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Presentation type:
AS – Atmospheric Sciences

EGU23-4082 | ECS | Orals | MAL31 | AS Division Outstanding Early Career Scientist Award Lecture

Multiphase buffer theory: explanations of contrasts in atmospheric aerosol acidity and its applications 

Guangjie Zheng

Acidity is one central parameter in atmospheric multiphase reactions, and strongly influences the climate, ecological and health effects of aerosols. Yet, the drivers of aerosol pH remain to be fully resolved. Here we investigated into this issue with thermodynamic models and observations. We find that aerosol pH levels in populated continental regions are widely buffered by the conjugate acid-base pair NH4+/NH3, and in aerosols an individual buffering agent can adopt different buffer pH values. To explain these large shifts of buffer pH, we propose a multiphase buffer theory, and show that aerosol water content and mass concentration play a more important role in determining aerosol pH in ammonia-buffered regions than variations in particle chemical composition. These results imply that aerosol pH and atmospheric multiphase chemistry are strongly affected by the pervasive human influence on ammonia emissions and the nitrogen cycle in the Anthropocene. We further investigated into the applications of the multiphase buffer theory. Exemplary applications include to help explain the formation of severe hazes in China, to quantify the contribution of different factors in driving the aerosol pH variations, and to provide the framework to reconstruct long-term trends and spatial variations of aerosol pH, etc. Further investigations on its applications in aerosol and cloud chemistry studies are needed.

How to cite: Zheng, G.: Multiphase buffer theory: explanations of contrasts in atmospheric aerosol acidity and its applications, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4082, https://doi.org/10.5194/egusphere-egu23-4082, 2023.

EGU23-9284 | Orals | MAL31 | Vilhelm Bjerknes Medal Lecture

Kilometer-resolution climate models: prospects and challenges 

Christoph Schär

Currently major efforts are underway toward refining the horizontal grid spacing of climate models to about 1 km, using both global and regional models. Such resolutions have been used for about a decade in limited-area numerical weather prediction applications and have demonstrated significant improvements in the representation of convective precipitation events (thunderstorms and rain showers). There is the well-founded hope that these benefits carry over to climate models, as the approach enables replacing the parameterizations of moist convection and gravity-wave drag by explicit treatments.

In this presentation, we will review three areas of km-resolution climate modeling. First, consideration will be given to an ensemble of km-resolution simulations from the CORDEX-FPS program on convection-permitting climate modelling, with a computational domain covering the greater Alpine region. This addresses the occurrence of short-term heavy precipitation events including their impacts such as flash floods, hail, and lightning. Results demonstrate the benefits of high computational resolution, in particular for the representation of short-term heavy events of severe weather. Second, we will present recent results from the projects trCLIM / CONSTRAIN carried out over the tropical and subtropical Atlantic, with the goal to assess the potential of the methodology to constrain estimates of the equilibrium climate sensitivity. It will be argued that km-resolution is a highly promising approach for constraining uncertainties in global climate change projections, due to improvements in the representation of tropical and subtropical clouds that goes along with an improved representation of the intertropical convergence zone (ITCZ).

Third, technical aspects of developing km-resolution global models will be addressed. Developing this approach requires a concerted effort between climate and computer sciences. Key challenges are the exploitation of the next generation hardware architectures using accelerators (e.g. graphics processing units, GPUs), the development of suitable approaches to overcome the output avalanche, and the consistent maintenance of the rapidly-developing model source codes on a number of different compute architectures. Despite these challenges, it will be argued that km-resolution GCMs with a capacity to run at 1 SYPD (simulated year per day), might be much closer than commonly believed. However, as the computational load of CMIP-style simulations is tremendous, alternative ways to exploit these models will be needed.

How to cite: Schär, C.: Kilometer-resolution climate models: prospects and challenges, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9284, https://doi.org/10.5194/egusphere-egu23-9284, 2023.

AS1 – Meteorology

EGU23-13 | Orals | AS1.1

An Integrated Coupling Framework for Atmospheric Dynamics and Physics 

Linjiong Zhou and Lucas Harris

Atmospheric resolved-scale air flow (dynamics) and sub-grid parameterizations (physics) are two essential components of a weather or climate model. These two independent components are coupled and advanced using the same time step, either parallel or sequentially split. However, traditionally dynamics and physics are engineered in isolation and developed independently in models. As a result, many parts of the physics run at a physically-inappropriate time frequency or with heat transfers that are inconsistent with the dynamics, leading to errors. In addition, physical parameterizations should contain dynamical and non-dynamical processes. We believe there are compelling reasons that dynamical processes, if resolved, should be taken care of by the dynamical core.

Our study proposes a novel integrated dynamics-physics coupling framework (Zhou and Harris, 2022) within the GFDL (Geophysical Fluid Dynamics Laboratory) weather-to-seasonal prediction system SHiELD (System for High-resolution prediction on Earth-to-Local Domains; Harris et al., 2020) that promises to resolve the above issues. We will present our integrated coupling framework and the development of integrated physical parameterization for this framework in detail. The performance of forecast experiments using the modeling system SHiELD with this integrated coupling framework will be highlighted, focusing on large-scale circulation, cloud and precipitation, hurricane, and convective-storm predictions.

How to cite: Zhou, L. and Harris, L.: An Integrated Coupling Framework for Atmospheric Dynamics and Physics, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13, https://doi.org/10.5194/egusphere-egu23-13, 2023.

EGU23-415 | ECS | Orals | AS1.1

Ensemble Forecast Sensitivity to Observations Impact (EFSOI) of a high impact weather event using a convection permitting data assimilation system. 

Gimena Casaretto, Maria Eugenia Dillon, Yanina Garcia Skabar, Juan Ruiz, Paula Maldonado, and Maximiliano Sacco

The improvement of numerical weather forecasts is a key element to predict high-impact weather events, associated with deep moist convection. The observations that are assimilated into numerical weather prediction systems are conformed by numerous data sets and their impact should be objectively evaluated. This can be efficiently estimated by the Forecast Sensitivity to Observation Impact (FSOI) methodology. In this study, we explore the application of the ensemble formulation of FSOI (EFSOI) in a convective scale regional data assimilation system over Sierras de Córdoba (Argentina), a data-sparse region with complex terrain characterized by the periodic occurrence of extreme precipitation and flash floods events. To evaluate the observation networks that result beneficial and detrimental for the forecast, the Weather Research and Forecasting model coupled with the Local Ensemble Transform Kalman Filter was used with 40 members. Convective scale analyses were obtained every 5 minutes, assimilating reflectivity data from a C-band radar and conventional and non-conventional surface weather stations (CSWS and NSWS). The experiment  was initialized on December 13 at 23 UTC and ran for 5 hours, until December 14 03 UTC. The experiment conducted was a case study within the intensive observing period of the RELAMPAGO-CACTI field campaign that was carried out during the 2018-2019 austral warm season in the center of Argentina. An independent data assimilation cycle using more observations and a different configuration is used in the experiments as verifying truth for the computation of forecast errors in EFSOI.

Results showed that all the observation sources had, on average, a positive impact on the 30 minute forecasts with a positive impact rate above 50%. However, when observations impacts are analyzed by geographic location, different results are evidenced. Most of the surface stations that evidence a detrimental impact in forecasts are located in the northern part of the region, probably due to a misrepresentation of the thermodynamic environment. Regarding radar reflectivity observations, values of positive impact rate above 50% dominate over all the region, demonstrating that, in general, they reduce the forecast errors. The results suggest that the observations with values of reflectivity beneath 15 dBZ have a larger amount of beneficial observations in lower levels than in upper levels.

This methodology is an approximation to quantify the impact of reflectivity and surface observations on a convective permitting forecast over the region. The results of this (and future) work can help to identify observation data sources detrimental for the data assimilation system, suggesting data selection criteria to assess improvements in this regional convective-scale data assimilation system where nonconventional observations such as radar data plays an essential role.

How to cite: Casaretto, G., Dillon, M. E., Garcia Skabar, Y., Ruiz, J., Maldonado, P., and Sacco, M.: Ensemble Forecast Sensitivity to Observations Impact (EFSOI) of a high impact weather event using a convection permitting data assimilation system., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-415, https://doi.org/10.5194/egusphere-egu23-415, 2023.

This study explores the potential impact of global navigation satellite system (GNSS) radio occultation (RO) data on the performance of satellite radiance data assimilation for the tropical cyclone formation forecast over the western North Pacific. The forecast experiments of 32 tropical disturbances in September−October 2019 are performed through a regional model. Either assimilation of GNSS RO data, radiance data, or both of them can improve the forecast skill and environmental moisture of tropical cyclone formation. However, the interaction between radiance and GNSS RO data can further increase moisture throughout the forecast period, compared to the experiment with only radiance data assimilation. Moreover, the improved vorticity patterns are different between the experiments with GNSS RO data and with radiance data. When both the GNSS RO and radiance data are assimilated, the improved vorticity pattern tends to the pattern improved by GNSS RO data assimilation. This may be attributed to the anchoring effect of GNSS RO data on satellite radiance data assimilation. Although radiance data volume is much larger than GNSS RO data, the interaction between GNSS RO and radiance data in the data assimilation process can significantly improve forecast performance.

How to cite: Teng, H.-F., Kuo, Y.-H., and Done, J.: Impact of radio occultation data on satellite radiance data assimilation performance in tropical cyclone formation forecast over the western North Pacific, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1079, https://doi.org/10.5194/egusphere-egu23-1079, 2023.

EGU23-1128 | ECS | Posters virtual | AS1.1

Modeling of wind conditions in Warsaw 

Tomasz Strzyzewski and Adam Jaczewski

Airflow is one of the most important weather parameters in a city. It is important for the air quality, the city's heat balance, pedestrian comfort and the safety of high-rise buildings. Local flow at the scale of streets and districts is difficult or impossible to capture in regional weather models. Computational Fluid Dynamic models are the solution. In this paper, the OpenFoam model was used to model wind direction and speed in specific meteorological situations. The results were compared with measurement stations in Warsaw, and the model was improved on their basis. An averaged Navier Stokes turbulence model was used under steady-stable flow conditions. The Darcy-Forchheimer model was used to take vegetation into account. The poster presents the first results of analyzes related to the spatial distribution of wind direction and speed, delineates areas at risk of low air quality and compares it with the results from measuring stations. In addition to the basic model, a model containing ground thermals was also created to study the extent and intensity of the urban heat island and to study the phenomenon of smog during temperature inversion in selected meteorological conditions. A comparative analysis of both models was made. The first results show that it is possible quite accurately to map airflow in a city. It also indicates that some existing ventilation channels of the city have been blocked or limited due to new investments. The most important ventilation channel is the Vistula valley, which is 500-600 m wide in Warsaw. However, due to the terrain, its most important role is not fulfilled during prevailing westerly winds, and then the air quality decreases, especially at low wind speeds. In most cases, the northern districts are also generally better ventilated (spatial distribution of buildings, higher wind speeds) than the southern districts, but this is not always visible when assessing air quality. The immediate vicinity also influences the aspects of mechanical ventilation of the city and the way buildings are heated. Districts that theoretically should have better conditions for air exchange are often areas of single-family houses and independent boiler rooms. The city centre, despite tighter development, is heated by the municipal heating plant, and they are not direct emitters of pollution. Another aspect is vehicle traffic. In the city centre, more vehicle traffic is another pollutant emitter. For this reason, pollutants specific to heating and traffic were analysed separately. The general problem in high-resolution city-scale modelling is the use of adequate computational power. This initially precludes using CFD models in meteorological nowcasting and short-term modelling.

How to cite: Strzyzewski, T. and Jaczewski, A.: Modeling of wind conditions in Warsaw, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1128, https://doi.org/10.5194/egusphere-egu23-1128, 2023.

EGU23-1463 | ECS | Orals | AS1.1

Docker container in DWD's Seamless INtegrated FOrecastiNg sYstem (SINFONY) 

Matthias Zacharuk, Christian Welzbacher, Isabel Schnoor, Nils Rathmann, Christian Eser, Florian Prill, and Ulrich Blahak and the SINFONY

At Deutscher Wetterdienst (DWD), the SINFONY project has been set up to develop a seamless ensemble prediction system for convective-scale forecasting with forecast ranges of up to 12 hours. It combines Nowcasting (NWC) techniques with numerical weather prediction (NWP) in a seamless way. So far NWC and NWP run on two different IT-Infrastructure levels. Due to the data transfer between both infrastructures, this separation slows down SINFONY, makes it complex and prone to disturbances. These disadvantages are solved by applying the interconnected part of the SINFONY on one single architecture using a Docker Container.

With this aim in view a Docker-Container of the respective NWC components is created and executed on the infrastructure of NWP, the high performance linux computing cluster (HPC) of DWD. In test applications we already observed a speed up of roughly 20% by using the Container on the HPC-cluster instead of using NWC-Tools on the initial NWC IT-Architecture. The Container is already implemented in DWD’s experimental tool BACY for the assimilation cycle.

A major innovation of SINFONY is the rapid update cycle (RUC), an hourly refreshing NWP procedure with a Forecast range of 8 hours, which will be extended to 12 hours soon. The container will be implemented to the RUC and used for the subsequent combination of NWP and NWC forecasts.

In the presentation I will explain what a container is and discuss opportunities and risks of this technology. I will introduce how building the Container is integrated to the CICD procedures at DWD, how and where the Container is implemented to BACY and discuss latest results for the implementation to the RUC.

How to cite: Zacharuk, M., Welzbacher, C., Schnoor, I., Rathmann, N., Eser, C., Prill, F., and Blahak, U. and the SINFONY: Docker container in DWD's Seamless INtegrated FOrecastiNg sYstem (SINFONY), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1463, https://doi.org/10.5194/egusphere-egu23-1463, 2023.

EGU23-1510 | ECS | Orals | AS1.1

Comparison of Arctic sea-ice albedo between CARRA and ERA5 reanalyses and satellite based CLARA-A2 

Viivi Kallio-Myers, Yurii Batrak, and Bin Cheng

With the ongoing climate change, the Arctic region is experiencing rapid warming. This has a profound effect on the sea-ice cover and, as a result, on the surface albedo. Surface albedo has a large impact on the energy balance of the region: a decrease in surface albedo leads to increased absorption of solar radiation and thus higher temperatures, ultimately leading to the albedo decreasing further. Information on the surface albedo is therefore necessary for various applications and climate studies. Atmospheric reanalysis products answer this need, providing consistent multiyear datasets with good spatial coverage.

We have studied the Arctic sea-ice albedo in two reanalyses. First is ERA5, a global atmospheric reanalysis by the ECMWF (European Centre for Medium range Weather Forecasts). ERA5 has a horizontal resolution of 31 km, and sea-ice is modelled with a one-dimensional sea-ice parameterisation scheme.

The second reanalysis is CARRA (Copernicus Arctic Regional ReAnalysis), a regional atmospheric reanalysis covering a part of the Arctic with two overlapping domains: the western domain centred around Greenland and the eastern over the European Arctic. The horizontal resolution is 2.5 km, and similarly to ERA5, sea-ice is modelled with a one-dimensional thermodynamic sea-ice scheme.

We compare the surface albedo of these two reanalyses to the satellite-based black-sky surface albedo product of the CLARA-A2.1 dataset (CM SAF cLoud, Albedo and surface RAdiation dataset from AVHRR data). Comparisons are made for April to September, 2000-2015, for the sea areas of the CARRA domains. In addition to a general assessment, four different regions within the domains are studied separately.

How to cite: Kallio-Myers, V., Batrak, Y., and Cheng, B.: Comparison of Arctic sea-ice albedo between CARRA and ERA5 reanalyses and satellite based CLARA-A2, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1510, https://doi.org/10.5194/egusphere-egu23-1510, 2023.

EGU23-1687 | Orals | AS1.1

Winter jet stream wind speed changes in the eastern North Atlantic 

Joel Tenenbaum and Paul Williams

We have published [ https://doi.org/10.1002/qj.4342 ] recent results on winter jet stream wind speed changes in the eastern North Atlantic: there is no change for the past 40 years but a statistically significant increase for the past roughly 20 years (2002-2020).  The increase shows up in both the Global Aircraft Data Set (GADS) observations from flight data recorders and the ERA5 reanalysis.  The wind speeds seem to track the North Atlantic Oscillation (NAO).  We can consider four possibilities: ( 1 ) synoptic fluctuation; ( 2 ) improved aircraft routing, though inconsistent with NAO correlations; ( 3 ) greater number of automated aircraft observations; ( 4 ) actual secular change in the polar jet exit region of the atmosphere.  This type of study must deal with subtleties of North Atlantic track system that includes aircraft step climbs.  We will present newer results on the secular increase in automated aircraft observations and the effects of including more recent Northern Hemisphere winters (2021 through, possibly, 2023).

How to cite: Tenenbaum, J. and Williams, P.: Winter jet stream wind speed changes in the eastern North Atlantic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1687, https://doi.org/10.5194/egusphere-egu23-1687, 2023.

EGU23-1830 | ECS | Posters on site | AS1.1

A statistical description method of global sub-grid topography for numerical models 

Yaqi Wang, Lanning Wang, Juan Feng, and Zhenya Song

Slope and aspect are important topographic elements for thermodynamics and dynamics of atmospheric circulation, especially for local radiation and topographic precipitation. We propose a simple realistic statistical method based on trigonometric function transformation to calculate sub-grid slope and aspect for describing the orographic characteristics of complex areas over the globe. It is found that the transformed conditional probability density function (PDF) conforms to the Gaussian distribution in most of the global areas (~98%), and this feature is not eliminated with the increasing of horizontal resolution. The reasonability of this method is tested over the Tibetan Plateau. The results show that the improvement ratio of surface solar radiation downward (SSRD) over the Tibetan Plateau improved significantly compared with the results from the grid average scheme, especially in autumn. The improvement of root mean square error (RMSE) is approximately 18.2 W/m2, and the improvement ratio reached 38.4%. The improvements of maximum and regional-averaged SSRD over the whole Tibetan Plateau were ~130 W/ m2 and ~44.3W/m2 respectively. Although we only consider the effect of sub-grid slope and aspect on solar shortwave radiation, which has a certain bias with the observation data, it is sufficient to prove the rationality of the statistical method compared with the unobstructed horizontal surfaces scheme (CTL). After that, we applied this sub-grid parameterization scheme for topographic vertical motion in CAM5 to revise the original vertical velocity by adding the topographic vertical motion and then resulting a significant improvement of simulation in precipitation over steep mountains.

How to cite: Wang, Y., Wang, L., Feng, J., and Song, Z.: A statistical description method of global sub-grid topography for numerical models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1830, https://doi.org/10.5194/egusphere-egu23-1830, 2023.

EGU23-2466 | ECS | Posters on site | AS1.1

Impact of changes in the cloud amount due to condensation processes on precipitation forecasting on the Korean Peninsula during the summer in the Korean Integrated Model 

Yeseo Park, Jeong-Ock Lim, Hyun-Joo Choi, Kyoungmi Cho, Seon-Kyun Baek, and Seong-Hoon Cheong

In numerical models, the amount of clouds affects atmospheric temperature through interaction with radiation. In the Korean Integrated Model (KIM), which has been in operation at the Korea Meteorological Administration since April 2020, the amount of clouds is determined from prognostic equation consisting of source and sink terms  by  physical processes such as planetary boundary layer (PBL) mixing, convection, advection, condensation, and evaporation. In the control KIM version, the temperature forcing used for calculating the rate of changes in time of saturation specific humidity which determines formation of cloud area due to condensation is calculated by considering those from all physical processes, such as radiation, cumulus convection, and turbulence, as well as cloud microphysical processes. However, we found the inconsistency between the cloud fraction and mixing ratio by using the methodology, so in this study, we modify the temperature forcing from all physical processes into that only due to the microphysical process. It is confirmed that the change in the amount of clouds changes the temperature and humidity of the atmosphere through the interaction between physical processes such as radiation, which also affects precipitation. 
In this study, to examine the effect of changes in cloud cover on precipitation in the Korean Peninsula, we perform one case study July 4, 2021 when precipitation in Gangwon occurs due to the convergence of air currents caused by east wind of high pressure in the eastern of Korea. Up to 172.5 mm of daily maximum precipitation was reported in the Gangwon region. In the 3-day forecast of the case, the control KIM  underestimates inland precipitation. But the trend of under-estimation is improved by increasing the amount of precipitation when the cloud amount is modified. The increase in precipitation mainly occurs in the large-scale precipitation due to the microphysical process. This is because the cloud amount generally increases in the Asian area including the Korean Peninsula, which makes the environment favor to the precipitation, by decreasing the temperature through the radiative cooling, in turn resulting the decrease in saturation vapor pressure. For the statistical evaluation of the precipitation performance, precipitation verification is also performed for one month in July, and it is found that ETS (Equivalent Threat Score) performance against the  reanalysis data on the Korean Peninsula is also improved.

How to cite: Park, Y., Lim, J.-O., Choi, H.-J., Cho, K., Baek, S.-K., and Cheong, S.-H.: Impact of changes in the cloud amount due to condensation processes on precipitation forecasting on the Korean Peninsula during the summer in the Korean Integrated Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2466, https://doi.org/10.5194/egusphere-egu23-2466, 2023.

EGU23-2827 | Posters on site | AS1.1

Ensemble sensitivity localization 

Philipp Johannes Griewank, Tobias Necker, and Martin Weissmann

Ensemble sensitivity is a tool to quantitatively determine which initial conditions influence a forecast quantity of choice. This information can then be used to understand the sources and dynamics of forecast uncertainty, quantify the impact of observations (e.g., E-FSOI), and determine where to best deploy observations to improve the forecast (e.g., observation targetting and network design). The ensemble sensitivity is calculated from the covariances of the initial ensemble to the forecast ensemble. Unfortunately, these covariances are prone to sampling errors due to the limited ensemble size. The most common approach in data assimilation to mitigate sampling errors is to apply distance-based damping, i.e., localization. This poster explores how to localize the sensitivity correctly and how it differs from analysis localization. Using simplified problems, we highlight the benefits and drawbacks of sensitivity localization and discuss its usefulness to numerical weather prediction applications.

How to cite: Griewank, P. J., Necker, T., and Weissmann, M.: Ensemble sensitivity localization, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2827, https://doi.org/10.5194/egusphere-egu23-2827, 2023.

EGU23-2982 | Orals | AS1.1

Advancing Operational Modeling Systems at NOAA’s Environmental Modeling Center: Transitioning to Unified Forecast System Applications 

Ivanka Stajner, Brian Gross, Vijay Tallapragada, Jason Levit, Arun Chawla, Avichal Mehra, Daryl Kleist, and Fanglin Yang

National Oceanic and Atmospheric Administration’s (NOAA’s) Environmental Modeling Center (EMC) is a lead developer of Numerical Weather Prediction (NWP) systems that also transitions to operations and maintains more than 20 numerical prediction systems that are used across the National Weather Service (NWS), the broader NOAA, by other United States (U.S.) federal agencies, and various other stakeholders. These systems are developed through a close collaboration with partners from the academic, federal and commercial sectors. EMC maintains, enhances and transitions-to-operations numerical forecast systems for weather, ocean, climate, land surface and hydrology, hurricanes, and air quality for the U.S. and the global community and for the protection of life and property and the enhancement of the economy.

 

NOAA’s Next Generation Global Prediction System (NGGPS) Project initiated a major shift in the development of operational Earth system predictions with a goal to simplify the National Centers for Environmental Prediction (NCEP) Production Suite using the Unified Forecast System (UFS) framework (https://ufscommunity.org/). EMC has taken a lead in further development and consolidation of NCEP’s operational systems into UFS based applications.  The UFS is being designed as a community-based, comprehensive atmosphere-ocean-sea-ice-wave-aerosol-land coupled Earth modeling system with coupled data assimilation and ensemble capabilities, organized around applications spanning local to global domains and predictive time scales ranging from sub-hourly analyses to seasonal predictions.  Disparate operational applications that have been developed and maintained by EMC in support of various stakeholder requirements are being transitioned to the UFS framework. The transition started a few years ago and is planned to continue over the next few years. The resulting applications will consolidate NCEP’s Production Suite into far fewer applications that share a set of common scientific components and technical infrastructure.  This approach is expected to accelerate the transition of research into operations and simplify maintenance of operational systems.

 

This talk describes major development and operational implementation projects at EMC over the last few years and the plans for the next five years (2023-2027), how those fit within the broader strategic plans of NOAA, and how these projects link with other model-related projects internally within NOAA and with the broader U.S. and international modeling community.

How to cite: Stajner, I., Gross, B., Tallapragada, V., Levit, J., Chawla, A., Mehra, A., Kleist, D., and Yang, F.: Advancing Operational Modeling Systems at NOAA’s Environmental Modeling Center: Transitioning to Unified Forecast System Applications, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2982, https://doi.org/10.5194/egusphere-egu23-2982, 2023.

EGU23-3025 | Posters on site | AS1.1

Effects of increasing horizontal and vertical resolution in Korean Integrated Model (KIM) 

Ja-Rin Park, Hae-Jin Kong, Hyun Nam, and Suk-Jin Choi

Since the dynamical core of Korean Integrated Model (KIM) was developed in the 1st phase (2011~2019) of KIAPS, we have been aiming to develop a variable resolution prediction system covering short to medium range in the 2nd phase (2020.9~2026). As a first step towards moving to km-scale resolution, we have increased the model resolution from 12 km to 8 km horizontally and 91 to 137 layers vertically. For increasing the resolution horizontally, dynamics core configurations and terrain elevation data were newly set up. For vertically, vertical coordinates of 137 layers followed that of the European Center for Intermediate Forecasting (ECMWF) Integrated Forecasting System (IFS), which has been increased vertical resolution throughout the troposphere and stratosphere comparing to 91 layers.
This study discusses the forecast impact of high-resolution KIM in terms of objective verification scores against observations and analyses. The overall conclusion for horizontal high-resolution is that it shows slightly positive in southern hemisphere and mainly neutral for northern hemisphere, but also some negative in tropics. One of distinguished results is increasing horizontal resolution leads to cooling in the temperature in the lower and upper troposphere. The cooling in the lower tropospheric over the tropics seems to come from smaller time step that has to be for smaller dx, which results in enlarged low cloud formation and thus more radiative cooling. In case of the upper troposphere, the cooling results from outgoing long-wave radiative cooling by decreasing hydrometeors in physical response to smaller grid spacing. The increase of vertical resolution had an effect of neutral to slight positive in northern hemisphere but showed significant degradation in tropics. To achieve the consistency and improvement for high-resolution model, it is necessary to understand the physical processes related to time step and horizontal and vertical grid spacing.

 

Acknowledgement
One of the authors, S-J Choi, wishes to acknowledge this study was supported by 2023 New Professor Support Program of Natural Science Research Institute in Gangneung-Wonju National University).

How to cite: Park, J.-R., Kong, H.-J., Nam, H., and Choi, S.-J.: Effects of increasing horizontal and vertical resolution in Korean Integrated Model (KIM), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3025, https://doi.org/10.5194/egusphere-egu23-3025, 2023.

NOAA is collaborating with the US weather and climate science community to develop the next generation fully coupled earth system modeling capability for both research and operational forecast applications across different temporal and spatial scales.    In this presentation we explore the possibility of running the UFS at convection-permitting resolution for global medium-range weather forecasting.  A few sensitivity experiments were performed at a global uniform 3-km resolution with and without parameterized convection.  Results were compared with the 13-km control experiments to investigate the impact of model resolution and convection parameterization on precipitation and cloud-radiation interaction.   Aerosol indirect effect on clouds is also tested and evaluated within this framework to understand its sensitivity to model resolution and parameterized convection.  Aerosol indirect effect occurs when aerosols act as cloud condensation nuclei and ice nuclei within clouds and consequently alter cloud radiative properties and cloud lifetime.   Using the Thompson double-momentum microphysics scheme, the number concentrations of water friendly aerosol and ice friendly aerosol are either diagnosed from the MERRA2 aerosol climatology or predicted and advected with source and sink terms derived from the climatology. The relations between clouds, radiation and precipitation with and without the presence of aerosol indirect effects are analyzed for simulations made at both the control 13-km and experimental 3-km UFS model resolutions.  

How to cite: Yang, F., Chen, A., and Moorthi, S.: Prototyping Convection-Permitting Global Weather Forecast and the Representation of Aerosol-Cloud-Radiation Interaction in the NOAA Unified Forecast System, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3038, https://doi.org/10.5194/egusphere-egu23-3038, 2023.

EGU23-3183 | ECS | Posters on site | AS1.1

Integration of the WRF Model With Fine-Scale Land Use Data to Simulate Extreme Rainfall Events 

Nagaraju Gaddam, Abhinav Wadhwa, Likhitha Pentakota, Gowri Reghunath, and Pradeep P Mujumdar

Urbanization results in drastic land alteration in which natural land cover is replaced by impermeable surfaces such as compacted soils, buildings and associated infrastructures. While the impact of urbanization on extreme rainfall is captured in satellite data to a great extent, its signal is frequently less obvious in station-level data. Also, the lack of local meteorological data hinders the development of adequate mitigation measures to reduce the impact of extreme rainfall scenarios. To regenerate the local meteorological data, numerical model-based simulations using global boundary conditions are required at finer Spatio-temporal scales. To this end, integrated land surface models which can provide the maximum likelihood of observed rainfall can be of great significance, especially in urban complexes. Weather Research Forecasting (WRF) model is one such numerical model that can lay down a framework to provide short-range weather forecasts by fixing site-specific physics-based parametrization schemes. This study demonstrates the application of the WRF model to provide building-scale weather forecasts based on the finer-scale Urban Canopy Model (UCM) and Local Climate Zonation (LCZ). The numerical modelling framework is set up for Bangalore city, India. Bangalore city is categorized as one of the major urban complexes with a total built-up area of 77.5%. The World Urban Database Access Portal Tool (WUDAPT), which is based on random forest classification of the ground truth training samples, is used to develop the LCZ database for the WRF model. A single-layer UCM is developed to indicate the importance of structural and aerial characteristics of static datasets with appropriate land features. WRF model runs are carried out based on global boundary conditions to provide a 24hr forecast with 3km and 1km spatial domain for the study area at an urban scale. The overall accuracy of 92% (for the built-up area) and 85% (for water bodies) is obtained for LCZs developed using the random forest classification in WUDAPT. In comparison to default configurations of WRF, the forecasts of WUDAPT-based LCZs have shown an improvement at both spatial and temporal scales. The bias (particularly the spatial shift) observed using the default WRF is reduced drastically, and the forecasts are well-matched with the observed Telemetric Rain Gauge (TRG) station rainfall datasets. Assessment of the maximum likelihood of extreme rainfall forecasts can provide a platform for the development of an integrated WRF hydrological configuration in the future. Such frameworks will be greatly beneficial for obtaining more accurate rainfall and flood forecasts.

How to cite: Gaddam, N., Wadhwa, A., Pentakota, L., Reghunath, G., and P Mujumdar, P.: Integration of the WRF Model With Fine-Scale Land Use Data to Simulate Extreme Rainfall Events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3183, https://doi.org/10.5194/egusphere-egu23-3183, 2023.

EGU23-3545 | ECS | Orals | AS1.1

The Role of Parameterized Momentum Flux on Biases in Tropical Cyclones and the Mean State in the Community Atmosphere Model 

Kyle Nardi, Colin Zarzycki, Vincent Larson, and George Bryan

With enhanced computational capacity, the treatment of subgrid processes in global Earth System Models (ESMs) has grown increasingly complex. Despite these enhancements, critical biases remain in the modeling of fundamental processes that govern both the mean climate and the development of extreme weather phenomena of high societal impact. Due to their potential to be better resolved in the next generation of ESMs, tropical cyclones (TCs) are extremes of particular interest. 

The importance of the parameterization of momentum flux within the boundary layer (PBL) for modeled TC structure has been established for numerical models run at a variety of spatial scales. However, few studies have specifically explored the modulation of TC structure by the PBL parameterization in a coarser-resolution ESM. In this study, we evaluate the role of the PBL scheme on modeled TC structure in the Community Atmosphere Model version 6 (CAM6), which is the atmospheric component of the Community Earth System Model version 2 (CESM2). CAM6 employs the Cloud Layers Unified by Binormals (CLUBB) scheme. To enhance generalizability of turbulent processes, we apply an experimental version of CLUBB (CLUBBX) with a prognostic formulation of momentum flux and a regime-specific formulation for the dissipation of turbulent eddies.  

We perform a sensitivity analysis, the Morris one-at-a-time (MOAT) method, to evaluate the influence of various tunable CLUBBX input parameters on process-based metrics that characterize TC structure in an idealized framework. We find that certain tunable CLUBBX parameters controlling vertical turbulent mixing in the PBL modulate key TC metrics like jet height, inflow angle, and surface heat flux. We further demonstrate that targeted perturbations to these influential parameters can reduce established ESM biases in modeled TC structure. 

However, in a global ESM, the accurate depiction of individual TCs should not come at the expense of the model’s depiction of the mean climate. Therefore, it is important to understand how the calibration of CAM6-CLUBBX impacts other aspects of the global and regional climate. We therefore repeat the MOAT sensitivity analysis on global ESM simulations to evaluate how these CLUBBX input parameters impact process-based climate metrics on regional and global scales. We leverage an ensemble approach with short, initialized runs (Betacast) to allow for computational tractability.  

We find that CLUBBX parameters that influence TC structure also influence various regionally and globally-averaged climate metrics, including thermodynamic profiles, cloud-radiative forcing, and surface wind stress, at short timescales (3 days). We further show that targeted perturbations to a handful of these influential input parameters can reduce global and regional biases in CAM6-CLUBBX at decadal timescales. We explore physical mechanisms for these demonstrated parameter sensitivities and discuss practical implications of targeted model tunings for long-term climate simulations. 

How to cite: Nardi, K., Zarzycki, C., Larson, V., and Bryan, G.: The Role of Parameterized Momentum Flux on Biases in Tropical Cyclones and the Mean State in the Community Atmosphere Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3545, https://doi.org/10.5194/egusphere-egu23-3545, 2023.

EGU23-3553 | Posters on site | AS1.1

A positive definite solution for an EDMF PBL scheme that includes a moist adjustment process 

Jian-Wen Bao, Evelyn Grell, Sara Michelson, and Song-You Hong

The eddy diffusivity and mass flux (EDMF) scheme for simulating turbulent transport in the operational Global Forecast System (GFS) shows a behavior due to a physical and numerical inconsistency in the scheme's numerical procedure to obtain detrained cloud water due to the moist nonlocal mixing and its associated moist adjustment.  One-dimensional simulations show that such inconsistency leads to an unphysical distribution of thermal tendencies and detrained cloud water near the simulated planetary boundary layer (PBL) top.  To solve this problem, a new procedure to obtain a positive definite solution from the scheme is proposed to solve the EDMF equations in the scheme. We will show the impact of this new solution procedure on the GFS performance.

How to cite: Bao, J.-W., Grell, E., Michelson, S., and Hong, S.-Y.: A positive definite solution for an EDMF PBL scheme that includes a moist adjustment process, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3553, https://doi.org/10.5194/egusphere-egu23-3553, 2023.

EGU23-3703 | Orals | AS1.1

Facilitating the development of complex models with the Common Community Physics Package and its Single-Column Model 

Ligia Bernardet, Grant Firl, Dustin Swales, Man Zhang, Mike Kavulich, Samuel Trahan, Weiwei Li, Jimy Dudhia, and Mike Ek

The Common Community Physics Package (CCPP) is a collection of atmospheric physical parameterizations and a framework that couples the physics for use in Earth system models. The CCPP Framework was developed by the U.S. Developmental Testbed Center (DTC) and is now an integral part of the Unified Forecast System (UFS). The UFS is a community-based, coupled, comprehensive Earth modeling system designed to support research and be the source system for NOAA‘s multi-scale operational numerical weather prediction applications. The CCPP is also being used in the experimental U.S. Navy Environmental Prediction sysTem Utilizing the NUMA  corE (NEPTUNE, which employs a modified version of the Non-hydrostatic United Model for the Atmosphere dynamical core) and is currently being integrated into the Community Atmosphere Model (CAM) utilized in the National Center for Atmospheric Research (NCAR) Community Earth System Model (CESM).

A primary goal for this effort is to facilitate research and development of physical parameterizations, while simultaneously offering capabilities for use in operational models. The CCPP Framework supports configurations ranging from process studies to operational numerical weather prediction as it enables host models to assemble the parameterizations in flexible suites. Framework capabilities include flexibility with respect to the order in which schemes are called, ability to group parameterizations for calls in different parts of the host model, and ability to call some parameterizations more often than others. Furthermore, the CCPP is distributed with a single-column model (SCM) that can be used to test innovations,  conduct hierarchical studies in which physics and dynamics are decoupled, and isolate processes to more easily identify issues associated with systematic model biases. The CCPP SCM can be driven using files in the DEPHY format (an internationally agreed-upon format for inputs and outputs of SCMs). This opens doors for collaborations using multiple initial and forcing datasets based on observational field campaigns. The CCPP SCM is also being updated to be forced by the UFS.

The CCPP v6.0.0 public release includes 23 primary parameterizations (and six supported suites), representing a wide range of meteorological and land-surface processes. Experimental versions of the CCPP also contain chemical schemes, making it possible to represent processes in which chemistry and meteorology are tightly coupled.

The CCPP is developed as open-source code and has received contributions from the wide community in the form of new schemes and innovations within existing schemes. In this presentation, we will provide an update on CCPP development and plans, as well as review existing resources for users and developers, such as the public releases, documentation, tutorial, and support mechanism. We will also provide information about the upcoming CCPP Visioning Workshop, indeed to be a forum for current and future CCPP users to learn about its capabilities and discuss requirements for new development. 

How to cite: Bernardet, L., Firl, G., Swales, D., Zhang, M., Kavulich, M., Trahan, S., Li, W., Dudhia, J., and Ek, M.: Facilitating the development of complex models with the Common Community Physics Package and its Single-Column Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3703, https://doi.org/10.5194/egusphere-egu23-3703, 2023.

EGU23-3781 | ECS | Orals | AS1.1

Appropriately representing convective heating is critical for predicting catastrophic heavy rainfall in 2021 in Henan Province of China 

Mingyue Xu, Chun Zhao, Jun Gu, Jiawang Feng, Gudongze Li, and Jianping Guo

An unprecedented heavy rainfall event occurred in Henan Province of central China during 19-20 July 2021. To investigate the impacts of predicted large-scale circulation on the regional convection-permitting prediction of this event, two sets of nested experiments with different convective parameterizations (GF and MSKF) in the outer domain and at convection-permitting resolution in the inner domain are performed with the Weather Research and Forecasting (WRF) model. The analysis found the prediction of “21.7” rainstorm at convection-permitting resolution in the inner domain is largely affected by convective scheme in the outer domain. The large-scale circulation forcing from the outer domain with different convective schemes is significantly different, which ultimately affects the circulation and precipitation in the refined region through lateral boundary forcing. The difference in regional prediction at convection-permitting resolution can be mitigated by adjusting convective latent heat parameterization in the outer domain. This work highlights that appropriately parameterizing convective latent heat is the key to provide reasonable large-scale forcing for regionally predicting this catastrophic heavy rainfall event at convection-permitting resolution, which may also be applicable to other events and other regions.

How to cite: Xu, M., Zhao, C., Gu, J., Feng, J., Li, G., and Guo, J.: Appropriately representing convective heating is critical for predicting catastrophic heavy rainfall in 2021 in Henan Province of China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3781, https://doi.org/10.5194/egusphere-egu23-3781, 2023.

The characteristic adjustment time scale τ is always defined as the time allowed for dissipation of Convective Available Potential Energy (CAPE) in convective parameterization schemes. Previous studies indicate that, in the cloud ensemble, τ is one of the most important parameters that have  the greatest influences on the global mean precipitation. Some research work has improved the Kain–Fritsch scheme in the regional model to realize the variable parameters. In the global model, some studies have used machine learning methods to optimize the parameters of the deep convection trigger function. However, changing constant parameters into variable parameters in the global model has not been explored. In our study, the Zhang-McFarlane (ZM) deep convection scheme is improved to realize the variable characteristic adjustment time scale parameter, so as to reduce the precipitation deviation in a global model. In the ZM deep convection scheme, τ is usually the default constant. While in this paper, we use CAPE to modulate τ and propose a calculation formula of τ. In the region where the mean precipitation amount bias is improved, the new scheme mainly increases the deep convective precipitation and reduces the large-scale and shallow convective precipitation. The modified scheme significantly improves the simulation of precipitation over the eastern equatorial Pacific Ocean and some steep terrain regions. The root mean square error of the mean precipitation amount over the eastern equatorial Pacific Ocean and the central Indo-Pacific Warm Pool in boreal summer is reduced after the new scheme is adopted in a global model with the horizontal resolution of 1° longitude and 1° latitude. Moreover, the simulations of precipitation over the Tibet Plateau and South America are also improved. The new scheme reduces the frequency of deep convective precipitation and increases the amount of deep convective precipitation each time.

How to cite: Wang, M. and Wang, L.: Simulation of Precipitation with a Variable Characteristic Adjustment Time Scale Parameter of Deep Convection in a Global AGCM, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4649, https://doi.org/10.5194/egusphere-egu23-4649, 2023.

EGU23-4730 | Posters on site | AS1.1

Status and plan of ensemble forecast system in Korea Meteorological Administration (KMA) 

Eun-Jung Kim, Hyun-Cheol Shin, Jong Im Park, Jong-Chul Ha, and Young-Cheol Kwon

The ensemble forecast system based on the Korea Integrated Model (KIM), which is developed for Korea’s own numerical weather prediction (NWP) model, has been in operation at Korean Meteorological Administration (KMA) since October 2021. KMA ensemble forecast system consists of 50 perturbation members (25 members for long-range forecast) and 1 control simulation. Four-dimensional LETKF (Local Ensemble Transform Kalman Filter) with additive and RTPS inflation scheme is used to make initial perturbation. 
Evaluation of forecast scores shows that our operational ensemble forecast system is generally more skillful compared to the deterministic simulation as forecast time is longer. Also, forecast with increased ensemble size produces better representation of atmospheric fields especially in higher latitudes. Details of results from operational ensemble system and impacts of increased ensemble size will be discussed with introducing a brief overview of our ensemble forecast system and development plan in future. 

How to cite: Kim, E.-J., Shin, H.-C., Park, J. I., Ha, J.-C., and Kwon, Y.-C.: Status and plan of ensemble forecast system in Korea Meteorological Administration (KMA), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4730, https://doi.org/10.5194/egusphere-egu23-4730, 2023.

EGU23-5548 | ECS | Orals | AS1.1

Exploitation of GNSS tropospheric gradients for severe weather Monitoring And Prediction (EGMAP): Project status and Initial results 

Rohith Muraleedharan Thundathil, Florian Zus, Galina Dick, and Jens Wickert

Data assimilation (DA) is a tool that is capable of combining observations and numerical weather models (NWMs) in an optimal manner. Current DA systems used by operational forecasting centres are constantly evolving and getting better than before. High-quality observations are very important for the accurate representation of variables in a weather model. In this study, we are incorporating Global Navigation Satellite System (GNSS) tropospheric gradients and Zenith Total Delays (ZTDs) into the Weather Research and Forecasting (WRF) model. WRF model has its operator already developed for the ZTDs and in this research, we are developing a new operator for the assimilation of tropospheric gradients. The assimilation of ZTDs, which are closely related to Integrated Water Vapor (IWV) above the GNSS station, has a positive impact on weather forecasts. On the other hand, tropospheric gradients are not yet assimilated by the weather agencies. Our research is based on a project titled “Exploitation of GNSS tropospheric gradients for severe weather Monitoring And Prediction” (EGMAP) focusing on the impact of GNSS tropospheric gradients and how it can be effectively used for operational forecasting of severe weather. EGMAP is funded by the German Research Foundation (DFG).

The observation operator currently in use for tropospheric gradients is based on a linear combination of ray-traced tropospheric delays (Zus et al., 2022). This observation operator is challenging to be implemented into an NWM DA system. We will thus rely on a more simple and fast observation operator which is based on the closed-form expression depending on the north–south and east–west horizontal gradients of atmospheric refractivity (Davis et al., 1993).

Initial testing of the operator is done on a 0.1 x 0.1-degree mesh configured over Central Europe in the WRF model with 50 vertical levels up to 50 hPa. The model configuration will be later upgraded to a convective-scale resolution after initial testing of the tropospheric gradient operator. Model forcing observations are derived from the National Centers for Environmental Prediction (NCEP) Global Forecast System (GFS) data at 0.25-degree resolution. Conventional observations are obtained from the European Centre for Medium-Range Weather Forecasts (ECMWF) and are the base dataset for the assimilation studies. The conventional datasets used for assimilation are restricted to surface stations (SYNOP observations) and radiosondes. Additionally, observations from roughly 100 GNSS stations are assimilated at each DA cycle. Three experiments are conducted: 1) Control run with only conventional data; 2) ZTD assimilation on top of the control run, and; 3) ZTD and tropospheric gradient assimilation on top of the control run. Initial DA tests are being performed with an automated rapid update cycle DA framework with 6 hourly intervals based on a deterministic three-Dimensional Variational (3DVar) DA system for the testing of ZTDs and tropospheric gradients. The DA system will be later upgraded to a probabilistic one based on the Hybrid 3DVar-Ensemble Transform Kalman Filter (-ETKF, Thundathil et al., 2021) and 4DEnVar. The EGMAP project status and initial results from the impact of GNSS-ZTDs and tropospheric gradients will be presented.

How to cite: Thundathil, R. M., Zus, F., Dick, G., and Wickert, J.: Exploitation of GNSS tropospheric gradients for severe weather Monitoring And Prediction (EGMAP): Project status and Initial results, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5548, https://doi.org/10.5194/egusphere-egu23-5548, 2023.

EGU23-6532 | Orals | AS1.1

Upper tropospheric convective outflow in ICON convection-permitting and parameterised set-up 

Edward Groot, Patrick Kuntze, Annette Miltenberger, and Holger Tost

The representation of upper tropospheric deep convective divergent outflow (UTDCDO) is compared between ICON-simulations with convection-permitting and convection parameterised set-ups (1 and 13 km resolution) for a convective event over Germany and the Alps on June 10th-11th 2019. Three hypotheses on those UTDCDO have been formulated using idealised Large Eddy Simulations and are now tested on ICON in a convection-permitting set-up: 1. Dimensionality affects the magnitude of UTDCDO in ICON; 2. Convective aggregation and organisation affects the magnitude of those convective outflows in ICON and 3. Convective momentum transport does not affect the magnitude of UTDCDO. A moving box is used to integrate mesoscale divergence, precipitation rate and convective momentum transport. Additionally, ellipse fitting is used to make estimates of convective organisation (dimensionality, area of convective precipitation, etc.).
Variability in UTDCDO at a given net latent heating rate is reduced in ICON with parameterised deep convection, compared to the convection-permitting set-up. Hints, but no conclusive results are found on the effect of dimensionality on the magnitude of UT divergent deep convective outflows. An impact of convective organisation and aggregation on UTDCDO is significant in the dataset: as a consequence of outflow collisions, UTDCDO increases sub-linearly with net latent heating. We also found a statistical relation between normalised UTDCDO and normalised convective momentum transport.  

How to cite: Groot, E., Kuntze, P., Miltenberger, A., and Tost, H.: Upper tropospheric convective outflow in ICON convection-permitting and parameterised set-up, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6532, https://doi.org/10.5194/egusphere-egu23-6532, 2023.

The sub-seasonal characteristics and prediction of rainfall over the Asian Monsoon Area during spring-summer transitional season (April-May-June) are investigated using a full set of hindcasts generated by the Dynamic Extended Range Forecast operational system version 2.0 (DERF2.0) of Beijing Climate Center, China Meteorological Administration. The onset and development of Asian summer monsoon and the seasonal migration of rain belt  over East Asia can be well depicted by the model hindcasts at various leads. However, there exist considerable differences between model results and observations, and model biases depend not only on lead time, but also on the stage of monsoon evolution. In general, forecast skill drops with  increasing lead time, but rises again after lead time becomes longer than 30 days, possibly associated with the effect of slowly-varying forcing or  atmospheric variability. An abrupt turning point of bias development appears around mid-May, when bias growths of wind and precipitation exhibit significant changes over the northwestern Pacific and South Asia, especially over the Bay of Bengal and the South China Sea. This abrupt bias change is  reasonably captured by the first two modes of multivariate empirical orthogonal function analysis, which reveals several important features associated  with the bias change. This analysis may provide useful information for further improving model performance in sub-seasonal rainfall prediction.

How to cite: Li, Q., Wang, J., and Yang, S.: Sub-seasonal Variations and Predictions of Precipitation over the Asian Monsoon Area with BCC_DERF2.0 in Spring-Summer Transition Season, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6653, https://doi.org/10.5194/egusphere-egu23-6653, 2023.

EGU23-7064 | ECS | Posters on site | AS1.1

Evaluation of Daily Temperature Extremes in the ECMWF ERA5 Reanalysis and Operational Weather Forecasts 

Francisco Lopes, Emanuel Dutra, and Souhail Boussetta

The daily maximum and minimum temperatures are among the most relevant meteorological variables in weather forecasts and climate monitoring. Their spatial and temporal evolution from synoptical to decadal scales are driven by numerous physical processes and climate feedbacks. Despite the significant improvements in weather forecasting over the last decades, forecasts of daily temperature extremes are still hampered by systematic errors. In this work we perform an integrated evaluation of the daily temperature extremes of the (i) ECMWF ERA5 reanalyses and (ii) ECMWF operational weather forecasts. The observations for the evaluation are taken from the Global Historical Climatology Network (GHCN) addressing: (i) the long-term assessment of the analysis produced by the ERA5 reanalysis, comprising a 40-year period (from 1980 to 2019); and (ii) the assessment of the ECMWF operational forecasts for a 5- year period (from 2017 to 2021). The evaluation carried out is global, however considering the GHCN station distribution and temporal availability, particular focus was given to four regions: Europe, Australia, East and West United States. The results identify a general underestimation of the daily maximum and overestimation of the daily minimum temperatures in both ERA5 analysis and operational forecasts, highlighting a known limitation of the ECMWF model in underestimating the diurnal temperature range. Our results also indicate a reduction of the errors in ERA5 when comparing the latest decade with the 1980’s, which is likely to be associated with an enhanced quality of the analysis due to a higher constrain emerging from the satellite data. The ERA5 analysis outperforms 1 day-ahead weather forecasts, which show some degree of improvement in the considered 5-year period, being associated with model upgrades.

 

This work was developed in the framework of the CoCO2 project. CoCO2 project has received funding from the European Union’s Horizon 2020 research and innovation programme under grant agreement No 958927.

How to cite: Lopes, F., Dutra, E., and Boussetta, S.: Evaluation of Daily Temperature Extremes in the ECMWF ERA5 Reanalysis and Operational Weather Forecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7064, https://doi.org/10.5194/egusphere-egu23-7064, 2023.

EGU23-7481 | ECS | Posters on site | AS1.1

Study of the 2 m temperature bias of the numerical weather forecasting model Arome over the French Alps 

Danaé Préaux, Ingrid Dombrowski-Etchevers, Isabelle Gouttevin, and Yann Seity

The Arome numerical weather prediction system is routinely used for weather forecasting over the mountains of the French Alps, Pyrénées and Corsica. However, its skills at temperature forecasting are altered by several 2 m temperature biases: (1) a cold bias at high altitude, (2) a low-altitude warm bias occurring in stably stratified layers and (3) a warm bias during snowfall situations.

Targeted numerical simulations (successive activation of some dynamic, physical and assimilation modifications) were carried out on the day of January 12, 2021, a problematic snowy situation in the Arve valley (Haute-Savoie, French Alps).

Over this period, the operational version of Arome has a mean absolute error (MAE) of 2.3°C in the valley. The increase of vertical resolution does not improve the performance of the model in the valley. The MAE is nevertheless decreased from 1.4 to 1.1°C in the mid-altitude range and from 1.5 to 1.2°C above 2000 m. Conversly, the use of a new surface scheme (ISBA-DIF) associated with a more complex snowpack model (ISBA-ES) allows to better represent the arrival of the warm front in the valley and reduces the error (to 1.8°C) whatever the altitude. The current surface scheme therefore seems too simplistic to correctly model soil-atmosphere interactions in the mountains. Forcing Arome with full-day data assimilation also reduces the bias in the valley (to 2.0°C). However, this experiment deteriorates the scores in the mid-altitude and high-altitude mountains. Furthermore, the situation has a poor initial state as biases are present even before the snow event starts. This may point towards deficiencies in the assimilation of in-situ data in mountain regions, that should be overcome in future work.

These results show that the warm bias during this snowy event has multiple origins. A carefull analysis of other situations will be needed to confirm and correct theses biases. 

How to cite: Préaux, D., Dombrowski-Etchevers, I., Gouttevin, I., and Seity, Y.: Study of the 2 m temperature bias of the numerical weather forecasting model Arome over the French Alps, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7481, https://doi.org/10.5194/egusphere-egu23-7481, 2023.

Infrasound waves generated by phenomena at the Earth’s surface can travel to these levels before returning to the surface and being detected. Observations like travel time, change in backazimuth angle, and trace velocity contain integrated information of all the levels the wave travelled through. These often include stratospheric and mesospheric levels which are otherwise poorly observed.
In this work we take a data assimilation technique, the Modulated Ensemble Transform Kalman Filter, which is commonly used in satellite data assimilation, and illustrate how it can be readily used for infrasound data assimilation. We highlight the similarities between the two problems, and the particular challenges in extracting information from summarised quantities. To our knowledge, this is the first work doing data assimilation with a full ray-tracing model as forward operator.

How to cite: Amezcua, J. and Näsholm, S. P.: Using satellite data assimilation techniques to combine infrasound observations and a full ray-tracing model to constrain atmospheric variables, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8665, https://doi.org/10.5194/egusphere-egu23-8665, 2023.

EGU23-8919 | Orals | AS1.1

PREVENIR: Japan-Argentina Cooperation Project for Heavy Rain and Urban Flood Disaster Prevention 

Takemasa Miyoshi, Celeste Saulo, Shigenori Otsuka, Juan Ruiz, Yanina G. Skabar, Arata Amemiya, Tomoo Ushio, Hirofumi Tomita, Tomoki Ushiyama, and Masaya Konishi

This presentation provides an overall summary of the project PREVENIR and recent activities about data assimilation and numerical weather prediction (NWP) research. PREVENIR is an international cooperation project between Argentina and Japan since 2022 for five years under the Science and Technology Research Partnership for Sustainable Development (SATREPS) program jointly funded by the Japan International Cooperation Agency (JICA) and the Japan Science and Technology Agency (JST). The main goal is to develop an impact-based early warning system for heavy rains and urban floods designed for two highly vulnerable urban basins in Argentina: one located in Buenos Aires Province and the other in Córdoba Province. PREVENIR takes advantage of leading research on simulations and Big Data Assimilation (BDA) with the Japan’s flagship supercomputer “Fugaku” and its predecessor “K” and develops a total package for disaster prevention, namely, monitoring, quantitative precipitation estimates (QPE), nowcasting, BDA and NWP, hydrological model prediction, warning communications, public education, and capacity building. Here, the Japanese leading institutions in the scientific research and operational services, i.e., RIKEN, Osaka University, the International Centre for Water Hazard and Risk Management (ICHARM), and the Japan Meteorological Agency (JMA) closely work with the Argentinian counterparts, i.e., the National Meteorological Service, the National Water Institute, and the National Research Council of Argentina under the strong support of JICA, JST, and Argentinian Foreign Affairs Ministry. Heavy rains and urban floods are important global issues under the changing climate. The total package for disaster prevention will be the first of its kind in Argentina and will provide useful tools and recommendations for the implementation of similar systems in other parts of the world.

How to cite: Miyoshi, T., Saulo, C., Otsuka, S., Ruiz, J., Skabar, Y. G., Amemiya, A., Ushio, T., Tomita, H., Ushiyama, T., and Konishi, M.: PREVENIR: Japan-Argentina Cooperation Project for Heavy Rain and Urban Flood Disaster Prevention, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8919, https://doi.org/10.5194/egusphere-egu23-8919, 2023.

EGU23-8950 | Posters on site | AS1.1

Exploring Domain Size for WRF High-Resolution Urban Rainfall Simulation 

Sichan Du, Lu Zhuo, Elizabeth J. Kendon, and Dawei Han

Abstract: With climate change, rainfall is expected to get more intense, leading to cities being increasingly at risk of urban flooding. Understanding local climate change over cities has therefore become a priority for the scientific community and city planners on building resilient cities and mitigating hydrometeorological disasters. Very high resolution (km-scale, ‘convection-permitting’) climate models are required to adequately represent cities and local rainfall extremes. Here we assess the Weather Research and Forecasting (WRF) model for simulating urban rainfall. Despite the wide application of WRF in rainfall simulations (including urban areas), there are limited investigations on the impact of the domain size and how to search for a suitable domain size over a particular city region.

To fill this knowledge gap, Newcastle upon Tyne is selected as the study area to simulate a summer heavy rainfall event with ERA5 (a fifth-generation dataset of global reanalysis developed by the European Centre for Medium-Range Weather Forecasts) as the input data and a radar product from the UK Met Office for validation. Accordingly, different domain sizes with the convection-permitting resolutions from 1 km to 4.5 km (increment: 0.5 km) are explored, and the hourly model outputs are compared with the radar observation data.

This study has proposed and tested a method to decide the most suitable domain size. By using eight assessment indexes (including pattern, cumulative time series, hourly time series, particular values (max/min/mean) as well as the seven statistical indicators of each data and overall data), there are two preliminary conclusions: 1) 200 km × 200 km is the best domain size for the single domain simulation; 2) For 200 km × 200 km or smaller domain sizes, higher resolution produces better results, but for 250 km × 250 km or large domain sizes, resolution sensitivity is opposite. Regarding next steps, the above procedure will be further investigated by applying it to more extreme rainfall case studies and to other cities in order to assess whether results here are generally applicable, and therefore the optimal domain configuration can be usefully applied to produce reliable urban rainfall simulations.

How to cite: Du, S., Zhuo, L., Kendon, E. J., and Han, D.: Exploring Domain Size for WRF High-Resolution Urban Rainfall Simulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8950, https://doi.org/10.5194/egusphere-egu23-8950, 2023.

EGU23-9199 | ECS | Orals | AS1.1

ECMWF-OpenIFS Climate Sensitivity to Horizontal Resolution and Time Step 

Abhishek Savita, Joakim Kjellsson, Robin Pilch Kedzierski, Wonsun Park, Mojib Latif, and Sebastian Wahl

We explored the sensitivity of the atmosphere general circulation model OpenIFS to horizontal resolution and time step. We conducted a series of experiments at different horizontal resolutions (i.e., 100, 50, and 25 km) while maintaining the same time step (i.e., 15 minutes), and using different time steps (i.e., 60, 30 and 15 minutes) at 100 km horizontal resolution. We find that the zonal wind bias over the Southern Ocean has significantly reduces at high horizontal resolution (i.e., 25 km), and that this improvement is evident too when using a coarse resolution model with smaller time step (i.e., 15 min and 100 km horizontal resolution). There is also evidence of improvements in the mid-latitude westerly jet in the Northern Hemisphere too, which is also sensitive to both model time step and horizontal resolution. We have also found that the biases in wave speed and wave amplitude reduce when we shorten the model time step or increase the model horizontal resolution. Therefore, it is clear that the improvement in the highest horizontal resolution (i.e., 25 km) simulation is a combination of both the enhanced horizontal resolution and shorter time step. We speculate that the improvement in the surface zonal wind bias in the coarse resolution with shorter time step (i.e., 15 min and 100 km horizontal resolution) simulation is mostly due to shallow convection that is intensified at shorter time step. In addition, we have also noticed improvements in the surface-air temperature when a high resolution and a smaller time step; however, the precipitation bias is independent of the model’s horizontal resolution and time step.

We propose based on OpenIFS that by reducing the time step in a coarse resolution atmospheric model (at least in OpenIFS), one can alleviate the surface-wind biases in the extratropics that is important for e.g., climate modeling in the Southern Ocean sector.

How to cite: Savita, A., Kjellsson, J., Pilch Kedzierski, R., Park, W., Latif, M., and Wahl, S.: ECMWF-OpenIFS Climate Sensitivity to Horizontal Resolution and Time Step, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9199, https://doi.org/10.5194/egusphere-egu23-9199, 2023.

Significant problems in numerical weather prediction modeling systems appear when the horizontal grid-spacing is between 20 km and 1 km and when deep convection is important. These scales are usually termed “Gray Scales”.  Techniques have been developed so that the behavior of the convective parameterization changes with the horizontal grid spacing of the model; such parameterizations are said to become “scale-aware”. Commonly used techniques involve applying a scaling approach to smoothly transition from parameterized to resolved convection. These are similar to an elegantly simple mathematical method originally developed by Arakawa et al. (2011), which scales the convective tendencies in dependence on the convective area fraction. Here we show that the scaling approaches are flawed, since they fail to consider the fact that the impacts of deep convection on those scales are not limited to one grid box, and usually – because of the scaling -- leads to light precipitation covering too much area, as we have previously shown in HRRR simulations. Any scaling approach is especially flawed in areas of light forcing (such as daytime heating) and in the tropics, when the explicit microphysics parameterization is not yet producing precipitation. We will show examples of these problems and discuss possible solutions as applied to NOAA’s new RRFS storm-scale modeling system.

How to cite: Grell, G., Li, H., and Freitas, S.: Flaws of scale-aware techniques in convective parameterizations, as discovered in NOAA’s operational convection-allowing modeling systems: an attempt to improve them., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10514, https://doi.org/10.5194/egusphere-egu23-10514, 2023.

A squall line system that occurred on 9-10 April 2016 over southern China was used to investigate the impact of incremental analysis update (IAU) initialization under the replay configuration on its forecasts. The ERA5 global reanalysis and the forecast field of the regional Weather Research and Forecasting (WRF) Model were used to construct the analysis increment. The results showed that IAU initialization reduced the imbalance caused by the introduction of the low-resolution global reanalysis into the high-resolution regional WRF model and retained the microphysical information in the forecast field of the regional WRF model, which reduced the spin-up time. Compared with the cold start run initialized directly by the ERA5 reanalysis, the linear structure and precipitation distribution of the squall line system using IAU initialization were closer to those in the observations. Further analyses indicated that the improvement of the squall line forecasts using IAU initialization was mainly related to the faster development of cold pool caused by retaining the microphysical information in the forecast field of the regional WRF model and the more favorable stratification conditions corrected by the IAU increment.

How to cite: gao, Y. and wang, X.: Impact of incremental analysis update initialization under the replay configuration on forecasts of a squall line event in southern China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11619, https://doi.org/10.5194/egusphere-egu23-11619, 2023.

EGU23-12177 | ECS | Orals | AS1.1

A multi-center exercise on the sensitivity of PAZ GNSS Polarimetric RO for NWP modeling 

Ramon Padullés, Estel Cardellach, Antía Paz, F. Joe Turk, Chi O. Ao, Kuo Nung Wang, Manuel de la Torre Juárez, Michael J. Murphy, Jennifer S. Haase, Katrin Lonitz, and Daisuke Hotta

A better understanding of the thermodynamics of heavy precipitation events is necessary towards improving weather and climate models and quantifying the impact of climate variability on precipitation. However, there are limited observations available to assess the thermodynamics model structure within heavy precipitation conditions.

In 2009, the Earth Observation Group at ICE-CSIC/IEEC conceived the polarimetric radio occultations (GNSS-PRO) technique with the aim to obtain simultaneous measurements of the vertical structure of precipitation and its associated thermodynamic state. Based on the standard GNSS radio occultation technique (GNSS-RO), polarimetric RO consists of an identical instrument working at two orthogonal linear polarizations (H,V) instead of the conventional circularly polarized antenna. This allows us to measure the differential phase delay at both ports, hypothesized to be positive in the presence of asymmetric hydrometeors (large raindrops, snowflakes, ice aggregates). This technique is being tested for the first time on the proof-of-concept mission Radio Occultations and Heavy Precipitation (ROHP) aboard PAZ satellite, operating since 2018. The results of the first 4 years of PRO observations already showed sensitivity to heavy precipitation and its associated cloud structures.

Such technique provides high quality thermodynamic observations of water vapor, temperature and pressure with high vertical resolution, along with the vertical measurements of the phase delay linked to the precipitation structure. This study focuses on comparing these observations with the simulations based on the outputs of several operational models and reanalysis for a set of selected cases. The main objectives of the study are: (1) To check if the models reproduce the main features of the actual data; (2) to assess whether different models/schemes result in different GNSS PRO observables, and whether these differences are larger than the measurement uncertainty; and (3) to examine the utility of PAZ GNSS PRO observations for model validation and diagnosis.

This effort provides insight on future methods to assimilate the PRO profile alongside other conventional (non-polarimetric) RO data, including work towards building a forward operator. The exercise includes comparisons with ECWMF operational model, ERA-5 reanalysis, the operational NWP at the Japan Meteorological Agency, and a near-real-time implementation of the WRF regional model over the northeastern Pacific produced at the Center for Western Weather and Water Extremes (CW3E) called West WRF, forced with ECMWF and GFS.

How to cite: Padullés, R., Cardellach, E., Paz, A., Turk, F. J., Ao, C. O., Wang, K. N., de la Torre Juárez, M., Murphy, M. J., Haase, J. S., Lonitz, K., and Hotta, D.: A multi-center exercise on the sensitivity of PAZ GNSS Polarimetric RO for NWP modeling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12177, https://doi.org/10.5194/egusphere-egu23-12177, 2023.

EGU23-12636 | ECS | Posters on site | AS1.1

Testing the AROME Hybrid 3DEnVar for convective-scale NWP over Austria 

Kaushambi Jyoti, Martin Weissmann, Philipp Griewank, and Florian Meier

Ensemble and hybrid ensemble-variational Data Assimilation (DA) methods incorporating ensemble-based flow-dependent error statistics into state estimation have emerged in recent decades. In a hybrid DA, the background error covariances are a combination of ensemble covariances and static climatology. The ensemble component provides flow-dependency and non-linear error growth critical for convective-scale models, and the static climatology mitigates the effects of a small ensemble size. Hybrid ensemble variational DA methods were recently implemented in the convective-scale NWP model AROME at Meteo-France.

We present our findings from testing Hybrid-3-Dimensional Variational Data Assimilation in convective-scale NWP model AROME over Austria. Given Austria's unique alpine orography, we investigate the impact of applying different weighting to flow-dependent covariances in hybrid DA for a summertime convection case over central Europe. In addition to the hybrid weights, we explore optimal ensemble size, the increase of ensemble size with a time-lagged approach as well as suitable localization settings. Finally, we compare our results to the 3-dimensional variational data assimilation (3DVar) operational model forecast of GeoSphere Austria and discuss the potential benefits, drawbacks, and challenges of using hybrid DA over traditional 3DVar.

Keywords: summertime convection; hybrid-3DEnVar; AROME NWP model; flow dependent background error covariance

How to cite: Jyoti, K., Weissmann, M., Griewank, P., and Meier, F.: Testing the AROME Hybrid 3DEnVar for convective-scale NWP over Austria, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12636, https://doi.org/10.5194/egusphere-egu23-12636, 2023.

EGU23-12877 | ECS | Orals | AS1.1

The influence of radiosonde observations on the sharpness and altitude of the tropopause 

Konstantin Krüger, Andreas Schäfler, George Craig, and Martin Weissmann

The shape, sharpness and altitude of the extratropical tropopause (TP) is strongly linked to the position and the strength of the subtropical and polar jet streams that determine the weather in the midlatitudes. However, current numerical weather prediction models fail to correctly represent the sharpness of the TP (i.e., the gradients of wind and temperature). In this study, we address the question if and how the assimilation of radiosonde observations influences the TP representation and whether it acts to sharpen or smooth near near-tropopause gradient.

We investigate the influence by comparing temperature, Brunt-Väisälä frequency (N²) and wind profiles of the observations (y), the model background (xb) and the analysis (xa) in tropopause-relative coordinates.

In total, we analyse more than 9000 radiosondes that were assimilated by the European Centre for Medium-Range Weather Forecast’s Integrated Forecast System (ECMWF IFS) over Canada, the Northern Atlantic and Europe during a one-month period in fall 2016. To test whether the diagnosed influence is caused by the assimilated radiosondes, we conducted a data denial experiment that excluded 500 radiosondes that were launched in the framework of the North Atlantic Waveguide and Downstream EXperiment (NAWDEX) field campaign. In observation space, we investigate the departures (i.e., the differences between y, xb and xa) in the control run (CTR) with all radiosondes considered and the denial run (DEN) without the NAWDEX radiosondes.

The observed minimum temperature at the TP is overestimated in the background forecast (warm bias, ~1 K). Above, in a layer 0.5-2 km, the temperature is underestimated (~0.5 K). Consequently, the sharpness of the TP which is diagnosed by the maximum of N² is also underestimated. We show that data assimilation is able to improve the temperature and to slightly strengthen the TP in the analysis, particularly in situations where the observed and model TP altitude fairly agree. In the data denial experiment we show that this influence exists in the CTR, but not in the DEN run, and thus can be attributed to the assimilation of the radiosonde data.

Regarding wind, we find an underestimation of the maximum wind at and below the TP (0.5-1 m s-1) and demonstrate that the assimilation of radiosonde winds is able to improve the wind profile across the TP. The bias and the positive influence are found to be stronger in situation of strong wind, i.e., the jet stream.

Although data assimilation is able to improve wind and temperature gradients across the tropopause by pulling the background closer to the observations, the individual analysis profiles still underestimate the sharpness of the tropopause. The misrepresented TP in models may impact the quality of weather and climate projections.

How to cite: Krüger, K., Schäfler, A., Craig, G., and Weissmann, M.: The influence of radiosonde observations on the sharpness and altitude of the tropopause, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12877, https://doi.org/10.5194/egusphere-egu23-12877, 2023.

EGU23-13110 | Orals | AS1.1

Recent progress and outlook for the ECMWF Integrated Forecasting System 

Gianpaolo Balsamo, Florence Rabier, Magdalena Balmaseda, Peter Bauer, Andy Brown, Peter Dueben, Steve English, Tony McNally, Florian Pappenberger, Irina Sandu, Jean-Noël Thepaut, and Nils Wedi

ECMWF recent improvements on scientific and technological fronts will be presented. In 2021 two new operational upgrades of the Integrated Forecasting System (IFS), cycles 47r2 and 47r3, have been introduced. In 2022 the ECMWF High-Performance Computing (HPC) facility has migrated from Reading, UK to a new data centre in Bologna, Italy, and on 18 October 2022 the operational system has been ported to a new supercomputer with enhanced capacity, that will pave the way for an increase in resolution in 2023 with the implementation of IFS cycle 48r1.

IFS Cycle 47r2 was first introduced on 11 May 2021 and its key features included changing the vertical resolution of the Ensemble forecast system (ENS) from 91 to 137 levels, the same used in the high-resolution forecast (HRES). This was made possible by introducing single precision arithmetic in both the HRES and ENS forecast systems. The single precision itself is neutral but enabled the ENS change which led to significant forecast skill improvement. Five months later, ECMWF introduced Cycle 47r3 operationally on 12 October 2021. This included major changes to the model physics that had been under development for several years. A more consistent formulation of boundary layer turbulence, new deep convection closure and cloud microphysics changes have increased the realism of the water cycle.

The next science upgrade, cycle 48r1, will be implemented in 2023 on our new HPC system in Bologna. This will see an enhancement of the ENS horizontal resolution to the TCo1279 grid (approximately 9km), the same resolution currently used by the HRES. There will also be an increase of the data assimilation resolution used in the incremental 4D-Var minimisation, and the use a new object orientated approach to run the 4D-Var atmospheric data assimilation (OOPS). Other important changes in 48r1 include running a daily 100 members extended range ensembles, introducing a new multi-layer snowpack model, and improving the atmospheric energy and water conservation.

Looking further ahead, future higher resolution capabilities will be accelerated by the digital twin developments under the European Commission Destination Earth programme, which will build km-scale capability for a range of potential future HPC architectures. Major efforts have been invested in the code scalability of the Integrated Forecasting System to be able to run on GPUs and investigating alternative dynamical core options. Data assimilation will evolve towards a fully coupled approach to maximise the exploitation of observations and benefit all components of the Earth system (atmosphere, land, ocean) in a consistent way. Machine Learning (ML) will be exploited to enhance the performance and efficiency of our systems. 

Finally, our Copernicus partnership with the European Commission has just entered its second phase. Synergistic interactions between meteorology and composition will be pursued for the mutual benefit of both and preparatory steps for next ECMWF climate reanalysis, ERA6, and new seasonal forecasting system, SEAS6, have already started. Several major upgrades in ERA6 and SEAS6 will aim at mitigating against systematic model biases to produce climate records with significantly improved time consistency, and enhanced reliability for extended-range predictions.

How to cite: Balsamo, G., Rabier, F., Balmaseda, M., Bauer, P., Brown, A., Dueben, P., English, S., McNally, T., Pappenberger, F., Sandu, I., Thepaut, J.-N., and Wedi, N.: Recent progress and outlook for the ECMWF Integrated Forecasting System, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13110, https://doi.org/10.5194/egusphere-egu23-13110, 2023.

EGU23-13449 | ECS | Posters on site | AS1.1

Ensemble-based regional reanalysis system for Central Europe: Development framework and outlook 

Alexander Kelbch, Thomas Spangehl, Michael Borsche, Thomas Rösch, and Florian Imbery

The development of regional reanalyses aims at the provision of high-resolution data sets that are suitable for climate applications and climate services. As the desired high-resolution information can barely be provided by either synoptic or remote sensing observation data, a growing interest in high-quality regional reanalyses is recognisable. Particular demand arises from the renewable energy sector. Further quality gains are expected by using an ensemble approach, e.g. by making available the desired uncertainty information when moving towards higher resolution. 
Within the framework of the Innovation Programme for applied Researches and Developments (IAFE) at Germany's national meteorological service (DWD) our project aims to develop and evaluate an operational ensemble-based regional reanalysis system incorporating the current NWP model of DWD (ICON). One final goal of the project is to provide a basic framework for user-oriented verification.  
We first present the Basic Cycling Environment (BACY) being mainly characterized by its modularity, robustness, user-friendlyness as well as its high complexity. Thus, our future reanalysis system will be a certain BACY version with "frozen" specifications. To assess BACY specifications such as model resolution, number of ensemble members, domain size and choice of output variables NWP simulations will be performed and first simulation results will be presented.

How to cite: Kelbch, A., Spangehl, T., Borsche, M., Rösch, T., and Imbery, F.: Ensemble-based regional reanalysis system for Central Europe: Development framework and outlook, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13449, https://doi.org/10.5194/egusphere-egu23-13449, 2023.

EGU23-14259 | ECS | Orals | AS1.1

Forecast sensitivity to the assimilation of observational data - two case studies for Australia 

Cassandra Rogers and Chris Tingwell

Australian weather forecasts use Numerical Weather Prediction (NWP) model output. Forecast accuracy is improved by assimilating a range of observational data which includes Australian Bureau of Meteorology station data. The significant investment by the Bureau of Meteorology in the national observing network, and the constant evolution of observational technologies, requires an ongoing assessment of the scientific value of the network components. Examining an objective measure of the impact of each assimilated observing system on the quality of short-term NWP forecasts can potentially guide planning and investment decisions related to network efficiency and effectiveness. 

Traditional techniques for assessing the impact of observations in NWP are inflexible (i.e. they require dedicated trials) and computationally expensive, but a widely used technique, known as adjoint-based Forecast Sensitivity to Observations (FSO), can provide forecast impact information continuously, flexibly, and in near real-time. We use archived FSO data to assess the relative forecast impact of in-situ data for different instruments and variables. We use two case studies to examine the impact of 1) three upper-air measurement instruments - radiosondes, aircraft, and a wind profiler - through the atmosphere at Sydney Airport, and 2) Automatic Weather Station surface observations along the Great Barrier Reef. These studies aim to provide network planners with information that can guide observations rationalisation decisions. 

How to cite: Rogers, C. and Tingwell, C.: Forecast sensitivity to the assimilation of observational data - two case studies for Australia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14259, https://doi.org/10.5194/egusphere-egu23-14259, 2023.

EGU23-14671 | ECS | Orals | AS1.1

A feature based perspective on upscale error growth. 

Sören Schmidt, Michael Riemer, and Tobias Selz

Atmospheric predictability is fundamentally limited by the upscale growth of initial small-scale, small-amplitude errors. Studying upscale error growth mechanism is essential to better understand this fundamental limitation. Upscale error growth is frequently investigated by spectral analysis. By design, however, spectral analysis is non-local. A local investigation of error growth in different flow configurations is desirable, though, to study the well-known flow dependence of error growth. We thus take here a complementary approach to spectral analysis and identify local regions of prominent errors as “error features”.

We have developed an automated algorithm to identify error features in gridded data and track their spatial and temporal evolution. Errors are considered in terms of potential vorticity (PV) and near the tropopause, where they maximize. A previously derived PV-error tendency equation is evaluated to quantify the different contributions to error growth in previously published upscale error growth experiments with the global prediction Model ICON from the German Weather Service. Errors in these experiments grow from very small initial-condition uncertainty (three orders of magnitude smaller than current-day uncertainty) and due to differences in the seeding of a stochastic convection scheme.

Spatial composites centered on the centroid of error features indicate that features are primarily generated ahead of an upper-tropospheric trough. The environment surrounding the features at the time of their first detection is characterized by locally enhanced lower to mid tropospheric moisture, latent heat release, and upper tropospheric divergence. Subsequently, this moist-diabatic nature of the error environment becomes gradually less prominent. The evaluating of process specific error growth rates enables to quantify the upscale growth mechanics in more detail. For this purpose, we integrate the growth rates over the respective area associated with an error feature. Examination of the combined growth rates of all features reproduces the previously found three-phased multi-scale upscale growth paradigm: Errors are first generated on the small scale by differences in latent heat release, then projected onto the tropopause region by associated differences in upper tropospheric divergent outflow, and finally amplified by nonlinear Rossby wave dynamics. The growth rates from a single feature, however, can substantially differ from the mean picture. Some features, e.g., go through the described stages in a cyclic sequence, and the main focus of the presentation will be on the differences between fast and slowly amplifying error features.

How to cite: Schmidt, S., Riemer, M., and Selz, T.: A feature based perspective on upscale error growth., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14671, https://doi.org/10.5194/egusphere-egu23-14671, 2023.

Precipitation characteristics are expected to change in the future as a consequence of global climate change. For example, high-intensity precipitation is expected to become more frequent in some areas of the world. The short time scales and small spatial scales of intense precipitation events pose challenges for numerical weather prediction (NWP) models. Measurements of precipitation characteristics from in-situ and remote sensing instrumentation are often available at much higher time resolution than common NWP model output, and need to be aggregated for validation studies. Here we present a methodology to enable the comparison of precipitation observations and model output at the time scale of the model time steps. Our analysis is focused on an extreme, convective precipitation event during 30th July 2019 in Bergen, Norway (60.38ºN, 5.33ºE, 12 m a.s.l.). We use high-resolution measurements of precipitation characteristics from a Micro Rain Radar Metek MRR-2, an Ott Parsivel2 Disdrometer, and a TPS-3100 Hotplate Pluviometer. Model precipitation was extracted from the operational NWP model MetCoOp that uses a horizontal grid spacing of 2.5 km and 65 vertical levels as part of the HARMONIE AROME model configuration. Using DDH (Diagnostics par Domaines Horizontaux), a novel tool for extracting prognostic variables from the model at a time-step resolution, we extracted a detailed dataset from a NWP model reforecast at every time step (75s), for a 62.5 by 62.5 km subdomain centred around the measurement site. We characterised precipitation by investigating five parameters, namely rain rate, liquid water content, mean volume diameter, the normalised intercept parameter, and terminal fall velocity. The newly developed methodology enabled a direct comparison of the observed precipitation characteristics with corresponding parameters from the model prediction for the convective rainfall event. Despite a generally reasonable correspondence between all parameters in the model and observations, the model struggled with underestimation of rainfall intensity during the high-intensity periods. The onset and intensity of precipitation depended strongly on location for the investigated event. Higher time resolution provided more detailed insight into intensity, timing and spatial variability of the modelled precipitation compared to the more commonly used hourly interval. Our new methodology can be easily applied to other precipitation events, such as frontal rainfall events, and thus provide process-level understanding of precipitation characteristics simulated by high-resolution NWP models. 



How to cite: Steinslid, M., Sodemann, H., and Kähnert, M.: Enabling the comparison of high-resolution precipitation observations with numerical weather prediction model simulations at every model time-step, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14882, https://doi.org/10.5194/egusphere-egu23-14882, 2023.

EGU23-15208 | Posters on site | AS1.1

Methods of weather forecasting and navigation in the N-Atlantic in the Middle Ages tested with a modern NWP tool 

Haraldur Ólafsson, Philipp Weitzel, Iman Rousta, Benoît Soula, and Léo Jacopin

Weather forecasting in the Middle Ages was most likely mostly based on persistence, and there are indications that persistence and correlation between elements of the sensible weather, in particular fog, helped in navigation in the N-Atlantic during the Viking age.

Investigation of the weather in the CARRA dataset, produced by dynamic downscaling, reveals that the connection between wind directions and fog is different on the leg between Iceland and Greenland from what it is between Iceland and Norway.  Consequently, the same navigational rules could not be applied on both these legs, making navigation from Iceland to Greenland even more difficult than navigation from Norway to Iceland.  This, in addition to very high frequency of fog and of strong winds in the vicinity of Greenland, made sailing and navigation between Iceland and the Medieval Nordic settlements in Greenland exceptionally difficult.    

How to cite: Ólafsson, H., Weitzel, P., Rousta, I., Soula, B., and Jacopin, L.: Methods of weather forecasting and navigation in the N-Atlantic in the Middle Ages tested with a modern NWP tool, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15208, https://doi.org/10.5194/egusphere-egu23-15208, 2023.

Numerical weather prediction (NWP) models are frequently used tools in operational weather forecasting. The NWP bases on current weather observations and processing of this data using computational models to forecast possible weather conditions. The aim of the study was to determine the optimal configuration of the Weather Research and Forecasting (WRF) model , version 4.2 (Skamarock et al. 2008), for more effective weather forecasting for the area of Poland. For model evaluation, we used observations from the IMWM-NRI network (above 50 meteorological stations). Numerical simulations were run using GFS model data was obtained from NOAA's NCEP servers. The WRF model was configured for a 3 km horizontal resolution grid, using unique parameterization settings for this model. Validation of forecast data was performed using statistical measures recommended by the WMO, e.g. mean error, mean absolute error, mean squared error, showing the values of forecast error. In this study, the model settings were configured based of other papers for Europe (Stergiou et al. 2017, Mooney et al. 2013, Kioutsioukis et al. 2016, Garcia-Diez et al. 2015, Carvalho et al. 2014, Santos Alamillos 2013), especially from its central part (Wałaszek et al. 2014, Kryza et al. 2017). The results of the work present statistical summaries of optimal model parameterization schemes, depending on their verifiability. Model configuration characterized by the best performance will be further examined over a longer time period (in the study, the average MAE for air temperature was 0.8°C). The research was funded by National Science Center (project number: 2017/27/N/ST10/00565)

How to cite: Kendzierski, S.: Influence of resolution and parameterization of the WRF model on the verifiability of weather forecast, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15595, https://doi.org/10.5194/egusphere-egu23-15595, 2023.

EGU23-15927 | Orals | AS1.1

Potential of accumulated parameterisation tendencies from AROME-Arctic for stochastic parameterisation erturbation patterns 

Harald Sodemann, Marvin Kähnert, Teresa Maaria Remes, Petter Ekrem, Rafael Grote, and Inger-Lise Frogner

Stochastic parameterisations are an important way to represent uncertainty in the deterministic forecasting models underlying ensemble prediction systems. Current stochastic parameterisation approaches use random correlation patterns that are unrelated to the atmospheric flow to induce coherent perturbations to parameterisations. Here we replace these patterns by accumulated tendency fields from parameterized physical processes in the HARMONIE-AROME system. Our rationale is that by perturbing the parameterisations with a field that reflects where parameterisations are most active, rather than random, the model obtains a more targeted increase in the degrees-of-freedom to represent forecasting uncertainty.

Here we study a large marine cold-air outbreak over the Norwegian Sea. Strong heat fluxes persisted near the ice edge, and shallow convection dominated in the center of the model domain. Perturbation fields are diagnosed from individual tendency diagnostics implemented in AROME-Arctic within ALERTNESS. Total physical tendencies for the horizontal winds, for temperature and humidity are accumulated with a time filtering throughout the 66 h forecast period.

Accumulated tendencies show overlapping and differing centers of activity. Wind parameterisations are active near the ice edge, and with smaller scale variability over land areas. Temperature tendency patterns show activity more confined to the ice edge, and the coast of northern Scandinavia. Such spatially coherent patterns of parameterisation activity are meaningfully related to current weather. To exploit the relation between parameterisation activity and weather patterns for ensemble perturbation, we conduct sensitivity tests of cloud parameterisation parameters in a single-column model version MUSC and the full model version. First results illustrate our progress towards the use of diagnostic perturbation patterns for stochastically perturbed perturbations in the HarmonEPS system.

How to cite: Sodemann, H., Kähnert, M., Remes, T. M., Ekrem, P., Grote, R., and Frogner, I.-L.: Potential of accumulated parameterisation tendencies from AROME-Arctic for stochastic parameterisation erturbation patterns, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15927, https://doi.org/10.5194/egusphere-egu23-15927, 2023.

EGU23-16670 | Orals | AS1.1

EURO1k: A high-resolution European weather model developed by Meteomatics 

Julie Thérèse Pasquier, Johannes Rausch, Alexander Stauch, and Martin Fengler

Accurate and precise weather forecasting is essential for a wide range of applications and industries, from agriculture to transportation to renewable energy. However, current weather models often struggle to represent the weather accurately due to limitations in spatial resolution. Global models with broad resolution are unable to represent small-scale weather features, such as convective thunderstorms or local wind patterns, while regional high resolution models are highly dependent on boundary conditions and typically provide forecasts for a small domain. To fill this gap, Meteomatics has developed the EURO1k model, the first pan-European weather model with a 1km2 resolution.

 

The EURO1k model consists of approximately 20 million grid points and is run 24 times per day, with a forecast horizon of 24 hours. It is based on the WRF (Weather Research and Forecasting) model and uses global ECMWF-IFS model data for boundary conditions. In addition to standard data sources such as weather stations, radar and satellite data, and radiosondes, the EURO1k model also ingests data from a network of Meteodrones, small unmanned aircraft systems (UAS) developed by Meteomatics which collect vertical atmospheric profiles up to 6000m in altitude. The high resolution of the EURO1k model allows it to accurately represent small-scale weather patterns, resulting in highly accurate and precise forecasts. This is evident in verifications against weather station observations, which show a very good agreement between model output and a range of weather variables including wind, temperature, and radiation.

 

Statistical analyses of EURO1k model output against observations from 5000 weather stations in Europe demonstrate better accuracy compared to other global and regional models. This has important implications for industry and the public. The EURO1k model can improve the forecasting of extreme weather events, allowing for better preparation and response. It can also enhance the prediction of renewable energy production, which depends on weather conditions. This increases the cost efficiency of renewable energies and help to reduce CO2 emissions. And, most importantly, it provides a more accurate and reliable weather forecast for communities across Europe. Overall, the EURO1k model represents a major advance in numerical weather prediction, bringing improved understanding and forecasting of the weather to a wide range of users.

How to cite: Pasquier, J. T., Rausch, J., Stauch, A., and Fengler, M.: EURO1k: A high-resolution European weather model developed by Meteomatics, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16670, https://doi.org/10.5194/egusphere-egu23-16670, 2023.

EGU23-16972 | Orals | AS1.1

LiDAR-based data assimilation during offshore transient events 

Mostafa Bakhoday-Paskyabi, Hai Bui, and Mohammadreza Mohammadpour Penchah

Atmospheric conditions and instabilities affect directly the performance of modern large offshore wind farms and several offshore operations, particularly farther offshore in deep waters. However, our current knowledge regarding to the atmospheric processes over a wide range of spatiotemporal scales needs further improvements by the use of measurements, and sophisticated modelling of Marine Atmospheric Boundary Layer (MABL) processes relevant to the offshore wind energy. Processes like gravity waves, Open Convective Cells (OCCs), Low Level Jets (LLJs) affect both horizontal and vertical structures of MABL flow fields and the interactions between the ambient flow and offshore constructions. For example, LLJs are common physical processes over the Southern North Sea. These transient events occur during stably stratified atmosphere with jet cores at heights between 150 m and 300 m. Strong positive and negative shears are observed below and above the nose of LLJ (i.e a maxima in the vertical wind profile). Structure, timing, shape, and characteristics of LLJs influence the loads on turbines and the overall power generation of offshore wind parks. Therefore, precise modelling and measurement of these episodes are highly important.

While advanced measurement systems such as LiDAR provides important information on formation and characteristics of LLJs, such measurements are sparse in time and space. On the other hand, modelling tools are sensitive in prediction of LLJ characteristics such as LLJ’s height, spatial position, and timing, the choice of initial and boundary conditions, and planetary boundary layer schemes used in the Numerical Weather Prediction models (NWPs).  Predictive skills of these models can be enhanced through assimilation of available quality observational data with NWPs like Weather Research and Forecasting (WRF) model.

 

In this study, we use the WRF model to model wind variability for a geographical area covering the FINO1 offshore meteorological met-mast and Alpha Ventus offshore wind park (in the Southern North Sea). We first examine the performance of WRF, with an appropriate configuration, in forecasting few LLJ events. We then apply a LiDAR-based data assimilation (for sometimes during 2015) and study how different DA techniques (namely observational nudging and 3DVAR) can improve the accuracy of wind forecasting and reduce the model uncertainity during the LLJ events.

How to cite: Bakhoday-Paskyabi, M., Bui, H., and Mohammadpour Penchah, M.: LiDAR-based data assimilation during offshore transient events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16972, https://doi.org/10.5194/egusphere-egu23-16972, 2023.

EGU23-16973 | Posters on site | AS1.1

Development of a New Microphysics Scheme with In-Cloud Processes for Weather Forecasting 

Songyou Hong, Haiqin Li, JIan-Wen Bao, and Jimy Dudhia

A new double-moment parameterization with in-cloud microphysical processes is developed for use in weather forecasting and climate studies. A main ingredient of the scheme utilizes a concept to represent the partial cloudiness effect on the microphysical processes, following the study of Kim and Hong (2018). The underlying assumption is that all the microphysical processes occur in a cloudy part of the grid box. Based on the long-term evaluation of the WRF Single-Moment (WSM) and WRF Double-Moment (WDM) schemes by WRF community, several revisions are made in microphysics terms, along with a newly introduced aerosol effect in ice processes. An aerosol-aware feature with prognostic aerosol emissions of sea salt, dust, anthropogenic and wildfire organic carbon for CCN is also designed. A mass-conserving Semi-Lagrangian sedimentation is re-configured for double-moment physics, which is superior to the conventional Eulerian algorithm in the context of the computational accuracy and numerical accuracy. The new scheme reproduces the storm structure in an idealized 2D testbed, accompanying better organized front-to-rear jets, cold pools, and convective updrafts, as compared to the results in the case of conventional microphysics. The wall-clock time is about a half in the US NOAA/GFS model, as compared to that of Thompson scheme.

How to cite: Hong, S., Li, H., Bao, J.-W., and Dudhia, J.: Development of a New Microphysics Scheme with In-Cloud Processes for Weather Forecasting, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16973, https://doi.org/10.5194/egusphere-egu23-16973, 2023.

EGU23-17383 | Orals | AS1.1

Automatic generation of a text forecast along a track 

Einar H. Guðmundsson, Ólafur Rögnvaldsson, and Karolina Stanislawska
Belgingur Ltd. has created a novel weather forecasting framework, called Weather On Demand – WOD, that can be deployed in the cloud and customised for any location world-wide at a very short notice.
 
A recent addition to the WOD system is a routing forecast option that generates a simple text forecast along a track provided by the end-user.
 
The process is such that a user provides a list of coordinates, where each coordinate pair is accompanied by a timestamp, via an API.

Points of interest are identified along the track. Most commonly these points are the locations of weather stations, as they are generally placed where weather conditions are of interest and the WOD system has additional machine learning interpolation mechanisms in development for weather stations. From this set, along with on-the-hour locations, a representative, refined, lower resolution track is assembled, for which high-resolution forecast data is pulled.

From that forecast data, the information most relevant to the user is highlighted. Any difficult conditions, as well as a segmented summary is generated in simple, succinct text, programmable in any language.

An ongoing extension of this feature is to develop a module that can create a simple text forecast for any user defined region.

The WOD software is maintained in Git and can be installed on suitable hardware in a matter of hours, bringing the full flexibility and power of the WRF modelling system at your fingertips.

How to cite: Guðmundsson, E. H., Rögnvaldsson, Ó., and Stanislawska, K.: Automatic generation of a text forecast along a track, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17383, https://doi.org/10.5194/egusphere-egu23-17383, 2023.

EGU23-17484 | Posters on site | AS1.1

Evaluating the Performance of WRF-Solar Model for 72-Hour Ahead Global Horizontal Irradiance Forecasting in West Africa: A Case Study of Ghana 

Windmanagda Sawadogo, Benjamin Fersch, Jan Bliefernicht, Stefanie Meilinger, and Harald Kunstmann

Accurate forecasting of solar irradiance is crucial for the integration of solar energy into the
power grid, power system planning, and the operation of solar power plants. The Weather
Research and Forecasting (WRF) model, with its solar radiation (WRF-Solar) extension, has
been used to forecast solar irradiance in various regions worldwide. However, the application
of the WRF-Solar model for global horizontal irradiance (GHI) forecasting in West Africa,
specifically in Ghana, has not been studied. This study aims to evaluate the performance of
the WRF-Solar model for GHI forecasting in Ghana, focusing on 3 health centers (Kologo,
Kumasi and Akwatia) for the year 2021. We applied a two one-way nested domain (D1=15
km and D2=3 km) to investigate the ability of the WRF solar model to forecast GHI up to 72
hours in advance under different atmospheric conditions. The initial and lateral boundary
conditions were taken from the ECMWF operational forecasts. In addition, the optical aerosol
depth (AOD) data at 550 nm from the Copernicus Atmosphere Monitoring Service (CAMS)
were considered. The study uses statistical metrics such as mean bias error (MBE), root mean
square error (RMSE), to evaluate the performance of the WRF-Solar model with the
observational data obtained from automatic weather stations in the three health centers in
Ghana. The results of this study will contribute to the understanding of the capabilities and
limitations of the WRF-Solar model for forecasting GHI in West Africa, particularly in
Ghana, and provide valuable information for stakeholders involved in solar energy generation
and grid integration towards optimized management of in the region.
Keywords: WRF-Solar; Global horizontal irradiance; Forecasting; West Africa; Ghana

How to cite: Sawadogo, W., Fersch, B., Bliefernicht, J., Meilinger, S., and Kunstmann, H.: Evaluating the Performance of WRF-Solar Model for 72-Hour Ahead Global Horizontal Irradiance Forecasting in West Africa: A Case Study of Ghana, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17484, https://doi.org/10.5194/egusphere-egu23-17484, 2023.

EGU23-17562 | Orals | AS1.1

Cut-cell Eta ensemble skill vs. ECMWF: Lessons learned 

Fedor Mesinger, Katarina Veljovic, Sin Chan Chou, Jorge L. Gomes, André A. Lyra, and Dušan Jovic

An experiment reported in Mesinger and Veljovic (JMSJ 2020) showed an
advantage of the Eta over its driver ECMWF ensemble members in placing 250 hPa jet
stream winds during a period of an upper tropospheric trough crossing the Rockies. A
byproduct of that experiment was that of the Eta ensemble switched to use sigma,
Eta/sigma, also achieving 250 hPa wind speed scores better than their driver members,
although to a lesser extent. Nevertheless, it follows that the Eta must include feature or
features additional to the eta coordinate responsible for this advantage over the
ECMWF.
An experiment we have done strongly suggests that the van Leer type vertical
advection of the Eta, implemented in 2007, is a significant contributor to this advantage.
In this experiment, having replaced a centered finite-difference Lorenz-Arakawa scheme
this finite-volume scheme enabled a successful simulation of an intense downslope
windstorm in the lee of the Andes.
While apparently a widespread opinion is that it is a disadvantage of terrain
intersecting coordinates that “vertical resolution in the boundary layer becomes reduced
at mountain tops as model grids are typically vertically stretched at higher altitudes,” a
very comprehensive 2006 NCEP parallel test gave just the opposite result. With
seemingly equal ABL schemes, the Eta showed a higher surface layer accuracy over
high topography than the NMM, using a hybrid terrain-following system (Mesinger, BLM
2022).
Hundreds of thousands of the Eta forecasts and experiments performed
demonstrate that the relaxation lateral boundary conditions almost universally used in
regional climate modeling (RCM)–in addition to conflicting with the properties of the
basic equations used–are unnecessary. Similarly, frequently applied in RCMs so-called
large scale or spectral nudging, being based on an ill-founded belief, should only be
detrimental if possible numerical issues of the limited area model used are addressed.
Note that this is confirmed by the results we refer to above.

How to cite: Mesinger, F., Veljovic, K., Chou, S. C., Gomes, J. L., Lyra, A. A., and Jovic, D.: Cut-cell Eta ensemble skill vs. ECMWF: Lessons learned, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17562, https://doi.org/10.5194/egusphere-egu23-17562, 2023.

EGU23-1129 | ECS | Posters virtual | AS1.2

High-resolution hail detection: probability of occurrence and size of hailstones based on weather radar data 

Krystian Specht, Jan Szturc, and Anna Jurczyk

The HAIL application was developed and implemented in the Institute of Meteorology and Water Management – National Research Institute (IMGW) as a component of the MeteoWarn system of detection and forecasting of dangerous weather phenomena. The application contains two algorithms: (i) hail detection and probability estimation; (ii) estimation of the maximum hail size that occurs in the event.

The probability of hail is determined using own hail detection algorithm based on fuzzy logic using the following weather radar products: the differential reflectivity (ZDR) and the exceedance of 0°C isotherm for echo top 40, 45, 50 dBZ (EHT40, EHT45, EHT50). Threshold have been introduced for the parameters to prevent false hail detection, above which hail is possible to occur. Additionally some other radar parameters: maximum reflectivity (CMAX), vertically integrated liquid water (VIL), constant altitude plan position indicator (CAPPI) on 4 km, and EHT are checked. The maximum hail size is calculated from the parameters: VIL, EHT50, and isotherm 0°C.

The developed algorithms were verified by observations in meteorological stations staffed by trained observers. The stations are limited to specific locations, but they are the most reliable and precise source of data about weather phenomena. Verification data for calibration are observations from synoptic stations and for hail size additionally observations from the European Severe Weather Database (ESWD). The results of the verification show good enough reliabilities of the two HAIL products. Validation based on the contingency table provided the following results: the probability of detection (POD) is 0.99, the false alarm ratio (FAR) is 0.02, and the critical success index (CSI) is 0.98. POD of no hail is 0.39, FAR is 0.38, and CSI is 0.31.

How to cite: Specht, K., Szturc, J., and Jurczyk, A.: High-resolution hail detection: probability of occurrence and size of hailstones based on weather radar data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1129, https://doi.org/10.5194/egusphere-egu23-1129, 2023.

EGU23-1345 | ECS | Orals | AS1.2

A Deep Learning-Based Bias Correction Method for Predicting Ocean Surface Waves in the Northwest Pacific Ocean 

Danyi Sun, Wenyu Huang, Yong Luo, Jingjia Luo, Jonathon S. Wright, Haohuan Fu, and Bin Wang

Ocean waves, especially extreme waves, are vital for air-sea interaction and shipping. However, current wave models still have significant biases, especially under extreme wind conditions. Based on a numerical wave model and a deep learning model, we accurately predict the significant wave height (SWH) of the Northwest Pacific Ocean. For each day in 2017-2021, we conducted a 3-day hindcast experiment using WAVEWATCH3 (WW3) to obtain the SWH forecasts at lead times of 24, 48, and 72hr, forced by GFS real-time forecast surface winds. The deep learning-based bias correction method is BU-Net by adding batch normalization layers to a U-Net, which could improve the accuracy. Due to the use of BU-Net, the mean Root Mean Squared Errors (RMSEs) of the SWH forecast from WW3 at lead times of 24, 48, and 72hr are reduced from 0.35m to 0.21m, 0.39m to 0.24m, and 0.43m to 0.30m, corresponding to drop percentages of 40%, 38%, and 30%, respectively. During typhoon passages, the drop percentages of RMSEs reach 45%, 42%, and 35% for three lead times. Therefore, combining numerical models and deep learning algorithms is very promising in ocean wave forecasting.

How to cite: Sun, D., Huang, W., Luo, Y., Luo, J., Wright, J. S., Fu, H., and Wang, B.: A Deep Learning-Based Bias Correction Method for Predicting Ocean Surface Waves in the Northwest Pacific Ocean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1345, https://doi.org/10.5194/egusphere-egu23-1345, 2023.

EGU23-1777 | Orals | AS1.2

Improving the ensemble forecast of precipitation in Europe by combining a stochastic weather generator with dynamical models  

Meriem Krouma, Lauriane Batté, Linus Magnusson, Damien Specq, Constantin Ardilouze, and Pascal Yiou

Ensemble forecasts of precipitation with sub-seasonal lead times offer  useful information for decision makers when they sufficiently sample the possible outcomes of trajectories. In this study, we aim to improve  precipitation ensemble forecast systems using a stochastic weather generator (SWG) based on analogs of the atmospheric circulation. This approach is tested for sub-seasonal lead times (from 2 to 4 weeks). The SWG ensemble forecasts  yield promising probabilistic skill scores for lead times of 5-10 days for precipitation (Krouma et al, 2022) and for lead times of 40 days for temperature   (Yiou and Déandréis, 2019) . In this work, we adapt the parameters of the SWG to optimize the simulation of European precipitations from ensemble dynamical reforecasts of ECMWF and CNRM. We present the HC-SWG forecasting tool (HC refers to Hindcast and SWG to the stochastic weather generator) based on a combination of dynamical and stochastic models.

We start by computing analogs of Z500 from the ensemble member reforecast of ECMWF (11 members) and CNRM (10 members). Then, we generate an ensemble of 100 members for precipitation over Europe. We evaluate the ensemble forecast of the HC-SWG using skill scores such as the continuous probabilistic score CRPS and ROC curve.

We obtain reasonable forecast skill scores for lead times up to 35 days for different locations in Europe (Madrid, Toulouse, Orly, De Bilt and Berlin). We compare the HC-SWG forecast with other precipitation forecasts to further confirm the benefit of our method. We found that the HC-SWG shows improvement against the ECMWF precipitation forecast until 25 days.

 

How to cite: Krouma, M., Batté, L., Magnusson, L., Specq, D., Ardilouze, C., and Yiou, P.: Improving the ensemble forecast of precipitation in Europe by combining a stochastic weather generator with dynamical models , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1777, https://doi.org/10.5194/egusphere-egu23-1777, 2023.

EGU23-4735 | Orals | AS1.2

GAN-based forecasting model via self-adaptive clustering approach 

Sojung An, Tae-Jin Oh, Inchae Na, Jiyeon Jang, Wooyeon Park, and Junghan Kim

Deep learning has been rapidly adopted in short-term precipitation prediction, such as simulating precipitation movement and predicting extreme weather events. Recently, generative adversarial neural networks (GANs) have been shown to be effective at dealing with field smoothing with increasing lead time. Several studies (Jing et al., 2019; Ravuri et al., 2021) demonstrated the potential of GAN by solving spatial smoothing problems and demonstrating reliable predictive performance. However, despite promising results from GANs, unbalanced datasets and human annotations can limit the predictive ability of deep learning and induce biased results. In addition, precipitation is a complex process that depends on various factors. Thus, approximating the model into a single latent space is a challenge, and furthermore, there is a risk of mode collapse. This study introduces an algorithm for predicting precipitation by clustering precipitation types using self-supervised learning (SSL) and estimating rainfall distribution according to precipitation types. First, we derive precipitation-type labels by self-clustering a generator that is a multi-layer ConvGRU. And then, we predict six-hour precipitation based on the gaussian distribution of each type. SSL improves the performance of precipitation forecasting based on type-specific representation learning through adaptive sampling in latent space. The proposed methodology was verified using hybrid surface rainfall (HSR) dataset at a spatial resolution of 500m with a resolution of 2,305 (longitude) × 2,881 (latitude) and a temporal resolution of 5 min. The images consist of 256×256 pixels from scaling down to a resolution of 4 km and are extracted at 30-minute intervals. Experimental results show that our method outperforms a state-of-the-art method on a six-hour prediction basis with a mean squared error and critical success index on unseen datasets. Also, the proposed algorithm can predict various precipitation types without spatial smoothing.

How to cite: An, S., Oh, T.-J., Na, I., Jang, J., Park, W., and Kim, J.: GAN-based forecasting model via self-adaptive clustering approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4735, https://doi.org/10.5194/egusphere-egu23-4735, 2023.

EGU23-5837 | Orals | AS1.2

Generating weather symbol data in IMPROVER 

Stephen Moseley, Ben Ayliffe, and Gavin Evans

The UK Met Office is developing an open-source probability-based post-processing system called IMPROVER (Integrated Model Post-Processing and Verification) to fully exploit our convection permitting, hourly cycling ensemble forecasts.  Post-processed MOGREPS-UK model forecasts are blended with deterministic UKV model forecasts and data from the coarser resolution global ensemble, MOGREPS-G, to produce seamless probabilistic forecasts from now out to 7 days ahead. For precipitation, an extrapolation nowcast is also blended in at the start.

A majority of the post-processing within IMPROVER is performed on gridded forecasts, with site-specific forecasts extracted as a final step, helping to ensure consistency. IMPROVER delivers a wide range of probabilistic products to both operational meteorologists and as input to automated forecast production. The system achieved operational acceptance in spring 2022 and will be used in operational products from spring 2023.

Weather symbols provide the general public with a simple, pictorial view of the weather for a time of interest and include sun and cloud conditions, mist and fog, hail and lightning, and three phases of precipitation, both as showers or continuous, and light or heavy. This talk describes how a deterministic most-likely weather type code is generated using a decision tree approach from probabilistic multi model IMPROVER data for 1 hour, 3 hour and daytime periods that are consistent with each other. Recent work to make these weather codes representative of a time-window, rather than an instant, will be discussed. We will present some verification, comparing IMPROVER weather symbols and the current operational Met Office symbols with SYNOP present weather reports.

How to cite: Moseley, S., Ayliffe, B., and Evans, G.: Generating weather symbol data in IMPROVER, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5837, https://doi.org/10.5194/egusphere-egu23-5837, 2023.

EGU23-7214 | Posters on site | AS1.2

Weather forecast downscaling for applications in smart agriculture 

Francesco Di Paola, Sabrina Gentile, Nicola Genzano, Elisabetta Ricciardelli, Filomena Romano, and Valerio Tramutoli

In the framework of the On Demand Services For Smart Agriculture (OD4SA) project, funded by PO FESR 2014-2020 from Regione Basilicata, Italy, a weather forecast service has been developed, for applications in smart agriculture and precision farming. It is based on the Weather Research and Forecasting (WRF) model and provides a daily 96-hour forecast of temperature and water vapor at 2 m altitude, wind speed and direction at 10 m altitude, atmospheric pressure, solar irradiance, and 1-hour accumulated rainfall, for the Southern Italy. Although encouraging advances in microscale modeling have been achieved in the last decade, the computational costs imposed by the state of the art do not allow for continuous operational forecasting at the sub-kilometer scale, useful for precision farming, especially in southern Italy that is characterized by a complex orography. To overcome this limit, an algorithm based on some Artificial Neural Networks (ANNs) has been developed, by using the WRF Large Eddy Simulation (LES) to build the training database at 240 m spatial resolution. Particular attention was paid to the analysis of the true spatial resolution of the WRF-LES outputs, to the definition of the ANNs topology and to the input selection, from over 250 inputs more than half has been discarded. The preliminary results show RMSE equal on average to 70% of those obtained by using the most common spatial interpolation methods.

How to cite: Di Paola, F., Gentile, S., Genzano, N., Ricciardelli, E., Romano, F., and Tramutoli, V.: Weather forecast downscaling for applications in smart agriculture, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7214, https://doi.org/10.5194/egusphere-egu23-7214, 2023.

EGU23-8628 | Posters on site | AS1.2

Discussion about bulk shear thresholds for severe weather environment that cause power outages and blow down towers of transmission and distribution lines in Southern Brazil 

Leonardo Calvetti, Luis Gabriel Cassol Machado, Cesar Beneti, Kerollyn Andrzejewski, Fabricio Pereira Harter, Marcelo Felix Alonso, and Sheila Radman Paz

Brazil has a country-wide interconnected grid of over 169,000 km of high voltage transmission lines. By 2026, an additional 20,000 km will expand the grid significantly. The main type of electrical energy transmission in Brazil is aerial for all sources of generation, including hydroelectric, wind and solar power plants, resulting in a network between the tropics to the subtropical regions up to -33 degrees latitude. In Southern Brazil there are 12.994.382 consumer units in the States, Rio Grande do Sul, Santa Catarina and Paraná.  One of the main causes of structural failures is associated with severe storms that produce loads that exceed the structural loading design criteria. In this work it has been investigating hindcast predictions with GFS and WRF for a high speed wind gust event that blew down towers in Southern Brazil during severe weather conditions between 2016 and 2022. It has analyzed eight high-impact events where towers or lines have failed or been shut down looking for convection parameters that indicate severe weather specifically for these impacts. In order to simulate a 48h forecast it was used the current operational GFS/GFDL V3 global model from NCEP/NOAA and 3-km resolution WRF runs. In seven of eight events the models were capable of simulating an environment conditions which meteorologists could elaborate an alert of high-impact severer weather for transmission lines and  could help the electric company's teams to execute a contingency plan.  Both GFS and WRF have indicated severe environments, but WRF has indicated better detailed areas of deep convection. In a sense of search thresholds that could be used in the future, some values of shear were found: 0-6km Shear 70-84 kt, 0-1 km Shear up to 40 kt, 0-3 km Shear up to 61 kt. The authors have not found specific thresholds for other variables such as the Convective available potential energy (CAPE) convective inhibition. The impact of the forecasts was analyzed according to the possible activities to be carried out by technicians in the prevention and repair of electrical systems and reduce the impact in outages.

How to cite: Calvetti, L., Cassol Machado, L. G., Beneti, C., Andrzejewski, K., Pereira Harter, F., Felix Alonso, M., and Radman Paz, S.: Discussion about bulk shear thresholds for severe weather environment that cause power outages and blow down towers of transmission and distribution lines in Southern Brazil, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8628, https://doi.org/10.5194/egusphere-egu23-8628, 2023.

EGU23-9531 | Orals | AS1.2

Latent diffusion models for generative nowcasting and uncertainty quantification of precipitation fields 

Jussi Leinonen, Ulrich Hamann, and Urs Germann

Deep generative modeling is able to generate highly realistic atmospheric fields, one prominent example being precipitation. So far, almost all studies have used generative adversarial networks (GANs) for this purpose, but recent progress in machine learning research has had a new class of methods called diffusion models replace GANs in many applications. Diffusion models have been often shown to be able to generate a wider variety of samples than GANs, suggesting that they might be able to better capture uncertainty in applications such as weather and climate where quantifying it is important.

In this presentation, we describe our research on using diffusion models for short-term prediction (nowcasting) of precipitation fields. We adapt the latent diffusion model used by Stable Diffusion (Rombach et al. 2022) to the this problem, predicting precipitation up to 3 hours ahead to the future at 5-min temporal resolution and 1-km horizontal resolution. Predictions can be produced as an ensemble where each member represent a possible future evolution of the precipitation field.

We show that our model:

  • generates highly realistic precipitation fields that are consistent with the past precipitation used as input.
  • outperforms the state-of-the-art GAN-based Deep Generative Models of Rainfall (DGMR) model by most relevant metrics.
  • performs particularly well at representing the uncertainty of its own predictions, as shown by uncertainty quantification methods developed for ensemble forecast verification.

Therefore, it appears that diffusion models are indeed suitable for generative modeling of precipitation fields with highly realistic representation of uncertainty. Our model architecture also permits multiple inputs data sources to be combined, in particular allowing seamless generative predictions to be made by exploiting observations and numerical weather predictions.

How to cite: Leinonen, J., Hamann, U., and Germann, U.: Latent diffusion models for generative nowcasting and uncertainty quantification of precipitation fields, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9531, https://doi.org/10.5194/egusphere-egu23-9531, 2023.

EGU23-9985 | Posters virtual | AS1.2

Predicting precipitation growth and decay with weather radar rainfall measurements 

Chen Li, Miguel Rico-Ramirez, Qin Wang, Weiru Liu, and Dawei Han

Recently, weather radar has been increasingly used to estimate precipitation for a variety of hydrological and meteorological applications, including real-time flood forecasting, severe weather monitoring and warning, and short-term precipitation forecasting. In very short range (0–6 h), many critical decisions are taken to ensure people’s safety. For example, the damage of a localized hazard of flood is high so that the warning of these severe weather is important. Forecasting precipitation in this time range the commonly relies on extrapolation-based nowcasting tools that exploit the persistence of the most recent weather radar observations. To obtain the best possible prediction skill in the 0–6-h range, one cannot solely rely on numerical weather prediction (NWP) but must also use the available observations in a more direct way. Weather radars are instruments capable to provide rainfall measurements with suitable spatial and temporal resolutions. The potential benefit of using radar rainfall in hydrology is huge, but practical hydrological applications of radar have been limited by the inherent uncertainties and errors in radar rainfall estimates. As radar nowcasts are essentially based on extrapolation from a series of consecutive radar scans, they are characterized by a high skill at the start of the forecast, but this decreases with lead time very rapidly, as extrapolation techniques generally do not account for growth and decay processes in the atmosphere (Golding 1998).

Machine learning algorithms can be trained with weather radar data to identify regions of precipitation growth and decay based on historical observations. Artificial neural networks (ANN) can be employed to learn the complex nonlinear dependence relating the growth and decay to the predictors, which are geographical location, motion vectors, temperature, precipitation and time (Foresti et al.2019). The precipitation motion field can be calculated by using the optical flow driven by weather radar data. Around 15-year of weather radar precipitation observations from Great Britain (GB) are used to derive precipitation growth and decay mainly due to orography. This paper will present the preliminary findings of predicting precipitation growth and decay in different regions in the UK.

 

How to cite: Li, C., Rico-Ramirez, M., Wang, Q., Liu, W., and Han, D.: Predicting precipitation growth and decay with weather radar rainfall measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9985, https://doi.org/10.5194/egusphere-egu23-9985, 2023.

Although tropical cyclone (TC) forecasts can fairly well capture the TC track and primary rainfall distribution, limited skills are found in forecasting TC structural changes and asymmetric gusty winds. The barrier to further understanding TC structural change is due mainly to the lack of observation, and it is difficult to have systematic 2-D wind analyses. Here, we developed a deep learning model — Deep Learning 2-D Structure Analysis Model for Tropical Cyclones (DSAT-2D) — to produce TC wind analysis in high-temporal-spatial resolutions based on generative adversarial networks (GAN). We use IR1 satellite observation and ERA5 reanalysis data as the model input for the DSAT-2D. The ASCAT surface wind data were collected and used as the label data. Note, however, that the ASACT analysis tends to underestimate winds greater than 15 m/s. Thus, we proposed several methods to fix this issue before training the model. Furthermore, other innovative designs in the DSAT-2D model include: (i) we regrid all data in a polar coordinate to better handle the TC tangential and radial features, and (ii) we also set the target of the DSAT-2D model as the TC radial wind and tangential wind.

Experiment results demonstrate that the DSAT-2D model can capture the TC asymmetric wind structure while possessing the capability of increasing the maximum estimation frequency from approximately 12 hours (e.g., ASCAT data) to less than one hour. The DSAT-2D model may help understand the TC asymmetric wind evolution and improve TC forecasts. Future applications of assimilating this value-added information into the numerical weather prediction model will also be discussed.

How to cite: Cheng, Y.-Y. and Chen, B.-F.: An End-to-end Deep Learning Approach for Analyzing Tropical Cyclone 2-D Surface Winds Utilizing Satellite Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10632, https://doi.org/10.5194/egusphere-egu23-10632, 2023.

EGU23-10645 | ECS | Orals | AS1.2

An Advanced Deep Learning Rainfall Forecasts Downscaling Method in Taiwan 

Rong-Cih Chang, Yung-Yun Cheng, and Buo-Fu Chen

Taiwan is a 35,808-km2 island with more than 100 peaks over 3,000 meters. The complex terrain in Taiwan makes forecasters more challenging to forecast rainfall in mesoscale and storm-scale. Besides, the spatial distribution of rainfall stations is quite uneven as well. Moreover, the forecast performance of both the European Centre for Medium-Range Weather Forecasts (ECMWF) and the Global Forecast System (GFS) is limited by Taiwan's complex terrain, having certain systematic deviations in rainfall forecasts. For example, the ECMWF forecast has underestimated heavy rainfall and over-predicted light rain in Taiwan. Consequently, to correct model deviations and provide better rainfall forecast products, advanced statistical or artificial intelligence (AI) methods should be studied.

This research applies the U-net neural network to generate downscaling rainfall prediction. We collected precipitation forecast data from the ECMWF (9 km resolution) and the GFS (22 km resolution) during 2021 as the model input. The Quantitative Precipitation Estimation and Segregation Using Multiple Sensor (QPESUMS) radar data from CWB is used as the label data. QPESUMS data can effectively help describe the complete spatial distribution of rainfall. The testing data is from the 2022 whole year. An innovative design of the proposed model is a geographical attention layer (GAL) in the U-net. The GAL helps to learn the geospatial characteristics from the QPESUMS rainfall observation. Moreover, this study uses a scale-separated loss function for model optimization, for which the rainfall is divided into large-scale smoothing and small-scale disturbance fields.

Results show that this U-net downscaling model successfully learns the feature and corrects the systematic bias in both global models, such as shifts in the rainfall caused by topographical lift and local circulation. Furthermore, based on the overall statistics of 2021, the performance diagram shows that the AI model corrects the over-prediction of light rain, while the critical success index in heavy rain is improved by 25 to 30%. The ongoing work of this research will apply generative adversarial networks to break the limitation of learning wrong features from the original forecast input data.

How to cite: Chang, R.-C., Cheng, Y.-Y., and Chen, B.-F.: An Advanced Deep Learning Rainfall Forecasts Downscaling Method in Taiwan, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10645, https://doi.org/10.5194/egusphere-egu23-10645, 2023.

Daily to monthly variations of precipitation directly affect the propagation of an emerging drought. To cope with adverse impacts, a skillful sub-seasonal forecast of precipitation is essential to track the evolution of the emerging drought and provide actionable information for stakeholder and water resources managers. This study evaluates the predictive performances of the Subseasonal Experiment (SubX) models (ECCC-GEPS6, EMC-GEFSv12, ESRL-FIMr1p1, GMAO-GEOS_V2p1, and RSMAS-CCSM4) for the precipitation variations during two recent long-term drought events (2007−2010 and 2013−2016) over the Korean Peninsula. Sub-seasonal prediction skill of SubX models are quantitatively evaluated via multiple verification metrics for ensemble, deterministic, and categorical forecasts. Results show that during the emergence of multi-year droughts, the intensification and persistence of drought severity are generally better predicted by SubX models than the weakening and recovery of the drought severity in all forecast times (1−4 weeks). The multi-model ensemble approach shows the best prediction skill, and EMC-GEFSv12 which has the most ensemble member presents the better predictive performance than other models. In addition, results from the sensitivity test to ensemble member size show that multiple ensemble member can enhance the prediction skills significantly up to eight ensemble members. Overall results suggest that the forecast of SubX on multi-year Korean Peninsula droughts can provide actionable information that helps manage water resources in a timely manner.

How to cite: Park, C.-K. and Kam, J.: Evaluation of the sub-seasonal forecasting skill of SubX models for precipitation during recent multi-year droughts over the Korean Peninsula, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10752, https://doi.org/10.5194/egusphere-egu23-10752, 2023.

EGU23-10909 | Posters on site | AS1.2

Prediction skill of Asian Dust Generation in hindcast data of Asian Dust Seasonal Forecasting Model (GloSea5-ADAM) 

Misun Kang, Woojeong Lee, Pil-Hun Chang, Mi-Gyeong Kim, and Kyung-On Boo

This study investigated the prediction skill of the Asian dust seasonal forecasting model (GloSea5-ADAM) on the Asian dust and meteorological variables related to the dust generation using hindcasts of GloSea5-ADAM for the period of 1991~2016 for East Asia. GloSea5-ADAM incorporates the dust generation algorithm of the Asian Dust and Aerosol Model (ADAM) into the Global Seasonal Forecasting System version 5 (GloSea5). The Asian dust and meteorological variables (10 m wind speed, 1.5 m relative humidity, and 1.5 m air temperature) depending on the combination of the initial dates in the sub-seasonal scale were compared to that from synoptic observation and ERA5 reanalysis data. The evaluation criteria used Mean Bias Error (MBE), Root Mean Square Error (RMSE), and Anomaly Correlation Coefficient (ACC). The Asian dust and meteorological variables in the source region (35~44°N, 90~115°E) showed high ACC in the prediction scale within one month. The best performances for all variables showed when the use of the initial dates closest to the prediction month based on MBE, RMSE, and ACC. ACC was as high as 0.4 in Spring when using the closest two initial dates. In particular, the GloSea5-ADAM shows the best performance of Asian dust generation with an ACC of 0.60 in the occurrence frequency of Asian dust in March when using the closest initial dates for initial conditions. This result showed that the performances could be improved by adjusting the number of ensembles considering the combination of the initial date.

 

How to cite: Kang, M., Lee, W., Chang, P.-H., Kim, M.-G., and Boo, K.-O.: Prediction skill of Asian Dust Generation in hindcast data of Asian Dust Seasonal Forecasting Model (GloSea5-ADAM), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10909, https://doi.org/10.5194/egusphere-egu23-10909, 2023.

EGU23-11043 | ECS | Orals | AS1.2

Precipitation Nowcasting Based on an Optimized Deep Learning Model Trained with Heterogeneous Weather Data 

Dian-You Chen, Chia-Tung Chang, and Buo-Fu Chen

    Due to the threat of extreme rainfall associated with mesoscale convective systems and summer afternoon thunderstorms, very short-term quantitative precipitation forecasting during 0−3 h is critical in Taiwan. In this study, deep learning models are developed for high-resolution quantitative precipitation nowcasting in Taiwan up to 3 h ahead. The baseline model based on the convolutional recurrent neural network is trained with a dataset containing radar reflectivity and rain rates at a granularity of 10 min. As previous works tend to produce overprediction in low-rainfall regions, the currently proposed model is improved and further driven by highly related heterogeneous weather data, including visible channel satellite observation, environmental winds, and environmental thermo-dynamical profiles. Note that an innovative “PONI module” is added to the deep learning model to integrate a variety of heterogeneous data with various spatial and temporal characteristics. Moreover, model performance is evaluated from statistical and spatial rescaling perspectives represented by R =  Ravg + R', where R denotes original rainfall, Ravg and R' are spatial moving averages and the values deviated from Ravg, respectively. Statistical verification shows that the Ravg of the new model outperforms the previous model, while the performance of R' is comparable. The new model integrated with heterogeneous data selected upon domain knowledge can restrain the nowcasts that overestimate in low-rainfall regions. Last but not least, quasi-operational verifications against other state-of-the-art techniques in Taiwan Central Weather Bureau are presented as follows: (1) the CSI of the first-hour prediction from the deep learning model is comparable with QPESUMS-QPF and better than RWRF and iTeen. (2) 3h ahead prediction CSI of RWRF and iTeen are inferior to the performance of deep learning model owing to their misprediction of rainfall regions. The deep learning model can accurately predict medium and extreme amounts of precipitation at a fraction of the computational cost.

How to cite: Chen, D.-Y., Chang, C.-T., and Chen, B.-F.: Precipitation Nowcasting Based on an Optimized Deep Learning Model Trained with Heterogeneous Weather Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11043, https://doi.org/10.5194/egusphere-egu23-11043, 2023.

So far, plenty of efforts have been pursued on the numerical weather prediction (NWP). However, systematic errors could never be ignored in the output applications. To supply the numerical forecasts with higher accuracies, statistical postprocessing is often expected to correct systemic biases and has been one of the key components of the forecasting suites. Based on the NWP models and taking advantages of the raw stepwise pattern projection method (SPPM), the neighborhood pattern projection method (NPPM) is newly proposed to postprocess the model outputs and to improve forecast skills of daily maximum and minimum temperatures (Tmax and Tmin) over East Asia for short-term timescales, as well as the Kalman filter based pattern projection method (KFPPM) for longer-term forecasts. For the short-term lead times of 1–7 days, the SPPM is slightly inferior to the benchmark of decaying averaging method, while its insufficiency decreases with increasing lead times. The NPPM shows manifest superiority for all lead times, with the mean absolute errors of Tmax and Tmin decreased by ~0.7° and ~0.9°C, respectively. Advantages of the SPPM and NPPM are both mainly concentrated on the high-altitude areas such as the Tibetan Plateau, where the raw model outputs show the most conspicuous biases. As for longer-term forecasts at the subseasonal timescale, the NPPM effectively calibrates the temperature forecasts at the early stage. However, with the growing lead times, it shows speedily decreasing skills and can no longer produce positive adjustments over the areas outside the plateaus. By contrast, the KFPPM consistently outperforms the other calibrations and reduces the forecast errors by almost 1.0°C and 0.5°C for Tmax and Tmin, respectively, both retaining superiorities to the random climatology benchmark till the lead time of 24 days. The optimization of KFPPM maintains throughout the whole range of the subseasonal timescale, showing most conspicuous improvements distributed over the Tibetan Plateau and its surroundings. Case experiments further demonstrate the above-mentioned features and imply the potential capability of the NPPM and KFPPM in improving forecast skills and disaster preventions for extreme temperature events. Besides, compared with the initial SPPM, they not only produces more powerful forecast calibrations, but also provides more pragmatic calculations and greater potential economic benefits in practical applications.

How to cite: Zhu, S., Lyu, Y., and Zhi, X.: Calibrations of Surface Air Temperature Forecasts at Short- and Long-term Timescales Based on Statistical Pattern Projection Methods, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11970, https://doi.org/10.5194/egusphere-egu23-11970, 2023.

EGU23-12127 | ECS | Orals | AS1.2

Exploiting radar polarimetry for nowcasting of convective hazards using deep learning 

Nathalie Rombeek, Jussi Leinonen, and Ulrich Hamann

Severe convective weather events, such as hail, lightning and heavy rainfall pose a great threat to humans and cause a considerable amount of economic damage. Nowcasting convective storms can provide precise and timely warnings and, thus, mitigate the impact of these storms. Dual-polarization weather radars are a crucial source of information for nowcasting severe convective events. These radars provide important information about the microphysics of the convective systems, on top of the rainfall rate and vertical structure of the reflectivity. Nevertheless, polarimetric variables, which can provide additional information about the size, shape and orientation of particles, are often not considered in nowcasting.

This work presents the importance of polarimetric variables as an additional data source for nowcasting thunderstorm hazards using machine learning, compared to using radar reflectivity alone. We add these data to the neural network architecture of Leinonen et al. 2022 (Seamless lightning nowcasting with recurrent-convolutional deep learning), which uses convolutional and recurrent layers and analyzes inputs from multiple data sources simultaneously. This network has a common framework, which enables nowcasting of hail, lightning and heavy rainfall for lead times up to 60 min with a 5 min resolution. The study area is covered by the Swiss operational radar network, which consists of five operational polarimetric C-band radars. In addition, we analyze the contribution of quality indices as an additional information source, which takes the uncertainty of the radar observations throughout the complex mountainous terrain and scanning strategy in Switzerland into account. Results indicate that including polarimetric variables and quality indices improves the accuracy of nowcasting convective storms.

How to cite: Rombeek, N., Leinonen, J., and Hamann, U.: Exploiting radar polarimetry for nowcasting of convective hazards using deep learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12127, https://doi.org/10.5194/egusphere-egu23-12127, 2023.

EGU23-12517 | ECS | Posters on site | AS1.2

The combined impact of model uncertainty on flow-dependent spatial predictability of convective precipitation 

Takumi Matsunobu, Christian Keil, Matjaž Puh, Christoph Gebhardt, and Chiara Marsigli

Accurate precipitation forecasts at kilometre scales are still a key challenge for convective scale ensemble prediction systems. We assess the spatial forecast skill-spread relationship for summer convection in 2021 and address the impact of considering model uncertainties from two physics parametrisations -- microphysics and planetary boundary layer turbulence -- together with initial and lateral boundary conditions uncertainties. To investigate their flow dependence all analyses are done conditionally to strong and weak synoptic convective forcing cases.
It is found that the spatial skill-spread relationship is highly dependent on synoptic forcing and the current operational ensemble forecasts are spatially underdispersive especially during weak synoptic control, whereas a good agreement is found during strong synoptic control. Case studies during weak synoptic control demonstrate that perturbations in the planetary boundary layer contribute to improving forecast skill and increase spread at small scales while microphysical perturbations contribute to spread increase across all scales. Overall, the combination of both perturbations seems to combine their individual impacts and thus benefits the spatial skill-spread relationship at most times and scales.

How to cite: Matsunobu, T., Keil, C., Puh, M., Gebhardt, C., and Marsigli, C.: The combined impact of model uncertainty on flow-dependent spatial predictability of convective precipitation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12517, https://doi.org/10.5194/egusphere-egu23-12517, 2023.

EGU23-12665 | ECS | Posters on site | AS1.2

Development of Geostationary Satellite Atmospheric Motion Vectors Forecasting Algorithm by CNN Model 

Hwayon Choi, Yong-Sang Choi, and Gyuyeon Kim

Atmospheric motion vector (AMV) is an important factor that affects most meteorological phenomena in numerical weather prediction. Despite of its significance, the conventional algorithm of moisture tracking for AMV calculated with most of remote sensing data uses the cross-correlation coefficient (CCC) method, resulting in low-resolution (target-based) output and much of errors. In addition, forecasting AMVs is impossible in conventional method because it requires water vapor data 10 minutes from the current time to calculate current winds. For better moisture flow tracking, convolutional neural network (CNN) frames were used that track motion, which is called optical flow estimation in computer vision. The pixel-based high-resolution AMVs are calculated by using the water vapor channel images into the PWC-Net (CNNs for optical flow using pyramid, warping, and cost volume). For each pixel, linear regression is used to forecast AMVs. The performance of the AMVs calculated by CNN was validated by comparing those results and the Korean geostationary satellite GEO-KOMPSAT-2A (GK2A) AMVs with wind fields of ERA5 data at 100-1000 hPa. Experiments used infrared brightness temperature images of three water vapor channels at 6.2 µm, 7.0 µm, and 7.3 µm over Korean Peninsula for 2022. As to root-mean-square vector differences (RMSVDs), the tracking performance of this study was found to be more accurate than the GK2A AMVs ­— 1.3 to 21.93 m/s more accurate for the cloudy sky and 0.32 to 14.9 m/s more accurate for the clear sky above 400 hPa. The results using the CNN model showed better moisture tracking performance than the conventional method, especially for low altitudes. It also enables to obtain higher resolution AMVs with pixel-based tracking rather than conventional target-based tracking. Furthermore, the mean RMSVDs of forecasted AMVs are 1.97 m/s, 2.66 m/s, 3.32 m/s, and 5.28 m/s when the forecast lead time is 10 min, 20 min, 30 min, and 1 hr, respectively. Consequently, high-resolution AMV forecasts with accuracy, which could not be calculated by the conventional method, were obtained by CNN model, and can be used to advance the accuracy of weather forecasting.

 

KEYWORDS: Moisture Tracking; Optical Flow; Atmospheric Motion Vectors; Wind Forecasting; Remote Sensing

How to cite: Choi, H., Choi, Y.-S., and Kim, G.: Development of Geostationary Satellite Atmospheric Motion Vectors Forecasting Algorithm by CNN Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12665, https://doi.org/10.5194/egusphere-egu23-12665, 2023.

EGU23-12924 | ECS | Orals | AS1.2

Short-term probabilistic forecast of cloudiness: a scale-dependent advection approach 

Alberto Carpentieri, Doris Folini, Daniele Nerini, Seppo Pulkkinen, Martin Wild, and Angela Meyer

Solar energy generation is highly volatile during the day due to the strong dependence on cloud dynamics, which limits its integration into the power grid (Smith et al., 2022). On the other hand, higher utilization of renewable energy is essential to tackle climate change. To increase the share of photovoltaic energy in the grid without jeopardizing grid stability, accurate forecasts are essential to ascertain the balance between energy demand and supply (David et al., 2021).

Photovoltaic energy production mainly depends on downwelling surface solar radiation (). SSR is accurately measured by pyranometers, but their spatial representativeness is limited to a few kilometers. By estimating the SSR from geostationary satellites, we can cover larger areas with high spatial and temporal resolutions, allowing us to track cloud motion.

Previous studies on probabilistic cloud motion focused on optical-flow methods without considering the temporal evolution of clouds as such. We address this issue by presenting a scale-dependent approach to forecast. Our approach is inspired by the works of Bowler et al., 2006 and Pulkkinen et al., 2019 on precipitation nowcasting. The novelty of our study is the utilization of different autoregressive models to forecast the temporal evolution of cloudiness of different spatial scales. Our work is motivated by the scale-dependent predictability of cloud growth and decay. By exploiting more than one autoregressive model, we can predict the noisy evolution of small scales independently of the more deterministic evolution of larger spatial scales.

Our preliminary results over Switzerland indicate that our model outperforms the probabilistic advection model based on Carriere et al., 2021 noise generation by reducing the continuously ranked probability score (CRPS) on the test set by 14%. Moreover, we demonstrate the advantage of cloudiness scale decomposition by comparing our model with the same approach without decomposition. We can reduce the CRPS by 6% and the RMSE by 5% by decomposing the images into multiple cascades

References

Bowler, N., C. Pierce, A. Seed, 2006, “STEPS: A probabilistic precipitation forecasting scheme which merges an extrapolation nowcast with downscaled NWP”, Quarterly Journal of the Royal Meteorological Society, 132, 620, pp. 2127–2155, doi:10.1256/qj.04.100.

Carriere, T., R. Amaro e Silva, F. Zhuang, Y. Saint-Drenan, P. Blanc, 2021, “A New Approach for Satellite-Based Probabilistic Solar Forecasting with Cloud Motion Vectors”, Energies, 14, doi:10.3390/en14164951.

David, M., M. Luis, P. Lauret, 2018, “Comparison of intraday probabilistic forecasting of solar irradiance using only endogenous data”, International Journal of Forecasting, 34, doi:10.1016/j.ijforecast.2018.02.003.

Pulkkinen, S., D. Nerini, A. Perez Hortal, C. Velasco-Forero, A. Seed, U. Germann, L. Foresti, 2019, “Systems: an open-source Python library for probabilistic precipitation nowcasting (v1.0)”, Geoscientific Model Development, 12, 10, pp. 4185–4219, doi:10.5194/gmd-12-4185-2019.

Smith, O., O. Cattell, E. Farcot, R. D. O’Dea, K. I. Hopcraft, 2022, “The effect of renewable energy incorporation on power grid stability and resilience”, Science Advances,  https://www.science.org/doi/abs/10.1126/sciadv.abj6734.

How to cite: Carpentieri, A., Folini, D., Nerini, D., Pulkkinen, S., Wild, M., and Meyer, A.: Short-term probabilistic forecast of cloudiness: a scale-dependent advection approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12924, https://doi.org/10.5194/egusphere-egu23-12924, 2023.

Quantitative precipitation nowcasting (QPN) is crucial for forecasting precipitation within the next several hours (generally up to 6) to prevent substantial socioeconomic damage. In general, ground radar data has been widely employed in QPN due to its high spatial-temporal resolution and more precise precipitation estimation than satellite. With the remarkable success of deep learning (DL), recent QPN studies have actively adopted DL using radar data. Although these studies yielded high skill scores in forecasting precipitation areas with a weak intensity (about 1 mm/h), they failed to effectively simulate the horizontal movement of precipitation areas and showed poor ability in forecasting precipitation with stronger intensities. In addition, despite the fact that the skill score is highly dependent on the characteristics of each precipitation event, there was a lack of evaluation over various precipitation cases. From the motivation that there can be room for improving QPN using the advanced DL model in video prediction, this study suggests the QPN model based on simple yet better video prediction (SimVP), which is a state-of-the-art DL model. We trained the SimVP model using radar data in South Korea from June to September (JJAS) for the period of 2019-2022, which includes the summer and early fall. In terms of the critical score index (CSI) with a lead time of 120 minutes (0.46, 0.23, and 0.09 for 1, 5, and 10 mm/h thresholds, respectively), the proposed model showed significant improvement over the existing DL models based on an evaluation from JJAS 2022. Considering different precipitation conditions, three case studies were conducted for heavy rainfall, typhoons, and fast-moving narrow convection events. The suggested model showed comparable or the highest CSI in 120 min with a 1 mm/h threshold in all cases, demonstrating robust performance (0.49, 0.69, and 0.29 for heavy rainfall, typhoon, and narrow convection, respectively). Qualitative evaluation of the proposed model also showed better results in terms of horizontal displacement movement and less underestimation than the other models. In addition, we further explored the possibility of real-time learning (RTL) with newly added radar data. By repeatedly optimizing DL model for currently facing precipitation events, RTL contributed to deep learning models predicting results more similar to actual radar patterns. It is expected that the proposed SimVP and RTL would serve as a new baseline for DL-based QPN due to their ease of implementation and enhanced performance. 

How to cite: Han, D., Choo, M., and Im, J.: A data-driven precipitation nowcasting framework using advanced deep learning model for video prediction and real-time learning approaches, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13644, https://doi.org/10.5194/egusphere-egu23-13644, 2023.

The accurate forecasting of the intensity of tropical cyclones (TCs) is able to effectively reduce the overall costs of disaster management. In this study, we proposed a deep learning-based model for TC forecasting with the lead time of 24, 48, and72 hours following the event, based on the fusion of geostationary satellite images and numerical forecast model output. A total of 268 TCs which developed in the Northwest Pacific from 2011 to 2019 were used in this study. The Communications system, the Ocean and Meteorological Satellite (COMS) Meteorological Imager (MI) data were used to extract the images of TCs, and the Climate Forecast System version 2 (CFSv2) provided by the National Center of Environmental Prediction (NCEP) was employed to extract atmosphere and ocean forecasting data. In this study, we suggested hybrid convolutional neural network (hybrid-CNN)-based TC forecasting models. It enables to efficiently consider not only the physical but also the spatial characteristics of variables. The Joint Typhoon Warning Center (JTWC) was used for validating the suggested model, and Korea Meteorological Administrator (KMA)-based operational TC predictions were utilized for evaluating the performance of the model. A hybrid-CNN-based prediction model obtained mean absolute errors (MAE) of 13.58, 16.48, and 21.64 kts and skill scores (SS) of 29%, 19%, and 1.6% for 24h, 48h, and 72h forecasts, respectively. Since the rapid intensification (RI) is one of the challenging tasks in the TC intensity prediction, the performance of suggested model for all RIs in 2019 were additionally evaluated. Compared to KMA-based predictions, the suggested models achieved average SS of 66%. Furthermore, using an explainable artificial intelligence (XAI) approach, it is possible to verify how the suggested model works for forecasting TC intensity and propose the feasibility of the suggested model in the meteorology field.

 

How to cite: Lee, J. and Im, J.: Deep learning-based tropical cyclone intensity prediction through synergistic fusion of geostationary satellite and numerical prediction model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14443, https://doi.org/10.5194/egusphere-egu23-14443, 2023.

EGU23-14544 | Orals | AS1.2

EUMETNET Nowcasting Programme 

Franziska Schmid, Anders Sivle, Solfrid Agersten, André Simon, and Aitor Atencia

One major task of the National Meteorological and Hydrological Services (NMHS) is the provision of consistent and integrated forecasting products from minutes to several days ahead (seamless forecasting). The former EUMETNET (European Meteorological Services’ Network) project ASIST (Application oriented analysis and very short-range forecast environment) which started in 2015 focused on the nowcasting and very short range forecasting. Then, it was extended to the EUMETNET Nowcasting Programme (E-NWC) which started in 2019 and will last until the end of 2023 with focus on nowcasting and also on seamless prediction.

In this presentation, the main objectives of the E-NWC Programme will be introduced. E-NWC supports NMHS in sharing expertise, experiences and best practices for developing and implementing nowcasting, very short-range forecasting and seamless prediction systems. Key activities lie in the exchange of information and experiences with the users during e.g. the every two years European Nowcasting Conference and the strong cooperation with the World Meteorological Organization (WMO) and EUMETSAT, and in summarizing the relevant findings in project reports and joint peer-reviewed papers. Highlights of this contribution comprehend a few results from studies and surveys carried out recently.

How to cite: Schmid, F., Sivle, A., Agersten, S., Simon, A., and Atencia, A.: EUMETNET Nowcasting Programme, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14544, https://doi.org/10.5194/egusphere-egu23-14544, 2023.

On 26 November 2022, an extreme rainfall event occurred over Ischia Island (Italy). It triggered a mudflow that swept over Casamicciola Terme town and caused 12 victims. Based on available rainfall data from 4 rain-gauge stations over the island, the precipitation values registered during the event were higher than the annual maxima values of the previous 15 years. With regards to 1 and 24 hours, the rain-gauge stations measured values between 40.6 and 57.6 mm, and between 145.4 and 176.8 mm, respectively. Since one of the main challenges during these phenomena is predicting rainfall sufficiently in advance in order to allow water managers to take action (issue warnings or real-time control), this study investigates how much time before the peak - or threshold exceedance - a machine learning model is able to capture the peak - or threshold exceedance. A model that predicts rainfall intervals and the corresponding probability of occurrence for lead times from 10 minutes to 6 hours is proposed. The model employs cumulative rainfall depths from recording stations in an area of 50 km radius from the Ischia Island as inputs for a Feed Forward Neural Network to nowcast rainfall in the 4 rain-gauges over the study area. Based on almost 400 rain events observed during years 2009-2022, 24 machine learning models were independently trained for each rain-gauge and each of the 6 lead-times - 10, 30, 60, 120, 180 and 360 minutes. The performance of each model was evaluated and compared using different metrics, both continuous (RMSE and MAE) and categorical (POD and FAR). In addition, the Eulerian Persistence (EP) was considered as a benchmark model. The rainfall nowcasts showed encouraging results. Even though for convective rain events the potential lead-time is short, the models produced consistent nowcasts for lead-times up to 2 hours. With probabilities of almost 90%, the thresholds exceedance was forecasted up to 1 hour before. As expected, predictive accuracy and probabilities gradually decreased as the lead-time increased, according to physically based models. Moreover, the proposed models outperformed the benchmark EP for all the lead-times and performance criteria. Results confirmed that the use of cumulative rainfall depths for precipitation nowcasting made this approach a promising tool for nowcasting purposes, and his flexibility and conceptual simplicity resulted in a rapid, easily replicable and convenient nowcasting approach. To conclude, the proposed models enhanced a first identification of critical thresholds, which should be further analysed in order to achieve a better, complementary understanding of the occurring phenomenon. 

Keywords: Precipitation nowcasting; Multi-step predictions; Rain-gauge measurements; Pattern recognition; Feed forward neural networks; Cumulative rainfall fields.

How to cite: Pirone, D., Del Giudice, G., and Pianese, D.: Machine Learning models for probabilistic rainfall nowcasting applied to a case study in Italy: the extreme rainfall event on 26 November 2022 over Casamicciola town, Ischia Island., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14545, https://doi.org/10.5194/egusphere-egu23-14545, 2023.

EGU23-14709 | ECS | Orals | AS1.2

Improving Dual-Polarization Radar-based rainfall estimation using Long Short-Term Memory Neural Networks 

Jiun-Liang Lin, Chia-Yu Hsu, and Li-Chiu Chang

Extreme hydrological events, which are highly concerned by local governments, hydraulic units and hazard response centers due to their potential to bring heavy rainfall and cause serious floods, have frequently occurred and impacts on Taiwan urban area in recent years under the circumstance of climate change and global warming. The frequent occurrence of high intense storm always leads to flooding-related disasters within a short period, which makes rainfall monitoring a disaster prevention. Therefore, this study utilizes Long Short-Term Memory Neural Networks (LSTM) and Back Propagation Neural Networks (BPNN) to extract the characteristics of radar observations and forecast rainfall with time 1-step-ahead to 6-step-ahead (T+1~T+6) in Taiwan’s capital, Taipei City. The data collection was included in the Shulin dual-polarization radar (RCSL) observations, such as differential phase shift, specific differential phase, reflectivity and doppler radial wind field, and rain gauge data from May 2021 to November 2021 in the Taipei City. With a view to capturing the movement of hydrometeors continually changes within the time step, an algorithm which can calculate velocity and direction of specific hydrometeors on two-dimensional matrix were developed and applied to simulate location of the specific hydrometeors on n-step-ahead (T+n). Finally, the rainfall forecast can be achieved by using the simulated location of specific hydrometeors and its physical properties from radar observations as input data to fit rainfall from the gauge. This study aims to investigate the relationship between short-duration rainfall and radar observations by artificial neural network (ANN), and forecast the rainfall  within a short period.

 

Keywords: Dual-Polarization Radar; Rainfall Estimation; Artificial Intelligence (AI), Artificial neural network (ANN); Long Short-Term Memory Neural Networks(LSTM)

How to cite: Lin, J.-L., Hsu, C.-Y., and Chang, L.-C.: Improving Dual-Polarization Radar-based rainfall estimation using Long Short-Term Memory Neural Networks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14709, https://doi.org/10.5194/egusphere-egu23-14709, 2023.

Reliable early forecasting of summer air temperature is important to effectively prepare and mitigate damage such as heat-related mortality and excessive electricity demand caused by heat waves and tropical nights. Numerical weather prediction (NWP) models have been used for operational forecasting of air temperature. However, NWP models have coarse spatial resolution due to massive computational resources arising from complex forecasting systems and unstable parameterization of NWP models, which make the uncertainty of prediction, consisting of systematic and random biases. Therefore, the objective of this study is to develop a novel deep learning-based statistical downscaling approach for the Global Data Assimilation and Prediction System (GDAPS) model’s summer air temperature forecasts over South Korea. This study developed the proposed statistical downscaling model through the decomposition into the temporal dynamics of daily air temperature forecast and spatial fluctuation by pixels. The daily temperature dynamic was estimated using a daily mean GDAPS temperature forecast with simple mean bias correction. The spatial fluctuation by pixels was obtained using the spatial anomaly of downscaled air temperature forecast by the U-Net model. The GDAPS model’s forecast data, present-day high spatial resolution satellite observations, and topography variables were used as input variables for training the U-Net model. The observations at weather stations were spatially interpolated using the regression-kriging, and then we used it as a target image for the U-Net model. The proposed U-net model was compared with the Local Data Assimilation and Prediction System (LDAPS), the dynamically downscaled model of the GDAPS, and the support vector regression (SVR)-based statistical downscaling model. For next-day Tmax and Tmin forecasts, the suggested U-net model showed better performance, having high coefficient of determination (R2) of 0.76 and 0.74 and root mean square error (RMSE) of 2.5 °C and 1.5 °C for next-day Tmax and Tmin forecasts, respectively. When analyzing the skill score (SS) values by stations of the U-Net model, it had remarkably high SS values at stations where the GDAPS had a high absolute value. For Tmax and Tmin forecasts with 1-7 days forecast lead time, the suggested model consistently provided better performance (higher spatial correlation and lower RMSE) than GDAPS and SVR. In addition, the U-net model showed a detailed spatial distribution most similar to that of the observations. These results demonstrated that the suggested model successfully corrected the bias of the GDAPS, improving not only the forecast accuracy but also the ability to capture the spatial distribution of Tmax and Tmin forecasts. Using the deep learning-based suggested model in this study, bias-corrected high spatial resolution air temperature forecasts with a relatively long forecast lead time in summer seasons can be successfully produced.

How to cite: Cho, D., Im, J., and Jung, S.: Deep learning-based statistical downscaling for short-term forecasting of summer air temperatures, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14894, https://doi.org/10.5194/egusphere-egu23-14894, 2023.

EGU23-14973 | ECS | Posters on site | AS1.2

Operational machine learning for the postprocessing of surface wind forecasts 

Daniele Nerini, Francesco Zanetta, Mathieu Schaer, Jonas Bhend, Christoph Spirig, Lionel Moret, and Mark A. Liniger

Forecasting winds at the local scale can be challenging due to the highly variable and complex nature of wind patterns, particularly in the case of complex terrain. In such cases, the accuracy of numerical weather prediction models (NWPs) is often limited by the quality of their initial conditions and their grid resolution. This is where the use of observational data through statistical postprocessing techniques can help to improve the quality of forecasts. 

Statistical postprocessing is nowadays an established component in operational weather forecasting that is used to improve the accuracy, resolution, and calibration of NWP ensemble forecasts with historical observations. In recent years, machine learning techniques have shown great potential in the field of postprocessing, thanks to their ability to deal with increasingly large volumes of data, and the capacity to capture complex relationships between forecasts and observations that are not explicitly represented in traditional postprocessing methods. 

To capitalize on machine learning for weather applications, and for it to gain acceptance and become a reliable technology for operational use, it is also crucial to consider the technical and engineering challenges that arise when implementing machine learning in a productive environment. MLOps, or Machine Learning Operations, is a set of practices that are used to manage and streamline the deployment, monitoring, and maintenance of machine learning models in production.  

We will present our recent experience with the development and operationalization of a statistical postprocessing system based on the use of neural networks to predict the probability distribution of forecasts of surface winds. Following MLOps best practices, our framework aims to improve the reproducibility and automation of most common tasks in a machine learning-based system, such as efficient data loading and manipulation, the monitoring and visualization of prediction quality, and the automation of model training and deployment pipelines. 

How to cite: Nerini, D., Zanetta, F., Schaer, M., Bhend, J., Spirig, C., Moret, L., and Liniger, M. A.: Operational machine learning for the postprocessing of surface wind forecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14973, https://doi.org/10.5194/egusphere-egu23-14973, 2023.

EGU23-15153 | Orals | AS1.2

Ensemble precipitation nowcasting by combination of generative and transformer deep learning models 

Gabriele Franch, Elena Tomasi, Virginia Poli, Chiara Cardinali, Marco Cristoforetti, and Pier Paolo Alberoni

This work introduces a novel deep-learning method for generating realistic ensembles nowcast of radar-based precipitation at a five-minute time resolution for the next 60 minutes and longer.

The proposed method is composed of a combination of two models: the first model is trained to compress and decompress the spatial domain into and from a discrete representation (tokens), while the second model evolves the compressed representation over time. Specifically, the compression and decompression model is based on a combination of a Quantized Variational Autoencoder with a Generative Adversarial Network, while the prediction over time leverages a Generative Pretrained Transformer (GPT) architecture.

This separation of concerns (discretized spatial compression/decompression and temporal extrapolation) adds several desirable features not present in more commonly used deep learning methods based on recurrent/convolutional deep learning architectures: 

  • transformer output probabilities can be leveraged to generate ensemble/probabilistic forecasts (without the need of injecting noise)
  • the discretized spatial representation can be used to characterize each token, adding interpretability and explainability to the model
  • the combination of transformer probabilities and token characterization can be used at inference time for forecasts conditioning based on external factors (e.g. NWP forecast output)

The presented architecture is trained and tested on a 7-year radar dataset of reflectivity composites of the Emilia-Romagna Region, Italy. The method is then applied at two different scales: regional, over Emilia-Romagna, and national, on the entire Italian domain, showing the adaptability of the approach to multiple spatial domains. We will present the performance of this model for both deterministic and ensemble settings by comparing it with respect to other commonly used extrapolation and deep learning methods.

How to cite: Franch, G., Tomasi, E., Poli, V., Cardinali, C., Cristoforetti, M., and Alberoni, P. P.: Ensemble precipitation nowcasting by combination of generative and transformer deep learning models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15153, https://doi.org/10.5194/egusphere-egu23-15153, 2023.

EGU23-15514 | Orals | AS1.2

Probabilistic Precipitation Nowcasting with Physically-Constrained GANs 

Matej Choma, Matej Murín, Jakub Bartel, Milly Troller, and Michal Najman

It is generally accepted that weather forecasts contain errors due to the chaotic nature of the atmosphere. Regression models, such as neural networks, are traditionally trained to minimize the pixel-wise difference between their predictions and ground truth. The major shortcoming of these models is that they express uncertainty about prediction with blurring, especially for longer prediction lead times. One way to tackle this issue is to use a generative adversarial network, which learns what real precipitation should look like during training. Coupled with a loss, such as Mean Squared or Mean Absolute Error, these networks can produce highly accurate and realistic nowcasts. As there is an inherent randomness in those networks, they allow to be sampled from, just like ensemble models, and various probabilistic metrics can be calculated from the samples. In this work, we have designed a physically-constrained generative adversarial network for radar reflectivity prediction. We compare this network to one without physical restraints and show that it predicts events with higher accuracy and shows much less variance among its samples. Furthermore, we explore fine-tuning the network to the prediction of severe weather events, as an accurate prediction of these benefits both automated warning systems and forecasters.

How to cite: Choma, M., Murín, M., Bartel, J., Troller, M., and Najman, M.: Probabilistic Precipitation Nowcasting with Physically-Constrained GANs, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15514, https://doi.org/10.5194/egusphere-egu23-15514, 2023.

EGU23-16271 | Posters virtual | AS1.2

Results of a GPS Zenith Total Delay data assimilation experiment over Italy 

Stefano Federico, Rosa Claudia Torcasio, Eugenio Realini, Giulio Tagliaferro, and Stefano Dietrich

The Mediterranean area is often struck by severe weather events and deep convective events because of the presence of the warm sea, the complex orography of the area, and the specific synoptic scale environment. This scenario is worsened by climate change because, as climate change is affecting many weather and climate extremes, and the frequency and intensity of heavy precipitation events have increased in most of the world.

Over the past years, the use of Numerical Weather Prediction (NWP) models, along with an increasing availability of computing power, led to an improvement of the forecast accuracy. However, NWPs have well-known difficulties in capturing the physical processes at small spatial and temporal scales which are involved in convective or severe weather events. 

In this work we study the impact of assimilating GPS-ZTD (Global Positioning System-Zenith Total Delay) on the precipitation forecast over Italy for the month of October 2019, characterized by several moderate to intense precipitation events. The Weather Research and Forecasting (WRF, version 4.1.3) is used with its 3DVar data assimilation system. The horizontal resolution is 3km while the vertical domain spans the whole troposphere and lower stratosphere.

A dense network of about 500 GPS receivers was used for data assimilation and verification of the atmospheric water content. The dataset was built collecting data from all the major national and regional GNSS permanent networks, achieving dense coverage over the whole area.

Results show that WRF underestimates the atmospheric water content for the period, and GPS-ZTD data assimilation reduced this underestimation by increasing the water content of the atmosphere. The GPS-ZTD data assimilation increases the precipitation forecast amount, and the model performance are improved up to 6h.

Results for a case study show that the GPS-ZTD data assimilation can improve the precipitation forecast in different ways: predicting rainfall missed by the model without data assimilation or better focusing the precipitation already predicted by the model without GPS-ZTD data assimilation on the impacted area, the main drawback being the prediction of false alarms.

 

How to cite: Federico, S., Torcasio, R. C., Realini, E., Tagliaferro, G., and Dietrich, S.: Results of a GPS Zenith Total Delay data assimilation experiment over Italy, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16271, https://doi.org/10.5194/egusphere-egu23-16271, 2023.

EGU23-360 | ECS | Orals | AS1.3

Factors influencing subseasonal predictability of Northern Eurasian cold spells 

Irina Statnaia, Alexey Karpechko, and Heikki Järvinen

The study focuses on identifying potential “windows of opportunity” for the enhanced predictability of extreme events, such as severe Northern Eurasian cold air outbreaks as these events have significant impacts on human health, energy use, agriculture and welfare.  The extended-range predictability of extreme events is closely related to the preceding large-scale circulation patterns and remote teleconnections. To assess the predictability of these events and attribute their causes we use ensemble hindcasts (i.e., reforecasts for dates in the past) from five prediction systems from the S2S database – namely, from the European Centre for Medium‐range Weather Forecasts (ECMWF), the United Kingdom Met Office (UKMO), Météo‐France (CNRM), Bureau of Meteorology (BoM), Japan Meteorological Agency (JMA). These models have long re-forecast periods and big ensemble sizes necessary to establish statistically robust results. Moreover, the comparison of the forecasts from these six models evaluates the ability of modern prediction systems to forecast extreme events well in advance and highlights the main sources of predictability. We subsample the hindcasts into two groups according to their skill to predict an extreme event beyond weather predictability horizon (lead time week 2 and 3) in order to study the systematic relationship between preceding conditions and the onset of extreme events. Next, we evaluate the flow configurations in the initial conditions: the state of the stratospheric polar vortex (SPV), the phase and amplitude of the Madden-Julian Oscillation (MJO) in the tropics, and the weather regimes over the North Atlantic and Europe. This analysis provides a systemic evaluation and understanding of the large-scale patterns that can potentially contribute to the onset of extreme events over Eurasia, therefore, extending their predictability. Our results show that in overall models tend to over-predict cold conditions after certain states of the remote drivers but there is case-to-case variability in the predictability of the individual events. Moreover, this study assesses and compares the results from several state-of-art predicting systems which provides useful information for model developers as well as for forecast users.

How to cite: Statnaia, I., Karpechko, A., and Järvinen, H.: Factors influencing subseasonal predictability of Northern Eurasian cold spells, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-360, https://doi.org/10.5194/egusphere-egu23-360, 2023.

EGU23-553 | ECS | Posters on site | AS1.3

The influence of the stratosphere on the North Atlantic storm track predictability in subseasonal-to-seasonal reforecasts 

Hilla Gerstman, Dominik Büeler, C. Ole Wulff, Michael Sprenger, and Daniela Domeisen

Extreme stratospheric polar vortex events, such as sudden stratospheric warmings (SSW) or extremely strong polar vortex (SPV) states, can have a prolonged downward impact, influencing surface weather for several weeks to months. These events often lead to changes in the midlatitude storm track position and associated cyclone frequency over the North Atlantic and Europe. Such changes can result in infrastructure damage and health impacts due to cyclone-associated extreme winds and the risk of flooding or heavy snowfall. However, there exists a strong inter-event variability in these downward impacts on the tropospheric storm track, leading to opposite predictions of the storm track response. Therefore, identifying the biases in the forecast of the downward impact of stratospheric polar vortex extremes can improve the predictability of extratropical winter storms on subseasonal-to-seasonal timescales, and has the potential to benefit society and stakeholders.

Using ECMWF reanalysis data and ECMWF reforecasts from the Subseasonal to Seasonal (S2S) Prediction Project database, we investigate the stratospheric influence on extratropical cyclones, identified with a cyclone detection algorithm. Following SSWs, there is an equatorward shift in cyclone frequency over the North Atlantic in reforecasts, and a poleward shift is observed after SPV events, consistent with the response in reanalysis. However, less than 70% of the reforecasts capture the sign of the cyclone frequency response over the North Atlantic during weeks 1-2 after SSWs, and less than 50% of the reforecasts capture the response during weeks 3-4. The cyclone forecasts following SPV events are generally more successful. We further discuss the differences in predictability of extratropical cyclones between the two types of stratospheric extremes.

The results provide new insights on the role of the stratosphere in subseasonal variability and predictability of extratropical cyclones during winter that can be used for forecasting their frequency and surface impacts.

How to cite: Gerstman, H., Büeler, D., Wulff, C. O., Sprenger, M., and Domeisen, D.: The influence of the stratosphere on the North Atlantic storm track predictability in subseasonal-to-seasonal reforecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-553, https://doi.org/10.5194/egusphere-egu23-553, 2023.

EGU23-861 | Orals | AS1.3

Boreal Summer Intraseasonal oscillation convective initiations in S2S models 

Daniel Simon and Neena Joseph Mani

Boreal summer Intraseasonal Oscillation (BSISO), with its 20–90 day periodicity characterised by northward propagation over the northern Indian Ocean and eastward propagation over the equatorial region, acts as a major source of predictability in the intraseasonal time scale. Predicting the initiation of BSISO over the equatorial Indian Ocean is of vital importance in the prediction of BSISO's northward advancement over the ISM domain. This study tries to investigate where we stand in terms of predicting the BSISO initiation and propagation, making use of the reforecasts available from the different operational forecasting centres part of the Sub-Seasonal-to-Seasonal (S2S) prediction project. The BSISO convective initiations over the Equatorial Indian Ocean are objectively identified using OLR MJO Index(OMI), and the ability of the models to simulate the initiation and propagation of BSISO is assessed. The BSISO propagation skill, quantified in 9 S2S models, ranges from 11 to 29 days, while the BSISO initiation skill, quantified in 4 out of 9 models, ranges from 11 to 16 days, which is systematically lower compared to the skill of the BSISO non-initiation stages. Two major regions of BSISO initiation were identified, one over the Western Equatorial Indian Ocean and another over the Eastern equatorial Indian Ocean. Over these identified initiation regions, observation show a buildup (reduction) of lower tropospheric moisture before (after) the BSISO initiation. Out of the 9 models considered, few capture either the buildup or reduction, while the majority of the models show biases in capturing the moisture buildup and reduction. Previous studies have emphasised the role of background moisture in the propagation of BSISO. The relationship between the background moisture gradient over the ISM domain and the BSISO propagation prediction skill is examined in the S2S models and a positive relationship is found.

How to cite: Simon, D. and Joseph Mani, N.: Boreal Summer Intraseasonal oscillation convective initiations in S2S models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-861, https://doi.org/10.5194/egusphere-egu23-861, 2023.

EGU23-953 | Posters on site | AS1.3

s2spy, a package to boost (sub) seasonal forecasting with artificial intelligence 

Yang Liu, Bart Schilperoort, Jannes van Ingen, Sem Vijverberg, Peter Kalverla, and Dim Coumou

Reliable (sub) seasonal (S2S) forecasts remain a huge scientific challenge. The lead-time is too long to benefit from the atmosphere’s inertial memory, but too short for the atmosphere’s boundary conditions to be felt strongly. Only for specific "windows of predictability" (i.e. specific regions, timescales and climatic background states), skillful forecasts are possible, in an otherwise largely unpredictable future. Due to a number of successes in S2S forecasting, the interest in machine learning (ML) is growing fast. However, we argue there is a need for more standardization, consensus on best practices, higher efficiency, and higher reproducibility. Typical S2S ML use-cases, such as (1) pure statistical forecasting based on observations, (2) transfer learning, and (3) post-processing of dynamical model ensembles, require a large coding and preprocessing effort. Such experiments are not trivial to set up, and without sufficient experience and expertise there is a large risk of improper cross-validation and/or improper and non-standard verification.

Within a 3-year project, we are developing a high-level Python package called s2spy. Our aim is to make ML workflows more transparent and easier to build, and to facilitate standardization and collaboration across the S2S community. s2spy also contributes to a higher reproducibility and works towards a wider acceptance of standards and best practices. We will present our vision and the capabilities of our package, show-casing that we can build a model from raw climate data up to verification and explanation in only a few lines of code.

How to cite: Liu, Y., Schilperoort, B., van Ingen, J., Vijverberg, S., Kalverla, P., and Coumou, D.: s2spy, a package to boost (sub) seasonal forecasting with artificial intelligence, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-953, https://doi.org/10.5194/egusphere-egu23-953, 2023.

EGU23-1102 | ECS | Orals | AS1.3

MJO-induced land-atmosphere feedbacks across East Africa 

Joshua Talib, Christopher Taylor, Bethan Harris, and Caroline Wainwright

Across East Africa, sub-seasonal rainfall variability predominantly depends on the phase of the Madden Julian Oscillation (MJO). Rainfall is enhanced during MJO phases 2 to 4, and suppressed during phases 6 to 8. Given that MJO-induced anomalous precipitation can persist beyond several days, a surface response is expected. Using earth observations and reanalysis data, in this presentation we will show how MJO-induced precipitation anomalies promote a surface response which feeds back onto local and regional atmospheric conditions.

              MJO-induced rainfall suppression across East Africa decreases surface soil moisture across the exit region of the Turkana jet. Reduced soil moisture increases surface sensible heat fluxes and elevates land surface temperatures. The drier and warmer surface reduces surface pressure and leads to an intensification of the Turkana jet. We conclude that on average approximately 11% of the anomalous jet speed is associated with surface-driven pressure fluctuations over the course of a single day. Since the Turkana jet controls moisture transport from low-lying regions of East Africa into Central Africa, we highlight that surface-induced jet variations impact rainfall totals across East Africa. Furthermore, due to the Turkana jet response to spatial variations in surface warming, we also identify that the magnitude of MJO-induced anomalous precipitation is influenced by surface conditions prior an MJO event. For example, when the surface over southern South Sudan is anomalously dry, MJO-induced precipitation suppression is greater. This presentation will highlight that to fully exploit predictability from the MJO, forecast models must correctly represent surface processes and land-atmosphere interactions. Future work evaluating sub-seasonal forecast models and improving the representation of land-atmosphere interactions will enhance the lead-time of early warning systems across East Africa.

How to cite: Talib, J., Taylor, C., Harris, B., and Wainwright, C.: MJO-induced land-atmosphere feedbacks across East Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1102, https://doi.org/10.5194/egusphere-egu23-1102, 2023.

EGU23-1187 | Orals | AS1.3 | Highlight

Deep-learning-based monthly precipitation forecast for Europe 

Ramon Fuentes-Franco and Klaus Zimmermann

We implement deep neural networks to forecast monthly precipitation over Europe. This architecture conformed by several convolutional layers and fully connected layers uses four different variables (surface temperature, west-east wind at 200 hPa, precipitation and sea level pressure) coming from seven different operational forecast systems (1. ECCC 2. MeteoFrance  3. DWD  4. JMA 5. NCEP  6. ECMWF  7. CMCC). The neural network is trained using observations from E-OBS, a gridded land-only observational dataset covering the whole European continent. This convolutional neural network is trained using the period 1993-2012 and the validation period is 2013-2016, which is the range that is available for all operational forecast systems. 

Comparing with precipitation from observations we show that forecasted precipitation from this Deep-Learning model shows small biases in the whole European continent when forecasting monthly precipitation, especially over Sweden (with a small overestimation of less than 0.2 mm/day). With some higher negative biases over Southern Europe (<-1 mm/day). In turn, the representation of the mean precipitation over specific months and seasons was also assessed, showing that during the validation period this method is able to reproduce properly the spatial features of mean precipitation over Europe and its intensity.

How to cite: Fuentes-Franco, R. and Zimmermann, K.: Deep-learning-based monthly precipitation forecast for Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1187, https://doi.org/10.5194/egusphere-egu23-1187, 2023.

EGU23-1286 | ECS | Orals | AS1.3

Wheat yields in Kazakhstan can successfully be forecasted using a statistical crop model 

Paula Romanovska, Bernhard Schauberger, and Christoph Gornott

The COVID-19 pandemic, recent extreme weather events around the globe and the invasion of Russian forces in Ukraine have led to a disrupted global food market. As the 12th largest global wheat exporter, Kazakhstan is fundamental for regional and global food security. Timely and reliable predictions of Kazakh wheat production could therefore improve food security planning and management in Central Asia and beyond.

In this session, we want to present a statistical weather-driven yield forecast model that is run with publicly available weather and yield data and requires low computational power, making it easily replicable. Decision makers in Kazakhstan have expressed high interest in using the forecast model as a replenishment to currently applied work-intensive forecasting methods. We stringently evaluated our model in a double out-of-sample validation and used it to forecast total national wheat production in a fully blind run for 2022.

Our results show that the model can successfully hindcast wheat yields at the oblast (regional) level up to two months before the harvest. The hindcast of wheat yields for 1993 to 2021 produces a median R2 of 0.69 for the full model run and R2 values of 0.60 and 0.37 for two levels of out-of-sample validations, respectively. Based on these yield estimates we provide a robust hindcast of the total wheat production for Kazakhstan with an R2 value of 0.86 (0.81 and 0.73 for two levels of out-of-sample validations). We forecast total wheat production in Kazakhstan for 2022 to be 12.4 million tonnes and thus 5 % above the production of the last year.

How to cite: Romanovska, P., Schauberger, B., and Gornott, C.: Wheat yields in Kazakhstan can successfully be forecasted using a statistical crop model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1286, https://doi.org/10.5194/egusphere-egu23-1286, 2023.

EGU23-1376 | ECS | Posters on site | AS1.3

New classification showing the stratospheric memory concept: towards a better seasonal prediction 

Alexis Mariaccia, Philippe Keckhut, and Alain Hauchecorne

A new method of classification based upon an empirical orthogonal functions (EOFs) analysis of zonal wind anomalies of the 70 winters from 1950 to 2020, extracted from ERA5, revealed that the winter stratosphere tends to follow four independent scenarios. The first three scenarios: the January, the February, and the Double modes, are all characterized by a perturbed evolution of the polar vortex due to significant sudden stratospheric warmings (SSWs) occurring in mid-winter, generally causing the reversing of zonal winds. Unsurprisingly, these modes contain the information of preferential important SSWs’ timings, events including minor and major SSWs, and final stratospheric warming’s timings. Thus, their patterns show that the mid-winter is often anti-correlated with the winter end. This result is consistent with the conclusion done in a recent study showing that the polar vortex on a given month is anti-correlated with its state 2-3 months earlier. While the last scenario illustrates an unperturbed polar vortex evolution during winter for which only the final stratospheric warming’s timing differs, either early and dynamical or late and radiative.

The study of the mean evolutions of wave-1 and wave-2 amplitude anomalies associated with these four scenarios reveals that they possess singular dynamic behavior, especially for the wave-1 activities, which are consistent with their mean evolutions of zonal mean zonal winds. Indeed, we found that the wave-1 activity drops systematically for each scenario when zonal winds weaken due to an important. In contrast, it is not the case for the wave-2 activity.

How to cite: Mariaccia, A., Keckhut, P., and Hauchecorne, A.: New classification showing the stratospheric memory concept: towards a better seasonal prediction, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1376, https://doi.org/10.5194/egusphere-egu23-1376, 2023.

EGU23-2752 | Posters on site | AS1.3

MJO-related China rainfall teleconnections in the MetUM 

Maria Joao Carvalho, Prince Xavier, and Kalli Furtado

During a Madden-Julian Oscillation (MJO) event, anomalous convection triggers a dynamical response with anomalous large-scale ascent and upper-tropospheric divergence outside the tropics creates interaction between the MJO and the extratropical weather, modes of global circulation and climate variability. The MJO is known to have an impact on China rainfall and regional circulation with enhanced/ suppressed rainfall in South China during the propagation of the MJO from the Indian Ocean into the western Pacific. As the MJO is considered a major source of predictability at subseasonal time scales, it is important to understand how climate models are representing the MJO and its remote effects. This study is aimed to investigate the modelled MJO and associated local effects in China precipitation using the Met Office Unified Model (MetUM). It was found that the response of the rainfall over South China is asymmetric, with the enhancement of rainfall during the Indian Ocean convective phases (phase 2) of the MJO being much stronger than the suppression during the west Pacific phases (phase 6). This response signal was mostly due to the increase in probability of extreme precipitation events rather than the increase in number of rainy days. Analysis of the modelled MJO and associated response shows, although the MJO is more realistically represented in the atmosphere-ocean coupled simulation, the atmosphere-only simulation showed more evidence of MJO-related remote effects in the rainfall patterns over China. The ocean-coupled simulation shows no significant response to the propagation of MJO-associated convection whereas the atmosphere-only simulation shows the correct pattern of enhancement and suppression of rainfall and associated regional circulation pattern changes. The differences found in the representation of remote effects between atmosphere-only and ocean-coupled simulations may be attributed to the air-sea interaction processes and to fundamentally different mean-state biases which affect not only the representation of the MJO but also the propagation of MJO-induced Rossby waves. 

How to cite: Carvalho, M. J., Xavier, P., and Furtado, K.: MJO-related China rainfall teleconnections in the MetUM, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2752, https://doi.org/10.5194/egusphere-egu23-2752, 2023.

EGU23-3039 | ECS | Orals | AS1.3

The Optimal Initial Condition of MJO Development 

Chun-Hao Chang and Kai-Chih Tseng

Madden-Julian Oscillation (MJO), an intraseasonal oscillation over the equatorial Indian ocean and Pacific, has profound impacts around the globe. Its extended-range life cycle (20-90 days) makes it the most important predictability source on subseasonal-to-seasonal timescales. While the mechanisms responsible for MJO's life cycle have been well  explored through the frameworks of moisture modes, and tropical wave dynamics, the mechanisms of initiation remain unsolved. By using linear inverse modeling (LIM) and incorporating different frameworks, this study investigates the processes resulting in MJO convection initiation. It is suggested that multi-scale interactions play a vital role in intraseasonal convection initiation over the Indian ocean. On intraseasonal timescales, the remnant of former MJO can create an environment favoring the convection development for the next event through modulating the prevailing circulations and moisture state (e.g., moisture advection). On shorter timescales (< 20 days), the optimal initial condition arises from the synoptic convergence/divergence of moisture flux, and the upper troposphere instability. 

How to cite: Chang, C.-H. and Tseng, K.-C.: The Optimal Initial Condition of MJO Development, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3039, https://doi.org/10.5194/egusphere-egu23-3039, 2023.

EGU23-5201 | ECS | Posters on site | AS1.3

How well in advance can we predict cold spells over France? 

Naveen Goutham, Hiba Omrani, Omar Himych, and Riwal Plougonven

France is committed to achieving climate neutrality by 2050. In this respect, the heating sector, one of the largest energy-consuming sectors in France, is undergoing rapid electrification. In 2022, electricity contributed to the heating of more than 40% of French dwellings. As a result, the French electricity demand is increasingly becoming thermosensitive. Accordingly, for every 1°C drop in temperature below the threshold (i.e., 15°C) during winter, the electricity demand increases by ~2.4 GW in France. With a notable share of French nuclear reactors reaching their end of service life, several recent episodes of widespread cold spells over France have raised concerns about energy security. Hence, anticipating cold spells well in advance is increasingly becoming important for the smooth operation of the energy sector. In this regard, we assess the predictability of several recent episodes of cold spells on seasonal timescales over France using the seasonal predictions from the European Centre for Medium-Range Weather Forecasts. Additionally, we test a recently developed statistical downscaling methodology in forecasting cold spells over France, using the forecasts of upper-level fields, which are better predicted than the surface fields. On comparing the dynamical and statistical predictions, we show that the statistical predictions, relying upon the information contained in the better-predicted upper-level fields, perform significantly better than the dynamical counterparts in predicting cold spells beyond a month.

How to cite: Goutham, N., Omrani, H., Himych, O., and Plougonven, R.: How well in advance can we predict cold spells over France?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5201, https://doi.org/10.5194/egusphere-egu23-5201, 2023.

EGU23-5397 | ECS | Orals | AS1.3 | Highlight

Factors influencing sub-seasonal forecast skill of Greenland Blockings 

Marisol Osman, Christian M. Grams, and Remo Beerli

Greenland blocking (GL) resembles the negative phase of the NAO and features a strong positive Z500 anomaly over Greenland and a zonally aligned negative anomaly stretching from the eastern North Atlantic into Northern Europe. The prevailing westerly flow is then deflected southward and extends into the Mediterranean. It causes melting events of the Greenland Ice Sheet which can impact global sea-level rise and has strong downstream impacts on Europe. It occurs year-round, although is more common in winter (11.7%) compared to summer (9.1%). GL is forecast with good ability by S2S models. This skill is driven by the performance in winter, when GL is persistent. In this study, we explore whether the skill of GL blocking can be linked to external meteorological drivers or the prevalence of specific meteorological features. Re-forecasts using the European Centre for Medium-Range Weather Forecasts for the 1999-2019 period are considered and compared against ERA Interim reanalysis over the same period. We focus on the factors affecting the skill, as depicted by the Brier Skill Score, from lead times 6 to 10 days, where the skill is 30% to 70% smaller than the skill at lead time 1 day.

Results show that most of the GL blocking events associated with low skill occur in spring. In this season, the model fails in forecasting the transition from Scandinavian Blocking to Greenland Blocking, in opposition to the rest of the seasons, when this transition is well predicted. The analysis of the role of large-scale processes that affect GL skill reveals that half of the forecasts of GL events initialized up to 30 days after a sudden stratospheric warming shows poor skill. In addition, the forecasts of GL events initialized with an active MJO in phase 6 and 7 present good skill whereas those forecast GL events initialized during an active MJO in phase 2 to 4 show poor skill. This link between large-scale factors and skill offers potential guidance in operational forecasting.

How to cite: Osman, M., Grams, C. M., and Beerli, R.: Factors influencing sub-seasonal forecast skill of Greenland Blockings, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5397, https://doi.org/10.5194/egusphere-egu23-5397, 2023.

EGU23-5665 | ECS | Orals | AS1.3

The seasonal teleconnections of the Indian Ocean Dipole to the North Atlantic region 

Tim Hempel, Antje Weisheimer, and Tim Palmer

The Indian Ocean Dipole (IOD) is a major source of seasonal climate variability in the
Indian Ocean. This dipole has strong impacts on the Indian Ocean region and through
teleconnections can influence the seasonal climate of remote regions like the North Pacific
and North Atlantic. A prominent example of this teleconnection from the IOD occurred
in the winter 2019/2020, where the IOD was in a positive state. This influenced the state
and predictability of the Northern Hemisphere extratropics. Thus, a good understand-
ing of the mechanism that transports information from the Indian Ocean to the North
Atlantic is desirable. In this contribution we investigate the special teleconnection of the
winter 2019/2020 and analyse the transport mechanism.
In model experiments with the OpenIFS from ECMWF we show that the NAO in the
winter 2019/2020 is influenced by the IOD and analyse the teleconnection mechanisms.
We use hindcast ensemble model experiments of the DJF season 2019/2020 to analyse
the behaviour of the IOD and its impact on the NAO. In the uncoupled OpenIFS the Sea
Surface Temperature (SST) boundary conditions are perturbed in regions of importance
to the NAO (like the ENSO region and the Indian Ocean). With these perturbations we
identify the relative importance of individual ocean regions to the state of the NAO in
the winter of 2019/2020.
We contrast the experiments with the perturbed SST conditions to the operational ECMWF
System5 forecast and ERA5. Experiments with the 2019/2020 SST’s in the In-
dian Ocean (with other boundary conditions set to climatology) reproduce many of the
observed atmospheric 2019/2020 features. In contrast, experiments with SST’s in the
Pacific show very different patterns to the observed 2019/2020 ones.
We identify eddy-mean-flow interactions as a mechanism that connects and transports
information from the Indian Ocean to the North Atlantic. With Hoskins E-Vectors we
show that anomalous eddy activity during IOD events impacts the position and strength
of the Northern Hemisphere extratropical jet. This interaction provides a teleconnection
mechanism in addition to the Rossby-wavetrain discussed in other studies.

How to cite: Hempel, T., Weisheimer, A., and Palmer, T.: The seasonal teleconnections of the Indian Ocean Dipole to the North Atlantic region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5665, https://doi.org/10.5194/egusphere-egu23-5665, 2023.

EGU23-5742 | Posters on site | AS1.3

S2S prediction of summer heatwaves in the Iberian Peninsula using convolutional networks 

Marie Drouard, Jorge Pérez-Aracil, David Barriopedro, Pablo G. Zaninelli, José M. Garrido-Perez, Dušan Fister, Sancho Salcedo-Sanz, and Ricardo García-Herrera

In this ongoing study we aim at using machine learning algorithms to better understand and improve southern Europe summer heatwave prediction on sub-seasonal to seasonal timescales (S2S). Summer heatwaves are extreme events that have large socio-economic impacts on mortality rate, crop yields, energy demand or water resources and southern Europe is particularly prone and vulnerable to such events.  

To do this, we train a convolutional network coupled with a multilayer perceptron to forecast with a 15-day and 1-month lead times the occurrence and intensity of heatwave in summer. This forecast model is trained with ERA5 data. The predictors fed to this model are monthly means of the SST, local soil moisture, outgoing longwave radiation, snow cover and sea-ice cover. The target is a monthly-mean heatwave index integrated over a sub-area of southern Europe. 

Here, we will present the initial results of this ongoing work and the next steps, focusing first on the Iberian Peninsula only. 

How to cite: Drouard, M., Pérez-Aracil, J., Barriopedro, D., Zaninelli, P. G., Garrido-Perez, J. M., Fister, D., Salcedo-Sanz, S., and García-Herrera, R.: S2S prediction of summer heatwaves in the Iberian Peninsula using convolutional networks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5742, https://doi.org/10.5194/egusphere-egu23-5742, 2023.

EGU23-6161 | Orals | AS1.3

The Dynamics and Structure of the Baroclinic Annular Mode 

Edwin Gerber, Madeleine Youngs, and Olivier Pauluis

As first explored by Thompson and Barnes (2014), hemispheric mean storm activity (or related quantities, such as the meridional eddy heat flux) exhibits periodicity on 20-30 day time scales.  They characterized this variability with the so-called Baroclinic Annular Mode, or BAM, a ring of enhanced eddy activity which is present in both hemispheres, but most pronounced in the south, which is less perturbed by zonal asymmetries relative to the north.   The mechanism behind this internally generated periodicity, however, has remained elusive.  We probe the dynamics and structure of the BAM on two fronts.  To understand the mechanism, we develop a minimal model that captures the essential dynamics: 2 layer quasi-geostrophic flow in a channel. By varying the geometry of the channel and the thermal and frictional forcing, we tease out the parameters that control the period and amplitude of the BAM.  The resulting changes in the BAM support the general framework of the charge-discharge mechanism proposed by Thompson and Barnes, but demand a more detailed explanation for the coupling between eddies and the mean baroclinicity that generates enhanced variability on subseasonal time scales.  On a second front, we apply dynamical mode decomposition (DMD) to atmospheric reanalyses of the Southern Hemisphere to quantify the structure of the southern BAM.  DMD captures BAM variability, providing additional information on relationships between the eddy kinetic energy and other mean and eddy quantities.  It suggests that moisture plays a fundamental role in the relationship between the eddy activity and baroclinicity, and that changes in stratification are more important than horizontal temperature gradients in the dynamics.    In this sense, the underlying BAM dynamics of vacillation between eddy and potential energy are remarkably robust, active in our moist atmosphere and in dry quasi-geostrophic systems where only the meridional temperature gradient can capture the available energy.

How to cite: Gerber, E., Youngs, M., and Pauluis, O.: The Dynamics and Structure of the Baroclinic Annular Mode, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6161, https://doi.org/10.5194/egusphere-egu23-6161, 2023.

EGU23-6511 | Posters on site | AS1.3

Evaluating Western North Pacific Tropical Cyclone Forecast in the Subseasonal to Seasonal Prediction Project Database 

Xiaochun Wang, Duane Waliser, Frederic Vitart, Xianan Jiang, and Shakeel Asharaf

The Daily Tropical Cyclone Probability (DTCP), defined as the probability of tropical cyclone occurrence within 500 km of a location in one day, is proposed and used in evaluating subseasonal to seasonal (S2S) predictions from the S2S Prediction Project Database, from May 1 to Oct. 31, 1999, to 2010. The ensemble reforecasts are collected from eleven operational centers, the BoM, CMA, ECCC, ECMWF, HMCR, ISAC, JMA, KMA, METFR, NCEP, and UKMO.  In both observation and these eleven forecast models, the DTCP is modulated by the Boreal Summer Intraseasonal Oscillation (BSISO), depicted by the two indices, BSISO1 and BSISO2. During BSISO1 phases 1, 5, 6, 7, and 8, the DTCP in the northwestern Pacific region is ~3.5 times higher. Similarly, during phases 1, 2, 3, 4, and 8 of BSISO2, the DTCP is  ~2.5 times higher.  Among the eleven models, the ECMWF model best reproduces the climatological DTCP and its modulation by the BSISO in the western North  Pacific region, followed by NCEP, KMA, JMA  models. Using the DTCP metric, the highest debiased Brier Skill Score of the eleven models is from ECMWF, which has a slightly less skillful prediction than the reference climatological forecast with lead time 11 to 30 days. The skill of the eleven models is higher during the non-active phases of tropical cyclone activity than their skill during the active phases.  The updated results based on the real-time tropical cyclone forecasts of the S2S Prediction Project Database  from these eleven systems will also be discussed.

How to cite: Wang, X., Waliser, D., Vitart, F., Jiang, X., and Asharaf, S.: Evaluating Western North Pacific Tropical Cyclone Forecast in the Subseasonal to Seasonal Prediction Project Database, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6511, https://doi.org/10.5194/egusphere-egu23-6511, 2023.

EGU23-7102 | ECS | Orals | AS1.3

Tropical cyclone precipitation skill in S2S models 

Jorge L Garcia-Franco, Chia-Ying Lee, Suzana Camargo, Michael Tippett, Daehyun Kim, Andrea Molod, and Young-Kwon Lim

Tropical cyclone precipitation (TCP) contributes a significant fraction of total annual rainfall and also is a frequent cause of extreme precipitation in many parts of the tropics. The climatology of TCP in the S2S models is characterized by dry biases in the North Atlantic and wet biases in most other basins,  specially in the Southern Indian Ocean and Australia. 
Biases in total precipitation (P), TCP and their ratio (TCP/P) are mostly positive in the multi-model ensemble mean and change very little with lead time. in these models the frequency biases are the dominant contribution to TCP biases. However, in some models, there are positive biases in average precipitation per each TC which contribute significantly to TCP biases at equatorial latitudes.

The prediction skill of these reforecasts is evaluated using skill scores such as the ranked probability skill score for TCP and the Brier Skill score for genesis and occurrence. The implication of these results is discussed for their relevance to mean and extreme precipitation prediction skill using S2S models.

How to cite: Garcia-Franco, J. L., Lee, C.-Y., Camargo, S., Tippett, M., Kim, D., Molod, A., and Lim, Y.-K.: Tropical cyclone precipitation skill in S2S models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7102, https://doi.org/10.5194/egusphere-egu23-7102, 2023.

EGU23-7168 | Orals | AS1.3

European S2S streamflow forecasting: Towards a seamless communication 

Ilias Pechlivanidis and Louise Crochemore

Information at the sub-seasonal to seasonal (S2S) time scale can be of high socio-economic value to a variety of users whose decision-making depends on climate variability. The usability of S2S forecasts generated by Numerical Weather Prediction (NWP) systems has increased over the years not only due to their skill improvement but also due to their potential to bridge the medium-range and seasonal horizons. The skill of the sub-seasonal (4-6 weeks ahead) and seasonal (6-12 months ahead) NWP-based forecasts in space and time depends on different factors, including the representation of the physical process, the initialization frequency and the spatial resolution. However, the NWP model setups differ between the two time horizons, and this consequently intrinsic differences between the two forecast products. To date, it has been subjectively accepted that during the first time horizons, e.g. up to 6 weeks ahead, the sub-seasonal forecasts are more informative than the seasonal forecasts, and hence all efforts on generating a seamless product are implemented through a direct merging of the two products. This unfortunately masks the potential for tailored seamless products that extract the best S2S information available.

Here, we evaluate the S2S hydro-meteorological forecasts from the ECMWF sub-seasonal (ENS-ER) and seasonal (SEAS5) products, aiming to identify their skill complementarity in space and time and further seamlessly communicate them for improved decision-making. Both the ENS-ER and the SEAS5 precipitation and temperature forecasts were bias-adjusted prior to forcing the E-HYPE hydrological model. The investigation focuses on the period 1999-2015. Overall, results highlight both spatial and temporal complementarities between the two systems, which is very encouraging for a seamless communication. In particular, ENS-ER-based hydro-meteorological forecast skill patterns appear to be more homogeneous spatially, while SEAS5-based forecasts ensure skill at longer forecast horizons. This diagnostic analysis is a step forward in hydro-climate services, indicating the tipping points in all European river systems for switching from ENS-ER to SEAS5 forecasts.

How to cite: Pechlivanidis, I. and Crochemore, L.: European S2S streamflow forecasting: Towards a seamless communication, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7168, https://doi.org/10.5194/egusphere-egu23-7168, 2023.

EGU23-7750 | ECS | Orals | AS1.3

Probabilistic predictions of global fire activity 

Miguel Ángel Torres-Vázquez, Andrina Gincheva-Norcheva, Amar Halifa-Marín, Juan Pedro Montavez, and Marco Turco

Seasonal forecasts of meteorological drought can help decision-making for weather-driven wildfires (Turco et al., 2018). However, one of the main drawbacks of drought prediction lies in the uncertainty of monitoring precipitation in near-real time. In this contribution we assess the predictability of the Standardized Precipitation Index (SPI) on a global scale, combining 11 datasets (DROP; Turco et al., 2020) as observed initial conditions with empirical and dynamic predictions of precipitation. The empirical predictions are based on the ensemble-based streamflow prediction system (ESP, an ensemble-based reordering of historical data) and the dynamics on the new generation seasonal prediction model developed by ECMWF (System 5; S5). Although both systems show comparable quality, S5 performs better at longer forecast timescales, especially over tropical regions.

Subsequently, we investigate whether the S5 seasonal forecasts can predict area burned anomalies on a global scale. To do so, we link the seasonal climate predictions of S5 to an empirical climate-fire model, using standard regression techniques in the framework of generalised linear models. The seasonal climate predictions of S5 have shown high and significant performance (with a mean relative operating characteristic “ROC” area value of 0.87) over a large fraction of the burnable area (~47%).

In summary, given that all data are publicy available in near real time, our results provide a basis for the development of a global probabilistic seasonal drought and burned area forecast product.

References

Turco, M., Jerez, S., Doblas-Reyes, F. J., AghaKouchak, A., Llasat, M. C., & Provenzale, A. (2018). Skilful forecasting of global fire activity using seasonal climate predictions. Nature Communications, 9(1), 1–9.

Turco, M., Jerez, S., Donat, M. G., Toreti, A., Vicente-Serrano, S. M., & Doblas-Reyes, F. J. (2020). A global probabilistic dataset for monitoring meteorological droughts. Bulletin of the American Meteorological Society, 101(10), E1628–E1644.

Acknowledgements

We acknowledge funding through the project ONFIRE, grant PID2021-123193OB-I00,funded by MCIN/AEI/ 10.13039/501100011033.

How to cite: Torres-Vázquez, M. Á., Gincheva-Norcheva, A., Halifa-Marín, A., Montavez, J. P., and Turco, M.: Probabilistic predictions of global fire activity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7750, https://doi.org/10.5194/egusphere-egu23-7750, 2023.

EGU23-8258 | Posters virtual | AS1.3

The Winter North Pacific Teleconnection in Response to ENSO and the MJO in Operational Subseasonal Forecasting Models Is Too Weak 

Chen Schwartz, Chaim Garfinkel, Wen Chen, Yanjie Li, Priyanka Yadav, and Daniela I.V. Domeisen

Teleconnection patterns associated with the Madden–Julian oscillation (MJO) and El Niño–Southern Oscillation (ENSO) impact weather and climate phenomena in the Pacific–North American region and beyond, and therefore accurately simulating these teleconnections is of importance for seasonal and subseasonal forecasts. Systematic biases in boreal midwinter ENSO and MJO teleconnections are found in eight subseasonal to seasonal (S2S) forecast models over the Pacific–North America region. All models simulate an anomalous 500-hPa geopotential height response that is too weak. This overly weak response is associated with overly weak subtropical upper-level convergence and a too-weak Rossby wave source in most models, and in several models there is also a biased subtropical Pacific jet, which affects the propagation of Rossby waves. In addition to this overly weak response, all models also simulate ENSO teleconnections that reach too far poleward toward Alaska and northeastern Russia. The net effect is that these models likely underestimate the impacts associated with the MJO and ENSO over western North America, and suffer from a reduction in skill from what could be achieved.

How to cite: Schwartz, C., Garfinkel, C., Chen, W., Li, Y., Yadav, P., and Domeisen, D. I. V.: The Winter North Pacific Teleconnection in Response to ENSO and the MJO in Operational Subseasonal Forecasting Models Is Too Weak, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8258, https://doi.org/10.5194/egusphere-egu23-8258, 2023.

Forecasts on sub-seasonal to seasonal (S2S) timescales have huge potential to improve early warning and anticipatory action ahead of high impact events. However, fully realising this potential predictability requires reliable forecasts that are communicated effectively so that they can support appropriate preparedness action. This study reflects on the African SWIFT (Science for Weather Information and Forecasting Techniques) S2S forecasting testbed which brought together researchers, forecast producers and forecast users from a range of African and UK institutions. The testbed used a co-production approach to pilot the provision of real-time bespoke S2S forecast products for applications. The S2S testbed supported decision-makers in a range of sectors and contexts. For example, informing food security decisions and hydropower energy planning in East Africa, supporting agricultural decision-making across West Africa, and, in health applications, increasing the lead-time for potential disease outbreaks.

 

This study critically reflects on the benefits and challenges of the co-production process within the S2S applications context. Specifically, while having direct access to the real-time S2S data allowed user-guided iterations to products to make them more actionable for their specific context. Some key lessons for effective co-production emerged. First, it is critical to ensure there is sufficient resource to support co-production, especially in the early co-exploration of needs. Second, all the groups in the co-production process require capacity building to effectively work in new knowledge systems. Third, evaluation should be ongoing and combine meteorological verification with decision-makers feedback. Ensuring the sustainability of project-initiated services within the testbed hinges on integrating the knowledge-exchanges between individuals in the co-production process into shaping sustainable pathways for improved operational S2S forecasting within African institutions.

How to cite: Hirons, L.: Using a co-production approach to support effective application of S2S forecasts in Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9342, https://doi.org/10.5194/egusphere-egu23-9342, 2023.

Extreme precipitation events (EPE), especially those leading to floods and landslides, are devastating to society. Predicting these events in advance can help disaster managers to carry out plans of action to respond effectively to any oncoming adverse events. Sub-seasonal forecasts, which aim to predict the weather with 2 weeks to 2 months in advance, can help to provide valuable and actionable information to disaster managers. Given the potential usefulness to end users, it is vital to assess the skill of sub-seasonal forecasts in predicting EPEs. However, given that precipitation is known to be a difficult variable to predict, the lead time at which forecasts are skilful may be limited. This study, therefore, aims to assess at which lead time sub-seasonal forecasts of atmospheric drivers of EPEs are skilful.

The study investigates the skill of the European Centre for Medium-Range Weather Forecast (ECMWF) sub-seasonal reforecast in predicting EPE over Italy from 2001 to 2020. A total of 100 EPEs are used as case studies. The variables evaluated are total precipitation, mean sea level pressure, geopotential height at 500 hPa and specific humidity at 850 hPa. Variables are averaged over the 5 days surrounding the date of the EPE. ERA5 is used as the reference dataset. Both deterministic and probabilistic metrics are used to assess the skill of the reforecast.

Results show that the skill for precipitation is limited to the first two weeks. Nevertheless, the ECMWF sub-seasonal product is skilful in predicting the atmospheric fields associated with the selected EPEs, such as MSLP and geopotential height, showing both reliability and discrimination beyond two weeks.

How to cite: Scott, W., Gaetani, M., and Fosser, G.: Skill assessment of sub-seasonal forecasts of different atmospheric variables related to extreme precipitation events over Italy, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10052, https://doi.org/10.5194/egusphere-egu23-10052, 2023.

EGU23-10243 | ECS | Orals | AS1.3

Improved subseasonal prediction of South Asian monsoon rainfall using data-driven forecasts of oscillatory modes 

Eviatar Bach, Venkat Krishnamurthy, Jagadish Shukla, Safa Mote, A. Surjalal Sharma, Eugenia Kalnay, and Michael Ghil

Predicting the temporal and spatial patterns of South Asian monsoon rainfall within a season is of critical importance due to its impact on agriculture, water availability, and flooding. The monsoon intraseasonal oscillation (MISO) is a robust northward-propagating mode which determines the active and break phases of the monsoon, and much of the regional distribution of rainfall. However, dynamical atmospheric forecast models predict this mode poorly. Data-driven methods for MISO prediction have shown more skill, but only predict the rainfall portion corresponding to MISO.

Here, we combine state-of-the-art ensemble precipitation forecasts from a high-resolution atmospheric model with data-driven forecasts of MISO using a novel method. The ensemble members of the detailed atmospheric model are projected onto a lower-dimensional subspace corresponding to the MISO dynamics, and are then weighted according to their distance from the data-driven MISO forecast in this subspace. We thereby achieve significant improvements in rainfall forecasts over India, as well as the broader monsoon region, at 10–30 day lead times, an interval that is generally considered as a predictability gap. Our results demonstrate the potential of leveraging the predictability of intraseasonal oscillations to improve extended-range forecasts; more generally, they point towards a future of combining dynamical and data-driven forecasts for Earth system prediction.

How to cite: Bach, E., Krishnamurthy, V., Shukla, J., Mote, S., Sharma, A. S., Kalnay, E., and Ghil, M.: Improved subseasonal prediction of South Asian monsoon rainfall using data-driven forecasts of oscillatory modes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10243, https://doi.org/10.5194/egusphere-egu23-10243, 2023.

EGU23-11267 | ECS | Posters on site | AS1.3

Impact of flux type variable exchange method in the atmosphere-ocean coupled version of the Korean Integrated Model (KIM) system for extended medium-range weather forecast 

Namgu Yeo, Eun-Chul Chang, Hajoon Song, Junseong Park, Eunjeong Lee, and Myung-Seo Koo

Extended medium-range prediction targets a period of up to 30 days, which is a longer period than medium-range (up to 15 days) and shorter than seasonal (up to 3 months) forecast. The atmospheric response to the initial condition significantly impacts predictability in medium-range prediction while ocean response which is a slower change compared to the atmosphere is also an important factor in extended medium-range prediction. Thus, it is important to consider not only initial forcing but also air-sea interaction containing ocean response in extended medium-range prediction. The interactions in the earth system model can be considered among the atmosphere, ocean, sea-ice, and ocean wave by coupling of each components. The Korean Integrated Model (KIM) system, which is a global atmospheric forecast model, was developed by the Korea Institute of Atmospheric Prediction Systems. Recently, the ocean and sea-ice model components have been coupled with the KIM atmosphere system, and continuous efforts are being made to improve its performance. The air-sea interaction in an atmosphere-ocean coupled system can be considered by exchanging the variables that require interaction between components with a coupler. The bulk type exchange method basically transfers state variables such as temperature, pressure, and wind, which are used to get flux variables that contain interacting information among the atmosphere, ocean, and sea-ice. The bulk method is simple but the energy budget at the interface among the model components may become inconsistent due to the use of different formulas during calculation of the flux variables. In this study, exchange variables are changed by replacing atmospheric state variables with flux and momentum variables, which are the final form used in the ocean model. It is found that the corrected flux and momentum of the ocean surface resulting from the flux type exchange method change the ocean structure, particularly over the low latitude region. The atmosphere reacts to the changed ocean state, affecting not only the lower atmosphere but also the upper atmosphere. The results show that the flux type variable exchange method has advantages for considering air-sea interaction, which would improve the performance of extended medium-range weather forecast compared to the bulk type exchange method.

Keywords: extended medium-range forecast, coupled model, air-sea interaction, bulk type method

Acknowledgement

This work was funded by the Korea Meteorological Administration Research and Development Program under Grant KMI2022-01210.

 

 

How to cite: Yeo, N., Chang, E.-C., Song, H., Park, J., Lee, E., and Koo, M.-S.: Impact of flux type variable exchange method in the atmosphere-ocean coupled version of the Korean Integrated Model (KIM) system for extended medium-range weather forecast, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11267, https://doi.org/10.5194/egusphere-egu23-11267, 2023.

Rain-fed agriculture constitutes more than 95 % of cropland in Germany. It depends heavily on rainfall patterns and the water storage capacities of top soil layers. Intense summer droughts with long-lasting lack of precipitation leads to yield loss in wheat, corn and sugar beet production in the last years 2018, 2019, 2020 and 2022. Hence, these drought events increase the requirement of long-range forecasts for precipitation and soil moisture, which could provide useful predictions for agricultural applications.

Here a coupled modelling attempt is presented, that combines the extended-range ENS-forecasts from the European Centre for Medium-Range Weather Forecasts (ECWMF) with the soil-vegetation-atmosphere-transfer (SVAT) impact model AMBAV to simulate the top soil moisture for subseasonal forecasts on a downscaled 5x5 km grid in Germany. A quality assessment of forecast ensemble means from July 2022 to November 2022 has been done with the corresponding hindcasts for the preceding 20 years. The mean squared error skill score (MSESS) of weekly averages reveals a significant forecast skill up to 4-6 weeks for soil moisture in the upper 60 cm in comparison to an AMBAV analysis run based on gridded weather station data. In contrast, the precipitation forecast skill is much lower and achieve only adequate forecast skill with lead times up to two weeks. Due to the low variability and persistence of soil moisture values, it is proposed, that this storage variable is well suited for climate services like agricultural drought predicting systems on subseasonal time scales. It could offer guidance with sufficient reliability for medium-term management adjustments like irrigation planning or reduced fertilizer usage in case of expected severe drought periods. Overall, the results of this study show the potential of subseasonal soil moisture forecasts for agricultural applications. Further research is needed to verify these findings and to extend the forecast analysis period to the entire year. Then the impact modelling system might contribute to the adaptation of agriculture to climate change in Germany.

How to cite: Leppelt, T.: Quality assessment of subseasonal soil moisture forecasts for agricultural applications in Germany, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11833, https://doi.org/10.5194/egusphere-egu23-11833, 2023.

EGU23-12537 | ECS | Posters on site | AS1.3

A sub-seasonal to seasonal prediction system with MPI-ESM 

Vimal Koul, Sebastian Brune, Cristian Febre, Daniela I.V. Domeisen, and Johanna Baehr

Current sub-seasonal prediction systems are traditionally based on models developed for numerical weather prediction. We present a different approach wherein we develop a sub-seasonal prediction system using a coupled Earth system model, the Max-Planck-Institute Earth system model (MPI-ESM), developed primarily for the use in climate prediction. We present results from initialized sub-seasonal reforecasts for the time period 1993-2017 from a 1st generation (CMIP5) seasonal-turned-sub-seasonal prediction system based on MPI-ESM including different components of the Earth system: atmosphere, land surface, ocean, and marine ecosystems. With our system we find (1) that atmospheric variables can be predicted with a quality and prediction horizon similar to what is found within the range of current sub-seasonal to seasonal prediction systems, (2) that extreme events as diverse as heatwaves over land, storm severity over Europe, and sudden stratospheric warmings can be skilfully predicted one to a few weeks ahead, (3) that sea surface temperatures can be skilfully predicted in the majority of large marine ecosystems for several weeks ahead, and (4) that sea ice area in the majority of Arctic seas can be skillfully predicted several weeks ahead. Our findings indicate that a coupled Earth system model like MPI-ESM can already be seamlessly used for sub-seasonal to seasonal (to decadal) climate predictions of different domains of the Earth system. Ultimately these results ask for the seamless approach to be embedded into the development of future coupled Earth system models.

How to cite: Koul, V., Brune, S., Febre, C., Domeisen, D. I. V., and Baehr, J.: A sub-seasonal to seasonal prediction system with MPI-ESM, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12537, https://doi.org/10.5194/egusphere-egu23-12537, 2023.

EGU23-13445 | ECS | Orals | AS1.3

Optimal transport for the multi-model combination of sub-seasonal ensemble forecasts 

Camille Le Coz, Alexis Tantet, Rémi Flamary, and Riwal Plougonven

Combining ensemble forecasts from several models has been shown to improve the skill of S2S predictions. One of the most used method for such combination is the “pooled ensemble” method, i.e. the concatenation of the ensemble members from the different models. The members of the new multi-model ensemble can simply have the same weights or be given different weights based on the skills of the models. If one sees the ensemble forecasts as discrete probability distributions, then the “pooled ensemble” is their (weighted-)barycenter with respect to the L2 distance.
Here, we investigate whether a different metric when computing the barycenter may help improve the skill of S2S predictions. We consider in this work a second barycenter with respect to the Wasserstein distance. This distance is defined as the cost of the optimal transport between two distributions and has interesting properties in the distribution space, such as the possibility to preserve the temporal consistency of the ensemble members.
We compare the L2 and Wasserstein barycenters for the combination of two models from the S2S database, namely ECMWF and NCEP. Their performances are evaluated for the weekly 2m-temperature over seven winters in Europe (land) in terms of different scores. The weights of the models in the barycenters are estimated from the data using grid search with cross-validation. We show that the estimation of these weights is critical as it greatly impacts the score of the barycenters. Although the NCEP ensemble generally has poorer skills than the ECMWF one, the barycenter ensembles are able to improve on both single-model ensembles (although not for all scores). At the end, the best ensemble depends on the score and on the location. These results constitute a promising first step before implementing this methodology with more than two ensembles, and ensembles having less contrasting skills.

How to cite: Le Coz, C., Tantet, A., Flamary, R., and Plougonven, R.: Optimal transport for the multi-model combination of sub-seasonal ensemble forecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13445, https://doi.org/10.5194/egusphere-egu23-13445, 2023.

EGU23-14682 | ECS | Posters on site | AS1.3

Characteristics of Tropical cyclones in sub-seasonal forecasting with GloSea5: Predictability in extreme ENSO phases and a climate regime shift 

Taehyung Kim, Eunji Kim, Minkyu Lee, Dong-Hyun Cha, Sang-Min Lee, Johan Lee, and Kyung-On Boo

Tropical Cyclone (hereafter, TC), a most destructive weather phenomenon that causes enormous socio-economic damage, occurs around 25 times every year in the western North Pacific, of which Korea is directly or indirectly affected by about 3 to 4 TCs every year. Even if it is affected by a small number of TCs, the damage could be unimaginably large. To preemptively prepare and respond to TCs, predictability on the sub-seasonal to seasonal (S2S) time-scale, over two weeks to two months is being emphasized. In this study, the characteristics of TCs in sub-seasonal forecasting with the Global Seasonal Forecast System 5 (GloSea5) of the Korea Meteorological Administration (KMA) were assessed over the western North Pacific (WNP). The predictability of GloSea5 was examined for its ability to reproduce observed TC climatology as well as changes in TC genesis with the El Niño-Southern Oscillation (ENSO) and a 1998/1999 climate regime shift. GloSea5 showed skilful performance in simulating the frequency and genesis spatial distribution of TCs in climatology and both extreme ENSO phases. Synoptic fields related to TC genesis were also reasonably captured, despite some systematic biases in those. GloSea5 performed well in terms of characteristics of changes in TC genesis due to the climate regime shift. However, there were biases in TC frequency before the regime shift and in changes in TC-related environmental fields. This study implies that GloSea5, which has a good predictive skill for TC genesis over the WNP, can be used as an operational model for sub-seasonal TC forecasting, although it requires continuous improvements to reduce systematic errors

How to cite: Kim, T., Kim, E., Lee, M., Cha, D.-H., Lee, S.-M., Lee, J., and Boo, K.-O.: Characteristics of Tropical cyclones in sub-seasonal forecasting with GloSea5: Predictability in extreme ENSO phases and a climate regime shift, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14682, https://doi.org/10.5194/egusphere-egu23-14682, 2023.

EGU23-15043 | ECS | Orals | AS1.3

Investigating the Role of Weather Patterns in Crop Yield Variability and Predictability 

Chris Knight, Abdou Khouakhi, and Toby Waine

Climate change is causing disruptions in Earth's weather patterns, leading to an increase in the frequency and severity of extreme weather events such as droughts, floods, frost, and heatwaves. These events can impact food production and lead to challenges in meeting the food needs of a growing population. Previous research has documented the role of temperature and precipitation during the growing season in explaining crop yield variability. For example, droughts and extreme heat can reduce cereal production by 9-10%.

Current crop yield models use only a few meteorological variables to represent weather conditions. However, weather patterns or weather regimes, (i.e., persistent, and recurrent flow patterns of the large-scale atmospheric circulation) can provide a more comprehensive view of weather conditions, and can be used to predict and characterise extreme weather events and explain crop yield variation.

In this study, we first conducted a literature review to examine the links between extreme weather events, such as heat waves, and droughts with weather patterns and regimes. One of the main findings of that review was the need to define what extreme weather is in the context of agriculture. The new definition is based on studies that identified optimal and terminal weather conditions for winter wheat at specific phenological stages. Using this definition of extreme weather, we analyse historic yields in East Anglia, UK, forming statistically based relationships between low yield years with a set of classified weather patterns from the UK Met Office. We focused on the weather patterns frequency of occurrence and persistence with additional consideration given to potential microclimates as we compare the effects weather patterns have on a specific farm with a long-term data set to the effects of the larger region. Preliminary analyses shows that a small number of these weather patterns are associated with high impact weather events that cause yield limiting conditions or physical damage to the crop such as wind lodging.

It is hoped that further research will lead to the development of a next-generation crop yield variation model taking into account the weather patterns, which can provide longer-term predictions of regional crop yield variability to help agri-businesses, crop insurers and farmers to facilitate decision making, respond effectively to regional and global crop production shocks and food price spikes, and develop adaptation strategies to reduce the potential impact of extreme weather events.

How to cite: Knight, C., Khouakhi, A., and Waine, T.: Investigating the Role of Weather Patterns in Crop Yield Variability and Predictability, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15043, https://doi.org/10.5194/egusphere-egu23-15043, 2023.

EGU23-15077 | ECS | Posters on site | AS1.3

Subseasonal prediction of the July 2021 extreme rainfall event over Henan China in S2S forecasting systems 

Yuhan Yan, Congwen Zhu, and Boqi Liu

Unprecedented heavy rainfall reaches the warming Earth more frequently, creating the need for effective risk-warning alerts that utilize subseasonal-to-seasonal (S2S) forecasting to integrate information from nowcasting, weather, and seasonal predictions. A record-breaking flooding event occurred in Zhengzhou, Henan Province of China during 17–23 July 2021, causing 398 total of deaths and vast economic losses.

A number of studies have shown this super severe heavy flooding occurred under the background of multiscale circulation interactions and the impacts of remote tropical cyclones. Here, we evaluated the predictability of this extreme rainfall event and the impacts of tropical cyclones (TCs) using subseasonal-to-seasonal (S2S) operational models. Most S2S models can reasonably predict the wet-in-north and dry-in-south monthly rainfall pattern over China in July. Only four models captured the location, probability, and sudden intensification of the Zhengzhou rainfall extremes in advance of one week, largely due to their reasonable prediction of the variability of the western North Pacific subtropical high in mid-latitudes. Although the chance of exceeding the new record daily rainfall is only approx. 0.7% in mid-late July, they provide a high probability of this heavy weekly rainfall one week in advance. However, the S2S models still underestimated the super extremeness of this event. The prediction discrepancies came from the poor predictability of Typhoon IN-FA and its impact on the daily evolution of the extreme rainfall event, even within a few days forecast lead. Compared with the observation, the prediction bias of tropical disturbance changed the environmental monsoon airflow to induce the earlier warning of rainfall extremes prior to the formation of IN-FA. After the formation of IN-FA, the prediction bias of the typhoon’s moving speed distorted the typhoon location, which incorrectly predicted the moisture convergence center and underestimated their remote impacts on this heavy rainfall event. Future research should improve our awareness of the challenges that remain in the S2S forecasts.

How to cite: Yan, Y., Zhu, C., and Liu, B.: Subseasonal prediction of the July 2021 extreme rainfall event over Henan China in S2S forecasting systems, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15077, https://doi.org/10.5194/egusphere-egu23-15077, 2023.

EGU23-15594 | ECS | Posters virtual | AS1.3

Hunting for “Windows of Opportunity” in Forecasts Across Timescales? Cross it 

Ángel G. Muñoz, Francisco Doblas-Reyes, Laurel DiSera, Markus Donat, Nube González-Reviriego, Albert Soret, Marta Terrado, and Verónica Torralba

Stakeholders in all socio-economic sectors require reliable forecasts at multiple timescales as part of their decision-making processes. Although basing decisions mostly on a particular timescale (e.g., weather, subseasonal, seasonal) is the present status quo, this approach tends to lead to missing opportunities for more comprehensive risk-management systems (Goddard et al. 2014).

 

While today a variety of forecasts are produced targeting distinct timescales in a routine way, these products are generally presented to the users in different websites and bulletins, often without an assessment of how consistent the predictions are across timescales. Since different models and strategies are used at different timescales by both national and international seasonal and subseasonal forecasting centers (Kirtman et al. 2014, Kirtman et al. 2017, Vitart et al. 2017), and skill is different at those timescales, it is key to guarantee that a physically consistent “bridging” between the forecasts exists, and that the cross-timescale predictions are overall skilful and actionable, so decision makers can conduct their work.

 

Here, we propose and explore a new methodology –that we call the Xit (“cross-it”) operator– based on the Liang-Kleeman information flow (e.g., Tawia Hagan et al. 2019) and wavelet spectra and entropy (e.g., Zunino et al. 2007), to “bridge” forecasts at different timescales in a smooth and physically-consistent manner.

 

In summary, the Xit operator (1) conducts a wavelet spectral analysis (e.g., Ng and Chan 2013, Zunino et al. 2007) and (2) a non-stationary time-frequency causality analysis (e.g., Tawia Hagan et al. 2019, Liang 2015) on forecasts at different timescales to assess cross-timescale coherence and physical consistency in terms of various sources of predictability. In principle, the approach permits to identify which “intrinsic” periods/scales (i) in the timescale continuum (t) are more suitable for the bridging to occur, and/or which ones can produce more skillful forecasts, by pointing to particular target times—i.e., potential windows of opportunity (Mariotti et al. 2020)—in the forecast period where wavelet entropy (uncertainty) is lower.

 

While the first component of the Xit operator, i.e., the wavelet spectral and entropy analysis (Zunino et al. 2007), is designed to identify the optimal time-frequency bands for cross-timescale bridging, the fact that two forecast systems (e.g., a subseasonal and a seasonal) exhibit significant wavelet coherence does not imply that bridging those systems will provide physically-consistent predictions. The second component of the Xit operator, i.e., the non-stationary causality analysis (Tawia Hagan et al. 2019), is thus designed to assess physical consistency of the bridging by analyzing the causal link between different climate drivers (acting at different timescales) and the forecast variable of interest.

How to cite: Muñoz, Á. G., Doblas-Reyes, F., DiSera, L., Donat, M., González-Reviriego, N., Soret, A., Terrado, M., and Torralba, V.: Hunting for “Windows of Opportunity” in Forecasts Across Timescales? Cross it, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15594, https://doi.org/10.5194/egusphere-egu23-15594, 2023.

EGU23-16178 | ECS | Posters virtual | AS1.3

Subseasonal forecasting of temperature and precipitation over India using a machine learning approach 

Prajwal Jadhav, Sreejith Op, and Sabeerali Thelliyil

Subseasonal forecasting is forecasting of the weather parameters, mainly temperature and precipitation, two weeks to two months in advance. Sub-seasonal variability accounts for a substantial portion of the summer rainfall over India. Prediction of sub-seasonal climate is of immense societal importance in agriculture planning, water management, emergency planning, etc. Using various weather parameters and ECMWF dynamical model forecasts as predictors, this study tries to investigate the weekly forecast of temperature and precipitation at 2-week, 3-week, and 4-week forecast horizon over India using a computationally inexpensive machine learning model-MultiLLR, which prunes out irrelevant predictors and integrates remaining predictors linearly for each target date. The model’s predictions calculated over the years 2019-2022 are as skilful as IMD’s Extended Range Forecasting System (ERFS). The skill of the model is better in the coastal region than in the inland part of India.

How to cite: Jadhav, P., Op, S., and Thelliyil, S.: Subseasonal forecasting of temperature and precipitation over India using a machine learning approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16178, https://doi.org/10.5194/egusphere-egu23-16178, 2023.

EGU23-16412 | ECS | Posters on site | AS1.3

The 2020-2023 La Niña: Did Cross-timescale Interference Fuel this Multi-year Event? 

Laurel DiSera and Ángel G. Muñoz

Beginning July 2020, the Niño 3.4 index crossed below the threshold to La Niña conditions and remained below a -0.4 sea surface temperature anomaly through the spring of 2023, impacting agriculture, livelihoods, and communities around the world. What caused this prolonged La Niña event and why was it sustained? How did the interaction between the different modes of climate variability influence the event? The internal dynamics of ENSO, the Indian Ocean Dipole, and the Madden-Julian Oscillation are studied here through a non-linear approach utilizing compositing techniques and both linear and non-linear wave superposition to identify what caused and prolonged the 2020-2023 La Niña event.

How to cite: DiSera, L. and Muñoz, Á. G.: The 2020-2023 La Niña: Did Cross-timescale Interference Fuel this Multi-year Event?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16412, https://doi.org/10.5194/egusphere-egu23-16412, 2023.

EGU23-16731 | ECS | Posters on site | AS1.3

Projected Future Changes in Equatorial Wave Spectrum in CMIP6 

Hagar Bartana, Chaim Garfinkel, Ofer Shamir, and Jian Rao

Changes of tropical wave-modes due to climate change will impact the predictability of the tropical atmosphere, and may impact extratropical weather as well. The simulations of convectively coupled equatorial waves and the Madden-Julian Oscillation (MJO) are considered in 13 state-of-the-art models from phase 6 of the Coupled Model Intercomparison Project (CMIP6).  We look at the wave-modes using frequency-wavenumber power spectra of the models and observations for Outgoing Longwave Radiation and zonal winds at 250 hPa. We analyze the spectra of the historical simulations and end of 21st century projections for the SSP245 and SSP585 scenarios.  The models simulate a spectrum quantitatively resembling that observed, though systematic biases exist. Most models project a future increase in power spectra for the MJO, while nearly all project a robust increase for Kelvin waves (KW) and weaker power values for most other wavenumber-frequency combinations. Models with a more realistic MJO in their control climate tend to simulate a stronger future intensification. In addition to strengthening, KW also shift toward higher phase speeds. The net effect is a more organized tropical circulation on intraseasonal timescales, which may contribute to higher intrinsic predictability in the tropics and to stronger teleconnections in the extratropics. In addition, those projected changes might be due to extratropical forcings, and more specifically due to changes in the North Pacific subtropical jet.

How to cite: Bartana, H., Garfinkel, C., Shamir, O., and Rao, J.: Projected Future Changes in Equatorial Wave Spectrum in CMIP6, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16731, https://doi.org/10.5194/egusphere-egu23-16731, 2023.

EGU23-604 | ECS | Posters on site | CL4.3

Boreal Spring Southern Hemisphere Climate Mode and Global Monsoon 

Shikhar Srivastava, Arindam Chakraborty, and Raghu Murtugudde

The global climatic pattern is governed by the dominant mode of variability in the tropics and the extratropic and their interaction. The extratropical atmosphere is much more vigorous than the tropics owing to sharp meridional temperature gradients in the mid-latitude. Especially on the decadal timescales, large signals are seen over the extratropical region than in the tropics. Here, we propose that during boreal spring, the second leading mode of climate variability in the Southern Hemisphere, has a decadal pattern. This mode is independent of the Southern Annular Mode (SAM), which represents the most dominant mode of climate variability in the Southern Hemisphere. The boreal spring climate of the Southern Hemisphere interacts with the tropics and significantly impacts the global climate, which is reflected in the global Monsoon rainfall. During the positive phase of the decadal mode, the global Monsoon rainfall is coherently suppressed. We propose a new finding highlighting that the Southern Hemisphere's extratropical forcing can significantly impact the tropical Pacific through subtropical pathways on the decadal to multidecadal timescale. The impact of such decadal climate variability is enormous and global and can add a new paradigm to the pursuit of improving decadal predictions of the global climate.

How to cite: Srivastava, S., Chakraborty, A., and Murtugudde, R.: Boreal Spring Southern Hemisphere Climate Mode and Global Monsoon, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-604, https://doi.org/10.5194/egusphere-egu23-604, 2023.

As a dominant pattern of the North Pacific sea surface temperature decadal variability, the Pacific Decadal Oscillation (PDO) has remarkable influences on the marine and terrestrial ecosystems. However, the PDO is highly unpredictable. Here, we assess the performance of the Coupled Model Intercomparison Project Phase 6 (CMIP6) models in simulating the PDO, with an emphasis on the evaluation of CMIP6 models in reproducing a recently detected early warning signal based on climate network analysis for the PDO regime shift. Results show that the skill of CMIP6 historical simulations remains at a low level, with a skill limited in reproducing PDO’s spatial pattern and nearly no skill in reproducing the PDO index. However, if the warning signal for the PDO regime shift by climate network analysis is considered as a test-bed, we find that even in historical simulations, a few models can represent the corresponding relationship between the warning signal and the PDO regime shift, regardless of the chronological accuracy. By further conducting initialization, the performance of the model simulations is improved according to the evaluation of the hindcasts from two ensemble members of the Decadal Climate Prediction Project (NorCPM1 and BCC-CSM2-MR). Particularly, we find that the NorCPM1 model can capture the early warning signals for the late-1970s and late-1990s regime shifts 5–7 years in advance, indicating that the early warning sig- nal somewhat can be captured by some CMIP6 models. A further investigation on the underlying mechanisms of the early warning signal would be crucial for the improvement of model simulations in the North Pacific.

How to cite: Ma, Y.: On the Pacific Decadal Oscillation Simulations in CMIP6 Models: A New Test‐Bed from Climate Network Analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5325, https://doi.org/10.5194/egusphere-egu23-5325, 2023.

Climate extremes can impact societies in various ways: from nuances in daily lives to full humanitarian crises. Droughts  are usually slow onset extremes but can be highly disruptive and affect millions of people every year. Warm temperature extremes (e.g. heat waves) can exacerbate droughts and their impacts and trigger a faster drought evolution. Combined drought and heat waves can lead to devastating consequences. For example, 2022 was a very active year in terms of drought or combined drought and heat waves, affecting particularly hard several regions of the world (e.g. Europe, China, southern South America and East Africa). In a context of risk management and civil protection, the use of operationally available seasonal climate forecasts can provide actionable information to reduce the risks and the impacts of these events on societies with different levels of development and adaptive capacities. 

 

Within the Copernicus Emergency Management Service (CEMS), the European and Global Drought Observatories (EDO and GDO, respectively) provide real time drought and temperature extreme monitoring products freely available and displayed through two dedicated web services. Recent efforts have been targeting the optimal integration and use of multi-system forecasting products to enhance the early warning component of the service. This contribution provides an overview of first results in terms of  initial multi-model skill assessment of forecasts available through the Copernicus Climate Change Service (C3S). It also discusses future avenues to improve skill in regions with limited predictability, for example by applying physically-based sampling techniques.    

How to cite: Acosta Navarro, J. C. and Toreti, A.: Seasonal forecasting of drought and temperature extremes as part of the Copernicus Emergency Management Service (CEMS), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5602, https://doi.org/10.5194/egusphere-egu23-5602, 2023.

EGU23-6000 | ECS | Orals | CL4.3

Seasonal forecasting of the European North West Shelf: Quantifying the persistence of the physical marine environment 

Jamie Atkins, Jonathan Tinker, Jennifer Graham, Adam Scaife, and Paul Halloran

The European North West shelf seas (NWS) support economic and environmental interests of several adjacent populous countries. Forecasts of physical marine variables on the NWS for upcoming months – an important decision-making timescale – would be useful for many industries. However, currently there is no operational seasonal forecasting product deemed sufficient for capturing the high variability associated with shallow, dynamic shelf waters. Here, we identify the dominant sources of seasonal predictability on the shelf and quantify the extent to which empirical persistence relationships can produce skilful seasonal forecasts of the NWS at the lowest level complexity. We find that relatively skilful forecasts of the typically well-mixed Winter and Spring seasons are achievable via persistence methods at a one-month lead time. In addition, incorporating observed climate modes of variability, such as the North Atlantic Oscillation (NAO), can significantly boost persistence for some locations and seasons, but this is dependent on the strength of the climate mode index. However, even where high persistence skill is demonstrated, there are sizeable regions exhibiting poor predictability and skilful persistence forecasts are typically limited to ≈ one-month lead times. Summer and Autumn forecasts are generally less skilful owing largely to the effects of seasonal stratification which emphasises the influence of atmospheric variability on sea surface conditions. As such, we also begin incorporating knowledge of future atmospheric conditions to forecasting strategies. We assess the ability of an existing global coupled ocean-atmosphere seasonal forecasting system to exceed persistence skill and highlight areas where additional downscaling efforts may be needed.

How to cite: Atkins, J., Tinker, J., Graham, J., Scaife, A., and Halloran, P.: Seasonal forecasting of the European North West Shelf: Quantifying the persistence of the physical marine environment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6000, https://doi.org/10.5194/egusphere-egu23-6000, 2023.

EGU23-7676 | Orals | CL4.3

Decadal Climate Variability and Predictability with a High-resolution Eddy-resolving Model 

Wei Zhang, Ben Kirtman, Leo Siqueira, and Amy Clement

Current global climate models typically fail to fully resolve mesoscale ocean features (with length scales on the order of 10 km), such as the western boundary currents, potentially limiting climate predictability over decadal timescales. This study incorporates high-resolution eddy-resolving ocean (HR: 0.1°) in a suite of CESM model experiments that capture these important mesoscale ocean features with increased fidelity. Compared with eddy-parametrized ocean (LR: 1°) experiments, HR experiments show more realistic climatology and variability of sea surface temperature (SST) over the western boundary currents and eddy-rich regions. In the North Atlantic, the inclusion of mesoscale ocean processes produces a more realistic Gulf Stream and improves both localized rainfall patterns and large-scale teleconnections. We identify enhanced decadal SST predictability in HR over the western North Atlantic, which can be explained by the strong vertical connectivity between SST and sub-surface ocean temperature. SST is better connected with slower processes deep down in HR, making SST more persistent (and predictable). Moreover, we detect a better representation of the air-sea interactions between SST and low-level atmosphere over the Gulf Stream, thus improving low-frequency rainfall variations and extremes over the Southeast US. The results further imply that high-resolution GCMs with increased ocean model resolution may be needed in future climate prediction systems.

How to cite: Zhang, W., Kirtman, B., Siqueira, L., and Clement, A.: Decadal Climate Variability and Predictability with a High-resolution Eddy-resolving Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7676, https://doi.org/10.5194/egusphere-egu23-7676, 2023.

Earth system predictability on decadal timescales can arise from both low frequency internal variability as well as from anthropogenically forced long-term changes. However, on these timescales, the chaotic nature of the climate system makes skillful predictions difficult to achieve even if we include information from climate change projections. Furthermore, it is difficult to separate the contributions from internal variability and external forcing to predictability. One way to improve skill is through identifying and harnessing initial conditions with more predictable evolution, so-called state-dependent predictability. We explore a neural network approach to identify these opportunistic initial states in the CESM2 large ensemble and subsequently explore how predictability may manifest in a future climate, influenced by both forced warming and internal variability. We use an interpretable neural network to demonstrate that internal variability will continue to play an important role in future climate predictions, especially for states of increased predictability.

How to cite: Gordon, E. and Barnes, E.: An interpretable neural network approach to identifying sources of predictability in the future climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8000, https://doi.org/10.5194/egusphere-egu23-8000, 2023.

EGU23-8296 | ECS | Orals | CL4.3 | Highlight

Better late than never: arrival of decadal predictions to the climate services arena 

Balakrishnan Solaraju-Murali, Dragana Bojovic, Nube Gonzalez-Reviriego, Andria Nicodemou, Marta Terrado, Louis-Philippe Caron, and Francisco J. Doblas-Reyes

Decadal prediction represents a source of near-term climate information that has the potential to support climate-related decisions in key socio-economic sectors that are influenced by climate variability and change. While the research to illustrate the ability of decadal predictions in forecasting the varying climate conditions on a multi-annual timescale is rapidly evolving, the development of climate services based on such forecasts is still in its early stages. This study showcases the potential value of decadal predictions in the development of climate services. We summarize the lessons learnt from coproducing a forecast product that provides tailored and user-friendly information about multi-year drought conditions for the coming five years over global wheat harvesting regions. The interaction between the user and climate service provider that was established at an early stage and lasted throughout the forecast product development process proved fundamental to provide useful and ultimately actionable information to the stakeholders concerned with food production and security. This study also provides insights on the potential reasons behind the delayed entry of decadal predictions in the climate services discourse and practice, which were obtained from surveying climate scientists and discussing with decadal prediction experts.

How to cite: Solaraju-Murali, B., Bojovic, D., Gonzalez-Reviriego, N., Nicodemou, A., Terrado, M., Caron, L.-P., and Doblas-Reyes, F. J.: Better late than never: arrival of decadal predictions to the climate services arena, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8296, https://doi.org/10.5194/egusphere-egu23-8296, 2023.

EGU23-8750 | Orals | CL4.3

A simple coupled assimilation approach for improved initialization of decadal climate predictions 

Tim Kruschke, Mehdi Pasha Karami, David Docquier, Frederik Schenk, Ramon Fuentes Franco, Ulrika Willén, Shiyu Wang, Klaus Wyser, Uwe Fladrich, and Torben Koenigk

We introduce a simple data assimilation approach applied to the coupled global climate model EC-Earth3.3.1, aiming at producing initial conditions for decadal climate hindcasts and forecasts. We rely on a small selection of assimilated variables, which are available in a consistent manner for a long period, providing good spatial coverage for large parts of the globe, that is sea-surface temperatures (SST) and near-surface winds.

Given that these variables play a role directly at or very close to the ocean-atmosphere interface, we assume a comparably strong cross-component impact of the data assimilation. Starting from five different free-running CMIP6-historical simulations in 1900, we first apply surface restoring in the model’s ocean component towards monthly means of HadISST1. After integrating this five-member ensemble with only assimilating SST for the period 1900-1949, we start additionally assimilating (nudging) 6-hourly near-surface winds (vorticity and divergence) taken from the ERA5 reanalysis from 1950 onwards. To mitigate the risk of model drifts after initializing the decadal predictions and to account for known instationary biases of the model, we assimilate anomalies of all variables that are calculated based on a 30-year running mean.

By assimilating near-surface data over several decades before entering the actual period targeted by the decadal hindcasts/forecasts for CMIP6-DCPP, we expect the coupled model to be able to ingest a significant share of observed climate evolution also in deeper ocean layers. This would then potentially serve as a source of predictive skill on interannual-to-decadal timescales.

We show that the presented assimilation approach is able to force the coupled model’s evolution well in phase with observed climate variability, positively affecting not only near-surface levels of the atmosphere and ocean but also deeper layers of the ocean and higher levels of the atmosphere as well as Arctic sea-ice variability. However, we also present certain problematic features of our approach. Two examples are significantly strengthened low-frequency variability of the AMOC and a wind bias resulting into generally reduced evaporation over ocean areas.

How to cite: Kruschke, T., Karami, M. P., Docquier, D., Schenk, F., Fuentes Franco, R., Willén, U., Wang, S., Wyser, K., Fladrich, U., and Koenigk, T.: A simple coupled assimilation approach for improved initialization of decadal climate predictions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8750, https://doi.org/10.5194/egusphere-egu23-8750, 2023.

The interdisciplinary research project "BayTreeNet" examines the reactions of forest ecosystems to climate dynamics. To establish a relationship between tree growth and climate, it is important to know that in the mid-latitudes, local climate phenomena often show a strong dependence on the large-scale climate weather types (WT), which significantly determine the climate of a region through frequency and intensity. Different WT show various weather conditions at different locations, especially in the topographically diverse region of Bavaria. The meaning of every WT is the physical basis for the climate-growth relationships established in the dendroecology sub-project to investigate the response of forests to individual WT at different forest sites. Complementary steps allow interpretation of results for the past (20th century) and projection into the future (21st century). One hypothesis is that forest sites in Bavaria are affected by a significant influence of climate change in the 21st century and the associated change in WT.

The automated classification of large-scale weather patterns is presented by Self-Organizing-Maps (SOM) developed by Kohonen, which enables visualization and reduction of high-dimensional data. The poster presents the SOM-setting which was used to classify the WT and the results of past environmental conditions (1990-2019) for different WT in Europe based on ERA5 data. Morover, it shows a future projection until 2100 for European WT and their respective environmental conditions. The projections are based on a novel GCM selection technique for two scenarios (ssp1-2.6 and ssp5-8.5) to obtain a range of the most likely conditions.

How to cite: Wehrmann, S. and Mölg, T.: GCM-based future projections of European weather types obtained by Self‑Organizing-Maps and a novel GCM selection technique, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8934, https://doi.org/10.5194/egusphere-egu23-8934, 2023.

EGU23-9520 | Orals | CL4.3

Estimating the significance of the added skill from initializations: The case of decadal predictions 

Bo Christiansen, Shuting Yang, and Dominic Matte

A considerable part of the skill in decadal forecasts often come from the forcings which are present in both initialized and un-initialized model experiments. This makes the added value from initialization difficult to assess. We investigate statistical tests to quantify if initialized forecasts provide skill over the un-initialized experiments. We consider three correlation based statistics previous used in the literature. The distributions of these statistics under the null-hypothesis that initialization has no added values are calculated by a surrogate data method. We present some simple examples and study the statistical power of the tests. We find that there can be large differences in both the values and the power for the different statistics. In general the simple statistic defined as the difference between the skill of the initialized and uninitialized experiments behaves best. However, for all statistics the risk of rejecting the true null-hypothesis is too high compared to the nominal value.

We compare the three tests on initialized decadal predictions (hindcasts) of near-surface temperature performed with a climate model and find evidence for a significant effect of initializations for small lead-times. In contrast, we find only little evidence for a significant effect of initializations for lead-times larger than 3 years when the experience from the simple experiments is included in the estimation.

How to cite: Christiansen, B., Yang, S., and Matte, D.: Estimating the significance of the added skill from initializations: The case of decadal predictions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9520, https://doi.org/10.5194/egusphere-egu23-9520, 2023.

EGU23-9986 | Posters on site | CL4.3

Probabilistic nonlinear lagged teleconnections of the sea surface temperature field 

Carlos Pires and Abdel Hannachi

The monthly anomaly sea surface temperature field over the global ocean exhibit probabilistic dependencies between remote points and lagged times, which are explained eventually by some oceanic or atmospheric bridge of information transfer. Despite much of the bivariate SST dependencies appear to be linear, others are characterized by robust and statistically significant nonlinear correlations. In order to enhance that, we present a general method of extracting bivariate (X,Y) dependencies, seeking for pairs of polynomials P(X) and Q(Y) which are maximally correlated. The method relies on a Canonical correlation Analysis (CCA) between sets of standardized monomials of X and Y, up to a certain (low) degree (e.g. 4). Polynomial coefficients are obtained from the leading CCA eigenvector. Polynomials are calibrated and validated over independent periods, being afterwards subjected to marginal Gaussian anamorphoses. The bivariate non-Gaussianity in the space of marginally Gaussianized polynomials remains residual because of the correlation concentration and maximization. Consequently, the bivariate Gaussian pdf or in alternative, a copula pdf in the space of maximally correlated polynomials can accurately approximate the bivariate dependency. That probabilistic model is then used to determine conditional pdfs, cdfs and probabilities of extremes.

The method is applied to various (X,Y) pairs. In the first example, X is an optimized polynomial of the El-Niño 3.4 index while Y is that index lagged to the future. For lags between 6 and 18 months, the nonlinear El-Niño forecast clearly surpasses the linear one, contributing to lower the El-Niño seasonal predictability barrier. In the second example, we relate El-Niño (X) with the lagged Atlantic multidecadal oscillation index (Y). Nonlinear, robust correlations appear, both for positive and negative lags up to 5 years putting in evidence Pacific-Atlantic basin oceanic teleconnections.

The above probabilistic (polynomial based) model appears to be a good candidate tool for the statistical (seasonal up to decadal) forecast of regime probabilities (e.g. dry/wet) and extremes, given certain antecedent precursors.

This work was funded by the Portuguese Fundação para a Ciência e a Tecnologia (FCT) I.P./MCTES through national funds (PIDDAC) – UIDB/50019/2020- IDL and the project JPIOCEANS/0001/2019 (ROADMAP: ’The Role of ocean dynamics and Ocean–Atmosphere interactions in Driving cliMAte variations and future Projections of impact–relevant extreme events’). Acknowledgements are also due to the International Meteorological Institute (IMI) at Stockholm University.

How to cite: Pires, C. and Hannachi, A.: Probabilistic nonlinear lagged teleconnections of the sea surface temperature field, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9986, https://doi.org/10.5194/egusphere-egu23-9986, 2023.

EGU23-13375 | ECS | Orals | CL4.3

Role of the subpolar North Atlantic region in skillful climate predictions for high northern latitudes: A pacemaker experiment 

Annika Drews, Torben Schmith, Shuting Yang, Steffen Olsen, Tian Tian, Marion Devilliers, Yiguo Wang, and Noel Keenlyside
Recent studies have suggested that the Atlantic water pathway connecting the subpolar North Atlantic (SPNA) with the Nordic Seas and Arctic Ocean may lead to skillful predictions of sea surface temperature and salinity anomalies in the eastern Nordic Seas. To investigate the role of the SPNA for such anomalies downstream, we designed a pacemaker experiment, using two decadal climate prediction systems based on EC-Earth3 and NorCPM. We focus on the subpolar extreme cold anomaly in 2015 and its subsequent development, a feature not well captured and predicted. The pacemaker experiment follows the protocol of the CMIP6 DCPP-A retrospective forecasts or hindcasts initialized November 1, 2014, but the models are forced to follow the observed ocean temperature and salinity anomalies in the SPNA from ocean reanalysis from November 2014 through to December 2019. Two sets of 10-year hindcasts are performed with 10 members for EC-Earth3 and 30 members for NorCPM. We here detail and discuss the design of this pacemaker experiment and present results, comparing with the initialized CMIP6 DCPP-A experiment assessing differences in decadal prediction skill outside the SPNA. We conclude that the pacemaker experiments show improved skill compared to the standard decadal predictions for the eastern Norwegian Sea, and therefore the SPNA is key for successful decadal predictions in the region.

How to cite: Drews, A., Schmith, T., Yang, S., Olsen, S., Tian, T., Devilliers, M., Wang, Y., and Keenlyside, N.: Role of the subpolar North Atlantic region in skillful climate predictions for high northern latitudes: A pacemaker experiment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13375, https://doi.org/10.5194/egusphere-egu23-13375, 2023.

EGU23-13639 | Orals | CL4.3

Seasonal prediction of UK mean and extreme winds 

Julia Lockwood, Nicky Stringer, Katie Hodge, Philip Bett, Jeff Knight, Doug Smith, Adam Scaife, Matthew Patterson, Nick Dunstone, and Hazel Thornton

For several years the Met Office has produced a seasonal outlook for the UK every month, which is issued to the UK Government and contingency planners.  The outlook gives predictions of the probability of having average, low, or high seasonal mean UK temperature and precipitation for the coming three-months.  In recent years, there has been increasing demand from sectors such as energy and insurance to include similar probabilistic predictions of UK wind speed: both for the seasonal mean and for measures of extreme winds such as storm numbers.  In this presentation we show the skill of the Met Office’s GloSea system in predicting seasonal (three-month average) UK mean wind and a measure of UK storminess throughout the year, and discuss the drivers of predictability.  Skill in predicting the UK mean wind speed and storminess peaks in winter (December–February), owing to predictability of the North Atlantic oscillation.  In summer (June–August), there is evidence that a significant proportion of variability in UK winds is driven by a Rossby wave train which the model has little skill in predicting. Nevertheless there are signs that the wave is potentially predictable and skill may be improved by reducing model errors.

How to cite: Lockwood, J., Stringer, N., Hodge, K., Bett, P., Knight, J., Smith, D., Scaife, A., Patterson, M., Dunstone, N., and Thornton, H.: Seasonal prediction of UK mean and extreme winds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13639, https://doi.org/10.5194/egusphere-egu23-13639, 2023.

EGU23-13736 | ECS | Posters on site | CL4.3

Decadal predictability of European temperature extremes. 

Eirini Tsartsali, Panos Athanasiadis, Stefano Tibaldi, and Silvio Gualdi

Accurate predictions of climate variations at the decadal timescale are of great interest for decision-making, planning and adaptation strategies for different socio-economic sectors. Notably, decadal predictions have rapidly evolved during the last 15 years and are now produced operationally worldwide. The majority of the studies assessing the skill of decadal prediction systems focus on time-mean anomalies of standard meteorological variables, such as annual mean near-surface air temperature and precipitation. However, the predictability of extreme events frequency may differ substantially from the predictability of multi-year annual or seasonal means. Predicting the frequency of extreme events at different timescales is of major importance, since they are associated with severe impacts on various natural and human systems. In the current study we evaluate the capability of state-of-the-art decadal prediction systems to predict the frequency of temperature extremes in Europe. More specifically, we assess the skill of a multi-model ensemble from the Decadal Climate Prediction Project (DCPP, 163 ensemble members from 12 models in total) to forecast the number of days belonging to heatwaves episodes during summer (June–August). We find statistically significant predictive skill over Europe, except for the United Kingdom and a large part of the Scandinavian Peninsula, most of which is associated with the long-term warming trend. We are progressing with the evaluation of other statistical aspects of extreme events, including warm and cold episodes during winter, and we are also investigating whether there is predictive skill beyond that stemming from the external forcing.  

How to cite: Tsartsali, E., Athanasiadis, P., Tibaldi, S., and Gualdi, S.: Decadal predictability of European temperature extremes., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13736, https://doi.org/10.5194/egusphere-egu23-13736, 2023.

EGU23-13789 | Posters on site | CL4.3

Do oceanic observations (still) matter in initializing decadal climate predictions over the North Atlantic ocean? 

Sebastian Brune, Vimal Koul, and Johanna Baehr

Earth system models are now regularly being used in inter-annual to decadal climate prediction. Such prediction systems based on CMIP5-generation Earth system models had demonstrated an overall positive impact of initialization, i.e. deriving initial conditions of retrospective forecasts from a separate data assimilation experiment, on decadal prediction skill. This view is now being increasingly challenged in the context of improvements both in CMIP6-generation Earth system models and CMIP6-evaluation of external forcing as well as in the context of ongoing transient climate change. In this study we re-evaluate the impact of atmospheric and oceanic initialization on decadal prediction skill of North Atlantic upper ocean heat content (0-700m) in a CMIP6-generation decadal prediction system based on the Max Planck Institute Earth system model (MPI-ESM). We compare the impact of initial conditions derived through full-field atmospheric nudging with those derived through an additional assimilation of observed oceanic temperature and salinity profiles using an ensemble Kalman filter. Our experiments suggest that assimilation of observed oceanic temperature and salinity profiles into the model reduces the warm bias in the subpolar North Atlantic heat content, and improves the modelled variability of the Atlantic meridional overturning circulation and ocean heat transport. These improvements enable a proper initialization of model variables which leads to an improved decadal prediction of surface temperatures. Our results reveal an important role of subsurface oceanic observations in decadal prediction of surface temperatures in the subpolar North Atlantic even in CMIP6-generation decadal prediction system.

How to cite: Brune, S., Koul, V., and Baehr, J.: Do oceanic observations (still) matter in initializing decadal climate predictions over the North Atlantic ocean?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13789, https://doi.org/10.5194/egusphere-egu23-13789, 2023.

EGU23-14755 | ECS | Posters on site | CL4.3

A low-dimensional dynamical systems approach to climate ensemble design and interpretation 

Francisco de Melo Viríssimo and David Stainforth

Earth System Models (ESMs) are complex, highly nonlinear, multi-component systems described by large number of differential equations. They are used to study the evolution of climate and its dynamics, and to make projection of future climate at both regional and global levels – which underpins climate change impact assessments such as the IPCC report. These projections are subject to several sorts of uncertainty due to high internal variability in the system dynamics, which are usually quantified via ensembles of simulations.

Due to their multi component nature of such ESMs, the emerging dynamics also contain different temporal scales, meaning that climate ensembles come in a variety of shapes and sizes. However, our ability to run such ensembles is usually constrained by the computational resources available, as they are very expensive to run. Hence, choices on the ensemble design must be made, which conciliate the computational capability with the sort of information one is looking for.

One alternative to gain information is to use low-dimensional climate-like systems, which consists of simplified, coupled versions of atmosphere, ocean, and other components, and hence capture some of the different time scales present in ESMs. This approach allows one to run very large ensembles, and hence to explore all sorts of model uncertainty with only modest computational usage.

In this talk, we discuss this approach in detail, and illustrate its applicability with a few results. Particular attention will be given to the issues of micro and macro initial condition uncertainty, and parametric uncertainty – including external, anthropogenic-like forcing. The ability of large ensembles to constrain decadal to centennial projections will be also explored.

How to cite: de Melo Viríssimo, F. and Stainforth, D.: A low-dimensional dynamical systems approach to climate ensemble design and interpretation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14755, https://doi.org/10.5194/egusphere-egu23-14755, 2023.

EGU23-15829 | ECS | Posters on site | CL4.3

Near term climate change in Emilia-Romagna (Italy) using CMIP6 decadal climate predictions 

Valeria Todaro, Marco D'Oria, Daniele Secci, Andrea Zanini, and Maria Giovanna Tanda

Ongoing climate change makes both short- and long-term adaptation and mitigation strategies urgently needed. While many long-term climate models have been developed and investigated in recent years, little attention has been paid to short-term simulations. The first attempts to perform multi-model initialized decadal forecasts were presented in the fifth Coupled Model Intercomparison Project 5 (CMIP5). Near-term climate prediction models are new socially relevant tools to support the decision makers delivering climate adaptation solutions on an annual or decadal scale. Recent improvements in decadal models were coordinated in CMIP6 and the World Climate Research Program (WCRP) Grand Challenge on Near Term Climate Prediction, as part of the Sixth Assessment Report of the Intergovernmental Panel on Climate Change (AR6, IPCC). The Decadal Climate Prediction Project (DCPP) provides decadal climate forecasts based on advanced techniques for the reanalysis of climate data, initialization methods, ensemble generation and data analysis. The initialization allows to consider the predictability of the internal climate variability reducing the prediction errors compared to those of the long-term projections, whose simulations do not take into account the phasing between the internal variability of the model and the observations. The aim of this work is to assess the near-future climate change in the Emilia-Romagna region in northern Italy until 2031. The hydrological variables analyzed are the daily precipitation and maximum and minimum temperature. An ensemble of models, with the highest resolution available, is used to handle the uncertainty in the predictions. Initially, to assess the reliability of the selected climate models, the hindcast data of the DCPP are checked against observations. Then, the DCPP predictions are used to investigate the variability of precipitation and temperature in the near future over the investigated area. Some climate features that are referenced to have an important impact on human health and activities are evaluated, such as drought indices and heat waves.

How to cite: Todaro, V., D'Oria, M., Secci, D., Zanini, A., and Tanda, M. G.: Near term climate change in Emilia-Romagna (Italy) using CMIP6 decadal climate predictions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15829, https://doi.org/10.5194/egusphere-egu23-15829, 2023.

EGU23-16034 | ECS | Posters on site | CL4.3

Seasonal forecast of the Sudden Stratospheric Warming occurrence 

Mikhail Vokhmyanin, Timo Asikainen, Antti Salminen, and Kalevi Mursula

The polar vortex in the wintertime Northern Hemisphere can sometimes experience a dramatic breakdown after an associated warming of the stratosphere during so-called Sudden Stratospheric Warmings (SSWs). These events are known to influence the ground weather in Northern Eurasia and large parts of North America. SSWs are primarily generated by enhanced planetary waves propagating from the troposphere to the stratosphere where they decelerate the vortex and lead to its breakdown. According to the Holton-Tan mechanism, the easterly direction of equatorial stratospheric QBO (Quasi-Biennial Oscillation) winds weakens the northern polar vortex by guiding more waves poleward. Recently, we found that during easterly QBO the occurrence rate of SSWs is modulated by the geomagnetic activity. We used the aa-index which is a good proxy for the energetic electron precipitations (EEP) responsible for the indirect effect on ozone. Our model shows that the breaking of the polar vortex is very likely to occur if the geomagnetic activity is weak. On the other hand, during westerly QBO, solar irradiance modulates the SSW occurrence: more SSWs happen under high solar activity.

How to cite: Vokhmyanin, M., Asikainen, T., Salminen, A., and Mursula, K.: Seasonal forecast of the Sudden Stratospheric Warming occurrence, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16034, https://doi.org/10.5194/egusphere-egu23-16034, 2023.

The state-of-the-art climate models suffer from significant sea surface temperature (SST) biases in the tropical Indian Ocean (TIO), greatly damaging the climate prediction and projection. In this study, we investigate the multidecadal atmospheric bias teleconnections caused by the TIO SST biases and their impacts on the simulated atmospheric variability. A set of century long simulations forced with idealized SST perturbations, resembling various persistent TIO SST biases in coupled climate models, are conducted with an intermediate complexity climate model. Bias analysis is performed using the normal-mode function decomposition which can differentiate between balanced and unbalanced flow regimes across spatial scales. The results show that the long-term atmospheric circulation biases caused by the TIO SST biases have the Matsuno-Gill-type pattern in the tropics and Rossby wavetrain distribution in the extratropics, similar to the steady state response to tropical heating. The teleconnection between the tropical and extratropical biases is set up by the Rossby wavetrain emanating from the subtropics. Over 90% of the total bias energy is stored in the zonal modes k≤6, and the Kelvin modes take 50-65% of the total unbalanced bias energy. The spatial and temporal variabilities have different responses to positive SST biases. In the unbalanced regime, variability changes are confined in the tropics, but the spatial variability increases whereas the temporal variability decreases. In the balanced regime, the spatial variability generally increases in the tropics and decreases in the extratropics, whereas the temporal variability decreases globally. Variability responses in the tropics are confined in the Indo-west Pacific region, and those in the extratropics are strong in the Pacific-North America region and the Europe. In the experiment with only negative SST biases, spatial and temporal variabilities increase in both regimes. In addition, the comparison between experiments indicates that the responses of the circulation and its variability are not sensitive to the structure and location of the TIO SST biases.

How to cite: Zhao, Y.-B., Žagar, N., Lunkeit, F., and Blender, R.: Long-term atmospheric bias teleconnection and the associated spatio-temporal variability originating from the tropical Indian Ocean sea surface temperature errors, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16899, https://doi.org/10.5194/egusphere-egu23-16899, 2023.

EGU23-946 | ECS | Orals | NP5.1

Combining Bayesian Neural Networks with explainable AI techniques for trustworthy probabilistic post-processing 

Mariana Clare, Zied Ben Bouallegue, Matthew Chantry, Martin Leutbecher, and Thomas Haiden

The large data volumes available in weather forecasting make post-processing an attractive field for applying machine learning. In turn, novel statistical machine learning methods that can be used to generate uncertainty information from a deterministic forecast are of great interest to forecast users, especially given the computational cost of running high resolution ensembles. In this work, we show how one such method, a Bayesian Neural Network (BNN), can be used to post-process a single global high resolution forecast for 2m temperature. This methodology improves both the accuracy of the forecast and adds uncertainty information, by predicting the distribution of the forecast error relative to its own analysis.

Here we assess both model and data uncertainty using two different BNN approaches. In the first approach, the BNN’s parameters are defined to be distributions rather than deterministic parameters, thereby generating an ensemble of models that can be used to quantify model uncertainty. In the second approach, the BNN remains deterministic but predicts a distribution rather than a deterministic output thereby quantifying data uncertainty. Our BNN results are benchmarked against simpler statistical methods, as well as statistics from the ECMWF operational ensemble.

Finally, in order to add trustworthiness to the BNN predictions, we apply an explainable AI technique (Layerwise Relevance Propagation) so as to understand whether the variables on which the BNN bases its prediction are physically reasonable or whether it is instead learning spurious correlations.

How to cite: Clare, M., Ben Bouallegue, Z., Chantry, M., Leutbecher, M., and Haiden, T.: Combining Bayesian Neural Networks with explainable AI techniques for trustworthy probabilistic post-processing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-946, https://doi.org/10.5194/egusphere-egu23-946, 2023.

EGU23-1365 | Posters virtual | NP5.1

Improving post-processing of East African precipitation forecasts using a generative machine learning model 

Bobby Antonio, Andrew McRae, Dave MacLeod, Fenwick Cooper, John Marsham, Laurence Aitchison, Tim Palmer, and Peter Watson

Existing weather models are known to have poor skill over Africa, where there are regular threats of drought and floods that present significant risks to people's lives and livelihoods. Improved precipitation forecasts could help mitigate the negative effects of these extreme weather events, as well as providing significant financial benefits to the region. Building on work that successfully applied a state-of-the-art machine learning method (a conditional Generative Adversarial Network, cGAN) to postprocess precipitation forecasts in the UK, we present a novel way to improve precipitation forecasts in East Africa. We address the challenge of realistically representing tropical convective rainfall in this region, which is poorly simulated in conventional forecast models. We use a cGAN to postprocess ECMWF high resolution forecasts at 0.1 degree resolution and 6-18h lead times, using the iMERG dataset as ground truth, and investigate how well this model can correct bias, produce reliable probability distributions and create samples of rainfall with realistic spatial structure. We will also present performance in extreme rainfall events. This has the potential to enable cost effective improvements to early warning systems in the affected areas.

How to cite: Antonio, B., McRae, A., MacLeod, D., Cooper, F., Marsham, J., Aitchison, L., Palmer, T., and Watson, P.: Improving post-processing of East African precipitation forecasts using a generative machine learning model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1365, https://doi.org/10.5194/egusphere-egu23-1365, 2023.

EGU23-2592 | ECS | Orals | NP5.1

U-Net based Methods for the Postprocessing of Precipitation Ensemble Forecasting 

Romain Pic, Clément Dombry, Maxime Taillardat, and Philippe Naveau

Most Numerical Weather Prediction (NWP) systems use statistical postprocessing methods to correct for bias and underdispersion errors made by ensemble forecasting. This underdispersion leads to an underestimation of extreme events. Thus, many statistical postprocessing methods have been used to take into consideration the extremal behavior of meteorological phenomena such as precipitation. State-of-the-art techniques are based on Machine Learning combined with knowledge from Extreme Value Theory in order to improve forecasts. However, some of the best techniques do not consider the spatial dependency between locations. For example, Taillardat et al. (2019) trains a different Quantile Regression Forest at each location of interest and Rasp & Lerch (2018) uses neural networks with an embedding for the station's information in order to train a global model.
The dataset used corresponds to 3-h precipitation amounts produced by the radar-based observations of ANTILOPE and the 17-members ensemble forecast system called PEAROME. The dataset spans over the south of France with a grid resolution of 0.025 degrees. Our method uses a U-Net-like neural network in order to take into account the spatial structure of the data and the output of our model is a parameterized law at each grid point. Among the choices available in the literature, we focused on the Extended Generalized Pareto Distribution  and the truncated logistic with a point mass in 0. The model is trained by minimizing the scoring rules such as the Continuous Ranked Probability Score, the Log-Score or weighted versions of the aforementioned scoring rules. The method developed here is then compared to the raw ensemble as well as state-of-the-art techniques through scoring rules, skill scores and ROC curves.

References :

  • L. Pacchiardi, R. Adewoyin, P. Dueben, and R. Dutta. Probabilistic forecasting with generative networks via scoring rule minimization. Dec. 2021. arXiv:2112.08217
  • M. Taillardat, A.-L. Fougères, P. Naveau, and O. Mestre. Forest-based and semiparametric methods for the postprocessing of rainfall ensemble forecasting. Weather and Forecasting, 34(3):617–634, jun 2019. doi: 10.1175/waf-d-18-0149.1.

How to cite: Pic, R., Dombry, C., Taillardat, M., and Naveau, P.: U-Net based Methods for the Postprocessing of Precipitation Ensemble Forecasting, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2592, https://doi.org/10.5194/egusphere-egu23-2592, 2023.

EGU23-2628 | ECS | Posters on site | NP5.1

Seasonal Weather Forecast Biases Dependence on Static and Dynamic Environmental Variables in the Alpine Region 

Sameer Balaji Uttarwar, Anna Napoli, Diego Avesani, and Bruno Majone

Global seasonal weather forecasts have inherent biases compared to observational datasets over mountainous regions. This can be attributed to the model's inaccurate representation of local and global environmental processes on the Earth. In this context, the objective of this study is to assess the variation of seasonal weather forecast biases with respect to static and dynamic environmental variables over the Trentino-South Tyrol region (north-eastern Italian Alps), characterized by complex terrain.

The research employs the latest fifth-generation seasonal weather forecast system (SEAS5) dataset produced by the European Center for Medium-Range Weather Forecast (ECMWF), available at a horizontal grid resolution of 0.125° x 0.125° with 25 ensemble members in a re-forecast period from 1981 to 2016. The reference dataset is a high-resolution gridded observation (250 m x 250 m) over the region of interest. The spatiotemporal variation of monthly weather (i.e., precipitation and temperature) forecast biases over the region is inferred using several statistical indicators at observational dataset grid resolution. The static and dynamic environmental variables (i.e., respectively, terrain characteristics and large-scale atmospheric circulation indices) are used univariately to interpret their relationship with monthly weather forecast biases using the linear regression technique. A statistically significant linear relation between monthly weather forecast biases and terrain characteristics, as well as large-scale atmospheric circulation indices, has been found depending on seasonality and ensemble members.

Given significant univariate linear correlation, a simple linear bias reduction model is developed and assessed by implementing a random subsampling technique in which the regression parameters are simulated by splitting the data into calibration (70%) and validation (30%). The results reveal a reduction in the monthly weather forecast bias over the region.

This study demonstrates that the local and global environmental variables should be explicitly considered in the bias correction and downscaling of the seasonal weather forecasts over complex terrain.

How to cite: Uttarwar, S. B., Napoli, A., Avesani, D., and Majone, B.: Seasonal Weather Forecast Biases Dependence on Static and Dynamic Environmental Variables in the Alpine Region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2628, https://doi.org/10.5194/egusphere-egu23-2628, 2023.

This work investigates several statistical tests in the context of probabilistic weather forecasting and ensemble postprocessing. The tests are commonly used for comparing predictive performance of e.g. two statistical postprocessing models.  

In the first part of the analysis a case study is conducted on temperature data consisting of observations and ensemble forecasts. The tests are applied to compare the performance of two probabilistic temperature forecasts at different stations, for different lead times, investigating several standard verification metrics to measure prediction performance. The analysis shows that the tests generally behave consistently in the context of temperature forecasts. However, for certain scenarios some tests might be be preferred over the others. In general, the combination of the original Diebold-Mariano test with the continuous ranked probability score (CRPS) to assess forecast accuracy leads to the most consistent and reliable results.

The second part of the analysis uses simulated data to investigate the general behaviour of the tests in different postprocessing scenarios as well as their size and power properties. Again, the original Diebold-Mariano test appears to perform most reliably and shows no noticeable inconsistent behaviour for different simulation settings.

How to cite: Möller, A. and Grupe, F.: Investigating properties of statistical tests for comparing predictive performance with application to probabilistic weather forecasting, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2701, https://doi.org/10.5194/egusphere-egu23-2701, 2023.

EGU23-2902 | ECS | Posters virtual | NP5.1

D-Vine Copula based Postprocessing of Wind Speed Ensemble Forecasts 

David Jobst, Annette Möller, and Jürgen Groß

Statistical postprocessing of ensemble forecasts has become a common practice in research to correct biases and errors in calibration. Meanwhile, machine learning methods such as quantile regression forests or neural networks are often suggested as promising candidates in literature. However, interpretation of these methods is not always straightforward. 
Therefore, we propose the D-vine (drawable-vine) copula based postprocessing, where for the construction of a multivariate conditional copula the graphical D-vine model serves as building plan. The conditional copula is based on this tracetable model using bivariate copulas, which allow to describe linear as well as non-linear relationships between the response variable and its covariates. Additionally, our highly data-driven model selects the covariates based on their predictive strength and thus provides a natural variable selection mechanism, facilitating interpretability of the model. Finally, (non-crossing) quantiles from the obtained conditional distribution can be utilized as postprocessed ensemble forecasts. 
In a case study for the postprocessing of 10 m surface wind speed ensemble forecasts with 24 hour lead time we compare local and global D-vine copula based models to the zero-truncated ensemble model output statistics (tEMOS) for different sets of predictor variables at 60 surface weather stations in Germany. Furthermore, we investigate different types of training periods for both methods. We observe that the D-vine based postprocessing yields a comparable performance with respect to tEMOS models if wind speed ensemble variables are included only and a significant improvement if additional meteorological and station specific weather variables are integrated. The case study indicates that training periods capturing seasonal patterns are performing best for both models. Additionally, we provide a criterion for calculating the variable importance in D-vine copulas and utilize it to outline which predictor variables are the most important for the correction of 10 m surface wind speed ensemble forecasts.

How to cite: Jobst, D., Möller, A., and Groß, J.: D-Vine Copula based Postprocessing of Wind Speed Ensemble Forecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2902, https://doi.org/10.5194/egusphere-egu23-2902, 2023.

EGU23-5821 | ECS | Posters on site | NP5.1

A multivariate approach to combine general circulation models using graph cuts 

Lucas Schmutz, Soulivanh Thao, Mathieu Vrac, and Gregoire Mariethoz

General circulation models (GCMs) are of extreme importance to making future climate projections. Those are used extensively by policymakers to manage responses to anthropogenic global warming and climate change.

To extract a robust global signal and evaluate uncertainties, individual models are often assembled in Multi-Model Ensembles (MMEs). Various approaches to combine individual models have been developed, such as the Multi-Model Mean (MMM) or its weighted variants.

Recently, Thao et al. (2022) proposed a model comparison approach based on graph cuts. Graph cut optimization was developed in the field of computer vision to efficiently approximate a solution for low-level computer vision tasks such as image segmentation (Boykov et al., 2001). Applied to MMEs, it allows selecting for each gridpoint the best-performing model and produces a patchwork of models that maximizes performances while avoiding spatial discontinuities. Thus, it considers the local performance of individual models in contrast with approaches such as MMM or similar methods that use global weights.

Here we propose a new multivariate combination approach of MMEs based on graph cuts. Compared to the existing univariate method, our approach ensures that the relationships between variables, that are present in GCMs, are locally preserved while providing coherent spatial fields. Moreover, we measure the local performance of models using the Hellinger distance between multi-decadal distributions. This allows a combination of models that is not only indicative of the average behavior (e.g. mean temperature or mean precipitation) but of the entire multivariate distribution, including more extreme values that have a high societal and environmental impact.

REFERENCES 

Boykov, Y., Veksler, O., & Zabih, R. (2001). Fast approximate energy minimization via graph cuts. IEEE Transactions on Pattern Analysis and Machine Intelligence, 23(11), 1222–1239. https://doi.org/10.1109/34.969114

Thao, S., Garvik, M., Mariethoz, G., & Vrac, M. (2022). Combining global climate models using graph cuts. Climate Dynamics, February. https://doi.org/10.1007/s00382-022-06213-4

How to cite: Schmutz, L., Thao, S., Vrac, M., and Mariethoz, G.: A multivariate approach to combine general circulation models using graph cuts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5821, https://doi.org/10.5194/egusphere-egu23-5821, 2023.

EGU23-8594 | ECS | Posters on site | NP5.1

Joint Generalized Neural Models and Censored Spatial Copulas for Probabilistic Rainfall Forecasting 

David Huk, Rilwan Adewoyin, and Ritabrata Dutta

This work develops a novel method for generating conditional probabilistic rainfall forecasts with temporal and spatial dependence. A two-step procedure is employed. Firstly, marginal location-specific distributions are modelled independently of one another. Secondly, a spatial dependency structure is learned in order to make these marginal distributions spatially coherent.
To learn marginal distributions over rainfall values, we propose a class of models termed Joint Generalised Neural Models (JGNMs). These models expand the linear part of generalised linear models with a deep neural network allowing them to take into account non-linear trends of the data while learning the parameters for a distribution over the outcome space.
In order to understand the spatial dependency structure of the data, a model based on censored copulas is presented. It is designed for the particularities of rainfall data and incorporates the spatial aspect into our approach. Uniting our two contributions, namely the JGNM and the Censored Spatial Copulas into a single model, we get a probabilistic model capable of generating possible scenarios on short to long-term timescales, able to be evaluated at any given location, seen or unseen. We show an application of it to a precipitation downscaling problem on a large UK rainfall dataset and compare it to existing methods.

How to cite: Huk, D., Adewoyin, R., and Dutta, R.: Joint Generalized Neural Models and Censored Spatial Copulas for Probabilistic Rainfall Forecasting, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8594, https://doi.org/10.5194/egusphere-egu23-8594, 2023.

EGU23-8824 | ECS | Posters on site | NP5.1

Evaluating probabilistic forecasts of extremes using continuous ranked probability score distributions 

Maxime Taillardat, Anne-Laure Fougères, Philippe Naveau, and Raphaël De Fondeville

Verifying probabilistic forecasts for extreme events is a highly active research area because popular media and public opinions are naturally focused on extreme events, and biased conclusions are readily made. In this context, classical verification methods tailored for extreme events, such as thresholded and weighted scoring rules, have undesirable properties that cannot be mitigated, and the well-known continuous ranked probability score (CRPS) is no exception.

Here, we define a formal framework for assessing the behavior of forecast evaluation procedures with respect to extreme events, which we use to demonstrate that assessment based on the expectation of a proper score is not suitable for extremes. Alternatively, we propose studying the properties of the CRPS as a random variable by using extreme value theory to address extreme event verification. An index is introduced to compare calibrated forecasts, which summarizes the ability of probabilistic forecasts for predicting extremes. The strengths and limitations of this method are discussed using both theoretical arguments and simulations.

How to cite: Taillardat, M., Fougères, A.-L., Naveau, P., and De Fondeville, R.: Evaluating probabilistic forecasts of extremes using continuous ranked probability score distributions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8824, https://doi.org/10.5194/egusphere-egu23-8824, 2023.

The ERA5 global reanalysis has been compared against a high-resolution regional reanalysis (COSMO-REA6) by means of scale-separation diagnostics based on 2d Haar discrete wavelet transforms. The presented method builds upon existing methods and enables the assessment of bias, error and skill for individual spatial scales, separately. A new skill score (evaluated against random chance) and the Symmetric Bounded Efficiency are introduced. These are compared to the Nash-Sutcliffe and the Kling-Gupta Efficiencies, evaluated on different scales, and the benefits of symmetric statistics are illustrated. As expected, the wavelet statistics show that the coarser resolution ERA5 products underestimate small-to-medium scale precipitation compared to COSMO-REA6. The newly introduced skill score shows that the ERA5 control member (EA-HRES), despite its higher variability, exhibits better skill in representing small-to-medium scales with respect to the smoother ensemble members. The Symmetric Bounded Efficiency is suitable for the intercomparison of reanalyses, since it is invariant with respect to the order of comparison.

How to cite: Casati, B., Lussana, C., and Crespi, A.: Scale-separation diagnostics and the Symmetric Bounded Efficiency for the inter-comparison of precipitation reanalyses, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9083, https://doi.org/10.5194/egusphere-egu23-9083, 2023.

EGU23-9328 | Orals | NP5.1

The EUPPBench postprocessing benchmark 

Jonas Bhend, Jonathan Demaeyer, Sebastian Lerch, Cristina Primo, Bert Van Schaeybroeck, Aitor Atencia, Zied Ben Bouallègue, Jieyu Chen, Markus Dabernig, Gavin Evans, Jana Faganeli Pucer, Ben Hooper, Nina Horat, David Jobst, Janko Merše, Peter Mlakar, Annette Möller, Olivier Mestre, Maxime Taillardat, and Stéphane Vannitsem

Statistical postprocessing of forecasts from numerical weather prediction systems is an important component of modern weather forecasting systems. A growing variety of postprocessing methods has been proposed, but a comprehensive, community-driven comparison of their relative performance is yet to be established. Important reasons for this lack include the absence of a fair intercomparison protocol, and, the difficulty of constructing a common comprehensive dataset that can be used to perform such intercomparison. Here we introduce the first version of the EUPPBench, a dataset of time-aligned medium-range forecasts and observations over Central Europe, with the aim to facilitate and standardize the intercomparison of postprocessing methods. This dataset is publicly available [1], includes station and gridded data, ensemble forecasts for training (20 years) and validation (2 years) based on the ECMWF system. The initial dataset is the basis of an ongoing activity to establish a benchmarking platform for postprocessing of medium-range weather forecasts. We showcase a first benchmark of several methods for the adjustment of near-surface temperature forecasts and outline the future plans for the benchmark activity. 

 

[1] https://github.com/EUPP-benchmark/climetlab-eumetnet-postprocessing-benchmark

How to cite: Bhend, J., Demaeyer, J., Lerch, S., Primo, C., Van Schaeybroeck, B., Atencia, A., Ben Bouallègue, Z., Chen, J., Dabernig, M., Evans, G., Faganeli Pucer, J., Hooper, B., Horat, N., Jobst, D., Merše, J., Mlakar, P., Möller, A., Mestre, O., Taillardat, M., and Vannitsem, S.: The EUPPBench postprocessing benchmark, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9328, https://doi.org/10.5194/egusphere-egu23-9328, 2023.

The established benefits of post-processing the results of multi-model ensembles, even by simple averaging, suggest a more radical approach: The models should be combined more frequently in run-time so as to form a single “supermodel”.  Simple nudging of models to one another, as frequently as the models might assimilate data from observations, combines model fusion with a reasonable degree of model autonomy.

Key to the success of the supermodeling approach is the phenomenon of chaos synchronization, known in the field of nonlinear dynamics, wherein two chaotic systems synchronize when connected through only a few of their variables, despite sensitive dependence on initial conditions. Synchronization gives rise to consensus among models. The nudging coefficients can be trained so that that consensus agrees with observations, because the effective dynamics of the trained supermodel, regarded as a single dynamical system, matches the dynamics of nature. Yet the number of independent nudging coefficients that must be trained is far less than the number of trainable parameters in a typical climate model.

It is expected that supermodeling will be especially useful for improving the representation of localized structures, such as blocking patterns, which will wash out if de-synchronized output fields of different models are combined by averaging.  We confirm a hypothesis that such coherent structures will synchronize even when the underlying fields do not, because the internal synchronization within each structure re-enforces synchronization between models: A configuration of CAM4 and CAM5 models, of different resolution, connected by nudging, exhibits correlated blocking activity even when the flows do not otherwise synchronize.  

We further explore the basis for correlated blocking activity in a pair of coupled quasi-geostrophic channel models. The local synchronization error is lower in a region of the channels where blocks form than elsewhere in the channels. Blocking correlations emerge as a vestige of “chimera synchronization”, the phenomenon in which complete synchronization of two spatially extended systems is intermittent in space as well as time. Such partial synchronization of different models in the regions of blocks - and of other structures such as jets, fronts, and large-scale convection - would be particularly useful for projecting climate-change patterns in extreme events associated with those structures.

How to cite: Duane, G., Schevenhoven, F., and Weiss, J.: Synchronization of Blocking Patterns in Diifferent Models, Connected So As to Form a “Supermodel” of Future Climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10153, https://doi.org/10.5194/egusphere-egu23-10153, 2023.

EGU23-11230 | Posters on site | NP5.1

Mathematical Properties of Continuous Ranked Probability Score Forecasting 

Clément Dombry, Romain Pic, Philippe Naveau, and Maxime Taillardat

The theoretical advances on the properties of scoring rules over the past decades have broaden the use of scoring rules in probabilistic forecasting. In meteorological forecasting, statistical postprocessing techniques are essential to improve the forecasts made by deterministic physical models. Numerous state-of-the-art statistical postprocessing techniques are based on distributional regression evaluated with the Continuous Ranked Probability Score (CRPS). However, theoretical properties of such minimization of the CRPS have mostly considered the unconditional framework (i.e. without covariables) and infinite sample sizes. We circumvent these limitations and study the rate of convergence in terms of CRPS of distributional regression methods. We find the optimal minimax rate of convergence for a given class of distributions. Moreover, we show that the nearest neighbor method and the kernel method for distributional regression reach the optimal rate of convergence in dimension larger than 2 and in any dimension, respectively.
Associated article: https://doi.org/10.1016/j.ijforecast.2022.11.001

How to cite: Dombry, C., Pic, R., Naveau, P., and Taillardat, M.: Mathematical Properties of Continuous Ranked Probability Score Forecasting, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11230, https://doi.org/10.5194/egusphere-egu23-11230, 2023.

It is often stated that the goal of probabilistic forecasting is to issue predictive distributions that are as sharp as possible, subject to being calibrated. To assess the calibration of ensemble forecasts, it is customary to employ rank histograms. Rank histograms not only assess whether or not an ensemble prediction system is calibrated, but they also reveal what (if any) systematic biases are present in the forecasts. This information can readily be relayed back to forecasters, helping to improve future predictions. Such is the utility of rank histograms, several extensions have been proposed to evaluate the calibration of probabilistic forecasts for multivariate outcomes. These extensions typically introduce a so-called pre-rank function that condenses the multivariate forecasts and observations into univariate objects, from which a standard rank histogram can be constructed. Several different approaches to construct multivariate rank histograms have been proposed, each of which differs in the choice of pre-rank function. Existing pre-rank functions typically aim to preserve as much information as possible when condensing the multivariate forecasts and observations into univariate objects. Although this is sensible when testing for multivariate calibration, the resulting rank histograms are often difficult to interpret, and are therefore rarely used in practice.        
We argue that the principal utility of these histogram-based diagnostic tools is that they provide forecasters with additional information regarding the deficiencies that exist in their forecasts, in turn allowing them to address these shortcomings more readily; interpretation is therefore a key requirement. We demonstrate that there are very few restrictions on the choice of pre-rank function when constructing multivariate rank histograms, meaning forecasters need not restrict themselves to the few proposed already, but can instead choose a pre-rank function on a case-by-case basis, depending on what information they want to extract from their forecasts. We illustrate this by introducing a range of possible pre-rank functions when assessing the calibration of probabilistic spatial field forecasts. The pre-rank functions that we introduce are easy to interpret, easy to implement, and they provide complementary information. Several pre-rank functions can therefore be employed to achieve a more complete understanding of the multivariate forecast performance. Finally, having chosen suitable pre-rank functions, tests for univariate calibration based on rank histograms can readily be applied to the multivariate rank histograms. We illustrate this here using e-values, which provide a theoretically attractive way to sequentially test for the calibration of probabilistic forecasts.

How to cite: Allen, S. and Ziegel, J.: Assessing the calibration of multivariate ensemble forecasts: E-values and the choice of pre-rank function, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11660, https://doi.org/10.5194/egusphere-egu23-11660, 2023.

EGU23-12232 | ECS | Posters on site | NP5.1

Impacts of uni- and multivariate bias adjustment methods on simulations of hydrological signatures in high latitude catchments 

Faranak Tootoonchi, Andrijana Todorović, Thomas Grabs, and Claudia Teutschbein

Climate models are used to generate future hydroclimatic projections for exploring how climate change may affect water resources. Their outputs, however, feature systematic errors due to parametrization and simplification of processes at the spatiotemporal scales required for impact studies. To minimize the adverse effects of such biases, an additional bias adjustment step is typically required.

Over the past decade, adjustment methods with different levels of complexity have been developed that consider one or several variables at a time, consequently adjusting one or multiple features of climate model simulations. Despite attempts in developing such methods and the growing use of some, the selection of methods for accurate simulation of streamflow remains subjective and still highly debated. In this study, we seek to answer whether sophisticated multivariate bias adjustment methods outperform simple univariate methods in the simulation of streamflow signatures.

To this end, we systematically investigated the ability of two simple univariate and two advanced multivariate methods to accurately represent various hydrological signatures relevant for water resources management in high latitudes. We offer practical guidelines for choosing the most suitable bias adjustment methods based on the objective of each study (i.e., hydrologic signatures of interest) and the hydroclimatic regime of the study catchments.

How to cite: Tootoonchi, F., Todorović, A., Grabs, T., and Teutschbein, C.: Impacts of uni- and multivariate bias adjustment methods on simulations of hydrological signatures in high latitude catchments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12232, https://doi.org/10.5194/egusphere-egu23-12232, 2023.

Spatial sampling remains a conundrum for verification. The observations that are required are rarely on a grid, nor are they homogenously spaced. They are often located where there are people, easy access and do not sample the variable in a representative way. In an aggregate sense, scores derived from such observation locations, will give areas with greater observation density more weight in the aggregate if the variations in network density are not accounted for. Furthermore the performance in some parts of the domain may not be represented at all if there are no observations there. Gridded analyses on the other hand often provide complete coverage, and offer great ease of use, but adjacent grid boxes are not independent. Given this relative wealth of coverage and uniform sampling, we tend to use all available grid points for computing aggregate scores for an area or region, despite knowing that this is likely to produce too-narrow confidence intervals and inflate any statistical significance that may be present. 

In this presentation a variety of approaches, both empirical and statistical, are explored to establish what we ought to include when computing aggregate scores. Three different empirical sampling approaches are compared to selections from statistical coverage or network design algorithms. The empirical options include what is termed “strict” sub-sampling, whereby a sample is taken from the full grid and the reduction in sample size is explored by systematically continually taking a sub-sample from the sub-sample. The second is a systematic reduction in sample size from the original grid whereby each sample is drawn from the original grid, taken every other grid point, then every 3rd grid point, every 4th etc. The third is a mean computed from N random draws of reducing sample size. These empirical options do not respect land or sea locations. They are purely intended at looking at the behaviour and stability of the sample score. The coverage design algorithms provide a methodology for deriving homogeneous samples for irregularly spaced surface networks over land, and regularly spaced sampling of grids over the ocean, to achieve an optimal blend of sampling for regions that cover both land and sea.  These sample sizes and sample scores are compared to a statistically computed effective sample size. 

Some interesting and surprising results emerge. One of which is that as little as 1% of the total number of grid points may be sufficient for measuring the performance of the forecast on a grid, though the proportion of the total will always be dependent on (to varying degrees) the variable, the threshold or event of interest, the metric or score, and the characteristics of the geographical region of interest. 

How to cite: Mittermaier, M. and Gilleland, E.: Exploring empirical and statistical approaches for determining an appropriate sample size for aggregate scores, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12242, https://doi.org/10.5194/egusphere-egu23-12242, 2023.

EGU23-12316 | Posters on site | NP5.1

On the reliability of bivariate forecasts 

Zied Ben Bouallegue

Reliability is a key attribute of an ensemble forecast. Typically, this means that one expects that the ensemble spread reflects the potential error of the corresponding ensemble mean forecast. In the realistic case of an unperfect forecast, reliability deficiencies can be diagnosed with tools such as the reliability diagram and the rank histogram. Along with the computation of scores, the use of these diagnostic tools is common practice in ensemble forecast verification when assessing univariate forecasts. But what does reliability mean in practical terms when assessing multivariate forecasts? Here the concept of reliability is revisited in the simplest of the multivariate cases: the bivariate forecast. As a result, we propose a set of new diagnostic tools with an emphasis on the cross-variable reliability aspect. Real case examples are used for illustration and discussion.

How to cite: Ben Bouallegue, Z.: On the reliability of bivariate forecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12316, https://doi.org/10.5194/egusphere-egu23-12316, 2023.

EGU23-13327 | ECS | Posters on site | NP5.1

Towards a machine learning based multimodel for precipitation forecast over the italian peninsula 

Luca Monaco, Roberto Cremonini, and Francesco Laio

Direct model output forecasts by Numerical Weather Prediction models (NWPs) present some limitations caused by errors mostly due to sensitivity to initial conditions, sensitivity to boundary conditions and deficiencies in parametrization schemes (i.e. orography).
These sources of error are unavoidable, and atmospheric chaotic dynamics make prediction errors spread rapidly in time in the course of the forecast, inducing both systematic and random errors.
Nonetheless, in the last 50 years, NWPs had a significant decrease in the impact of these sources of errors, even in the long-term forecast, thanks for instance to an ever-increasing computational capability, but their relevance is still not neglectable.
Moreover, different NWPs present specific different pros and cons which are findable empirically. For instance, in the case of precipitation forecast in north-west Italy, low-resolution models (e.g. ECMWF-IFS) are more reliable in terms of space and time in predicting the average precipitation, while high-resolution models (e.g. COSMO-2I) tend to forecast better the maximum precipitation. Research purposes apart, actual limitations must be seen in an operational context, where weather forecasts’ skillfulness and associated uncertainty are information of the utmost importance to the forecaster and in general to the user of a certain forecasts system.

To tackle these limitations of NWPs and the need for an uncertainty-quantified meteorological forecast, we propose a machine learning-based multimodel post-processing technique for precipitation forecast. We focus on precipitation since it is the most important variable in the issue of spatially localized weather alert notice by the Italian Civil Protection system and at the same time it is one of the most challenging variables to forecast. 
We use a Convolutional Neural Network (CNN) to obtain deterministic and probabilistic forecast grids over 24h up to 48h focusing on North-West Italy, using several high and low-resolution deterministic NWPs as input and using high-resolution rain-gauge corrected radar observations for the training. The effect of the usage of different convolutional parameters (e.g. stride, padding) is taken into account. The deterministic output grid is chosen as the grid with the lowest mean square error obtained during the training, and it is compared with the linear regression of the input NWPs and with every single model. The probabilistic output grid is generated by considering the statistical ensemble of the twenty grids with the lowest mean square error obtained during the training, and it is compared with the logistic regression of the input NWPs and with ECMWF-EPS as a benchmark, both at different precipitation thresholds.

How to cite: Monaco, L., Cremonini, R., and Laio, F.: Towards a machine learning based multimodel for precipitation forecast over the italian peninsula, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13327, https://doi.org/10.5194/egusphere-egu23-13327, 2023.

In recent years neural networks have successfully been applied to probabilistic post-processing of numerical weather prediction forecasts. In the Bernstein Quantile Networks (BQN) method predictive quantile distributions are specified by Bernstein polynomials and their coefficients linked to input features through flexible neural networks. However, precipitation presents an additional challenge due to its mixed distributed nature with a considerable proportion of dry events for short accumulation periods. In this presentation, it is demonstrated how the BQN method can be modified to mixed distributed variables like precipitation by introducing a latent variable and treating zero precipitation cases as censored data. The method is tested on both synthetic and real precipitation forecast data and compared to an approach where a model of the probability of precipitation is combined with a model of precipitation amounts using the laws of probability.

 

How to cite: Bremnes, J. B.: Censored Bernstein quantile networks for probabilistic precipitation forecasting, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13849, https://doi.org/10.5194/egusphere-egu23-13849, 2023.

EGU23-14425 | ECS | Posters on site | NP5.1

Lead time continuous statistical post-processing of ensemble weather forecasts 

Jakob Wessel, Chris Ferro, and Frank Kwasniok

Numerical weather prediction (NWP) models usually output their forecasts at a multiplicity of different lead times. For example, the Met Office ensemble prediction system for the UK (MOGREPS-UK) predicts atmospheric variables on a 2.2km grid for up 126h on hourly and sub-hourly timesteps. Even though for applications, information is often required on this range of lead times, many post-processing methods in the literature are either applied at fixed lead time or by fitting individual models for each lead time. This is also the case in systems used in practice such as the Met Office IMPROVER system. However, this is 1) computationally expensive because it requires the training of multiple models if users are interested in information at multiple lead times and 2) prohibitive because it restricts the training data used for training post-processing models and the usability of fitted models.

In this work we investigate lead time dependence of ensemble post-processing methods by looking at ensemble forecasts in an idealized Lorenz96 system as well as temperature forecast data from the Met Office MOGREPS-UK system. First, we investigate the lead time dependence of estimated model parameters in non-homogenous Gaussian regression (NGR -- a standard ensemble post-processing technique) and find substantial smoothness. Secondly, we look at the usability of models fitted for one lead time and employed at another to then thirdly fit models that are “lead time continuous”, meaning they work for multiple lead times simultaneously by including lead time as a covariate using spline regression. We show that these models can achieve similar performance to the classical “lead time separated” models, whilst saving substantial computation time. Fourthly and finally we make first steps towards the development of a cheap computational model including seasonality and working continuously over the lead time, needing to be fit only once.

How to cite: Wessel, J., Ferro, C., and Kwasniok, F.: Lead time continuous statistical post-processing of ensemble weather forecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14425, https://doi.org/10.5194/egusphere-egu23-14425, 2023.

EGU23-14560 | ECS | Posters on site | NP5.1

Quantile regression forests for post-processing ECWMF ensemble precipitation forecasts: hyperparameter optimization and comparison to EMOS 

Eva van der Kooij, Antonello Squintu, Kirien Whan, and Maurice Schmeits

Ensemble forecasts are important due to their ability to characterize forecast uncertainty, which is fundamental when forecasting extreme weather. Ensemble forecasts are however often biased and underdispersed and thus need to be post-processed.

A common approach for this is the use of ensemble model output statistics (EMOS), where a parametric distribution is fitted with a limited number of predictors. With recent advances in computer science and increased amounts of data available, machine learning techniques, like random forests, are becoming more popular for high dimensional regression problems. In this research, we explore the use of the quantile regression forest (QRF), a random forest adapted for conditional quantile estimation, applied to medium range gridded probabilistic precipitation forecasts. QRFs are non-parametric and allow for a larger number of predictors, which means they can possibly consider more dependencies that might otherwise not be captured with a simple EMOS.

A QRF takes several hyperparameters that influence the way the decision trees in the forest are constructed. We explore the minimum number of samples needed in a leaf to split it (minimum node size) and the number of predictors explored in each split (mtry). A hyperparameter space is constructed by setting ranges for both minimum node size and mtry, and the optimal hyperparameter set is determined by performing a cross validated grid search. Here, each model is assessed based on the continuous ranked probability skill score (CRPSS). For comparison, EMOS is applied with a zero-adjusted gamma (ZAGA) distribution, using a limited number of predictors that are physically correlated to precipitation. Both methods are verified on a separate testing data set and evaluated using several scores, including CRPSS and Brier skills score (BSS).

We consider 4 years (November 2018 – October 2022) of archived operational ECMWF-IFS ensemble forecasts for the Netherlands. The data is split into November 2018 – October 2021 for training and cross-validation, and October 2021 – October 2022 for testing, separating data for season, initialization time and lead-time. Forecasts are post-processed up to +10 days. Ensemble statistics on 60+ forecast variables are used as predictors. Spatially and temporally aggregated, gauge-adjusted radar observations are used as predictand. The raw ensemble is considered as the benchmark.

The results of this research will determine what method will be used to post-process the ensemble precipitation forecasts in the context of the early warning center (EWC) of the Royal Netherlands Meteorological Institute. The most suitable method could differ between shorter and longer lead times.

How to cite: van der Kooij, E., Squintu, A., Whan, K., and Schmeits, M.: Quantile regression forests for post-processing ECWMF ensemble precipitation forecasts: hyperparameter optimization and comparison to EMOS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14560, https://doi.org/10.5194/egusphere-egu23-14560, 2023.

EGU23-14712 | ECS | Orals | NP5.1

NWP model updates and post-processing: a strategy for an EMOS model on ECMWF wind gusts forecasts 

Antonello A. Squintu, Eva van der Kooij, Kirien Whan, and Maurice Schmeits

In the framework of KNMI’s Early Warning Center (EWC), ECMWF ensemble (ENS) predictions are used to issue medium-range forecasts of severe weather. Timely forecasts of wind gusts extremes are important to prevent potential damage. However, ensemble forecasts are affected by biases and under- or over-dispersion. These errors lead to a reduction in the skill of the forecasts, especially for long lead-times and for extreme cases, such as windstorms and deep convective episodes. Hence, statistical post-processing is a fundamental step in the establishment of a skillful weather alert system for extreme wind gust events.     

However, weather models like ECMWF-IFS are subject to frequent updates, which include changes in the calculation of certain diagnostic variables and by consequence in statistical features of their ensemble distribution. This is the case for ECMWF wind gusts forecasts, whose bias has been reduced with the last update in October 2021. Therefore, the use of pre-update wind gusts forecasts in the training of the post-processing model must be considered with care.

In the context of the development of an Ensemble Model Output Statistics (EMOS) model, this limitation has been tackled by reconstructing wind-gusts forecasts with a preliminary EMOS model. This step has been performed by including in the regression those variables that are used by ECMWF for the calculation of wind gusts, which were less affected by the update.

The reconstructed wind gusts forecasts have been added to a set of summary statistics of the ensemble distribution of variables physically related to wind gusts. A process of forward selection has been applied to identify the most relevant contributions to the general EMOS model, highlighting reconstructed wind gusts as the most important predictor for all lead-times.

The post-processed forecasts obtained with this experimental EMOS model have been verified and compared to those calculated with a conventional EMOS model (performed ignoring the above caveats) and with the results of a non-parametric Quantile Regression Forest. These models have been trained on the same period (2018-2021) and tested on the period that has followed the update (2021-2022), including only grid-points and stations that cover the territory of the Netherlands and distinguishing between summer and winter half-years. The method showing the best performance will be employed operationally for the post-processing of ECMWF-ENS wind gust forecasts over the Netherlands and will be used in the EWC weather alert system.

How to cite: Squintu, A. A., van der Kooij, E., Whan, K., and Schmeits, M.: NWP model updates and post-processing: a strategy for an EMOS model on ECMWF wind gusts forecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14712, https://doi.org/10.5194/egusphere-egu23-14712, 2023.

EGU23-15152 | ECS | Posters on site | NP5.1

Towards sub-kilometer resolution probabilistic analysis of surface wind in complex terrain 

Francesco Zanetta, Daniele Nerini, Matteo Buzzi, and Mark A. Liniger

Correctly representing surface wind is critical for applications such as renewable energy, snow modelling or warning systems. However, numerical weather prediction models with their limited resolution cannot fully represent the strong variability due to complex topography. Downscaling techniques – functionally equivalent to postprocessing when the ground truth is given by observational data - can achieve remarkable results in reducing systematic biases of raw models and can be calibrated to yield accurate probabilistic information at any point in space. 

These techniques can be further improved at analysis time by including real-time measurements, allowing to produce a probabilistic sub-grid resolution analysis of surface wind. Such a product would enable other interesting applications, such as detailed climatologies or nowcasting, and could serve as a ground truth for training deep learning-based postprocessing models with generative approaches, allowing to model spatially and temporally consistent ensembles.  

The first important challenge is to integrate measurements in a statistically optimized and efficient way. Here, we share our ongoing work and preliminary results in a comparative analysis of different approaches, from naïve interpolations to geostatistical techniques or novel approaches based on neural networks. The analysis is based on a multi-year archive of hourly wind observations and NWP analyses from the operational COSMO-1E model over Switzerland. 

How to cite: Zanetta, F., Nerini, D., Buzzi, M., and Liniger, M. A.: Towards sub-kilometer resolution probabilistic analysis of surface wind in complex terrain, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15152, https://doi.org/10.5194/egusphere-egu23-15152, 2023.

EGU23-17348 | Orals | NP5.1

Postprocessing of ensemble precipitation forecasts over India using weather types 

Martin Widmann, Noemi Gonczol, Michael Angus, and Robert Neal

Accurate predictions of heavy precipitation in India are vital for impact-orientated forecasting, and an essential requirement for mitigating the impact of damaging flood events. Operational forecasts from non-convection-permitting models can have large biases in the intensities of heavy precipitation, and while convection-permitting models can perform better, their operational use over large areas is not yet feasible. Statistical postprocessing can reduce these biases for relatively little computational cost, but few studies have focused on postprocessing forecasts of monsoonal rainfall.

We present a postprocessing method for operational precipitation forecasts based on local precipitation distributions for 30 Indian weather types. It is applied to ensemble forecasts for daily precipitation with 12km spatial resolution and lead times of up to 10 days from the Indian National Centre for Medium Range Weather Forecasting (NCMRWF) Ensemble Prediction System (NEPS). The method yields local probabilistic forecasts that are the weighted mean of the observed local precipitation distributions for each weather type, with weights given by the relative frequency of the weather types in the forecast ensemble.

The general forecast skill is determined through the Continuous Ranked Probability Skill Score (CRPSS) and the skill for predicting the exceedance of the local 90th percentile is quantified through the Brier Skill Score (BSS). The CRPSS shows moderate improvement over most of India for forecasts with one day lead time, and substantial improvements almost everywhere for longer lead times. The BSS for one day forecasts indicates a spatially complex pattern of higher and lower performance, while for longer lead times the forecasts for heavy precipitation are improved almost everywhere. The improvements with respect to both measures are particularly high over mountainous or wet regions. We will also present reliability diagrams for the raw and postprocessed forecasts of threshold exceedances.

 

 

How to cite: Widmann, M., Gonczol, N., Angus, M., and Neal, R.: Postprocessing of ensemble precipitation forecasts over India using weather types, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17348, https://doi.org/10.5194/egusphere-egu23-17348, 2023.

EGU23-3730 | PICO | AS1.6

Simulating atmospheric dust and its radiative impact with a global variable-resolution model 

Chun Zhao, Jiawang Feng, Qiuyan Du, Mingyue Xu, Jun Gu, and Zhiyuan Hu

In this study, a global variable-resolution modeling framework of atmospheric dust and its radiative feedback is introduced and evaluated. In this model, atmospheric dust is simulated simultaneously with the meteorological fields, and dust-radiation interaction is included. Five configurations of global mesh with the refinement at different resolutions and over different regions of interest are used to explore the impacts of regional refinement on modeling dust lifecycle at regional and global scales. The model produces reasonably the overall magnitudes and spatial variabilities of global dust metrics such as surface mass concentration, total deposition, AOD, and radiative forcing compared to observations and previous modeling results. Two global variable-resolution simulations with mesh refinement over major deserts of North Africa (V16km-NA) and East Asia (V16km-EA) simulates less dust emissions and smaller dry deposition rate inside the refined regions due to the weakend near-surface wind speed caused by better resolved topographic complexity at higher resolution. Dust mass loading over North Africa is close to each other between V16km-NA and U120km, while over East Asia, V16km-EA simulates higher dust mass loading. Over the non-refined areas with the same resolution, the difference between global variable-resolution and uniform-resolution experiments also exist, which is partly related to their difference in dynamic time-step and the coefficient for horizontal diffusion. Refinement at convection-permitting resolution around the Tibet Plateau (TP) leads to significantly different dust and precipitation around the TP against coarse resolution, which implies that dust-precipitation interaction over this area deserves further investigation with this  global variable-resolution modeling framework in future. 

How to cite: Zhao, C., Feng, J., Du, Q., Xu, M., Gu, J., and Hu, Z.: Simulating atmospheric dust and its radiative impact with a global variable-resolution model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3730, https://doi.org/10.5194/egusphere-egu23-3730, 2023.

EGU23-3983 | PICO | AS1.6

Indirect and direct aerosol feedback in the global and regional scale NOAA UFS Weather Model 

Haiqin Li, Georg Grell, Ravan Ahmadov, Johana Romero-Alvarez, Li Zhang, Eric James, Barry Baker, Joseph Olson, Shan Sun, Jordan Schnell, and Ning Wang

Aerosols play a significant role in the radiation and atmospheric precipitation physics of microphysics and convection, and have a significant impact on air quality, visibility, public health, aviation, and climate. A physics suite, which includes the aerosol-aware double momentum Thompson-Eidhammer microphysics scheme (TH-E MP), the scale-aware and aerosol-aware Grell-Freitas (GF) convection scheme, and the MYNN-EDMF boundary layer and shallow cloud scheme, was developed at NOAA Global System Laboratory (GSL). The GSL physics suite is applied in the FV3GFS global model and the Rapid Refresh Forecast System (RRFS) regional model. We also developed the RRFS – Smoke and Dust model (RRFS-SD) at NOAA GSL with the Common Community Physics Package (CCPP), which is designed to facilitate a host-model agnostic implementation of physics parameterizations. Because of the interactive and strongly coupled nature of chemistry and physics, it is natural to allow for the smoke, dust and other chemical modules to be called directly from the physics suite. Here we embedded the plume rise modules for wildfire, sea-salt, dust, and anthropogenic emission modules into the regional model of RRFS and global UFS model using CCPP as subroutines of physics. The prognostic emissions of sea-salt, and organic carbon are combined to represent the “water friendly” aerosol emission, while the prognostic emission of dust is used to represent “ice friendly” aerosol emission for TH-E MP. With this implementation, we examined the aerosol indirect feedback when using the TH-E scheme in the global FV3GFS forecast with C768 (~13km) horizontal resolution and 127 vertical levels. There are significant cloud-radiation responses to the aerosol differences, and the severely positive precipitation bias over Europe and North America is significantly alleviated when applying this aerosol emission method for indirect feedback. We also examined the smoke direct feedback to the radiation in the RRFS-SD with 3km horizontal resolution and 64 vertical layers for September, 2020 during which the western US experienced extreme wildfires. The aerosol direct feedback run significantly improves the forecast of aerosol optical depth, surface 2m air temperature, 10m wind speed, and radiation fluxes.

How to cite: Li, H., Grell, G., Ahmadov, R., Romero-Alvarez, J., Zhang, L., James, E., Baker, B., Olson, J., Sun, S., Schnell, J., and Wang, N.: Indirect and direct aerosol feedback in the global and regional scale NOAA UFS Weather Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3983, https://doi.org/10.5194/egusphere-egu23-3983, 2023.

The Chinese Meteorology Administration chemistry model CUACE is online integrated into the mesoscale operational weather prediction (NWP) model (GRAPES_Meso5.1) and aerosol-cloud-radiation interaction is achieved to establish the first version (V1) of chemistry-weather (CW) interacted model GRAPES-Meso5.1/CUACE CW V1. The most polluted winter 2016-2017 is selected to study the meteorology impacts on haze/fog prediction, the impact of aerosol-radiation, aerosol-cloud and CW interaction (ARI, ACI, CWI) on haze/fog prediction and NWP. Single way model without CWI displays reasonable PM 2.5 and visibility prediction in general. However, modeled PM2.5 peaks are underestimated and visibility valleys are overestimated during haze/fog pollution, the underestimation of relative humidity (RH) contributes major to this misestimation; CWI model cut the negative bias of PM 2.5 peaks and the positive bias of visibility valleys. The improvement of 5km and 3km low visibility by CWI during severe haze/fog period is more obvious than that of 10 km, which just compensates for the largest deficiency in low visibility prediction related with severe haze/fog by single way model; The NWP including sea level pressures, relative humidity(RH), temperature, wind speed are also improved by CWI from surface to upper troposphere; ARI contributes larger to the predicted PM2.5 ,visibility and NWP improvement than that of ACI, their relative contributions varies with model vertical height and the overlapping condition of cloud and aerosols. Due to the joint contribution of RH and PM2.5, CWI’s improving on visibility is larger than PM2.5. This study illustrates the importance of including CWI in air quality prediction model.

How to cite: Wang, H.: Chemistry-Weather Interacted Model System GRAPES_Meso5.1/CUACE CW V1.0: Development, Evaluation and Application in Better Haze/fog Prediction in China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4025, https://doi.org/10.5194/egusphere-egu23-4025, 2023.

The representation of aerosol–cloud interaction (ACI) and its impacts in the current climate or weather model remains a challenge, especially for severely polluted regions with high aerosol concentration, which is even more important and worthy of study. Here, ACI is first implemented in the atmospheric chemistry model GRAPES_Meso5.1/CUACE by allowing for real-time aerosol activation in the Thompson cloud microphysics scheme. Two experiments are conducted focusing on a haze pollution case with coexisting high aerosol and stratus cloud over the Jing–Jin–Ji region in China to investigate the impact of ACI on the mesoscale numerical weather prediction (NWP). Study results show that ACI increases cloud droplet number concentration, water mixing ratio, liquid water path (CLWP), and optical thickness (COT), as a result improving the underestimated CLWP and COT (reducing the mean bias by 21% and 37%, respectively) over a certain subarea by the model without ACI. A cooling in temperature in the daytime below 950 hPa occurs due to ACI, which can reduce the mean bias of 2 m temperature in the daytime by up to 14% (∼ 0.6 ℃) in the subarea with the greatest change in CLWP and COT. The 24 h cumulative precipitation in this subarea corresponding to moderate-rainfall events increases, which can reduce the mean bias by 18%, depending on the enhanced melting of the snow by more cloud droplets. In other areas or periods with a slight change in CLWP and COT, the impact of ACI on NWP is not signifificant, suggesting the inhomogeneity of ACI. This study demonstrates the critical role of ACI in the current NWP model over the severely polluted region and the complexity of the ACI effect.

How to cite: Zhang, W., Wang, H., and Zhang, X.: Aerosol–cloud interaction in the atmospheric chemistry model GRAPES_Meso5.1/CUACE and its impacts on mesoscale numerical weather prediction under haze pollution conditions in Jing–Jin–Ji in China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4146, https://doi.org/10.5194/egusphere-egu23-4146, 2023.

EGU23-11392 | PICO | AS1.6

Simulating direct and semi-direct effect of aerosols on subseasonal prediction: climatology versus interactive aerosols in the UFS model 

Shan Sun, Gregory Frost, Georg Grell, Li Zhang, Barry Baker, Jessica Meixner, and Anning Cheng

We investigate the aerosol direct and semi-direct effect on subseasonal prediction using NOAA’s fully coupled Unified Forecast System (UFS) model, which includes the atmospheric model FV3 with the Global Forecast System (GFS) physics package V17, MOM6 ocean model, WW3 wave model and CICE6 sea ice model. A systematic twin experiment is carried out: (i) UFS with prescribed aerosol climatology and (ii) UFS coupled to interactive aerosols from the GOCART aerosol module. Both experiments are deterministic 32-day hindcasts with monthly initialization over multiple years.

The modeled aerosol optical depth (AOD) in both experiments is in good agreement with the MODIS satellite observations. The AOD from the experiments with interactive aerosols captured the interannual variability seen in the observations. The estimated radiative forcing from the aerosol radiation interaction in these two sets of experiments is similar in the multi-year average. However, the advantage in the experiments with interactive aerosols can be seen clearly when simulating radiative forcing in the extreme dust storm and biomass burning events. Changes in cloud and precipitation are small between these two sets of experiments.

How to cite: Sun, S., Frost, G., Grell, G., Zhang, L., Baker, B., Meixner, J., and Cheng, A.: Simulating direct and semi-direct effect of aerosols on subseasonal prediction: climatology versus interactive aerosols in the UFS model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11392, https://doi.org/10.5194/egusphere-egu23-11392, 2023.

EGU23-13739 | PICO | AS1.6 | Highlight

Project FOCI - Non-CO2 Forcers and Their Climate, Weather, Air Quality and Health Impacts 

Tomas Halenka, Ranjeet Sokhi, and Alexander Baklanov

While overall global warming with the causes and global processes connected to well-mixed CO2, and its impacts on global to continental scales are well understood with a high level of confidence, there are knowledge gaps concerning the impact of many other non-CO2radiative forcers leading to low confidence in the conclusions. This relates mainly to specific anthropogenic and natural precursor emissions of short-lived GHGs and aerosols and their precursors. These gaps and uncertainties also exist in their subsequent effects on atmospheric chemistry and climate, through direct emissions dependent on changes in e.g., agriculture production and technologies based on scenarios for future development as well as feedback of global warming on emissions, e.g., permafrost thaw. In addition to the atmospheric radiative forcing (gaseous or aerosols), albedo changes connected to land use and land cover can play a role, depending on the adaptation or mitigation measures included in different scenarios.

The main goal of the EC Horizon Europe project FOCI (from the call HORIZON-CL5-2021-D1-01-0 Improved understanding of greenhouse gas fluxes and radiative forcers, including carbon dioxide removal technologies), is to assess the impact of key radiative forcers, where and how they arise, the processes of their impact on the climate system, to find and test an efficient implementation of these processes into global Earth System Models and into Regional Climate Models, eventually coupled with CTMs, and finally to use the tools developed to investigate mitigation and/or adaptation policies incorporated in selected scenarios of future development targeted at Europe and other regions of the world. We will develop new regionally tuned scenarios based on improved emissions to assess the effects of non-CO2 forcers. Mutual interactions of the results and climate services producers and other end-users will provide feedback for the specific scenarios preparation and potential application to support the decision-making, including climate policy.

How to cite: Halenka, T., Sokhi, R., and Baklanov, A.: Project FOCI - Non-CO2 Forcers and Their Climate, Weather, Air Quality and Health Impacts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13739, https://doi.org/10.5194/egusphere-egu23-13739, 2023.

EGU23-15355 | PICO | AS1.6

Changes to the IFS atmospheric composition model in support to the CAMS update for CY49R1. 

Samuel Remy, Vincent Huijnen, Chabrillat Simon, Swen Metzger, Jason Williams, Daniele Minganti, Christine Bingen, Mihai Alexe, and Johannes Flemming

The Integrated Forecasting System (IFS) of ECMWF is core of the Copernicus Atmosphere Monitoring Service (CAMS) to provide global analyses and forecasts of atmospheric composition, including reactive gases, as well as aerosol and greenhouse gases. The CAMS global model consists of the aerosol model of the IFS, IFS-AER, which is a sectional-bulk scheme, while the chemistry scheme is based on a CB05-based carbon-bond mechanism, with the option to couple this to BASCOE-based stratospheric chemistry. The composition model is updated regularly, aligned with updates of ECMWF’s operational meteorological model. Here we report on updates planned for the operational version after next, referred to as CY49R1. This concerns revisions on a large range of topics, as developed over the recent years, and therefore impacting many aspects of chemistry and aerosol composition in troposphere and stratosphere. Main aspects concern:

  • A review of the representation of polar stratospheric clouds and of their impact on stratospheric ozone,
  • An extension of IFS-AER to represent stratospheric sulfate aerosols, coupled with CB05 and BASCOE precursor gases,
  • An upgrade of gas-particle partitioning through the implementation of EQSAM4Clim in the IFS,
  • Computation of aerosol, cloud and rain pH, and use of the update pH values in aqueous chemistry,
  • A combined representation of aerosols and chemistry deposition processes (wet and dry),
  • Update of aerosol optics, including a simple representation of dust asphericity and hygroscopic growth,
  • Update of PM diagnostic output

In this contribution we provide an overview of expected changes with emphasis on changes in composition modeling aspects. We will present their expected impact on key atmospheric composition aspects, including air quality performance across major pollution regions across the world, aerosol optical depth, dust, and stratospheric composition products.

How to cite: Remy, S., Huijnen, V., Simon, C., Metzger, S., Williams, J., Minganti, D., Bingen, C., Alexe, M., and Flemming, J.: Changes to the IFS atmospheric composition model in support to the CAMS update for CY49R1., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15355, https://doi.org/10.5194/egusphere-egu23-15355, 2023.

EGU23-15547 | ECS | PICO | AS1.6 | Highlight

Introduction to the AQ-WATCH multi-model air quality forecast system 

Cathy Wing Yi Li, Mikhail Sofiev, Renske Timmermans, Richard Kranenburg, Gabriele Pfister, Rajesh Kumar, Adrien Deroubaix, Nicolas Huneeus, Mariel Opazo, Tomas Caballero, Dan Mo, Xuelei Zhang, Lukas Hubert Leufen, Felix Kleinert, Martin Schultz, Claire Granier, Sara Basart, Olivier Salvi, Bastien Caillard, and Guy Brasseur

AQ-WATCH (Air Quality: Worldwide Analysis and Forecasting of Atmospheric Composition for Health) is an international consortium, which co-develops and co-produces tailored products and services derived from space and in situ observational data for improving air quality forecasts and attribution. For this purpose, AQ-WATCH develops a supply chain leading to innovative downstream products and services for providing air quality information tailored to the identified needs of international users. This presentation will focus on one of the AQ-WATCH products, the AQ-WATCH air quality forecast system. Air quality forecast models provided by the AQ-WATCH consortium are set up for the focus regions in Asia and the Americas, based on the templates of Copernicus European and MarcoPolo-Panda Asian ensembles, but with much higher resolution and reliance on regional emission and observational information. The models are established over the focus regions using the meteorological and emission data taken from Copernicus repositories and other national archives and refined with local information wherever available. Each forecast model is then evaluated using local observational datasets and with the needs of the stakeholders. Machine learning workflows are being incorporated into the forecast system to improve both results from individual models and the model ensembles based on bias correction from observation data. Lessons learnt from model comparison in the focus regions will be presented. At last, the potential application of the system prototype, as well as the other AQ-WATCH products, namely the global and regional air quality atlas, the air quality attribution & mitigation, the dust and fire forecasts, and the fracking analysis tool, to other regions of the world will be discussed.

How to cite: Li, C. W. Y., Sofiev, M., Timmermans, R., Kranenburg, R., Pfister, G., Kumar, R., Deroubaix, A., Huneeus, N., Opazo, M., Caballero, T., Mo, D., Zhang, X., Leufen, L. H., Kleinert, F., Schultz, M., Granier, C., Basart, S., Salvi, O., Caillard, B., and Brasseur, G.: Introduction to the AQ-WATCH multi-model air quality forecast system, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15547, https://doi.org/10.5194/egusphere-egu23-15547, 2023.

EGU23-15869 | PICO | AS1.6

Extension and evaluation of the Integrated Forecast System (IFS) cycle 49R1 to stratospheric aerosols and chemistry for the global Copernicus Atmospheric Monitoring Service (CAMS) 

Christine Bingen, Simon Chabrillat, Quentin Errera, Vincent Huijnen, Swen Metzger, Daniele Minganti, Samuel Rémy, Jason Williams, and Johannes Flemming

The ECMWF’s Integrated Forecast System (IFS) is the global atmospheric model used by the Copernicus Atmospheric Monitoring Service (CAMS) to provide analyses and forecasts on atmospheric composition. Currently, the CAMS global model includes the aerosol model of the IFS, the aerosol module IFS-AER making use of a sectional-bulk scheme, and the chemistry scheme based on a CB05-based carbon-bond mechanism, with the option to couple this to stratospheric chemistry module BASCOE. The combined BASCOE will be used operationally in the CAMS global system starting from the upgrade to cycle 48R1 planned in June 2023. This abstract focuses on further developments related to stratospheric chemistry and aerosols that are to be implemented in the future operational cycle 49R1, as well as on a first evaluation of IFS’ performances in representing stratospheric aerosols and chemistry against different datasets.

Initially focussing on the troposphere, IFS-AER has been extended to include and represent stratospheric sulfate aerosol processes, keeping the existing tracers. The extended IFS-AER(strato) has been coupled to IFS(BASCOE) through the gaseous sulphuric acid tracer, to the IFS radiation scheme, and to the 4Dvar assimilation scheme. The evaluation of aerosol aspects makes use of aerosol datasets (aerosol extinction, AOD, …) from the Global Ozone Monitoring by Occultation of Stars (GOMOS, onboard Envisat), and the Global Space-based Stratospheric Aerosol Climatology (GloSSAC), based on different cases studies including quiescent and (highly) volcanic periods. It has also been tested against reference simulations from WACCM-CARMA. These intercomparisons show a reasonable agreement against retrieval datasets such as GloSSAC and reference simulations from WACCM-CARMA. In quiescent conditions, the new system showed a decreasing trend with respect to the reference datasets.

BASCOE includes a simple PSC parameterization, which has been updated and tuned in cycle 49R1. In order to assess the impact of this upgrade, we evaluate the composition of the polar lower stratosphere during the winter-spring seasons ("ozone hole" events) of 2008, 2009 and 2020 above the Antarctic and 2009, 2011, 2012 and 2020 above the Arctic, with a focus on 5 key species observed by Aura-MLS. This evaluation demonstrates the capacity of IFS(BASCOE) to forecast the chemical composition of the polar lower stratosphere above both the Arctic and the Antarctic for several years with very different evolution of the polar vortex. While further improvements are desirable and will require an overhaul of the PSC parameterization, the current performance allows us to study the interannual variability of ozone hole episodes.

How to cite: Bingen, C., Chabrillat, S., Errera, Q., Huijnen, V., Metzger, S., Minganti, D., Rémy, S., Williams, J., and Flemming, J.: Extension and evaluation of the Integrated Forecast System (IFS) cycle 49R1 to stratospheric aerosols and chemistry for the global Copernicus Atmospheric Monitoring Service (CAMS), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15869, https://doi.org/10.5194/egusphere-egu23-15869, 2023.

EGU23-16081 | ECS | PICO | AS1.6

Impact of the use of biofuels on the formation of ultrafine particles in southeastern Brazil 

Alejandro Herman Delgado Peralta and Maria de Fatima Andrade

Southeastern Brazil is the most developed and populous region with 89.5 million of inhabitants, according to the Instituto Brasileiro de Geografia e Estatística (IBGE) for 2021. The main metropolitan and industrialized areas are concentrated in its four states (São Paulo, Minas Gerais, Rio de Janeiro and Espírito Santo). One of them comprises the Metropolitan Area of São Paulo (MASP) with 7.3 million vehicles that releases air pollutant -gas and ultrafine particles- to the atmosphere due to the use of different fuel types; light-duty vehicles consume ethanol, gasohol (85% gasoline and 25% hydrous ethanol) or natural gas, and heavy vehicles (i.e., buses and trucks) run on diesel. So, frequently high concentrations of air pollutants (ozone and fine particles) in urban areas are above the recommended limits suggested by the World Health Organization (WHO) with high health risk mainly for children and elderly. The biggest concern is the high health risk of exposing the population to ultrafine particles, also called nanoparticles. Consequently, it is important to understand the formation of ultrafine particles, whether they are emitted directly or formed in the atmosphere. 

We study the formation processes of ultrafine particles in the scenario of fuel change in the road transport sector, including a greater use of biofuels. The air quality modeling system will analyze the impact of different scenarios in urban areas in southeastern Brazil. We begin with the air quality simulation for the current conditions as the base case scenario using the WRF-Chem model. As the main data input, we use emission data with two temporal profile distributions (monthly and hourly time average). First, we use available monthly anthropogenic emission's data processed by the European Copernicus Atmosphere Service (CAMS). Secondly, we added hourly road transport emission calculated with the LAPAT model, which use emission factors derived from measurements in experimental campaigns in tunnels where light and heavy vehicles circulate within the MASP. This simulation test with the WRF-Chem model considers the MOZART-MOSAIC mechanism and additional emissions from other sources such as biomass burning and chemical initial and boundary conditions from the CAM-Chem model. Experimental data and measurements of meteorological and air quality parameters will support the work to evaluate the performance of the model’s results.

How to cite: Delgado Peralta, A. H. and Andrade, M. D. F.: Impact of the use of biofuels on the formation of ultrafine particles in southeastern Brazil, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16081, https://doi.org/10.5194/egusphere-egu23-16081, 2023.

EGU23-16085 | PICO | AS1.6

Impact of pH computation from EQSAM4Clim on inorganic aerosols in the CAMS system 

Swen Metzger, Samuel Rémy, Vincent Huijnen, Jason Williams, Simon Chabrillat, Christine Bingen, and Johannes Flemming

The Integrated Forecasting System (IFS) of ECMWF is used within the Copernicus Atmosphere Monitoring Service (CAMS) to provide global analyses and forecasts of atmospheric composition, including aerosols as well as reactive trace gases and greenhouse gases. Inorganic gas/aerosol equilibrium involving the major sulphate and nitrate anions, i.e., H2SO4/HSO4-/SO42- and HNO3/NO3-, largely determines the aerosol acidity, while the gas/liquid/solid phase partitioning of semi-volatile cations, NH3/NH4+, and the liquid/solid partitioning of non-volatile mineral cations, particularly Ca2+, Mg2+, and K+, overall control the gas-liquid-solid aerosol equilibrium partitioning of reactive nitrogen compounds. For the NO3- and NH4+ equilibrium, our recent developments have focused on EQSAM4Clim, which has been recently integrated into the IFS as a computationally efficient means of describing aerosol pH in a global modeling system.

EQSAM4Clim is used in the IFS to estimate gas-liquid-solid partitioning and the aerosol associated liquid water content, which is subsequently used to estimate the associated aerosol, cloud and rain acidity. The aerosol, cloud and rain pH is computed by considering the liquid water (H2O) content in the respective liquid water phase using either the aerosol associated water computed by EQSAM4clim, and if present, the cloud and/or rain water of the IFS. The pH is coupled to the aqueous phase chemistry in IFS(CB05) and in the wet deposition of SO2 and NH3, which in-turn affects the aerosol composition through changes in the SO2/SO42-, NH3/NH4+and HNO3/NO3- partitioning, the aerosol associated liquid water content and solution pH.

Here we present first results of the of the impact of improved aerosol acidity in the solution (aerosol/cloud/rain water) on PM2.5 forecasts simulated in the IFS which are subject to gas-particle partitioning. In particular, the NH4+, NO3- and SO42- concentrations have been compared against observational datasets at the surface, showing promising improvements as a direct result of the new pH computations. When coupling the EQSAMClim pH into the aqueous phase chemistry routine, the surface concentrations of SO42- and the SO2 + SO42- wet deposition fluxes are improved over most of Europe, but degraded over parts of US. The relative impact of the improved pH appears generally small as compared to other related changes such as updates in aqueous chemistry rates. In the pH coupling, the aqueous chemistry component dominates the impact on the wet deposition of SO2/NH3. All of these results are highly dependent on the emissions input (SO2/NOx/NH3). 

How to cite: Metzger, S., Rémy, S., Huijnen, V., Williams, J., Chabrillat, S., Bingen, C., and Flemming, J.: Impact of pH computation from EQSAM4Clim on inorganic aerosols in the CAMS system, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16085, https://doi.org/10.5194/egusphere-egu23-16085, 2023.

EGU23-17426 | PICO | AS1.6

Extending and Improving JEDI-based Global Aerosol Data Assimilation System for UFS-Aerosols 

Bo Huang, Mariusz Pagowski, Cory Martin, Andrew Tangborn, Maryam Abdi-Oskouei, Jérôme E. Barré, Shobha Kondragunta, Georg Grell, and Gregory Frost

A global aerosol data assimilation (DA) system based on the ensemble-variational (EnVar) application in the Joint Efforts for Data assimilation Integration (JEDI) was recently developed for the Global Ensemble Forecast System - Aerosols (GEFS-Aerosols) in operations at NOAA/NWS/NCEP. The aerosol optical depth (AOD) retrievals at 550 nm are assimilated to improve the GEFS-Aerosols initial conditions and its subsequent forecasts. To account for aerosol emission uncertainty in the ensemble forecasts and thus enhance AOD assimilation, a stochastically-perturbed emission (SPE) approach was implemented in the Common Community Physics Package (CCPP)-based GEFS-Aerosols. The performance of this JEDI-based EnVar aerosol DA system has been evaluated using the CCPP-based GEFS-Aerosols in the near-real time (NRT) experiments at NOAA/OAR/GSL and the global aerosol reanalysis products that  assimilate 550 nm AOD retrievals from the the Visible Infrared Imaging Radiometer Suite (VIIRS) instruments and the Moderate Resolution Imaging Spectroradiometer (MODIS) instruments, respectively. The NRT experiment results are displayed on the GSL website (https://ruc.noaa.gov/projects/nrt/Aerosol-DA/). Both the NRT experiment results and global aerosol reanalyses demonstrate that compared to the six-hour forecasts without AOD assimilation, the analyses and subsequent six-hour forecasts resulting from AOD assimilation show significantly improved agreement with AOD retrievals from VIIRS, MODIS and the Aerosol Robotic NETwork (AERONET), and AOD analyses/reanalyses from NASA and ECMWF. Although AOD retrievals, due to their column-integral nature, provide limited information regarding aerosol compositions and vertical profiles, AOD assimilation in our experiments generally contributes to improved aerosol analyses and forecasts verified against those from NASA and ECMWF.  

One of the ongoing Unified Forecast System (UFS)-Research to Operations (R2O) efforts aims to integrate and improve aerosol prediction within UFS (hereafter referred to as UFS-Aerosols). UFS-Aerosols will eventually replace the standalone GEFS-Aerosols for operations at NOAA/NWS/NCEP. Compared to GEFS-Aerosols, UFS-Aerosols is coupled with NASA's second-generation Goddard Chemistry Aerosol Radiation and Transport (GOCART) model including additional nitrate aerosol species, adopts improved biomass burning and dust emissions, and allows for aerosol-radiation interactions. Motivated by the promising results of assimilating AOD for GEFS-Aerosols and to advance aerosol assimilation and prediction in UFS, we are extending and improving this JEDI-based EnVar aerosol DA system for UFS-Aerosols. It requires further development of AOD forward operator, its tangent linear and adjoint models in JEDI’s Unified Forward Operator (UFO) to accommodate additional nitrate aerosol species in UFS-Aerosols. Enhancements to this DA system for UFS-Aerosols include implementing SPE within UFS-Aerosols to improve background ensemble and implementing assimilation of log-transformed AOD within JEDI to better satisfy the Gaussian assumptions in the DA update. To evaluate these new developments for UFS-Aerosols, cycled DA experiments will be performed to assimilate 550 nm AOD retrievals from VIIRS instruments on board NOAA’s satellites, and verified against various aerosol observations and reanalyses. Results will be presented.

How to cite: Huang, B., Pagowski, M., Martin, C., Tangborn, A., Abdi-Oskouei, M., E. Barré, J., Kondragunta, S., Grell, G., and Frost, G.: Extending and Improving JEDI-based Global Aerosol Data Assimilation System for UFS-Aerosols, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17426, https://doi.org/10.5194/egusphere-egu23-17426, 2023.

Including prognostic atmospheric composition (AC) simulations in numerical weather predication or climate modelling application to exploit AC – weather feedbacks is often prohibited by the high computational cost of adding complex AC simulation to the weather or climate model.  There are in principle two approaches to solve this problem: (i) drastically reduce the complexity of the aerosol and chemistry simulations in the weather model, or (ii)  safe cost by reducing the spatial resolution of the model components simulating the AC processes and implement a coupling mechanism.  

At ECMWF a dual configuration forecast (dcfc) approach for the of the Integrated Forecasting System (IFS) has been developed based on the infrastructure for Object-Oriented Prediction System (OOPS). It enables the coupled simulation of a high-resolution application and a low-resolution application of the IFS and a coupling mechanism. The low-resolution model instance simulates the aerosol and chemistry-processes as activated for the operational AC forecasts by the Copernicus Atmosphere Monitoring Service (CAMS)  

We show first scientific results of this dual configuration forecast (dcfc) for a sever dust storm event in Europe in March 2022. We will discuss to what extent and at what computational cost the dcfc application can forecast the meteorological impact of the dust on radiation and 2m temperatures. We will compare the dcfc result to the more expensive integrated IFS-CAMS configuration as well as to NWP forecast using the aerosol climatology as currently applied in the ECMWF operational weather forecasts.  

How to cite: Flemming, J. and Hamrud, M.: A multiple gird approach for atmospheric composition - aware NWP forecasts with the ECMWF forecast system, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17501, https://doi.org/10.5194/egusphere-egu23-17501, 2023.

EGU23-17561 | ECS | PICO | AS1.6 | Highlight

High-resolution dynamical downscaling of present and future air quality over the South Asia-Cordex domain with a focus on the megacity Delhi, India 

Ummugulsum Alyuz, Ranjeet Sokhi, Kester Momoh, Vikas Singh, Chandra Venkataraman, Arushi Sharma, Ganesh Gupta, Kushal Tibrewal, Ravindra Khaiwal, Suman Mor, and Gufran Beig and the PROMOTE Team

Through a NERC/MOES funded project, PROMOTE, analysis based on WRF and CMAQ models has been conducted to understand the impact of road transport emissions on air quality over Delhi. NCEP/FNL 1 data was used to drive WRF with four nested domains over India with resolutions of 45km, 15 km, 5 km, and 1.6 km for 2018. EDGAR v5.0 emission inventory (for 2015) 2 and Cam-Chem initial and boundary condition data 3 were used to drive the CMAQ model. In the baseline runs, all domains were considered without any change in emissions, while in Scenario 1, road transport sector was removed in the third domain (5km) covering Delhi region. Model performance for NOx, NO2, PM10, PM2.5 and O3 was evaluated with available observations, recognising that air quality and meteorological datasets were limited for the period analysed. In the later part of the study, OSCAR model 4 was used to predict the high-resolution air quality over Delhi and estimate the contributions from road transport emissions. Relative contributions to Delhi's air quality from local and regional long range transport sources are discussed. 

As part of a NERC funded COP26 project on Climate Adaptation for India, an overarching goal of this study is to quantify how air quality changes in South Asia in a changing climate under SSP245 (middle-of-the-road scenario) 5. A dynamical downscaling process was implemented and bias-corrected Coupled Model Intercomparison Project Phase 6 (CMIP6) data 6 was used to drive Weather Research and Forecasting (WRF) model simulations. Simulations have been conducted for the South Asia-Cordex domain for 2015 (representative of 2011-2020 years) and 2050 (representative of 2046-2055 years) with a 27 km grid resolution. The Community Multiscale Air Quality (CMAQ) model was driven with an average of ten years meteorology with future land use land cover, initial and boundary conditions, and future emissions 7 for India. To assess the impact of averaged meteorology on the CMAQ performance, the CMAQ model was run with both ten years' averaged meteorology around 2015 (2011-2020) and only 2015 meteorology.

Although averaging ten years around the desired year suppresses the diurnal variations, it provides an indication of monthly changes in climate and air quality variables. Under the selected SSP245 scenario, the CMAQ model predicted monthly means of PM2.5 anomalies (2050-2015) range over India between 8 to 41 μg/m3. Significant change is PM2.5, PM10, NOx, and O3 anomalies, especially in the urban regions of India, such as Delhi, before and after the Monsoon months (June to October) have been observed.

Financial Support: We acknowledge funding from NERC/MOES (Reference: NE/P016391/1) for the PROMOTE project and NERC funding (Reference: 2021COPA&R48Sokhi) for the COP26 Improving adaptation strategies for climate extremes and air pollution affecting India project.

References

1 NCEP/NOAA/U.S. 2015,  https://doi.org/10.5065/D65Q4T4Z.

2 Crippa M. et al. (2019): http://data.europa.eu/89h/377801af-b094-4943-8fdc-f79a7c0c2d19

3 Buchholz, R. R. et al, (2019). https://doi.org/10.5065/NMP7-EP60

Singh V, et al. (2020) Environmental Pollution, 257, 113623

5 van Vuuren, D.P. et al. (2011). Climatic Change 109, 5. https://doi.org/10.1007/s10584-011-0148-z

6 Xu, Z. et al.  (2021). Sci Data 8, 293. https://doi.org/10.1038/s41597-021-01079-3

7 SMoG-India v1 2015 and 2050 emissions dataset, NERC project.

How to cite: Alyuz, U., Sokhi, R., Momoh, K., Singh, V., Venkataraman, C., Sharma, A., Gupta, G., Tibrewal, K., Khaiwal, R., Mor, S., and Beig, G. and the PROMOTE Team: High-resolution dynamical downscaling of present and future air quality over the South Asia-Cordex domain with a focus on the megacity Delhi, India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17561, https://doi.org/10.5194/egusphere-egu23-17561, 2023.

EGU23-1439 | ECS | Posters on site | AS1.7

Using MPAS model to forecast the Convectively Induced Turbulence 

Haoming Chen, Xiaoming Shi, Chiristy Yan-yu Leung, Ping Cheung, and St Chan

Convectively induced turbulence (CIT) is a serious aviation hazard and it is challenging to forecast the CIT in the region near convection. Previous studies used reginal model with high resolution or global model with low resolution and selected empirical indices to diagnose the turbulence. In this study, we used The Model for Prediction Across Scales (MPAS) to simulate some cases of CIT reported near Hong Kong. MPAS allows us to use convection-permitting resolution in the interested area while including the global-large scale circulation with coarser resolutions in other regions. The eddy dissipation rate (EDR) is computed to diagnose the potential occurrence of CIT. We compared three methods for calculating EDR from the resolved flow in the MPAS, the first one based on second order structure function, the second one based on Scale-Similarity in Large Eddy Simulation (LES) and the third is Near Cloud Turbulence (NCT) diagnostics by using Convective Gravity Wave Drag. Comparing with the NOAA Graphical Turbulence Guidance (GTG) product and flight data suggests that computing EDR with Scale-Similarity is more effective and accurate than second order structure function and NCT diagnostics. Resolution is also an important factor in forecast, we tested the method in mesh with different resolutions but similar distributions, the results from low resolution simulations can generate a useful turbulence pattern forecast, but the intensity is weak, highlighting the value of high resolution simulations that can resolve convection. We evaluated the sensitivity to several model physics and numeric options in simulations. Those variations can change the EDR prediction by influencing the intensity and the life cycle of the convection. No particular scheme produces systematically more intense turbulence than others, suggesting varying model physics captures some stochasticity of convection. Compared with flight records of EDR along the flight routes, MPAS could produce in three out of five cases showing maximum EDR is close to the observed intensity of turbulence (EDR>0.4). However, in the other two cases, the results are not satisfactory mainly because of significant location biases of the predicted convection. We also add initial condition perturbation-based large ensemble in one case and find it possible to improve the prediction of the failed cases by influencing the position of the convection. Further work should be conducted to prioritize the ensemble members since only a few members can capture the turbulence and doing the average will erase them easily.

How to cite: Chen, H., Shi, X., Leung, C. Y., Cheung, P., and Chan, S.: Using MPAS model to forecast the Convectively Induced Turbulence, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1439, https://doi.org/10.5194/egusphere-egu23-1439, 2023.

EGU23-2556 | ECS | Orals | AS1.7

SST-driven changes in cloud radiative heating in RCEMIP models and observations 

Blaž Gasparini, Aiko Voigt, Giulio Mandorli, and Claudia Stubenrauch

The interactions of ice particles with radiative fluxes in tropical high clouds substantially alter the heating structure within the atmosphere, also known as cloud radiative heating (CRH). CRH influences the upper-tropospheric temperature structure and thus modulates the strength and position of tropical and extratropical circulations. Moreover, it influences the life cycle of tropical high clouds through longwave destabilization of the cloud layer and lifting of clouds by absorption of both shortwave and longwave radiation by ice crystals. A possible change of CRH, for example, due to global warming, can substantially alter the tropical climate.Despite a large body of work that has explored interactions between clouds and radiation, responses of CRH to global warming remain largely unknown. We therefore use idealized SAM cloud-resolving model simulations, the RCEMIP multimodel dataset, and a 15-year-long satellite-derived CRH dataset to explore changes in CRH under different sea surface temperatures.

To a first approximation, the upper tropospheric CRH shifts nearly isothermally to a higher altitude level following a surface warming. In addition, upper-tropospheric CRH in 27 of the 32 analyzed models increase by 0.5 to 10%/K, with a mean value of about 3%/K. Interestingly, the CRH increases despite decreases in upper tropospheric ice water content and cloud fraction. The increase in CRH can be to a large extent explained by an increase in atmospheric transmissivity due to a 2-3 km vertical shift of high clouds, in an environment with decreased air density. Similarly, all models simulate an increase in the upper tropospheric clear-sky radiative cooling in warmer conditions.

Additionally, the CRH response to surface warming can be largely predicted by assuming a nearly isothermal vertical shift of upper tropospheric CRH profiles (as per the fixed anvil temperature hypothesis) following a warmer moist adiabat and by considering the increase in CRH magnitude due to changes in atmospheric density. Therefore, if we know the CRH of a reference climate state, we can, to a good approximation, estimate its response to surface warming.

The modeled CRH vertical shift and increase are confirmed by a 15-year-long satellite-derived tropical CRH dataset. The years with the highest SSTs lead to the most positive CRH that is shifted to higher levels, similarly to what is simulated by RCEMIP models.

How to cite: Gasparini, B., Voigt, A., Mandorli, G., and Stubenrauch, C.: SST-driven changes in cloud radiative heating in RCEMIP models and observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2556, https://doi.org/10.5194/egusphere-egu23-2556, 2023.

The vertical structure of large-scale tropical circulations is determined by their complex coupling with both deep and shallow convection. This is reflected in our theoretical frameworks for understanding the tropical precipitation distribution, which consist of “deep” theories that focus on overturning circulations that extend throughout the depth of the troposphere and “shallow” theories that focus on low-level convergence driven by boundary-layer pressure gradients. While both types of theories suggest links between low-level thermodynamic fields and the precipitation distribution, shallow theories highlight the importance of the distribution of surface temperature, while deep theories additionally highlight the importance of the low-level humidity. 

Here we use idealised cloud-permitting simulations to elucidate the physical factors that control the vertical structure of tropical circulations. We first demonstrate how the influence of convective entrainment on the lapse rate can act to change the vertical structure of deep tropical circulations, with implications for the behaviour of precipitation in the current and future climate. We further investigate the interaction between deep and shallow tropical circulations  by simulating an idealised overturning circulation over varying surface conditions. By independently varying the sea-surface temperature and moisture availability, the low-level temperature and moisture distributions are manipulated such that the predictions of “deep" and “shallow" theories of the circulation may be distinguished. The results provide insight into the relative roles of oceanic SST gradients and land-ocean contrasts in determining the climatological precipitation distribution in the tropics.

How to cite: Singh, M.: Shallow and Deep Circulations in the Tropical Atmosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3078, https://doi.org/10.5194/egusphere-egu23-3078, 2023.

Radiative-convective equilibrium is the simplest possible way to phrase many questions about a deep-convecting atmosphere and is accessible by a wide range of model types. The radiative-convective equilibrium project (RCEMIP) provides a common configuration, but reveals a large spread in the simulated climate across models, including profiles of temperature and relative humidity. Here we use simple models and theory to understand the intermodel spread in CAPE, relative humidity, and their responses to warming.

Across the RCEMIP ensemble, temperature profiles are systematically cooler than a moist adiabat, consistent with theory that they are set by dilute ascent. As horizontal grid spacing is reduced in models with explicit convection from 1 km to 200 m, CAPE and relative humidity increase. Across all models, CAPE increases with warming at a rate (14-19%/K) greater than that expected from the Clausius-Clapeyron relation. We find that there is higher CAPE (greater instability) in models that are on average moister in the mid-troposphere, which is consistent with the simple plume model of Romps (2016) in which both instability and relative humidity depend on entrainment and precipitation efficiency. The sign of the relationship suggests that differences in entrainment drive the intermodel spread. This relationship is true across both models with explicit and parameterized convection.

To more explicitly evaluate the drivers of the intermodel spread, we use the Romps (2016) model to diagnose theory-implied values of entrainment and precipitation efficiency given the simulated values of CAPE and relative humidity. We then decompose the the variability across models in CAPE and relative humidity (and their responses to warming) into contributions from entrainment, precipitation efficiency, and the depth of the convecting layer. Targeted microphysics parameter perturbation experiments with an individual cloud-resolving model in which precipitation efficiency is varied and explicitly diagnosed provide proof of concept for this decomposition technique. 

How to cite: Wing, A. and Singh, M.: Control of Tropical Stability and Relative Humidity in Radiative-Convective Equilibrium Simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3532, https://doi.org/10.5194/egusphere-egu23-3532, 2023.

The initiation of deep convection in a diurnal cycle is still one of the most important uncertainties in a climate numerical model. This is partially due to our poor understanding of the physical mechanisms leading to the transition from shallow to deep convection. In this work, we discuss the role of shallow cumulus clouds in the initiation of deep convection. By using a simple entraining plume model, we show that the interaction between an active and a passive shallow cumulus helps the former to reach higher altitudes and, in the right conditions, may initiate deep convection. It is also shown that the organization of passive and active clouds due to the formation of cold pools may act as a positive feedback. Furthermore, based on the proposed mechanism, a stochastic triggering function is derived, which can be implemented in climate models. As an important feature, the stochastic function is scale-aware, which makes it suitable for simulations at the gray-zone.

How to cite: Vraciu, C.-V.: The role of passive shallow cumuli in the transition from shallow to deep convection, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3561, https://doi.org/10.5194/egusphere-egu23-3561, 2023.

EGU23-4079 | ECS | Orals | AS1.7

Identifying the Deep-inflow Mixing Features in Orographically Locked Diurnal Convection 

Yu-Hung Chang, Wei-Ting Chen, Chien-Ming Wu, Yi-Hung Kuo, and J. David Neelin

This study focuses on the deep-inflow mixing features of the orographically locked diurnal convection, involving interactions between local circulation and the thermodynamic environment of the convection. Under the weak synoptic weather regime, orographically locked diurnal convection is a typical summertime phenomenon in Taiwan, a tropical island in the Asian monsoon region. Numerical simulations are carried out using the vector vorticity equation model with high-resolution Taiwan topography (TaiwanVVM), which can appropriately simulate the characteristics of diurnal convection and the evolution of boundary layer and local circulation. The semi-realistic approach, simplified by observed soundings as the uniform initial condition over the entire domain, emphasizes the decisive environmental factors that modulate the development of convection, representing the variability of the background environment by the ensembles. The analyses by the deep-inflow mixing framework, including the locally-derived convective structures and the upstream moist static energy (MSE) transport, improve the understanding of the interactive physical processes in the boundary layer development and local circulation evolution of orographically locked diurnal convection over complex topography. The convective structures of the deep-inflow mixing, increasing vertical velocity and convective mass flux with height through a deep lower-tropospheric inflow layer, are found in strong convective updraft columns within heavily-precipitating systems over precipitation hotspots. While the topography constrains the location of the convection, enhanced convective development is associated with higher upstream MSE transport through this deep-inflow layer via local circulation, augmenting the rain rate by 35% in precipitation hotspots. The results highlight the importance of non-local dynamical entrainment of the deep-inflow, transporting MSE via local circulation to supply the growth of orographically locked diurnal convection. Thus, the deep-inflow mixing framework can serve as the theoretical basis for describing the orographic locking feature of diurnal convection over complex topography. Guided by the simulations, the Storm Tracker mini-radiosondes are released upstream of the precipitation hotspot, targeting observations within the most common deep-inflow path. Initial field measurements support the presence of high MSE transport within the deep-inflow layer when organized convection occurs at the precipitation hotspot.

How to cite: Chang, Y.-H., Chen, W.-T., Wu, C.-M., Kuo, Y.-H., and Neelin, J. D.: Identifying the Deep-inflow Mixing Features in Orographically Locked Diurnal Convection, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4079, https://doi.org/10.5194/egusphere-egu23-4079, 2023.

EGU23-4150 | Orals | AS1.7

New GSRM global warming simulations and active sensors reveal robust changes of tropical convergence zones in cloud ice space 

Maximilien Bolot, Lucas Harris, Kai-Yuan Cheng, Peter Blossey, Christopher Bretherton, Spencer Clark, Alex Kaltenbaugh, Timothy Merlis, Linjiong Zhou, and Stephan Fueglistaler

Change of the intertropical convergence zone (ITCZ) with global warming has important consequences for the regulation of the tropical climate and for future precipitation projections. Most of the volume of the ITCZ is filled with ice associated with convective anvils, which opens the perspective of using the response of ice clouds to study changes of the tropical convergence zones with global warming. Past studies have shown a decrease of tropical high-cloud fraction with surface warming, whereby the response of anvil clouds is used to interpret the response of ice clouds as a whole. However, tropical clouds organize over a very wide range of scales, meaning that the response of ice clouds is more complex. In particular, precipitating deep convection may represent a small volume of total cloudiness, but it concentrates most of the ascending motion in the tropics and is therefore of crucial importance for the dynamics. Here we show how the high resolution in next generation convection-resolving climate models and in observations can be leveraged to directly measure the response of precipitating deep convection with surface warming in the ice signal. For this purpose, we use the first year-long simulations of global warming ever performed with a Global Storm Resolving Model (GSRM) at 3 km resolution. These simulations use the eXperimental System for High-resolution prediction on Earth-to-Local Domains (X-SHiELD), developed at the Geophysical Fluid Dynamics Laboratory (GFDL). By tracking the response of tropical clouds to surface warming from the response of ice water path (IWP), the vertical integral of ice mixing ratio, we show that the response of precipitating deep convection can be identified at high resolution and that this response, marked by an increase in frequency of very deep convective cores and a decrease in frequency of more moderate convection, is robust in model and active sensor observations. We discuss this result and show how it promotes a simple view of the changes of tropical convergence zones in ice-based coordinates.

How to cite: Bolot, M., Harris, L., Cheng, K.-Y., Blossey, P., Bretherton, C., Clark, S., Kaltenbaugh, A., Merlis, T., Zhou, L., and Fueglistaler, S.: New GSRM global warming simulations and active sensors reveal robust changes of tropical convergence zones in cloud ice space, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4150, https://doi.org/10.5194/egusphere-egu23-4150, 2023.

EGU23-4711 | Posters virtual | AS1.7

Sensitivity of projected storm track and jet latitude changes to the parameterization of convection: implications for mechanisms of the future poleward shift 

Ian White, Chaim Garfinkel, Benny Keller, Orli Lachmy, Ed Gerber, and Martin Jucker

While a poleward shift of the jet stream and storm track in response to increased greenhouse gases appears to be robust, the magnitude of this change
is uncertain and differs across models, and the mechanisms for this change are poorly constrained. An intermediate complexity GCM is used to explore
the factors governing the magnitude of the poleward shift and the mechanisms involved. The degree to which parameterized subgrid-scale convection is inhibited has a leading-order effect on the poleward shift, with a simulation with more convection (and less large-scale precipitation) simulating a significantly weaker shift, and eventually no shift at all if convection is strongly preferred over large-scale precipitation. Many of the mechanisms that have been proposed to lead to the poleward shift are present in all simulations (even those with no poleward shift), and hence we can conclude that these mechanisms are not of leading-order significance for the poleward shift in any of the simulations. In contrast, the thermodynamic budget is able to diagnose the reason the jet and storm track shift differs among the simulations, and helps identify midlatitude latent heat release as the crucial differentiator. These results have implications for intermodel spread in the jet, hydrological cycle, and storm track response to increased greenhouse gases in intermodel comparison projects.

How to cite: White, I., Garfinkel, C., Keller, B., Lachmy, O., Gerber, E., and Jucker, M.: Sensitivity of projected storm track and jet latitude changes to the parameterization of convection: implications for mechanisms of the future poleward shift, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4711, https://doi.org/10.5194/egusphere-egu23-4711, 2023.

EGU23-4968 | ECS | Posters on site | AS1.7

Evaluating Memory Properties in Convection Schemes Using Idealised Tests 

Yi Ling Hwong, Maxime Colin, Philipp Aglas, Caroline Muller, and Steven Sherwood

Two structural assumptions are frequently employed in convective parameterisation: the diagnostic and quasi-equilibrium assumptions. The former assumes an instantaneous relationship between the large-scale environment (“macrostate”) and subgrid-scale convective activity, while the latter postulates that convective processes are almost in equilibrium with slowly evolving large-scale forcing at all times. Both assumptions do not take into account the role of convective memory (“microstate” memory), which is defined as the dependence of convection on its own history. Here, we present the memory behaviour of three convection schemes by comparing their responses in two idealised RCE experiments in single-column models (SCMs) to those of a cloud-resolving model (CRM). Three main findings from these tests will be discussed. First, when the large-scale environment is held constant (“FixMacro”), precipitation remains invariant in time with the Zhang-McFarlane scheme, confirming that the scheme does not parameterise convective memory and is fully diagnostic. The org scheme (Mapes & Neale, 2011) displays similar behaviour to the CRM in that precipitation increases in the first moments after FixMacro starts, with larger entrainment rates associated with slower growth. However, its logarithmic growth shape differs from that of the CRM, which displays exponential growth, and can be explained using the scheme’s governing equations. Second, when the prognostic convective memory variable is set to zero at one time step (essentially wiping out microstate memory), the org scheme displays remarkably similar behaviour to the CRM, with precipitation dropping to zero and then recovering to its RCE value over a recovery time scale tmem. In comparison, precipitation in the LMDZ cold pool scheme (Grandpeix & Lafore, 2010) responds in the opposite direction: it grows and then falls back to its RCE value. Finally, the mean and temporal variance of the org variable were found to correlate strongly with memory strength (tmem), indicating that org has captured important aspects of convective memory. Overall, our results indicate that the org and LMDZ cold pool schemes partially, but do not fully capture CRM memory behaviour and are limited by their structural assumptions. They also demonstrate the usefulness of our simple idealised experiments to probe the memory behaviour of convection schemes. 

How to cite: Hwong, Y. L., Colin, M., Aglas, P., Muller, C., and Sherwood, S.: Evaluating Memory Properties in Convection Schemes Using Idealised Tests, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4968, https://doi.org/10.5194/egusphere-egu23-4968, 2023.

EGU23-5898 | ECS | Posters on site | AS1.7

On the organization of passive shallow cumulus clouds 

Andrei Marin and Cristian-Valer Vraciu

The shallow cumulus clouds are ubiquitous in the atmosphere, populating a large part of the subtropical oceans. They may play a strong climate feedback due to their cooling effect on the Earth atmosphere. As a result, a large number of studies investigated the organization of cumulus clouds and their interaction with the climate. However, the organization of passive shallow clouds and their impact on the atmospheric convection and climate change received very limited attention. In this work, we perform a series of large eddy simulations in order to investigate how the organization and the total cloud cover depends on the relative humidity of the environment. We show that although the active cumulus clouds only show a weak correlation with the relative humidity, the passive clouds are very sensitive to it. We show thus that the cloud cover of the shallow cumuli is very sensitive to the relative humidity which could be very important in the context of the climate change. Furthermore, we formulate a conceptual picture to explain the organization of passive shallow cumulus clouds.

How to cite: Marin, A. and Vraciu, C.-V.: On the organization of passive shallow cumulus clouds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5898, https://doi.org/10.5194/egusphere-egu23-5898, 2023.

EGU23-6933 | ECS | Orals | AS1.7

Investigating Convective Self-Aggregation in the Transition from Land to Sea 

Irene L. Kruse and Jan O. Haerter

Within the atmospheric modelling community, a large focus in recent years has been on the concept of Convective Self-Aggregation (CSA): In an environment of radiative convective equilibrium, with homogeneous initial conditions and a constant-temperature tropical sea surface, convection can spontaneously aggregate into domain-wide patterns of persistent dry areas and constrained rainy areas over a temporal timescale of weeks to months. CSA, albeit still a modeling paradigm, could reveal the mechanisms behind some of the convective organization observed in the tropics.

This process of forming domain-wide structure can be accelerated to the order of days by imposing oscillating surface temperatures with a large enough amplitude [1]. The ‘diurnally aggregated’ cloud field is similar to CSA as it also constrains the surface rain field to certain parts of the domain. Further, pattern formation was found to initiate first as persistent dry patches in the uppermost layers of the simulated atmosphere. The dry patches subsequently penetrate through to the subcloud layer [2].

In this work we investigate how diurnal surface temperature amplitudes, typical of tropical land, affect the formation of persistent dry patches and the spatio-temporal extent of the emergent mesoscale convective systems. We run a set of cloud resolving simulations initialized with typical profiles of temperature and humidity. We impose a large-amplitude diurnally oscillating surface temperature, which we then set to constant at different times, to see the effect on the diurnally aggregated cloud field. We present the results of this study, which show a strong dependence on the degree of aggregation over ‘land’, in determining the aggregation over ‘sea’, and a form of hysteresis arises.

 

1. Haerter, Jan O., Bettina Meyer, and Silas Boye Nissen. ‘Diurnal Self-Aggregation’. Npj Climate and Atmospheric Science 3, no. 1 (30 July 2020): 1–11. https://doi.org/10.1038/s41612-020-00132-z.
2. Jensen, Gorm G., Romain Fiévet, and Jan O. Haerter. ‘The Diurnal Path to Persistent Convective Self-Aggregation’. Journal of Advances in Modeling Earth Systems 14, no. 5 (2022): e2021MS002923. https://doi.org/10.1029/2021MS002923.

 

How to cite: Kruse, I. L. and Haerter, J. O.: Investigating Convective Self-Aggregation in the Transition from Land to Sea, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6933, https://doi.org/10.5194/egusphere-egu23-6933, 2023.

The difficulty to accurately represent atmospheric convection in numerical weather forecasts contributes to persistent biases in weather and climate simulations – particularly tropical precipitation. Convection-permitting global forecasts are an improvement on global models with parametrized convection schemes, however it is not yet clear whether they improve forecast skill to match or improve upon the current approach of nesting a convection-permitting high-resolution regional model inside a global model with parameterized convection. This is far less computationally expensive than running a global convection-permitting model.

To test this, the Met Office is coordinating a UK K-scale project nesting high resolution (2.2 km) limited area models (LAMs) within global models that have between 5 and 10 km grid resolution. We compare these nested regional models with two different global simulations, run with parameterised and explicit convection science configurations. The 2.2 km resolution LAMs encompass a variety of domains focussing on both tropical land and ocean regions.

Our current work seeks to investigate if and where we see differences in model evolution between the high-resolution nested LAM approach and the explicit convection global driving model.  We focus on an active MJO event in January 2018 where enhanced convection propagated across the Indian Ocean and impacted the Maritime continent. For high-impact events such as this, do we see a marked change in the model forecast when explicitly simulating convection globally rather than in a regional limited area model (as currently used in operational forecasts)? Further, are differences between the global convection permitting and LAM forecasts more pronounced over ocean-dominated regions where the amplitude of the diurnal cycle of convection is smaller?

This talk will summarise our findings in the context of the wider K-scale project, evaluating how our recent work contributes to the development of more accurate weather forecasts.

How to cite: Macholl, J., Jones, R., and Lewis, H.: Globally modelling explicit convection: how does it compare with the nested limited area model approach at high horizontal resolutions?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7082, https://doi.org/10.5194/egusphere-egu23-7082, 2023.

EGU23-7224 | Posters on site | AS1.7

Parametrization of dust storms in the Sahel by cold pools 

Mamadou Lamine Thiam, Frédéric Hourdin, Jean-Yves Grandpeix, Catherine Rio, and Amadou Thierno Gaye

The cold pools, created below cumulonimbus from the evaporation of precipitation, generate the strong winds responsible for the large dust storms called “haboobs” which appear in the Sahel in summer. Most global climate models do not take into account these types of dust emissions due to lack of parameterization of cold pools and associated gusts (Marsham et al. 2011 ; Pantillon et al. 2015).

The introduction of a parameterization of cold pools in the LMDZ climate model has improved the representation of convection, and in particular of the diurnal cycle of continental precipitation in the tropics (Rio et al. 2009). The aim of this work is to develop a parameterization of gusts related to cold pools in order to take into account ‘‘hoobobs’’ in LMDZ model. To do this, we use Large Eddy Simulations (LES) performed on an oceanic domain and in Radiative-Convective Equilibrium (RCE) mode. We use a LES of an oceanic RCE case, easier to analyze because the temperatures are uniform on the surface and therefore the cold pools easier to detect. Before developing a gust parameterization, we evaluate the cold pools parameterization in LMDZ on this RCE case, which has never been done so far. If the comparison confirms the relevance of the scheme and its qualitative match to the LES behavior, is also led to substantial improvements and adjustments to this scheme. Next, we analyze the wind distributions in the LES in order to construct a parametrization based on a probability distibution function of the subgrid scale distribution of the wind which will allow us to take into account the effect of gusts on dust storms. The parametrization relates the moments of the distribution to large-scale wind speed, the spreading speed of the cold pools and the surface fraction covered by the latter. In the following, we will test the parametrization on the LMDZ model by focusing on dust storms in the Sahel during the rainy season.

How to cite: Thiam, M. L., Hourdin, F., Grandpeix, J.-Y., Rio, C., and Gaye, A. T.: Parametrization of dust storms in the Sahel by cold pools, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7224, https://doi.org/10.5194/egusphere-egu23-7224, 2023.

EGU23-9002 | ECS | Posters on site | AS1.7

A Lagrangian View to the Evolution of Convective Updrafts 

Thomas Hutton, John Thuburn, and Robert Beare

The representation of cumulus convection is a known source of uncertainty within current weather and climate models. Where model resolution is too coarse to accurately resolve convection, parameterisations are required to estimate the impact of small-scale convective processes. High resolution large eddy simulations (LES) can be used to diagnose many aspects of convective processes, such as heat and momentum budgets and rates of entrainment. However, LES is computationally expensive, making it impossible to use within operational models. This study aims to bridge the gap between current coarser models and LES by developing a stochastic Lagrangian model to represent an ensemble of air parcels. Vertical velocity, liquid water potential temperature, and total specific humidity are predicted following the ensemble of parcels. The random motions associated with turbulence are represented by a stochastic term within the w-tendency equation. The mean fields which the parcels interact with are defined by an ensemble average of nearby parcels. Several fixers have been developed to ensure that conservation properties are respected. At the current stage of development, the model can represent dry convective boundary layer and shallow convection cases. A theoretical study of the stochastic differential equations is useful to verify the self-consistency of the model and also as a tool for calibrating various parameters within the model. A key question for this project is how well the stochastic parcel model can replicate the statistics of LES results. This will act as a measure of the model’s success, allowing for a deeper understanding on accurately modelling convective processes. Due to the Lagrangian nature of the model, analysis can be conducted upon how the parcels’ characteristics change over time as the parcels experience smaller-scale convective processes such as entrainment. Ultimately, results from this model may yield better understandings of small-scale convective processes. This can create potential for improvements to parameterisations in operational models, reducing model uncertainty generated by convective processes.

How to cite: Hutton, T., Thuburn, J., and Beare, R.: A Lagrangian View to the Evolution of Convective Updrafts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9002, https://doi.org/10.5194/egusphere-egu23-9002, 2023.

The intrinsic failure of eddy-diffusion parameterizations in representing upward transport of heat in the convective boundary layer, recognized since the 70s, has lead to various propositions of parameterizations like counter-gradient terms and third order closures to account for the asymmetry of the vertical transport. An approach that is now well recognized consists in combining a mass flux parameterization of the organized structures of the convective boundary layer with a local TKE closure for small scale turbulence. The idea traces back to a proposition by Chatfield and Brost (1987) and is since often referred to as the Eddy Diffusion Mass Flux (EDMF) approach. The “thermal plume model” developed for LMDZ was the first EDMF scheme published and tested in a climate model (Hourdin et al., 2002). It was first introduced in the LMDZ5B atmospheric component of the IPSL model for CMIP5. However, this first version suffered from youth problems. It is only for CMIP6A, about 20 years after the development of the parameterization, that a first satisfactory version of the model was delivered. Through years, and more often with this last version, the key role of the representation of shallow convection on many component of the system has been realized: 1) the ventilation of air by the subsiding air around thermal plumes dries the surface, reinforcing the near surface evaporation. Representing this convection correctly both over trade winds and subsiding regions in the tropics, together with the associated cumulus and stratocumulus clouds, is one of the key for the reduction of the East Tropical Ocean warm bias; 2) the preconditioning of the deep convection by a phase of shallow convection is a key for a correct representation of the phasing of the diurnal cycle of convective rainfall over continents; 3) the strong diurnal cycle of the convective boundary layer in desert areas is essential to well represent the maximum of near surface wind in the morning, responsible for a maximum of dust emission, when the momentum of the nocturnal low level jet is brought suddenly back toward the surface when reached by the developing dry convection. 4) the thermal plume model being active about on half of the globe all the time, it controls the transport of all trace elements, with some non linear effects when the emissions themselves show a diurnal cycle. In this presentation, we review these lessons learned with LMDZ, identify the issues which should require further developments, and expose how new machine assisted techniques allow to reconcile improvement of parameterizations at process scale and climate model improvement.

Chatfield, R. B., & Brost, R. A. (1987). A two-stream model of the vertical transport of trace species in the convective boundary layer. Journal of Geophysical Research, 92, 13,263–13,276

Hourdin, F., Couvreux, F., & Menut, L. (2002). Parameterisation of the dry convective boundary layer based on a mass flux representation of thermals. Journal of the Atmospheric Sciences, 59, 1105–1123

How to cite: Hourdin, F. and Rio, C.: On the importance of dry and cloudy boundary layer convection and of its parameterization in climate models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9438, https://doi.org/10.5194/egusphere-egu23-9438, 2023.

EGU23-9855 | ECS | Posters on site | AS1.7

Tracking Convective Storms and their Environments with the tobac Tracking Package 

Sean Freeman, Rick Schulte, Gabrielle Leung, and Sue van den Heever

Understanding how convective storms respond to changes in their environment on a local scale is critical to begin to elucidate how Earth’s changing climate will affect storms globally. There is now a vast amount of storm-scale observational data, including from geostationary and low-earth orbiting satellites and ground-based observing systems. However, employing these datasets to build comprehensive databases of convective storms and the local environments that form them requires new analysis methodologies. Here, in preparation for the NASA INCUS satellite mission, we have used the tobac tracking package to identify, track and analyze storms and their environments with these big datasets. Using tobac to track storms with geostationary satellite and ground-based radar data, we have built a comprehensive, months-long database of convective storms over their entire lifetime. For each individual convective storm, the database contains their formation environments (including convective available potential energy, wind shear, etc.), evolution over time, and, where applicable, additional data, such as those from low earth orbiting satellites. In this presentation, we will employ this vast database of clouds and storms to quantify the relationship, on a storm scale, between thermodynamic and dynamic environments and storm properties, including lifetime, growth rate, and ice and liquid water paths. 

How to cite: Freeman, S., Schulte, R., Leung, G., and van den Heever, S.: Tracking Convective Storms and their Environments with the tobac Tracking Package, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9855, https://doi.org/10.5194/egusphere-egu23-9855, 2023.

EGU23-11285 | Orals | AS1.7

Tropical Convection through the Lens of the INCUS Mission 

Susan van den Heever, Ziad Haddad, Brenda Dolan, Sean Freeman, Leah Grant, Pavlos Kollias, Gabrielle Leung, Johnny Luo, Peter Marinescu, Derek Posselt, Kristen Rasmussen, Prasanth Sai, Richard Schulte, Graeme Stephens, Rachel Storer, and Hanii Takahashi

The convective mass flux within tropical convection influences the large-scale circulation, drives cloud radiative forcing, has integral links to the production of fresh water, and impacts extreme weather. CMF forms the focus of the recently selected Investigation of Convective Updrafts (INCUS) mission to be launched in 2026. This NASA mission is comprised of 3 spacecraft, all of which will carry a Ka-band cloud radar. One spacecraft will also carry a passive microwave radiometer. The 3 smallsats are to be separated by time intervals of 30, 90 and 120 seconds, thus allowing for the rapid and systematic sampling of the same storm with all three spacecraft. These time intervals (delta-ts) also facilitate the investigation of the magnitude and evolution of CMF, which will be examined as a function of storm type, storm lifecycle and environmental properties. INCUS will therefore provide the first global systematic investigation into CMF and its evolution within deep tropical convection.

A wide range of research tasks have been conducted in preparation for the INCUS mission and the development of the INCUS algorithms including: (1) running and analyzing extensive suites of large-domain, high-resolution model simulations; (2) examining ground-based Doppler radar observations obtained using adaptive scanning techniques during several recent field campaigns; and (3) evaluating anvil characteristics using passive microwave radiometer and geoIR data. This talk will focus on three specific highlights arising from these modeling and observational analyses. First, we will examine the temporal scales of updraft variability. Second, we will analyze the relationship between ice water path cores and convective updrafts. Finally, we will demonstrate proof of the INCUS delta-t concept linking changes in reflectivity to CMF through the use of ground-based radar analyses.

How to cite: van den Heever, S., Haddad, Z., Dolan, B., Freeman, S., Grant, L., Kollias, P., Leung, G., Luo, J., Marinescu, P., Posselt, D., Rasmussen, K., Sai, P., Schulte, R., Stephens, G., Storer, R., and Takahashi, H.: Tropical Convection through the Lens of the INCUS Mission, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11285, https://doi.org/10.5194/egusphere-egu23-11285, 2023.

EGU23-12581 | ECS | Posters on site | AS1.7

No evidence of spatial feedbacks causing convective clustering in the Tropical Western Pacific 

Alejandro Casallas, Adrian Tompkins, and Michie De Vera

Idealized high-resolution models show spontaneous aggregation of tropical convection on the beta-mesoscale driven by radiative feedbacks, and the resulting drying implies a potentially important impact on climate sensitivity missing in classic convective parameterization schemes. Here, we combine multiple state-of-the-art observations and reanalysis of the tropical atmosphere and ocean in a 1000 x 700 km region in the tropical Western Pacific warm pool region, along with numerical models and machine learning techniques to demonstrate that in boreal summer, while radiative and surface fluxes act to cluster convection, the convection remains in a random configuration as evidenced by very limited spatial variability in total column humidity. Instead, in the winter/spring period, when the warm pool is displaced southwards, the region lies on the warm pool boundary with stronger north-south surface temperature gradients. Convection usually remains strongly organized in these periods but is interspersed with occasional random episodes. This entails a sudden flipping into the random state associated with the southerly flow anomalies that advect convection and humidity over the cooler sea surface temperature (SST) regions. Observations and models suggest that this advection of humidity is the principal driver of organization and disorganization of convection and that diabatic feedbacks instead always act to try and cluster convection. Results also indicate that when convection is organized, the atmosphere is significantly drier than when convection is random and that the Longwave (LW) clear-sky top of atmosphere flux is significantly larger in the organized state, principally due to the moisture differences between both configurations. The LW all-sky flux difference between both states is less significant compared to the LW clear-sky because it is largely driven by the cloud cover, which, although smaller for the organized state, does not differ significantly. These differences between organized and random convective states, and the role of the diabatic processes in providing forcing for aggregation, mostly reproduce the findings of idealized models. However, this study indicates that in the real tropical atmosphere diabatic forcing is inadequate to lead to aggregation on its own over homogeneous SSTs, and instead, spatial SST gradients and large-scale dynamics are key to driving aggregation and determining its breakup over the warm pool region.

How to cite: Casallas, A., Tompkins, A., and De Vera, M.: No evidence of spatial feedbacks causing convective clustering in the Tropical Western Pacific, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12581, https://doi.org/10.5194/egusphere-egu23-12581, 2023.

EGU23-13504 | Posters virtual | AS1.7

Response of Mature Storms to Soil Moisture State in Global Hotspot Regions 

Emma Barton, Cornelia Klein, Christopher Taylor, John Marsham, and Douglas Parker

Mesoscale Convective Systems (MCSs) represent some of the most intense and destructive thunderstorms in the world. Understanding the physical processes that drive these storms and influence their characteristics is vital for hazard prediction and mitigation. 

A significant amount of research in the “natural laboratory” of West Africa has shown that soil moisture heterogeneity on different spatial scales can influence the location of convective initiation (10s of km) and the intensification of remotely triggered storms (100s of km).

Previous studies have demonstrated that the control of soil moisture state on convective initiation identified in West Africa is also important elsewhere in the world whereas very little is known about the influence of surface conditions on travelling storms in other regions.

In the current work we combine satellite observations and reanalysis data to characterise the impact of pre-storm soil moisture conditions on the atmospheric environment and characteristics of mature storms in seven MCS hotspot regions, West Africa, South Africa, South America, Great Plains, India, China and Australia. 

We observe a clear latitudinal dependence of the coupling signal with distinct differences between regions where convection is predominately driven by monsoonal or frontal dynamics. However our results suggest that in all regions, large-scale (100s of km) soil moisture gradients are having an impact on convection within mature MCSs through moderation of the climatological temperature gradient in the lower atmosphere, which influences factors that favour convection such as shear and convergence.

How to cite: Barton, E., Klein, C., Taylor, C., Marsham, J., and Parker, D.: Response of Mature Storms to Soil Moisture State in Global Hotspot Regions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13504, https://doi.org/10.5194/egusphere-egu23-13504, 2023.

EGU23-13744 | Posters on site | AS1.7

The Diurnal Cycle of the Cloud Radiative Effect of Deep Convective Clouds over Africa from a Lagrangian Perspective 

William Jones, Martin Stengel, and Philip Stier

Tropical deep connective clouds (DCCs) have large top of atmosphere (ToA) cloud radiative effects (CREs) in both the shortwave (SW) and longwave (LW), which both have average magnitudes of greater than 100 Wm-2. Due to the opposite sign of the two components, the overall ToA CRE is generally assumed to average to approximately 0 Wm-2. Although there are a number of mechanisms that contribute to this balance, the fact that the daytime only SW CRE balances with the LW CRE indicates that the diurnal lifecycle of DCCs is a key component of this balance. Understanding how the diurnal cycle of DCCs influences their CRE is vital for understanding how any changes in their diurnal cycle of these clouds may influence the climate.

 

A year-long dataset of retrieved cloud properties and derived broadband radiative fluxes has been produced by the ESA Cloud CCI project using temporally highly resolved satellite observations. Using a novel method, we are able to detect and track both isolated DCCs and large, mesoscale convective systems (MCSs) over their entire lifecycle. We explicitly retrieve the cloud properties and CREs of DCCs over Africa, and how these properties change over the lifecycle of approximately 100,000 observed clouds. We find that the mean anvil SW CRE greatly varies depending on the initiation time of day and the lifetime of the DCC, whereas the LW CRE is consistent throughout the diurnal cycle and varies primarily with cloud top temperature.

 

As a result of our study we can confirm that the mean observed ToA CRE of all DCCs (integrated over area and lifetime) is indeed approximately 0 Wm-2, but very few DCCs individually have mean CREs near this value. Instead, we find that DCCs occurring during the daytime have a large cooling effect, and those at nighttime have a warming effect, resulting in a bimodal distribution. While MCSs make the largest contribution to the overall effect due to their large areas and lifetimes, because they tend to exist during both nighttime and daytime the overall magnitude of their ToA CREs tend to be smaller than those of isolated DCCs. As a result, factors which influence the diurnal cycle of deep convection – such as changes in CAPE generation or convective inhibition – may have a more important influence on the properties of isolated DCCs rather than larger MCSs.

How to cite: Jones, W., Stengel, M., and Stier, P.: The Diurnal Cycle of the Cloud Radiative Effect of Deep Convective Clouds over Africa from a Lagrangian Perspective, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13744, https://doi.org/10.5194/egusphere-egu23-13744, 2023.

EGU23-13748 | ECS | Posters on site | AS1.7

Sub-mesoscale temperature variability in observed and simulated convective cold pools 

Bastian Kirsch, Leah D. Grant, Nicholas M. Falk, Christine A. Neumaier, Jennie Bukowski, Felix Ament, and Susan C. van den Heever

The spatial and temporal variability of air temperature represents the imprint of various meteorological processes, ranging from microscale turbulence to synoptic-scale weather systems. Convective cold pools, formed by evaporatively cooled downdrafts of precipitating clouds, are known to be an important source of mesoscale variability over mid-latitude land. Cold pools both directly perturb the near-surface temperature field and influence variability by controlling larger-scale convective organization. However, their impact on the sub-mesoscale (100 m to 10 km) temperature variability is unclear due to insufficient observational data. Consequently, the validation of sub-mesoscale variability in numerical weather prediction (NWP) and Large-Eddy Simulation (LES) models is also impeded.

In this study, we apply the variogram framework to determine sub-mesoscale temperature variability in observations as well as in idealized and realistic simulations of cold pool events. The basis of the analyses are actual and virtual observations of a dense network of 99 surface measurement stations as part of the Field Experiment on Submesoscale Spatio-Temporal Variability in Lindenberg (FESSTVaL) conducted in eastern Germany during summer 2021. The observed variogram averaged over the lifetime of a cold pool shows enhanced temperature variance at scales between about 1 km and 15 km compared to well-mixed boundary layer conditions, although the magnitude of the perturbation strongly varies for single time steps. Except for the intensification phase, the cold pool generally reduces the temperature variability at sub-km scales compared to pre-cold pool conditions. This suggests smoothing of sub-km temperature gradients by enhanced mixing near the surface as well as damped turbulent surface fluxes.

Idealized cold pool simulations at LES grid spacings capture the overall variogram shape and evolution well but show the largest uncertainty for sub-km scales as compared to the observed variograms. The results are sensitive to the sampled lifetime stage of the cold pool, its environmental conditions, and the model representation of dissipation time scales and turbulent surface fluxes. These findings can help to identify the spatial and temporal scales of variability that are relevant to correctly simulate convective processes in the atmosphere and their interaction with the land surface.

How to cite: Kirsch, B., Grant, L. D., Falk, N. M., Neumaier, C. A., Bukowski, J., Ament, F., and van den Heever, S. C.: Sub-mesoscale temperature variability in observed and simulated convective cold pools, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13748, https://doi.org/10.5194/egusphere-egu23-13748, 2023.

EGU23-13971 | ECS | Posters on site | AS1.7

The Relationship Between Isolated Deep Convection Initiation and Topography in the North China Area 

Guilin Lu, Yangze Ren, Shizuo Fu, and Huiwen Xue

The characteristics of isolated deep convection initiation (DCI) and its relation to topography in the North China area are studies statistically and numerically. The infrared brightness temperature data from satellite Himawari-8 are utilized to identify DCI events in three summers. A total of 2534 DCI events are obtained and their locations show clustering over mountains and hills, suggesting the significance of local topography. Topography is described with elevation and relief amplitude. DCI events and grid boxes are counted. DCI events per grid box increases with elevation and relief amplitude. Among different types of topography, DCI is favored in mountains and hilly areas. Moreover, the morning cloud cover condition also shows notable impact on the relation of DCI and topography. For the regime characterized with less morning clouds (regime one), DCI strongly depends on elevation and relief amplitude, while for the regime with more morning clouds (regime two), topography shows a moderate impact on DCI. The time of DCI events are also recorded, and regime one shows a stronger diurnal variation and a peak occurring 2 hours earlier than that of regime two. The synoptic patterns show the difference of large-scale environment between the two regimes, which can explain their differences in DCI to some extent. To clarify the mechanism of topographic effect in DCI process, quasi-idealized numerical simulation in North China is conducted with WRF. The averaged 6-hourly ERA-Interim reanalysis data, which can maintain the major patterns of large-scale circulations, are inputted into the model as initial and boundary conditions. The elevation and relief amplitude of the study domain is varied in the model. The preliminary result shows that the speed of upscale convection growth changes with elevation and relief amplitude, which indicates that mechanisms involving topography-induced variation of solar heating may exist and need further numerical study. We suggest that special attention should be paid to elevation and relief amplitude (or topography type), as well as morning cloud cover condition when forecasting DCI in the North China area and mountainous areas around the world.

How to cite: Lu, G., Ren, Y., Fu, S., and Xue, H.: The Relationship Between Isolated Deep Convection Initiation and Topography in the North China Area, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13971, https://doi.org/10.5194/egusphere-egu23-13971, 2023.

EGU23-14317 | ECS | Orals | AS1.7

Using statistical emulation to quantify microphysical uncertainties for the Andreas hailstorm in 2013 

Lena Frey, Corinna Hoose, Michael Kunz, Annette Miltenberger, and Patrick Kuntze

We investigate microphysical uncertainties in hailstorms using statistical emulation in a single model framework with the objective to disentangle the relative contributions from aerosols, microphysical parameters and environmental conditions to the uncertainty in cloud-, precipitation- and hail-related parameters.

Our selected case study is the Andreas hailstorm on 28 July 2013 in the Neckar Valley and over the Swabian Jura in Southwest Germany. We perform model simulations on cloud-resolving scale with the numerical weather prediction model ICON coupled with the aerosol module ART (ICON-ART). We use a two-moment cloud microphysics scheme with a representation of ice nucleation by dust aerosols.
We generated a perturbed parameter ensemble (PPE) to sample uncertainties in cloud-, precipitation- and hail related parameters. Six parameters from the categories aerosols, microphysics and environmental conditions were jointly perturbed, namely the cloud condensation nuclei (CCN) and ice nuclei (IN) concentrations, the riming efficiency of graupel and hail, the convective available potential energy (CAPE) and vertical wind shear. The defined parameter ranges are based on forecast analysis and literature. We used the maximin Latin hypercube algorithm to distribute the parameters well-spaced in the six-dimensional parameter uncertainty space. For these six parameters, an ensemble of 90 members was generated and in addition a smaller independent ensemble of 45 members serves for validation.

We used the Gaussian process emulation and developed emulators for hail- and precipitation related output variables. To quantify contributions to the uncertainty in the output variables from the perturbed parameters individually as well as interactions between them, a variance-based sensitivity analysis was performed. We will present first results, which reveal the importance of the CCN concentration for controlling the number concentration of hail particles as well as the CCN concentration and environmental conditions for controlling the amount of hail and precipitation in the model. The geographical distribution of hail and precipitation shows a large variety among the ensemble members, with storm tracks shifted further to the north or south compared to the reference simulation. The path of the storm track is thereby mainly controlled by CAPE and the vertical wind shear, however, aerosol parameters seem to be important for the development of multiple storm tracks. 

How to cite: Frey, L., Hoose, C., Kunz, M., Miltenberger, A., and Kuntze, P.: Using statistical emulation to quantify microphysical uncertainties for the Andreas hailstorm in 2013, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14317, https://doi.org/10.5194/egusphere-egu23-14317, 2023.

EGU23-14672 | ECS | Posters on site | AS1.7

Modulation of Maritime Continent convection by the MJO: differences between parametrized and explicit convection 

Dan Shipley, Emma Howard, and Steven Woolnough

Convection over the Maritime Continent has large impacts for local extreme weather, as well as for global weather and climate. However, this convection and its impacts are poorly represented in current weather and climate models. This is largely due to complex multi-scale interactions between convection and the ocean, intricate island coastlines and topography, equatorial waves, and larger-scale dynamics such as the Madden-Julian oscillation (MJO). In order to better understand the modulation of convection by the MJO, and its representation in current models, we developed a new modelling suite that couples the Met Office Unified Model to a thermodynamic mixed-layer ocean model with additional corrections to account for ocean dynamics. This allows two-way interactions between the atmosphere and ocean on convection-relevant timescales without the expense of a full dynamical ocean model. We present results from simulations of 10 DJF seasons over the Maritime Continent at grid spacings of 12km (with a mass flux convection scheme) and 2km (without).  

We investigated the modulation of large-scale convective heating and moistening by MJO phase in both models. We show that: 

  • The 2km suite has more variability by MJO phase, and this variability is more realistic than that in the 12km suite when compared to observational data; 
  • There is more variability in the type of convection (defined by the shape of heating/moistening profiles) between MJO phases in the 2km suite; 
  • The dominant variation is between different types of convection in the two suites. 

We also present preliminary results on the modulation by the MJO of basic properties of the cloud field like feature size, and feature isotropy.  

How to cite: Shipley, D., Howard, E., and Woolnough, S.: Modulation of Maritime Continent convection by the MJO: differences between parametrized and explicit convection, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14672, https://doi.org/10.5194/egusphere-egu23-14672, 2023.

EGU23-15870 | ECS | Orals | AS1.7

Extreme Precipitation in Tropical Squall Lines 

Sophie Abramian, Caroline Muller, and Camille Risi

Squall lines are the consequence of the interaction of low-level shear with cold pools associated with convective downdrafts. Beyond a critical shear amplitude, squall lines tend to orient themselves at an angle with respect to the low-level shear. While the mechanisms behind squall line orientation seem to be increasingly well understood, uncertainties remain on the implications of this orientation. Roca & Fiolleau 2020 show that long lived mesoscale convective systems, including squall lines, are disproportionately involved in rainfall extremes in the tropics. One may then question whether the orientation of squall lines has an impact on rainfall extremes, and if so, why.

Using a cloud-resolving model, we perform idealized simulations of tropical squall lines by imposing a vertical wind shear in radiative-convective equilibrium. Our results show that precipitation extremes in squall lines are 40% more intense in the critical case and remain 30% superior in the supercritical regime. With a theoretical scaling of precipitation extremes (Muller & Takayabu 2019), we show that the condensation rates control the amplification of precipitation extremes in tropical squall lines, mainly due to its dynamic component. The critical case is not only optimal for squall line orientation, but also for the cloud base velocity intensity of new convective cells.

How to cite: Abramian, S., Muller, C., and Risi, C.: Extreme Precipitation in Tropical Squall Lines, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15870, https://doi.org/10.5194/egusphere-egu23-15870, 2023.

EGU23-1071 | Orals | AS1.8

Radiation, Clouds, and Self-Aggregation in RCEMIP Simulations 

Chris Holloway, Kieran Pope, Thorwald Stein, and Todd Jones

The responses of tropical anvil cloud and low-level cloud to a warming climate are among the largest sources of uncertainty in our estimates of climate sensitivity. However, most research on cloud feedbacks relies on either global climate models with parameterized convection, which do not explicitly represent small-scale convective processes, or small-domain models, which cannot directly simulate large-scale circulations. We investigate how self-aggregation, the spontaneous clumping of convection in idealized numerical models, depends on cloud-radiative interactions with different cloud types, sea surface temperatures (SSTs), and stages of aggregation in simulations that form part of RCEMIP (the Radiative-Convective Equilibrium Model Intercomparison Project). Analysis shows that the presence of anvil cloud, which tends to enhance aggregation when collocated with anomalously moist environments, is reduced in nearly all models when SSTs are increased, leading to a corresponding reduction in the aggregating influence of cloud-longwave interactions. We also find that cloud-longwave radiation interactions are stronger in the majority of General Circulation Models (GCMs), typically resulting in faster aggregation compared to Cloud-system Resolving Models (CRMs). GCMs that have stronger cloud-longwave interactions tend to aggregate faster, whereas the influence of circulations is the main factor affecting the aggregation rate in CRMs.

How to cite: Holloway, C., Pope, K., Stein, T., and Jones, T.: Radiation, Clouds, and Self-Aggregation in RCEMIP Simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1071, https://doi.org/10.5194/egusphere-egu23-1071, 2023.

EGU23-2791 | ECS | Orals | AS1.8

Turbulence properties inside and outside trade-wind cumulus clouds 

Jakub Nowak, Marta Wacławczyk, and Szymon Malinowski

Shallow trade-wind cumulus clouds originate from thermals which rise from the turbulent subcloud layer and penetrate high enough to reach their lifting condensation level. Those thermals transport heat and moisture into the cloud layer. Analogously, the subject of such a transport can be the small-scale turbulence.

Turbulence measurements near the cloud base and in the subcloud layer were performed in the course of the EUREC4A field campaign by the ATR research aircraft in a large number of repeatable flight segments (Brilouet et al., 2021). In this study, we exploit this extensive dataset to derive properties of turbulence corresponding to short 'local' domains, of the size of the order of 100 m, e.g. turbulence kinetic energy dissipation rate, anisotropy and inertial range scaling. Taking advantage of the substantial amount of data provided by the EUREC4A measurements, we compare the statistics of those parameters between the areas inside cumulus clouds, outside them at the same altitude and at three levels inside the subcloud layer.

Such a comparison indicates that the character of small-scale turbulence inside cumulus clouds can be considered comparable to the one observed in the subcloud layer but significantly differs from that observed at the same level outside the clouds. As the cloud fraction at cloud base is typically rather a small number (about 4% during EUREC4A), it is in consequence inherently difficult for large scale models to accurately parameterize the intensity of turbulence and mixing in the trade-wind regime.

How to cite: Nowak, J., Wacławczyk, M., and Malinowski, S.: Turbulence properties inside and outside trade-wind cumulus clouds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2791, https://doi.org/10.5194/egusphere-egu23-2791, 2023.

EGU23-4127 | ECS | Posters virtual | AS1.8

Cloud Feedback on Earth's Long-Term Climate Simulated by a Near-Global Cloud-Permitting Model 

Mingyu Yan, Jun Yang, Yixiao Zhang, and Han Huang

The Sun becomes brighter with time, but Earth's climate is roughly temperate for life during its long-term history; for early Earth, this is known as the faint young Sun problem (FYSP). Besides the carbonate-silicate feedback, recent researches suggest that a long-term cloud feedback may partially solve the FYSP. However, the general circulation models they used cannot resolve convection and clouds explicitly. This study re-investigates the clouds using a near-global cloud-permitting model without cumulus convection parameterization. Our results confirm that a stabilizing shortwave cloud feedback does exist, and its magnitude is ≈6 W m−2 or 14% of the energy required to offset a 20% fainter Sun than today, or ≈10 W m−2 or 16% for a 30% fainter Sun. When insolation increases and meanwhile CO2 concentration decreases, low-level clouds increase, acting to stabilize the climate by raising planetary albedo, and vice versa.

How to cite: Yan, M., Yang, J., Zhang, Y., and Huang, H.: Cloud Feedback on Earth's Long-Term Climate Simulated by a Near-Global Cloud-Permitting Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4127, https://doi.org/10.5194/egusphere-egu23-4127, 2023.

EGU23-4307 | ECS | Orals | AS1.8

The Sugar-To-Flower Shallow Cumulus Transition Under the Influences of Diel Cycle and Free-Tropospheric Mineral Dust 

Pornampai Narenpitak, Jan Kazil, Takanobu Yamaguchi, Patricia Quinn, and Graham Feingold

A shallow cumulus cloud transition from a sugar to flower type of organization occurred under a layer of mineral dust on 2nd February 2020, during the multinational Atlantic Tradewind Ocean-Atmosphere Mesoscale Interaction Campaign (ATOMIC) and the Elucidating the Role of Clouds-Circulation Coupling in Climate (EUREC4A) campaigns. Lagrangian large eddy simulations following an airmass trajectory along the tradewinds are used to explore radiative impacts of the diel cycle and mineral dust on the sugar-to-flower (S2F) cloud transition. The large-scale meteorological forcing is derived from the ECMWF Reanalysis 5th Generation (ERA5) and based on aerosol measurements from the U.S. Ronald H. Brown Research Vessel and the French ATR-42 Research Aircraft during the field campaigns. A 12-hr delay in the diel cycle accelerates the S2F transition at night, leading to more cloud liquid water and precipitation. The aggregated clouds generate more and stronger cold pools, which alter the original mechanism responsible for the organization. Although there is still mesoscale moisture convergence in the cloud layer, the near-surface divergence associated with cold pools transports the subcloud moisture to the drier surrounding regions. New convection forms along the cold-pool edges, generating new flower clouds. The modulation of the surface radiative budget by free-tropospheric mineral dust poses a less dramatic effect on the S2F transition. Mineral dust releases longwave radiation, reducing the cloud amount at night, and absorbs shortwave radiation during the day, cooling the boundary-layer temperature and increasing the overall cloud amount. Cloud-top radiative heating because of more clouds strengthens the mesoscale organization, enlarging the aggregate areas, and increasing the cloud amount further.

How to cite: Narenpitak, P., Kazil, J., Yamaguchi, T., Quinn, P., and Feingold, G.: The Sugar-To-Flower Shallow Cumulus Transition Under the Influences of Diel Cycle and Free-Tropospheric Mineral Dust, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4307, https://doi.org/10.5194/egusphere-egu23-4307, 2023.

EGU23-4689 | Posters virtual | AS1.8

What explains the population of daytime, optically-thin clouds below one km in the marine trade wind region? 

Paquita Zuidema, Isabel McCoy, Michael Perez, and Sunil Baidar

The cloud fraction of shallow non-precipitating cumulus residing at the lifting condensation level (LCL) increases in the afternoon, most evident in airborne lidar observations from EUREC4A. Observations from the HALO platform and from the R/V Ronald H. Brown are used to articulate the responsible process. Three hypotheses are investigated: 1) afternoon increases of the ocean sea surface temperature help support buoyancy fluxes that lift air parcels to saturation, as seen in tropical regions under low wind speeds; 2) shortwave absorption of the sub-cloud layer helps deepen the sub-cloud layer, so that its mixed-layer height can reach the LCL; 3) clouds form where the cloud layer is already moist. We invite the reader to take a moment here to choose which hypothesis you think is correct.

Analysis to date suggests #3 is the correct explanation. If so, then the next question is to identify why the daytime cloud layer is more or less moist in some places and times. Ideas for this can either be moisture redistribution from shallow circulations occurring at scales of approximately 200 km, or, moisture transport occurring at larger scales. These will be explored prior to the meeting, as well as ramifications for the diurnal cycle.

How to cite: Zuidema, P., McCoy, I., Perez, M., and Baidar, S.: What explains the population of daytime, optically-thin clouds below one km in the marine trade wind region?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4689, https://doi.org/10.5194/egusphere-egu23-4689, 2023.

The subtropical marine stratocumulus-to-cumulus cloud transition and associated cloud size distributions are studied using Large-Eddy Simulations based on EUREC4A data. The simulations with the DALES code follow a Lagrangian trajectory from initially overcast stratocumulus to the tropical shallow cumulus region at the HALO flight site near Barbados, covering four days and three complete diurnal cycles. Mean state and bulk properties for different domain sizes are evaluated against aircraft data. In addition, time-continuous high-frequency data from Geostationary Operational Environmental Satellite (GOES) are used to investigate the evolution of cloud size distributions, focusing on the diurnal evolution of mesoscale cloud features. TOA brightness temperature data from GOES is used at a spatial resolution of 2x2 km2 to characterize cloud populations and cloud morphology. These are compared to TOA brightness temperatures calculated from DALES output using the RRTOV simulator, as applied to subdomain-averages of similar dimensions. We find that the simulation with the largest domain size (100x100 km2) best reproduces the observed boundary layer and cloudy states at the HALO target site. The same applies to the amplitude and evolution of cloud cover as detected by GOES. The upstream nocturnal flower cloud organization is also reproduced, albeit with a slight time delay. 

How to cite: Ghazayel, S. and Neggers, R.: Evaluation of the diurnal evolution of flower cloud organization in multi-day Lagrangian large-eddy simulations based on EUREC4A against GOES satellite data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4907, https://doi.org/10.5194/egusphere-egu23-4907, 2023.

Mesoscale vertical velocity is a key element to understand links between clouds, radiation and circulation. However, in situ measurements of this variable remain sparse and costly.

Here, we present a method to estimate clear-sky free tropospheric mesoscale vertical motion from rapid-scan geostationary satellite radiance measurements in the water vapour absorption band. Subsidence is indeed associated with drying and a decrease of emission level height (and conversely for ascendance). Under basic physical assumptions, the associated temporal changes in brightness temperature can be quantitatively related to vertical velocity.

The retrieval method is evaluated against in situ observations from EUREC4A and OTREC field campaigns that sampled respectively the winter trades and the intertropical convergence zone. Although suffering from significant error bars (+/-4hPa/hr), retrievals are able to reproduce the general temporal evolution and spatial patterns of mid-tropospheric mesoscale vertical motion.

The retrieval method is further evaluated using kilometer-scale simulations associated with a radiative transfer code. Basic climatological features are captured such as the distribution of mesoscale vertical velocity or its influence on cloud cover.

Despite notable drawbacks, the method is able to provide time-continuous estimations of vertical velocity in clear sky regions of the whole tropical belt at the scale of the pixel of the satellite imager. First results suggest that mesoscale (20-200km) vertical velocity structures are ubiquitous in the tropical free troposphere.

These observations could prove valuable for studying dynamical links between deep convection and its environment, especially in association with the new generation of satellites, that will provide measurements of in-cloud convective mass flux and clear-sky time-continuous water vapour and temperature profiles.

How to cite: Poujol, B. and Bony, S.: A method to estimate clear sky mesoscale vertical motion from geostationary satellite imagery, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5009, https://doi.org/10.5194/egusphere-egu23-5009, 2023.

EGU23-5585 | Orals | AS1.8

Impact of elevated Saharan Air layer on shallow marine convection 

Silke Gross, Manuel Gutleben, and Martin Wirth

Mineral dust is one of the major contributors to the global aerosol load with the Sahara being its largest source. Dust particles can be transported over many days and thousands of kilometers. The main transport route spans from Africa over the Atlantic Ocean towards the Caribbean. Most of the time dust-transport takes place in the so-called Saharan Air Layer (SAL).  During its transport the SAL affects the Earth’s atmosphere by scattering and absorption of solar and terrestrial radiation, and by changing cloud evolution and cloud properties. The main season for the transatlantic dust transport is during the boreal summer months. However, dust can be transported towards the Caribbean also during wintertime, although this happens with less frequency.

Airborne lidar measurements with the combined water vapor differential absorption and high spectral resolution lidar system WALES provide simultaneous measurements of the water vapor mixing ratio and of aerosol properties. We use the measurements during the NARVAL-II experiment in August 2016 and during the EUREC4A experiment in January/February 2020 to characterize the long-range transported SAL in summer- and in wintertime, and to investigate its radiative effect and its impact on the subjacent shallow marine trade wind convection. We found, that a small amount of water vapor embedded in the SAL has a strong impact on the radiative heating effect of this layer and consequently also on the atmosphere’s stability. During summertime, when the SAL is well separated from the marine boundary layer, the radiative effect of the SAL dominates. The evolution of shallow marine clouds below the SAL is suppressed. In wintertime, the SAL is transported at lower altitudes and the dust layer is frequently mixed into the marine boundary layer. During this time of the year the effect of the SAL on the evolution and lifetime of marine trade wind convection is much more complex, as the dust particles within the SAL might additionally act as cloud or ice nuclei.

In our presentation we will give an overview of the performed measurements and the radiative transfer calculations. We will present the radiative effects of the separated summertime SAL, and show first results of the impact of the wintertime SAL on the atmosphere’s stability and cloud properties.

How to cite: Gross, S., Gutleben, M., and Wirth, M.: Impact of elevated Saharan Air layer on shallow marine convection, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5585, https://doi.org/10.5194/egusphere-egu23-5585, 2023.

EGU23-5796 | Posters on site | AS1.8

Tracking Clouds: Comparing Geostationary Satellite Observations and Model Data 

Felix Müller, Torsten Seelig, and Matthias Tesche

Tracking clouds has multiple applications. It is used for short-term weather forecasting as well as long-term weather and climate analyses. Our long-term goal is to investigate cloud life cycles under different conditions, such as marine or continental areas, over deserts, or in areas with increased anthropogenic aerosols. This is a key element in understanding cloud radiation effects and the human influence on the cloud life cycle.

To identify clouds and their trajectories, we are using Particle Image Velocimetry [1] which is well-known for measuring velocities in fluid dynamics. These velocity fields are used to predict the positions of clouds in the next timestep. The predicted positions are then compared to the observed positions to match clouds across timesteps. The algorithm can work on any geostationary satellite data set or equivalent model data [2].

Currently we are comparing satellite data from the EUREC4A campaign [3] (observed by the Advanced Baseline Image onboard the GOES-16 satellite) and model output from ICON-LEM [4]. Both datasets are located east of Barbados in the Caribbean Sea. This is done to benchmark the model settings and to identify which of the three model resolution best captures the satellite data. The cloud tracking allows us to look at the lifetimes of the clouds and the development of cloud physical properties over the lifetime of a cloud. This leads to a more refined investigation into the cloud behavior.

The presented results are twofold. Firstly, we will show a direct comparison of individual cloud trajectories between observed and model data to establish a deeper understanding of the methodology and datasets. Secondly, we will look at the distributions of clouds sizes and lifetimes to compare different resolutions of model data to the observed satellite data.

 

References:

[1] Raffel et al. (2007) "Particle Image Velocimetry - A Practical Guide", Springer Verlag, doi: 10.1007/978-3-540-72308-0

[2] Seelig et al. (2021) "Life cycle of shallow marine cumulus clouds from geostationary satellite observations", in JGR: Atmospheres, doi: 10.1029/2021JD035577

[3] EUREC4A campaign: www.eurec4a.eu

[4] Dipankar et al. (2015) “Large eddy simulation using the general circulation model ICON”, in Journal of Advances in Modeling Earth Systems 7(3): 963-986, doi: 10.1002/2015MS000431

How to cite: Müller, F., Seelig, T., and Tesche, M.: Tracking Clouds: Comparing Geostationary Satellite Observations and Model Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5796, https://doi.org/10.5194/egusphere-egu23-5796, 2023.

EGU23-7513 | Posters virtual | AS1.8

Sub-cloud layer winds in the vicinity of trade-wind cumulus 

Louise Nuijens and Mariska Koning

Sailors have long used cumulus clouds to guide their ships into areas of favourable winds. On the upwind side of cumulus clouds, the clouds’ thermal circulation would add momentum to the prevailing flow, while on the downwind side, the opposing branch of the circulation would reduce the flow. In this study, we take a simple approach to evaluating this sailors’ theorem and visualise the winds in the sub-cloud layer in the vicinity of shallow cumulus clouds. This is done by collocating cloud radar and wind lidar profiling measurements during EUREC4A on board the RV Meteor and at the BCO for a six-month period. Is there evidence for a thermal circulation in the wind surrounding clouds, or for plume-like structures that support a mass-flux approach? We will discuss our findings for clouds of increasing depth, for which clustered convection and cold pool gustiness become increasingly important.

How to cite: Nuijens, L. and Koning, M.: Sub-cloud layer winds in the vicinity of trade-wind cumulus, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7513, https://doi.org/10.5194/egusphere-egu23-7513, 2023.

EGU23-8842 | ECS | Posters on site | AS1.8

Evaluation of mass flux closures using EUREC4A observations 

Raphaela Vogel and Juan Pedro Mellado

Determining the shallow-convective mass flux at cloud base is the principle closure needed in convective parameterizations. Closure methods are usually developed and tested based on large-eddy simulations of a limited number of idealized cases. Here we evaluate how well common closures reproduce the magnitude and variability of the cloud-base mass flux observed during the recent EUREC4A field campaign upstream Barbados. The true observed mass flux is estimated as a residual of the sub-cloud layer mass budget from the circular dropsonde arrays at the 200km scale. To assess the closures, we diagnose all parameters of the chosen closures from the same dropsonde data or from coincident turbulence and cloud measurements of a second aircraft. Preliminary results suggest that (i) both variability in the area fraction and vertical velocity scales should be accounted for to reproduce the observed mass flux variability, (ii) methods using the turbulence kinetic energy to approximate the vertical velocity scale outperform methods based on the subcloud convective velocity scale, and (iii) the closure formulations should be general enough to remain useful when applied to other data and regimes.

How to cite: Vogel, R. and Mellado, J. P.: Evaluation of mass flux closures using EUREC4A observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8842, https://doi.org/10.5194/egusphere-egu23-8842, 2023.

EGU23-8935 | ECS | Orals | AS1.8

How do environmental mesoscale heterogeneities influence the trade-wind cloud organization? 

Thibaut Dauhut, Fleur Couvreux, and Dominique Bouniol

Cumuli clouds in the trade winds are a great source of uncertainty for the future climate as their net radiative effect is hardly represented in global models. The spatial organization of these clouds, that drives their radiative effect, has been categorized into 4 major patterns: Sugar, Flower, Gravel and Fish (Bony et al. 2020). The processes governing their spatial organization and the relationships with the environmental properties remain however unclear. This study investigates the sensitivity of the Flower organization to the environmental mesoscale heterogeneities in water vapor and winds. A case of Flower organization, producing 100-km wide cloud clusters, is selected from the EUREC4A-ATOMIC campaign that took place east of Barbados in January-February 2020. A Large-Eddy Simulations using the Meso-NH model and a 100-m horizontal grid-spacing has been extensively validated by satellite and aircraft high-resolution observations (Dauhut et al., 2022) and serves as a reference. By removing alternatively the humidity or the wind heterogeneities, we show that mesoscale humidity anomalies play a critical role in driving cloud organisation into Flower. Further investigations indicate that humidity heterogeneities in the cloud layer influence the development of a shallow mesoscale circulation and have a larger impact than the heterogeneities in the sub-cloud layer. Different chains of processes are proposed to explain such a sensitivity.

How to cite: Dauhut, T., Couvreux, F., and Bouniol, D.: How do environmental mesoscale heterogeneities influence the trade-wind cloud organization?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8935, https://doi.org/10.5194/egusphere-egu23-8935, 2023.

EGU23-10014 | ECS | Orals | AS1.8

How shallow circulations couple to moisture in the trades - A perspective from satellites 

Geet George, Dominique Bouniol, and Fleur Couvreux

Measurements over the north-Atlantic trade wind regions from the recent EUREC4A field campaign (ElUcidating the RolE of Cloud–Circulation Coupling in ClimAte) have revealed a large variability in mesoscale (ca. 200 km) vertical velocity. This variability is primarily attributable to shallow mesoscale overturning circulations (SMOCs) , which have also been shown to influence mesoscale moisture variability. From EUREC4A observations, it is found that the mesoscale horizontal divergence (D) averaged over the mixed layer covaries strongly with surface D. We exploit this finding by using satellite observations of surface divergence to understand SMOCs further. We mainly use WindSAT measurements for surface divergence due to its larger swath compared to scatterometers and its superior performance under precipitating conditions. In WindSAT observations, surface divergence shows a negative correlation with integrated water vapour (IWV), but also shows the large variance when IWV is large, indicating that there might be two regimes in the divergence-moisture relationship. To further investigate the divergence-moisture relationship, we perform object-identification in the IWV field and characterize surface divergence therein. A synergy with geostationary cloudiness fields from GOES-16 helps us further interpret these characteristics in the context of the spatial organization of clouds. As satellite observations go beyond the space-time coverage of field campaigns, we are able to document (a) statistics of the spatial scales of SMOCs as well as (b) some consistent relationships between SMOCs and atmospheric moisture.

How to cite: George, G., Bouniol, D., and Couvreux, F.: How shallow circulations couple to moisture in the trades - A perspective from satellites, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10014, https://doi.org/10.5194/egusphere-egu23-10014, 2023.

EGU23-10638 | Orals | AS1.8

Moisture export by shallow convective mixing during EUREC4A 

Adriana Bailey, David Noone, and Dean Henze

In 2020, the EUREC4A (ElUcidating the RolE of Clouds-Circulation Coupling in ClimAte) field mission set out to investigate the role of shallow convective mixing in regulating trade cumulus and their influence on global climate. Recent results from this mission refute the idea that shallow convective mixing reduces cloudiness, as previous studies had argued. Instead, they suggest that shallow convective mixing is positively correlated with cloudiness when both are modulated by mesoscale circulations. Here, we provide independent evidence that further substantiates these findings. Using the unprecedented collection of water isotopic data sampled during EUREC4A, we derive estimates of total moisture exported from the sub-cloud layer by shallow convective mixing. We also derive vertical profiles of exported sub-cloud layer moisture, which allow us to investigate how shallow convective mixing alters the vertical structure of thermodynamic quantities and clouds. We show a strong association between the amount of moisture exported, the top-heaviness of the exported-moisture profile, the trade wind inversion height, and the average cloud top altitude. All increase when large cloud decks are present, indicating a role for mesoscale convective organization. We extend the analysis with remotely sensed isotope ratios in order to investigate the associations between mixing, moisture export, and cloudiness on larger scales (in both time and space) and to examine the conditions that favor convective organization at the mesoscale.

How to cite: Bailey, A., Noone, D., and Henze, D.: Moisture export by shallow convective mixing during EUREC4A, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10638, https://doi.org/10.5194/egusphere-egu23-10638, 2023.

EGU23-10781 | Posters virtual | AS1.8

Evaluation of Trade Wind Mesoscale Morphology Evolution and Transitions 

Isabel L. McCoy, Paquita Zuidema, Sunil Baidar, Raphaela Vogel, Ryan Eastman, Hauke Schulz, and Alan Brewer

Mesoscale cloud morphology patterns in the trade-winds can be grouped by their distinct appearance, size, and radiative properties into four categories: Sugar, Gravel, Flowers, and the synoptically driven Fish. Two occurrence pathways for the larger boundary-layer cloud organization structures were observed during the wintertime 2020 EUREC4A-ATOMIC joint campaign: i) regional Gravel persistence and ii) transitions to Gravel and Flowers from smaller Sugar clouds. Understanding the contributions to larger cloud structure occurrence under pathways of persistence vs. transitions from smaller clouds has utility in predicting their occurrence under climate change. Two EUREC4A-ATOMIC case studies are developed for these respective pathways during multi-day periods when observational platforms were longitudinally distributed across the ocean in parallel with Barbados. A Lagrangian analysis framework is developed by using for/backward 30-hr boundary layer trajectories initialized every 3-hr from the RV Ronald H. Brown (i.e., the mid-evolution reference platform) to connect upwind (e.g., the Northwest Tropical Atlantic Station buoy) and downwind (e.g., the Barbados Cloud Observatory) platforms. This synergistic, multi-platform campaign dataset is supplemented with satellite observations and reanalysis. Motion-stabilized Doppler-lidar observations at the RV Ronald H. Brown and the Barbados Cloud Observatory allow us to examine characteristics of cloud and plume dynamics in addition to the impact of environmental conditions expected to influence cloud organization and development (e.g., surface wind speeds, energy and moisture fluxes, stability, entrainment, large- and meso-scale subsidence, and aerosols). Eulerian differences between key platforms over the campaign period are evaluated and campaign findings are further extended using multi-year Lagrangian analysis.

How to cite: McCoy, I. L., Zuidema, P., Baidar, S., Vogel, R., Eastman, R., Schulz, H., and Brewer, A.: Evaluation of Trade Wind Mesoscale Morphology Evolution and Transitions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10781, https://doi.org/10.5194/egusphere-egu23-10781, 2023.

EGU23-10856 | ECS | Orals | AS1.8

Evaluating hm-scale simulations of trade wind clouds using EUREC4A data 

Hauke Schulz, Stevens Bjorn, and Robert Wood

Recent observations revealed that meso-scale patterns of shallow convection in the downwind trades can be connected to specific atmospheric environments whose characteristics are not solely from within the trades but have traces from tropical or mid-latitudinal origin depending on the pattern. As a consequence of this co-variability of patterns and air-mass characteristics, a different feedback to a changing climate is anticipated and will be modulated by the observed, pattern-dependent net cloud radiative effects. By conducting large-eddy simulations we evaluate how well current climate models reproduce this co-variability in cloudiness and its environment and whether the meso-scale patterns are represented due to the observed mechanisms. To capture the full range of patterns and its processes these simulations are done on large-scale domains with grid-spacings of 625m, 312m and 156m and focus on the EUREC4A field campaign time period. By repeating the simulation with an increased aerosol load, we reveal pattern-dependent sensitivities. With frequently raining patterns showing the largest response, the importance of different processes depending on the meso-scale organization is emphasized.

How to cite: Schulz, H., Bjorn, S., and Wood, R.: Evaluating hm-scale simulations of trade wind clouds using EUREC4A data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10856, https://doi.org/10.5194/egusphere-egu23-10856, 2023.

Cloud cover products from multiple satellite projects are long enough to provide a robust evaluation of climate models. Using global atmosphere models forced by observed sea-surface temperature and employing satellite simulator software, three generations of the Community Atmosphere Model are evaluated. This inter-generational comparison shows how the cloud radiative effect has improved through time but cloud cover has shown only modest improvements over the past decade. Diagnostics are introduced that allow a decomposition of spatial biases to separately evaluate systematic errors in the mean from the spatial variability. Errors in cloud properties are evaluated using a dynamical regimes analysis to connect the climatological errors to the large-scale circulation. Two closely related, current-generation models, CESM2 and E3SM, are compared to show how slightly different model development and tuning decisions can impact the the cloud climatology. Leveraging multiple long-term satellite data sets suggest that despite improvements through time, there remain significant systematic errors in cloud cover. It is suggested that simultaneously constraining cloud radiative effect and cloud cover, and therefore reducing the longstanding "too few, too bright" bias, is feasible and could improve climate projections. 

How to cite: Medeiros, B.: Satellite-based evaluation of cloud cover through three generations of global atmosphere models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10934, https://doi.org/10.5194/egusphere-egu23-10934, 2023.

EGU23-11082 | Orals | AS1.8

The impact of dry intrusions on midlatitude cold-air outbreak cloud transitions 

George Tselioudis, Florian Tornow, Andrew Ackerman, and Ann Fridlind

Cold-air outbreaks (CAOs) form marine boundary layer (MBL) clouds that undergo rapid overcast-to-broken cloud regime transitions, initiated by substantial rain. CAOs are usually accompanied by dry intrusions (DIs) that subside as free-tropospheric (FT) air into the postfrontal sector of mid-latitude storms. For an exemplary cold-air outbreak in the NW Atlantic that showed faster transitions (corresponding to reduced extents of overcast clouds) closer to the low-pressure system, we posit that varying transitions are caused by an uneven meteorological pattern imposed by the prevailing DI. We compile satellite observations, reanalysis fields, and Lagrangian large-eddy simulations (LES) translating along MERRA2-based trajectories to show that postfrontal trajectories closer to the low-pressure system are uniquely favorable to rain formation (and, thus, cloud transitions) as they show (1) weaker FT subsidence rates, (2) greater FT humidity, (3) greater MBL windspeeds, and (4) a colder MBL as well as reduced lower-tropospheric stability. We present an updated conceptual view of postfrontal cloud formation that may guide future investigations.

How to cite: Tselioudis, G., Tornow, F., Ackerman, A., and Fridlind, A.: The impact of dry intrusions on midlatitude cold-air outbreak cloud transitions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11082, https://doi.org/10.5194/egusphere-egu23-11082, 2023.

EGU23-11662 | ECS | Orals | AS1.8

High spatial resolution retrieval of cloud droplet size distribution from polarimetric specMACS observations and application to simulated data 

Veronika Pörtge, Tobias Kölling, Anna Weber, Lea Volkmer, Claudia Emde, Tobias Zinner, Linda Forster, and Bernhard Mayer

We present novel remote sensing observations of cloud droplet size distributions retrieved from polarimetric observations of the wide-field airborne imaging system specMACS. The measurements were collected during the EUREC4A field campaign which took place in January and February 2020 in the trade wind region east of Barbados. We focus on observations of the cloudbow which is an optical phenomenon that results from single scattering of sunlight by liquid droplets close to the cloud top. The cloudbow signal strongly depends on the cloud droplet size distribution. By fitting model simulations (stored in a look-up table) to the cloudbow observations, both the effective radius and the effective variance (i.e., the width) of the droplet size distribution are retrieved. Traditional retrieval techniques based on total reflectance measurements are able to determine the effective radius but do not provide information on the effective variance. However, to fully understand cloud growth processes and the interaction between clouds and solar radiation, both parameters must be known. Furthermore, the cloudbow is only weakly affected by 3-D radiative transfer effects which is beneficial since these are usually a problem for traditional methods.

High-resolution maps of the cloud droplet size distribution with a spatial resolution of 100 m by 100 m are presented. The maps reveal patterns within the cloud droplet size distribution at cloud top that could originate from mechanisms like entrainment or mixing processes. We further show first results of an application of the retrieval to simulated specMACS observations. The images were generated using the 3-D radiative transfer model MYSTIC and are based on realistic LES cloud field simulations. We will investigate limitations and uncertainties of the retrieval using the simulated dataset.

How to cite: Pörtge, V., Kölling, T., Weber, A., Volkmer, L., Emde, C., Zinner, T., Forster, L., and Mayer, B.: High spatial resolution retrieval of cloud droplet size distribution from polarimetric specMACS observations and application to simulated data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11662, https://doi.org/10.5194/egusphere-egu23-11662, 2023.

EGU23-12257 | Orals | AS1.8

Complementary approaches in self-supervision to exploit EUREC4A measurements and satellite observations for cloud systems over North Atlantic trades 

Dwaipayan Chatterjee, Sabrina schnitt, Paula Bigalke, Claudia Acquistapace, and Susanne Crewell

The cloud systems of the North Atlantic trades (NAT) have been a topic of curiosity due to significant uncertainty in their physical characteristics, physical process understanding across various spatial and temporal scales, and their impact on the regional climate system. Initial research has provided the causal link for cloud systems having distinct organizational aspects (formerly described as Sugar, Gravel, Fish, and Flower) with the net radiative flux over the region. Questions have been raised about how the changing climate will influence the frequency of occurrence of these cloud regimes and how the net radiative impact will change the regional climate system.

 

However, cloud systems represent a continuous spectrum where not-so-visually distinct systems also occur. Existing clustering mechanisms sort organizations into separate classes. Yet, in reality, the organization often does not align with those pre-defined classes but transitions amongst them or simply occurs in a continuous spectrum. Using two complementary neural networks in self-supervision (without human interference), we investigate the representation learning of cloud systems both in a continuous space describing a cloud system spectrum and in a discreet space aiming to identify distinct cloud systems. 50,000 GOES-ABI cloud optical depth NAT images from 2017 – 2021 covering the EUREC4A study area are randomly cropped to 256 x 256 pixels and sorted/labeled by the machine.

 

We study the climatological representation of EUREC4A’s cloud patterns in the continuous embedding space. We follow the Maria S. Merian ship track inside the feature space matching the ship-based atmospheric remote sensing and ERA5 profiles with the K-nearest satellite images. This analysis examines the consistency of the environmental conditions for cloud systems identified as close to each other in the continuous feature space. We investigate the relationship between the net cloud radiative effect and the radiative flux characteristics in the continuous space, finding a strong functional relationship with the cloud system’s pattern and distributions.

 

In the discrete space, we aim to identify the optimal number of classes that could represent the continuous space. We also aim to understand if these discrete classes correspond to the categories identified in the physical and visual space. Moreover, to better understand the decision of the neural network for a particular cloud pattern, we visualize the network’s focus in the activation space. We find that different self-attention heads of the neural network learn to focus on different semantics of the cloud system distribution.

 

Finally, we found that different regularizations applied during the training of the network directly impact the representation learning of the cloud system, and we show how to use such regularizations to improve the understanding of cloud systems.

How to cite: Chatterjee, D., schnitt, S., Bigalke, P., Acquistapace, C., and Crewell, S.: Complementary approaches in self-supervision to exploit EUREC4A measurements and satellite observations for cloud systems over North Atlantic trades, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12257, https://doi.org/10.5194/egusphere-egu23-12257, 2023.

EGU23-12306 | Posters on site | AS1.8

First applications of the Virga-Sniffer – a new tool to identify precipitation evaporation using ground-based remote-sensing observations 

Heike Kalesse-Los, Anton Kötsche, Andreas Foth, Johannes Röttenbacher, Teresa Vogl, and Jonas Witthuhn

The dominant cloud type in the subtropical Atlantic is the trade wind cumulus with a cloud base located near the lifting condensation level (LCL) below 1 km. Other common clouds in this region with their base above 1 km are stratiform cloud layers or cloud edges near the trade wind inversion at 2-3 km. Precipitation in all these clouds mainly forms at temperatures above freezing point by collision and coalescence. Therefore, precipitation generally occurs as light rain/drizzle from stratiform cloud layers or as showers from well-developed trade wind cumuli. Precipitation underneath a cloud base is often visible as fall streaks. If the precipitation evaporates before reaching the ground, these fall streaks are called virga.

Combined continuous long-term ground-based remote-sensing observations with vertically pointing cloud radar and ceilometer are well-suited to identify these precipitation evaporation fall streaks. Here we show the first application of a new open-source tool, the Virga-Sniffer which was developed within the frame of RV Meteor observations during the ElUcidating the RolE of Cloud–Circulation Coupling in ClimAte (EUREC4A) field experiment in Jan–Feb 2020 in the Tropical Western Atlantic. In the simplest approach, it detects virga from time-height fields of cloud radar reflectivity and time series of ceilometer cloud base height. The Virga Sniffer was applied to RV Meteor observations during EUREC4A and statistical results as well as an evaporation case study are presented. Spectral W-band radar data from a fall streak, identified as virga by the Virga-Sniffer, was used to calculate evaporative cooling rates. Sensitivity studies were performed to investigate the influence of vertical wind and relative humidity uncertainties.  Possible future applications of the Virga-Sniffer within the frame of EUREC4A include detailed studies of precipitation evaporation with a focus on cold pools or cloud organization, or distinguishing moist processes based on water vapor isotopic observations.

How to cite: Kalesse-Los, H., Kötsche, A., Foth, A., Röttenbacher, J., Vogl, T., and Witthuhn, J.: First applications of the Virga-Sniffer – a new tool to identify precipitation evaporation using ground-based remote-sensing observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12306, https://doi.org/10.5194/egusphere-egu23-12306, 2023.

The representation of shallow tradewind cumulus clouds in climate models accounts for the majority of inter-model spread in climate projections, highlighting an urgent need to understand these clouds better. In particular, their spatial organisation appears to cause a strong impact of their radiative properties and dynamical evolution. The precise mechanisms driving different forms of convective organisation which arise both in nature and in simulations are, however, currently unknown.

We show how the continuum of convective organisation states can be analysed as an emergent  property of the embedding space representation learnt by a neural network through unsupervised learning.  Specifically we will use a technique to extract an estimate of the manifold in a high-dimensional space on which possible states of convective organisation lie.  Through composition of reanalysis and observations onto this manifold we are able to extract the characteristics of the atmosphere which coincide with different forms of convective organisation, and further we are able to map transitions between different states of organisation and study how these develop.

We will show results from analysing: a) what the radiative properties of different forms of organisation are, b) what atmospheric characteristics coincide with different forms of organisation and c) what transitions occur when following air-masses along Lagrangian trajectories.  Specifically, we find: a) net radiation changes significantly between different forms of organisation, b) agreement with previous studies on the importance of boundary layer wind-speed and to some degree atmospheric stability, and c) we are able to succinctly capture what transitions occur between regimes.

How to cite: Denby, L.: Charting the realms of Convective Cloud Organisation using Unsupervised Learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12508, https://doi.org/10.5194/egusphere-egu23-12508, 2023.

In January and February 2020, the joint EUREC4A/ATOMIC field campaign took place in the Tropical Atlantic near Barbados, with the goal to advance our understanding of the interplay between clouds, convection and circulation including their role in climate change. Within the scope of this campaign, several unique satellite-based datasets have been collected, including very high-spatial resolution multispectral images with 10x10m² pixel size acquired by polar-orbiting Copernicus Sentinel-2 satellites. In this presentation, the first analysis of these high-resolution observations focused on tropical trade cumuli is given. This cloud type is characterized by small-scale spatiotemporal variability that is unresolved at the spatial resolution of current meteorological satellite imagers.

Using the high-resolution Sentinel-2 observations, we will show the clouds can be considered as individual objects with associated properties, such as shape and size parameters, but also their mean radiative properties. A novel technique will be presented for deriving cloud height from Sentinel-2 observations, which exploits the geometric relationship between cloud objects and their shadows. Furthermore, the cloud fraction and cloud size distribution are calculated for various trade cumulus scenes. The uncertainties arising from choices in our cloud detection scheme will be discussed.

We show that a substantial fraction of clouds has equivalent diameters below the pixel size of commonly used meteorological satellite instruments. Consequently, and consistent with previous studies, the cloud size distribution and domain-average cloud fraction from coarse-resolution satellite imagers are shown to be biased and highly sensitive to pixel resolution. In addition, a large fraction of pixels identified as cloudy contains significant clear-sky contributions, and it is no longer possible to characterize clouds as objects. We will discuss how this affects the accuracy of cloud property determination and biases estimates of cloud radiative forcing.

How to cite: Ritter, O., Bley, S., and Deneke, H.: Object-based characterization of Tropical Trade Cumuli During the EUREC4A/ATOMIC Field Campaign using Sentinel-2 observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13751, https://doi.org/10.5194/egusphere-egu23-13751, 2023.

Cloud resolving models run to equilibrium in idealized simulations of radiative-convective equilibrium often show the deep convection spontaneously transitioning from random organization to a state where convection in aggregated into clusters.  This results in a drier mean state and aggregation could be important for climate sensitivity, and is missing in classical parameterization schemes.  However, the onset and nature of the equilibrium, and the sensitivity to lower boundary conditions, differs dramatically between models that use different representations of moist physics and diffusion parameterizations, and varying dynamical cores.  In order to shed light on this, we develop a highly idealized, spatially explicit, stochastic reactive-diffusive model for the column relative humidity in the tropics.

The model is run to equilibrium and it is found that, depending on the model parameter settings and experimental framework, it can produce equilibrium states where the convection remains random, or states where the convection is highly aggregated. Many results of the full-physics models are reproduced, such as their sensitivity to model resolution and domain size, with aggregation more likely using coarse grid sizes and larger domains. The simple model thus allows to explain these sensitivities of the full physics models, with convective nearest-neighbor distances constrained to decrease with smaller domains or higher resolution, which reduces the spatial heterogeneity of column humidity and makes aggregation less likely.  Expanding on these arguments, we use dimensional analysis to combine the model parameters that describe how sensitive convection is to humidity, the subsidence drying rate, and the spreading of humidity by advection and diffusion processes, along with the domain size and resolution.  Using large ensembles of over 1000 simulations, we demonstrate that aggregation occurs at a precise critical value of the resulting dimensionless parameter, which will refer to as the aggregation number.   We suggest that the aggregation number could prove useful to diagnose the differences between full physics models of the atmosphere. 

How to cite: Tompkins, A. and Biagioli, G.: A dimensionless parameter to predict spontaneous convective aggregation onset in a idealized stochastic-diffusive model of radiative-convective equilibrium, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14609, https://doi.org/10.5194/egusphere-egu23-14609, 2023.

EGU23-14787 | ECS | Orals | AS1.8

Reponse of precipitation to dynamics in global-storm resolving models 

Lucile Ricard, Athanasios Nenes, Claudia Stephan, and Fabrizio Falasca

Most climate models show a precipitation increase with warming that is smaller than the increase in moisture, which requires a weakening of the convective mass flux and a slowing of the overturning circulation. In this study we use global-storm resolving models (DYAMOND models) to identify the systematic relationships between the precipitation, the vertical velocity and the overturning circulation in the tropics. The cloud-resolving simulations that are 40-day long in winter allow us to study the dynamical response of precipitation over a wide range of spatial scales. A data reduction and inference method, δ-MAPS, provides an efficient way to reduce the complexity and dimensionality of high-resolution simulations. We use the domains identified in 2d fields of atmosphere mass content of water vapor – interpreted as regions of homogeneous precipitable water – as preferential domains to derive the isentropic distribution of vertical mass transport and the isentropic streamfunction. The isentropic analysis consists in sorting the air parcels in terms of equivalent potential temperature, which offers a simple representation of the convective overturning. A multiscale decomposition allows us to quantify the contribution of the mesoscale circulation in comparison to the large-scale overturning circulation. Finally, the results are compared between the different DYAMOND models to evaluate the intermodel spread. By doing so, we evaluate to what extent the spread in precipitation in model ensemble may arise from the differences in representation of the overturning circulation at different scales.

How to cite: Ricard, L., Nenes, A., Stephan, C., and Falasca, F.: Reponse of precipitation to dynamics in global-storm resolving models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14787, https://doi.org/10.5194/egusphere-egu23-14787, 2023.

EGU23-14814 | Orals | AS1.8

The WInd VElocity Radar Nephoscope (WIVERN): a candidate mission for the ESA Earth Explorer 11 

Alessandro Battaglia, Anthony Illingworth, Frederic Tridon, Ali Rizik, Paolo Martire, and Filippo Emilio Scarsi

The WIVERN (WInd VElocity Radar Nephoscope) concept, now in Phase 0 of the ESA Earth Explorer program, promises to complement Doppler wind lidar by globally observing, for the first time, the vertical profiles of winds in cloudy areas. The mission will also strengthen the cloud and precipitation observation capability of the Global Observing System by providing unprecedented revisit time of cloud and precipitation vertical profiles. The mission hinges upon a single instrument, i.e., a dual-polarization Doppler W-band scanning cloud radar with a 3 m circular aperture non-deployable main reflector. The WIVERN antenna conically scans a large swath (of about 800 km) around nadir at an off-nadir angle of about 38o at 12 rpm (revolutions per minute). This viewing geometry allows daily revisits poleward of 50°, 50-km horizontal resolution, and approximately 1-km vertical resolution. A key element is the use of closely spaced pulse pairs one of which is H polarised the other V polarised, so that the target does not have time to reshuffle, and, providing there is no significant cross-talk between the two returns, the high velocities associated with wind storms can be retrieved. 

In this paper we will discuss the scientific objectives of the mission and will outline some of the technical challenges of the measuring technique. In particular we will discuss how to correct for wind biases introduced by the satellite motion and wind shear across the beam, how to account for cross-talk between the H and V returns due to depolarisation by meteorological targets, how to calibrate the instrument and how to identify mis-pointing of the antenna that could affect Doppler accuracy. We will also present examples of Level 1 products via an end to end simulations applied to high resolution cloud resolving models and expected performances of the instrument in terms of cloud/precipitation and wind coverage.

How to cite: Battaglia, A., Illingworth, A., Tridon, F., Rizik, A., Martire, P., and Scarsi, F. E.: The WInd VElocity Radar Nephoscope (WIVERN): a candidate mission for the ESA Earth Explorer 11, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14814, https://doi.org/10.5194/egusphere-egu23-14814, 2023.

EGU23-17058 | ECS | Posters on site | AS1.8

Measuring meso-scale gradients in the Arctic during HALO-(AC)³ 

Fiona Paulus, Roel Neggers, Gunilla Svensson, and Michail Karalis

Boundary layer cloud transitions at high latitudes play a key role in Arctic climate change, and are partially controlled by large-scale dynamics such as subsidence. While measuring large- and mesoscale divergence has proven notoriously difficult, the recent NARVAL and EUREC4A airborne campaigns in the subtropics have finally achieved this goal using multiple dropsondes releases in circular patterns. If this method also works at high latitudes is still an open research question, given the considerable differences in atmospheric dynamics. Answering this question was one of the main objectives of the recent HALO-(AC)^3 field campaign near Svalbard in Spring 2022. Circular dropsonde patterns were realized during various research flights by two airplanes, independently sampling Cold Air Outbreaks (CAO) in the Fram Strait with multiple dropsondes. This study presents a first overview of the results. We find that the method indeed yields reliable estimates of mesoscale gradients in the Arctic, yeilding robust vertical profiles of both subsidence and vorticity. Sensitivity to aspects of the method is investigated, including dependence on sampling area and the divergence calculation. Ongoing work to drive targeted Lagrangian high resolution simulations of the observed CAOs exclusively with HALO-(AC)³ data will be briefly discussed.

How to cite: Paulus, F., Neggers, R., Svensson, G., and Karalis, M.: Measuring meso-scale gradients in the Arctic during HALO-(AC)³, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17058, https://doi.org/10.5194/egusphere-egu23-17058, 2023.

EGU23-17350 | ECS | Orals | AS1.8

On the properties of greenCu: continental, organized shallow clouds 

Tom Dror, Ilan Koren, Orit Altaratz, Michael D. Chekroun, and Vered Silverman

Prevalent over the world’s oceans and continents, shallow clouds still comprise a main aspect of the uncertainty related to cloud feedback and climate sensitivity. Compared to shallow clouds over the ocean, confined to specific marine environments, shallow cumulus (Cu) over land occur in diverse locations throughout the globe.

Motivated by an intriguing observation regarding the universality of continental shallow Cu fields regardless of their geographical location, we explore their similarities. We combine satellite observations, along with machine learning classification and numerical modelling to show that these cloud fields share many important properties, such as the patterns they form and their tendency to form over and near forests and vegetated lands, thus termed greenCu.

Moreover, we show that in spite of their occurrence in different climatic regions, from the tropics to mid- and high-latitudes, greenCu fields are associated with similar large-scale meteorological conditions.

How to cite: Dror, T., Koren, I., Altaratz, O., Chekroun, M. D., and Silverman, V.: On the properties of greenCu: continental, organized shallow clouds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17350, https://doi.org/10.5194/egusphere-egu23-17350, 2023.

Spring precipitation over the southeastern Tibetan Plateau (SETP) produces more than 34% of annual precipitation, which is comparable to summer precipitation. This pre-monsoon rainfall phenomenon, influenced synthetically by atmospheric circulations and topography, makes the SETP an exception to its surroundings. Here, fine-scale characteristics and typical synoptic backgrounds of this unique phenomenon have been investigated. The spring precipitation over the SETP is characterized by high frequency at hourly scale, with a single diurnal peak at night. Event-based analysis further demonstrates that the spring precipitation is dominated by long-lasting nocturnal rainfall events. From early to late spring, the dominant synoptic factor evolves from terrain-perpendicular low-level winds to atmospheric moisture, influencing the spatial heterogeneity and fine characteristics of the spring precipitation. The westerly-dominated type, featured by lower geopotential height over the TP and enhanced westerlies along the Himalayas, produces limited-area precipitation at those stations located at topography perpendicular to low-level winds. In contrast, the moisture-dominated type is featured by an anomalous cyclone over the Bay of Bengal and induces widespread precipitation around the SETP, which is the leading contributor to the spring precipitation there. Due to the moist environment and weak instability, the spring precipitation influenced by the moisture-dominated type is characterized by long-lasting nocturnal events, with a large portion of weak precipitation. Findings revealed in this study complete the picture of spring precipitation influenced by different dominant synoptic factors over the SETP, which deepen the current understanding of the joint influence of circulation and topography on the hydrological cycle of complex terrains.

How to cite: zhao, Y., li, J., ren, L., li, N., and li, P.: Fine-scale characteristics and dominant synoptic factors of spring precipitation over complex terrain of the southeastern Tibetan Plateau, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1347, https://doi.org/10.5194/egusphere-egu23-1347, 2023.

The seasonal migration of the Intertropical Discontinuity (ITD) is critical for monitoring seasonal moist convective processes and associated rainfall over West Africa. This study constitutes a new analysis of the seasonality of moist convection over West Africa, relative to the ITD, based on NASA's Atmospheric Infrared Sounder (AIRS) measurements from 2003-2018. Results show that AIRS resolves the seasonal march of the ITD, including its inherent diurnal-scale variations. AIRS captures the north - south daytime skin temperature dipole around the ITD, with greater relative temperatures to the north, especially during March - August. In the vicinity of the nighttime ITD, AIRS profiles indicate increased instability that is characteristic of nocturnal thunderstorm propagation. On thunderstorm days, the mean latitude of the AIRS-derived ITD is displaced 3o , 0.2o, and 2o north of its DJF, MAM, and SON climatological positions, respectively, and 1.2o south in JJA. The findings of this study are critical to building local tropical weather forecasting capacity and capabilities in West Africa.

How to cite: Osei, M.: Observation of the moist convective environment of West Africa by the Atmospheric InfraRed Sounder, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1683, https://doi.org/10.5194/egusphere-egu23-1683, 2023.

EGU23-3406 | ECS | Posters on site | AS1.9

Enhanced climatology of large hail in the UK: Radar-derived diurnal cycle and storm mode 

Henry Wells, John Hillier, Freya Garry, Nick Dunstone, Huili Chen, Abdullah Kahraman, William Keat, and Matthew Clark

Large hail, with a diameter of at least 20 mm, is a hazard associated with severe convective storms (SCS) that can cause significant damage. Understanding of atmospheric environments conducive to large hail is underpinned by catalogues of past events. Because of the small footprint of hail events, these often rely on crowdsourced reports. In the UK, the relative rarity of large hail and low public awareness of SCS hazards makes obtaining a complete set of reports difficult, and in many cases the precise time of the hail is not recorded. In this study, the two major databases of UK large hail reports are merged for the first time. Composite radar reflectivity data are used to verify and enhance 260 reports since 2006. Time of the hail and the basic storm mode (isolated, clustered or linear) are visually estimated from animations. Compared to the UK’s most severe historic hailstorms (1800–2004), our quality controlled climatology of all sizes of large hail shows a diurnal cycle with a slightly broader peak. Around 55% of large hail events are associated with isolated cells, while 34% have supercellular characteristics, a much lower proportion than found in the USA. The full event set (1979–2022), comprising over 850 reports, is used to update the seasonal, spatial and size distributions of large hail in the UK. We intend that this hail event set forms part of a multi-hazard analysis of UK SCS, also including tornadoes and extreme rainfall, and its relationship to background atmospheric conditions. The effect of climate change on UK SCS will be investigated through past and future trends in these background conditions.

How to cite: Wells, H., Hillier, J., Garry, F., Dunstone, N., Chen, H., Kahraman, A., Keat, W., and Clark, M.: Enhanced climatology of large hail in the UK: Radar-derived diurnal cycle and storm mode, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3406, https://doi.org/10.5194/egusphere-egu23-3406, 2023.

EGU23-4332 | Orals | AS1.9

A Merger-Formation Bow Echo Caused by Low-Level Mesovortex in South China 

Qiqing Liu, Xin Xu, Kun Zhao, and Ang Zhou

Based on operational radar observations and high-resolution analyses from the Variational Doppler Radar Analysis System (VDRAS), a bow echo producing high-winds and heavy rainfall that occurred over South China in the pre-rainy season is studied. Results show that this bow echo developed from a quasi-linear convective system (QLCS) and acquired a well-defined bow shape after merging with a pre-line convective cell (CC). Interestingly, the rear-inflow jet (RIJ), which has been well recognized to play a key role in the formation of a bow echo, was absent in this merger-formation bow echo (MFBE). This is ascribed to the weak cold pool and line-end vortices generated within the QLCS as it developed in the monsoon environment of high humidity and weak low-level vertical wind shear.

A new pathway of bow echo formation was proposed instead, which highlighted the importance of the low-level mesovortex (MV) on the leading edge of the QLCS. The MV originated from a weak vertical vorticity band ahead of the QLCS. Vertical vorticity budget analyses revealed that the enhanced stretching effect during the QLCS-CC merger was the main cause of the growth of the MV. The well-developed MV thereby provided a RIJ-like flow wrapping cyclonically from north of the QLCS, forcing the QLCS to distorted into a bow echo. This MV contributed foremost to the near surface gales as well.

Combined with the well-resolved dynamical processes aforementioned, observations from an S band polarimetric radar are employed, aiming to uncover the microphysical and dynamical structures and their interaction processes accounting for the heavy rainfall. The precipitation was shown to be featured of high concentration of large hydrometeors, with maxima basically limited within the intensified MV. The deep QLCS developing far above the freezing level favored for significant ice-phase processes, further enhancing rain rate through melted graupel and hail. High spatiotemporal correlation between the precipitation extremes and the MV suggests the non-negligible role the MV played to determine the microphysics process of this precipitation, which required more detailed researches next.

How to cite: Liu, Q., Xu, X., Zhao, K., and Zhou, A.: A Merger-Formation Bow Echo Caused by Low-Level Mesovortex in South China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4332, https://doi.org/10.5194/egusphere-egu23-4332, 2023.

EGU23-5208 | ECS | Posters on site | AS1.9 | Highlight

Dynamical Impacts of Warm-Starting Operational Weather Models over Africa 

Fran Morris, James Warner, Caroline Bain, Juliane Schwendike, Doug Parker, and Jon Petch

Weather models which allow explicit convection can add value to weather forecasting by improving the intensity and timing of precipitating systems and their dynamics, which is particularly valuable in the tropics where moist diurnal convection dominates. In West Africa, convection can become organised to form mesoscale convective systems which are crucial for supplying water but may have devastating impacts, and while convection-permitting models improve forecasts, issues remain in the implementation of operational convection-permitting models. A major problem is initialising weather models in the tropics, where measurements are sparse and weather systems are dominated by nonlinear diabatic processes, which makes data assimilation challenging. Currently, the UK Met Office runs a regional operational convection-permitting model in Africa, the Tropical Africa Model, which is initialised using lower-resolution global models. However, the global models have extremely limited convective-scale structures and as a result, there is a spin-up time of around 12-18 hours before the model begins to accurately reflect precipitation.

To counteract this problem, a “warm-starting” method has been trialled. The warm-starting technique blends large-scale features from the global model and fine-scale fields below a certain length scale from previous runs of the high-resolution model to use as an initial state in a new model run. It combines the more realistic convective structures of the regional model and the more accurate synoptic conditions in the global model. Not only is the approach cheaper and quicker than traditional data assimilation, both in terms of development and computational cost, but it also shows demonstrable improvements in the representation of precipitation for the first 12 hours of the model and beyond relative to simulations where the model has simply been initialised with the global model (a “cold-start”). The cold-start simulations appear to consistently predict rainfall that is too intense even beyond the first 12 hours.

We investigate why warm-starting models produces more realistic rainfall distributions by examining the dynamical structures: producing statistics of rainfall objects as forecasts evolve and examining their connection to the dynamics. We examine the energetics of convection in the convection-permitting models, aiming to provide a justification for the scale length at which we include structure from previous model runs using this technique.

How to cite: Morris, F., Warner, J., Bain, C., Schwendike, J., Parker, D., and Petch, J.: Dynamical Impacts of Warm-Starting Operational Weather Models over Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5208, https://doi.org/10.5194/egusphere-egu23-5208, 2023.

EGU23-5258 | ECS | Orals | AS1.9

Comparison of Mesoscale Convective Systems in a Seasonal Convection-Permitting Simulation With Observations Over the Indian Monsoon Zone 

Manisha Tupsoundare, Sachin Deshpande, Zhe Feng, Medha Deshpande, Subrata Kumar Das, and Harshad Hanmante

The largest type of deep convection, mesoscale convective systems (MCSs), regulate changes in the hydrological cycle and large-scale tropical circulation. During the Indian summer monsoon (June-September), synoptic-scale systems move across the monsoon zone, causing MCSs to form frequently. MCSs cause widespread and heavy rain throughout the monsoon zone. Past MCS studies in India used either observations or simulation in a short period or with case studies approach. Studies on structure and evolution of MCSs highlighting the organization of convection over the monsoon zone are lacking.

In this study, a 4-month, convection-permitting simulation is conducted over the Indian monsoon zone using the Weather Research Forecast (WRF) model with 4-km grid spacing and two microphysics parameterizations and is compared with observations to evaluate composite MCS characteristics and microphysics sensitivities. We first apply a cloud-tracking algorithm to two high-resolution observation data sets, NASA global merged infrared brightness temperature (IR Tb) and GPM IMERG surface precipitation to identify and track individual MCS events during monsoon. Ground-based S-band radar observations are used to examine the 3-D structures of storms embedded within the tracked MCSs and analyze evolution of convective, stratiform and anvil components of the MCSs. A similar cloud-tracking algorithm is then applied to WRF simulated data (radar reflectivity, IR Tb and precipitation) to identify and track MCS in model simulation. As a result, the observed and simulated MCSs are consistently identified and tracked, making it possible to compare WRF MCS population statistics with observed MCSs.

Results show that the properties of MCS including composite evolution, and frequency distribution are reasonably captured by the two simulations with some noticeable differences. In general, the Thompson simulation produces better agreement with observations for convective area and precipitation amount, MCS propagation speed but exhibits underestimation of stratiform area. The composite evolution of simulated MCS cloud and precipitation structures showed a gradual increase from convective initiation to around the first half of the MCSs lifetime, which was consistent with observations. The MCS eccentricity reaches to minimum value at maximum horizontal extent, indicating a quasi-circular shape of MCS. We observed that PDF of MCS precipitation intensity largely agrees well with observations. The highest altitude reached by intense convective cores (30-dBZ echo-tops) is 8 km, but the model significantly underestimates it. The detailed comparison of multiple aspects of MCSs (e.g., initiation, size, intensity, lifetime, propagation) and embedded storms (e.g., convective-stratiform areas) and associated precipitation between the simulation and observations for one monsoon season will be discussed.

How to cite: Tupsoundare, M., Deshpande, S., Feng, Z., Deshpande, M., Das, S. K., and Hanmante, H.: Comparison of Mesoscale Convective Systems in a Seasonal Convection-Permitting Simulation With Observations Over the Indian Monsoon Zone, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5258, https://doi.org/10.5194/egusphere-egu23-5258, 2023.

EGU23-5342 | ECS | Orals | AS1.9

Sensitivity of simulated mesoscale convective systems over East Asia to the treatment of convection in a high-resolution GCM 

Puxi Li, Mark Muetzelfeldt, Reinhard Schiemann, Haoming Chen, Jian Li, Kalli Furtado, and Moran Zhuang

Mesoscale convective systems (MCSs) downstream of the Tibetan Plateau (TP) exhibit unique precipitation features. These MCSs can have damaging impacts and there is a critical need for improving the representation of MCSs in numerical models. However, most global climate models are typically run at resolutions that are too coarse to reasonably resolve MCSs, and it is still unclear how well higher-resolution global models can reproduce the precipitation characteristics of MCSs. In this study, the sensitivity of MCSs simulated by a global high resolution (~10km), atmosphere-only climate model to different treatments of convection (with and without parametrized convection, and a hybrid representation of convection) have been investigated. The results show that explicit convection (i.e., non-parameterized) can better reproduce the observed pattern of MCS precipitation over the East Asian Summer Monsoon (EASM) region. In general, explicit convection better simulates the diurnal variability of MCSs over the eastern China, and is able to represent the distinctive diurnal variations of MCS precipitation over complex terrain particularly well, such as the eastern TP and the complex terrain of central-northern China. It is shown that explicit convection is better at simulating the timing of initiation and subsequent propagating features of the MCS, resulting in better diurnal variations and further a better spatial pattern of summer mean MCS precipitation. All three experiments simulate MCS rainfall areas which are notably smaller than those in observations, but with much stronger rainfall intensities, implying that these biases in simulated MCS morphological characteristics are not sensitive to the different treatment of convection.

How to cite: Li, P., Muetzelfeldt, M., Schiemann, R., Chen, H., Li, J., Furtado, K., and Zhuang, M.: Sensitivity of simulated mesoscale convective systems over East Asia to the treatment of convection in a high-resolution GCM, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5342, https://doi.org/10.5194/egusphere-egu23-5342, 2023.

EGU23-6107 | ECS | Posters on site | AS1.9 | Highlight

Deforestation and changes in rainfall across the Amazon – reducing uncertainty using a continental scale convection permitting domain 

Richard Bassett, Luis Garcia-Carreras, Douglas Lowe, Lincoln Alves, Gilberto Fisch, Kate Halladay, Ron Kahana, and José Veiga

The Amazon rainforest holds more than 40% of all remaining tropical rainforest and is a key component of the climate system. The scale of deforestation in the Amazon significantly impacts both local and global climates. Under a business-as-usual scenario as much as 40% of the Brazilian Amazon rainforest will be lost by 2050. Despite the magnitude of these changes and its importance, the overall effects of deforestation on rainfall remain uncertain. Land-use change influences rainfall through a variety of mechanisms acting at local to continental scales. As such, previous research indicates conflicting responses to rainfall depending on the scales studied. In reality, rainfall processes interact across these scales, but until recently have been impossible to capture within a single model due to computational expense. Consequently we are unable to rely on these simulations as future estimations of rainfall for such a sensitive and anthropogenically impacted region as the Amazon.

 

In this study, we overcome these limitations by running convection permitting simulations (horizontal resolution 4.5km) over a large domain (6000km covering the majority of South America) using a Tropical configuration of the UK Met Office Unified Model. The high-resolution and continental-scale of these simulations present an opportunity to reduce the uncertainty in Amazonian rainfall estimates within a single model and ensures rainfall processes and interactions across scales are captured. To investigate the impacts of deforestation we will include a series of land-use sensitivity runs making use of a range of socioeconomic scenarios to 2050. Here we present initial results from our simulations, indicating how localised storms, mesoscale convective systems and large-scale circulations respond to land-use change.

How to cite: Bassett, R., Garcia-Carreras, L., Lowe, D., Alves, L., Fisch, G., Halladay, K., Kahana, R., and Veiga, J.: Deforestation and changes in rainfall across the Amazon – reducing uncertainty using a continental scale convection permitting domain, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6107, https://doi.org/10.5194/egusphere-egu23-6107, 2023.

EGU23-6994 | Posters on site | AS1.9

Grid spacing effects on convection initiation and aerosol-cloud interactions: A case study of a supercell storm from the Swabian MOSES 2021 field campaign 

Christian Barthlott, Beata Czajka, Martin Kohler, Corinna Hoose, Michael Kunz, Harald Saathoff, and Hengheng Zhang

The predictability of deep moist convection is subject to large uncertainties, mainly due to inaccurate initial and boundary data, incomplete description of physical processes, or uncertainties in microphysical parameterizations. In this study, we present hindcasts of a supercell storm that occurred during the Swabian MOSES field campaign in southwestern Germany in summer 2021. The supercell storm of 23 June 2021 passed directly over the main observation site equipped with various instruments, allowing a detailed comparison of simulations and observations. The preconvective radiosonde observations revealed suitable conditions for supercell development, i.e., low convective inhibition, moderate convective available potential energy, sufficient deep-layer shear, and a Bulk Richardson number of 22. Numerical simulations were performed with the ICOsahedral Non-hydrostatic (ICON) model using two horizontal grid spacings (i.e., 2 km/1 km) with a single-moment and a double-moment microphysics scheme. The double-moment scheme allows us to study aerosol effects on clouds and precipitation with cloud condensation nuclei (CCN) concentrations ranging from low to very high. Numerical results show that all 2-km model realizations do not simulate convective precipitation at the correct location and time. For the 1-km grid spacing, changes in aerosol concentration resulted in large changes in convective precipitation, causing the supercell to disappear completely in some simulations. Only the 1-km model run, which assumes a clean environment, is able to realistically capture the supercell storm. During the Swabian MOSES field campaign, aerosol particle concentrations and size distributions were continuously measured with an optical particle counter from June to August 2021. The day of the supercell storm was characterized by the lowest potential CCN values of the month, suggesting that the low aerosol concentration in the successful model run is a reasonable assumption for this case study. Possible reasons for the discrepant model results, i.e., effects of grid spacing on convection initiation and detailed analyses of microphysical process rates, are discussed. These results demonstrate the benefits of using an aerosol-aware double-moment microphysics scheme at high model resolution for convection initiation and cloud evolution, and that the use of different CCN concentrations can determine whether a supercell is successfully simulated or not.

How to cite: Barthlott, C., Czajka, B., Kohler, M., Hoose, C., Kunz, M., Saathoff, H., and Zhang, H.: Grid spacing effects on convection initiation and aerosol-cloud interactions: A case study of a supercell storm from the Swabian MOSES 2021 field campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6994, https://doi.org/10.5194/egusphere-egu23-6994, 2023.

EGU23-9500 | Posters on site | AS1.9

Investigating links among heatwaves, precipitation, and land use types using the Convection-Permitting Model in the Southwest UK for the 2022 boreal summer 

Kwok Pan Chun, Yasemin Ezber, Emir Toker, Michelle Simões Reboita, Rosmeri Porfirio da Rocha, Bayu Christoforus Risanto, Omer Yetemen, Thanti Octavianti, Nevil Quinn, Omer Lutfi Sens, and Christopher Castro

To improve sub-seasonal forecasts, different global initiatives generate continental convection-permitting simulations for resolution less than 10 kilometres for multiple decades. These simulations, however, are based on land use maps with only single urban type. In this study, we explore how the density and height information of the urban canopy based on Local Climate Zones (LCZs) affect the dynamics among temperatures, precipitation and land use types for the 2022 summer heatwave in the Southwest UK. Four numerical experiments at a 3 km grid are run by switching off the parameterization of deep-convection in the Weather Research and Forecasting (WRF) models. These experiments are based on (i) the no urban scenario, (ii) the default MODIS land use scheme, (iii) the building environment parameterization (BEP), and (iv) the building energy model (BEM).

Results show that the cold advection over the UK led to downward motion according to a Q-vector analysis. The regional downward motion caused the formation of a heat dome. It is against the hypothesis that the 2022 summer heatwave was due to the hot circulation from Spain and equatorial Africa. Even though four land use schemes have similar simulated cold advection across the UK, our findings show that land use types affected water recycling due to local convection differently. These differences were related to the strength of rainstorms at the dissipating heatwave stage. Our results suggest that urban areas were more likely to have more persistent heatwaves since the intensity of rainstorms was affected by the lower local water recycling. This advanced understanding of the UK heatwave mechanism based on regional advection conditions and local convection processes will guide us on how to improve our sub-seasonal forecast in the urban area.

How to cite: Chun, K. P., Ezber, Y., Toker, E., Simões Reboita, M., Porfirio da Rocha, R., Risanto, B. C., Yetemen, O., Octavianti, T., Quinn, N., Sens, O. L., and Castro, C.: Investigating links among heatwaves, precipitation, and land use types using the Convection-Permitting Model in the Southwest UK for the 2022 boreal summer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9500, https://doi.org/10.5194/egusphere-egu23-9500, 2023.

EGU23-10212 | ECS | Orals | AS1.9 | Highlight

Severe hail in France: reconstruction of Storm Ela’s and late June 2022 hailstorms 

Davide Panosetti, Christopher Allen, Obaidullah Yaqubi, and Orane Thollon

Hail is by far the greatest contributor to insured losses from severe convective storms on an annual basis. Individual severe convective storm outbreaks can cause hail losses well above EUR 1 bn. In May and June 2022 a series of such events impacted France, Germany and Belgium. Of these, those occurring on 19-22 June 2022 were particularly damaging as they hit the large metropolitan region of Ile-de-France. There were many reports of large hailstones, causing significant damage to property and motor vehicle. Total insured hail loss estimates in France alone exceeded EUR 2.4 bn, of which EUR 1.34 bn of property loss and EUR 1.08 bn of motor vehicle loss. These were the largest hail events in France in terms of losses since Storm Ela’s, which on 9-10 June 2014 resulted in insured hail losses in excess of 900 mn in 2021 EUR.

Common denominator to these two impactful events were persistent meteorological situations conducive to large-scale severe convective storms for several consecutive days. These compounded with local conditions favorable for the development of severe hail. Maximum hailstone sizes of 12 cm in diameter were observed in the administrative regions of Centre-Val-De-Loire (Ela) and Occitanie (June 2022). In this study we present a reconstruction of these events based on eye-witness reports cross-referenced with weather radar data. We analyze the synoptic configurations and pre-convective environments that characterized them, with particular focus on those properties and features that are peculiar to severe hail-forming thunderstorms. These event reconstructions are part of our effort to construct a Realistic Disaster Scenario (RDS) model for France and Belgium to stress test both individual client portfolios and the market as a whole.

How to cite: Panosetti, D., Allen, C., Yaqubi, O., and Thollon, O.: Severe hail in France: reconstruction of Storm Ela’s and late June 2022 hailstorms, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10212, https://doi.org/10.5194/egusphere-egu23-10212, 2023.

The topography plays an essential role in initiation and development on precipitating clouds, therefore has a profound effect on the ultimate spatial distributions of precipitation. This study investigates the fine-scale characteristics of synoptic-induced precipitation over Southwest China, a region characterized by a sequence of steep mountains aligned roughly north-south. Based on the convection-permitting simulation for a realistic case, the results show that the model successfully reproduces the observed precipitation, which is induced by a low-level shear line over Southwest China. The spatial distribution of precipitation over three small-scale mountains (named as M1, M2 and M3 from east to west) exhibits distinct inhomogeneity. The precipitation is notably enhanced on the leeward slope of M1, the high-altitude area of M2, as well as the windward slope of M3, which is driven by the steep topography relief, through exerting dominant influences on the local atmospheric circulations. Further results of the high-resolution experiment shows that the thermal instabilities and topographic lifting over the high-altitude ridges are beneficial to the enhanced precipitation. In addition, the small-scale vortex generated on the leeward slope of M1, as well as the convergence zones established over M2 and the windward slope of M3, dynamically contribute to the intensification of precipitation over these three small-scale mountains. In sensitivity simulation with the terrain height of M2 reduced to the comparable height as the other two mountains, the enhanced precipitation decreases significantly over M2. The dynamic blocking effect of M2 on airflow is weakened, leading to the maximum precipitation over M3 moving to its mountaintop.

How to cite: Zhang, M., Li, J., and Li, N.: Spatial inhomogeneity of synoptic-induced precipitation in a region of steep topographic relief, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10335, https://doi.org/10.5194/egusphere-egu23-10335, 2023.

It has been known that potential vorticity (PV) diagnostics can be employed to (a) evaluate large-scale dynamics of hurricane movement, and (b) assess the storm’s influence on its own track. Moreover, PV variations and temperature adjustments at the tropospheric interior and the associated general circulation theory are closely related to the surface PV. Diagnosis of the surface PV is, however, complicated due to data availability/coarse-resolution configurations across the wide terrain in topographic regions. In this work we develop a high-resolution configuration for the Gulf of Mexico (GoM) region for employing in the Weather Research and Forecasting (WRF) model to study Hurricanes Harvey and Ida. The new configuration includes horizontal resolutions of 5 km and 1.67 km in the main and nest domains, respectively; 55 vertical heights (potential pressure levels) are also considered. Forecasts of Hurricane Harvey for 132-hours (5days + 12 hrs), and Hurricane Ida for 78-hours (3days + 6 hrs) are performed, and outputs are stored at every 15 minutes. It is shown that surface PV changes its sign when the Hurricane Harvey/Ida arrives over the land while PV at high altitudes are conserved. We show that the surface PV change is due to the change of vertical temperature gradient at the surface (i.e. change of surface layer stability). These dynamical evolutions are coincident with an increase in precipitation rate and accumulated precipitation of hurricane aftermath. We discuss how these meteorological processes can possibly influence hurricane movements.

How to cite: Khani, S. and Dawson, C. N.: Potential vorticity and surface layer stability in hurricane movement: case studies of Hurricanes Harvey and Ida, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11156, https://doi.org/10.5194/egusphere-egu23-11156, 2023.

EGU23-11509 | ECS | Posters on site | AS1.9

A study on the diurnal variation of the snowfall structure in the western coastal region of the Korean Peninsula. 

Soojin Yoo, Eun-Chul Chang, and GyuWon Lee

 On the western coastal region of the Korean Peninsula in the winter, heavy snowfall occurs due to air mass modification which is called the western coast snowfall. The western coast snowfall occurs through a mechanism similar to the lake effect snowfall that is formed over the Great Lakes in the North America. In the winter season, cold and dry northwesterly wind blowing from the south-eastern flank of the Siberian High is formed over the Yellow Sea. The cold and dry air mass from the continent gets heat and moisture from the ocean when it passes over the relatively warm sea surface, , which invigorate snow clouds. The snow clouds generated over the ocean flow into the western coastal region by the westerly winds, hence predicting when the snow clouds flow into the land is important for snowfall forecast. Although the western coast snowfall can persist for several days when the synoptic environment is maintained, diurnal fluctuations in snowfall inflow appears during the snowfall cases. In this study, the diurnal variation of snowfall inflow on the western coastal region was investigated by analyzing of the dynamic/thermodynamic factors affecting the diurnal variation. The western coast snowfall shows snowfall inflow into the land in the evening, then inflow decreases after sunrise, with the snowfall becoming concentrated over the ocean, and the snowfall inflow increases after sunset. The diurnal variation of the snowfall inflow structure appears with the diurnal variation of the dynamic/thermodynamic structure according to the solar radiation diurnal cycle. During the evening, as the temperature of the lower troposphere over the land decreases due to radiative cooling, the lower troposphere thermal stability increases. After sunrise, the planetary boundary layer (PBL) height grows due to radiative heating, and the wind in the lower troposphere weakens, limiting the snowfall inflow to 9 LST, where both factors affect simultaneously. In addition, as the lower troposphere temperature over the land decreases, the land-sea horizontal temperature contrast increases, and the density wall of the colder land blocks the inflow of the snowfall. On the other hand, during the daytime, the lower troposphere temperature of the land rises due to radiative heating and the thermal stability decreases. As the horizontal temperature contrast decreases and the PBL height decreases after sunset, the lower troposphere wind becomes stronger, which allows the snowfall penetrates into the land. According to the time lag in heating/cooling by radiation of the lower troposphere, it is analyzed that the time point of snowfall inflow interruption (increasing) appears after sunrise (sunset).

 

Acknowledgement

This work was supported by the National Research Foundation of Korea (NRF) grant funded by the Korea government(MSIT) (No. 2021R1A4A1032646).

How to cite: Yoo, S., Chang, E.-C., and Lee, G.: A study on the diurnal variation of the snowfall structure in the western coastal region of the Korean Peninsula., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11509, https://doi.org/10.5194/egusphere-egu23-11509, 2023.

EGU23-14475 | ECS | Posters on site | AS1.9

Changes in land surface effects on organised convection in a convection-permitting climate projection 

Cornelia Klein, Emma Barton, and Christopher Taylor

Convection-permitting (CP) climate simulations represent a major advance in capturing land surface effects on convection. From observational analyses in West Africa, we know that land surface conditions are a major driver of storm initiation as well as intensification during later stages of the storm life cycle. Dry soils of 10 km to several 100s of km scale can cause anomalous warming of the planetary boundary layer and affect horizontal circulations, regional moisture convergence as well as instability. However, to date it remains unclear whether, in a warming climate, larger and more intense storms may change the scale and frequency of surface patterns, feeding back on these identified processes. Here, we evaluate the ability of a pioneering convection-permitting (4.4km) pan-African climate simulation to capture the observed land effects on the pre-convective environment in West Africa and subsequent storm characteristics. This is compared to a CP climate projection representing a decade under a very high emission scenario around 2100 in order to reveal potential changes in process interactions and consequences for organised convection in the future. 

How to cite: Klein, C., Barton, E., and Taylor, C.: Changes in land surface effects on organised convection in a convection-permitting climate projection, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14475, https://doi.org/10.5194/egusphere-egu23-14475, 2023.

EGU23-14661 | ECS | Posters on site | AS1.9

Analysis of the impact of selected sources of uncertainty on precipitation simultaions of summer convection over Central Europe 

Beata Czajka, Christian Barthlott, Martin Kohler, Andreas Wieser, and Corinna Hoose

In this study we investigate the impact of several selected sources of uncertainty on convective precipitation prediction. For this purpose, we conduct numerical simulations with the ICOsahedral Non-hydrostatic (ICON) model for two consecutive days in June, 2021, on which deep moist convection triggered by different synoptic forcing occurred over southwestern Germany. We use single- and double-moment microphysics schemes and vary the initial soil moisture, grid spacing, and cloud condensation nuclei (CCN) concentration. We compare the results with measurements conducted on the same two days during the Swabian MOSES (Modular Observation Solutions for Earth Systems) field campaign. We find that the applied dry bias (initial soil moisture in the model reduced by 25%) much better represents the actual soil moisture conditions and leads to an improved quantitative precipitation forecast when compared to radar-derived precipitation amounts. Furthermore, the model resolution impacts the precipitation amount, intensity, and the timing of convection initiation: while 1-km runs show the least root mean square error for 24-hour precipitation sums, the onset of convective precipitation in 2-km resolution runs matches better the observations. However, the overall impact of this factor is not always systematic. The comparison of several radiosounding-derived convective indices (e.g. lifted index, convective available potential energy, convective inhibition) with model data yield many non-systematic results. For instance, CCN concentrations do not seem to have any significant impact on any of the calculated indices. At the same time, runs with coarser resolution (2-km) often better depict the temporal development of CAPE but overestimate its amount.

How to cite: Czajka, B., Barthlott, C., Kohler, M., Wieser, A., and Hoose, C.: Analysis of the impact of selected sources of uncertainty on precipitation simultaions of summer convection over Central Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14661, https://doi.org/10.5194/egusphere-egu23-14661, 2023.

EGU23-15734 | ECS | Posters on site | AS1.9

Do Mesoscale Convective Systems precipitation follows the Clausius-Clapeyron relationship? 

Nicolas Da Silva and Jan Haerter

Floods related to heavy precipitation are common over Europe during both the warm and the cold seasons. In a way to better understand these heavy precipitation systems and their potential evolution in a warming climate, several studies investigated the dependency of precipitation extremes to temperature over Europe (e.g. Lenderink et al., 2008; Berg et al., 2013). It was found that the scaling of precipitation extremes can exceed the scaling expected from the Clausius-Clapeyron (CC) relationship, relating temperature to the water holding capacity of the atmosphere. While several potential explanations were proposed, a recent study (Lochbihler et al., 2017) noted the important role of large systems in determining this “super-CC” scaling over the Netherlands.

Building on this study, we further investigate the role of Mesoscale Convective Systems (MCS) in determining the temperature precipitation relationship over Europe. The detection and tracking of MCSs is based on the recent Integrated Multi-satellitE Retrievals for Global Precipitation Measurement (IMERG; Huffman et al., 2019) satellite precipitation climatology. We use the EUropean Cooperation for LIghtning Detection (EUCLID) lightning dataset to distinguish between stratiform (or shallow convective) and deep convective rain patches without introducing bias in precipitation intensity. We select the temperature upstream of the MCS tracks, as a proxy of the moisture source involved in the formation of MCS precipitation.

MCS can display strong dynamical features such as the rear inflow jet or cold pools, of which the effects on precipitation as well as their changes with temperature are still unclear. It suggests that MCS precipitation may deviate significantly from the CC scaling. Additionally, the processes involved in MCS precipitation may differ depending on the stage of the MCS life cycle. We thus characterize the temperature dependency of MCS precipitation and their 2-D structure at different stages of their life cycle. This work contributes to better understanding the drivers of MCS precipitation and how these may evolve in a warming climate.

References

Berg, P., Moseley, C., & Haerter, J. O. (2013). Strong increase in convective precipitation in response to higher temperatures. Nature Geoscience, 6(3), 181-185.

Huffman GJ, Stocker EF, Bolvin DT, Nelkin EJ, Tan J. 2019. GPM IMERG final precipitation L3 half hourly 0.1 degree x 0.1 degree V06, Greenbelt, MD, Goddard Earth Sciences Data and Information Services Center. doi: 10.5067/GPM/IMERG/3B-HH/06

Lenderink, G., & Van Meijgaard, E. (2008). Increase in hourly precipitation extremes beyond expectations from temperature changes. Nature Geoscience, 1(8), 511-514.

Lochbihler, K., Lenderink, G., & Siebesma, A. P. (2017). The spatial extent of rainfall events and its relation to precipitation scaling. Geophysical Research Letters, 44(16), 8629-8636.



How to cite: Da Silva, N. and Haerter, J.: Do Mesoscale Convective Systems precipitation follows the Clausius-Clapeyron relationship?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15734, https://doi.org/10.5194/egusphere-egu23-15734, 2023.

EGU23-16303 | ECS | Orals | AS1.9 | Highlight

Environmental Precursors to Mesoscale Convective Systems 

Mark Muetzelfeldt, Robert Plant, and Hannah Christensen

Mesoscale convective systems (MCSs) are important components of the Earth’s weather and climate systems. They produce a large fraction of tropical rainfall and their top-heavy heating profiles can feedback onto atmospheric dynamics. Understanding the large-scale environmental precursor conditions that cause their formation is normally done as case studies or on a regional basis. Here, we take a global view on this problem, linking tracked MCSs to the environmental conditions that lead to their growth and maintenance. We consider common variables associated with deep convection, such as CAPE, total column water vapour and moisture convergence. We take care to distinguish between conditions associated with deep convection, and conditions associated with MCSs specifically. Furthermore, we pose the question in a way that is useful for the development of an MCS parametrization scheme, by asking what environmental conditions lead to MCS occurrence, instead of locating an MCS and then finding the associated conditions.

How to cite: Muetzelfeldt, M., Plant, R., and Christensen, H.: Environmental Precursors to Mesoscale Convective Systems, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16303, https://doi.org/10.5194/egusphere-egu23-16303, 2023.

EGU23-22 | Orals | AS1.10

Observational and Modeling Studies of High Ice Water Content Clouds: Implications for Process–Oriented Understanding 

Greg McFarquhar, Yongjie Huang, Yachao Hu, Peter Brechner, Alexei Korolev, Hugh Morrison, Jason Milbrandt, Mengistu Wolde, Cuong Nguyen, and Alain Protat

High ice water content (HIWC) regions with small ice crystals, where ice water contents (IWCs) are greater than 1.5 g m-3 and median mass diameters (MMDs) less than about 300 micrometers, occur above tropical mesoscale convective systems (MCSs) and can have detrimental impacts on aircraft engines. Data collected by the French Falcon aircraft and the National Research Council of Canada Convair-580 during the 2014 and 2015 High Altitude Ice Crystals and High Ice Water Content (HAIC/HIWC) projects are revisited here along with coordinated modeling studies to investigate processes that can produce such HIWCs. In particular, data collected from 2014 in the vicinity of Darwin Australia and from 2015 in the vicinity of Cayenne French Guyana are used to determine how bulk microphysical properties (e.g., number concentration, IWC, median volume diameter) and characteristics of ice crystal size distributions (i.e., multimodal nature, parameters fit to gamma distributions for each mode) vary with environmental conditions such as temperature, vertical velocity, MCS age, distance from MCS core, and surface characteristics. It is determined that temperature and vertical velocity are the biggest controls of small ice crystals, but younger cells, stronger convective strengths and closer proximity to convective cores also increase the relative importance of small crystals.

Numerical simulations conducted using the Weather Research and Forecasting model with four different bulk microphysics schemes generally reproduce the observed temperature, dew-point, and wind structure. However, comparison of regime-specific observations against properties simulated over Cayenne using a variety of existing parameterization schemes show that although the coverage and evolution of convection is well predicted, simulations overestimate the intensity and spatial extent of observed airborne X-band radar reflectivity and do not well depict the peak of observed size distributions with maximum dimensions between 0.1 and 1 mm. To explore formation mechanisms for large numbers of small ice crystals, a series of simulations varying the representation of secondary ice production (SIP) processes were conducted. Simulations including one of three SIP mechanisms separately (i.e., the Hallett–Mossop mechanism, fragmentation during ice–ice collisions, and shattering of freezing droplets) did not replicate the observed ratio of number concentration divided by IWC. However, the simulation including all three SIP processes produced HIWC regions consistent with observations in terms of number concentration and radar reflectivity, which was not replicated using the original P3 two-ice category configuration that only included the Hallett-Mossop mechanism. In summary, observations and simulations show primary ice production plays a key role in generating HIWC regions at temperatures < -40 Celsius, shattering of freezing droplets dominates ice particle production in HIWC regions between -15 and 0 Celsius during the early stage of convection, and fragmentation during ice–ice collisions dominates between -15 and 0 Celsius during the later stage of convection and between -40 and -20 Celsius over the whole convection period. This study thus shows the dominant role of SIP processes in the formation of numerous small crystals in HIWC regions. Implications for future measurement and modeling needs are discussed.

How to cite: McFarquhar, G., Huang, Y., Hu, Y., Brechner, P., Korolev, A., Morrison, H., Milbrandt, J., Wolde, M., Nguyen, C., and Protat, A.: Observational and Modeling Studies of High Ice Water Content Clouds: Implications for Process–Oriented Understanding, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-22, https://doi.org/10.5194/egusphere-egu23-22, 2023.

EGU23-829 | ECS | Posters on site | AS1.10

Improving the Balloon-borne Ice Cloud Particle Imager (B-ICI) 

János Stenszky and Thomas Kuhn

Atmospheric constituents, such as aerosols and clouds, greatly affect the
radiative properties of the atmosphere. Clouds play a substantial role in this
radiative balance. To better understand the contribution of cirrus clouds im-
proved modelling and in-situ observations are needed.
For further improving current climate-modelling parameters, accurate pa-
rameterization of these clouds are required. From in-situ measurements, the
size distribution of cirrus ice particles, their concentration and shape param-
eters can be determined. This can be achieved with the iBalloon-borne Ice
Cloud particle Imager (B-ICI). Campaigns done with the B-ICI and resulting
parameetrizations have contributed to more accurate characterization of cirrus
clouds.
The B-ICI is collecting and imaging ice particles with a pixel resolution
of 1,65 µm/pixel. With detailed image analysis at this accuracy particles >
20µm can be distinguished, dimensions and concentration can be derived, and
particles can be sorted according to their shape. An improved version of B-ICI
is currently being developed. This new version of the instrument is primarily
improving image quality to enable easier and more automated image processing.
Secondarily, changes in the design will reduce the weight of the instrument
and simplify the method for sampling of ice particles. A more light-weight
instrument will allow adding other sensors. In particular, an optical particle
counter to measure aerosol and small ice particles will be added to the B-ICI.
This addition of an optical particle counter will result in more accurate size
distributions in addition of providing complementary aerosol measurements. In
this paper, we will highlight these changes and improvements in the B-ICI set-
up.

How to cite: Stenszky, J. and Kuhn, T.: Improving the Balloon-borne Ice Cloud Particle Imager (B-ICI), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-829, https://doi.org/10.5194/egusphere-egu23-829, 2023.

EGU23-2309 | ECS | Posters on site | AS1.10

An idealized model to assess the impact of gravity waves on ice crystal populations in the Tropical Tropopause Layer 

Milena Corcos, Albert Hertzog, Riwal Plougonven, and Aurélien Podglajen

The role of gravity waves on microphysics of tropical cirrus clouds and air parcel dehydration was studied using the combination of Lagrangian observations of temperature fluctuations and a 1.5 dimension model. High frequency measurements during isopycnal balloon flights were used to resolve the gravity wave signals with periods ranging from 15min to a few days. The detailed microphysical simulations with homogeneous freezing, sedimentation and a crude horizontal mixing represent the slow ascent of air parcels in the Tropical Tropopause Layer. A reference simulation describes the slow ascent of air parcels in the tropical tropopause layer, with nucleation occurring only below the cold point tropopause with a small ice crystals density. The inclusion of the gravity waves modifies drastically the low ice concentration vertical profile and weak dehydration found during the ascent alone: numerous events of nucleation occur below and above the cold point tropopause, efficiently restoring the relative humidity over ice to equilibrium with respect to the background temperature, as well as increase the cloud fraction in the vicinity of the cold-point tropopause. The increased ice crystal number and size distribution agree better with observations.

How to cite: Corcos, M., Hertzog, A., Plougonven, R., and Podglajen, A.: An idealized model to assess the impact of gravity waves on ice crystal populations in the Tropical Tropopause Layer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2309, https://doi.org/10.5194/egusphere-egu23-2309, 2023.

The HIAPER Cloud Radar (HCR) is a 94 GHz W-band radar deployed in an underwing pod on the NCAR HIAPER aircraft. We use dual polarized Doppler observations collected in three major field campaigns:

  • The Cloud Systems Evolution in the Trades (CSET) study focused on the characterization of the cloud fields in the stratocumulus and the fair-weather cumulus regimes within the subtropical easterlies over the northern Pacific.
  • Motivated by challenges in their modeling, Southern Ocean clouds were observed south of Tasmania during the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES).
  • Deep convective clouds in a tropical environment were the focus in the Organization of Tropical East Pacific Convection (OTREC) field campaign.

In this study we classify clouds sampled by HCR in these very different environments into twelve categories, based on the clouds’ convective and stratiform characteristics. We calculate dimensional and convective properties of the clouds in the different categories and contrast and compare derived statistics. We analyze updraft regions observed in all cloud categories, their dimensions and velocities. Characteristics of precipitation shafts from the precipitating clouds, such as precipitation fraction or strength are also provided.

How to cite: Romatschke, U.: Cloud properties from airborne radar observations collected in field campaigns, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2868, https://doi.org/10.5194/egusphere-egu23-2868, 2023.

EGU23-2964 | Orals | AS1.10

Implementing a process-based contrail parametrization in the Unified Model 

Timmy Francis, Alex Rap, Kwinten Van Weverberg, James Manners, Kalli Furtado, Weiyu Zhang, Piers Forster, and Cyril Morcrette

     The global aviation fleet modifies cloudiness through contrail formation and their subsequent competition with natural cirrus for ambient water vapor, along with enhanced ice-nuclei concentrations from aircraft soot emissions. Contrails form in the upper troposphere at temperatures below 233 K and pressures below 300 hPa, when plume gases from jet engines, having appreciable water vapor content, saturate with respect to liquid water (Schmidt-Appleman Criterion, SAC). Realistic assessments of the aviation-induced modifications to global cloud cover demand improved representation of contrails and their interaction with background cloudiness in climate models. We have implemented a process-based parametrization of contrail cirrus, that applies to both young (≤ 5 h) and aged contrails, in the UK Met Office Unified Model, version 12.0. Contrail cirrus is introduced as a new prognostic cloud class, forming in the parametrized, fractional ice supersaturated area which then undergoes advection, depositional growth, sublimation and sedimentation. The proxy for the fractional supersaturated area is calculated using the same total water PDF as used for natural cirrus but with a different critical relative humidity, rcc - a value at which part of the model grid box is at least ice-saturated. The persistence of contrails being allowed in the ice supersaturated areas, the simulated coverage is not confined to flight corridors, but is advected to air traffic free zones as well. The simulated annual mean global coverage due to young contrails is 0.13%, with the main traffic areas of Europe and North America having the maximum coverage. Similar to natural cirrus, the contrail ice particles reflect the solar short-wave (SW) radiation and trap outgoing long-wave (LW) radiation, thereby modifying the radiative balance of the Earth’s atmosphere. Contrail cirrus is radiatively active in the model with forcing studies enabled via a ‘double radiation call’ approach, wherein parallel runs of the radiation scheme ‘with’ (prognostic) and ‘without’ (diagnostic) the contrail radiative effects isolates the contrail-induced perturbations. Contrails are seen to induce a short-wave cooling and long-wave warming and the net (SW+LW) direct top-of-atmosphere radiative forcing by young contrails amounts globally to 0.5 mWm-2, with the peak forcing seen along the main air traffic areas of North America, Europe and East Asia. The implementation of this process-based parametrization in the UM enables the simulation of the life cycle of persistent contrails, and can provide valuable insights to the aviation-induced modifications to the global cloud cover.

How to cite: Francis, T., Rap, A., Van Weverberg, K., Manners, J., Furtado, K., Zhang, W., Forster, P., and Morcrette, C.: Implementing a process-based contrail parametrization in the Unified Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2964, https://doi.org/10.5194/egusphere-egu23-2964, 2023.

EGU23-4195 | ECS | Posters on site | AS1.10

Modeling Secondary Ice Processes on a midlatitude squall line 

Jie Gao and Huiwen Xue

Secondary ice processes (SIPs) can produce ice crystals with a number concentration much higher than that of ice nucleating particles (INPs) in mixed-phase clouds, and therefore influence cloud glaciation and precipitation. But the role of SIPs in midlatitude continental mesoscale convective systems (MCSs) such as squall lines is still unknown. This study investigates the relative importance of rime splintering, freezing drop shattering, and collision breakup in the mature stage of a squall line case in North China on 18 August 2020 using the WRF model. The simulations show that collision breakup has the most pronounced effect on ice production, and rime splintering plays a secondary role. It is because ice multiplication from SIPs can feedback to collision breakup and rime splintering in different ways. Collision breakup has a positive feedback because the numerous snow and graupel from SIPs in turn promote a higher collision breakup rate, while rime splintering is limited by itself and also limited by collision breakup because the weaker riming due to the two SIPs leads to a lower rime splintering rate. Freezing drop shattering has a negligible effect on ice production because there are few large droplets in the mature stage. Collision breakup can also redistribute surface precipitation in the squall line, which decreases in the convective region and increases in the stratiform region. The influence of aerosols as CCN and INPs on SIPs is further studied. Preliminary simulation results show that the effects of aerosol concentration on the rate of SIPs and anvil ice concentration are nonlinear. The mechanism remains to be analyzed.

How to cite: Gao, J. and Xue, H.: Modeling Secondary Ice Processes on a midlatitude squall line, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4195, https://doi.org/10.5194/egusphere-egu23-4195, 2023.

EGU23-5000 | ECS | Orals | AS1.10

Airborne observations of riming in arctic mixed-phase clouds during HALO-(AC)3 

Nina Maherndl, Maximilian Maahn, Manuel Moser, Johannes Lucke, Mario Mech, and Nils Risse

Ice crystal formation and growth processes in mixed-phase clouds (MPCs) are not sufficiently understood leading to uncertainties of atmospheric models in representing MPCs. One of these processes is riming, which occurs when liquid water droplets freeze onto ice crystals. Riming plays a key role in precipitation formation in MPCs by efficiently converting liquid cloud water into ice. However, riming is challenging to observe directly and there are only few studies quantifying riming in Arctic MPCs.

In this study, we derive the normalized rime mass 𝑀 to quantify riming. We use airborne data collected during the (AC)3  field campaign HALO-(AC)3  performed in 2022. For this campaign, two aircraft were flying in formation collecting closely spatially collocated and almost simultaneous in situ and remote sensing observations. We aim to quantify 𝑀 by two methods. First, we present an Optimal Estimation algorithm to retrieve 𝑀 from measured radar reflectivities. We find 𝑀 by matching measured with simulated radar reflectivities 𝑍𝑒obtained from in situ particle number concentration observations. As forward operators, we use the Passive and Active Microwave radiative TRAnsfer tool (PAMTRA) and empirical relationships of 𝑀 and particle properties. The latter are derived via aggregation and riming model calculations. Second, we derive 𝑀 from in situ measured particle shape. We calculate the complexity 𝜒 of in situ measured particles, which relates particle perimeter to area. We then derive 𝑀 from empirical relationships that were again obtained from synthetic particles. We compare the obtained 𝑀 derived by both methods and evaluate the occurrence of riming in terms of meteorological conditions and macrophysical cloud properties to understand external drivers and variability of riming. This will lead to a better understanding of riming and thereby helps to improve modelling of this important arctic MPC process.

How to cite: Maherndl, N., Maahn, M., Moser, M., Lucke, J., Mech, M., and Risse, N.: Airborne observations of riming in arctic mixed-phase clouds during HALO-(AC)3, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5000, https://doi.org/10.5194/egusphere-egu23-5000, 2023.

EGU23-5002 | ECS | Orals | AS1.10

Identification of cirrus formation regimes using cluster analysis of back trajectories and satellite data 

Kai Jeggle, David Neubauer, and Ulrike Lohmann

In recent years our understanding of cirrus cloud processes has been significantly advanced. However, a large uncertainty regarding the influence of cirrus formation mechanisms on the microphysical properties, and hence radiative properties of cirrus clouds still remains. This leads to uncertainty in global climate models and climate change projections. In this work we aim to identify different cirrus formation regimes and analyze their influence on cirrus microphysical properties. We combine DARDAR-Nice satellite observations with Lagrangian back trajectories of meteorological and aerosol reanalysis data on the Northern Hemisphere. Our goal is to classify observed cirrus clouds by means of their trajectories and investigate the trajectories' influence on observed cirrus microphysical properties. With our data-driven nested clustering approach we identify different meteorological regimes that lead to cirrus formation. We are also able to isolate the effect of dust ice nucleating particle (INP) exposure along the trajectory from meteorological variability.

We identify four different meteorological clusters that lead to characteristic cirrus cloud microphysical properties and can be associated with liquid origin and in-situ formed cirrus clouds. Furthermore, we find that dust concentrations in cirrus cloud back trajectories are significantly higher compared to cloud free trajectories with comparable meteorological conditions. This indicates the importance of dust acting as INP during heterogeneous nucleation. The magnitude of the dust concentration, however, has only a negligible effect on cirrus microphysical properties.

How to cite: Jeggle, K., Neubauer, D., and Lohmann, U.: Identification of cirrus formation regimes using cluster analysis of back trajectories and satellite data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5002, https://doi.org/10.5194/egusphere-egu23-5002, 2023.

EGU23-5327 | Orals | AS1.10

Ice multiplication in simulated deep convective clouds with the ICON model 

Cunbo Han, Corinna Hoose, and Viktoria Dürlich

Ice multiplication processes have been recognized to play an important role in the forming of cloud ice crystals, and multiple mechanisms have been proposed to describe ice multiplication. Ice multiplication processes have been investigated for a variety of cloud types, but mostly for stratiform clouds or shallow cumulus, which do not reach temperatures of homogeneous freezing. In this study, sensitivity experiments are performed to study the role of ice multiplication in the developing stages of deep convective clouds. A double-moment cloud physics scheme was adopted. Except as the default Hallett-Mossop rime splintering process, two additional ice multiplication processes, which are droplet shattering during the freezing of supercooled drops and the collisional breakup of ice particles, are implemented. Moreover, two different parameterization schemes for the collisional breakup of ice particles. Simulation results reveal that the ice multiplication processes have a significant impact on the cloud microphysical properties and thermodynamic phase distribution within the cloud. At the cloud top, the fingerprint of ice multiplication is weaker. Collisional breakup is found to dominate ice multiplication, and the collisional breakup process rate is larger than rime splintering and droplet shattering process rates by 4 and 3 orders of magnitude, respectively. The ice enhancement factor (the ratio of ice mass or number in simulations with and without ice multiplication) has a strong vertical variation, with the maximum around -10°C and -25°C. Besides, the cascade effect on ice cloud number concentration was also investigated.

How to cite: Han, C., Hoose, C., and Dürlich, V.: Ice multiplication in simulated deep convective clouds with the ICON model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5327, https://doi.org/10.5194/egusphere-egu23-5327, 2023.

EGU23-6077 | ECS | Posters on site | AS1.10

Representation of Arctic mixed-phase clouds in ECMWF forecasts during ACLOUD 

Hanno Müller, Johannes Röttenbacher, Michael Schäfer, André Ehrlich, and Manfred Wendisch

The representation of Arctic clouds in numerical weather prediction models is challenging, especially for mixed-phase clouds with both a liquid and ice phase present. We compare measurements conducted during the Arctic CLoud Observations Using airborne measurements during polar Day (ACLOUD) campaign, which took place in May/June 2017 northwest of Svalbard, Norway, with the operational ‘Atmospheric Model high resolution’ configuration (HRES) of the Integrated Forecasting System (IFS), operated by the European Centre for Medium-Range Weather Forecasts (ECMWF). Instead of using cloud retrieval products from airborne remote sensing, the comparison is performed in the observational space of spectral solar irradiances reflected by the clouds. To allow such an analysis along the flight track at flight level, the operational ecRad radiation scheme of the IFS is used in offline mode. Besides the HRES model output, vertical profiles of concentrations of trace and greenhouse gases provided by the ECMWF Atmospheric Composition Reanalysis 4 serve as the input for ecRad. The ability of the IFS to realistically represent the airborne radiation measurements collected during ACLOUD is evaluated for flight sections above sea ice and open ocean. Inconsistencies between the upward irradiance observed during ACLOUD and the simulations by ecRad are found and may originate from uncertainties introduced by the cloud fraction, the cloud phase, the sea ice albedo, and the ice optics parameterization. Our analysis aims to separate the influence of the different macro- and microphysical parameters on the upward irradiance. To disentangle the impact of these parameters, the spectral irradiance is analyzed where e.g. the impact of liquid and ice phase can be separated. Different case studies give insight into a sub-grid cloud cover variability that is not seen by the IFS above open ocean and an overestimation of the measurements by ecRad above sea ice that can be explained by the lack of cloud brightness. EcRad is additionally run with improved ice optics parameterizations. The choice of the applied ice optics becomes more important with an increasing ice water path of the clouds and is investigated in detail within the near-infrared bands of ecRad.

How to cite: Müller, H., Röttenbacher, J., Schäfer, M., Ehrlich, A., and Wendisch, M.: Representation of Arctic mixed-phase clouds in ECMWF forecasts during ACLOUD, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6077, https://doi.org/10.5194/egusphere-egu23-6077, 2023.

EGU23-6114 | ECS | Posters on site | AS1.10

Climatological analysis of warm conveyor belt contributions to UTLS moisture content 

Ziyan Guo, Cornelis Schwenk, Maxi Boettcher, Nils Brast, Philip Reutter, and Annette Miltenberger

The Upper Troposphere-Lower Stratosphere (UTLS) is a transition region for coupled dynamical, chemical and microphysical processes. These coupled processes play an essential role in climate change. Water vapor, ozone and aerosols in the UTLS region have important impacts on the Earth’s radiation budget. Systematic biases in UTLS moisture are known to exist in global climate models. Understanding the sources of UTLS moisture and quantifying the transport processes that control water vapor and clouds in the UTLS can provide important insights into the model uncertainties and improve model simulations. In the extratropics ascending airstreams in extratropical cyclones, particularly the warm conveyor belt (WCB), and deep convection are thought to be the most important sources of UTLS moisture. Here, we utilize ERA5 reanalysis data and IAGOS aircraft measurements to quantify the contribution of WCBs to UTLS moisture for the decade 2010 to 2019. WCB outflow regions are defined using Lagrangian trajectories. The moisture anomaly in the WCB outflow compared to average UTLS moisture content is quantified as well as its evolution over the 2 days after WCB ascent. ERA5 suggests significant positive moisture anomalies in the WCB outflow that persists over several days. Finally, ERA5 UTLS moisture content is compared to IAGOS humidity measurements with a particular focus on WCB outflow regions. In summary, we present a comprehensive climatological picture of the role of WCB moisture transport for the UTLS composition.

How to cite: Guo, Z., Schwenk, C., Boettcher, M., Brast, N., Reutter, P., and Miltenberger, A.: Climatological analysis of warm conveyor belt contributions to UTLS moisture content, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6114, https://doi.org/10.5194/egusphere-egu23-6114, 2023.

Recent experiments and modelling studies suggest that secondary ice production (SIP) may close the gap between observed Arctic ice nucleating particle (INP) concentrations and ice crystal number concentrations (Ni). Here we explore model sensitivities with respect to the complexity of different INP parameterisations in numerical simulations under the premiss that Ni is governed by SIP. Idealised, cloud-resolving simulations are performed for the marine cold air outbreak cloud deck sampled during M-PACE (cloud-top temperature of -17°C) with the ICOsahedral Nonhydrostatic (ICON) model.

Droplet shattering (DS) of rain drops according to Phillips et al. (2018), and collisional breakup (CB) (Phillips et al. 2017) were implemented and tested in addition to the existing Hallet-Mossop (HM) rime splintering implemented in ICON’s state-of-the-art two-moment bulk microphysics scheme. Furthermore, a fully prognostic temperature-dependent budget representation of INP (Solomon et al. 2015) was implemented and contrasted to a less sophisticated time-relaxation formulation of atmospheric INP concentrations.

Overall, 16 different model experiments (24h runs) were performed and analysed. Despite the considerable amount of uncertainty remaining with regard to ice production mechanisms and their process representation in numerical models we conclude from these experiments that: (i) Ni-enhancement through SIP can close the gap between measured and simulated Ni concentrations during M-PACE in ICON consistent with previous studies (e.g. Sotiropoulou et al. 2020; Zhao et al. 2021), (ii) only simulations where DS dominates the SIP signal (potentially amplified by CB) capture the vertical Ni in-cloud profile correctly, (iii) INP recycling remains necessary for MPC maintenance during M-PACE even if Ni is dominated by SIP, and (iv) experiments using a computationally more efficient relaxation-based prognostic parameterisation of primary nucleation are statistically invariant from simulations considering a prognostic INP budget.

How to cite: Possner, A., Pfannkuch, K., and Ramadoss, V.: Interplay between Primary and Secondary Ice Production (SIP) in Arctic Mixed-Phase Clouds (MPCs) as simulated for the M-PACE campaign in ICON, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6658, https://doi.org/10.5194/egusphere-egu23-6658, 2023.

Warm conveyor belts (WCB) are regions of large-scale coherent airflow within extratropical cyclones that rapidly ascend from the boundary layer to the upper troposphere. During their ascent, WCBs transport water vapour and cloud condensate to the upper troposphere, and thereby significantly contribute to the moisture content of the extra-tropical upper troposphere-lower stratosphere (UTLS) as well as upper tropospheric cloudiness. UTLS moisture content and cloudiness are important for the radiative budget of the Earth and future changes thereof, but are often poorly represented in numerical models and reanalysis products. A detailed quantitative understanding of the processes governing water transport in WCBs provides vital clues to the origin of these biases and for evaluating predicted future changes in WCB moisture transport. Furthermore, recent studies have found that deep and embedded convection play an important role in WCBs. This points to the necessity of high-resolution simulations, that are well validated with observational data to provide a “benchmark” for coarser-resolution global (climate) models. Here we investigate the physical processes governing WCB moisture transport in simulations of a case-study from the WISE campaign with a particular focus on (i) the impact of grid spacing (including the use of convection parameterisations) on WCB moisture transport, (ii) the microphysical processes controlling moisture loss from the WCB, and (iii) the cloud microphysical properties of the cirrus clouds in the WCB outflow.

To this end we conducted two ICON simulations of an extratropical cyclone using (i) a global (~13km resolution), convection-parameterizing and (ii) a doubly nested (~13km, ~6km and ~3km resolution) convection permitting set up. In both set-ups online trajectories are calculated that capture convective ascent and allow for a Lagrangian analysis of WCB moisture transport and WCB cloud structure.

The Lagrangian metrics show large differences in ascent timescales and the efficiency with which water is transported from the boundary-layer to the UTLS. It is shown that this impacts the UTLS moisture content in the WCB outflow region. Local changes in UTLS moisture content induced by different representations of convection are shown to project onto larger-scale structures in the moisture and cloud fields over the 1-2 days after WCB ascent.

How to cite: Schwenk, C. and Miltenberger, A.: Physical processes controlling warm conveyor belt moisture transport to the UTLS and dependence on model resolution, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6987, https://doi.org/10.5194/egusphere-egu23-6987, 2023.

EGU23-7012 | ECS | Posters on site | AS1.10

Quantification of the Radiative Effect of Arctic Cirrus by Airborne Radiation Measurements - A Case Study 

Johannes Röttenbacher, Hanno Müller, André Ehrlich, and Manfred Wendisch

Observations of cloud related processes in the Arctic are needed to evaluate the representation of clouds in weather and climate models and to improve our understanding of processes of Arctic amplification and Arcitc-midlatitude linkages. One remaining uncertainty of the Arctic climate system are cirrus clouds and their influence on the radiative budget. Arctic cirrus is known to warm the climate system on annual average, especially when present over the sea ice covered central Arctic. 
The HALO-(AC)³ airborne campaign in spring 2022 investigated changes within air masses on their way in and out of the central Arctic with the High Altitude LOng Range research aircraft (HALO), which was equipped with a suite of remote sensing instrumentation. Two flights were used to explicitly investigate the cloud radiative effect of single layer isolated cirrus between 81 and 90 degrees North.
Flight legs above and below the cirrus with measurements of spectral solar irradiance from the Spectral Modular Airborne Radiation measuremenT system (SMART) make a direct estimation of the cloud radiative effect possible. The cirrus was sufficiently thick to reduce the transmission of solar radiation by around 25%. However, significant inhomogeneities in the cirrus were observed.
We present a case study of the radiative effect of Arctic cirrus and compare airborne irradiance measurements to simulations from an offline run of the ecRad radiation scheme which is operationally used in the ECMWF's Integrated Forecasting System.

How to cite: Röttenbacher, J., Müller, H., Ehrlich, A., and Wendisch, M.: Quantification of the Radiative Effect of Arctic Cirrus by Airborne Radiation Measurements - A Case Study, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7012, https://doi.org/10.5194/egusphere-egu23-7012, 2023.

EGU23-7035 | Orals | AS1.10

Characterization of Tropical Tropopause Layer clouds combining balloon-borne and space-borne observations 

Thomas Lesigne, Francois Ravetta, Aurélien Podglajen, Dung Tran, Jérôme Bureau, Vincent Mariage, Jacques Pelon, and Alain Hauchecorne

Tropical Tropopause Layer clouds have a significant impact on the Earth's radiative budget and regulate the amount of water vapor entering the stratosphere. They are a key component of the climate system but their observation is still challenging. The Strateole-2 project aims at a  better understanding of dynamical, transport, and processes in the Tropical Tropopause Layer (TTL) using long-duration super-pressure balloons flying for several months in the lower stratosphere along the equator belt. From October 2021 to late January 2022, three microlidars flew onboard stratospheric balloons, slowly drifting just a few kilometers above the clouds. These observations have unprecedented sensitivity to thin cirrus and provide a fine scale description of cloudy structures both in time and space. Statistical comparisons with spaceborne lidar CALIOP are discussed, highlighting the unique ability of the microlidar to detect optically thin clouds. The modulation of outgoing longwave radiation by tropical clouds is also investigated using the balloon-borne observations. 

How to cite: Lesigne, T., Ravetta, F., Podglajen, A., Tran, D., Bureau, J., Mariage, V., Pelon, J., and Hauchecorne, A.: Characterization of Tropical Tropopause Layer clouds combining balloon-borne and space-borne observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7035, https://doi.org/10.5194/egusphere-egu23-7035, 2023.

EGU23-7474 | Posters on site | AS1.10

Measurements of microphyscs in cold air Outbreks 

Tom Choularton and Gary Lloyd and the M-phase ACAO

Measurements were made in 2 sets of cold air outbreaks using the UK FAAM BAE 146  research aircraft. The first set were performed in March 2022 over the Eastern Atlantic the second set were perform in October to early November 2022 in the Western Atlantic over the Labrador Sea based in Goose Bay, Eastern Canada. In each set of experiments the focus was to study the evolution of the cloud microphysics as influenced by Cloud condensation nuclei, ice nuclei and secondary ice processes  in the stratocumulus clouds being advected southwards over progressively warmer sea until cloud break-up occurred into convective clouds. The aims were to improve the treatment of these cloud types in Global climate models and weather forecast models. These projects formed part of m-Phase funded by NERC as part of its Cloud Sense programme and ACAO a Met office program to study these clouds.A range of aerosol and cloud microphysical equipment was used in the 2 projects which will be discussed in the presentation.Analysis of the data set including a new novel Holographic instrument is still underway at the time of writing; however, some preliminary results indicate that:

  • Generally the ice crystal number concentration exceeded the ice nucleus concentrations measured at the same temperature
  • Some regions consisted entirely of super cooled water
  • A range of secondary ice particle production mechanisms were observed including ice splinter production during riming and droplet shattering on freezing after capture by ice crystals
  • Generally if the convective region was reached by the aircraft then secondary ice production was greater than in the stratocumulus region
  • Precipitation was mostly in the ice phase

How to cite: Choularton, T. and Lloyd, G. and the M-phase ACAO: Measurements of microphyscs in cold air Outbreks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7474, https://doi.org/10.5194/egusphere-egu23-7474, 2023.

EGU23-8660 | Orals | AS1.10

A Global Merged Diurnal Ice/Snow Cloud Product from Spaceborne Passive Microwave Observations and Its Applications to Model Evaluation 

Jie Gong, Chenxi Wang, Dong Wu, Yiding Wang, Leah Ding, and Donifan Barahona

Ice cloud and floating snow play critical roles in Earth’s energy budget and hydrological cycle. Their diurnal variation is tightly coupled with convection development life cycle, hence it also greatly impacts the diurnal cycle of surface precipitation and top of the atmosphere radiation. Due to the high degree of freedom of ice crystal microphysical properties, remote sensing of ice/snow cloud is challenging for passive spaceborne sensors.

In this work, we present a global diurnal ice/snow cloud product by merging three spaceborne passive microwave sensor observations together (GPM-GMI, NPP-ATMS, and MT-SAPHIR). This dataset includes ice water path (cloud ice + falling snow), cloud top height (CTH) and cloud bottom height (CBH) at pixel level between 2015 – 2016, and monthly gridded values at 2deg X 2deg X 2 hours grid scale. The convolutional neural network (CNN) approach is adopted for the algorithm development by learning from collocated CloudSat observations, and the Monte Carlo dropout method is used for uncertainty estimation. A customized loss-function is developed to retrieve cloud mask and mass together.

We evaluated the retrieval at collocated pixels as well as against other independent field campaign and ground-based measurements. Diurnal and semi-diurnal distributions of the IWP will be presented. We will also demonstrate how we use this product to evaluate model performance on capturing the general distribution and diurnal variation of the frozen hydrometeors in the atmosphere.

How to cite: Gong, J., Wang, C., Wu, D., Wang, Y., Ding, L., and Barahona, D.: A Global Merged Diurnal Ice/Snow Cloud Product from Spaceborne Passive Microwave Observations and Its Applications to Model Evaluation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8660, https://doi.org/10.5194/egusphere-egu23-8660, 2023.

EGU23-9818 | ECS | Orals | AS1.10

A novel approach to investigate Cirrus cloud formation 

Tim Lüttmer and Peter Spichtinger

Warm conveyor belts (WCB) lead to formation of horizontally wide spread Cirrus clouds in the upper troposphere. However, the contribution of different ice formation processes and the resulting micro- and macrophysical properties of the Cirrus ,e.g., their radiative effects are still poorly understood. We want to especially address the research question of in-situ vs. liquid origin ice formation.

Common microphysics bulk schemes only consider a single ice class which includes sources from multiple formation mechanisms. We developed and implemented a two-moment microphysics scheme in the atmosphere model ICON that distinguishes between different ice modes of origin including homogeneous nucleation, deposition freezing, immersion freezing, homogeneous freezing of water droplets and secondary ice production from rime splintering, frozen droplet shattering and collisional break-up, respectively. Each ice mode is described by its own size distribution, prognostic moments and unique formation mechanism while still interacting with all other ice modes and microphysical classes like cloud droplets, rain and rimed cloud particles.

Using this novel microphysics scheme we can determine the contribution of the various ice formation mechanisms to the total ice content. For the first time this allows us to directly investigate the competition of in-situ and liquid origin Cirrus as well as homogeneous and heterogeneous ice nucleation with regards to environmental conditions and choice of microphysical parameterisations.

We performed an ensemble of simulations for selected WCB cases to cover a range of microphysical properties and compared the results of our liquid origin vs in-situ analysis with other Cirrus categorization algorithms.

How to cite: Lüttmer, T. and Spichtinger, P.: A novel approach to investigate Cirrus cloud formation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9818, https://doi.org/10.5194/egusphere-egu23-9818, 2023.

EGU23-10696 | Posters on site | AS1.10

How important are secondary ice processes – preliminary results from FOR-ICE 

Luisa Ickes, Montserrat Costa Surós, Patrick Eriksson, Hannah Frostenberg, Paraskevi Georgakaki, Maria Gonçalves Ageitos, Hanna Hallborn, Anna Lewinschal, Eleanor May, Athanasios Nenes, David Neubauer, Carlos Pérez García-Pando, Ulrike Proske, and Georgia Sotiropoulou

Global climate models poorly represent mixed-phase clouds, which leads to uncertainties in cloud radiative forcing and precipitation. In the FORCeS ice experiment (FOR-ICE) we compare three global climate models (ECHAM-HAM, NorESM, EC-Earth) and show which processes are crucial for a realistic representation of cloud ice and supercooled water in each global climate model framework using the factorial method as a statistical approach. A specific focus of the experiments is on secondary ice production (SIP) - which apart from one mechanism (rime splintering) is typically not represented in models, even if observations of ice crystal concentrations of ice crystal number in warm mixed-phase clouds often exceed available ice nuclei by orders of magnitude. We evaluate the importance of three SIP mechanisms combined (rime splintering, ice-ice collisions, and droplet shattering) compared to all other processes that can modulate ice mass and number in mixed-phase clouds: ice nucleation, sedimentation, and transport of ice crystals, and the Wegener-Bergeron-Findeisen process. To describe SIP we adopt two approaches: an explicit microphysical representation of the processes, and a parameterization based on a random forest regression of high-resolution two-year simulations in the Arctic using the polar Weather Research and Forecast model (polar-WRF). Satellite observations are used to evaluate if including descriptions of SIP leads to a more realistic representation of mixed phase clouds.

How to cite: Ickes, L., Costa Surós, M., Eriksson, P., Frostenberg, H., Georgakaki, P., Gonçalves Ageitos, M., Hallborn, H., Lewinschal, A., May, E., Nenes, A., Neubauer, D., Pérez García-Pando, C., Proske, U., and Sotiropoulou, G.: How important are secondary ice processes – preliminary results from FOR-ICE, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10696, https://doi.org/10.5194/egusphere-egu23-10696, 2023.

EGU23-11199 | Orals | AS1.10

Secondary ice production - No evidence of a productive rime-splintering mechanisms during dry and wet growth 

Susan Hartmann, Johanna Seidel, Alice Keinert, Alexei Kiselev, Thomas Leisner, and Frank Stratmann

Mixed-phase clouds are essential elements in Earth’s weather and climate system. Atmospheric observation of mixed-phase clouds occasionally demonstrated a strong discrepancy between the ice particle and ice nucleating particle number concentration of several orders of magnitude at modest supercooling [1, 4, 6]. Various secondary ice production (SIP) mechanisms have been hypothesized which can increase the ice particle number concentration by multiplication of primary ice particles [2, 3].

In this study, we focus on SIP as a result of droplet-ice collisions, commonly known as rime-splintering or Hallett-Mossop (HM) process. During riming supercooled droplets collide with an ice particle and freeze upon impact and lead to the formation of secondary ice particles. Our main objectives are to quantify the number of secondary ice particles and to learn more about the underlying physics. Therefore, we conducted laboratory experiments at IDEFIX (Ice Droplets splintEring on FreezIng eXperiment) in which small droplets collide with a fixed ice particle of 1 mm in diameter. IDEFIX is designed to simulate atmospheric relevant conditions regarding temperature, humidity, impact velocities and collision rates. The riming process was observed with high-speed video microscopy and infrared thermography to visualize the growing rimer structures and the surface temperature of the riming ice particle, respectively. Further, the secondary ice particles were counted via inertial impaction on a supercooled sugar solution in the ice counting device (cut off diameter of 2 µm) developed at IMK-AAF, KIT.

The following parameters were investigated: the air temperature was varied between -4°C and -10°C, the ice-droplet impact velocities were set either to 1 ms-1 or 3 ms-1, and the lognormal droplet size distribution was adjusted to have the mode diameter between 18 µm and 30 µm with the standard deviation between 1.6 µm and 8.4 µm. Under these conditions, the collisions rates between droplets and rimer were between 102 and 10mm-1s-1 , as determined from the video records and with a rimer heat balance model [5] using measured surface temperature as input data. Thus, the simulated riming process is typical for convective clouds; both dry and wet growth could be realized in IDEFIX. We found no efficient and reproducible secondary ice production during riming within the range of the investigated parameters. The amount of secondary ice particles produced in all our experiments was well below the values expected from the HM mechanism [3, 7], where several hundreds of secondary ice particles per mg rime were found at optimal conditions. Six potential SIP cases (out of 31) could be identified where ice was detected in the ice counting device. Four of them could be attributed to rime spicules break-off due to sublimation.

[1] Crosier, J., et al. 2011, DOI: 10.5194/acp-11-257-2011.

[2] Field, P.R., et al. 2016, DOI: 10.1175/amsmonographs-d-16-0014.1.

[3] Korolev, A. and T. Leisner 2020, DOI: 10.5194/acp-20-11767-2020.

[4] Luke, E.P., et al. 2021, DOI: 10.1073/pnas.2021387118.

[5] Pruppacher, H.R. and J.D. Klett, Microphysics of Clouds and Precipitation. 2010, Springer Dordrecht.

[6] Taylor, J.W., et al. 2016, DOI: 10.5194/acp-16-799-2016.

How to cite: Hartmann, S., Seidel, J., Keinert, A., Kiselev, A., Leisner, T., and Stratmann, F.: Secondary ice production - No evidence of a productive rime-splintering mechanisms during dry and wet growth, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11199, https://doi.org/10.5194/egusphere-egu23-11199, 2023.

EGU23-11386 | Orals | AS1.10

Large-eddy simulation of a two-layer boundary-layer cloud system from the Arctic Ocean 2018 expedition 

Annica M. L. Ekman, Ines Bulatovic, Julien Savre, Michael Tjernström, and Caroline Leck

The most common type of cloud in the Arctic latitudes is mixed-phase stratocumulus. These clouds play a critical role in the Arctic energy budget. Previous observations in the central (north of 80° N) Arctic have shown a high occurrence of prolonged periods of a shallow, single-layer mixed-phase stratocumulus at the top of the boundary layer (altitudes ~300-400m). However, recent observations from the summer of 2018 showed a prevalence of a two-layer boundary-layer cloud system. Here we use large-eddy simulation to examine the maintenance of one of the cloud systems observed in 2018 as well as the sensitivity of the cloud layers to different micro- and macro-scale parameters. We find that the model generally reproduces the observed thermodynamic structure well, with two near-neutrally stratified layers in the boundary layer caused by a low cloud (located within the first few hundred meters) capped by a lower temperature inversion, and an upper cloud layer (based around one kilometer or slightly higher) capped by the main temperature inversion of the boundary layer. The investigated cloud structure is persistent unless there are low aerosol number concentrations (<5 cm-3), which cause the upper cloud layer to dissipate, or high large-scale wind speeds (>8.5 m s-1), which erode the lower inversion and the related cloud layer. These types of changes in cloud structure led to a substantial reduction of the net longwave radiation at the surface due to a lower emissivity or higher altitude of the remaining cloud layer. The findings highlight the importance of better understanding and representing aerosol sources and sinks over the central Arctic Ocean. Furthermore, they underline the significance of meteorological parameters, such as the large-scale wind speed, for maintaining the two-layer boundary-layer cloud structure encountered in the lower atmosphere of the central Arctic.

How to cite: Ekman, A. M. L., Bulatovic, I., Savre, J., Tjernström, M., and Leck, C.: Large-eddy simulation of a two-layer boundary-layer cloud system from the Arctic Ocean 2018 expedition, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11386, https://doi.org/10.5194/egusphere-egu23-11386, 2023.

EGU23-13062 | Orals | AS1.10

A probabilistic approach to determine the thermodynamic cloud phase using passive satellites 

Johanna Mayer, Luca Bugliaro, Florian Ewald, and Christiane Voigt

The cloud thermodynamic phase (ice / mixed-phase / liquid) is a crucial parameter to understand the earth radiation budget, hydrological cycle and atmospheric thermodynamic processes. The phase partitioning of clouds and their parameterization in global climate models have therefore become of particular interest.

To improve our understanding of the frequency of occurrence and temporal evolution of cloud phase, geostationary passive sensors can be very useful due to their wide field of regard and high temporal resolution. However, the retrieval of cloud phase using passive instruments is challenging since the spectral signature of the phase is weak compared to other parameters of the clouds and atmosphere. Especially the distinction between ice and mixed-phase clouds is difficult and previous efforts to retrieve cloud phase often only distinguished between ice and liquid phase.

We present a new method to detect clouds and retrieve their phase using the passive instrument SEVIRI aboard the geostationary satellite Meteosat Second Generation. The method uses probabilities derived from active observations (the Lidar-Radar product DARDAR) of cloud top phase. Combining these probabilities for different SEVIRI channels gives probabilities for the presence of a cloud and for its cloud top phase. Our probabilistic approach includes a measure of uncertainty and allows us to distinguish between ice, mixed-phase, supercooled liquid, and warm liquid clouds. The method is tested against active satellite measurements and shows good agreement. Finally, we discuss its advantages and limitations. In the future, we plan to use our method to study the microphysical (such as optical thickness and effective radii) and macrophysical (such as temporal evolution and extent) properties of ice and mixed-phase clouds.

How to cite: Mayer, J., Bugliaro, L., Ewald, F., and Voigt, C.: A probabilistic approach to determine the thermodynamic cloud phase using passive satellites, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13062, https://doi.org/10.5194/egusphere-egu23-13062, 2023.

EGU23-14023 | ECS | Posters on site | AS1.10

Unraveling secondary ice production in winter orographic clouds through a synergy of in-situ observations, remote sensing and modeling 

Paraskevi Georgakaki, Anne-Claire Billault-Roux, Eliot Perrin, Romanos Foskinis, Georgia Sotiropoulou, Franziska Vogel, Maria Gini, Konstantinos Eleftheriadis, Ottmar Moehler, Satoshi Takahama, Alexis Berne, and Athanasios Nenes

The representation of orographic clouds in numerical weather prediction models remains a great challenge, as a consequence of our incomplete understanding of the microphysical processes acting on them and the complex interactions between the large-scale and orographic flow dynamics. Mixed-phase conditions are frequently occurring in orographic clouds, highlighting the importance of correctly simulating the microphysical evolution of ice- and liquid-phase hydrometeors. In this study we employ the mesoscale Weather Research and Forecasting (WRF) model to investigate the drivers of intense snowfall events observed during the Cloud-AerosoL InteractionS in the Helmos background TropOsphere (CALISHTO) campaign, that took place from Fall 2021 to Spring 2022 at Mount Helmos in Peloponnese, Greece. Vertical profiles of reflectivity, Doppler velocity, as well as full Doppler spectra measured by a vertically pointing W-band (94 GHz) Doppler cloud radar, in synergy with Doppler and aerosol depolarization lidar data, help gain insight into the snowfall microphysics involved and set the basis for evaluating the performance of the WRF model. A radar simulator coupled with WRF enables the direct comparison between the mesoscale simulations and remote sensing products, and allows us to find the optimal model set-up that minimizes deviations from the observations. Comparing the modeled ice crystal number concentrations (ICNCs) with the Ice Nucleating Particles (INPs) measured in-situ at the Helmos High Altitude Monitoring Station (2314 m, 42°N 05' 30'', 34°E 14' 25'') by the Portable Ice Nucleation Experiment (PINE) instrument, we seek to quantify the ice enhancement factors due to secondary ice production (SIP) or seeding ice particles and their potential role in enhancing orographic precipitation. The synergy between high-resolution modeling and radar observations gives us the opportunity to infer SIP signatures from remote sensing observations, which is an important outcome given the abundance of the latter.

How to cite: Georgakaki, P., Billault-Roux, A.-C., Perrin, E., Foskinis, R., Sotiropoulou, G., Vogel, F., Gini, M., Eleftheriadis, K., Moehler, O., Takahama, S., Berne, A., and Nenes, A.: Unraveling secondary ice production in winter orographic clouds through a synergy of in-situ observations, remote sensing and modeling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14023, https://doi.org/10.5194/egusphere-egu23-14023, 2023.

EGU23-14247 | ECS | Posters on site | AS1.10

Studying secondary ice production mechanisms: from a remote sensing and hydrometeors dynamics perspective 

Florian Le Roy De Bonneville, Yasmin Aboel Fetouh, Jan Cermak, Corinna Hoose, Emma Järvinen, Thomas Leisner, and Markus Uhlmann

Ice crystal number concentrations were often found to be orders of magnitude higher than the number concentration of ice nucleating particles; a finding that indicated the presence of secondary ice production (SIP).  Although 6 mechanisms of SIP have been both discovered and theorized, it is still not fully understood and the recent studies have been inconclusive in identifying the dominant process in real conditions.  This lack of constraint of ice multiplication adds to the uncertainty of cloud simulations in climate models. Studying SIP is challenging due to the various interfering factors involved.
In this study, we attempt to further our knowledge in understanding the SIP mechanisms using two different but complementary approaches. The first consists of using remote sensing tools such as Himawari-8 and MODIS retrievals in addition to the SOCRATES in-situ data to identify the presence of SIP and categorize the possible mechanism involved.
The second approach utilizes numerical simulations to further understand these mechanisms that are potentially responsible for SIP, but through the study of the dynamics of the different particles (ice crystals, supercooled droplets, graupel...) involved in these processes. In this approach we focus on the characteristics of the particles, such as their diameter and concentration, as well as the presence of turbulence, that are crucial in describing their movement and the feasibility of the mechanisms under study. 

How to cite: Le Roy De Bonneville, F., Aboel Fetouh, Y., Cermak, J., Hoose, C., Järvinen, E., Leisner, T., and Uhlmann, M.: Studying secondary ice production mechanisms: from a remote sensing and hydrometeors dynamics perspective, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14247, https://doi.org/10.5194/egusphere-egu23-14247, 2023.

EGU23-14329 | ECS | Posters on site | AS1.10

Investigating ice cloud formation mechanisms from satellite observations and Lagrangian transport and microphysics models 

Athulya Saiprakash, Patrick Konjari, George Horner, Christian Rolf, Martina Krämer, and Odran Sourdeval

Ice clouds are challenging because of the high complexity and diversity of their composition  (microphysics) as well as formation and growth processes. As a result, there has been little constraint from observations until recently, resulting in significant limitations in our understanding and representation of ice clouds. A major problem with satellite measurements is the lack of information on the environmental context, which is necessary to identify and understand the formation mechanism and evolution of clouds; these renditions indeed only represent a snapshot of the state of a cloud and its microphysical properties at a given time. This work tackles this issue by providing additional metrics on ice cloud history and origin along with operational satellite products.

Here, we present a novel framework that combines geostationary satellite observations with Lagrangian transport and ice microphysics models, in order to obtain information on the history and origin of air parcels that contributed to their formation. The trajectory of air parcels encountered along the DARDAR-Nice track has been traced using the air mass transport models CLAMS (Chemical LAgrangian Model of the Stratosphere). CLaMS - Ice model is jointly used to simulate cirrus clouds along trajectories derived by CLaMS. This approach provides information on the cloud regime as well as the ice formation (in-situ vs liquid origin) pathway. For tropical cirrus of convective origin, a Time Since Convection dataset from geostationary observations can also be incorporated into this approach. Preliminary results of this approach obtained on case studies representative of multiple cloud types will be shown here.

How to cite: Saiprakash, A., Konjari, P., Horner, G., Rolf, C., Krämer, M., and Sourdeval, O.: Investigating ice cloud formation mechanisms from satellite observations and Lagrangian transport and microphysics models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14329, https://doi.org/10.5194/egusphere-egu23-14329, 2023.

EGU23-15307 | Orals | AS1.10

Do detrained cirrus clouds have memory of the deep convection they came from? 

George Horner and Edward Gryspeerdt

The large cirrus outflows that arise from deep convection play a vital role in modulating the energy balance of the Earth’s atmosphere. One important question is how much do the initial conditions of the deep convection influence the subsequent evolution of the detrained cirrus, and if these initial conditions are important, over what timescales do they matter? Characterising how these cirrus outflows evolve over their entire lifetime, and how they might change in response to anthropogenic emissions is important in order to understand their role in the climate system and to constrain past and future climate change.

Building on the ‘Time Since Convection’ product used in Horner & Gryspeerdt (2023), this work investigates how the initial conditions of the deep convection influence the subsequent evolution of the detrained cirrus- in particular, how does the timing, location, and meteorological environment of the deep convection alter the detrained cirrus, and for how long are these initial conditions important for the cirrus properties- is there a ‘memory’ of the initial conditions of the deep convection imprinted on the properties of the cirrus hours or days after the initial deep convection has dissipated? To answer this question, data from the DARDAR, ISCCP, and CERES products are used to build a composite picture of the radiative and microphysical properties of the clouds, which is investigated under varying initial conditions.

The initial state of the convection is found to have a considerable impact on cirrus development under a variety of conditions. The diurnal cycle, particularly the timing of the convection, is a strong control on the cloud radiative effect, particularly in regions of strong convective activity. The initial aerosol perturbation is also shown to play a role in cirrus development, both in the large scale properties of the cirrus and the microphysical properties.

This demonstrates a potential time dependent impact of aerosol and convection on cloud properties and provides a template for future studies of cloud development incorporating diverse sets of measurements.

How to cite: Horner, G. and Gryspeerdt, E.: Do detrained cirrus clouds have memory of the deep convection they came from?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15307, https://doi.org/10.5194/egusphere-egu23-15307, 2023.

EGU23-15602 | ECS | Orals | AS1.10

Differences in microphysical properties of cirrus at high and mid latitudes from airborne measurements 

Elena De La Torre Castro, Tina Jurkat-Witschas, Armin Afchine, Valerian Hahn, Simon Kirschler, Martina Krämer, Johannes Lucke, Nicole Spelten, Heini Wernli, Martin Zöger, and Christiane Voigt

Cirrus in mid latitudes (<= 60° N) are often affected by aviation and pollution while cirrus in high latitudes (> 60° N) develop in a more pristine atmosphere. In this study, we compare the microphysical properties of cirrus measured in mid latitudes and cirrus measured in high latitudes. The analyzed properties are: the ice crystal number concentration (N), effective diameter (ED) and ice water content (IWC) of cirrus from in situ measurements during the CIRRUS-HL campaign in June and July 2021. We use a combination of cloud probes covering ice crystals sizes between 2 and 6400 µm. The differences in cirrus properties are investigated with dependence on altitude and latitude and we show that there exist differences between mid-latitude and high-latitude cirrus. An increase in ED and a reduction in N is observed in high-latitude cirrus compared to mid-latitude cirrus.

In order to investigate the cirrus properties in relation to the region of formation, we also combine our measurements with 10-day backward trajectories to identify the location of cirrus formation and the cirrus type: in situ or liquid origin cirrus. According to the latitude of cloud formation and latitude of the measurement, we classify the cirrus in three groups: cirrus formed and measured at mid latitudes (M-M), cirrus formed at mid latitudes and measured at high latitudes (M-H) and cirrus formed and measured at high latitudes (H-H). This analysis shows that part of the cirrus measured at high latitudes are actually formed at mid latitudes and therefore influenced by mid-latitude air masses. We discuss the differences of the cirrus properties under this new classification. Our study helps to advance the understanding of upper-tropospheric cirrus properties at mid and high latitudes in summer and the influence of anthropogenic perturbations.

How to cite: De La Torre Castro, E., Jurkat-Witschas, T., Afchine, A., Hahn, V., Kirschler, S., Krämer, M., Lucke, J., Spelten, N., Wernli, H., Zöger, M., and Voigt, C.: Differences in microphysical properties of cirrus at high and mid latitudes from airborne measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15602, https://doi.org/10.5194/egusphere-egu23-15602, 2023.

EGU23-15765 | Posters on site | AS1.10

Sensitivity of Satellite Lidar-Radar Cirrus Retrievals to PSD Assumptions: DARDAR-Nice v2 and Simulator 

Odran Sourdeval, Irene Bartolome Garcia, Guillaume Penide, and Martina Krämer

Ice clouds constitute a challenge to satellite remote-sensing due to the variability of their microphysical properties. A central parameter to understand and represent ice clouds in modelling as well as in remote-sensing is the ice particle size distribution (PSD), whose shape largely varies depending on the environmental conditions in which the ice cloud has formed and evolved. This shape is typically assumed in satellite retrieval algorithm, for instance as a mono-modal gamma-modified distribution. Our representation of PSDs has greatly improved over the last decades, largely due to novel parameterisation methods as well as the increasing availability and accuracy of in-situ measurements that can serve as a solid basis to calibrate retrieval algorithms.

This study investigates the impact of the PSD shape assumptions on cirrus retrievals obtained from lidar-radar satellite observations (DARDAR-Nice), with a strong focus on the ice crystal number concentration. Recent in-situ measurements from the JULIA dataset were recently processed to propose new parameterisations of the PSD that offer a better representation of small ice concentrations. The added-value of considering the observed bi-modality when representing PSDs for remote sensing applications was also discussed. We here assess the consequences of including such new parameterisations in DARDAR-Nice. Comparisons between v1 and v2 (offering updated PSD assumptions) of this satellite product are also discussed.

Finally, preliminary results from a DARDAR-Nice simulator will be shown. This simulator allows to perform synthetic lidar-radar observations and retrievals on high-resolution cloud model outputs. Comparisons between the model “truth” and synthetic retrievals will be investigated and discussed in the context of underlying PSD assumptions.

How to cite: Sourdeval, O., Bartolome Garcia, I., Penide, G., and Krämer, M.: Sensitivity of Satellite Lidar-Radar Cirrus Retrievals to PSD Assumptions: DARDAR-Nice v2 and Simulator, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15765, https://doi.org/10.5194/egusphere-egu23-15765, 2023.

EGU23-15890 | ECS | Posters on site | AS1.10

Organization of SIP mechanisms among basic cloud types 

Akash Deshmukh, Vaughan Phillips, Deepak Waman, Sachin Patade, Aaron Bansemer, and Ashok Gupta

 Clouds are a fundamental aspect of the Earth’s atmosphere. One of the major challenges in cloud-resolving models (CRM) is the formation and generation of new cloud ice particles from pre-existed ice and liquid. Based on the basic broad cloud types, it is helpful to distinguish between their fundamental microphysical properties. The four basic cloud types are defined as: (1) warm-based convective and stratiform clouds; and (2) cold-based convective and stratiform clouds. Recent studies of ice initiation in clouds have shown that most ice particles in the mixed-phase region of clouds are from secondary ice production (SIP) mechanisms but have generally concentrated on only one specific cloud system.

In this study, Aerosol-Cloud model (AC) is used. AC includes the four mechanisms of secondary ice production as follows: ice-ice collisional breakup, raindrop freezing fragmentation, Hallett-Mossop (HM) process and sublimational breakup. The intent is to generalize the contribution of each SIP mechanism among basic cloud types. The numerical simulations are performed using our AC for each cloud type and validated against in-situ cloud observations. The observational data is collected during four different cloud observational campaigns, each representing a contrasting cloud type than others.

Here, we study the contributions from each process of SIP (HM process, ice-ice collisional breakup, raindrop-freezing fragmentation and sublimational breakup) by performing control simulations of each basic cloud type. For the warm cloud convective clouds, the HM process prevails near freezing level and contributes significantly from 0 to -15oC. In cold-based convective clouds, the ice-ice collisional breakup is the most dominating SIP mechanism in each cloud type. In warm-based stratiform clouds, the HM process dominates the contribution of ice in the -5 to -15oC temperature range for updrafts up to 8 m/s. In the slightly warm-based convective clouds, the breakup due to ice-ice collision is the most dominating mechanism for the convective updrafts between -5oC and cloud top temperatures. 

How to cite: Deshmukh, A., Phillips, V., Waman, D., Patade, S., Bansemer, A., and Gupta, A.: Organization of SIP mechanisms among basic cloud types, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15890, https://doi.org/10.5194/egusphere-egu23-15890, 2023.

A new CALIPSO satellite retrieval for cirrus clouds has been developed over the last 1.5 years that retrieves ice particle number concentration, effective diameter, and ice water content.  It compares favorably with in situ measurements from many field campaigns around the world.  This talk would briefly describe the new method targeting single-layer cirrus clouds and focus on new findings resulting from this retrieval, relating them to climate model predictions.  These results indicate that there are two types or categories of cirrus clouds.  Type 1 cirrus appear to form through heterogeneous ice nucleation (het), have visible optical depths < 0.3, and are most abundant; they are what most people visualize as a “cirrus cloud”.  Type 2 cirrus may form through a combination of het and homogeneous ice nucleation, have visible optical depths > 0.3 (with visible extinction coefficients typically 4 times greater than type 1 cirrus), and are often associated with warm fronts, orographic gravity waves, and other lifting processes.  However, type 2 cirrus clouds constitute 76% to 88% (depending on latitude) of the estimated net cloud radiative effect of all cirrus clouds.  Based on comparisons between retrieved and predicted ice particle number concentrations and effective diameters, these type 2 cirrus clouds are poorly represented in climate models, possibly partly due to the predicted dependence of ice nucleation on layer-average pre-existing ice (not realistic near cloud top where ice nucleation occurs).  Predicted ice nuclei concentrations may also need revising. 

How to cite: Mitchell, D. and Garnier, A.: Characterizing two types of cirrus clouds that differ in nucleation mechanism and radiative effect, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16885, https://doi.org/10.5194/egusphere-egu23-16885, 2023.

EGU23-643 | ECS | Orals | AS1.11

Cloud cover estimation using different methods exploiting solar radiation measurements at various sites in Antarctica 

Claudia Frangipani, Raul Cordero, Adriana M. Gulisano, Angelo Lupi, Hector A. Ochoa, Penny Rowe, and Vito Vitale

Observations at the surface in Antarctica have always been challenging, but cloud observations are particularly scarce due to different factors, among which the polar night and lack of instruments and observers. One way to obtain information on cloud cover, and fill the gap, is through broadband radiation measurements thanks to methods based on the effect that clouds have on solar and terrestrial radiation. In this work three different algorithms have been studied and implemented: i) Long et al.[1] method, which exploits global and diffuse shortwave radiation components; ii) Kasten and Czeplak[2], based on global shortwave component alone; iii) APCADA[3] algorithm, which requires longwave downward radiation measurements and meteorological variables data, and is specially chosen as it yields results also at (polar) night. Different methods were selected to adapt to the data available at each site and to cross-check the results. The algorithms are tested on common-time data sets from three different stations: Marambio (64°14’50’’S - 56°37’39’’W), where upward and downward components for shortwave and longwave radiation are measured along with diffuse shortwave radiation; Professor Julio Escudero (62°12’57’’S - 58°57’35’’W) where downward shortwave and longwave radiation data are available; and Concordia (75°05’59’’S - 123°19’57’’E) where data on all components of both solar and terrestrial radiation are collected. Before any computation, data quality control is executed following tests[4] recommended by the Baseline Surface Radiation Network[5], showing good quality for all three data sets. Sky conditions depend on the location of the stations: Marambio and Escudero are coastal sites located on islands on opposite sides of the Antarctic Peninsula where cloudy skies are expected to occur, while Concordia is situated on the East Antarctic Plateau where the sky should be clearer. Such expectations are confirmed by the preliminary results obtained from the tested algorithms, indicating that clouds occur very often with almost scarce clear sky periods at the coastal stations. 

 

Bibliography
[1] Long C. N., Ackerman T. P., Gaustad K. L., and Cole J. N. S. (2006): “Estimation of fractional sky cover from broadband shortwave radiometer measurements”, J. Geophys. Res. 111, doi: 10.1029/2005JD006475
[2] Dürr B. and Philipona R. (2004): “Automatic cloud amount detection by surface longwave downward radiation measurements”, J. Geophys. Res. 109, doi: 10.1029/2003JD004182
[3] Kasten F., Czeplak G. (1980): “Solar and terrestrial radiation dependent on the amount and type of cloud”, Solar Energy 24, doi: 10.1016/0038-092X(80)90391-6
[4] Long and Shi (2008): “An automated quality assessment and control algorithm for surface radiation measurements”, Open Atm. Science J. 2, doi: 10.2174/1874282300802010023
[5] https://bsrn.awi.de/

How to cite: Frangipani, C., Cordero, R., Gulisano, A. M., Lupi, A., Ochoa, H. A., Rowe, P., and Vitale, V.: Cloud cover estimation using different methods exploiting solar radiation measurements at various sites in Antarctica, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-643, https://doi.org/10.5194/egusphere-egu23-643, 2023.

EGU23-667 | ECS | Orals | AS1.11 | Highlight

Cloud and precipitation profiles from observations  and Polar-WRF simulations over Vernadsky station (western Antarctic Peninsula) during austral winter 2022 

Anastasiia Chyhareva, Svitlana Krakovska, Irina Gorodetskaya, and Lyudmyla Palamarchuk

Intense moist intrusions originating from the lower latitudes of the Pacific Ocean have been found to have a significant impact on the Antarctic Peninsula (AP), including enhancement of surface melt events, increased runoff, reduction in sea-ice cover and ice shelves destabilization. Clouds play an important role in the surface energy budget during these events and in precipitation formation. Precipitation phase and amounts determine local and regional surface mass and energy budget. Our  research focuses on cloud and precipitation microphysical and dynamic characteristics over the AP region, using  ground based remote sensing at the Ukrainian Antarctic Station Akademic Vernadsky Moreover, an enhanced radiosonde program was launched during the austral winter at the Vernadsky station as part of the Year of Polar Prediction in the Southern Hemisphere (YOPP-SH) international initiative (May-August 2022). Here we present detailed analysis of one of the Targeted Observing Periods (TOPs) during an intense moisture and heat intrusion affecting the AP.

Although there is a lot of research on the atmospheric processes over the AP region, the local dynamic and microphysical characteristics of clouds and precipitation are still poorly understood and misrepresented in the models due to the lack of direct measurements, particularly in winter.

Further we performed  Polar-WRF model simulations, forced by ERA5 reanalysis and configured with Morrison double moment cloud microphysical scheme. The simulations were run at 1-km spatial resolution with 10-minute temporal output centered over the Vernadsky region. Simulation results were verified with precipitation properties derived from Micro Rain Radar-Pro measurements and radiosonde profiles. We found that there is  more snow in PolarWRF outputs in comparison to MRR-Pro measurements. Thus it does not represent mixed phased precipitation properly. At the same time Polar WRF shows warm temperature bias compared to radiosounding. 

Measurements and model output are used to analyze cloud ice and water particle distribution, thickness and precipitation particle spectra over the Vernadsky station and the AP mountains during the extreme precipitation events in the Antarctic Winter. In overall there were five TOPs over the AP region. However, not all of them were associated with extreme precipitation on Vernadsky station.

Our preliminary results show the importance of the transition between dry and wet snowfall during intense moisture transport events at the AP (particularly remarkable during winter at the location of Vernadsky station). Polar-WRF shows differences in simulating the timing and intensity of such transitions probably related to the biases in temperature profiles influencing the melting layer height.

How to cite: Chyhareva, A., Krakovska, S., Gorodetskaya, I., and Palamarchuk, L.: Cloud and precipitation profiles from observations  and Polar-WRF simulations over Vernadsky station (western Antarctic Peninsula) during austral winter 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-667, https://doi.org/10.5194/egusphere-egu23-667, 2023.

EGU23-901 | ECS | Orals | AS1.11 | Highlight

Warm Temperature Anomalies Associated with Snowfall in Antarctica 

Aymeric Servettaz, Cécile Agosta, Christoph Kittel, and Anaïs Orsi

Antarctica, the coldest and driest continent, is home to the largest ice sheet. A common feature of polar regions is the warming associated with snowfall, as moist oceanic air and cloud cover contribute to increase the surface temperature. Consequently, the ice accumulated onto the ice sheet is deposited under unusually warm conditions. Here we use the polar-oriented atmospheric model MAR to study the statistical difference between average and snowfall-weighted temperatures. Most of Antarctica experiences a warming scaling with snowfall, although with strongest warming at sites with usually low accumulation. Heavier snowfalls in winter contribute to cool the snowfall-weighted temperature, but this effect is overwritten by the warming associated with atmospheric perturbations responsible for snowfall, which particularly contrast with the extremely cold conditions in winter. Disturbance in apparent annual temperature cycle and interannual variability may have major implications for water isotopes, which are deposited with snowfall and commonly used for paleo-temperature reconstructions.

How to cite: Servettaz, A., Agosta, C., Kittel, C., and Orsi, A.: Warm Temperature Anomalies Associated with Snowfall in Antarctica, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-901, https://doi.org/10.5194/egusphere-egu23-901, 2023.

On the East Antarctic Plateau, in winter, rapid warming events originated by the advection of warm, moist air from lower latitudes, cause the disruption of the stable thermal structure of the atmosphere, and can be linked to the warming of the Plateau region itself. Continuous monitoring of these events can shed light on temperature trends in East Antarctica, trends which are still not clearly defined in terms of origin and amount.

Since the main mechanism acting in the warming events is the strong increase in cloud cover linked to the higher water content of the advected air, for a systematic monitoring of warming phenomena a simultaneous detection of water vapor vertical profile and cloud properties is needed. These two tasks can be both performed through the analysis of spectrally resolved atmospheric downwelling emitted radiances.

The REFIR (Radiation Explorer in the Far Infrared) Fourier transform spectroradiometer was installed at Concordia station, in the Dome C region of the Antarctic Plateau, in December 2011, and it has been performing continuous measurement since then. REFIR measures the downwelling atmospheric radiance in the 100-1500 cm-1 (6.7-100 µm) spectral interval, with a resolution of 0.4 cm-1, and with a repetition rate of about 10 minutes. The measured spectral interval extends from the far infrared, which includes the water vapor rotational band, to the atmospheric window region (8-14 µm), which provides information about the radiative effects of clouds.

A dedicated inversion code was developed to retrieve vertical profiles of water vapor and temperature from the measured emission spectra. The retrieved profiles allow for the monitoring of the evolution of the vertical structure of the troposphere on a 10 minutes timescale, whereas the spectral radiance itself provides, in a more direct way, information on the cloud cover. Therefore, the dataset produced by the REFIR instrument allow us to detect and obtain statistics about warming events in the Dome C region.

How to cite: Bianchini, G., Belotti, C., Di Natale, G., and Palchetti, L.: Exploiting a decadal time-series of spectrally resolved downwelling infrared radiances at Dome C, Antarctica to assess the occurrence of advective warming events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1528, https://doi.org/10.5194/egusphere-egu23-1528, 2023.

EGU23-5075 | Orals | AS1.11

Measuring snowfall properties with the open-source Video In Situ Snowfall Sensor 

Maximilian Maahn, Nina Maherndl, and Isabelle Steinke

We do not know the exact pathways through which ice, liquid, cloud dynamics, and aerosols are interacting in clouds while forming snowfall but the involved processes can be identified by their fingerprints on snow particles. The general shape of individual crystals (dendritic, columns, plates) depends on the temperature and moisture conditions during growth from water vapor deposition. Aggregation can be identified when multiple individual particles are combined into a snowflake. Riming describes the freezing of cloud droplets onto the snow particle and can eventually form graupel. In order to exploit these unique fingerprints of cloud microphysical processes, optical in situ observations are required.

The Video In Situ Snowfall Sensor (VISSS) was specifically developed for a campaign in the high Arctic (MOSAiC) to determine particle shape and particle size distributions. Different to other sensors, the VISSS minimizes uncertainties by using two-dimensional high-resolution images, a large measurement volume, and a design limiting the impact of wind. Tracking of particles over multiple frames allows determining fall speed and particle tumbling. The instrument design and software will be released as open-source. Here, we present the design of the instrument, show how particles are detected and tracked and introduce first results from campaigns in the high Arctic (MOSAiC), in the Colorado Rocky Mountains (SAIL), and in and Hyytiälä (Finland).  

How to cite: Maahn, M., Maherndl, N., and Steinke, I.: Measuring snowfall properties with the open-source Video In Situ Snowfall Sensor, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5075, https://doi.org/10.5194/egusphere-egu23-5075, 2023.

EGU23-5650 | ECS | Orals | AS1.11

Mixed-phase Multilayer Clouds in the Arctic: A Simulation Study using ICON 

Gabriella Wallentin, Corinna Hoose, Peggy Achtert, and Matthias Tesche

Multilayer clouds (MLCs), defined as individual, vertically overlapping clouds, are frequently occurring worldwide but have been far less studied than single layered clouds. Earlier studies have suggested a clear abundance of MLCs in the Arctic compared with the rest of the world and with data from the MOSAiC campaign in 2019-2020 we have classified multilayered clouds at a 52% frequency of occurrence. The microphysical interaction between these cloud layers is expected to be complicated, such as the seeder- feeder mechanism, and we thus employ a model to further investigate these clouds. 

Cases from the MOCCHA campaign in 2018 as well as the MOSAiC campaign in 2019-2020 have been selected for MLC occurrences. These cloud systems vary from vertically distinct layers with no potential of seeding (subsaturated layer of >3km) to a doubly layered system within the boundary layer with frequent seeding events. The structure of the former can be simulated at a coarse grid spacing, provided appropriate initial conditions and aerosol concentration, whilst the latter is highly dependent on initial and boundary conditions, resolution, and parameterisation for the boundary layer. 

Together with an analysis of the measurements on board of the ships, the ICON (ICOsahedral Non-hydrostatic) model was deployed. The simulations are run with refined nests down to 75 meters horizontal grid spacing in ICON-LEM. Initial and boundary data are supplied by both ICON Global and IFS. As the Arctic aerosol contribution is yet to be parameterised, we are further making use of the prognostic aerosol module ART (Aerosol and Reactive Trace gases) developed by KIT, set up specifically for cloud condensation nuclei activation for sea salt and sulfate. 

Various sensitivity experiments have been performed on these case studies including (i) sensitivity to microphysical parameters, such as CCN and INP parameterisation and concentration, (ii) sensitivity to horizontal and vertical resolution as well as (iii) initial and boundary condition impacts on resolving the cloud layers. Furthermore, the aerosol concentration has been scaled, in the existing parameterisations in ICON, to represent the measurements on site as well as prognostically run using ICON-ART. 

Preliminary results on the modelled multilayer cloud system highlight a high dependency on the initial and boundary data quality as well as domain resolution while the microphysics have a smaller impact on the formation and detailed structure of the multilayer cloud system.

How to cite: Wallentin, G., Hoose, C., Achtert, P., and Tesche, M.: Mixed-phase Multilayer Clouds in the Arctic: A Simulation Study using ICON, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5650, https://doi.org/10.5194/egusphere-egu23-5650, 2023.

EGU23-5802 | ECS | Orals | AS1.11

Transforming cloudy air masses and surface impacts: a case study confronting MOSAiC observations, reanalyses and coupled model simulations 

Sandro Dahlke, Amélie Solbès, Matthew D. Shupe, Christopher J. Cox, Marion Maturilli, Annette Rinke, Wolfgang Dorn, and Markus D. Rex

Variability in the components of the Arctic surface energy budget and the atmospheric boundary layer (ABL) structure are to a large extent controlled by synoptic-scale changes and associated air mass properties. The transition of air masses between the radiatively clear and cloudy states, along with their characteristic surface impacts in radiation and ABL structure, can occur in either direction and on short time scales. In both states as well as during the transition, insufficient model representation of radiative processes and cloud microphysical properties cause biases in numerical weather prediction- and climate models. We employ observations from radiosondes, MET tower, and the ShupeTurner cloud microphysics product, which itself synthesizes a wealth of instruments, for the classification of an event of transition between low-level mixed phase cloud and clear conditions. The observed air mass properties and transition process are compared to ERA5 reanalysis data and output from a simulation of the coupled regional climate model HIRHAM-NAOSIM which applied non-spectral nudging to ERA5 in order to reproduce the observed synoptic-scale changes. The approach highlights the potential of event-based analysis of transformations of cloudy Arctic air masses by confronting models with observations.

 

How to cite: Dahlke, S., Solbès, A., Shupe, M. D., Cox, C. J., Maturilli, M., Rinke, A., Dorn, W., and Rex, M. D.: Transforming cloudy air masses and surface impacts: a case study confronting MOSAiC observations, reanalyses and coupled model simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5802, https://doi.org/10.5194/egusphere-egu23-5802, 2023.

EGU23-5876 | ECS | Orals | AS1.11

Airborne measurements of the cloud impact on the surface radiative energy budget in the Fram Strait 

Sebastian Becker, André Ehrlich, Michael Schäfer, and Manfred Wendisch

Clouds play an important role in the climate system of the Arctic. The interaction of clouds with atmospheric radiation has a significant influence on the radiative energy budget (REB) of the Arctic surface, which is quantified by the surface cloud radiative effect (CRE). Due to the counteraction of the cooling effect of clouds in the solar and their warming effect in the thermal-infrared spectral range, the total CRE depends on a complex interplay of the illumination, surface, thermodynamic, and cloud conditions.

To characterize the CRE for a variety of environmental conditions, broadband radiation measurements were performed during three seasonally distinct airborne campaigns. The flights were conducted over sea ice and open ocean surfaces in the eastern Fram Strait. The analysis focusses on the differences of the CRE with respect to the different campaigns and surface types. It was found that clouds cool the open ocean surface during all campaigns. In contrast, clouds mostly have a warming effect on sea ice–covered surfaces, which neutralizes during mid-summer. Given the seasonal cycle of the sea ice distribution, these results imply a cooling effect of clouds on the surface during the sea ice minimum in late summer and a warming effect during the sea ice maximum in spring in the Fram Strait region. The variability of, e. g., cloud and synoptic conditions causes deviations of the CRE from these statistics. In particular, the study presents the evolution of the CRE during selected cases of warm air intrusions and marine cold air outbreaks.

How to cite: Becker, S., Ehrlich, A., Schäfer, M., and Wendisch, M.: Airborne measurements of the cloud impact on the surface radiative energy budget in the Fram Strait, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5876, https://doi.org/10.5194/egusphere-egu23-5876, 2023.

EGU23-6007 | ECS | Orals | AS1.11

Impact of Atmospheric Rivers on Poleward Moisture Transport and Arctic Climate on Interannual Timescales 

Marlen Kolbe, Jeroen Sonnemans, Richard Bintanja, Eveline van der Linden, Karin van der Wiel, Kirien Whan, and Imme Benedict

The projected increase in poleward moisture transport (PMT) towards warmer climate has mainly been linked to the larger moisture holding capacity of warmer air masses. However, the future of interannual fluctuations of PMT and associated driving mechanisms are fairly uncertain. This study demonstrates the extent to which atmospheric rivers (ARs) explain the interannual variability of PMT, as well as related variables such as temperature, precipitation and sea ice. Such linkages help to clarify if extreme precipitation or melt events over Arctic regions are dominantly caused by the occurrence of ARs. A main focus is set on the impact of ARs on Arctic sea ice on interannual timescales, which so far has been poorly studied, and varies from colder to warmer climates.

To robustly study these interannual linkages of ARs and Arctic Climate, we examine Arctic ARs in long climate runs of one present and two future climates (+2°C and +3°C), simulated by the global climate model EC-Earth 2.3. To enhance the significance of the results, three different moisture thresholds were used to detect ARs. Further, the use of additional thresholds relative to the 2°C and 3° warmer climates allowed a distinction between thermodynamic and dynamic processes that lead to changes of ARs from colder to warmer climates. It is found that most PMT variability is driven by ARs, and that the share of ARs which explain moisture transport increases towards warmer climates. We also discuss the role of the position and strength of the jet stream in driving AR variability and highlight the importance of ARs in generating interannual fluctuations of Arctic climate variables such as temperature and precipitation.

How to cite: Kolbe, M., Sonnemans, J., Bintanja, R., van der Linden, E., van der Wiel, K., Whan, K., and Benedict, I.: Impact of Atmospheric Rivers on Poleward Moisture Transport and Arctic Climate on Interannual Timescales, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6007, https://doi.org/10.5194/egusphere-egu23-6007, 2023.

EGU23-7246 | Orals | AS1.11 | Highlight

HALO-(AC)3: Airborne Observations of Arctic Clouds in Airmass Transformations 

André Ehrlich, Manfred Wendisch, Marcus Klingebiel, Mario Mech, Susanne Crewell, Andreas Herber, and Christof Lüpkes and the HALO-(AC)3 team

Clear indications of the phenomenon of Arctic Amplification include the above-average increase of the near-surface air temperature and the related dramatic retreat of sea ice observed in the last decades. The mechanisms behind these features are widely discussed. Especially the role of clouds and of air mass transports into and out of the Arctic associated with related transformation processes are still poorly understood. Therefore, the HALO-(AC)3 campaign was performed to provide observations of meridional air mass transports and corresponding transformations in a quasi-Lagrangian approach. Three research aircraft equipped with state-of-the-art instrumentation performed measurements over the Arctic ocean and sea ice in March/April 2022. The German High Altitude and Long Range Research Aircraft (HALO), equipped with a comprehensive suite of active and passive remote sensing instruments and dropsondes, was operated from Kiruna, Sweden. The flight pattern covered long distances at high altitudes up to the North Pole probing air masses multiple times on their way into and out of the Arctic. The Polar 5 (remote sensing) and Polar 6 (in-situ) aircraft from the Alfred Wegener Institute operated in the lower troposphere out of Longyearbyen in the lower troposphere over Fram Strait West of Svalbard. Several coordinated flights between the three aircraft were conducted with Polar 6 sampling in-situ aerosol, cloud, and precipitation particles within the boundary layer, Polar 5 observing clouds and precipitation from above roughly at 3 km altitude, and HALO providing the large scale view on the scene following air masses.
The observations cover a major warm air intrusion event with atmospheric river embedded bringing warm and moist air far into the Arctic. Multiple cold air outbreaks were characterized in their initial stage close to the sea ice edge with Polar 5 and 6 and in a quasi-Lagrangian perspective with HALO, which allowed to quantify the air mass transformation by changes of thermodynamic profiles, large scale subsidence, and cloud properties over a period of 24 hours. Single events of high latitude Arctic cirrus and the formation of a polar low are included in the data set. The presentation reports on first results of the campaign by illustrating the capabilities of the multi-aircraft operation.

How to cite: Ehrlich, A., Wendisch, M., Klingebiel, M., Mech, M., Crewell, S., Herber, A., and Lüpkes, C. and the HALO-(AC)3 team: HALO-(AC)3: Airborne Observations of Arctic Clouds in Airmass Transformations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7246, https://doi.org/10.5194/egusphere-egu23-7246, 2023.

EGU23-7692 | ECS | Orals | AS1.11

The effect of cloud top cooling on the evolution of the Arctic boundary layer observed by balloon-borne measurements 

Michael Lonardi, Christian Pilz, Elisa F. Akansu, André Ehrlich, Matthew D. Shupe, Holger Siebert, Birgit Wehner, and Manfred Wendisch

The presence of clouds significantly affects Arctic boundary layer dynamics. However, the accessibility of clouds over the Arctic sea ice for in-situ observations is challenging. Measurements from tethered balloon platforms are one option to provide high-resolution data needed for model evaluation.

The tethered balloon system BELUGA (Balloon-bornE moduLar Utility for profilinG the lower Atmosphere) was deployed to profile the boundary layer at the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC), and in Ny-Alesund. A set of scientific payloads for the observation of broadband radiation, turbulence, aerosol particles, and cloud microphysics properties were operated to study the interactions in the cloudy and cloud-free boundary layer.

Measurements obtained under various cloud conditions, including single-layer and multi-layer clouds, are analyzed. Heating rates profiles are calculated to validate radiative transfer simulations and to study the temporal development of the cloud layers. 

The in-situ observations display the importance of radiation-induced cloud top cooling in maintaining stratocumulus clouds over the Arctic sea ice. Case studies also indicate how the subsequent turbulent mixing can lead to the entrainment of aerosol particles into the cloud layer.

How to cite: Lonardi, M., Pilz, C., Akansu, E. F., Ehrlich, A., Shupe, M. D., Siebert, H., Wehner, B., and Wendisch, M.: The effect of cloud top cooling on the evolution of the Arctic boundary layer observed by balloon-borne measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7692, https://doi.org/10.5194/egusphere-egu23-7692, 2023.

EGU23-8107 | ECS | Orals | AS1.11 | Highlight

The extraordinary March 2022 East Antarctica heatwave 

Jonathan Wille and the East Antarctica heatwave project

Between March 15-19th 2022, East Antarctica experienced an unprecedented heatwave with widespread 30-45° C temperature anomalies across the ice sheet. This record-shattering event saw numerous monthly temperature records being broken including a new all-time temperature record of -9.4 °C on March 18th at Concordia station despite March typically being a transition month to the Antarctic coreless winter. The driver for these temperature extremes was an unprecedently intense atmospheric river (AR) advecting heat and moisture deep into the Antarctic interior. The scope of the temperature records spurred a large, diverse collaborative effort to study the heatwave’s meteorological drivers, impacts, and historical climate context using an array of observations, models, and analysis techniques. 

 From these efforts, we present the following

  • Temperature observations and records
  • Meteorological drivers including tropically forced Rossby wave activity along with AR and warm conveyor belt dynamics
  • Radiative forcing impacts on surface temperatures and inversions
  • Surface mass balance impacts
  • Discussion of the AR impacts on isotope and cosmic ray measurements from Concordia station
  • AR influence on the Conger Ice Shelf disintegration
  • Event return time analysis
  • Implications on past climate reconstructions
  • Future event likelihood from IPSL-CM6 simulations

How to cite: Wille, J. and the East Antarctica heatwave project: The extraordinary March 2022 East Antarctica heatwave, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8107, https://doi.org/10.5194/egusphere-egu23-8107, 2023.

EGU23-8500 | ECS | Orals | AS1.11

The effects of warm air intrusions in the high arctic on cirrus clouds 

Georgios Dekoutsidis, Silke Groß, and Martin Wirth

In the last decades scientist have noticed that the average global temperature of the Earth has been increasing. Moreover, the arctic is warming significantly faster than the global average, a phenomenon labeled Arctic Amplification. Two atmospheric components contributing to the warming of the atmosphere in the arctic are water vapor and cirrus clouds. Both have an effect on the radiation budget of the atmosphere and more specifically the longwave radiation. A Warm Air Intrusion (WAI) event is defined as the meridional transport of warm, water-vapor-rich airmasses into the arctic. During such events large amounts of water vapor can be transported into the arctic, which also leads to high supersaturations aiding the formation and longevity of cirrus clouds. There is a strong hypothesis that WAI events in the high arctic are becoming more frequent, so it is important to study the effects these events have on the macrophysical and optical properties of cirrus clouds in the arctic.

The HALO-(AC)3 flight campaign was conducted in March/April 2022 with the central goal of studying WAI events in the arctic regions of the Northern Hemisphere. For this campaign the German research aircraft HALO was equipped with remote sensing instrumentation, including the airborne LIDAR system WALES which we use in this study. WALES is a combined water vapor differential absorption and high spectral resolution lidar. It provides water vapor measurements in a 2D field along the flight track. We combine these measurements with ECMWF temperature data and calculate the Relative Humidity with respect to ice (RHi) inside and in the vicinity of cirrus clouds. For each flight we studied the synoptic situation and created two groups: One containing flights were cirrus that formed in arctic airmasses were measured and another were cirrus were measured during WAI events, henceforth arctic cirrus and WAI cirrus respectively. Our main goal is to compare the humidity characteristics inside and in the vicinity of arctic cirrus clouds and WAI cirrus clouds.

For the arctic cirrus we find that 49 % of the in-cloud data points are supersaturated with RHi mostly below the lower threshold for heterogeneous nucleation (low HET). The cloud-free air around these clouds has a supersaturation percentage of 8.5 %. The WAI cirrus are measured in a wider temperature range and also have a significantly higher supersaturation percentage inside as well as in the cloud-free air, 61.7 % and 9.3 % respectively. The majority is again in the low HET regime. Additionally, WAI cirrus are on average geometrically thicker than arctic cirrus. Finally, regarding the vertical distribution of RHi within these clouds we find that WAI cirrus have their highest supersaturations near the cloud top and become gradually subsaturated towards cloud-bottom. On the other hand, arctic cirrus have their highest supersaturations near cloud-middle, with lower supersaturations at cloud-top and subsaturated cloud-bottom.

How to cite: Dekoutsidis, G., Groß, S., and Wirth, M.: The effects of warm air intrusions in the high arctic on cirrus clouds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8500, https://doi.org/10.5194/egusphere-egu23-8500, 2023.

EGU23-9110 | Posters on site | AS1.11

Multi-year precipitation characteristics based on in-situ and remote sensing observations at the Arctic research site Ny-Ålesund, Svalbard 

Kerstin Ebell, Christian Buhren, Rosa Gierens, Melanie Lauer, Giovanni Chellini, Sandro Dahlke, and Pavel Krobot

Precipitation is a key variable in the hydrological cycle. However, observations of precipitation are quite challenging and even more so in remote locations such as the Arctic. The Arctic is experiencing a rapidly changing climate with a strong increase in near-surface air temperature, known as Arctic Amplification. In particular, the Svalbard archipelago is located in the warmest region of the Arctic and reveals the highest temperature increase (Dahlke and Maturilli, 2017). Such changes also affect the hydrological cycle. For example, climate models reveal a strong increase in precipitation in the Arctic (McCrystall et al., 2021) with rain becoming the most dominant precipitation type (Bitanja and Andry, 2017). Continuous detailed observations, which can also be set in context to satellite products and reanalyses data, are necessary to better understand precipitation and precipitation related processes in the Arctic.

In this study, we make use of the complementary precipitation observations performed as part of the Transregional Collaborative Research Centre on Arctic Amplification TR172 (http://www.ac3-tr.de; Wendisch et al., 2017) at the Arctic research station AWIPEV at Ny-Ålesund, Svalbard, to analyze precipitation characteristics in detail. The observations include an OTT Pluvio2 weighing gauge, an OTT Parsivel2 distrometer and a METEK MRR-2 micro rain radar (MRR). While the Pluvio and the Parsivel provide information on surface precipitation amount and type, the MRR provides information on the vertical structure of precipitation up to a height of 1 km. Measurements are available since spring/summer 2017 allowing for an analysis of more than 4 years of data.

First results show that the yearly precipitation amount based on Pluvio ranges from 306 mm to 552 mm (values are uncorrected for undercatch). Using the one-minute resolved data of Parsivel, precipitation frequency is highly variable within the different months ranging from 0.4 % to 18.8 % with solid precipitation being the most dominant type typically from September to March and liquid precipitation in the months May to August. In addition to monthly and yearly statistics, we will also characterize and analyze in detail the individual precipitation events. One question to be addressed is how much of the precipitation is related to atmospheric rivers (ARs). ARs are long, narrow, and transient corridors of strong horizontal water vapor transport which account for 80-90 % of the poleward moisture transport. Although their occurrence in the Arctic is limited, they are a significant source of rain and snow in the Arctic. Understanding linkages between precipitation and weather events and using observational data to evaluate models and reanalysis in the current climate will aid developing more accurate future predictions.

How to cite: Ebell, K., Buhren, C., Gierens, R., Lauer, M., Chellini, G., Dahlke, S., and Krobot, P.: Multi-year precipitation characteristics based on in-situ and remote sensing observations at the Arctic research site Ny-Ålesund, Svalbard, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9110, https://doi.org/10.5194/egusphere-egu23-9110, 2023.

EGU23-9323 | Posters on site | AS1.11

Observations of ice optical and microphysical properties in Arctic low-level mixed-phase clouds during ACLOUD 

Emma Järvinen, Franziska Nehlert, Guanglang Xu, Fritz Waitz, Guillaume Mioche, Regis Dupuy, Olivier Jourdan, and Martin Schnaiter

Observations of late spring and summer time stratiform clouds over pack ice, marginal sea ice zone and open water during the ACLOUD campaign have shown that relatively high ice particle number concentrations up to 35 L-1 are observed in cases where cloud top temperatures are between -3.8 and -8.7°C. This elevation in ice crystal number can likely be linked with secondary ice production. Simultaneous measurements of ice optical properties showed that a relative low asymmetry parameter between 0.69 and 0.76 can be associated with the mixed-phase cloud ice crystals. The condensed water path is dominated by the liquid phase at the cloud top in most of the studied cases except in one case study of a system with embedded convection where ice extinction exceeded the liquid extinction. Radiative transfer simulations have shown that the ice phase in low-level mixed-phase clouds, otherwise dominated by liquid phase, can also be radiatively important in cases where ice phase contributes to the cloud top extinction. This highlights the importance of an accurate vertical information of ice extinction within Arctic low-level clouds. The results of this study provide an important basis for testing and improving cloud microphysical parameterizations in models in order to accurately predict Arctic warming.

How to cite: Järvinen, E., Nehlert, F., Xu, G., Waitz, F., Mioche, G., Dupuy, R., Jourdan, O., and Schnaiter, M.: Observations of ice optical and microphysical properties in Arctic low-level mixed-phase clouds during ACLOUD, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9323, https://doi.org/10.5194/egusphere-egu23-9323, 2023.

EGU23-9784 | ECS | Posters on site | AS1.11

Airborne Closure of Moisture Budget inside Arctic Atmospheric Rivers 

Henning Dorff, Heike Konow, Vera Schemann, Davide Ori, Mario Mech, and Felix Ament

Among arctic moist air intrusions, atmospheric rivers (ARs) provide substantial moisture transport over long distances poleward. Along their corridors, warm and moist air masses undergo various transformation processes and can cause regional sea ice decline, especially when they induce precipitation as rain. Quantifying the components of the atmospheric moisture budget in arctic ARs is key to elucidate their precipitation efficiency. We close the AR moisture budget by measurements of the High Altitude LOng range research aircraft (HALO) during the recent HALO-(AC)³ campaign (Spring, 2022) in the vicinity of the Fram Start and Arctic ocean.

Our analysis is based on a strong AR event that HALO observed on two consecutive days during the occurrence of a sequence of moist air intrusions mid of March 2022. Dropsondes detect the vertical atmospheric profile and therefrom quantify the integrated water vapour transport (IVT) along AR cross sections. Applying regression methods then allows calculating the divergence of IVT. Since the limited number of dropsondes may deteriorate such calculations, we estimate the arising uncertainties using the ICOsahedral Nonhydrostatic model (ICON) in a storm-resolving configuration. Retrieved moisture profiles from the microwave radiometer (HAMP) further complement the sporadic sonde-based moisture profiles. We use the nadir cloud and precipitation radar mounted aboard HALO to derive precipitation rates along the flight curtains.

As the comparison with ICON suggests, the set of dropsondes to derive the IVT divergence within a reasonable range. The advection of moisture is roughly twice as strong as mass convergence. Both components act on different heights, with convergence dominating in the boundary layer (0-1 km) near the low-level jet, whereas moisture advection is more elevated (1-4 km). The strongest moisture convergence arises in the warm prefrontal AR sector while precipitation dominates slightly westwards in the AR centre. The investigated AR event caused rain over sea-ice with a melting layer up to 1.5 km. While there was less IVT on the second observation day, mean precipitation increased from the first day. Model simulations show that evaporation makes only a small contribution to the budget.  Within the ICON simulations, the comparison of precipitation purely based on the along-track radar curtain against that over the entire AR corridor indicates that the along-track curtain captures the mean precipitation intensity of the AR corridor, but misrepresents its spatial variability. However, the HALO devices outperform the ICON simulations in terms of the vertical variability of moisture conversion processes.

How to cite: Dorff, H., Konow, H., Schemann, V., Ori, D., Mech, M., and Ament, F.: Airborne Closure of Moisture Budget inside Arctic Atmospheric Rivers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9784, https://doi.org/10.5194/egusphere-egu23-9784, 2023.

EGU23-10197 | Orals | AS1.11

Atmospheric moisture intrusion into the Arctic: sources, impact, and trends 

Hailong Wang, Rudong Zhang, Yufei Zou, Weiming Ma, Philip Rasch, and Travis O'Brien

Atmospheric water vapor plays an enormously important role in the water cycle and energy budget of the Arctic. Water vapor in the Arctic also participates in many important feedback mechanisms influencing the climate response to forcing agents and the Arctic amplification. In this study, we conduct analysis of atmospheric moisture transport into the Arctic based on reanalysis products and CMIP6 model simulations. We are particularly interested in the episodic atmospheric-river-like features (AR or moisture intrusion) that play an important role in delivering water to the Arctic. Based on the method of using column-integrated meridional vapor transport for characterizing AR events, we find that the mean AR frequency peaks in the Atlantic sector in all seasons except that it’s more zonally widespread in summer. An increasing trend in the Arctic AR frequency in the recent decades identified from ERA5 can be captured by few CMIP6 models. The historical Arctic AR frequency, sea ice concentration and Arctic warming are highly correlated. Atmospheric circulation patterns that drive the interannual and decadal Arctic AR variation contribute substantially to the historical Arctic warming. We also use the Community Earth System Model (CESM), equipped with a water tagging capability, to quantify contributions of surface evaporation within the Arctic versus from lower-latitude regions as a source of water to the Arctic and characterize moisture transport pathways that control the Arctic water vapor distribution.

How to cite: Wang, H., Zhang, R., Zou, Y., Ma, W., Rasch, P., and O'Brien, T.: Atmospheric moisture intrusion into the Arctic: sources, impact, and trends, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10197, https://doi.org/10.5194/egusphere-egu23-10197, 2023.

EGU23-10530 | ECS | Orals | AS1.11 | Highlight

Central tropical Pacific convection drives extreme high temperatures and surface melt on the Larsen C Ice Shelf, Antarctic Peninsula 

Kyle Clem, Deniz Bozkurt, Daemon Kennett, John King, and John Turner

Northern sections of the Larsen Ice Shelf, eastern Antarctic Peninsula (AP) have experienced dramatic break-up and collapse since the early 1990s due to strong summertime surface melt, linked to strengthened circumpolar westerly winds. Here we show that extreme summertime surface melt and record-high temperature events over the eastern AP and Larsen C Ice Shelf are triggered by deep convection in the central tropical Pacific (CPAC), which produces an elongated cyclonic anomaly across the South Pacific coupled with a strong high pressure anomaly over Drake Passage. Together these atmospheric circulation anomalies transport very warm and moist air to the southwest AP, often in the form of “atmospheric rivers”, producing strong foehn warming and surface melt on the eastern AP and Larsen C Ice Shelf. Therefore, variability in CPAC convection, in addition to the circumpolar westerlies, is a key driver of AP surface mass balance and the occurrence of extreme high temperatures.

How to cite: Clem, K., Bozkurt, D., Kennett, D., King, J., and Turner, J.: Central tropical Pacific convection drives extreme high temperatures and surface melt on the Larsen C Ice Shelf, Antarctic Peninsula, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10530, https://doi.org/10.5194/egusphere-egu23-10530, 2023.

EGU23-11436 | Orals | AS1.11 | Highlight

Moisture transport into the Arctic in a past and future climate 

Sabine Eckhardt, Tove Svendby, Birthe Steensen, Gunnar Myhre, Ada Germundsen, and Dirk Olivie

The Arctic is warming at a faster rate than the rest of the globe. There are both remote and local mechanism identified driving this process. While albedo changes and atmospheric stability happens within in the Arctic, transfer transport processes, both in the ocean and atmosphere, heat and moisture into the Arctic. These processes can be analysed in a Eulerien way, by observing the fluxes through a curtain defining the Arctic or/and by Lagrangian analysis which follows this transport processes all the way from uptake in the mid/high latitudes until the inflow into the Arctic. 

We use a Lagrangian Particle Transport model FLEXPART running with ECMWF reanalysis data as well as with data from the norwegian earth system model NorESM, which represents the future climate scenarios until 2100. In this way we investigate the inflow of moisture and energy for the last 50 years, but can also project it in the future by considering the climate model output.

We find that the the transport through the 65N Latitude, defining the Arctic area is highly inhomogenious in space, but has also a distinct seasonal variability. The end of the storm tracks, especially the Northern Atlantic stormtrack show the most important region of inflow. While moisture origins over ocean areas in winter, continental areas in summer act as a source. The patterns in the reanalysis data from ECMWF and in the climate simulations are very similar. Those patterns are stable over time, but intensify in a warming climate.

How to cite: Eckhardt, S., Svendby, T., Steensen, B., Myhre, G., Germundsen, A., and Olivie, D.: Moisture transport into the Arctic in a past and future climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11436, https://doi.org/10.5194/egusphere-egu23-11436, 2023.

EGU23-11620 | Posters on site | AS1.11

Analyzing the development of cold air outbreaks and warm air intrusions based on remote sensing and dropsonde data from (AC)3 campaigns 

Marcus Klingebiel, Lukas Monrad-Krohn, Benjamin Kirbus, Mario Mech, André Ehrlich, and Manfred Wendisch

Within the framework of (AC)3, four airborne campaigns were conducted in the vicinity of Svalbard to investigate the Arctic airmass transformations during warm air intrusions (WAI) and marine cold air outbreaks (CAO). In this study, we will take a deeper look into the development process of CAOs starting from the marginal sea-ice zone towards the open ocean, using data from active and passive remote sensing instruments. In addition, we will present data from more than 450 dropsondes launched during the HALO-(AC)3 campaign and analyze the development of the vertical profiles along WAIs and CAOs. This is done by using a Lagrangian analysis of the campaign, which delivers same-day and next-day trajectory matches of the HALO flights.

How to cite: Klingebiel, M., Monrad-Krohn, L., Kirbus, B., Mech, M., Ehrlich, A., and Wendisch, M.: Analyzing the development of cold air outbreaks and warm air intrusions based on remote sensing and dropsonde data from (AC)3 campaigns, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11620, https://doi.org/10.5194/egusphere-egu23-11620, 2023.

EGU23-11951 | ECS | Posters on site | AS1.11

Influence of atmospheric rivers, cyclones and fronts on precipitation in the Arctic – a climatological perspective 

Melanie Lauer, Annette Rinke, Irina Gorodetskaya, Michael Sprenger, Mario Mech, and Susanne Crewell

The enhanced warming in the Arctic compared to the global mean – a phenomenon called Arctic Amplification - has different effects, including impacts on the hydrological cycle and thus the precipitation. In the Arctic, there are two major sources of moisture leading to increased precipitation formation: The enhanced local evaporation due to the missing insulation due to reduced sea-ice cover and the increased poleward moisture transport which is often associated with atmospheric rivers (ARs).

Previous studies have shown that ARs are a significant source for rain and snow in the Arctic. ARs are dynamically linked to the extratropical cyclones and fronts. Thus, AR-related precipitation can be not only concentrated within the AR itself, but also occur within the cyclone and frontal boundaries. Therefore, we developed a new method to distinguish precipitation within the AR shape and the precipitation related to cyclones and fronts based on ERA5 reanalysis. Thereby, we estimate how much precipitation occurs within AR, cyclone and frontal boundaries, separately and overlapping together. We applied this method for different case studies during two campaigns performed at and around Svalbard within the Collaborative Research Center “Arctic Amplification: Climate Relevant Atmospheric Surface Processes, and Feedback Mechanisms (AC)3”. Differences in the contributions of ARs, cyclones and fronts to the total precipitation could be identified comparing the both campaigns. During the early summer campaign (ACLOUD), precipitation (both rain and snow) was more confined within the AR shapes, especially in the area in which the AR is connected to fronts. In contrast, during the early spring campaign (AFLUX), precipitation (predominantly snow) was more restricted to the cyclone regions without connection to ARs and fronts. Generally, a higher precipitation intensity was found within ARs, especially when they are connected with cyclones and fronts.

In a climatological perspective, we apply this method to the ERA5 reanalysis data (1979 - 2020) to quantify the occurrence and influence of ARs and related cyclones and fronts. For this extended analysis, we consider the whole Arctic. This allows us to analyse the change of precipitation (in terms of type and frequency) related to the different weather systems during the last four decades. Furthermore, we can assess seasonal differences. In summary, we can investigate in which regions ARs, cyclones and fronts have a greater impact and if and how it also depends on different surface types (sea ice, open ocean, and land).

This work is supported by the DFG funded Transregioproject TR 172 “Arctic Amplification (AC)3“.

How to cite: Lauer, M., Rinke, A., Gorodetskaya, I., Sprenger, M., Mech, M., and Crewell, S.: Influence of atmospheric rivers, cyclones and fronts on precipitation in the Arctic – a climatological perspective, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11951, https://doi.org/10.5194/egusphere-egu23-11951, 2023.

EGU23-13074 | ECS | Orals | AS1.11

Linking aerosol size distribution and hygroscopicity to cloud droplet formation at an Arctic mountain site 

Ghislain Motos, Gabriel Freitas, Paraskevi Georgakaki, Jörg Wieder, Wenche Aas, Chris Lunder, Radovan Krejci, Julie T. Pasquier, Jan Henneberger, Robert O. David, Claudia Mohr, Paul Zieger, and Athanasios Nenes

The regulation of energy transfer by clouds and fog is a key process affecting the climate of the Arctic, a region that exhibits frequent cloud cover and suffers an extreme vulnerability to climate change. Measurements were performed over a whole year at the Zeppelin station, Ny-Ålesund, Svalbard, Norway from October 2019 to October 2020 in the framework of the NASCENT campaign (Ny-Ålesund AeroSol Cloud ExperimeNT). Aiming at a better understanding of the susceptibility of cloud droplet formation, we analyzed particle number size distributions obtained from differential mobility particle sizers and chemical composition derived from filter samples and an aerosol chemical speciation monitor. Combined with updraft velocity information from a wind lidar and an ultrasonic anemometer, the data were used as input parameters for a state-of-the-art cloud droplet formation parameterization to investigate the particle sizes that can activate to cloud droplets, the levels of supersaturation as well as potential cloud droplet formation and its susceptibility to aerosol. We showed that low aerosol levels in fall and early winter led to clouds that are formed under an aerosol-limited regime, while higher particle concentrations centered around the Arctic Haze together with a drop in cloud supersaturation could be linked to periods of updraft velocity-limited cloud formation regime. In the latter case, we observed that the maximum number of cloud droplets forming - also called the limiting droplet number - and the updraft velocity follow a relationship that is universal, as proved by similar studies previously performed in different environments and cloud types. Finally, we successfully performed a droplet closure, proving, for the first time, the ability of our cloud droplet parameterization to predict cloud droplet number not only in liquid clouds but also in mixed-phase clouds with a very high degree of glaciation. This closure suggests that rime splintering may not be significant enough to affect droplet concentrations, which is consistent with previous observations and model simulations.

How to cite: Motos, G., Freitas, G., Georgakaki, P., Wieder, J., Aas, W., Lunder, C., Krejci, R., T. Pasquier, J., Henneberger, J., O. David, R., Mohr, C., Zieger, P., and Nenes, A.: Linking aerosol size distribution and hygroscopicity to cloud droplet formation at an Arctic mountain site, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13074, https://doi.org/10.5194/egusphere-egu23-13074, 2023.

EGU23-13124 | ECS | Posters on site | AS1.11

Assessing Arctic low-level clouds and precipitation from above - a radar perspective 

Imke Schirmacher, Susanne Crewell, Katia Lamer, Mario Mech, and Manfred Wendisch

According to satellite-based estimations, a lot of clouds over the Arctic Ocean occur below
2 km. Most information on Arctic low-level clouds come from CloudSat radar measurements.
However, CloudSat lacks a complete representation of low-level clouds because the blind
zone masks the lowest kilometer and the coarse spatial sampling conceals cloud patterns.
Thus, higher resolved observations of cloud characteristics are needed to determine how
the cloud fraction varies close to the ground and how it depends on surface characteristics
and meteorological situation.

Our study investigates the low-level hydrometeor fraction of Arctic clouds over the ocean
using airborne remote sensing measurements by the Microwave Radar/radiometer for Arctic
Clouds (MiRAC) flown on the Polar 5 aircraft. Four campaigns have been conducted in the
vicinity of Svalbard during different seasons: ACLOUD, AFLUX, MOSAiC-ACA, and HALO-
AC3. We convolute the MiRAC radar reflectivity measurements to adapt the fine MiRAC and
coarse CloudSat resolution. The convoluted measurements are compared with the original
airborne observations over all campaigns to investigate the effects of CloudSat’s spatial res-
olution, clutter mask, and sensitivity on the low-level hydrometeor fraction. Measurements
reveal high hydrometeor fractions of up to 60% in the lowest 1.5 km, which CloudSat would
miss due to the blind zone. CloudSat would especially underestimate half of the total pre-
cipitation. During cold air outbreaks, when rolling cloud structures evolve, CloudSat over-
estimates the hydrometeor fraction most. Moreover, CloudSat does not resolve the separate
layers of multilayer clouds but rather merges them because of its coarse vertical resolution.

How to cite: Schirmacher, I., Crewell, S., Lamer, K., Mech, M., and Wendisch, M.: Assessing Arctic low-level clouds and precipitation from above - a radar perspective, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13124, https://doi.org/10.5194/egusphere-egu23-13124, 2023.

EGU23-13191 | ECS | Orals | AS1.11

The evolution of clouds in Arctic marine cold air outbreaks 

Rebecca Murray-Watson and Edward Gryspeerdt

Marine cold air outbreaks (MCAOs) are important parts of the high-latitude climate system and are characterised by strong surface fluxes generated by the air-sea temperature gradient. These fluxes promote cloud formation, which can be identified in satellite imagery by the distinct transformation of stratiform cloud 'streets' into a broken field of cumuliform clouds downwind of the outbreak. This evolution of cloud morphology changes the radiative properties of the cloud and therefore is of importance to the surface energy budget.  

While the drivers of stratocumulus-to-cumulus transitions have been extensively studied for subtropical clouds, such as aerosols or the sea surface temperature gradient, the factors influencing transitions at higher latitudes are relatively poorly understood. This work uses reanalysis data to create a set of composite trajectories of cold air outbreaks moving off the Arctic ice edge and co-locates these trajectories with data from multiple satellites to generate a unique view of cloud development within cold air outbreaks. 

Clouds embedded in MCAOs have distinctive properties relative to clouds following other, more stable trajectories in the region. The initial instability and aerosol environments have distinct impacts on cloud development within outbreaks. The strength of the outbreak has a lasting effect on the magnitude of cloud properties along the trajectory. However, it does not strongly affect the timing of the transition to cumuliform clouds. In contrast, the initial aerosol concentration changes the timing of cloud break-up rather than the size of the cloud response.

How to cite: Murray-Watson, R. and Gryspeerdt, E.: The evolution of clouds in Arctic marine cold air outbreaks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13191, https://doi.org/10.5194/egusphere-egu23-13191, 2023.

EGU23-13388 | Posters on site | AS1.11

Occurrence of multilayer clouds and ice-crystal seeding during the Arctic Ocean 2018 and MOSAiC research campaign 

Peggy Achtert, Matthias Tesche, Gabriella Wallentin, and Corinna Hoose

Previous research on arctic clouds has focused on single-layer clouds. However, the occurrence of multi-layer clouds in the Arctic is of importance, since in such systems upper clouds can influence the phase of lower clouds. This is the case when ice crystals fall from above into supercooled liquid water clouds and trigger the formation of mixed-phase clouds.

The aim of our project is to investigate the occurrence of multi-layer clouds and seeding using the combination of radiosonde and cloud radar observations. The focus is on the MOSAiC campaign. In order to classify and interpret the results, previous measurements will be used as well.

During the Arctic Ocean 2018 campaign multi-layer clouds were observed 56% of the time and 48 % showed a likelihood of seeding. Previous satellite studies on multi-layer-clouds showed an occurrence of 11 %. During the MOSAiC campaign multi-layer clouds occurred around 50 % of the time and showed a latitude dependency, with more multi-layer clouds north of 84°N.

How to cite: Achtert, P., Tesche, M., Wallentin, G., and Hoose, C.: Occurrence of multilayer clouds and ice-crystal seeding during the Arctic Ocean 2018 and MOSAiC research campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13388, https://doi.org/10.5194/egusphere-egu23-13388, 2023.

EGU23-14418 | ECS | Orals | AS1.11

Simulating the effects of Ice-nucleating particles in Antarctica in COSMO-CLM² 

Florian Sauerland, Niels Souverijns, Anna Possner, Heike Wex, Preben Van Overmeiren, Alexander Mangold, Kwinten Van Weverberg, and Nicole van Lipzig

The remoteness of the Antarctic continent has important implications for the microphysical properties of clouds: In particular, the rare abundance of ice-nucleating particles (INP) limits the primary nucleation of ice crystals. Yet, persistent mixed-phase clouds with ice crystal number concentrations of 0.1-1l-1 are still observed in the Arctic and Antarctic. However, the ability of regional climate models to reproduce these mixed-phase clouds remains limited, much like the knowledge about their climatological effects. Thus, we added a module to the regional climate model COSMO-CLM² aimed at improving the parametrisation of the aerosol-cycle, which allows us to prescribe different concentrations of INPs. We examined the model response to different concentrations by running it in an area around the Belgian Princess Elisabeth Station in Dronning Maud Land for one month and with four different concentration settings: The first, corresponding to the low end of INP concentrations we observed at the station, the second, corresponding to the high end of INP concentrations we observed at the station, and the third and fourth, to the low and high end of continental observations. The performance was evaluated by comparing the simulation results with radar and ceilometer observations taken at the station. Finally, we analysed the differences between the four simulations to determine the overall sensitivity of the model to variability in INP concentrations, which allows us to draw conclusions about the importance of accurately simulating processes related to ice nucleation, and about the climatological implications that a change in aerosol concentrations would have.

How to cite: Sauerland, F., Souverijns, N., Possner, A., Wex, H., Van Overmeiren, P., Mangold, A., Van Weverberg, K., and van Lipzig, N.: Simulating the effects of Ice-nucleating particles in Antarctica in COSMO-CLM², EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14418, https://doi.org/10.5194/egusphere-egu23-14418, 2023.

EGU23-15022 | ECS | Posters on site | AS1.11

Impact of Atmospheric Rivers on the Arctic Surface Energy Budget 

Sofie Tiedeck, Benjamin Kirbus, Melanie Lauer, Susanne Crewell, Irina Gorodetskaya, and Annette Rinke

Atmospheric Rivers (ARs) are long, narrow atmospheric structures which carry anomalously warm and moist air from lower latitudes into higher latitudes. Therefore, ARs are discussed to contribute to Arctic Amplification due to water vapor feedback and cloud-radiation processes. The detailed impact on the surface energy budget (SEB), however, is not fully understood.

We analyze the impact of ARs on the SEB of an early winter and spring case study, using ERA5 reanalysis data and model output from limited area simulations of ICON (ICON-LAM). Both cases show less energy loss of the surface compared to climatology, especially due to more downward longwave radiation and less upward sensible heat. The effect depends on the surface type, open ocean or sea ice. Next, we provide a climatological perspective on the impact of Atmospheric Rivers on the SEB based on ERA5.

How to cite: Tiedeck, S., Kirbus, B., Lauer, M., Crewell, S., Gorodetskaya, I., and Rinke, A.: Impact of Atmospheric Rivers on the Arctic Surface Energy Budget, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15022, https://doi.org/10.5194/egusphere-egu23-15022, 2023.

EGU23-16007 | ECS | Orals | AS1.11

One year of Aerosol and Cloud measurements in Rothera on the Antarctic Peninsula 

Floortje van den Heuvel, Tom Lachlan-Cope, Jonathan Witherstone, Joanna Dyson, Freya Squires, Daniel Smith, and Michael Flynn

Our limited understanding of clouds is a major source of uncertainty in climate sensitivity and climate model projections. The Southern Ocean is the largest region on Earth where climate models present large biases in short and long wave radiation fluxes which in turn affect the representation of sea surface temperatures, sea ice and ultimately large scale circulation in the Southern Hemisphere. Evidence suggests that the poor representation of mixed phase clouds at the micro- and macro scales is responsible for the model biases in this region. The Southern Ocean Clouds (SOC) project is a multi-scale, multi-platform approach with the aim of improving understanding of aerosol and cloud microphysics in this region, and their representation in numerical models.

In February 2022 we installed a suite of instruments at the Rothera research station on the Antarctic peninsula to measure the physical and chemical properties of aerosol, the number concentrations of Cloud Condensation Nuclei and Ice Nucleating Particles, and cloud height and thickness all year round. Here we will report the first observations and statistics of one full year of aerosol and cloud measurements from the Rothera research station.

How to cite: van den Heuvel, F., Lachlan-Cope, T., Witherstone, J., Dyson, J., Squires, F., Smith, D., and Flynn, M.: One year of Aerosol and Cloud measurements in Rothera on the Antarctic Peninsula, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16007, https://doi.org/10.5194/egusphere-egu23-16007, 2023.

EGU23-2324 | Orals | AS1.12

Observing the dynamics of deep convection using a tandem of spaceborne microwave radiometers 

Helene Brogniez, Remy Roca, Jean-Pierre Chaboureau, Franck Auguste, Ilhem Gharbi, Thomas Lefebvre, Thomas Fiolleau, and Dominique Bouniol

Deep convection plays a fundamental role in the climate system by transporting from the lower layers of the atmosphere to the free troposphere, air, water and momentum. Although its study has been the subject of intense and rich scientific activities for decades, our ignorance of the vertical distribution of convective movements in the heart of convective cells is today an important scientific and operational obstacle. Only space-borne observations can meet the needs in documentation necessary to progress on the science of the water and energy cycle and simultaneously improve numerical forecasting systems. Pending the emergence (hypothetical) of microwave missions in geostationary orbit with high repeatability (~ 1 minute), an approach based on satellite constellations in convoys could provide a first response.

The “Convective Core Observations through MicrOwave Derivatives in the trOpics”, or C2OMODO for short, proposes to rely on 2 passive microwave radiometers with a multispectral sampling of the 183 and 325 GHz lines in a mini-train of 2 satellites. The time-spacing of 60 to 180sec between the 2 swaths encompasses information on the updraft motions of hydrometeors, and is thus used to characterize the intensity and the size of individual updrafts in deep convective systems.

We will present this original observational strategy, associated to the NASA / AOS general framework, as well as its expected added-value for the characterization of deep convection.

How to cite: Brogniez, H., Roca, R., Chaboureau, J.-P., Auguste, F., Gharbi, I., Lefebvre, T., Fiolleau, T., and Bouniol, D.: Observing the dynamics of deep convection using a tandem of spaceborne microwave radiometers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2324, https://doi.org/10.5194/egusphere-egu23-2324, 2023.

EGU23-3105 | Posters on site | AS1.12

Insight of deep convection and sea surface wind gusts link through collocated GEO and LEO data 

Yu Li, Tran Vu La, Ramona-Maria Pelich, Marco Chini, Patrick Matgen, and Christophe Messager

Convective system (CS) is an extreme weather event occurring regularly over the subtropical and tropical regions such as the Gulf of Guinea, the Gulf of Mexico, Lake Victoria, Southeast Asia, India, and Australia. Certain CS types, i.e., mesoscale CS, supercell convective storms, squall lines, are disastrous for human life, infrastructures, and economic activities since they can produce strong surface winds, heavy rainfall, and significant lightning. Over the last decades, the CS observing, monitoring, and forecasting have been much improved thanks to a dense network of GEOstationary (GEO) satellites, including Meteosat, GEOS, Himawari, and Gaofen, covering Europe, Africa, America, and the Asia Pacific, respectively. However, the observation and prediction of the extreme weather events associated with deep convection are still a big challenge since they often occur suddenly, develop quickly, and become intense in a short time (several hours). Such unpredicted features are a significant issue for the numerical weather prediction models. While the prediction of intense rainfall associated with deep convection is still ongoing, the estimation of surface convective wind gusts has some important advancements. La et al. [1-2] indicated Sentinel-1 C-band Synthetic Aperture Radar (SAR) data with a high spatial resolution and wide swath bring significant advantages for observing and estimating ocean surface convective wind gusts. Indeed, through the images acquired by the Sentinel-1 Low Earth Orbit (LEO) satellite, one can observe convective wind patterns at both mesoscales and sub-mesoscales, as well as wind hot spots (15-25 m/s) at a small scale. The studies [1-2] also showed the relationship between surface wind patterns and deep convective clouds observed on Meteosat GEO images. In particular, the collocation of Sentinel-1, Aeolus Lidar, and Meteosat devices [3] enabled a multi-dimensional view of deep convection and its vertical and horizontal dynamics.

Following the previous studies, we illustrate in this paper more interesting cases of multi-dimensional CS observations by the collocated GEO and LEO sensors. They include sea surface convective wind patterns observed by Sentinel-1 LEO, intense downdrafts detected by Aeolus Lidar LEO, and deep convective clouds observed by Meteosat GEO. These cases expected to strengthen the relationship between deep convection and strong surface winds over the sea. In particular, we present the assessment of surface convective wind gust estimates through comparisons to in situ wind measurements by the moored buoys and weather stations. This work is a significant step to strengthen the conclusion that the high-intensity radar backscattering observed on Sentinel-1 C-band SAR images is associated with surface convective wind gusts rather than induced by precipitation.

[1] T. V. La and C. Messager, "Convective System Observations by LEO and GEO Satellites in Combination," IEEE JSTARS, vol. 14, pp. 11814-11823, 2021, doi: 10.1109/JSTARS.2021.3127401.

[2] T. V. La and C. Messager, "Different Observations of Sea Surface Wind Pattern Under Deep Convection by Sentinel-1 SARs, Scatterometers, and Radiometers in Collocation," IEEE JSTARS, vol. 15, pp. 3686-3696, 2022, doi: 10.1109/JSTARS.2022.3172375.

[3] La, T. V., & Messager, C. (2021). Convective system dynamics viewed in 3D over the oceans. Geophysical Research Letters, 48(5), e2021GL092397.

How to cite: Li, Y., La, T. V., Pelich, R.-M., Chini, M., Matgen, P., and Messager, C.: Insight of deep convection and sea surface wind gusts link through collocated GEO and LEO data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3105, https://doi.org/10.5194/egusphere-egu23-3105, 2023.

EGU23-4910 | Posters on site | AS1.12

Evaluating the L-MEB forward radiative transfer model for the assimilation of SMOS observations 

Mozhdeh Jamei and Ebrahim Asadi Oskouei

Satellite observations play an important role in providing the initial conditions for the Numerical Weather Prediction (NWP) models. Satellite data are assimilated into the first estimate provided by NWP models using a radiative transfer model. The impact of satellite observations significantly depends on the accuracy of the simulation performed by the radiative transfer (RT) models. In recent years, there have been significant advances in RT modeling for microwave and infrared observations, which are not sensitive to the surface. However, in the case of sensitive surface observations such as Soil Moisture and Ocean Salinity (SMOS) satellite observations, the assimilation has been limited by inaccuracy in the forward calculations. This study investigates the accuracy of the L-band Microwave Emission of the Biosphere (L-MEB) RT model for SMOS frequencies using high-quality in-situ observations as input. The L-MEB model is the forward RT model used in the SMOS L2 algorithm, specifically developed to simulate brightness temperature (TB) over the land surfaces at different incidence angles (between 0° and 60°). The L-MEB model simulated the SMOS TB data with the horizontal (H) and vertical (V) polarization at the lowest SMOS incidence angles at the meteorological stations over Iran.The land cover at these stations is either bare soil or low vegetation. The comparison between simulated TB and the SMOS TB products showed a suitable RMSE and a relatively low bias for horizontally and vertically polarized channels. The relatively low bias can justify the assimilation of SMOS observations into the data assimilation systems. However, cross-comparison of the RT models used at the NWP centers and the RT models such as L-MEB, which were mainly developed to work with the SMOS data, is required to ensure that the operational RT models used at the NWP centers meet the same accuracy.

 

How to cite: Jamei, M. and Asadi Oskouei, E.: Evaluating the L-MEB forward radiative transfer model for the assimilation of SMOS observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4910, https://doi.org/10.5194/egusphere-egu23-4910, 2023.

It has long been known that microphysics parameterizations are among leading sources of model uncertainty in storm and convective scale weather prediction.  The uncertainty results from combination of imperfect knowledge of the microphysics processes, inability to explicitly resolve them at computationally feasible spatial and phase-space resolutions, as well as from inherent limited predictability of micro to turbulent scale processes.   Representing these in the context of improving probabilistic prediction skill using ensembles has been the subject of many studies, but remains an outstanding problem.  The problem is especially acute in storm and convective scale ensemble prediction, where there may be strong coupling of errors between ensemble data assimilation and forecasting. 

Over the last decade, the inclusion of stochastic representation of model uncertainty associated with physical parameterizations has emerged as a viable approach for representing the intrinsic uncertainties of the microphysical parameterizations.  This study examines sensitivity of storm scale ensemble simulations to representation of microphysics parameterization uncertainties using a cloud resolving model.  We compare several stochastic parameter (SP) perturbation methods, including various parameter distributions and parameter covariance models, applied to physical parameters in a bulk microphysics parameterization.  The study follows a prior study, in which a 1D column version of the 3D cloud resolving model was used to test non-stochastic and several SP perturbation methods for which the parameter perturbation statistical distributions were based on Markov Chain Monte Carlo (MCMC) inversions with synthetic observations. That study indicated that SP schemes produce significantly more ensemble variance of microphysics states than non-stochastic, and that inclusion of parameter covariances, and specifically those that vary with the state of the system, improve their performance.

The current study investigates impacts of SP scheme configurations on microphysics with dynamical feedbacks in 3D ensemble simulations.  The statistical parameter distributions used for the SP scheme are obtained as in the 1D study using MCMC inversions with synthetic observations. The results are evaluated in terms of changes to the ensemble mean and variance of microphysical and dynamical states and the simulated column integral microphysics-sensitive satellite-based observable quantities. We discuss the results and note the implications for convective scale ensemble data assimilation and forecasting. 

How to cite: Vukicevic, T., Posselt, D., and Jurlina, S.: Evaluation of stochastic parameter representation of microphysics parameterization uncertainty for convective scale ensemble data assimilation and prediction, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5714, https://doi.org/10.5194/egusphere-egu23-5714, 2023.

Data assimilation techniques can improve the simulation of regional precipitation and temperature over complex regions. Nowadays, regional climate simulations using convection-permitting scales are becoming available, but the number of those simulations including an additional data assimilation scheme is rather small because of their high computational costs. Hence, it is important to evaluate the effect of data assimilation schemes for such convection-permitting simulations, and to determine if data assimilation produces any improvement in the simulation of temperature or precipitation fields.

To investigate this, we employ the Weather Research and Forecasting model (WRF; version 3.8.1) to dynamically downscale the state-of-the-art ERA5 reanalysis over Western Europe. A 3 km spatial resolution grid is employed, together with 51 vertical levels. The temporal resolution of the WRF outputs is one hour. Two model configurations are tested in two experiments spanning the period 2010-2020 after a one-year spin-up. In the first experiment (NoDA), after the initialization of the model, the boundary conditions drive the model. The second experiment (DA) is configured the same way as NoDA, but the additional 3DVAR data assimilation step (WRFDA) is run every six hours (00, 06, 12 and 18 UTC – analysis times). Observations obtained from the PREPBUFR dataset (NCEP ADP Global Upper Air and Surface Weather Observations) are employed, and only those included inside a 120 min window around analysis times were assimilated. For DA, monthly varying background error covariance matrices were created. In both cases, the model uses the Noah-MP land surface model, and high-resolution daily-varying SST fields from the NOAA OI SST v2 data set instead of the SST field from ERA5.

The results of this study show that both experiments produce similar monthly precipitation patterns to those from observational data sets such as IMERG and CHIRPS, or the reanalysis ERA5. However, in general, and particularly during summer months, DA produces larger amounts of precipitation than NoDA. These amounts are in line with those from CHIRPS. In terms of temperature, DA show colder temperatures than NoDA in most of the months, which again are similar to those from observational data sets such as CRU or EOBS. The monthly temperature patterns of both experiments are similar to those from both observational data sets. These results highlight the fact that NoDA already is able to generate reliable precipitation and temperature fields compared to diverse gridded observational data sets, but the 3DVAR data assimilation can additionally improve the performance of the regional model when convection-permitting scales are employed.

How to cite: González-Rojí, S. J. and Raible, C. C.: The effect of 3DVAR data assimilation and convection-permitting scales on the simulation of precipitation and temperature over Western Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6378, https://doi.org/10.5194/egusphere-egu23-6378, 2023.

EGU23-7868 | Posters on site | AS1.12

Learning model parameters from observations by combining data assimilation and machine learning 

Tijana Janjic, Yvonne Ruckstuhl, and Stefanie Legler

Parametrization of microphysics as well as parametrization of processes in the surface and boundary layers typically contain several tunable parameters. The parameters are not observed and are only crudely known. Traditionally, the numerical values of these model parameters are chosen by manual model tuning, leading to model errors in convection permitting numerical weather prediction models. More objectively, parameters can be estimated from observations by the augmented state approach during the data assimilation or by combing data assimilation with machine learning (ML).

If the parameters are updated objectively according to observations, they are flexible to adjust to recent conditions, their uncertainty is considered, and therefore the uncertainty of the model output is more accurate. To illustrate benefits of online augmented state approach, Ruckstuhl and Janjic (2020) show in an operational convection-permitting configuration that the prediction of clouds and precipitation is improved if the two-dimensional roughness length parameter is estimated. This could lead to improved forecasts of up to 6 h of clouds and precipitation. However, when parameters are estimated by the augmented state approach, stochastic model for the parameters needs to be pre-specified to keep the spread in parameters. Alternatively, Legler and Janjic (2022) investigate a possibility of using data assimilation for the state estimation while using ML for parameter estimation in order to overcome this problem. We train two types of artificial neural networks as a function of the observations or analysis of the atmospheric state.  The test case uses perfect model experiments with the one-dimensional modified shallow-water model, which was designed to mimic important properties of convection. Through perfect model experiments we show that Bayesian neural networks (BNNs) and ensemble of point estimate neural networks (NNs) are able to estimate model parameters and their relevant statistics. The estimation of parameters combined with data assimilation for the state decreases the initial state errors even when assimilating sparse and noisy observations.

How to cite: Janjic, T., Ruckstuhl, Y., and Legler, S.: Learning model parameters from observations by combining data assimilation and machine learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7868, https://doi.org/10.5194/egusphere-egu23-7868, 2023.

Deep convective cloud systems are one of the leading contributors to weather related disasters, provide much of the fresh water used by society, and contribute significantly to the interactions among weather and climate. Convection is known to be influenced strongly by the characteristics of its environment, including the vertical structure of temperature, moisture, and wind. It has also been shown in many numerical modeling studies to be sensitive to the assumptions made in the representation of cloud processes.

 

This presentation will explore the relative influence of environmental (extrinsic) factors and cloud microphysical parameter (intrinsic) uncertainty in the evolution of tropical deep convection. The effect of both types of factor on the energy and water cycle, as well as on convective dynamics and heating, are shown. Ensemble Monte Carlo experiments quantify convective storm sensitivity, while ensemble data assimilation experiments provide traceability from convective outcomes to control factors. The results have implications for modeling, data assimilation, and the design of future observing systems.

How to cite: Posselt, D.: The relative sensitivity of convective simulations to perturbations in initial conditions and microphysics parameters, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8429, https://doi.org/10.5194/egusphere-egu23-8429, 2023.

EGU23-9488 | Orals | AS1.12 | Highlight

Predictive hazards from convective systems with deep learning 

Jussi Leinonen, Ulrich Hamann, Ioannis Sideris, and Urs Germann

Convection is a complex spatiotemporal process, which has made it a particularly attractive application for deep learning, which excels at both spatial and temporal reasoning. We have developed deep learning models for predicting the occurrence of hazards caused by convective storms, so that this information may be used by forecasters, emergency services and infrastructure managers to respond to the threats caused by these hazards.

Our network is based on a recurrent-convolutional architecture that can process input data at multiple resolutions. It issues probabilistic predictions of hazard occurrence, currently up to 1 hour to the future. As inputs, we use data from weather radars, geostationary satellites, ground-based lightning detections, numerical weather predictions and digital elevation models. We have studied the importance of each data source to the quality of the predictions, finding that radar-based inputs contribute most to the prediction quality; however, some hazards can be well predicted also without radar, indicating that it is plausible to create warning systems for these hazards in areas where radar networks are not available.

In this presentation, we will describe the model architecture and case studies, as well as our experiences so far in bringing the model to real-time use by forecasters and automated warning systems at MeteoSwiss. We will also discuss future directions of this research.

How to cite: Leinonen, J., Hamann, U., Sideris, I., and Germann, U.: Predictive hazards from convective systems with deep learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9488, https://doi.org/10.5194/egusphere-egu23-9488, 2023.

Clouds are the first area-wide observable signal of convection. Although heavily used in nowcasting applications, the use of cloud-affected satellite observations in data assimilation is very limited.

This work aims to estimate the potential impact of assimilating cloud-affected satellite observations of visible (0.6 µm) and near thermal infrared wavelength (6.2 µm and 7.3 µm) relative to the impact of assimilating radar reflectivity observations. The observation types are evaluated in observing system simulation experiments (OSSE) featuring two cases: isolated and scattered supercells. In the first case, a supercell is triggered by a warm bubble (temperature perturbation) with uncertain location and strength but equal evolution in time. In the second case, random perturbations give rise to numerous supercells scattered throughout the domain, which are in different stages of their lifetime. Observations are simulated using the radiative transfer model RTTOV/MFASIS and assimilated by the Ensemble Adjustment Kalman Filter in the Data Assimilation Research Testbed (DART). The Weather Research and Forecasting (WRF) model at 2-km grid resolution was used for forecasts. 

Results show that the forecast impact is notably different in the two cases. For example, the Fractions Skill Score of precipitation and cloudiness indicates that satellite observations can be as beneficial as three-dimensional radar reflectivity observations in the first case, in which the prior contains no error in the stage of storm development but only in horizontal position and strength. Hence, the vertical structure information contained in three-dimensional radar reflectivity does not seem to add value compared to satellite observations, resulting in a similar impact of both observation types. In the second case, however, three-dimensional radar observations constrain the vertical structure and improve upon forecasts that only use satellite observations.

How to cite: Kugler, L. and Weissmann, M.: Assimilating cloud-affected visible & infrared satellite observations in idealized simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9876, https://doi.org/10.5194/egusphere-egu23-9876, 2023.

EGU23-10418 | ECS | Orals | AS1.12

Assessing the added value of Aeolus winds in the ECCC forecast system 

Chih-Chun (Gina) Chou, Paul J. Kushner, and Stéphane Laroche

The European Space Agency (ESA)’s Aeolus mission, launched in August 2018, provides the first global horizontal line-of-sigh (HLOS) wind profile measurements. Many Numerical Weather Prediction (NWP) centres, including ECMWF, DWD, Météo-France, Met-Office and ECCC, have shown that assimilating Aeolus winds improves overall forecast skill, especially in the tropics and data-sparse regions. To better characterize the locations and drivers of improved skill from Aeolus, we use a series of Observing System Experiments (OSEs) with the ECCC Global Deterministic Prediction System (GDPS) covering the period July to September 2019 and December 2019 to March 2020. Three experiments are used: CNTRL, CNTRL+Aeolus, and CNTRL-winds. All the observations assimilated in the GDPS are included in the CNTRL experiment. The Aeolus winds are added in the CNTRL+Aeolus experiment and the operational wind observations are withheld in the CNTRL-wind experiment. The impact of the operational winds and Aeolus are quantified by comparing the forecast error of the CNTRL-winds and CNTRL experiments with the CNTRL and CNTRL+Aeolus experiments. 

As expected, the operational winds improve the tropospheric forecast over the tropics the most, with a normalized forecast error of 8% for the wind field. By adding the Aeolus winds, which account for less than 1% of the observations, the tropospheric forecast further improves by 0.7-0.9% over the tropics and the Arctic, and by 0.5-0.6% over the data-sparse Southern Hemisphere extra-tropics. The added value of Aeolus winds is further highlighted when its impact on forecasts as a function of length scale is investigated, using a spherical harmonic decomposition. The impact is measured as the difference of the 250-hPa kinetic energy forecast error spectra between experiments. The impact of operational winds and Aeolus is dominated by the transient component whose impact is nearly four times greater than the impact on the mean component. The operational winds largely improve the forecast of global scale to intermediate scale in the short-range forecasts. The impact then decreases as forecast range increases. On the other hand, the impact of Aeolus is mostly seen in the intermediate to large scale range with a peak around spherical harmonics of degree 9 (scales about 4000 km), and is the smallest on day 1 and increases until days 4 to 5. This analysis suggests that Aeolus winds provide estimates of the wind state that are valuable and complementary to that provided from current operational winds.

How to cite: Chou, C.-C. (., Kushner, P. J., and Laroche, S.: Assessing the added value of Aeolus winds in the ECCC forecast system, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10418, https://doi.org/10.5194/egusphere-egu23-10418, 2023.

The NASA TROPICS Earth Venture (EVI-3) CubeSat constellation mission will provide nearly all-weather observations of 3-D temperature and humidity, as well as cloud ice and precipitation horizontal structure, at high temporal resolution to conduct high-value science investigations of tropical cyclones. TROPICS will provide rapid-refresh microwave measurements (median refresh rate of approximately 60 minutes for the baseline mission) over the tropics that can be used to observe the thermodynamics of the troposphere and precipitation structure for storm systems at the mesoscale and synoptic scale over the entire storm lifecycle. The TROPICS constellation mission comprises four 3U CubeSats (5.4 kg each) in two low-Earth orbital planes. Each CubeSat comprises a Blue Canyon Technologies bus and a high-performance radiometer payload to provide temperature profiles using seven channels near the 118.75 GHz oxygen absorption line, water vapor profiles using three channels near the 183 GHz water vapor absorption line, imagery in a single channel near 90 GHz for precipitation measurements (when combined with higher resolution water vapor channels), and a single channel at 205 GHz that is more sensitive to precipitation-sized ice particles. TROPICS spatial resolution, measurement sensitivity, and calibration accuracy and stability are all comparable with current state-of-the-art observing platforms. Two launches for the TROPICS constellation mission are planned for the Summer of 2023. Data will be downlinked to the ground via the KSAT-Lite ground network. NASA's Earth System Science Pathfinder (ESSP) Program Office approved the separate TROPICS Pathfinder mission, which launched on June 30, 2021, in advance of the TROPICS constellation mission as a technology demonstration and risk reduction effort. The TROPICS Pathfinder mission continues to yield excellent data over 18+ months of operation and has provided an opportunity to checkout and optimize all mission elements prior to the primary constellation mission. This presentation will describe the on-orbit results for the successful TROPICS Pathfinder precursor mission and will describe the recent development progress for the TROPICS constellation mission and discuss recent activities to improve the data latency and generation of near-real-time products for forecasting applications.

How to cite: Blackwell, W.: 18+ Months of Tropical Cyclone and Convective Storm Observations with the NASA TROPICS Pathfinder Satellite, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10494, https://doi.org/10.5194/egusphere-egu23-10494, 2023.

EGU23-10561 | ECS | Orals | AS1.12

High-frequency microwave satellite radiances data assimilation using NICAM-LETKF in the OSSE framework 

Rakesh Teja Konduru, Jianyu Liang, and Takemasa Miyoshi

This study investigates the impact of high frequency, such as 3-hourly and 1-hourly satellite microwave radiances, in global atmospheric data assimilation. To understand the impact of such a high-frequency satellite radiances data assimilation, we designed an observing system simulation experiment (OSSE) using the global NICAM-LETKF system at 56 km horizontal resolution. A free run was conducted with the NICAM model and treated as the reference (Nature) for the OSSE experiments. With the NICAM-LETKF system, we conducted five experiments, without data assimilation (NoDA), with only conventional data assimilation but not satellite radiances (NoSat), 6-hourly (6H), 3-hourly (3H), and 1-hourly (1H) satellite clear-sky radiances assimilation. The results showed that satellite microwave radiances assimilation improved the forecast of air temperature and wind over the global ocean compared to NoSat experiments. With the increase in the assimilation frequency of the satellite radiances, the air temperature and winds showed improvement in their representation over the ocean but degraded over land. Over the ocean, microwave radiances assimilation improved the typhoon eyewall wind intensities and its structure for 1H satellite radiances assimilation compared to 6H. These improvements in the wind intensities are prominent during the landfall stage of the typhoon. Forecasting landfall storms' strong winds are essential for disaster prevention and mitigation.

How to cite: Konduru, R. T., Liang, J., and Miyoshi, T.: High-frequency microwave satellite radiances data assimilation using NICAM-LETKF in the OSSE framework, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10561, https://doi.org/10.5194/egusphere-egu23-10561, 2023.

EGU23-10858 | Orals | AS1.12

Parametrizing the evolution of convective updraft vertical velocities 

Ziad Haddad, Sai Prasanth, Sue van den Heever, Peter Marinescu, Sean Freeman, and Derek Posselt

Moisture convergence, latent heat, upper-level divergence all contribute to the genesis and growth of convective updrafts. In order to characterize the morphology of this evolution, and identify its constituent modes, we analyzed a large data set of synthetic updrafts simulated using a convection-resolving differential-equation solver run at high spatial and temporal resolutions (respectively 100 meters and 10 seconds). The analysis started by fitting each simulated updraft with a 6-parameter analytic representation, so that the joint statistics of the 6 parameters and of their evolution in time can be quantified. The first result is that an effective 6-parameter representation does exist and approximates the vertical profiles with a residual relative error whose r.m.s. value is smaller than 10% for 59% of all cases, and smaller than 20% for 89% of all cases. The r.m.s value of the absolute error is smaller than 0.4 m/s for 97% of all cases. Having established the suitability of this approximation, the variability of the 6 parameters for the 2-minute average Wa of a profile W was quantified, as was the variability of the evolution of W – Wa over a two-minute interval. The analysis reveals that 4 scalars suffice to capture the bulk of the variability of the evolution of convective updrafts. The modes (spanning the range of values of these 4 scalars) turn out to be related to the maximum amplitudes of w and to the heights at which they are achieved. This description paves the way toward the characterization of the environmental determinants of updraft evolution and, in turn, the determination of the effects of updraft characteristics on upper-level air density, divergence and the resulting anvil clouds.

How to cite: Haddad, Z., Prasanth, S., van den Heever, S., Marinescu, P., Freeman, S., and Posselt, D.: Parametrizing the evolution of convective updraft vertical velocities, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10858, https://doi.org/10.5194/egusphere-egu23-10858, 2023.

EGU23-11119 | Posters on site | AS1.12

The development of a detailed mineralogical database from satellite remote sensing products, towards an improved representation of dust transport in NWP simulations. 

Nikolaos S. Bartsotas, Olga Sykioti, Christos Spyrou, Kostas C. Douvis, Vassilis Amiridis, Christos Zerefos, and Stavros Solomos

A broad spectrum of environmental processes such as radiation, cloud formation, ocean fertilization and human health are affected from the presence of mineral dust. The transport of dust particles is dictated by the prevailing meteorological conditions as well as the composition and physiochemical properties of the particles themselves. Which, in turn, are bound to the soil mineralogy at the source region.

Numerical weather prediction models can estimate the transport of dust particles, yet a more refined mineralogical categorization can significantly improve the dust transport estimations and  increase preparedness for implications on weather, biogeochemistry and health. This novel mineralogical representation is derived from multi-spectral satellite remote sensing sensors (Sentinel 2A) over a limited area around Lake Chad in Sahara desert by taking into account dust particle characteristics such as size, composition and optical properties. The mineralogy map will be implemented in WRF/CHEM model to improve the accuracy of atmospheric simulations. The final product will be juxtaposed against current state-of-the-art mineralogical products such as the NASA’s Earth Surface Mineral Dust Source Investigation (EMIT) mission. Dust transport simulations will be compared against field measurements from Antikythera PANGEA station in the Mediterranean and ASKOS campaign in the Atlantic Ocean.

How to cite: Bartsotas, N. S., Sykioti, O., Spyrou, C., Douvis, K. C., Amiridis, V., Zerefos, C., and Solomos, S.: The development of a detailed mineralogical database from satellite remote sensing products, towards an improved representation of dust transport in NWP simulations., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11119, https://doi.org/10.5194/egusphere-egu23-11119, 2023.

EGU23-12321 | ECS | Orals | AS1.12

Predictability of moist convection through ensemble-based convective-scale data assimilation 

Masashi Minamide and Derek Posselt

The development of atmospheric deep moist convection has been a challenging topic for numerical weather prediction, due to its chaotic nature of the development with multi-scale physical interactions. We recently found that greater than 20-km scale (as commonly known as meso-α (2000-200 km) and meso-β (200-20 km) scales) initial features helped to constrain the general location of convective activity with a few hours of lead time, but meso-γ (20-2 km) or even smaller scale features with less than 30-minute lead time were identified to be essential for capturing the spatiotemporal features of individual convection. To examine the potentials of ensemble-based data assimilation in capturing the individual convective development, as well as the subsequent development of severe weather events, we have conducted large ensemble convection-permitting data assimilation experiments with all-sky infrared satellite radiances from the latest-generation geostationary satellites. We found that the greater number of ensembles more effectively suppressed the spurious correlation for convective-scale data assimilation. However, the exact signals of convective development were not clearly captured in covariances even with thousands of ensemble members. These results suggest the potential limitation of the traditional “Eulerian” (i.e. physical grid-based) ensemble approach in convective-scale data assimilation.

How to cite: Minamide, M. and Posselt, D.: Predictability of moist convection through ensemble-based convective-scale data assimilation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12321, https://doi.org/10.5194/egusphere-egu23-12321, 2023.

EGU23-13441 | Posters on site | AS1.12

Impact study of Aeolus/ALADIN bias correction in the KIM data assimilation system 

Hyemin Shin, Jeon-Ho Kang, and In-Hyuk Kwon

The Aeolus Atmospheric Laser Doppler Instrument (ALADIN) sensor onboard Aeolus provides the Horizontal Line Of Sight (HLOS) wind. The satellite-based HLOS wind profile data is significant because it complements the southern hemisphere, tropical and polar regions where existing wind observations are insufficient. The KMA also assimilates the HLOS wind for the operational data assimilation (DA) system since 2021, showing slightly positive impacts on average in the analysis field. However, it was confirmed that the impacts were relatively lower than those of the leading centers and limited due to systematic or random errors in the observation. 
In this study, we tested if we could enhance the positive impacts by applying the bias correction (BC) method to the HLOS wind observation. To this end, the Total Least Squares (TLS) were tested to conduct on the KIM Package for Observation Processing (KPOP) system, which is a system to provide well-qualified observations to the DA system. It shows better statistics in the mean and standard deviation of the first guess departures (O-B) by applying the TLS BC method with -0.19 m/s and 3.30 m/s from -0.44 m/s and 6.22 m/s, relatively. Detailed impacts on the analysis and forecast fields from the cycling experiments will be presented.

How to cite: Shin, H., Kang, J.-H., and Kwon, I.-H.: Impact study of Aeolus/ALADIN bias correction in the KIM data assimilation system, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13441, https://doi.org/10.5194/egusphere-egu23-13441, 2023.

Convection-permitting data assimilation requires observations with high spatial density and high temporal frequency to provide information on appropriate scales for high resolution forecasting. Those observation types (e.g., geostationary satellite data) were found to exhibit strong spatial error correlations. Explicitly introducing correlated error statistics in the assimilation may increase the computational complexity and parallel communication costs of the matrix-vector multiplications with the observation precision matrices (the inverse observation error covariance matrices). Therefore, without suitable approaches we cannot take full advantage of the new observation uncertainty estimates. In this work, we present a new numerical approximation method, called the local SVD-FMM, which is developed based on a particular type of the fast multipole method (FMM) using a singular value decomposition (SVD), and a domain localization approach. The basic idea of the local SVD-FMM is to divide the observation domain into boxes of (approximately) equal size and then separates the calculations of the matrix-vector products according to the domain partition. These calculations can be done in parallel with very low communication overheads. Moreover, the local SVD-FMM is easy to implement and applicable to a wide variety of the precision matrices. We applied the local SVD-FMM in a simple variational data assimilation system and found that the computational cost of the variational minimisation was dramatically reduced while preserving the accuracy of the analysis. This new method has the potential to be used as an efficient technique for practical data assimilation applications where a large volume of observations with mutual error correlations needs to be assimilated in a short period of time.

How to cite: Hu, G. and Dance, S. L.: A Novel Numerical Approximation Method for Computations with Spatially Correlated Observation Error Statistics in Data Assimilation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14476, https://doi.org/10.5194/egusphere-egu23-14476, 2023.

EGU23-17558 | ECS | Posters on site | AS1.12

Toward the Application of Nonlinear Ensemble Data Assimilation Methods to Convective-Scale Parameter Estimation 

Hristo Georgiev Chipilski and Derek Posselt

Recent work has demonstrated that convective-scale model parameters, such as those related to cloud microphysical schemes, are nonlinearly related to dynamic/thermodynamic variables in forecasts and observations. This leads to errors when data assimilation (DA) schemes based on linear-Gaussian assumptions are used to estimate the uncertain model parameters. Nonlinear modifications to the standard ensemble Kalman filter (EnKF) have been shown to perform better for systems governed by convective dynamics, and recent algorithms leveraging advances in AI/ML appear to be especially promising.

 

In this talk, we will present results from previous experiments that demonstrate how and why linear EnKF methods fall short for the challenging task of nonlinear parameter estimation. We will discuss the potential improvements that may result from a new class of ensemble DA algorithms leveraging the powerful framework of latent Gaussian models. In particular, two generalizations of the classical EnKF will be described – one which exploits the special mathematical properties of invertible neural networks (ECTF) and another one based on ideas from measure transport in the context of two-step ensemble filtering (TGA-EnKF). The advantages of these new methods will be illustrated through idealized DA experiments, which will then motivate further discussion on their applicability to convective-scale DA problems.

How to cite: Chipilski, H. G. and Posselt, D.: Toward the Application of Nonlinear Ensemble Data Assimilation Methods to Convective-Scale Parameter Estimation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17558, https://doi.org/10.5194/egusphere-egu23-17558, 2023.

EGU23-10 | ECS | Posters on site | AS1.13

Tropical cyclone Vayu under climate change scenario RCP 8.5 

Pubali Mukherjee and Balaji Ramakrishnan

 

The Northern Indian Ocean has witnessed the genesis of several devastating cyclones over the years due to the typical warm climate. The effect of climate change on these cyclones is an essential topic of research owing to the socio-economic impacts of these cyclones on the coastlines. Climate change is expected to influence the various synoptic parameters of these storms, like translational speed, intensification, frequency, etc. Most of the studies about the impact of climate change on cyclones have been done related to the Atlantic and Pacific Oceans; very few have explored the storms of the Indian Ocean in this context. Considering this context, the present study attempts to understand the track, intensity, and synoptic parameters of Tropical cyclone Vayu-June 2019 under the climate change scenario of RCP 8.5 with the Community Earth Systems Model, CESM data simulated with GPU-based WRF-ARW model. The model is simulated at a 9km single domain with a selected set of physical settings based on the previous studies on the cyclones of the Northern Indian Ocean. The track and intensity of the simulated storm are compared with the present-day hurricane Vayu from the IMD best track estimates.

Interestingly under RCP 8.5, unlike the present-day cyclone Vayu, under RCP 8.5, Vayu would have made landfall along the west coast of India with a sustained wind speed of ~ 15 m/s w. At the same time, he presents a scenario in Vayu weakened over the ocean due to several interactions with the mid-latitude westerlies. The results indicate a considerable change in the future thermodynamics under which Vayu sustained the intensity till landfall. Under RCP 8.5 simulations, the initial posting error is high; other than that, the coming cyclone Vayu seemed to follow a similar track as the present-day storm except for the landfall.

Regarding wind speed intensity, Vayu under RCP 8.5 shows equal wind intensity as that of the present day, with similar underestimation at the mature stage of the storm. The initial results of this study indicate that changes in large-scale thermodynamics in future warming scenarios can influence the modulations in track and intensity of a very severe cyclonic storm like Vayu. Such results highlight the importance of closely monitoring Arabian Sea cyclones to understand the impending disaster mitigations under probable warming scenarios.

 

 

How to cite: Mukherjee, P. and Ramakrishnan, B.: Tropical cyclone Vayu under climate change scenario RCP 8.5, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10, https://doi.org/10.5194/egusphere-egu23-10, 2023.

EGU23-44 | ECS | Posters on site | AS1.13

Influence of MJO on cyclone activity in the north Indian Ocean and Western North Pacific 

Rahul Raghudhas, Jayanarayanan Kuttippurath, Arun Chakraborty, and Akhila Rajeev

We investigate the changes in cyclogenesis and tropical cyclone (TC) activity by the warped life cycle of MJO triggered by the two-fold expansion of the warm pool that occurred during the period of the past 40 years (1979-2019). To study the impact of MJO on TC genesis and activity, we have used the genesis potential index (GPI), accumulated cyclonic energy (ACE) and frequency of cyclones in the active, moderately active and non-active periods of MJO in the North Indian Ocean (NIO) and Western North Pacific (WNP). We find an inverse characteristic of anomalies of relative humidity, vertical wind shear, absolute vorticity, potential intensity, GPI and sea surface temperature over the tropical region between active and non-active years of MJO (1979-2019). High TC activity is experienced during the moderately active years of MJO over the Bay of Bengal (BoB) and WNP. The impact of MJO on TC activity over WNP from October to December (OND) is not particularly dominant during the active years. The genesis of TCs over the Arabian Sea (AS) have also increased during the active years of MJO; indicating that the impact of MJO is increasing over AS. In addition, stalling of eastward propagation of MJO is noticed over the Maritime Continent (MC) during the active and moderately active MJO years. After phase 5, a strong decline in the trend of the phase duration over WNP is noticed, which can be attributed to the reduced TC genesis and activity over WNP during the MJO active years. Reduced MJO activity during OND over WNP, along with lower absolute vorticity and vertical velocity, resulted in lower TC activity and genesis. Our analysis reveals the basin dependency of TC activity and genesis over AS, BoB and WNP due to the stalled propagation of MJO over MC by the extended Indo-Pacific warm pool driven by anthropogenic activities.

How to cite: Raghudhas, R., Kuttippurath, J., Chakraborty, A., and Rajeev, A.: Influence of MJO on cyclone activity in the north Indian Ocean and Western North Pacific, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-44, https://doi.org/10.5194/egusphere-egu23-44, 2023.

EGU23-75 | ECS | Orals | AS1.13

Kelvin Waves and Tropical Cyclogenesis: Connections to Convection and Moisture 

Quinton Lawton and Sharanya Majumdar

In recent years, research has illuminated a distinct relationship between Convectively Coupled Kelvin Waves (CCKWs) and tropical cyclone (TC) formation. In basins that support TCs, there is a pronounced increase in the number of TC genesis events 1-3 days following the passage of a CCKW’s convectively-active phase. It has been hypothesized that this lagged relationship could be the result of the modification of environmental and kinematic factors by the CCKW. However, little work has been done to try to connect these environmental changes to the processes involved in TC genesis. Observational and modeling studies alike have indicated that the development of TCs may be intimately tied to convective-radiative feedbacks and pre-moistening of the atmosphere. How might CCKWs be impacting these processes?

To investigate this, we leverage a 39-year database of African Easterly Waves (AEWs) and associated TC genesis events in the Atlantic Ocean basin from 1981 to 2019. Environmental composites of ERA5 reanalysis and satellite data show an increase in column specific humidity and convective coverage beginning two days prior to TC genesis. This supports previous hypotheses of AEW trough preconditioning. A moist static energy (MSE) variance budget surrounding AEWs is also calculated. This analysis indicates that the dominant source of MSE variance during TC genesis – a proxy for convective aggregation – are longwave-radiative feedbacks, further solidifying the role of convection-related feedbacks in TC development.

Environmental fields around developing AEWs are then composited relative to passing CCKWs. Convectively-active CCKWs temporarily promote an increase in convection, specific humidity, and relative vorticity around AEWs. AEW-CCKW passages are shown to be quite common, with 76% of all developing AEWs passing at least one CCKW in their lifetime. We also compare AEW-CCKW passages that result in TC genesis versus those that do not. The primary discriminator between these two outcomes appears to be convective coverage and diabatic heating at the time of CCKW passage. There is also a pronounced increase in the longwave-radiative feedback term following the CCKW passage for cases that result in TC genesis.

While it is hard to separate the simultaneous effects of a multi-day TC genesis process from that of passing CCKWs, this analysis provides at least circumstantial evidence that CCKW-related modifications to convection and humidity could play an indirect role in preconditioning the AEW and a direct role in strengthening radiative-convective feedbacks. These results also motivate investigation of AEW-CCKW interactions in numerical simulations, which may be more suited to investigate cross-scale interactions and better determine causality.

How to cite: Lawton, Q. and Majumdar, S.: Kelvin Waves and Tropical Cyclogenesis: Connections to Convection and Moisture, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-75, https://doi.org/10.5194/egusphere-egu23-75, 2023.

EGU23-127 | ECS | Posters on site | AS1.13

Dynamic circulations and Windward Flow over Reunion Island 

samira El Gdachi, Pierre Tulet, and Anne Réchou

Numerical Weather Prediction models still have difficulties to predict local-scale phenomena, such as thermal breezes circulation.  They are local driven wind systems that form over coastal zones (sea/land breeze) or mountainous terrain (slope/valley breeze), produced by the buoyancy effects associated with the diurnal cycle of heating and cooling of the lower atmospheric layers (Zardi et Whiteman, 2013). These circulations can drive abrupt changes that generate localized wind gusts, extreme precipitation, air pollution episodes in the lower layers, or sea state perturbations. 

The characteristics of the volcanic and tropical island of Reunion Island  (Indian Ocean, 21°07’S, 55°32’E) offer an exceptional natural field of investigation for these process studies. The meteorological circulations on Reunion Island have been extensively studied by Lesouëf et al. (2010), Durand et al. (2014), Tulet et al. (2017), Foucart et al. (2018), and Réchou et al. (2019). These works show that the island is affected by a regime of southeast trade winds, which is intense in winter (June-August) and moderate to weak in summer (December to February). This weather regime is the cause of intense winds on the southwest and northeast edges of the island and a branch of northwesterly leeward circulation forcing in the northwest of the island (Maïdo area). In this region, thermal circulations are added to this regional circulation. This return loop occurs almost daily in this part of the island in the boundary layer. The oceanic air masses are advected on the slopes of the Maïdo area by the sea and valley breezes. This convection on the mountain slopes causes an almost daily formation of clouds, which are generally weakly developed vertically and generally with low water content. 

An intensive measurement campaign BIOMAÏDO (Bio-physicochemistry of tropical clouds at Maïdo) took place from 11 March to April 7, 2019, at Réunion Island, in order to study the chemical and biological composition of the air mass, the formation processes of secondary organic matter in heterogeneous environments, the dynamics and the evolution of the boundary layer, and the macro and micro-physical properties of clouds.  

In this study, we detail and analyze the dynamics circulations using the observations of the campaign and compare them to a high-resolution (100m horizontal resolution) numerical simulation with the Meso-NH model. Such a model turned during the selected days in which a dynamical connection between the sites was found (Rocco et al., 2022).

The preliminary results have shown that a vertical resolution smaller than a few meters (~1m)  is needed to capture the katabatic flows and the structure of the valley boundary layer, these circulations have an abrupt variation (~1 hour) and the anabatic flow takes nearly 1 h to arrive to the top of the mountain. 

The temporal and spatial structure of this breezes regimes is analyzed with the use of the wet bulb potential temperature (Davies-Jones., 2007), and the turbulence kinetic energy budgets determined by the numerical model;  this study aims to quantify which processes have the most important role during the diurnal breeze evolution. 

How to cite: El Gdachi, S., Tulet, P., and Réchou, A.: Dynamic circulations and Windward Flow over Reunion Island, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-127, https://doi.org/10.5194/egusphere-egu23-127, 2023.

In this study we have conducted a survey of Mixed Rossby-Gravity (MRG) wave events in the upper troposphere and quantified their association with the intrusions of extratropical disturbances for the period 1979-2019. MRG events are identified by projecting the equatorial meridional winds at 200 hPa onto the meridional structure of theoretical MRG waves2390 MRG events are identified and majority (61%) of them occurred during May-October months, and 65% of the total MRG events occurred over the central-east Pacific and Atlantic Ocean domains. Not only the frequency of occurrence but also the amplitude, wavenumber and trapping scale of the MRG events are found to exhibit a clear seasonality. MRG events associated with intrusions of extratropical disturbances are identified as when the potential vorticity on the 350K isentropic surface at 15° latitude exceeded 1 PVU in the vicinity of the MRG events. We find that 37% of the MRG events are intrusion MRG events and a large majority (88%) of such events occurred over the central-east Pacific and Atlantic Ocean domains. It is also noteworthy that nearly 70% of such intrusions occurred in the winter Hemisphere where the westerly wind ducts are well developed. Over the central-east Pacific during Northern Hemispheric (NH) winter, it is observed that the amplitude of intrusion MRG events are larger and have a larger meridional extent compared to non-intrusion MRG events. They also exhibit a similar spatial scale as the extratropical disturbances implying that resonant interactions may be a primary mechanism for the genesis of MRG events. During NH summer, on the other hand, MRG events are primarily triggered by convective processes and the extratropical disturbances may be instrumental in amplifying their amplitude. 

How to cite: Keshri, S. and Ettammal, S.: A survey of Mixed Rossby-Gravity waves and quantification of their association with extratropical disturbances., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-845, https://doi.org/10.5194/egusphere-egu23-845, 2023.

EGU23-873 | ECS | Orals | AS1.13

Role of land in the unusual track of cyclones Gulab and Shaheen 

Ashish Navale and Karthikeyan Lanka

Cyclones lead to heavy precipitation in a very short period causing severe damage to life and socio-economy along its track. Globally, it is projected that there will be an increase in extreme weather events, which will lead to flooding in places like the Indian subcontinent because of irregular monsoon patterns and cyclonic storms. Extremely rare climatic events occasionally display unexpected phenomena, and cyclone Gulab and Shaheen's formation was one such extraordinary occurrence. Cyclone Gulab developed over the Bay of Bengal on 25th September 2021. The cyclone moved westward and made landfall on the east coast of India in the state of Andhra Pradesh on 26th September. Cyclone Shaheen formed in the North East Arabian sea from the remnants of cyclone Gulab. Although these cyclones were not particularly powerful compared to others in this region, it followed a very unusual track. As the cyclone entered the land, it started losing energy but continued to move across the Indian peninsula as a low-pressure system before emerging into the North Eastern Arabian Sea. Favorable atmospheric and oceanic factors for cyclogenesis in this region caused the system to reintensify on 1st October 2021. The system continued to move westward steadily for two days and intensified into a severe cyclonic storm, Shaheen. On 3rd October, cyclone Shaheen made landfall on the Northeastern coast of Oman and made history as the first severe cyclone to strike the Northern coast of Oman for one and a half-century.

After the landfall of cyclone Gulab, the low-pressure system sustained over land and eventually developed into cyclone Shaheen, suggesting that land was a significant source of moisture. Thus, in this study, we quantified the moisture contributed by land in the form of evapotranspiration to the cyclones Gulab and Shaheen. We used an Eulerian water tracking technique incorporated in the state-of-the-art Weather Research and Forecasting (WRF) model to track moisture. The model allows us to specify a source region of moisture originating as evapotranspiration, which can be tracked throughout the atmosphere. This moisture is tracked till it results in precipitation or advects out of the domain. The precipitation associated with this tracked moisture is termed recycled precipitation. ERA5, a fifth-generation ECMWF atmospheric reanalysis data, is used to set up the model's initial and boundary conditions. The microphysical, cumulus, and planetary boundary layer schemes used are WSM6, Kain-Fritsch, and YSU, respectively. Eulerian water tracking being one of the most accurate tracking techniques, will enable us to get accurate contributions of different regions and land use to the cyclonic system. In this study, we mainly focus on the contributions of moisture from the forested areas and understanding the role of antecedent soil moisture in sustaining the low-pressure system across the Indian landmass. Our results showed that Northeast India and Myanmar's dense vegetated regions contributed copious amounts of moisture to the cyclonic systems in the Bay of Bengal.

How to cite: Navale, A. and Lanka, K.: Role of land in the unusual track of cyclones Gulab and Shaheen, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-873, https://doi.org/10.5194/egusphere-egu23-873, 2023.

EGU23-923 | ECS | Orals | AS1.13

Uncovering the Intrinsic Intensity-Size Relationship of Tropical Cyclones 

Jie Sun, Ming Cai, Guosheng Liu, Ruikai Yan, and Da-Lin Zhang

The central theme of this study is to explore if and how the intensity of a tropical cyclone (TC) is related to its size. This subject has puzzled atmospheric scientists since the work of Depperman (1947) but the existence of this relationship still remains elusive. The improved understanding of the intensity-size relationship of TCs will help coastal communities to prepare for the maximum potential damage as both the intensity and size have important impacts on wind damages, storm surges, and flooding. This study considers 33 years (1988–2020) of TC records of maximum surface winds and radii of maximum and gale-force winds over the North Atlantic Basin derived from the Extended Best Track Dataset. Analysis of these TC records reveals a robust positive correlation between loss of earth and relative angular momentum. This finding together with the inspiration from the seminal work of Emanuel and his collaborators leads us to combine absolute angular momentum and its frictional loss as a radially invariant quantity, referred to as “effective absolute angular momentum” (eAAM), for radial profiles of TC surface winds. It is demonstrated that the eAAM model can reproduce the observed complex intensity-size relationship of TCs, which can be further reduced to a quasi-linear one after factoring out the angular momentum loss and the radius of maximum surface winds. The findings of this study would not only advance our understanding of the complex TC intensity-size relation, but also allow for operational assessments of TC severity and potential damage just using its outer wind information.

How to cite: Sun, J., Cai, M., Liu, G., Yan, R., and Zhang, D.-L.: Uncovering the Intrinsic Intensity-Size Relationship of Tropical Cyclones, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-923, https://doi.org/10.5194/egusphere-egu23-923, 2023.

This study examines the role of tropical dynamics in the formation of global tropical cyclone (TC) clusters. Using theoretical analyses and idealized simulations, it is found that global TC clusters can be produced by the internal dynamics of the tropical atmosphere, even in the absence of all landmass surface and zonal sea surface temperature (SST) anomalies. Theoretical analyses of a two-dimensional InterTropical Convergence Zone (ITCZ) model reveal indeed some large-scale stationary waves whose zonal and meridional structures could support the formation of TC clusters at the global scale. Additional idealized simulations using the Weather Research and Forecasting (WRF) model confirm these results for a range of experiments. Specifically, the examination of two common tropical wave types including the equatorial Rossby (ER) wave and the equatorial Kelvin (EK) wave shows that ER waves could develop a stationary structure for a range of zonal wavenumbers $m\in[5-11]$, while EK waves do not. This modeling result is consistent with the ITCZ analytical model and suggests that large-scale ER waves could support stationary "hot spots" for global TC formation without any zonal SST anomalies. The findings in this study offer different insights into the importance of tropical waves in producing global TC clusters beyond the traditional explanation based on zonal SST variability.   

How to cite: Kieu, C. and Vu, T.-A.: On the Roles of Tropical Waves in the Formation of Global Tropical Cyclone Clusters, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1258, https://doi.org/10.5194/egusphere-egu23-1258, 2023.

Rapid intensification/weakening (RI/RW) refers to a significant increase/decrease in tropical cyclone (TC) intensity over a short period of time. A TC can also undergo multiple RI/RW events during its lifetime, and these events pose a significant challenge for forecasting TC activity. In fact, RW is one major source of large intensity forecasting errors as well as RI. These processes can be associated to particular large-scale conditions, both in terms of atmospheric drivers - such as vertical wind shear or dry air intrusion - and oceanic drivers - such as sea surface temperature (SST) gradient.

In this work we aim to verify the ability of the new CMCC-CM3 model (a preliminary version of the General Circulation Model that will take part to the 7th Coupled Model Intercomparison Project - CMIP7 effort) in representing Tropical Cyclone activity with a particular focus on RI and RW. The simulations used in this work have been provided within the EU project BlueAdapt at a 25km horizontal resolution in atmosphere and ocean components, ensuring the representation of realistic TCs both in terms of spatial variability and intensity. Less agreement is found in representing RI/RW timing and duration, but better results are obtained, compared to the previous version of the model CMCC-CM2. The role of the ocean in determining RI and RW is also investigated.

How to cite: Scoccimarro, E. and Peano, D.: Rapid Intensification and Rapid Weakening of Tropical Cyclones, as represented by the CMCC-CM3 Climate Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1541, https://doi.org/10.5194/egusphere-egu23-1541, 2023.

EGU23-1692 | Orals | AS1.13 | Highlight

The slowdown tends to be greater for stronger tropical cyclones 

Yuan Sun, Wei Zhong, Hongrang He, and Yao Yao

Understanding the impact of climate change on tropical cyclones (TCs) has become a hot topic. The slowdown of TC translation speed contributes greatly to the locally accumulated TC damage. While the recent observational evidence shows that TC translation speed has decreased globally by 10% since the mid-twentieth century, the robustness of the trend is questioned by other studies as effects of changes in observational capability can strongly affect the global trend. Moreover, none of the published studies considered dependence of TC slowdown on TC intensity. This is the caveat of these analyses as the effect of TC slowdown is closely related to TC intensity. Here, we investigate the relationship between TC translation speed trend and TC intensity, and reveal possible reasons for the trend. We show that the global slowing trend without weak TC moments (≤ 17 m s-1) is about double of that with weak TC moments in a recent study. This is because the slowing trend is dominated by strong TCs’ trend. Stronger (weaker) TCs tend to be controlled more by upper-level (lower-level) steering flow, and the calculated trend of upper-level steering flow is much larger than that of lower-level steering flow. This may be an important reason for the large difference between the slowing trend without weak TC moments and that with weak TC moments. Furthermore, the changes of TC tracks (including inter-basin trend and latitudinal shift), which are partly attributed to data inhomogeneity, make a much larger contribution to the slowing trend, compared with the weakening of tropical circulation, which is related to anthropogenic warming.

How to cite: Sun, Y., Zhong, W., He, H., and Yao, Y.: The slowdown tends to be greater for stronger tropical cyclones, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1692, https://doi.org/10.5194/egusphere-egu23-1692, 2023.

EGU23-1799 | ECS | Orals | AS1.13

Role of subtropical Rossby waves in governing the track of cyclones in the Bay of Bengal 

Vineet Singh, Roxy Mathew Koll, and Medha Deshpande

The cyclones during November in the Bay of Bengal follow two distinct tracks. Analysis for the period 1982–2019 shows that some cyclones move
west-northwestward and make landfall at the Odisha, Andhra Pradesh or Tamil Nadu coast of India, or the Sri Lanka coast, while others move north-northeastwards and make landfall at the West Bengal, Bangladesh or Myanmar coast. Our analysis shows there is a significant difference in the steering winds governing these two different cyclone tracks. The north-northeastward moving cyclones are associated with an anomalous upper-level cyclonic circulation over India which is part of a subtropical Rossby wave train triggered by an anomalous upper-level convergence over the Mediterranean region. This wave train propagates along the subtropical westerly jet from the east Atlantic/Mediterranean region and reaches the Indian subcontinent in 4 days. It induces an anomalous cyclonic circulation over the Indian landmass and provides south-to-north and west-to-east steering over the Bay of Bengal, causing the cyclones to move in a north-northeastward direction. On the other hand, for west-northwestward moving cyclones, there is no Rossby wave intrusion over the Indian subcontinent, hence the cyclones move in a west-northwestward direction assisted by the beta effect and climatological winds which are from east to west over the south and central Bay of Bengal. This shows that the track of cyclones in the north Indian Ocean can be modulated by atmospheric changes in the extratropics and can act as a precursor for the prediction of the track of cyclones in this region.

How to cite: Singh, V., Mathew Koll, R., and Deshpande, M.: Role of subtropical Rossby waves in governing the track of cyclones in the Bay of Bengal, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1799, https://doi.org/10.5194/egusphere-egu23-1799, 2023.

EGU23-2007 | ECS | Orals | AS1.13

Mid-Level Dry Air Intrusions over the southern Maritime Continent 

Ashar Aslam, Juliane Schwendike, Simon Peatman, Cathryn Birch, Massimo Bollasina, and Paul Barrett

Patterns in extreme precipitation across the Maritime Continent in Southeast Asia are known to be modulated by many processes, from large-scale modes of variability such as the Madden-Julian Oscillation and planetary waves, to finer-scale processes such as the diurnal cycle. Transient mid-level dry air intrusions are an example of a process not extensively studied over the Maritime Continent, which has the potential to influence rainfall patterns.  

Through Lagrangian trajectory and event composite analyses, we use a humidity metric which identifies mid-level dry air intrusions. These intrusions originate from upper-level disturbances along the subtropical jet. Mid-level cyclonic circulation anomalies northwest of Australia from December-February (DJF) intensify westerlies in the southern Maritime Continent, advecting dry air eastward. In contrast, mid-level anticyclonic circulation anomalies northwest of Australia from June-August (JJA) intensify southern Maritime Continent easterlies, advecting dry air westward. The resultant transport direction of associated air parcels is also dependent on the seasonal low-level monsoon circulation, and potentially convective entrainment.  

Dry air intrusions are found to be important in influencing low-level wind circulations and rainfall patterns in the southern Maritime Continent. Dry air suppresses rainfall over seas near to the southern Maritime Continent in both seasons. Further suppression matches intrusions trajectories, such as over southern Maritime Continent islands in DJF, and the Indian Ocean in JJA. In both seasons, there is enhanced rainfall to the east of the intrusion, where there is moist return flow to the extratropics.  

How to cite: Aslam, A., Schwendike, J., Peatman, S., Birch, C., Bollasina, M., and Barrett, P.: Mid-Level Dry Air Intrusions over the southern Maritime Continent, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2007, https://doi.org/10.5194/egusphere-egu23-2007, 2023.

Convectively coupled equatorial Rossby waves (CCERWs) are an intrinsic part of the spectrum of tropical weather systems, and can bring extreme precipitation to tropical locations. They are usually interpreted as modified versions of the theoretical dry equatorial Rossby wave solutions of the shallow water equations. However, the structure and dynamics of CCERWs are rather different to their theoretical cousins. Here, a vorticity budget is presented for both theoretical equatorial Rossby waves and for CCERWs (based on reanalysis data). The different strengths of the vorticity budget terms between the theoretical waves and CCERWs gives insights into CCERW propagation and growth mechanisms, and provides a focus and testbed for future model and forecast improvements.

How to cite: Matthews, A.: Vorticity budget of convectively coupled equatorial Rossby waves: propagation and growth mechanisms, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2020, https://doi.org/10.5194/egusphere-egu23-2020, 2023.

EGU23-2857 | Orals | AS1.13

Organization of Tropical East Pacific Convection Field Project 

Zeljka Stone, David Raymond, and Stipo Sentic

The OTREC (Organization of Tropical East Pacific Convection) field project took place from August 5 to October 3, 2019. The operational center was in Liberia, Costa Rica. During OTREC, we performed 127 research flight hours in the area of the Eastern Pacific and southwest Caribbean. We deployed 648 dropsondes in a grid to evaluate mesoscale thermodynamic and vorticity budges. We also used the Hiaper Cloud Radar to determine the characteristics of cloud populations. Both of these tools were deployed from the NSF/NCAR Gulfstream V aircraft.

The Eastern Pacific has a strong cross-equatorial gradient in sea surface temperature. The southwest Caribbean exhibits uniform ocean temperatures. The two regions together provide a broad range of atmospheric conditions and a great deal of diversity in convective behavior.

The main goal of the project was to study convection in diverse environments to improve global weather and climate models. In this talk I will present an overview of OTREC, the highlights of the field project and the results that OTREC has yielded that include the thermodynamics of the environment and the vertical mass flux profiles. In particular, column relative humidity, low to mid-tropospheric moist convective instability, and convective inhibition are shown to be useful predictors for moisture convergence, and hence rainfall.

How to cite: Stone, Z., Raymond, D., and Sentic, S.: Organization of Tropical East Pacific Convection Field Project, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2857, https://doi.org/10.5194/egusphere-egu23-2857, 2023.

EGU23-3335 | ECS | Orals | AS1.13

Tropical Cyclones in High-Resolution Global Climate Simulations with the IPSL Model 

Stella Bourdin, Sébastien Fromang, Arnaud Caubel, Josefine Ghattas, Yann Meurdesoif, and Thomas Dubos

The availability of a new icosahedral dynamical core (DYNAMICO) for the IPSL model was the opportunity to participate in the HighResMIP protocol. We present the results of four historical 1950-2015 atmosphere-only (forced SST) simulations at horizontal resolutions equal to 200, 100, 50, and 25 km. We compare them with two simulations that use the same configuration but were performed with the previous longitude-latitude dynamical core at 250 and 75km horizontal resolutions.

We use these simulations to perform the first assessment of Tropical Cyclones (TC) in the IPSL model. This evaluation is done across four resolutions, gathering methodologies from recent literature (Roberts et al., 2020 a&b; Moon et al., 2020; Chavas et al., 2017; Camargo et al., 2020; Bourdin et al., 2022).
We first show that the results obtained with DYNAMICO compare favorably with the previous dynamical core of the IPSL model.
Then, we analyze how increasing horizontal resolution from 200km to 50km improves the TC climatology. Our results align with the current expectation that frequency and geographical distribution get closer to the observation but that the intensity is still significantly under-resolved.
In the highest-resolution simulation TC activity in the North Atlantic basin is well represented in terms of geographical distribution and inter-annual variability. However, regional biases remain, especially in the Western North Pacific, where there is a significant deficit in TC number and a shift of activity towards the east of the basin. These regional biases are robust with resolution but are not associated with any obvious climatological bias in the simulations.
Finally, we study composites, TC size, and life cycles to document the physics of the model's TCs. They show that the model simulates realistic TC structures with primary and secondary circulations, an eyewall, and a warm core. TC size diminishes with resolution and less so with intensity.

We conclude that the IPSL model is able to simulate a realistic climatology of Tropical Cyclones at 25 km horizontal resolution, with maximum intensities limited by the current maximum resolution.

How to cite: Bourdin, S., Fromang, S., Caubel, A., Ghattas, J., Meurdesoif, Y., and Dubos, T.: Tropical Cyclones in High-Resolution Global Climate Simulations with the IPSL Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3335, https://doi.org/10.5194/egusphere-egu23-3335, 2023.

Tropical cyclone activity usually negatively affects people’s lives in coastal countries, especially in East-Asia including China. In order to reduce the effect, various approaches are utilized to study tropical cyclones. The Murray and Simmonds Cyclone Tracking algorithm, which has been mainly used in tracking extratropical cyclones, is, for the first time, applied to detect and track tropical cyclones in the West-Pacific based on mean sea level pressure data. Since this algorithm only requires one variable field as input, if it would achieve similar performance as other more complex tracking algorithms, this could be a good algorithm to use for construction of large physically consistent tropical cyclone event sets.

In the presentation, a preliminary evaluation on the performance of the Murray and Simmonds Cyclone Tracking algorithm on tracking tropical cyclones in West-Pacific, using ERA5 and IBTrACS, will be presented. The sensitivity of the performance of the algorithm on different parameter settings will also be discussed. Furthermore, the added value of combining the Murray and Simmonds Cyclone Tracking algorithm and an impact-based storm tracking algorithm, WiTRACK, from the disaster risk reduction and mitigation perspective will also be demonstrated.

How to cite: Zhang, X., Leckebusch, G. C., and Ng, K. S.: Objective Tracking of Tropical Cyclones and their Impact on Relevant Wind Fields in the West-Pacific for Construction of Physically Consistent Event Sets, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3390, https://doi.org/10.5194/egusphere-egu23-3390, 2023.

EGU23-3628 | Orals | AS1.13 | Highlight

Forced trends in the tropical Pacific and global tropical cyclones: An investigation using a statistical-dynamical downscaling model 

Chia-Ying Lee, Suzana Camargo, Adam Sobel, Richard Seager, Boniface Fosu, and Kevin Reed

The response of tropical cyclone activity to anthropogenic radiative forcing remains uncertain, with even the direction of the change uncertain in some respects (e.g., TC frequency), both globally and regionally. One important source of uncertainties is the Pacific zonal SST gradient. At the interannual time scale, this SST gradient, through the El Niño Southern Oscillation, is known to strongly influence global TC activity. Global climate models in CMIP5/6 generations project this SST gradient to weaken and lead to a more El Niño-like mean state in the future. Observations over the past several decades, however, show a strengthening of the SST gradient and thus a more La Niña-like mean state. While the observed strengthening of the SST gradient may be due to natural variability or merely an observational issue, some recent studies have marshalled evidence, backed up with modeling, to argue that the projected weakening is erroneous and a consequence of a common climatological cold tongue bias that has persisted in a few generations of global climate models. If the above argument is correct, at the transient forced response of Pacific SST over the upcoming decades will be towards a La Niña-like mean state, in contrast to the climate models. This means that the projected trends in TC activity from current state-of-the-art global climate models may be incorrect in some basins. In this presentation, we will report an initial investigation of the above problem using synthetic TCs from the Columbia tropical cyclone HAZard model (CHAZ) downscaled from CMIP6 models. Although all show El Niño-like forced responses, we will group the CMIP6 models/members based on the magnitudes of their climatological cold tongue biases, their historical trends of the zonal and meridional SST gradients, and the correlation between their trends and the observed one. For each stratified group, we will then evaluate SST gradient projections and how these projections affect the large-scale atmospheric and oceanic environment conditions that are important to TC activity and thus influence the forced trends in the CHAZ-CMIP6 downscaled TCs.  This work will inform on how much a potential model bias towards the wrong sign of the tropical Pacific zonal SST gradient change matters for projections of global TCs.

How to cite: Lee, C.-Y., Camargo, S., Sobel, A., Seager, R., Fosu, B., and Reed, K.: Forced trends in the tropical Pacific and global tropical cyclones: An investigation using a statistical-dynamical downscaling model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3628, https://doi.org/10.5194/egusphere-egu23-3628, 2023.

EGU23-3655 | ECS | Orals | AS1.13

A new born theory for the genesis and dynamics of Madden–Julian oscillation-like structure 

Masoud Rostami, Bowen Zhao, and Stefan Petri

By means of a new multilayer pseudo-spectral moist-convective thermal rotating shallow-water (mcTRSW) model in a full sphere, we present a possible equatorial adjustment beyond Gill’s mechanism for the genesis and dynamics of the Madden–Julian oscillation (MJO). According to this theory, an eastward-propagating MJO-like structure can be generated in a self-sustained and self-propelled manner due to nonlinear relaxation (adjustment) of a large-scale positive buoyancy anomaly, depressed anomaly, or a combination of these, as soon as this anomaly reaches a critical threshold in the presence of moist convection at the Equator. This MJO-like episode possesses a convectively coupled “hybrid structure” that consists of a “quasi-equatorial modon” with an enhanced vortex pair and a convectively coupled baroclinic Kelvin wave (BKW), with greater phase speed than that of dipolar structure on an intraseasonal time-scale. Interaction of the BKW, after circumnavigating the entire Equator, with a new large-scale buoyancy anomaly may contribute to excitation of a recurrent generation of the next cycle of MJO-like structure. Overall, the generated “hybrid structure” captures a few of the crudest features of the MJO, includingits quadrupolar structure, convective activity, condensation patterns, vorticity field, phase speed, and westerly and easterly inflows in the lower and upper troposphere. Although moisture-fed convection is a necessary condition for the “hybrid structure” to be excited and maintained in the proposed theory in this study, it is fundamentally different from moisture-mode theories, because the barotropic equatorial modon and BKW also exist in “dry” environments, while there are no similar “dry” dynamical basic structures in moisture-mode theories. The proposed theory can therefore be a possible mechanism to explain the genesis and backbone structure of the MJO and to converge some theories that previously seemed divergent (DOI:10.1002/qj.4388). 

How to cite: Rostami, M., Zhao, B., and Petri, S.: A new born theory for the genesis and dynamics of Madden–Julian oscillation-like structure, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3655, https://doi.org/10.5194/egusphere-egu23-3655, 2023.

Tropical Cyclone Debbie (2017) made landfall near Airlie Beach on 28 March 2017 causing 14 fatalities and an estimated US$2.67B economic loss and was ranked as the most dangerous cyclone to hit Australia since TC Tracy in 1974. In addition to the extreme flooding as TC Debbie moved onshore and down the east coast of Australia, it intensified rapidly just offshore from Category 2 to Category 4 in approximately 18 hours and finally made landfall as a Category 4 TC, causing widespread and disastrous damage.

 

A high-resolution WRF simulation (1-km horizontal, and 10-min temporal resolution) is used to analyze the inner-core structure and evolution during the offshore rapid intensification period in the current conditions and potential future change. In current condition, Debbie’s a rapid intensification (RI) stage is characterized by three rounds of eyewall breakdown into mesovortices and re-development events. Each round of breakdown and re-establishment brings high potential vorticity and equivalent potential temperature air back into the eyewall, re-invigorating eyewall convection activity and driving intensification. The potential future changes in the inner-core structure and eyewall evolution will also be discussed using WRF with the Coupled Model Intercomparison Project Phase 6 (CMIP6) perturbed conditions to better assess the possible TC intensity change under different climate change scenarios.

How to cite: Deng, D. and Ritchie, E.: High-resolution simulation of Tropical Cyclone Debbie (2017):The current and future changes in the inner-core structure and evolution during offshore intensification., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3704, https://doi.org/10.5194/egusphere-egu23-3704, 2023.

EGU23-3718 | Orals | AS1.13

Relationship between the Tropical Cyclone Forecast Skill and the Western North Pacific Summer Monsoon in the ECMWF Monthly Ensemble 

Hsiao-Chung Tsai, Tzu-Ting Lo, Meng-Shih Chen, Yun-Jing Chen, Jui-Ling Kuo, and Han-Yu Hsu

In this study, week-1 to week-4 forecasts of tropical cyclones (TCs) in the western North Pacific are evaluated. The CWB TC Tracking System 2.0 (Lo et al. 2021) is used to objectively detect TCs in the 46-day ECMWF ensemble (ENS) forecasts in the 2021 season and also the reforecasts during 2001-2020. Preliminary evaluations of the probabilistic TC activity forecasts in the 20-year reforecasts show promising forecast skills. The reliability diagrams indicate slight over-forecasting bias in the weeks 1-4 forecasts, and the AUCs (Area Under Curves) are ranging from 0.91 (week-1) to 0.80 (week-4). The relationship between the TC activity forecast skill and the western North Pacific summer monsoon (WNPSM) is also investigated. The WNP monsoon index (WNPMI) proposed by Wang et al. (2001) is computed to provide a measure for the summer monsoon, and the TC forecast skills are evaluated under different levels of the WNPMI. To identify the potential false alarms, a spatial-temporal track clustering technique (Tsai et al. 2019) is implemented to objectively group similar vortex tracks in the 51-member forecasts. The corresponding ensemble mean track for each cluster is then used for performing the event-based verifications after the end of season. More details about the TC forecast verifications in weeks 1-4 using the ECMWF monthly ensemble will be presented in the meeting.

How to cite: Tsai, H.-C., Lo, T.-T., Chen, M.-S., Chen, Y.-J., Kuo, J.-L., and Hsu, H.-Y.: Relationship between the Tropical Cyclone Forecast Skill and the Western North Pacific Summer Monsoon in the ECMWF Monthly Ensemble, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3718, https://doi.org/10.5194/egusphere-egu23-3718, 2023.

EGU23-3995 | ECS | Orals | AS1.13

Impact of the MJO on the extreme precipitations in the Mexican Valley 

Liset V. Proveyer and Alejandro Jaramillo

This research aims to determine how the Madden-Julian oscillation (MJO) influences extreme summer precipitation events in the Metropolitan Area of the Mexican Valley (MAMV). Using the Real-time Multivariate MJO Index (RMM), we found a higher frequency of days with extreme events during phases 1 and 2 of the MJO (wet phases), with the lowest occurrence during phases 6, 7, and 8 (dry phases). These frequencies are associated with positive (negative) humidity anomalies in the whole atmospheric column of the study region during the wet (dry) phases. The interaction of a humid flow from the Caribbean Sea with the mountain systems of the region plays a fundamental role in the occurrence of deep convection. Also, the formation of mesoscale convective systems in the central region of the Mexican territory contributes to the moisture content in the Mexican Valley. We used the Dynamic Recycling Model to quantify the relative contributions of different source regions to the atmospheric humidity in MAMV. We found that the greatest contributions to the humidity anomalies are from the Caribbean Sea and Central Mexico during the wet phases of the MJO. During the remaining phases, we observe a weakening of the humid flow from the east as the Caribbean low-level jet intensifies. Additionally, during phases 7 and 8, the mountainous systems that limit the MAMV constitute natural barriers to the flow of humidity that tends to be predominantly from the eastern Pacific. The MAMV is highly vulnerable to extreme precipitation events and their effects, such as pluvial floods and landslides. Therefore, studying the phenomena that modulate these extreme events is essential to improve their predictability and perform better risk management.

How to cite: Proveyer, L. V. and Jaramillo, A.: Impact of the MJO on the extreme precipitations in the Mexican Valley, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3995, https://doi.org/10.5194/egusphere-egu23-3995, 2023.

EGU23-4002 | Posters on site | AS1.13

Effect of the Coastal Large-Scale Environment on the Tropical Diurnal Cycle 

Eric Maloney, Michael Natoli, Emily Riley Dellaripa, Hien Bui, Charlotte DeMott, and Ewan Short

Environmental conditions supporting offshore propagation of diurnal precipitation near tropical coastlines are examined. In particular, the effect of the near-coastal background wind, moisture, and surface wind speed and fluxes on offshore precipitation propagation is assessed for the Philippines, northern Australia, and Panama Bight region near Colombia. Reanalysis fields, satellite precipitation, surface wind speed (from the CYGNSS satellite), and flux observations, and the Cloud Model 1 (CM1) are used in this work. In general, a moist offshore environment and enhanced wind-driven surface fluxes support offshore propagation of strong diurnal convective disturbances. Near the west coast of Luzon, a weak offshore wind in the lower free troposphere also supports offshore propagation, as often occurs in the transition phases of the boreal summer intraseasonal oscillation from suppressed to enhanced daily mean convection. Vertically-integrated moist static energy budget analysis is used to support these results. Sensitivity tests with the CM1 verify the importance of weak offshore flow and a moist offshore environment for supporting offshore propagation of diurnal precipitation.

How to cite: Maloney, E., Natoli, M., Riley Dellaripa, E., Bui, H., DeMott, C., and Short, E.: Effect of the Coastal Large-Scale Environment on the Tropical Diurnal Cycle, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4002, https://doi.org/10.5194/egusphere-egu23-4002, 2023.

EGU23-4126 | ECS | Posters on site | AS1.13

A Dynamical Framework to Understand and Predict the Indian Summer Monsoon Low Pressure Systems 

K. S. S. Sai Srujan, Sukumaran Sandeep, and Hariprasad Kodamana

About 60% of the rainfall during the Indian Summer Monsoon (ISM) is manifested by the synoptic-scale storms form over North Bay of Bengal (BoB) and the adjacent land area known as “Low-Pressure Systems” (LPS). Unlike tropical cyclones, the storms during this season (LPSs) are embedded in the background monsoon flow, which makes them difficult to predict, considering the chaotic nature of the monsoon. Nearly one-third of these synoptic-scale storms are formed due to the amplification of disturbance which is propagating from the Western North Pacific (WNP) (categorized as “downstream LPS”). We observed an association of tropical cyclones (TCs) originating over WNP with the genesis mechanisms of downstream LPS over the BoB. The TCs over the WNP are classified into different clusters based on different features like length, genesis location, landfall, etc., using the gaussian mixture models. We found that four major clusters of WNP TCs are responsible for triggering 83% of the downstream LPS genesis. We established a causality using the transfer entropy analysis between the fluctuations in mean sea-level pressure over BoB and the Rossby wave activity over the WNP prior to the initiation of an LPS.

Our results suggest a plausible prediction of downstream LPS at least a week ahead. The current generation of climate models has low skill in simulating the LPS; understanding the dynamics behind the genesis of LPS is the way to improve the LPS-related precipitation in climate models. The recent advancement in using AI/ML in predicting various weather and climate phenomena, including our recent study in predicting the synoptic-scale sea-level pressure using the ConvLSTM model explains the importance of dynamics-based data-driven ML models to predict complex weather patterns. Understanding the dynamics of such physical phenomena will help in identifying the appropriate predictors for the data-driven ML models.

How to cite: Srujan, K. S. S. S., Sandeep, S., and Kodamana, H.: A Dynamical Framework to Understand and Predict the Indian Summer Monsoon Low Pressure Systems, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4126, https://doi.org/10.5194/egusphere-egu23-4126, 2023.

EGU23-4491 | ECS | Orals | AS1.13

Influence of the MJO on extreme precipitation events over the Eastern Pacific Ocean 

Luis Lazcano and Christian Domínguez

The Madden-Julian Oscillation (MJO) is the main mode of intraseasonal variability over the tropics. We aim to explore the MJO modulation on extreme precipitation events by analyzing atmospheric variables from ERA5 and oceanic variables from the NOAA and HYCOM reanalysis over the Eastern Pacific Ocean from May to November during the 1982-2018 period. The Real-time Multivariate MJO Index (RMM) is used to define the MJO phases. Only strong MJO phases are considered for this study. During MJO phases 3-7, the Eastern Pacific Ocean warm pool goes through a large expansion, but rainfall decreases near the Mexican Pacific coast. On the other hand, MJO phases 8, 1, and 2 induce an increase in precipitation over the continental part of the Middle Americas, making extreme precipitation events more frequent, but these phases decrease the warm pool extension near the Pacific coast. Additionally, the MJO compounds are classified according to El Niño Southern Oscillation (ENSO) years. MJO phases under Neutral and El Niño years have similar patterns in the atmospheric variables. However, these patterns drastically change in MJO phases under La Niña years, as the warm pool expansion decreases and the decrease/increase in rainfall is more intense compared to Neutral and El Niño years. We also noticed that the warm pool expansion and extreme precipitation events do not occur simultaneously. There is a lag of 7 days, as previous studies found but for the Indian Ocean. We conclude that these results are important to understand the air-ocean coupling for MJO and its application for sub-seasonal forecasts.

How to cite: Lazcano, L. and Domínguez, C.: Influence of the MJO on extreme precipitation events over the Eastern Pacific Ocean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4491, https://doi.org/10.5194/egusphere-egu23-4491, 2023.

EGU23-4550 | ECS | Orals | AS1.13

On the critical layer interaction of the stratospheric Kelvin waves 

Ahmed Shaaban and Paul Roundy

Stratospheric Kelvin waves are known to be absorbed by the background flow via mechanical and thermal damping and, to less extent, by the critical layer interaction. Critical layer interaction occurs when the Kelvin waves' phase speed approaches the background flow's speed. This study aims to depict the structure of the Kelvin waves while approaching the critical layer, where the phase speed of the wave matches the speed of the background flow. In the time domain, the wavelet filtering technique filters Kelvin waves at a specific location and phase speeds using ERA-I zonal wind. Linear regression yields the pattern of specific phase speed's Kelvin wave. Yet, the critical layer interaction of the Kelvin waves with the environmental flow could be studied by choosing a background environment in which its flow speed matches the wave's phase speed, which could be implemented using the varying-coefficient regression technique. We found that the in-phase relationship between the zonal wind and height, associated with the structure of the Kelvin waves, relaxes with the decreasing of the Doppler-shifted speed; then, at a further reduction of the Doppler-shifted speed, the Gill pattern appears. Furthermore, Kelvin waves were found to be absent under an environment of westerly shear.

How to cite: Shaaban, A. and Roundy, P.: On the critical layer interaction of the stratospheric Kelvin waves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4550, https://doi.org/10.5194/egusphere-egu23-4550, 2023.

EGU23-4664 | ECS | Posters on site | AS1.13

Record-breaking rainfall accumulations in eastern China produced by Typhoon In-fa (2021) 

Xin Huang, Johnny C. L. Chan, Ruifen Zhan, Zifeng Yu, and Rijin Wan

Persistent heavy rainfall produced by western North Pacific (WNP) tropical cyclones (TCs) can lead to widespread flooding and landslides in Asian countries. On July 2021, unprecedent rainfall amount occurred when Typhoon In-fa passed through the highly populated eastern China. While the associated synoptic features have been analyzed, the extreme characteristics and return periods of rainfall induced by In-fa remain unexplored. Analyses of rainfall data from a WNP TC database of the China Meteorological Administration (CMA) show that Typhoon In-fa not only produces record-breaking rainfall accumulations at individual surface stations, but generates unprecedent rainfall amounts for the whole area of eastern China. Quantitatively, 2, 4, 11, 24 and 55 stations are exposed to once in 200-, 100-, 50-, 20- and 10-year extreme TC rainfall accumulations, respectively, and total rainfall at 75 stations reaches a record high since 1980. Overall, the return period is up to ~481 years for the total rainfall amount accumulated in eastern China during the 1980-2019 baseline. The extremely long rainfall duration is identified as key to the torrential rains in the Yangtze River Delta before In-fa changes its direction of movement from northwestward to northeastward, while the extreme rain rate plays a dominant role in the northern areas afterwards. Probabilities of occurrence of such an unprecedented TC rainfall event have increased in most (~75%) of the eastern China during the period of 2000-2019 compared with those during 1980-1999. Our study highlights the likely increase in risk of extreme TC-induced rainfall accumulations which should be considered in disaster risk mitigation.

How to cite: Huang, X., Chan, J. C. L., Zhan, R., Yu, Z., and Wan, R.: Record-breaking rainfall accumulations in eastern China produced by Typhoon In-fa (2021), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4664, https://doi.org/10.5194/egusphere-egu23-4664, 2023.

EGU23-4688 | Orals | AS1.13

Contribution of tropical cyclone seeds in the poleward shift of the tropical cyclone formation 

Jung-Eun Chu, Axel Timmermann, Pavan Harika Raavi, Sun-Seon Lee, Johnny C. L. Chan, and Hung Ming Cheung

Tropical cyclones (TCs), the generic name for typhoons, are among the most destructive natural hazards. It is important to understand how climate change affects TC frequency, to minimize human and economic losses. Some studies have suggested that the number of TCs will decrease, and their formation will shift poleward. However, there is a major lack of fundamental understanding of the origin and development of the TCs from the initial precursory vortex, called a TC seed. The changes in the number of TC seeds and their survival rate (i.e., the proportion that successfully develops into TCs) will eventually control the future TC frequency. However, key challenges are mainly due to a lack of consensus in TC seed definition and a lack of computing resources for TC modeling.

This study aims to meet the above challenges, through the following three tasks: (1) to identify the representation of TC seeds based on three different definitions from early-stage to matured stage; (2) to investigate the future changes in TC seeds and survival rate and their contribution to the poleward shift in TC genesis location; and (3) to unravel the physical mechanisms responsible for the change in response to climate change. We use a high-resolution fully-coupled Community Earth System Model (CESM) with an atmospheric resolution of 0.25° and an ocean resolution of 0.1° with present-day, doubling, and quadrupling CO2 concentrations. Our results show TC seeds defined by early-stage definition show more equatorward distribution with a strong connection to vertical velocity than those defined by matured stage. Interestingly, all three definitions exhibit a statistically significant reduction in the frequency of TC seeds while that in survival rate is not significant. Details of the methods and mechanisms will be further discussed during the presentation. The outcomes of this project will strengthen fundamental scientific knowledge of the TC seeds and their future change mechanisms, as well as provide a scientific basis for future risk assessment and precautionary strategies.

How to cite: Chu, J.-E., Timmermann, A., Raavi, P. H., Lee, S.-S., Chan, J. C. L., and Cheung, H. M.: Contribution of tropical cyclone seeds in the poleward shift of the tropical cyclone formation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4688, https://doi.org/10.5194/egusphere-egu23-4688, 2023.

EGU23-4734 | Posters on site | AS1.13

Investigation of TC track uncertainty using multiple ensembles for the official TC forecast 

Jinyeon Kim, Dongjin Kim, Daejoon Kim, Joohyung Son, and Dong-Ju Ham

The official tropical cyclone information in Korea includes a deterministic forecast position of TC center and its uncertainty with the 70% probability circle, which is statistically determined by previous 3 year’s operational track errors. Therefore, the current probability circle does not represent situational uncertainty. In this study, it is investigated for using an ensemble prediction system (EPS) to represent the TC position uncertainty with three different methods: circle (CIR), ellipse with an along-track and a cross-track axes (EAC), ellipse with eigenvector axes (EEV). Five single EPSs, ECMWF, NCEP, UKMO-UM, JMA and KMA-UM, and two multiple ensembles, a simple one (SME) and a calibrated one (CME) which coincides the ensemble means, were evaluated. The methods and the ensembles were verified for 5 days with the hit rate which is defined as the percentage of the observed TC central positions within circles or ellipses.
In order to verify the new probability areas as well as the operation, the hit rate which is defined as the percentage of the observed TC central positions within 70% probability circle or ellipses were used. The operational radii have over 70% hit rate, around 0.8 for all forecast times. It means that the official forecast skill is getting better year by year and the current circle is overestimated. EPS based circle or ellipse showed better performance apart from the EAC. In more detail, the CME for both circle and ellipse method outperformed the operational method until 48 forecast hours. Since the five single EPSs were under-spread at this time, the multiple ensembles could overcome this shortage. After 72 forecast hours, SME and CME are too overspread, so that a single EPS is more likely to be consistent with the 70% probability area.
Although it is definitely sure that the EPS based one is better, there are still limitations to use them. It is difficult to say which method is the best because performance of methods is different according to the forecast time and to get other organizations’ EPS data in real time. Nevertheless, utilizing ensemble for TC track is valuable information since EPS can provide the best method for estimating uncertainty. 

How to cite: Kim, J., Kim, D., Kim, D., Son, J., and Ham, D.-J.: Investigation of TC track uncertainty using multiple ensembles for the official TC forecast, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4734, https://doi.org/10.5194/egusphere-egu23-4734, 2023.

EGU23-4792 | Posters on site | AS1.13

Characteristics of rapidly intensifying tropical cyclones in the South China Sea, 1980-2016 

Lei Yang, Xi luo, Fenghua Zhou, Dongxiao Wang, and Weiqiang Wang

The differences in the characteristics of the rapid intensification (RI) during the TCs that form in the SCS (referred as local TCs) and that
enter the SCS from the western North Pacific (WNP; referred as entering TCs) have not been well studied, which could contribute the inaccuracy
of current TC intensity forecast in the SCS. In this study, we used TC observations, reanalysis data and model experiments to analyze the RI
occurrences during local TCs and entering TCs in 1980e2016. We found that the significant interannual and interdecadal variations in RI
occurrences during local eastward-moving TCs were related to the strong intraseasonal oscillation (ISO) over the SCS and the WNP under La
Nina conditions. RI during local westward-moving TCs showed insignificant variations as a result of the complex interactions among the
monsoon trough, ISO and the large-scale circulation. RI during entering TCs showed strong interdecadal variations, with increased RI after
1997, even though the total number of entering TCs has decreased since 1997, which is a result of a higher number of entering TCs in the
northwestern quadrant of the WNP, a stronger ISO and weak vertical windshear over the SCS and east of the Philippines under negative phase of
Pacific Decadal Oscillation. The different variations and related mechanisms of RI indicates that distinct forecasting factors should be considered
for intensity prediction during local eastward- and westward-moving TCs and entering TCs.

How to cite: Yang, L., luo, X., Zhou, F., Wang, D., and Wang, W.: Characteristics of rapidly intensifying tropical cyclones in the South China Sea, 1980-2016, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4792, https://doi.org/10.5194/egusphere-egu23-4792, 2023.

EGU23-5056 | ECS | Orals | AS1.13

Relationships of the Diurnal Pulse to Structure and Intensity of Tropical Cyclones 

Xinyan Zhang and Weixin Xu

The radially-outward propagating, cloud-top cooling, diurnal pulse (DP) is a prominent feature in tropical cyclones (TCs) that has important implications for changes in TC structure and intensity. By using an objective diurnal-pulse identification algorithm, this study characterizes DPs both globally and regionally over various ocean basins and examines their relationships to TC structure and intensity. Active DPs (ACTDPs) occur on 52% of TC days globally. They are the most frequent over the Northwest Pacific (NWP, 60.4%). The median duration and propagation distance of ACTDPs are 12–15 h and 500–600 km, respectively. Some ACTDPs (20–25%) last longer than 18 h and propagate as far as 700–800 km. Although the mean propagation speed of ACTDPs is 11–13 m s-1, persistent ACTDPs (lasting >15 h) mostly propagate at speeds similar to internal inertial gravity waves (5–10 m s-1). Most ACTDPs initiate in the inner core overnight, in phase with inner-core deep convection. Nearly half of the ACTDPs are coupled with the outward propagation of precipitation within TCs. The TC inner-core deep convection is significantly enhanced on ACTDP days. Specifically, the 20 dBZ echo top in the upshear quadrant of TCs rises the most evidently with the occurrence of the ACTDP, leading to a more symmetric structure of the inner-core convection. The occurrence ACTDPs may promote the rapid intensification (RI) of TCs. The frequency and duration of ACTDPs are strongly correlated with the TC intensification rate. RI TCs have a markedly higher frequency of the very long-duration ACTDPs (≥15h) and longer mean pulse duration than steady-state and gradually intensifying TCs. Overall, the DP is a potentially useful signal for the RI of TCs.

How to cite: Zhang, X. and Xu, W.: Relationships of the Diurnal Pulse to Structure and Intensity of Tropical Cyclones, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5056, https://doi.org/10.5194/egusphere-egu23-5056, 2023.

Mixed Rossby-Gravity (MRG) Waves are westward propagating synoptic scale equatorial disturbances which play a crucial role in the formation of tropical cyclones and tropical depressions, and they constitute a significant part of various modes of tropical variability such as the Madden-Julian Oscillation (MJO) and Quasi-Biennial Oscillation (QBO). In this study, we have investigated the trends and Inter Annual Variability (IAV) in the occurrence of upper tropospheric MRG events using ERA-I reanalysis data for the period 1979-2018. The MRG events are identified by projecting the upper tropospheric meridional winds onto the theoretical spatial structure of MRG waves. A steady increasing trend is observed in the occurrence of MRG events which is contributed by the MRG events associated with the intrusion of extratropical disturbances. The possible factors that govern the observed trends and IAV in the occurrences of MRG events are El Nino Southern Oscillation (ENSO), MJO and extratropical forcing. The MRG events over the central and Eastern Pacific contribute maximum to the IAV. ENSO explains about 25% of the IAV. It exhibits a positive correlation with non-intrusion MRG events and a negative correlation with intrusion MRG events. These observations have been investigated by exploring the strength and the extent of the westerly duct at 200 hPa and the Outgoing Longwave Radiation (OLR) during El Nino and La Nina years over the central-Eastern Pacific ocean. The convectively active state of the MJO over the Western Pacific explains 20% of the IAV over the central-Eastern Pacific. Besides ENSO, MJO exhibits a diametrically opposite correlation with intrusion and non-intrusion MRG events. The antisymmetric heating with respect to the equator, associated with the MJO, enhances non-intrusion MRG events. The subtropical easterlies forbid the intrusion of extratropical disturbances, thereby lowering the occurrences of intrusion MRG events. The increasing trend in the intrusion of extratropical disturbances explains the observed trend in the upper tropospheric MRG events. Such an increasing trend is not observed in the strength or extent of the upper tropospheric westerly duct over the central-Eastern Pacific.

How to cite: Na, M., Keshri, S., and Ettammal, S.: Major Factors Governing the Trends and Interannual Variability in the Occurrences of Mixed Rossby-Gravity Wave Events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5340, https://doi.org/10.5194/egusphere-egu23-5340, 2023.

This study investigated rapid intensification (RI, +30 kt in 24 h) and rapid weakening (RW, -20 kt in 24 h) for Typhoon Trami (2018) using the Weather Research and Forecasting V4.2 with the three-dimensional Price-Weller- Pinkel ocean model. As with the previous Typhoon Lan (2017) case study, the three-dimensional relative humidity field reproduced from Tropical Cyclones-Pacific Asian Research Campaign for the Improvement of Intensity Estimations/Forecasts dropsonde data and Himawari-8 satellite imagery was assimilated during every tropical cyclone dynamical initialization process. Specifically, dropsonde data obtained from two aircraft campaigns for Lan and Trami is used. Numerical results showed that compared to without this special data assimilation, Trami’s RI and RW simulations were better improved with this special data assimilation with respect to track and intensity forecasts. Around the RI period, vertical wind shear noticeably decreased and convective bursts (vertical velocity ≥ 3 m s-1 with 30 dBZ at 2 km height) significantly increased during the RI period. With these favorable ambient and storm inner-core environments, Trami quickly formed an eye structure. After RI and slow intensification periods, Trami eventually reached the Category 5 Saffir-Simpson hurricane scale. This maximum intensity was almost maintained until it had turned northwards. After that, as its translation speed significantly decreased, RW occurred with substantial upwelling. This upwelling caused a stable boundary layer and made significant asymmetry of surface heat fluxes and convective clouds. During this significant sea surface cooling period, deep convective cells were significantly suppressed in the eyewall area. As a result, Trami underwent RW during this period. To sum up, Trami’s RI may be associated with the reduction of negative dynamic forcing around the RI period, whereas Trami’s RW may be related to negative thermodynamic forcing by ocean cooling with a very slow translation speed during the RW period. More numerical results and detailed analyses of Trami’s RI and RW will be shown in the 2023 EGU General Assembly.

 

Keywords: dropsonde data assimilation, tropical cyclone dynamical initialization, rapid intensification, rapid weakening, WRF atmosphere and ocean coupled model

 

Acknowledgment

This work was funded by the Korea Meteorological Administration Research and Development Program under Grant KMI2022-00410.

 

How to cite: Lee, J., Chang, E.-C., Ito, K., and Wu, C.-C.: Effects of the Assimilation of Relative Humidity Reproduced From T-PARCII and Himawari-8 Satellite Imagery Using Dynamical Initialization and Ocean Coupled Model: A Case Study of Typhoon Trami (2018), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5434, https://doi.org/10.5194/egusphere-egu23-5434, 2023.

EGU23-5825 | ECS | Orals | AS1.13

GPM-DPR observed microphysical characteristics of the Arabian Sea tropical cyclone 

Amit Kumar, Atul Kumar Srivastava, and Manoj Kumar Srivastava

The precipitation characteristics of tropical cyclones (TCs) formed between 2014-2021 over the Arabian Sea during the onset phase of monsoon and after the monsoon (post-monsoon) seasons have been investigated through the space-borne dual-frequency precipitation radar of the Global Precipitation Measurement (GPM-DPR) satellite level 2, V07 observation. In a cloud that is producing precipitation, the two-dimensional frequency distribution of the liquid water content (LWC; g/m2) and non-liquid water content (IWC; g/m2) exhibits a clear seasonal and cloud-type dependence. For the precipitating cloud of stratiform origin of TCs in the monsoon and post-monsoon seasons, a significant part of rain droplets is present in the LWC limit of 0-800 g/m2 and the IWC limit of 0-350 g/m2. In contrast to the stratiform precipitation associated with the TCs, the LWC quantity is additionally more, and IWC is less for the convective origin precipitating cloud. In the monsoon and post-monsoon season, the mean values of the mass-weighted mean diameter, Dm (mm), are 1.29 (1.47) mm and 1.27 (1.31) mm, respectively, for the stratiform (convective) cyclonic cloud. It is noticed that when the value of Dm increases, the normalised intercept parameters (Nw) decrease, regardless of the season and cloud type related to the TCs. While stratiform precipitation contains a considerably high concentration of smaller-sized rain droplets during both seasons, the number concentration of bigger rain droplets is significantly high during convective precipitation. From the contoured frequency with altitude diagram (CFAD) plots for Dm and Ze for the cyclonic cloud in both seasons, we observe a large concentration of ice and supercooled liquid particles available above the melting layer and a significant concentration of rain droplets in liquid state present below the melting layer. We derived the contribution of the different microphysical processes (break-up, size-sorting, collision-coalescence, and evaporation processes) in the rain droplets formation below the melting layer. It is found that the process of collision-coalescence is predominating microphysical process for convective precipitation. The break-up process is a primary microphysical process in the precipitating cloud of stratiform origin.

 

How to cite: Kumar, A., Srivastava, A. K., and Srivastava, M. K.: GPM-DPR observed microphysical characteristics of the Arabian Sea tropical cyclone, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5825, https://doi.org/10.5194/egusphere-egu23-5825, 2023.

EGU23-6086 | Orals | AS1.13

Influence of Potential Vorticity Structure on North Atlantic Tropical Cyclone Activity 

Ulrike Lohmann, Bernhard Enz, David Neubauer, and Michael Sprenger

Tropical cyclones are among the most devastating natural phenomena that can cause severe damage when hitting land. Some of this damage could be prevented with more reliable short-term and seasonal forecasts. In the wake of the poorly forecast 2013 North Atlantic hurricane season, Rossby wave breaking has been linked to tropical cyclone activity measured by the accumulated cyclone energy. Here, ERA5 reanalysis data and HURDAT2 tropical cyclone data are used to show that the latitude of the 2 potential vorticity unit (PVU) contour on the 360 K isentropic surface in the western North Atlantic is linked to changes in vertical wind shear and relative humidity during the month of September.

A more equatorward position of the 2 PVU contour is linked to an increase in vertical wind shear and a reduction in relative humidity, as manifested in an increased ventilation index, in the tropical western North Atlantic during September. The more equatorward position of the 2 PVU contour is further linked to a reduction in the number of named storms, hurricane days, hurricane lifetime, and number of tropical cyclones making landfall due to changes in genesis location. In summary, the 2 PVU contour latitude in the western North Atlantic can therefore potentially be used as a predictor in seasonal and sub-seasonal forecasting.

How to cite: Lohmann, U., Enz, B., Neubauer, D., and Sprenger, M.: Influence of Potential Vorticity Structure on North Atlantic Tropical Cyclone Activity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6086, https://doi.org/10.5194/egusphere-egu23-6086, 2023.

EGU23-6157 | ECS | Posters on site | AS1.13

Intensification mechanisms of tropical cyclones 

Andrea Polesello, Caroline J. Muller, Claudia Pasquero, and Agostino N. Meroni

Wind Induced Surface Heat Exchange (WISHE) mechanism is considered very important for tropical cyclone intensification in a large part of the scientific literature([1], [2], [3] ): heat flux from the ocean increase with increasing wind speed, building up a positive feedback on the intensification.
Simple WISHE-based models of tropical intensification predict that tropical cyclones intensify up to a steady state at the Potential Intensity (PI), obtained from the balance of heat supply rate from the ocean and dissipation rate in the boundary layer and dependent on boundary conditions only ([1]). The main problem of such models is the fact that they typically drastically simplify the convective motion within the cyclone, assuming a troposphere neutral to moist convection. ([4]).
In our work we tested these predictions in idealized numerical experiments performed using the non-hydrostatic, high-resolution model System for Atmospheric Modelling (SAM). The results showed a significantly different intensity evolution, with the cyclone undergoing a oscillation in surface wind speed with peak intensity significantly lower than the PI.
This intensity evolution was related to that of the environmental conditions along the whole air column: convective heating exports latent and sensible heat in the middle-upper troposphere, increasing environmental air buoyancy and so reducing CAPE. Radiative heating from the clouds further stabilizes the upper troposphere, weakening convection and thus cyclone intensity. After the intensity decay phase the upper level air surrounding the cyclone cools down through radiation emission: entrainment of cold air by the cyclone itself rebuilts CAPE and triggers a new intensification. Despite this work showed some limits in the predictivity of WISHE theory, WISHE feedback itself was proved to be fundamental for tropical cyclone intensification with a sensitivity numerical experiment.

 

[1]  K. Emanuel et al., “Tropical cyclones,” Annual review of earth and planetary sciences, vol. 31,
no. 1, pp. 75–104, 2003

[2]  K. A. Emanuel, “An Air-Sea Interaction Theory for Tropical Cyclones. Part I: Steady-State
Maintenance.,” Journal of Atmospheric Sciences, vol. 43, pp. 585–605, Mar. 1986.

[3]  C. J. Muller and D. M. Romps, “Acceleration of tropical cyclogenesis by self-aggregation
feedbacks,” Proceedings of the National Academy of Sciences, vol. 115, no. 12, pp. 2930–
2935, 2018.

[4]  K. A. Emanuel, “The behavior of a simple hurricane model using a convective scheme based
on subcloud-layer entropy equilibrium,” Journal of Atmospheric Sciences, vol. 52, no. 22,
pp. 3960 – 3968, 1995.

How to cite: Polesello, A., Muller, C. J., Pasquero, C., and Meroni, A. N.: Intensification mechanisms of tropical cyclones, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6157, https://doi.org/10.5194/egusphere-egu23-6157, 2023.

EGU23-6549 | ECS | Orals | AS1.13

Extreme precipitation in South Sulawesi triggered by equatorial waves and its representation in MetUM forecasts 

Natasha Senior, Adrian Matthews, Ben Webber, Beata Latos, and Dariusz Baranowski

The Indonesian island of Sulawesi lies at the heart of the Maritime Continent, a region prone to extreme rainfall. On seasonal timescales, rainfall frequency and intensity increases during the monsoon season (Nov-March). On subseasonal scales, rainfall is modulated by the Madden-Julian Oscillation (MJO) which increases moisture and moisture convergence in its active phase. Higher frequency modes include convectively coupled equatorial waves which influence rainfall variability on daily timescales. On 22nd January 2019, these large-scale meteorological drivers coincided resulting in the South Sulawesi region experiencing its largest flood on record. Specifically, the extreme rainfall event was linked to a convectively coupled Kelvin wave (CCKW) and a convectively coupled equatorial Rossby wave (CCERW) embedded within an active MJO envelope, as well as a cross equatorial cold surge (Latos et al, 2021). Interactions between these modes resulted in increased moisture transport and convergence that lead to the development of a mesoscale convective system (MCS) over Java and the Java Sea on 21st January 2019. This MCS traversed towards Sulawesi bringing extreme rainfall to the region in the evening and overnight on the 22nd reaching its peak mid-afternoon. Cases like this present a unique challenge for forecasters, to not only to accurately represent the individual equatorial modes but their interactions. In the present work we study the MCS in reanalysis and satellite data and discuss how the various equatorial modes contributed to its development. Then we examine its representation in different convection permitting Met Office Unified Model (MetUM) configurations. We find that the MetUM performed well in capturing the trajectories of the equatorial modes, however the representation of the MCS itself varies between ensemble members and model configurations. We further examine how well the RAL1T+ configuration represents the equatorial modes through comparing filtered fields of daily model data at fixed lead times to those in observations.

How to cite: Senior, N., Matthews, A., Webber, B., Latos, B., and Baranowski, D.: Extreme precipitation in South Sulawesi triggered by equatorial waves and its representation in MetUM forecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6549, https://doi.org/10.5194/egusphere-egu23-6549, 2023.

As tropical cyclones (TCs) undergo extratropical transition (ET), they develop distinct frontal boundaries across the resulting extratropical cyclone. In the North Atlantic Ocean (NATL), this can often happen near the Gulf Stream (GS). Previous work has demonstrated that the GS can influence the development of fronts in midlatitude winter cyclones. The mechanisms of air-sea interactions associated with WBCs occur at multiple spatiotemporal scales, with the extent and exact nature of those interactions debated within the literature. Could the influence of the GS on frontal development in midlatitude winter storms also apply to storms undergoing ET? Here, we present both an observational-based statistical analysis, as well as results from case-study simulations, of a possible pathway for the GS to influence TCs undergoing ET via local small-scale SST gradient changes.

Composites of NATL TCs indicate that the magnitude of the GS sea surface temperature (SST) gradient in the time prior to the TC passing is significantly weaker for TCs that begin the ET process but ultimately do not complete it, compared with TCs that do complete ET. Using a simple index of the GS SST gradient strength, both the sensible heat flux gradient and, to a lesser degree, lower-tropospheric diabatic frontogenesis are shown to scale with the local SST gradient used in this index. Our results suggest that there is some support for a mechanism in which the GS SST gradient influences the sensible heat flux gradient and subsequent surface diabatic frontogenesis in the region, impacting the favorability of the environment for a passing TC to complete ET.

To investigate this possible mechanism more closely and establish causality, we use the Weather Research and Forecasting (WRF) model to test case study simulations of Hurricane Teddy as it undergoes ET near the GS. We analyze this by modifying the magnitude and strength of the local grid point-scale SST gradient strength associated with the GS in the North Atlantic in the days prior to Teddy passing over the GS. These different simulations are then compared to determine impacts in terms of the track, intensity, frontal development, strength of both the adiabatic and diabatic frontogenesis, during Teddy’s ET. These results provide insight into the dynamical mechanisms by which surface forcing could exert an influence on ET.

How to cite: Jones, E., Wing, A., and Parfitt, R.: Investigating A Potential Pathway for Gulf Stream Influence on the Extratropical Transition of North Atlantic Tropical Cyclones, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6628, https://doi.org/10.5194/egusphere-egu23-6628, 2023.

EGU23-6722 | Orals | AS1.13 | Highlight

Impact of Deforestation in the Maritime Continent on the Madden–Julian Oscillation 

Chuing-Wen June Chang, Min-Hui Lo, Wan-Ling Tseng, Yu-Cian Tsai, and Jia-Yuh Yu

Deforestation is a major issue affecting both regional and global hydroclimates. This study investigated the effect of deforestation in the Maritime Continent (MC) on tropical intraseasonal climate variability. Using a global climate model with Madden–Julian Oscillation (MJO) simulations, we examined the effect of deforestation over the MC region by replacing the forest canopy with grassland. The results revealed that under constant orographic and land–sea contrast forcing, the modification of the canopy over the MC altered the characteristics of the MJO. We noted the amplification of the MJO and increases in wet–dry fluctuation and the zonal extent. We analyzed more than 100 MJO cases by performing K-means clustering and determined that the continuous propagation of the MJO over the MC increased in 35% and 61% of the total 110 cases in the control and deforestation experiments, respectively. This phenomenon was associated with more substantial vanguard precipitation, increased soil moisture, and a suppressed diurnal cycle in land convection. Furthermore, when the MJO convection was over the Indian Ocean (IO), we observed the enhancement of low-level moisture over the MC region in the deforestation experiment. Grassland surface forcing provides a thermodynamic source for triggering instability in the atmosphere, resulting in low-level moisture convergence. The MJO exhibited a stronger energy recharge–discharge cycle in the deforestation experiment than in the control experiment, and this difference between the experiments enlarged from the IO to MC.

 

How to cite: Chang, C.-W. J., Lo, M.-H., Tseng, W.-L., Tsai, Y.-C., and Yu, J.-Y.: Impact of Deforestation in the Maritime Continent on the Madden–Julian Oscillation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6722, https://doi.org/10.5194/egusphere-egu23-6722, 2023.

The variation of the thermodynamic cycle and energy of tropical cyclones (TCs) under vertical wind shear (VWS) is analyzed, and its associated TC thermal and dynamical structure evolutions are explored. The thermodynamic cycles extracted using the Mean Airflow as Lagrangian Dynamics Approximation (MAFALDA) method show that the maximum energy obtained by the TC decreases with the reduction of storm intensity in VWS. The thermodynamic cycles of sheared TC experience a two-stage evolution. During the early stage, the ascending branch of the MAFALDA cycle shifts toward lower entropy, which is attributed to the reduction of the entropy in the eyewall and the increase of the upward motion and entropy outside the eyewall. In the latter stage, the entropy increases, and the downward motion weakens in the ambient and upper troposphere, allowing the descending legs shifts toward high values of entropy. A backward Lagrangian diagnostic of air parcels associated with variations in thermodynamic cycles is employed to analyze the relative importance of distinct pathways. In addition to the low-, mid-, and upper-level ventilation pathways, the enhanced inner and outer rainbands, outward advection of high entropy air in mid- and upper-troposphere eyewall, the outflow layer with reduced height, and the inflow below the outflow layer are also important for the reduction of the energy gained by TC.

How to cite: Liu, Z.-Q. and Tan, Z.-M.: How Vertical Wind Shear Impacts Tropical Cyclone by Different Thermodynamic Pathways: Energetics and Lagrangian Analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6747, https://doi.org/10.5194/egusphere-egu23-6747, 2023.

EGU23-6758 | ECS | Posters on site | AS1.13

The Decadal Variation of Eastward-Moving Tropical Cyclones in the South China Sea During 1980–2020 

Xi luo, Lei Yang, Sheng Chen, Dong Liang, Johnny C. L. Chan, and Dongxiao Wang

The track of tropical cyclones (TCs) formed in the South China Sea (SCS) can be divided into eastward and westward directions. Significant decadal variation during 1980–2020 only exists in the number of eastward-moving TCs, especially during July–September, with 47% TCs moving eastward during 1994–2004 (Period II), 22% during 1980–1993 (Period I) and only 15% during 2005–2020 (Period III). This decadal change is related to the zonal shift of Western Pacific Subtropical High (WPSH). An eastward-retreated WPSH during 1994–2004 leads to upward motion and westerly flow anomaly over the northern SCS, and therefore favors TC genesis and eastward motion. The eastward-retreated WPSH is associated with a warm sea surface temperature anomaly over the tropical western-central Pacific which induces a cyclonic flow and weakens the WPSH. With the weaker modulation of WPSH, stronger intraseasonal oscillation (ISO) in the SCS during Period II favors eastward-moving TCs due to the westerly flow associated with the ISO.

How to cite: luo, X., Yang, L., Chen, S., Liang, D., Chan, J. C. L., and Wang, D.: The Decadal Variation of Eastward-Moving Tropical Cyclones in the South China Sea During 1980–2020, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6758, https://doi.org/10.5194/egusphere-egu23-6758, 2023.

EGU23-7841 | ECS | Posters on site | AS1.13

The diurnal cycle of precipitation over the Maritime Continent: characterisation in observations and models 

Jack Mustafa, Adrian Matthews, Rob Hall, Karen Heywood, and Marina Azaneu

The meteorological diurnal cycle over the Maritime Continent is a major component of observed variability and features see-sawing of intense precipitation from over land through the afternoon and evening to over surrounding seas and oceans through the night into the morning. This high-frequency land-locked mode of variability interacts with lower-frequency propagating modes of tropical variability, such as the Madden-Julian Oscillation, therefore accurate forecasting of downstream impacts of these intraseasonal modes of variability depends on accurate understanding and model representation of the diurnal cycle.

In this presentation we compare the observed diurnal cycle of precipitation with the diurnal cycle generated by regional hindcast runs of the UK Met Office Unified Model with parameterised and with explicitly-resolved convection. A novel characterisation framework is used to quantify the cycle at each location in order to optimise the intuitive simplicity and the completeness of the characterisation.

How to cite: Mustafa, J., Matthews, A., Hall, R., Heywood, K., and Azaneu, M.: The diurnal cycle of precipitation over the Maritime Continent: characterisation in observations and models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7841, https://doi.org/10.5194/egusphere-egu23-7841, 2023.

EGU23-7870 | Orals | AS1.13 | Highlight

Ocean-Atmosphere Observations from Uncrewed Saildrones and Gliders during the 2022 Atlantic Hurricane Season 

Gregory Foltz and the 2022 NOAA Saildrone Hurricane Observations Team

During the 2022 Atlantic hurricane season, uncrewed systems were used in an innovative and coordinated effort to measure the upper ocean and air-sea interface inside and outside of tropical cyclones. The main objectives were to advance understanding of air-sea interactions in and around tropical cyclones and aid forecaster situational awareness, with the ultimate goal of improving tropical cyclone intensity forecasts. The uncrewed systems included seven saildrones and five underwater gliders that operated in the western Atlantic Ocean, Caribbean Sea, and Gulf of Mexico. Nearly collocated and simultaneous measurements were acquired by an underwater glider and saildrone through the eye of Hurricane Fiona south of Puerto Rico in September. Another saildrone was directed through Fiona after it had intensified to a Category 4 Hurricane in the North Atlantic, measuring sustained winds of 35 m/s and significant wave height of 15 m. Two other saildrones obtained measurements in Fiona when it was a tropical storm east of the Caribbean and as a Category 1 hurricane north of Puerto Rico. Later in September, after Hurricane Ian made landfall in southwestern Florida and then re-intensified to a hurricane east of Florida, a saildrone was directed through its center, measuring winds of 29 m/s and an air-sea temperature difference of 8 deg. C near the Gulf Stream. This presentation gives an overview of the 2022 effort and the data acquired, discusses challenges and lessons learned, and looks toward the future of uncrewed systems observations in tropical cyclones.

How to cite: Foltz, G. and the 2022 NOAA Saildrone Hurricane Observations Team: Ocean-Atmosphere Observations from Uncrewed Saildrones and Gliders during the 2022 Atlantic Hurricane Season, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7870, https://doi.org/10.5194/egusphere-egu23-7870, 2023.

EGU23-8613 | ECS | Orals | AS1.13

Veer and shear in the tropical cyclone lower boundary-layer 

Sara Müller, Xiaoli Guo Larsén, and David Verelst

Tropical cyclones are associated with extreme wind speeds, enhanced turbulence, vertical wind shear, and veer. All these elements increase loads acting on structures such as wind turbines, bridges, and high-rise buildings. While most studies focus on maximal wind speeds in tropical cyclones, we analyze wind shear and veer in the lowest 300 m of the atmosphere, which is relevant for wind energy applications. We use the Weather Research and Forecasting model to model and analyze the distribution and spatial structure of wind shear and veer in Typhoon Megi (2016) at different radii. We found maximal mean shear and veer in the eyewall region. Shear and veer are on average smaller in the rainbands, but their respective distribution is positively skewed due to spatially organized outliers. These outliers are associated with convective cells and downdrafts, that propagate over structures with speeds of around 30 ms⁻¹. Consequently, structures experience rapid changes in shear and veer. We further analyze vertical cross-sections through convective cells and their propagation velocity. The study highlights differences in characteristics of the low-level wind field between the eyewall region and rainbands, which suggest distinct forces acting on structures.

How to cite: Müller, S., Guo Larsén, X., and Verelst, D.: Veer and shear in the tropical cyclone lower boundary-layer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8613, https://doi.org/10.5194/egusphere-egu23-8613, 2023.

EGU23-8675 | ECS | Posters on site | AS1.13

The influence of weather patterns and the Madden-Julian Oscillation on extreme precipitation over Sri Lanka 

Akshay Deoras, Andrew G. Turner, and Kieran M. R. Hunt

Sri Lanka is affected by extreme precipitation events every year that cause floods, landslides, and tremendous economic losses. Unlike for other countries in South Asia such as India, there has been a limited investigation of weather patterns associated with extreme precipitation events in Sri Lanka. In this study, we use the ERA5 reanalysis dataset to understand the association between extreme precipitation events and 30 weather patterns, which were originally derived to represent the variability of the Indian climate during January–December 1979–2016. Furthermore, we analyse the modulation of extreme precipitation events by the Madden-Julian Oscillation (MJO). We also use the daily rainfall data from 51 meteorological stations in Sri Lanka to take some account of the observational uncertainty.

We find that weather patterns that are most common during the northeast monsoon (December–February) and second intermonsoon (October–November) seasons produce the highest number of extreme precipitation events. Moreover, extreme precipitation events occurring during these two seasons are more persistent than those during the southwest monsoon (May–September) and first intermonsoon (March–April) seasons. The frequency of extreme precipitation events is enhanced (suppressed) in MJO phases 1–4 (5–8) for most weather patterns. The results of this study could benefit meteorologists, hydrologists, and researchers in developing forecasting products based on the identification of these weather patterns and MJO phases in numerical weather prediction and the subseasonal-to-seasonal prediction models, envisaging improved disaster preparedness in Sri Lanka.

How to cite: Deoras, A., Turner, A. G., and Hunt, K. M. R.: The influence of weather patterns and the Madden-Julian Oscillation on extreme precipitation over Sri Lanka, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8675, https://doi.org/10.5194/egusphere-egu23-8675, 2023.

EGU23-8710 | ECS | Orals | AS1.13

Has there been a recent shallowing of tropical cyclones? 

Tsz-Kin Lai and Ralf Toumi

Many aspects of tropical cyclone (TC) properties at the surface have been changing but any systematic vertical changes are unknown. Here we document a recent trend of high thick clouds of TCs. The global inner-core high thick cloud fraction measured by satellite has decreased from 2002 to 2021 by about 10% per decade. The TC inner-core surface rain rate is also found to have decreased during the same period by a similar percentage. This suppression of high thick clouds and rain has been largest during the intensification phase of the strongest TCs. Hence, these two independent and consistent observations suggest that the TC inner-core convection has weakened and that TCs have become shallower recently at least. For this period the lifetime maximum intensity of major TCs has not changed and this suggests an increased efficiency of the spin-up of TCs.

How to cite: Lai, T.-K. and Toumi, R.: Has there been a recent shallowing of tropical cyclones?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8710, https://doi.org/10.5194/egusphere-egu23-8710, 2023.

EGU23-8949 | ECS | Orals | AS1.13

Impact of tropical waves on rainfall modulation and heavy rainfall event occurrence over western equatorial Africa 

Marlon Maranan, Idene-Flore Mantho T., Andreas H. Fink, Derbetini A. Vondou, Peter Knippertz, and Roderick van der Linden

Tropical waves, particularly convectively coupled equatorial waves (CCEWs), are known to modulate rainfall in tropical Africa on intraseasonal down to convective time scales, the latter of which includes the dynamics of heavy rainfall events. Data scarcity in large parts of Africa, especially in equatorial Africa, has long prevented a clearer picture on the regional variability of extreme rainfall. Thus, making use of globally gridded satellite data and a unique in-situ rainfall dataset for Cameroon, this study aims for a systematic comparison of the role of tropical waves on the occurrence and variability of intense rainfall over western equatorial Africa.

For the study period 2001-2019 in a selected domain over Cameroon, heavy daily rainfall (i.e. the 20% strongest and spatially most extensive) events are identified using both the satellite-based rainfall estimates of the Integrated Multi-satellite Retrievals for Global Precipitation Measurement (IMERG) and largely unique station data from the Karlsruhe African Surface Station-Database (KASS-D). The outgoing longwave radiation (OLR) dataset of the National Oceanic and Atmospheric Administration (NOAA) are then used (a) to support evidence of the occurrence of the intense rainfall events, and (b) to apply a wavenumber-frequency filtering in order to evaluate the co-occurrence of tropical waves around these events. These include the fast modes such as Kelvin waves and tropical disturbances (TD), in the study region commonly represented by African Easterly Waves (AEWs), as well as slow modes represented by equatorial Rossby waves and the Madden-Julian Oscillation (MJO). Finally, to account for regional differences in seasonal rainfall characteristics, the analysis is performed for a southern and northern sub-domain during the bi-modal (March–May/September–November) and unimodal (May–October) rainy seasons, respectively.

Results show that: 1) the passage of Kelvin waves and TDs have the strongest impact on daily rainfall rates in the two sub-regions, whereas the effect of the MJO is the weakest ; 2) the modulation by Kelvin waves is strongest in southern Cameroon whereas that of TDs is strongest in the north; 3) there is a shift between the wet wave phases in OLR and rainfall (IMERG, KASSD); 4) up to 78% of the cases with heavy rain coincide with the passage of a tropical wave; 5) Kelvin and TD are again the most likely to be associated with a heavy rainfall event, featuring an up to five times higher local wave intensity as compared to the other waves.

To further test potential dependencies of results on the applied wave identification method, tropical waves have also been identified with a 2D spatial projection method based on parabolic cylinder functions (PCFs) using horizontal wind fields from ERA5. Here, first results suggest that the projection method overall yields less intense and slower Kelvin waves. Furthermore, the occurrence of a Kelvin wave appears to be related to heavy rainfall to a lesser degree compared to the wavenumber-frequency approach. This potentially stresses the importance of a careful choice of the suitable wave identification method for a given application, the details of which are currently evaluated.

How to cite: Maranan, M., Mantho T., I.-F., Fink, A. H., Vondou, D. A., Knippertz, P., and van der Linden, R.: Impact of tropical waves on rainfall modulation and heavy rainfall event occurrence over western equatorial Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8949, https://doi.org/10.5194/egusphere-egu23-8949, 2023.

The very active month of September 2020 included the formation of 10 named storms, the most on record for the month of September, and 5 concurrent tropical cyclones (TCs) in the North Atlantic basin on September 14th. The Model for Prediction Across Scales (MPAS) is used to explore potential opportunity to predict TC activity out to 4 weeks. First, the MPAS model climatology for September TC activity is established. Next, the predictability of an active September is explored using MPAS simulations with initial atmospheric and oceanic conditions from the global forecast system (GFS) and compared with MPAS climatology. MPAS simulations for 2020 are initialized over the last two weeks of August and run freely through September. The total number of TCs, TC days, accumulated cyclone energy (ACE), and the track density are each evaluated relative to observations. In addition, the simulations resulting in the most and least active month are analyzed in further detail to understand why those model simulations predicted an active or inactive September. Lastly, differences with and without a regionally refined 3 km mesh are explored.

How to cite: Nystrom, R. and Judt, F.: Predictions of North Atlantic tropical cyclone activity out to 4 weeks with global MPAS simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10481, https://doi.org/10.5194/egusphere-egu23-10481, 2023.

EGU23-10920 | Posters on site | AS1.13

Characteristics of Mesoscale Convective Systems in the Philippines 

Ma. Cathrene Lagare, Takeshi Yamazaki, and Junshi Ito

Mesoscale convective systems (MCSs) are organized clusters of convection that often bring in heavy to extreme rainfall, which can cause devastating effects such as flooding, landslides, and significant crop and infrastructural damages. Studies on severe weather in the Philippines, a part of the Maritime Continent where frequent and intense convective activities occur, focus predominantly on synoptic-scale systems (e.g., tropical cyclones). The characteristics of MCSs in the Philippines remain understudied. 

Motivated by this research gap, a long-term MCS climatology over the Philippines was constructed using the global MCS tracking database of Feng et al. (2021), and its large-scale environments are investigated to understand the formation of MCSs. Preliminary results show that large-scale flows largely affect MCS formation. MCSs occur more frequently during the peak of the Asian summer monsoon (JJA), producing large rainfall amounts over the west of the Philippines. Meanwhile, the Asian winter monsoon during DJF has a different effect on MCS formation in the Philippines as it does not directly correspond to high occurrences of MCSs. However, the convective systems during DJF still produce high rainfall amounts over the east of the Philippines. Based on these results, additional analyses for the MCSs during the boreal winter are conducted. 

 

Reference:

Feng, Z., Leung, L. R., Liu, N., Wang, J., Houze Jr, R. A., Li, J., ... & Guo, J. (2021). A global high-resolution mesoscale convective system database using satellite-derived cloud tops, surface precipitation, and tracking. Journal of Geophysical Research: Atmospheres, 126(8), e2020JD034202.

How to cite: Lagare, Ma. C., Yamazaki, T., and Ito, J.: Characteristics of Mesoscale Convective Systems in the Philippines, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10920, https://doi.org/10.5194/egusphere-egu23-10920, 2023.

In a recent model evaluation of the African Easterly Wave (AEW) that became Helene (pre-Helene; 2006) over the Atlantic, the wave was categorized as a mixed-off-equatorial moisture mode during tropical cyclogenesis as it evolved under weak temperature gradient balance. It was found that the simulated pre-Helene waves were more intense and overall slower than in ERA5, especially the wave that evolved in a more moisture-rich environment. The growth and propagation of the wave were related to the position of the convection with respect to the center of the wave vortex. The influence of environmental moisture on wave propagation before and during genesis remains an open question. Motivated by the recent findings, in this study, moisture sensitivity experiments are performed with a convection-permitting model to further evaluate the moisture dependency of the pre-Helene wave and later tropical cyclogenesis. The Model for Prediction Across Scales (MPAS) regional configuration is used to allow altering initial and lateral boundary conditions of relative humidity (RH) through the entire atmospheric column using ERA5 pressure-level data. Preliminary results reveal that over land the strength of the wave-trough meridional flow is related to mid-to-upper-level diabatic heating tendencies from clouds located in the northerly phase of the wave and to the lack of shallow convection within the vortex. In MOIST (RH x 1.2 experiment), the wave moves slower, yet organized convection propagates out of phase with the wave speed, ultimately weakening the wave and subsequent tropical cyclogenesis. In CONTROL, where the wave propagates faster, the phasing between wave and convection supports a stronger wave prior to genesis and ultimately genesis when compared to MOIST. A moister atmosphere (MOIST) favors a larger fraction of shallow convection (bottom heavy and weaker updrafts) at the center and ahead of the vortex, detraining the mid-troposphere and weakening the mid-tropospheric vorticity. This leads to a wave that weakens prior to genesis compared to CONTROL as well as a more abrupt decrease in speed prior to genesis. The lack of cloud microphysics heating tendencies in DRY (RH x 0.5 experiment) resulted in a weaker mid-to-upper-level circulation but stronger surface-to-low-level winds. The lack of moisture is detrimental to the simulated pre-Helene; however, a moister environment does not necessarily result in a more intense wave or tropical cyclogenesis event. A wave that propagates more slowly (‘moist wave’ versus ‘dry wave’), does not necessarily favor growth. For further growth, convection that is in phase with the vortex should be deep moist convection.

How to cite: Núñez Ocasio, K. and Davis, C.: Wave Propagation and Growth Dependency to Environmental Moisture: A Case of an Atlantic Tropical Cyclogenesis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10985, https://doi.org/10.5194/egusphere-egu23-10985, 2023.

This study investigated long-term changes of tropical cyclones (TCs) activity and rainfall produced by TCs, hereafter TC-rainfall, over Vietnam in the period of 1979-2021. Furthermore, it is investigated how rainfall changes are influenced by the North Pacific (NP) pattern.

First, it was found that TC activity has not changed significantly in its frequency, and its related rainfall including TC and tropical depression (TDs) produced rainfall, hereafter TCTD-rainfall over entire Vietnam. On the other hand, significant increasing trend of TC activity (XX per 10 year), TC-rainfall (65 mm per 10 year), TCTD-rainfall (75 mm per 10 year), and total rainfall (440 mm per 10 year) is found in North Vietnam in the period of 1979-2021. However, TC, TD activity, TC-rainfall and TCTD-rainfall did not show any significant trends in Central and South Vietnam. Second, decadal and inter-decadal variation of rainfall in North Vietnam are significantly correlated with the North Pacific (NP) pattern during autumn season (October-December). Negative (positive) phases of the NP is characterized by a low (high) sea level pressure (SLP) located over the northern North Pacific Ocean and anomalously warm (cold) sea surface temperature (SST) over central and eastern tropical Pacific, resulting in to less (more) TCs activity and rainfall events over the South China Sea and Vietnam. In summary, it is found that rainfall produced by TCTD exhibits significantly increasing trend in North Vietnam, as well as total rainfall and the NP pattern plays an active role in altering rainfall anomalies in North Vietnam in the decadal and inter-decadal timescales.

How to cite: Thi Ngoc Huyen, H. and Yoon, J.-H.: Tropical Cyclone produced rainfall trends in Vietnam and their relationship with the North Pacific (NP) pattern during 1979 – 2021, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11096, https://doi.org/10.5194/egusphere-egu23-11096, 2023.

EGU23-12007 | Posters on site | AS1.13

Statical prediction system of the typhoon intensity using Numerical Weather Prediction model for correction 

Jeong-Ho Bae, Jung-Rim Lee, Seong-Hee Won, and Dong-Ju Ham

The accuracy of tropical cyclone (TC) forecasts from NWP models have been improved especially for the track. Relatively, TC intensity forecasts still include huge uncertainties though the dynamics, physics processes, and resolutions of NWP systems become higher in both horizontal and vertical. For this reason, many operational centers and academia for TC forecasts implemented statistical prediction systems and Artificial Intelligence (AI) algorithms based on long-term dynamic model forecasts for better predictions of typhoon intensity.
The National Hurricane Center (NHC) developed the Statistical Hurricane Intensity Prediction Scheme (SHIPS) which is a statistical model based on NWP forecasts (parameters from atmosphere and ocean). Also, infrared imagery from geostationary satellite is used as predictors for the regression. SHIPS is implemented for the North Atlantic and East Pacific regions. Otherwise, the Joint Typhoon Warning Center (JTWC) implemented this model for the Northwest Pacific region. Also, Korea Meteorological Administration (KMA) and Japan Meteorological Administration (JMA) developed the statistical based typhoon prediction systems (called STIPS and TIFS, respectively). However, the accuracy of these systems is not stable because it is not easy to define the tendency of NWP forecasts for TC intensity. 
The National Typhoon Center of KMA developed a new statistical model (Statistical Prediction Intensity of Korea mEteorological administrator, SPIKE) for typhoon intensity prediction based on ECMWF forecast. While the ECMWF Integrated Forecast System (IFS) has an excellent performance in forecasting track of typhoons, the intensity tends to be underestimated compared to typhoons analysis information. 
SPIKE is basically developed as a multi-linear regression model, and its predictors are extracted from the IFS forecast. The average prediction error of typhoon intensity of SPIKE in 2022 decreased by about 30% compared to the ECMWF forecasts. However, there was still a limitation, especially for cases of rapid intensification (RI). More studies to reflect real-time intensity, cloud development, center location, and prediction errors of the model are conducted. Then, the second multi-linear regression model to account for these parameters is developed. Finally, an additional improvement of about 30% was achieved. Also, the performance for RI cases developing more than 35 knots within 24 hours was greatly improved. 

How to cite: Bae, J.-H., Lee, J.-R., Won, S.-H., and Ham, D.-J.: Statical prediction system of the typhoon intensity using Numerical Weather Prediction model for correction, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12007, https://doi.org/10.5194/egusphere-egu23-12007, 2023.

EGU23-12516 | ECS | Posters on site | AS1.13

The inner life of the Atlantic ITCZ 

Julia Windmiller and Bjorn Stevens

The intertropical convergence zone (ITCZ) is a central component of the global circulation system, but remarkably little is known about the dynamical and thermodynamical structure of the convergence zone itself. This is true even for the structure of the low-level convergence that gives the ITCZ its name. Following on from the major international field campaigns in the 1960s and 70s, we performed extensive atmospheric profiling of the Atlantic ITCZ during a ship-based measurement campaign aboard the research vessel SONNE in summer 2021. Combining the data we collected during our north-south crossing of the ITCZ with reanalysis data shows that there are generally two low-level convergence lines that roughly mark the southern and northern edges of the region of intense precipitation. Based on the location of these two edges, we construct a composite view of the structure of the Atlantic ITCZ. The ITCZ, far from being simply a region of enhanced deep convection, has a rich inner life, i.e., a rich dynamical and thermodynamic structure that changes throughout the course of the year and has a northern edge that differs systematically from the southern edge. 

How to cite: Windmiller, J. and Stevens, B.: The inner life of the Atlantic ITCZ, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12516, https://doi.org/10.5194/egusphere-egu23-12516, 2023.

EGU23-13886 | ECS | Posters on site | AS1.13

Influence of Indian Summer Monsoon on the Post-Monsoon Cyclones 

Feba Francis, Vikas Kushwaha, and Ashok Karumuri

The North Indian Ocean (NIO) has two Tropical cyclone (TC) seasons, i.e., pre-monsoon and post-monsoon. We find that the Indian summer monsoon (ISM) has an influence on the frequency of cyclones in the post-monsoon in the NIO. Flood years show a higher frequency of TCs, and drought years show a lesser frequency of TCs than normal years. By the examination of Grey-Sikka parameters for cyclogenesis, we show that during the drought years, the mid-tropospheric humidity, low-level vorticity, and Tropical Cyclone Heat Potential are lower than in normal years and the vertical shear is higher over most of the NIO. These factors lead to the reduced cyclonic frequency in the Bay of Bengal during drought years and more frequent cyclones in flood years, though the relation is more ambiguous in the Arabian Sea. This study builds an unexplored relation between ISM and TCs in the NIO and would help in improving TC seasonal prediction.

How to cite: Francis, F., Kushwaha, V., and Karumuri, A.: Influence of Indian Summer Monsoon on the Post-Monsoon Cyclones, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13886, https://doi.org/10.5194/egusphere-egu23-13886, 2023.

EGU23-14195 | ECS | Posters on site | AS1.13

Machine learning-based bias correction for tropical cyclone track simulation of the WRF model over the western North Pacific 

Kyoungmin Kim, Donghyuck Yoon, Dong-Hyun Cha, and Jungho Im

The tropical cyclone (TC) tracks are usually simulated with the numerical models, which have an intrinsic error, although the performance of numerical models is continuously improving. Recently, machine learning has been suggested as a good tool to correct the intrinsic error of the model outputs. This study used an artificial neural network (ANN) to correct the error of TC tracks hindcasted by the Weather Research and Forecasting (WRF) model over the western North Pacific (WNP). TCs whose intensity was higher than tropical depression (i.e., tropical storm, severe tropical storm, and typhoon) from June to November were hindcasted, and TC positions at 72 h were set as the target of bias correction. WRF model output, best track data, and wind field of reanalysis were used as input variables of ANN. The structure of ANN was optimized for TCs during 2006-2015, and the optimized ANN was verified for TCs from 2016-2018. In the verification of ANN, TCs were classified using k-mean clustering to analyze the results of bias correction because the performance of the numerical model for the TC track varied depending on the region of WNP. The ANN corrected the error of WRF by 8.81% for four clusters where ANN was most effective. Moreover, the post-processing was applied to other clusters with less effect of ANN. Consequently, ANN with post-processing improved the accuracy of WRF by 4.34%.

How to cite: Kim, K., Yoon, D., Cha, D.-H., and Im, J.: Machine learning-based bias correction for tropical cyclone track simulation of the WRF model over the western North Pacific, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14195, https://doi.org/10.5194/egusphere-egu23-14195, 2023.

EGU23-14848 | ECS | Posters on site | AS1.13

Multivariate forecasting of tropical cyclones using combined neural networks. 

Yegor Hudozhnik and Andreas Windisch

Tropical Cyclones (TCs) are extremely dangerous and destructive events which pose a danger to human lives every year. Conventional TC forecasting methods are computationally intensive and require a relatively large amount of energy and time.

In the light of climate change due to the process of global warming, the behavior of TCs may change, and therefore require the use of modern, more flexible learning methods for estimation and forecasting.

In recent years, the study of the application of Deep Learning (DL) in this area proved to be highly effective. These methods are designed to facilitate the prediction process, as well as automatically detect possible trends that may occur over time.

In this work, an application of neural networks such as LSTMs and GRUs is investigated to forecast tracks and classify the evolution of TC systems using satellite image data series as an input, where historical track data and the satellite image data are used to train the network. Particular attention is paid to adaptivity of DL approaches to recent trends and edge cases.

How to cite: Hudozhnik, Y. and Windisch, A.: Multivariate forecasting of tropical cyclones using combined neural networks., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14848, https://doi.org/10.5194/egusphere-egu23-14848, 2023.

EGU23-15063 | Orals | AS1.13

Physical mechanisms of offshore propagation of convection in the Maritime Continent 

Simon Peatman, Cathryn Birch, Juliane Schwendike, John Marsham, Chris Dearden, Stuart Webster, Emma Howard, Steven Woolnough, Ryan Neely, and Adrian Matthews

The Maritime Continent, located within the Indo-Pacific warm pool, experiences some of the most intense convective rainfall on Earth, with a pronounced diurnal cycle. The spatio-temporal variability of convection, its organisation and its offshore propagation away from the islands overnight all depend on many factors including the topography of island coastlines and mountains, and large-scale weather phenomena such as the Madden-Julian Oscillation, El Niño–Southern Oscillation and equatorial waves. However, numerical weather prediction and climate models typically suffer from considerable biases in simulating the diurnal convection and its propagation, hence there is a need to improve our understanding of the underlying physical mechanisms of these phenomena.

While the nocturnal offshore propagation of convection is often thought to be forced by gravity waves triggered by land-based diurnal convection, alternative hypothesized mechanisms exist in the literature, related to the propagation of the offshore land breeze and cold pools. Using convection-permitting simulations of selected case studies of convection propagating offshore from Sumatra, we find a squall line propagating overnight due to low-level convergence caused by the land breeze and environmental winds. This is reinforced by cold pools, which we diagnose using model tracers. However, gravity waves also play a role, triggering localized (non-organized) convection which does not itself propagate, but can appear as propagation along wave trajectories when compositing the diurnal cycle over many days.

The investigation is extended to other coastlines in the Maritime Continent, using convection-permitting simulations for 900 days during boreal winters, to demonstrate broader evidence for these physical mechanisms; to understand why the offshore propagation occurs on some days but not others; and to show how the strength, timing and causes of offshore propagation vary for different Maritime Continent islands, due to variations in the large-scale winds, orography and the topography of coastlines.

How to cite: Peatman, S., Birch, C., Schwendike, J., Marsham, J., Dearden, C., Webster, S., Howard, E., Woolnough, S., Neely, R., and Matthews, A.: Physical mechanisms of offshore propagation of convection in the Maritime Continent, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15063, https://doi.org/10.5194/egusphere-egu23-15063, 2023.

The organization and propagation of inner rainbands of landfalling Typhoon Cempaka (2021) during rapid intensification (RI) are investigated from two ground-based Doppler radars. Dual-Doppler analysis based on ground-based radars provide long-lasting high temporal and spatial three dimensional wind fields to examine the possible mechanisms for the organization of inner rainbands. In the early period when the convections were preferentially located inside the RMW, deformation plays an important role in the formation of inner rainbands. Convective cells were advected by the cyclonically rotating tropical cyclone swirling flow while being deformed into spiral shapes. In the later period when the convections were preferentially located outside the RMW, positive part of wavenumber-2 reflectivity associated with the rainband is collocated with the positive component of wavenumber-2 vorticity. The wavenumber-2 reflectivity moved at an azimuthal phase speed of 64.5% of the local tangential wind and very close to the theoretically predicted speed. It is evident that vortex Rossby wave is associated with the organization of rainband in the later stage.

How to cite: Fan, X.: Differences in the Formation and Evolution of the Inner Rainbands during the Rapid Intensification of Typhoon Cempaka (2021), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15194, https://doi.org/10.5194/egusphere-egu23-15194, 2023.

EGU23-15259 | ECS | Orals | AS1.13

Impacts of the MJO and Equatorial Waves on Tracked Mesoscale Convective Systems Over Southeast Asia 

Julia Crook, Fran Morris, Rory Fitzpatrick, Simon Peatman, Juliane Schwendike, Thorwald Stein, Cathryn Birch, and Sam Hardy

Southeast Asia is a region dominated by intense convection and characterised by the high-impact weather associated with synoptic scale tropical depressions, typhoons, or tropical cyclones (TCs). However, more localised convection such as mesoscale convective systems (MCSs) can also produce intense precipitation which can be a major risk for loss of lives and property for the communities in the region. Due to these high-impact weather features, its complex orography, and the significant impact of large-scale weather features on its meteorological variability, predicting weather in Southeast Asia is of great importance and scientific interest, but is a challenge. We aim to characterise the distribution of MCSs in the region and capture how the systems are modulated by the Madden-Julian Oscillation (MJO) and equatorial waves. 

MCSs in Southeast Asia between 2015 and 2020 were tracked using Himawari satellite data, their associated rainfall estimated using IMERG, and classified by lifetime and propagation speed. TC-related rainfall was also deduced using data from IBTrACS to identify certain cloud clusters as associated with TCs. Between 10S and 10N, MCSs account for 45-70% of the precipitation between November and April, and over most of the region, the fractional MCS contribution to rainfall is higher than average on extreme wet days (>55%). Long-lived  (>12 hours) MCSs contribute disproportionately, providing 84% of the rainfall despite comprising only 34% of all MCSs.

The MJO modulates MCS rainfall in a similar way to total rainfall, contributing >50% of the total rainfall anomaly, with the number of MCSs being greater in convectively active phases. However, in the West part of the region there are more fast-moving MCSs in the active MJO phases and more slow-moving MCSs in the inactive phases, resulting in fast-moving MCSs having a greater impact on the MJO-associated variation in MCS rainfall. This variation in MCS rainfall is larger in the West part of the region than the East. Meanwhile, variation in the area-mean rainfall rate within the storms, and sizes of storms were less well correlated with MCS rainfall in different phases; when areas were large, area-mean rainfall rate was generally low, and vice versa, providing compensating effects.

In the low-level convergence phase of an equatorial Kelvin wave, MCS rainfall and non-organized rainfall both increase, accounting for 20-50% of local rainfall anomalies, a pattern which is again enhanced in the West of the region. By contrast, Westward-propagating Mixed Rossby-Gravity waves, and Rossby-1 waves, do not strongly modulate MCS rainfall, and instead their rainfall anomalies are dominated by TC-related rainfall.

These relationships between MCSs and the MJO and Kelvin waves provide useful insight into forecasting MCSs in Southeast Asia by utilising knowledge of the synoptic weather regimes that are or will be affecting the region.

How to cite: Crook, J., Morris, F., Fitzpatrick, R., Peatman, S., Schwendike, J., Stein, T., Birch, C., and Hardy, S.: Impacts of the MJO and Equatorial Waves on Tracked Mesoscale Convective Systems Over Southeast Asia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15259, https://doi.org/10.5194/egusphere-egu23-15259, 2023.

EGU23-15866 | ECS | Orals | AS1.13

Investigation of the microphysical processes during the rapid intensity changes of tropical cyclones over the Bay of Bengal: A modelling approach 

Yerni Srinivas Nekkali, Krishna Kishore Osuri, Ananda Kumar Das, and Dev Niyogi

Tropical cyclones (TCs) are one of the natural destructive weather phenomena. The accurate prediction of TC intensity is dependent on the understanding of the physical processes behind that. This study exposes the importance of microphysical (MP) processes in the rapid intensity changes of cyclones. For this, tropical cyclone simulations were made from the WRF model with a double nested (9 km-Static and 3 km-moving nests) configuration. This study shows that the heating generated by the MP processes in the TC’s inner-core region is highly (moderately) correlated with precipitated (non-precipitated) hydrometeors. During the rapid intensification (RI) period, heat-released microphysical processes such as condensation, freezing due to the accretion of liquid hydrometeors with ice particles, and deposition, etc., are dominant as compared to cooling-induced processes. In addition, the saturated envelope in the TC Phailin (2013) is responsible for more convection, heating, and hence consecutive RI episodes. While dry air intrusion hampers the prolonged RI episodes in TC Fani (2019). However, rapid weakening (RW) in TC Lehar (2013) is promoted by asymmetric, limited convection, and hence, lesser heating. During this RW period, the warm rain (ice) microphysical processes mainly produce heating (cooling).

How to cite: Nekkali, Y. S., Osuri, K. K., Das, A. K., and Niyogi, D.: Investigation of the microphysical processes during the rapid intensity changes of tropical cyclones over the Bay of Bengal: A modelling approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15866, https://doi.org/10.5194/egusphere-egu23-15866, 2023.

EGU23-15922 | Orals | AS1.13

The Potential of the W-band polarization diversity Doppler radar envisaged for the WIVERN mission for sampling tropical cyclones 

Frederic Tridon, Alessandro Battaglia, and Anthony Illingworth

The WIVERN (WInd VElocity Radar Nephoscope) mission, currently under the Phase-0 of the ESA Earth Explorer program, promises to complement AEOLUS Doppler wind lidar by globally observing, for the first time, vertical profiles of winds in cloudy areas. The objective of this work is to assess the potential of WIVERN for sampling tropical cyclones from the long-term CloudSat dataset. Realistic WIVERN synthetic observations are produced thanks to the recently developed end to end simulator of the WIVERN dual-polarization Doppler conically scanning 94 GHz radar based on CloudSat reflectivity observations and ECMWF co-located winds. The resulting multi-year dataset provides statistics on how well the WIVERN mission can sample the cloud systems associated to tropical cyclones and monitor their genesis and lifecycle. The analysis of the results provides statistics for addressing the following questions for tropical systems: What is the frequency of reliable wind estimates as a function of height? What is the effect of ghost echoes produced by cross-polarization? What is the impact of noise error and how often will the 94 GHz radar signal be fully attenuated by rain?

How to cite: Tridon, F., Battaglia, A., and Illingworth, A.: The Potential of the W-band polarization diversity Doppler radar envisaged for the WIVERN mission for sampling tropical cyclones, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15922, https://doi.org/10.5194/egusphere-egu23-15922, 2023.

Characterizing inflow structure is important to better represent tropical cyclone impacts in numerical models. While much research has considered the impact of storm translation on the distribution of inflow angle, comparatively less research has examined its distribution relative to the environmental wind shear. This study analyzes data from 3,655 dropsondes in 44 storms to investigate the radial and shear-relative distribution of surface inflow angle. Emphasis is placed on its relationship with intensity change. The results show that the radial variation in the inflow angle is small and not significantly dependent on the shear magnitude or intensity change rate. In contrast, the azimuthal distribution of the inflow angle shows a significant asymmetry, with the amplitude of the asymmetry increasing with shear magnitude. The maximum inflow angle is located in the downshear side. The degree of asymmetry is larger in the outer core than in the eyewall. Intensifying storms have a smaller degree of asymmetry than steady-state storms under moderate shear.

How to cite: Ming, J.: The Shear-Relative Variation of Inflow Angle and Its Relationship to Tropical Cyclone Intensification, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16246, https://doi.org/10.5194/egusphere-egu23-16246, 2023.

EGU23-16512 | ECS | Posters on site | AS1.13

Spatial and temporal variability of floods in Indonesia based on governmental data, Twitter messages and paper reports 

Beata Latos, Dariusz Baranowski, Maria Flatau, Jens de Bruijn, Katarzyna Barabasz, Michał Łabuz, Donaldi Permana, and Jaka Paski

Indonesia, with its tropical and monsoonal climate, is exposed to heavy precipitation and enormous rainfall accumulation which results in weather-driven hazards, including extreme rainfall events and floods. There are several conventional sources of data to estimate potential of anomalously high precipitation in Indonesia, including rain gauge data, satellite data and meteorological reanalysis. Even though they allow assessment of precipitation variability, their usefulness is limited by biases and data gaps. Furthermore, assessment of a variability in precipitation patterns is not the same as identification of their adverse societal effects, such as floods.  

Due to the proliferation of social media, these conventional data sets can be supplemented with crowd-sourced information that can potentially provide longer-term, accurate records and cover a larger area. In this study, we demonstrated that Twitter is a useful source for flood detection and created a flood database. Twitter-based flood database is derived for subregions of major islands within Indonesia: Java, Sumatra, Borneo and Sulawesi, and validated against data from governmental reports and local paper articles. Results show that Twitter-based retrieval performs well in comparison with other sources, but only in regions characterized by sufficiently large pool of active users. 

Flood events and extreme rainfall events (defined using in-situ and satellite data) were compared in terms of their spatial and temporal distribution, as well as their meteorological drivers. In general, on each of the island, there is a seasonal cycle: a wet season during boreal winter, when the Southeast Asian monsoon provides an environment supportive of rain events, and a dry season during boreal summer. On intraseasonal scale, Madden-Julian Oscillation (MJO) creates the conditions favorable for weather extremes. MJO activity causes an increase in the local rainfall rate, with a significant increase in a chance of observing extreme precipitation during favorable MJO phase.  

How to cite: Latos, B., Baranowski, D., Flatau, M., de Bruijn, J., Barabasz, K., Łabuz, M., Permana, D., and Paski, J.: Spatial and temporal variability of floods in Indonesia based on governmental data, Twitter messages and paper reports, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16512, https://doi.org/10.5194/egusphere-egu23-16512, 2023.

EGU23-16737 | Orals | AS1.13

Three Dimensional Wind and Rain Aircraft-Based Observations within the Hurricane Inner Core 

Zorana Jelenak, Joe Sapp, Paul Chang, Clayton Bjorland, James Carslwell, and Stephen Guimond

The three dimensional observations of wind and rain within the inner core of major hurricanes in the Atlantic basin were collected utilizing the Imaging Wind and Rain Profiler (IWRAP) on board a National Oceanographic Atmospheric Administration (NOAA) P-3 aircraft during the 2020-2022 hurricane seasons. With 30 m vertical and 150 m horizontal resolution, these measurements represent the highest resolution hurricane boundary layer (HBL) observations collected to date with a remote sensing instrument. State of the art IWRAP radar control and data acquisition system collects both in-phase (I) and quadrature (Q) signals for the entire observational profile. This allows for the full spectrum to be derived by utilizing a series of Fast Fourier Transforms (FFTs) on every single range gate resulting in the availability of the observations within lowest 500 m of the HBL. Previously, these observations were only possible from drop sondes. High resolution reflectivity profiles are processed into both three dimensional wind and rain products utilizing Ku- and C-band microwave observations. Over the course of three hurricane seasons, observations of 9 major hurricanes were collected and processed.

            With its unprecidented resolution these measurements are providing insights into turbulant processes within HBL of the major hurricanes and can possibly lead into new HBL parametarization of the hurricane models. Validation of measurements were carried out with flight level aircraft measurements, Step Frequency Microwave Radiometer surface wind measurements and Tail Doppler Radar 3d Wind and Reflectivity data.

            The measurement technique, collected data, validation results and data availability will be discussed and presented.

How to cite: Jelenak, Z., Sapp, J., Chang, P., Bjorland, C., Carslwell, J., and Guimond, S.: Three Dimensional Wind and Rain Aircraft-Based Observations within the Hurricane Inner Core, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16737, https://doi.org/10.5194/egusphere-egu23-16737, 2023.

EGU23-16746 | Posters on site | AS1.13

A study on precipitation characteristics of Kal Baishakhi: a premonsoon thunderstorm event 

Srinivasa Ramanujam Kannan

Kal Baishaki, a heavy thunderstorm event, recurs yearly during the premonsoon period (March-May) over the Indo-Gangetic plain and northeastern part of India. The event is highlighted by vigorous thunderstorm activity often associated with lightning and heavy to very heavy precipitation. Though the event has significant health and economic impact, the precipitation characteristics are not clearly understood. This is mainly due to a lack of continuous observation across a vast area covering West Bengal, Jharkhand, Orissa, Bihar, Assam, and other northeastern states of India. Precipitation measuring instruments onboard the Tropical Rainfall Measuring Mission satellite, followed by the Global Precipitation Measurement Mission, have provided an unprecedented data set that provides rainfall estimates at a high spatial, but sparsely temporal scale. The accuracy of data products has been refined over the years by comparing them with measurements from ground stations worldwide. The present work aims to consider rainfall data measured between 2001 and 2020 using remotely sensed instruments to analyse the precipitation characteristics of the significant rain event using a time series analysis approach.

How to cite: Kannan, S. R.: A study on precipitation characteristics of Kal Baishakhi: a premonsoon thunderstorm event, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16746, https://doi.org/10.5194/egusphere-egu23-16746, 2023.

EGU23-716 | ECS | Posters on site | AS1.14

Analysis of the Genesis Potential Index in Subtropical Cyclones off the Coast of Brazil 

João Gabriel Martins Ribeiro, Gabriel Teodoro da Paz, Michelle Simões Reboita, Luiz Felippe Gozzo, Glauber Willian de Souza Ferreira, and Rosmeri Porfírio da Rocha

The coastal region of southern and southeastern Brazil, which is part of the South Atlantic Ocean basin, is a genesis region for subtropical cyclones and, therefore, is susceptible to weather changes caused by these systems. The first named subtropical cyclone in the South Atlantic basin was Anita in 2010. Since then, some studies on subtropical cyclones have been carried out, but there are still several questions to be investigated. Thus, this study aims to: (a) describe the main physical mechanisms of genesis of the subtropical cyclones that were named in the South Atlantic Ocean between 2010 and 2021 and (b) identify the value of the Genesis Potential Index (GPI) between the pre-cyclogenesis and the phase in which these systems acquire subtropical characteristics. The rationale for analyzing the CPI is that we want to identify a possible pattern that helps in operational weather forecasting. The main database used in the study is the ERA5 reanalysis. Of the 14 cyclones studied, only two systems did not have cyclogenesis with subtropical characteristics, but acquired it 24 hours after cyclogenesis. The results indicate that 5 cyclones have a genesis associated with mid-level troughs in the atmosphere, and 9 with blocking patterns (cutoff low type). As most of the cyclones studied occur in an environment with blocking structure, this indicates that the condition of weak vertical wind shear is an important factor for subtropical cyclones. As the GPI does not show a standard value in the 14 cyclones studied, between pre-cyclogenesis and the moment when these systems become subtropical, as it varies from 0.35 in the Deni genesis to 22.71 in the Anita genesis, perhaps it is not possible to use it with a threshold in operational practices. The authors thank Programa de P&D regulado pela ANEEL e empresa Engie Brasil Energia e a Companhia Energética Estreito for the financial support.

How to cite: Ribeiro, J. G. M., da Paz, G. T., Reboita, M. S., Gozzo, L. F., Ferreira, G. W. D. S., and da Rocha, R. P.: Analysis of the Genesis Potential Index in Subtropical Cyclones off the Coast of Brazil, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-716, https://doi.org/10.5194/egusphere-egu23-716, 2023.

Previous studies showed that the midlatitude atmospheric circulation generally shifts poleward in response to climate change induced by increased greenhouse gas concentration, including the midlatitude storm track and the eddy-driven jet. The magnitude of this shift varies widely between different climate models and depends on the season, hemisphere and longitude. In this study we aim to reexamine the connection between the shifts of the sensible eddy heat flux and the eddy-driven jet in response to climate change and the role of diabatic heating and latent eddy heat flux in this relation. Our approach is to use the constraints of the zonally averaged heat and momentum budgets in order to connect the eddy-driven jet latitude to the heat budget terms. First, we examine the relation between the eddy-driven jet latitude and the eddy heat flux latitude in the inter-model spread of CMIP6 models. We find that the latitudinal separation between the eddy heat flux and eddy-driven jet depends on the amount of diabatic heating in the midlatitude midtroposphere, which varies widely between different models. This relation is explained based on the heat and momentum budgets.

Next, we use an idealized general circulation model with interactive water vapor and full radiation. We customized the model with different levels of saturation vapor pressure by increasing CO2 concentration and by increasing the humidity factor in the Clausius-Clapeyron relation. We found that in both the cases the atmospheric circulation responds in a similar way and the heat budget terms shift upward and poleward, signifying an upward and poleward shift of the storm track. We found that when the diabatic heating rises upward and strengthens enough over the midlatitude mid-troposphere in response to climate change, the adiabatic cooling by the Ferrel cell rising branch balances the diabatic heating and an equatorward shift of the eddy driven jet and the Ferrel cell is observed. These results provide further insight to the relation between the responses of the midlatitude circulation and the poleward energy flux terms to climate change.

How to cite: Ghosh, S., Lachmy, O., and Kaspi, Y.: The latitudinal shift of the midlatitude atmospheric circulation in response to climate change and the role of midlatitude diabatic heating, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1801, https://doi.org/10.5194/egusphere-egu23-1801, 2023.

EGU23-1812 | ECS | Orals | AS1.14

Extreme rainfall events in Morocco: spatio-temporal characteristics and climate drivers 

Abdelaziz Chaqdid, Alexandre Tuel, Abdelouahed EL Fatimy, and Nabil EL Moçayd

Extreme precipitation drives a series of natural disasters such as floods, flash floods, landslides, or crop losses. These disasters directly impact people's lives, their homes, and their food security. Located at the edge of the subtropics, on the northern edge of the Sahara desert, Morocco is particularly vulnerable to extreme precipitation. Indeed, between 1951 and 2015, Morocco experienced more than 35 major floods, which resulted in significant material and human losses. Understanding the spatio-temporal characteristics of extreme precipitation is key to better predicting and mitigating the risks associated with extreme precipitation events (EPEs). Yet, the spatio-temporal distribution and physical drivers of extreme precipitation in Morocco remain poorly understood. To address this gap, we apply temporal and spatial clustering methods to precipitation data from the ERA5 database as well as from observational databases to identify the main drivers of EPEs in Morocco. We find that Morocco exhibits five spatially coherent regions in terms of EPE timing, corresponding to mixed influences of large-scale extratropical and tropical weather systems. Indeed, EPEs in northern regions are caused by weather patterns similar to the negative phase of the North Atlantic Oscillation (NAO), associated with strong upper air flow enhanced by Greenland blocking and Rossby wave breaking (RWB). By contrast, extreme precipitation in southern regions is associated with tropical-extratropical interactions. There, EPEs are linked to an intense water vapor transport from the tropics and a relatively weak upper air flow.

How to cite: Chaqdid, A., Tuel, A., EL Fatimy, A., and EL Moçayd, N.: Extreme rainfall events in Morocco: spatio-temporal characteristics and climate drivers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1812, https://doi.org/10.5194/egusphere-egu23-1812, 2023.

EGU23-1890 | Orals | AS1.14

The thermodynamic differences between winter cyclones from midlatitudes and high latitudes 

Dandan Tao, Camille Li, Richard Davy, Shengping He, Clio Michel, and Andrea Rosendahl

Cyclones carry heat and moisture that impact local conditions along their path. Cyclones with different origins can, however, have different life cycles and cause different impacts. To quantify differences in the thermodynamic evolution of cyclones originating from different latitudes during wintertime, we separate the cyclones according to their origin (cyclogenesis location):  midlatitude (ML) cyclones originating in the North Atlantic and high-latitude (HL) cyclones originating in the Nordic Seas and Barents Seas. It is found that HL cyclones generally carry lower thermodynamic energy as they originate in a cold environment. In contrast, ML cyclones have much higher thermodynamic energy throughout their lifecycle, even though they lose a large amount of heat as they travel long distances from their origin towards the Arctic. For a given region in the high latitudes (e.g., the Barents Sea), the mean vertical profiles of temperature and moisture from the HL group are colder and drier compared to the ones from the ML group, but the maximum values in the HL group can reach those of the ML group. Further analysis for the top 10% warmest profiles in the HL group suggests that these HL cyclones form in a preconditioned warm and moist environment. The precondioning is set up by the large-scale circulation with influences from the upstream North Atlantic. Under special conditions, the formation of high latitude cyclones in a preconditioned warm and moist environment can lead to extreme warming events in the deep Arctic like the one during New Year’s 2015/16.

How to cite: Tao, D., Li, C., Davy, R., He, S., Michel, C., and Rosendahl, A.: The thermodynamic differences between winter cyclones from midlatitudes and high latitudes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1890, https://doi.org/10.5194/egusphere-egu23-1890, 2023.

EGU23-2195 | ECS | Orals | AS1.14

Origin of low-tropospheric potential vorticity in Mediterranean cyclones 

Alexander Scherrmann, Emmanouil Flaounas, and Heini Wernli

Mediterranean cyclones are extratropical cyclones, typically of smaller size and weaker intensity than other cyclones that develop over the main open ocean storm tracks. Nevertheless, Mediterranean cyclones can attain high intensities, even comparable to the ones of tropical cyclones, and thus cause large socio-economic impacts in the densely populated coasts of the region. After cyclogenesis takes place, a large variety of processes are involved in the cyclone’s development, contributing with positive and negative potential vorticity (PV) changes to the lower-tropospheric PV anomalies in the cyclone center. Although the diabatic processes that produce these PV anomalies in Mediterranean cyclones are known, it is still an open question whether they occur locally within the cyclone itself or remotely in the environment (e.g., near high orography) with a subsequent transport of high-PV air into the cyclone center. This study introduces a Lagrangian method to determine the origin of the lower-tropospheric PV anomaly, which is applied climatologically to ERA5 reanalysis and to 12 monthly simulations, performed with the IFS model. We define and quantify so-called "cyclonic" and "environmental" PV and find that the main part of the lower-tropospheric PV anomaly (60%) is produced within the cyclone, shortly prior (-12 h) to the cyclones’ mature stage. Nevertheless, in 19.5% of the cyclones the environmental PV production near the mountains surrounding the Mediterranean basin plays a significant role in forming the low-tropospheric PV anomaly, and therefore in determining the intensity of these cyclones. The analysis of PV tendencies from the IFS simulations reveals that the major PV production inside the cyclone is typically due to convection and microphysics, whereas convection and turbulent momentum tendencies evoke most of the positive PV changes in the environment.

How to cite: Scherrmann, A., Flaounas, E., and Wernli, H.: Origin of low-tropospheric potential vorticity in Mediterranean cyclones, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2195, https://doi.org/10.5194/egusphere-egu23-2195, 2023.

EGU23-4675 | ECS | Posters on site | AS1.14

Storms and associated damages in Norway 

Ashbin Jaison, Asgeir Sorteberg, Clio Michel, and Øyvind Breivik

Extreme winds account for more than half of Norway’s insurance claims related to natural hazards [1]. Quantifying windstorm-damage relations is crucial to prepare for and mitigate the effects of future wind events. However, there has never been an attempt to quantify windstorm-damage relations at the municipality level in Norway. The work in hand employs four different damage functions at the municipality level of Norway. Along with the newly proposed modified Prahl damage function [2], an ensemble means of the damage estimates are tested for 356 municipalities in Norway. We evaluate the damage functions in terms of forecast accuracy. The spatial distribution of losses suggests severe damages along the west coast of Norway. Further inland in Norway, there are seldom any losses due to Norway’s unique topography and demography. The losses above the 99.7th percentile in each municipality constitute 85% of total national loss, and we focus on this extreme loss class. A significant agreement between the observed and estimated losses at the municipality and national levels indicates that the damage functions are suited for forecasting storm-induced damages. The damage functions are also able to successfully reconstruct the spatial spread and pattern of losses caused by very extreme windstorms.

References

1] Finance Norway, Natural Disaster Statistics (NASK), (2019)
[2] B.F. Prahl et al., Applying stochastic small-scale damage functions to German winter storms, Geophysical Research Letters 39, (2012)

 
 

How to cite: Jaison, A., Sorteberg, A., Michel, C., and Breivik, Ø.: Storms and associated damages in Norway, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4675, https://doi.org/10.5194/egusphere-egu23-4675, 2023.

EGU23-5690 | ECS | Posters on site | AS1.14 | Highlight

Investigating the predictability of Mediteranean cyclones and their severity 

Benjamin Doiteau, Florian Pantillon, Matthieu Plu, Laurent Descamps, and Thomas Rieutord

Cyclones are essential elements of the climate and of the water cycle in the Mediterranean. The most intense of them lead to natural disasters because of their violent winds and extreme rainfall, which can cause significant damage to the territories bordering the Mediterranean (coast and mountain ranges). Reliable forecasts of cyclones are therefore essential to better anticipate and prevent their societal impact. However, their predictability is often limited by their particularities: smaller cyclones with a shorter life cycle than in the North Atlantic, complex topography, interactions with the relatively warm sea and air masses laden with dust from the Sahara.

We investigate the predictability of Mediterranean cyclones in a systematic framework using an ensemble prediction system. A reference dataset was first obtained by tracking cyclones in the ERA5 reanalysis (1979-2021), using an algorithm developped for the North Atlantic and adapted for the Mediterranean region. We then investigated the predictability using ARPEGE ensemble reforecasts in a homogeneous configuration over 22 years (2000-2021).

We restricted the study on 500 cases, which were selected using a storm severity index based on wind gusts and adapted for the Mediterranean region. The cases were then divided in several categories following their dynamical context, their intensity and their geographical origin. The predictability of the reforecasts was finally quantified on each of those categories, using probabilistic scores on cyclone trajectories (along and cross track error) and on intensities (mean sea level pressure and storm severity index).

While past studies have been limited by the fact that regular updates of operational forecasting systems do not allow the predictability of cases to be compared with each other, the homogeneous configuration of the ARPEGE ensemble reforecasts makes it possible to systematically identify the limitation to the predictability of Mediterranean cyclones.

How to cite: Doiteau, B., Pantillon, F., Plu, M., Descamps, L., and Rieutord, T.: Investigating the predictability of Mediteranean cyclones and their severity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5690, https://doi.org/10.5194/egusphere-egu23-5690, 2023.

A large number of intense cyclones occur every year in the Mediterranean basin, a relatively small and densely populated region, but also a worldwide climate-change hotspot. Given their importance for the variability of the regional climate and its extremes, Mediterranean cyclones have lately attracted much of attention, especially due to the broad range of severe socio-economic and environmental impacts that they produce.

This talk aims at summarizing the concentrated knowledge of the last decade on the dynamics, climatology and relevant impacts of Mediterranean cyclones. We will especially focus on the processes that take place in different spatiotemporal scales triggering cyclogenesis and turning Mediterranean cyclones into catastrophic storms. We will also discuss the role of the unique regional geographical features therein, along with the influence of the latitudinal location of the Mediterranean basin. Finally, we will discuss the different subtypes of Mediterranean cyclones that develop in the region, devoting special attention to medicanes, i.e. cyclones with tropical characteristics and subjects of numerous recent studies. Througout the talk, research perspectives that advance the field of Mediterranean cyclones as a whole will be highlighted, along with current trends in community efforts within the framework of MedCyclones COST Action that address relevant topics to the complex dynamics of Mediterranean cyclones and consequent severe socio-economic impacts.

How to cite: Flaounas, E.: Mediterranean cyclone dynamics and climatology: current knowledge and research perspectives, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6278, https://doi.org/10.5194/egusphere-egu23-6278, 2023.

EGU23-6570 | Posters on site | AS1.14

Cloud-radiative heating shapes idealized extratropical cyclones by changing atmospheric stability 

Aiko Voigt, Behrooz Keshtgar, and Klara Butz

"All models are wrong. Some are wrong in a useful manner.” (adapted by the authors from George Box) In this presentation, we utilize an error in the surface flux formulation of the ICON-NWP numerical weather prediction model to elucidate how cloud-radiative heating affects the intensity of idealized extratropical cyclones.

We present idealized baroclinic life cycle simulations with two versions of the global atmosphere model ICON-NWP. Both versions simulate the same cyclone when run without radiative heating, but disagree when cloud-radiative heating is allowed to affect atmospheric temperature and the cyclone evolution. In version 2.1, taking into account cloud-radiative heating leads to a weaker cyclone, while in version 2.6 a stronger cyclone results. The simulations use a new modeling technique for which only cloud-radiative heating interacts with the cyclone and clear-sky radiative heating is omitted. The technique circumvents changes in the mean state due to clear-sky radiative heating that has complicated the interpretation of previous work.

A defining difference between the two model versions is the amount of simulated low-level clouds. Compared to version 2.6, version 2.1 simulates twice as many low-level clouds and a twice as strong cooling of the planetary boundary layer by cloud-radiative heating. While the increase in low-level clouds is tied to an error in the surface flux formulation in version 2.1 that was corrected in version 2.6, the error provides an opportunity to probe the impact of cloud-radiative heating in the boundary layer (below 2 km) versus the free-troposphere (above 2 km). Sensitivity studies show that negative cloud-radiative heating in the boundary layer from the tops of low-level clouds weakens the cyclone by making the atmosphere more stable. At the same time, they show that negative cloud-radiative heating near the tropopause from the tops of high-level clouds strengthens the cyclone by decreasing atmospheric stability. The changes in stability are particularly evident in regions of upward motion.

Overall, our results indicate that the vertical distribution of clouds and their radiative heating are an important factor for the dynamics of extratropical cyclones and that model differences in the simulation of low-level clouds can translate to model differences in cyclone intensity.

How to cite: Voigt, A., Keshtgar, B., and Butz, K.: Cloud-radiative heating shapes idealized extratropical cyclones by changing atmospheric stability, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6570, https://doi.org/10.5194/egusphere-egu23-6570, 2023.

EGU23-6629 | ECS | Posters on site | AS1.14

Effects of climate variability and change on cyclones in the Mediterranean 

Onno Doensen, Martina Messmer, Woon Mi Kim, and Christoph Raible

The Mediterranean is characterized by a high extratropical cyclone activity. These cyclones are an important source for water availability in the region, but at the same time they have the potential to cause extreme weather in the form of precipitation and wind extremes. The Mediterranean is heavily affected by the ongoing anthropogenic climate change, which is expected to have a profound effect on cyclones in this area. In this study, we investigate the effects of internal climate variability and anthropogenic climate change on the characteristics of Mediterranean cyclones. The analysis is based on two simulations from the Community Earth System Model 1.2 (CESM): a seamless simulation spanning 3500 years from 1500 BCE to 2012 CE and a simulation of future RCP8.5 scenario from 2013 to 2300 CE. The simulations have a 1.9°x2.5° horizontal resolution, and cyclones are identified using an established detection and tracking algorithm. Comparison with the ERA5 reanalysis for the period 1981–2010 shows that CESM is able to realistically represent cyclone frequency on a global scale, though it slightly underestimates cyclone activity in the Mediterranean. Our results indicate that cyclone activity in the Mediterranean varies on interdecadal to centennial time scales before 1850 CE. These variations are linked to positive and negative climate anomalies and fluctuations in strength of several modes of circulation, such as the North Atlantic Oscillation. The variations caused by internal variability are, however, of smaller magnitude than the effects of future climate change on the Mediterranean cyclones. In the RCP8.5 scenario, Mediterranean cyclones will become less frequent based on our simulation, and cyclone related precipitation will decrease in addition to that, which is contrary to what is being observed in other important storm track regions, such as the North Atlantic. We hypothesize that the changes in cyclone characteristics are more pronounced in the Western Mediterranean than in the Eastern Mediterranean. Overall, the study suggests that cyclone activity in the Mediterranean is projected to leave the bandwidth of variability of the last 3500 years near the end of the century.

How to cite: Doensen, O., Messmer, M., Kim, W. M., and Raible, C.: Effects of climate variability and change on cyclones in the Mediterranean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6629, https://doi.org/10.5194/egusphere-egu23-6629, 2023.

Extratropical cyclone airstreams, such as warm conveyor belts (WCBs), are linked to strong precipitation along with latent heat release at low levels and, thus, changes in the low-level PV distribution. Previous studies have shown significant changes in PV anomalies in a future climate under the RCP8.5 scenario, which are also associated with changes in strong near-surface winds. However, the source of these PV anomalies is still unclear, especially at upper levels. Based on the 1% strongest winter-cyclones in the North Atlantic (NA) region over the two periods 1990-2000 and 2091-2100, we adopt a Lagrangian perspective to investigate such changes in CESM Large Ensemble simulations.
Backward trajectories are computed to explicitly identify the contributions of diabatic processes to future changes in cyclone-associated PV anomalies. Moreover, the role of specific airstreams in PV generation/destruction is examined with Lagrangian composites.
The results show a sinificant change in the mean trajectory properties 24 hours before the maximum cyclone intensity at low and upper levels. This period of 24 hours is taken to construct Lagrangian composites at 700 hPa and 250 hPa, which provide insights into changes in WCB and dry intrusion (DI) airstreams. We further analyze these airstrem changes by constructing cross sections downstream (WCB regime) and at the equatorward side (DI regime) of the cyclone center.
In general, increased diabatic heating along backward trajectories amplifies positive PV anomalies near the cyclone center at both lower and upper levels in a warmer future climate. More specifically, a poleward and upward shift of the WCBs with a larger PV production at middle levels are is found. DIs near the cyclone center are projected to be responsible for stronger PV production at low levels to the south of the cyclone center. At upper levels, the decreased PV anomaly to the south of the cyclone center results from a combined effect of a decreased climatological PV in the NA region and a shift in the origin of the air masses. The increasing importance of diabatic processes in a wamer climate suggests that a better representation of these processes in climate models is necessary to reduce uncertainties.

How to cite: Dolores-Tesillos, E. and Pfahl, S.: Future changes in North Atlantic winter cyclones in CESM-LE simulations from a Lagrangian-composite perspective, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6851, https://doi.org/10.5194/egusphere-egu23-6851, 2023.

EGU23-7236 | ECS | Posters on site | AS1.14

Objective assessment of storm surge risk in the German Bight – historical events and future climate change 

Laura Schaffer, Nico Becker, Ludwig Schenk, Claudia Hinrichs, Gabriel Ditzinger, Nils H. Schade, Daniel J. Befort, and Tim Kruschke

Storm surges in the German Bight can have great destructive potential. This includes devastating floods, structural damage to infrastructure, and even loss of life. The most important driver of storm surge events in the German Bight is strong winds from north-westerly directions, often related to intense extra-tropical cyclones travelling from the North Atlantic into the North Sea region.

Making use of an objective, impact-oriented identification and tracking scheme, we analyse storm events related to storm surges in the German Bight. This particular version of the tracking algorithm includes the so-called Storm Surge Severity Index (SSSI) and is used as a complementary tool in operational forecasting by the German Federal Maritime and Hydrographic Agency (BSH). The SSSI takes wind speed and direction into account and intends to quantify storm surge risk in the German Bight. However, to date, the SSSI has never been systematically evaluated for past storm surge events. To fill this gap and to prove that the SSSI can be used as a proxy for storm surge risk, we analyse the relationship between SSSI values of past storm events and the associated water levels recorded in the German Bight using ERA5 atmospheric reanalysis data. Moreover, we analyse potentially storm surge-relevant storms in a multi-model ensemble of global climate model simulations to assess potential future changes in storm surge risk in the German Bight.

How to cite: Schaffer, L., Becker, N., Schenk, L., Hinrichs, C., Ditzinger, G., Schade, N. H., Befort, D. J., and Kruschke, T.: Objective assessment of storm surge risk in the German Bight – historical events and future climate change, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7236, https://doi.org/10.5194/egusphere-egu23-7236, 2023.

EGU23-8826 | ECS | Orals | AS1.14

Global climatology of cyclone clustering in present and future climates 

Chris Weijenborg, Thomas Spengler, and Matthew Priestley

Cyclone clustering, the swift succession of multiple extratropical cyclones in a geographically confined region during a short period of time, constitutes a large fraction of European weather extremes. The idea that several cyclones follow a similar track dates back to the centennial concept of cyclone families of Bjerknes and Solberg. To investigate the dynamical causes of cyclone clustering, it is necessary to diagnose the occurrence of cyclone clustering and to determine their characteristics. So far, most diagnostics focused either on local impact or on a statistical analysis of storm recurrence. While the first cannot be applied globally, the latter is difficult to relate to individual events. We therefore use a novel method to globally detect cyclone clustering that is closer to the original concept of Bjerknes and Solberg, where extratropical cyclones follow similar tracks within a given time period.

Using this novel cyclone clustering diagnostic based on spatio-temporal distance between cyclone tracks, we analyse cyclone clustering globally in Era-Interim for the period 1979 until 2016 as well as for 10 CMIP6 models. We separate the cyclone clusters into two types: one representing the ‘classical’ bjerknes-type clusters, and one representing more stationary clusters. We find that cyclone clustering mainly occurs along the climatological storm tracks, with the bjerknes-type more common at the western side of the storm tracks, while the stationary-type of cyclone clusters occurs more downstream. In general, clustered cyclones are stronger than non-clustered cyclones. While CMIP6 models feature a slight bias towards an equatorward shift of the storm tracks, cyclone clustering in a future climate occurs more poleward. Furthermore, the average number of storms per cluster decreases in a future climate, though the mean intensity of the cyclones that are clustered increases slightly.

How to cite: Weijenborg, C., Spengler, T., and Priestley, M.: Global climatology of cyclone clustering in present and future climates, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8826, https://doi.org/10.5194/egusphere-egu23-8826, 2023.

EGU23-9393 | ECS | Orals | AS1.14

Growing Pacific Linkage with Western North Atlantic Explosive Cyclones 

Jacob Stuivenvolt-Allen, Simon S.-Y. Wang, Yoshimitsu Chikamoto, Jonathan Meyer, and Zachary Johnson

Explosive cyclones (ECs), defined as developing extratropical cyclones that experience pressure drops of at least 24 hPa in 24 hours, are impactful weather events which occur along highly populated coastal regions in the eastern United States. These storms occur due to a combination of atmospheric and surface processes, such as jet stream intensification and latent heat release. Even though previous literature has elucidated the role of these processes in EC formation, the sources of interannual variability that impact seasonal EC frequency are not well known. To analyze the sources of interannual variability, we track cases of ECs and dissect them into two spatial groups: those that formed near the east coast of North America (coastal) and those in the North Central Atlantic (high latitude). The frequency of high-latitude ECs is strongly correlated with the North Atlantic Oscillation, a well-known feature, whereas coastal EC frequency exhibits a growing relationship with an atmospheric wave-train emanating from the North Pacific in the last 30 years. This wave-train pattern of alternating high-and-low pressure resulted in heightened upper-level divergence and baroclinic instability along the east coast of North America. Using a coupled model experiment, we show that the tropical Pacific Ocean and North Pacific oceans are the main driver of this atmospheric wave train and the subsequent enhancement seasonal baroclinic instability in the North Atlantic.

How to cite: Stuivenvolt-Allen, J., Wang, S. S.-Y., Chikamoto, Y., Meyer, J., and Johnson, Z.: Growing Pacific Linkage with Western North Atlantic Explosive Cyclones, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9393, https://doi.org/10.5194/egusphere-egu23-9393, 2023.

EGU23-9411 | ECS | Posters on site | AS1.14

Explosive Cyclones in the Mediterranean Sea exploiting ERA5 dataset: detection, classification, statistical and synoptic analysis of their occurrance 

Cosimo Enrico Carniel, Rossella Ferretti, Antonio Ricchi, Gabriele Curci, Mario Marcello Miglietta, Marco Reale, Piero Serafini, Evan David Wellmeyer, and Dino Zardi

In the semi-enclosed basin of the Mediterranean Sea, a wide variety of cyclone mechanisms are known to develop, including baroclinic waves coming from the Atlantic, Mediterranean cyclones originating from the cut-off of baroclinic waves, Warm Seclusions, Tropical-Like Cyclones (TLC), Rapid-Cyclogeneses (RC) and Intense Mediterranean Cyclones (IMC). Depending on the cyclone's type, the characteristic frequency of appearance can vary, ranging from tens per month to around 1-1.5 per year, as in the TLC case. RCs are among the rarest and probably most intense and destructive cyclone events that can develop in nature; they usually originate at high latitudes, during wintertime, and mainly over the sea, preferring areas with high Sea Surface Temperature (SST) gradients. It is generally accepted that these events are described by quick drop of pressure, close to 1hPa/hr for 24 hours, within the eye of the cyclone. Several recent studies investigated the formation of RC’s over Mediterranean Basin (MB). RCs formation is an extremely complicated process, and in the MB  it is mostly driven by dry air intrusions from the stratosphere and by the trigger of Atmospheric Rivers.

Using ERA5 dataset, we firstly conducted a physical and dynamical analysis of the most intense cyclone events occurred in the Mediterranean basin in the period 1979-2020, identifying factors which triggered, generated and contributed to the intensification of such events. According to Sanders’ and Gyakum’s definition of Bergeron, a parameter which describes RCs’ deepening rate and varies from 28mb/(24h) at the pole to 12 mb/(24h) at latitude 25°N, we were able to classify them in the three aforementioned categories. With the help of EOF analysis, we outlined synoptic configuration more likely to drive the phenomena, highlighting the role of SCAND index and NAO-. Moreover, we have investigated the deepening with a new promising approach involving the use of 6 hours timespans, in order to single out the cyclones with higher gradients of pressure and faster evolution in semi enclosed basins. Further analysis is being undertaken to determine the cyclones’ phase and their main morphological characteristics, as well as their correlation with atmospheric rivers and SST anomalies exhibited by the Central Mediterranean Basin.

How to cite: Carniel, C. E., Ferretti, R., Ricchi, A., Curci, G., Miglietta, M. M., Reale, M., Serafini, P., Wellmeyer, E. D., and Zardi, D.: Explosive Cyclones in the Mediterranean Sea exploiting ERA5 dataset: detection, classification, statistical and synoptic analysis of their occurrance, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9411, https://doi.org/10.5194/egusphere-egu23-9411, 2023.

EGU23-10041 | ECS | Posters on site | AS1.14

Tropical and extratropical circulation biases and the Southern Hemisphere Hadley cell width 

Pia Freisen, Julie Arblaster, Christian Jakob, and José Rodriguez

The widening of the Southern Hemisphere tropical meridional circulation has been attributed to various forcings from increased greenhouse gases, ozone depletion and natural variability. While climate models can reproduce some characteristics of this observed change, there is some uncertainty in the operating mechanisms and driving regions setting the edge of the tropical circulation. Here we examine the impacts of systematic model biases of the atmosphere-only Unified Model onto the simulation of the Southern Hemisphere tropical extent. We utilise nudging experiments with prescribed sea-surface temperatures, where potential temperature and horizontal winds are relaxed back to reanalysis for a 20-year period. Specifically, experiments with regionally-defined bias correction aide to determine the influence of remote model biases on the tropical width. The experiments are applied to different tropical width metrics previously identified to measure the boundary between the tropical to extratropical circulation. We uncover a more consistent improvement of the location of the Hadley cell edge by correcting Southern Hemisphere extratropical circulation biases, than tropical ones. The analysis is further expanded to the range of atmosphere-only model simulations of the Coupled Model Intercomparison Project Phase 6 (CMIP6). We explore the relationships between tropical and extratropical biases and the models’ representation of the Hadley cell.

How to cite: Freisen, P., Arblaster, J., Jakob, C., and Rodriguez, J.: Tropical and extratropical circulation biases and the Southern Hemisphere Hadley cell width, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10041, https://doi.org/10.5194/egusphere-egu23-10041, 2023.

EGU23-10466 | Posters on site | AS1.14

Extratropical storm track activity change in future climate change scenarios 

Ui-Yong Byun, Eun-Chul Chang, Joowan Kim, Donghyun Cha, Joong-Bae Ahn, and Seung-Ki Min

In the mid-latitudes, synoptic-scale phenomena like high and low-pressure systems generate the variability of the regional-scale weather system. To identify the weather variability of extra-tropical region storm track activity has been analyzed based on observations since the mid-nineteenth century. After early-stage research that directly counted the movement of cyclones, the time filtering method based on grid analysis has been used for an isolated disturbance with periods of 2~7 days. This bandpass filtering method has the advantage of being able to examine the distribution and the variability of the storm track spatially in vertical and horizontal space.

In this study, we confirm the storm track activity in the East Asia region using the dynamical down-scale results from CORDEX (COordinated Regional climate Downscaling EXperiment) East Asia projects. We verify the reproducibility and confirm the temporal change in the storm track activity from various RCM data. In addition to the historical period, we examine the difference in storm track intensity over future climate change scenarios. Through this, we also discuss the role of added value from RCM.

 

This work was funded by the Korea Meteorological Administration Research and Development Program under Grant KMI2022-01210.

How to cite: Byun, U.-Y., Chang, E.-C., Kim, J., Cha, D., Ahn, J.-B., and Min, S.-K.: Extratropical storm track activity change in future climate change scenarios, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10466, https://doi.org/10.5194/egusphere-egu23-10466, 2023.

EGU23-10857 | ECS | Posters on site | AS1.14

An assessment of extreme precipitation within cyclone composites using ERA5 

Cameron McErlich, Adrian McDonald, and James Renwick

Extra-tropical cyclones are key components of the atmospheric general circulation due to their ability to transport large quantities of heat, moisture, and momentum. Cyclones are an important contributor to extreme weather as their passage is associated with strong winds, and large precipitation accumulations. Here we connect a cyclone compositing scheme with regionally derived distributions of precipitation to present a framework for classifying spatially dependent extremes relative to the cyclone centre. Using this framework, cyclone composites for both average (50th percentile) and extreme (90th and 98th percentile) precipitation are derived from ERA5 reanalysis output. Composites are then partitioned into different stages of the cyclone lifecycle to assess the spatial and temporal evolution of precipitation extremes. We find that most extreme precipitation occurs within the comma-cloud structure close to the cyclone centre, with the extreme precipitation occurrence and intensity occurring in that region. Extreme precipitation is also identified to be largest during the period of deepening before the maximum cyclone intensity is reached. These regions of the cyclone correspond to places where large fractions of precipitation are above the extreme threshold. Strong spatial correlation are also seen between the average and extreme precipitation during the deepening phase for the precipitation mean, occurrence and fraction. This correlation weakens as the cyclone evolves and as the threshold used to determine extreme precipitation increases.

How to cite: McErlich, C., McDonald, A., and Renwick, J.: An assessment of extreme precipitation within cyclone composites using ERA5, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10857, https://doi.org/10.5194/egusphere-egu23-10857, 2023.

EGU23-12391 | ECS | Posters on site | AS1.14

High-resolution loss modeling for European Windstorms 

Dhirendra Kumar, Len Shaffrey, Richard Dixon, Hannah Bloomfield, Paul Bates, and John Hillier

European windstorms are a frequent and damaging natural hazard that can cause loss of human life and damage to property and infrastructure. As there is a high degree of uncertainty in climate projections, it is crucial to understand the physical risks and economic losses at regional and local scales associated with European Windstorms. In this study, we develop a simple model to estimate historical windstorm losses over the European region. The model uses winds from the ERA5 reanalysis and different exposure datasets based on countrywide total insured property values, gross domestic product, and historical population density.

We find that the estimated losses associated with major historical storms in North-western Europe and estimated average EU-wide losses are comparable to the reported estimates and those from propriety vendor models. However, estimated losses from windstorms in France and Germany are lower than reported. Differences in the estimated losses are attributed to the contrasts in the regional-level exposure within and between different exposure datasets. We also tested the sensitivity of regional-level vulnerabilities and find that accounting for regional-level vulnerability differences slightly improves the biases in countrywide losses. Further, we also find that the major contribution to the estimated losses comes from the United Kingdom, France, and Germany for most of the storm seasons, and thus it is important to correctly represent the exposure and vulnerabilities over these countries. The ability of the model to estimate reported losses is also limited by the representation of the winds in ERA5, which has limited skill in representing the hazard footprint, especially for specific storms such as the Great October Storm of 1987.

Keywords: Losses, Windstorms, Climate Change, Natural Hazards

How to cite: Kumar, D., Shaffrey, L., Dixon, R., Bloomfield, H., Bates, P., and Hillier, J.: High-resolution loss modeling for European Windstorms, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12391, https://doi.org/10.5194/egusphere-egu23-12391, 2023.

EGU23-12526 | ECS | Posters virtual | AS1.14

Volcanically induced increase in extra-tropical cyclone frequency 

Laurits Andreasen, Joona Corner, Peter Abbott, Victoria Sinclair, Felix Riede, and Claudia Timmreck

Volcanic eruptions are well known to influence Earth's temperature, however, how eruptions influence the atmosphere's circulation pattern, especially on the scale of everyday weather is poorly understood. Changing Earth's temperature can affect temperature gradients which in turn could affect baroclinicity and hence high- and mid-latitude weather. Yet, to what extent volcanic eruptions do in fact exert  such an influence is not clear.

To answer this, we followed two independent lines of investigation: First, we query the Greenland ice-core proxy record for Indications of increased extra-tropical cyclone frequency that correlates with evidence for volcanism. This is done by comparing the storm proxy sea salt (a substance transported to the ice sheet by wind)  with the volcanological proxy sulfur. Secondly, we simulate eruptions with the MPI-ESM1.2 Earth System Model and use the TRACK algorithm to explore how extra-tropical cyclone frequency is affected in the model  experiments. Both approaches suggest that volcanic eruptions impact high- and mid-latitude weather by increasing the number of extra-tropical cyclones especially at higher latitudes. A detailed interrogation of the simulated eruption scenarios suggests that this increase in cyclone frequency is associated with features such as an increase in isentropic slopes and sea-ice extent most commonly found under  colder climate regimes and is the reverse of what one finds in more equable climates such as that projected for the future.

How to cite: Andreasen, L., Corner, J., Abbott, P., Sinclair, V., Riede, F., and Timmreck, C.: Volcanically induced increase in extra-tropical cyclone frequency, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12526, https://doi.org/10.5194/egusphere-egu23-12526, 2023.

EGU23-13180 | ECS | Posters on site | AS1.14

Drivers of large footprints of extreme winds and rainfall and their projected future changes 

Colin Manning, Elizabeth Kendon, Hayley J. Fowler, Jennifer L. Catto, Steven C. Chan, and Philip Sansom

Extratropical cyclones produce extreme surface wind speeds and heavy rainfall which can individually and jointly influence impacts and potentially produce large aggregate impacts. Within this study, we assess the UKCP 12-member ensemble of local convection-permitting 2.2 km climate projections. We quantify the likelihood of cyclones producing large footprints of both extreme winds and rainfall over the UK in a control (1981-2000) and future (2061-2080, RCP8.5) climate simulation. Following this, we characterise the convective and frontal drivers of wet and windy conditions within cyclones, and identify the characteristics of cyclones, their tracks and interactions with the jet stream that contribute to the occurrence of large, combined footprints in the control and future simulations. The future simulations project an increased probability of extratropical cyclones producing extremely wet and windy conditions in the same storm, as well as an increase in the land area covered by such conditions. In both the control and future simulations, combined wet and windy extremes largely occur close to cold and warm fronts, likely due to the warm conveyor belt which produces heavy rainfall (due its ascent over the frontal boundaries) and high winds (when occurring within a region of tight pressure gradients). Cyclone composites reveal that the largest changes in joint extremes are closely located within the sector of cyclones where we expect to see the warm conveyor belt, suggesting their change arises partly through the response of this shared driver rather than being a simple consequence of increased rainfall due to thermodynamics. In further analysis, we identify favourable conditions and cyclone characteristics that lead to cyclones producing large rainfall and wind footprints over the UK.

How to cite: Manning, C., Kendon, E., Fowler, H. J., Catto, J. L., Chan, S. C., and Sansom, P.: Drivers of large footprints of extreme winds and rainfall and their projected future changes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13180, https://doi.org/10.5194/egusphere-egu23-13180, 2023.

EGU23-13914 | Posters on site | AS1.14

Decadal variability of extreme winds and potential storm losses in Europe using large RCM ensembles 

Jisesh Sethunadh, Joaquim G. Pinto, Patrick Ludwig, Hendrik Feldmann, and Florian Ehmele

Windstorms (major winter storms) are one of the most important natural hazards in Europe. Despite the large observed socioeconomic losses, the impact of windstorms and its decadal variability is not yet fully understood. This study aims to assess the loss potentials associated with European windstorms and the variability in the wind speed climatology across Europe. We use the 12,500-years LAERTES-EU (LArge Ensemble of Regional climaTe modEl Simulations for EUrope) RCM ensemble to study the spatio-temporal distribution and variability of windstorms over Europe. LAERTES-EU is validated against reanalysis data (ERA5) and available ground-based station observations. The associated windstorm losses are estimated by computing statistics of extreme wind speeds and related indices. Different loss indices are validated using historical loss data from the insurance sector. The results reveal that the loss index (LI) is a good proxy for the estimation of potential losses associated with windstorms across Europe in winter. The derived statistics of extreme windstorms such as return periods (RP) show hardly any change in the severity and frequency of windstorms during the covered period 1900-2028, but a strong decadal variability is apparent.

How to cite: Sethunadh, J., Pinto, J. G., Ludwig, P., Feldmann, H., and Ehmele, F.: Decadal variability of extreme winds and potential storm losses in Europe using large RCM ensembles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13914, https://doi.org/10.5194/egusphere-egu23-13914, 2023.

EGU23-13929 | ECS | Posters on site | AS1.14

European windstorm risk at the regional scale under recent and future climate conditions 

Inovasita Alifdini, Julia Moemken, and Joaquim G. Pinto

European windstorms are among the natural hazards with the highest economic losses. We investigate the impact of European windstorms under recent and future climate conditions at high spatial resolution. With this aim, we use hourly surface wind data at 30 km resolution from ERA5 reanalysis for 1959-2021, and 3-hourly surface wind data at 12.5 km resolution from 60 different global-to-regional climate model (GCM-RCM) chains from EURO-CORDEX (EUR-11). The windstorm activity is compared in 30-year periods from the historical events (1976-2005) to the future events (under RCP8.5 scenario) at global warming levels (GWL) of +2°C and +3°C.  We apply different indices (meteorological index and loss index) to quantify the severity of windstorms and to estimate the corresponding impacts. For the historical period, storm Wiebke in 1990 (storm names as used by the German Weather Service DWD) caused the highest loss for Central Europe, followed by storm Lothar in 1999. The United Kingdom and Germany are countries in Central Europe that have the highest loss index (more vulnerable to the European windstorms). The results from the EURO-CORDEX ensemble show only small changes in windstorm activity between the historical period and the different GWLs, but display decadal variability.

How to cite: Alifdini, I., Moemken, J., and Pinto, J. G.: European windstorm risk at the regional scale under recent and future climate conditions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13929, https://doi.org/10.5194/egusphere-egu23-13929, 2023.

EGU23-14410 | ECS | Posters on site | AS1.14

Estimating worst-case European windstroms, and worst-case seasons, using seasonal forecasts. 

Jacob Maddison, Jennifer Catto, Stefan Siegert, and Sandra Hansen

Windstorms pose continual risk to Europe. Among their associated hazards, strong near-surface winds can be particularly damaging, threatening infrastructure, life and billions of pounds in insured losses. Insurers (and reinsurers) therefore need to prepare for the potential cost of extreme windstorms. Storm severity indices (SSIs) have been developed to quantify the potential losses associated with windstorm winds. Here, the most extreme windstorms that could potentially occur in the current climate are estimated using seasonal forecast data together with a cyclone-tracking algorithm, and their potential losses quantified using an SSI. As maximum wind gusts, the typical input variable for SSIs, are not available in the seasonal forecast dataset, a method is developed to calculate SSIs using wind speed data and a bias correction used to convert to SSI values representative of those obtained when calculated using wind gusts. Nearly 700 extended winter seasons of forecast data are analysed, representing a much larger sample of potential windstorms compared to that available from reanalysis or observational products. The storm track is reasonably well represented in the seasonal forecast data: spatial features are similar to those in a reanalysis, but there exists a slight poleward bias and underestimation of number of storms per season (maximal underestimation of around 10%). Additionally, distributions of SSI values for several countries in Europe are similar in the forecast data and reanalysis. Together, these suggest that the seasonal forecast data is suitable for analysing windstorm statistics and informing on potential extreme storms. We give estimates of worst-case storms, and worst-case seasons, that are identified in the forecast data and compare to those seen in a reanalysis, highlighting the potential insurance loss implications.

How to cite: Maddison, J., Catto, J., Siegert, S., and Hansen, S.: Estimating worst-case European windstroms, and worst-case seasons, using seasonal forecasts., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14410, https://doi.org/10.5194/egusphere-egu23-14410, 2023.

EGU23-14446 | ECS | Orals | AS1.14

A framework for understanding the correlation between aggregated losses of compound events 

Toby Jones, David Stephenson, and Matthew Priestley

The risk from individual natural hazards (such as extratropical cyclones) can be large, but the aggregate loss over yearly timescales is significantly greater. For example, wind damage from the three major European windstorms in February 2022 caused more than €3.5 billion of insured losses.

This study proposes a random sum modelling framework for understanding the correlation between aggregate risks that occur from compound events. By considering the frequency and intensities of compound events as random variables, the framework provides an expression for correlation between two random sums (which each represent different types of loss from compound events).

The framework shows that this correlation will generally increase monotonically towards one as the dispersion (clustering) of the number of events increases. Under certain conditions, the correlation will always monotonically increase with dispersion.

The framework has been illustrated by applying it to annual sums from 1980-2020 using wind speed and precipitation as proxy measures for insured loss. This is calculated from ERA5 reanalysis data which includes 39587 storm events and covers the European region and Atlantic Ocean (from 30°N 100°W to 75°N 40°E).

The framework performs well, capturing the general behaviour of the correlation, with large positive correlation over the N. Atlantic Ocean and weaker correlations over European land regions.

How to cite: Jones, T., Stephenson, D., and Priestley, M.: A framework for understanding the correlation between aggregated losses of compound events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14446, https://doi.org/10.5194/egusphere-egu23-14446, 2023.

EGU23-14695 | Posters on site | AS1.14

Assessing the boundaries of seasonal forecast skill for European winter storms from different hindcast suites 

Gregor C. Leckebusch, Lisa Degenhardt, Elleanor Berrie, Kelvin S. Ng, and Elisa Spreitzer

European winter storms are a significant threat to communities, public infrastructure, and private and commercial properties. On seasonal timescales, potential predictability was evidenced in recent state-of-the-art seasonal hindcast suites e.g., the UK Met Office’s GloSea5. Related positive and potentially usable forecast skill for frequency and intensity measures were based on pre-season model initialisation around the beginning of November for the following core winter (DJF) season’s assessment.

This study expands on these findings by analysing extended lead times of seasonal forecast into autumn and late summer before the winter season. Here, in a systematic way, a multi-model ensemble of hindcasts is analysed to evaluate current models’ capability to forecast the seasonal activity for initialisations from September to November. First results indicate potential predictability precursors already from the September initialisations for storm frequencies. These results vary from model to model though. The presentation will discuss differences between models as well as lead times for both, storm frequency and intensity.

How to cite: Leckebusch, G. C., Degenhardt, L., Berrie, E., Ng, K. S., and Spreitzer, E.: Assessing the boundaries of seasonal forecast skill for European winter storms from different hindcast suites, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14695, https://doi.org/10.5194/egusphere-egu23-14695, 2023.

EGU23-408 | ECS | Posters on site | CL2.2

El Niño Southern Oscillation influence over the Orinoco low-level jet variability 

Alejandro Builes, Johanna Yepes, and Hernán D. Salas

We studied the most active season of the Orinoco Low-Level jet (OLLJ), December-January-February (DJF), during the El Niño-Southern Oscillation canonical phases, El Niño and La Niña. In particular, we studied the occurrence days of the jet in each month, wind speed, moisture transport and precipitation over northern south America. In terms of the occurrence of the OLLJ, during El Niño in January, the jet exhibits its highest reduction with changes up to 24% in the eastern Colombian plains. On the contrary, during La Niña, the jet exhibits an increase between 6–16% in the frequency of occurrence mainly located in the eastern Colombian plains and the border between Colombia, Ecuador and Peru. Although the diurnal cycle of the OLLJ windspeed remains unaltered during the ENSO phases the maximum decrease (increase) up to -2m/s (up to 1 m/s) during El Niño (La Niña). Regarding moisture transport there is a gradual reduction during the season in both ENSO phases reaching up to 18 gm-1 kgm-1 during El Niño, and the precipitation also shows a reduction of around 5 mm/day. In conclusion, during DJF at the ENSO canonical phases the OLLJ shows changes in its occurrence along the jet corridor, and the region experiences changes in both moisture transport and precipitation.

How to cite: Builes, A., Yepes, J., and Salas, H. D.: El Niño Southern Oscillation influence over the Orinoco low-level jet variability, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-408, https://doi.org/10.5194/egusphere-egu23-408, 2023.

EGU23-410 | Orals | CL2.2

Phase-Locking between precipitation and El Niño-Southern Oscillation over northern South America 

Hernán D. Salas, Germán Poveda, Óscar J. Mesa, Alejandro Builes-Jaramillo, Niklas Boers, and Jürgen Kurths

We study phase-locking between the El Niño - Southern Oscillation (ENSO) and precipitation at inter-annual time scales over northern South America. To this end, we characterize the seasonality of the regional patterns of sea surface temperature, surface pressure levels, and precipitation anomalies associated with the states of the canonical ENSO. We find that the positive (negative) precipitation anomalies experienced in northern South America differ from those previously reported in the literature in some continental regions. In particular, the Orinoco Low-level Jet corridor separates two regions with negative (positive) rainfall anomalies during El Niño (La Niña), which are located in the Guianas (northeastern Amazon) and the Caribbean. Moreover, we show that the ENSO signal is phase-locked with the inter-annual rainfall variability in most of the study regions although some areas exhibit phase-locking without a significant change in the anomalies of precipitation. This suggests that ENSO could induce changes only in terms of phases and not so in terms of magnitude. This work provides new insights into the non-linear interactions between ENSO and hydro-climatic processes over the tropical Americas.

How to cite: Salas, H. D., Poveda, G., Mesa, Ó. J., Builes-Jaramillo, A., Boers, N., and Kurths, J.: Phase-Locking between precipitation and El Niño-Southern Oscillation over northern South America, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-410, https://doi.org/10.5194/egusphere-egu23-410, 2023.

EGU23-1522 | ECS | Orals | CL2.2

Future climate response to observed extreme El Niño analogues 

Paloma Trascasa-Castro, Yohan Ruprich-Robert, and Amanda Maycock

Model simulations show a robust increase in ENSO-related precipitation variability in a warmer climate, but there remains uncertainty in whether the characteristics of ENSO events themselves may change in the future. Our study aims to disentangle these effects by addressing how the global impacts of observed large El Niño events would change in different background climate states covering the preindustrial, present and future periods.

Pacemaker simulations with the EC-Earth3-CC model were performed replaying the 3 strongest observed El Niño events from the historical record (1982/83, 1997/98, 2015/16). Model tropical Pacific sea surface temperature (SST) anomalies were restored towards observations, while imposing different background states, mimicking past, present and future climate conditions (following the SSP2-4.5). All variables outside the restoring region evolve freely in a coupled-atmosphere ocean transient simulation. For each start date, 30 ensemble members with different initial conditions were run for 2 years. Using this approach we ask ‘what impacts would arise if the observed El Niño occurred in the past or future’?

In response to the same imposed El Niño SST anomalies, precipitation anomalies are shifted towards the Eastern equatorial Pacific in the future compared to the present day, leading to changes in the extratropical response to El Niño. Some examples are an amplification of the surface temperature response over north-eastern North America, northern South America and Australia in boreal winter. We link the changes of El Niño related tropical Pacific precipitation to a decrease in the climatological zonal SST gradient in the equatorial Pacific, as we move from past to future climatologies, which potentially leads to a higher convection sensitivity to SST anomalies over the Central and Eastern equatorial Pacific in the future. Interestingly, the simulations indicate there has already been an intensification of El Niño impacts between present day and preindustrial, which is comparable to the differences found between future and present. This nonlinear behaviour highlights the need to understand potential changes to convection thresholds in the tropical Pacific to be able to explain El Niño teleconnections under climate change scenarios. Ongoing work is exploring the changes in atmospheric circulation that lead to the overall intensification of El Niño impacts that we show in our study.

How to cite: Trascasa-Castro, P., Ruprich-Robert, Y., and Maycock, A.: Future climate response to observed extreme El Niño analogues, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1522, https://doi.org/10.5194/egusphere-egu23-1522, 2023.

EGU23-1960 | Posters on site | CL2.2

Two regimes of inter-basin interactions between the Atlantic and Pacific Oceans on interannual timescales 

Jae-Heung Park, Sang-Wook Yeh, Jong-Seong Kug, Young-Mean Yang, Hyun-Su Jo, Hyo-Jeong Kim, and Soon-Il An

Understanding the inter-basin interactions between the Atlantic and Pacific Oceans is of great concern due to their substantial global climatic implications. By analyzing observational reanalysis datasets (1948-2020), we found that there are two regimes in Atlantic–Pacific inter-basin interactions: (i) the Pacific-driven regime, and (ii) the Atlantic-driven regime. In the Pacific-driven regime before the mid-1980s, the El Niño-Southern Oscillation (ENSO) in winter effectively drives the primary mode of sea surface temperature anomaly (SSTA) in the tropical Atlantic (i.e., NTA mode) in boreal spring. The NTA mode has a meridional contrast of SSTA along the Atlantic Intertropical convergence zone due to the ENSO effect, similar to the Atlantic Meridional Mode. Whereas, in the Atlantic-driven regime after the mid-1980s, the ENSO effect on the NTA becomes remarkably weaker, so that the NTA mode is featured with a SSTA monopole. Notably, the NTA mode without the meridional contrast of SSTA is capable of modulating an ENSO event. Our analyses of the latest climate models participating in the Coupled Model Intercomparison Project (CMIP) phases 6 support the hypothesis that the two regimes engendered by the Atlantic-Pacific inter-basin interactions are likely due to natural variability.

How to cite: Park, J.-H., Yeh, S.-W., Kug, J.-S., Yang, Y.-M., Jo, H.-S., Kim, H.-J., and An, S.-I.: Two regimes of inter-basin interactions between the Atlantic and Pacific Oceans on interannual timescales, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1960, https://doi.org/10.5194/egusphere-egu23-1960, 2023.

EGU23-2136 | ECS | Posters on site | CL2.2

A multi-modal representation of El-Niño Southern Oscillation Diversity 

Jakob Schlör, Antonietta Capotondi, and Bedartha Goswami

Sea surface temperature anomalies (SSTA) associated with the El-Niño Southern Oscillation (ENSO) show strong event-to-event variability, known as ENSO diversity. El Niño and La Niña events are typically divided into Eastern Pacific (EP) and Central Pacific (CP) types based on the zonal location of peak SSTA. The separation of these types is usually based on temperature differences between pairs of predefined indices, such as averages over boxes in the Eastern and Central Pacific or the two leading Principal Components of tropical SSTA. 
Using results from unsupervised learning of SSTA data, we argue that ENSO diversity is not well described by distinctly separate classes but rather forms a continuum with events grouping into "soft'' clusters. We apply a Gaussian mixture model (GMM) to a low-dimensional projection of tropical SSTA to describe the multi-modal distribution of ENSO events. We find that El-Niño events are best described by three overlapping clusters while La-Niña events only show two "soft'' clusters. The three El-Niño clusters are described by i) maximum SSTA in the CP, ii) maximum SSTA in the EP, and iii) strong basin-wide warming of SSTA which we refer to as the "super El-Niño'' cluster. The "soft'' clusters of La-Niña correspond to i) anomalous cool SST in the CP and ii) anomalously cool SST in the EP. We estimate the probability that a given ENSO event belongs to a chosen cluster and use these probabilities as weights for estimating averages of atmospheric variables corresponding to each cluster. These weighted composites show qualitatively similar patterns to the typically used averages over EP and CP events. However, the weighted composites show a higher signal-to-noise ratio in the mid-latitudes for the "super El-Niño'' events. 
We further apply our approach to CESM2 model data and discuss the potential of GMM clustering for evaluating how well ENSO diversity is captured in Global Circulation models.

How to cite: Schlör, J., Capotondi, A., and Goswami, B.: A multi-modal representation of El-Niño Southern Oscillation Diversity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2136, https://doi.org/10.5194/egusphere-egu23-2136, 2023.

An information theory based framework is developed to assess the predictability of the ENSO complexity, which includes different types of the ENSO events with diverse characteristics in spatial patterns, peak intensities and temporal evolutions. The information theory advances a unique way to quantify the forecast uncertainty and allows to distinguish the predictability limit of each type of event. With the assistance of a recently developed multiscale stochastic conceptual model that succeeds in capturing both the large-scale dynamics and many crucial statistical properties of the observed ENSO complexity, it is shown that different ENSO events possess very distinct predictability limits. Beyond the ensemble mean value, the spread of the ensemble members also has remarkable contributions to the predictability. Specifically, while the result indicates that predicting the onset of the eastern Pacific (EP) El Ninos is challenging, it reveals a universal tendency to convert strong predictability to skillful forecast for predicting many central Pacific (CP) El Ninos about two years in advance. In addition, strong predictability is found for the La Nina events, corresponding to the effectiveness of the El Nino to La Nina transitions. In the climate change scenario with the strengthening of the background Walker circulation, the predictability of sea surface temperature in the CP region has a significant response with a notable increase in summer and fall. Finally, the Gaussian approximation exhibits to be accurate in computing the information gain, which facilitates the use of more sophisticated models to study the ENSO predictability.

How to cite: Fang, X. and Chen, N.: Quantifying the Predictability of ENSO Complexity Using a Statistically Accurate Multiscale Stochastic Model and Information Theory, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2209, https://doi.org/10.5194/egusphere-egu23-2209, 2023.

EGU23-2470 | ECS | Orals | CL2.2

The Dynamics of the El-Niño Southern Oscillation (ENSO) Diversity 

Priyamvada Priya, Dietmar Dommenget, and Shayne McGregor

This study investigates the observed El-Niño Southern Oscillation (ENSO) dynamics for the eastern Pacific (EP) and central Pacific (CP) events. Here we use the recharge oscillator (ReOsc) model concept to describe the ENSO phase space, based on the interaction of sea surface temperatures in the eastern equatorial Pacific (T) and thermocline depth (h), for the different types of ENSO events. We further look at some important statistical characteristics, such as power spectrum and cross-correlation, as essential parameters for understanding the dynamics of ENSO. The results show that the CP and EP events are very different in the ENSO phase space and less well described by the ReOsc model than a T index-based model. The EP events are closer to the idealised ReOsc model, with clear propagation through all phases of the ENSO cycle and strongly skewed towards the El-Niño and subsurface ocean heat discharge states. The CP events, in turn, do not have a clear propagation through all phases and are strongly skewed towards the La-Nina state. Also, the CP events have a slower cycle (67 months) than the EP events (50 months). Further, the CP events collapse after the La-Nina phase, whereas the EP events appear to collapse after the discharging phase. The characteristics out-of-phase cross-correlation between T and h is nearly absent for the CP events, suggesting that the interaction between T and h is not as important as for the EP or the canonical ENSO events. Furthermore, the coupling factor of T and h is smaller for the CP events than the EP events, implying that the CP events are not influenced much by T and h interactions. This study will provide new insight to understand these events by developing a dynamical approach to explain the observed ENSO dynamics for the EP and CP events in the ReOsc model framework.

How to cite: Priya, P., Dommenget, D., and McGregor, S.: The Dynamics of the El-Niño Southern Oscillation (ENSO) Diversity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2470, https://doi.org/10.5194/egusphere-egu23-2470, 2023.

EGU23-2477 | Posters on site | CL2.2

ENSO phase space dynamics with an improved estimate of the thermocline depth 

Dietmar Dommenget and Priyamvada Priya

The recharge oscillator model of the El Niño Southern Oscillation (ENSO) describes the ENSO dynamics as an interaction and oscillation between the eastern tropical Pacific sea surface temperatures (T) and subsurface heat content (thermocline depth; h), describing a cycle of ENSO phases. h is often approximated on the basis of the depth of the 20oC isotherm (Z20). In this study we will address how the estimation of h affects the representation of ENSO dynamics. We will compare the ENSO phase space with h estimated based on Z20 and based on the maximum gradient in the temperature profile (Zmxg). The results illustrate that the ENSO phase space is much closer to the idealised recharge oscillator model if based on Zmxg than if based on Z20. Using linear and non-linear recharge oscillator models fitted to the observed data illustrates that the Z20 estimate leads to artificial phase dependent structures in the ENSO phase space, which result from an in-phase correlation between h and T. Based on the Zmxg estimate the ENSO phase space diagram show very clear non-linear aspects in growth rates and phase speeds. Based on this estimate we can describe the ENSO cycle dynamics as a non-linear cycle that grows during the recharge and El Nino state, and decays during the La Nina states. The most extreme ENSO states are during the El Nino and discharge states, while the La Nina and recharge states do not have extreme states. It further has faster phase speeds after the El Nino state and slower phase speeds during and after the La Nina states. The analysis suggests that the ENSO phase speed is significantly positive in all phases, suggesting that ENSO is indeed a cycle. However, the phase speeds are closest to zero during and after the La Nina state, indicating that the ENSO cycle is most likely to stall in these states.

How to cite: Dommenget, D. and Priya, P.: ENSO phase space dynamics with an improved estimate of the thermocline depth, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2477, https://doi.org/10.5194/egusphere-egu23-2477, 2023.

EGU23-3263 | ECS | Orals | CL2.2

Model Resolution Effects on ENSO and its Teleconnections 

Ned Williams, Adam Scaife, and James Screen

The El Niño-Southern Oscillation (ENSO) influences climate on a global scale and is a source of long-range predictability. Accurate modelling of the impact of ENSO requires accurate representation of teleconnections as well as of ENSO itself. We consider a set of CMIP6 models and assess the effect of increasing model resolution on ENSO and its boreal winter teleconnections. The spatial structure, strength and asymmetry of both ENSO and its teleconnection to the extratropical North Pacific are considered. We find evidence of an improved El Niño teleconnection in high resolution models, but this effect is weaker for La Niña. We aim to establish whether ocean or atmospheric resolution is the primary driver of resolution-based trends, and we evaluate the relevance of mean state biases on these trends. 

How to cite: Williams, N., Scaife, A., and Screen, J.: Model Resolution Effects on ENSO and its Teleconnections, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3263, https://doi.org/10.5194/egusphere-egu23-3263, 2023.

EGU23-3278 | ECS | Posters on site | CL2.2

Oceanic and Atmospheric Feedbacks Associated with the Spreading of Pacific Coastal Niño Events 

Daniel Rudloff and Joke Lübbecke

In early 2017 a very strong coastal warming occurred off the coast of Peru. This event, which caused heavy rainfalls and flooding over land, marked the strongest so called ‘Pacific Coastal Niño Event’ observed. Most intriguing about this event was the fact that the central Pacific was not showing any significant anomalies during that time. Since then several studies have investigated Pacific Coastal Niños but the exact mechanisms of how such events behave are still not clear. While most studies focus on their onset mechanisms, we here analyze their evolution and decay and in particular their connection to the central equatorial Pacific.

To address those questions, we are using the coupled climate model FOCI (Flexible Ocean Climate Infrastructure). Starting from a long control simulation with pre-industrial conditions we perform sets of 2-year long sensitivity experiments in which a coastal warming is generated by a local wind stress anomaly utilizing a partial coupling approach. Once the warming is initiated by reduced upwelling the wind forcing is switched off and the model can evolve freely, which enables us to investigate the evolution and decay of the warming. The approach allows to vary the forcing in strength, location and timing. By starting from different conditions in terms of equatorial heat content and applying the forcing during different months, the influences of both the background state of the equatorial Pacific during the Coastal Niño and the seasonality of the coastal warming are investigated. To understand which factors influence the spreading of the warm anomaly we analyze both local coastal feedbacks, which lead to an alongshore extension of the anomaly, and equatorial feedbacks that are crucial for a spreading along the equator.

How to cite: Rudloff, D. and Lübbecke, J.: Oceanic and Atmospheric Feedbacks Associated with the Spreading of Pacific Coastal Niño Events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3278, https://doi.org/10.5194/egusphere-egu23-3278, 2023.

EGU23-3440 | ECS | Posters on site | CL2.2

New insight into multi-year La Niña dynamics from the perspective of a near-annual ocean process 

Fangyu Liu, Wenjun Zhang, Fei-Fei Jin, Feng Jiang, Julien Boucharel, and Suqiong Hu

The El Niño-Southern Oscillation (ENSO) exhibits highly asymmetric temporal evolutions between its warm and cold phases. While El Niño events usually terminate rapidly after their mature phase and show an already established transition into the cold phase by the following summer, many La Niña events tend to persist throughout the second year and even re-intensify in the ensuing winter. While many mechanisms were proposed, no consensus has been reached yet and the essential physical processes responsible for the multi-year behavior of La Niña remain to be illustrated. Observations show that a unique ocean physical process operates during multi-year La Niña events. It is characterized by rapid double reversals of zonal ocean current anomalies in the equatorial Pacific which exhibits a fairly regular near-annual periodicity. Analyses of mixed-layer heat budget reveal comparable contributions of the thermocline and zonal advective feedbacks to the SST anomaly growth for the first year of multi-year La Niña events; however, the zonal advective feedback plays a dominant role in the re-intensification of La Niña events. Furthermore, the unique ocean process is identified to be closely associated with the preconditioning heat content state in the central to eastern equatorial Pacific before the first year of La Niña, which sets the stage for the future re-intensification of La Niña. The above-mentioned oceanic process can be largely reproduced by state-of-the-art climate models despite systematic underestimation, providing a potential predictability source for the multi-year La Niña events.

How to cite: Liu, F., Zhang, W., Jin, F.-F., Jiang, F., Boucharel, J., and Hu, S.: New insight into multi-year La Niña dynamics from the perspective of a near-annual ocean process, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3440, https://doi.org/10.5194/egusphere-egu23-3440, 2023.

EGU23-3598 | Orals | CL2.2 | Highlight

Prediction Challenges from Errors in Tropical Pacific Sea Surface Temperature Trends 

Michelle L'Heureux, Michael Tippett, and Wanqiu Wang

Initialized, monthly mean predictions of the tropical Pacific Ocean are made against the backdrop of a warming climate, and it is unclear to what extent these predictions are impacted by trends.  Here, we analyze the forecast models that comprise the North American Multi-Model Ensemble (NMME) and uncover significant linear trend errors that have consequences for the tropical Pacific basin and ENSO variability.  All models show positive trend errors over the eastern equatorial Pacific over the 1982-2020 hindcast and real-time period.  These positive trend errors interact with the mean bias of each respective model, reducing, over time, the bias of models that are too cold and increasing the bias of models that are too warm.  These trend errors lead to a tropical Pacific that is too warm and too wet over the basin, and is significantly correlated with an increase in El Niño false alarms.  Finally, we explore the consequences of these tropical Pacific Ocean trend errors on predictions of global precipitation anomalies. 

How to cite: L'Heureux, M., Tippett, M., and Wang, W.: Prediction Challenges from Errors in Tropical Pacific Sea Surface Temperature Trends, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3598, https://doi.org/10.5194/egusphere-egu23-3598, 2023.

EGU23-3631 | Posters on site | CL2.2

Multiyear ENSO dynamics as revealed in observations, CMIP6 models, and linear theory 

Tomoki Iwakiri and Masahiro Watanabe

El Niño–Southern Oscillation (ENSO) events occasionally recur one after the other in the same polarity, called multiyear ENSO. However, the dynamical processes are not well understood. This study aims to elucidate the unified mechanisms of multiyear ENSO using observations, CMIP6 models, and the theoretical linear recharge oscillator (RO) model. We found that multiyear El Niño and La Niña events are roughly symmetric except in some cases. The composite multiyear ENSO reveals that anomalous ocean heat content (OHC) in the equatorial Pacific persists beyond the first peak, stimulating another event. This prolonged OHC anomaly is caused by meridional Ekman heat transport counteracting geostrophic transport induced recharge–discharge process that otherwise acts to change the OHC anomaly. A meridionally wide pattern of sea surface temperature observed during multiyear event is responsible for the Ekman heat transport. CMIP6 multi-model ensemble shows a significant correlation between the ENSO meridional width and the occurrence ratio of multiyear ENSO. A multiyear ENSO-like oscillation was simulated using the linear RO model that incorporates a seasonally varying Bjerknes growth rate and a weak recharge efficiency representing the effect of Ekman transport. When the recharge efficiency parameter was estimated using reanalysis data based on geostrophic transport alone, a multiyear ENSO rarely occurred, confirming the importance of Ekman transport in retarding the recharge–discharge process.

How to cite: Iwakiri, T. and Watanabe, M.: Multiyear ENSO dynamics as revealed in observations, CMIP6 models, and linear theory, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3631, https://doi.org/10.5194/egusphere-egu23-3631, 2023.

EGU23-3637 | ECS | Posters on site | CL2.2

Is a Preceding Strong El Niño Required to Generate Multi-year La Niña? 

Ji-Won Kim, Jin-Yi Yu, and Baijun Tian

By analyzing observational data covering the period from 1900 to 2021, we show that the known mechanism linking multi-year La Niña with a preceding strong El Niño has been overemphasized. A majority of multi-year La Niña (64%; 7 out of 11 events) do not require a preceding strong El Niño to generate their 2nd-year La Niña. We find that the negative phase of the Pacific Meridional Mode (PMM) during 1st-year La Niña’s decaying spring, rather than the preceding strong El Niño, offers the key mechanism to produce 2nd-year La Niña, resulting in a multi-year La Niña. It is further found that the westward extension of the 1st-year La Niña cold sea surface temperature anomalies, which interacts with the eastern edge of the western Pacific warm pool, is a key factor inducing the negative PMM. The negative PMM mechanism to generate multi-year La Niña is also applied to the 3rd-year La Niña of multi-year La Niña, giving rise to a triple-dip event. The possible reason(s) how and why a multi-year La Niña can become either a double-dip or a triple-dip event will be discussed.

How to cite: Kim, J.-W., Yu, J.-Y., and Tian, B.: Is a Preceding Strong El Niño Required to Generate Multi-year La Niña?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3637, https://doi.org/10.5194/egusphere-egu23-3637, 2023.

EGU23-4180 | Orals | CL2.2

Why is El Nino warm? 

Stephan Fueglistaler, Laure Resplandy, and Allison Hogikyan

El Nino years stand out in the global average temperature time series as record-warm years. The coupled atmosphere-ocean dynamics leading to warming in the climatologically cold equatorial Eastern Pacific are well understood, but cannot be the cause for the very strong signal in global average temperarture. The latter must be caused by an increase in subcloud Moist Static Energy (MSE) in the domain of highest subcloud MSE where atmospheric deep convection couples the surface, boundary layer and free troposphere. Transformation of the data from geographical space to sea-surface temperature (SST) percentiles eliminates the large spatial see-saws in all variables arising from the geographic reorganization of the general circulation, and brings to light the mechanism: While in the Eastern Pacific region oceanic heat uptake is reduced (corresponding to a heat flux out of the ocean), the deep convective domain sees a heat flux from the atmosphere into the ocean. We show that this heat flux into the ocean at the high end of SSTs - the opposite of the canonical perspective of a warming due to a heat flux from the ocean to the atmosphere - is mechanically forced: surface wind speeds are lower in regions of active deep convection than in ENSO neutral (and La Nina) years. The resulting reduced evaporation leads to the increase in subcloud MSE that causes the global temperature signal.

How to cite: Fueglistaler, S., Resplandy, L., and Hogikyan, A.: Why is El Nino warm?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4180, https://doi.org/10.5194/egusphere-egu23-4180, 2023.

The equatorial Atlantic zonal sea surface temperature (SST) gradient, which has significant climatic and biogeochemical effects, is closely associated with the equatorial Pacific zonal SST gradient through Walker circulation on seasonal and interannual time scales. However, discrepancies in current SST datasets mean that its long-term trend is not well understood. Here, using multiple datasets, we find a robust weakening long-term trend (i.e., greater warming in the east than west) in the equatorial Atlantic zonal SST gradient over the period 1900–2010 in all datasets. We also find that this weakening trend is closely linked to the tropical Pacific cold tongue mode (CTM), which corresponds to a strong increasing long-term trend of zonal SST gradient along the equatorial Pacific (i.e., warming in the west and cooling in the east). Specifically, the long-term cooling SST anomalies associated with the CTM modify the Walker circulation, and leads to weaker trade winds over the western equatorial Atlantic. These in turn deepen the thermocline in the eastern equatorial Atlantic, and cause the weakening long-term trend of SST gradient along the equatorial Atlantic. The long-term trend of the CTM is induced by ocean dynamical feedback in response to global warming, suggesting that global warming could affect the equatorial Atlantic zonal SST gradient via the CTM. Our results provide a novel explanation of the linkages between the long-term trend of equatorial Atlantic zonal SST gradient and the CTM under global warming, which carries important implications for the relationship between global warming and the equatorial Atlantic zonal SST gradient.

How to cite: Li, Y.: Long-term trend of equatorial Atlantic zonal SST gradient linked to the tropical Pacific cold tongue mode under global warming, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4360, https://doi.org/10.5194/egusphere-egu23-4360, 2023.

EGU23-4971 | ECS | Orals | CL2.2

Indo-Pacific teleconnection changes during the Holocene: model-proxy comparison 

Isma Abdelkader Di Carlo, Pascale Braconnot, Mary Elliot, and Olivier Marti

The teleconnections between the Indian and Pacific Oceans are very complex, involving multiple modes of variability and phenomena such as the El Niño-Southern Oscillation, Indian Ocean Dipole, Indian Ocean Basin mode, and the Asian monsoon. Their interactions are complex because changes in one of these phenomena affect the others. Insufficient agreement exists on the predicted evolution of mean states of both basins and the impacts of climate variability in this region in response to increasing CO2 emissions. To better constrain Indo-Pacific interactions, we have studied the Holocene period. We consider four transient simulations from three General Circulation Models (GCM) and a collection of paleo-archives from the Holocene in the Indo-Pacific region. Our study allows us to put into perspective the links between long-term changes in variability and in the mean state. The main driver is insolation and trace gases (CO2) that have increased the mean sea surface temperature of the tropical ocean over the last 6,000 years. Our first results show that modeled trends in the regional long-term variability are in agreement, but differences are observed when we analyze the data at shorter interannual timescales. We also explain why the simulations differ or agree with the paleoclimate reconstructions. One way is to look at the relative role of temperature and salinity in determining the changes in δ18O recorded by the various climate archives. 

How to cite: Abdelkader Di Carlo, I., Braconnot, P., Elliot, M., and Marti, O.: Indo-Pacific teleconnection changes during the Holocene: model-proxy comparison, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4971, https://doi.org/10.5194/egusphere-egu23-4971, 2023.

EGU23-5205 | ECS | Posters on site | CL2.2

Impact of tropical SSTs on the monthly signal over the North Atlantic-European region 

Sara Ivasić, Ivana Herceg Bulić, and Margareta Popović

Targeted numerical simulations were designed to test the potential impact of tropical sea surface temperatures (SSTs) on the geopotential heights at 200 hPa (GH200) signal over the North Atlantic-European region. Five experiments with SST anomalies prescribed in different areas, acting as lower boundary forcing, were created with an intermediately complex atmospheric general circulation model (ICTP AGCM). In the AGCM experiments, the SST forcing was prescribed globally, in the tropical zone of all oceans, only in the tropical Atlantic, tropical Indian Ocean and limited to the tropical Pacific. All of the simulations covered a 156-year-long period.

The monthly GH200 signal was calculated based on the difference between the ensemble mean of each experiment and the climatological mean for the considered period. In addition, to inspect the impact of the El Niño-Southern Oscillation (ENSO), the signal was calculated for ENSO and non-ENSO years, respectively. Here, the ENSO years were classified according to the value of the late-winter Niño3.4 index.

Additionally, each experiment’s monthly signal was averaged over the signal maximum over the North Atlantic-European region. The characteristics of the spatially averaged signal were compared to the signal averaged over a similar signal maximum observed over the Pacific North American region.

Results have shown that the GH200 signal is the strongest in the late-winter months in all experiments. The AGCM experiment with SST boundary forcing prescribed only in the tropical Atlantic consistently had the smallest signal amplitude. The strongest signal linked to ENSO events was found in the experiment with the SST forcing prescribed only in the tropical Pacific. The signal averaged over the NAE maximum generally yields smaller values than the PNA maximum average. Also, the differences between the (non) ENSO signal and the signal for all years are less pronounced in the case of the NAE maximum average.

How to cite: Ivasić, S., Herceg Bulić, I., and Popović, M.: Impact of tropical SSTs on the monthly signal over the North Atlantic-European region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5205, https://doi.org/10.5194/egusphere-egu23-5205, 2023.

EGU23-5310 | ECS | Orals | CL2.2

Distinct and reproductible northem hemisphere winter teleconnection pattern during strong El Niño events : relative roles of Sea Surface Temperature forcing and atmospheric nonlinearities 

Margot Beniche, Jérôme Vialard, Matthieu Lengaigne, Aurore Voldoire, Srinivas Gangiredla, and Nicholas Hall

The strengthening and north-eastward shift of El Niño Northern hemisphere winter teleconnections relative to those of La Niña is a well-known asymmetry of ENSO (El Niño Southern Oscillation). It is generally attributed to atmospheric nonlinearities associated with the Sea Surface Temperature (SST) threshold for tropical deep convection. Here, we re-examine these teleconnection asymmetries in the context of ENSO SST pattern diversity. We find that the asymmetries are mainly attributable to strong El Niño events (eg. 1982-83, 1997-98, 2015-16), both in observations and in ensemble simulations with the atmospheric component of the CNRM-CM6 model. This strong El Niño teleconnection pattern also results in specific impacts, characterized by enhanced rainfall along the United States (US) west coast and warm anomalies over Canada and the Northern US. Our ensemble simulations further indicate that moderate “Eastern Pacific” El Niño events exhibit teleconnection patterns that are similar to those of “Central Pacific” El Niño, or to the opposite of La Niña events. We also find that the teleconnection spread between ensemble members or events is reduced for strong El Niño relative to moderate El Niño or La Niña events, with important implications for predictability. Sensitivity experiments in which the atmospheric model is forced by the opposite of observed SST anomalies are used to assess the mechanisms inducing the strong El Niño teleconnection pattern. In addition to the well-known influence of atmospheric nonlinearities, these experiments reveal an important contribution from the Eastward-shifted SST pattern during strong El Niño events.

 

How to cite: Beniche, M., Vialard, J., Lengaigne, M., Voldoire, A., Gangiredla, S., and Hall, N.: Distinct and reproductible northem hemisphere winter teleconnection pattern during strong El Niño events : relative roles of Sea Surface Temperature forcing and atmospheric nonlinearities, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5310, https://doi.org/10.5194/egusphere-egu23-5310, 2023.

The amplitude of El Niño/Southern Oscillation (ENSO) varied considerably over the last 140 years, for which we have relatively reliable Sea Surface Temperature (SST) observations over the tropical Pacific. The difference between periods of high and low ENSO amplitude results mainly from the number of strong Eastern Pacific (EP) El Niños, while the amplitude of Central Pacific (CP) El Niños is comparable in both periods. Further, the asymmetry of ENSO, i.e. that the SST anomalies during El Niño are on average stronger and located further to the east than during La Niña, covaries with ENSO amplitude in observations, indicating that the number of strong EP El Niño events dominates both ENSO amplitude and asymmetry variations.

We find similar relations in the 40 historical runs of the Large Ensemble with the CESM1-CAM5-BGC model that can simulate the ENSO asymmetry quite realistically.  Further, there is a strong relation between the ENSO amplitude and the tropical Pacific mean state, indicating that a warmer eastern equatorial Pacific favors more EP El Niños due to a lower convective threshold in that area. We also analyze the spatial asymmetry and amplitude asymmetry of the atmospheric and oceanic feedbacks and show that the spatial asymmetry is more pronounced in the atmospheric feedbacks, while the amplitude asymmetry is more pronounced in the oceanic feedbacks, and that both together form the observed asymmetry of ENSO.  A comparison with 360 years-long CESM1 experiments with a -4.0 K colder and +3.7 K warmer mean state indicates that the present-day ENSO may be in a transition zone between a CP El Niño dominated ENSO state and an EP El Niño dominated ENSO state and that ENSO may lock-in into the EP El Niño dominated state under global warming.

Finally, our analysis of ENSO-amplitude variability in preindustrial control simulations of the CMIP6 database supports a strong relation of ENSO amplitude and asymmetry with the number of strong EP El Niño events.

How to cite: Bayr, T., Lübbecke, J. F., and Latif, M.: The role of strong Eastern Pacific El Nino events in ENSO-amplitude variability in Observations and Climate Models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6109, https://doi.org/10.5194/egusphere-egu23-6109, 2023.

Using observational analysis and numerical experiments, we identify that the dipole mode of 
spring surface wind speed (SWS) over the Tibetan Plateau (TP) could act as a trigger for subsequent winter El 
Niño–Southern Oscillation events. During the positive phase of spring SWS dipole mode (south-positive and 
north-negative), a self-sustaining “negative sensible heating–baroclinic structure” prevails over the western TP, 
which is characterized by negative surface sensible heating anomalies, anomalous low-level anticyclones, and 
mid–high-level cyclones. The “negative sensible heating–baroclinic structure” stimulates the surface westerly 
wind anomalies over the tropical western Pacific in May through two pathways, favoring the occurrence of 
subsequent El Niño events. One is through weakening the zonal monsoon circulation over the tropical Indian 
Ocean and the Walker circulation over the tropical western Pacific. The other is modulating the air–sea 
interaction over the North Pacific through triggering Rossby waves. The negative SWS dipole mode tends to 
induce La Niña events.

How to cite: Yu, W.: Potential Impact of Spring Thermal Forcing Over the Tibetan Plateau on the Following Winter El Niño–Southern Oscillation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6401, https://doi.org/10.5194/egusphere-egu23-6401, 2023.

EGU23-7693 | Orals | CL2.2

Atmospheric nonlinearities strong contribution to the skewed ENSO amplitude and phase transition 

Jérôme Vialard, Srinivas Gangiredla, Matthieu Lengaigne, Aurore Voldoire, Takeshi Izumo, and Eric Huilyardi

ENSO features prominent asymmetries, in terms of amplitude, spatial pattern and phase-transition between warm and cold events. Here we examine the contribution of atmospheric nonlinearities to ENSO asymmetries through a set of forced experiments with the CNRM-CM6 AGCM and the NEMO OGCM. Control experiments can reproduce the major atmospheric and oceanic asymmetries of ENSO, with stronger signals east of the dateline for strong El Niño events, and west of it for strong La Niñas. Ensemble atmospheric experiments forced by observed ENSO SST anomalies and their opposites allow diagnosing asymmetries in air-sea heat and momentum fluxes directly attributable to atmospheric nonlinearities. They indicate that atmospheric nonlinearities are largely attributable to nonlinearities in the rainfall-SST relation and act to enhance El Niño atmospheric signals east of the dateline and those of La Niña west of it. An ocean simulation where the non-linear signature of air-sea fluxes is removed from the forcing reveals that asymmetries in the ENSO SST pattern are primarily due to atmospheric nonlinearities, and result in a doubling of eastern Pacific warming during the peak of strong El Niño events and a 33% reduction during that of strong La Niña events. Atmospheric nonlinearities also explain most of the observed prolonged eastern Pacific warming into boreal summer after the peak of strong El Niño events. Overall, these results imply that properly simulating the nonlinear relationship between SST and rainfall in CGCMs is essential to accurately simulate asymmetries in ENSO amplitude, spatial pattern and phase transition. Finally, we discuss the inherent limitations to our two-tier forced approach.

How to cite: Vialard, J., Gangiredla, S., Lengaigne, M., Voldoire, A., Izumo, T., and Huilyardi, E.: Atmospheric nonlinearities strong contribution to the skewed ENSO amplitude and phase transition, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7693, https://doi.org/10.5194/egusphere-egu23-7693, 2023.

EGU23-7791 | Posters on site | CL2.2

The multiverse future of ENSO diversity in large ensembles of climate models 

Bastien Dieppois, Nicola Maher, Antonietta Capotondi, and John O'Brien

El Niño Southern Oscillation (ENSO) shows large differences from one event to another in terms of its intensity, spatial pattern, and temporal evolution, which are typically referred to as “ENSO diversity”. While such differences in ENSO patterns are associated with different regional climate impacts throughout the world, influencing the skill of impact prediction systems, large uncertainties remain concerning its potential future evolution and trends. The location and intensity of ENSO events are indeed strongly influenced by internal/natural climate variations, limiting the detection of forced changes.

Here, we exploit the power of single model initial-condition large ensembles (SMILEs) from 13 fully coupled climate models from both CMIP5 and CMIP6 (totalling 580 realizations in historical and SSP-RCP scenarios) to first examine the ability of climate models to simulate realistic diversity of ENSO events compared to multiple observational datasets, and then use those models to characterize future trajectories in the location and intensity of El Niño and La Niña events. We define the location of ENSO events as the longitude of the absolute maximum (the intensity) of sea-surface temperature anomalies (SSTa) during boreal Winter (December-February) in the equatorial Pacific. Future projections of ENSO diversity are assessed in terms of joint probability distributions of ENSO events’ location and intensity.

While some models show a degree of diversity in the location and intensity of events that are comparable with observed statistics, other models tend to favour the occurrence of eastern or central Pacific events. Such contrasting performances during the historical period are found to be associated with different future trajectories of ENSO diversity: i) models favouring the occurrence of eastern Pacific events (e.g., ACCESS-ESM1-5, CanESM2, and 5) show a westward shift in event location over the 21st century; ii) models simulating ENSO events anomalously westward tend to show an eastward shift in event locations and an increased intensity in the 21st century (e.g., CESM1 and 2, CSIRO-MK3-6-0, GFDL-CM3, GFDL-ESM2M, MIROC-ES2L, MIROC6). Nevertheless, we note that models showing the closest match to observed statistics during the historical period also present a westward shift in ENSO locations and a slight increase in intensity in the 21st century (e.g., GFDL-SPEAR and IPSL-CM6-LR).

Although the physical cause of model discrepancies remains unclear, this study provides a broader perspective on expected ENSO changes over the 21st century in different models and highlights the spread of projections among models.

How to cite: Dieppois, B., Maher, N., Capotondi, A., and O'Brien, J.: The multiverse future of ENSO diversity in large ensembles of climate models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7791, https://doi.org/10.5194/egusphere-egu23-7791, 2023.

EGU23-8299 | ECS | Orals | CL2.2

Effect of Indian Ocean Dipole on ocean meridional heat transport depends on ENSO 

Kay McMonigal and Sarah Larson

Meridional heat transport within the Indian Ocean can drive climate and ecosystem impacts, by changing ocean temperature. Previous studies have linked variability in meridional heat transport to Indian Ocean Dipole (IOD) and El Niño-Southern Oscillation (ENSO). Recent studies have shown that some IOD events are caused by ENSO (termed “ENSO forced IOD”), while other events occur without ENSO (termed “internal IOD”). It is unclear whether these different kinds of IOD have different effects on the ocean. By comparing a climate model that includes ENSO to the same climate model but with ENSO dynamically removed, we show that internal IOD does not lead to variability in Indian Ocean meridional heat transport. However, ENSO forced IOD does lead to meridional heat transport variability. This is due to differing wind patterns associated with each kind of IOD event. These results suggest that the ecosystem and climate effects of IOD likely depend upon whether the IOD occurs with or without ENSO. 

How to cite: McMonigal, K. and Larson, S.: Effect of Indian Ocean Dipole on ocean meridional heat transport depends on ENSO, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8299, https://doi.org/10.5194/egusphere-egu23-8299, 2023.

EGU23-8733 | ECS | Orals | CL2.2

Stochastic perturbations of El Nino Southern Oscillations (ENSO) : a Wiener chaos approach 

Yusuf Aydogdu, Peter Baxendale, and N. Sri Namachchivaya

The phenomena of El Nino Southern Oscillations (ENSO) is modeled by coupled atmosphere-ocean mechanism together with sea surface temperature (SST) budget at the equatorial Pacific and has a significant impact on the global climate.  We consider a modeling framework that was originally developed by Majda and co-workers in (Chen et al. 2018; Thual et al. 2016), which is physically consistent and amenable to detailed analysis. The coupled model is mainly governed by the equatorial atmospheric and oceanic Kelvin and Rossby waves and it is shown that stochastic forcing gives rise to the model anomalies and unpredictable behavior. The purpose of our work is to investigate the influence of randomness on the model dynamics,  construct the appropriate model components with stochastic noise and calculate the statistical properties. We also provide analytical and numerical solutions of the model to prove the convergence of the numerical scheme developed in our work. 

We use Wiener-Chaos Expansion (WCE) to study stochastic ENSO models. The WCE method is based on reducing stochastic partial differential equations (SPDEs) into an infinite hierarchy of deterministic PDEs called propagators-Fourier modes (Lototsky and Rozovsky, 2006) and represents the stochastic solution as a spectral decomposition of deterministic components with respect to a set of random Hermite bases. We solve the WCE propagators, which are forced by a set of complete orthonormal bases,  by applying numerical integration and finite-difference methods. We compare WCE-based results with Monte Carlo simulations of SPDEs.

Our results depict that the mean and variance of the solutions obtained from the WCE method provide remarkably accurate results with a reasonable convergence rate and error range.  We first test the WCE-based method on the ocean  model with white noise and show that 10-Fourier modes are able to approach the theoretical variance values. We also show that the OU process with a specific noise strength and dissipation over a one-time period can be recovered with less than 50-Fourier modes for the ENSO model.  To illustrate the particular weight of variance, we also generate the ensembles of solutions by using different stochastic bases. We also derive the analytical formulation of propagators for the coupled model with nonlinear SST by using the properties of Wick polynomials that construct the foundation of numerical schemes. 

How to cite: Aydogdu, Y., Baxendale, P., and Namachchivaya, N. S.: Stochastic perturbations of El Nino Southern Oscillations (ENSO) : a Wiener chaos approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8733, https://doi.org/10.5194/egusphere-egu23-8733, 2023.

EGU23-8904 | Orals | CL2.2

Forecasting the El Niño type well before the spring predictability barrier 

Josef Ludescher, Armin Bunde, and Hans Joachim Schellnhuber

The El Niño Southern Oscillation (ENSO) is the most important driver of interannual global climate variability and can trigger extreme weather events and disasters in various parts of the globe. Depending on the region of maximal warming, El Niño events can be partitioned into 2 types, Eastern Pacific (EP) and Central Pacific (CP) events. The type of an El Niño has a major influence on its impact and can even lead to either dry or wet conditions in the same areas on the globe. Here we show that the zonal difference ΔTWP-CP between the sea surface temperature anomalies (SSTA) in the equatorial western Pacific and central Pacific is predictive of the type of an upcoming El Niño. When at the end of a calendar year, ΔTWP-CP is positive, an El Niño event developing in the following year will probably be an EP event, otherwise a CP event. Between 1950 and present, the index correctly indicates the type of 18 out of 21 El Niño events (p = 9.1⋅10-4).
For early actionable forecasts, the index has to be combined with a forecast for the actual onset of an El Niño event. The previously introduced climate network-based forecasting approach provides such forecasts for the onset of El Niño events also by the end of the calendar year before onset. Thus a combined approach can provide reliable forecasts for both the onset and the type of an event: at a lead time of about one year, 2/3 of the EP El Niño forecasts and all CP El Niño forecasts in the regarded period are correct. The combined model has considerably more predictive power than the current operational type forecasts with a mean lead time of about 1 month and should allow early mitigation measures.

How to cite: Ludescher, J., Bunde, A., and Schellnhuber, H. J.: Forecasting the El Niño type well before the spring predictability barrier, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8904, https://doi.org/10.5194/egusphere-egu23-8904, 2023.

Since the early 1990s the Pacific Walker circulation has strengthened, while SSTs in the eastern equatorial Pacific became colder, which is opposite to future model projections. Whether these trends, evident in many climate indices especially before the 2015 El Niño, reflect the coupled ocean-atmosphere response to global warming or the negative phase of the Pacific Decadal Oscillation (PDO) remains debated. Here we show that sea surface temperature (SST) trends during 1980-2020 are dominated by three signals: a spatially uniform warming trend, a negative PDO pattern, and a Northern Hemisphere/Indo-West Pacific warming pattern. The latter pattern, which closely resembles the transient ocean thermostat-like response to global warming emerging in a subset of CMIP6 models, shows cooling in the central-eastern equatorial Pacific but warming in the western Pacific and tropical Indian ocean. Together with the PDO, this pattern drives the Walker circulation strengthening. CMIP6 historical simulations appear to underestimate this pattern, contributing to the models’ inability to replicate the Walker cell strengthening. We further discuss how such changes in the Walker circulation can effect ENSO.

Reference:  Heede, U. and A.V. Fedorov, 2023: Colder eastern equatorial Pacific and stronger Walker circulation in the early 21st century: separating the forced response to global warming from natural variability. In press, GRL

How to cite: Fedorov, A. and Heede, U.: Colder eastern equatorial Pacific and stronger Walker circulation in the early 21st century: an Indo-Pacific ocean thermostat  versus natural variability, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10347, https://doi.org/10.5194/egusphere-egu23-10347, 2023.

EGU23-10801 | Orals | CL2.2 | Highlight

Causes and Consequences of the Prolonged 2020-2023 La Niña 

Michael J. McPhaden, Nahid Hasan, and Yoshimitsu Chikamoto

The tropical Pacific has witnessed three successive years of unusually cold sea surface temperatures, with peak anomalies in late 2020, 2021 and 2022.  These conditions represent the first "triple dip" La Niña of the 21st century with major climatic impacts felt around the world.  Three year La Niña events are rare but not unprecedented; similar events occurred in 1998-2001 and in 1973-76.  A leading hypothesis for multi-year La Niñas is that they occur on the rebound from preceding extreme El Niños which, through recharge oscillator dynamics, drain the equatorial band of upper ocean heat content leaving a large heat deficit that takes multiple years to recover. The current multi-year La Niña does not conform to this scenario--antecedent conditions in the tropical Pacific in 2019 were characterized by a borderline El Niño that did not lead to a large upper ocean heat content discharge. What caused the this La Niña is thus a topic of considerable interest.  In this presentation we hypothesize that tropical inter-basin interactions were instrumental in initiating and prolonging the event. In particular, we suggest that the event was triggered from the Indian Ocean by a record Indian Ocean Dipole in late 2019, then boosted in 2021 by unusually warm conditions in the tropical Atlantic involving the strongest Atlantic Niño since the 1970s. Whether climate change may have played a role in these developments will be discussed.

How to cite: McPhaden, M. J., Hasan, N., and Chikamoto, Y.: Causes and Consequences of the Prolonged 2020-2023 La Niña, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10801, https://doi.org/10.5194/egusphere-egu23-10801, 2023.

EGU23-11500 | Orals | CL2.2

Representation of tropical SST trends in ECMWF seasonal hindcasts and implications for recent ENSO forecasts 

Michael Mayer, Magdalena Alonso Balmaseda, and Steffen Tietsche

Operational seasonal forecasts are routinely issued with their bias removed, which is estimated from hindcasts covering a sufficiently long period. An increased number of false alarms for the occurrence of El Nino by various dynamical forecasting systems in recent years challenges the view that forecast biases are stationary. Here we assess the ability of ECMWF’s operational seasonal prediction system SEAS5 to represent observed trends in tropical SSTs since 1993, with a focus on the Pacific.

SEAS5 hindcasts overestimate SST warming in the equatorial Pacific when compared to observations. Although present for all start dates, the trend error is most pronounced for May starts. As a result, SEAS5 forecasts in recent years tended to predict too warm ENSO states despite bias correction. The hindcasts also fail to reproduce the observed meridional dipole in SST trends in the eastern Pacific, with warming in the northern and cooling in the southern subtropics. We assess several numerical experiments to investigate the role of the evolving ocean observing system, the ocean data assimilation system, and the atmospheric model. Results show that the increase in Argo observations amplifies the spurious trends in the hindcasts, which points to biases in the ocean initial conditions when observational constraints are lacking prior to Argo. Furthermore, observed-SST experiments show that the atmospheric model is unable to reproduce the magnitude of increasingly northward winds that are observed in the eastern equatorial Pacific, which are associated with the meridional structure of observed SST trends and have been speculated to reduce ENSO variability. This suggests that shortcomings of the atmospheric model physics further contribute to the system’s inability to predict the recent triple La Nina period. The results call for more sophisticated calibration methods of seasonal forecasts and ultimately improved models and initialization to provide more reliable ENSO forecasts under varying background conditions.

How to cite: Mayer, M., Alonso Balmaseda, M., and Tietsche, S.: Representation of tropical SST trends in ECMWF seasonal hindcasts and implications for recent ENSO forecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11500, https://doi.org/10.5194/egusphere-egu23-11500, 2023.

There are large interannual variations in the area integral of the Pacific-wide annual-mean net surface heat fluxes within 5o of the equator. They are shown to be very well correlated (r2 = 0.75) with the zonal-mean, annual-mean, zonal component of the surface wind stress on the equator, both in UK-HadGEM3 coupled climate simulations and in the ERA5 wind-stress and DEEPC net surface heat flux re-analyses. For the model data the corresponding correlations are small for monthly means (r2 = 0.25) but are large (r2 > 0.6) for time-mean periods between 6 months and 10 years (the latter being calculated from 700 year pre-industrial control simulations). The amplitude of these annual mean fluctuations in the DEEPC net surface heat fluxes is almost twice as large as that in the UK-HadGEM3 simulations. Comparison of the area-mean fields in the Nino3 and Nino4 regions from 4 member ensembles of N216O025 historical simulations with the ERA5 winds, DEEPC heat fluxes and EN4 ocean re-analyses shows that the model’s mean values and seasonal cycle of the zonal wind stress and net surface heat flux agree well with the re-analyses. In the Nino3 region however the model’s surface temperature is 1.5oC colder than the re-analyses and the depth of the 20oC isotherm (t20d) is between 10 and 15 m shallower than that in EN4.  Comparison of the amplitudes of El Nino and La Nina composite anomalies in the Nino3 and Nino4 regions shows that the surface temperature anomalies are well simulated but that the amplitudes of the wind stress anomalies in Nino4 and the t20d anomalies and surface heat flux anomalies in Nino3 are about half those in ERA5, EN4 and DEEPC respectively. These findings are somewhat similar to those from the (lower resolution)  Kiel Climate Model. The characteristic spatial patterns of the surface fields might be used to attribute the differences between the model and re-analysis net surface fluxes to particular component fluxes (e.g. the surface latent heat flux and the surface solar flux). It is also a plausible hypothesis that the under-estimation of these variations in the net surface heat fluxes is a significant contributor to the signal-to-noise paradox.       

 

How to cite: Bell, M.: HadGEM3  underestimates interannual variations in heat fluxes, zonal winds and thermocline displacements  in the tropical Pacific, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12824, https://doi.org/10.5194/egusphere-egu23-12824, 2023.

EGU23-13335 | ECS | Posters on site | CL2.2

Using Causal Discovery to Clarify Observed and Simulated Relationships Between ENSO and Other Ocean Basins 

Rebecca Herman and Jakob Runge

Observed sea-surface temperatures in various ocean basins are confounded by anthropogenic and natural radiative forcing and by teleconnections to modes of internal variability, especially the El Nino Southern Oscillation (ENSO). While confounding due to anthropogenic and natural forcing can be removed in coupled simulations, confounding due to ENSO is unavoidable. When not appropriately characterized and quantified, this confounding can obscure causal relationships between various ocean basins and atmospheric phenomena of huge humanitarian import, such as monsoon rainfall, with implications for attribution of past disasters and prediction of the future. These relationships have been difficult to characterize in part because observational data is limited and simulated data may not represent the observed climate system. This study uses causal discovery to examine the coupled relationships between ENSO and other ocean basins in simulations and observations. We begin by evaluating the (L)PCMCI(+) causal discovery algorithms under various conditions and assumptions on data generated by two continuous idealized models of ENSO: the classic Zebiak-Cane model and a simple stochastic dynamical model proposed by Thual, Majda, Chen, and Stechmann. We then apply the causal discovery algorithms to seasonally and spatially-averaged sea surface temperature (SST) indices for ENSO and other ocean basins in preindustrial control simulations from the Coupled Model Intercomparison Project Phase 6. We discuss the robustness of the results, and the differences between the causal relationships in different General Circulation Models. Finally, we apply the causal learning algorithm to observed SST, and discuss to what extent simulated relationships can be used to learn about the observed climate system. We additionally demonstrate the implications of this study for other scientific questions, specifically for understanding variability in Sahel Monsoon rainfall.

How to cite: Herman, R. and Runge, J.: Using Causal Discovery to Clarify Observed and Simulated Relationships Between ENSO and Other Ocean Basins, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13335, https://doi.org/10.5194/egusphere-egu23-13335, 2023.

EGU23-13812 | ECS | Orals | CL2.2

ENSO–IOD Inter-Basin Connection Is Controlled by the Atlantic Multidecadal Oscillation 

Jiaqing Xue, Jing-Jia Luo, Wenjun Zhang, and Toshio Yamagata

The interactions between El Niño-Southern Oscillation (ENSO) and Indian Ocean Dipole (IOD) are known to have great implications for global climate variability and seasonal climate predictions. Observational analysis suggests that the ENSO–IOD inter-basin connection is time-varying and related to the Atlantic Multidecadal Oscillation (AMO) with weakened ENSO–IOD relationship corresponding to AMO warm phases. A suite of Atlantic pacemaker simulations successfully reproduces the decadal fluctuations in ENSO–IOD relationship and its link to the AMO. The warm sea surface temperature (SST) anomalies associated with the AMO drive a series of Indo-Pacific mean climate changes through tropical-wide teleconnections, including the La Niña-like mean SST cooling over the central Pacific and the deepening of mean thermocline depth in the eastern Indian Ocean. By modulating ocean–atmosphere feedback strength, those mean state changes decrease both ENSO amplitude and the Indian Ocean sensitivity to ENSO forcing, therefore decoupling the IOD from ENSO.

How to cite: Xue, J., Luo, J.-J., Zhang, W., and Yamagata, T.: ENSO–IOD Inter-Basin Connection Is Controlled by the Atlantic Multidecadal Oscillation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13812, https://doi.org/10.5194/egusphere-egu23-13812, 2023.

EGU23-15824 | ECS | Orals | CL2.2

Future Changes in the early winter ENSO teleconnections to the North Atlantic European region 

Muhammad Adnan Abid and Fred Kucharski

North Atlantic European (NAE) winter climate variability is strongly modulated through the stratospheric and tropospheric pathways, where El Niño-Southern Oscillation (ENSO) teleconnections play an important role. Recent studies showed intra-seasonal changes of the ENSO response in the NAE circulation anomalies from early to late winter.  One mechanism for this behavior is that the Indian Ocean (IO) dominate over the direct ENSO teleconnections in early winter favoring an in-phase North Atlantic Oscillation (NAO) response over NAE region. On the other hand, the direct ENSO response dominates in latter half of winter, where it projects onto the opposite phase of the NAO. In present study, we analyze the early to late winter ENSO-NAE teleconnections in future climate projections by adopting the sixth assessment report Coupled Model Intercomparison Project (CMIP6) model datasets. During early winter, we noted an increase in the ENSO-induced precipitation variability in the Pacific as well as over western and central Indian Ocean, while decrease is noted over the eastern IO. Moreover, a strengthening of the ENSO and Indian connections are noted in almost all models except few, where these connections are not well represented in the present climate. Interestingly, the changes in ENSO forced wave train are noted, which may lead to the negative NAO like circulation anomalies over the NAE region in future compared to the present climate. 

How to cite: Abid, M. A. and Kucharski, F.: Future Changes in the early winter ENSO teleconnections to the North Atlantic European region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15824, https://doi.org/10.5194/egusphere-egu23-15824, 2023.

EGU23-16921 | Orals | CL2.2

The role of spatial shifting in El Niño/Southern Oscillation complexity 

Sulian Thual and Boris Dewitte

The El Niño-Southern Oscillation (ENSO) represents the most consequential fluctuation of the global climate system, with dramatic societal and environmental impacts. Here we show that the spatial shifting movements of the Walker circulation control the ENSO space-time complexity in a major way. First, we encapsulate the process in a conventional recharge-discharge oscillator for the ENSO by replacing the regionally fixed sea surface temperatures (SST) index against a warm pool edge index. By doing so, we can model essential ingredients of ENSO diversity and nonlinear behavior without increasing the complexity of the dynamical model. Second, we propose a data-driven method for estimating equatorial Pacific SST variability resulting from spatial shifting. It consists in time-averaging conditions respective to the evolving warm pool edge position, then generating back SST data with reduced dimensionality (one degree of freedom) from the movements of the resulting "shifted-mean" profile. It is shown that the shifted-mean SST generated in this fashion reasonably reconstructs observed interannual SSTs both in terms of amplitude and pattern diversity. We discuss implications of the present paradigm of spatial shifting for understanding ENSO complexity, including tropical basins interactions.

How to cite: Thual, S. and Dewitte, B.: The role of spatial shifting in El Niño/Southern Oscillation complexity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16921, https://doi.org/10.5194/egusphere-egu23-16921, 2023.

EGU23-307 | ECS | Orals | AS1.17

Circulation aspects associated with heat wave events over Iraq 

Hasanain Al-Shamarti, Thomas Birner, and Philip Rupp

Heat waves lead to increased mortality due to heat exhaustion and heatstroke, wildfire, reduced agricultural yields, increased energy demand, economic predicaments and other societal issues. Heat wave events over the Middle-East have received far less attention compared to events elsewhere. Here, we provide a comprehensive characterization of heat wave events over Iraq, covering the period 1980-2019.
We use ERA5 reanalysis data for Northern summer (June-July-August) to identify heat waves in daily maximum 2-m temperature (Tmax) data and study them using composite analyses and clustering. We define a heat wave event if the Tmax anomaly exceeds the 90th percentile over three consecutive days, provided this threshold exceedance covers at least 50% of our target area.

The composite-mean evolution of daily Tmax anomalies demonstrates that our heat waves typically strengthen gradually over the week preceding the central day with a sharp decline in strength at positive lags, reaching an average maximum anomaly of ~3.7 K at the central day. We find the heat waves to extend from the Arabian peninsula northward across Iraq toward southwestern Russia. Clustering of all heat wave events reveals two dominant flow anomaly patterns that roughly distinguish early from late summer events.

The first cluster (early summer events) is associated with anomalous anticyclonic flow associated with a quasi-stationary upper-level high pressure system to the north-east of Iraq precisely over Caspian sea. This anomalous anticyclonic flow is embedded in a Rossby wave train that initially propagates along the north Atlantic wave-guide, then further equatorward along the North African-Asian jet just before the central day. Our composite-mean evolution for this first cluster further shows mid-tropospheric subsidence over the Zagros mountains, i.e., upstream of our heat wave target area. Downslope Foehn winds appear to enhance the heat wave over Iraq.

In contrast, the second cluster is primarily composed of late-summer events and shows strong anomalies in the Shamal winds - a pronounced low-level north-westerly jet along the western edge of the Zagros mountains. During these late summer heat wave events the Shamal jet is substantially weakened or even reversed, transporting warm air from the Persian gulf into the target region. 

 

How to cite: Al-Shamarti, H., Birner, T., and Rupp, P.: Circulation aspects associated with heat wave events over Iraq, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-307, https://doi.org/10.5194/egusphere-egu23-307, 2023.

EGU23-459 | ECS | Posters on site | AS1.17

Investigating the Hadley Cell and eddies with varying sea surface temperature gradients 

Abu Bakar Siddiqui Thakur, Jai Sukhatme, and Nili Harnik

We examine the tropical meridional overturning circulation in an aquaplanet GCM with fixed orbital parameters and uniform insolation angle. The atmosphere is forced by an imposed non-interactive sea surface temperature (SST) distribution which is varied between present-day Earth-like to a latitudinally uniform profile. A conventional Hadley Cell (HC) -like flow is observed in all experiments along with the poleward transport of energy and momentum. In simulations forced by a non-zero SST gradient, latent heat released from organized convection near the equator sets up a deep tropical cell. Rossby wave activity generated near the extratropical surface propagates upward and turns equatorward on reaching the tropopause. These waves break on the edge of the HC, fluxing heat and momentum poleward and reinforcing a thermally direct cell in the same sense as the HC. When the SST distribution becomes globally uniform, the traditional midlatitude Rossby waves are trapped near the surface as the mean flow inhibits their upward propagation. But, near the tropopause, baroclinicity generates waves that ride on a sharp upper tropospheric potential vorticity gradient. These waves propagate downwards towards the lower equatorial troposphere and transport angular momentum out of the tropics. Together with a dominant MJO-like mode, which facilitates near-equatorial convergence, this leads to a conventional tropical overturning circulation. As the SST gradient weakens, the HC moves from a regime intermediate to thermally and eddy-driven to one that's strongly influenced by eddies. Moreover, the thermal structure of the troposphere becomes uniform with weak gradients, and for flat SSTs, the tropopause in the midlatitudes is also set by convection. A Transformed Eulerian Mean perspective is consistent with this view and highlights the diabatic nature of the midlatitude circulation in the limit of flat sea surface temperatures.

How to cite: Thakur, A. B. S., Sukhatme, J., and Harnik, N.: Investigating the Hadley Cell and eddies with varying sea surface temperature gradients, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-459, https://doi.org/10.5194/egusphere-egu23-459, 2023.

Extratropical Rossby waves intrude over tropical region as well as the Indian region and exert significant influence on the weather features. Over Indian region, the pre-monsoon is a dry summer season. During this season, several studies have identified drivers of heatwaves based on different aspects such as the synoptic-scale systems, regional factors, and large-scale teleconnection patterns around the globe (Perkins 2015). Essentially these drivers identified for the Indian region do not describe the heatwave events as the intensification of some modes. Midlatitude heatwaves, on the other hand, are identified as the extreme phase of Rossby Wave mode amplification. However, over the Indian region studies do not explicitly point out the existence of temperature intraseasonal modes during April-May over the Indian region, and it is not clear if some of the drivers of heatwaves can also explain the April-May temperature variations during heatwaves as derivatives (or amplification) of some subseasonal modes. This study identifies the dominant pair of the intrinsic mode of temperature intraseasonal oscillations (ISO) related to subtropical and extratropical Rossby waves, which can also explain the heatwave spikes.

            The ISO modes are derived using the empirical orthogonal function analysis of the detrended surface temperature and further regression analysis demonstrates the dynamical origin of these spatial modes. It is found that both the modes are driven by the mid-latitudinal Rossby waves which propagate towards the Indian region following the ‘preferred teleconnection pathways’ (Ambrizzi and Hoskins 1997). The dominant mode is related to the subtropical westerly jet waveguide, and the second mode is induced by the extratropical to European eddy-driven jet which follows the Europe-Middle East-Indian Ocean pathway. From the different phases of the oscillation obtained from these modes, two phases are favorable for the extreme temperature events and these two phases account for more than 50% of the extreme event occurred over the Indian region.

            Global warming is however steering these two inherent modes of ISOs in surface temperature with the first mode having a significant decreasing trend and the second mode showing an increasing trend. The modal difference in trend is likely to be related to the weakening of the subtropical jetstream waveguide and the strengthening of the extratropical jetstream in a warming scenario (Archer and Caldeira 2008). The usefulness of this study is that the ISOs defined in this study could explain the maximum number of extreme temperature events occurring over the Indian region as a projection on two temperature modes. The modal trend could also account for the regional asymmetry of warming over the Indian region in the global warming scenario, and is related to the trend in jetstream waveguide those steers these modes towards the Indian region.

References

Ambrizzi T, Hoskins BJ (1997) Stationary rossby-wave propagation in a baroclinic atmosphere. Q J R Meteorol Soc 123:919–928. https://doi.org/https://doi.org/10.1002/qj.49712354007

Archer CL, Caldeira K (2008) Historical trends in the jet streams. Geophys Res Lett 35:. https://doi.org/https://doi.org/10.1029/2008GL033614

Perkins SE (2015) A review on the scientific understanding of heatwaves—Their measurement, driving mechanisms, and changes at the global scale. Atmos Res 164–165:242–267. https://doi.org/https://doi.org/10.1016/j.atmosres.2015.05.014

How to cite: Saradambal, L. and Chattopadhyay, R.: Propagation of Mid-Latitudinal Rossby waves along the Jetstream waveguides and their Role in Summer Temperature Intraseasonal Oscillations and Extremes over the Indian Region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1199, https://doi.org/10.5194/egusphere-egu23-1199, 2023.

We examine regional and seasonal variations of extratropical storm tracks and their maintenance in terms of a column-mean local wave activity budget.  Seasonal climatology of wave activity in ERA5 reveals spatial and temporal variations of storm tracks in both hemispheres broadly consistent with previous studies based on other metrics. The seasonal-mean budget consists of horizontal convergence of wave activity fluxes, input from the surface (the upward Eliassen-Palm flux), a small storage, and the residual. When averaged hemispherically, surface injection of wave activity due to baroclinic instability and forced stationary waves is balanced by a negative residual (dissipation) due to mixing and radiative damping.

However, the budget terms show considerable zonal, meridional and seasonal variations, especially in the Northern Hemisphere. Wave activity migrates downstream from a source region to a sink, where the residual is negative and largely balanced by flux convergence. In addition to the surface sources in the regions of strong baroclinicity, the residual term, though negative on average, shows significant positive values where cloud water abounds, suggesting diabatic (and/or nonquasigeostrophic) sources of wave activity.

By reconstructing the budget driven by a fixed transport velocity and damping rate evaluated from the seasonal climatology but suppressing the positive residual values, we estimate the impact of diabatic sources on the mean wave activity. It is found that the diabatic sources contribute to 26% and 20%, respectively, of North Atlantic and North Pacific storm track activities in winter, 28% of wave activity over the Pacific Northwest in summer, and 34% of activity in the Indo-western Pacific sector of the austral storm track in summer.

How to cite: Nakamura, N.: How much does diabatic heating affect storm track activity?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2533, https://doi.org/10.5194/egusphere-egu23-2533, 2023.

Clustering extreme rainfall events are successive occurrences over multiple regions. As climate continues to warm up, cluster occurrence is becoming a prevailing feature of extreme weather events and leading to significant socioeconomic impacts. Understanding the associated atmospheric teleconnection patterns and their underlying mechanisms can help quantify their risk, i.e., the probability of occurrence and severity of cluster extremes in the future. In this study, we identified over 400 events of clustering extreme rainfall events over South Asia, East Asia, and North America in the past 42 years. Diagnostic analyses of these events reveal the diversity of teleconnection that paved the road to the events. Three Rossby wave patterns: (1) circum-Pacific Rossby wave, (2) cross-Pacific Rossby wave, and (3) Pacific anticyclone Rossby wave breaking, are the major synoptic-scale dynamics responsible for clustering rainfall events. Specifically, the circum-Pacific Rossby wave dominates in autumn and early winter, while the cross-Pacific Rossby wave pattern prevails during the Indian summer monsoon season. The occurrence frequency of the anticyclone Rossby wave breaking does not show significant seasonal differences.

The key driving mechanisms behind these wave patterns are: 1) The poleward propagation of the circum-Pacific wave can be excited by the heating anomaly originating in the tropics. 2) The mid-latitude cross-Pacific Rossby wave is a portion of the circum-global teleconnection pattern. This recurrent Rossby wave connects Asia and North America, influenced by the Indian summer monsoon. 3) Pacific anticyclone Rossby wave breaking is a quasi-stationary synoptic wave pattern causing persistent extreme weather. The frequency of this pattern increases significantly during La Niña years with a relatively weak subtropical jet. The single or synergistic effects of these three patterns cause the cluster occurrence of extreme rainfall. Findings from this work offer a better understanding of rainfall teleconnection and tropic/midlatitude interaction.

How to cite: Song, Y. and Lu, M.: Cluster occurrence of extreme rainfall events over Indo-Pacific and their associated diverse Rossby wave patterns, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2751, https://doi.org/10.5194/egusphere-egu23-2751, 2023.

EGU23-3115 | ECS | Posters on site | AS1.17

Jet streaks from a PV gradient perspective: A Lagrangian analysis of diabatic-adiabatic interaction in km-scale simulations 

Mona Bukenberger, Stefan Rüdisühli, and Sebastian Schemm

The jet stream is a circumpolar global band of high wind speeds in the upper troposphere. Meridional meanders of the jet lead to high-impact weather events and may synchronize them over thousands of kilometres. As a Rossby waveguide, the jet influences paths of synoptic-scale eddies, which in turn alter jet dynamics. Coherent regions of enhanced wind speed, so-called jet streaks, typify the jet locally and anomalously strong jet streaks often coincide with extreme precipitation and wind events.

Despite their relevance, process understanding remains limited regarding the formation of jet streaks in interaction with lower-level weather systems. The same is true for the influence of jet streaks on Rossby wave evolution. One way to further the understanding of jet streak dynamics is to study the interaction between adiabatic and diabatic processes during jet streak evolution. However, the relative importance of those processes is difficult to disentangle. 

This study utilises a Lagrangian-based PV gradient perspective by applying it to a jet streak relative coordinate system to obtain composites throughout the lifecycles of multiple jet streak events. The theoretical foundation of this approach is the link between the horizontal isentropic PV gradient and wind speed. Local maxima of the normalised isentropic PV gradient are collocated with centers of jet streaks. As PV is conserved under adiabatic and frictionless flow, the PV gradient perspective allows for an investigation of diabatic-adiabatic interaction.

We analyse a convection-resolving 1.1 km COSMO simulation in the eastern North Atlantic in autumn 2016, using PV gradient analysis and online air parcel trajectories to separate diabatic and adiabatic contributions to jet streak development. Cloud processes play an important role in the establishment and maintenance of a strong event, while the dynamics of a weaker jet streak is dominated by effects of adiabatic deformation.

After demonstrating the approach in two case studies, we present results from a composite analysis of multiple jet streak events to achieve a more systematic understanding of diabatic-adiabatic interaction during their evolution.

How to cite: Bukenberger, M., Rüdisühli, S., and Schemm, S.: Jet streaks from a PV gradient perspective: A Lagrangian analysis of diabatic-adiabatic interaction in km-scale simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3115, https://doi.org/10.5194/egusphere-egu23-3115, 2023.

EGU23-3912 | ECS | Posters on site | AS1.17

The Role of North American Convective Storms on Jet Stream Dynamics: A Negative Potential Vorticity Perspective 

Alexander Lojko, Andrew Winters, Christiane Jablonowski, and Ashley Payne

Synoptic-scale filaments of negative potential vorticity (PV) in the northern hemisphere tropopause can form adjacent to the jet stream in the presence of convection and moderate shear (i.e., severe thunderstorm environments). Case-studies have shown that synoptic-scale negative PV can influence in-situ jet stream dynamics. Negative PV arises due to strong vorticity in convective updrafts, driven by the horizontal gradient of diabatic heating (O < 10 km).  Its origin from scales not resolvable by contemporary global weather models can thus also impinge on jet stream forecast skill.

Nevertheless, little is still known about the characteristics of synoptic-scale negative PV. How frequently is it observed? And what are its ‘typical’ impacts on the jet stream?

Focusing on North America where severe thunderstorms are frequent, we design an algorithm that tracks the temporal evolution of closed contours of upper-level, negative PV air using ERA5 data. We composites instances in which it is in close-proximity to (‘interacts with’) the jet stream and assess its dynamical response. The role of negative PV on jet evolution and its downstream response over the Atlantic is facilitated through a combination of lagged composite analysis and K-means clustering.

Our composite results in combination with preliminary high-resolution model simulations highlight that elongated bands of negative PV frequently interact with the jet stream, intensify jet wind maxima and may serve as an amplification source for Rossby waves.

How to cite: Lojko, A., Winters, A., Jablonowski, C., and Payne, A.: The Role of North American Convective Storms on Jet Stream Dynamics: A Negative Potential Vorticity Perspective, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3912, https://doi.org/10.5194/egusphere-egu23-3912, 2023.

EGU23-3942 | ECS | Orals | AS1.17

Persistent anomalies of the North Atlantic jet stream and associated surface extremes over Europe 

Vera Melinda Galfi and Gabriele Messori

Persistent unusual configurations of the North Atlantic jet stream affect the weather and climate over Europe. We focus on winter and on intraseasonal and seasonal time scales, and study persistent jet anomalies through the lens of large deviation theory using CMIP6 simulations of the MPI-ESM-LR model and ERA5 reanalysis data. Our results show that persistent temperature and precipitation extremes over large European regions are anomalously frequent during the unusual, persistent jet configurations we identify. Furthermore, the relative increase in frequency of surface extremes is larger as we consider more intense surface extremes and/or more extreme jet anomalies. The highest extreme event frequencies at the surface are observed in case of precipitation over the Mediterranean and Western Europe during anomalously zonal and/or fast jet events, pointing to these jet anomalies matching rather homogeneous large-scale atmospheric configurations with a clear surface footprint. Additionally, our results emphasise the usefulness of large deviation rate functions to estimate the frequency of occurrence of persistent jet anomalies, and more generally of unusual, persistent atmospheric circulation patterns.

How to cite: Galfi, V. M. and Messori, G.: Persistent anomalies of the North Atlantic jet stream and associated surface extremes over Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3942, https://doi.org/10.5194/egusphere-egu23-3942, 2023.

EGU23-5448 | ECS | Orals | AS1.17

A new atmospheric background state to diagnose local waveguidability 

Christopher Polster and Volkmar Wirth

Rossby waveguides constrain the propagation of Rossby waves by ducting eddy activity along paths of enhanced waveguidability in the atmosphere. Conceptually, waveguidability is the property of an eddy-free background state on which waves exist as perturbations. Because eddies are always present in the atmosphere, a procedure is required to separate the waves from the background. The choice of procedure is of practical importance when diagnosing waveguides. For example, a zonal-mean background state is easy to compute from data and often used, but does not allow for longitudinal variation of waveguidability. It has also been shown to exhibit waveguide artifacts in the presence of finite-amplitude eddies.

We introduce a new procedure to obtain an eddy-free background state for the analysis of waveguides in the atmosphere. It utilizes a redistribution (so-called zonalization) of Ertel potential vorticity on isentropes to remove eddies, including those of finite amplitude, while retaining local information. Because the procedure can be applied to instantaneous data without a need for temporal aggregation, it is suitable for causal analyses and can be applied to forecast data without lead time restrictions. Our construction is based on the "slowly evolving background state" by Nakamura and Solomon (2011) and Methven and Berrisford (2015), with additions and approximations to achieve a pragmatic compromise between theoretical grounding, usability and ease of computation.

The effectiveness of the procedure to meaningfully separate waves and the background state is illustrated with reanalysis data. Rossby waveguides are diagnosed from the background-state PV fields with a gradient-based metric. We show that our localized procedure leads to regional differences in the diagnosed waveguidability and discuss the existence of circumglobal waveguides.

How to cite: Polster, C. and Wirth, V.: A new atmospheric background state to diagnose local waveguidability, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5448, https://doi.org/10.5194/egusphere-egu23-5448, 2023.

EGU23-5969 | ECS | Posters on site | AS1.17

Winter North Atlantic jet variability under global warming: Past trends and future projections 

Alejandro Hermoso and Sebastian Schemm

Regional weather variability and the occurrence of extreme weather events are highly connected to the position of jet streams. Climate models generally project a poleward shift of the jets under the influence of anthropogenic warming. However, ERA5 reanalysis data show that the North Atlantic jet stream in winter has roughly remained in place. We investigate the mechanisms that lead to this behavior.  The analysis reveals that upper-level temperature trends produce a reduction in stability that leads to an increase in baroclinicity. Furthermore, momentum convergence is also intensified across the jet core, producing an acceleration of the jet and not a weakening as suggested by arguments based solely on the Artic amplification. 

 

Numerical simulations from an ensemble of fully coupled climate simulations run with the Community Earth System Model under the SSP3.7 scenario are also analyzed along with idealized warming experiments in an aquaplanet setup with a zonal asymmetry in sea surface temperature. The climate simulations exhibit a large spread during the historical period and only a few ensemble members reproduce the observed trends, suggesting that trends only based on ensemble means could lead to misleading projections. Additionally, the aquaplanet runs display high sensitivity to the location of the asymmetry. This provides a supplementary argument in support of inspecting all individual climate projections as small variations in the original jet position can lead to large disparities in the projected trends. 

How to cite: Hermoso, A. and Schemm, S.: Winter North Atlantic jet variability under global warming: Past trends and future projections, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5969, https://doi.org/10.5194/egusphere-egu23-5969, 2023.

EGU23-7466 | ECS | Orals | AS1.17

On the relationship between Atmospheric Blocking and Arctic Amplification 

Marco Cadau, Giorgia Fosser, Simona Bordoni, Gianmaria Sannino, and Marco Gaetani

Atmospheric blocking is known to be one of the most important drivers of large-scale atmospheric variability at mid-high latitudes. Blocking events consist of a disruption and/or deceleration of the mean westerly circumpolar flow, and are generally associated with large-scale high-pressure patterns, which may be connected with the occurrence of climate extremes, such as heat waves and cold spells. Atmospheric dynamics in the Arctic region may be very important in shaping the spatial and temporal patterns of blocking at mid-high latitudes, and consequently the occurrence of associated climate extremes. In particular, Arctic Amplification (AA), namely the recent amplified warming in the Arctic region compared to lower latitudes, has recently been argued to have an impact on blocking patterns and behaviour at mid-high latitudes.

The objective of this study is to investigate the most relevant mechanisms playing a role in the relationship between blocking and Arctic Amplification, by analysing the variability and frequency of the associated spatial patterns at various timescales using variables from the ERA5 reanalysis dataset for the time interval 1959-2022. Blocking events are detected based on geopotential height gradients between mid- and high-latitude regions, while Arctic Amplification is quantified as the difference of 1000hPa temperature between high and mid latitudes.

The climatological number of events per year and their average lifetime, along with the long-term trends and their relationship with the AA are analysed. Furthermore, possible mechanisms linking blocking variability and the AA are explored through the analysis of the jetstream dynamics and teleconnection patterns in the Northern Hemisphere.

How to cite: Cadau, M., Fosser, G., Bordoni, S., Sannino, G., and Gaetani, M.: On the relationship between Atmospheric Blocking and Arctic Amplification, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7466, https://doi.org/10.5194/egusphere-egu23-7466, 2023.

Since 1980, the U.S. experienced 338 different billion-dollar weather and climate disasters, with greater than 25% (n = 96) of these occurring in the cold season of December–March. These events can have lasting societal and economic impacts that make diagnosing their likelihood of occurrence in the next week, season, or decade an important problem in the context of our changing climate. This analysis will focus on a case study of the predictability and dynamics of the 2021 US cold air outbreak (CAO) and provide a multiscale overview of the event on subseasonal-to-seasonal (S2S) timescales. The analysis of the dynamics focuses on the role of the stratospheric recovery from the January 2021 sudden stratospheric warming and a stratospheric Rossby wave reflection event in the context of the development of high amplitude flow in early February 2021. The second part considers the ability of S2S forecast models to resolve the predecessor events to this CAO. The predictability of this CAO and the role of the stratosphere in the development of CAO are considered by analyzing both high-top and low-top S2S forecast model from the S2S prediction Project Database.

How to cite: Lang, A.: The dynamics and predictability of US winter extremes—a multiscale case study of the 2021 U.S. cold air outbreak, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7975, https://doi.org/10.5194/egusphere-egu23-7975, 2023.

EGU23-8062 | ECS | Orals | AS1.17

Potential Role of Inter-Basin Interactions in Eurasian Summer Blocking 

Lina Boljka, Nour-Eddine Omrani, Ho-Nam Cheung, Noel Keenlyside, Hisashi Nakamura, Clemens Spensberger, and Fumiaki Ogawa

Atmospheric blocking events are persistent tropospheric weather patterns that are associated with extreme events, such as heatwaves. In the summer, they primarily occur at high latitudes, e.g., over northern Eurasia. However, blocking frequency over these regions is underestimated in climate models, and often overestimated over the midlatitudes, while causes for such discrepancies remain elusive. To improve model representation of blocking frequency, it is important to understand different processes that affect it. Here, we explore blocking frequency in a reanalysis and experiments with an atmospheric general circulation model forced with different sea surface temperature (SSTs) profiles. The configurations range from an idealized no SST-front experiment and prescribing idealized SST-front in different regions to prescribing realistic climatological SSTs. Surprisingly, this reveals that more idealized (realistic) experiments lead to more (less) realistic blocking frequency. We find that weaker (less realistic) blocking frequency over northern Eurasia is primarily caused by the circulation changes related to SST gradients over the North Pacific. This suggests an important role of inter-basin interactions between the Atlantic and the Pacific. Additionally, tropical teleconnections can also play a role. This may suggest that models struggle with circulation response to SSTs in boreal summer, especially over the North Pacific. Thus, this work has implications for simulating (future) summer heat (and other) extremes over the high latitudes.

How to cite: Boljka, L., Omrani, N.-E., Cheung, H.-N., Keenlyside, N., Nakamura, H., Spensberger, C., and Ogawa, F.: Potential Role of Inter-Basin Interactions in Eurasian Summer Blocking, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8062, https://doi.org/10.5194/egusphere-egu23-8062, 2023.

The successful prediction of heatwave onsets on the medium-range forecast time scale (here, 5-12 days) mainly relies on the adequate forecasting of large-scale Rossby wave patterns and their dynamics. In the mid-latitude regions of Europe, lasting heatwaves are often associated with a substantial blocking of the large-scale atmospheric flow due to amplified and/or breaking Rossby waves. To characterize such anomalous flow configurations, which may come in different patterns, we adopt the concept of Euro-Atlantic weather regimes. Based on Empirical Orthogonal Function analysis and subsequent k-means clustering, this widely-used metric reduces the complexity of the atmospheric flow field by projecting it onto the seven main modes of synoptic-scale variability in this domain.  In this study, we therefore examine heatwave characteristics in different European regions in relation to Euro-Atlantic weather regimes. A focus is set on the question to which extent the medium-range predictability of heatwave onsets depends on the current or preceding weather regime as well as to flow anomalies further upstream or other potential precursors not directly related to Rossby wave dynamics such as abnormally dry soils. 

Heatwaves are objectively diagnosed as a 90th percentile exceedance in 2m maximum temperatures for a minimum of 3 days in both a local and regional context.  Using ERA-5 data for the period 1979-present, we find that British and Scandinavian heatwaves are mainly associated with classic blocking regimes (Scandinavian and European blocking), whereas the picture is more diverse for Central Europe where the „no regime“ case is also frequently observed. Remarkably, over the last 20 years, European heatwaves associated with a European blocking seem to be significantly related to pre-existing anomalously dry soils over large parts of Northern America which is, however, not the case for heatwaves related to any other weather regime. 

The medium-range predictability of heatwaves is investigated for the period 2001-2018, using hindcast ensembles of two state-of-the art weather forecast models ECMWF-IFS and GEFS-v12, by means of usual metrics such as 500hPa geopotential anomaly correlation coefficients (ACC) and 850hPa temperature mean absolute errors. Preliminary results with a focus on Central Europe suggest that heatwaves in this region seem to be slightly more predictable (roughly one more day until ACC drops below 0.8) when they occur in conjunction with a Scandinavian or European blocking compared to the case with no apparent regime. This may be explained by the overall more transient and phase-error prone nature of the „no regime“-type heatwaves. Interestingly, heatwaves with the worst predictability at 10 days lead time show an intensified jet stream over the Atlantic one week prior and a slight tendency toward wetter than normal soils over North America and Central Europe.

Finally, we also investigate to which extent medium-range forecasts of local maximum temperatures further depend on more local, diabatic processes (soil moisture, cloud cover forecast) and whether there are systematic differences between lead times and weather regimes.

How to cite: Lemburg, A. and Fink, A. H.: Investigating European heatwaves and their medium-range predictability in relation to weather regimes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8139, https://doi.org/10.5194/egusphere-egu23-8139, 2023.

EGU23-8210 | Orals | AS1.17

A linearized approach to study stability and waveguidability of barotropic Rossby waves 

Antonio Segalini, Jacopo Riboldi, Volkmar Wirth, and Gabriele Messori

The propagation and the characteristics of Rossby waves are influenced by the large-scale background flow where they occur: for instance, the role of upper-level jet streams in promoting Rossby wave propagation along preferred directions (so-called “waveguidability”) is a classic problem in climate dynamics. We propose a linear framework to study barotropic Rossby waves over a spherical domain for arbitrary orographic forcing and zonal background flow configurations, including cases with localised single and double jet streams. The approach allows to analytically obtain the steady-state linear flow response to orographic forcing without performing lengthy numerical integrations, together with the flow evolution as a combination of few modes composed by the various eigensolutions of the unforced problem (thus independent of the forcing). The connection between jet strength and waveguidability noticed by previous studies is confirmed. Background flow states featuring a strong jet stream are also prone to barotropic instability.

The eigenvalue analysis reveals the spatial structure of the associated Rossby modes and their growth rates, allowing to detect the presence of instabilities. We notice that, even in presence of a damping term, some background flow configurations allow wave instabilities to exist. According to the linear theory, the flow should diverge from the equilibrium state, since some waves are linearly unstable. Nonlinear simulations are performed to provide insights about the waves evolution in the unstable case. Such simulations reveal two interesting effects: 1) a damping effect operated by the nonlinear terms (i.e., the flow is unstable linearly but stable nonlinearly) for medium jet strengths; 2) a quasi-periodic behaviour around the unstable equilibrium state for the strongest jets, indicating the existence of a limit cycle. The linear analysis was still able to capture the unstable equilibrium state at the center of the limit cycle and to provide insights about the spatial structure of the dominant modes. These results indicate the usefulness of linearized approaches in the development of a reduced-order model to describe the barotropic instability mechanisms driving spherical Rossby waves.

How to cite: Segalini, A., Riboldi, J., Wirth, V., and Messori, G.: A linearized approach to study stability and waveguidability of barotropic Rossby waves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8210, https://doi.org/10.5194/egusphere-egu23-8210, 2023.

EGU23-8331 | ECS | Orals | AS1.17

Extremes of meridional energy transports in Northern Hemisphere mid-latitudes across zonal wavenumbers and dominant weather regimes 

Valerio Lembo, Federico Fabiano, Vera Melinda Galfi, Rune Grand Graversen, Valerio Lucarini, and Gabriele Messori

Extremes in extratropical meridional energy transports in the atmosphere are associated with the dynamics of the atmosphere at multiple spatial scales, from planetary to synoptic. This is related to the nature of amplifying baroclinic waves, that are fundamentally intermittent and sporadic, significantly affecting the net seasonal transport across latitudes. Here, we use the ERA5 reanalysis data to perform a wavenumber decomposition of meridional energy transports in the Northern Hemisphere mid-latitudes during winter and summer. Extreme transport events are linked to atmospheric circulation anomalies and dominant weather regimes, identified by clustering 500 hPa geopotential height fields. Partitioning the extreme events across zonal wavenumber highlights the different role of scales in different seasons and regions. In general, planetary-scale waves determine the strength and meridional position of the synoptic-scale baroclinic activity with their phase and amplitude. During winter, large wavenumbers (k = 2–3) are key drivers of the meridional-energy-transport extremes, and planetary- and synoptic-scale transport extremes virtually never co-occur. In summer, extremes are associated with higher wavenumbers (k = 4–6), identified as synoptic-scale motions. Focusing on recently occurred exceptionally strong summertime heat waves and wintertime cold spells, we notice that regime structures of these events are typical of extremely large poleward meridional energy transports.

How to cite: Lembo, V., Fabiano, F., Galfi, V. M., Graversen, R. G., Lucarini, V., and Messori, G.: Extremes of meridional energy transports in Northern Hemisphere mid-latitudes across zonal wavenumbers and dominant weather regimes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8331, https://doi.org/10.5194/egusphere-egu23-8331, 2023.

EGU23-8399 | ECS | Posters on site | AS1.17

Jet Regimes Induced by Stratification Changes in a Dry Dynamical Core Model 

Pablo Conrat Fuentes, Thomas Birner, and Hella Garny

The tropical circulation is typically not well represented in idealized models used to study jet dynamics. 
We implement a convective relaxation algorithm into a dry dynamical core model following Schneider and Walker (2006) to improve the representation of the driving mechanism behind the subtropical jet: the tropical meridional overturning.
We study the dependence of the general circulation on the vertical stratification set by a convective relaxation scheme.
Varying tropospheric lapse rates produces two jet regimes that are characterized by the distance between the subtropical jet and the eddy-driven jet.
The separated jet state features distances of more than 12° latitude between subtropical and eddy-driven jet and is dominant in simulations with higher tropospheric static stability.
Both jets approximately coincide in the joined jet regime, which is dominant in lower stability simulations.

In addition to a steady state analysis, transitions from one regime to the other are induced by changes in convective lapse rate.
Regime changes are also observed as events produced by natural variability in some of the model runs.
This time-dependent perspective shows that the structure of net Rossby wave dissipation in the upper troposphere, measured by the Eliassen-Palm flux divergence, is crucial in order to understand the regimes.
Jet merge and split events are mediated by upper tropospheric momentum flux variability.
They are preceded by heat flux variability and are tied to variations in the hemispheric eddy kinetic energy.
The results are also interpreted through the concept of criticality, relating meridional and vertical gradients in potential temperature.
The analysis highlights the importance of static stability and its changes to mid-latitude jet dynamics.

How to cite: Conrat Fuentes, P., Birner, T., and Garny, H.: Jet Regimes Induced by Stratification Changes in a Dry Dynamical Core Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8399, https://doi.org/10.5194/egusphere-egu23-8399, 2023.

EGU23-8465 | ECS | Posters on site | AS1.17

Long-term variability of Rossby Wave Breaking events over the Indian subcontinent 

Biyo Thomas, Ravi Kumar Kunchala, Bhupendra Bahadur Singh, and Niranjan Kumar Kondapalli

The synoptic scale upper level Rossby wave breaking (RWB) has a great influence on the weather pattern on the underlying regions. The RWB events have been studied extensively in the mid-latitude regions as it is prone to such events which often lead to extreme weather conditions. However, studies are elusive especially over the Indian sub-continent except few cases. RWB climatology and variability on monthly, interannual as well as on decadal scales is still poorly understood over this region. To address these shortcomings, in this study, we have used the reanalysis data and implemented a contour searching algorithm to identify RWB events over the period 1979-2021. Using the implemented algorithm, we have detected 513 RWB events for the study period which we further use to examine RWB climatology and variability over the subcontinent (5-40oN, 55-105oE). Our results suggest a significant increase in the number of RWB events per year during the last  two decades, as well as an increase in the intensity over the northwest region of the Indian subcontinent. We note that the RWB frequently affects the northwest region in winter, which later shows a shift in peak number of occurrences of RWB towards central India at the end of winter. This shift is linked to seasonal changes in the background zonal wind in the upper-troposphere. Also, the monthly climatology of vertical intrusions of the PV streamers indicate that intrusions are stronger during winter than other months. In addition, the role of RWB on the dynamical changes of the atmosphere such as anomalies of wind circulation patterns and moisture content is analyzed using composite analysis. The variability of the RWB events and its linkages with global sea surface temperature particularly conditions in the Pacific Ocean have also been studied.

How to cite: Thomas, B., Kunchala, R. K., Singh, B. B., and Kondapalli, N. K.: Long-term variability of Rossby Wave Breaking events over the Indian subcontinent, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8465, https://doi.org/10.5194/egusphere-egu23-8465, 2023.

When different weather extremes occur at multiple locations at the same time, their aggregated impact can exceed the one of the individual events. Examples can be concomitant summer heatwaves over major breadbasket regions, leading to potential food shortages at the global scale, or the connection between cold spells over North America and windstorms over Europe. These compound events often attract a broad interest by the media and society, as anomalous weather conditions seem to occur “everywhere at the same time”. If it is possible to identify a physical linkage between them, those separate extremes can be considered as parts of a single, spatially compounding weather extreme. Pinpointing a common physical driver is not trivial, however, and it might well be that such extreme events just co-occur by coincidence.

This overview presentation will discuss how the linear and nonlinear dynamics of Rossby waves can help to understand spatially compounding extremes. Examples of linear dynamics involve the propagation of Rossby wave packets across broad portions of the middle latitudes, aided by the presence of upper-level waveguides. The link between extreme weather and atmospheric blocking, on the other hand, can be seen as involving a nonlinear sort of dynamics. Analytical, idealized and data-driven approaches to the study of Rossby waves can shed light on the drivers of spatially compounding extremes, and result in useful tools to study how the drivers of such extremes are being affected by anthropogenic global warming.

How to cite: Riboldi, J.: On the connection between Rossby waves and spatially compounding weather extremes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8587, https://doi.org/10.5194/egusphere-egu23-8587, 2023.

EGU23-8620 | ECS | Posters on site | AS1.17

Variability of beta-plane zonal jets 

Wenzhong Wang and Peter Haynes

The dynamics of the mid-latitude atmospheric jet is an important component of internal variability in real and modelled climate. The variability may also potentially affect the response to deterministic external forcing, with implications for seasonal prediction including the ‘signal-to-noise’ paradox. Recent research has used ad hoc probabilistic approaches to investigate the paradox but has given little dynamical insight into the behaviour observed in models. This motivates further dynamical study of the factors determining variability and response to forcing. We use a simple stochastically forced barotropic model containing the essential mechanisms for beta-plane jet variability to conduct a range of numerical experiments. We consider first the dependence of the behaviour on the damping time scale and on the amplitude and latitudinal width of stochastic forcing that is statistically homogeneous in longitude. We consider leading empirical orthogonal functions of the zonal mean wind velocity, use these as quantifiers of jet behaviour, and analyse the amplitude, latitudinal structure, and autocorrelation time scale of the simulated variability. We move on to examine cases where there is imposed longitudinal variation. An appropriate decorrelation time scale of the zonal jet stream could be displayed by the model, partly depending on the damping time scale. We conduct experiments with applied forcing to determine whether the basic prediction of the fluctuation-dissipation theorem, that response to forcing is proportional to the autocorrelation time scale for natural variability, holds in this system. This simple dynamical model has good implications for a physical understanding of jet persistence and the signal-to-noise paradox. 

How to cite: Wang, W. and Haynes, P.: Variability of beta-plane zonal jets, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8620, https://doi.org/10.5194/egusphere-egu23-8620, 2023.

EGU23-9353 | ECS | Posters on site | AS1.17

A Thermal Wind Perspective of Driving Changes in Jet Stream Patterns 

Mehmet Sedat Gözlet, Joakim Kjellsson, and Mojib Latif

It is evident that the jet streams are becoming more erratic and unstable in a changing climate. We investigate changes both in position and speed of the midlatitude jet streams at 300 hPa in  31 Atmospheric Model Intercomparison Project (AMIP) runs and the ERA5 reanalysis dataset investigating the ability of the thermal wind concept to explain changes in place and the regime of the jet streams, which are disturbed by Arctic amplification, is the core of this work. All data covers the period 1979-2014. 
 
It is revealed that the changes in jet stream magnitude and position in the multi-model mean (MMM) can largely be explained by the thermal wind. We also discovered that the AMIP models reproduce trends in jet position and strength seen in  ERA5. Yet it is a must to state that when inspecting individual models, we find that some models can reproduce ERA5 trends in NH. The large variance in modelled trends, however, leads to a poorly represented MMM.
 
In the end, the jet stream plays a significant role in shaping global weather patterns and is affected by changing climate as becoming more wobbly and unstable. The potential impact of Arctic warming on the jet stream and how it may lead to more extreme weather events in the mid-latitudes is taken under inspection from the window of thermal wind concept with this study. 

How to cite: Gözlet, M. S., Kjellsson, J., and Latif, M.: A Thermal Wind Perspective of Driving Changes in Jet Stream Patterns, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9353, https://doi.org/10.5194/egusphere-egu23-9353, 2023.

EGU23-9918 | ECS | Orals | AS1.17

Extreme weather in the Southern Hemisphere in early 2022: from Rossby waves to planetary-scale conditions 

Andries Jan De Vries, Jake William Casselman, Hilla Afargan-Gerstman, Shingirai Shepard Nangombe, Romain Pilon, Emmanuele Russo, Wolfgang Wicker, Priyanka Yadav, and Daniela I.V. Domeisen

In early 2022, several extreme weather events occurred in the Southern Hemisphere. Devastating floods killed more than 500 people in South Africa (11-12 April) and about 26 people in eastern Australia (24-28 February and 25-31 March), while an unprecedented heatwave broke temperature records in Antarctica (16-22 March). This study presents a multiscale perspective of the atmospheric processes associated with these extreme events from synoptic to planetary scales. Equatorward Rossby wave breaking facilitated the transport of moist air from tropical oceans to the subtropical regions affected by the extreme precipitation events, while poleward Rossby wave breaking forced an intrusion of warm and moist extratropical air masses into the Antarctic Peninsula. Southern hemispheric extratropical wave activity demonstrated relatively normal conditions during February and March, while wave energy reached extremely large values for wave number 5 during April. From a planetary-scale perspective, we investigate how tropical variability, including the El-Nino Southern Oscillation (ENSO; in a La Nina phase) and the Madden-Julian Oscillation (MJO), modulates large-scale atmospheric circulation patterns, extratropical wave activity, and Rossby wave breaking. Overall, this study clarifies the role of regional and remote atmospheric processes in the recent weather extremes in the Southern Hemisphere.

How to cite: De Vries, A. J., Casselman, J. W., Afargan-Gerstman, H., Nangombe, S. S., Pilon, R., Russo, E., Wicker, W., Yadav, P., and Domeisen, D. I. V.: Extreme weather in the Southern Hemisphere in early 2022: from Rossby waves to planetary-scale conditions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9918, https://doi.org/10.5194/egusphere-egu23-9918, 2023.

Wind-driven dust emission from dry, exposed land surfaces plays an important role in the climate system, and also contributes to severe weather and public health hazards around the world. In the past several years, the Northern Hemisphere midlatitude region was stuck by several extreme dust storms with severe socioeconomic and environment consequences within and beyond the dryland source areas. For instance, the 26-27 May 2018 salt storm from the dried-up Aral Sea was considered a first-of-its-kind ecological catastrophe over Central Asia. In March 2021, northern China was hit by the worst sand storm in a decade. Later in November, Uzbekistan recorded the worst dust storm through the country’s meteorological record. Currently, significant knowledge and methodological gaps exist in characterizing the multivariate compound dust events. This study is a first attempt to develop a multivariate approach and ground-based climatology to improve our knowledge of the historical variations, spatial distributions, and governing factors of extreme dust outbreaks over the drylands of Central and East Asia. Detailed case studies will also be conducted to elucidate the role of tropic Pacific and Arctic warming and Rossby wave activities in triggering recent extreme dust events.

How to cite: Xi, X.: A first look at the multivariate extreme dust outbreak over Northern Hemisphere midlatitudes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10425, https://doi.org/10.5194/egusphere-egu23-10425, 2023.

EGU23-12319 | ECS | Orals | AS1.17

Heatwaves of 2018: connecting large-scale to synoptic scale circulation 

Maria Pyrina and Daniela Domeisen

The intensity of heat extremes has been increasing in recent decades, with several recent notable heatwaves afflicting highly populated areas. Previous studies have related heatwaves to slow moving amplified Rossby waves, due to the formation of circumglobal teleconnections (i.e., European heatwaves of 2003 and 2010). Other studies have found that there is a statistical link between high amplitude upper-tropospheric transient Rossby wave packets (RWPs) and increased probability of lower-tropospheric temperature extremes. These non-circumglobal RWP amplitudes were found to be better linked to temperature extremes than Fourier amplitudes quantifying circumglobal waviness, including the European heatwaves of 2003 and 2010. In the summer of 2018, several record-breaking and persistent heatwaves occurred simultaneously around the globe and were linked to an amplified hemisphere-wide wavenumber 7 circulation pattern. Here, we investigate the relation of the synoptic RWPs and the circumglobal characteristics of atmospheric circulation characteristics with the heatwaves during 1998-2018, with a focus on the heatwaves that occurred during the summer of 2018.  Preliminary results show that the dominant circumglobal pattern for the 2018 summer heat extremes was dominated by a zonal wavenumber 6 circulation pattern and that its amplitude was connected to high amplitude RWPs that occur across the Northern Hemisphere.

How to cite: Pyrina, M. and Domeisen, D.: Heatwaves of 2018: connecting large-scale to synoptic scale circulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12319, https://doi.org/10.5194/egusphere-egu23-12319, 2023.

EGU23-12703 | ECS | Orals | AS1.17

Intransitive Atmosphere Dynamics Leading to Persistent Hot–Dry or Cold–Wet European Summers 

Ruud Sperna Weiland, Karin van der Wiel, Frank Selten, and Dim Coumou

Persistent hot–dry or cold–wet summer weather can have significant impacts on agriculture, health, and the environment. For northwestern Europe, these weather regimes are typically linked to, respectively, blocked or zonal jet stream states. The fundamental dynamics underlying these circulation states are still poorly understood. Edward Lorenz postulated that summer circulation may be either fully or almost intransitive, implying that part of the phase space (capturing circulation variability) cannot be reached within one specific summer. If true, this would have major implications for the predictability of summer weather and our understanding of the drivers of interannual variability of summer weather. Here, we test the two Lorenz hypotheses (i.e., fully or almost intransitive) for European summer circulation, capitalizing on a newly available very large ensemble (2000 years) of present-day climate data in the fully coupled global climate model EC-Earth. Using self-organizing maps, we quantify the phase space of summer circulation and the trajectories through phase space in unprecedented detail. We show that, based on Markov assumptions, the summer circulation is strongly dependent on its initial state in early summer with the atmospheric memory ranging from 28 days up to ~45 days. The memory is particularly long if the initial state is either a blocked or a zonal flow state. Furthermore, we identify two groups of summers that are characterized by distinctly different trajectories through phase space, and that prefer either a blocked or zonal circulation state, respectively. These results suggest that intransitivity is indeed a fundamental property of the atmosphere and an important driver of interannual variability.

How to cite: Sperna Weiland, R., van der Wiel, K., Selten, F., and Coumou, D.: Intransitive Atmosphere Dynamics Leading to Persistent Hot–Dry or Cold–Wet European Summers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12703, https://doi.org/10.5194/egusphere-egu23-12703, 2023.

EGU23-14014 | Orals | AS1.17

Potential impact of tropopause sharpness on jet latitude 

Thomas Birner and Lina Boljka

The wintertime extratropical general circulation may be viewed as being primarily governed by interactions between Rossby waves and the background flow. These Rossby waves propagate vertically and meridionally away from their sources and amplify within the core of the tropopause-level jet, which acts as a waveguide. The strength of this waveguide is in part controlled by tropopause sharpness, which itself is a function of the strength of tropopause inversion layer (TIL), a layer of enhanced static stability just above the tropopause. Here, we report a strong relation between interannual-to-multidecadal variations in the strength of the midlatitude TIL and jet latitude in a reanalysis and climate models. Similar relationships hold for the variability across climate models. Experiments with a mechanistic model show that a sharper tropopause promotes an intensified general circulation and an equatorward shifted jet.

Reference: https://doi.org/10.1038/s41612-022-00319-6

How to cite: Birner, T. and Boljka, L.: Potential impact of tropopause sharpness on jet latitude, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14014, https://doi.org/10.5194/egusphere-egu23-14014, 2023.

EGU23-14529 | Posters on site | AS1.17

Summer jet stream response to global af-/reforestation and deforestation 

Iris Manola, Dim Coumou, Fei Luo, Suqi Guo, Felix Havermann, Steven De Hertog, Quenting Lejeune, Inga Menke, Julia Pongratz, Carl Schleussner, Sonia Seneviratne, and Wim Thiery

 

Global-scale af-/reforestation (A/R) and deforestation substantially changes the Earth’s energy and water fluxes, thereby affecting the large-scale atmospheric circulation and thus have significant impacts on weather systems. During summer, A/R and deforestation induced changes in the soil moisture are shown to have an impact on the planetary wave response through the jet stream. Such changes might lead to high-amplitude, quasi-stationary circumglobal Rossby waves that have been associated with extreme summer heatwaves and persistent high-impact extremes. In this study we investigate how idealized global land use and land management changes can alter the boreal summer circulation with a focus on the response of the jet stream. For the analysis we conducted model experiments with three fully coupled Earth System Models (EC-EARTH, MPI-ESM and CESM). Each scenario run for 160 years from which we analyze the final 30 years.  A control run with constant current land use and land management is compared to a global A/R and a global deforestation (global cropland expansion) simulation. In order to assess clean land-atmosphere interactions, all simulations are kept with constant present-day atmospheric forcings (year 2014). We investigate the potential changes in the amplitude of the waves, the likelihood of quasi-stationary wave activity, and of summer blockings within the three different simulations, and the weather consequences that such changes lead to.

How to cite: Manola, I., Coumou, D., Luo, F., Guo, S., Havermann, F., De Hertog, S., Lejeune, Q., Menke, I., Pongratz, J., Schleussner, C., Seneviratne, S., and Thiery, W.: Summer jet stream response to global af-/reforestation and deforestation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14529, https://doi.org/10.5194/egusphere-egu23-14529, 2023.

EGU23-15986 | ECS | Posters on site | AS1.17

Projected changes on quasi-resonant amplification by CMIP5 and CMIP6 toward the persistence in extreme summer weather events 

Sullyandro Oliveira Guimarães, Michael E. Mann, Stefan Rahmstorf, Stefan Petri, Kai Kornhuber, Dim Coumou, Byron A. Steinman, Daniel Brouillette, and Shannon Christiansen

 
High-amplitude quasi-stationary atmospheric Rossby waves with zonal wave numbers 6 to 8 associated with the phenomenon of quasi-resonant amplification (QRA) have been linked to persistent summer extreme weather events in the Northern Hemisphere. We project future occurrence of QRA events based on an index derived from the zonally averaged surface temperature field, comparing results from CMIP5 and CMIP6 (Coupled Model Intercomparison Projects) climate projections. Under the scenarios analyzed, there is a general agreement among models, with most simulations projecting a substantial increase in QRA index. Larger increases are found among CMIP6-SSP585 (42 models, 46 realizations) models with 85% of models displaying a positive trend, as compared with as compared with 60% of CMIP5-RCP85 (35 models, 75 realizations), and a reduced spread among SSP585 models. The CMIP6-SSP370 (24 models, 28 realizations) simulations display qualitatively similar behavior to SSP585, indicating a substantial increase in QRA events under business-as-usual emissions scenarios. Our analysis suggests that anthropogenic warming will likely lead to an even more substantial increase in QRA events (and associated summer weather extremes) than our previous analysis of CMIP5 simulations.

How to cite: Oliveira Guimarães, S., E. Mann, M., Rahmstorf, S., Petri, S., Kornhuber, K., Coumou, D., A. Steinman, B., Brouillette, D., and Christiansen, S.: Projected changes on quasi-resonant amplification by CMIP5 and CMIP6 toward the persistence in extreme summer weather events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15986, https://doi.org/10.5194/egusphere-egu23-15986, 2023.

EGU23-16490 | Posters on site | AS1.17

On the role of Rossby wave phase speed for persistent temperature extremes 

Wolfgang Wicker and Daniela Domeisen

Case studies of mid-latitude summer heatwaves commonly regard stationary synoptic-scale Rossby waves as the primary dynamical forcing. Whether this relationship between upper-tropospheric Rossby wave phase speed and persistent temperature extremes can be generalized is less clear. Here, we evaluate interannual and intra-seasonal variability of Rossby wave phase speed in reanalysis datasets employing circumglobal spectral analysis and investigate episodes with a low or a high zonal phase speed, respectively. Locally, we find evidence of Rossby wave phase preferences during episodes with a low phase speed, where preferred locations of ridges coincide with regions of increased heatwave frequency, but globally, there is no indication of an increased heatwave frequency. Unexpectedly, the finding of Rossby wave phase preferences and increased heatwave frequency also hold for episodes with a high phase speed, although in different areas of the summer hemisphere mid-latitudes. These findings, in particular about episodes with a zonal phase speed, will improve our mechanistic understanding of the dynamical drivers of heatwaves.

How to cite: Wicker, W. and Domeisen, D.: On the role of Rossby wave phase speed for persistent temperature extremes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16490, https://doi.org/10.5194/egusphere-egu23-16490, 2023.

EGU23-16756 | ECS | Orals | AS1.17

Role of Quasi-resonant Planetary Wave Dynamics in Winter Precipitation Extremes over India’s High Mountain Region 

Nischal Sharma, Raju Attada, and Kieran M.R. Hunt

Abstract

Extreme precipitation during winter over the western Himalayas (WH) is associated with western disturbances embedded in sub-tropical westerly jet streams, which are potentially linked to planetary wave dynamics. In this study, we explore a possible connection of quasi-resonant amplification (QRA) to precipitation extremes observed over WH using the global high-resolution reanalysis ERA5 during the period 1979-2019. Precipitation extremes have been identified using percentile approach (peak over threshold) where daily precipitation amount from the entire time series of precipitation exceeds the 95th percentile threshold at a particular grid point. Our analysis suggests that substantially magnified, quasi stationary mid-latitude planetary waves with zonal wavenumbers 6 to 8 accompany these extremes, highlighting the influence of QRA phenomenon. Furthermore, we also identified a fingerprint for QRA occurrence in terms of the zonally averaged surface temperature field. Lastly, we classified extreme precipitation intensities and various related key variables using k-means clustering and analyzed the wavenumbers associated with different categories. Our results underpin the significant role of the QRA mechanism in amplification of planetary waves, in turn, favoring western Himalayan precipitation extremes. Detailed results will be discussed.

Keywords: Quasi-resonant amplification, zonal wavenumber, precipitation extremes, western Himalayas

*E-mail of corresponding author: rajuattada@iisermohali.ac.in

How to cite: Sharma, N., Attada, R., and Hunt, K. M. R.: Role of Quasi-resonant Planetary Wave Dynamics in Winter Precipitation Extremes over India’s High Mountain Region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16756, https://doi.org/10.5194/egusphere-egu23-16756, 2023.

Indian Ocean Dipole (IOD) is an air-sea coupled variability in the Tropical Indian Ocean (TIO), which strongly impacts climate variability over the Indian Ocean rim countries. Though many positive IODs co-occurred with El Niño Southern Oscillation (ENSO), IODs do evolve independently, suggesting the possible role of internal dynamics of the Indian Ocean. In this study, the subtropical IOD (SIOD) is reported as one of the triggers for non-ENSO IODs. The study highlights the existence of cyclic feedback between IOD and SIOD through tropical subtropical interaction, a possible mechanism for the biennial tendency of both IOD and SIOD modes. The positive SIOD induce warming in the southwest of the Subtropical South Indian Ocean (SSIO) during April-May months and creates a meridional cell with subsidence over the southwestern TIO region (10oS). The subsidence expands the existing anticyclonic circulation over SSIO towards the equator and develops easterlies along the equator, warming the western TIO region. A zonal-vertical cell with convection over the western TIO and subsidence over the eastern TIO originates during June-July, which subsequently generates positive IOD in the following months. The positive IOD triggers negative SIOD by developing a stationary Rossby wave train in the midlatitudes. The southeastern anticyclonic circulation develops during the IOD peak season as Gill’s response initiates warm SST anomalies in the northeastern subtropics. As a result of the warming, the evolution of upper-level divergence and high absolute vorticity gradient over the subtropics generate an equivalent barotropic Rossby wave number 3 pattern in the extratropics. The cyclonic circulation over the southwest SSIO related to this Rossby wave pattern creates cold SST anomalies there. The cooling in the southwest and the warming in the northeast SSIO persisted from the IOD peak season, which strengthened the cyclonic circulation over SSIO, reinforcing the existing negative and positive SST anomalies through a positive feedback mechanism and generating negative SIOD, which peaks in the following January-March months.

How to cite: Sebastian, A. and Gnanaseelan, C.: Coupled feedback between the tropics and subtropics of the Indian Ocean with emphasis on the coupled interaction between IOD and SIOD, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-373, https://doi.org/10.5194/egusphere-egu23-373, 2023.

Tropical cyclone (TC) activity varies substantially yearly, and tropical cyclone-related damage also changes. Longer-term prediction of tropical cyclones plays an important role in reducing the wear and human loss caused by TCs. In this study, we have used a Causal-network-based algorithm to find the main development regions and precursors responsible for TC genesis and intensification. However, all the extreme events are interconnected through various global links. Therefore, analysis of the teleconnection and correlation of Tropical Cyclones with El Nino Southern Oscillation (ENSO), Indian Ocean Dipole (IOD), and North Atlantic Oscillation (NAO) during the satellite era (1980-2020) over the North Indian Ocean (NIO) basins using this Causal Effect Network (CEN) based algorithms is checked. The most appropriate metric for cyclone energy is Accumulated Cyclone Energy (ACE); its correlation with the various factors are investigated. We examined the variation in TCs activity during all three phases (positive, negative, and neutral phases).

The results show an increasing trend in ACE over the NIO region during that specific period. The duration of most intense cyclones is increased, but their frequency decreases in this period. A shift in ACE starts after 1997 and still rises significantly. Analysis of Sea Surface Temperature (SST), Vertical Wind Shear (VWS) between 850 and 250 hPa, mid-tropospheric (800 hPa) Relative Humidity (RH), low level (850 hPa) Relative Vorticity (RV), and Tropical Cyclone Heat Potential (TCHP) is done, and it shows positive changes and variability of ACE. These results may help get better knowledge about the atmospheric or oceanic teleconnections between the events, and improved tropical cyclone prediction can help reduce the loss caused by the TCs.        

How to cite: kumar sagar, A.: identification of robust predictors of tropical cyclones using causal effect network over the north indian ocean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-502, https://doi.org/10.5194/egusphere-egu23-502, 2023.

EGU23-595 | ECS | Posters on site | CL4.6

Intra-decadal variability of the Indian Ocean shallow meridional overturning circulation during boreal winter 

Rahul Pai, Anant Parekh, Jasti S Chowdary, and Gnanaseelan Chellappan

The variability of Indian Ocean shallow meridional overturning circulation (SMOC) is studied using the century-long ocean reanalysis simple ocean data assimilation (SODA) data. Though SMOC exhibits stronger southward transport during boreal summer, it displays stronger variability during boreal winter. The spectrum analysis of the winter SMOC index reveals the presence of the highest amplitude between 5 to 7 years at 95% confidence level, suggesting the dominance of intra-decadal SMOC variability. The robustness of intra-decadal SMOC variability is also confirmed in different ocean reanalysis data sets. Composite analysis of filtered upper Ocean Heat Content, sea level, thermocline depth, and Sea Surface Temperature anomalies for strong (weak) SMOC years show negative (positive) anomalies over north and East of Madagascar. Correlation analysis, of filtered SMOC index and sea level pressure (zonal winds) over the Indian Ocean, found a significant negative (positive) correlation coefficient north of 40 °S (around 10 °S) and a significantly positive (negative) correlation coefficient over the 45 °S to 70 °S (20 °S to 50 °S and north of 5 °S). This meridional pattern of the correlation coefficient for sea level pressure, manifesting the out-of-phase relationship between sub-tropics and high latitude mean sea level pressure, resembles Southern Annular Mode (SAM). We conclude that the intra-decadal variability of mean sea level pressure leads to zonal wind variation around 10 °S modulating SMOC, which in turn affects the upper ocean thermal properties in the east and north of Madagascar. This study for the first time brought out coherent intra-decadal evolution of SAM and SMOC during boreal winter.

How to cite: Pai, R., Parekh, A., Chowdary, J. S., and Chellappan, G.: Intra-decadal variability of the Indian Ocean shallow meridional overturning circulation during boreal winter, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-595, https://doi.org/10.5194/egusphere-egu23-595, 2023.

EGU23-864 | ECS | Posters on site | CL4.6

The Teleconnection of Indian Summer Monsoon Clouds with Global Predictors: An Unexplored Measure for Coupled Model development 

Ushnanshu Dutta, Anupam Hazra, Hemantkumar S Chaudhari, Subodh Kumar Saha, Samir Pokhrel, and Utkarsh Verma

The teleconnection studies regarding Indian summer monsoon (ISM) clouds are not focused on detail from both observational and modeling aspects. This is despite the fact that clouds play a seminal role in governing rainfall variability through the modulation of heating and induced circulation. Therefore, we find it essential to explore whether the inter-annual variability of ISM clouds is also remotely influenced by the slowly varying predictable component e.g. Sea Surface Temperature (SST). 

The findings reveal the linkage of observed TCF (and rainfall) over the ISM region with slowly varying forcing (e.g., global SST). The observed/reanalysis teleconnection pattern of TCF-SST is almost similar to that of rainfall-SST.In the long-term period, TCF and SST show a strong and positive correlation with Extra-Tropics (R ~ 0.41), NAO (R ~ 0.51), and AMO (R ~ 0.41) SST regions, in addition to canonical ENSO teleconnection (R ~ −0.39). This is better captured in CMIP6-MME than in CMIP5-MME. The representation of the global teleconnection pattern has been significantly improved in participating models from CMIP5 to CMIP6. The teleconnection with extra-tropics and north Atlantic mode of variability is markedly enhanced in CMIP6-MME compared to CMIP5-MME. The present study has also shown the lag correlations in the teleconnection analysis, i.e., the correlation of June–September (JJAS) mean of rainfall/TCF with October–December (OND) SST from observation/reanalysis, CMIP5-MME, and CMIP6-MME. The CMIP6-MME performs better than CMIP5-MME as compared to observation/reanalysis. 

Thus, the improved understanding of the teleconnection of cloud variables with ENSO and other predictors (ET, NAO, and AMO) will help researchers take up the challenges of improving the ISMR skill far ahead using the new generation coupled climate models. This may facilitate reliable seasonal ISM forecasting.

Keywords: Indian Summer Monsoon, Clouds, Teleconnection, CMIP5, CMIP6

How to cite: Dutta, U., Hazra, A., Chaudhari, H. S., Saha, S. K., Pokhrel, S., and Verma, U.: The Teleconnection of Indian Summer Monsoon Clouds with Global Predictors: An Unexplored Measure for Coupled Model development, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-864, https://doi.org/10.5194/egusphere-egu23-864, 2023.

EGU23-1944 | ECS | Orals | CL4.6

ENSO-driven abrupt phase shift in North Atlantic Oscillation in early January 

Xin Geng, Jiuwei Zhao, and Jong-Seong Kug

El Niño-Southern Oscillation (ENSO) teleconnections exhibit a strong dependency on seasonally and intraseasonally varying mean states, which leads to impactful short-term variations in regional climate. The North Atlantic Oscillation (NAO)-ENSO relation is a typical example, in that its phase relationship reverses systematically between the early and late winter. However, the details and underlying mechanisms of this relationship transition are not well understood yet.

Here based on observations and an ensemble of atmosphere-only climate model simulations, we first reveal that this NAO phase reversal occurs synchronously in early January, which indicates strong abruptness. We demonstrate that this abrupt NAO phase reversal is caused by the change in ENSO-induced Rossby wave-propagating direction from northeastward to southeastward over the northeastern North American region, which is largely governed by a climatological alteration of the local jet meridional shear. We also provide evidence that the North Atlantic intrinsic eddy–low-frequency flow feedback further facilitates and amplifies the NAO responses. This abrupt NAO phase reversal signal is strong enough during the ENSO winter to be useful for intraseasonal climate forecasting in the Euro-Atlantic region.

How to cite: Geng, X., Zhao, J., and Kug, J.-S.: ENSO-driven abrupt phase shift in North Atlantic Oscillation in early January, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1944, https://doi.org/10.5194/egusphere-egu23-1944, 2023.

Weather type classification is a well-established and thoroughly researched field of study in atmospheric sciences. One of its applications is the analysis of occurrence of and transitions between large scale synoptic types. This is typically done by calculating the moving average of, or estimating linear or polynomial fits to relative frequencies. The presented work points out the theoretical inconsistencies implied by such approaches and, instead, employs binomial and multinomial logistic regression for consistent estimation of long-term trends in occurrence and transition probabilities between synoptic types, while assuming first-order Markovian behaviour throughout. The methodological framework's functioning is demonstrated using two prominent examples of weather type classification schemes with regional focus on Germany and central Europe. Temporal refinement to seasonal and monthly level and aggregation into combined groups of classes allows for tracing of observed trends, providing a more comprehensive understanding of the systems investigated. The results, by and large, fit in well with expectations about circulatory changes suggested by research about global warming induced climate change and can be verified by existing research in some cases. Inspection of transition probability changes allows for differentiation between changes in occurrence probability caused by changes in the mean vs. changes in circulatory dynamics. Limitations and favourable implementational details of the approach are determined and the Wald Null test is recommended for assessing statistical significance.

How to cite: Schoeller, H.: Occurrence and Transition Probabilities for two Weather Classification Systems over Germany, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2004, https://doi.org/10.5194/egusphere-egu23-2004, 2023.

EGU23-2125 | Orals | CL4.6

Resolving weather fronts increases the large-scale circulation response to Gulf Stream SST anomalies 

Robert Jnglin Wills, Adam Herrington, Isla Simpson, and David Battisti

Canonical understanding based on general circulation models (GCMs) is that the large-scale circulation responds only weakly to extratropical sea-surface temperature (SST) anomalies, compared to the larger influence of tropical SST anomalies. However, the horizontal resolution of modern GCMs, which ranges from roughly 200 km to 25 km, is too coarse to fully resolve mesoscale atmospheric processes such as weather fronts. Here, we investigate the large-scale atmospheric circulation response to idealized Gulf Stream SST anomalies in a variable resolution version of the Community Atmospheric Model (CAM6), with regional grid refinement of 14 km over the North Atlantic, and compare it to versions with 28-km regional grid refinement and global 111-km resolution. The high-resolution simulations show a large positive response of the wintertime North Atlantic Oscillation (NAO) to positive SST anomalies in the Gulf Stream, a 1-standard-deviation NAO anomaly for 2°C SST anomalies. The lower-resolution simulations show a much weaker response, and in some cases, a different spatial structure of the response. The enhanced large-scale circulation response at high resolution results from an increase in resolved vertical motions, which enables SST forcing to have a larger influence on transient-eddy heat and momentum fluxes. In response to positive SST anomalies, these processes contribute to a stronger North Atlantic jet that varies less in latitude, as is characteristic of the positive phase of the NAO. Our results suggest that the atmospheric circulation response to extratropical SST anomalies is fundamentally different at higher resolution. Regional refinement in key regions offers a potential pathway towards improving simulation of the atmospheric response to extratropical SST anomalies and thereby improving multi-year regional climate predictions.

How to cite: Jnglin Wills, R., Herrington, A., Simpson, I., and Battisti, D.: Resolving weather fronts increases the large-scale circulation response to Gulf Stream SST anomalies, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2125, https://doi.org/10.5194/egusphere-egu23-2125, 2023.

EGU23-5034 | ECS | Orals | CL4.6

Impact of tropical eastern Pacific warming bias on Caribbean climate 

Marta Brotons Blanes, Rein Haarsma, and Nadie Bloemendaal

During the last decades, CMIP5 models simulate a warming trend in the tropical eastern Pacific that has not been present in observations (Seager et al., 2019). Associated with this, the Walker circulation has experienced a westward migration while CMIP5 models simulate an eastward migration. This mismatch is still present in CMIP6 models and might affect climate projections worldwide. In the Caribbean region, CMIP6 models project a strong drying at the end of the 21st century. El Niño-like changes in the Walker circulation are the dominant teleconnections driving the Caribbean drying. The models that project a strong Caribbean drying also simulate generally a strong equatorial eastern Pacific warming trend over the recent decades. Thus, the mismatch between observed and simulated warming trends over the equatorial eastern Pacific questions the reliability of the Caribbean precipitation projections. The warming bias might also have implications for tropical cyclones’ projections in the Atlantic and Pacific through the effect of vertical wind shear, which is related to shifts in the Walker circulation. In addition, the double Intertropical Convergence Zone (ITCZ) bias might be influenced by the mismatching trends. The strong influence of El Niño-Southern Oscillation (ENSO) dynamics on the world’s climate demands more in-depth studies addressing the drivers of the Walker circulation and the equatorial Pacific warming bias.

How to cite: Brotons Blanes, M., Haarsma, R., and Bloemendaal, N.: Impact of tropical eastern Pacific warming bias on Caribbean climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5034, https://doi.org/10.5194/egusphere-egu23-5034, 2023.

Climate change affects the hydrological cycle and induces extreme weather events, such as storms, floods and droughts. Adaptation to climate change needs to be based on assessments of future impacts. The new generation of Coupled Model Inter-comparison Project Phase 6 (CMIP6) is widely used in future flood prediction and drought risk assessment. However, many studies have found that CMIP6 global climate models for simulating land surface water and energy fluxes have significant biases, which poses a problem for using CMIP6 as input data for hydrological impact studies. Therefore, the output of CMIP6 cannot be directly used in hydrological models to project the impacts of future climate change. To overcome this problem, the correction of model output towards observations for its subsequent application in climate change impact studies has now become a standard procedure. And hydrological simulations generally use bias corrected output. But bias correction methods cannot really correct bias. The commonly used bias correction approaches only force the model outputs to match observations, and does not consider the mechanisms within the model and the interaction between variables. This study systematically evaluates water and energy fluxes of CMIP6 model over the Tibetan Plateau. Results show that the inter-model variability is substantial in temperature simulations. Snow that the largest component of the cryosphere responds significantly to changes in temperature. In the study, we study snow depth simulations corresponding to temperature simulations of different models over the Tibetan Plateau. Based on the water balance formula, analysis of how water balance fluxes respond to temperature changes in CMIP6, and determine the sources of error and ultimately lead to improved predictions.

How to cite: Liu, S., Liu, Z., and Duan, Q.: Evaluation of CMIP6 models for water and energy fluxes and analysis of source of errors over the Tibetan Plateau, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5066, https://doi.org/10.5194/egusphere-egu23-5066, 2023.

EGU23-5176 | ECS | Orals | CL4.6

Global warming induces more internally generated extremes of North Atlantic Oscillation and East Atlantic pattern 

Quan Liu, Johann Jungclaus, Daniela Matei, and Juergen Bader

Increased weather and climate extreme events are often attributed solely to either human-induced climate change or internal variability, under the assumption that external forcing does not influence the internal variability. However, with the development of single-model initial-condition large ensembles, recent research shows the impact of global warming on internal variability. This study investigates how global warming influences the North Atlantic Oscillation (NAO) and the East Atlantic (EA) pattern, which are the dominant large-scale circulation/teleconnection modes in the North Atlantic sector.

The study analyzes the geopotential height data of the Max Planck Institute Grand Ensemble (MPI-GE)  with 100 ensemble members. The internal variability is quantified as the deviation from the ensemble mean. The influence of global warming on the internal variability is checked with a 1pcCO2 experiment, where the  concertation is increased by 1% every year. This experiment provides a scenario for relatively strong global warming based on increasing greenhouse gas concentration alone. The extreme NAO and EA are defined as those years where the indexes are above (positive extremes) or below (negative extremes) 2 standard deviations.

The results show increases in extreme events, especially negative extremes, for both NAO and EA during wintertime, in a warmer climate. While NAO extremes increase consistently across the whole troposphere, EA extremes increase more at higher altitudes (500hpa-200hpa) than at lower altitudes. The warming effect of positive extreme NAO over northern Eurasia gets weaker, while the cooling effect of negative extreme NAO over northern Eurasia gets stronger. The effects of both, positive and negative extremes of EA, extend eastward till Eastern Asia. Overall, this study underlines the impact of global warming onto the internal variability of NAO and EA.

How to cite: Liu, Q., Jungclaus, J., Matei, D., and Bader, J.: Global warming induces more internally generated extremes of North Atlantic Oscillation and East Atlantic pattern, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5176, https://doi.org/10.5194/egusphere-egu23-5176, 2023.

EGU23-5279 | Orals | CL4.6

Reconciling conflicting evidence for the cause of the observed early 21st century Eurasian Cooling 

Stefan Sobolowski, Stephen Outten, and Camille Li

Arctic amplification of global warming is accompanied by a dramatic decline in sea ice. This, in turn, has been linked to cooling over the Eurasian subcontinent over recent decades, most dramatically during the period 1998-2012. Such a coherent and pronounced cooling is a counterintuitive impact under global warming. Some studies have proposed a causal teleconnection from Arctic sea ice retreat to Eurasian wintertime cooling; others argue that Eurasian cooling is mainly driven by internal variability. Overall, there is an impression of strong disagreement between those holding the “ice-driven” versus “internal variability” viewpoints. We offer an alternative framing that shows that the sea ice and internal variability views can be compatible. Key to this is viewing Eurasian cooling through the dual lens of dynamics (linked primarily to internal variability with a small contribution from sea ice; cools Eurasia) and thermodynamics (linked to sea ice retreat; warms Eurasia). This framing, combined with recognition that there is uncertainty in the hypothesized mechanisms themselves, allows both viewpoints (and others) to co-exist and contribute to our understanding of Eurasian cooling. A simple autoregressive model shows that strong Eurasian cooling is consistent with internal variability, with some periods being more susceptible to strong cooling than others. Rather than posit a “yes-or-no” causal relationship between sea ice and Eurasian cooling, a more constructive way forward is to consider whether the cooling trend was more likely given the observed sea ice loss, as well as other sources of low-frequency variability. Taken in this way both sea ice and internal variability are factors that affect the likelihood of strong regional cooling in the presence of ongoing global warming. Improving our understanding of the underlying mechanisms is critical for quantifying regional responses and impacts as well as producing reliable near-term climate predictions. 

How to cite: Sobolowski, S., Outten, S., and Li, C.: Reconciling conflicting evidence for the cause of the observed early 21st century Eurasian Cooling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5279, https://doi.org/10.5194/egusphere-egu23-5279, 2023.

EGU23-5775 | ECS | Orals | CL4.6 | Highlight

Impacts of a weakened AMOC on the European climate 

Katinka Bellomo, Virna Meccia, Roberta D'Agostino, Federico Fabiano, Sarah Larson, Jost von Hardenberg, and Susanna Corti

Previous studies have shown that the response of the Atlantic Meridional Overturning Circulation (AMOC) to increasing greenhouse gas forcing is a key driver of inter-model uncertainties. While all models project an AMOC decline, the inter-model spread in the decline rate drives very different climate change impacts, including temperature, precipitation, and large-scale atmospheric circulation patterns. Here we investigate the impacts of a weakened AMOC by performing idealized climate model experiments using EC-Earth3, a state-of-the-art GCM participating in CMIP6. We compare results from a control experiment run under preindustrial forcing, with an experiment in which we force a weakened AMOC by applying a virtual salinity flux in the North Atlantic/Arctic basin. Here we analyze previously unexplored aspects of the climate response to a weakened AMOC, focusing on impacts on wintertime daily timescales in the Euro-Atlantic region.

We find that a weakened AMOC forces an overall drier climate over most of Europe; however, some regions especially in northwestern Europe experience an increase in the number of very wet days. We investigate drivers of precipitation changes by performing a moisture budget and analyzing the association with changes in weather regimes at daily timescales. We find that an increase in the occurrence of the NAO+ days (going from a frequency of ~26% of occurrence to above 42%) together with an enhanced and more central jet, favors drier conditions over southern Europe and wetter conditions over northwestern Europe. Further, enhanced but drier storms cause dryness over Europe while thermodynamic processes per se, namely the Clausius-Clapeyron constraint on temperature, play a second role. Finally, we explore these relationships in additional experiments in which we keep the AMOC constant in a forced 4xCO2 experiment by applying a reversed virtual salinity flux, which allows us to separate the effects of 4xCO2 forcing from the weakened AMOC on climate change impacts. Our results have broader implications for understanding the role of the AMOC response on future climate change, allowing us to separate the impacts of the AMOC from those of the CO2 increase.

How to cite: Bellomo, K., Meccia, V., D'Agostino, R., Fabiano, F., Larson, S., von Hardenberg, J., and Corti, S.: Impacts of a weakened AMOC on the European climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5775, https://doi.org/10.5194/egusphere-egu23-5775, 2023.

The central role of tropical sea surface temperature (SST) variability in modulating Northern Hemisphere (NH) extratropical climate has long been known. However, the prevailing pathways of teleconnections in observations and the ability of climate models to replicate these observed linkages remain elusive. Here, we apply maximum covariance analysis between atmospheric circulation and tropical SST to reveal two co-existing tropical-extratropical teleconnections albeit with distinctive spatiotemporal characteristics. The first mode, resembling the Pacific-North American (PNA) pattern, favors a Tropical-Arctic in-phase (warm-Pacific-warm-Arctic) teleconnection in boreal spring and winter. The second mode, predominant in summer and autumn, is manifested as an elongated Rossby-wave train emanating from the tropical eastern Pacific that features an out-of-phase relationship (cold-Pacific-warm-Arctic) between tropical Pacific SST and temperature variability over the Arctic. This Pacific-Arctic teleconnection (PARC) mode partially explains the observed summertime warming around the Arctic. The reliability of climate models to replicate these leading teleconnections is of primary interest in this study to improve decadal prediction on regional climate. While climate models participating in CMIP6 appear to successfully simulate the PNA mode and its temporal characteristics, the majority of models’ skill in reproducing the PARC mode is obstructed by apparent biases in simulating low-frequency SST and rainfall variability over the tropical eastern Pacific and the summer climatological mean flow over the North Pacific. Considering the contribution of the PARC mode in shaping low frequency climate variations over the recent decades from the tropics to the Arctic, improving models’ capability to capture the PARC mode is essential to reduce uncertainties associated with decadal prediction and climate change projection over the NH.

How to cite: Feng, X.: Possible causes of model biases in simulating Tropical-Arctic teleconnections in CMIP6, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6017, https://doi.org/10.5194/egusphere-egu23-6017, 2023.

EGU23-6966 | ECS | Orals | CL4.6

Opposite Impacts of Interannual and Decadal Pacific Variability in the Extratropics 

Melissa Seabrook, Doug Smith, Nick Dunstone, Rosie Eade, Leon Hermanson, Adam Scaife, and Steven Hardiman

It is well established that the positive phase of El Niño Southern Oscillation (ENSO) tends to weaken the Northern Hemisphere stratospheric polar vortex (SPV), promoting a negative North Atlantic Oscillation (NAO). Pacific Decadal Variability (PDV) is characterised by a pattern of sea surface temperatures similar to ENSO, but its impacts are more uncertain: some studies suggest similar impacts of ENSO and PDV on the SPV and NAO, while others find the opposite. We use climate model experiments and reanalysis to find further evidence supporting opposite interannual and decadal impacts of Pacific variability on the extratropics. We propose that the decadal strengthening of the SPV in response to positive PDV is caused by a build-up of stratospheric water vapour leading to enhanced cooling at the poles, an increased meridional temperature gradient and a strengthened extratropical jet. Our results are important for understanding decadal variability, seasonal to decadal forecasts and climate projections.

How to cite: Seabrook, M., Smith, D., Dunstone, N., Eade, R., Hermanson, L., Scaife, A., and Hardiman, S.: Opposite Impacts of Interannual and Decadal Pacific Variability in the Extratropics, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6966, https://doi.org/10.5194/egusphere-egu23-6966, 2023.

EGU23-7011 | ECS | Orals | CL4.6

AMOC variations modulated by Tropical Indio-Atlantic SST Gradient 

Brady Ferster, Leonard Borchert, Juliette Mignot, and Alexey Fedorov

A potential future slowdown or acceleration of the Atlantic Meridional Overturning Circulation (AMOC) would have profound impacts on global and regional climate. Recent studies have shown that AMOC responds, among many other processes, to anthropogenic changes in tropical Indian ocean (TIO) temperature. However, internal unforced co-variations between these two basins are largely unexplored as of yet. Here, we use the ERSST v5, HadISST v1, and COBE v2 gridded observational products for the period 1870-2014, as well as dedicated simulations with coupled climate models, and show that internal changes in sea surface temperature gradients between the Indian and Atlantic Ocean (SSTgrad) can drive teleconnections that influence internal variations of North Atlantic climate and AMOC.

We separate the unforced observed component (i.e., internal signal) from the forced signal following the residuals method presented by Smith et al. (2019). In the absence of direct AMOC observation we estimate AMOC variability from an SST index (SSTAMOC; Caesar et al., 2018). We find a robust observed relationship between the unforced tropical SSTgrad and SSTAMOC when TIO leads by ~25 years. This time-lag is in line with a recently described mechanism of anomalous tropical Atlantic rainfall patterns that originate from TIO warming and cause anomalously saline tropical Atlantic surface water which slowly propagate northward into the subpolar North Atlantic, ultimately altering oceanic deep convection and AMOC (Hu and Fedorov, 2019; Ferster et al. 2021). Our study now suggests that it is the tropical SSTgrad that drives those AMOC changes, with a limited role for the western tropical Pacific. Pre-industrial control simulations with the IPSL-CM6A-LR model confirm this relationship, indicating a time lag of ~25 years between SSTgrad and SSTAMOC variations. These simulations also confirm that the SSTAMOC is representative of unforced AMOC variations when SSTAMOC leads by 5 years. This work therefore indicates that an unforced pathway between tropical ocean temperature and AMOC exists with a ~20 year lag, which opens the potential for using SSTgrad as precursor to predict future AMOC changes.

 

Caesar, L., Rahmstorf, S., Robinson, A., Feulner, G., & Saba, V. (2018). Observed fingerprint of a weakening Atlantic Ocean overturning circulation. Nature, 556(7700), 191-196.

Ferster, B. S., Fedorov, A. V., Mignot, J., & Guilyardi, E. (2021). Sensitivity of the Atlantic meridional overturning circulation and climate to tropical Indian Ocean warming. Climate Dynamics, 1-19.

Hu, S., & Fedorov, A. V. (2019). Indian Ocean warming can strengthen the Atlantic meridional overturning circulation. Nature climate change, 9(10), 747-751.

Smith, D. M., Eade, R., Scaife, A. A., Caron, L. P., Danabasoglu, G., DelSole, T. M., ... & Yang, X. (2019). Robust skill of decadal climate predictions. Npj Climate and Atmospheric Science, 2(1), 1-10.

How to cite: Ferster, B., Borchert, L., Mignot, J., and Fedorov, A.: AMOC variations modulated by Tropical Indio-Atlantic SST Gradient, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7011, https://doi.org/10.5194/egusphere-egu23-7011, 2023.

A detailed assessment of climate variability of the Baltic Sea area for the period 1958-2009 (Lehmann et al. 2011) revealed that recent changes in the warming trend since the mid-1980s, were associated with changes in the large-scale atmospheric circulation over the North Atlantic. The analysis of winter sea level pressure (SLP) data highlighted considerable changes in intensification and location of storm tracks, in parallel with the eastward shift of the North Atlantic Oscillation (NAO) centres of action. Additionally, a seasonal shift of strong wind events from autumn to winter and early spring existed for the Baltic area. Lehmann et al. (2002) showed that different atmospheric circulation regimes force different circulation patterns in the Baltic Sea. Furthermore, as atmospheric circulation, to a large extent, controls patterns of water circulation and biophysical aspects relevant for biological production, such as the vertical distribution of temperature and salinity, alterations in weather regimes may severely impact the trophic structure and functioning of marine food webs (Hinrichsen et al. 2007). To understand the processes linking changes in the marine environment and climate variability, it is essential to investigate all components of the climate system which of course include also the large-scale atmospheric circulation. Here we focus on the link between changes/shifts in the large scale atmospheric conditions and their impact on the regional scale variability over the Baltic Sea area for the period 1950-2021. This work is mostly an extension of previous studies which focused on the response of the Baltic Sea circulation to climate variability for the period 1958-2008 (Lehmann et al. 2011, Lehmann et al. 2014). Now extended time series ECMWF ERA 5 reanalysis for 7 decades are available, highlighting recent changes in atmospheric conditions over the Baltic Sea. The main focus of this work is to identify predominant large scale atmospheric circulation patterns (climate regimes) on a monthly/seasonal time scale influencing the regional atmospheric circulation over the Baltic Sea area. Furthermore, long-term changes on the annual to decadal time scale will also be investigated.

How to cite: Lehmann, A., Post, P., and Myrberg, K.: Changing impact of the large-scale atmospheric circulation on the regional climate variability of the Baltic Sea for the period 1950-2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8461, https://doi.org/10.5194/egusphere-egu23-8461, 2023.

EGU23-10582 | Orals | CL4.6 | Highlight

Impacts of oceanic warming patterns versus CO2 radiative forcing on the Hadley Circulation 

Yong Sun, Gilles Ramstein, Alexey V. Fedorov, Lin Ding, and Bo Liu

The Hadley circulation (hereafter HC) is one of the most prominent meridional overturning circulations in the climate system. In addition to maintaining energy balance and momentum exchange in tropics and extratropics, it can also shape the Intertropical Convergence Zone (ITCZ) and subtropical dry arid zones by regulating the hydrological cycle in tropical and extratropical regions. Weakening and expanding HC and narrowing of the ITCZ are projected with human greenhouse gas emissions. However, no consensus has been achieved regarding the relative importance of direct CO2 radiative effect and indirect effects via SST changes in shaping the future HC changes. This limits our deep understanding of the climate impacts imposed by changes in the HC. Here we analyze a broad range of CMIP5 experiments and show that future changes in SST patterns play the leading role in the determining the future changes in HC and ITCZ. In addition, a series of individual basin perturbation experiments were conducted at 1.5°C, 2°C, and 3°C temperature thresholds to identify key basins that determine HC strength, edges, and ITCZ locations. Our work highlights the overwhelming role of future tropical Indian Ocean warming on the HC and ITCZ changes.

How to cite: Sun, Y., Ramstein, G., Fedorov, A. V., Ding, L., and Liu, B.: Impacts of oceanic warming patterns versus CO2 radiative forcing on the Hadley Circulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10582, https://doi.org/10.5194/egusphere-egu23-10582, 2023.

EGU23-11826 | ECS | Posters on site | CL4.6

Precipitation weather typing over the South Pacific: application to the TRMM satellite product calibration 

Oscar Mirones, Joaquín Bedia, Juan A. Fernández-Granja, Sixto Herrera, Sara O. Van Vloten, Andrea Pozo, Laura Cagigal, and Fernando J. Méndez

In the South Pacific region, the precipitation patterns are mostly driven by a number of processes operating at spatial and temporal scales. One of the most important features is the South Pacific Convergence Zone (SPCZ).

Five Daily Weather Types (WT) of precipitation are presented, based on Principal Component Analysis (PCA) and k-means clustering using ERA5 precipitation and atmospheric circulation variables such as mean sea-level pressure (SLP), day-to-day difference of mean daily SLP or northward and eastward 10-m wind component fields, able to capture distinct precipitation spatio-temporal patterns, interpretable in terms of salient regional climate features such as the SPCZ state and tropical cyclone activity. We then undertake a weather-type conditioned calibration of the TRMM (Tropical Rainfall Measuring Mission) product using in-situ rain gauge records from the PACRAIN database as reference. “Conditioning” is here based on applying separate statistical corrections for each of the generated WTs, since biases might be dependent on specific atmospheric situations that can be partially captured by the clustering procedure, thus adapting the correction factors to specific synoptic conditions. 

Our results indicate that the WT-conditioned calibration provides an overall marginal added value over the unconditioned approach, although it makes a significant difference for a better correction of extreme rainfall events, critical in many impact studies. The approach can be extended to compound extreme events, in which several variables are involved (e.g. precipitation, sea level, wind, etc.), in order to better preserve multi-variable consistency.

How to cite: Mirones, O., Bedia, J., Fernández-Granja, J. A., Herrera, S., Van Vloten, S. O., Pozo, A., Cagigal, L., and Méndez, F. J.: Precipitation weather typing over the South Pacific: application to the TRMM satellite product calibration, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11826, https://doi.org/10.5194/egusphere-egu23-11826, 2023.

EGU23-11931 | ECS | Posters virtual | CL4.6

The Large-Scale Climate of Alaska - The Effects of the Pacific Decadal Oscillation on the Climate of Alaska 

Jasper Heuer, Martin Stuefer, and Lea Hartl

The climate of the state of Alaska is influenced not only by regional anthropogenic climate change, but also by the effects of large-scale ocean atmosphere systems like the Pacific Decadal Oscillation (PDO). Whereas positive anomalies in the PDO index coincide with warmer (sea surface) temperatures in the Gulf of Alaska and across the state, negative anomalies have the opposite effect. After analyzing the strength and direction of the correlation between the PDO index and the average temperatures in each of the 13 climate divisions of Alaska – both annually, as well as seasonally (DJF, MAM, JJA, and SON) – it becomes apparent, that the PDO affects the southern coastal and Panhandle regions much stronger than the Interior and North Slope. Over the course of a year, the correlations are strongest during the winter months, decrease during the spring and summer, only to increase again in the fall. Since the effects of large-scale circulations such as the PDO are changing under the influence of natural and anthropogenic climate change, reliable predictions on the future of the Alaskan climate are extremely complicated. In the future, further analysis is needed to support policy makers in their efforts to help adept the state’s ecosystems and economies to the changing climate.

How to cite: Heuer, J., Stuefer, M., and Hartl, L.: The Large-Scale Climate of Alaska - The Effects of the Pacific Decadal Oscillation on the Climate of Alaska, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11931, https://doi.org/10.5194/egusphere-egu23-11931, 2023.

EGU23-12678 | ECS | Orals | CL4.6

Classification of Atmospheric Circulation Patterns That Trigger Rainfall Extremes in the Sudan-Sahel Region 

Manuel Rauch, Jan Bliefernicht, Patrick Laux, and Harald Kunstmann

A better understanding of the rainfall variability and extremes in tropical regions is crucial for the development of improved statistical and numerical approaches used for climate research and weather prediction. In this study, we present a novel fuzzy rule-based method for classifying atmospheric circulation patterns relevant to heavy rainfall in the Sudan-Sahel region over West Africa. In the first step, we determine large-scale atmospheric patterns to describe important seasonal features of the West African Monsoon like the movement of Saharan Heat Low over the African continent. In the second step, meso-scale monsoon patterns are classified to better describe rainfall variability and extremes during the monsoon period. In addition to a comprehensive predictor screening using more than 30 variables at different atmospheric levels, a detailed sensitivity analysis is performed, which aims to improve the transferability of the classification approach to an independent dataset. Furthermore, crucial aspects of the methodological development of fully automatic classification approaches are addressed. Using mean sea level pressure and stream function fields (700hPa) as final predictor variables, we identified 23 circulation patterns as robust solution to represent key atmospheric processes and rainfall variability in the study region. The two wettest patterns are distinguished by an enhanced Saharan Heat Low and cyclonic rotation near the study region, suggesting the presence of a tropical wave trough and triggering about 50% of the rainfall extremes on 6.5% of the days. The identified atmospheric circulation patterns are currently used to develop a variety of improved statistical approaches for this challenging region, such as pattern-dependent bias correction, geostatistical interpolation, and simulation. 

How to cite: Rauch, M., Bliefernicht, J., Laux, P., and Kunstmann, H.: Classification of Atmospheric Circulation Patterns That Trigger Rainfall Extremes in the Sudan-Sahel Region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12678, https://doi.org/10.5194/egusphere-egu23-12678, 2023.

EGU23-13294 | ECS | Orals | CL4.6

Regime-oriented causal model evaluation of Atlantic-Pacific teleconnections in CMIP6 

Soufiane Karmouche, Evgenia Galytska, Jakob Runge, Gerald Meehl, Adam Phillips, Katja Weigel, and Veronika Eyring

Regime-oriented causal model evaluation of Atlantic-Pacific teleconnections in CMIP6

Abstract:

The Pacific Decadal Variability (PDV) and the Atlantic Multidecadal Variability (AMV) are two important modes of long-term internal variability that significantly impact the climate system and its spatio-temporal changes. In this study, we use a regime-oriented causal discovery method (Karmouche et al, 2022) to examine the changing interactions between the PDV and AMV. The results of this analysis are used to evaluate the ability of models participating in the Coupled Model Intercomparison Project Phase 6 (CMIP6) to represent the observed changing interactions between the PDV, AMV, and their extra-tropical teleconnections.

Applying the regime-oriented causal discovery method to reanalysis time series revealed that the interactions between AMV and PDV differ from one regime to the other. The results also show that there are both direct and indirect connections between the Atlantic and Pacific oceans, which are established through various teleconnection patterns.

In order to evaluate the ability of climate models to represent these observed interactions, we applied the same regime-oriented causal discovery method to the CMIP6 Large Ensemble historical simulations. We show that several models performed well in simulating the observed causal patterns when AMV and PDV are "out-of-phase", and that the two models with the largest number of members generally outperformed other models in simulating observed causal patterns during longer regimes. This work shows how causal discovery on LEs complements the available diagnostics and statistics metrics of climate variability to provide a powerful tool for climate model evaluation.

Karmouche, S., Galytska, E., Runge, J., Meehl, G. A., Phillips, A. S., Weigel, K., and Eyring, V.: Regime-oriented causal model evaluation of Atlantic-Pacific teleconnections in CMIP6, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2022-1013, 2022.

How to cite: Karmouche, S., Galytska, E., Runge, J., Meehl, G., Phillips, A., Weigel, K., and Eyring, V.: Regime-oriented causal model evaluation of Atlantic-Pacific teleconnections in CMIP6, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13294, https://doi.org/10.5194/egusphere-egu23-13294, 2023.

EGU23-13299 | Orals | CL4.6

Drivers of the Annual Cycle of Rainfall over Central Africa: The Role of Water Vapor and the Mid-Tropospheric Meridional Circulation 

Georges-Noel T. Longandjo, Bellinda Mashoene Monyela, and Mathieu Rouault

The Intertropical Convergence Zone (ITCZ), with its twice-annual passage over central Africa, is considered as the main driver of the rainfall seasonality. But recently, this paradigm was challenged. To find out what are the main drivers of the annual cycle of rainfall over central Africa, we present a simple comprehensive paradigm with both local forcings and regional-scale processes playing crucial role. Due to the local evaporative cooling effect, the foot of the ascending branch of Hadley cells occurs where the temperature is the warmest, indicating a thermal low. This distorts the southern Hadley cell by developing its bottom-heavy structure. As result, both shallow and deep Hadley cells coexist over central Africa year–round. The deep mode is associated with poleward branches at upper levels that transport the atmospheric energy. The shallow mode is characterized by a meridional return flow in the mid-troposphere that transports the water vapour instead of lower branches as widely reported. This favours the building-up of the mid-tropospheric moisture flux convergence with a limited contribution of the midlevel easterly jet, conducive to deep convection. Embedded in this strong rising branch of Hadley cells at midlevels, the intense convective rainfall, and with it the rainfall maximum position, is seasonally controlled by the dynamics of the midlevel shallow meridional return flow. This highlights the interhemispheric rainfall contrast over central Africa and outlines its unimodal seasonality. On the other hand, forced by the Congo basin cell, the precipitable water regulates the deep convection from the vegetated surface of Congo basin, acting as a continental sea. This nonlinear mechanism separates the rainfall into three distinct regimes – (i) the moisture-convergence-controlled regime, with convective rainfall exclusively occurring in the rainy season and (ii) the local evaporation-controlled regime with drizzle and (iii) the precipitable-water-controlled regime, with exponential increase of rainfall that both occur during the dry season.

How to cite: Longandjo, G.-N. T., Monyela, B. M., and Rouault, M.: Drivers of the Annual Cycle of Rainfall over Central Africa: The Role of Water Vapor and the Mid-Tropospheric Meridional Circulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13299, https://doi.org/10.5194/egusphere-egu23-13299, 2023.

In this communication, we will present results from an analysis of the variability of the vertically averaged (i.e., barotropic) atmospheric circulation simulated by climate models, which integrate the current Coupled Model Intercomparison Project (CMIP6). The variabilities in two ensembles of Atmospheric Model Intercomparison Project (AMIP) simulations were compared with the variabilities in two ensembles of fully coupled simulation counterparts of the current CMIP6 (Castanheira and Marques, 2022).

The atmospheric models simulate less variability of the barotropic atmospheric circulation over the Northern Atlantic and more variability over the North Pacific when compared with the corresponding variabilities in the ERA5 reanalysis (“observations”), at intraseasonal and interannual scales. When integrated over the whole globe, the variability in the coupled climate simulations is smaller than the variability in the corresponding AMIP simulations. The smaller global variability of the coupled simulations results in no mean overestimation of the subtropical jet variability in the North Pacific, but further underestimation of the jet stream variability in the Northern Atlantic. The results suggest that the reduction of the biases in the barotropic atmospheric variability over the North Pacific, in the coupled climate simulations, is achieved through compensating biases in the mean Sea Surface Temperatures (SSTs). Moreover, the reduction of the positive biases in the North Pacific seems to be associated with a reduction of the excitation of the most unstable barotropic mode of the atmospheric circulation, which contributes also to a reduction of the barotropic atmospheric variability in the North Atlantic region.

 Acknowledgements: The CESAM is supported by FCT/MCTES through the project UIDP/50017/2020+ UIDB/ 50017/20201+LA/P/0094/2020.

References

Castanheira, J. M., Marques, C. A. F. (2022). Biases of the Barotropic Atmospheric Circulation Variability in CMIP6 Models. Journal of Climate,  Vol. 35, 5071–5085 DOI: 10.1175/JCLI-D-21-0581.1. 

How to cite: Castanheira, J. M. and Marques, C. A. F.: How can the most unstable barotropic mode of atmospheric models contribute for the explanation of atmospheric variability biases of climate models in the North Atlantic?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13716, https://doi.org/10.5194/egusphere-egu23-13716, 2023.

EGU23-13726 | ECS | Posters on site | CL4.6

Causal drivers of central Amazon precipitation variability during austral summer 

Emily Henningsen, Giorgia Di Capua, and Reik V. Donner

The South American monsoon system is one key component of the regional climate of South America, and its interannual as well as intraseasonal variability is of great relevance for water availability over vast parts of the continent. To further develop advanced prediction systems for hydro-meteorological conditions, a better understanding of the underlying atmospheric as well as coupled ocean-atmosphere and land-atmosphere processes governing the intraseasonal variations of rainfall is of paramount importance.

 

In this work, we focus on rainfall variability over the central Amazon basin (CAB) as a particularly vulnerable region during the peak season of the monsoon (December to February). In order to identify causal precursors of CAB rainfall variability and their mutual causal interdependence structure, we employ a causal discovery tool called Peter and Clark Momentary Conditional Information (PCMCI) algorithm to monthly average sea surface temperature (SST), mean sea level pressure (MSLP) and precipitation fields from reanalysis data sets for two different time periods, 1950-2020 and 1979-2020. As a first step, anomaly maps and correlation maps are used to identify potential candidate drivers of the precipitation variability in the CAB at lead times of up to three months. The causal effect networks resulting from the subsequent application of the PCMCI algorithm unveil the causal dependencies of different climate phenomena with CAB rainfall variability during austral summer, confirming previous results based on standard correlation analyses and allowing for a quantitative assessment of the different effects.

 

Among others, we find that SST changes in the tropical Pacific Nino1+2 region close to the South American west coast have a causal effect on CAB precipitation, with lower SSTs promoting more rainfall with a lag of one to two months. Notably, we do not find any similar statistically significant causal impact of SST variations in the Nino3.4 region in the central tropical Pacific, which is commonly most closely associated with the El Niño Southern Oscillation. Additionally, the obtained causal effect networks demonstrate that the Southern Annular Mode (SAM) causally influences the Amundsen Sea Low (ASL), which in turn causally affects the CAB rainfall. Both links are negative, i.e. a positive SAM mode leads to a deeper ASL with a lag of one month, and a deeper ASL supports higher precipitation in central Amazonia with a lag of three months. Finally, SST variability in the tropical North Atlantic as well the Madden-Julian Oscillation do not show a significant causal relationship with CAB rainfall. Our obtained findings are qualitatively consistent among the two different time periods. However, when analyzing data starting only after 1979, some links increase in strength while generally less causal links show up in the networks.

How to cite: Henningsen, E., Di Capua, G., and Donner, R. V.: Causal drivers of central Amazon precipitation variability during austral summer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13726, https://doi.org/10.5194/egusphere-egu23-13726, 2023.

EGU23-14053 | ECS | Posters virtual | CL4.6

Cyclonic development in the Mediterranean Basin in CMIP6 models using a neural network approach 

George Blougouras, Kostas Philippopoulos, Chris G. Tzanis, and Constantinos Cartalis

The Mediterranean basin is located between the subtropical high-pressure belt and the mid-latitude westerlies and is characterized by complex topography. Its orography, the relatively warm Mediterranean Sea, which is a source of energy and moisture, and the land-sea interactions result in significant cyclonic behavior in the synoptic and sub-synoptic scales. Due to its high sensitivity to climate change forcings, the Mediterranean region is considered a climate change hot spot, with impacts, such as the decline in the projected precipitation, leading to increasing aridification in an already water-stressed area. The above highlight the importance of examining the cyclonic development in the area and assessing the respective changes under different climate change scenarios. In this research, unsupervised machine learning algorithms are used in order to objectively identify cyclonic development in the Mediterranean basin using CMIP6 data for a subset of the different shared socio-economic pathways (SSP) that explore a wide range of possible future outcomes. In more detail, Sea Level Pressure from selected CMIP6 models is used as an input in a Self-Organizing Map (SOM) which is trained to identify the cyclone activity in the Mediterranean Basin for the 1981-2010 reference period. The ability of the network in terms of identifying effectively cyclogenesis regions and the transition probabilities is evaluated. The trained SOM is used to classify CMIP6 mid-century (2031-2060) projections and changes in the frequencies of occurrence of cyclonic development. These are evaluated in terms of physical drivers and regionally specific mechanisms. Examining the responses of cyclonic development to different forcing scenarios will not only shed light on the physical and dynamical processes that govern these circulations but will also allow identifying high–risk regions with potential socio-economic impacts.

How to cite: Blougouras, G., Philippopoulos, K., Tzanis, C. G., and Cartalis, C.: Cyclonic development in the Mediterranean Basin in CMIP6 models using a neural network approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14053, https://doi.org/10.5194/egusphere-egu23-14053, 2023.

EGU23-15027 | ECS | Orals | CL4.6

Representation of relationship between PDO and global precipitation in CMIP6 models 

Jivesh Dixit, Vikram M. Mehta, and Krishna M. AchutaRao

Decadal Climate Variability (DCV) modes perturb regional climatic parameters across the globe at multi-year timescales. Precipitation is one such climatic parameter of socio-economic importance.

Our study examines the ability of Coupled Model Intercomparison Project Phase 6 (CMIP6) models in representing the observed teleconnection of DCV modes; Pacific Decadal Oscillation (PDO) and Tropical Atlantic SST Gradient with the global precipitation. We chose the subset of CMIP6 models that participate in both historical and hindcast experiments.

In this study we examine the relationship between the model's ability to simulate the long-term DCV pattern and its ability to simulate the teleconnection between DCV mode and global precipitation.

HadGEM3-GC31-MM and MPI-ESM-1-2-HR, which simulate the observed global SST anomaly pattern in the warm phase of PDO considerably well, also simulate observed global precipitation patterns during the warm phase of PDO quite well in regions like  central India, Europe, North- and South-America, Eastern Africa, Eastern Australia etc. However, BCC-CSM2-MR and NorCPM1 fail to effectively simulate observed precipitation patterns in the warm phase of PDO in regions like, North- and South-America, Africa etc. 

Hence, we found that models that are able to simulate the PDO pattern of SST are also able to represent the teleconnection between PDO modes and precipitation across the globe. We also examined the regression pattern of wind circulation, and the regression pattern of converging and diverging parts of the wind with PDO index. Models that better represent the observed warm phase of PDO pattern, also well represent the observed circulation pattern in respective phases of PDO. Similar analysis is also performed for TAG.


Keywords: Decadal Climate Variability (DCV), CMIP6, historical experiments, teleconnection, precipitation.

How to cite: Dixit, J., Mehta, V. M., and AchutaRao, K. M.: Representation of relationship between PDO and global precipitation in CMIP6 models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15027, https://doi.org/10.5194/egusphere-egu23-15027, 2023.

EGU23-15646 | ECS | Posters on site | CL4.6

Characterization of Mediterranean large-scale atmospheric circulation based on Jenkinson-Collison Weather Type classification. 

Juan Antonio Fernández-Granja, Ana Casanueva, Joaquín Bedia, Swen Brands, and Jesús Fernández

The evaluation of new generations of global climate models (GCMs) with respect to their large-scale circulation features is crucial for model development and has recently been brought into focus by the downscaling community, interested in the suitability of GCMs for downscaling purposes. In such evaluation experiments, additional uncertainties emerge from differences among the reference datasets used for evaluation, typically reanalyses. In this context, weather typing techniques are a useful tool for the classification of the full diversity of data into a few recurrent patterns that can serve as objective characterizations of either global or regional atmospheric circulation. A well-known weather typing classification algorithm is the Jenkinson-Collison Weather Type (JC-WT, Jenkinson and Collison 1977) approach. Although the methodology was originally developed for the British Isles (Lamb, 1972), the JC-WT approach can in principle be applied to any mid-to-high latitude region (Jones et al, 2013). Fernandez-Granja et al (2023) extended the limits of applicability from 23.5º to 80º latitude on both hemispheres, but the suitability of the method is questionable for certain seasons over some areas of the globe, such as the Mediterranean region in summer.

In this study, we first explore the applicability of the JC classification over the Mediterranean by linking the JC-WTs with main northern hemisphere teleconnection indices and blocking conditions. Further, the diversity of JC-WTs and occurrence of the unclassified type are used to examine the suitability of the method. Results show that the application of the JC-WT classification is physically meaningful in large parts of the domain. Secondly, fundamental characteristics of the JC-WTs such as transition probabilities between consecutive types and persistence of the dominant JC-WTs (number of time-steps staying in the same type) obtained for five different reanalyses are compared. Important differences among reanalyses are found, especially in summer, which may bring additional uncertainties when the method is used in model evaluation experiments. 

References:

Fernández-Granja, J. A., Brands, S., Bedia, J., et al (2023) Exploring the limits of the Jenkinson–Collison weather types classification scheme: a global assessment based on various reanalyses. Climate Dynamics. DOI: 10.1007/s00382-022-06658-7

Jenkinson A., Collison F. (1977) An initial climatology of gales over the north sea. synoptic climatology branch memorandum. Meteorological Office, 62

Jones P.D., Harpham C., Briffa K.R. (2013) Lamb weather types derived from reanalysis products. International Journal of Climatology 33(5):1129–1139. DOI: 10.1002/joc.3498

Lamb H. (1972) British isles weather types and a register of daily sequence of circulation patterns 1861-1971. Meteorological Office, Geophysical Memoir 116:1–85

How to cite: Fernández-Granja, J. A., Casanueva, A., Bedia, J., Brands, S., and Fernández, J.: Characterization of Mediterranean large-scale atmospheric circulation based on Jenkinson-Collison Weather Type classification., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15646, https://doi.org/10.5194/egusphere-egu23-15646, 2023.

EGU23-15694 | Posters on site | CL4.6

Heat Waves over Eastern Balkans: A statistical analysis, possible causes and physical drivers. 

Hristo Popov and Oleg Stepanyuk

Heat wave is a period of prolonged abnormally high surface temperatures relative to those normally expected. Heat waves may form when high pressure system strengthens and remains over a region from several days up to several weeks. Severe and exceptional heat waves, such as those that occurred over the Balkans (2007), France (2003), or Russia (2010), are associated with increased mortality, health hazards, reduced personal work productivity and have significant economic impacts by compromising agricultural harvest. Extremely high air temperature values in the Balkan Region are associated with anticyclones formed at the Azores maximum or high-pressure ridges and advections of hot air from the south and southwest.

In our study we perform statistical analysis of the occurrence, durability and intensity of the heat waves over the Balkan Peninsula for the period 1980-2020 based on historical satellite and reanalysis datasets. We analyse correlation between heat waves occurrence and North Atlantic Oscillation Index and certain historical meteorological data for Atlantic and Mediterranean regions aiming to figure out possible causes and physical drivers of this phenomena. One of the mid-term goals of the project is to develop a CNN based predictive system for short and long-time forecasting of extreme weather conditions over the Balkans.

 

How to cite: Popov, H. and Stepanyuk, O.: Heat Waves over Eastern Balkans: A statistical analysis, possible causes and physical drivers., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15694, https://doi.org/10.5194/egusphere-egu23-15694, 2023.

EGU23-16668 | ECS | Orals | CL4.6

Emergence of Low-Frequency Temperature Variability in Instrumental Data and Model Simulations 

Raphael Hébert and Thomas Laepple

The amplitude and spatial distribution of low-frequency natural variability is determinant for regional climate projections, but it is still poorly understood. 

 

In a previous study, pollen-based temperature reconstructions were used to quantify spatial patterns of millennial temperature variability. This showed an inverse relationship across timescales with sub-decadal variability from instrumental data in extra-tropical regions over land (Hébert et al., 2022, under review). We concluded that due to varying marine influence, regions characterized by stable oceanic climate at sub-decadal timescales experience stronger long-term variability while continental regions with higher sub-decadal variability show weaker long-term variability. Indications of this relationship could also be inferred from instrumental data alone as regions of low sub-decadal variability were more likely to exhibit a steeper increase of variability over multi-decadal timescales and vice versa. 

 

In the current work, the relationship found in the instrumental data was further investigated using different instrumental products. In addition, a large multi-model ensemble of CMIP6 models, as well as single-model ensembles, were considered for analysis and it was found that they do not systematically reproduce the relationship found in the instrumental data. This indicates a fundamental deficiency in the model simulations with regard to the mechanism driving the emergence of low-frequency climate variability. This characteristic being related to multi-decadal variability thus has important significance for multi-decadal regional climate projections and might be used as an emergent constraint in model evaluation and inter-comparison.

How to cite: Hébert, R. and Laepple, T.: Emergence of Low-Frequency Temperature Variability in Instrumental Data and Model Simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16668, https://doi.org/10.5194/egusphere-egu23-16668, 2023.

EGU23-16755 | Orals | CL4.6

An Atlantic interhemispheric teleconnection established by South American summer monsoon 

Wan-Ling Tseng, Yi-Chi Wang, Yu-chi Lee, Huang-Hsiung Hsu, and Noel Keenlyside

This paper reports the structure of an interhemispheric atmosphere–ocean coupling pattern, which occurs over the Atlantic Ocean from January to February, and refers to it as the Atlantic symmetric pattern (ASP). The ASP occurs in the middle–upper troposphere, with two trains of cyclonic–anticyclonic–cyclonic anomalous circulations aligned meridionally over the Atlantic Ocean. The sea surface temperature (SST) signature of the ASP, which is composed of a distinct SST dipole, is the leading mode of the interannual SST of the Southwest Atlantic Ocean. Experiments with the linear baroclinic model shows that the interhemispheric wave trains of the ASP can be excited as a Gill-type response to convection in the South American monsoon system and the South Atlantic convergence zone. Further studies are warranted to elucidate other aspects of the ASP, including teleconnection in the Northern Hemisphere and interactions with other climatic modes.

How to cite: Tseng, W.-L., Wang, Y.-C., Lee, Y., Hsu, H.-H., and Keenlyside, N.: An Atlantic interhemispheric teleconnection established by South American summer monsoon, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16755, https://doi.org/10.5194/egusphere-egu23-16755, 2023.

EGU23-16955 | Posters on site | CL4.6

Tropical to extratropical interactions in the Southern Hemisphere 

Julie Arblaster

Tropical variability has long been identified as having an important influence on climate variability and change in the Southern Hemisphere (SH). In all three ocean basins, heating from tropical convection can generate stationary Rossby waves that propagate polewards and eastwards towards Antarctica, influencing temperature and rainfall patterns along the way. Recent studies have also highlighted the reverse – an influence of the polar regions on changes further north, for example, the stratospheric weakening of the SH polar vortex that contributed to the prolonged drought and extreme fire weather in Australia in the spring and summer of 2019. On longer timescales, the climate of the Southern Hemisphere has undergone significant changes over the past 30-50 years. The extratropical atmosphere has seen a shift to a more positive phase of the Southern Annular Mode and a stronger and more poleward eddy-driven jet, particularly in austral summer. While the influence of anthropogenic forcing such as ozone depletion and increasing greenhouse gases on these changes is well-established, the importance of tropical to extratropical interactions in shaping some recent events is becoming more evident. Examples include the deepening of the Amundsen Sea Low which has been associated with tropical Pacific decadal variability and the rapid decline in Antarctic sea ice in 2016 which was linked to a record positive Indian Ocean Dipole event. Recent insights into tropical to extratropical interactions, including the mechanisms through which they operate and links to observed changes on interannual to interdecadal timescales will be discussed.

How to cite: Arblaster, J.: Tropical to extratropical interactions in the Southern Hemisphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16955, https://doi.org/10.5194/egusphere-egu23-16955, 2023.

EGU23-1251 | PICO | AS1.19

Towards an implementation of topography in a next-generation gravity-wave parameterisation 

Ulrich Achatz, Ray Chew, and Stamen Dolaptchiev

The Multi-Scale Gravity Wave Model (MS-GWaM) uses raytracing-based modelling that supports transient gravity-wave parametrisation. The state-of-the-art implementation of MS-GWaM in the upper-atmosphere ICON model solves the raytracing equations in three dimensions and accounts for background (non-orographic) and convective gravity-wave sources. Our work extends the capabilities of MS-GWaM to include orography gravity-wave sources, and we present methods and preliminary results towards this goal. Specifically, we first determine the spectral representation of the topography in each ICON grid cell via Fourier fitting. We then apply linear theory to obtain a representation of the bottom boundary for the raytracer. Finally, the bottom boundary serves as an initial condition for the raytracer-based parametrisation of orographic gravity waves. Preliminary results indicate that a judicious setup of this bottom boundary allows for an optimal tradeoff between computational efficiency and a sufficiently accurate representation of the underlying topography.

How to cite: Achatz, U., Chew, R., and Dolaptchiev, S.: Towards an implementation of topography in a next-generation gravity-wave parameterisation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1251, https://doi.org/10.5194/egusphere-egu23-1251, 2023.

EGU23-2661 | PICO | AS1.19

Comparison between a non orographic gravity wave drag scheme and constant level balloons in the QBO region 

Francois Lott, Raj Rani, Aurelien Podglajen, Francis Codron, Lionel Guez, Albert Hertzog, and Riwal Plougonven

The parameterization scheme that represents gravity waves due to convection in LMDz-6A, the atmospheric components of the IPSL coupled climate model (IPSLCM6), is directly compared to Strateole-2 balloon observations made in the lower tropical stratosphere from November 2019 to February 2020. The input meteorological fields necessary to run the parameterization offline are extracted from the ERA5 reanalysis and correspond to the instantaneous meteorological conditions found underneath the balloons. In general, we find a fair agreement between measurements of the momentum fluxes due to waves with periods less than 1hr and the parameterization. The correlation of the daily values between the observations and the results of the parameterization is around 0.4, which is statistically elevated considering that we analyse around 600 days of data and surprisingly good considering that the parameterization has not been tuned: the scheme is just the standard one that helps producing a Quasi-Biennial Oscillation in the IPSLCM6 model. Online simulations also show that the measured values of momentum fluxes are well representative of the zonally and averaged values of momentum fluxes needed in LMDz-6A to simulate a QBO. The observations also show that longer waves with periods smaller than a day carry about twice as much flux as waves with periods smaller than an hour, which is a challenge since the low period waves that make the difference are potentially in the “grey zone” of most climate models

How to cite: Lott, F., Rani, R., Podglajen, A., Codron, F., Guez, L., Hertzog, A., and Plougonven, R.: Comparison between a non orographic gravity wave drag scheme and constant level balloons in the QBO region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2661, https://doi.org/10.5194/egusphere-egu23-2661, 2023.

EGU23-3226 | ECS | PICO | AS1.19

Investigation of Secondary Gravity Wave Variability using a 3-Field-of-View Doppler-Rayleigh Lidar in Kühlungsborn, Germany 

Robin Wing, Michael Gerding, Gerd Baumgarten, Irina Strelnikova, Eframir Franco-Diaz, and Mohamed Mossad

Recent interpretations of atmospheric gravity wave propagation have emphasized the importance of secondary and higher-order gravity waves.  One implication of multi-stage vertical coupling of gravity waves could be an increased probability of measuring larger vertical wavelengths than would be expected from a primary gravity wave.  These secondary waves are also expected to be intermittent in time and localized in space, which means that lidars are an excellent technique for detecting these phenomena.  We present lidar gravity wave measurements from temperatures and winds using a zenith pointing beam and two 25-degree off-zenith beams. In each lidar field-of-view, gravity wave energy is estimated as a function of vertical wavelength and period using a Morlet wavelet analysis.  This analysis is conducted at multiple altitudes in each of the three beams to determine small-scale horizontal variability, which could indicate small-scale wave activity associated with primary wave breaking.

How to cite: Wing, R., Gerding, M., Baumgarten, G., Strelnikova, I., Franco-Diaz, E., and Mossad, M.: Investigation of Secondary Gravity Wave Variability using a 3-Field-of-View Doppler-Rayleigh Lidar in Kühlungsborn, Germany, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3226, https://doi.org/10.5194/egusphere-egu23-3226, 2023.

EGU23-3495 | ECS | PICO | AS1.19

Comparing gravity waves sampled from a kilometre-scale IFS run to AIRS satellite observations 

Emily Lear, Corwin Wright, Neil Hindley, and Inna Polichtchouk

Gravity waves are small-scale atmospheric waves which transport energy and momentum. These waves impact the large scale circulation and increasing our understanding of them is therefore important to support improvements to weather and climate models. This presentation focusses on gravity waves in the stratosphere using data from a high resolution run of the European Centre for Medium-Range Weather Forecasts (ECMWF) Integrated Forecasting System (IFS) operated at a kilometre-scale spatial resolution, the Atmospheric Infrared Sounder (AIRS) on NASA’s Aqua satellite and the ECMWF ERA5 reanalysis. For this comparison, the IFS run and ERA5 are resampled using the AIRS observational filter. Data are examined during the first 2 weeks of November, as the high resolution model was initialised on the 1st of this month. Wave properties were found using the 2D+1 S-Transform, a spectral analysis technique, which has been previously applied to AIRS data. Asia and surrounding regions are investigated, because preliminary studies of AIRS data suggested strong gravity wave activity in this region during this time period. Gravity waves can also be seen in the high resolution model and ERA5 data at similar times and locations as those in the observations. Higher amplitude gravity waves can be seen in nighttime AIRS data compared to the resampled models. The horizontal wavelengths in the data sets are generally similar in areas of peak gravity wave activity for nighttime data. Weather models are advancing rapidly and kilometre scales, such as the experimental IFS run, could become operational in the next decade. At these grid scales, gravity waves must be resolved instead of parameterized so the models need to be tested to see if they do this correctly. This work provides information on how a cutting edge model resolves gravity waves compared to observations.

How to cite: Lear, E., Wright, C., Hindley, N., and Polichtchouk, I.: Comparing gravity waves sampled from a kilometre-scale IFS run to AIRS satellite observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3495, https://doi.org/10.5194/egusphere-egu23-3495, 2023.

EGU23-4081 | PICO | AS1.19

Transient Tropopause Waves 

Andreas Dörnbrack

Horizontally short gravity waves are often observed near the tropopause. Here, airborne observations of mountain waves over southern Scandinavia are used to characterize these waves and to detect non-stationary modes. A series of two-dimensional numerical simulations is used to explain the generation of these transient wave modes that are trapped in the lowermost stratosphere and propagate horizontally downstream along the tropopause inversion layer. The numerical results reveal on which external parameters the properties of the short waves depend on. It turns out that the interaction of wave breaking aloft in the middle atmosphere and the tropospheric flow is the essential process explaining the generation of these non-stationary modes. Their characteristics is controlled by the sharpness of the tropopause inversion layer, the strength of the orographic forcing and, partially, by the spectra of the underlying orography exciting the vertically propagating mountain waves.

How to cite: Dörnbrack, A.: Transient Tropopause Waves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4081, https://doi.org/10.5194/egusphere-egu23-4081, 2023.

EGU23-4866 | ECS | PICO | AS1.19

Link between orographic gravity wave parameterizations and resolved dynamics in CMIP6 models. 

Dominika Hájková, Petr Šácha, and Petr Pišoft

Internal gravity waves (GWs) have an important influence on the atmospheric energy transport and momentum budget. Consideration of the GWs – related processes is necessary in modelling and conceptual models of the atmosphere. GWs cover a broad spectrum of wavelengths from few to thousands of kilometres. Hence, they cannot be fully resolved by the global climate models (GCMs) and have to be parameterized. Although recent efforts with satellite observations and high-resolution models have been improving tuning and constraints of the GWs parameterizations, there is still a large uncertainty concerning the effects of GWs in GCMs. This is unwanted due to large impact of GWs on the atmospheric dynamics.

In our research we focus on orographic GW (OGW) parameterizations used in CMIP6 simulations. We compare the OGW induced drag from 7 different OGW parameterizations used in 9 different models, establishing the simulation-unique tuning of free parameters for majority of them. The comparison shows large, unexpected differences between simulations, which can be partly traced to the tuning or type of the parameterization. We also analyze intermodel differences in zonal mean winds and Eliassen-Palm flux divergence to trace the effects of the differences in OGW drag. Particularly, our results demonstrate a strong correlation between resolved wave drag and OGW drag in the models. Overall, our study gives an additional motivation for further improvements of the OGW parameterization schemes, with the aim of lowering the uncertainty of the future climate projections.

How to cite: Hájková, D., Šácha, P., and Pišoft, P.: Link between orographic gravity wave parameterizations and resolved dynamics in CMIP6 models., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4866, https://doi.org/10.5194/egusphere-egu23-4866, 2023.

EGU23-4928 | ECS | PICO | AS1.19

Quantification of gravity wave drag in ERA5 reanalysis 

Zuzana Procházková, Petr Pišoft, and Petr Šácha

Internal gravity waves (GWs) are a ubiquitous component of atmospheric dynamics, propagating both horizontally and vertically through the atmosphere, interacting with other flow components and affecting regional to large-scale dynamics. Due to the wide spectrum of GWs, model dynamics in general circulation models (GCMs) can resolve only part of the spectrum, leaving the effects of the unresolved part to be inserted by parametrisations. The analysis of high-resolution atmospheric datasets with resolved GWs allows us to understand GW dynamics and their effects on the mean flow, even in the long-term time-scales. In addition to this, such analysis enables validation of the parametrised effects and potential improvements of the parametrisations. In the presented work, we analyse resolved GWs in the ECMWF‘s ERA5 reanalysis, evaluating their effects on the flow through the GW drag.

How to cite: Procházková, Z., Pišoft, P., and Šácha, P.: Quantification of gravity wave drag in ERA5 reanalysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4928, https://doi.org/10.5194/egusphere-egu23-4928, 2023.

EGU23-6108 | PICO | AS1.19

Cirrus cloud formation by gravity waves 

Stamen Dolaptchiev, Peter Spichtinger, Manuel Baumgartner, and Ulrich Achatz

Vertical ascent due to gravity waves (GW) represents one important formation mechanism for cirrus clouds, i.e., clouds consisting solely
of ice crystals. Further, GWs can substantially influence the microphysical cloud properties and cloud life cycle, which are crucial
for the radiative impact of the cirrus clouds. Here we investigate the interactions between high-, mid- or low-frequency GWs and cirrus
clouds in the tropopause region. Utilizing asymptotic analysis reduced equations are derived for the self-consistent description of the
cirrus dynamics forced by a monochromatic GW. This allows for the construction of prototype parameterization of the number nucleated ice
crystals. The GW-cirrus interactions are studied further in cloud resolving large eddy simulation and the results are used to evaluate
the asymptotic parameterization.

How to cite: Dolaptchiev, S., Spichtinger, P., Baumgartner, M., and Achatz, U.: Cirrus cloud formation by gravity waves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6108, https://doi.org/10.5194/egusphere-egu23-6108, 2023.

EGU23-8137 | ECS | PICO | AS1.19

Ray-tracing global gravity wave observations in 21 years of AIRS data 

Phoebe Noble, Corwin Wright, Neil Hindley, and Tracy Moffat-Griffin

Gravity waves have a variety of different sources including wind flow over mountains, convection and jet stream instabilities. Yet when working with observations of gravity waves we can only make informed guesses of their sources. In this work we use GROGRAT to backwards ray trace stratospheric observations of gravity waves globally to learn more about their origins.

We use observations of temperatures at 40km altitude observed by the AIRS (Atmospheric InfraRed Sounder) instrument on NASA’s Aqua satellite. From these observations we extract temperature perturbations and use the 3D Stockwell transform to derive gravity wave properties such as momentum flux, horizontal wavelength, vertical wavelength. These gravity waves are then backwards ray traced through the ERA5 atmosphere. The significance in this work lies in the volume: we ray trace 21 years (2002-2022) of AIRS data globally, representing by far the largest such observational dataset ever reverse ray-traced.

By investigating the lowest traceable altitude of these rays, we can attribute the gravity waves to their sources (orographic gravity waves will originate near the surface whilst convective waves will have a higher origin). We can also investigate the horizontal propagation of orographic gravity waves from specific mountain ranges and how this changes seasonally. This work aims to answer the question: “Where do gravity waves observed by AIRS come from?”

How to cite: Noble, P., Wright, C., Hindley, N., and Moffat-Griffin, T.: Ray-tracing global gravity wave observations in 21 years of AIRS data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8137, https://doi.org/10.5194/egusphere-egu23-8137, 2023.

EGU23-8145 | PICO | AS1.19

Simulation of the quasi-biennial oscillation using a fully 3D transient gravity-wave parameterization 

Young-Ha Kim, Georg Voelker, Gergely Bölöni, Günther Zängl, and Ulrich Achatz

Using a 3-dimensional (3D) Lagrangian ray-tracing approach, a realistic gravity-wave (GW) parameterization has been developed: Multi-Scale Gravity Wave Model (MS-GWaM). It is a unique and useful tool to simulate and study the 3D transient dynamics of GWs and their interactions with various meteorological phenomena. We implement MS-GWaM into the ICOsahedral Non-hydrostatic model (ICON) and conduct a simulation of the quasi-biennial oscillation (QBO). A particular focus of the study is on the effect of oblique propagation and transient dynamics of GWs on the simulated QBO dynamics. Source spectra of GWs in MS-GWaM are calculated online using the convective latent heat modeled by ICON's cumulus parameterization, as the QBO dynamics is sensitive to the source spectra. In the GW-source scheme a tuning parameter, the areal fraction of convective cells in a model grid cell, is used to produce a reasonable QBO period. In the simulation result, the amplitude of the QBO is realistic in the middle stratosphere but underestimated in the lower stratosphere. The easterly QBO wind is shorter in height than that of the observed QBO. It is notable that in the solstice seasons when the convective activity is maximal off the equator (~8°), GWs with relatively large horizontal wavelengths tend to propagate equatorward from the active convection region. This oblique propagation leads to an effective coupling between the GWs and the QBO. Another simulation is performed using the same experimental setup except that in MS-GWaM the horizontal propagation is neglected and the steady-state assumption is used, as in conventional GW parameterizations. The QBO in this simulation exhibits a large difference from that using the 3D transient MS-GWaM: The QBO has a much longer period (~4 years) and its easterly phase descends a bit less. QBO jets tend to form off the equator in the solstice seasons, centered on the latitudes of active convection.

How to cite: Kim, Y.-H., Voelker, G., Bölöni, G., Zängl, G., and Achatz, U.: Simulation of the quasi-biennial oscillation using a fully 3D transient gravity-wave parameterization, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8145, https://doi.org/10.5194/egusphere-egu23-8145, 2023.

EGU23-9196 | ECS | PICO | AS1.19

MS-GWaM - A three dimensional transient parameterization for internal gravity waves in atmospheric models 

Georg Sebastian Voelker, Young-Ha Kim, Gergely Bölöni, Günther Zängl, and Ulrich Achatz

Internal gravity waves (IGWs) are important distributors of energy and momentum in a stratified atmosphere. While most IGWs are presumably excited at lower altitudes their effects are most important between the upper troposphere and the mesopause (~85km). During propagating - both in the vertical and the horizontal - nonlinear IGWs can exert a wave drag on the large-scale winds, interact with the large-scale potential temperature, and influence transport and mixing of atmospheric constituents such as aerosols or greenhouse gases.

In state-of-the art weather and climate prediction models subgrid-scale IGWs are typically parameterized neglecting both the horizontal wave propagation (single-column assumption), the transient wave behavior including its effect on wave-mean-flow interactions (steady-state assumption) as well as time dependent wave generation. While being computationally efficient the missing physics, however, may lead to model errors and inaccurate predictions under varying boundary conditions. The potential importance of the horizontal wave propagation and wave transience has been shown in various theoretical, numerical and experimental studies.

The transient Multi Scale Gravity Wave Model (MS-GWaM) - implemented in the high-top model UA-ICON - aims to improve these shortcomings by allowing for transient and three dimensional wave propagation. The parameterization is based on a multi scale WKBJ analysis of the compressible atmosphere and includes various non-orographic wave sources, non-dissipative wave-mean-flow interactions as well as wave breaking. Internally, the parameterized gravity waves are treated as Lagrangian volumes with the dynamics prescribed by the well known gravity wave modulation equations. A suitable projection method of wave properties onto the unstructured model grid facilitates the calculation of wind and temperature tendencies. What is more, an efficient parallelization of the ray-tracing scheme allows for simulations in reasonable computation times, being much faster than corresponding wave resolving runs.

While satisfactorily reproducing the observed zonal-mean wind and potential temperature climatology the model results reveal new insight into the detail of the role of IGWs in the atmosphere. In particular, probability density functions of wave momentum fluxes exhibit the typical observed long tails (i.e. wave intermittency) which cannot be reproduced with steady-state parameterizations. Moreover, the three dimensional distribution of wave momentum and wave action fluxes differ greatly when relaxing the single-column assumption. As an example the well known three dimensional refraction of IGWs into polar jets can be shown.

How to cite: Voelker, G. S., Kim, Y.-H., Bölöni, G., Zängl, G., and Achatz, U.: MS-GWaM - A three dimensional transient parameterization for internal gravity waves in atmospheric models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9196, https://doi.org/10.5194/egusphere-egu23-9196, 2023.

From March to December 2014, Loon LLC flew 107 super-pressure balloons in the lower stratosphere over the Southern Ocean. Their GPS sampling frequency of 1Hz allowed them to sample motion associated with atmospheric internal gravity waves generated by the Andes mountains, small islands, and non-orographic sources such as fronts. Analyzing the balloons’ data time series using wavelets, we present distributions of the gravity waves’ momentum fluxes, phase speeds, and wavelengths, both in the time-mean and as they vary from month to month. Many climate models parameterize gravity waves using a phase speed-momentum flux relationship, so we focus on the relationship between those quantities.

How to cite: Green, B. and Sheshadri, A.: Gravity Wave Phase Speeds, Wavelengths, and Momentum Fluxes Observed Above the Southern Ocean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9679, https://doi.org/10.5194/egusphere-egu23-9679, 2023.

EGU23-11529 | ECS | PICO | AS1.19

Modelling horizontal propagation of orographic Gravity Waves in climate models 

Sebastian Rhode, Roland Eichinger, Peter Preusse, Hella Garny, and Lukas Krasauskas

Gravity waves (GWs) transport energy within the atmosphere both in vertical and horizontal direction. While the former is considered in climate models via parameterizations, the latter is often not modeled in most long time simulations. Especially orographic GWs can propagate horizontally more than 1000 km from their sources, however, and thereby de- or accelerate winds in completely different regions. To remedy this, we present a model that is capable of describing orographic GW sources and the associated GWs and their propagation in the atmosphere. From this, we can approximate general propagation pattern, which in the following can be used in climate models (here EMAC) to improve the orographic GW parameterization. The first simulations show strong redistribution of wave drag from land masses and thereby a closing of the gap of missing wave drag at 60°S.

How to cite: Rhode, S., Eichinger, R., Preusse, P., Garny, H., and Krasauskas, L.: Modelling horizontal propagation of orographic Gravity Waves in climate models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11529, https://doi.org/10.5194/egusphere-egu23-11529, 2023.

EGU23-12273 | PICO | AS1.19

The CAIRT earth explorer 11 mission: a way towards global gravity wave momentum budgets 

Peter Preusse, Inna Polichtchouk, Scott Osprey, Joern Ungermann, Sebastian Rhode, Martyn Chipperfield, Quentin Errera, Felix Friedl-Vallon, Bernd Funke, Sophie Godin-Beekmann, Alex Hoffmann, Alizee Malavart, Piera Raspollini, Björn-Martin Sinnhuber, Pekka Verronen, and Kaley Walker

Retrieving global observations of gravity waves (GW) from recent satellite missions is challenging. Nadir viewing satellites such as AIRS provide directional momentum fluxes, but lack fine vertical resolution and hence observe only those GW with exceptionally high intrinsic phase speed. Limb scanning instruments such as HIRDLS and SABER have only a single measurement track and hence provide only an estimate of absolute GW momentum flux. In addition, the sparse along-track sampling of these limb sounders introduce uncertainties in horizontal wavelength. GPS-RO can provide GW profile triplets, allowing in principle the horizontal direction of GW propagation to be inferred, but these triplets are rare. Finally, direct wind measurements from Aeolus are restricted in altitude to less than ~25km and only provide the wind component in the direction of the lidar beam from one observational track. In consequence, also Aeolus cannot reveal horizontal propagation direction and GW momentum flux.

This situation could be dramatically improved by bringing a limb imager into space. A limb imager combines the very dense spatial sampling of a nadir viewing instrument with the high vertical resolution of a limb sounder. This will provide an almost complete description of the vertical spectrum of GWs, necessary for inferring drag estimates. Such global GW momentum flux data would for the first time allow to retrieve a global momentum budget from the mid-troposphere to the upper mesosphere.

The changing-atmosphere infra-Red Tomography (CAIRT) mission candidate for ESA's earth explorer 11 proposes a limb imager for spatial sampling of 25 km across-track, 50 km along-track and 1 km in the vertical. From this we expect to infer directional GW momentum fluxes from the tropopause to 70 km or higher. This will allow longstanding scientific questions to be addressed such as the quantification of tropospheric GW sources and their related phase speed spectra and the identification of secondary wave generation in the stratosphere and lower mesosphere. Considering the momentum flux at higher altitudes, secondary wave generation competes with oblique GW propagation which allows GWs from low latitude sources to reach the high latitudes mesosphere and thus avoid critical levels. In general, two-way interaction with the background flow will be considered via the modulation of the GW spectrum by the winds and the mean wind accelerations by the GWs. In this contribution we will outline the CAIRT instrument concept, give an overview of the mission’s objectives and demonstrate its potential using simulated observations.

How to cite: Preusse, P., Polichtchouk, I., Osprey, S., Ungermann, J., Rhode, S., Chipperfield, M., Errera, Q., Friedl-Vallon, F., Funke, B., Godin-Beekmann, S., Hoffmann, A., Malavart, A., Raspollini, P., Sinnhuber, B.-M., Verronen, P., and Walker, K.: The CAIRT earth explorer 11 mission: a way towards global gravity wave momentum budgets, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12273, https://doi.org/10.5194/egusphere-egu23-12273, 2023.

EGU23-12882 | PICO | AS1.19

Gravity wave signatures in mesospheric/lower thermospheric winds caused by Hunga Tonga-Hunga Ha‘apai volcanic eruption identified by CONDOR and the Nordic Meteor Radar Cluster 

Gunter Stober, Alan Liu, Alexander Kozlovsky, Zishun Qiao, Masaki Tsutsumi, Njål Gulbrandsen, Satonori Nozawa, Mark Lester, Evgenia Belova, Johan Kero, and Nicholas Mitchell

Gravity waves are a major source of the middle atmospheric short-term variability. The Hunga Tonga-Hunga Ha‘apai volcanic eruption provided a unique opportunity to study gravity wave propagation around the globe from a well-defined source. The eruption triggered several atmospheric signatures including a lamb wave (troposphere/stratosphere/mesosphere) and a package of gravity waves. Here we present results of gravity wave signatures found in mesospheric winds leveraging multi-static meteor radar networks such as the Nordic Meteor Radar Cluster and CONDOR. We were able to identify the eastward and westward propagating gravity waves. Furthermore, it was possible to estimate the intrinsic wave properties such as a horizontal wavelength of approximately 1600-2000 km and an intrinsic phase speed of 200 m/s.

How to cite: Stober, G., Liu, A., Kozlovsky, A., Qiao, Z., Tsutsumi, M., Gulbrandsen, N., Nozawa, S., Lester, M., Belova, E., Kero, J., and Mitchell, N.: Gravity wave signatures in mesospheric/lower thermospheric winds caused by Hunga Tonga-Hunga Ha‘apai volcanic eruption identified by CONDOR and the Nordic Meteor Radar Cluster, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12882, https://doi.org/10.5194/egusphere-egu23-12882, 2023.

 The momentum transport by orographic gravity waves (OGWs) plays an important role in driving the large-scale circulation throughout the atmosphere, which is subject to parameterization in numerical models. Current parameterization schemes commonly assume that the unresolved OGWs are hydrostatic, typically only valid for waves with large horizontal scale, weak winds and high stability. These schemes were originally developed for coarse-resolution numerical models and, as a result, captured the first-order effects of unresolved OWGs. With the increase in the horizontal resolution of state-of-the-art numerical models, unresolved OGWs are of smaller horizontal scales and may be more influenced by nonhydrostatic effects (NHE), thus challenging use of the hydrostatic assumption. Based on the analytical formulae of nonhydrostatic OGWs derived in our recent study, this work revises the orographic gravity wave drag (OGWD) parameterization scheme employed in the Model for Prediction Across Scales (MPAS) by accounting for NHE. Global simulations are conducted to investigate NHE on the momentum transport of parameterized OGWs and their impact on the simulated large-scale circulation. NHE are found to be the most evident in regions of complex terrain where the subgrid-scale orography is narrow. As NHE act to reduce the surface wave momentum flux (WMF) of OGWs, the revised scheme tends to inhibit wave breaking in the lower troposphere and transport more WMF upward, leading to an enhancement of OGWD in the upper troposphere and lower stratosphere. Over Antarctica, where the largest zonal-mean NHE occur, the OGWD-induced meridional circulation is strengthened, which helps reduce the cold pole and westerly wind biases associated with a too strong polar vortex, thereby alleviating the delayed breakdown of the Antarctic polar vortex in late spring and early summer, a bias commonly found in climate models.

How to cite: Xu, X., Zhang, R., Teixeira, M., van Niekerk, A., and Li, R.: A parametrization scheme accounting for non-hydrostatic effects on vertically propagating orographic gravity waves and implementation in the Model for Prediction Across Scales (MPAS), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13248, https://doi.org/10.5194/egusphere-egu23-13248, 2023.

EGU23-14145 | ECS | PICO | AS1.19

Comparison of Stratospheric Gravity Waves in a High-resolution General Circulation Model with 3-D Satellite Observations 

Haruka Okui, Corwin Wright, Neil Hindley, and Kaoru Sato

Recently, high-resolution satellite instruments and general circulation models (GCMs) which resolve gravity waves explicitly are becoming available. However, because of their small temporal and spatial scales, the entire spectral range of gravity waves cannot be fully detected by global observations or simulated by a GCM. To enhance our understanding of the characteristics of gravity waves in the middle atmosphere, quantitative comparison between observed and model-simulated gravity waves is of great importance. The aim of this study is to make a quantitative comparison between gravity waves observed by the Atmospheric Infrared Sounder (AIRS) on NASA’s Aqua satellite and those simulated by a gravity-wave permitting GCM, named JAGUAR. As a nadir-viewing satellite instrument, AIRS has relatively high horizontal resolution varying from ~13.5 km to ~41 km and coarse vertical resolution of 7–20 km over the altitude range of 15–60 km. JAGUAR is a hydrostatic spectral GCM with a T639 triangular truncation. This model contains 340 layers from the ground to the model top of ~150 km with a constant log-pressure height interval of 300 m. We first applied a vertical filter simulating the observational filter of AIRS to the output data of hindcast simulations in the 2018/19 boreal winter performed with JAGUAR. Then, the filtered model data were resampled as AIRS observational granules. Gravity waves were extracted by subtracting a fourth-order polynomial fit in the cross-track direction of a granule, whose data length is 1780 km. A three-dimensional Stockwell transform was utilized to examine the amplitudes and wavelengths of dominant waves. Stratospheric gravity waves in the model results are compared with those in AIRS observations. It was shown that amplitude, zonal momentum flux, and meridional momentum flux of the gravity waves are in good agreement between the JAGUAR and AIRS data. These results support the validity of studies on gravity waves and their roles in the middle atmosphere by using the JAGUAR model. Peaks of gravity-wave amplitudes are observed along the winter eastward jet and summer westward jet. The peaks located in the former region got weaker, and the latter got stronger as the stratospheric sudden warming in January 2019 progressed. Compared to waves in the model data without the vertical filter applied, dominant waves in the filtered model data are half the amplitude in the regions where strong gravity waves are observed. This difference is most remarkable in eastern Eurasia, where the vertical wavelengths of dominant waves are relatively short. This fact implies the importance of careful consideration on the underestimation of wave amplitudes due to AIRS observational filter especially where waves having short vertical wavelengths are likely dominant.

How to cite: Okui, H., Wright, C., Hindley, N., and Sato, K.: Comparison of Stratospheric Gravity Waves in a High-resolution General Circulation Model with 3-D Satellite Observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14145, https://doi.org/10.5194/egusphere-egu23-14145, 2023.

EGU23-14447 | PICO | AS1.19

Observation of Gravity Waves and Turbulence at the Polar Night Jet 

Gerd Baumgarten, Eframir Franco-Diaz, Jens Fiedler, Michael Gerding, Ralph Latteck, Mohammed Mossad, Thoralf Renkwitz, Irina Strelnikova, Boris Strelnikov, and Robin Wing

The polar night jet, i.e., the edge of the polar vortex, maximises in the altitude range of 30 km to 70 km. The polar vortex is known to affect even underlying layers and the weather. The polar night jet shows the highest mean wind speeds observed in the atmosphere and likely plays an important role in multi-step vertical coupling not only from the ground, but also from the upper atmosphere downward.

Direct measurements of the polar night jet’s extreme atmospheric motion are rare and limited to a few rocket soundings or locations with dedicated remote sensing techniques.

 

We operate lidar and radar instruments capable of measuring temperatures and winds above northern Norway (ALOMAR, 69°N) and northern Germany (Kühlungsborn, 54°N). The instruments have observed the atmosphere frequently inside and outside the Polar Vortex for more than 10 years.

Using lidar measurements of temperatures and winds allows for studying up- and downward-propagating gravity waves in complicated dynamical situations that are often found at the polar vortex edge. Observing simultaneously up- and downward propagating waves may indicate gravity wave breakdown as well as the generation of secondary gravity waves and turbulence. Turbulence is frequently detected using the MAARSY VHF radar. So called Polar Mesosphere Winter Echoes (PMWE) are observed if sufficient ionisation and turbulence exist.

We will discuss the relationship between waves, turbulence, and the polar vortex based on lidar and radar observations.

How to cite: Baumgarten, G., Franco-Diaz, E., Fiedler, J., Gerding, M., Latteck, R., Mossad, M., Renkwitz, T., Strelnikova, I., Strelnikov, B., and Wing, R.: Observation of Gravity Waves and Turbulence at the Polar Night Jet, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14447, https://doi.org/10.5194/egusphere-egu23-14447, 2023.

EGU23-14959 | ECS | PICO | AS1.19

Oblique propagation and refraction of mountain waves over the Andes observed by GLORIA and ALIMA during the SouthTRAC campaign 

Lukas Krasauskas, Bernd Kaifler, Sebastian Rhode, Joern Ungermann, Wolfgang Woiwode, and Peter Preusse

The SouthTRAC measurement campaign was held in Argentina from September to November 2019 using the HALO research aircraft. One of the main goals of the campaign was gravity wave (GW) study in the region of Southern Andes: a global hotspot for GW activity. The measurements included air temperature data from the IR limb imaging spectrometer GLORIA jointly developed by FZJ and KIT, as well as ALIMA, an upward looking lidar developed by DLR, and in situ instruments. GLORIA's viewing direction can be panned between 45° and 135° with respect to the flight direction. Combining this capability with flight paths that encircle the observed atmospheric region, multiple measurements of the same air mass can be performed, allowing for 3D tomography of the atmosphere with a vertical resolution down to 250 m and horizontal resolution of around 25 km. GLORIA provides data below the flight altitude of the HALO aircraft (up to 15 km), while ALIMA observations cover the altitude range between 20 and about 60 km. GLORIA is the airborne demonstrator of the satellite based infrared limb imager CAIRT proposed as the Earth Explorer 11 candidate.  

During a research flight on 20-21 September, a large amplitude mountain wave was observed over the Andes. GLORIA 3D data showed a complex temperature structure with several overlapping gravity wave families at altitudes of 9 to 14 km above the mountain ridges. The amplitudes and 3D wave vectors for each of those families were determined by performing a least-squares fit of harmonic disturbances to the GLORIA temperature data. These wave parameters were then used to initialise a ray-tracer (GROGRAT ray-tracing code was used) and follow the path of the waves as they propagated upwards and away from the mountain range. The results of this study could be summarised as follows:

  • Many of the waves observed by GLORIA in the 9-14 km altitude range propagated into the regions observed by ALIMA in 25-40 km altitudes. There was very good agreement between ALIMA data and GLORIA data-initialised ray tracing results: GWs observed by GLORIA were shown to propagate into the same regions where waves were seen by ALIMA and their spectral characteristics also closely matched ALIMA observations.
  • Oblique GW propagation was directly observed, including propagation of some GWs toward the upwind side of the Andes mountain range. Oblique propagation also resulted in significant meridional transport of zonal gravity wave momentum flux (GWMF).
  • We observed strong horizontal GW refraction, with some wave vectors turning by more than 50°. This resulted in significant momentum exchange between waves and the background flow outside of wave generation and breaking regions. 
  • We also use the GLORIA data to study the time dependence (as a result of changing winds) of the mountain wave pattern over the Andes.

How to cite: Krasauskas, L., Kaifler, B., Rhode, S., Ungermann, J., Woiwode, W., and Preusse, P.: Oblique propagation and refraction of mountain waves over the Andes observed by GLORIA and ALIMA during the SouthTRAC campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14959, https://doi.org/10.5194/egusphere-egu23-14959, 2023.

EGU23-15558 | ECS | PICO | AS1.19

The impact of subgrid-scale gravity waves on the Brewer-Dobson circulation 

Gökce Tuba Masur, Young-Ha Kim, and Ulrich Achatz

The Brewer-Dobson circulation (BDC) is a meridional circulation mainly driven through mean-flow forcing by Rossby-wave breaking that is, however, also influenced by gravity waves (GW). As some part of GW dynamics is subgrid-scale in numerical climate and weather prediction models, an appropriate wave parameterization and later an accurate separation of the drivers are necessary to understand the impact of the subgrid-scale GWs on the BDC.

Polichtchouk et al. (2018) explored the sensitivity of BDC to the parameterized GW drag by separating the drivers of the residual circulation using the downward-control principle. Even in relatively high-resolution simulations, the parameterized drags are found to significantly contribute to the BDC in the lower stratosphere, especially for northern hemisphere winter-pole downwelling.

We parameterize subgrid-scale GWs in the Lagrangian ray-tracing scheme Multi-Scale Gravity-Wave Model (MS-GWaM) (Bölöni et al. 2021; Kim et al. 2021). MS-GWaM includes interactions between the GW field and the resolved flow, which are neglected in the traditional GW parameterization schemes. It has been implemented successfully into of the Icosahedral Non-hydrostatic (ICON) model in its upper-atmosphere configuration. Using the MS-GWaM output, we diagnose the sensitivity of the BDC using the downward-control principle.

How to cite: Masur, G. T., Kim, Y.-H., and Achatz, U.: The impact of subgrid-scale gravity waves on the Brewer-Dobson circulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15558, https://doi.org/10.5194/egusphere-egu23-15558, 2023.

EGU23-336 | ECS | Posters virtual | AS1.21

Linking Atmospheric Moisture Transport to Extreme Precipitation Events Associated with Floods over India 

Akash Singh Raghuvanshi and Ankit Agarwal

The primary component of the atmospheric branch of the water cycle is atmospheric moisture transport, and its amplitude has a strong influence on drought and precipitation extremes. Vertically integrated water vapor transport (IVT) is evaluated to assess atmospheric moisture transport (AMT) over the Indian Subcontinent. Linkages to flood-causing extreme precipitation events are understood using case studies that were in accordance with their intense rainfall conditions and flooding that resulted in huge losses over a specified region. Using a high-resolution daily gridded rainfall data set, an attempt has been made to analyze the spatiotemporal characteristics of atmospheric moisture transport (AMT) responsible for extreme events. The spatiotemporal characteristics of specific rainfall events associated with the occurrence of AMT show the existence of a strong relationship between the presence of high AMT and extreme precipitation events for the northwestern region where AMT penetrates inland and for the east coast region where AMT makes landfalls. Further analysis suggests that extreme precipitation events are predominantly influenced by the strong moisture convergence associated with the low-level pressure systems, wind speed, and wind direction developed in the vicinity of affected regions.

How to cite: Singh Raghuvanshi, A. and Agarwal, A.: Linking Atmospheric Moisture Transport to Extreme Precipitation Events Associated with Floods over India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-336, https://doi.org/10.5194/egusphere-egu23-336, 2023.

EGU23-1553 | ECS | Orals | AS1.21

Sources of Moisture to Extreme Atmospheric Rivers: a storm Denis case study 

Ferran Lopez-Marti, Lichuan Wu, Gabriele Messori, and Anna Rutgersson

Moisture transport within atmospheric rivers (ARs) is a complex combination of processes, with convergence of moisture with different origin and its changes over the life cycle of an AR. The water vapour budget in an AR enables us to understand the contribution of the different moisture sources and sinks (horizontal transport, local evaporation and precipitation). Here, we focus on how these contributed to the formation and development of the exceptional AR associated with storm Denis that occurred in February 2020 leading to the 3rd highest UK average daily rainfall since 18911.

We use the WRF-ARW numerical limited-area atmospheric model to simulate the life-cycle of the AR in the North Atlantic basin. We use a resolution of 0.09º, and a domain covering both the AR’s formation region close to the Gulf of Mexico to the landfall region in northern and central Europe. Moreover, we performed two sets of sensitivity experiments by reducing the tropical moisture transport, and the sensible heat flux in specific areas of the oceanic basin to assess how these two main components affect the water vapour balance within the AR. We also defined a threshold to map the AR and used a centroid-based method to track its path in order to measure the shift of its location and intensity through time in the different experiments.  

Our findings reveal significant relationships between the reduction of tropical moisture and a change of the location of the AR. The analysis also detected regional and temporal changes in the water vapour budget due to the perturbations done in the sensitivity experiments. In addition, relative importance of moisture sources are assessed. As such, our work provides a new case study to unravel feedback processes and the influence to the AR characteristics when perturbing the water vapour balance.


1 Davies, Paul A., et al. "The wet and stormy UK winter of 2019/2020." Weather 76.12 (2021): 396-402.

How to cite: Lopez-Marti, F., Wu, L., Messori, G., and Rutgersson, A.: Sources of Moisture to Extreme Atmospheric Rivers: a storm Denis case study, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1553, https://doi.org/10.5194/egusphere-egu23-1553, 2023.

EGU23-1738 | ECS | Posters virtual | AS1.21

The spatial variability in isotopic composition of surface snow and snowpits on the East Antarctic Ice Sheet 

Agnese Petteni, Mathieu Casado, Barbara Stenni, Giuliano Dreossi, Elise Fourré, Amaelle Landais, Joel Savarino, Andrea Spolaor, Barbara Delmonte, Silvia Becagli, and Massimo Frezzotti

The water isotope composition of snow precipitations, archived in the Antarctic ice sheet every year, is an important proxy of climatic conditions. This signal depends on several parameters such as local temperature, altitude, moisture source areas and air mass pathways.

However, especially in areas where snow accumulation is very low (as on the East Antarctic Plateau), the isotopic composition is affected by additional spatial variability induced by the interactions between the atmosphere and snow surface, and the pristine signal may be modified through isotopic exchanges, sublimation processes and mechanical mixing originated from wind action.

Here, we present the isotopic composition (δD and δ18O) and the second-order parameter d-excess of surface snow and snowpit samples collected during the Italian-French campaign in Antarctica (2019-2020). The sampling sites cover the area from Dumont D'Urville to Concordia Station and from Concordia Station towards the South Pole (EAIIST – East Antarctic International Ice Sheet Traverse). These data, compared with a previous dataset of Antarctic surface snow isotopic composition (Masson-Delmotte et al. 2008), are analyzed to determine the variability of the spatial relationship between precipitation isotopic composition and local temperature in relation to geographical parameters (latitude, distance from the coast and elevation). The interpretation of these factors determining the isotope signature is the base to better define the amount of the effects caused by subsequent interaction between atmosphere and surface snow, and by the wind action.

Understanding the spatial variability of this proxy, which strongly decreases the signal-to-noise ratio, could permit to improve the use of the “isotopic thermometer” to quantify past changes in temperature based on the stable isotopic record of deep ice cores.

How to cite: Petteni, A., Casado, M., Stenni, B., Dreossi, G., Fourré, E., Landais, A., Savarino, J., Spolaor, A., Delmonte, B., Becagli, S., and Frezzotti, M.: The spatial variability in isotopic composition of surface snow and snowpits on the East Antarctic Ice Sheet, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1738, https://doi.org/10.5194/egusphere-egu23-1738, 2023.

Stable isotope ratios of oxygen (δ18Op) and hydrogen (δDp) record information about the hydrological cycle. These signals are preserved in natural archives, such as speleothems, stalagmites, ice cores, and pedogenic carbonates. Recent studies have used these proxy records of water isotopologues to reconstruct the evolution of paleoclimates, paleoenvironments, and even tectonic-related changes in surface elevations. However, such reconstructions require information about the atmospheric dynamics that drive the spatial variability of isotopic ratios. δ18Op and δDp are known to reflect the history of air masses, surface temperature, precipitation, and synoptic-scale atmospheric teleconnection patterns like the North Atlantic Oscillation (NAO). Climate-driven variations in these data can complicate their interpretation of geologic processes. The NAO is the predominant mode of inter-annual and seasonal variability that controls the weather and climate system across the North Atlantic region and continental Europe. The influence of the NAO on the Global Network of Isotopes in Precipitation (GNIP) stations records of δ18Op and δDp across Europe was previously studied in the winter season when the NAO impacts are well defined. 

Here we build upon previous work by (1) investigating the present-day NAO-δ18Op and -δDp relationships and their associated atmospheric dynamics and causal mechanism in all seasons, and (2) studying the NAO’s influence on the δ18O and δD in precipitation in the late Cenozoic. We focus on the latter since many δ18Op- and δDp-based studies tackle problems in the Late Cenozoic. In addition, important characteristics of such pressure systems (e.g., the location of the centers of maximum and minimum pressures and axis of polarity) may change over longer (centennial to geological) time scales in response to different forcings such as atmospheric CO2, paleogeography, orbital changes, and land-surface cover. To achieve the study’s first goal, we explore the NAO-δ18Op and -δDp link by tracking the NAO in the ERA5 reanalysis data and relating its variability with GNIP observational data across Europe. For the second goal, we use the isotope-enabled Atmospheric General Circulation Model ECHAM5-wiso to perform time-specific, high spatial resolution (paleo)climate simulations with (paleo)environmental conditions of the middle Miocene (~14 Ma), the mid-Pliocene (~3 Ma), the Last Glacial Maximum (~21 ka), the mid-Holocene (~6.5 ka), the pre-industrial (the reference year 1850) and the present-day (1979-2000). We then transfer the analyses from the first step to our paleoclimate simulation output, using the present-day simulation for calibration. Our results help reconstruct the NAO from proxy archives and provide context for more refined interpretations of the isotopic ratios of rainwater in proxy archives.

How to cite: Boateng, D., G. Mutz, S., and A. Ehlers, T.: The influence of North Atlantic Oscillation on oxygen and hydrogen stable isotopes in precipitation of the Late Cenozoic: implications on paleoenvironment reconstructions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1752, https://doi.org/10.5194/egusphere-egu23-1752, 2023.

In East Asia, summer monsoon rainbands usually stretch for thousands of kilometers in the east-west direction and are capable of producing heavy rainfall intensity of 20-40 mm day-1 on average, rendering them the culprit of many devastating historical floods. Despite the previous endeavor to understand their formation dynamics and hazards, the atmospheric water cycle of these rainband systems remains surprisingly poorly understood. In this study, we leverage backward moisture tracking to demystify the dominant moisture pathways and sources that feed the East Asian rain belt events during the warm season (April to September) from 1981 to 2018. The simulations were conducted using a semi-Lagrangian dynamical recycling model (DRM) forced by hourly-0.25˚ ERA5 reanalysis. In virtue of an Expectation-Maximization (EM)-based curve clustering, we classify up to 15 moisture pathways along four main corridors reaching the Somali Jet, South Asia, the Bay of Bengal and the Pacific basin. Long-range moisture pathways turn out to dominate high-impact monsoon rainbands, coinciding well with the role of planetary-scale atmospheric rivers in triggering extreme rainfall over East Asia. The result also highlights the importance of terrestrial moisture pathways and sources in supplying rain belts. Back-tracing the moisture pathways and atmospheric rivers unravels interesting couplings of pre-existing weather systems. The terrestrial moisture pathways over South Asia turn out to link to circumglobal wave trains at the upper levels up to a two-week lead time. The findings here bridge the knowledge gap in the regional hydrological cycle of the disastrous East Asian rain belts. The pre-existing weather systems uncovered by tracking the moisture and atmospheric rivers also provide potential predictability of heavy precipitation in East Asia.

How to cite: Lu, M., Cheng, T. F., and Dai, L.: Improved Understanding of the East Asian Monsoon Rainbands and Dynamics Via Lagrangian Moisture Tracking and Atmospheric Rivers Analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2474, https://doi.org/10.5194/egusphere-egu23-2474, 2023.

Abstract

Summer (June to August) precipitation over the Three-River Headwaters’ (TRH) region has experienced a significant dry-to-wet transition during 1979-2020. The transition could have been caused by changed atmospheric circulations, which was modulated by oceanic forcings. This study intends to improve our understanding of the summer precipitation variability over the TRH region under the influence of oceanic modes. The combined effect of three interdecadal oceanic modes [Pacific decadal oscillation (PDO), Atlantic multidecadal oscillation (AMO), and Indian Ocean Basin mode (IOBM)] on the interdecadal dry-to-wet transition was examined, using composite analysis on HadISST and the fifth generation ECMWF reanalysis (ERA5) datasets. The results show that in positive AMO and negative PDO phases, a zonally oriented teleconnection wave train is generated across the Eurasian mid-to-high latitudes, propagating from the North Atlantic to northern East Asia along the westerly jet. This results in a weakened and northward-shifted westerly jet. Furthermore, the enhanced and northward-shifted Western Pacific Subtropical High (WPSH) brings water vapor from the Pacific Ocean, and cyclonic circulation over the Arabian Sea increases the amount of water vapor entering the TRH region. In positive IBOM phases, the warm Indian Ocean induces an anomalous anticyclone over the Bay of Bengal, and anomalous southwesterly delivers abundant water vapor from the Indian Ocean to the TRH region, which overlaps with the vapor transport caused by a positive AMO and PDO. As the Atlantic and Northern Pacific Oceans warm, the enhanced Walker circulation suppresses the ascending motion in the central Pacific and enhances the equatorial easterly, which in turn strengthens the anomalous anticyclone over the Bay of Bengal. As a result, the summer precipitation over the TRH is further increased. The analysis shows that the combined effect of the three oceanic modes played an important role in the dry-to-wet transition.

How to cite: Liu, X., Yang, M., Chen, D., and Wang, H.: The dry-to-wet transition of summer precipitation over the Three-River Headwaters’ region: the role played by three interdecadal oceanic modes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3316, https://doi.org/10.5194/egusphere-egu23-3316, 2023.

EGU23-3551 | ECS | Orals | AS1.21

Global warming triggers the notable rise in water vapour: implications for global climate change 

Vikas Kumar Patel and Jayanarayanan Kuttippurath

Among all greenhouse gases (GHGs), atmospheric water vapour is the most abundant and has huge influence on the Earth’s radiation budget, and plays decisive role in regional weather processes. Unlike other GHGs, which are controlled by emissions, atmospheric water vapour is influenced by the surface temperature. Here, we examine the long-term changes in global and regional water vapour using satellite and reanalysis datasets. The annual mean water vapour shows very high values in tropics and low values in the polar and high terrain regions. A clear seasonal cycle is observed in the water vapour, with high values in summer (25–65 kg/m2) and small values in winter (5–20 kg/m2), except in the tropics. The high values in summer is maily due to the enhanced evapotranpiration driven by surface air temperature, and water vapour transport by winds. There is a significant rise in annual mean global water vapour, driven by global warming, about 0.025–0.1 kg/m2/yr for the period 1980–2020. Furthermore, higher positive trends in water vapour is also observed in arid regions (Sahara, Arabian and Thar desert), Indian subcontinent and the Arctic. The higher values of water vapour trends in the Arctic is due to the significant rise in temperature there. Similarly, the increase in water vapour in desert regions is due to water vapour transport from nearby oceans. The associated radiative effects on short-wave at the surface varies from -5 to -70 W/m2 over the tropical radiosonde stations, and the smallest of about -5– -10 W/m2 in the polar regions. This study, therefore,  shows that there is significant rise in water vapour across the latitudes, which could further increase the global temperature through positive feedback mechamism and thus, change global and regional climate.

Keywords: Water Vapour, Evapotranspiration, Global Warming, Arctic, Desert; Radiative Effects

   

How to cite: Patel, V. K. and Kuttippurath, J.: Global warming triggers the notable rise in water vapour: implications for global climate change, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3551, https://doi.org/10.5194/egusphere-egu23-3551, 2023.

EGU23-3606 | ECS | Orals | AS1.21

Estimating the origin of precipitation: uncertainties associated with atmospheric moisture tracking models 

Jessica Keune, Imme Benedict, Chris Weijenborg, Dominik L. Schumacher, Akash Koppa, and Diego G. Miralles

Precipitation is the largest freshwater flux that enables life on land. However, climate change is projected to increase the frequency and intensity of extreme precipitation events, which often culminate in droughts and floods with devastating impacts on humanity and the environment. To better understand the dynamics of precipitation in a changing climate, recent studies aimed to unravel the interaction between evaporation and precipitation. To do so, atmospheric moisture tracking models have often been employed to determine the origins of precipitation and establish source–sink relationships. However, due to the lack of sufficient and accurate observations to evaluate these models, their estimated source regions of precipitation often remain unvalidated. Nonetheless, the number of studies using such models is increasing, even if only a few have addressed associated uncertainties and even fewer employed multiple models.

Here, we advocate the need for moisture tracking model intercomparisons to advance this field of study. Therefore, we provide an overview of models and methods that track moisture through the atmosphere and determine the origins of precipitation. Further, we highlight conceptual differences between these models and demystify assumptions hidden in the analysis of source regions. Using selected case studies, we illustrate the uncertainty associated with the origin of precipitation and highlight the need for coordinated model comparisons using multiple models. Finally, we present our plans to engage with the entire moisture tracking community to collaborate on prospective model intercomparison studies. Through these efforts, we wish to raise awareness about the uncertainties inherent in moisture tracking approaches and achieve a better understanding of the drivers of precipitation in a changing climate.

How to cite: Keune, J., Benedict, I., Weijenborg, C., Schumacher, D. L., Koppa, A., and Miralles, D. G.: Estimating the origin of precipitation: uncertainties associated with atmospheric moisture tracking models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3606, https://doi.org/10.5194/egusphere-egu23-3606, 2023.

EGU23-4543 | Orals | AS1.21

Changing length scales of moisture transport — their isotopic imprint and implications for remote moisture dependence 

Adriana Bailey, Hansi Singh, Jesse Nusbaumer, Mathieu Casado, Alexandre Cauquoin, Kyle Heyblom, and John Worden

Isotope ratios in water vapor record evaporation (E) and precipitation (P) along moisture transport paths. At low latitudes, the path-integrated E-P signal is dominated by local E and P, providing an indicator of tropical water balance. In contrast, at high latitudes, E and P patterns upstream overwhelm local signals, reflecting the dependence on remote moisture sources. This dependence defines the length scales of moisture transport.

 

In the zonal mean, moisture transport length scales can be represented visually in two dimensions by moist isentropic surfaces, along which poleward moisture transport occurs. These surfaces explain why Rayleigh distillation reasonably approximates meridional variations in high-latitude isotope ratios while also providing a physical basis for why polar isotope-temperature relationships are distinct in space and time. 

 

Isotopically enabled GCM simulations and short-duration Antarctic ground-based observations both lend support for the isentropic view of moisture transport. They also suggest that this framework provides a simple means to predict changes in length scale in a warmer climate, assuming zonal-mean humidity changes follow Clausius-Clapeyron scaling. However, isotopic observations with the vertical resolution and temporal coverage necessary to easily evaluate recent and expected future variations in moist isentropic transport are lacking.

 

Here, we consider two possible alternative methods for testing predictions about long-term moisture length-scale changes with isotopic observations. Using the two-decade-long AIRS satellite record, we consider the extent to which mid-free tropospheric hydrogen isotope ratios, normalized by humidity, can provide a measure of length scale in a total-column sense. Second, we ask to what extent moist isentropic transport is set by episodic events, such as warm conveyor belts, that can be observed by infrequent but high-vertical-resolution airborne isotopic measurements. We discuss the implications of enhanced transport efficiency, expected in a warmer future, for increasing length scales and strengthening hydrological dependencies between remote locations.

How to cite: Bailey, A., Singh, H., Nusbaumer, J., Casado, M., Cauquoin, A., Heyblom, K., and Worden, J.: Changing length scales of moisture transport — their isotopic imprint and implications for remote moisture dependence, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4543, https://doi.org/10.5194/egusphere-egu23-4543, 2023.

Vapor from anthropogenic emissions accounted for a significant proportion of the urban atmospheric water due to the process of urbanization. Fossil fuel combustion-derived vapor (CDV) is one of the main sources of anthropogenic water. Due to the extremely low d-excess (δD - 8*δ18O) value of CDV (-206.7‰ weighted average from different kinds of fossil fuels), stable hydrogen and oxygen isotope can be a promising method to partition CDV from other natural sources. Considering several limitations of long-term in-situ measurement of water isotopes in the urban area, this study explored the possibility to use IsoRSM, an isotopic-enable regional spectral model to simulate the emission situation of CDV.

Two experiments were made respectively in Salt Lake City, USA for one month and in Beijing, China for one year. A fixed emitting rate of CDV with a fixed isotopic ratio was added to the evaporation process of the model in the urban domains (2°×2°) of these two cities, and the result indicated that the addition of CDV could significantly decrease the d-excess of water vapor, especially when the boundary layer was stable. The modified d-excess fitted better with the time series and diurnal variation of in-situ observation than the simulation without CDV in Salt Lake City and in the summer monsoon season of Beijing. Furthermore, the addition of CDV also resulted in an obvious negative correlation between vapor d-excess and specific humidity.  In the simulations, the fraction of CDV in the total atmospheric water in January of Salt Lake City reached more than 20% with an average value of 3.4%, and the peak values mainly occurred when the stability of the atmosphere was relatively high. The mean CDV fraction in the monsoon season of Beijing would also be 2.3%. The CDV fraction calculated from vapor d-excess was slightly lower than moisture tracer method. In summary, the bias of d-excess simulation from IsoRSM in the stable boundary layer periods could be improved by adding CDV emission into the local evaporation process.

How to cite: Yang, Y. and Yoshimura, K.: Isotopic Simulation of Combustion-derived Vapor Emission in Urban Areas Using Regional Spectral Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4656, https://doi.org/10.5194/egusphere-egu23-4656, 2023.

EGU23-4775 | ECS | Orals | AS1.21

Heavy Water Isotope Precipitation in Inland East Antarctica Accompanied by Strong Southern Westerly Winds during the Last Glacial Maximum 

Kanon Kino, Alexandre Cauquoin, Atsushi Okazaki, Taikan Oki, and Kei Yoshimura

Stable water isotope signals in inland Antarctic ice cores have provided wealth of information about past climates. This study investigated atmospheric circulation processes that influence precipitation isotopes in inland Antarctica associated with atmospheric circulations in the southern mid-latitudes during the Last Glacial Maximum (LGM, ~21 000 year ago). A couple of probable climates during this climate period were simulated using the isotope-enabled atmospheric general circulation model MIROC5-iso. Our results showed a steepened meridional sea surface temperature gradient in the southern mid-latitudes associated with a strengthening of the southern westerlies. This change in the atmospheric circulation enhanced the intrusion of warm and humid air from low latitudes that contributes to precipitation events, inducing heavy water isotope precipitation inland East Antarctica. Our results suggest that past southern westerlies can be constrained using water isotopic signals in Antarctic ice cores.

How to cite: Kino, K., Cauquoin, A., Okazaki, A., Oki, T., and Yoshimura, K.: Heavy Water Isotope Precipitation in Inland East Antarctica Accompanied by Strong Southern Westerly Winds during the Last Glacial Maximum, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4775, https://doi.org/10.5194/egusphere-egu23-4775, 2023.

EGU23-4927 | Posters on site | AS1.21

Impact of colder vs. warmer tropical sea-surface temperature on water isotopes in precipitation during the Last Glacial Maximum 

André Paul, Thejna Tharammal, Martin Werner, Stefan Mulitza, and Alexandre Cauquoin

Using the isotope-enabled atmospheric general circulation models iCAM5 and ECHAM6-wiso, we investigate the impact of relatively colder vs. warmer tropical sea-surface temperature on isotopes in precipitation during the Last Glacial Maximum. We forced the two models by the same sets of pre-industrial (PI) and Last Glacial Maximum (LGM) surface boundary conditions; the latter were taken from GLOMAP (Paul et al., 2021), which in turn were based on the MARGO project (MARGO Project Members, 2009) and recent estimates of Last Glacial Maximum sea-ice extent.

To test the sensitivity to changes in tropical sea-surface temperature, we deliberately increased respectively decreased the reconstructed tropical sea-surface temperature by about 1.5 °C. We compared our model results to reconstructions from ice cores (cf. Risi et al., 2010) and speleothems (cf. Comas-Bru et al., 2020).  However, the resulting changes in water isotopes in precipitation were surprisingly small and difficult to detect, hence the sensitivity to changes in tropical sea-surface temperature is rather low. We discuss our results as well as the prospect of utilizing more sensitive proxy data that would allow to discriminate between the two sceanrios.

How to cite: Paul, A., Tharammal, T., Werner, M., Mulitza, S., and Cauquoin, A.: Impact of colder vs. warmer tropical sea-surface temperature on water isotopes in precipitation during the Last Glacial Maximum, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4927, https://doi.org/10.5194/egusphere-egu23-4927, 2023.

EGU23-5260 | ECS | Posters virtual | AS1.21

How meteorological and cloud processes affect water isotopes in a tropical rain shadow region? 

Nimya Sheena Sunil and Saikat Sengupta

Stable water isotopes can be used as natural tracers of various physical processes in the atmospheric water cycle. The isotopic signal is modulated by several meteorological and cloud microphysical processes such as moisture recycling, advection, condensation, evaporation, etc. The interaction of these processes with water isotopes are often complex in tropical orographic regions especially in the lee side of the mountains which are, in general,  rain shadow regions. Disentangling the roles of these process in the water isotope variability is very important considering these regions host a gamut of natural archieves from which decadal to centennial scale climate have been reconstructed earlier. Towards this, the current study presents daily rain and ground level vapour isotope observations in a tropical Indian rain-shadow region.The analyses shows that mesoscale convections affect both water isotope values significantly. A considerable isotopic exchange between rain and vapour is also noted in the sub cloud layer suggesting a strong control of sub cloud processes in the isotope values. Using an 1-D model, the role of all these process in the isotope values are further evaluated.     

How to cite: Sheena Sunil, N. and Sengupta, S.: How meteorological and cloud processes affect water isotopes in a tropical rain shadow region?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5260, https://doi.org/10.5194/egusphere-egu23-5260, 2023.

In 2019, a record-breaking drought happened in the middle reaches of the Lancang-Mekong River Basin (M-LMRB), which brings about 650 million dollars in economic loss and affected 17 million residences. As climate change evolute, the LMRB is suffering from increasingly frequent and intensive drought with the mechanisms remaining unclear. This study analyzed the water vapor circulation of the drought event in 2019 based on the land-atmosphere water budget and backward trajectory model. Results show that the precipitation of the M-LMRB from May to October 2019 was 71.9% of the climatological mean (1959-2021). The moisture transported from the Indian Ocean, Bay of Bengal, and Pacific Ocean, which are the main moisture sources of the region, was found to decrease through the backward trajectory model. From the comparison of the atmospheric circulation of 2019 and the climatology, the anomalous anticyclone in the BOB, the anomalous westerlies in the Northeast Indian Ocean, and the anomalous cyclone in the Western Pacific Ocean were found to facilitate the stronger export of water vapor jointly. Therefore, the dynamic processes should be more responsible for the extreme drought event of the LMRB in 2019 than the thermodynamics processes. The findings of this study provide new insights into understanding mechanisms of climate change affecting extreme drought events through the atmospheric circulation and are helpful to the risk management of droughts under climate change.

How to cite: Gong, G., Zhang, S., and Liu, J.: The anomalous water vapor circulation in an extreme drought event in the middle reaches of the Lancang-Mekong River Basin, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6262, https://doi.org/10.5194/egusphere-egu23-6262, 2023.

EGU23-7569 | ECS | Posters on site | AS1.21

Identifying the origin of precipitation moisture within the tropical cyclones outer radius in the North Atlantic basin 

Albenis Pérez-Alarcón, Patricia Coll-Hidalgo, José C. Fernández-Alvarez, Rogert Sorí, Ricardo M. Trigo, Raquel Nieto, and Luis Gimeno

Tropical cyclones (TCs) are one the principal natural hazards for coastal regions in tropical and subtropical latitudes. On a global scale, around 90 TCs form annually, and approximately 16% of them originated in the North Atlantic (NATL) basin. Heavy rainfall, one of the major hazards associated with TCs, can cause catastrophic flash flooding, landslide and related health and socio-economic problems. Therefore, understanding the precipitation origin during the passage of TCs is important to significantly aid in disaster mitigation and risk analysis. This work seeks to identify the origin of precipitation moisture within the TCs outer radius in the NATL basin from 1980 to 2018 by applying a Lagrangian moisture tracking method to air parcel trajectories. The TC information (intensity and position) was retrieved from the HURDAT2 database, while the outer radius was from the TCSize dataset. The pathways of air parcels that precipitated within the TC outer radius were obtained from the global outputs of the FLEXible PARTicle dispersion (FLEXPART) model fed by ERA-Interim reanalysis provided by the European Center for Medium-Range Weather Forecasts. The spatial moisture sources pattern exhibited a north-south split around 10ºN, coinciding with the mean position of the Intertropical Convergence Zone (ITCZ) during the boreal summer. The highest moisture contribution (~39%) during the genesis and peak of maximum intensification was from the tropical Atlantic Ocean north of ITCZ, including ~11% from the Caribbean Sean and ~6% from the Gulf of Mexico, followed by the western NATL (WNATL) with 23.8% and eastern NATL (ENATL) with 16.6%. Curiously, ~10% of moisture was from the Atlantic Ocean south of ITCZ and ~2% from the eastern Pacific Ocean. During the dissipation phase, the moisture sources shifted poleward as TCs moved, with the highest moisture support (~60.3%) from the subtropical north Atlantic Ocean (WNATL + ENATL) and ~11.2% from the NATL north of 50ºN. This behaviour shows that moisture sources for TCs precipitation are located circa to their positions. Indeed, by investigating the moisture uptake pattern along the TCs trajectories, we detected that the highest moisture uptake generally occurred within 3-5º from the TC track. Likewise, the moisture uptake within 2000 km from the TC centre was approximately two times higher during the rapid intensification than during the slow intensification process. Furthermore, the relative position of moisture sources to the TC centre changed from 24 hours before the extratropical transition (ET) process to 24 hours after. That is, before ET, the moisture sources were located in the southwest-south sector, while after ET appeared in the west-southwest sector. Overall, this work provides new insights into the TCs' climatology in the NATL basin. Additionally, these findings can be used as a reference to understand future changes in the origin of precipitation moisture for TCs precipitation under different climate changes scenarios.

How to cite: Pérez-Alarcón, A., Coll-Hidalgo, P., Fernández-Alvarez, J. C., Sorí, R., Trigo, R. M., Nieto, R., and Gimeno, L.: Identifying the origin of precipitation moisture within the tropical cyclones outer radius in the North Atlantic basin, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7569, https://doi.org/10.5194/egusphere-egu23-7569, 2023.

EGU23-8256 | Posters on site | AS1.21

How will climate change affect the isotope composition of meteoric water in the Mediterranean area? 

Marcello Liotta, Giuseppe Castorina, Simona Simoncelli, and Annalisa Cherchi

The relationship between the isotopic composition of precipitation in the Mediterranean Sea, the atmospheric circulation patterns over the region and groundwater properties has been topic of investigation in recent years. Overall, the link between the isotopic composition of precipitation and the Mediterranean climate raises the question of how future climate change could affect the isotope ratios of precipitation and groundwater. Past and future atmospheric properties (i.e. humidity, evaporation, precipitation and winds) over the Mediterranean region can be used to investigate the past and possibly understand future characteristics of meteoric water isotope composition. In order to evaluate how the climate change will affect the isotope composition of meteoric water, we re-evaluated previous rain events in light of well-defined climate framework. The main objective is to retrieve information on the atmospheric circulation systems based on ERA5 reanalysis and relate climate features with the isotope composition of selected rain events. This will allow to identify the most appropriate parameters needed to constrain the circulation systems responsible for those events and their isotope composition. Preliminary results to infer scenario-based considerations on the evolution of the meteoric recharge will be shown and discussed.

How to cite: Liotta, M., Castorina, G., Simoncelli, S., and Cherchi, A.: How will climate change affect the isotope composition of meteoric water in the Mediterranean area?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8256, https://doi.org/10.5194/egusphere-egu23-8256, 2023.

EGU23-9014 | ECS | Posters on site | AS1.21

Moisture sources projections under climate change for Atmospheric Rivers landfalling the Iberian Peninsula 

José C. Fernández-Alvarez, Albenis Perez-Alarcon, Jorge Eiras-Barca, Alexandre Ramos, Gleisis Alvarez-Socorro, Stefan Rahimi, Raquel Nieto, and Luis Gimeno

A combination of Flexpart-WRF simulations forced with ERA5 and the CESM2 model incorporated in the CMIP6 project to infer a series of changes over the present century in the behavior of the landfalling ARs arriving at the Iberian Peninsula was used. Potential changes in the strength and position of their main moisture sources are also studied first in the literature. In general terms, a gradual strengthening in the intensity of these events is expected, observable from an increase in the amount of moisture transported, while no significant changes in the net number of events are observed. A northward shift in the position of the centroids has also been detected. In relation to the moisture sources, an increase in the contribution of these sources to the moisture content is expected, compatible with Clausius-Clapeyron amplification.

How to cite: Fernández-Alvarez, J. C., Perez-Alarcon, A., Eiras-Barca, J., Ramos, A., Alvarez-Socorro, G., Rahimi, S., Nieto, R., and Gimeno, L.: Moisture sources projections under climate change for Atmospheric Rivers landfalling the Iberian Peninsula, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9014, https://doi.org/10.5194/egusphere-egu23-9014, 2023.

EGU23-9026 | ECS | Posters on site | AS1.21

Reconciling the moisture sources of the extreme flood event in July 2021 over western Europe 

Imme Benedict, Chris Weijenborg, Thomas Vermeulen, Jessica Keune, Harald Sodemann, Ruud van der Ent, and Peter Kalverla

From the 12th to the 15th of July 2021, Western Europe was confronted with an abnormal amount of precipitation leading to extreme floods and enormous damage in western Germany, Belgium, Luxembourg and the south of The Netherlands. Locally, almost thrice as much as the monthly precipitation amount was observed, culminating in 175 mm of rain in just two days. Dynamically, a stationary upper-level cut-off low was the driver of moisture transport to the region resulting in the extreme precipitation over a large area. A follow-up step to unravel the hydrometeorology of the event, is to understand the evaporative regions (moisture sources) that contributed to the event. In literature, these different source region contributions were presented, either indicating the importance of transpiration from vegetation over North America and Europe, or highlighting the role of the Baltic sea, which experienced a heatwave and high evaporation rates at the same time.

Here, we reconcile the moisture sources of the flood event in July 2021 and its uncertainties by comparing the results from three different moisture tracking models (WaterSip, HAMSTER & WAM-2layers) forced with ERA5. By further addressing model-internal sensitivities, we (can) provide a thorough estimate of the uncertainty of contributions from different regions to precipitation during the extreme event, and we ascertain the mechanisms that played a role. Our first results confirm that central Europe is the largest contributor of moisture for precipitation during the event (45 – 90%), whereas the Baltic contributed very little (0 – 5%), thereby contrasting results from recent single-model studies. However, substantial differences were found between the moisture tracking models indicating the need to better understand where those difference arise from and employ multi-model moisture tracking intercomparison studies in the future. 

How to cite: Benedict, I., Weijenborg, C., Vermeulen, T., Keune, J., Sodemann, H., van der Ent, R., and Kalverla, P.: Reconciling the moisture sources of the extreme flood event in July 2021 over western Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9026, https://doi.org/10.5194/egusphere-egu23-9026, 2023.

EGU23-9251 | ECS | Orals | AS1.21 | Highlight

AR-tracks: A new comprehensive global catalog of atmospheric rivers 

Sara M. Vallejo-Bernal, Tobias Braun, Norbert Marwan, and Jürgen Kurths

Atmospheric rivers (ARs) are filaments of extensive water vapor transport in the lower troposphere. They play a crucial role in the global water cycle and are a main source of fresh water for the mid-latitudes. However, very intense and persistent ARs are important triggers of heavy rainfall events and have been associated with natural and economical damage. Further motivated by their high impacts, in the last decade occurrences of ARs have been intensively studied, detection algorithms have been developed, and multiple AR catalogs have been produced. As a common approach, the detection of ARs is based on localizing anomalous atmospheric transport of moisture, usually by setting an absolute threshold on vertically integrated vapor transport (IVT) and/or vertically integrated water vapor (IWV) fields. Behind this methodology, there is the implicit assumption of stationary atmospheric moisture levels, which is not necessarily true for long periods under the context of a warming atmosphere. Also, these thresholds have proven to vary regionally which results in often excluded low-level ARs.

Here, we introduce AR-tracks, a global, high-resolution catalog of atmospheric rivers that we have developed based on the Image-Processing-based Atmospheric River Tracking (IPART) algorithm, using IVT estimates of the ERA5 reanalysis data set. As opposed to conventional detection methods, IPART calculates anomalies of the IVT field at the synoptical spatiotemporal scale of ARs and is, therefore, free from magnitude thresholds and stationarity assumptions. The resulting catalog displays a list of AR events, with a spatial resolution of 0.75° x 0.75° and a temporal resolution of 6 hours, covering the period between 1979 and 2019. For each AR, we provide common parameters such as the time and location of the landfall, the respective IVT value, the area, the width, and the length of the AR. Moreover, we also track the contour and the axis of each AR, the position of the centroid, and the proportion of the AR that is located over ocean and land, and over the different continents.

To show the potential of this new catalog, we study the spatiotemporal variability of European ARs between 1979-2019, analyzing the robustness of our results for distinct parameter choices in the definition of AR-tracks. We also use a novel power spectral measure to identify periodic cycles in the occurrence of European ARs, revealing spatially heterogeneous seasonal and multi-annual periodicities. Finally, we discuss the role of land-falling ARs as a trigger of heavy precipitation events in the regional domain.

With the extensive data we provide in this new catalog, we aim at contributing to the further understanding of the role of ARs in global climate dynamics, as long-lived ARs having cross-continent tracks can be reliably traced through their tropical/subtropical origins to high-latitude landfall, and novel topics such as inland penetration of ARs can be studied.

How to cite: Vallejo-Bernal, S. M., Braun, T., Marwan, N., and Kurths, J.: AR-tracks: A new comprehensive global catalog of atmospheric rivers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9251, https://doi.org/10.5194/egusphere-egu23-9251, 2023.

EGU23-9436 | ECS | Orals | AS1.21

Unravelling the sources of moisture for precipitation events in a flood-prone Indian basin 

Rajat Choudhary, Chandrika Thulaseedharan Dhanya, and Ashvani Kumar Gosain

Global warming has resulted in frequent occurrences of hydrological extremes, especially floods, across the globe. Flooding may lead to significant loss of life and economic damage. The increase in these flood events is due to the short intense rainfall events. Finding the geographical sources of the moisture that causes these short intense rainfall events is an important step toward predicting extreme events. The present research intends to investigate moisture sources for precipitation events over the flood-prone Indian Basin. Using the lagrangian moisture diagnostic, the research will look at moisture sources below the boundary layer as well as variations above the boundary layer from 1980 to 2018 during the Indian Summer Monsoon season. The study will also look at how the contribution from various sources varies over the course of the Indian Summer Monsoon Rainfall season. This work will enhance our understanding of the hydrological cycle and assist with a variety of related issues, including water resource planning, weather forecasting, land and water management, and more.

How to cite: Choudhary, R., Dhanya, C. T., and Gosain, A. K.: Unravelling the sources of moisture for precipitation events in a flood-prone Indian basin, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9436, https://doi.org/10.5194/egusphere-egu23-9436, 2023.

EGU23-9668 | Orals | AS1.21

Interrogating the influence of shallow convective mixing on low-level clouds with observations of stable water isotopes 

Sylvia Dee, Jun Hu, Adriana Bailey, Jesse Nusbaumer, Christiana Sasser, and John Worden

Low-cloud feedbacks contribute large uncertainties to climate projections and estimated climate sensitivity. A key physical process modulating low-cloud feedbacks is shallow convective mixing between the boundary layer and the free troposphere. However, there are challenges in acquiring observational estimations of shallow convective mixing with global coverage. To this end, we propose a novel approach to constraining convective mixing using stable water vapor isotope profiles from satellite retrievals. We demonstrate that the vertical gradient of water vapor δD between the boundary layer and free troposphere can be used to track shallow convective mixing, especially over the trade-wind regions. We also evaluate this metric of shallow convective mixing against the EUREC4A experiment data. Analyzing isotopes in water vapor alongside low-cloud properties from satellite retrievals, we find that low-cloud fraction appears insensitive to convective mixing in trade cumulus regions. Our results suggest that satellite-derived observations of the relationship between shallow convective mixing and low-cloud are regionally-dependent, and strong shallow convective mixing is associated with moistening of the free troposphere in the tropics. The new estimations of low-cloud properties and their relationship with changes in convective mixing using water isotopes house potential to improve the simulation of low-cloud feedbacks in numerical simulations, refining estimates of climate sensitivity.

How to cite: Dee, S., Hu, J., Bailey, A., Nusbaumer, J., Sasser, C., and Worden, J.: Interrogating the influence of shallow convective mixing on low-level clouds with observations of stable water isotopes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9668, https://doi.org/10.5194/egusphere-egu23-9668, 2023.

 

Understanding rainfall and its extremes is essential for quantifying weather and climate related risks, and the management of water resources. However, climate projections of rainfall have large uncertainties because of differing sensitivities to changes in dynamic, thermodynamic and microphysical factors. Emergent statistical constraints derived from observations and high resolution simulations can be used to reduce these uncertainties, but must be based on process understanding to be robust.

Our recent work shows that clustering rainfall data into regions of similar wet day frequency, regardless of geographical separation, uncovers a strong correlation between wet day occurrence and daily rainfall accumulation distributions. This relationship is robust across a range of observational datasets with differing spatial resolutions.

We hypothesise that this relationship shows that the presence or absence of precipitation generating weather systems (atmospheric rivers, cyclones, fronts and mesoscale convective storms) rather than their individual intensities is critical for daily rainfall totals. In this presentation, we will first examine whether the probability of specific dynamic, thermodynamic and microphysical states drives wet day occurrence. We will also use feature analysis and tracking schemes to identify how the distribution of each of these dynamic, thermodynamic and microphysical states varies for each precipitation generating weather system. This potentially allows a quantification of the importance of different precipitation generating systems for different wet day occurrences and how each contributes to daily accumulation distributions. This expands on previous work which has shown that atmospheric rivers, cyclones, fronts and mesoscale convective storms have varying relationships to rainfall and their extremes. In particular, it allows us to identify their relative importance and explains their relative efficacy for precipitation generation.

How to cite: McDonald, A.: Understanding the relative importance of different precipitation generating weather systems and quantifying their efficiencies, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10922, https://doi.org/10.5194/egusphere-egu23-10922, 2023.

EGU23-11452 | ECS | Posters on site | AS1.21

Stable isotope ratios (δ2H, δ18O and δ17O) of precipitation in Seoul, Korea, during 2016-2020 

Songyi Kim, Yeongcheol Han, Jangil Moon, Yalalt Nyamgerel, and Jeonghoon Lee

Precipitation plays an important role in the global hydrological cycle, and its stable isotope ratio (δ2H, δ18O and δ17O) provides useful information for atmospheric circulation in forming precipitation. However, understanding of precipitation stable isotope ratio in mid-latitude is limited by an insufficient and restricted interpretation of hydrological and meteorological processes based on insufficient datasets. To improve domain knowledge, we monitored the water stable isotopes of rainwater and snowfall in Seoul, Korea, during the period of 2016-2022. The δ2H, δ18O and δ17O values varied from -120.3 to 3.9 ‰, from -16.58 to 1.21 ‰ and from -8.76 to 0.65 ‰, respectively with characteristic seasonal patterns. The prominent patterns were the isotopic depletion during winter (Dec-Feb; the mean δ2H of -9.39 ‰) under the influence of the Siberian High system and the isotopic enrichment during the spring (Mar-May; the mean δ2H of -2.6 ‰) affected by the Asia monsoon system. The summer season was characterized by the lowest deuterium excess (δ2H­ – 8 x δ18O; 7.4 ‰). As the interplay of the northeast Asia monsoon, and the Siberian High and the North Pacific High was the major cause of the seasonality of the isotope values, their covariance with temperature or the amount of precipitation was weak. The local meteoric water line had a lower slope and intercept (δ2H = 7.67 x δ18O + 9.28) compared to the global meteoric water line. Another local meteoric water line between δ17O and δ18O appeared to be δ17O = 0.5312 x δ18O + 0.0068 with a greater slope and intercept than its global meteoric line.

How to cite: Kim, S., Han, Y., Moon, J., Nyamgerel, Y., and Lee, J.: Stable isotope ratios (δ2H, δ18O and δ17O) of precipitation in Seoul, Korea, during 2016-2020, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11452, https://doi.org/10.5194/egusphere-egu23-11452, 2023.

Shallow clouds, ubiquitous in the trade-wind region, substantially contribute to the cooling of the Earth's climate through their shortwave radiative effect. Their response to climate change is unclear, contributing to a large part of the uncertainty of climate projections. The cloud fraction at cloud base, in particular, has been identified as a key parameter for the spread of modelled feedback of these clouds to climate change. Therefore, understanding the processes controlling the variability of cloudiness at cloud base is of utmost importance. Stable water vapour isotopes reflect the integral of moist atmospheric processes encountered by the vapour since evaporation from the ocean surface. This study focuses on stable water isotopes variability from aircraft observations with the French ATR research aircraft and high-resolution isotope-enabled simulations in the winter trades near Barbados at cloud base. Nested convection resolving COSMOiso simulations at 10, 5 and 1 km grid spacing during the EUREC4A field experiment period are used, which have been thoroughly evaluated using observations from different platforms. The three main findings are: (i) contrasting isotope and humidity characteristics in clear-sky versus cloudy cloud base environments emerge due to vertical transport on time scales of 12 hours, which (ii) are associated with local, convective circulations, and show a clear diel cycle; (iii) the cloud base isotope signals are, in addition, sensitive to variations in the large-scale circulation on time scales of several days, which shows on average a Hadley-type subsidence but occasionally much stronger descent related to extratropical dry intrusions. This investigation, based on stable water isotopes in high-resolution simulations in combination with trajectory analyses reveals, in a physically plausible way, how dynamical processes at different scales act in concert to produce the observed humidity variations at the cloud base of trade wind cumuli.

How to cite: Aemisegger, F. and Villiger, L.: A process-oriented model evaluation using EURECA water isotope field observations in the North Atlantic trades reveals the imprint of the atmospheric circulation at different scales, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12083, https://doi.org/10.5194/egusphere-egu23-12083, 2023.

EGU23-12634 | Orals | AS1.21

Early Holocene Laurentide Ice Sheet retreat influenced summer atmospheric circulation in the North American Arctic: Evidence from precipitation isotope and temperature proxy records and a climate model 

Elizabeth Thomas, Allison Cluett, Michael Erb, Nicholas McKay, Jason Briner, Isla Castañeda, Megan Corcoran, Owen Cowling, Devon Gorbey, Kurt Lindberg, and Jeffrey Salacup

Changes in ice sheet size and configuration impact global moisture and heat transport, but few proxy records examine these impacts. High-latitude precipitation-isotope proxy records are often interpreted to reflect temperature change, but can also reflect changes in moisture source. We present independent sub-centennial-scale records of summer temperature and summer precipitation δ2H from the same lake sediment archive on northeastern Baffin Island. We also examine published TraCE-21k transient model simulation results. These records span from 12 to 7 ka, when the Laurentide Ice Sheet underwent major retreat. The correlation structure between summer temperature and precipitation δ2H on northeastern Baffin Island changed from negative to positive around 10 ka. We interpret this change in correlation structure to indicate a shift in moisture sources to northeastern Baffin Island. TraCE-21k results suggest that moisture sources in this region are controlled by the relative strength of the high pressure systems and associated anticyclonic circulation over the Greenland and Laurentide ice sheets. We therefore interpret the proxy records as follows: when the Laurentide high dominated prior to 10 ka, northerly winds brought cold, dry Arctic air to the region, allowing 2H-enriched local sea breezes to provide most of the moisture to Baffin Island. After 10 ka, the Greenland high dominated, causing southerly flow to carry warm, moist, 2H-depleted air masses to northeastern Baffin Island. Regional centennial-scale cooling events caused by periodic freshwater inputs to the Labrador Sea throughout the Early Holocene were also associated with intervals of 2H-enriched summer precipitation. This study provides evidence that atmospheric circulation was influenced by the waning continental ice sheets. Similar ice-sheet influences are critical to consider when interpreting precipitation isotope proxy records spanning periods of dramatic ice-sheet change. These results demonstrate that precipitation isotopes can reflect changes in atmospheric circulation in the geologic record.

How to cite: Thomas, E., Cluett, A., Erb, M., McKay, N., Briner, J., Castañeda, I., Corcoran, M., Cowling, O., Gorbey, D., Lindberg, K., and Salacup, J.: Early Holocene Laurentide Ice Sheet retreat influenced summer atmospheric circulation in the North American Arctic: Evidence from precipitation isotope and temperature proxy records and a climate model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12634, https://doi.org/10.5194/egusphere-egu23-12634, 2023.

EGU23-12841 | ECS | Posters on site | AS1.21

Precipitation origin in atmospheric rivers from a global perspective: first steps 

Alfredo Crespo-Otero, Damián Insua-Costa, and Gonzalo Míguez-Macho

Atmospheric rivers (ARs) are filaments of enhanced moisture in the atmosphere, usually located in subtropical zones and mid-latitudes over oceanic areas. These structures are able to transport huge water vapor amounts, so that when they make landfall and the water vapor is forced upwards, they often cause heavy or even extreme rainfall, thus increasing the odds of catastrophic flooding. Given their potential effects on our daily lives, a better understanding of their physical properties is therefore needed. 

One of the most studied and debated ARs properties in recent years is the origin of the moisture in them. Despite the numerous scholars dealing with this topic, moisture sources for precipitation in ARs have not yet been investigated from a global and climatological perspective.  Here we present a first attempt to fill this gap by selecting different ARs events across the globe and subsequently simulating them with the FLEXPART model, enabled to calculate Lagrangian trajectories of individual air particles. In addition, we use state-of-the-art techniques to process and bias-correct FLEXPART outputs in other to accurately estimate precipitation origins. Our preliminary results reveal that ARs can tap from multiple moisture sources and that the contributions of the latter vary widely from case to case. Therefore, we conclude that moisture uptake in ARs is more complex and varied than previously known.  

How to cite: Crespo-Otero, A., Insua-Costa, D., and Míguez-Macho, G.: Precipitation origin in atmospheric rivers from a global perspective: first steps, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12841, https://doi.org/10.5194/egusphere-egu23-12841, 2023.

EGU23-13348 | ECS | Orals | AS1.21

Investigating diurnal ecosystem scale H2O and CO2 isotope fluxes in an irrigated semi-arid environment during the LIAISE 2021 field campaign 

Robbert Moonen, Getachew Adnew, Oscar Hartogensis, Jordi Vila-Guerau de Arellano, and Thomas Röckmann

Validation of gas exchange fluxes in models has been challenging due to the lack of ecosystem scale exchange fluxes partitioned into soil, plant and atmospheric components. One promising method to partition turbulent fluxes uses the exchange process dependent fractionation of molecules like CO2 and H2O. When applying this method to short spatiotemporal scales, an isotope flux (δ-flux) needs to be resolved. Few have attempted to measure this δ-flux as the required instrumentation only became available in recent years. In our presentation we will discuss observations made during the LIAISE 2021 field campaign using an EC system, Picarro L-2130i H2O isotope analyser, and Aerodyne TILDAS-CS CO2 isotope analyser. This campaign took place in the summer of 2021 in the heavily irrigated Ebro River basin near Lleida, Spain embedded in a semi-arid region.

We will present procedures to estimate and scrutinize the central δ-flux variable. To this end we calculated co-spectra of the relevant signals and compared their frequency dependent contributions. One relevant finding is that mole fractions and isotope ratios measured with the same instrument can be offset in time by more than a minute, thereby impacting the resulting δ-fluxes. Additionally, we found asymmetric signal loss between net ecosystem fluxes and δ-fluxes. We will show that such effects impact flux partitioning severely and indicate how they can be tackled using physically sound corrections. Only when such corrections and verifications are made, ecosystem flux partitioning can be applied to validate conceptual land-atmosphere exchange models. Such models will calculate the diurnal variability of CO2 and H2O isotopologue concentrations, and link local to regional scales, all with the purpose of better constraining current and future exchange fluxes. 

How to cite: Moonen, R., Adnew, G., Hartogensis, O., Vila-Guerau de Arellano, J., and Röckmann, T.: Investigating diurnal ecosystem scale H2O and CO2 isotope fluxes in an irrigated semi-arid environment during the LIAISE 2021 field campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13348, https://doi.org/10.5194/egusphere-egu23-13348, 2023.

EGU23-13629 | ECS | Posters on site | AS1.21

A new theoretical framework for parameterizing nonequilibrium fractionation during evaporation from the ocean 

Marina Duetsch, Christopher W. Fairall, Peter N. Blossey, and Richard P. Fiorella

The evaporation isotope model proposed by Craig and Gordon (1965) is used in most atmospheric isotope models for the parameterization of fractionation during evaporation from the ocean. It describes the isotope ratios in the evaporation flux as a function of the isotope ratios in liquid water and the atmosphere, relative humidity, the equilibrium fractionation factor, and the nonequilibrium fractionation factor (kiso). Of these parameters, kiso is the most uncertain. Many isotope models use the formulation of Merlivat and Jouzel (1979), which parameterizes kiso as a function of wind speed and distinguishes between a smooth and a rough regime to account for the fact that waves act as roughness elements, inducing perturbations that significantly influence gas transfer rates. The resulting discontinuity in kiso and therefore isotope ratios, which usually occurs at around 7m/s wind speed, has been disputed by several empirical studies, based on measurements of deuterium excess and 17O-excess in the near-surface boundary layer. However, a theoretical framework, which would be in line with the measurements, is still lacking. Here, we present a new approach to parameterizing kiso by explicitly accounting for the influence of wave drag on the momentum flux near the surface. Following recent work by Cifuentes-Lorenzen et al. (2018), we add a third wave-induced component to the total momentum flux, in addition to the viscous and turbulent components, and extend the definition of the eddy viscosity to account for the loss of friction velocity due to ocean waves and the fall-off of turbulence close to the surface. The new scheme predicts a slight decrease of kiso with wind speed, similar to the values from Merlivat and Jouzel (1979) if the smooth-regime parameterization were used at all wind speeds. In a second step, we incorporate the new parameterization into the isotope-enabled Community Earth System Model, and run nudged simulations for the years 2000-2020, to analyze the effect on vapor and precipitation isotopes. While δD and δ18O remain nearly unaffected, the deuterium excess tends to be higher in the simulation with the new scheme than in the control simulation, especially in regions with high wind speeds.

 

References

Cifuentes-Lorenzen, A., Edson, J. B., and Zappa, C. J. (2018). Air–sea interaction in the southern ocean: Exploring the height of the wave boundary layer at the air–sea interface. Bound.-Layer Meteorol., 169(3), 461-482.

Craig, H. and Gordon, L. I. (1965). Deuterium and oxygen 18 variations in the ocean and the marine atmosphere. In Stable Isotopes in Oceanographic Studies and Paleo-Temperatures, pp. 9–130. Lab. Geol. Nucl., Pisa, Italy.

Merlivat, L. and Jouzel, J. (1979). Global climatic interpretation of the deuterium-oxygen 18 relationship for precipitation. J. Geophys. Res., 84(C8):5029–5033.

How to cite: Duetsch, M., Fairall, C. W., Blossey, P. N., and Fiorella, R. P.: A new theoretical framework for parameterizing nonequilibrium fractionation during evaporation from the ocean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13629, https://doi.org/10.5194/egusphere-egu23-13629, 2023.

A continuous bi-weekly water isotope analysis (δ18O, δD, and d-excess) was done since 2015 from a subtropical reservoir (Feitsui Reservoir) in northern Taiwan. The Feitsui reservoir is an important national freshwater system, as it provides water for the large urban population of Taipei. The isotopic data reveals a multiyear pattern and it closely follows the rainfall isotopic composition. We made a simple mass-balance model using the rainfall isotopic composition, inflow and outflow volumes, and meteorological parameters that fit well (R2 = 0.55; p-value < 0.05) with the observed isotopic composition of the reservoir. Based on this model, we estimated reservoir isotopic composition for the previous 20 years (2001-2021). The model also well reproduced a few years of historical data reported in the literature. In the model, we noted two conspicuous patterns: (1) multiyear cyclicity in δ18O and d-excess, and (2) a long-term enriching trend in δ18O. These patterns were not so obvious in rainfall because of the strong seasonality, which gets diluted in the reservoir because of the longer water residence time (~6 months). However, these patterns became visible in rainfall isotopes after removing the seasonal cycles. The observed multiyear patterns do not resemble with the known multiyear global processes, such as ENSO, PDO, and the East Asian Monsoon Index. However, the role of these global processes cannot be ruled out completely. We believe that because of the unique geographical location of the island, multiple moisture sources (South China Sea and central/northern China), dual monsoons (summer and winter monsoons), and complex hydrometeorological processes, the signals of these multiyear global processes get modulated and modified. The long-term enriching trend in δ18O seems to be a consequence of climate change. The enriching trend is more vivid during the winters than summers. This indicates the possible role of global warming and the expansion of the tropics because the Tropics of Cancer passes through central Taiwan. There also remains a significant knowledge gap in understanding the role of winter monsoons in East Asia. This study highlights the importance and the need for rigorous climatic research in Taiwan because of its unique location which makes it highly sensitive to climate change. This study may also have implications for paleoclimatic studies because it highlights the complex hydrometeorology of the region.

How to cite: Oza, H., Wang, C.-H., and Liang, M.-C.: Enigmatic Multi-Year Oscillations in Water Isotopic Composition of East Asia: Insights from a Subtropical Reservoir, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13842, https://doi.org/10.5194/egusphere-egu23-13842, 2023.

EGU23-14175 | ECS | Posters on site | AS1.21

Stable water vapour isotopes as integrated tracers of moisture sources, transport and deposition during warm air intrusions in the Arctic 

Camilla F. Brunello, Florian Gebhardt, Annette Rinke, Hanno Meyer, Moein Mellat, Silvia Bucci, Marina Dütsch, Ben G. Kopec, Jeffery M. Welker, and Martin Werner

Air-mass intrusions arriving from the mid-latitudes introduce moisture and heat into the Arctic and perturb cloud properties. These events have a strong impact on the water cycle as their frequency and intensity control the inter-annual variability of mean surface air temperature, humidity and energy budget. Warm air intrusions are all short-lived events related to blocking situations of the large-scale circulation, however, the characteristics of each individual air intrusion depend on the season, the sourcing of the air masses, the characteristics of the boundary layer and the surface conditions during the long-range transport.

In this study, we use atmospheric water vapour isotopes (H216O, H218O, HD16O) to trace the origin of the moisture and to gain insights into the exchange processes occurring during four distinct warm air intrusion events, recorded during a one-year expedition in the Central Arctic. Stable water isotopes can track feedback loops and exchange processes between the hydrological compartments of the Arctic, because evaporative sources, phase changes and interactions within hydrological compartments all have specific imprints on the isotopic compositions. Continuous observations of near-surface atmospheric vapour were obtained onboard RV Polarstern during the MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) drifting expedition in 2019-2020. By combining a moisture source diagnostic to the particle dispersion model FLEXPART, we constrain the magnitude and the location of the surface moisture uptake into the air masses.

We found that the moisture transported during the events originated from different locations, namely lower North Atlantic sector (<70°N), upper North Atlantic (>70°N), continental Siberia and sea-ice. The different evaporative conditions over these regions are key to determine the distinct isotopic signature of the sampled air masses. Further, we observe opposite sensitivity of d-excess to local temperature and humidity in the moisture sourced from the sea-ice. D-excess is a second order isotope parameter interpreted as a diagnostic of non-equilibrium fractionation. We further investigate the mechanisms leading to non-equilibrium phase changes and we examine the roles of: (i) mixed-phase cloud formation where water vapour is supersaturated with respect to ice, (ii) evaporation from leads and melt ponds, and (iii) changes in vapour isotopes with respect to snow on sea ice during sublimation/deposition regimes.

With this work we aim at better understanding the transport of mid-latitudes moisture into the Central Arctic region and identifying the moisture exchange processes with the Arctic cryosphere. In view of the projected increase of frequency and duration of warm air intrusions in the Arctic, our study contributes to understanding the mechanistic consequences of such short-lived events on the whole Arctic water cycle. 

How to cite: Brunello, C. F., Gebhardt, F., Rinke, A., Meyer, H., Mellat, M., Bucci, S., Dütsch, M., Kopec, B. G., Welker, J. M., and Werner, M.: Stable water vapour isotopes as integrated tracers of moisture sources, transport and deposition during warm air intrusions in the Arctic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14175, https://doi.org/10.5194/egusphere-egu23-14175, 2023.

EGU23-14988 | Orals | AS1.21

Identifying the convective and stratiform rainfall regimes using stable isotopic measurement 

Pramit Kumar Deb Burman, Supriyo Chakraborty, Amey Datye, Abida Choudhury, Milind Mujumdar, Pm Mohan, Nirmali Gogoi, Rajendra Trivedi, Dipankar Sarma, Abhijit Bora, and Neha Trivedi

It still remains an intriguing question in weather and climate research on identifying the convective rainfall from stratiform. In a future warmer climate, this will be important to know to predict the changing pattern of rain intensity and distribution and to plan an efficient usage of water resources. Although quite a few methods have been proposed to address this question, such as cloud top temperature value, height-integrated ice and cloud water paths, brightness temperature, drop size distribution etc., the fidelity and validity of those vary widely, and hence their applicability remains limited. In this work, we propose a method to identify these two rainfall regimes using a combination of surface and remote sensing measurements. We collected the rainwater samples daily at Port Blair, Sagar and Tezpur in India as part of a project CRP F31006, funded by the International Atomic Energy Agency (IAEA). We measured the 18O content in these collected rainwater samples by measuring its fractionation (δ18O) using a Triple Isotope Water Analyzer by Los Gatos Research, USA. Among these sites, Port Blair is an island on the Bay of Bengal near the tropics, Sagar is an inland location in central India's dry, arid climate and Tezpur is located in the wet and heavily forested northeast India. Whereas Port Blair is situated very close to the tropics, Sagar and Tezpur are closer to the subtropics. The dual-frequency precipitation radar in the global precipitation measurement (GPM) program provides the convective and stratiform rainfall records by looking at radar reflectivities. We utilize these records to estimate the area-averaged stratiform rainfall fraction over each of these locations. We find that the relation between rain intensity and stratiform rainfall fraction can be represented by a logarithmic regression, whereas, the relation between δ18O and rain intensity can be represented by linear regression. However, the logarithmic regression weakens with latitude, and, the slope of the linear relation changes from slightly negative to slightly positive. The three sites considered here are located under different environmental conditions (oceanic to continental, semi-arid to forest, southwest to northeast monsoon zones, etc.) and house different vegetation types. To better understand the underlying processes governing such relations, we also study the impact of different meteorological variables in regulating these relations. Based on our study, the δ18O can be used as a proxy to identify the relative contributions of convective and stratiform rain types in the total rainfall over a region.

How to cite: Deb Burman, P. K., Chakraborty, S., Datye, A., Choudhury, A., Mujumdar, M., Mohan, P., Gogoi, N., Trivedi, R., Sarma, D., Bora, A., and Trivedi, N.: Identifying the convective and stratiform rainfall regimes using stable isotopic measurement, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14988, https://doi.org/10.5194/egusphere-egu23-14988, 2023.

The sensitivity of coarse-grained daily extreme precipitation to sea surface temperature is analyzed using satellite precipitation estimates over the 300–302.5 K range. A theoretical scaling is proposed, linking changes in coarse-grained precipitation to changes in fine-scale hourly precipitation area fraction and changes in conditional fine-scale precipitation rates. The analysis reveals that the extreme coarse-grained precipitation scaling with temperature (∼7%/K) is dominated by the fine-scale precipitating fraction scaling (∼6.5%/K) when using a 3 mm/h fine-scale threshold to delineate the precipitating fraction. These results are shown to be robust to the selection of the precipitation product and to the percentile used to characterize the extreme. This new coarse-grained scaling is further related to the well-known scaling for fine-scale precipitation extremes, and suggests a compensation between thermodynamic and dynamic contributions or that both contributions are small with respect to that of fractional coverage. These results suggest that processes responsible for the changes in fractional coverage are to be accounted for to assess the sensitivity of coarse-grained extreme daily precipitation to surface temperature.

How to cite: Muller, C., Roca, R., and De Meyer, V.: Precipitating Fraction, Not Intensity, Explains Extreme Coarse-Grained Precipitation Clausius-Clapeyron Scaling With Sea Surface Temperature Over Tropical Oceans, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16367, https://doi.org/10.5194/egusphere-egu23-16367, 2023.

EGU23-17506 | ECS | Posters on site | AS1.21

Moisture source changes of precipitation in Europe under SSP1-2.6 and SSP3-7.0 warming 

Janina Tschirschwitz, Martin Werner, Qinggang Gao, Louise Sime, and Camilla F. Brunello

When global temperature increases, the atmosphere will be able to hold more water,
as described by the Clausius-Clapeyron equation. It is thus hypothesised that the global
water cycle will intensify under a warming climate. This might lead to more intense and more
frequent extreme precipitation events and might also affect the atmospheric circulation.
This project investigates how moisture sources of precipitation over the European
continent will change under SSP1-2.6 and SSP3-7.0 warming, using the atmospheric
general circulation model ECHAM6-wiso. A present day simulation (1990-2020), nudged to
ERA5 reanalysis, and a future simulation for each investigated SSP (2070-2099), nudged to
respective CMIP6 coupled model output, are conducted. Using numerical water tracers, the
model is able to trace precipitation back to its point of evaporation, characterised by latitude
and longitude.
Our results suggest that, under warming, the source latitude and longitude of
precipitation in Europe will change across all seasons. The magnitude of change depends
on the strength of the warming. These changes in source latitude and longitude reflect
changes in the mid-latitude wind patterns and atmospheric circulation.

How to cite: Tschirschwitz, J., Werner, M., Gao, Q., Sime, L., and Brunello, C. F.: Moisture source changes of precipitation in Europe under SSP1-2.6 and SSP3-7.0 warming, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17506, https://doi.org/10.5194/egusphere-egu23-17506, 2023.

EGU23-469 | ECS | PICO | HS7.9 | Highlight

Revegetation impacts on moisture recycling over Loess Plateau in China 

Mingzhu Cao, Weiguang Wang, Lan Wang-Erlandsson, and Ingo Fetzer

Moisture recycling of local water sources through evaporation allows a region to maintain precipitation in the same region. Many studies have shown that deforestation can reduce evaporation and downwind rainfall, and it has been suggested that reforestation conversely increase evaporation and downwind rainfall. Precipitation has been observed to increase over China’s Loess Plateau over the past two decades, coinciding with the start of the Grain for Green project - the largest active revegetation programme attempted in the world. However, the contribution of revegetation to the increase in precipitation is yet unknown. Here, we aim to quantitatively analyze the relationship between revegetation, evaporation, and locally recycled moisture. Based on the ERA5 reanalysis data, we used the modified Water Accounting model-2 layers (WAM-2layers) to track the recycling moisture over the Loess Plateau. Preliminary results indicate that local recycling moisture (Er) accounted for almost one-tenth of the annual precipitation, and seems to have a decreasing trend, which was more evident after 2000. Meanwhile, the contribution of local evaporation to local precipitation appears to decrease during both 1982-1999 and 2000-2015, while the decreasing trend has been slightly amplified after the revegetation. Spatially, Er over the Loess Plateau showed a decreasing trend from southeast to northwest. Significant increasing trend of Er can be identified in the northern part of the plateau during 1982-1999. However, after the implement of the Green for Grain Project, most area over the Loess Plateau showed a decreasing trend, which is significant in the east. Thus, contrary to popular wisdom, the revegetation appears to have led to a decrease in evaporation and subsequent recycling, and the increase in precipitation seems to have other causes. These results are subject to high data uncertainty, and further research is needed to better understand the hydroclimatic effects of revegetation projects under climate change.

How to cite: Cao, M., Wang, W., Wang-Erlandsson, L., and Fetzer, I.: Revegetation impacts on moisture recycling over Loess Plateau in China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-469, https://doi.org/10.5194/egusphere-egu23-469, 2023.

EGU23-965 | ECS | PICO | HS7.9

Ecohydrological dynamics in the Central American and Andean Páramo: Insights from a modelling analysis using a Budyko-type model for non-stationary conditions 

Germain Esquivel-Hernández, Ricardo Sánchez-Murillo, Giovanny M. Mosquera, Patricio Crespo, Rolando Célleri, Juan Pesantez, Braulio Lahuatte, and Enzo Vargas-Salazar

The Páramo is a high‐elevation tropical grassland ecosystem that plays an important role in the regional water cycle of Central America and the northern Andes. However, refined information about the ecohydrological partitioning in these mountainous biomes is scarce. This work aimed to assess sub-annual or monthly variations in the ecohydrological conditions along a N-S transect with three Páramo sites: Chirripó (Costa Rica) and El Carmen and Cajas (north and south Ecuador, respectively). A Budyko-type model for conditions under which evapotranspiration surpasses precipitation using monthly meteorological observations and evapotranspiration products (May 2016-April 2019) was applied to evaluate short-term ecohydrological dynamics based on the aridity index and precipitation partitioning in the Páramo sites. Stronger hydroclimatic variations were found in Chirripó than in the Andean Páramos, related with significant increments in the evaporative index (AET/P) during the dry season. We also found a clear separation between Chirripó and the Ecuadorian Páramos owing to a higher ecohydrological resilience (i.e., similar trajectories in the energy excess or 1- AET/PET and the water excess or Q/P) in Chirripó during dry season and a more effective regulation by the additional water available to evapotranspiration besides direct precipitation (y0, range: 37 – 90 %). Our results reveal the complex ecohydrological functional properties of the Páramo and its sensitivity to future moisture changes (e.g., ENSO cycles) that could alter its water yield synchronicity. 

How to cite: Esquivel-Hernández, G., Sánchez-Murillo, R., Mosquera, G. M., Crespo, P., Célleri, R., Pesantez, J., Lahuatte, B., and Vargas-Salazar, E.: Ecohydrological dynamics in the Central American and Andean Páramo: Insights from a modelling analysis using a Budyko-type model for non-stationary conditions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-965, https://doi.org/10.5194/egusphere-egu23-965, 2023.

EGU23-1031 | ECS | PICO | HS7.9

Spatial and temporal patterns and influencing factors of carbon and water cycles in different permafrost types on the Qinghai-Tibet Plateau 

Xiang Wang, Guo Chen, Qi Wu, Longxi Cao, Joseph Awange, and Mingquan Wu

Understanding changes in water use efficiency (WUE) and its drivers in terrestrial ecosystems on the Qinghai-Tibet Plateau is important to reveal the response of carbon and water cycle to climate change in the area sensitive to the environment. However, the patterns of carbon and water cycles in different frozen soil zones in this area are not well understood to our knowledge. This study explores the spatial and temporal patterns of WUE, gross primary production (GPP), and evapotranspiration (ET) from 2001 to 2020 at six frozen soil zones (short-time frozen ground; thin seasonally frozen ground; middle-thick seasonally frozen ground; mountain permafrost; predominantly continuous and island permafrost; predominantly continuous permafrost) on the Qinghai-Tibet Plateau with different degrees of freezing based on remote sensing data. The climatic, edaphic, and botanic parameters influencing these patterns were then investigated. The results show that: (1) the WUE, GPP, and ET all generally increased from 2001-2020 for each type of frozen soil ecosystem although the significance and the slope of the trends differed, (2) the WUE and GPP gradually decreased as the degree of freezing increased, while ET first increased and then decreased with the freezing gradient, and (3) enhanced vegetation index was the first important variable influencing WUE for all types of frozen soil regions except for the area of short-time frozen ground. Our results highlight that the freezing degree of soil could influence the evaluation of the water-carbon cycle on the Qinghai-Tibet Plateau.

How to cite: Wang, X., Chen, G., Wu, Q., Cao, L., Awange, J., and Wu, M.: Spatial and temporal patterns and influencing factors of carbon and water cycles in different permafrost types on the Qinghai-Tibet Plateau, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1031, https://doi.org/10.5194/egusphere-egu23-1031, 2023.

Water is crucial for human health, food and industrial production, ecosystem services, and climate and weather systems. As a major contributor of renewable freshwater over land, humans have been studying the origin of continental precipitation for nearly a century. From the moisture budget perspective, local evapotranspiration in a vast part of the Earth’s surface is effectively smaller than local precipitation. This entails the role of moisture advection in sustaining continental precipitation. However, previous trajectory-based quantification appeared to underestimate the global “continental precipitation recycling (CPR)” ratio –– that is, the fraction of continental precipitation originating from evapotranspiration. To this end, the present study completed a 40-year (1971-2010) tracking of moisture from continental precipitation using a three-dimensional Lagrangian tracking model and optimized water accounting diagnostics. Our Lagrangian tracking confirms that 62% of continental precipitation stems from evapotranspiration, aligning well with the water budget-based estimates in the literature. Across the globe, non-local terrestrial sources dominate 1˚-scale precipitation in nearly 70% of the land areas, together with the greatest continental moisture feedback in the interior of South America, Africa and Eurasia. Seasonally, the CPR ratio anomalies are markedly different between the mid-to-high latitudes and monsoon regions worldwide, from which two kinds of moisture source-regulated hydroclimate are generalized. For transboundary water governance, perennial source hotspots for continental precipitation are identified, including the biome-rich Amazon and Congo rainforests and other major watersheds within 30˚ equatorward. Leveraging the backward “WaterSip” and the forward “WaterDrip” algorithms, we propose two ubiquitous processes of cascading moisture recycling (CMR) that formulate a cascade of regional water cycles. The watershed-scale CMR metrics quantify the hidden interdependence between the regional water cycles through moisture recycling. Overall, by closing the gap in the estimate of the CPR ratio, this work updates the understanding of the moisture recycling, feedback and cascading characteristics of the continental atmospheric water cycle. The outcome sheds light on the potential vulnerability of local precipitation in response to the modification of non-local land surface fluxes by human activities.

How to cite: Cheng, T. F. and Lu, M.: Updated Understanding of Continental Precipitation Recycling Using Global 3-D Lagrangian Tracking, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1887, https://doi.org/10.5194/egusphere-egu23-1887, 2023.

EGU23-2768 | ECS | PICO | HS7.9

Hydrological response to anthropogenic activities and climate change in the southern Caspian Sea, Iran 

Alireza Sharifi Garmdareh, Ali Torabi Haghighi, and Ritesh Patro

Rivers play a vital role in supplying fresh water for various sectors. During the last decades, increasing anthropogenic activities and climate change have altered river flow regimes around the globe. Rivers flow in the southern Caspian Sea in Iran has altered due to water-intensive socio-economic development and climate change. To assess and quantify the impact of anthropogenic activities and climate change on river flow regimes, the elasticity-based methods and the Budyko hypothesis were applied to 40 rivers on the closest gauges to the Caspian Sea were selected. Furthermore, to evaluate spatial/temporal change in hydrometeorological variables, two non-parametric methods, including the modified Mann-Kendall method (MK3) and Innovative Trend Analysis (ITA), were applied. The results showed an alarming trend of increasing temperature and potential evapotranspiration and decreasing rivers’ flow in the southern Caspian sea. Assessing and quantifying the impact of anthropogenic activities and climate change on river flow alteration indicated that anthropogenic activities (accounting for 83.3%) played a dominant role in river flow alteration that led to inflow to the Caspian Sea decline by about 2,412 MCM annually. In addition, the inflow to the Sea has decreased by about 551 MCM every year due to the impact of climate change. Decreasing the inflow to the Caspian Sea can accelerate the declining trend of the Sea level, which leads to boosts eutrophication conditions in the Sea, and negatively affect the ecosystem and economics of the Caspian Sea. Therefore, an appropriate adoption approach must be taken into account to alleviate the environmental and socio-economic issues in the southern Caspian Sea.

How to cite: Sharifi Garmdareh, A., Torabi Haghighi, A., and Patro, R.: Hydrological response to anthropogenic activities and climate change in the southern Caspian Sea, Iran, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2768, https://doi.org/10.5194/egusphere-egu23-2768, 2023.

Irrigation practice has impacts on the natural environment by changing the water and energy balance at the land surface and thereby interacting with the atmosphere. To quantify such impacts and estimate irrigation water demand, process-based hydrological models with a representation of irrigation practice are often used. However, the applicability of existing irrigation schemes is limited to arid and semi-arid regions. Likewise, it is still lack of more sophisticated irrigation schemes that can be particularly applicable to humid regions. This study presents the newly developed Crop-classified Dynamic Irrigation (CDI) scheme that has been two-way coupled into the land surface-hydrologic model Noah-HMS. Such development allows to distinguish the different irrigation practices for "rice" and "non-rice" crops and to estimate irrigation water demand. We have applied the newly developed model to an important grain and industrial crop production base in southern China, namely, Poyang Lake Basin (PLB), where the sown area of rice accounts for more than 60% of the sown area of all crops. As compared to the widely used, traditional Dynamic Irrigation (DI) scheme, the CDI-incorporated Noah-HMS improves the simulations of water and energy balance over the PLB from 2007 to 2015, especially irrigation water amount simulation. The relative error for irrigation water amount of CDI (DI) is -18.1% (-56.8%). In terms of surface water balance, the inclusion of irrigation practice has larger impacts on the simulated soil moisture (+1.7%) during dry years than that (+0.9%) during wet years, while has larger impacts on the simulated surface runoff (4.6%) in wet years than that (2.4%) in dry years. In terms of surface energy balance, irrigation practice leads to increased latent heat flux by 0.9 W/m2 (1.4%), decreased sensible heat flux by 0.5 W/m2 (1.3%), decreased ground heat flux by 0.02W/m2 (5.0%), and increased net radiation by 0.09 W/m2 (0.1%). Such impacts on the surface water and energy balance become more pronouncing at local scale especially over the intensively irrigated areas, for example the Nanchang city region. We conclude that our Crop-classified Dynamic Irrigation scheme is especially beneficial for applications in multiple cropping humid regions. Furthermore, our modeling development has the potential to be further extended into the fully coupled atmospheric-hydrologic modeling systems with a more holistic representation of human activities.

How to cite: Yang, Q., Wei, J., Yang, C., and Yu, Z.: Impacts of Farmland Irrigation on Land Surface Water and Energy Balance over a Humid Region: Development and Benefits of a Crop-Classified Dynamic Irrigation Scheme in Noah-HMS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4290, https://doi.org/10.5194/egusphere-egu23-4290, 2023.

EGU23-5016 | PICO | HS7.9 | Highlight

Moisture Recycling in the Amazon: a study using WRF with water vapor tracers 

Francina Domínguez and Jorge Eiras-Barca

This work analyzes the sources, sinks and stores of moisture that originates as Amazonian evapotranspiration (ET) from daily to annual timescales. To do this, we use the Weather Research and Forecast (WRF) regional meteorological model with the added capability of water vapor tracers to track the local evapotranspired moisture. The tracers reveal a strong diurnal cycle of Amazonian water vapor which had not been previously reported. This signal is related to the diurnal cycle of ET, convective precipitation and advected moisture. ET's contribution to atmospheric moisture increases from early morning into the afternoon. Some of this moisture is rained out through convective storms in the early evening. Later in the night and following morning, strong winds associated with the South American Low Level Jet advect moisture downwind. The beating pattern becomes apparent when visualizing the Amazonian water vapor as an animation.

How to cite: Domínguez, F. and Eiras-Barca, J.: Moisture Recycling in the Amazon: a study using WRF with water vapor tracers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5016, https://doi.org/10.5194/egusphere-egu23-5016, 2023.

EGU23-6508 | PICO | HS7.9 | Highlight

Assessing the impact of large-scale afforestation on the atmospheric water cycle of the Loess Plateau in China 

Lei Tian, Shuoyu Chen, Baoqing Zhang, and Baotian Pan

Afforestation has been regarded as an appropriate way to mitigate climate change and enhance ecosystem services. How afforestation affects the availability of water resources is a hot topic in the science community. Most current studies investigate the impact of afforestation on water resources through offline modeling or observation on a small spatial scale. However, the atmospheric water cycle (AWC) is also an important aspect that can alter the availability of water resources, especially on a large spatial scale. With an investment of about US$54.57 billion, the Chinese government implemented the world’s largest afforestation project, the Grain for Green Program (GFGP), to curb the severe soil erosion over the Loess Plateau (LP) since 1999. Here we focused on this ideal platform, the LP, to explore the impact of large-scale afforestation on the processes related to the atmospheric water cycle. We adopted two different approaches to discern the hydroclimatic effect of the GFGP. This first approach used the reanalysis dataset to compare the hydroclimatic states before (1982–1998) and after (1999–2018) the GFGP. Since the reanalysis dataset cannot separate the impact of climate change and afforestation, this study also applied a regional climate model (the Weather Research & Forecasting Model, WRF) to isolate the net hydroclimatic effect of the GFGP by controlled experiments. In particular, the WRF model was driven by two land surface conditions with/without the implementation of the GFGP. We found both approaches reached similar conclusions. Results show the vegetation coverage fraction over the LP increased by 3.15% decade−1 induced by the GFGP. The climatological precipitation and evapotranspiration (ET) increased by 54.62 and 22.56 mm, respectively, after starting the GFGP in 1999. The large-scale afforestation intensifies the atmospheric water cycle over the LP. In addition, based on the dynamic precipitation recycling model, we also found the precipitation recycling ratio approximately increased by 1%. The GFGP alters the regional circulation by influencing diabatic heating, and moisture convergence, resulting in more moisture being advected from the south boundary, thus more atmospheric moisture was retained in the LP. Additionally, the internal branch of the AWC contributes to about 15% of the increased precipitation, while the contribution of the external branch is about 85%. Moreover, the GFGP remotely affects the water vapor budget in the downwind areas. Our work enriched the current understanding of how afforestation affects the water cycle from a precipitation recycling perspective and can help policy-makers to make science-informed afforestation strategies.

How to cite: Tian, L., Chen, S., Zhang, B., and Pan, B.: Assessing the impact of large-scale afforestation on the atmospheric water cycle of the Loess Plateau in China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6508, https://doi.org/10.5194/egusphere-egu23-6508, 2023.

EGU23-6883 | ECS | PICO | HS7.9 | Highlight

Local moisture recycling across the globe 

Jolanda Theeuwen, Arie Staal, Obbe Tuinenburg, Bert Hamelers, and Stefan Dekker

Atmospheric moisture recycling describes how moisture evaporated from land precipitates over land. It explains how shifts in terrestrial evaporation due to land cover changes may affect precipitation and freshwater availability across scales. Recycling at regional and continental scales has been studied using different methods, such as offline and online moisture tracking models and bulk recycling models. Although recycling at regional and continental scales is relatively well understood, it has only recently become possible to study local moisture recycling across the globe. Recent developments in offline moisture tracking resulted in a dataset including a 10-year climatology (2008-2017) of atmospheric moisture connections from evaporation source to precipitation sink at a spatial scale of 0.5° (Tuinenburg et al., 2020). We used this data to calculate the local moisture recycling ratio, which we define as the fraction of evaporated moisture that precipitates within a distance of 0.5° (typically 50 km) from its source. Furthermore, we identify variables that correlate with the local moisture recycling ratio to assess its underlying processes. On average, 1.7% (st. dev. = 1.1%) of terrestrial evaporated moisture returns as local precipitation annually. However, there is large spatial and temporal variability with peak values over mountainous and wet regions and in summer. Wetness (i.e., precipitation and precipitation minus evaporation), orography, latitude, convective available potential energy, wind speed and total cloud cover have moderate to strong correlations with the local moisture recycling ratio. Interestingly, we find peaks in the local moisture recycling ratio at latitudes where air ascends due to the Hadley cell circulation (i.e., at 0° and 60°). These results suggest that wet regions characterized by ascending air and low wind speeds are favourable for high local moisture recycling ratios. This knowledge can be used to strategically recycle water using nature-based solutions or irrigation to minimize the usage of freshwater availability. For example, for the tropics and mountainous regions globally, and for the Mediterranean regions on the Northern Hemisphere, an increase in evaporation through for example, regreening has a relatively large contribution to local precipitation due to the relatively large local moisture recycling ratios here. These results suggest the potential to enhance freshwater availability with land cover changes, e.g., regreening.

 

References

Tuinenburg, Obbe A., Jolanda J.E. Theeuwen, and Arie Staal. "High-resolution global atmospheric moisture connections from evaporation to precipitation." Earth System Science Data 12.4 (2020): 3177-3188.

How to cite: Theeuwen, J., Staal, A., Tuinenburg, O., Hamelers, B., and Dekker, S.: Local moisture recycling across the globe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6883, https://doi.org/10.5194/egusphere-egu23-6883, 2023.

EGU23-7687 | ECS | PICO | HS7.9

Towards using multi-dimensional structures in climate variables to detect anthropogenic changes 

Marius Egli, Sebastian Sippel, Vincent Humphrey, and Reto Knutti

Precipitation (P) and evapotranspiration (ET) play a crucial role in the water cycle and have a significant impact on water resources and the energy balance of the Earth's surface. However, it remains a challenge, in particular on regional scales, to detect changes in hydrological variables and attribute them to anthropogenic or natural influences. Traditional studies that aim to detect or attribute changes in atmospheric variables often consider only a single variable at a time. This makes detecting changes in hydrological variables challenging due to large internal variability, the lack of long-term observational coverage and partly poor mechanistic understanding of land-atmosphere coupling processes in a changing climate.

 

However, because P and ET are related to various other atmospheric variables, such as temperature, humidity, and sea level pressure, the detection of anthropogenic influences may be conducted in principle within a broader multivariate space. Here, we aim at exploiting multivariate relationships to more robustly detect anthropogenic changes to the hydrological cycle at the regional or up to continental scale. We train statistical models from coupled Earth system models to learn the relationships between relatively well observed variables and more poorly observed ones, like P and ET. We demonstrate that such models can predict and extract patterns of forced change in P and ET, albeit somewhat contingent on the realism of the simulation of the Earth system model. The main advantage is that the method does not rely on sparse observations of P and ET, and instead relies on covariates which are more abundantly and reliably observed.

 

We demonstrate the effectiveness of this approach in a climate-model-as-truth framework, showing that it can capture a wide range of possible hydrological responses produced by the different climate models. We also apply the statistical model to observations to identify forced changes in P and ET that have already occurred. For example, we see an increase in ET in the northern hemisphere likely induced by a reduction in aerosol emissions. Our results show that this method can infer changes in P and ET that may have taken place, in principle even without the need for direct observations of those variables and can provide constrained projections of future water resources and energy balance.

How to cite: Egli, M., Sippel, S., Humphrey, V., and Knutti, R.: Towards using multi-dimensional structures in climate variables to detect anthropogenic changes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7687, https://doi.org/10.5194/egusphere-egu23-7687, 2023.

EGU23-7867 | ECS | PICO | HS7.9 | Highlight

The importance of the plant physiological response to rising CO2 in projections of future water availability 

Jessica Stacey, Richard Betts, Andrew Hartley, and Lina Mercado

Reliable and useful future projections of water scarcity are vital for incorporating into climate policy and national adaptation plans for building climate resilience. However, projections of water scarcity are often based on hydrology models which do not include an important climate feedback affecting the water cycle: the response of plant physiology to rising atmospheric CO2, or “physiological forcing”. With higher atmospheric CO2, plant physiology can affect the water cycle in two contradictory ways. Plant stomata do not open as widely in higher CO2, and therefore transpiration rates are lower, leaving relatively more water in the ground increasing runoff and soil moisture. However, faster rates of photosynthesis with higher CO2 also encourages greater leaf area, and thus higher overall canopy transpiration (even though transpiration of an individual stomata still decreases). The influence of physiological forcing on physical quantities within the water cycle such as transpiration and runoff have been well studied; however, there is a requirement to quantify how this translates to human impacts and more policy-relevant metrics on water resources, such as the water scarcity index. I will present findings from experiments using the Joint UK Land Environmental Simulator (JULES) forced with four earth system models which quantify and highlight the importance of including the plant physiological response in water-related impact studies.

How to cite: Stacey, J., Betts, R., Hartley, A., and Mercado, L.: The importance of the plant physiological response to rising CO2 in projections of future water availability, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7867, https://doi.org/10.5194/egusphere-egu23-7867, 2023.

EGU23-7976 | ECS | PICO | HS7.9 | Highlight

Modeling the Impacts of Deforestation: local drying of the atmosphere and potential effect on downwind precipitation. 

Clément Devenet, Nathalie de Noblet, Catherine Ottlé, Nicolas Viovy, and Frédérique Chéruy

The Amazon rainforest is a vital component of the hydrological cycle of South America. Its evapotranspiration is an essential supply of atmospheric moisture for precipitation in more southern regions of the continent. The potential impacts of deforestation on precipitation in these distant regions are yet not fully understood.

The present research project aims at quantifying the deficit of evapotranspiration occurring at the location of deforestation, focusing on the southern part of Amazonia, which has experienced intense deforestation since the 80s. We first use the ORCHIDEE land surface model forced with the reanalysis dataset CRU-JRA to simulate the impacts of an imposed land cover change: from observed states of vegetation cover to a massive extension of croplands. The ORCHIDEE model computes all the components of evapotranspiration, giving, in turn, the expected deficit of atmospheric moisture at the location of the land cover change.

Then, thanks to existing datasets connecting any place on Earth with the area that supplies its moisture through the atmosphere, we link this deficit with downwind locations highly dependent on this upwind evapotranspiration for its precipitation. From there, we draw hypotheses about the potential changes in precipitation amounts and seasonality.

In the project’s second phase, these hypotheses are tested against land-atmosphere coupled simulations produced with the IPSL global climate model, nudged to winds from the ERA5 reanalysis. The model grid is zoomed on the South American continent to better describe the atmospheric transport in the region. The land-atmosphere coupled simulations provide information on the atmospheric feedback induced by the land cover change, confirming or invalidating the hypotheses. Since land cover affects not only water fluxes but also energy fluxes, the coupled model experiments give us insights into the atmospheric processes at stake, the changes in cloudiness and local convection, and the potential shifts in precipitation location or timing.

How to cite: Devenet, C., de Noblet, N., Ottlé, C., Viovy, N., and Chéruy, F.: Modeling the Impacts of Deforestation: local drying of the atmosphere and potential effect on downwind precipitation., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7976, https://doi.org/10.5194/egusphere-egu23-7976, 2023.

EGU23-8061 | ECS | PICO | HS7.9

Exploring the human influence on surface water availability in the contiguous United States 

Sara Alonso Vicario, Maurizio Mazzoleni, and Margaret Garcia

Finding which factors control the spatial variability of surface runoff is fundamental for assessing regional surface water availability. These controlling factors drive the water balance and vary from physio-climatic catchment attributes to anthropogenic activities. A few studies evaluated these factors in the Contiguous United States on catchments with non-human influence (Abatzoglou & Ficklin, 2017). Yet, a comprehensive analysis of the human influence on surface water availability is still missing.

Here, we employed a parametric Budyko-based framework to assess the long-term runoff sensitivity in the last 30 years of 502 catchments in the Contiguous United States. We linked the Budyko-based framework's landscape parameter with an extensive set of 50 climatic, topographic, anthropogenic, and soil factors that were previously found influential on partitioning precipitation into evapotranspiration and runoff. The catchments belong to the GAGES-II database (Falcone, 2010) and have been grouped in reference and human-impacted basins (urban and agricultural) using the most updated land cover data of 2019. A stepwise multiple linear regression model is developed to find the most significant factors in the partitioning depending on the most extensive human activity on the basin and assess their interactions. Also, we analyzed how anthropogenic activities (e.g., irrigated agriculture, urban settlements) alter the effect of climate variables.

Preliminary results suggest that cultivated land is the second most important factor in explaining runoff variability in agricultural basins, and urban settlements increase the runoff in catchments with a high interannual variability of precipitation.

 

References

Abatzoglou, J. T., & Ficklin, D. L. (2017). Climatic and physiographic controls of spatial variability in surface water balance over the contiguous United States using the Budyko relationship. Water Resources Research, 53(9), 7630–7643. https://doi.org/10.1002/2017WR020843

Falcone, J. A., Carlisle, D. M., Wolock, D. M., & Meador, M. R. (2010). GAGES: A stream gage database for evaluating natural and altered flow conditions in the conterminous United States. Ecology, 91(2), 621–621. https://doi.org/10.1890/09-0889.1

How to cite: Alonso Vicario, S., Mazzoleni, M., and Garcia, M.: Exploring the human influence on surface water availability in the contiguous United States, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8061, https://doi.org/10.5194/egusphere-egu23-8061, 2023.

EGU23-10635 | PICO | HS7.9

Uncertainties in global future projection of potential evapotranspiration using SSP scenarios 

Young Hoon Song, Eun-Sung Chung, Seung Taek Chae, and Jin Hyuck Kim

Evapotranspiration (ET) is the amount of water lost from the global surface, and it represents water and Earth's energy cycle. The intensity and frequency of climate variables have been changed because of the ongoing climate crisis, leading to increased climate disasters, such as heat waves and droughts. The abrupt climate crisis affects the variation of ET because climate variables highly influence ET. However, the future potential ET (PET) estimates include various uncertainty resulted from the variations in the projection of climate variables. In this context, the uncertainty in the projected future PETs should be quantified for the high reliability. Therefore, this study projected future global PET using Penman-Monteith (PM) for the near (2031-2065) and far (2066-2100) futures and quantified the corresponding uncertainty. The six climate variables of 14 CMIP6 GCMs were used for estimating historical PET which were compared to those from the NCEP/NCAR reanalysis data using the five evaluation metrics. The changes in PETs for four Shared Socio-economic Pathways (SSPs) scenarios were calculated for the near and far futures compared to the historical period (1980-2014). Subsequently, the uncertainties of PETs were quantified using the reliability ensemble average method. As a result, the future PET in high latitudes showed the most significant variability compared to the other latitudes. The future PET in the southern hemisphere was higher than the historical PET. Especially the PET in the mid-latitudes of southern hemisphere was the highest among the other latitudes. In addition, the uncertainty of PET was the highest in the high latitudes of the northern hemisphere while the mid-latitude in the northern was the lowest. This study provides insight into evaluating the global water cycle based on PET and helps establish appropriate policies for climate impact assessment.

How to cite: Song, Y. H., Chung, E.-S., Chae, S. T., and Kim, J. H.: Uncertainties in global future projection of potential evapotranspiration using SSP scenarios, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10635, https://doi.org/10.5194/egusphere-egu23-10635, 2023.

EGU23-10652 | ECS | PICO | HS7.9

Atmospheric moisture exchanges between the Magdalena River basin and its surroundings. 

Paola Andrea Giraldo Ramirez, Ruben Dario Molina Santamaria, and Juan Fernando Salazar Villegas

Atmospheric moisture transport is a fundamental process in the climate system, critical for the hydrological cycle and water security on land. Moisture exchanges between a basin and its surroundings determine water availability and may change over time due to climate change and other human impacts. Understanding how and why these atmospheric fluxes change under global change is critical for river basins supporting water security in different regions. Here we focused on the Magdalena River basin in northwestern South America, a critical basin for water and energy security in Colombia. We quantified moisture exchanges for the entire watershed and different segments (defined by the boundaries between neighboring basins). We used monthly data between 1979 and 2021 from the ERA5 reanalysis to look for possible changes, including trends. Our results provide new insights into the dynamics of moisture exchanges between the basin and its surroundings. In addition, we found evidence of statistically significant trends likely related to anthropic effects, mainly deforestation and climate change. These results have implications for water security analyses in this region, where there are few studies of this type, and simultaneously generate new insights for decision-making related to water management and transboundary water security in the Magdalena river basin.

How to cite: Giraldo Ramirez, P. A., Molina Santamaria, R. D., and Salazar Villegas, J. F.: Atmospheric moisture exchanges between the Magdalena River basin and its surroundings., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10652, https://doi.org/10.5194/egusphere-egu23-10652, 2023.

EGU23-12671 | ECS | PICO | HS7.9 | Highlight

WRF with age-weighted water tracers: implementation, application, and new insights into the regionally accelerated atmospheric hydrological cycle under global warming 

Jianhui Wei, Joël Arnault, Thomas Rummler, Benjamin Fersch, Zhenyu Zhang, Patrick Olschewski, Patrick Laux, and Harald Kunstmann

Atmospheric water residence time, here defined as time between the original evaporation and the returning of its respective water masses to the land surface as precipitation, is a measure of the speed of the atmospheric hydrological cycle. Traditional analytical methods are generally limited by crude assumptions in the coupling between the land surface and the atmosphere, and hence are not applicable to regions with complex monsoon systems under a changing climate. To this end, we have implemented the age-weighted water tracers into the Weather Research and Forecasting WRF model, namely, WRF-age, to follow the atmospheric water pathways and to derive atmospheric water residence times accordingly. The newly developed, physics-based WRF-age is used to regionally downscale the reanalysis of ERA-Interim and the MPI-ESM Representative Concentration Pathway 8.5 scenario (RCP8.5) simulation for an East Asian monsoon region, i.e., the Poyang Lake basin, for two 10-year slices of historical (1980-1989) and future (2040-2049) times. In comparison to the historical WRF-age simulation, the future 2-meter air temperature rises by 1.3 °C and precipitation decreases by 38% under RCP8.5 on average. In this context, global warming leads to decreased atmospheric residence times of the column-integrated water vapor (from 22 to 13 hours) and column-integrated condensed moisture (from 26 to 14 hours) in the atmosphere over the basin, but slightly increased atmospheric residence times of surface precipitation (from 12 to 15 hours) in agreement with reduced the precipitation amounts. Our findings demonstrate that global warming increases the complexity of regional atmospheric water cycle, especially the associated changes in the residence times of atmospheric water states of matter.

How to cite: Wei, J., Arnault, J., Rummler, T., Fersch, B., Zhang, Z., Olschewski, P., Laux, P., and Kunstmann, H.: WRF with age-weighted water tracers: implementation, application, and new insights into the regionally accelerated atmospheric hydrological cycle under global warming, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12671, https://doi.org/10.5194/egusphere-egu23-12671, 2023.

EGU23-12775 | PICO | HS7.9

Introducing project ITHACA: Investigation of the Terrestrial HydrologicAl Cycle Acceleration 

Yannis Markonis, Mijael Rodrigo Vargas Godoy, Johanna Blöcher, Riya Dutta, Shailendra Pratap, Rajani Pradhan, Alexander Kazantsev, Petr Bašta, Akbar Rahmati, Arnau Sanz i Gil, Vishal Thakur, Hossein Abbasizadeh, Oldřich Rakovec, Martin Hanel, Petr Máca, Rohini Kumar, and Simon Papalexiou

ITHACA is a 5-year project that aims to benchmark the terrestrial water cycle intensification. Our goal is to estimate the past range of the hydrological cycle variability, determine the present state of its acceleration, and understand its future impacts on the terrestrial water availability. To achieve this, we combine multi-source data products, stochastic analysis, and process-based hydrological modeling from regional to global scale. Here, we present the preliminary results after the completion of its first year, which come with multiple homogenized datasets of water cycle components, R software packages for data pre-processing and data-driven analyses, and methodological suggestions and insights for the cross-scale quantification of water cycle changes. We also discuss the current challenges and the future steps of the project, highlighting the numerous opportunities for active collaboration.  

How to cite: Markonis, Y., Vargas Godoy, M. R., Blöcher, J., Dutta, R., Pratap, S., Pradhan, R., Kazantsev, A., Bašta, P., Rahmati, A., Sanz i Gil, A., Thakur, V., Abbasizadeh, H., Rakovec, O., Hanel, M., Máca, P., Kumar, R., and Papalexiou, S.: Introducing project ITHACA: Investigation of the Terrestrial HydrologicAl Cycle Acceleration, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12775, https://doi.org/10.5194/egusphere-egu23-12775, 2023.

EGU23-13142 | PICO | HS7.9

An engineering approach to land-surface controlled convective precipitation 

Sarah Warnau and Bert Hamelers

In the summer of 2022, several records of hot and dry conditions were broken in Europe, resulting in problems of water availability that are projected to increase further, especially in the Mediterranean basin. The reason for this drying trend is twofold: There is a reduction in precipitation, and an increase in evaporative demand due to climate warming. For climate mitigation and adaptation, solutions are needed to counteract this drying trend. A technological innovation that can be considered is enhancing surface evaporation by evaporating sea water using solar energy. The aim of this research is to examine whether this technology can potentially be used to address the reduction in precipitation. Therefore, we study under which conditions enhanced surface evaporation leads to more convective precipitation and how much water is required to achieve this.

For convective precipitation to occur, several conditions must be met. These include the atmospheric boundary layer (ABL) crossing the lifting condensation level (LCL), moist air parcels reaching their level of free convection (LFC), and the convective available potential energy (CAPE) surpassing a certain threshold (e.g. 400 J/kg). These conditions can be affected by turbulent fluxes of heat and moisture from the surface. Here we use a zero-dimensional mixed layer "slab" model which describes the evolution of the convective ABL height up to the LCL-crossing and the potential temperature and specific humidity of the mixed layer. From this model we obtain an implicit analytical relationship between the integrals of surface fluxes of heat and moisture that cause the LCL and ABL to cross. The relationship between these integrated surface fluxes varies depending on the initial and free atmospheric conditions.

As a case study, we examine the Ebro basin in northeastern Spain. We use the analytical expression of the LCL-crossing with the observational data from the LIAISE campaign to estimate:

  • how many days during the 2021 summer months could enhanced surface evaporation theoretically have led to an LCL-crossing,

  • the amount of water required in such cases, and

  • the changes to the LFC and CAPE that this evaporation enhancement could cause.

Preliminary results indicate that the LCL-crossing relationship between the integrated surface fluxes strongly depends on the initial and free atmospheric temperatures. This has implications for the areas where the technology could potentially benefit the water availability. Since convective precipitation is only controlled by the surface under specific atmospheric conditions, climate warming can cause areas to go from surface controlled to being too hot for the technology to be able to trigger convective precipitation.

Our research provides a preliminary assessment of the potential of this technology to counteract the drying trend in the Mediterranean basin. Further research is needed to evaluate the amount of precipitation that can be expected from the technology, as well as the effects of the technology on local evaporative demand, evapotranspiration, and heat stress.

How to cite: Warnau, S. and Hamelers, B.: An engineering approach to land-surface controlled convective precipitation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13142, https://doi.org/10.5194/egusphere-egu23-13142, 2023.

EGU23-13426 | ECS | PICO | HS7.9

Upwind land-use change impacts on wetland vulnerability 

Simon Felix Fahrländer, Lan Wang-Erlandsson, Agnes Pranindita, Lauren Seaby Andersen, and Fernando Jaramillo

Research on the protection and preservation of wetlands has traditionally focused on direct human drivers and impacts of climate change occurring in their upstream hydrological basin. However, since precipitation falling in the hydrological basin comprises both oceanic and terrestrial evaporation originating mostly outside of the basin boundaries, upwind land use and hydroclimatic changes affecting this supply of precipitation also need to be assessed. This study assesses the vulnerability of 40 wetlands of international importance to land use and hydroclimatic changes occurring upwind (i.e., in their precipitationsheds). We here use a dataset containing atmospheric moisture flows in combination with evaporation from natural and current vegetation to analyse the impact of extra-basin vegetation changes on the precipitation over the wetland basins. The analysis shows that historical land-use conversion has already caused reduced incoming precipitation into most wetland hydrological basins. The strongest effects are seen in (sub)tropical wetlands in South America, Africa and Asia and especially those located downwind of large agricultural areas. Based on our results and current wetland decline rates, we find that wetland sites in China, India, South America and Sub-Saharan Africa are especially threatened by hydroclimatic and vegetation changes outside of their basins. Additionally, larger basins appear to be more reliant on evaporation from within their basin boundaries than smaller hydrological basins. Using wetland ecosystems as an exemplary case, this study stresses the need to incorporate downwind effects to land-use changes in sustainable ecosystem management approaches. Since the transition from potential natural vegetation to agricultural land is often associated with changes in evaporation, land conversion may affect the resilience of wetland water availability. Following this analysis of the upwind moisture sources of wetland basins, future studies should investigate the potential effect of wetland loss on downwind precipitation patterns.

How to cite: Fahrländer, S. F., Wang-Erlandsson, L., Pranindita, A., Andersen, L. S., and Jaramillo, F.: Upwind land-use change impacts on wetland vulnerability, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13426, https://doi.org/10.5194/egusphere-egu23-13426, 2023.

EGU23-13859 | PICO | HS7.9

Collaborative moisture tracking with WAM2layers v3 

Peter Kalverla, Imme Benedict, Ruud van der Ent, and Chris Weijenborg

Atmospheric moisture tracking is a valuable technique for understanding the physical processes that drive (extreme) precipitation and drought in our changing climate. By following where precipitated moisture originally evaporated (backtracking) or where evaporated moisture eventually precipitates (forward tracking) we can gain valuable insights into the connection of large-scale weather systems and hydrometeorological events, land-atmosphere interactions, or the impact of land-use changes on water availability.

The WAM2layers model is an Eulerian moisture tracking code that solves the water balance equation for tagged moisture in gridded model output data. With the increasing resolution of weather and climate models, however, data handling and performance have become serious constraints. Over the past year, we have worked on a new version of WAM2layers (github.com/WAM2layers/WAM2layers), in which we tackle these computational challenges and make a substantial upgrade to the user- and developer-friendliness of the model. The most important changes are summarized below.

Usability: the new version of WAM2layers separates configuration from code. This makes it possible to run many different model simulations without modifying the source code. The model can now be run with a single command, supplying a configuration file as an input argument. It is even possible to use the model without copying the code. Simply install the wam2layers Python package from PyPI.

Modularity: we have made a stricter separation between preprocessing steps, the actual tracking code, and utilities for analysing the results. This is important, for example, for working with multiple datasets. So far, we've worked with ERA5 data. Adding support for other datasets requires no modifications to the tracking code, only a separate preprocessing script.

Documentation: the new version of the model comes with documentation on ReadTheDocs. The documentation includes theory, installation instructions, a complete user guide, and contributing guidelines.

Collaborative development: previous versions of the model were already available on GitHub, but further development often happened offline and without coordination. From the start of this project, we have opened up the development process such that everyone can ask questions, raise issues, and open pull requests. The brand-new documentation includes instructions for anyone willing to contribute. We believe this shift represents a modern perspective on collaborative research practice.

How to cite: Kalverla, P., Benedict, I., van der Ent, R., and Weijenborg, C.: Collaborative moisture tracking with WAM2layers v3, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13859, https://doi.org/10.5194/egusphere-egu23-13859, 2023.

As cities around the world are growing at a rapid pace, the need to understand their impact on the regional to local climate has become more crucial.  Urban settlements are more affected by extreme weather than rural areas. Localised circulation patterns, the topography of the region and micro-scale systems induced by Land-Use Land-Cover (LULC) can modify regional flows to produce unique patterns in the urban region. National Capital Region (NCR) - Delhi, the second biggest urban settlement globally, reported an almost ~20 fold increase in urban and built-up areas in past decades. NCR urbanisation during the past few decades caused a corresponding increase up to 3–5 and 2–4 K in values of LST and T2m, respectively, while a decrease in the magnitude of surface winds up to 2 m s−1 was noted. The LULC plays a crucial role in meteorological models because they determine the crustal properties that interfere with the exchange of energy, moisture, and momentum between the land surface and the atmosphere. This study attempts to assess the impact of legitimate present-state LULC based on AWiFS in the mesoscale model for simulating monsoon weather over NCR Delhi. The newly implemented AWiFS LULC precisely distinguishes the default MODIS classification used in the model framework. Overall, the AWiFS-based simulations showed an improved performance in predicting the study period during the monsoon.

How to cite: Chalakkal, J. B. and Mohan, M.: Impact of accurate representation of Land Use/Land Cover over the National Capital Region (NCR) Delhi in simulating Monsoon Weather, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-605, https://doi.org/10.5194/egusphere-egu23-605, 2023.

EGU23-2418 | Posters on site | ITS2.8/AS1.23

Probabilistic Rainy Season Onset Prediction over the Greater Horn of Africa based on Long-Range Multi-Model Ensemble Forecasts 

Michael Scheuerer, Titike Bahaga, Zewdu Segele, and Thordis Thorarinsdottir

Most of the socioeconomic activities in the Greater Horn of Africa (GHA) region are rain dependent, and economic sectors such as agriculture, hydroelectric power generation, and health would greatly benefit from reliable information about onset, cessation, intensity, and frequency of rainfall. 
In a seasonal climate forecast at lead times on the order of weeks or months, uncertainty about these variables is significant, making a case for probabilistic forecasting where uncertainties are communicated along with the forecast.

We present results of an evaluation of the skill of probabilistic rainy season onset forecasts over GHA, which were derived from bias-corrected, long-range, multi-model ensemble precipitation forecasts. A careful analysis of the contribution of the different forecast systems to the overall multi-model skill shows that the improvement over the best performing individual model can largely be explained by the increased ensemble size. An alternative way of increasing ensemble size by blending a single model ensemble with climatology is explored and demonstrated to yield better probabilistic forecasts than the multi-model ensemble. Both reliability and skill of the probabilistic forecasts are better for OND onset than for MAM and JJAS; for the two latter, forecasts are found to be late biased and have only minimal skill relative to climatology. While the overall level of skill is limited in our setup where predictions are made at a horizontal resolution of 0.25 degrees, we find that especially OND forecast skill increases substantially under a metric that evaluates the forecasts at coarser spatial scales.

How to cite: Scheuerer, M., Bahaga, T., Segele, Z., and Thorarinsdottir, T.: Probabilistic Rainy Season Onset Prediction over the Greater Horn of Africa based on Long-Range Multi-Model Ensemble Forecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2418, https://doi.org/10.5194/egusphere-egu23-2418, 2023.

Western Equatorial Africa (WEA) is characterized by a long and cloudy dry season extending from June to September. So far, no study has investigated the intra-seasonal characteristics of this dry season especially its onset and cessation dates. In our study, the onset and cessation dates are determined over the 38-year period 1983–2020, using daily surface solar radiation (SSR) data from CMSAF SARAH-2. The maximum and minimum values of the cumulative anomalies of a regional index, for each year, are used to extract the onset and cessation dates. The mean onset date of the dry season in the region is May 17, the mean cessation date is October 3. We obtain very distinct anomaly patterns of SSR but also of low-level clouds and precipitation before/after the onset/cessation dates. The onset and cessation dates show strong year-to-year variability but no significant trend is detected over the 4 decades studied. Lastly, the cumulative anomalies for each year are also used to classify the dry seasons according to the SSR intra-seasonal evolution. Three types of years are obtained which are associated to different patterns of SST anomalies in the tropics.

How to cite: Ouhechou, A., Philippon, N., and Morel, B.: Detection and characterization of the onset and cessation dates of the dry season in Western Equatorial Africa based on solar radiation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4418, https://doi.org/10.5194/egusphere-egu23-4418, 2023.

EGU23-5395 | Posters virtual | ITS2.8/AS1.23

Potential shift of rainy seasons’ onset and cessation under climate change scenarios in West Africa 

Torsten Weber, Imoleayo E. Gbode, Amadou Coulibaly, Daniel Abel, Karin Ziegler, Jean-Bosco B. Zoungrana, Seydou B. Traore, and Heiko Paeth

Information on the onset and cessation of rainy seasons is an important prerequisite for planning the sowing of crops in West Africa. A late onset, but also too early cessation of a rainy season, has a direct impact on plant growth and thus on the crop yield in the region. However, onset and cessation dates of rainy seasons can change under future climatic conditions. Therefore, this information is key for stakeholders and decision-makers to mainstream climate change into agricultural activities and policies for better adaptation in the region.

To obtain information on the onset and cessation of rainy seasons on a regional scale under future climate change, Regional Climate Models (RCMs) are applied to dynamically downscale global climate projections generated by Earth System Models (ESMs). Therefore, regional climate projections provide more detailed information due to the higher spatial resolution compared to the climate projections generated by ESMs.

The study will show initial results on the onset and cessation of rainy seasons in West Africa under two emission scenarios using the Representative Concentration Pathways (RCPs) 2.6 and 8.5 for the end of the century (2071-2100 vs. 1981-2010). The regional climate projections are taken from the Coordinated Output for Regional Evaluations (CORE) embedded in the WCRP Coordinated Regional Climate Downscaling Experiment (CORDEX) for Africa with a spatial resolution of about 25 km. In this initiative, three different RCMs (REMO2015, RegCM4-7, and CCLM5-0-15) were applied to perform the downscaling process.

How to cite: Weber, T., Gbode, I. E., Coulibaly, A., Abel, D., Ziegler, K., Zoungrana, J.-B. B., Traore, S. B., and Paeth, H.: Potential shift of rainy seasons’ onset and cessation under climate change scenarios in West Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5395, https://doi.org/10.5194/egusphere-egu23-5395, 2023.

The Climate Predictability Tool (CPT) is a well established tool for creating calibrated objective predictions of seasonal rainfall anomalies, and is used for this purpose by many institutions including  the IGAD Climate Prediction and Applications Centre (ICPAC)  to create operational forecasts for the Greater Horn of Africa wet seasons. CPT can also be used to predict other variables such as wet season onset. Such predictions require a non spatially dependent definition of onset, in our case we define onset as the number of days into the season when rainfall reaches 10% of seasonal rainfall for that location. The CPT forecasts are created by detecting relationships between predictions of precipitation and SST from global dynamical forecasting systems and observed onset patterns using Canonical Correlation Analysis (CCA).  CPT has the advantage that skill statistics are automatically produced for assessing the performance of the forecasts. CPT forecasts of Short rains (October-December) onset have been found to have useful skill.

How to cite: Colman, A.: Hybrid dynamical/statistical forecasts of wet season onset using CCA, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7802, https://doi.org/10.5194/egusphere-egu23-7802, 2023.

Monsoon onset is the most awaited event for more than a billion people in India because monsoon rainfall is a source of life for the population. The abruptness of the transition to monsoon and its spatial and temporal variability from year to year are key features of the phenomenon that makes predicting the monsoon's onset a scientific challenge. According to Ananthakrishnan and Soman, 1988, [1], the onset of a monsoon is a transition from a regime of sporadic rainfall to spatially organized and temporally sustained rainfall. Our recent study [2] added a single word to this definition by discovering that a transition to monsoon is a 'critical' transition. We defined two states in the transition: pre-monsoon and monsoon. Between two states must be a critical point - a threshold in the atmospheric variables (near-surface air temperature, relative humidity). We found that the monsoon begins when the variables overcome a critical threshold. This funding allowed us to develop and successfully implement [3] the methodology of the long-term forecast of monsoon onset and withdrawal in Central India, Northern Telangana, and Delhi: 40 days before the onset date and 70 days before the withdrawal date. Building on these findings, I move forward to understand how to describe the critical conditions for a local onset and withdrawal of monsoon in every state in India, where the monsoon forecast desperately needs.

Here, I present a definition of monsoon onset for every location based on critical values of three atmospheric variables: temperature (Tc), relative humidity (RHc), and outgoing longwave radiation (OLRc). The OLR is included in the critical points set because it is a crucial indicator for the upcoming monsoon characterizing convective activity, implying scarcity or deep convective clouds. The critical values (Tc, RHc, OLRc) for every location can be revealed from the historical observations: near-surface temperature and relative humidity at 1000 hPa from NCEP/NCAR reanalysis and OLR data from NOAA. The three critical points do not always appear simultaneously; the dates might differ from one to three days. Hence, monsoon onset occurs when all three variables pass a critical threshold. I anticipate the definition to be a starting point for other monsoon-related applications, such as planning agriculture season, the water and energy recourses management.

Importantly, a vulnerable period could appear between monsoon onset and sustainable rainfall - a dry spell after initial rainfall strongly affecting the agriculture sector. I work towards a deeper understanding of the precursors of a dry spell and its extremes and uncover how to avoid false alarms that are disastrous for farming.

ES acknowledges the financial support of the B-EPICC project (18_II_149_Global_A_Risikovorhersage) funded by FFO.

[1] Ananthakrishnan R., and M. K. Soman, 1988: The onset of southwest monsoon over Kerala: 1901-1980. J. Climatol., 8, 283–296.

[2] Stolbova, V., E. Surovyatkina, B. Bookhagen, and J. Kurths (2016): Tipping elements of the Indian monsoon: Prediction of onset and withdrawal. GRL 43, 1–9 [doi:10.1002/2016GL068392]

[3] https://www.pik-potsdam.de/members/elenasur/forecasting-indian-monsoon/welcome-to-the-pik-monsoon-page-1

How to cite: Surovyatkina, E.: Local onset of monsoon defined by critical values of atmospheric variables: Indian summer monsoon case, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8441, https://doi.org/10.5194/egusphere-egu23-8441, 2023.

EGU23-10749 | ECS | Posters on site | ITS2.8/AS1.23

Delayed response of the onset of the summer monsoon over the Bay of Bengal to land–sea thermal contrast 

Sun Weihao, Liu Yimin, and Wu Guoxiong

The mechanisms involved in the onset of the Bay of Bengal summer monsoon (BOBSM) were studied using reanalysis data and numerical model experiments. Results revealed that the weak meridional land–sea thermal contrast (LSTC) over the northern BOB in early spring enhances the lower-tropospheric easterly belt along 10°–15°N, which is unfavorable for the BOBSM onset. The BOBSM onset is driven by the cumulative impact of this LSTC along with the LSTC in the meridional direction across the equator and in the zonal direction across the tropics, together with air–sea interactions. While the LSTC intensifies over the northern BOB, a near-surface northward cross-equatorial flow develops south of India, inducing springtime zonal flow and surface sensible heating over the southern BOB and a pair of cyclones straddling the equator over the central Indian Ocean at 700 hPa. The zonal LSTC in the tropics generates near-surface cyclones over land and anticyclones over the sea. This induces a zonal SST warm pool around 10°N, which produces vertical westerly wind shear to the north and weakens the wintertime easterly aloft and the anticyclone to its north. As the cyclone over southern India develops eastward, the cyclone below 700 hPa develops northward over the eastern BOB in response to the enhancing tropical westerly and surface sensible heating. The wintertime anticyclonic belt and easterly belt split, and the southerly carries water vapor northward over the eastern BOB, heralding the onset of the BOBSM and presenting a delayed response to the springtime LSTC changes.

How to cite: Weihao, S., Yimin, L., and Guoxiong, W.: Delayed response of the onset of the summer monsoon over the Bay of Bengal to land–sea thermal contrast, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10749, https://doi.org/10.5194/egusphere-egu23-10749, 2023.

EGU23-12235 | ECS | Posters on site | ITS2.8/AS1.23

Characterizing the growing period using seasonal rainfall onset dates in the semi-arid region of Tanzania 

Jacob Joseph, Anthony Whitbread, Reimund Roetter, and Elena Surovyatkina

Rainfall characteristics such as onset and cessation dates, seasonal rainfall amount, and distribution significantly impact agricultural production in rainfed systems. Studies have found that timely crop planning is necessary to maximize crop production and increase the resilience and sustainability of the rain-fed system. Thus, timely and accurate prediction of seasonal rainfall characteristics is crucial to enhance effective crop planning and minimize climate-induced crop production risks. The present study used seasonal rainfall onset dates computed using a long-term dataset, i.e., 1935–2020, acquired from the Tanzania Meteorological Authority (TMA) using Liebmann’s method to characterize the growing period in the semi-arid region of Tanzania—Kongwa district. Liebmann’s method was used due to its proven suitability in both hydrological and agronomical applications. We further used the well-known climate indices, i.e., the SOI (Southern Oscillation Index), the IOD (Indian Ocean Dipole), and NINO 3.4 averaged over the July–September period in the decision tree model, to predict the onset dates and characterize the growing period. We found the late-onset seasons—two weeks after the 7th of December—had lower rainfall (17% less than the climatological mean) and were at least 15 days shorter than the climatologically normal growing period. Moreover, the variability in seasonal rainfall in the late-onset season (CV = 28%) was found to be at least 5% higher than in the early-onset season. Late-onset seasons had a 40% chance of receiving the minimum amount of rainfall required for high-water-demand cereals like maize (450 mm). We also found SOI to be a good predictor of onset dates compared to NINO 3.4 and IOD. The SOI predicted well both normal and late-onset infections—50% and 68% precision (hit rate), respectively—compared to the IOD and NINO 3.4, whose precision was less than 10% in predicting the late onset and about 63% in predicting the normal onset. Although our results are useful to guide crop planning before the season, we recommend further studies to examine the agronomical and economic impacts the onset dates would have on crop productivity.

How to cite: Joseph, J., Whitbread, A., Roetter, R., and Surovyatkina, E.: Characterizing the growing period using seasonal rainfall onset dates in the semi-arid region of Tanzania, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12235, https://doi.org/10.5194/egusphere-egu23-12235, 2023.

EGU23-12834 | Posters on site | ITS2.8/AS1.23

Rainy season onset and cessation over the Greater Horn of Africa area: definitions and forecasts. 

Rondrotiana Barimalala, Masilin Gudoshava, Teferi Demissie, Stefan Sobolowski, Erik Kolstad, and Michael Scheuerer

The demand for more accurate forecasts in rainy season onset, length and cessation has significantly increased over the Greater Horn of Africa area. Recent failed rainy seasons, and an extended drought over much of the region, have highlighted the need for both reliable and timely forecasts so that action can be taken proactively rather than reactively. One of the major challenges in the weather and climate science community is how to appropriately define and characterize onset in such a way that is both robust and useful to the stakeholders.

As part of the EU H2020 project CONFER (Co-production of Climate Services for east Africa), we revisit the rainfall onset and cessation definitions used over the subcontinent, with a particular focus on the large discrepancies, reaching up to 50 days, in the onset and cessation dates that emerge from different definitions. The climate over the Greater Horn of Africa is highly variable with most of the region classified as arid and semi-arid and only a few areas classified as humid. A regionalization of the thresholds used in the definitions that more accurately accounts for user needs and the amount of total rainfall an area receives is suggested. These regional details are then combined with a probabilistic approach developed in CONFER, based on a widely available multi-model seasonal forecast ensemble, to predict rainy season onset over the Greater Horn of Africa area.

How to cite: Barimalala, R., Gudoshava, M., Demissie, T., Sobolowski, S., Kolstad, E., and Scheuerer, M.: Rainy season onset and cessation over the Greater Horn of Africa area: definitions and forecasts., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12834, https://doi.org/10.5194/egusphere-egu23-12834, 2023.

EGU23-14836 | ECS | Posters on site | ITS2.8/AS1.23

Evaluating the Performance of the WRF model in reproducing the Rainfall Onset and Cessation  over Eastern  Africa 

Masilin Gudoshava, Titike Bahaga, Rondrotiana Barimalala, Stefan Sobolowski, Zachary Atheru, Teferi Demissie, and Guleid Artan

Knowledge of the onset, cessation and length of the rainy season is important for decision-making in various climate sensitive sectors over Eastern Africa. In the agricultural sector for example the forecast information on these characteristics can be used to decide on when and what to plant.  We customize the Weather Research and Forecasting (WRF) model over the region and evaluate the skill of producing the onset and cessation over the region. The WRF regional climate model is utilised in sub-seasonal to seasonal forecasting over the region.  We utilize the threshold on accumulated rainfall method for calculating the rainfall onset and cessation as is currently done operationally over the region by the IGAD Climate Prediction and Applications Centre.   The customization experiments focus on the land surface, cumulus and microphysics schemes for the long rains (March-April- May), June to September and the short rains (October-November-December). In this study 3 land surface schemes, 5 cumulus and 6 microphysics schemes are utilized in combination with other physics schemes.  The WRF model is able to simulate the seasonal rainfall over the region. In addition it is shown that some physics combinations represent the onset and cessation  dates  better compared to others. The preliminary results  highlight the usefulness of the WRF model in reproducing the onset and cessation characteristics over the region. 

How to cite: Gudoshava, M., Bahaga, T., Barimalala, R., Sobolowski, S., Atheru, Z., Demissie, T., and Artan, G.: Evaluating the Performance of the WRF model in reproducing the Rainfall Onset and Cessation  over Eastern  Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14836, https://doi.org/10.5194/egusphere-egu23-14836, 2023.

While it is well known that the interannual variability of Kiremt (boreal summer) Rains in Ethiopia is forced by Sea Surface Temperature (SST) in the Pacific Ocean, the mechanisms for ENSO-Kiremt Rains teleconnections and the role of other oceans are not fully understood. In this study, the Ethiopian Kiremt Rains interannual variability was analyzed using observational data and higher-resolution SST-forced ICON experiments for the period 1981–2017. Such fine-grid global and two-way nests over the Greater Horn of Africa (GHA) were carried out here for the first time. The physical mechanisms that link ENSO influence on the Kiremt Rains in the model and ERA5 reanalysis are also investigated. It is found that the model reasonably simulates the main features of the JJAS rainfall climatology over GHA and also reproduces horizontal wind intensity and patterns at (150, 600, 850, and 925- hPa) levels over Africa. It is shown that there is a substantial skill in reproducing the leading modes of Kiremt Rains interannual variability (r = 0.64), given the SSTs are known. The results suggest that the majority (> 50%) of Kiremt Rains anomalies are driven by Equatorial Pacific SST variability, while the SST effects from other regions counteracted ENSO impact in the model. Consistent with previous studies, it is found that the El Niño phase of the ENSO drives a corresponding large-scale circulation anomaly, which weakens the monsoon trough over the Arabian Peninsula, and descending motion and upper-level convergence right over Ethiopia. The subsidence over the GHA region induces upper (lower) level westerly (easterly) wind anomalies over North Africa, weakening Tropical Easterly Jet, Somali Low-Level Jet, and reducing the moist westerly from Atlantic and Congo basin, and thus a reduction of Kiremt Rains over Ethiopia. The opposite pattern is considered under La Niña events and enhanced surface westerlies leading to wetter Kiremt Rains. This mechanism represents an anomalous Walker-type circulation for the ENSO-Kiremt Rains teleconnection. The results will have ramifications for climate model improvement and seasonal forecast improvement in Ethiopia and GHA.

How to cite: Bahaga, T.: Representation of the Mean Climate and Interannual Variability of Kiremt Rains over the Ethiopian Highlands within ICON AMIP Simulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16914, https://doi.org/10.5194/egusphere-egu23-16914, 2023.

The  onset  of  the  southwest  monsoon  over  Kerala  (Southern tip of India) is  very  crucial  as  it  marks  the  beginning  of  the rainy  season  for  Indian  land  mass.  The  onset  of  the  broad  scale  Asian  monsoon  occur  in  many  stages  associated with the significant  transitions  in  the  large-scale  atmospheric  and  ocean  circulations  over  the  region.  Along with this, the changes in sea surface temperature (SST) and convective activity over the north Indian Ocean also play crucial roles during the onset and advance of monsoon over India. Recent analysis (based on data from 1971 to 2019) by India Meteorological Department (IMD) on the onset & withdrawal of southwest monsoon over India compared to the earlier onset and withdrawal dates (based on the rainfall data from 1901 to 1940) has found variations in onset and withdrawal dates over different parts of India.

 

        The variability of SST and convective activity over the north Indian Ocean (Bay of Bengal and Arabian Sea) on inter-annual time scales and their association with the onset and withdrawal of southwest monsoon over India has been analysed by using 42-year (1980-2021) monthly mean outgoing longwave radiation (OLR) data. The 42-year period is categorised into two groups of 21 years each (Former: 1980-2000 & Later: 2021-2021). The inter-annual variability of SST shows significant increasing trends over the Arabian Sea and the Bay of Bengal with a comparatively higher rate of increase of SST over the Arabian Sea. Associated with this increasing SST, the degree of moist static convective instability and associated convective rainfall is also increasing during later period compared to the former period with a magnitude of difference is higher over the Arabian Sea compared to the Bay of Bengal.

         The analysis also indicated that there is a rapid progress of monsoon to the north after its onset over the southern tip of India leading to early onset over parts of northern India.  Similarly, there is a delayed withdrawal of monsoon from northwest India in later period compared to the former period, which is basically, due to the increasing convective activity over the north Arabian Sea and neighbourhood during the onset and withdrawal phase of monsoon.

How to cite: Pattanaik, D. R.: Recent Changes in Onset and Withdrawal Characteristics of Monsoon over India in Relation to Variability of SST and Convection over the Indian Ocean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17236, https://doi.org/10.5194/egusphere-egu23-17236, 2023.

EGU23-17545 | Posters virtual | ITS2.8/AS1.23

Major drivers of East African Monsoon variability and improved prediction for Onset dates 

Indrani Roy, Alberto Troccoli, and Meshack Mliwa

Monsoon rain and its year-to-year variability have a profound influence on Africa’s socio-economic structure by heavily impacting agricultural and energy sectors.  The current study focuses on major drivers of the east African Monsoon during October-November-December (OND) which is a common onset window for various rainfall patterns, unimodal or bimodal. Major drivers of monsoon rain in the East African sector, covering Tanzania, Malawi, Kenya and Somalia could be different in early or extended boreal winter, due to the relative positioning of the Intertropical convergence zone and its seasonal migration -hence the location and season is the focus here.

Two drivers viz. Indian Ocean Dipole (IOD) and El Niño Southern Oscillation (ENSO) both separately  indicate very strong positive connections with monsoon(OND) rain. Not only is a strong significant correlation present in OND season with zero seasonal lag, but the signal is also present even a season ahead (before four months too).  This is also confirmed using various data sources, detrending the data, using regression technique and covering even earlier as well as later periods.  To further strengthen results, a compositing technique is applied that can additionally identify strong signals when different combinations of ENSO and IOD phases act as confounding factors. Results of precipitation anomaly suggest that when IOD and ENSO are both on the same phase in July-August-September (JAS), a significant OND rainfall anomaly is noticed around the east African sector: a deficit (excess) of monsoon rain when both drivers are in the negative (positive) phase. Walker circulation seems to play a major part in transporting signals, via reversing its ascending or descending branch over the regions, when IOD and ENSO are in the same phase. These results can be used for prediction purposes and interestingly, that criterion of IOD and ENSO being of same phase in JAS was again matched in 2022 (both negative) and hence it was possible to deliver early warnings for a deficit in the rain, a season ahead.

Methods to compute the Monsoon Onset as determined by meteorological services such as the Tanzania Meteorological Authority rely on various thresholds (these can vary according to the country). To overcome some of the biases with such methods, other definitions of ‘Onset’ take into account cumulative rainfall amount: these have also been tested. Late (early) Onsets dominate years when ENSO and IOD are both in their negative (positive) phases during the JAS season. The cumulative rainfall and Onset days are correlated such that early Onsets are usually associated with more seasonal rainfall and vice versa. Uncertainty in cumulative rain as well as the Onset date of the OND Monsoon is reduced to a large degree when years are categorised based on ENSO and IOD phases of the previous season. Such results have implications for future planning in optimizing agricultural and energy outputs, mitigating severe consequences and losses, alongside taking advantage of favourable weather scenarios. It will impact the livelihoods of millions of Africans. 

How to cite: Roy, I., Troccoli, A., and Mliwa, M.: Major drivers of East African Monsoon variability and improved prediction for Onset dates, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17545, https://doi.org/10.5194/egusphere-egu23-17545, 2023.

EGU23-37 | Orals | AS1.24

Nonlinear intensification of monsoon low pressure systems by the BSISO 

Kieran Hunt and Andrew Turner

More than half of the rainfall brought to the Indian subcontinent by the summer monsoon is associated with low-pressure systems (LPSs). Yet their relationship with the Boreal Summer Intraseasonal Oscillation (BSISO) – the dominant intraseasonal forcing on the monsoon – is only superficially understood. Using reanalysis data, we explore the relationship between the BSISO and LPS intensity, propagation, and precipitation, and associated underlying mechanisms.

The BSISO has a large impact on mean monsoon vorticity and rainfall as it moves northward – maximising both in phases 2-3 over southern India and phases 5-6 over northern India – but a much weaker relationship with total column water vapour. 
We present evidence that LPS genesis also preferentially follows these phases of the BSISO.
We identify significant relationships between BSISO phase and LPS precipitation and propagation: for example, during BSISO phase 5, LPSs over north India produce 51% heavier rainfall and propagate northwestward 20% more quickly.
Using a combination of moisture flux linearisation and quasigeostrophic theory, we show that these relationships are driven by changes to the underlying dynamics, rather than the moisture content or thermodynamic structure, of the monsoon.

Using the example of LPSs over northern India during BSISO phase 5, we show that the vertical structure of anomalous vorticity can be split into contributions from the BSISO background circulation and the nonlinear response of the LPS to anomalous BSISO circulation. Complementary hypotheses emerge about the source of this nonlinear vorticity response: nonlinear frictional convergence and secondary barotropic growth. We show that both are important. The BSISO imparts greater meridional shear on the background state, supporting LPS intensification. The BSISO background and nonlinear LPS response both contribute significantly to anomalous boundary layer convergence, and we show through vortex budget arguments that the former supports additional LPS intensification in boundary layer while the latter supports faster westward propagation.

This work therefore yields important insights into the scale interactions controlling one of the dominant synoptic systems contributing to rainfall during the monsoon.

How to cite: Hunt, K. and Turner, A.: Nonlinear intensification of monsoon low pressure systems by the BSISO, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-37, https://doi.org/10.5194/egusphere-egu23-37, 2023.

EGU23-49 | ECS | Posters on site | AS1.24

Subseasonal strength reversal of the East Asian winter monsoon 

Wogu Zhong and Zhiwei Wu

As one of the most significant circulation systems over the Northern Hemisphere in the cold season, the East Asian winter monsoon (EAWM) has been broadly investigated from the seasonal-mean perspective, while subseasonal variations in the EAWM still remain ambiguous. Based on Season-reliant Empirical Orthogonal Function (S-EOF) analysis, this study shows that the subseasonal strength reversal of the EAWM (SR-EAWM), featuring a weaker (or stronger) EAWM in early winter (December) and a stronger (or weaker) EAWM in late winter (January-February), is a distinct leading mode of the month-to-month variation of the EAWM. The weak-to-strong SR-EAWM is characterized by an anomalous low over Eurasia and a weakened East Asian major trough (EAT) in early winter, with an intensified Siberian High and a deepened EAT in late winter. The SR-EAWM is preceded by surface air temperature anomalies over Davis Strait (DST) and those over central-eastern North America (CENAT) in September-October. The DST mainly influences the SR-EAWM in early winter through a “sea ice bridge” of the November Baffin Bay sea ice concentration anomaly (BBSIC). The BBSIC could intensify the DST in December by altering surface heat flux, thus exciting a downstream atmospheric response and modulating the strength of the EAT in early winter. The preceding CENAT affects the SR-EAWM in late winter by inducing an “ocean bridge” of the western North Atlantic sea surface temperature anomaly (WNASST). The WNASST can persist into late winter and then significantly affects the SR-EAWM by regulating Eurasian circulation anomalies and the downstream EAT. The bridge roles of the BBSIC and WNASST can be further verified by a linear baroclinic model. Finally, two physical-empirical models are established using the DST/BBSIC and the CENAT indices, respectively. Both exhibit promising prediction skills. The results highlight that the DST, BBSIC, and CENAT are crucial predictability sources for the SR-EAWM.

How to cite: Zhong, W. and Wu, Z.: Subseasonal strength reversal of the East Asian winter monsoon, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-49, https://doi.org/10.5194/egusphere-egu23-49, 2023.

Understanding the natural variability of Indian summer monsoon (ISM) is a crucial aspect relevant for decadal climate predictions and climate change studies. The multidecadal variability of ISM is known to have a close association with the Atlantic multidecadal oscillations (AMO). Several teleconnection pathways have been suggested to explain the co-variability of the AMO and ISM in multidecadal timescales. One hypothesis is that the AMO modulates the interannual North Atlantic Oscillation (NAO) mode and there by influences the monsoon via Eurasian temperature modulations. Direct atmospheric teleconnection, across Eurasia, through upper-level circulation anomalies has also been attributed to the observed AMO-ISM relationship. Another possibility is the AMO modulating the monsoon via the Pacific pathway through the atmospheric bridge mechanism and associated modulations of the Hadley-Walker circulations. The Last millennium (LM) (851-1848) climate simulations part of the PMIP3/CMIP5 gives an opportunity to better understand the fidelity of climate models in capturing the AMO-ISM teleconnection mechanisms. In this study we explore how well the proposed mechanisms are represented in eight global climate models (GCM) LM simulations. Such a study, assessing the validity of different AMO-monsoon teleconnection mechanisms in different model climates provides crucial information about how reliable the respective GCMs may be in making decadal climate predictions.

How to cite: Dutta, A., Sivankutty, R., and Joseph Mani, N.: Investigating the Atlantic-Indian summer monsoon multidecadal teleconnections in the PMIP3/CMIP5 Last Millennium simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-191, https://doi.org/10.5194/egusphere-egu23-191, 2023.

EGU23-426 | ECS | Orals | AS1.24

Role of background moisture in dictating the Intraseasonal Rainfall over Bay of Bengal 

Aditya Kottapalli and Vinayachandran Pn

The northward propagating intraseasonal Oscillation (ISO) is one of the dominant modes of tropical variability during Boreal summers. Several mechanisms have been proposed to explain northward propagation. Yet the factors that decide the ISO rainfall over a particular region remains elusive. in this  study we show that the ISO rainfall anomalies weaken across the south Bay of Bengal (SBoB) before they re-strengthen over the north Bay of Bengal (NBoB). We use the moisture budget to understand the reason for the same. We find that the horizontal moisture flux convergence predominantly controls the ISO rainfall anomalies over the two regions. Further analyses reveal that the convergence of background moisture by the ISO wind perturbations decides the ISO rainfall structure. We hypothesize that the weaker rainfall anomalies in the SBoB result from the weaker background column relative humidity and moisture, which do not allow the initial dynamic perturbations to grow as fast as they do in an environment with stronger background relative humidity and moisture (NBoB). 

How to cite: Kottapalli, A. and Pn, V.: Role of background moisture in dictating the Intraseasonal Rainfall over Bay of Bengal, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-426, https://doi.org/10.5194/egusphere-egu23-426, 2023.

EGU23-436 | ECS | Orals | AS1.24

Role of thermodynamic processes in driving Monsoon Intraseasonal Oscillations (MISO) away from the Equator 

Rajat Masiwal, Vishal Dixit, and Ashwin K Seshadri

Monsoon intraseasonal oscillation (MISO) is an important aspect of the monsoon variability on various timescales, accounting for short-term variability as well as about 40% of total seasonal rainfall variance. MISO plays an important role in modulating the active (wet) and break (dry) spells of monsoon, and its low-frequency component has a time period of 30-60 days and exhibits northward propagation from the equatorial Indian Ocean to the Himalayan foothills. This northward propagation is generally attributed to generation of positive barotropic vorticity to the north of the previous convection centre. However, using ERA5 reanalysis composites we show that the relation between convection centre and positive barotropic vorticity undergoes significant change as MISO propagates away from the equator. Close to the equator (0-15°N), barotropic voriticty is either in-phase or leads rainfall, whereas further poleward (15°N-25°N), this relationship reverses and rainfall leads vorticity by 1-2 days. This contrast is closely tied to changes in the vertical structure of vorticity: near the equator, the vorticity maximum lies in the middle troposphere, while poleward of 15°N it is in the lower troposphere. The vorticity budget at each pressure level reveals the importance of vertical advection of vorticity for its near-barotropic structure, together with the importance of thermodynamic influences on vorticity, especially poleward where the vortex stretching term grows. Such findings point to the central role of feedback on the dynamics from the thermodynamic processes away from the equator. Furthermore, it closely ties the ability of models to reproduce MISO to their ability to represent convective processes.

 

How to cite: Masiwal, R., Dixit, V., and Seshadri, A. K.: Role of thermodynamic processes in driving Monsoon Intraseasonal Oscillations (MISO) away from the Equator, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-436, https://doi.org/10.5194/egusphere-egu23-436, 2023.

EGU23-546 | ECS | Posters on site | AS1.24

Precipitation and temperature variability in Vietnam during Marine Isotope Stage 3 from terrestrial biomarkers 

Trang Tran, Lora Stevens-Landon, Jessica Tierney, Patrick Murphy, and Tich Vu-Van

Southeast (SE) Asia is located in a transitional zone where hydroclimate is controlled by both the Indian and East Asian summer monsoon branches. Recent proxy-based studies and climate models suggest that the hydroclimate of SE Asia may be out of phase with neighboring regions, such as India and China. However, we lack sufficient proxy records to verify this postulation or to identify spatial and temporal variations. This study reconstructs both past temperatures and effective moisture in Central Vietnam during Marine Isotope Stage 3 (approximately 50,00 to 30,000 years BP) to determine how these two climate variables relate in the past. Terrestrial temperatures and precipitation are reconstructed using biomarkers (branched glycerol dialkyl glycerol tetraethers, brGDGT) and compound-specific isotope analyses (carbon and hydrogen-isotopic values of leaf wax n-acids, δ13Cwax, and δDwax) from a buried peat deposit in the Central Highlands of Vietnam. The brGDGTs-derived annual temperatures range from 22.9 to 26.2°C and show a warming trend coincident with a weakening of summer insolation. A coincident and gradual enrichment of δ13Cwax from 47 to 33 kyr BP suggests a transition from C3 to C4 vegetation dominance. Such a response could signal an overall decrease in precipitation or a shift in the seasonality of precipitation. The δDwax data, however, do not indicate an overall drying trend, which supports the idea that a shift in the seasonality of rainfall, along with higher annual temperatures, is driving the vegetation change. In addition, the δDwax records may exhibit a trend opposite to a site in Thailand. We argue that the isotopic variability in the precipitation of Central Vietnam reflects the shift in moisture sources along with the shift in seasonality. In this case, an increase in amount of precipitation derived from the South China Sea in winter months is marked by rain enriched in δ2H-which could also be interpreted as a decrease in precipitation. The increase in rainfall during winter monsoon months (e.g. winter) in the Central Highlands of Vietnam does not appear to reach Thailand. We recommend that the precipitation proxies should be applied with knowledge of regional climate context and argue that better geographic representation of monsoonal climates is necessary to fully understand and model this critical climate system.

How to cite: Tran, T., Stevens-Landon, L., Tierney, J., Murphy, P., and Vu-Van, T.: Precipitation and temperature variability in Vietnam during Marine Isotope Stage 3 from terrestrial biomarkers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-546, https://doi.org/10.5194/egusphere-egu23-546, 2023.

EGU23-658 | ECS | Posters on site | AS1.24

The complexity of South China Sea summer monsoon onset 

Tian Ma and Weidong Yu

The complexity of the South China Sea (SCS) summer monsoon (SCSSM) onset is mainly reflected in the interaction of multiscale processes that include the seasonal cycle, 10-25-day ISO (HISO), 30-60-day ISO (LISO). In this study, the characteristics and mechanism of the HISO and LISO and their interaction with the background field are investigated when they trigger the SCSSM onset base on newly released reanalysis and remote sensing data for the period of 1979–2020.

The SCSSM onsets always are triggered by the second westward HISO or first northward LISO when the control of subtropical high pressure weakens on the SCS. The first HISO can be seen as a signal that the control is weak enough, and the SCSSM is about to onset. The SCSSM can also be established without the effects of the HISO or LISO, but the date would be put off. Based on the budget analysis of column-integrated moist static energy (MSE), the interaction between the easterly trade winds and the zonal gradient of MSE anomalies is considered the dominant reason for the HISO that can successively propagate westward from the western North Pacific. The SSTa-induced turbulent heat flux and the interaction between the mean southerly and the meridional gradient of the MSE anomaly are both important for the northward LISO from the equatorial Indian Ocean when it triggers the SCSSM onset. For the simulation and forecasting of the SCSSM onset, we put more emphasis on the role of the HISO because it is a more active process.

How to cite: Ma, T. and Yu, W.: The complexity of South China Sea summer monsoon onset, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-658, https://doi.org/10.5194/egusphere-egu23-658, 2023.

The study addresses the role of climate change on the interaction between the Indian Summer monsoon rainfall (ISMR) and western north Pacific (WNP) convective activities. We have examined two high-resolution climate model simulations, with and without anthropogenic forcing (i.e., HIST and HISTNAT), using a variable resolution model. The study is supplemented by detailed diagnostics and innovative techniques like causal network analysis which bring out the interaction of convective activities between the two regions which is altered by the influence of anthropogenically forced climate change. Our results shows that the weakening of ISMR re-orient the cross-equatorial winds along with large-scale moisture transport towards the western tropical Pacific which significantly increase the genesis potential index (GPI) over the region by 9.6%. Further we noted the probability of the occurrence of extremely low sea-level pressure (SLP) i.e., SLP < 995.5 hPa around areas near Taiwan and part of Chinese mainland is significantly higher by 10.3 % in the HIST simulation as compared to that of HISTNAT. The use of causal effect network analysis showed a significant causative link between the Indian monsoon circulation index (IMI), WNP tropical cyclone activity (GPI) and winds over the tropical Indo-Pacific (IPWND). The results show a weakening of the IMI can lead to possible enhancement of GPI and IPWND, with a certain time-lag. It is noteworthy to mention that the time lag of interaction between the IMI, GPI and IPWND are different in the two simulations with a significantly shorter time scales in HIST (~ 5 days) compared to that of HISTNAT where it is significantly larger (>20 days).

How to cite: Sagar, A., Krishnan, R., and Sabin, T. P.: Weakening of South Asian monsoon circulation and its interaction with western north Pacific tropical convective activities in a changing climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-696, https://doi.org/10.5194/egusphere-egu23-696, 2023.

EGU23-715 | Orals | AS1.24

CMIP6 projections of the South American Monsoon Lifecycle: comparison with pre and post statistical downscaling 

Michelle Reboita, Glauber Ferreira, and João Gabriel Ribeiro

The climate of a great part of South America presents two well-defined seasons: one dry, in general, from April to September, and another wet, from October to March, which characterizes a monsoon regime. As most of the energy generation in this monsoon region is hydroelectric, precipitation is a target of several studies. In this context, the South America Monsoon (SAM) lifecycle (onset, demise, and duration) in projections of eight global climate models (GCMs) of the Coupled Model Intercomparison Project Phase 6 (CMIP6) is analyzed in this study using two approaches: (a) the original GCM outputs downloaded from the Earth System Grid Federation (ESGF) and (b) after application of the statistical downscaling (SD) technique. Daily precipitation data from the Climate Prediction Center (CPC), with a horizontal resolution of 0.5o, are used as a reference. So, the final resolution of the GCMs after applying the Quantile Delta Mapping (QDM) is the same as CPC. SAM lifecycle is identified with a similar methodology from Liebman and Marengo published in 2001, which is based on the accumulated daily precipitation anomalies. The rainy season is considered to be the period during which precipitation exceeds its climatological annual average, then a positive slope indicates the rainy season. Note that this methodology is proper to be applied in projections because it does not assume any threshold. Initial results indicate a shorter lifetime of SAM at the end of the century.  The authors thank the Programa de P&D regulado pela ANEEL: empresa Engie Brasil Energia e Companhia Energética Estreito, MC&E, FAPEMIG, CAPES and CNPq for the financial support.

How to cite: Reboita, M., Ferreira, G., and Ribeiro, J. G.: CMIP6 projections of the South American Monsoon Lifecycle: comparison with pre and post statistical downscaling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-715, https://doi.org/10.5194/egusphere-egu23-715, 2023.

In this study, we present the results of a regional model (regional spectral model-regional ocean model [(RSM-ROMS]) simulation of the South Asian Summer Monsoon (SASM). The RSM-ROMS integration is carried out at 20 km grid spacing over a period of 25 years (1986–2010). The simulation is forced by global atmospheric and oceanic reanalysis. The RSM-ROMS simulation shows a realistic alignment of the simulated rainfall along the orographic features of the domain. Furthermore, the RSM-ROMS simulates the observed feature of convection over continental SASM region being more vigorous with dominance of mixed warm and cold phase hydrometeors in contrast to the dominance of the warm rain process in the neighboring tropical oceans. Similarly, the upper ocean features of contrasting mixed layer and thermocline depths between the northern and equatorial Indian Ocean are also simulated in the RSM-ROMS. Intra-Seasonal Oscillation (ISO) of the SASM at 10–20 and 20–70 days are also simulated in the RSM-ROMS with many of its features verifying with observations. For example, the 20–70 days ISO are of higher amplitude and its meridional propagation is slower in Bay of Bengal compared to that over Arabian Sea. Additionally, RSM-ROMS shows 12.3 Monsoon Low Pressure Systems (LPSs) per season that is comparable to 14.6 per season from observations. Furthermore, the observed intraseasonal contrasts of LPS between the wet and dry spells of ISO is also reproduced in the RSM-ROMS.

How to cite: Misra, V. and Jayasankar, C. B.: Dynamic Downscaling the South Asian Summer Monsoon From a Global Reanalysis Using a Regional Coupled Ocean-Atmosphere Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1014, https://doi.org/10.5194/egusphere-egu23-1014, 2023.

Tibet plateau plays very crucial roles in globle climate system, and the precipitation is  one of the main factors in Tibet plateau climate system, Based on GPCC monthly precipitation data and ERA5 monthly precipitation reanalysis data from 1961 to 2016, this study analyzes the spatio-temporal distribution and evolution of plateau precipitation during the May-September monsoon period under the background of global warming. Try to analyze the mechanism reason affecting precipitation variation in different regions. The precipitation in the South part of Tibet plateau began to increase in May, and advance to the northwest part of Tibet plateau during the July and August, and began to back to the south in September. According to The decomposition of the empirical orthogonal function (EOF), we divided the Tibet plateau into north and south two parts by the mount tunggula, on the interannual variability, percentage of precipitation in the monsoon plateau exists reverse change relation, precipitation showed a trend of slight decrease in the south part of plateau, plateau in northern precipitation shows ascendant trend on decadal scale, rate of precipitation in the plateau there are shocks between 3 to 5 years in 7-9 or 11 years. There is a north-south inverse change rate in the precipitation in the plateau during the monsoon period. The analysis of the relationship between the monthly precipitation data and the atmospheric circulation in the south and north of the Plateau shows that the precipitation in the south of the Plateau is affected by the South Asian monsoon, while the precipitation in the north of the plateau is related to the Rossby wave of the subtropical westerly jet. In other words, the precipitation in the southern part of the plateau is mainly controlled by summer risk, while the precipitation in the northern part of the plateau is affected by subtropical westerly winds.

 

Keyword: Tibetan Plateau,Precipitation,Circulation,South asia monsoon,Jet stream

How to cite: Wang, H. and Hu, Z.: The North-South variation and mechanism of the precipitation over the Tibetan Plateau during the monsoon in the past 60 years, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1193, https://doi.org/10.5194/egusphere-egu23-1193, 2023.

EGU23-2011 | Posters on site | AS1.24

Increased intra-seasonal variability in Indian summer monsoon precipitation in a warming climate 

Sukumaran Sandeep and Neelesh Kumari

The characteristics of Indian summer monsoon (ISM) precipitation have been changing in a warming climate. We examined the intra-seasonal variability of daily mean ISM rainfall over central India in 20 CMIP6 models. The daily precipitation variance is found to have increased in the last 20 years of SSP585 runs compared to the 1981 – 2000 period of historical all forcing simulations. The mean ISM precipitation also shows an increase in the same period. The future changes in seasonal mean precipitation and the intra-seasonal variance in daily precipitation with respect to the historical period are scaled with the corresponding change in the surface temperature over the ISM domain. The changes in the seasonal mean precipitation do not show any significant relationship with the surface temperature change. However, the changes in the daily variance of ISM precipitation scale linearly with the changes in temperature. These results suggest that the ISM precipitation will become more erratic in a warming environment.

How to cite: Sandeep, S. and Kumari, N.: Increased intra-seasonal variability in Indian summer monsoon precipitation in a warming climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2011, https://doi.org/10.5194/egusphere-egu23-2011, 2023.

EGU23-2025 | Orals | AS1.24

Processes controlling the South American Monsoon response to Climate Change 

Robin Chadwick, Jorge Garcia-Franco, and Lincoln Alves

CMIP6 future climate projections consistently show a drying trend during the onset of the South American monsoon, which has the potential for large ecological and societal impacts in this region. This trend is also present in a high-resolution regional convection-permitting simulation over the South American domain. Here, the processes responsible for this drying trend are examined using a number of idealised experiments and analysis techniques. The main driver is shown to be remote sea surface temperature (SST) warming - rather than local radiative or plant physiological responses to increased CO2 - with both large-scale uniform SST warming and patterned regional warming playing important roles. The role of uniform SST warming on the South American monsoon onset is examined in more detail using a moist static energy budget approach, building on hypotheses from a previous single model study. The atmospheric circulation response to patterned SST warming is examined using a local overturning circulation partioning technique, allowing a link between the South American monsoon region and specific regions of ocean warming to be identified.

How to cite: Chadwick, R., Garcia-Franco, J., and Alves, L.: Processes controlling the South American Monsoon response to Climate Change, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2025, https://doi.org/10.5194/egusphere-egu23-2025, 2023.

Monsoon influences the well-being of billions of people in tropical and subtropical regions. The accelerated climate change and monsoon coupling with other large-scale climatic phenomena make their prediction challenging. Therefore, improvement in understanding and prediction of monsoons has become essential. Recent studies have emphasized the role of arctic region in influencing the tropical climate and its potential to cause more persistent extreme events. Therefore, it is imperative to explore the arctic region for its strategic advantage and combat climate change. In this direction, our work aims to unravel the association between the Arctic region and the Indian summer monsoon (ISM). We quantify the influence of the Arctic region on Indian summer monsoon rainfall (ISMR) using statistical parameters. The sea ice extent and Arctic Oscillation Index were correlated with the precipitation in India at seasonal and monthly scale. The Arctic Oscillation index was able to explain around 7-10% of variability in precipitation. The increased magnitude and frequency of precipitation in India are significantly related to decreased sea ice extent indicated by negative correlation coefficient ranging from 0.3-0.6.

How to cite: kulkarni, S. and Agarwal, A.: Unraveling the association between artic region and Indian summer monsoon – an empirical study, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2111, https://doi.org/10.5194/egusphere-egu23-2111, 2023.

EGU23-2159 | ECS | Posters virtual | AS1.24

Climatic effects of the Indian Ocean tripole on the western United States in boreal summer 

Yazhou Zhang and Jianping Li

The Indian Ocean tripole (IOT) is an independent mode of ocean–atmosphere circulation centered on the tropical Indian Ocean. This study explores the physical mechanisms of the IOT affecting the western United States climate variation during the boreal summer. We find that the IOT is significantly correlated with both western United States summer surface temperature and precipitation anomalies. During positive IOT events, the westerly wind anomalies over the northern Indian Ocean are intensified by two cross-equator airflows over the tropical eastern Indian Ocean and the east coast of Africa. The resulting convergence of air over the northern Bay of Bengal–Indochina Peninsula–northern South China Sea (NBB–IP–NSCS) region (80°–125°E, 15°–25°N) exacerbates the surplus precipitation there. Serving as a heat source, these NBB–IP–NSCS precipitation anomalies can excite a circum-global teleconnection-like (CGT–like) pattern that propagates eastward from west-central Asia towards North America along the Asia subtropical westerly jet, further influencing local circulation anomalies. Development of strong anticyclonic circulation over the western United States enhances descending motion and divergence there, resulting in negative precipitation anomalies. This circulation anomaly also induces the diabatic heating anomalies through allowing more solar radiation to reach the ground surface, further increasing the surface temperature anomalies. Meanwhile, the increased tropospheric temperature also raises local surface temperatures by modulating the adiabatic air expansion and compression. Ultimately, the CGT-like pattern associated with NBB–IP–NSCS precipitation anomalies sets up an atmospheric bridge by which the IOT can impact summer climate in the western United States.

How to cite: Zhang, Y. and Li, J.: Climatic effects of the Indian Ocean tripole on the western United States in boreal summer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2159, https://doi.org/10.5194/egusphere-egu23-2159, 2023.

EGU23-2322 | ECS | Orals | AS1.24

Extratropical Stratospheric Air Intrusions Over the Western North Pacific and the Genesis of Downstream Monsoon Low-Pressure Systems 

Vishnupriya Selvakumar, Suhas Ettamal, and Sandeep Sukumaran

Low-pressure systems (LPS) are convectively coupled vortices that contribute nearly half of the summer monsoon rainfall over the Indian subcontinent. About one-third of the boreal summer monsoon LPS are caused by downstream amplification of westward propagating disturbances from the western North Pacific (WNP). Analysis of downstream LPS events from 1979 to 2017 reveals that 43% of them are caused by extratropical stratospheric air intrusions over the WNP. Stratospheric air intrusions lead to high tropospheric potential vorticity (PV), and the downstream vortex seeds are observed to initiate and intensify to the southwest of the PV anomalies. The PV anomalies can deform the temperature in its neighborhood and cause adiabatic lifting, which in turn can induce and intensify low-level cyclonic vortices. The subsequent intensification of the low-level vortex is aided by deep convection, observed to the southwest of the PV anomaly, through vortex stretching and low-level PV generation by diabatic heating.

How to cite: Selvakumar, V., Ettamal, S., and Sukumaran, S.: Extratropical Stratospheric Air Intrusions Over the Western North Pacific and the Genesis of Downstream Monsoon Low-Pressure Systems, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2322, https://doi.org/10.5194/egusphere-egu23-2322, 2023.

EGU23-2469 | ECS | Orals | AS1.24

Australian Summer Monsoon Bursts: A Moist Static Energy Budget Perspective 

Sarthak Mohanty, Christian Jakob, and Martin Singh

The Australian monsoon's wet season is associated with sequences of wet and dry conditions known as bursts and breaks, which usually have timescales of a week or two. There are several hypotheses for the physical processes involved in monsoon bursts, ranging from the effects of the Madden-Julian Oscillation to extratropical influences.

We analyse rainfall bursts in Northern Australia using a moist static energy (MSE) budget framework. First, we separate the bursts into pre-monsoon, monsoon, and post-monsoon based on simple monsoon onset and retreat criteria. We then apply ERA5 data to calculate the MSE budget for each burst and construct composite bursts for each of the three types.

We find that the horizontal advection of MSE over the tropical northern Australian convergence zone is the most critical term in the budget for the day-to-day precipitation variation. An analysis of the MSE-related gross moist stability (GMS) reveals that the GMS framework is able to predict periods of convective growth and decay before and after monsoon bursts, with the exception of the pre-monsoon bursts which do not follow the characteristic evolution of tropical convective systems. We hypothesise that this is because pre-monsoon bursts have a stronger extratropical influence. We find that the growth phase of convection in monsoon and post-monsoon bursts is associated with a notable reduction of the advection of dry air into the monsoon region. We show that this is likely the result of a rearrangement of the circulation ahead of the burst.  

How to cite: Mohanty, S., Jakob, C., and Singh, M.: Australian Summer Monsoon Bursts: A Moist Static Energy Budget Perspective, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2469, https://doi.org/10.5194/egusphere-egu23-2469, 2023.

EGU23-2580 | ECS | Orals | AS1.24

Land evaporation biases link to East Asian rainfall shifts across AMIP simulations 

Ruth Geen, Marianne Pietschnig, Shubhi Agrawal, Dipanjan Dey, F. Hugo Lambert, and Geoffrey Vallis

State-of-the-art models show significant climatological biases in their simulation of East Asian Summer Monsoon (EASM) rainfall, with biases even more pronounced in atmosphere-only simulations versus simulations with a coupled-ocean. It has further been noted that systematic evapotranspiration biases occur locally over East Asia, and globally over land, in simulations both with and without a coupled ocean. Here, we explore a possible role for evapotranspiration in EASM precipitation biases.

Idealized model simulations are presented in which the parameterization of land evaporation is modified. The results suggest a feedback whereby excessive evapotranspiration over East Asia can result in cooling of land, a weakened monsoon low, and a shift of rainfall from the Philippine Sea to China, moistening land and further fueling evapotranspiration. Cross-model regressions against evapotranspiration over China indicate that a similar pattern of behavior is seen in Atmosphere Model Intercomparison Project (AMIP) simulations.

In AMIP, the feedback is not explained by a too-intense global hydrological cycle or by differences in radiative processes. Analysis of land-only simulations indicates that evapotranspiration biases are present even when models are forced with prescribed meteorological conditions. These biases are strengthened when the land model is coupled to the atmosphere, suggesting a role for land-model errors in driving atmospheric biases. Coupled atmosphere-ocean models are shown to have similar evapotranspiration biases to those in AMIP over China, but different precipitation biases, including a northward shift in the Intertropical Convergence Zone over the Pacific and Atlantic oceans.

How to cite: Geen, R., Pietschnig, M., Agrawal, S., Dey, D., Lambert, F. H., and Vallis, G.: Land evaporation biases link to East Asian rainfall shifts across AMIP simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2580, https://doi.org/10.5194/egusphere-egu23-2580, 2023.

EGU23-3466 | Posters on site | AS1.24

Understanding changes in West African monsoon precipitation in response to increased CO2 

Harry Mutton, Robin Chadwick, Matthew Collins, and Hugo Lambert

Projections of future West African monsoon (WAM) precipitation change in response to increased greenhouse gases are uncertain, and an improved understanding of the drivers of WAM precipitation change is needed to help aid model development and better inform adaptation policies in the region. Here, we address two of these drivers: the direct radiative effect of increased CO2 (referring to the impact of increased CO2 in the absence of SST changes), and the impact of a uniform SST warming. Atmosphere only models are used to investigate the response, finding that these two drivers have opposing impacts on WAM precipitation. In response to the direct radiative effect, an increase in precipitation is caused by a northward shift and a weakening of the shallow meridional circulation over West Africa, advecting less dry air into the monsoon rainband. In contrast, the uniform SST warming causes a decrease in precipitation due to a strengthening of the shallow meridional circulation and enhanced moisture gradients between the moist monsoon airmass and the dry desert airmass. These changes in the shallow meridional circulation are shown to be caused by large scale temperature changes as well as the more localised impact of a soil moisture feedback mechanism over the Sahel. It is then shown that the processes discussed are relevant to the intermodel uncertainty in WAM projections across a range of CMIP6 models.

How to cite: Mutton, H., Chadwick, R., Collins, M., and Lambert, H.: Understanding changes in West African monsoon precipitation in response to increased CO2, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3466, https://doi.org/10.5194/egusphere-egu23-3466, 2023.

EGU23-3747 | ECS | Orals | AS1.24

Impact of vegetation on the boreal summer monsoon precipitation over India: an energetics viewpoint. 

Jerry B Samuel, Arindam Chakraborty, and Anagha Paleri

The heterogeneities arising out of surface variabilities, land-sea contrasts, aerosol concentrations, and the influence of orography define the intricate characteristics of regional monsoon systems. The amount of precipitation India receives during the boreal summer monsoon season can be modulated by land surface processes due to its influence on moisture availability and atmospheric stability. This study investigates the impact of vegetation changes on the seasonal mean precipitation over Indian land using fully coupled global climate model (GCM) simulations with idealized land cover. In addition, an  energetics framework is employed to unravel the physical mechanisms/pathways connecting vegetation and rainfall. In general, evaporation enhances with an increase in forest cover. However, this does not translate to a similar increase in all-India averaged precipitation. Using the energetics approach, we find that precipitation changes primarily happens via three different thermodynamic pathways. We also find the regions where each pathway is dominant. The relative dominance of these pathways in various areas leads to spatial inhomogeneities in the precipitation response due to vegetation changes. Human intervention, including agricultural expansion, has reshaped the landscape of India in the last century, altering the nature of land-atmosphere interactions. The results from this study, that land cover plays a significant role in modulating the regional characteristics of seasonal monsoon precipitation, are particularly important in this context. The findings in this study also have broader ramifications since the dominant region-specific mechanisms identified are expected to be valid for other forcings and are not just limited to the scenarios considered here. A unified framework connecting these various forcings with monsoon variability would be of great practical importance, and the present study is an advancement in this regard.

How to cite: Samuel, J. B., Chakraborty, A., and Paleri, A.: Impact of vegetation on the boreal summer monsoon precipitation over India: an energetics viewpoint., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3747, https://doi.org/10.5194/egusphere-egu23-3747, 2023.

The Indo-Pacific warm pool (IPWP) is enclosed by a 28 ◦C isotherm and plays a vital role in controlling tropical circulations. However, the effects of changes in regional warm pool sea surface temperatures (SSTs) on the circulations remain unexplored. To do this, we divided the IPWP into the Indian and Pacific sectors and distinguished their responses to natural variability and global warming. And then, we examined the impacts of the interannual variability (IAV) in warm pool SST on the tropical Hadley, Walker, and monsoon circulations. The Hadley circulation was affected by warm pool SST warming, i.e., warmer SSTs over the warm pool strengthened the upward branch of Hadley circulation, whereas the downward branch was weakened and strengthened in the Northern and Southern Hemispheres. Walker circulation was strengthened (weakened) in the warming (natural) mode. Consequently, the Walker circulation is weakened since the natural variability of warm pool SST plays a more dominant role than the warming trend of SSTs over the warm pool. It is notable that warm pool warming has little impact on monsoon circulation. Our findings highlight the different roles of the IAV of warm pool regions in each tropical circulation as part of the warming trend and natural variability. Furthermore, an increase in precipitation is limited up to a specific SST, although SST becomes warmer. We defined this specific SST as Saturation Threshold SST (STT). Under a warming climate, future changes in STT over the IPWP and its mechanism will be shortly shown in this presentation.

How to cite: Kim, H.-R. and Ha, K.-J.: Impact of the Indo-Pacific Warm Pool on the Tropical Circulations and Changes in Saturation Threshold SST, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4743, https://doi.org/10.5194/egusphere-egu23-4743, 2023.

The Himalayas are an essential driver of the monsoon and climate system. However, river flooding during the monsoon impacts the most densely populated region of Himalayan downstream regions annually. Previous studies also reported elevation-dependent warming, rainfall changes, ice-sheet melting, and extremes in the Himalayas. Nevertheless, due to complicated orography, Himalayan precipitation dynamics remain quantitatively limited on a spatial scale compared to other monsoon regions. In the context of climate change, recent studies show how melting glaciers and snow, along with monsoonal rains causing recurrent floods, play a role. This study examined the last 43 years (1979-2021) to emphasize the interannual variability. We found a robust signal over in the Eastern Himalayas, where the orographic features and process plays a dominant role. Further analysis indicates Monsoonal rainfall is the main factor, rather than melting snow for these unusually extreme years. Regional monsoonal circulation connected to Walker circulation controls the variability of Himalayan monsoonal rainfall via circulation linkages. Our findings illustrate the wet and dry response mechanisms in the eastern Himalayas. The conclusions are drawn from this work highlight the role of natural variability, which might help understand Himalayan floods and their predictability.

 

Keywords Himalayas, Interannual variability, Monsoon dynamics, Orographic features, River floods

How to cite: Kad, P. and Ha, K.-J.: Dynamics and characteristics of monsoonal orographic rainfall variability over Eastern Himalaya, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4950, https://doi.org/10.5194/egusphere-egu23-4950, 2023.

The changes in the Indian summer monsoon rainfall under anthropogenic climate change would have a large socio-economic impact. The thermodynamic effect of the climate change on future monsoon rainfall is well understood with an overall increase in precipitation as the atmosphere moistens. Understanding the dynamical effect of climate change especially from the changes in the drivers of the monsoon remains challenging. Here we show that the observed western Indian monsoon rainfall has an increasing trend over the last 120 years. We find this observed trend is connected with the trend in the tropical Pacific zonal sea surface temperature (SST) gradient, where the western tropical Pacific or the warm pool region of the Pacific Ocean is warming faster than the eastern side. Applying a storyline approach to the future evolution of the zonal tropical Pacific SST gradient in 38 global climate models from the latest Coupled Model Intercomparison Project phase 6, we find a consistent connection in the models between the western Indian monsoon rainfall change and the strength of the change in the zonal tropical Pacific SST gradient under global warming. The models which warm more in the western compared to the eastern side of the tropical Pacific have higher rainfall increases over western India during the monsoon season. This link is associated with an anomalous easterly wind coming from the western tropical Pacific and converging over western India, leading to higher rainfall in both observations and models. This result suggests that future changes in the western Indian monsoon rainfall would depend on the changes in the strength of the zonal gradient of the tropical Pacific Ocean SST.

How to cite: Ghosh, R. and Shepherd, T. G.: Strengthening tropical Pacific zonal temperature gradient linked with increasing West Indian Monsoon rainfall, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5985, https://doi.org/10.5194/egusphere-egu23-5985, 2023.

EGU23-6151 | Posters on site | AS1.24

Response of the Indian monsoon to a warming Indian ocean 

Bidyut Bikash Goswami

The Indian summer monsoon rainfall (ISMR) has been declining since the middle of the last century. However, recently (since about 2002) it is reported to have revived. For these observed changes in the ISMR, several explanations have been reported. Among these explanations, the warming of the Indian Ocean is considered a major one. However, we still do not fully understand the response of the atmosphere to this warming. Here we report that warming in the Indian Ocean (focusing on the eastern side of it where the sea surface temperatures are climatologically very warm) drives atmospheric responses that oppose Indian summer monsoon circulation and reduces ISMR. 

How to cite: Goswami, B. B.: Response of the Indian monsoon to a warming Indian ocean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6151, https://doi.org/10.5194/egusphere-egu23-6151, 2023.

EGU23-6573 | Orals | AS1.24

Why is there a systematic bias in the Asian Monsoon in the Met Office Unified Model? 

Kalli Furtado, Gill Martin, David Sexton, John Rostron, and Paul Field

Many global-climate models have substantial biases in their predictions of the Asian monsoon. For example, the Met Office Unified Model predicts a  monsoon trough that is too zonal and therefore underestimates summer rainfall over south and east Asia. These errors have persisted over many cycles of research-to-operations, and appear robust to significant developments in all major parametrizations in the model. Here, we address a simple question: why are these biases systematic? That is, why have they not been removed by optimization of parameters in the model's physics? Using a Perturbed Parameter Ensemble of AMIP simulations, we show that a strong constraint exists which prevents the Unified Model from simultaneously producing an unbiased monsoon and unbiased global top-of-atmosphere radiation fluxes. We use this constraint to define a scalar parameter, the "structural bias"  of the ensemble, the magnitude of which measures the conflict between the constraints and therefore how "untunable" the model is. We identify the drivers of this parameter, show that it is related to an inability to independently affect the properties of tropical and extra-tropical clouds, and suggest ways in which it could be reduced in future model versions.

How to cite: Furtado, K., Martin, G., Sexton, D., Rostron, J., and Field, P.: Why is there a systematic bias in the Asian Monsoon in the Met Office Unified Model?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6573, https://doi.org/10.5194/egusphere-egu23-6573, 2023.

EGU23-6671 | ECS | Orals | AS1.24

Boreal Summer Intraseasonal Oscillation extreme rainfall propagation modulated by Pacific sea surface temperatures 

Felix Strnad, Jakob Schlör, Ruth Geen, Niklas Boers, and Bedartha Goswami

Intraseasonal variability of extreme rainfall events (EREs) during the South Asian Summer Monsoon season is dominated by the Boreal Summer Intraseasonal Oscillation (BSISO). However, deviations from its canonical north-eastward propagation are poorly understood, posing challenges to the prediction of EREs and climate modeling. Here, we combine a climate network-based approach determining regions of synchronously occurring EREs with
a clustering analysis of zonal and meridional BSISO propagation patterns which reveals three distinct modes: canonical north-eastward, eastward-blocked, and stationary propagation. We show that Pacific sea surface temperature background states determine the propagation mode. In particular, El Niño (La Niña)-like conditions favor the stationary (eastward-blocked) mode by modifying the zonal and meridional overturning circulation structures and the strength of the BSISO Kelvin wave component. The uncovered mechanism for BSISO diversity has implications for the predictability of large, spatially extensive EREs in South Asia and the development of early warning signals on a time horizon of 3-5 weeks.

How to cite: Strnad, F., Schlör, J., Geen, R., Boers, N., and Goswami, B.: Boreal Summer Intraseasonal Oscillation extreme rainfall propagation modulated by Pacific sea surface temperatures, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6671, https://doi.org/10.5194/egusphere-egu23-6671, 2023.

EGU23-7258 | Orals | AS1.24

Uncertainty in Sahel precipitation change: a storyline approach 

Paul-Arthur Monerie, Michela Biasutti, Juliette Mignot, Elsa Mohino, Benjamin Pohl, and Guiseppe Zappa

Future changes in Sahel precipitation are uncertain because of large differences between projections of various climate models. We assess the effect of climate change on Sahel precipitation in summer and for the end of the 21st century. We show that uncertainty in Sahel precipitation is associated with uncertainty at simulating future changes in surface air temperature over the northern Hemisphere. We point out the Atlantic Ocean and Euro-Mediterranean surface air temperature as drivers of the Sahel precipitation change uncertainty. We use a storyline approach, a statistical method, to construct scenarios of changes in Sahel precipitation, whose differences only depend on future changes in Atlantic Ocean and Euro-Mediterranean surface air temperature. We show that uncertainty in changes in Atlantic Ocean and Euro-Mediterranean surface air temperature explains up to 50% of Sahel precipitation change uncertainty. The approach also allows selecting models to better understand uncertainty in Sahel precipitation change, focusing on the mechanisms at play. We suggest that reducing uncertainty in the future warming of the North Atlantic and the Euro-Mediterranean areas would then allow reducing uncertainty in future changes in Sahel precipitation.

How to cite: Monerie, P.-A., Biasutti, M., Mignot, J., Mohino, E., Pohl, B., and Zappa, G.: Uncertainty in Sahel precipitation change: a storyline approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7258, https://doi.org/10.5194/egusphere-egu23-7258, 2023.

It has been argued in recent studies that the source of dry air originating over the desert regions of the West Asia i.e. Middle East intrudes over the continental India during the boreal summer resulting in more prolonged dry spells over India. Singh and Sandeep (2021, Clim Dyn) showed the existence of a huge reservoir of moist deficit air over the northern Arabian Sea at 850-hPa. In addition to this, it has been argued that low level jet undergo weakening and broadening prior to monsoon break phase in feedback to an increased barotropic instability. Furthermore, the monsoon low-level jet which transports the moisture to the continental landmass in the active phase acts as a main carrier in transporting this dry air towards the continental India during the break phase of the summer monsoon. In order to investigate the thermodynamic effects of dry air intrusion activity during dry phases of the Indian Summer Monsoon (ISM), isentropic analysis is performed on climate models simulations of Coupled Model Intercomparison Project Phase 6 (CMIP6). Here, we analyze the specific humidity and wind fields at 316 K isentropic level. The negative specific humidity anomalies of multi models average (MMA) signifies the pattern of dry air advection which shows that a large fraction of the moisture deficit is being transported to the continental India from the northern Arabian Sea, and only a small contribution comes from West Asia. The lead-lag composites of anomalous wind vectors and relative vorticity of MMA at 316 K isentrope clearly show a weakening of the monsoon circulation associated with the break conditions. The anomalous anti-cyclonic circulation pattern propagates westwards from the Bay of Bengal which is a well known feature of the monsoon break spells.  

KEYWORDS: Low level jet; Dry air intrusion; Indian Summer Monsoon 

How to cite: Singh, R. and Sandeep, S.: A thermodynamical study of dry air intrusion activity over India during dry phases of summer monsoon in CMIP6 models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7948, https://doi.org/10.5194/egusphere-egu23-7948, 2023.

EGU23-8550 | ECS | Posters on site | AS1.24

Indian Ocean heat transport and its role in developing SST pattern in the post-monsoon season in CMIP6 models 

Rajendran Saran and Sukumaran Sandeep

The cross-equatorial oceanic heat transport (OHT) in the Indian Ocean during boreal summer is an integral component of the Indian summer monsoon (ISM). This OHT is believed to be a crucial factor in the interannual variability of ISM. Thus, a deeper understanding of OHT in climate model simulations is needed for the understanding of the simulated interannual variability of monsoon. Here we examine the Indian Ocean meridional OHT and how the OHT in the summer monsoon season impacts the development of SST patterns in the post-monsoon season. Our results show that the post-monsoon SST positively correlates with OHT during the summer monsoon in western IO and negatively correlates in the southeastern Indian Ocean. Further, it reveals that the OHT during summer monsoon explains the dipole pattern of SST in the post-monsoon over the equatorial Indian Ocean. This study also investigates how anomalous OHT during monsoon months contributes to the persistence of marine heat waves (MHW) in the post-monsoon season. Both CMIP6 models and observations suggest enhanced and persistent MHWs in the post-monsoon season are linked to stronger OHT during the summer season.

How to cite: Saran, R. and Sandeep, S.: Indian Ocean heat transport and its role in developing SST pattern in the post-monsoon season in CMIP6 models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8550, https://doi.org/10.5194/egusphere-egu23-8550, 2023.

EGU23-9295 | Posters on site | AS1.24

Mid-Latitude Controls on Monsoon Onset and Progression (the MiLCMOP project) 

Andrew Turner, Ambrogio Volonte, and Marlene Kretschmer

The Indian monsoon is critical since it supplies most of the water for drinking, sanitation, industry and agriculture for a billion people.  The onset of monsoon typically starts in southern India by 1 June, taking up to 6 weeks to cover the country.  Meanwhile, during the monsoon, variations on time scales of a week or more give rise to periods of excess and reduced rainfall, known as active and break events.

Being able to better predict the onset of the rains, their progression, and of active and break events in the monsoon would be of great.  The timing of monsoon onset is already known to be influenced by tropical variability such as the Madden-Julian Oscillation.  New research has shown that the mid-latitudes also exert a powerful control, but the full extent of this extratropical role in monsoon onset progression and in the timing of active and break periods is poorly quantified and understood.

The team behind the new MiLCMOP project earlier led the INCOMPASS field campaign to India, taking new measurements and generating new hypotheses on how the monsoon is controlled, including the concept that monsoon progression can be described as a “tug-of-war” between tropical and extratropical airmasses.  This "tug-of-war" is an unsteady process, with a back and forth of the two airmasses before the moist tropical flow takes over for the rest of the season.

This poster describes some of the preliminary results on which the project is designed and explains the approach that MiLCMOP will use, including established techniques and development of new metrics to quantify the interactions between monsoon progression and extratropical forcing.  These methods will include use of vorticity budgets and Lagrangian feature tracking, applied to reanalysis and model data in case study years of fast and slow onset behaviour, to determine the dominant mechanisms controlling monsoon progression.  New model experiments will be designed and performed to isolate the mechanisms by which extratropical drivers affect monsoon onset and its progression.  Finally, novel causal inference techniques will be used to disentangle the effects of extratropical drivers from those in the tropics.

The MiLCMOP project will eventually answer the following key questions:  (1) How are the pace and steadiness of Indian monsoon progression affected by interactions with the extratropics?  (2) What are the mechanisms of extratropical control on monsoon progression and variability?  (3) In what way do the causal extratropical and tropical drivers of ISM progression offset or reinforce each other and can the competing roles of tropical and extratropical processes be generalised to other monsoons?

How to cite: Turner, A., Volonte, A., and Kretschmer, M.: Mid-Latitude Controls on Monsoon Onset and Progression (the MiLCMOP project), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9295, https://doi.org/10.5194/egusphere-egu23-9295, 2023.

EGU23-9398 | ECS | Orals | AS1.24

Monsoon Planet: Bimodal rainfall distribution due to barrier-structure in pressure field 

Anja Katzenberger, Anders Levermann, Georg Feulner, and Stefan Petri

Monsoon systems are transporting water vapour and energy across the globe, making them a central component of the global circulation system. Changes in different forcing parameters have the potential to fundamentally change the monsoon characteristics as indicated in various paleoclimatic records. Here, we use the Atmosphere Model version 2 developed at the Geophysical Fluid Dynamics Laboratory (GFDL-AM2) and couple it with a slab ocean to analyse the monsoon's sensitivity to changes in different forcing parameters on a planet with idealized topography. This Monsoon Planet concept of an Aquaplanet with a broad zonal land stripe allows to reduce the influence of topography and to access the relevant meridional monsoon dynamics. In the simulations that enable monsoon dynamics, a bimodal rainfall distribution develops during the monsoon months with one maximum over the tropical ocean and the other one over land. The intensity and expansion of the land monsoon depends on the relative height of a local maximum in the surface pressure field that is acting as a barrier and determines the landward moisture transport. This dynamic is emerging during the course of one year, but also occurs when varying different parameters in a sensitivity analysis (slab ocean depth, sulfate aerosols, carbon dioxide, solar constant, land albedo). This structure of a bimodal rainfall distribution and a pressure-barrier located between the two maxima is also present in the Westafrican monsoon.

How to cite: Katzenberger, A., Levermann, A., Feulner, G., and Petri, S.: Monsoon Planet: Bimodal rainfall distribution due to barrier-structure in pressure field, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9398, https://doi.org/10.5194/egusphere-egu23-9398, 2023.

EGU23-9428 | ECS | Posters on site | AS1.24

East Asian summer precipitation in AWI-CM3: Comparison with observations and CMIP6 models 

Jian Shi, Christian Stepanek, Dmitry Sein, Jan Streffing, and Gerrit Lohamnn

Owing to the complicated spatial-temporal characteristics of East Asian precipitation (EAP), climate models have limited skills in simulating the modern Asian climate. This consequently leads to large uncertainties in simulations of the past EAP variation and future projections. Here, we explore the performance of the newly developed Alfred Wegener Institute Climate Model, version 3 (AWI-CM3) in simulating the climatological summer EAP. To test whether the model’s skill depends on its atmosphere resolution, we design two AWI-CM3 simulations with different horizontal resolutions. The result shows that both simulations have acceptable performance in simulating the summer mean EAP, generally better than the majority of individual models participating in the Climate Modelling Intercomparison Project (CMIP6). However, for the monthly EAP from June to August, AWI-CM3 exhibits a decayed skill, which is due to the sub-seasonal movement of the western Pacific subtropical high bias. The higher resolution AWI-CM3 simulation shows an overall improvement relative to the one performed at a relatively lower resolution in all aspects taken into account regarding the EAP. We conclude that AWI-CM3 is a suitable tool for exploring the EAP for the observational period. Having verified the model’s skill for modern climate, we suggest employing the AWI-CM3, especially with high atmosphere resolution, also for applications in paleoclimate studies and future projections.

How to cite: Shi, J., Stepanek, C., Sein, D., Streffing, J., and Lohamnn, G.: East Asian summer precipitation in AWI-CM3: Comparison with observations and CMIP6 models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9428, https://doi.org/10.5194/egusphere-egu23-9428, 2023.

EGU23-9482 | Orals | AS1.24

Where the north wind meets the sea: rainfall variability and change and its implications for food security in the Sahel 

Timmo Gaasbeek, Ruud van der Ent, Dim Coumou, Rein Haarsma, and Sander Keulers

Many factors have been suggested to explain variability and change in Sahel rainfall. Of those, sea surface temperature (SST) in the Eastern Mediterranean Sea (EMS) and zonal moisture flux south of the Sahel show strong correlations. Based on observational and reanalysis data on temperature, pressure, wind and moisture flux, this paper identifies a mechanism that explains both correlations. The mechanism hinges on the Jebel Marra massif and the Ethiopian highlands, where the mesoscale convective systems (MCSs) develop that bring most of the rain to the Sahel. We find that cold SST anomalies in the EMS between June and September cause a greater trans-Sahara temperature contrast and coincide with high pressure over Libya, resulting in stronger northerlies towards Sudan. This prevents Tropical Atlantic moisture from reaching the MCS genesis region, which reduces the seasonal northward spread of Sahel rainfall and of the Atlantic intertropical convergence zone, which in turn suppresses the development of the west-African westerly jet and the African westerly jet and inhibits Atlantic moisture from reaching the MCS genesis region, thus further reducing Sahel rainfall. Anomalous moisture transport from the Mediterranean does not play a role. Mediterranean SST variability raises questions about the future development of Sahel rainfall. If a new dry period materialises, this will have substantial implications on food production in the region. There are however opportunities for mitigating against the effects of such a dry period.

How to cite: Gaasbeek, T., van der Ent, R., Coumou, D., Haarsma, R., and Keulers, S.: Where the north wind meets the sea: rainfall variability and change and its implications for food security in the Sahel, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9482, https://doi.org/10.5194/egusphere-egu23-9482, 2023.

The phase shift of climatic systems in decadal or interdecadal scale, also called as regime shift has occurred in East Asian Summer Monsoon (EASM) in the past. For example, the shifts of the late 1970s, mid 1990s, and early 2000s are the typical examples. Before and after these shifts, dominant teleconnection mode affecting the EASM had changed. On the other hand, the shift of early 2000s has not extensively investigated. Here, it is examined the characteristics of this particular shift in relation to variability of East Asian jet during summer. First, regime shifts earlier and in the early 2000s are detected based on the variance of summer East Asian jet. Second, the teleconnection pattern that influence summer East Asian jet was changed from the Atlantic-Eurasian (AEA) pattern to distinctly different zonal pattern around extratropical region of Eurasian. Finally, it was found that after this regime shift the land-atmosphere coupling induced by variability of soil moisture also strengthened. It is hypothesized that enhanced linkage between jet in the upper atmosphere and surface heat flux over Inner East Asia is a key mechanism of enhancing variability of the East Asian summer jet, i.e., the regime shift in 2000s. These results imply that over drier region, the regional climatic system might response more sensitively to regional-scale change on surface level than large-scale influence, such as wave-train.

How to cite: Nam, J. and Yoon, J.-H.: Regime shift of Jet over East Asian summer Monsoon in the early 2000s: its detection and dynamical driver, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11107, https://doi.org/10.5194/egusphere-egu23-11107, 2023.

The present study is aimed to investigate the rainfall characteristics of Monsoon Deep Depressions (MDD) originating over the Bay of Bengal (BoB) basin using a coupled ocean-atmospheric model (COAWST) and a stand-alone atmospheric (WRF) model with a lead time of up to 72h. It is found that though the tracks of the four MDDs considered in the study have been reasonably simulated, the intensity was overestimated in both sets of simulations compared to India Meteorological Department (IMD) best estimates. Upon decomposition of the contributors to the rainrate for the composite of the storms in the deep depression (DD) phase, it was found that the moisture sources/sinks play a more important role than the cloud sources/sinks in modulating the rainfall processes. Further analysis of the moisture sources/sinks showed that the horizontal and vertical advection are the major drivers in modulating the contribution of the moisture sources/sinks. The validation of rainfall using CMORPH datasets suggested that the coupled simulations had a higher skill in rainfall prediction. Furthermore, the composite of different components of moisture sources/sinks (especially vertical advection) was found to be more realistically simulated in COAWST compared to WRF upon validation with MERRA datasets. Analysis of the composite energetics showed that scarcity of bulk kinetic energy in the later hours of the DD phase in COAWST led to the dissipation of the storm core, which led to better prediction of rainfall. On the other hand, a re-intensification of the storm core by means of condensational heating led to an overestimation of rainfall in WRF, which finally resulted in lower skill in rainfall prediction. In spite of the stand-alone atmospheric model capturing the horizontal moisture incursion in the lower levels significantly, the better representation of the vertical structure enabled the coupled model to capture the precipitation features more realistically, increasing skill in rainfall prediction.

How to cite: Chakraborty, T., Pattnaik, S., and Baisya, H.: A Numerical Study to Investigate Precipitation Features of Monsoon Deep Depressions over Bay of Bengal: Comparison of Coupled and Control Simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11257, https://doi.org/10.5194/egusphere-egu23-11257, 2023.

EGU23-12313 | ECS | Posters on site | AS1.24

Zonal Momentum Balance in South Asian Summer Monsoon: Forces and Changing Winds 

Pankaj Upadhyaya and Saroj K. Mishra

The balance of forces for the South Asian Summer Monsoon (SASM) gives valuable insights for the understanding of the mean circulation and the changes it has undergone in the past. In this study, we have analyzed the zonal momentum balance for SASM for the last few decades (1950-2010) using reanalysis data to understand the changes in different forces and relate them with the changes in the associated circulation. In the lower level (925 hPa), the Pressure Gradient Force (PGF), Coriolis Force (CF), and Residual Force (RF, which includes the unresolved sub-grid scale process and frictional terms) are found to be the dominant terms of the zonal momentum balance for SASM with a magnitude of order 10-4m sec-2 whereas, horizontal advection and eddy force terms are negligible with one or more order lesser in magnitude. The residual force can be estimated by Rayleigh friction induced by turbulence, particularly over ocean points, which, however, is not a good measure of the same over the land points because of high irregularity. The momentum balance at the upper level (200 hPa) is between the PGF, CF, and the advection term, unlike the lower level, where the residual force does not seem to be dominant. In the free troposphere, the Convective Momentum Transfer or in other words convective friction is a good estimator of the RF, which represents the vertical transport of momentum. The changes in SASM circulation in the past can be apprehended by looking into the changes in these vital forces that drive the motion.

How to cite: Upadhyaya, P. and Mishra, S. K.: Zonal Momentum Balance in South Asian Summer Monsoon: Forces and Changing Winds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12313, https://doi.org/10.5194/egusphere-egu23-12313, 2023.

EGU23-12760 | ECS | Posters on site | AS1.24

Developed a climate modeling framework for India                  

Debi Prasad Bhuyan and Saroj Kanta Mishra

A better representation of the poorly understood sub-grid scale processes in the Global Circulation Model is imperative for the skilful simulation of the Indian Summer Monsoon (ISM). We customized the parametrizations for deep convection, gravity wave, and surface layer; incorporated them into the NCAR Community Atmosphere Model 5.0 (NCAR CAM5, base model). The modified deep convective parametrization includes dynamic tau (dynamic convective adjustment timescale), which allows a spatiotemporally varying tau instead of constant tau and the stochastic entrainment rate in place of a fixed entrainment rate. Similarly, the modified gravity wave parametrization facilitates estimating the response of upper-level gravity wave drag induced from secondary sources. Likewise, the modified surface layer parametrization enables a better representation of near-surface variables as well as surface fluxes. The simulations of default and customized NCAR CAM5 have been carried out for eleven years (one year for spin-up and the rest ten years considered for analysis). The analysis has been performed for two major climate change indicators, i.e., temperature and precipitation for the ISM season (June to September). The model simulated near-surface temperature and precipitation during ISM were evaluated against observation (Indian Meteorological Department). A significant improvement has been noted in simulating the total precipitation pattern and magnitude over India, as well as for surface air temperature, particularly over northern India. In addition, based on performance, the customized model alleviates some of the long-standing biases evident in the default NCAR CAM5 simulation over India. Furthermore, compared to the base model, the customized model realistically simulates the annual cycle of precipitation, medium and extreme precipitation rates, meridional tropospheric temperature gradient, upper (200 hPa) and lower (850 hPa) tropospheric winds, Madden Julian Oscillation, and equatorial waves. The study’s findings illustrate the significance of model parametrizations towards improving the ISM simulation. Meanwhile, the modeling framework would be essential for credible future climate projections of India and would become a vital tool for policymakers and diverse stakeholders.

Keywords: Indian Summer Monsoon, NCAR CAM5, Deep convection, Gravity wave, Surface layer

How to cite: Bhuyan, D. P. and Mishra, S. K.: Developed a climate modeling framework for India                 , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12760, https://doi.org/10.5194/egusphere-egu23-12760, 2023.

EGU23-12805 | Orals | AS1.24

Indian summer monsoon versus mid-latitude drivers of boreal summer tropospheric circulation and heat extremes in the eastern Mediterranean 

Giorgia Di Capua, Dominik Diedrich, Evangelos Tyrlis, Daniela Matei, and Reik V. Donner

The lower tropospheric circulation over the eastern Mediterranean during boreal summer is markedly characterized by northerly winds known as the Etesians (Tyrlis et al., 2013). These winds are accompanied by large scale subsidence and clear skies, and can mitigate the emergence of heat waves by bringing colder air from the Eurasian landmass. Here, we employ Causal Effect Networks, obtained by applying the Peter and Clark Momentary Conditional Independence (PCMCI) causal discovery algorithm (Runge, 2018), to identify causal precursors of the Etesians both in mid-latitude circulation fields and tropical convective activity at two different intraseasonal time scales (3 and 7-day average). We identify wave train activity over the North Atlantic and North American region and convective activity over the Arabian Sea and western coast of the Indian peninsula to be causal precursors of Etesians winds defined as 850 hPa meridional wind variations over the eastern Mediterranean at a lag of 3-to-6 days. In general, the influence of tropical drivers, i.e. the Indian summer monsoon (ISM) system,  is found to be stronger than that of the mid-latitude wave train, thus corroborating the hypothesis that the ISM affects the circulation over the Mediterranean and Northeast Africa, as suggested by the monsoon-desert mechanisms (Rodwell and Hoskins, 1996). Moreover, at longer time scales (7 to 14-day lag), the main causal influence comes from tropical convective activity over the Indian peninsula, while the effect of the mid-latitude circulation weakens and becomes not significant. We finally employ event coincidence analysis to explore the relationship between Etesians and heat extremes in the eastern Mediterranean and assess the presence of trends in the strength of Etesians outbreaks at intraseasonal variability in the historical period.

References

Rodwell, M. J. and Hoskins, B.: Monsoons and the dynamics of deserts, Q. J. R. Meteorol. Soc., 122, 1385–1404, 1996.

Runge, J.: Causal network reconstruction from time series: From theoretical assumptions to practical estimation, 28, 075310, https://doi.org/10.1063/1.5025050, 2018.

Tyrlis, E., Lelieveld, J., and Steil, B.: The summer circulation over the eastern Mediterranean and the Middle East: Influence of the South Asian monsoon, Clim. Dyn., 40, 1103–1123, https://doi.org/10.1007/s00382-012-1528-4, 2013.

How to cite: Di Capua, G., Diedrich, D., Tyrlis, E., Matei, D., and Donner, R. V.: Indian summer monsoon versus mid-latitude drivers of boreal summer tropospheric circulation and heat extremes in the eastern Mediterranean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12805, https://doi.org/10.5194/egusphere-egu23-12805, 2023.

EGU23-13539 | ECS | Posters on site | AS1.24

Characteristics of spectral energetics during excess and deficient rainfall years in India 

Ravi Dhishana and Sarvesh Kumar Dubey

Significant spatial and temporal deviations from the seasonal mean precipitation, such as severe droughts (deficient rainfall) and floods (excess rainfall), have a major influence on India. The non-linear energy interactions between the various scale atmospheric systems are important as they play a crucial role in the Indian summer monsoon variability. Since studies have yet to look at the whole energy budget of the southwest monsoon, it is necessary to accurately capture these energy exchanges to represent the monsoon circulation better. In this study, we found the exact nature of complex non-linear energy interactions of synoptic-scale mainly low-pressure systems (LPSs) and Intraseasonal Oscillation (lSO) 30-60 day scale with other scales, including the seasonal mean, Indian Ocean Dipole (IOD), and El Niño–Southern Oscillation (ENSO) using the in-scale and out of scale energetics. These energy interactions are calculated in the frequency domain for the Indian monsoon region using the ECMWF ERA-5 data for 72 years (1950-2021) during the monsoon season (JJAS). Since the seasonal mean kinetic energy is highly correlated with the seasonal mean rainfall, we explored how these energy exchanges vary during excess and deficient rainfall years. We also found that the ISO and synoptic scale systems influence the interannual variability of the Indian Summer Monsoon mainly through the interactions with the mean flow. In addition, the monsoon mean flow and most energy exchanges show a significant relationship at the upper level (200 hPa) and lower level (850 hPa) atmosphere.

How to cite: Dhishana, R. and Dubey, S. K.: Characteristics of spectral energetics during excess and deficient rainfall years in India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13539, https://doi.org/10.5194/egusphere-egu23-13539, 2023.

EGU23-13727 | ECS | Orals | AS1.24

Characteristics of African Sahel Precipitation in global storm-resolving Climate Models 

Dorian Spät, David Schuhbauer, and Aiko Voigt

The simulation of precipitation in the African Sahel region is challenging for current global climate models. These models conventionally work with grids with horizontal resolution larger than 100 km and therefore must use parametrization schemes to simulate deep convection. The nextGEMS project, on the other hand, performs global simulations with two new climate models (adapted versions of ICON and IFS) with fine resolutions of a few kilometers. At such high resolution, deep convection is resolved, which allows for a much more realistic representation of precipitation. This is particularly promising for simulating convection in the African Sahel, where most precipitation originates from mesoscale convective systems resolved at these simulation scales. 

We present a preliminary analysis of the cycle two nextGEMS simulations focusing on Sahel precipitation and the West African monsoon. We show that some characteristics of precipitation, such as low autocorrelation with one day lag, are much closer to measurements compared to conventional climate models. We also discuss some of the problems that still persist in the simulations and compare the two models depending on different features of Sahel precipitation.

How to cite: Spät, D., Schuhbauer, D., and Voigt, A.: Characteristics of African Sahel Precipitation in global storm-resolving Climate Models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13727, https://doi.org/10.5194/egusphere-egu23-13727, 2023.

EGU23-13868 | ECS | Orals | AS1.24

Causal Drivers Behind Enhanced Rainfall Activity OverNorthern Indian 

Luisa E. Aviles Podgurski, Giorgia Di Capua, and Reik V. Donner

The Western (WHF) and Eastern Himalayan foothills (EHF) are two densely populated regions that experience extreme precipitation events during the Indian summer monsoon (ISM) season lasting typically from June to September [1, 2]. Therefore, a better understanding of the processes controlling ISM intraseasonal variability is of great relevance.

In our present work we identify and quantify causal relationships at short lead-times (three to nine days) between characteristic remote and local climate patterns and the precipitation over the WHF and EHF. More specifically we apply the so-called response-guided causal precursor detection (RGCPD) scheme that builds on the Peter and Clark momentary conditional dependence (PCMCI) algorithm [3]. The employed method is based on concepts of information theory and statistical mechanics, and allows to identify strongly interdependent climate patterns associated with the ISM and to distinguish between spurious and truly causal links. Finally, causal effect networks (CENs) visually summarise the identified causal links between different variables, indicating the directionality, time lag and magnitude of the causal effect.

Our analysis reveals that WHF rainfall variability is influenced by mid-latitude teleconnections such as the circumglobal teleconnection index and seems to be driven by similar precursors and time scales as the precipitation over central India [4]. In contrast, CENs indicate that the EHF rainfall is characterised by faster dynamics compared to the WHF and whilst it is also driven by mid-latitude teleconnections, a different set of atmospheric processes appears to play a major role in its variability. Specifically, a unique and strong causal connection to the tropical western Pacific is revealed, manifesting itself in the geopotential height at 500 hPa and the mean sea-level pressure. A thorough analysis of this signal indicates a Gill-type response to a heat sink over the equatorial Pacific, that may be associated with the Madden-Julian oscillation (MJO) and suggests a link between suppressed MJO phases and enhanced rainfall activity over the EHF region. Thus, our analysis hints to a connection between break spells of the ISM, where large parts of the Indian landmass experience reduced precipitation activity, and enhanced rainfall activity over the EHF region.

References
[1] Vellore, R., et al., On the anomalous precipitation enhancement over the Himalayan foothills during monsoon breaks, Clim. Dynam. 43, 2009-2031 (2014).
[2] Vellore, R., et al., Monsoon - extratropical circulation interactions in Himalayan extreme rainfall, Clim. Dynam. 46, 3517-3564 (2016).
[3] Runge, J., Causal network reconstruction from time series: From theoretical assumptions to practical estimation, Chaos 28, 075310 (2018).
[4] Di Capua, G., et al., Tropical and mid-latitude teleconnections interacting with the Indian summer monsoon rainfall: a theory-guided causal effect network approach, Earth Syst. Dyn., 11, 17-34 (2020).

How to cite: Aviles Podgurski, L. E., Di Capua, G., and Donner, R. V.: Causal Drivers Behind Enhanced Rainfall Activity OverNorthern Indian, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13868, https://doi.org/10.5194/egusphere-egu23-13868, 2023.

EGU23-14204 | ECS | Orals | AS1.24

Modeling the impact of the urban land-use on the Indian Summer Monsoon precipitation 

Renaud Falga and Chien Wang

The urban areas can modify the local and regional climate through various processes. They can indeed modify the water cycle and precipitations, either through the modification of land-use, or through effects induced by the emissions of anthropogenic aerosols. The thermodynamical perturbations induced by the presence of urban land-use, including the urban heat island effect, are known to induce rainfall modification due to perturbation of the flow and enhancement of the convective activity. However, this impact has yet to be clarified in a large scale, highly energetic system like the Asian Monsoon system. Using the high resolution meso-scale atmospheric model Meso-NH, we investigated the impact of urban land-use on the precipitation during the Indian Summer Monsoon, including the influence on extreme events. The results of this study will be presented and discussed.

How to cite: Falga, R. and Wang, C.: Modeling the impact of the urban land-use on the Indian Summer Monsoon precipitation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14204, https://doi.org/10.5194/egusphere-egu23-14204, 2023.

EGU23-14372 | ECS | Posters on site | AS1.24

Investigating the Causes of Poleward Shift in Monsoon Low-level Jet 

Sukumaran Sreepriya, Krishna Mirle AchutaRao, and Sukumaran Sandeep

Recent studies using coupled model simulations and observation datasets suggest a poleward shift and overall weakening of Indian Summer Monsoon (ISM) circulation (Sandeep and Ajayamohan, 2015). Their investigation using experiments from the fifth phase of coupled model Inter-comparison project (CMIP5) indicate a poleward migration of the monsoon low-level jet (LLJ), with the magnitude of shift  linked to the degree of warming. 

Here we investigate the changes in monsoon LLJ in multiple reanalysis datasets as well as historical and future scenario simulations of the sixth phase of coupled model Inter-comparison project (CMIP6). The latitudinal location of LLJ is defined as the latitude of zero absolute vorticity over the Arabian Sea, following Tomas and Webster (1997). Although all reanalysis datasets show a poleward shift in LLJ since late 1970s, the magnitude of shift varies among them. The multi model ensemble of CMIP6 historical simulations show a northward shift of 0.4 degrees in LLJ. The ensemble mean of SSP585 simulations show a northward shift in LLJ by 0.8 degrees in the 2081 - 2100 period. The changes in the latitudinal position of LLJ and the land-sea temperature difference are significantly correlated, with a Pearson correlation coefficient of 0.81 and 0.67 for the ensemble means of historical and SSP585 runs, respectively. This suggests that the underlying dynamics of the monsoon circulation is changing in a warming climate.

References

Sandeep, S., & Ajayamohan, R. S. (2015). Poleward shift in Indian summer monsoon low level jetstream under global warming. Climate Dynamics, 45(1), 337-351.

Tomas, R. A., & Webster, P. J. (1997). The role of inertial instability in determining the location and strength of near‐equatorial convection. Quarterly Journal of the Royal Meteorological Society, 123(542), 1445-1482.

How to cite: Sreepriya, S., Mirle AchutaRao, K., and Sandeep, S.: Investigating the Causes of Poleward Shift in Monsoon Low-level Jet, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14372, https://doi.org/10.5194/egusphere-egu23-14372, 2023.

EGU23-16193 | ECS | Orals | AS1.24

Rise in Rainfall of South Asian Monsoon Low-Pressure Systems 

Vishnu Sasidharan Nair, William R. Boos, Mark D. Risser, Travis A. O’Brien, Paul A. Ullrich, and William D. Collins

Cyclonic low‐pressure systems (LPS) are the dominant synoptic‐scale rain-bearing system of the South Asian summer monsoon. Traditionally categorized by intensity as monsoon lows, monsoon depressions, and more intense cyclonic storms, LPS produce intense rainfall and floods in some of the world’s most densely populated regions. Yet the contribution of the relatively weak lows vs. the stronger depressions to extreme rainfall and its trends remains unknown; this knowledge gap is particularly troubling because historical trends in LPS have been difficult to assess due to changes in the observing network. Future projections have also remained highly uncertain due to the inability of many coarse-resolution climate models to accurately simulate LPS.

Here we use satellite and gauge-based precipitation estimates with atmospheric reanalyses to show that precipitation in monsoon depressions has become more intense in recent decades. This intensification has occurred as humidity over parts of India increased more rapidly than nearly anywhere else on Earth. Precipitation in depressions has risen at a relative rate larger than that of specific humidity, suggesting that upward motion in depressions has become more intense; vertical motion trends in a state-of-the-art reanalysis, which incorporates nearly all long-term climate forcings, are consistent with this hypothesis. We also examine changes in South Asian LPS precipitation simulated by an ensemble of high-resolution global models, which we find skillfully represent these storms. Future trends in total LPS precipitation, including in monsoon depressions, lie near an approximate Clausius–Clapeyron rate (7%/K) in the multi-model mean. This change in LPS rain rates contributes to a projected future increase in seasonal mean and extreme precipitation over South Asian land. Adaptation to future changes in human exposure to hydrological extremes thus requires careful monitoring, accurate multi-decadal projections, and skilful short-term forecasts of the interaction of the humidity field with the dynamics of monsoon LPS.

How to cite: Sasidharan Nair, V., R. Boos, W., D. Risser, M., A. O’Brien, T., A. Ullrich, P., and D. Collins, W.: Rise in Rainfall of South Asian Monsoon Low-Pressure Systems, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16193, https://doi.org/10.5194/egusphere-egu23-16193, 2023.

India has tropical monsoon climate with significant regional variability in rainfall and temperature, where precipitation is closely connected to precipitable water vapour (PWV). Here, the satellite and reanalysis data are applied to study the spatial and temporal changes of PWV over India in 1980–2020. We have also analysed its potential drivers such as precipitation, surface temperature and evapotranspiration during the same period. The distribution of annual PWV depicts the highest values over the east coast (40–50 mm) and lowest in western Himalaya (< 10 mm). The seasonal distribution shows highest PWV during monsoon (June-July-August-September, about 40–65 mm). Similarly, the monthly cycle of PWV shows the lowest amount in January, which gradually increases with time until it peaks in July, and then decreases thereafter. Interannual variations in PWV show a peak in 1997–1998, which is related to the strong El-Nino Southern Oscillation (ENSO) event during that period. Among the sources, sinks and drivers, evapotranspiration (0.6-–0.9), precipitation (0.7–0.9) and surface temperature (0.5–0.6) are highly correlated with PWV throughout India. The PWV trends in India are found significantly positive (0.6–0.9), which can be attributed to recent increase in surface temperature and thus the rise in atmospheric moisture.  This is concern for regional climate change as PWV is directly connected to water vapour and thus, to temperature and climate.

How to cite: Sarkar, S.: Long-term changes in precipitable water vapour over India derived from satellite and reanalyses data for the past four decades (1980–2020), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-184, https://doi.org/10.5194/egusphere-egu23-184, 2023.

EGU23-394 | ECS | Posters on site | AS1.25

Multi-source assessment of uncertainty over the tropical ocean 

Rajani Kumar Pradhan and Yannis Markonis

The tropical ocean, which receives a substantial volume of precipitation and evapotranspiration, has a greater impact on Earth's energy and water balance. Yet, considerable studies have been focused on the Earth's terrestrial precipitation, whereas very little attention has been given to the oceanic region. Despite the advancement of satellite and reanalysis precipitation estimates, relatively few studies explored these estimates over the oceans. In this context, we quantitatively evaluate and inter-compare the state-of-the-art satellite, reanalysis, and merged precipitation products over the tropical oceans. We use a suite of various gridded and well-known precipitation datasets such as the Integrated Multisatellite Retrieval for Global Precipitation Measurement (IMERG), Global satellite Mapping of Precipitation (GSMaP), European Centre for Medium-Range Weather Forecast (ECMWF) Reanalysis v5 (ERA5), and Multi-Source Weighted-Ensemble Precipitation (MSWEP) products to comprehensively estimate the tropical oceanic precipitation and its spatial and temporal variation. In particular, we are looking into the estimates of the total mean precipitation and its inter-annual variation. In addition, the discrepancies among various precipitation estimates are analysed as a function of different spatial and temporal scale to assess their uncertainty over tropical ocean for the first time. This study will provide deep insights into the precipitation characteristic and its spatio-temporal variability across the tropical ocean. Moreover, such information will help to revisit the estimation of the global water budget components in the near future.

How to cite: Pradhan, R. K. and Markonis, Y.: Multi-source assessment of uncertainty over the tropical ocean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-394, https://doi.org/10.5194/egusphere-egu23-394, 2023.

High spatiotemporal resolution satellite precipitation products (herein SPPs) have great potential for investigating rainfall dynamics, including diurnal rainfall (DR). However, the relative performances of these products are regionally specific and unknown in most places. This talk presents our recent works on evaluating and applying various SPPs in studying the summer DR events in Taiwan and Luzon (an Island of Philippines nearby Taiwan). In the first part of the talk, we evaluated the four post-real-time SPPs (including TRMM-3B42 v7, IMERG-F v5, IMERG-F v6, and GSMaP v7) in studying DR events in Taiwan. Our results show that IMERG-F v6 outperforms the other SPPs more accurately (both quantitatively and qualitatively) in depicting the summer rainfall variations in Taiwan at multiple timescales (including mean status, daily, and diurnal), using more than 400 rain-gauge observations as the baseline for comparison. IMERG-F v6 also performs better than other SPPs in capturing the characteristics of DR activities. In the second part of the talk, we further evaluated the near-real-time (NRT) products of IMERG v6 (i.e., IMERG-L and IMERG-E) and GSMaP v7 (i.e., GSMaP-NRT and GSMaP-Gauge-NRT) in depicting the variation in DR in Taiwan. Two sub-components of DR variation, daily mean (Pm) and anomalies (ΔP), were evaluated, and ΔP was further separated into diurnal (S1) and semi-diurnal (S2) harmonic modes. Compared with surface observations, all NRT products underestimated Pm and ΔP; however, IMERG products are relatively better than GSMaP products in most of the examined spatial characteristics. Furthermore, temporal analysis shows that only IMERG-E depicts the phase evolution of both S1 and S2, similar to surface observations. Finally, we showed some potential use of IMERG-F v6 and TRMM-3B42 v7 in studying the long-term changes in the summer DR activities over Luzon and its adjacent seas during 2000-2019.

How to cite: Huang, W.-R., Hsu, J., and Liu, P.-Y.: Evaluation and application of satellite precipitation products in studying the summer diurnal rainfall events in Taiwan and Luzon, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-915, https://doi.org/10.5194/egusphere-egu23-915, 2023.

The Global Precipitation Measurement (GPM) mission was launched in February 2014 as a joint mission between JAXA from Japan and NASA from the United States.  GPM carries a state of the art dual-frequency precipitation radar and a multi-channel passive microwave radiometer that acts not only to enhance the radar’s retrieval capability, but also as a reference for a constellation of existing satellites carrying passive microwave sensors.  In April 2022, GPM approved V 7 of its precipitation products starting with GMI and continuing with the constellation of radiometers.  The precipitation products from these sensors are consistent by design and show relatively minor differences in the mean global sense.  Validation results will be shown for work done over the Continental United States using a Radar/Gauge composite as truth, and Kwajalein atoll to represent truth over tropical oceans.  The validation results are a necessary but not sufficient component to quantify the algorithm’s uncertainties.  Good results for bias, MAR and RMSE are demonstrated.  Validation results, however, are only able to assess errors at their own sites, and systematic errors, in particular, are not actually systematic, but regime dependent errors that vary as a function of how well the algorithm assumptions are captured at the validation sites.   This talk will explore ways of validating not by location, but by precipitation states that, the environment that the precipitation evolves in, as a way of obtaining robust statistics of individual precipitation states that are universal and can be applied with confidence to areas outside the validation domain.

How to cite: Kummerow, C.: The GPM Radiometer Algorithm - from Validation to Uncertainties, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-954, https://doi.org/10.5194/egusphere-egu23-954, 2023.

Snow, on the ground and falling to the surface, plays an important part in the global water cycle, yet the measurement of it remains problematic. The estimation of falling snow (or frozen precipitation) is difficult and relies upon the interpretation of observations from passive microwave sensors. However, the relationship(s) between the passive microwave observations and falling snow at/near the surface is very much dependent upon the type of snow (ice) crystals present which vary greatly between different precipitating weather systems. To date, much work has concentrated observations from current sensors using the 150/166 GHz and the 183.31 GHz water vapour channels to extract the scattering signature associated with frozen hydrometeors. However, the TROPICS pathfinder mission, launched in June 2021 into a near polar orbit, carries a new radiometer that provides an opportunity to assess the impact of including observations at 204.8 GHz. Such measurements are more sensitive to ice particles, resulting in a greater scattering signature, while being less sensitive to the water vapour around the 183.31 GHz region. Preliminary results are encouraging and will be presented here. A number of case studies, including lake-effect snowfall (November 2022) and widespread snow across North America (mid-December 2022), will be explored in detail. These initial results show observations at 204.8 GHz provide additional information that improves snow delineation and estimation: this is of great significance for the upcoming EUMETSAT EPS-SG missions.

How to cite: Milani, L. and Kidd, C.: Assessing the potential of frequencies around 205 GHz for improving snowfall estimation., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1484, https://doi.org/10.5194/egusphere-egu23-1484, 2023.

EGU23-1718 | Orals | AS1.25

Deep learning for uncertainty quantification of satellite retrievals of precipitation: Case studies in two complex terrain regions 

Haonan Chen, Liping Wang, Yun-Lan Chen, Pingping Xie, Chia-Rong Chen, and Tony Liao

The performance of various composite satellite precipitation products is severely limited by their individual passive microwave (PMW)-based retrieval uncertainties because the PMW sensors have difficulties in resolving heavy rain and/or shallow orographic precipitation systems, especially during small scale precipitation events. Characterizing the error structure of PMW retrievals is crucial to improving precipitation mapping at different space-time scales. This paper presents an ensemble learning framework to quantify the uncertainties associated with satellite precipitation products with an emphasis on orographic precipitation. A deep convolutional neural network is devised, which utilizes ground-based radar and gauge blended precipitation estimates as target labels to train satellite precipitation products in order to extract the uncertainty features involved in the satellite products. An ensemble strategy is designed to boost the performance of individually trained deep learning models. The ensemble model is then applied to multiple domains with different geophysical characteristics. The precipitation products derived using the NOAA/Climate Prediction Center morphing technique (CMORPH) over Taiwan and the coastal mountain region in the western United States are used to demonstrate the deep learning-based bias correction performance. The impact of topography on satellite-based precipitation retrievals is quantified. The results show that the orographic gradients have a strong influence on precipitation retrievals in complex terrain regions. The accuracy of CMORPH is dramatically enhanced after applying the ensemble learning-based bias correction technique, indicating the great potential of machine learning in improving satellite precipitation retrievals.

How to cite: Chen, H., Wang, L., Chen, Y.-L., Xie, P., Chen, C.-R., and Liao, T.: Deep learning for uncertainty quantification of satellite retrievals of precipitation: Case studies in two complex terrain regions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1718, https://doi.org/10.5194/egusphere-egu23-1718, 2023.

EGU23-2792 | Orals | AS1.25

Operational Real-Time Production of CMORPH2 

Pingping Xie, Eric Sinsky, Shaorong Wu, David DeWitt, Donald Garrett, and Wanqiu Wang

Real-time production of the second generation CMORPH (CMORPH2) has been migrated to and executed at a NOAA / NWS required operational environment, the NWS/NCEP Central Operation (NCO) and Climate Prediction Center (CPC) Compute Farm (CF) effective December 2022.  CMORPH2 real-time production was routinely implemented on a research and development environment at NOAA/CPC since April 2017. Successful migration of the production system to the 7/24 operational environment ensures the production of the high-resolution, high-quality global precipitation analysis at a much higher stability and reduced production latency of one hour, satisfying a requirement for an observational analysis to be infused into operational forecast models and routine field operations.

Inputs to the CMORPH2 real-time production include rainfall and snowfall rate retrievals from passive microwave (PMW) measurements aboard more than 10 low earth orbit (LEO) satellites, precipitation estimates derived from infrared (IR) observations of geostationary (GEO) and LEO platforms, and model precipitation forecast from the NCEP operational global forecast system (GFS).  These inputs are first inter-calibrated to ensure quantitative consistencies. The inter-calibrated PMW retrievals and IR-based precipitation estimates are then propagated from their respective observation times to the target analysis time along the cloud motion vectors from both the forward and backward directions. The propagated PMW and IR based precipitation estimates are finally integrated into a single field of global precipitation through the Kalman Filter framework. In addition to the total precipitation, fraction of solid precipitation is computed from the surface air temperature and other surface meteorological variables using the algorithm of Sims and Liu (2015).

The CMORPH2 satellite precipitation analysis is constructed on a 0.05o latitude/longitude over the entire globe (90oS-90oN) and in a 30-minute temporal resolution. The real-time production is first generated at a very short latency of one hour and then refreshed with any newly available inputs once every 30 minutes up to 12 hours of latency for improved accuracy when inouts from all sources are available in most cases. The CMORPH2 real-time production is utilized by several important users including the NWS Aviation center (AWC), Weather Prediction Center (WPC), and NWS Alaska Office, and pushed to the AWIPS for field applications. 

Work is under way to examine the CMORPH2 real-time production as a function of region, season, precipitation type, and production latency, and to further improve the CMORPH2 through infusing the PMW precipitation retrievals from the NOAA Direct Broadcast (DB) systems and refining the GEO IR based precipitation estimates. Results will be reported at the 2023 EGU Meetings.

How to cite: Xie, P., Sinsky, E., Wu, S., DeWitt, D., Garrett, D., and Wang, W.: Operational Real-Time Production of CMORPH2, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2792, https://doi.org/10.5194/egusphere-egu23-2792, 2023.

EGU23-2870 | ECS | Orals | AS1.25

Understanding the influence of urban form on the spatial pattern of precipitation 

Yanle Lu, Qi Li, Zhou Yu, John Albertson, Xiaodong Chen, Haonan Chen, Angeline Pendergrass, and Leiqiu Hu

Urban areas are known to modify the spatial pattern of precipitation climatology. Existing observational evidence suggests that precipitation can be enhanced downwind of a city, albeit other locations of precipitation enhancement have also been reported. Among the proposed mechanisms that modify the precipitation, the thermodynamic and aerodynamic processes in the urban lower atmosphere interact with the synoptic conditions and could play a key role in determining the resulting spatial variability of precipitation. In addition, these processes are intricately shaped by urban form characteristics, such as the spatial extent of the impervious land. This study aims to unravel how different urban forms impact the spatial organizations of precipitation climatology under different synoptic conditions. We use the Multi-Radar Multi-Sensor (MRMS) quantitative precipitation estimation data products and analyze the hourly precipitation maps for a selected set of cities across the continental United States from the years 2015 to 2021. Results suggest that a statistically significant downwind enhancement of precipitation does exist in about four-fifths of these cities, while the magnitude is comparable to previous findings. Additionally, we find that the precipitation distribution tends to be more clustered for higher wind speed; the location for precipitation maxima is located closer to the city center under low synoptic winds but shifts towards the urban-rural interface under high wind conditions. The magnitude of downwind precipitation enhancement is highly dependent on wind directions and is positively correlated with the city size for the south, southwest, and west directions. This study provides observational proof through a cross-city analysis that the spatial pattern of urban precipitation can be attributed to the modified atmospheric processes by distinct urban forms.

How to cite: Lu, Y., Li, Q., Yu, Z., Albertson, J., Chen, X., Chen, H., Pendergrass, A., and Hu, L.: Understanding the influence of urban form on the spatial pattern of precipitation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2870, https://doi.org/10.5194/egusphere-egu23-2870, 2023.

EGU23-2893 | Orals | AS1.25

V07 Reprocessing of Global Precipitation Measurement (GPM) Mission Data Suite 

Erich Franz Stocker, John Kwiatkowski, and Owen Kelley

Periodic reprocessing of the complete GPM data suite is an integral part of thescience processing strategy for the GPM mission. The first publicly available data was identified by the data product version V04 in 2014. In 2017 product version V05 for the radiometer products and in 2018 V06 for the radar products were completed.This reprocessing cycle extended the radar data  back to the TRMM era (1997) and radiometer data back to 1987.  It also officially integrated a considerable amount of earlier data into the GPM data suite. Reprocessing cycle V07 began at the end of 2021 with the radar based data and completed in May 2022 with all the radiometer data. The V07 version had significant changes in radar data because of a change in the Ka radar scanning strategy in May 2018 that allowed the Ka radar to cover the  entire swath of the Ku radar. This allowed dual frequency retrieval across the entire Ku swath rather than just in the interior.  The GPROF precipitation retrieval for the radiometers reverted back to a probablistic output. This presentation will summarize these major changes as well as other algorithm changes that improved the precipitation retrieval.  It will  also present other data that the mission makes available to users. 

How to cite: Stocker, E. F., Kwiatkowski, J., and Kelley, O.: V07 Reprocessing of Global Precipitation Measurement (GPM) Mission Data Suite, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2893, https://doi.org/10.5194/egusphere-egu23-2893, 2023.

EGU23-2945 | ECS | Orals | AS1.25

Machine Learning-based Probabilistic Precipitation Estimation with the GOES-16 Advanced Baseline Imager 

Shruti A. Upadhyaya, Pierre-Emmanuel Kirstetter, and Robert J. Kuligowski

This study introduces a new machine learning-based probabilistic quantitative precipitation estimate (PQPE) retrieval that uses observations from the GOES-16 Advanced Baseline Imager (ABI) across the CONUS at 5 min temporal resolution and ~2 km spatial resolution. It is developed and evaluated using the Ground Validation Multi-Radar/Multi-Sensor (GV-MRMS) system as a benchmark, and features Convolutional Neural Network (CNN) machine learning. Key advances include (1) the design of a three-dimensional CNN model to retrieve the distribution of precipitation rate instead of a single deterministic value; (2) a comprehensive set of predictors based on spatio-temporal information from infrared ABI channels and complemented by environmental conditions from Numerical Weather Prediction (NWP) models; and (3) using probabilities of occurrence for different precipitation type (e.g., convective and stratiform), retrieved from a separate machine learning  model as predictors in the CNN model. Precipitation type predictors allow a single model to be used seamlessly for all precipitation types. The analysis reveals that combining predictors based on satellite and NWP data leads to improved performance, with the greatest improvement in the stratiform precipitation type. The use of probabilities of precipitation type as predictors contributes significantly to the improved performance of the quantitative precipitation retrievals. Furthermore, improvements in conditional biases are demonstrated for all precipitation rates when compared to a deterministic CNN model.

How to cite: Upadhyaya, S. A., Kirstetter, P.-E., and Kuligowski, R. J.: Machine Learning-based Probabilistic Precipitation Estimation with the GOES-16 Advanced Baseline Imager, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2945, https://doi.org/10.5194/egusphere-egu23-2945, 2023.

EGU23-2961 | Orals | AS1.25

Lessons Learned in V07 IMERG 

George Huffman, David Bolvin, Robert Joyce, Eric Nelkin, and Jackson Tan

The Global Precipitation Measurement (GPM) mission combines passive microwave (PMW) and infrared (IR) satellite data, together with other data to create the Integrated Multi-satellitE Retrievals for (IMERG) precipitation product on a (nearly) global 0.1° half-hour grid.  Experience with Version 06 datasets revealed deficiencies that the algorithm team has addressed in creating the new Version 07 datasets.

Input precipitation estimates from the Goddard Profiling (GPROF) algorithm (which retrieves precipitation from passive microwave sensor data), the GPM Combined Radar-Radiometer Algorithm (CORRA), and the new Precipitation Estimation from Remotely Sensed Information Using Artificial Neural Networks–Dynamic Infrared Rain Rate (PDIR) algorithm (retrieving precipitation from IR data) all represent advances over the V06 inputs.  For V07, several issues have been addressed, and many algorithm improvements have been implemented.  These include refining the Kalman filter to approximately preserve the local histogram of precipitation rates (Scheme for Histogram Adjustment with Ranked Precipitation Estimates in the Neighborhood, or SHARPEN), and applying the Kalman filter even when a PMW overpass occurs.  Furthermore, a long-standing bug in the geolocation that shifted grid values 0.1° to the east in the latitude band 70°N-S has been corrected.  Other changes in V07 include a hierarchical selection among motion vector sources to address deficiencies in the precipitation propagation near orography, an update to the precipitation phase specification for improved consistency with current inputs, and climatological adjustment of the near-real-time Early and Late Runs to the Final Run (which includes monthly precipitation gauge analyses).  Extensive development work was directed at unexpected biases in the V06 products, leading to 1) calibrations that now employ the entire swath widths of CORRA and GPROF GPM Microwave Imager (GMI) precipitation estimates (rather than spatially coincident data), and 2) coarsening the CORRA resolution to approximately match the GPROF-GMI footprint scale.  The latter provides more consistent histograms for building the calibrations.

It is anticipated that the retrospective analysis for V07 will be well underway at the time of the meeting.  Changes between V06 and V07 will illustrate the cumulative result of the improvements implemented in V07.  The current status of processing and plans for future development will also be discussed.

How to cite: Huffman, G., Bolvin, D., Joyce, R., Nelkin, E., and Tan, J.: Lessons Learned in V07 IMERG, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2961, https://doi.org/10.5194/egusphere-egu23-2961, 2023.

EGU23-3081 | ECS | Posters on site | AS1.25

Variation in bright band height during the passage of a typhoon observed with wind profiler radars 

Kyung Hun Lee, Byung Hyuk Kwon, Yujin Kim, Jiwoo Seo, and Geon Myeong Lee

When snow particles fall and pass through the melting layer, they melt from the surface and change into rain particles. At this time, due to the difference in permittivity between ice and water, reflectivity appears large, and this is called the bright band (BB). Since the BB causes confusion in the precipitation estimation of weather radar, many studies on BB detection have been conducted to improve the quantitative precipitation estimation accuracy of weather radar and the performance of numerical models. Wind profiler radar (WPR) is useful for vertical structure analysis of mesoscale convective systems with excellent temporal and vertical spatial resolution. We analyzed the bright band of Typhoon HAISHEN passing near the Korean Peninsula from 00 UTC on September 06 to 00 UTC on September 07, 2020 by 9-site WPR. As the HAISHEN approached, distinct precipitation patterns and BB were detected with vertical signal to noise ratio and vertical radial velocity. The BB height gradually increased as the typhoon approached, and decreased as it moved away. Therefore, the precipitation converged in the front of the typhoon and originated from a stratiform structure. It is known that the BB height depends on local factors such as ground temperature and topography. However, the BB height in Jeju Island and Chupungnyeong, located on the mountain boundary at about 240 m above sea level, showed 3-4 km and 4-5 km, respectively. In order to understand the structure of a rapidly developing precipitation cell, it is necessary to investigate the dynamic parameters which are optimal to retrieve based on WPR.

How to cite: Lee, K. H., Kwon, B. H., Kim, Y., Seo, J., and Lee, G. M.: Variation in bright band height during the passage of a typhoon observed with wind profiler radars, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3081, https://doi.org/10.5194/egusphere-egu23-3081, 2023.

EGU23-3385 | ECS | Orals | AS1.25

Evaluation of precipitation satellite products and ground-based radars during two case studies over France in 2022 

Antoine Causse, Jean-Luc Baray, Céline Planche, and Emmanuel Buisson

Precipitations are a crucial and extremely valuable source of water for humanity’s food production and for its own consumption but droughts or even floods can be potential causes of considerable damages to crops, infrastructures or properties and life-threatening situation. Precipitations are characterised by a high spatial and temporal variabilities. Hence, multiple rain gauges, precipitation radars and satellite-based estimates gridded datasets are necessary to quantify rain accumulation at local, regional and global scales.

Rain gauges observations tend to observe the amount of precipitable water locally providing rain rates for an equivalent surface of less than 1 m². Weather radars estimate the rain fields over a surface at high spatio-temporal resolution (~1km for space and several minutes for the time). Finally, the satellite-related estimates of precipitation, mainly based on the estimates made by infrared (IR) and passive or active microwave (PMW or AMW) sensors, have been developed and studied in the last decades. Moreover, new innovative satellite skills provide rain estimates from the attenuation of broadband communication satellite link signals at Ka-band.

This work evaluated the behaviour of two precipitation radar products: the French radar product PANTHERE and the pan-European radar mosaic product OPERA, and 11 satellite precipitation products: GHE, PDIR, IMERG Early v6, IMERG Late v6, CMORPH v0.x, CMORPH-RT v0.x, GSMaP-NRT v8, GSMaP-NRT-GC v8, GSMaP-NOW, GSMaP-NOW-GC and Databourg. This study has been performed against the observation made the RADOME rain gauge network with more than 500 stations over the French territory. All datasets are aggregated at hourly temporal resolution and are compared using a point-to-pixel method during two notable case studies: a 3-days April 2022 event and a 4-days June 2022 event. It is shown that radar products tend to be more reliable on the estimation of precipitation accumulation while PMW datasets tend to underestimate rain rates compared to the observations whereas IR datasets has the potential to overestimate these values.

How to cite: Causse, A., Baray, J.-L., Planche, C., and Buisson, E.: Evaluation of precipitation satellite products and ground-based radars during two case studies over France in 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3385, https://doi.org/10.5194/egusphere-egu23-3385, 2023.

EGU23-4123 | Posters on site | AS1.25

Evaluation of WRF physics ensemble performance in forecasting extreme precipitation events over Germany 

Rafaella - Eleni P. Sotiropoulou, Ioannis Stergiou, and Efthimios Tagaris

The effectiveness of numerical weather prediction models in forecasting precipitation and temperature extremes is highly dependent on the correct combination of the parameterization schemes as well as the grid resolutions used. For precipitation, the parameterization schemes of microphysics, cumulus and the planetary boundary layer are decisive for the correct forecast of the event. The WRF model is one of the most widely used numerical weather prediction models to estimate such extreme phenomena. In order to identify the optimal combination of these parameterizations for the European region, WRF is used here to simulate eight extreme precipitation events that occurred in the Schleswig–Holstein and Baden–Wurttemberg regions in Germany. The events were selected from the German Weather Service (DWD) catalog and exceeded DWD severe weather warning level 3 (i.e., precipitation > 40 mm/h – W3). A two-way nesting approach is used with 9 and 3 km spatial resolutions. The initial and boundary conditions are obtained from the ERA5 dataset at 0.25° × 0.25° resolution. To model each event, thirty different parameterization configurations were used, accounting for all possible combinations of five microphysics (MP), three cumulus (CU), and two planetary boundary layer (PBL) parameterization methods, yielding a total of 240 simulations. To determine the performance skill of each setup, the multi-criteria decision analysis Technique for Order of Preference by Similarity to Ideal Solution (TOPSIS) is employed. Six categorical and five statistical metrics are used as input in the TOPSIS algorithm to calculate each member's performance rank. The analysis conducted here revealed that an increase in the grid spatial resolution from 9 km to 3 km did not result in a substantial improvement in the accuracy of the forecast in time or in the estimation of precipitation intensity. When considering each event individually, the optimal combination, according to the TOPSIS ranking algorithm, is seasonally and geographically dependent, with specific members appearing more frequently in the top-ranking positions. When all events are treated as one to determine the best performing simulating members, the Morrison double-moment (MDM) scheme, along with the Grell-Freitas (GF) CU and the YSU PBL schemes, is found to be the most effective set up, followed by the WRF single-moment 5-class, along with the GF and the YSU schemes.

How to cite: Sotiropoulou, R.-E. P., Stergiou, I., and Tagaris, E.: Evaluation of WRF physics ensemble performance in forecasting extreme precipitation events over Germany, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4123, https://doi.org/10.5194/egusphere-egu23-4123, 2023.

EGU23-4215 | Posters on site | AS1.25

Satellite remotely-sensed data for studying the impact of climate change on crop evapotranspiration in Cyprus 

Silas Michaelides, George Papadavid, Diofantos Hadjimitsis, and Georgios Kountios

Recent studies have shown that climate change is likely to affect the agricultural sector in Cyprus. In the present study, crop water requirements in each of the 1995–2004 and 2010-2019 decades are estimated, by employing the same methodology, and subsequently compared. The aim is to investigate whether there has been any significant change regarding the crop water requirements of the most water-intensive crops in Cyprus. For the estimation of the crop evapotranspiration, the FAO Penman-Monteith methodology is used, as this has been adapted to satellite data. Remote-sensing data from Landsat TM/ETM+/OLI were employed.

Five water-intensive crops are in the focus of this research: citrus, bananas, colocasi, potatoes, and avocado. For each of these crops, estimations of the crop evapotranspiration were performed, considering three agricultural areas on the island where these crops are grown:  Pafos, Polis, and Famagusta.

The results have shown that there is no significant effect of climate variation on crop evapotranspiration, despite the fact that some climatic factors have exhibited a change on the island of Cyprus; the mean values for the most water-intensive trees/crops in Cyprus in the 1994–2004 decade have shown no significant difference from the mean values in the 2010–2019 decade, for all the crops and all agricultural areas. From the statistical analysis performed, it can be concluded that the climate change which has been documented in the past decades has not impacted significantly the crop evapotranspiration.

The authors would like to express their thanks to the Agricultural Research Institute for providing the proper resources for applying the specific methodology. Also, the authors acknowledge the ‘EXCELSIOR’: ERATOSTHENES: EΧcellence Research Centre for Earth Surveillance and Space-Based Monitoring of the Environment H2020 Widespread Teaming project (www.excelsior2020.eu). The ‘EXCELSIOR’ project has received funding from the European Union’s Horizon 2020 research and innovation programme under Grant Agreement No 857510, from the Government of the Republic of Cyprus through the Directorate General for the European Programmes, Coordination and Development and the Cyprus University of Technology.

How to cite: Michaelides, S., Papadavid, G., Hadjimitsis, D., and Kountios, G.: Satellite remotely-sensed data for studying the impact of climate change on crop evapotranspiration in Cyprus, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4215, https://doi.org/10.5194/egusphere-egu23-4215, 2023.

EGU23-4247 | Orals | AS1.25

Statistical uncertainty analysis-based precipitation merging (SUPER): A new framework for improved global precipitation estimation 

Jianzhi Dong, Wade T.Crow, Xi Chen, Natthachet Tangdamrongsub, Man Gao, Shanlei Sun, Jianxiu Qiu, Lingna Wei, Hongkai Gao, and Zheng Duan

Multi-source merging is an established tool for improving large-scale precipitation estimates. Existing merging frameworks typically use gauge-based precipitation error statistics and neglect the inter-dependence of various precipitation products. However, gauge-observation uncertainties at daily and sub-daily time scales can bias merging weights and yield sub-optimal precipitation estimates, particularly over data-sparse regions. Likewise, frameworks ignoring inter-product error cross-correlation will overfit precipitation observation noise. Here, a Statistical Uncertainty analysis-based Precipitation mERging framework (SUPER) is proposed for addressing these challenges. Specifically, a quadruple collocation analysis is employed to estimate precipitation error variances and covariances for commonly used precipitation products. These error estimates are subsequently used for merging all products via a least-squares minimization approach. In addition, false-alarm precipitation events are removed via a reference rain/no-rain time series estimated by a newly developed categorical variable merging method. As such, SUPER does not require any rain gauge observations to reduce daily random and rain/no-rain classification errors. Additionally, by considering precipitation product inter-dependency, SUPER avoids overfitting measurement noise present in multi-source precipitation products. Results show that the overall RMSE of SUPER-based precipitation is 3.35 mm/day and the daily correlation with gauge observations is 0.71 [−] – metrics that are generally superior to recent precipitation reanalyses and remote sensing products. In this way, we seek to propose a new framework for robustly generating global precipitation datasets that can improve land surface and hydrological modeling skill in data-sparse regions.

How to cite: Dong, J., T.Crow, W., Chen, X., Tangdamrongsub, N., Gao, M., Sun, S., Qiu, J., Wei, L., Gao, H., and Duan, Z.: Statistical uncertainty analysis-based precipitation merging (SUPER): A new framework for improved global precipitation estimation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4247, https://doi.org/10.5194/egusphere-egu23-4247, 2023.

This study evaluates efficacy of rainfall kinetic energy (KE) and rain intensity (I) relationship through field observations under different wind conditions.  KE-I relationship is critical for various applications.  For example, rain-induced soil erosion, for which KE is an important indicator of potential rain splash erosion, may cause severe environmental and agricultural issues during, especially, heavy rainfall events.  Fertilizers removed from the soil due to rain-induced erosion pollute waterbodies, silt up the basin, and reduce basin capacity that may trigger flooding.  In this study, the KE-I relationship was investigated using raindrop size and fall speed measurements by a disdrometer and wind speed measurements by a 3D Ultrasonic anemometer.  Rainfall events considered in this study were selected from a 3-year long field campaign conducted at our outdoor rainfall laboratory located on the West campus of the University of Texas at San Antonio, Texas, USA.  Using these measurements, different KE-I relationships reported in the literature were evaluated through statistical analyses.  A new parameterization for the KE-I relationship was also developed based upon our field observations, and wind-induced effects on KE-I relationship are discussed.  The results of this investigation with potential implications will be discussed in this presentation.  This material is based upon work supported by the National Science Foundation under Grants No. AGS-1741250.

How to cite: Testik, F. and Saha, R.: Assessing Rainfall Kinetic Energy – Rain Intensity Relationship through Field Observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4299, https://doi.org/10.5194/egusphere-egu23-4299, 2023.

This study investigated the impacts of low-level thermodynamic structure and water vapor on heavy rainfall events in the southern Korean Peninsula during the 2016 summer intensive observation period. An intensive dataset of mobile observation vehicle (MOVE), with high temporal resolution rawinsonde soundings and global navigation satellite system (GNSS) observations in Geochang (GC) supersite, was used. We divided study events into two heavy rainfall cases to compare the characteristics of representative summer heavy rainfall with different synoptic conditions. Case 1 has localized heavy rainfall associated with the Changma (summer monsoon) and Case 2 has convective instability. The temporal behavior of precipitable water vapor (PWV) retrieved from the MOVE-GNSS data demonstrated that during Case 1, heavy rainfall events experience a steep decrease after a long increasing trend. However, the most intense rainfall events occurred after a rapid increase in PWV during Case 2. In Case 1, the mean static stability at >2 km altitude was variable for all periods (in the order of after > before > during rainfall), whereas in Case 2, this was less variable with time and had generally higher convective instability close to the surface, compared with Case 1. In addition, Case 1 demonstrated the progression of a vertical wind structure connected with a quasi-stationary frontal passage (e.g., veering winds at low levels before rainfall), whereas Case 2 demonstrated a nearly homogeneous southwesterly wind from the surface to an altitude of 5 km.

How to cite: Kim, Y.-J. and Lim, B.: Study on the thermodynamic characteristics of heavy rainfall events in the southern Korean Peninsula, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4680, https://doi.org/10.5194/egusphere-egu23-4680, 2023.

EGU23-4687 | Orals | AS1.25

JAXA Earth Observation Overview for measuring the Global Water Cycle 

Riko Oki, Takuji Kubota, Misako Kachi, Kosuke Yamamoto, and Moeka Yamaji

Japan Aerospace Exploration Agency (JAXA) currently operates six Earth observation missions for water cycle and climate studies, disaster mitigation, and various application studies including weather forecasts. One of six missions, the Global Precipitation Measurement (GPM) is an international mission to achieve highly accurate and highly frequent global precipitation observations (Hou et al. 2014, Skofronick-Jackson et al. 2017). The GPM mission consists of the GPM Core Observatory jointly developed by U.S. and Japan and Constellation Satellites that carry microwave radiometers and provided by the GPM partner agencies. The GPM Core Observatory, launched on February 2014, carries the Dual-frequency Precipitation Radar (DPR) by JAXA and the National Institute of Information and Communications Technology (NICT) (Kojima et al. 2012, Iguchi 2020).

 

Regarding future satellite missions, Global Change Observation Mission - Water "SHIZUKU" (GCOM-W) follow-on mission (AMSR3) with high-frequency channels (166 & 183 GHz) will be installed on the Global Observing Satellite for Greenhouse gases and Water cycle (GOSAT-GW) satellite (Kasahara et al. 2020). Japan will provide the world's first satellite-based cloud vertical motion information by the Cloud Profiling Radar (CPR) to the Earth Clouds, Aerosols and Radiation Explorer (EarthCARE), Europe-Japan joint mission (Illingworth et al. 2015, Wehr et al. 2023). JAXA is currently conducting R&D of the Precipitation Measuring Mission carrying the Ku-band Doppler Precipitation Radar to succeed and expand currently operating GPM/DPR.

 

It is also required to evolve combined use of multi-satellite to provide the “best” information to users. Under the GPM mission, the Global Satellite Mapping for Precipitation (GSMaP) produces high-resolution and frequent global rainfall map based on multi-satellite passive microwave radiometer observations with information from the Geostationary InfraRed (IR) instruments (Kubota et al. 2020). Output product of GSMaP algorithm is 0.1-degree grid for horizontal resolution and 1-hour for temporal resolution. The GSMaP near-real-time version product (GSMaP_NRT) has been in operation at JAXA since November 2007 in near-real-time basis, and browse images and binary data available at JAXA GSMaP web site (http://sharaku.eorc.jaxa.jp/GSMaP/).

JAXA also collaborates with model development community to expand satellite data utilization in various fields. With the goal of providing reliable water cycle information and achieving integrated water resources management, JAXA has developed the global hydrological simulation system “Today’s Earth (TE)” under the joint research with University of Tokyo (Ma et al. 2021). To provide the products with better accuracy, rainfall from the GSMaP is used for TE-Global GSMaP version. The Over 50 hydrological variables are now accessible through the web page and ftp site of the “TE-Global” system (https://www.eorc.jaxa.jp/water/).

JAXA continues to provide useful satellite-based information related to the global water cycle.

How to cite: Oki, R., Kubota, T., Kachi, M., Yamamoto, K., and Yamaji, M.: JAXA Earth Observation Overview for measuring the Global Water Cycle, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4687, https://doi.org/10.5194/egusphere-egu23-4687, 2023.

EGU23-4731 | Posters on site | AS1.25

Estimation of raindrop size distribution from polarimetric radar measurements at C-band 

Ahoro Adachi, Takahisa Kobayashi, and Akihito Umehara

Many studies have proposed methods to estimate the raindrop size distribution (DSD) parameters from polarimetric radar data as a part of rain attenuation correction and/or rainfall rate estimation algorithms, in which a modified gamma distribution model has been often used to characterize the natural variation of DSD. The parameters that determine the modified gamma DSD are a shape parameter μ, median volume diameter D0 or slope parameter Λ, and a number concentration N0 or its normalized version NW. While D0 (or Λ) and NW can be retrieved relatively straightforward from the polarimetric radar measurements, estimation of shape parameter is not an easy task. Instead, empirical relations including μ-Λ and/or μ-D0 relations derived from surface measurements of DSD are widely used to estimate μ implicitly.

   Adachi et al. (2015) proposed a method to estimate the three parameters of the DSD from polarimetric radar data without any assumptions of relationship among the parameters. In that method, they assumed a constant shape parameter in a range profile. However, this assumption may not be satisfied if the radar is sampling mixed convective/stratiform echoes that simultaneously exist in a single profile. Theoretically, on the other hand, a shape parameter can be estimated from a correlation coefficient ρHV at each range gate (e.g., Thurai et al. 2008). However, to estimate shape parameters with a method of this kind, it is necessary to obtain a correlation coefficient with quite high accuracy, for which a very long sampling time is needed to apply it to radars to satisfy this condition for most radar measurements. The MRI C-band polarimetric radar is equipped with solid-state transmitters, which enable the radar to make observations of correlation coefficient with high accuracy in a relatively short time, especially in high-SNR regions. Thus, we have developed an algorithm to estimate a shape parameter at each range gate both from correlation coefficient and differential reflectivity along with D0 and NW, and compared it with surface measurements.

How to cite: Adachi, A., Kobayashi, T., and Umehara, A.: Estimation of raindrop size distribution from polarimetric radar measurements at C-band, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4731, https://doi.org/10.5194/egusphere-egu23-4731, 2023.

Raindrop size distributions (DSDs) are the main tool for describing and discussing rain microphysics. They play a crucial role in remote sensing of precipitation and extensive efforts have been devoted to measuring and modeling them. However, when it comes to DSDs in extreme rain, very few, reliable, results are available. Using numerical simulations, Srivastava (1978, 1982) and List (1988) theorized that for high enough rainfall intensities (>40 mm/h), DSDs should converge toward a stationary state where drop coalescence and breakup are in dynamical equilibrium with each other. In such conditions, the shape of the DSDs should be constant and the particle number concentration should be proportional to the rain rate. However, reliable evidence of such transitions toward a “number-controlled” remains scarce and many researchers have contested its existence.

In this study, high-quality DSD observations from a network of 7 optical disdrometers belonging to the Ruisdael observatory for Dutch atmospheric science are used to take a new, fresh look at the issue. The main research questions are:

  • Is there empirical evidence for a transition from size to number-controlled regimes at high rainfall intensities in the Netherlands?
  • What parametric model best fits DSDs at high rainfall rates?
  • Can the super-CC scaling of sub-hourly rainfall extremes with temperature highlighted by Lenderink et al. (2008) be explained by changes in DSDs?

To address the questions above, we analyze characteristic drop sizes (Dm, D0), number concentrations (NT, Nw) and state variables (LWC, Z, Zdr) for different classes of rainfall intensities and temperatures and study the shape of DSDs by comparing the goodness of fit of various parametric DSD models. We look at non-parametric descriptors such as the relative number of small versus large drops and study the scaling laws linking different moments of the DSD in heavy rain using single and double-normalization frameworks to assess possible convergence toward number-controlled regime at higher intensities.

How to cite: Schleiss, M.: The microstructure of heavy rainfall in the Netherlands, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4933, https://doi.org/10.5194/egusphere-egu23-4933, 2023.

EGU23-5291 | ECS | Orals | AS1.25

Understanding the Polarimetric Radio Occultation observable differential phase shift with the help of the NEXRAD polarimetric weather radars 

Antía Paz Carracedo, Ramon Padullés Rulló, and Estel Cardellach Galí

Lack of knowledge about the physical processes controlling heavy precipitation arises from the limited number of simultaneous observations of the vertical structure of precipitation and its thermodynamic environment. These limitations are caused by the degradation that the signals of some spaced-based sensors suffer in presence of thick clouds or the lack of high vertical resolution thermodynamic measurements.
To overcome this problem, the ROHP (Radio Occultation and Heavy Precipitation) experiment provides high-quality thermodynamic profiles (temperature, pressure, water vapor pressure, etc.) and vertical information of the hydrometeors, simultaneously. This proof-of-concept experiment led by the Institut de Ciències de l’Espai (ICE-CSIC, IEEC) in collaboration with NOAA, UCAR, and NASA/Jet Propulsion Laboratory, is carried out aboard the Spanish low earth orbiter (LEO) PAZ. Its objective is to test the new Polarimetric Radio Occultation (PRO) concept, and it has been operating since 2018. The standard radio occultation technique consists of tracking the signals emitted by a Global Navigation Satellite System (GNSS) satellite from a LEO satellite that is rising or occulting behind the Earth’s limb. The novelty that PRO offers is that GNSS signals are collected using two different linearly polarized antennae (horizontal and vertical) as opposed to the standard technique, where GNSS signals are acquired using a circularly polarized antenna. Consequently, we can obtain an observable called the differential phase shift, defined as the difference in the accumulated phase delay between both polarizations (H-V). Since the hydrometeors surrounding heavy precipitation events stand out for being oblate spheroid-like, we will have an associated accumulated phase shift if rays are crossing heavy precipitation.
For the sake of continuing with the validation of the PRO technique, we make use of the polarimetric weather data provided by the Next Generation Weather Radars (NEXRAD). NEXRAD is the network of dual-polarized Doppler radars operating at the S-band, that covers all the United States territory. By comparing the differential phase shift obtained with PAZ and the observables from NEXRAD, we can analyze the polarimetry of both systems. In this study, we focus on the vertical structures of NEXRAD-provided specific differential phase shift (Kdp) that can be compared to the PAZ observable accounting for some geometry and frequency factors. This comparison will help us to better understand the PAZ observables, and ultimately to better understand the microphysics underlying heavy precipitation events.

How to cite: Paz Carracedo, A., Padullés Rulló, R., and Cardellach Galí, E.: Understanding the Polarimetric Radio Occultation observable differential phase shift with the help of the NEXRAD polarimetric weather radars, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5291, https://doi.org/10.5194/egusphere-egu23-5291, 2023.

EGU23-5356 | Orals | AS1.25

Trends of precipitation variables on different datasets 

Romana Beranova and Radan Huth

It is a well-established fact that different types of data (station, gridded, reanalysis) possess different statistical characteristics, e.g. for higher-order moments, extremes, and trends. In this contribution we examine the long-term changes in precipitation characteristics on different data sources over Europe. We calculate and display differences between the datasets and attempt to identify causes for the differences and for specific behavior of the datasets. We used data from stations across Europe (ECA&D project), gridded data (E-OBS) and reanalysis (NCEP/NCAR, JRA-55). We mainly analyze the trends of the seasonal total amount, intensity and probability of precipitation. Long-term trends of seasonal values of precipitation variables and their statistical significance are calculated by non-parametric methods (Mann-Kendall test, Kendall statistic). The analysis is conducted on a seasonal basis, with emphasis on winter and summer. We found that each of the datasets has its advantages and drawbacks. Trends in reanalysis deviate considerably from the other datasets mainly because the type and amount of data assimilated into them change in time. The weakness of the grid data sets is the unstable number of stations entering the interpolation in time, and the lack of representativeness of some climate stations is the main disadvantage of the station data.

How to cite: Beranova, R. and Huth, R.: Trends of precipitation variables on different datasets, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5356, https://doi.org/10.5194/egusphere-egu23-5356, 2023.

EGU23-5822 | ECS | Orals | AS1.25

Analysis of Precipitation Extremes Using High Resolution Ensemble-based Dataset for India 

Anagha Peringiyil and Manabendra Saharia

Grid-based meteorological estimates are indispensable in a wide variety of contexts. In India, most of the existing precipitation datasets are deterministic and have limitations when it comes to expressing the inherent uncertainties in data. Existing gridded datasets for India were created using a similar process, which comprised a multi-stage quality check, followed by methods such as Shepard's interpolation and probabilistic interpolation. This paper focus on the development of ensemble based gridded product for India named as, Indian Meteorological Ensemble Dataset (IMED) for 30 years. Additionally, this paper also discusses the analysis of precipitation extremes over Indian region. IMED (Indian Meteorological Ensemble Dataset) creates a daily ensemble precipitation product for the specified grid using gauge station readings as input, together with spatial variables such as latitude, longitude, elevation, and slope for the period of 30 years from 1991 to 2020. Daily, thirty distinct ensemble members are generated with a resolution of 0.25 degrees. IMD (Indian Meteorological Department) gridded precipitation data, CHIRPS gridded precipitation data and ERA5 land precipitation are compared with the mean of the developed ensemble members. In addition, a sensitivity analysis carried out to find out the possible combination of input parameters such as search radius, number of neighbouring stations to be considered, and number of ensembles to be used etc. and found that the combination 80, 25, 30 respectively gives better performance in terms of the quality of developed dataset as well as the time complexity. The generated ensemble has generally strong reliability and discrimination of events of different magnitudes and it is comparable to other widely used hydrometeorological datasets, although there are significant distinctions. The correlation coefficient between IMED and station precipitation data is 0.972, which is greater than the correlation coefficient between IMD gridded precipitation data and station precipitation data. Ensemble precipitation datasets are especially useful in places with substantial meteorological uncertainty, since practically all available deterministic datasets encounter formidable difficulties in obtaining reliable estimations.

How to cite: Peringiyil, A. and Saharia, M.: Analysis of Precipitation Extremes Using High Resolution Ensemble-based Dataset for India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5822, https://doi.org/10.5194/egusphere-egu23-5822, 2023.

EGU23-5991 | Posters virtual | AS1.25

A wind tunnel investigation on the ventilation coefficients of hailstones 

Alexander Theis, Laura Werner, Subir Mitra, Stephan Borrmann, and Miklós Szakáll

The rate of change of mass of a hailstone by diffusion is affected by its motions. In a stationary pure diffusive case the water vapor distribution around a spherical hailstone is spherically symmetric having rather weak water vapor gradients. However, when a hailstone falls in the air, the flow field and hence the water vapor distribution around the hailstone is asymmetric showing much stronger water vapor gradients which are high at the upstream side and lower at the rear side of the hailstone. When averaged over the whole surface area of the hailstone the mass transfer to or from the falling hailstone surface is always higher compared to a pure diffusive case. This convective enhancement is given by the ventilation coefficient. Thus, to reliably quantify growth or sublimation rates of falling hailstones with models, it is necessary to know their ventilation coefficients. The rate of change of mass is proportional to the rate of change of heat. Therefore, the growth or sublimation of hailstones has not only implications on the humidity of the ambient air but also the vertical temperature profile of the atmosphere and consequently cloud and storm dynamics.

However, there is a lack of experimental studies on the ventilation coefficient of spherical hailstones in the literature. There are just three experimental studies available – all dating back to the 1960’s – which investigate the heat and mass transfer of spherical and oblate hailstones, but all were measured under accretional growth and melting conditions, respectively.

Therefore, experiments in the Mainz vertical wind tunnel were carried out to determine ventilation coefficients of spherical hailstones during sublimation. We investigated stones with diameters between 1 and 3 cm or, equivalently, Reynolds numbers between 10.000 and 45.000. The spherical hailstones were produced by freezing water in moulds and introduced into the wind tunnel. While freely floating at their terminal velocities the hailstones lost mass due to sublimation. The temperature in the tunnel was set to -5°C and relative humidities were rather low, i.e. between 30 % and 50 % with respect to ice, to facilitate sublimation. The mass of the hailstones was measured before and after the wind tunnel measurements from which we calculated the rate of change of mass in the convective case. The recordings of temperature and dew point were used to calculate the rate of change of mass for the pure diffusive case. The ratio of these rates is, by definition, the ventilation coefficient, which was calculated and parameterized as a function of the Reynolds number.

How to cite: Theis, A., Werner, L., Mitra, S., Borrmann, S., and Szakáll, M.: A wind tunnel investigation on the ventilation coefficients of hailstones, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5991, https://doi.org/10.5194/egusphere-egu23-5991, 2023.

EGU23-6110 | Orals | AS1.25

Twenty years of radar data from a single C-band radar - Potentials and drawbacks in rainfall statistics 

Søren Thorndahl and Christoffer Bang Andersen

In terms of spatial and temporal information, weather radar data offers notable advantages when used for rainfall statistics compared to rain gauge records. In the past, long-term statistics were only possible through the use of rain gauge records. However, the availability of more than one decade of radar data now allows for a more detailed analysis of rainfall variability in both space and time.

For radar-based statistical analyses to be a reliable alternative to rain gauge statistics, it is essential to have high-quality, consistent data that is free of errors. While advancements in technology, such as dual polarimetric estimation, have improved our ability to quantify rainfall intensities with radar, it is still necessary to utilize "ground truth" records from rain gauges to adjust and ensure the accuracy of the radar estimates. In extreme value statistics where long-term continuous records are required, it is necessary to not only utilize the latest technology but also to adjust and verify older data (e.g. pre dual-pol. data or data with lower spatial and temporal resolution)

This abstract present data from a 20-year radar series single radar from Denmark, where several analyses with regard to rainfall statistics have been conducted. We describe and quantify challenges in bias adjustment, advection interpolation to improve temporal resolution, duration-dependent biases, spatial scaling issues comparing points and pixels, subpixel variability, range dependence in rainfall estimates, etc.

We apply the data to develop extreme value statistics based on peak-over-threshold ranking and stochastic storm transposition. Furthermore, we examine spatial variability using radar-based areal reduction factors as well as spatial correlation analyses and severity diagrams. The analyses and application of radar data are conducted with an aim towards application in urban hydrology.

How to cite: Thorndahl, S. and Andersen, C. B.: Twenty years of radar data from a single C-band radar - Potentials and drawbacks in rainfall statistics, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6110, https://doi.org/10.5194/egusphere-egu23-6110, 2023.

EGU23-6374 | ECS | Posters on site | AS1.25

Characterization of Extreme Rainfall Events Classes in the Tropical Andes by Using Weather Radar Data 

Gabriela Urgilés, Johanna Orellana-Alvear, Jörg Bendix, and Rolando Célleri

Extreme rainfall is characterized by a high spatio-temporal variability. This variability is exacerbated in mountain areas, such as the tropical Andes, where the complex orography and mesoscale atmospheric processes have an enormous influence on the rainfall processes. Particularly the analysis of extreme rainfall events in the Ecuadorian Andes has remained a challenge due the lack of high spatio-temporal resolution operational observing systems. However, the recent availability of rainfall radar data in this area enables an improvement of our knowledge about those extremes. Here, we presented a study that aims to identify specific types of extreme rainfall events based on a clustering approach and to analyze their spatio-temporal characteristics. The study is based on three years of data collected from an X-band scanning weather radar that was located at 4450 m a.s.l in the Tropical Andes of southern Ecuador, delivering high resolution (5min, 500m) data. Several extreme rainfall events were identified, which were selected based on a rainfall accumulation threshold and visual inspection. Then, extreme rainfall events characteristics (e.g., rain rate, duration, rainfall accumulation, hour and month of occurrence) were identified for each event. Then, the k-means clustering was applied to the events using their rainfall characteristics. The main idea of this algorithm is to cluster a set of objects by accounting for their similarities. In our presentation, we will show the three major types of extreme rainfall events resulting from our analysis as well as the marked differences in their rainfall characteristics. The first type of extreme-events showed the highest values of intensity and the lowest values of duration. Also, two extreme-events types showed predominant months and hours of occurrence. In addition, the site of occurrence of the spatial nucleus of maximum intensity of the first type was located at higher elevations. We will show that the typology of extreme rainfall events improves our knowledge about the spatio-temporal characteristics in the tropical Andes. 

How to cite: Urgilés, G., Orellana-Alvear, J., Bendix, J., and Célleri, R.: Characterization of Extreme Rainfall Events Classes in the Tropical Andes by Using Weather Radar Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6374, https://doi.org/10.5194/egusphere-egu23-6374, 2023.

EGU23-6602 | ECS | Orals | AS1.25

Assessment of preselected Satellites and Reanalysis Precipitation Products using ground observations over the Upper and the Middle Drâa catchment, central-east of Morocco. 

Athmane Khettouch, Mohammed Hssaisoune, Thomas Hermans, Aziz Aouijil, and Lhoussaine Bouchaou

In most ungauged areas, validation of precipitation gridded satellite products is fundamental to provide precipitation information with high accuracy and spatial-temporal resolution. Drâa river basin (DRB) in southeastern Morocco is one of ten driest watersheds worldwide with a limited network of rain-measured stations. However, literatures investigations have shown the necessity of strong climatic datasets to conduct water resources management. In this study, five satellite precipitation products with high spatio-temporal resolution were evaluated including: the latest version of Climate Hazards Group InfraRed Precipitation with Stations (CHIRPS V2.0), the atmospheric reanalysis dataset for the global climate by the ECMWF (ERA5-Land), the latest version of Multi-Source Weighted-Ensemble Precipitation (MSWEP V2.2), Precipitation Estimation from Remotely Sensed Information using Artificial Neural Networks-Cloud Classification System-Climate Data Record (PERSIANN-CCS-CDR) and Tropical Applications of Meteorology using SATellite data and ground-based observations (TAMSAT V3.1). The evaluation was conducted in terms of their performance in capturing occurred precipitation events and reliable amounts. The Monthly and seasonal precipitation amounts determined by these products at different altitude levels were evaluated against available rain gauge observations for a period of 81 months using point-to-pixel method and with reference to continuous, categorical and volumetrics indices. The only available station belonging to SYNOP weather network (Surface Synoptic Observations) with more than 40 years of data was included to advance our conclusion regarding the performance of a given P-dataset. The achieved results show that the best performance was obtained for ERA5-Land and MSWEP V2.2 for monthly and seasonal time-step, respectively, while CHIRPS V2.0 followed by TAMSAT V3.1 and PERSIANN-CCS-CDR perform the worst. The expected results will cover the performance of each P-dataset for different sub-seasons, elevation, intensities and their ability to detect extreme rain events. The outcomes of this investigation provide valuable information in one of the most scarcely gauged and arid Moroccan watersheds, indicating which P-dataset could be an alternative to rain gauges measurement.

Key words: Drâa river basin (DRB), ungauged arid areas, precipitation satellite products, ground observations. 

How to cite: Khettouch, A., Hssaisoune, M., Hermans, T., Aouijil, A., and Bouchaou, L.: Assessment of preselected Satellites and Reanalysis Precipitation Products using ground observations over the Upper and the Middle Drâa catchment, central-east of Morocco., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6602, https://doi.org/10.5194/egusphere-egu23-6602, 2023.

EGU23-6662 | ECS | Orals | AS1.25

The High lAtitude sNowfall DEtection aLgorithm for ATMS (HANDEL-ATMS): a new algorithm for snowfall retrieval at the high latitudes 

Andrea Camplani, Daniele Casella, Paolo Sanò, and Giulia Panegrossi

Snowfall detection and quantification are challenging tasks in the Earth science field. Ground-based instruments provide only punctual measurements, and therefore the development of satellite-based snowfall retrieval methods is necessary for the implementation of a global monitoring system of snowfall. In particular, Passive Microwave (PMW) radiometric measurements are used for snowfall remote sensing: the retrieval is based on the scattering effect of the snowflakes visible in the high-frequency channels (> 80 GHz) on the upwelling radiation. However, the detection is made difficult by the weakness of this signature and by the contamination by the background surface emission/scattering signal. This phenomenon is particularly evident at high latitudes, where the prevalence of very light snowfall events and the extremely cold and dry environmental conditions make snowfall retrieval very difficult. The exploitation of operational microwave sounders on near-polar orbits such as the Advanced Technology Microwave Sounder (ATMS) allows for a very good coverage at high latitudes. Moreover, the wide range of channels (from 22 GHz to 183 GHz), allows for a radiometric characterization of the surface at the time of the overpass.

In this work the High lAtitude sNow Detection and rEtrieval aLgorithm for ATMS (HANDEL-ATMS), a new snowfall retrieval algorithm developed especially for high latitude environmental conditions and based on the ATMS observations, is described. The algorithm is based on the use of ATMS-CPR coincidence dataset, i. e. a dataset where each ATMS multichannel observation is associated with a vertical snow profile obtained by the CloudSat Cloud Profiling Radar (CPR) and therefore it is possible to analyze the relationship between the vertical precipitation structure and the PMW measurements in a direct way, without using simulated datasets.

The algorithm is composed of three main modules. The first module, based on the PMW Empirical clod Surface Classification Algorithm (PESCA), exploits ATMS low-frequency channel observations to obtain the surface classification and radiometric characterization at the time of the overpass. The second module estimates a set of clear-sky simulated brightness temperatures (TBs) by exploiting the previously derived surface radiometric properties. The clear-sky TBs set is compared with the observed TBs to highlight the snowfall signature. The third module is composed of four neural networks, which have been tuned against the CPR snowfall products. These networks, which exploit the deviation of the ATMS TBs from the clear-sky simulated TBs and the PESCA surface classification flag as inputs, return as outputs a snowfall detection flag and the surface snowfall rate estimate. HANDEL-ATMS shows very good detection capabilities - POD = 0.83, FAR = 0.18 and HSS=0.68. Estimation error statistics show an overestimation of very light snowfall events, but a good agreement for more intense events with respect to CPR snowfall products. The analysis of the results for an independent ATMS-CPR coincidence dataset and of selected snowfall events evidence the capability of HANDEL-ATMS to well detect and estimate snowfall also in presence of extreme environmental conditions typical of higher latitudes – dry and cold atmosphere and snow-covered background surface.

How to cite: Camplani, A., Casella, D., Sanò, P., and Panegrossi, G.: The High lAtitude sNowfall DEtection aLgorithm for ATMS (HANDEL-ATMS): a new algorithm for snowfall retrieval at the high latitudes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6662, https://doi.org/10.5194/egusphere-egu23-6662, 2023.

Due to its geographic location and unique climatic circumstances, the Galápagos archipelago is renowned for its exceptional and high endemic biodiversity. Nevertheless, due to limited access to the permanent freshwater body in the archipelago, the freshwater budget is almost exclusively dependent on precipitation. However, with the lack of spatial and temporal distribution of rainfall information, it is not easy to understand the short- and long-term dynamics of rainfall in the Galápagos.

The poster presents the new satellite-based rainfall retrieval algorithm, the Galápagos Rainfall Retrieval (GRR), which offers the potential for a high spatio-temporal resolution (2 km, 10 min) rainfall product in near real-time for the Galápagos archipelago.

The algorithm is proposed to combine physical methods with machine learning in which sequences of Geostationary Earth Orbit infrared (GEO-IR) images are used to retrieve both cold season Garua drizzle and warm season convective rainfall.

In the first step, a threshold technique and spectral differences are used to identify the cloudy regions and distinguish the low, middle, and high clouds. Next, the cloud-covered region will go under a different entity-based classification method (e.g., slope test/ML algorithm) for each cloud type to detect the low stratus/Garua drizzle and potentially convective core regions. The next test follows for all detected potentially convective core regions based on cloud formation over time and space to examine whether they are likely to be decaying. If the convective core is classified as decaying, it is labelled stratiform rain; otherwise, it is labelled as the active convective core.

Finally, the rainfall assignment will be performed by training the random forest regression models. The convective and stratiform cells will be trained based on microwave-only IMERG-V06 rainfall data separately, meanwhile the cloudsat would be used to train the rainfall rate for the Garua detected regions.  By the end, all of these steps are combined together as GRR product. The algorithm of GRR product will be developed for the time period 1/1/2022-1/1/2023 and then it would be applied to the entire available GOES-16 dataset.

The validation will be conduct by: i) independent microwave-only IMERG-V06 rainfall data/cloudsat not used for model training ii) recently installed automated weather stations (AWS) network with high temporal resolution of 10 minutes covering a W-E and luff-lee transects over three islands (Isabela, S. Cruz, S. Cristóbal).

How to cite: Turini, N., Delgado Maldonado, B., and Bendix, J.: High spatio-temporal rainfall algorithm over Galápagos archipelago using multispectral GOES-16 infrared brightness temperatures: the GRR product, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6938, https://doi.org/10.5194/egusphere-egu23-6938, 2023.

EGU23-7215 | ECS | Orals | AS1.25

Assessing the wind-induced bias for an impact disdrometer using numerical simulation and wind tunnel experiments 

Enrico Chinchella, Arianna Cauteruccio, and Luca G. Lanza

Wind is a recognised source of environmental bias in precipitation measurements, affecting both catching and non-catching instruments. The latter are a family of precipitation measuring instruments that do not require the collection of hydrometeors inside a reservoir (see e.g., Lanza et al., 2021). All instruments behave like bluff-body obstacles when exposed to wind and produce strong velocity gradients and turbulence near their sensing volume, with considerable impact on the measurement accuracy.

Among them, impact disdrometers present a roughly cylindrical shape, sometimes not fully radially symmetric, and operate by measuring the kinetic energy of incoming hydrometeors. In this work, the wind-induced measurement bias is assessed for the Vaisala WXT-520 gauge, for liquid precipitation, using Computational Fluid Dynamics (CFD) simulation and a Lagrangian Particle Tracking (LPT) model.

The OpenFOAM software was used to run CFD simulations, considering three different wind directions and seven different wind speeds (1, 2.5, 5, 7.5, 10, 15 and 20 m/s). CFD results showed significant updraft upstream of the instrument sensing area and a limited dependency on the wind direction. The numerical model was further validated using wind tunnel measurements performed in the DICCA laboratory on a real gauge.

The obtained airflow field was used as the basis for an uncoupled LPT model to compute trajectories of drops of various diameters (0.25, 0.5, 0.75 and from 1 to 8 mm) while approaching the instrument sensing area. Drops were injected in the simulation domain, starting from a regular grid, with a vertical velocity equal to their terminal velocity and a horizontal velocity equal to the undisturbed wind speed.

A Kinematic Catch Ratio (KCR) is defined as the ratio between the kinetic energy transferred to the sensor in windy conditions and the kinetic energy that would have been transferred in still air conditions. Results shows that at low wind speed (1 and 2.5 m/s) the reduction in fall velocity produced by the updraft reduces the total kinetic energy, resulting in KCR < 1, especially for the smaller drops. However, the increase in kinetic energy experienced by drops carried by strong wind is predominant with respect to the updraft, resulting in KCR values much larger than unity.

Analogously, the Kinematic Collection Efficiency (KCE) can be defined once a Drop Size Distribution (DSD) is chosen. KCE values showed a similar behaviour, with values close to unity at low wind speed, but significantly larger when increasing the wind speed.

Wind also affects the DSD sensed by the instrument, since drops with increased kinetic energy are detected as having a larger diameter. Therefore, the gauge tends to overestimate the number of drops at each drop size bin, showing a shift of the DSD towards the larger diameters, that increases with increasing the wind speed.

References:

Lanza, L. G., Merlone, A., Cauteruccio, A., Chinchella, E., Stagnaro, M., Dobre, M., ... & Parrondo, M. (2021). Calibration of non‐catching precipitation measurement instruments: A review. Meteorological Applications, 28(3), e2002. https://doi.org/10.1002/met.2002

How to cite: Chinchella, E., Cauteruccio, A., and Lanza, L. G.: Assessing the wind-induced bias for an impact disdrometer using numerical simulation and wind tunnel experiments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7215, https://doi.org/10.5194/egusphere-egu23-7215, 2023.

The Tibetan Plateau (TP) plays a vital role in Asian hydrological climate. However, there is a lack of quantitative estimate on TP’s effect on snowfall over China. Some trending views include that the TP acts as a giant wall, blocking cold outbreaks and protecting southern China from severe snowstorm. Here, through topography experiments with and without the TP, we demonstrate that, compared to the world without the TP, the presence of the TP decreases snowfall in northern China by 60% due to drastically reduced moisture, while it promotes snowfall in southern China by 1500%, especially from November to March, through attracting cold air from the north and moisture from the south to southern China. The presence of the TP increases winter relative humidity substantially in southern China, which reduces human comfort. This work refutes some trending views and helps us correctly recognize TP’s role in China’s winter climate.

How to cite: Wang, L. and Yang, H.: Tibetan Plateau increases the snowfall in southern China: a refutation to some trending views, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7526, https://doi.org/10.5194/egusphere-egu23-7526, 2023.

Quantitative precipitation estimates obtained from satellite data are of critical importance to research and applications. Not only is precipitation a key component of important water and energy cycles, but the immediate societal benefits offered by reliable products are undeniable.

The complex terrain of the Peruvian Andes creates significant challenges to precipitation retrievals from space and to the establishment of dense ground monitoring networks. Nonetheless, for the communities and authorities of the region (home to nearly one third of the Peruvian population), this information is vital.

The performance of the quasi-global Integrated Multi-Satellite Retrievals for Global Precipitation Measurement (IMERG) V06 was assessed in Peru as part of Project e-Andes. Data covering the period between 2011 and 2020 were compared against gauge data from 35 stations maintained by SENAMHI. The gauges are located in the Andes and arid Pacific coast. Mean Pearson correlation values ranged from 0.34 (Early, Daily), to 0.80 (Final, Monthly), showing a clear improvement with temporal aggregation and from Early to Final runs. The trend was also observed across other metrics including Bias, RMSE, and MAE.

 Challenges to the validation of IMERG Final in sparsely gauged regions is also discussed. The study was an important component of capacity-building efforts and the development of user networks. The information provides important guidance for the development of monitoring services that incorporate both IMERG and gauge networks to create estimates with reduced bias.

How to cite: Mantas, V. and Caro, C.: Performance of quantitative precipitation estimates in the complex terrain of the Peruvian Andes. IMERG V06 and the development of user-driven downstream applications., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7860, https://doi.org/10.5194/egusphere-egu23-7860, 2023.

EGU23-8456 | Posters on site | AS1.25

Operational Quantitative Precipitation Estimation Algorithm in Southern Brazil - An Update Blending Dual Polarization Weather Radar Network with Raingauges and Satellite Data 

Cesar Beneti, Leonardo Calvetti, Fernanda Verdelho, Rodrigo Rocha Junior, Jeova Silva Junior, and Vinicius Cebalhos

Quantitative estimation of precipitation (QPE) of high resolution, accurate and in real-time, increases the potential of weather radars for many applications, such as flash flood forecasting and hydropower production and distribution management. Using polarimetric variables from dual-polarization weather radars has already shown significant improvements in quantitative precipitation estimation in many countries with diverse weather. In Brazil, in the past ten years, we have seen an increase in dual-polarization weather radar coverage, mostly S-Band and some X-Band, concentrated in the southern parts of the country, an area prone to severe weather with high precipitation and lightning due to mesoscale convective systems. This region's significant economic activity is agriculture and energy production, accounting for more than 33% of the hydro energy generation used in the country. Therefore, the improvement of precipitation estimation is a necessary goal. However, the use of weather radar's QPE depends on calibration, good fit with rain gauges and distrometers, good data filtering, target’s distance from the radar, orography (i.e., relative to the topography), and signal propagation, as well as other factors.  A multi-sensor integration approach of remotely sensed precipitation estimation using weather satellites and weather radar with rain gauges improves the accuracy of hydrological models compared to a model using only rain gauge data. A quantitative precipitation estimation algorithm called SIPREC (System for Integrated PRECipitation) has been used operationally for more than 15 years, combining data from different sources, such as weather radar, rain gauge, and satellite. Precipitation estimates are obtained through an automated precipitation classification scheme based on reflectivity structures. This approach aggregates data from rain gauges by interpolation while maintaining the spatial distribution of the radar or satellite measurement. Statistical results indicate that the method can reduce radar and satellite data errors. This method is an essential advantage in an operational environment since it does not require frequent processing to update the weights as in other known schemes. However, this approach does not solve problems such as uncertainties related to Z-R estimation, spatial variability, and the one-hour temporal resolution. To improve the SIPREC algorithm, we used machine learning classification and regression methods to address the problem of precipitation estimation using dual polarization variables and rain gauge. An enhanced satellite precipitation estimation using GOES-16 data also replaced the previous dataset, and a new quality control algorithm for the network of weather radars was also applied to the dataset. A performance evaluation study shows improvements in precipitation estimation, primarily when used in real-time in an operational environment. This paper presents the results of this evaluation, with applications in severe weather events with high precipitation in the area.

How to cite: Beneti, C., Calvetti, L., Verdelho, F., Rocha Junior, R., Silva Junior, J., and Cebalhos, V.: Operational Quantitative Precipitation Estimation Algorithm in Southern Brazil - An Update Blending Dual Polarization Weather Radar Network with Raingauges and Satellite Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8456, https://doi.org/10.5194/egusphere-egu23-8456, 2023.

In semi-arid contexts, the strong spatiotemporal fluctuation of rainfall and the sparsity of the rain gauge (RG) measurement networks are the main limitations for water resources management. Freely available satellite-based rainfall estimates can be a potential source of information to cop data limitations over poorly gauged regions. Thus, the main aim of this work was to investigate how eight Spatial Rainfall Products (SRP, ARC-2, CHIRPSp25, CHIRPSp5, CMORPH-CRT, GPM-IMERG, PERSIANN-CDR, RFE-2, and TRMM-3B42) can be able to reproduce the observed monthly rainfall over a semi-arid context. The SRP estimates were directly evaluated against the RG observations. Then, bias correction techniques were used to account for the bias in the SRPs. The results indicated that the SRPs poorly correlate with the daily rainfall patterns (with Pearson Correlation Coefficients (PCCs) mostly below 0.5) but agreed with the monthly observations. The agreement was stronger over the lowlands than over the mountainous region. Overall, out of all the considered SRPs, IMERG (with a short-term record) and PERSIANN (with a long-term record) performed the best. Still, the monthly SRP estimates were significantly biased as the large rainfall totals were frequently underestimated. However, when the bias correction was applied remarkable improvement in the SRP’s performance was observed. The different adopted correction techniques yielded close results, with a slight prevalence of the Cumulative Distribution Function (CDF) over the Linear Scaling (LS), and Simple Linear Regression (SLR) techniques. Still, to reliably adjust the bias in the SRP estimates, LS and SLR should be preferred over the CDF technique, as they demonstrated more spatially consistent performance after validation.

How to cite: Ouatiki, H., Boudhar, A., and Chehbouni, A.: Can Bias correction Techniques Improve Remote Sensing-based Rainfall Estimates in a Semi-Arid Context: Case of the Oum Er-Rbia River Basin in Morocco, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8537, https://doi.org/10.5194/egusphere-egu23-8537, 2023.

EGU23-8700 | Posters on site | AS1.25

Advancing Precipitation Measurements from the NASA TROPICS Mission. 

Chris Kidd, Toshi Matsui, William Blackwell, Scott Braun, Robert Leslie, and Zach Griffith

A major challenge for measuring precipitation from space is the need to properly capture the spatial and temporal variability of precipitation. This requires that all available observations from precipitation-capable sensors are exploited. Passive microwave sensors are fundamental in providing reliable observations since they relate to the precipitation particles themselves. Passive microwave sounding instruments have been developed for cubesats, such as for the Time-Resolved Observations of Precipitation structure and storm Intensity with a Constellation of Smallsats (TROPICS) mission. The TROPICS pathfinder was launched in June 2021 into a polar orbit, carrying the TROPICS Millimeter-wave Sounder (TMS) with frequencies ranging from 91.655 to 204.8 GHz. The Precipitation Retrieval and Profiling Scheme (PRPS) has been adapted for use with the TMS based upon a 4-channel ATMS-DPR a priori database. This surrogate database is built upon coincident observations from the NPP and NOAA-20 ATMS sensors and the precipitation retrievals from the GPM DPR. The main limitation of the current database is that it is limited to just four closely matched channels, one at 89/91 GHz and the three around the 183.31 GHz water vapour absorption lines. The limited number of TMS vs DPR observations early in the mission precluded their use to generate a viable database: however, a reasonable number of coincident observations are now available to provide an insight into the use of the full range of TMS channels in the retrieval scheme. A total of about 1200 coincident TROPICS/GPM overpasses are available since launch, providing about 2 million matched footprints. Comparisons between the full 12-channel TMS database and the 4-channel ATMS database show a good degree of improvement, although refinement of channel weighting is deemed necessary, not least due to the high inter-channel correlations present within the 118 and 183 GHz channel groups. However, validation of the resulting precipitation products against the IMERG precipitation product indicate that the retrievals from the TMS are comparable as those from similar cross-track sounding instruments (such as GPROF retrievals from the MHS and ATMS).

How to cite: Kidd, C., Matsui, T., Blackwell, W., Braun, S., Leslie, R., and Griffith, Z.: Advancing Precipitation Measurements from the NASA TROPICS Mission., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8700, https://doi.org/10.5194/egusphere-egu23-8700, 2023.

EGU23-9191 | ECS | Posters on site | AS1.25

Machine Learning-driven Infilling of precipitation recordings over Germany 

Danai Filippou, Étienne Plésiat, Johannes Meuer, Hannes Thiemann, Thomas Ludwig, and Christopher Kadow

Weather radars are a significant component of modern precipitation recordings,as they provide information with high spatial and temporal resolution. However, radars as a tool for weather applications emerged only after the 1950s. AI/ML methods have proven to be successful when it comes to determining patterns and connections between related fields in space and time. Moreover, AI/ML methods have exhibited remarkable skill in infilling missing climate information (see Kadow et al. 2020). Desired outcomes of the project include using these AI/ML techniques to build a spatial precipitation field by combining station and radar data. We will use data from two well-known datasets: RADOLAN and COSMO-REA2. The validity of this digital twin will be investigated by comparing its output with other reanalysis data (e.g. ERA5). Further evaluation can be carried out by testing the radar field’s accuracy in detecting extreme precipitation events in the past (e.g. heavy rain events in the summer of 2021 in Western Germany). We aim for the creation of a radar field that will be successfully projected in the past. Moreover, it will uncover new information on regional climatology, especially in areas where station data is sparse.

How to cite: Filippou, D., Plésiat, É., Meuer, J., Thiemann, H., Ludwig, T., and Kadow, C.: Machine Learning-driven Infilling of precipitation recordings over Germany, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9191, https://doi.org/10.5194/egusphere-egu23-9191, 2023.

EGU23-9527 | Orals | AS1.25

Estimating and Simulating Precipitation Uncertainty Data for Large-Scale Hydrologic Applications 

Daniel Wright, Samantha Hartke, Zhe Li, Kaidi Peng, Aaron Alexander, and Yuan Liu

The usefulness of satellite multi-sensor precipitation and other large-scale precipitation products in hydrologic applications can be hindered by substantial uncertainty. In parts of the world with few ground observations of precipitation, such uncertainty is difficult to quantify. At the same time, how to cope with the characterize and model the spatiotemporal structure of this uncertainty has been called a grand challenge within the precipitation community. We present progress on two fronts which, when combined, addresses this grand challenge. Rather than relying on ground reference data to quantify uncertainty in NASA’s IMERG precipitation dataset, we instead use the dual-frequency precipitation radar aboard the NASA/JAXA GPM platform. This uncertainty information is then fed into the Space-Time Rainfall Error and Autocorrelation Model (STREAM), which uses an uncalibrated anisotropic and nonstationary spatiotemporal correlation modeling approach to stochastically generate ensemble precipitation fields that depict the uncertainty inherent in IMERG. We then use these ensemble fields to examine the effects of precipitation uncertainty in several hydrologic applications, including flood monitoring and prediction of water and energy fluxes. Ensemble-based hydrologic simulations outperform those based on IMERG and help reveal the spatiotemporal scales and hydrologic variables for which precipitation uncertainty is critical. The approach is compatible with other continental-to-global scale precipitation estimates such as those from numerical weather models, and can also be used in precipitation downscaling contexts. We are developing a set of open-source tools to facilitate its usage.

How to cite: Wright, D., Hartke, S., Li, Z., Peng, K., Alexander, A., and Liu, Y.: Estimating and Simulating Precipitation Uncertainty Data for Large-Scale Hydrologic Applications, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9527, https://doi.org/10.5194/egusphere-egu23-9527, 2023.

EGU23-9544 | ECS | Orals | AS1.25

Nearly instantaneous probabilistic retrievals of Rain over Africa 

Adrià Amell, Patrick Eriksson, Lilian Hee, and Simon Pfreundschuh
How much has rained in the last minutes anywhere in Africa? Contrary to Europe or North America, a dense network of weather radars providing this information is not available on the African continent. A new product, Rain over Africa, aims to find an answer to the question by retrieving rain rates from Meteosat geostationary infrared images and making them available to the public within minutes from satellite downlink. By using geostationary observations, rain retrievals with a resolution of 3-5 km and 15 min update time can be offered.

Machine learning is at the core of Rain over Africa. The GPM DPR and GMI combined precipitation L2B product was exploited to train a convolutional neural network. The trained model outputs a pixel-wise rain rate distribution free from traditional assumptions, enabling not only point estimates such as an expected value, but also non-Gaussian error estimates or likelihoods of extreme events by computing tail probabilities. Moreover, the Rain over Africa retrievals compare similar to the IMERG Late Run product, but can offer additional statistics at a finer spatiotemporal resolution, with a product latency of few minutes instead of hours.

Further details on the model and its performance, characteristics of the Rain over Africa product, how to access the data, and data availability, combined with a product outlook, will be given in this presentation.

How to cite: Amell, A., Eriksson, P., Hee, L., and Pfreundschuh, S.: Nearly instantaneous probabilistic retrievals of Rain over Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9544, https://doi.org/10.5194/egusphere-egu23-9544, 2023.

The assessment and interpretation of an extreme hydrometeorological event and the consequent impacts such as flash floods, especially within urban environment, is of high interest, especially in the Anthropocene era. Global warming intensifies Urban Heat Island resulting in local intense convective precipitation over a densely urbanized area.  Urbanization on one hand, increases the sensible heat flux  and transports more water vapor, mixing it into the upper atmosphere and on the other hand, increases the surface roughness and as a consequence mechanical turbulence drives low-level convergence resulting in enhanced intensity and frequency of convectional extreme precipitation (Nastos and Zerefos, 2007; Li et al., 2023).

In this study, we focus on an extreme summer convective event on August 24, 2022, in Athens, Greece, where the precipitation intensity reached instantly 116 mm/h and the visibility was limited to 600m. More specifically, we analyzed and compared the H03B product of EUMETSAT Hydrology Satellite Applications Facility (HSAF) with the ground-based OTT PARSIVEL Laser-based optical Disdrometer measurements.

Product H03B is based on the infrared (IR) electromagnetic spectrum from the SEVIRI instrument on board of Meteosat Second Generation satellites. The product is generated at the 15-min imaging rate of SEVIRI, and the spatial resolution is consistent with the SEVIRI pixel. Precipitation is obtained by combining IR equivalent blackbody temperatures at 10.8 μm with rain rates from polar microwave measurements.

OTT PARSIVEL Disdrometer is ideal for simultaneous measurement of PARticle SIze and VELocity of all liquid and solid precipitation. It detects and identifies 8 different precipitation types as drizzle, mixed drizzle/rain, rain, mixed rain/snow, snow, snow grains, freezing rain and hail. Besides, it provides drop size distributions on the ground and a function to derive a local Z/R relation – ready to be used to adjust the radar data.

The findings of the combined analysis showed that, towards early warning of convective precipitation in urban areas, combined high temporal resolution measurements carried out by satellites and ground based disdrometer measurements could provide a high-performance regional early warning system.

Keywords: extreme convective precipitation, EUMETSAT HSAF, PARSIVEL, rain rate, Athens

Acknowledgement: This work is co-financed by Iceland, Liechtenstein, Norway European Economic Area (EEA) Grants 2014 – 2021 and Greek Public Investments Program.

References:

  • Panagiotis T. Nastos, Christos S., Zerefos (2007), On extreme daily precipitation totals at Athens, Greece. Advances in Geosciences10, DOI: 5194/adgeo-10-59-2007
  • Chenxi Li, Xihui Gu, Louise J. Slater, Jianyu Liu, Jianfeng Li, Xiang Zhang, Dongdong Kong (2023), Urbanization-Induced Increases in Heavy Precipitation are Magnified by Moist Heatwaves in an Urban Agglomeration of East China. Journal of Climate, 36 (2), 693–709, DOI: https://doi.org/10.1175/JCLI-D-22-0223.1

How to cite: Nastos, P. T. and Matsangouras, I. T.: Combined Analysis of a convective precipitation event in Athens, Greece, by utilizing the H03B product of EUMETSAT HSAF and ground-based OTT PARSIVEL Laser-based optical Disdrometer measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9737, https://doi.org/10.5194/egusphere-egu23-9737, 2023.

EGU23-9756 | Posters on site | AS1.25

The observed changes in the precipitation regime in Romania – constraints for river restoration 

Dana Maria Constantin (Oprea), Giorgiana Daiana Lüftner, Raul Gabriel Ilea, Ionuț Andrei Șandor, and Gabriela Ioana-Toroimac

The success of river restoration depends on precipitation and their hydrological effects. In the context of global warming, an increase in the frequency of extreme events has been observed, with a rapid alternation between periods of excess precipitation with floods and periods of deficit precipitation with drought. Understanding the spatio-temporal variability of the precipitation regime allows to set guidelines for river restoration at a large scale. The main aim of the study is to analyze the variability and observed changes in the precipitation regime in Romania. The research is based on the monthly amounts and maximum precipitation in 24 hours data recorded at 23 meteorological stations, which are part of the Regional Basic Synop Network (RBSN) and belong to the National Meteorological Administration (NMA), for the period 1981 – 2020. Based on these monthly data, the annual, seasonal and semestrial precipitation amounts were calculated. Standardized anomalies and decadal averages were also calculated both annually and for the months January, April, July and October, which are considered typical months from a climatic point of view. The analysis of changes in the precipitation regime is completed by calculating linear trends and statistical significance at annual and seasonal level by applying the Mann-Kendall statistical test. From the analysis of these monthly data of the precipitation amounts, it was found that from January or February to June or July, the monthly precipitation regime shows ascending values, which then gradually decrease until the end of the year. The annual precipitation amounts, at the level of Romania, decrease from west to east as a consequence of oceanic influence’s decrease in the same direction. The variation of the average decennial values of the precipitation amounts indicates increases and decreases from one decade to another, but without significant changes. The trend of average monthly precipitation amounts is predominantly decreasing, but without being statistically significant according to the Mann-Kendall test. In Romania, in the transitional temperate continental climate, the great variability of precipitation in time can be a drawback for self-sustainable river restoration.

D.M. (Oprea) Constantin, I.A. Șandor and G. Ioana-Toroimac were supported by a grant of the Ministry of Research, Innovation and Digitization, CNCS - UEFISCDI, project number PN-III-P1-1.1-TE-2021-0600, within PNCDI III.

How to cite: Constantin (Oprea), D. M., Lüftner, G. D., Ilea, R. G., Șandor, I. A., and Ioana-Toroimac, G.: The observed changes in the precipitation regime in Romania – constraints for river restoration, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9756, https://doi.org/10.5194/egusphere-egu23-9756, 2023.

EGU23-9890 | Orals | AS1.25

Precipitation observations and simulations during the LIAISE-2021 field campaign 

Joan Bech, Mireia Udina, Eric Peinó, Francesc Polls, Albert García-Benadí, and Marta Balagué

Within the framework of the GEWEX initiative  “Land surface Interactions with the Atmosphere over the Iberian Semi-arid Environment” (LIAISE), the WISE-PreP project was carried out to study precipitation processes aiming to characterize possible differences in precipitation induced by surface characteristics (irrigated vs non-irrigated areas) in NE Spain. Specific deployed instrumentation during the 2021 campaign included three sites equipped each with a vertical radar Doppler Micro Rain Radar (MRR) and a laser disdrometer (PARSIVEL), plus an additional PARSIVEL disdrometer, covering both irrigated and non-irrigated sites. Time series of vertical precipitation profiles and in-situ drop size distributions were recorded to study microphysical processes and related variables including precipitation intensity or convective vs stratiform rainfall regimes.

First results show higher accumulated precipitation in the non-irrigated area (eastern area) than those in irrigated area (western area) in summer 2021, a feature also observed in summers for a previous reference period (2010-2019). Maximum and minimum daily temperatures were higher in irrigated areas than in non-irrigated areas. Both results are consistent with current climatology based on monthly precipitation and temperature that indicate the existence of a zonal gradient that increases semi-arid conditions (drier and warmer) from the east to the west. Disdrometer derived 1-min rainfall rate distributions presented some differences between the irrigated and non-irrigated areas during summer, unlike the other seasons when surface conditions are more similar in both areas. An overview of additional results obtained with numerical simulations using the WRF model is also provided. This research was supported by projects WISE-PreP (RTI2018-098693-B-C32) and ARTEMIS (PID2021-124253OB-I00) and the Water Research Institute (IdRA) of the University of Barcelona.

How to cite: Bech, J., Udina, M., Peinó, E., Polls, F., García-Benadí, A., and Balagué, M.: Precipitation observations and simulations during the LIAISE-2021 field campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9890, https://doi.org/10.5194/egusphere-egu23-9890, 2023.

EGU23-10762 | Orals | AS1.25

Hydrometeor Identification for GPM DPR 

Chandra V Chandrasekar and Minda Le

 

The GPM science implementation plan articulates the new frontiers of space-based precipitation observations, including new insights into vertical storm structure and microphysics [1]. The DPR algorithms are a key part of the process as discussed in the GPM science implementation the last updated DPR Algorithm Theoretical Basis Document (GPM/DPR ATBD 2021) document. Dual-frequency precipitation radar (DPR) onboard the GPM satellite has extended scan pattern to full swath mode for both Ku- and Ka-band since May 2018.  

 

The objective of the level-2 DPR algorithms are to derive radar only meteorological quantities meaning general characteristics of the precipitation, correction for attenuation and estimation of precipitation water content, rainfall rate and, when dual-wavelength data are available, information on the particle size distributions in rain and snow. The DPR Level-2 algorithms consist of several modules including the classification (CSF) module. Currently, our team plays a key role in the international DPR algorithm development group and is responsible for the dual-frequency algorithms development in the classification module. These algorithms include rain type classification, melting region detection, surface snowfall identification, graupel and hail detection etc. [2]-[4]. 

 

It is a unique advantage for space radar to provide a hydrometeor type over the globe while ground based observations are limited to the regions of deployment. Among the algorithms of current DPR classification module, most of the products are two dimensional with either a “flag” or “type” (or etc.) on a Latitude / Longitude surface. In this research, we will add a range-bin based hydrometeor type for DPR full swath data to enhance the classification module. This three-dimensional hydrometeor identification feature is the next frontier built upon our knowledge of hydrometeor classification development for DPR. 

 

This algorithm has been applied to various precipitation types and validated successfully with either ground based weather radar or airborne weather radar observations from field experiments such as OLYMPEX. Validation for cases with extreme hydrometeor type as hail are also performed with GMI-based approach and illustrate meaningful comparisons.  

 

 

 

How to cite: Chandrasekar, C. V. and Le, M.: Hydrometeor Identification for GPM DPR, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10762, https://doi.org/10.5194/egusphere-egu23-10762, 2023.

EGU23-10873 | ECS | Posters on site | AS1.25

Spatial downscaling of IMERG precipitation estimates using statistical techniques 

Stavros Stathopoulos and Alexandra Gemitzi

The aim of this study was to spatially downscale the Precipitation Estimates (PEs) from the Global Precipitation Measurement (GPM) mission, using the Integrated Multi-satellite Retrievals for GPM (IMERG), over a complex region in Greece. For this purpose, the Multivariate Linear Regression (MLR) and the Residual Correction (RC) techniques were utilized, in conjunction with remote sensing cloud properties from the Moderate Resolution Imaging Spectroradiometer (MODIS) instrument, onboard Aqua satellite, namely Cloud Optical Thickness (COT), Cloud Effective Radius (CER) and Cloud Water Path (CWP). The downscaled PEs were then validated using regional rain gauges’ measurements. According to our analysis, the 0.01o downscaled IMERG PEs were found to be more accurate than the original 0.1o IMERG data, over the region. In addition, the implementation of the RC technique to the 0.01o downscaled PEs was observed to improve the performance of the MLR downscaling method. This research was funded by the EU project titled: WATERLINE project id CHIST-ERA-19-CES-006.

How to cite: Stathopoulos, S. and Gemitzi, A.: Spatial downscaling of IMERG precipitation estimates using statistical techniques, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10873, https://doi.org/10.5194/egusphere-egu23-10873, 2023.

EGU23-11068 | Orals | AS1.25

Recent Advances in Quantitative Precipitation Estimation using Passive Microwave Observations from the Temporal Experiment for Storms and Tropical Systems (TEMPEST) 

Steven C. Reising, Venkatchalam Chandrasekar, Chandrasekar Radhakrishnan, Shannon T. Brown, Todd C. Gaier, and Sharmila Padmanabhan

The Temporal Experiment for Storms and Tropical Systems – Demonstration (TEMPEST-D) mission demonstrated the first global observations from a multi-frequency microwave radiometer on a CubeSat.  The TEMPEST-D CubeSat was deployed from the ISS in July 2018 and operated in low Earth orbit nearly continuously for three years until it re-entered the Earth’s atmosphere in June 2021. This NASA Earth Venture Technology mission exceeded expectations in terms of scientific data quality, instrument calibration, radiometer stability, and mission duration. TEMPEST-D brightness temperatures were validated using scientific and operational microwave sensors, including GPM/GMI and four MHS sensors on NOAA and ESA/EUMETSAT satellites. These comparison sensors operate at similar frequencies to TEMPEST-D, observing at the 87 GHz window channel, and at 164, 174, 178 and 181 GHz for water vapor sounding, cloud water and precipitation retrievals. TEMPEST-D was shown to have comparable or better performance to much larger operational sensors, in terms of calibration accuracy, precision, stability and instrument noise, during its nearly 3-year mission.

TEMPEST-D performed detailed observations of the microphysics of hurricanes, typhoons and tropical cyclones during three consecutive hurricane seasons. Nearly simultaneous observations by TEMPEST-D and JPL’s RainCube weather radar demonstrated a high degree of correlation between complementary passive and active microwave measurements of convective storms and tropical cyclones from the two CubeSats.  TEMPEST-D periodically performed along-track scanning measurements, providing the first space-borne demonstration of “hyperspectral” microwave sounding observations to retrieve the height of the planetary boundary layer with high precision.

The highly successful, stable operation of the TEMPEST-D instrument on a 6U CubeSat for nearly three years suggests myriad future opportunities to enhance microwave sounding and imaging of water vapor, clouds and precipitation. During the TEMPEST-D development, a nearly identical TEMPEST sensor was produced for risk reduction. The second sensor was delivered to the U.S. Space Force and integrated with NASA/JPL’s Compact Ocean Wind Vector Radiometer (COWVR). On December 21, 2021, COWVR and TEMPEST were launched from KSC as part of STP-H8 for 3 years of operations on the ISS. COWVR and TEMPEST-H8 have performed coordinated observations of Earth’s oceans and atmosphere from the ISS since January 7, 2022. TDRSS allows for near real-time communications from the ISS to ground, and STP-H8 plans to ingest COWVR and TEMPEST microwave observations into short- and medium-term weather forecasting models.

Quantitative precipitation estimates from TEMPEST-D on-orbit observations have been produced using a machine-learning approach.  Precipitation retrievals over continental storms as well as land-falling hurricanes demonstrated excellent agreement with multiradar/multisensor system (MRMS) quantitative precipitation estimates (QPE). These retrievals are currently being expanded from CONUS-only to a global basis using the IMERG precipitation dataset.  Similar techniques are being applied to TEMPEST-H8 observations from the ISS to provide retrievals of water vapor profiles, cloud liquid water, cloud ice water, and precipitation.

How to cite: Reising, S. C., Chandrasekar, V., Radhakrishnan, C., Brown, S. T., Gaier, T. C., and Padmanabhan, S.: Recent Advances in Quantitative Precipitation Estimation using Passive Microwave Observations from the Temporal Experiment for Storms and Tropical Systems (TEMPEST), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11068, https://doi.org/10.5194/egusphere-egu23-11068, 2023.

The specific differential phase Kdp is defined as the slope of range profiles of the differential propagation phase shift Φdp between horizontal and vertical polarization states observed by polarimetric radar. The Kdp is an important parameter for meteorological applications because it is proportional to precipitation particle concentrations and size and closely related to rain intensity. Past studies showed that the high Kdp value above the environmental 0 °C level potentially is an early indicator of heavy rain produced by summertime deep convection.

In autumn and winter, the stratiform precipitation system is the primary source of rainfall in north Taiwan. Additionally, embedded convective cells could lead to intense rain rates. But these cells’ top is not always developed higher than 0 °C level. This study uses a C-band polarimetric radar located in north Taiwan to discuss the evolution of Kdp and related rainfall of several heavy rain events in autumn. The application of Kdp to quantitative rainfall estimation is also illustrated.

The result shows that the value of Kdp > 2° km-1 is closely related to the movement and intensity of the severe rainfall area (> 60 mm h-1). Kdp > 2.0° km-1 occurs for more than 30 minutes, which is related to the location of rainfall of 100mm in 3 hours. The development height of Kdp >1.5° km-1 reaches the melting level, or there is a core area with Kdp >3.0° km-1 below the melting level, which will cause local heavy rainfall on the ground in the next 10 to 20 minutes (>10 mm in 10 minutes). Kdp > 3.0° km-1 occurs for more than 1 hour, which is related to the rainfall of up to 200mm in 3 hours.

How to cite: Jung, C.-J. and Jou, B. J.-D.: Application of specific differential phase as indicator for severe rainfall produced by shallow convection, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11118, https://doi.org/10.5194/egusphere-egu23-11118, 2023.

EGU23-11345 | Orals | AS1.25

NASA Particle and Single-Scattering Database (PaSS-DB) in Support of Particulate Matter Retrievals 

Kwo-Sen Kuo, Ines Fenni, Robert Schrom, Ian Adams, Dai Hai Ton, George Huffman, and Scott Braun

A significant portion of the atmospheric particulate matters are irregular without symmetry, e.g., dust particles, ice crystals, snowflakes, etc. Some of them are of heterogeneous composition, e.g., melting hydrometeors and droplets with inclusions. Solving the electromagnetic scattering problem for these particles are computationally intensive. It becomes impractical and very inefficient to repeatedly solve the same problem. Moreover, due to the lack of symmetry, every orientation of the particle has a unique solution, generating considerably greater volumes of data than the solutions for particles with nice symmetry. Storing the solutions and making them accessible is far more sensible, economical, and thus sustainable. The Particle and Single-Scattering Database, PaSS-DB, initiative aims to catalog, warehouse, and disseminate these atmospheric particles and their electromagnetic scattering solutions using an enterprise-grade database management system and a web interface. We report the early progress of the effort in this presentation.

How to cite: Kuo, K.-S., Fenni, I., Schrom, R., Adams, I., Ton, D. H., Huffman, G., and Braun, S.: NASA Particle and Single-Scattering Database (PaSS-DB) in Support of Particulate Matter Retrievals, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11345, https://doi.org/10.5194/egusphere-egu23-11345, 2023.

EGU23-11499 | ECS | Orals | AS1.25

High-resolution gridded dataset of precipitation and temperature for Trentino-Alto Adige 

Pranav Dhawan, Daniele Dalla Torre, Andrea Menapace, Bruno Majone, and Maurizio Righetti

A high temporal (hourly) and high spatial resolution (250-meter) multi-decadal (1991 - 2021) gridded dataset of mean temperature and precipitation is presented for the complex mountain area of Trentino-Alto Adige in the north-eastern region of the Alps in Italy. This dataset was obtained from more than 300 meteorological stations covering the entire region of Trentino-Alto Adige as well as the neighbouring countries and regions of Italy. The observed dataset underwent quality checks and quality control such as gross error limit check, two-sided continuity check, persistence check and others for both meteorological variables however, no gap-filling procedure was undertaken in order to keep the originality of the dataset. Using the processed dataset, kriging interpolation technique was used to generate a gridded hourly dataset of the meteorological metered variables on a high spatial resolution grid of 250m x 250m. The accuracy of the kriging dataset was evaluated by a leave-one-out cross-validation approach, wherein the station in consideration is omitted, to remove self-influence, and the time series is reconstructed using the neighbouring stations. For the entire time period and region, the hourly temperature and precipitation show no bias, with a mean absolute error (MAE) of about 1.2 °C and 0.1 mm, comparable with state-of-art high-resolution datasets. This new dataset provides valuable insight into the spatio-temporal distribution of temperature and precipitation for highly variable topography experiencing distinct climatic conditions for the region of Trentino-Alto Adige and it helps to validate climate models for monitoring climate change at the regional level. Moreover, gridded datasets support the modelling of extreme events and climate variance, which are crucial for a range of climate impact assessments.

How to cite: Dhawan, P., Dalla Torre, D., Menapace, A., Majone, B., and Righetti, M.: High-resolution gridded dataset of precipitation and temperature for Trentino-Alto Adige, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11499, https://doi.org/10.5194/egusphere-egu23-11499, 2023.

EGU23-11506 | ECS | Orals | AS1.25

Detecting shallow precipitation from conical-scanning radiometer observations using a Random Forest model over the Netherlands 

Linda Bogerd, Kirien Whan, Chris Kidd, Christian Kummerow, Veljko Petkovic, Hidde Leijnse, Aart Overeem, and Remko Uijlenhoet

Over the past decades, spaceborne radiometers have proven to be valuable input to realize a global coverage of precipitation estimates. However, retrieving accurate shallow precipitation estimates from radiometers remains challenging. The signal related to precipitation formed close to the Earth’s surface is difficult to distinguish from dry weather, especially over land.  Despite the relatively low precipitation rates that are often associated with shallow precipitation, its persistent presence results in a significant contribution to the total amount of rainfall over the mid- and high latitudinal regions. Hence, correct identification is important.

This study aimed to improve our understanding of the radiometric signatures of shallow precipitation from passive microwave observations by implementing a Random Forest (RF) model. RF is chosen because of its limited risk of overfitting and the ability to physically interpret the resulting model structure and parameters. The RF model is applied to brightness temperature observations from all channels onboard the Global Precipitation Measurement (GPM) Microwave Imager (GMI) during 2017-2020 over The Netherlands (52°N). A high-quality gauge-adjusted radar product is used as reference. The echo top height retrieved from the two radars in The Netherlands (Herwijnen and Den Helder) are used to classify the GMI footprints to either dry, shallow (<3km) or non-shallow (>3km) regime.

Hyperparameter settings, such as the depth of the model, and choices such as the number of years the model is trained on or the threshold to classify footprint as dry, shallow, or non-shallow regime have a limited effect on the performance of the RF. In general, the model tends to wrongly classify dry footprints as wet (both shallow and non-shallow). The model showed a seasonal dependency, with the best performance in summer. Preliminary results also showed a strong seasonal effect when excluding all footprints within 40km distance of the coast. These results indicate that four different parameter sets representing each season are required. Furthermore, the specific years the model is trained or tested on are found to strongly affect its performance. Currently, additional variables (such as ERA5 freezing level, two-meter air temperature) and simultaneous observations from the GPM dual-frequency precipitation radar (DPR), are included to further improve and understand the performance of the RF model.

How to cite: Bogerd, L., Whan, K., Kidd, C., Kummerow, C., Petkovic, V., Leijnse, H., Overeem, A., and Uijlenhoet, R.: Detecting shallow precipitation from conical-scanning radiometer observations using a Random Forest model over the Netherlands, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11506, https://doi.org/10.5194/egusphere-egu23-11506, 2023.

EGU23-12109 | ECS | Orals | AS1.25

Dependence of GPM IMERG products on precipitation intensity in Catalonia. 

Eric Peinó, Joan Bech, and Mireia Udina

Satellite precipitation estimates (SPE) offer an excellent way to complement information on the spatio-temporal distribution of precipitation in semi-arid regions, such as Catalonia (NE Spain). The network of automatic weather stations of the Meteorological Service of Catalonia is used to evaluate the performance of the Integrated Multisatellite Estimates for GPM (IMERG). The semi-hourly scale analysis considered five categories related to precipitation intensity (light, moderate, heavy, very heavy, and torrential) and an analysis of two case studies of extreme precipitation was performed. Results found indicate that IMERG tends to overestimate light precipitation, while showing underestimates (errors above 60%) of cumulative precipitation in the rest of the intensity thresholds. This behaviour is related to the variability of precipitation on a point scale provided by the rain gauges and the uncertainties generated in the meshing process of the IMERG products. For high precipitation intensities, a time lag appears between satellite estimates and observations, related to the fact that the estimated precipitation may transform differently from the actual cloud movement. In addition, errors may be directly associated with the lack of information from the passive microwave (PMW) sensor. Finally, it is concluded that while IMERG can capture the spatio-temporal variability of the region in general, it has significant shortcomings in the detection of extreme sub-daily precipitation events. This research has been funded by projects WISE-PreP (RTI2018-098693-B-C32) and ARTEMIS (PID2021-124253OB-I00) and the Institute for Water Research (IdRA) of the University of Barcelona.

How to cite: Peinó, E., Bech, J., and Udina, M.: Dependence of GPM IMERG products on precipitation intensity in Catalonia., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12109, https://doi.org/10.5194/egusphere-egu23-12109, 2023.

EGU23-13779 | ECS | Posters on site | AS1.25

Development of a Python Framework (pyRadman) for QPE using radar and CML data at DWD 

Malte Wenzel, Christian Vogel, Maximilian Graf, Tanja Winterrath, and Christian Chwala

The daily life of everybody is affected by weather, especially by precipitation events. Climate projections indicate that the number and intensity of heavy rain events could increase in future. Therefore, the interest to improve QPE has increased rapidly, particularly for assurances, public infrastructure and flood risk management.

Currently, the QPE is calculated by using the RADOLAN algorithm of Deutscher Wetterdienst. This algorithm combines the data of 17 weather radars and roughly 1,200 rain gauges in Germany by adjusting the radar reflectivity to the precipitation amount measured at the ground. The adjustment process is done every 10 minutes using the hourly total of radar and rain gauge data. Due to the rain gauge data delivery the adjustment process is delayed by 25 minutes. For this reason, short convective precipitation events can only be observed insufficiently.   

Therefore, the RADOLAN algorithm has to be adapted to improve the QPE based on shorter data accumulation time and contemporary data delivery. One approach is to use almost real-time available data from the telecommunication network. Rainfall leads to attenuation of the signal level of commercial microwave links (CMLs). The path integral of the attenuation along one sender-receiver pair can be related to a certain precipitation amount. Germany is covered by several thousands (~130,000 in total) of CMLs, which can potentially be used to quantify rainfall events. Especially in urban areas the density of CMLs exceeds the density of meteorological networks rain gauges clearly. Therefore, it becomes possible to observe convective extreme weather events with higher temporal and spatial resolution.

Within the project HoWa-PRO, the Deutscher Wetterdienst (DWD) collaborates with University of Augsburg, Karlsruhe Institute of Technology in Garmisch-Partenkirchen, and Ericsson. One of the first tasks is to set up a continuous data flow from Ericsson to DWD. To investigate different combinations of data sources and adjustment intervals, a fast, flexible and expandable software framework for combining and processing this data has to be developed.      

We present first results of QPE after adjustment using different combinations of data e.g. CML+radar data and gauge+radar data. These results were analyzed and compared to show the potential of using opportunistic data from CMLs for radar adjustment.

How to cite: Wenzel, M., Vogel, C., Graf, M., Winterrath, T., and Chwala, C.: Development of a Python Framework (pyRadman) for QPE using radar and CML data at DWD, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13779, https://doi.org/10.5194/egusphere-egu23-13779, 2023.

EGU23-13962 | ECS | Orals | AS1.25

Analysis of Various Gauge Adjusted Merged Satellite Rainfall Products : A study for Major River Basins of Western India. 

Saurabh Choubey, Rina Kumari, Shard Chander, and Prashant Kumar

Precipitation is the most significant component of the global water and energy cycle associated directly with major Earth system processes- atmospheric circulation, clouds and water vapor and overall regulation of the biogeochemical cycle. Precipitation also has a major contribution in maintaining the socio-economic stability of the world as it is the primary source of freshwater and directly affects the food and water security. Extreme weather events associated with precipitation such as floods, droughts, landslides etc. are likely to intensify under current climate change scenarios which could induce mass migration and human conflicts due to unavailability of food and freshwater resources. Hence, accurate precipitation estimates are crucial in enhancing our understanding of the changing earth system processes and management of water resources through numerical weather predictions and hydrological forecasting. In this study, we evaluated the performance of a satellite-gauge merged rainfall product (GSMaP-IMD, 0.1×0.1) with a gauge based observational data (Indian Meteorological Department (IMD) daily gridded rainfall, 0.25×0.25) and two global satellite-based rainfall products- IMERG Final-run and GSMaP-CPC (standard JAXA product, GSMaP-Gauge) over 4 major river basins of Western India for the southwest monsoon period during 2000-2020.  

Results indicate that GSMaP-IMD better represents the overall distribution of rainfall over the river basins. The cumulative rainfall distribution over the study area is represented more realistically than other two datasets, especially at higher rainfall intensity (mm/day). GSMaP-IMD has smaller root mean squared error and higher correlation coefficient value than IMERG and GSMaP-CPC during the observation period. The distribution of low and moderate rainfall improved remarkably in case of GSMaP-IMD compared to the other products. Temporally, higher rainfall events are not represented accurately by IMERG and GSMaP-CPC which is improved in GSMaP-IMD. Overall, it is observed that IMERG overestimated the high rainfall events while GSMaP-CPC underestimated it whereas GSMaP-IMD showed improvement in estimating the events over the study area. The probability of detecting true rainfall events is further improved in GSMaP-IMD for all the basins. IMERG shows higher false rainfall bias over regions with high rainfall intensity which is reduced in GSMaP-CPC and further improved in GSMaP-IMD. The total ability of a dataset to capture actual rainfall events (Critical Success Index) is further enhanced for GSMaP-IMD. Finally, IMERG shows a large negative bias in detecting low rainfall events while GSMaP-CPC shows large positive bias in detecting high rainfall spatially. This systematic error is reduced in the GSMaP-IMD rainfall product. The results indicate that the IMERG and GSMaP-CPC have difficulties in detecting low and high rainfall events and further have systematic error which is due to the orographic effects and regional characteristics in southwest monsoon. Overall, satellite-gauge merged rainfall dataset performed better than the satellite-based products over major river basins of Western India. The integration of in-situ rainfall data from gauges and radars in future with satellite products at regional scale is found to improve the bias characteristics in IMERG and GsMAP-CPC which is significant in improving the availability of rainfall dataset for regional hydrological modelling applications, numerical weather predictions and water resource management. 

 

How to cite: Choubey, S., Kumari, R., Chander, S., and Kumar, P.: Analysis of Various Gauge Adjusted Merged Satellite Rainfall Products : A study for Major River Basins of Western India., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13962, https://doi.org/10.5194/egusphere-egu23-13962, 2023.

EGU23-14066 | Posters on site | AS1.25

An improved MSG SEVIRI wet-dry product based on a convolutional neural network 

Rebecca Wiegels, Andreas Wagner, Julius Polz, Luca Glawion, and Christian Chwala

Adequate spatial coverage of precipitation measurements is not available for large regions. Many countries are only equipped with networks of meteorological stations to measure precipitation based on sparse point measurements. Attenuation data from commercial microwave links (CML) allow precipitation estimates over existing networks, such as the cellular network. However, the processing of the data requires a distinction between wet and dry. Here, satellite data in countries of the Global South play a significant role, as they can be used in place of conventional reference data to distinguish between dry periods and precipitation events.

Deep Learning (DL) can be used to develop a dry indicator based on geostationary satellite data that can be applied for dry-wet classification in CML processing. A convolutional neural network is used to process visual and infrared cloud information from geostationary satellites and to create a dry indicator. Satellite derived products exist, such as the NWC SAF products PC and PC-Ph, and are utilized as baseline products. The baseline products and the DL based dry indicator developed in this work (DL product) are evaluated with radar and station data in Germany.

The evaluation shows that the developed DL product improves the performance at day and especially at nighttime. Limitations in detecting the correct rain field area is reduced by the DL product. In total the DL product improves the Matthews Correlation Coefficient value by about 0.05 compared to the PC-Ph product. 

How to cite: Wiegels, R., Wagner, A., Polz, J., Glawion, L., and Chwala, C.: An improved MSG SEVIRI wet-dry product based on a convolutional neural network, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14066, https://doi.org/10.5194/egusphere-egu23-14066, 2023.

EGU23-14775 | Posters on site | AS1.25

Combinations of CML wet/dry corrections based on MSG SEVIRI data in Germany 

Andreas Wagner, Rebecca Wiegels, Maximilian Graf, Julius Polz, and Christian Chwala

Data from commercial microwave links (CML) operated by mobile network providers is attenuated by precipitation. The line integral of the precipitation intensity can be calculated from this attenuation and is used as a complement to common precipitation measurements. A major issue in CML signal processing is the distinction between dry and wet time steps. In addition to time series-based methods, precipitation patterns based on weather radar or satellite are also used.

One aim of our work is to evaluate the suitability of MSG SEVIRI data as a wet/dry indicator. The advantage of SEVIRI is the almost global coverage with a resolution of about 4x6 km in the middle latitudes, every 15 minutes. We apply two products from NWCSAF that derive the probability of precipitation from a combination of SEVIRI channels. Our study is based on 3901 CMLs in Germany for the summer of 2021. We evaluate the performance differences at various precipitation intensities as well as between daytime and nighttime since fewer SEVIRI channels are available at night. Another aim of our work is to investigate the possibilities of improvements by a combination of time series and SEVIRI-based wet/dry detections.

Our results show at least equivalent performance of SEVIRI compared to common time-series-based methods. The Matthews Correlation Coefficient (MCC) values for combinations are even better. This is especially the case for light precipitation. In addition, there are also no deteriorations for individual CMLs compared to common methods.

How to cite: Wagner, A., Wiegels, R., Graf, M., Polz, J., and Chwala, C.: Combinations of CML wet/dry corrections based on MSG SEVIRI data in Germany, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14775, https://doi.org/10.5194/egusphere-egu23-14775, 2023.

EGU23-14994 | ECS | Orals | AS1.25

Improved QPE for the Ahr flooding event using weather radar and CML data 

Maximilian Graf, Julius Polz, JuYu Chen, Tanja Winterrath, Silke Trömel, and Christian Chwala

Extreme floods are one of the most severe natural disasters. In a recent example, long-lasting heavy rainfall over central Europe led to devastating flooding in several catchments in Germany and Belgium on the 14th and 15th of July 2021. The valley of the river Ahr in the German state of Rhineland-Palatinate was heavily affected by this flooding with over 100 casualties and a loss of over 20 billion Euros. Quantitative precipitation estimation (QPE) during this event was affected by several issues. Rain gauge measurements suffered from underestimation and were not available due to power outages towards the end of the event. Weather radar measurements underestimated the rainfall amount due to pronounced vertical gradients of precipitation below the melting layer. Rainfall products from these two sensors were not able to explain the discharge values within the Ahr catchment.A potential solution to improve the rainfall estimation for the Ahrtal event and radar rainfall estimation in general is to add additional rainfall information. This is commonly done by adjusting the radar derived rainfall fields to rain gauges. Here we use opportunistic sensors, namely commercial microwave links (CMLs), which have previously not been used for radar adjustment. We show QPE based on different radar products, each of them with and without an adjustment via CML rainfall estimates. We use the unadjusted RADOLAN product RY and two own polarimetric radar QPEs, of which one is enhanced with specific corrections based on MRR data and combined with a local X-Band gap-filling radar. We perform additive and multiplicative adjustment of the radar QPEs on an hourly basis with CML data, taking into account the path-averaging nature of the CML observations. Our results show that the CML adjustment significantly improves RADOLAN-RY and the polarimetric product without enhancement. The enhanced polarimetric product is already in very good agreement with the reference data and hence is not improved much. The applied enhancements from MRR and X-Band radar data are currently not suitable for operational usage, though. Radar-adjustment with CML data, which is available in real-time without delay, hence provides a suitable solution to improve operational QPE.

How to cite: Graf, M., Polz, J., Chen, J., Winterrath, T., Trömel, S., and Chwala, C.: Improved QPE for the Ahr flooding event using weather radar and CML data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14994, https://doi.org/10.5194/egusphere-egu23-14994, 2023.

EGU23-15222 | Orals | AS1.25

CML rainfall estimation in Africa: Recent results, challenges and suggested solutions 

Christian Chwala, Moumouni Djibo, Maximilian Graf, Julius Polz, François Zougmoré, and Harald Kunstmann

Many studies have already shown that attenuation data from commercial microwave link (CML) networks can be used to derive rainfall information, also on a country-wide scale. Particularly in regions with coarse station networks and without radar coverage, CMLs provide an attractive solution to increase the spatial and temporal coverage of rainfall observations. There are, however, several challenges that we face when transferring the successful applications from Europe to developing countries. In this contribution we present recent results from dense CMLs networks in two African cities, discuss the challenges that we are facing when trying to expand CML rainfall estimation, and present potential solutions to tackle these challenges.

We show rainfall maps with temporal resolution of 15-minutes derived from CML networks in the city of Ouagadougou (Burkina Faso) and the city of Lusaka (Zambia). There is only one rain gauge for comparison in each city, which limits the options for validation. However, comparison of the CML-derived rainfall maps with the gauges shows good agreement. These results clearly show the large potential of the dense CML networks in African cities for rainfall observation. 

Country-wide rainfall estimation based on CML data in developing countries can not always be done in the same manner, as e.g. in Germany. Based on our experience, a large number of CMLs in developing countries are long 7-GHz CMLs. At these frequencies the path attenuation is less sensitive to rainfall and the long CMLs seem more prone to fluctuations during dry periods. This makes the data processing more challenging. We suggest that a combination of CML data processing with data from geostationary satellites is considered a basic requirement and not only an option for further improvement. While this combination is methodologically feasible, it implies large organizational efforts. Either large amounts of satellite data have to be moved to the individual institutions that do CML data processing, or CML data, which is hard to get access to, has to be transferred to an institution that has direct access to the satellite data.

To be able to bring rainfall estimation from a combination of CML and geostationary satellite data to an operational level, simplified access to CML data and concerted processing is required. We do not suggest a final solution, but we present ideas to initiate a discussion that should pave the way towards making operational usage of CML data in developing countries a reality.

How to cite: Chwala, C., Djibo, M., Graf, M., Polz, J., Zougmoré, F., and Kunstmann, H.: CML rainfall estimation in Africa: Recent results, challenges and suggested solutions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15222, https://doi.org/10.5194/egusphere-egu23-15222, 2023.

EGU23-15447 | ECS | Posters on site | AS1.25

New insights into the wet antenna attenuation effect based on data from a dedicated field experiment with CML antennas 

Jonas Tiede, Uwe Siart, Christian Chwala, and Harald Kunstmann

The monostatic field experiment ATTRRA2 uses six dual-polarized, customary CML antennas which operate at different frequency bands. The experiment is installed at the TERENO field site in Fendt, Germany. A mounted camera provides pictures of the antenna radomes, and, thereby, visual information about the wetness distribution on the antennas. On-site disdrometers provide a reference for the rainfall intensity. Transmit-receive signal level (TRSL) data commonly used for quantitative precipitation estimation (QPE) is recorded into a minutely sampled time series together with the so-called antenna mismatch factor. The latter provides additional information about the radome condition in this use case and, thereby, serves as a proxy measurement of the wet antenna attenuation (WAA). Careful analysis of the data yields new insights into the temporal dynamics of WAA, especially during dewy periods before actual rain and drying periods after rain events. A comparison with established WAA correction methods shows that the proposed one performs promisingly, especially during periods of high TRSL fluctuations. A remaining challenge is the long-term stability of the instrument which will be specifically addressed in the future.

How to cite: Tiede, J., Siart, U., Chwala, C., and Kunstmann, H.: New insights into the wet antenna attenuation effect based on data from a dedicated field experiment with CML antennas, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15447, https://doi.org/10.5194/egusphere-egu23-15447, 2023.

The Dual-frequency Precipitation Radar (DPR) on NASA's core Global Precipitation Measurement satellite is the first space-borne instrument that offers an opportunity of a dual-wavelength radar retrieval of the size and the mass concentration of hydrometeors, i.e., two microphysical parameters that control the mass flux through the weather systems. Our focus is placed on DPR observations over the stratiform rain where the analysis revealed a sharp increase in mass flux from ice to rain phase in the official algorithm. This is inconsistent with the expectation that mass flux varies little across the bright band. The proposed algorithm imposes continuity of the precipitation rate across the bright band which additionally helps in deriving bulk ice density. It is based on Bayes' rule with riming parameterized by the “fill-in” model. The radar reflectivity are simulated using the scattering models corresponding to realistic snowflake shapes. The algorithm is validated using the co-located polarimetric radar data collected for the GPM ground validation program. In the future, this dataset will be used for multi-frequency radar studies that aim at constructing high quality training datasets for artificial intelligence algorithms that are necessary to analyse the huge volume of data that will be generated by upcoming space missions such as the one proposed by Tomorrow.io

How to cite: Mroz, K. and Battaglia, A.: Characteristics of ice over stratiform rain: Global statistics from the Dual-frequency Precipitation Radar and the proposed retrieval scheme, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15803, https://doi.org/10.5194/egusphere-egu23-15803, 2023.

EGU23-16155 | Posters on site | AS1.25

Analysis of satellite precipitation products during the monsoon floods in Pakistan in 2022 

Giulia Panegrossi, Sidra Batool, Daniele Casella, Leo Pio D'Adderio, Paolo Sanò, Stefano Sebastianelli, Claudio Giorgi, and Davide Melfi

On 24-26 August 2022 Pakistan has suffered one of its most severe floods.  The excessive monsoon rainfall throughout the summer, which was worsened by shorter bursts of extremely heavy rain that affected the regions of Sindh and Balochistan, directly contributed to the flooding. According to reports, Pakistan experienced more than three times its typical rainfall in August, making it the wettest month since 1961. The strong monsoon moist currents and thermal lows started from Arabian Sea penetrating into entire area of Balochistan and Sindh, and spread over upper and central parts of the country. The moist currents from the Bay of Bengal penetrating during the entire monsoon season
from mid-June to September resulted in floods and land sliding across Pakistan, causing human casualties as well as widespread destruction of homes and infraructure. Floods cannot be entirely avoided, but their harmful effects can be significantly managed with careful planning and adequate preparation. The use of operational satellite precipitation products could facilitate prompt and accurate monitoring (and forecasting) as well as the implementation of impact-minimizing strategies, reducing vulnerability to floods.

The European Organization for the Exploitation of Meteorological Satellites (EUMETSAT) application facility on Support to Operational Hydrology and Water Management (H SAF) (http://h-saf.eumetsat.int/) provides operational satellite products of important hydrological parameters, including snow cover and water equivalent, soil moisture, surface rain rate and cumulated rainfall. Among these, H SAF generates a near-real time (NRT) product providing instantaneous surface precipitation rate over the Meteosat Second Generation (MSG) Indian Ocean Data Coverage (IODC) every 15 minutes at 3-5 km spatial resolution (H SAF product ID H63). H63 is based on the rapid update blending technique combining passive microwave (PMW) precipitation rate estimates and IR measurements from MSG SEVIRI.  On the other hand, since the beginning of March 2014, the NASA Global Precipitation Measurement (GPM) mission (https://gpm.nasa.gov/missions/GPM) Integrated Multi-satellite Retrievals for GPM (IMERG) product provides quasi-global (60 N-60 S) precipitation rate estimates every 30 min at 0.1°x0.1° spatial resolution, combining information from the GPM constellation of PMW radiometers available over the majority of the Earth's surface with IR satellite measurements.

This study proposes a comprehensive overview about the performance evaluation of IMERG (Early and Late run) and H63 products using rain gauges data in Pakistan, for the August 2022 Pakistan Flood event. Gauge-based rainfall data from the high-density climate station network of the Metrological Department Pakistan (PMD), are compared with NASA GPM IMERG rainfall products, and with H SAF and H63 rainfall product. Hourly and daily precipitation estimates are derived from the satellite products over specific regions entirely covered by 32 PMD stations. The goal of the study is to evaluate the performance of IMERG and H63 by means of a cross-comparison with rain gauges data (considered as the ground truth) using both statistical and graphical methods and analyze the results considering local environmental conditions. We also illustrate, through selected rainfall event cases and sub-regions, how insufficient coverage by PMW radiometers can lead to larger discrepancies in the IMERG and H63 estimates with respect to the ground measurements.

How to cite: Panegrossi, G., Batool, S., Casella, D., D'Adderio, L. P., Sanò, P., Sebastianelli, S., Giorgi, C., and Melfi, D.: Analysis of satellite precipitation products during the monsoon floods in Pakistan in 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16155, https://doi.org/10.5194/egusphere-egu23-16155, 2023.

EGU23-16639 | Posters on site | AS1.25

Building an EPS-SG Microwave Imager Retrieval Suite: Level-1 Proxy Data Record 

Veljko Petković, Patrick Stegmann, Huan Meng, Ralph Ferraro, and John Xun Yang

Following the success of MetOp, EUMETSAT Polar System Second Generation (EPS-SG) will provide satellite observations from polar orbit to support Numerical Weather Prediction and climate monitoring in the 2024 to mid-2040's timeframe. Designed to fly on board the EPS-SG satellite-B series and cover 19-183 GHz frequency range, Microwave Imager (MWI) is expected to deliver high-quality measurements of radiometric properties relevant to precipitation, clouds, near-surface ocean winds and snow/ice cover. With goal to build an enterprise MWI retrieval in support to NOAA operational Environmental Data Records (EDRs) productiondevelopment of new and adaptation of the existing microwave imager algorithm procedures are underway at University of MarylandAs part of this effort and to ensure timely delivery of day-1 retrievals, we simulate MWI level-1 data over prolonged periods of time (up to 12 months) using radiative transfer techniques. Two datasets will be presented. The first, oriented towards precipitation retrieval development, relies on Global Precipitation Measurement (GPM) Dual-frequency Precipitation Radar (DPR) observations to construct a state vector in radiative transfer calculations. The second dataset relies exclusively on ERA5 parameters. Two radiative transfer models have been considered in the production of simulated MWI brightness temperatures: a) Community Radiative Transfer Model (CRTM) and b) Edington model. Each model uses MWI observation geometry, following DPR and GCOM-W1 AMSR2 sampling, respectively. To deliver the product, CRTM has been updated by, for this purpose derived, MWI coefficients using an idealized Spectral Response Function at each of the 26 channels. When compared to the common channels of AMSR2 sensorthe simulations reflect exceptionally high accuracy. In addition to the methodology and proxy data sets, preliminary results for MWI precipitation EDR retrieval will be presented.

How to cite: Petković, V., Stegmann, P., Meng, H., Ferraro, R., and Yang, J. X.: Building an EPS-SG Microwave Imager Retrieval Suite: Level-1 Proxy Data Record, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16639, https://doi.org/10.5194/egusphere-egu23-16639, 2023.

EGU23-16922 | Posters on site | AS1.25

Development of a Low-cost Precipitation Observation Network in Africa 

Paul Kucera and Martin Steinson

Accurate and reliable real-time monitoring and dissemination of observations of atmospheric and hydrologic conditions in general is critical for a variety of research and real-time monitoring applications.  Precipitation observations provide critical information for wide variety of applications ranging from drought monitoring for agriculture application and resource staging in extreme drought regions to water resource monitoring for freshwater allocation and hydroelectric power generation.  In many regions of the World, especially in Africa, weather observation network density has been declining over the past few decades.  The University Corporation for Atmospheric Research (UCAR) with support from USAID, is leading an initiative to develop low-cost hydrometeorological instrumentation (e.g., automatic weather stations, rain gauges, stream gauges) as solution to increase observation networks in sparsely observed regions of the world. We have started a new initiative to use low-cost observation network to support the Famine Early Warning Systems Network (FEWS NET: https://fews.net/). The goal of the project is to improve the number of observations (temporally and spatially) in these regions to improve the quality of the FEWS NET products.  These data will be open and publicly available to the scientific community for other applications (e.g., satellite precipitation product evaluation, weather and hydrological prediction, etc.).  The presentation will provide an overview of the low-cost observation technology and plans for the development of the precipitation monitoring network in Africa.

How to cite: Kucera, P. and Steinson, M.: Development of a Low-cost Precipitation Observation Network in Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16922, https://doi.org/10.5194/egusphere-egu23-16922, 2023.

EGU23-17124 | Posters virtual | AS1.25

Statistical and hydrological evaluation of precipitation estimates and simulations from the remote sensing technologies and WRF modeling over the Peruvian Andes region 

Mengye Chen, Yongjie Huang, Zhi Li, Albert Johan Mamani Larico, Ming Xue, Yang Hong, Xiao-Ming Hu, Hector Mayol Novoa, Elinor Martin, Renee McPherson, Andres Vitaliano Perez, and Isaac Yanqui Morales

Peruvian Andes region has been proven in multiple studies to be one of a few regions have poor performance of many global precipitation estimations, due to its complex terrain and extreme interruption of atmospheric movement by the Andes mountain. This study provides an evaluation over two Peruvian local precipitation products PISCO and RAIN4PE, along with a regional dynamic downscaled WRF model simulation, and GPM-IMERG. The precipitation products were evaluated against local rain gauge data and used as the forcing data for CREST-VEC model to test the uncertainties of the precipitation products in a extremely dry region in Peru. This study readdress the accuracy issue of precipitation products in the Peruvian Andes region, and highlights the importance of using WRF modeling simulation to ‘fill-the-blank’ of heterogenous rain gauge distribution, when remote-sensing technologies fail to perform in this area.

How to cite: Chen, M., Huang, Y., Li, Z., Mamani Larico, A. J., Xue, M., Hong, Y., Hu, X.-M., Mayol Novoa, H., Martin, E., McPherson, R., Vitaliano Perez, A., and Yanqui Morales, I.: Statistical and hydrological evaluation of precipitation estimates and simulations from the remote sensing technologies and WRF modeling over the Peruvian Andes region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17124, https://doi.org/10.5194/egusphere-egu23-17124, 2023.

EGU23-17303 | Posters on site | AS1.25

Improving Cross-Track Scanning Radiometers’ Precipitation Retrieval over Ocean by Morphing 

Yalei You, George Huffman, Christa Peters-Lidard, Joseph Munchak, Jackson Tan, Scott Braun, Chris Kidd, Sarah Ringerud, William Blackwell, John Xun Yang, Eric Nelkin, and Jun Dong

Previous studies showed that conical scanning radiometers greatly outperform cross-track scanning radiometers for precipitation retrieval over ocean. This study demonstrates a novel approach to improve precipitation rates at the cross-track scanning radiometers’ observation time by propagating the conical scanning radiometers’ retrievals to the cross-track scanning radiometers’ observation time. The improved precipitation rate is a weighted average of original cross-track radiometers’ retrievals and retrievals propagated from a conical scanning radiometer. Results show that the morphed precipitation rates agree much better with the reference. The degree of improvement depends on several factors, including the propagated precipitation source, the time interval between the cross-track scanning radiometer and the conical scanning radiometer, the precipitation type (convective versus stratiform), the precipitation events’ size, and the geolocation. The study has potential to greatly improve high-impact weather systems monitoring (e.g., hurricanes) and multisatellite precipitation products. It may also enhance the usefulness of future satellite missions with cross-track scanning radiometers on board.

How to cite: You, Y., Huffman, G., Peters-Lidard, C., Munchak, J., Tan, J., Braun, S., Kidd, C., Ringerud, S., Blackwell, W., Xun Yang, J., Nelkin, E., and Dong, J.: Improving Cross-Track Scanning Radiometers’ Precipitation Retrieval over Ocean by Morphing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17303, https://doi.org/10.5194/egusphere-egu23-17303, 2023.

To study climate change we rely on global climate models (GCMs) but their resolution is coarse to investigate impacts at the local scale. Hence, a downscaling task is required for the use of these coarse-resolution outputs. In this sense, statistical downscaling methods (SDMs) are commonly applied to analyse the local impacts. Furthermore, a quantification of the uncertainty share of the SDMs is advised to complement the results. However, many choices need to be done before their application and these decisions can bias the outcome of the analysis. This work examines the SDMs’ uncertainty share to evaluate to what extent the different adopted strategies can impact the climate change signal (CCS) associated with the study. For this, eleven research indicators (six representing precipitation extremes) are used with four future scenarios, 28 state-of-art GCMs, and 15 SDMs of two different types (change factor and quantile mapping methods). The uncertainty involved is quantified by the variance decomposition procedure. Three different decisions are tested:

(i) The selection of the Coupled Model Intercomparison Project (CMIP) era. The uncertainty shares in phases five and six (CMIP5 and CMIP6, respectively) are compared.  

(ii) The selection of the SDM ensemble based on the SDMs’ methodological construction. More specifically, based on an ensemble of five methods of change factor type (including an event-based change factor weather generator) and an ensemble of ten methods of quantile mapping.

(iii) The selection of the optimal SDM ensemble number. Different unique SDMs combinations are tested from k-ensemble members in [2,n] with n as the ensemble with the largest number of members (n=15).

To complement the analysis, the outcomes of the CCSs from all the combinations in (ii) and (iii) are analysed. The results showed that the uncertainty quantification of the SDMs is not sensitive to the selection of the CMIP era. However, this choice is important if the focus is on the GCMs and future scenarios. Hence, it is preferable (but not mandatory) to perform the analysis with the most recent era. The selection of the SDMs based on a methodological construction might bias the conclusions. Therefore, it is better to include methods from all possible types since the results showed that the more methods included in the downscaling, the more reliable the estimation of the SDMs’ uncertainty share. The CCS seems to strongly depend on the choice of the SDM ensemble, and it tends to converge from different k-ensemble members in [2,n] towards the largest ensemble (n). Hence, CCSs from large SDM ensembles will be more reliable. Future work must extend the analysis into different climatological regions and include more methods from all the possible types.

How to cite: Mendoza Paz, S. and Willems, P.: The statistical downscaling methods’ uncertainty share as a measure for adopted strategies in downscaling studies for climate change, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-83, https://doi.org/10.5194/egusphere-egu23-83, 2023.

Rainfall Intensity-Duration-Frequency (IDF) curves are widely used in studies related to planning, design, and operation of various water control (e.g., barrages, dams, levees) and conveyance structures (e.g., culverts, spillways, storm sewers) for mitigating risk associated with floods attributable to extreme precipitation. In many parts of the globe, precipitation data are limited, and the network of gauges is sparsely distributed. Therefore, the use of only at-site data for the construction of IDF curves could have large uncertainties. To overcome this impediment, regional IDF relationships could be developed by regional frequency analyses (RFA) which uses information pooled from several meteorologically similar sites. Recently, there is growth in the use of fine spatial scale remote-sensing precipitation products to arrive at IDF relationships for ungauged locations, as the spatial coverage of these products is exhaustive. However, recent studies indicate that most of the remote sensing products underestimate the precipitation intensities corresponding to different durations and return periods and also perform worse at shorter time scales (e.g., daily and sub-daily). Although remote sensing products can be corrected for biases before use in developing the IDF relationships, there is ambiguity in the choice of bias correction methods. Furthermore, in sparsely gauged locations, the availability of only a limited number of ground observation stations for bias correction enhances uncertainty in the developed IDF relationships. In addition, relying on only one satellite product may not be meaningful, as the skill of different satellite products varies across the globe. Also, the conventional practice of developing IDF curves considering the stationary assumption may lead to large biases in estimates of precipitation extremes in a changing climate. To address these issues, this study proposes a novel methodology to develop non-stationary regional IDF relationships for use in climate change scenarios. The methodology involves nonstationary RFA utilizing fine grid-scale daily precipitation derived by merging multiple satellite-based precipitation products and ground-based precipitation products for homogenous extreme precipitation regions (EPRs). The merging of different products is achieved using a novel random forest-based regression method. Effectiveness of the proposed methodology is demonstrated through a case study on Karnataka state in India, which extends over approximately 0.2 million square kilometers. The homogenous EPRs are delineated in the study area using ensemble cluster analysis of the relevant predictor variables/covariates. Non-stationary regional IDF curves are developed using the proposed methodology corresponding to different CMIP6 climate change scenarios, considering an ensemble mean precipitation derived from eleven GCMs (General Circulation Models). The curves are compared with those obtained using conventional stationary methods considering block-maxima and partial duration series of extreme precipitation.

How to cite: Goel, A. and Srinivas, V. V.: Deriving Regional IDF Curves for Data-Sparse Areas in Climate Change Scenarios using Merged Satellite and Ground-based Precipitation and GCMs, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-304, https://doi.org/10.5194/egusphere-egu23-304, 2023.

EGU23-624 | ECS | Orals | HS7.2

The unintended usage of precipitation reanalysis products: Downscaling of daily precipitation time series to hourly values using reanalysis products for parameter estimation 

Hannes Müller-Thomy, Jana Kellner, Patrick Nistahl, Nejc Bezak, Katarina Zabret, and Kai Schröter

High-resolution precipitation time series are required for numerous applications in hydrology. For data-scarce regions, precipitation reanalysis products (PRP) are a promising data source. We validated two PRP for Slovenia and identified biases, which disable a direct usage of the PRP. However, the PRP were used for the parameter estimation of a cascade model to disaggregate daily time series, which exist for long periods for the whole country. The so assimilated data benefits from the advantages from both datasets: the daily rainfall amounts from the observations and the high-resolution temporal structure from the PRP. The disaggregated time series show a superior representation of the observed high-resolution point and areal precipitation time series in comparison to the PRP themselves, and their usage is recommended instead. The developed concept can be transferred to other data-scarce regions.

In more detail, from the latest PRP two are most promising due to their spatial and temporal resolution: ERA5-Land (raster width ~9 km width, temporal resolution of 1 h) and REA6 (6 km, 1 h). ERA5-Land and REA6 are evaluated in space and time by continuous and event-based characteristics as well as precipitation extreme values for five recording stations and 20 catchments in Slovenia. Both PRP show underestimations of dry spell duration, wet spell amount and average intensity, while wet spell duration is overestimated. For extreme values with 1 h duration both PRP lead to underestimations, whereby the bias increases with the return period. The identified biases are larger for ERA5-Land than for REA6. The PRP time series were used for the parameter estimation of a micro-canonical cascade model to disaggregate observed daily values to hourly values. The so estimated parameters differ from station-based estimations, e.g. probabilities for the generation of dry time steps (P(1/0), P(0/1)) are underestimated. Nevertheless, starting from observed daily rainfall amounts the disaggregated time series show a superior representation of the high-resolution precipitation characteristics in comparison to ERA5-Land and REA6. This conclusion is based on all studied precipitation characteristics.

How to cite: Müller-Thomy, H., Kellner, J., Nistahl, P., Bezak, N., Zabret, K., and Schröter, K.: The unintended usage of precipitation reanalysis products: Downscaling of daily precipitation time series to hourly values using reanalysis products for parameter estimation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-624, https://doi.org/10.5194/egusphere-egu23-624, 2023.

EGU23-668 | ECS | Orals | HS7.2

Effects of Super-Extremes in the evaluation of the design rainfall: a case study in Northern Italy 

Paola Mazzoglio, Ilaria Butera, and Pierluigi Claps

In recent years, several major rainfall events have been observed in Italy, with amounts that have broken previous all-time records. Several questions concerning the adequacy of the statistical tools that we have at our disposal to determine the "real" rarity of these events emerge, especially considering the limited availability of long and complete rainfall records. In this work, we investigate the influence of "Super-Extremes" on the rainfall regional frequency analysis framework. More specifically, we consider the all-time Italian record events up to now, some of which were observed in 2021 (377.8 mm / 3h, 496 mm / 6h, 740.6 mm / 12h).

The approach is undertaken through a rainfall regional frequency analysis performed over the North-West of Italy based on the patched kriging (PK) technique. PK requires a year-by-year application of ordinary kriging, that overcomes the data inconsistency by considering all the time series, without the need to discard those shorter than a specific length. The morphology of the areas is quite complex, which implies that extremes are expected to be influenced by the elevation: the orographic gradient is computed and removed and, for each duration, the sample variogram is evaluated as the mean of the annual variograms weighted on the number of active rain gauges for any year.

The sequential application of the ordinary kriging allows to reconstruct both a "rainfall data cube" and a "variance data cube" in the (x, y, t) space. A complete series of measured and estimated values are obtained by coring the data cube along the time axis in each location. The cored series are then used to compute the L-moments, in a framework that assigns weights based on the kriging variance, to consider the different nature of the data (measured and estimated). To overcome possible inconsistencies of the L-moment, a bias-correction procedure is applied to preserve the coefficient of variation from the smoothing effect induced by the spatial interpolation.

The methodology is applied to short-duration (1 to 24 hours) annual maximum rainfall depths recorded by rain gauges coming from the Improved Italian – Rainfall Extreme Dataset (I2-RED). The effects in the local frequency curves when introducing new record-breaking data are examined and commented, in view of the role that these values assume in the surrounding region.

How to cite: Mazzoglio, P., Butera, I., and Claps, P.: Effects of Super-Extremes in the evaluation of the design rainfall: a case study in Northern Italy, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-668, https://doi.org/10.5194/egusphere-egu23-668, 2023.

EGU23-736 | ECS | Orals | HS7.2

Parameterization-based uncertainties in RegCM simulations over the Carpathian region in a wet year 

Tímea Kalmár, Rita Pongrácz, and Ildikó Pieczka

Precipitation is one of the most important climate variables in many aspects due to its key impact on agriculture, water management, etc. Furthermore, extreme precipitation events can lead to excess surface water and floods and are becoming an amplifying societal cost as a result of urbanization and our warming climate. However, it remains a challenge for climate models to realistically simulate the regional patterns, temporal variations, and intensity of precipitation. Detailed knowledge about extreme precipitation events is important for advanced predictions on weather-to-climate time scales. The difficulty arises from the complexity of precipitation processes within the atmosphere stemming from cloud microphysics, cumulus convection, large-scale circulations, planetary boundary layer processes, and many others. This is especially true for heterogeneous surfaces with complex orography such as the Carpathian region.

In order to quantify the impact of the use of different parameterization schemes on regional climate model outputs, hindcast experiments were completed applying RegCM4.7 to the Carpathian region and its surroundings at 10-km horizontal resolution using ERA-Interim reanalysis data as initial and boundary conditions. In this study, 24 simulations were carried out by using various combinations of the physics schemes (2 land surface, 2 microphysics, 3 cumulus and 2 boundary layer schemes) for the year 2010, which was the wettest year in the region since the beginning of the regular measurements. Each parameterization combination leads to different simulated climates, so their spread is an estimate of the model uncertainty arising from the representation of the unresolved phenomena. The analysis of the RegCM ensemble indicates systematic precipitation biases, which are linked to different physical mechanisms in the summer and winter seasons.

Based on the results, RegCM is sensitive to the applied convection scheme, but the interactions with the other schemes (e.g., land surface or microphysics) affect not only the total precipitation, but also the convective and stratiform precipitation in some cases. Due to the different treatment of moisture in the schemes, there are differences not only between the representation of the precipitation cycle, but also in other climatological variables such as soil moisture, temperature and cloud cover.

How to cite: Kalmár, T., Pongrácz, R., and Pieczka, I.: Parameterization-based uncertainties in RegCM simulations over the Carpathian region in a wet year, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-736, https://doi.org/10.5194/egusphere-egu23-736, 2023.

EGU23-1126 | ECS | Orals | HS7.2

Developing precipitation datasets for mountain regions in a changing climate 

Keith Shotton, Elizabeth Lewis, David Pritchard, and Nick Rutter

Around 22% of the global population depend on mountain runoff for their water supply. Due to its importance for future water resources, as well as flood and drought planning, an improved understanding of spatial precipitation patterns in mountain regions is needed. Precipitation gauge networks are sparse and traditional methods of interpolation yield inadequate precipitation fields for poorly gauged mountain catchments.

This research project builds on a new method, Random Mixing, to generate multiple random spatial daily precipitation fields, conditioned on gauge observations. The Random Mixing algorithm has so far been tested on larger, densely gauged catchments. This project adapts the approach for a sparsely gauged, small 9.1 km2 mountain catchment, Marmot Creek Research Basin in Alberta, Canada, where elevations range between 1600 m and 2825 m above sea level (a.s.l.). Quality-controlled total precipitation (i.e., rainfall and snowfall) gauge observations, for an 11-year period, from three weather stations around the catchment have been used to condition the random spatial fields.

To optimise selection of the most plausible fields, ensemble hydrological simulations are run, initially using a Python-coded version of the HBV spatially-distributed conceptual model, on a 50 m2 regular model grid. Optimisation involves the use of metrics, primarily Nash-Sutcliffe Efficiency (NSE) and bias, to identify the fields that result in the best match between observed and simulated streamflows. Sensitivity of these fields to seasonality, elevation and precipitation intensity is tested.

Results so far are promising. Even with very few gauges, improving the way that spatial covariance relationships between gauge locations are represented in the model has enhanced the quality of the spatial fields. The biggest improvement to date is from explicitly modelling the precipitation / elevation relationship, introducing gradients, and applying daily dry day and wet day parameters to each grid cell across the model domain.

Intended future work will aim to further refine the process using a physically-based spatially distributed model, the Cold Regions Hydrological Model (CRHM). Spatial fields generated using other random methods will be used to evaluate the performance of the new technique. Long time-period flood frequency curves generated using each approach will be compared. Different methods of phase partitioning will be evaluated to identify impacts on extreme flooding which is often controlled by snowpack melt. Climate change perturbations will be applied to generate potential future flood estimates.

How to cite: Shotton, K., Lewis, E., Pritchard, D., and Rutter, N.: Developing precipitation datasets for mountain regions in a changing climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1126, https://doi.org/10.5194/egusphere-egu23-1126, 2023.

EGU23-1157 | ECS | Posters on site | HS7.2

Spatial downscaling of rainfall fields using a multiple-point geostatistics-based approach 

Wenyue Zou, Guanghui Hu, Pau Wiersma, Shuiqing Yin, Grégoire Mariethoz, and Nadav Peleg

High-resolution gridded rainfall product at sub-daily and kilometer scales is required for many hydrological applications. In ungauged catchments, gridded rainfall data are often obtained through remote sensing, primarily satellites, whose spatial resolution is too coarse and requires to be downscaled to a finer resolution. The challenge is not only to downscale the rainfall intensity but also to downscale the spatial structure of rainfall fields, as both elements are essential for assessing the surface hydrological response. For this purpose, we further developed the stochastic multiple-point geostatistics (MPS) method, which enables the downscaling of long-term coarse-gridded rainfall using only a few years of high-resolution rainfall observations. We describe the methodology and demonstrate an application whereby long time series (1998-2019) of hourly CMORPH rainfall dataset are downscaled from 7 km to 1 km resolution based on training images from the 1-km CMPAS dataset available for a much shorter period (2015-2020), taking the area of Beijing as a case study. We show that the downscaled rainfall fields are following the expected spatial structure. Moreover, the downscaled rainfall intensities are consistent with station-based rainfall observations. And the heavy rainfall intensities at the 99th quantile match those expected due to the change in spatial scale and the application of an areal reduction factor. The results indicate that MPS preserves the spatial structure and downscales rainfall intensities well, especially for heavy rainfall, even if limited high-resolution training data is available. The proposed downscale approach can be applied to other rainfall datasets and in other regions.

How to cite: Zou, W., Hu, G., Wiersma, P., Yin, S., Mariethoz, G., and Peleg, N.: Spatial downscaling of rainfall fields using a multiple-point geostatistics-based approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1157, https://doi.org/10.5194/egusphere-egu23-1157, 2023.

EGU23-1357 | ECS | Orals | HS7.2

Is WaPOR precipitation data reliable over Iran? 

Mohsen Moghaddas and Massoud Tajrishy

As a result of satellite observations, ground observations, and data assimilation, global precipitation datasets have been developed for regions like Iran, where ground observations are limited. This study presents a comprehensive evaluation of WaPOR precipitation dataset over Iran at daily time scale. We considered a period of three years from 2019 to the end of 2021 and 394 synoptic rain gauges are used for the assessment. Daily WaPOR precipitation data at 250m scale downloaded and compared pixel-to-point with in-situ data. In addition, the WaPOR data and stations data were compared based on time classification (seasonal), location in the main catchment basins of Iran, and elevation above sea level. Calculating MSE, R score, RMSE and MSLE between real data(stations) and predict data(Wapor) shows some important result: 1. From the time point of view, WaPOR has best performance in summer (MSE = 4.94 and MSLE = 0.16) 2. Location, the best performance is related to stations of the catchment areas of the eastern part of Iran (Qaraqom basin with MSE = 11.9 and eastern border basin with MSE = 6.26) and the worst performance is related to the catchment area of the Caspian Sea (Mazandaran Sea basin with MSE = 64.06). 3. For analyzing the effect of elevation on precipitation, we divided the stations into 5 groups with an interval of approximately 600 meters (according to the lowest and highest elevation, which is -25 meters and 2965 meters). The best performance is related to stations with an altitude between 572 and 1170 meters (MSE = 21.61) and the worst is related to stations with an altitude between 1768 and 2366 meters (MSE = 43.79). 4. Moreover, on average for each station, in the three years of study (1096 days), we have 166 days (with standard deviation 119 days) that station has recorded precipitation but WaPOR dataset didn’t represent any record, so it’s not appropriate for daily hydrological models. 5. The difference between the three-year precipitation total at the station and the WaPOR precipitation total is 449.6 mm on average (with standard deviation 724.5).

How to cite: Moghaddas, M. and Tajrishy, M.: Is WaPOR precipitation data reliable over Iran?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1357, https://doi.org/10.5194/egusphere-egu23-1357, 2023.

EGU23-2705 | ECS | Posters on site | HS7.2

Impact of Spatio-Temporal Disaggregation of Rainfall on Hydrological Modelling 

Vemuri Harini, Abhinav Wadhwa, and Pradeep P. Mujumdar

Uncertainty assessment of rainfall patterns and the accompanying hydrological effects is essential to formulate effective adaptation strategies. Although the problem of equifinality in hydrological modelling has long been debated, its impact on hydrological analysis has not been sufficiently investigated. Traditional calibration techniques assume that input error is minimal, which might add a bias to the parameter estimates and impair the model predictions. Existing methods to overcome this issue are often weak due to both challenges in comprehending sampling errors in rainfall and processing limitations during parameter estimation. Such approaches consider structural and parameter uncertainties, whereas input and calibration data errors are often unaccounted for. This study aims to enhance the computational effectiveness of uncertainty analysis and separate the sources of uncertainty. Also, the implications of model input uncertainty to coupled human-natural-hydrologic systems and environmental changes are evaluated. A regression-based technique is developed to measure the level of uncertainty in the monsoon precipitation patterns for an urban catchment in Bangalore city, India. Sub-hourly rainfall datasets for various stations are estimated using disaggregation techniques such as scale-invariance and k-nearest neighbours-based methods. These datasets are fed into a hydrological model to connect the proposed method with the common framework for hydrological modelling. The findings demonstrate that the performance of a hydrological model is highly dependent on the spatio-temporal scale of the input rainfall in urban catchments where flash flood situations are envisaged.

How to cite: Harini, V., Wadhwa, A., and P. Mujumdar, P.: Impact of Spatio-Temporal Disaggregation of Rainfall on Hydrological Modelling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2705, https://doi.org/10.5194/egusphere-egu23-2705, 2023.

EGU23-3697 | ECS | Posters on site | HS7.2

Accounting for Precipitation Asymmetry in a Multiplicative Random Cascade Disaggregation Model 

Kaltrina Maloku, Benoit Hingray, and Guillaume Evin

Multiplicative random cascades (MRC) have been widely used for the disaggregation of coarse-resolution time series (e.g. daily) to high-resolution ones (e.g. sub-hourly). With MRCs, the amount of precipitation at any time step is partitioned into two parts, attributed respectively to the first and second sub-division of this time step. The partition is repeated throughout the cascade levels until the final temporal resolution is achieved.

In the so-called micro-canonical MRCs, the partition is conservative. The rainfall amounts R1 and R2 attributed respectively to the first and second sub-divisions of the considered time step (with rainfall amount R0), are expressed as R1=W1·R0 and R2=W2·R0 where the weights W1 and W2 are complementary, i.e.  W1+W2=1. The possible values of W1 are:

Therefore, for a given time step, the disaggregation is determined by the value of  W:=W1.

The probabilities p01, p10 and the distribution fW+ define the cascade generator of the MRC. For a given location, they have been found to depend on different factors. The cascade generator depends for instance on temporal scale, on precipitation intensity and on precipitation temporal asymmetry, i.e. on the temporal pattern of precipitation amounts Ri-1,Ri,Ri+1 around the amount of precipitation to disaggregate Ri (e.g. Olsson, 1998; Hingray and BenHaha, 2005). p01 tends to be higher than p10 in the case of a so-called "ascending" precipitation pattern (Ri-1<Ri<Ri+1) and,  p01 tends to be smaller than p10  in the case of a "so-called" descending pattern (Ri-1>Ri>Ri+1). Different models have been proposed to estimate p01,p10 and fW+ . Analytical scaling models are used very often because very convenient for simulation, but to date, they have disregarded the dependency on asymmetry (Paschalis et al., 2014).

Our work presents an analytical MRC modelling framework that merges the strengths of some of the different MRC models proposed in past years, allowing the cascade generator to depend in a continuous way on temporal scales, precipitation intensity and precipitation asymmetry.

We first define a precipitation asymmetry index and show how it influences the parameters of the cascade generator. This index is used to model the scaling dependency on asymmetry. We then compare four different analytical MRC models that account for the dependency on the temporal scale, precipitation intensity and/or precipitation asymmetry. An application to 81 stations in Switzerland is presented where the performance of the models is assessed. Including the asymmetry of precipitation in a model brings significant improvements in the reproduction of observed temporal persistence of precipitation in the disaggregated time series. The proposed model, with a simple parametrization, shows a great potential for regionalization, thus for the application of the approach to sites with coarse-resolution data only.

 

References

Hingray, B., Ben Haha, M., 2005. Statistical performances of various deterministic and stochastic models for rainfall series disaggregation. Atmospheric Research 77, 152–175.doi:10.1016/j.atmosres.2004.10.023.

Olsson, J., 1998. Evaluation of a scaling cascade model for temporal rainfall disaggregation. Hydrology and Earth System Sciences 2, 19–30. doi:10.5194/hess-2-19-1998.

Paschalis, A., Molnar, P., Fatichi, S., Burlando, P., 2014. On temporal stochastic modeling of precipitation, nesting models across scales. Advances in Water Resources 63, 152–166. doi:10.1016/j.advwatres.2013.11.006.

How to cite: Maloku, K., Hingray, B., and Evin, G.: Accounting for Precipitation Asymmetry in a Multiplicative Random Cascade Disaggregation Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3697, https://doi.org/10.5194/egusphere-egu23-3697, 2023.

EGU23-4747 | ECS | Orals | HS7.2

Stochastic Simulation of Realistic Continuous Snow Depth Time Series 

Jeongha Park and Dongkyun Kim

We propose an approach for stochastic simulation of realistic continuous snow depth time series using a snow depth estimation model and a stochastic weather generation model. The snow depth estimation model consists of three steps: (1) determination of the precipitation type, (2) estimation of  the snow ratio, and (3) estimation of the decreased snow depth. In the first step, air temperature and relative humidity are used as indicators to determine the type of precipitation when precipitation occurs. In the second step, when the type is determined as snow, the snow ratio is estimated, converting the depth of precipitation into depth of fresh snow. Here, the air temperature is used as an indicator to estimate the snow ratio using sigomidal relationship with the snow ratio. In the last step, the amount of decreased snow depth was estimated using a novel temperature index snowmelt equation considering a trend of depth-dependent decreasing snow depth. The snow depth estimation model was applied to the four snowiest meteorological stations of Korea and yielded high Nash Sutcliffe efficiency values which ranged between 0.745 and 0.875 for calibration, and ranged between 0.432 and 0.753 for validation. This calibrated snow depth estimation model was then applied to the simulated weather time series (precipitation, temperature, and relative humidity) from the stochastic weather generation model to simulate continuous snow depth time series. The simulated snow depth data accurately reproduced standard and extreme value statistics of the observed data, the latter of which were consistent with the estimates provided in Korean Building Code. Then, the model was extended to investigate the influence of climate change on the future snow depth. For this, future weather statistics were obtained by applying factor of change to the current weather statistics and then were used to calibrate the weather generation model. Lastly, the future snow depth time series for three future time windows (2021-2040, 2041-2070, and 2071-2100) were simulated using future weather time series and snow depth estimation model.

 

This research was supported by a grant(2022-MOIS61-003) of Development Risk Prediction Technology of Storm and Flood for Climate Change based on Artificial Intelligence funded by Ministry of Interior and Safety(MOIS, Korea).

How to cite: Park, J. and Kim, D.: Stochastic Simulation of Realistic Continuous Snow Depth Time Series, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4747, https://doi.org/10.5194/egusphere-egu23-4747, 2023.

EGU23-4828 | Posters on site | HS7.2

Investigating the quality of radar composites in a mountainous region in northeastern Thailand 

Punpim Puttaraksa Mapiam, Monton Methaprayun, Apiniti Jotisankasa, and Thom Bogaard

Composite radar products are made by combining radar scans of multiple radar stations into a single product to improve the quality of the radar product in overlapping region and to visualize the distribution and movement of precipitation over a large area. The reliability of radar composites depends on radar data quality, as each radar measurement is influenced by, among others, atmospheric conditions, interference with other sources, and the radar specifications. The quality of rain radar composites is critical as these products will be used for near real-time forecasting of hydrometeorological hazards. This research aims to investigate the controlling factors influencing the quality of radar composites over a hazard-prone mountainous region in northeastern Thailand. In this study we evaluate and quantify the rain radar composites by looking at four quality indexes among the distance to the radar station (DTR), the height of the beam above the ground (HTG), the radar beam blockage fraction (BBF), and the radar reflectivity fraction between the composited radar stations (RRF). For our overarching research to build a near real-time forecasting system for landslide and flashflood warnings in the Khao Yai National Park, Lamtakong basin and surroundings. Hereto, local cells of high intensity precipitation should be derived with highest accuracy. Two rain radar stations were selected: Sattahip, 220 kilometer southwest and Phimai, 140 kilometer North of the Lamtakong basin. Automatic rain gauges in the overlapping area were used to evaluate the radar composite product during storm events in 2020. The results indicated that specific quality indexes could be used to identify areas with inaccurate or unreliable raw data. This was a particular advantage in areas where the radar beam was (partly) blocked by an obstacle and underestimated the intensity of the storm. The BBF was the most important quality index in the study area. Moreover, combining the BBF with the RRF could increase the accuracy and reliability of radar rainfall estimates. Overall, using radar composites with raw radar data quality control can play an essential role in improving near real-time nowcasting for further natural hazard mitigation in the mountainous area.

How to cite: Mapiam, P. P., Methaprayun, M., Jotisankasa, A., and Bogaard, T.: Investigating the quality of radar composites in a mountainous region in northeastern Thailand, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4828, https://doi.org/10.5194/egusphere-egu23-4828, 2023.

EGU23-5224 | Posters on site | HS7.2

Projected changes in precipitation variability over Europe in CMIP6 climate models 

Eva Plavcová, Romana Beranová, Radan Huth, and Ondřej Lhotka

Changes in the amount, intensity, frequency and type of precipitation are observed in some places over recent decades (IPCC 2021). While much effort has been devoted to analyzing long-term changes in mean values and extremes, studies on changes in precipitation variability have been rather scarce. Long-term changes in climate variability are, nevertheless, an important aspect of the climate change with various impacts on society and environment. Therefore it is necessary to know whether and how the precipitation variability will change in the future. To this end, it is important that it is simulated correctly by recent climate models. In our study, we analyze outputs from an ensemble of different CMIP6 global climate models and several reanalyses and gridded observed datasets. We study long-term changes in day-to-day precipitation variability and how they differ between various datasets for the historical and current climate. We evaluate how successful the climate models are in reproducing precipitation variability, while identifying biases and errors common to all models or to groups of models. We analyze projected changes of short-term precipitation variability in model simulations over the whole 21st century. We focus on the North Atlantic-European sector. We consider wet-to-wet and dry-to-dry transition probabilities as a measure of short-term precipitation variability, focusing on winter and summer seasons separately.

 

Ref.: IPCC, 2021: Summary for Policymakers. In: Climate Change 2021: The Physical Science Basis. Contribution of Working Group I to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change [Masson-Delmotte, V., P. Zhai, A. Pirani, S.L. Connors, C. Péan, S. Berger, N. Caud, Y. Chen, L. Goldfarb, M.I. Gomis, M. Huang, K. Leitzell, E. Lonnoy, J.B.R. Matthews, T.K. Maycock, T. Waterfield, O. Yelekçi, R. Yu, and B. Zhou (eds.)].

How to cite: Plavcová, E., Beranová, R., Huth, R., and Lhotka, O.: Projected changes in precipitation variability over Europe in CMIP6 climate models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5224, https://doi.org/10.5194/egusphere-egu23-5224, 2023.

EGU23-5717 | ECS | Posters on site | HS7.2

Testing the performance of different WRF planetary boundary layer parameterizations schemes in the precipitation simulation under different Weather Regimes 

Joana Martins, David Carvalho, Alfredo Rocha, and Susana Cardoso Pereira

Surface meteorology is dominated by atmospheric boundary layer processes. Due to their typical low spatial resolution, numerical weather prediction models are not able to explicitly resolve such sub-grid scale processes, and as such use physical parameterization schemes to implicitly take into account these processes' influence on atmospheric variables. It is well known that the performance of such physical parameterization schemes depends on the atmospheric state of each location, season, etc.

This work aims to investigate the performance of six different WRF PBL parameterization schemes in the simulation of the precipitation over continental Portugal, under different weather regimes, or weather types. For this, a set of six weather regimes, which represent 96% of Portugal's atmospheric states were identified and for each WR, six different PBL parameterization schemes were tested.

Preliminary results show that for the entire region, the lowest spacial mean difference between observations and simulations is shown by the TEMF scheme parameterization for the positive phase of the North Atlantic Oscillation (NAO +) and Scandinavian height Weather Regimes,  MYJ for Summer Pattern, Anti-blocking (AB) and negative phase of the North Atlantic Oscillation (NAO -), and ACM2 scheme for Blocking (BLO) Weather Regime.

How to cite: Martins, J., Carvalho, D., Rocha, A., and Cardoso Pereira, S.: Testing the performance of different WRF planetary boundary layer parameterizations schemes in the precipitation simulation under different Weather Regimes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5717, https://doi.org/10.5194/egusphere-egu23-5717, 2023.

EGU23-6081 | ECS | Posters on site | HS7.2

Investigating the effects of extreme rainfall trends on the flow capacity of streams over the Northeast United States 

Stergios Emmanouil, Andreas Prevezianos, Andreas Langousis, and Emmanouil N. Anagnostou

While various research efforts investigate the direct effects of climate change on hydrometeorological variables, the incidental consequences of extreme rainfall trends on the flow capacity of open channels remains an open question. Hydrological modeling for the assessment of flood events and the organization of protection strategies usually include precipitation fields transformed by climate change factors. The latter, however, simply account for the relation (frequently through a ratio) between past and future Intensity-Duration-Frequency (IDF) values. Along these lines, epistemic uncertainties introduced by the choice of the IDF estimation techniques and/or the extensive incorporation of climate model simulations are accounted for through the application of safety factors on the yielded results. Yet, this practice may lead to a misestimation of flood risk, accompanied by costly, yet ineffective, protective measures. Moreover, the employment of high-resolution distributed hydrological models over extensive areas can be computationally cumbersome, while introducing an additional layer of uncertainty. In this study, we attempt to link the occurrence of channel overflowing to the evolution of the magnitude and frequency of extreme rainfall over the Northeast United States. More precisely, we: a) use measured streamflow data offered by the United States Geological Survey (USGS) during the 41-year period from 1979 to 2019, to assess the rate of occurrence of flood events over gauge locations across the study domain, and b) link the observed evolution of the aforementioned overflow rates to that of extreme rainfall for different return periods and durations of temporal averaging. In this context, we attempt to develop a conceptual basis for studying the effects of climate change on the linkage between rare precipitation events and the reliability of existing channels.

How to cite: Emmanouil, S., Prevezianos, A., Langousis, A., and Anagnostou, E. N.: Investigating the effects of extreme rainfall trends on the flow capacity of streams over the Northeast United States, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6081, https://doi.org/10.5194/egusphere-egu23-6081, 2023.

EGU23-6267 | ECS | Posters on site | HS7.2

Daily extremes from the MSWEP global rainfall dataset compared to estimates from buoy networks through MEVD-based downscaling 

Giorgio Dalmasso, Emmanouil Anagnostou, Luca Brocca, Elsa Cattani, Gaby Gruendemann, Lanxin Hu, Sante Laviola, Vincenzo Levizzani, Francesco Marra, Christian Massari, Efrat Morin, Efthymios Nikolopoulos, Ruud van Der Ent, Enrico Zorzetto, and Marco Marani

Estimating the frequency of extreme precipitation events, both locally and over extended areas, is key for developing risk reduction measures in present and future climates. Large areas of the world are characterized by sparse or absent rain-gauge networks, which poses significant challenges to the estimation of extreme events in many applications. Remote sensing and reanalysis datasets may contribute to filling some of these gaps, but their use meets some important obstacles: 1) remote sensing/reanalysis rainfall estimates are defined at coarse resolutions, thereby preventing direct validations against ground observations; 2) they usually span a ~20-year observation period, making it difficult to estimate the frequency of large extremes; 3) they suffer from significant uncertainties. Using the novel Metastatistical Extreme Value Distribution (MEVD) and a recent statistical downscaling technique, we compare ground and satellite-based/model estimates of rainfall to quantify the improvement achieved through downscaling in high-quantile quantification. We focus on ocean rainfall observations, which are rarely considered in validating global databases, from the Tao-Triton, Pirata, and Rama buoy networks. We quantify the estimation uncertainty for point extremes associated with the MSWEP rainfall dataset. We find that the MEVD-based extreme value downscaling approach generally improves point extreme estimates. 

How to cite: Dalmasso, G., Anagnostou, E., Brocca, L., Cattani, E., Gruendemann, G., Hu, L., Laviola, S., Levizzani, V., Marra, F., Massari, C., Morin, E., Nikolopoulos, E., van Der Ent, R., Zorzetto, E., and Marani, M.: Daily extremes from the MSWEP global rainfall dataset compared to estimates from buoy networks through MEVD-based downscaling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6267, https://doi.org/10.5194/egusphere-egu23-6267, 2023.

EGU23-6571 | ECS | Posters on site | HS7.2

Analysis of Projected Changes in Seasonal Precipitation Amounts for Central Asia Using the CMIP6 Multi-Model Ensemble Approach 

M. Tufan Turp, Nazan An, Zekican Demiralay, B. Cem Avcı, and M. Levent Kurnaz

Particularly due to its arid and semi-arid nature, the environmental, ecological and socio-economic systems of Central Asia are under serious threat of climate change. Depending on the climate change in Central Asia, water resources spread over limited physiographic regions in the domain, grasslands and related livestock are the elements that will be adversely affected by the negative changes. The vital resource in the arid and semi-arid Central Asia region, which is a kind of large continental rain shadow basin surrounded by mountains, is therefore water. For this reason, in this study, the changes in the total precipitation for Central Asia, which is the core region of the Asia continent and one of the 14 main domains of the COordinated Regional climate Downscaling EXperiment (CORDEX), were examined within the scope of Coupled Model Intercomparison Project-Phase 6 (CMIP6) models. In the study, a multi-model ensemble mean approach was applied in order to investigate the projected changes in seasonal precipitation amounts for three different future quarters (i.e., 2025-2049, 2050-2074, and 2075-2099) with respect to the reference period of 1975-1999 under various Shared Socioeconomic Pathways (i.e., SSP1-2.6, SSP2-4.5, SSP3-7.0, and SSP5-8.5).

Acknowledgement: This research has been supported by Boğaziçi University Research Fund Grant Number 19367. 

How to cite: Turp, M. T., An, N., Demiralay, Z., Avcı, B. C., and Kurnaz, M. L.: Analysis of Projected Changes in Seasonal Precipitation Amounts for Central Asia Using the CMIP6 Multi-Model Ensemble Approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6571, https://doi.org/10.5194/egusphere-egu23-6571, 2023.

EGU23-6866 | ECS | Orals | HS7.2

Sub-kilometre resolution climate model data: Added benefits in the representation of extreme precipitation? 

Emma Dybro Thomassen, Karsten Arnbjerg-Nielsen, Hjalte J. D. Sørup, Peter L. Langen, Jonas Olsson, Rasmus A. Pedsersen, and Ole B. Christensen

Climate change impact on extreme precipitation is of great importance to society. Small-scale, short-term events can have massive social and socioeconomic consequences. The present study analyses a new sub-kilometre (750 m) HARMONIE-Climate1 model simulation driven by ERA5 reanalysis data. The new sub-kilometre climate model data (750 m) is compared to NorCP data2 from climate models in 3, 5, and 12 km grid spacing, rain gauge station data and reanalysis data in 31 and 79 km resolution. The study examines a case area covering Denmark for five cloudburst seasons (April – October). The study aims to analyse how convective events are represented in the climate model data across grid resolution, and if an added benefit can be identified moving to sub-kilometre resolution.

Extreme convective events are analysed across datasets with respect to diurnal cycle, intensity levels and spatial structure. This is done at both hourly and sub-hourly scales. The 750 m climate model performs better for most metrics. However, climate models with 3 and 5 km grid spacing also perform well. The added computational and storage cost of the sub-kilometre scale experiments, thus only results in limited added benefit for this specific model set-up. Analysing hourly and sub-hourly temporal scales shows that the model performance varies between different temporal scales. The convection-permitting models, in general, represent hourly extremes much better than sub-hourly extremes. The sub-hourly scale is, therefore, essential to analyse to assess the model performance of convective events.

1 Belušić D, De Vries H, Dobler A, Landgren O, Lind P, Lindstedt D, Pedersen RA, Carlos Sánchez-Perrino J, Toivonen E, Van Ulft B, et al (2020) HCLIM38: A flexible regional climate model applicable for different climate zones from coarse to convection-permitting scales. Geosci Model Dev 13:1311–1333. https://doi.org/10.5194/gmd-13-1311-2020

2 Lind P, Lindstedt D, Kjellström E, Jones C (2016) Spatial and Temporal Characteristics of Summer Precipitation over Central Europe in a Suite of High-Resolution Climate Models. J Clim 29:3501–3518. https://doi.org/10.1175/JCLI-D-15-0463.1

How to cite: Dybro Thomassen, E., Arnbjerg-Nielsen, K., J. D. Sørup, H., L. Langen, P., Olsson, J., A. Pedsersen, R., and B. Christensen, O.: Sub-kilometre resolution climate model data: Added benefits in the representation of extreme precipitation?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6866, https://doi.org/10.5194/egusphere-egu23-6866, 2023.

EGU23-6981 | ECS | Orals | HS7.2

High-resolution simulations of tropical island thunderstorms: Does an increase in resolution improve the representation of extreme rainfall? 

Martin Bergemann, Todd Lane, Scott Wales, Sugata Narsey, and Valentin Louf

Recent increases in computational resources have led to the application of kilometre- and sub-kilometre-scale simulations in research, numerical weather prediction, and climate modelling alike. Despite anticipated improvements with resolution, there is still considerable work needed to evaluate how well such models improve the representation of intense convection. In this study we conduct ensemble simulations with kilometre- and sub-kilometre-scale horizontal grids to investigate intense convective events in the tropical island thunderstorm system Hector, which frequently occurs over the Tiwi Islands in North Australia. To avoid losing information through spatio-temporal averaging we apply a tracking algorithm to simulated and observed storms. When compared with observations, the model storms exhibit a lack of propagation across the study domain. In general, simulated storms are too intense but too small and too short-lived. This is especially true for the sub-kilometre simulations, where storms are more intense, smaller, and more numerous than in the kilometre-scale counterparts. We argue that size and duration errors compensate for storm number and intensity errors, which could lead to misleading interpretations when only comparing time and space averages of rainfall fields. Investigating some properties of the simulated storms suggests that storms with high rainfall intensities have stronger updrafts in the sub-kilometre model and are accompanied by an increase in cold pool intensity. The results and their resolution sensitivities highlight that the remaining parametrisations and their many tuning parameters in high-resolution set-ups influence the representation of convective storms in such models.

How to cite: Bergemann, M., Lane, T., Wales, S., Narsey, S., and Louf, V.: High-resolution simulations of tropical island thunderstorms: Does an increase in resolution improve the representation of extreme rainfall?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6981, https://doi.org/10.5194/egusphere-egu23-6981, 2023.

EGU23-7682 | ECS | Orals | HS7.2

A stochastic rainfall model with intensity dependent autocorrelations. 

András Bárdossy and Faizan Anwar

The space-time behaviour of precipitation is very complex. The knowledge of the dependence structures in space and time is very important for the assessment of flood risks. There are many different models available for stochastic simulations of precipitation time series. Most of the models are constructed such that the simulated time series match the autocorrelation structure of the observations in time along with the reproduction of spatial correlations. However, both auto and spatial correlations are value dependent i.e., if it is the upper or the lower tail. High and low intensity values have different dependence structures which have a significant influence on simulated extremes in space. In this presentation, first indicator correlations are introduced to show the intensity dependence of precipitation both in space and time at various resolutions. Then, a stochastic simulator based on gradual change of the correlations for the values in different parts of the distributions is introduced. The idea is that value dependent correlation is changed in such a way that the overall values remains same as that of a reference but not when considering values in different sections of the distributions alone. The model is applied to a large number of German catchments with hourly temporal resolution. The results are carefully analysed and compared to classical approaches.

How to cite: Bárdossy, A. and Anwar, F.: A stochastic rainfall model with intensity dependent autocorrelations., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7682, https://doi.org/10.5194/egusphere-egu23-7682, 2023.

EGU23-7751 | ECS | Orals | HS7.2

A Coarse-to-Fine Deep Learning Framework for High-Resolution Future Precipitation Map Generation 

Shan Zhao, Zhitong Xiong, and Xiao Xiang Zhu

Precipitation nowcasting, aiming to predict the rainfall intensity in the near future (usually 0-2h) [1], is crucial for urban planning, flood monitoring, agriculture management, and so on. Numerical weather modeling (NWP) takes a variety of data sources as the input of complex computer models that use mathematical equations to simulate the behavior of the atmosphere. Limited by the time needed for model spin-up, the performance in the short near future is not satisfactory. Deep learning (DL)-based method fills in the gap by treating nowcasting as a video prediction problem. The Convolutional LSTM [2] extracts spatial information when dealing with temporal series. The Generated Adversarial Network (GAN)-based [3] method shows potential in simulating the realisticness of the precipitation field. However, training such a model is very time-consuming and data-demanding [3] [4]. Different from natural images, the precipitation field to be estimated usually has a larger spatial size. Moreover, the convolutional layers tend to oversmooth the output and eliminate the small patterns that are important for the meteorologists to make the decision. Thus, we proposed a two-stage framework: the first one is to train an RNN-based model on the coarse field. The second is to downscale and style transfer from the coarse field to high-resolution precipitation maps based on GAN and Graph Convolutional Network (GCN). The coarse prediction will act as a constraint to the finer scale output and allows re-assignment of the spatial distribution of intensities. Such probabilistic output prevents the overestimation of the intensity. RNN is good at capturing long-range characteristics, and GCN [5] can extract local and neighborhood information, thus these two channels are naturally complementary to improve both local patterns and global accuracy scores. The GAN is used to make final output similar to real precipitation maps such as radar scans. To train the model, we downloaded the 2006-2016 ERA5 total precipitation at 0.25-degree spatial resolution and the DWD radar map [6] at 1km spatial resolution. We expect our model can capture the overall coverage of rainfall events and depict the spatial details. More importantly, this alleviates the data shortage problem, i.e., high-resolution precipitation nowcasting at places without ground-based radar stations can be acquired.

 

[1] Shi, Xingjian, et al. "Deep learning for precipitation nowcasting: A benchmark and a new model." Advances in neural information processing systems 30 (2017).

[2]Shi, Xingjian, et al. "Convolutional LSTM network: A machine learning approach for precipitation nowcasting." Advances in neural information processing systems 28 (2015).

[3] Ravuri, Suman, et al. "Skilful precipitation nowcasting using deep generative models of radar." Nature 597.7878 (2021): 672-677.

[4] Sønderby, Casper Kaae, et al. "Metnet: A neural weather model for precipitation forecasting." arXiv preprint arXiv:2003.12140 (2020).

[5] Shi, Yilei, Qingyu Li, and Xiao Xiang Zhu. "Building segmentation through a gated graph convolutional neural network with deep structured feature embedding." ISPRS Journal of Photogrammetry and Remote Sensing 159 (2020): 184-197.

[6] Ayzel, Georgy, Tobias Scheffer, and Maik Heistermann. "RainNet v1. 0: a convolutional neural network for radar-based precipitation nowcasting." Geoscientific Model Development 13.6 (2020): 2631-2644.

How to cite: Zhao, S., Xiong, Z., and Zhu, X. X.: A Coarse-to-Fine Deep Learning Framework for High-Resolution Future Precipitation Map Generation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7751, https://doi.org/10.5194/egusphere-egu23-7751, 2023.

EGU23-8567 | ECS | Posters on site | HS7.2

A parsimonious and efficient statistical method to correct large scale precipitation products: Empirical Conditional Probability (ECP)method 

Shima Azimi, Christian Massari, Silvia Barbetta, and Riccardo Rigon

Satellite-based precipitation products show significant bias with respect to ground-based data which prevents their use in several geophysical applications. In this study, we developed a method, the “Empirical Conditional Probability (ECP) method”, to augment the information of remotely sensed precipitation products using ground-based observation. The method relaxes the assumption of Gaussianity typical of many statistical processors which is a strong limitation specifically for the heavily skewed and intermittent daily precipitation signal leading to problems such as extrapolation to extreme values. We proposed a non-parametric and parsimonious approach to optimally merge the satellite and ground-based data.

The performance of our developed method is investigated in different experiments using the Climate Hazards Group InfraRed Precipitation with Station data (CHIRPS) precipitation product. Rain gauges are assumed as a priori information (predictors) about the true precipitation and is used to provide its posterior probabilistic estimation by our proposed empirical conditional probability approach. We compare our method with the classical Quantile mapping (QM) correction method to evaluate the added value of our approach.

The analysis was carried out in Aosta Valley, a region located in northern Italy with a dense rain gauge network. The time series was split into two sub-periods: 2008-2021 was used for generating the posterior distribution of precipitation and 2005-2007 was used for the validation of the method. The results demonstrated that the corrected CHIRPS product by our method is superior with respect to the original CHIRPS product and the corrected one with QM during both split periods (i.e., it performs better in terms of KGE, R, NSE, and RMSE). In a second experiment, using the proposed method, the posterior probability distribution of precipitation has been obtained according to the kriged ground-based precipitation data. In this way, instead of having gridded single-value data, a range of expected values is available for each pixel.

The idea of using uncertainty assessment for the satellite data (specifically precipitation) is going toward having cubic uncertainty-conscious satellite products with a range of expected values. Furthermore, since the ECP method is based on ground data, we investigated the sensitivity of the method to the density of rain gauges.

How to cite: Azimi, S., Massari, C., Barbetta, S., and Rigon, R.: A parsimonious and efficient statistical method to correct large scale precipitation products: Empirical Conditional Probability (ECP)method, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8567, https://doi.org/10.5194/egusphere-egu23-8567, 2023.

EGU23-9370 | Orals | HS7.2

Stochastic simulation of daily precipitation extremes in West Africa 

Jan Bliefernicht, Manuel Rauch, Marlon Maranan, Andreas Fink, and Harald Kunstmann

West Africa is one of the most data-poor regions in the world. In-situ precipitation observations are not available for many sites or contain many data gaps, thus leading to uncertainties and biases in hydrological studies in this region. To address this fundamental problem, we present a straightforward stochastic approach based on turning bands to simulate daily precipitation fields. Our approach is based on meta-Gaussian frameworks that generate Gaussian random fields, which are transformed into "real-world" precipitation fields using transfer functions. The simulation approach is tested for multiple extremes (1991 – 2016) in the Ouémé river basin in West Africa using different model settings and the most comprehensive station-based precipitation dataset available for this region. The evaluation shows that our approach is a valuable tool for simulation of daily precipitation fields and clearly outperforms classical interpolation techniques (e.g., ordinary kriging). Moreover, the simulation method can be conditioned on observations, uses only a small set of parameters and is an efficient algorithm for ensemble generation of precipitation fields for ungauged areas and design events.  In our West African research projects FURIFLOOD, the precipitation simulations are used as input information for hydrological modeling to reconstruct observed flood events and to create improved hazard maps for this region. Overall, the application of this advanced technique contributes to a better understanding of precipitation uncertainties and to the provision of improved station-based precipitation products for this challenging region.  

 

How to cite: Bliefernicht, J., Rauch, M., Maranan, M., Fink, A., and Kunstmann, H.: Stochastic simulation of daily precipitation extremes in West Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9370, https://doi.org/10.5194/egusphere-egu23-9370, 2023.

The knowledge of the statistical variability of precipitation (P) at short durations (≤24 h) is necessary to support engineering applications and hydrologic modeling. In this talk, we provide novel insights into the seasonal and spatial variability of two statistical properties of short-duration P that have received less attention, including the spatiotemporal correlation structure (STCS) and the marginal distribution. To this end, we design a framework based on multisite Monte Carlo simulations with the Complete Stochastic Modeling Solution (CoSMoS) which we test using a dense network of 223 high-resolution (30 min) rain gages with more than 20 years of observations in central Arizona. We first show that an analytical model and a three-parameter probability distribution capture the empirical STCS and marginal distribution of P, respectively, across Δt’s from 0.5 to 24 h and the summer and winter seasons. We then conduct Monte Carlo multisite stochastic simulations of P time series with CoSMoS, which reveal that the statistical properties of short-duration P exhibit significant seasonal differences, especially at low Δt. In summer, the STCS of P is weaker and the distributions are heavy-tailed because of the dominance of localized convective thunderstorms. Winter P has instead stronger STCS and lighter tails of the distributions as a result of more widespread and longer frontal systems. The Monte Carlo experiments also demonstrate that, in most cases, P is characterized by a homogeneous and isotropic STCS across the region, and by parameters of the marginal distribution that are constant for the shape and dependent on elevation for scale and P occurrence. The only exception is winter P at Δt ≥ 3 h, where anisotropy could be introduced by the motion of frontal storms, and additional factors are required to explain the variability of the scale parameter. The findings of this work are useful for improving stochastic P models and validating convection-permitting atmospheric models.

How to cite: Mascaro, G., Papalexiou, S., and Wright, D.: Utility of Multisite Stochastic Simulations to Characterize and Model the Seasonal and Spatial Variability of Short-Duration Precipitation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10062, https://doi.org/10.5194/egusphere-egu23-10062, 2023.

The intensity and frequency of extreme rainfall events are likely to increase under projected climate change scenarios. Given the adverse socio-economic impacts of these extreme events, we need to model their risk to develop effective policies for adaptation and mitigation. Simulating local hydrometeorological processes at the resolutions essential for assessing impacts and planning is computationally expensive using global climate models. Thus, there is a demand for efficacious downscaling from the coarse-resolution climate model outputs to the finer local scales of interest. Here, we develop a dynamic data-driven model coupled with physics, to downscale coarse-resolution climate model outputs (0.25° × 0.25°) to high-resolution (0.01° × 0.01°) rainfall. The downscaled rainfall is initially estimated by actively searching data on a manifold to learn the downscaling function incrementally using an iterative Gaussian process (GP). Upon convergence, the “first-guess” downscaled rainfall field, along with a physics-based estimation of orographic rainfall are processed by an adversarial learning framework (GAN) to refine finer-scale details. A stochastic sampling model and optimal estimation are used to correct the biases and obtain the final rainfall super-resolution fields. We assess the skill of the proposed model, using ERA5 reanalysis data and Daymet observation data at different terrain conditions (plain and hilly), and show that the downscaled rainfall closely matches the ground truth spatial patterns and extreme rainfall risk. By comparing the performance of individual components of our model (GAN, GP, and Physics) we find that the combined model outperform the individual components, and the GAN accounts for the maximum performance gain of the downscaling model.

How to cite: Saha, A. and Ravela, S.: Downscaling Precipitation Extremes Using Physics-coupled Dynamic Data Driven Adversarial Learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10931, https://doi.org/10.5194/egusphere-egu23-10931, 2023.

Tuning is now recognised as a key step in climate modelling, and the rise of machine learning techniques is increasing the number of targets used to tune these models. There are several reasons to focus on continental surface tuning. Firstly, a significant part of the sources of uncertainty in regional climate projections lie in the interactions between the atmosphere and the land surface. Secondly, the quality of climate change impact studies highly depends on a good representation of the climate at the surface. Finally, tuning at the surface can benefit from observational sites that provide multivariate, in situ hourly data of many meteorological, radiative and turbulent flux variables.

The objective here is to constrain the water and energy balances at the atmosphere-continental surface interface in the IPSL GCM, using as reference the in-situ observations of the SIRTA instrumented site (Paris suburb). A configuration of the coupled atmosphere (LMDZ) and continental surface (ORCHIDEE) model is set up on a zoomed grid in order to have a 30 km side mesh on the SIRTA point while keeping a reasonable computational cost. In addition, the winds (and possibly the temperature and humidity) are nudged towards the ERA5 reanalyses in order to compare the weather sequences observed at SIRTA with those of the climate model. This nudging technique allows a significant part of the internal variability of the local meteorology simulated by the GCM to be removed and to compare observations and model on a day-to-day basis. An essential step in setting up the tuning of this configuration is to assess the different sources of uncertainty involved. In this presentation, the characterisation of the uncertainties associated with the choice of configuration and the internal variability will be addressed more specifically, with a focus on clouds and precipitation.

In order to characterise the uncertainty linked to the internal variability, we compare the precipitation variability of a simulation ensemble with perturbed initial conditions with that of a perturbed physical ensemble obtained by machine-assisted exploration of the free parameters of the models. The internal variability of the precipitation simulated at SIRTA is found to be of the same order of magnitude as the parametric sensitivity, especially during convective periods, which questions the possibility of a tuning against SIRTA observations. We use a rainfall product (combining radar and rain gauges) from Météo-France in order to evaluate both the representation of spatial and temporal variability in a wider area around SIRTA and the associated uncertainty for tuning. We also present results concerning the uncertainty due to the configuration based on sensitivity tests to the grid configuration and the nudging setup. Finally, we evaluate the part of the precipitation variability due to the soil response by imposing an evaporation factor on the study area. We show how this configuration can be used in the atmosphere model tuning strategy, as it allows to get rid of the rainfall evaporation feedback.

How to cite: Coulon Decorzens, M. and Hourdin, F.: Assessment of precipitation variability sources in a GCM for the implementation of a tuning methodology using in-situ observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12080, https://doi.org/10.5194/egusphere-egu23-12080, 2023.

EGU23-13343 | Posters on site | HS7.2

The Application of Informational Predictability to Rainfall Data 

Alin-Andrei Carsteanu and Félix Fernández Méndez

Informational predictability, as defined in Fernández Méndez et al. [Stoch. Environ. Res. Risk Assess. (2023), submitted for publication] is based on the normalized complement of the expected value of the logarithm of the conditional probability, to be precise, this refers to the probability of the predicted events, when conditioned upon their respective predictors. The present work focuses on balancing the precision of the prediction, as measured by the narrowness of the predicted intervals, against the respective probabilities of a correct prediction, which finally amounts to maximizing the informational predictability. The data are high-resolution temporal rainfall intensity series, measured by an optical rain gauge.

How to cite: Carsteanu, A.-A. and Fernández Méndez, F.: The Application of Informational Predictability to Rainfall Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13343, https://doi.org/10.5194/egusphere-egu23-13343, 2023.

EGU23-13346 | ECS | Posters on site | HS7.2

The impact of vertical mixing schemes on the position of the ITCZ in the eastern tropical Pacific 

Chiara De Falco, Priscilla A. Mooney, and Jerry Tjiputra

The presence of a double Intertropical Convergence Zone (ITCZ) in the tropical Pacific is a persistent feature of global coupled ocean-atmosphere models that gives rise to excessive precipitation south of the equator. The ITCZ position is extremely sensitive to changes in the magnitude and distribution of the Sea Surface Temperature (SST) in the tropical band, due to the strong coupling between SST and convective precipitationThe complexity of the air-sea interactions makes it hard to disentangle the different mechanisms at play to identify the main driving processes behind this ubiquitous bias. Here, we use a coupled ocean-atmosphere regional model, the Coupled-Ocean-Atmosphere-Wave-Sediment Transport (COAWST) Modeling System, to investigate the impact that different parametrizations of the oceanic vertical mixing have on the water column dynamic, SST and subsequently the convective precipitation distribution in the eastern tropical Pacific. The model includes an atmospheric component, the Weather Research and Forecast Model (WRF), and an oceanic component, the Regional Ocean Modeling System (ROMS). The same atmospheric setup, with a resolution of 20km, has been forced with observed SSTs and with two ocean parameterizations. Different temperature gradients and oceanic stratification give rise to a double ITCZ or to a southward shift of the maximum precipitation band. Particularly in late winter and spring, a surface warming of a few degrees south of the equator around 5°S affects the distribution of the sea level pressure. The consequent changes in the surface wind pattern impact the usually asymmetric behavior of the trade winds, the south easterlies are no longer able to cross the equator and converge in the ITCZ in the northern hemisphere.  

How to cite: De Falco, C., Mooney, P. A., and Tjiputra, J.: The impact of vertical mixing schemes on the position of the ITCZ in the eastern tropical Pacific, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13346, https://doi.org/10.5194/egusphere-egu23-13346, 2023.

EGU23-14002 | ECS | Orals | HS7.2

On the improved ensemble of multi-source precipitation through joint automated machine learning-based classification and regression 

Hao Chen, Tiejun Wang, Carsten Montzka, Huiran Gao, Ning Guo, Xi Chen, and Harry Vereecken

Accurate precipitation representation at local and global scales will greatly improve our understanding of climate system changes. However, no precipitation estimate consistently has the lowest errors (systematic biases, random error, and rain/no-rain classification error) under varying environmental gradients, resulting in considerable uncertainty when investigating mechanisms and making predictions. Multiple Source Precipitation Ensemble (MSEP) is regarded as an indispensable approach to this challenge. Based on an automatic machine learning workflow, we propose an MSPE framework that uses machine learning classification and regression jointly. Six distinct precipitation products (e.g., satellite- and reanalysis-based estimates) and their ensembles based on different framework strategies were examined comprehensively at 818 gauges across China and 500 randomly selected sites (representing ungauged regions). The unique features of MSPE were investigated, including the necessity of assigning spatiotemporal dynamic weights and the usage of machine learning classification and regression jointly. Results demonstrated that MSPE could effectively reduce both random and classification errors associated with precipitation occurrences. In addition, the capacity to generalize and the interpretability of the ML models developed within the framework were compared and discussed in depth. We also summarized the current framework's limitations and potential expansions. The framework presented in this research is expected to be a robust and flexible framework for the global application of ensembles of precipitation estimates from numerous scales, data sources, and time periods.

How to cite: Chen, H., Wang, T., Montzka, C., Gao, H., Guo, N., Chen, X., and Vereecken, H.: On the improved ensemble of multi-source precipitation through joint automated machine learning-based classification and regression, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14002, https://doi.org/10.5194/egusphere-egu23-14002, 2023.

EGU23-14531 | Orals | HS7.2

A CP conditioned hybrid weather generator 

Ross Pidoto and Uwe Haberlandt

Long continuous time series of meteorological variables such as temperature and precipitation are required for applications such as derived flood frequency analyses. Observed time series are however generally too short, too sparse in space, or incomplete, especially at the sub-daily timestep. Stochastic weather generators allow an alternative to using observations, being able to generate time series of arbitrary length which are then used as input to hydrological models.

A hybrid hourly space-time weather generator has been developed based on a stochastic alternating renewal rainfall model. Modelling of non-rainfall climate variables is achieved using a non-parametric k-nearest neighbour (k-NN) resampling approach, which is coupled to the space-time rainfall model via rainfall state.

Circulation pattern (CP) or weather pattern classifications can be useful as a conditioning variable for stochastic rainfall models and weather generators. One primary use is the downscaling of future climate scenarios. Furthermore, CP conditioned models may better simulate rainfall and other climate variables through a better partitioning of observations into distinct rainfall and weather types.

Previous research has shown that the point rainfall model performs better, particularly regarding extremes, if conditioned on an optimised fuzzy-rule based objective weather pattern classification. Appropriate model revisions have now been made to allow the full hybrid space-time weather generator to also be conditioned on this classification.

This study assesses the performance of the weather pattern conditioned hybrid weather generator compared to the previous seasonal (summer-winter) conditioned model. For testing, 400 meso-scale catchments across Germany were selected. 

How to cite: Pidoto, R. and Haberlandt, U.: A CP conditioned hybrid weather generator, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14531, https://doi.org/10.5194/egusphere-egu23-14531, 2023.

EGU23-14968 | ECS | Orals | HS7.2

Determination of the spatial scaling relationship of rainfall extremes using radar data 

Golbarg Goshtsasbpour, Uwe Haberlandt@iww.uni-hannover.de, Ashish Sharma, Abbas El Hachem, Jochen Seidel, and Andras Bardossy

Climate models and their future projections, are normally provided in coarse spatial resolutions which makes them an imprecise source of information for certain hydrological purposes. Finding the proficient means of downscaling such data is one of the open questions of climate research. Previous research has shown that, the rainfall extremes show self-similarity in time and that a relatively similar behavior exists in regard to the spatial scale as well (Veneziano et al 2002). This study aims at determining the spatial scaling relationship of the rainfall extremes by using fine grids of radar datasets and upscaling them. In an empirical manner by aggregating the radar rainfall cells in space and for different cell sizes with a = 1, 2, 3, …12 km and for different durations of d = 5 min, 15 min 30 min, 1 hr, 2 hr, 4 hr, …, 24 hr the Annual Maximum Series are extracted. Using the AMS of different spatial and temporal scales and applying the Koutsoyiannis et at. 1998 method for rainfall extreme value analysis, the probability distribution function is fitted. Assessing the changes of the PDF parameters with the scale, with a logarithmic transformation on both variables; ln(parameter) vs. ln(scale), can show the sought relationship. The preliminary results of the study show definable non-linear relationships for location and scale parameters of the GEV distribution and the eta parameter of the Koutsoyiannis et al. 1998 parametrization.

 

Koutsoyiannis, D. Kozonis, and A. Manetas, A mathematical framework for studying rainfall intensity-duration-frequency relationships, Journal of Hydrology, 206 (1-2), 118–135, doi:10.1016/S0022-1694(98)00097-3, 1998.

Veneziano, Daniele; Furcolo, Pierluigi (2002): Multifractality of rainfall and scaling of intensity-duration-frequency curves. In Water Resour. Res. 38 (12), 42-1-42-12. DOI: 10.1029/2001WR000372.

How to cite: Goshtsasbpour, G., Haberlandt@iww.uni-hannover.de, U., Sharma, A., El Hachem, A., Seidel, J., and Bardossy, A.: Determination of the spatial scaling relationship of rainfall extremes using radar data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14968, https://doi.org/10.5194/egusphere-egu23-14968, 2023.

EGU23-15320 | ECS | Orals | HS7.2

High spatial and temporal resolution precipitation over Mediterranean basin for Digital Twin Earth Hydrology and 4dMED projects 

Paolo Filippucci, Hamidreza Mosaffa, Luca Brocca, and Christian Massari

The Mediterranean basin is a complex environment characterized by both exceptional biodiversity and intense human presence. This environment is already highly influenced by the anthropogenic activities, but their importance is expected to rise up due to the forecasted increase of population (from 480 million people to 520-570 million by 2030) and ongoing climate change. These conditions will trigger an increase of human pressures, including urbanization, industrialization, the expansion of intensive agriculture activities (i.e., irrigation) and aquaculture, thus threatening the natural resources availability, and specifically the water availability. Droughts, floods and landslides events are already stepping up in this environment, making it urgent to develop models systems capable to predict the extreme complex and widespread climate variations of this area.

ESA recognized the crucial role of this region by funding the Digital Twin Earth (DTE) Hydrology Evolution and the 4dMED projects, specifically dedicated to reconstruct the Mediterranean terrestrial water cycle at 1km spatial and 1 day temporal resolution and to develop a prototype of Digital Twin for the entire Mediterranean basin, which can be used for the prediction of hydrological extremes, the management of the water resource cycle and the simulation of the changes that the system may undergo. To reach those objectives, the latest developments of Earth Observation (EO) data as those derived from the ESA-Copernicus missions will be exploited together with in situ observations, hydrological and hydraulic models, artificial intelligence tools and advanced digital platform functionalities.

Among the hydrologic variables datasets generated within these projects, precipitation holds a major role due to its influence on the natural hazards occurrence. Here, we show the procedure adopted to generate the high spatial and temporal resolution precipitation product over the Mediterranean region by downscaling and merging different satellite and in-situ precipitation products. The obtained dataset is evaluated against high resolution observed data in several region of the Mediterranean basin, in order to assess its performance with respect to others EO derived precipitation datasets.

How to cite: Filippucci, P., Mosaffa, H., Brocca, L., and Massari, C.: High spatial and temporal resolution precipitation over Mediterranean basin for Digital Twin Earth Hydrology and 4dMED projects, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15320, https://doi.org/10.5194/egusphere-egu23-15320, 2023.

EGU23-706 | ECS | PICO | HS7.1

Multi-scale comparison of rainfall measurement with the help of a disdrometer and a mini vertically pointing Doppler radar 

Mateus Seppe Silva, Rodrigo Vieira Casanova Monteiro, Jerry Jose, Auguste Gires, Ioulia Tchiguirinskaia, and Daniel Schertzer

Local rainfall measurements can be done in a significant range of methods which rely on very different underlying measurement concepts and assumptions. As an illustration, mechanical rain gauges collect small rainfall amounts; optical disdrometers assess size and velocity of each drop passing through a sampling area, while  Doppler sensors derive a rain rate from estimated average fall velocity. Hence, the quality of the measurements can vary a lot, depending on factors such as rain drop size, wind velocity, rain rate etc. Understanding the differences between various technologies enables us to determine the most reliable device depending on each raining condition. This research aims to compare the performance of two of those devices: the optical disdrometer Parsivel2 (manufactured by OTT) and a mini Doppler radar part of a mini Meteorological Station (manufactured by Thies). The comparison was done with two research focuses: by evaluating the scaling features of the fields measured by both instruments utilizing the framework of Universal Multifractals (UM) to have a performance assessment valid across scales and not only separated scales, and by analyzing the influence of physical parameters namely drop size, wind velocity and rainfall rate in the performance of the devices.

The data used was collected on a meteorological mast located in the Pays d’Othe wind farm, 110km southeast of Paris. This measurement campaign is part of the RW-Turb project (https://hmco.enpc.fr/portfolio-archive/rw-turb/; supported by the French National Research Agency (ANR-19-CE05-0022). The mast is operated with two sets of devices, one around 75m in height and the other around 45m. The observation time step of the Parsivel2 is of 30 seconds, and it measures full binned drop size and velocity distribution, while the mini station provides data (rainfall, 2D wind, temperature, pressure, humidity) with 1 second time step. In general, the mini-doppler radar is found to measure a smaller amount of rain with regards to the  Parsivel2. More precisely, we found that the mini doppler radar returned very low rain measurements when subjected to rain conditions with a bigger mean drop size (Dm), and that heavy wind was related to a non-detection of the field in situations with light rain. Scaling analysis enabled us to show that mini Doppler radar exhibited white noise from observation scale smaller than 4s. Hence, it was used only with large time steps. UM analysis also revealed different scaling behaviour for mini Doppler radar rain data at finer temporal resolution than that of Parsivel (30 s).

 

 

How to cite: Seppe Silva, M., Vieira Casanova Monteiro, R., Jose, J., Gires, A., Tchiguirinskaia, I., and Schertzer, D.: Multi-scale comparison of rainfall measurement with the help of a disdrometer and a mini vertically pointing Doppler radar, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-706, https://doi.org/10.5194/egusphere-egu23-706, 2023.

EGU23-2689 | PICO | HS7.1

Precipitation measurement based on satellite data and machine learning 

Lu Yi, Zhangyang Gao, Zhehui Shen, Haitao Lin, Zicheng Liu, Siqi Ma, Stan Z. Li, and Ling Li

Satellite infrared (IR) data, with high temporal resolution and wide coverages, have been commonly used in precipitation measurement. However, existing IR-based precipitation retrieval algorithms suffer from various problems such as overestimation in dry regions, poor performance in extreme rainfall events, and reliance on an empirical cloud-top brightness-rain rate relationship. To solve these problems, a deep learning model using a spherical convolutional neural network was constructed to properly represent the Earth's spherical surface. With data inputted directly from IR band 3, 4, and 6 of the operational Geostationary Operational Environmental Satellite (GOES), the new model of Precipitation Estimation based on IR data with Spherical Convolutional Neural Network (PEISCNN) was first trained, tested and validated. Compared to the commonly used IR-based precipitation product PERSIANN CCS (the Precipitation Estimation from Remotely Sensed Information Using Artificial Neural Network, Cloud Classification System), PEISCNN showed significant improvement in the metrics of POD, CSI, RMSE and CC, especially in the dry region and for extreme rainfall events. The PEISCNN model may provide a promising way to produce an improved IR-based precipitation product to benefit a wide range of hydrological applications.

How to cite: Yi, L., Gao, Z., Shen, Z., Lin, H., Liu, Z., Ma, S., Li, S. Z., and Li, L.: Precipitation measurement based on satellite data and machine learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2689, https://doi.org/10.5194/egusphere-egu23-2689, 2023.

EGU23-4992 | PICO | HS7.1

The Fresnel Platform for Greater Paris: enhancing the urban resilience with the fully distributed and physically based model, Multi-Hydro 

Guillaume Drouen, Daniel Schertzer, Auguste Gires, and Ioulia Tchiguirinskaia

The aim of the Fresnel platform of École des Ponts ParisTech is to develop research and innovation on multiscale urban resilience. To achieve this goal, it is therefore conceived as a SaaS (Software as a Service) platform, providing data over a wide range of space-time scales and appropriate softwares to analyse and simulate them over this range.

To study the different technical solutions of the water cycle in an urban environment at different scales, RadX now provides a user-friendly graphical user interface to run simulation using a fully distributed and physically based model: Multi-Hydro.

This model that has been developed at École des Ponts ParisTech, from four open-source software applications already used separately by the scientific community. Its modular structure includes a surface flow module, sewer flow module, a ground flow module and a precipitation module. It is able to simulate the quantity of runoff and the quantity of rainwater infiltrated into unsaturated soil layers from any temporally-spatially varied rainfall event at any point of the peri-urban watersheds. The spatial and temporal variation of meteorological, hydrological, geological and hydrogeological data across the model area is described in gridded form of the input as well as the output from the model.

The use of RadX as a graphical user interface gives users the ability to easily customize the input data for their simulation. They can, for instance, modify the land use to study the effect of urban climate mitigation strategies like green roofs. They can select real hydrological events measured by the ENPC X-Band radar as rainfall input, but also generate virtual rainfall events. To ease the interpretation of the simulation, RadX can render interactive 2D and 3D graphics directly in the users' web browser by the use of open source libraries that focus on performance using low level graphic API. For example, it gives the user an intuitive and efficient way to spot singular points of the infiltration output display. Users can also download the file outputs to use in their GIS software.

Other components can be integrated to RadX to satisfy the particular needs with the help of visual tools and forecasting systems, eventually from third parties. Developments are still in progress, with a constant loop of requests and feedback from the scientific and professional world.

How to cite: Drouen, G., Schertzer, D., Gires, A., and Tchiguirinskaia, I.: The Fresnel Platform for Greater Paris: enhancing the urban resilience with the fully distributed and physically based model, Multi-Hydro, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4992, https://doi.org/10.5194/egusphere-egu23-4992, 2023.

The microphysical processes were found to be vital in facilitating the system evolution for a merger-formation bow echo (MFBE) in southeast China, where the reinforced precipitation enhanced the cold pool strength via evaporation cooling. However, current numerical model failed to accurately perform such processes, suggesting the large uncertainties for microphysical schemes in simulating MFBE events in southeast China. In this study, three microphysics schemes including Thompson (THOM), Morrison (MORR), and Weather Research and Forecasting Double-Moment 6-Class (WDM6) schemes were evaluated by comparing against polarimetric observations and Variational Doppler Radar Analysis System (VDRAS) analyses. The three schemes captured the basic kinematic structures for this MFBE event after assimilating radar radial velocities, but all underpredicted the cold pool strength by ∼25%. Particularly, THOM produced the best raindrop size distributions (DSDs) and precipitation pattern, and the larger raindrop size bias and the weak cold pool strength were owing to the relatively low rain breakup efficiency and inefficient rain evaporation, respectively. By decreasing the cutoff diameter of rain breakup parameterization from the default 1.6–1.2 mm (i.e., increasing breakup efficiency) and increasing evaporation efficiency by threefold in THOM, the simulated DSDs and precipitation were greatly improved, and the cold pool strength was significantly increased from 77% to 99% compared to that in VDRAS analyses. This study illustrated a plausible approach of combining polarimetric radar retrievals and VDRAS analyses as bases to adjust THOM default settings in simulating a MFBE event in southeast China with physical characteristics more consistent with observations. Since microphysical processes vary from convective organizations and climate regions, it is recognized more cases studies are needed in the future to examine the validity and approach in this study to improve simulations and predictions of MFBEs in southeast China.

How to cite: Zhao, K., Zhou, A., Lee, W.-C., and Huang, H.: Evaluation and Modification of Microphysics Schemes on the Cold Pool Evolution for a Simulated Bow Echo in Southeast China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6808, https://doi.org/10.5194/egusphere-egu23-6808, 2023.

EGU23-7987 | ECS | PICO | HS7.1

Spatiotemporal pattern of precipitation in the Pearl River basin, China from 1951 to 2015 

shirong Cai, Kunlong Niu, Xiaolin Mu, and Xiankun Yang

Precipitation is one of the most important factors in hydrological cycle and climate change. Due to global climate change, the global and regional hydrological cycle has been changed significantly, and the precipitation pattern has changed, which made natural disasters happened more frequent. In this study, we taken the Pearl River Basin as a case study area and used APHRODITE dataset to investigate the spatiotemporal trend of precipitation during the period of 1951-2015 based on six extreme rainfall indices recommended by the WMO. Then, the MK test was used to verify their trend and analyze the temporal and spatial variability. The results indicated that: (1) The annual PRCPTOT in the Pearl River Basin displayed an increasing trend with an increasing rate of 0.019mm/yr. Although the number of annual rainy days was decreasing, the annual SDII exhibited an increasing trend. The annual R95P and RX1day exhibited an increasing trend, but the R95D and CWD showed a decreasing trend. The seasonal PRCPTOT increased in summer and winter, but decreased in spring and autumn. R95P and SDII displayed an increasing trend in four seasons. (2) The annual variation of PRCPTOT increased from west to east, the trend of SDII, R95P and RX1day were similar with PRCPTOT, but the high value of R95D happened in the middle and lower reaches of Xijiang River, and CWD increased from north to south. Except autumn, the seasonal spatial distribution of PRCPTOT, SDII and R95P were similar. In spring and winter, the spatial distribution of PRCPTOT, SDII and R95P increased from west to east, and from north to south in summer, indicating that the Beijiang River basin and Dongjiang River basin had a higher flood risk. (3) MK test of indices shown that the Yunnan-Guizhou Plateau was becoming drier, and the risk of extreme rainfall was increasing in the Beijiang River basin and Dongjiang River basin. The study results are valuable for future water resources management and ecological environment protection in the Pearl River Basin.

How to cite: Cai, S., Niu, K., Mu, X., and Yang, X.: Spatiotemporal pattern of precipitation in the Pearl River basin, China from 1951 to 2015, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7987, https://doi.org/10.5194/egusphere-egu23-7987, 2023.

EGU23-9256 | PICO | HS7.1

Improving shape-dependent snow fall speed relationships using different particle size parameters 

Thomas Kuhn, Salomon Eliasson, and Sandra Vázquez-Martín

Meteorological forecast models, notably snowfall predictions, require accurate knowledge of the properties of snow particles, such as their size, cross-sectional area, mass, shape, and fall speed. Therefore, measurements of individual snow particles’ fall speed and their cross-sectional area, from which a size parameter and area ratio can be derived, provide very useful datasets. We have compiled such a dataset from measurements with the Dual Ice Crystal Imager (D-ICI) in Kiruna during several winter seasons from 2014 to 2019. Using that data, we have previously studied shape-dependent relationships between fall speed and particle size, cross-sectional area, and particle mass. While we had used maximum dimension as the size parameter, we have found that it seems unsuitable for certain shapes like columnar particles. Here, we investigate which particle size parameter should be used depending on the shape or if one size parameter is suitable for all shapes. With a more suitable particle size parameter, we aim to improve the relationships between fall speed and particle size and mass.

How to cite: Kuhn, T., Eliasson, S., and Vázquez-Martín, S.: Improving shape-dependent snow fall speed relationships using different particle size parameters, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9256, https://doi.org/10.5194/egusphere-egu23-9256, 2023.

EGU23-10190 | PICO | HS7.1

A novel methodology for remote sensing retrieval of rainfall rates 

Massimiliano Ignaccolo and Carlo De Michele
We propose a new methodology for rainfall rate retrieval from remote sensing observations using 166 datasets from 76 different locations on Earth's surface. The method rests upon the data science parametrization of the drop size distribution [Ignaccolo and De Michele (2022) : https://doi.org/10.1175/JHM-D-21-0211.1]. It retrieves the possible triplets (drop count, mean diameter of the drop size distribution, skewness of the drop size distribution) associated with given values of the horizontal and vertical reflectivities. We demonstate how this novel approach is superior to a standard one based upon the mass weighted diameter, normalized intercept and gamma functional form for the drop size distribution. 
 

How to cite: Ignaccolo, M. and De Michele, C.: A novel methodology for remote sensing retrieval of rainfall rates, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10190, https://doi.org/10.5194/egusphere-egu23-10190, 2023.

In previous work [Aguilar Flores et al., Stoch. Environ. Res. Risk Assess. (2021) 35: 1681-1687], distributional convergence of breakdown coefficients (BDCs) to symmetric probability distribution functions of weights in discrete-scale multiplicative cascades has been shown. Asymmetric weights distributions, however, cannot become the limiting functions of symmetric BDC distributions. A procedure has been devised and is presented herein for the computation of the limiting distributions in the aforementioned cases, involving a convolution that is identified with the first-level BDCs probability distribution, and thereby can be used for the purpose of model validation in otherwise non-ergodic single realizations of multiplicative cascade models.

How to cite: Aguilar Flores, C. and Carsteanu, A. A.: Breakdown coefficients of multiplicative cascades having asymmetrically distributed generators with bounded essential range, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10237, https://doi.org/10.5194/egusphere-egu23-10237, 2023.

EGU23-12061 | ECS | PICO | HS7.1

Classification of snow and rainfall using commercial microwave links 

Erlend Øydvin, Rasmus Falkeid Hagland, Vegard Nilsen, Mareile Astrid Wolff, and Nils-Otto Kitterød

The use of Commercial microwave links (CMLs) to estimate rainfall has been under investigation for the past 15 years. CMLs still seem like a promising supplement to standard measurement methods. So far, CMLs have almost exclusively been applied for rainfall only situations. It is expected that different precipitation types affect the CML signal strength and error sources differently. For CML applications in high latitude countries with frequent and extended periods with snowfall and mixed precipitation, an extension of the classification methods for these precipitation types is needed. 

In this presentation we study how the CML signal attenuation is affected by different precipitation types and how those can be used to classify the different events. We use nearby disdrometers as a ground truth reference and CML data from different climatological conditions in Norway.

How to cite: Øydvin, E., Hagland, R. F., Nilsen, V., Wolff, M. A., and Kitterød, N.-O.: Classification of snow and rainfall using commercial microwave links, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12061, https://doi.org/10.5194/egusphere-egu23-12061, 2023.

EGU23-12265 | PICO | HS7.1

Using Opportunistic Rainfall Sensing to improve Areal Precipitation Estimates and Run-off Modelling – The Case Study of the Ahr Flood in July 2021 

Jochen Seidel, András Bárdossy, Micha Eisele, Abbas El Hachem, Christian Chwala, Maximilian Graf, Harald Kunstmann, Norbert Demuth, and Nicole Gerlach

On 14 and 15 July 2021, heavy and prolonged precipitation caused flooding in large areas in western Germany and adjacent regions. The Ahr River valley in the Federal State of Rhineland-Palatinate was particularly affected, with numerous fatalities and large-scale damage. Due to the spatio-temporal variability of precipitation and failure of several gauging stations, the estimation of the flood triggering areal precipitation as well as determination of peak discharges is associated with high uncertainties.

In this study, we present results where data from opportunistic sensors (commercial microwave links (CML) and personal weather stations (PWS)) were used to interpolate hourly precipitation sums for the Ahr catchment. The data from the opportunistic sensors was quality controlled, filtered and interpolated using the methods from Graf et al. (2021). This precipitation data was compared to a gauge adjusted weather radar product from the German Weather Service DWD as well as interpolated rain gauge data. In order to determine the maximum discharges at the gauges in the Ahr, flood was simulated with the water balance model LARSIM (Large Area Runoff Simulation Model) using the aforementioned precipitation products as input data.

The results show that the areal precipitation obtained from opportunistic sensors yielded higher sums than the gauge adjusted radar products and the interpolated gauge data, especially in the northern part of the Ahr catchment where the station density of the conventional rain gauges was not sufficient to capture the spatial variability of this extreme event. Furthermore, the modelled run-offs using the precipitation input from opportunistic sensors yielded higher and more plausible peak discharges than the ones with the gauge adjusted weather radar product. This suggests that the radar underestimated precipitation due to attenuation. The difference in the resulting peak discharges point to the fact that due to the saturated soils any additional precipitation during the flood event in July 2021 lead to a direct run-off effect.

 

References:

Graf, M., El Hachem, A., Eisele, M., Seidel, J., Chwala, C., Kunstmann, H., & Bárdossy, A. (2021). Rainfall estimates from opportunistic sensors in Germany across spatio-temporal scales. Journal of Hydrology: Regional Studies, 37, 100883.

How to cite: Seidel, J., Bárdossy, A., Eisele, M., El Hachem, A., Chwala, C., Graf, M., Kunstmann, H., Demuth, N., and Gerlach, N.: Using Opportunistic Rainfall Sensing to improve Areal Precipitation Estimates and Run-off Modelling – The Case Study of the Ahr Flood in July 2021, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12265, https://doi.org/10.5194/egusphere-egu23-12265, 2023.

EGU23-12880 | PICO | HS7.1

Modelling Typhoon Rainfall with Universal Multifractal 

Ching-Chun Chou, Auguste Gires, and Li-Pen Wang

Universal Multifractal (UM) has been a useful tool to model rainfall processes across a wide range of spatialtemporal scales. Double Trace Moment (DTM) is a technique that helps estimate parameters for the UM model. Based upon the estimated UM parameters, a discrete random cascade process can be used to generate samples with realistic rainfall properties. UM parameters are of physical meanings, representing the levels of mean intermittence (C1) and the changing rate of the mean intermittency deviating from the average field (α, know as the multifractality index), respectively. Therefore, these parameters are also widely used to characterise rainfall features across scales. UM has been tested in many countries under various weather conditions. However, its applications to extreme storm events, such as typhoons, are limited. In light of this, this study intends to analyse UM’s capacity of capturing and modelling extreme storm events recorded by a rainfall monitoring network in the South of Taipei City. On the roof of the Civil Engineering Research Building at National Taiwan University, an innovative extreme rainfall monitoring campaign has been set up and collecting high-quality rainfall measurements at fine timescales over the past two years. Rainfall data from several extreme rainfall events, including four typhoons and 10+ thunderstorms, has been collected. In this work, high-resolution rainfall time series from the laser disdrometer for typhoon Nalgae is used for analysis. Rainfall measurements are first aggregated from the native 10-second resolution to 80-second and coarser resolution and then downscaled back to 10-second to verify the downscaling results. The UM analysis is conducted in three different ways. The first way is to apply UM analysis to the entire time series. The resulting parameters are α = 1.32 and C1 = 0.108. Then, the time series is equally divided into 16 sections such that the temporal variations in rainfall features can be observed. Similarly to the first way, the second way applies the ’standard’ UM analysis but to each section. This leads to α ranging from 1.1 to 1.9 and C1 from 0.05 to 0.18. Finally, the third way applies ’ensemble’ UM analysis that concatenates divided sections into a single matrix. This results in α = 1.55 and C1 = 0.125. The derived parameters are then used to sample 10-second rainfall estimates with a discrete cascade process. The performance is quantified based upon the capacity of preserving observed extreme features. We first analyse the ranges of α and C1 resulting from the samples downscaled from the first and the third ways. We can see that the resulting α ranging from 1.2 to 1.8 and C1 from 0.06 to 0.16, which fails resembling the aforementioned variability of the UM parameters (i.e. 1.1−1.9 and 0.05−0.18). In fact, only the second way leads to satisfactory result. This preliminary study suggests that typhoon rainfall experiences drastic behaviour changes within a short period, which requires a more ’dynamic’ way to model these changes well. Similar analyses will be conducted over other collected typhoons and thunderstorm events to see if the findings can be generalised.

How to cite: Chou, C.-C., Gires, A., and Wang, L.-P.: Modelling Typhoon Rainfall with Universal Multifractal, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12880, https://doi.org/10.5194/egusphere-egu23-12880, 2023.

EGU23-13080 | ECS | PICO | HS7.1

Challenges in the usage of commercial microwave links for the generation of transboundary German-Czech rainfall maps 

Nico Blettner, Martin Fencl, Vojtěch Bareš, Christian Chwala, and Harald Kunstmann

Attenuation data from commercial microwave links (CMLs) has proven useful for estimating rainfall. Their major benefits are a high abundance in most regions on earth, a high resolution in time, close to ground measurement, and the absence of installation costs and efforts. The spatial and temporal coverage of CMLs would theoretically enable the generation of continental rainfall maps for various aggregation times.

However, there exist limitations that have so far inhibited rainfall estimation on larger scales. The data is generally obtained on a national basis from different network providers and networks can vary significantly in characteristics such as frequency and length distributions. CML data requires careful processing that depends on these characteristics and which has so far been adjusted to independent data sets only.

In this study we investigate what kind of processing is required to use independent and heterogeneous CML data sets for the generation of transboundary rainfall maps. We use 3900 CMLs from Germany and 2500 CMLs from the Czech Republic. The German data set is rather evenly distributed with respect to spatial coverage, frequencies and lengths. The Czech data set, on the other hand, varies significantly more in all these regards: it is characterized by dense networks of short CMLs in the cities, a large share of CMLs with E-Band frequency, and hence a large range of sensitivities.

We find that quality control is important especially when dealing with independent data sets. We propose several algorithms and the consideration of network characteristics when combining two CML data sets, and show how adapted but straightforward processing allows the generation of transboundary rainfall maps.

How to cite: Blettner, N., Fencl, M., Bareš, V., Chwala, C., and Kunstmann, H.: Challenges in the usage of commercial microwave links for the generation of transboundary German-Czech rainfall maps, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13080, https://doi.org/10.5194/egusphere-egu23-13080, 2023.

In an attempt to get the best parameter estimations of the theoretically consistent IDF (Intensity Duration Frequency) models of rainfall intensity for the entire state of Baden Wuerttemberg, three well-defined optimization algorithms such as Differential Evolution (DE), Nelder Mead (NM), and TNC Truncated Newton (TNC) are taken into account for comparison.

Seven-parametric IDF model contains mean intensity µ, intensity scale parameters λ1, λ2 , time scale parameter α, fractal/smoothness parameter Μ, Hurst parameter Η, exponent of the expression of probability dry θ,  and tail index ξ, which are obtained by minimizing the error between empirical k-moments and model quantiles. Error metric focusing on distribution quantiles x(k,T) is thus minimized for all available scales k and a series of return periods T . Non-linear solver is chosen to perform this step as these errors are non-linear functions of the parameters.

All results are demonstrated visually, and a final decision is made on the basis of precisely fitted parameter values to the model. This crucial step will also assist us in finding the optimum design values for stormwater and floods.

How to cite: Amin, B. and Bárdossy, A.: Comparative Analysis of Parameter Optimization of Theoretically Consistent IDF Models of Rainfall Intensity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14215, https://doi.org/10.5194/egusphere-egu23-14215, 2023.

EGU23-14295 | PICO | HS7.1

OpenMRG: Open data from Microwave links, Radar, and Gauges for rainfall quantification in Gothenburg, Sweden 

Remco (C.Z.) van de Beek, Jafet Andersson, Jonas Olsson, and Jonas Hansryd

In a changing climate accurate measurements and near-real time rainfall monitoring are essential for sustainable societies. Commercial microwave links (CMLs) offer a great alternative, or addition, to traditional sensors, like rain gauges and radar. While CMLs are a great source of opportunistic sensors the data from CMLs are usually limited by their accessibility for both research and actual implementation. To help in gaining better access and research into CML-derived rainfall we present a dataset at 10 second resolution with true coordinates for 364 bi-directional CMLs gathered during a pilot study in Gothenburg, Sweden over a three-month period (June-August 2015). These data are complemented by additional data from 11 high-resolution rain gauges (ten 1 min and one 15 min) and radar data (5 min and 2 km resolution) from the Swedish operational weather radar composite over the Gothenburg area.

Analysis of the data show that data collection is very complete, with 99.99% of the CMLs, 100% rain gauges and 99.6% of the radar data available. The gauge data shows that around 260mm rainfall was measured during this period with 6% precipitation during 15-minute intervals. At the Torslanda gauge on 28 July 2015 one the of the most intense events was observed during the three-month period with a peak intensity of 1.1 mm min−1. The CML data reflect this event well and show a drop of around 27 dB during the peak intensity. Radar data also showed a good distribution of the reflectivity of the precipitation with some measurements above 40 dBZ, which is commonly taken as an indication of convective precipitation. Some low intensity clutter was also found, mostly around -15 dBZ.

The data are accessible at https://doi.org/10.5281/zenodo.7107689 (Andersson et al., 2022). The sharing of these Open high-resolution data of Microwave links, radar and gauges (OpenMRG) should enable further research in microwave-link based environmental monitoring. In the longer term we hope that this dataset will also contribute to easier access of CML data and help in the development of the merging of multi-sensor products.

How to cite: van de Beek, R. (C. Z. )., Andersson, J., Olsson, J., and Hansryd, J.: OpenMRG: Open data from Microwave links, Radar, and Gauges for rainfall quantification in Gothenburg, Sweden, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14295, https://doi.org/10.5194/egusphere-egu23-14295, 2023.

The safety of autonomous vehicles will depend critically on the performance of sensors (such as 77GHz radar), which will degrade in the presence of propagation losses during severe weather events. Variations in the drop size distribution lead to significant uncertainty in attenuation estimates. As part of the UK government's commitment to the safe introduction of autonomous vehicles, and in collaboration with the National Physical Laboratory, we have set up a series of observing platforms at Met Office Cardington to measure a multitude of weather-related variables such as temperature, pressure, illumination, precipitation particles, fog, etc. In this contribution, I will cover our work on characterising the rain drop size distribution, using a network of 5 disdrometers located 125m apart, and returning a drop size distribution every minute. From the spectra, we derived an estimate of the attenuation, including an estimate of the uncertainty.

How to cite: Husnoo, N. and Jones, D.: The impact of drop size distribution variability and rainfall attenuation on autonomous vehicle sensors, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14407, https://doi.org/10.5194/egusphere-egu23-14407, 2023.

Weather radar provides rainfall estimates at high resolution in both space and time, which is useful for many hydrological applications. Despite this, the radar rainfall estimation process introduces many sources of error, impacting the reliability of results obtained from the radar rainfall estimates. Key error sources include signal attenuation, radar calibration issues, ground clutter contamination, variability in the drop-size distribution and variation in the vertical profile of reflectivity. To gain an improved understanding of potential limitations, and the corresponding uncertainty of rainfall rates, the impact of these errors has been systematically investigated, developing a radar error model by inverting the rainfall estimation process.

To this end, an ensemble of realistic rainfall events is simulated, and working backwards in a stochastic manner gives an ensemble of weather radar images, corresponding to each rainfall event, at each time step. The radar error model includes random noise effects, drop-size distribution errors, sampling estimation variance and importantly, attenuation effects. To allow for direct comparisons, standard radar processing methods are applied to each radar image, to obtain corrected ‘best guess’ rainfall estimates which would be obtained from each weather radar ensemble member in real world applications. The difference between the simulated and corrected rainfall for each ensemble member is then treated as the uncertainty corresponding to the radar rainfall estimation process.

A simple measure is introduced, to help understand how often errors result in a rainfall signal completely irretrievable, referred to as ‘rainfall shadow’. Areas of rainfall that are ‘shadowed’ are defined as pixels where the simulated ‘true’ rainfall rate is significant, but the ensemble member has less than 10% of the original signal. This is equivalent to considering where a significant rainfall rate has been completely lost, and would therefore be irretrievable using standard correction methods, to quantify the frequency of occurrence in real-world radar rainfall applications. The impact of location of rainfall within images is considered, by introducing the second moment of area for radar images, in order to quantify the proximity of intense rainfall to the radar transmitter.

Results show relationships between rainfall shadows and high bias and uncertainty in rainfall estimates, related to the amount of rainfall (i.e. proportion and rates) in images. More central rainfall also results in higher errors and higher variability. The minimum likelihood of occurrence of rainfall shadows showed that 50% of event images have at least 3% of significant rainfall shadowed. In addition, 25% of images had a shadowed area of over 45km2, with the minimum largest shadow in one area for 5% of images exceeding an area of 50km2. This gap would result in an underestimation of the impact of potential floods, showing that weather radar has potential for important information to be lost. A model framework for representing this uncertainty in the radar rainfall estimation process provides methodology for assessing the impacts of radar rainfall errors on hydrological applications.

How to cite: Green, A., Kilsby, C., and Bardossy, A.: Quantifying the uncertainty corresponding to the radar rainfall estimation process:  an inverse model for radar attenuation error, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14569, https://doi.org/10.5194/egusphere-egu23-14569, 2023.

EGU23-14766 | PICO | HS7.1

Multiscale Characteristics of West African Summer Monsoon Precipitation Derived from UCadMet Network Observations 

Belen Rodríguez de Fonseca, Luis Durán Montejano, Alvaro González Cervera, Auguste Gires, Cheikh Modou Noreyni Fall, Abdou Lahat Dieng, Amadou Thierno Gaye, and Elsa Mohino

Since 2012 a joint Université Cheikh Anta Diop de Dakar and Universidad Complutense de Madrid meteorological observation network (UCadMet) has been in place in the city of Dakar (Senegal). During the last years, the observation and data storage systems have been considerably improved. Last summer of 2022, a laser disdrometer was installed providing  detailed information on the size and speed of precipitation with a time resolution of one minute. Observations from several tipping bucket rain gauges are available also at the same site. Summer 2022 has been anomalously rainy in West Africa, with large precipitation events during the African monsoon season, which seems to be enhanced by a La Niña situation in the Pacific. These events have proven to be particularly suitable for evaluating the performance of the installed observing systems and for drawing some conclusions about the characteristics of monsoon precipitation in this region not only at different time scales, but also across scales (from 1 min to season). Commonly used rain rate together with drop size distribution are used to access information on rainfall microphysics. This analysis allows the design of future lines of action considering climate change, for which large precipitation events are expected to become more frequent.

How to cite: Rodríguez de Fonseca, B., Durán Montejano, L., González Cervera, A., Gires, A., Fall, C. M. N., Dieng, A. L., Gaye, A. T., and Mohino, E.: Multiscale Characteristics of West African Summer Monsoon Precipitation Derived from UCadMet Network Observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14766, https://doi.org/10.5194/egusphere-egu23-14766, 2023.

EGU23-15902 | ECS | PICO | HS7.1

Correction of hourly radar precipitation data based on rain-gauges values: what is the most efficient method for hydrologic modeling purposes? 

Andrea Citrini, Georgia Lazoglou, Adriana Bruggeman, George Zittis, Giovanni Pietro Beretta, and Corrado Camera

The effectiveness of a hydrologic model is largely driven by the availability and nature of the input data. Among these, many studies proved precipitation to be the most important because it regulates the amount of water entering the system. Spatially continuous precipitation data can be obtained from radar technology. However, radar precipitation values are an indirect measure, and it is widely believed that their use in hydrologic modelling is complicated due to the presence of bias. The use of radar data is increasingly problematic in mountain regions where elevation plays a key role on precipitation, creating significant variations in few kilometers. Also, mountains can lead to a shadow effect of the radar beam.

The research objective is to integrate precipitation data derived from the radar into a partially distributed hydrologic model, running in an area with complex morphology. The study area is a portion of Upper Valtellina valley (about 2300 km2), located within the Alpine belt on the border between Italy and Switzerland, and characterized by an elevation range between 350 and 3400 m a.s.l. The hourly series of 22 rain-gauges (18 Italian and 4 Swiss stations) and hourly precipitation from a radar dataset (1km x 1km resolution, from MeteoSWISS) from 2010 to 2020 are used. The mean bias between the series extracted in the radar cells at the station locations and the series measured by rain-gauge is around -28%, indicating a general underestimation of the radar data. The targets of the correction techniques are the precipitation series at the centroids of the sub-basins defined by the hydrologic model.

For the correction, two approaches are tested: (i) the radar precipitation is corrected in every centroid of the hydrologic model subbasins (point-based correction); (ii) the radar precipitation is adjusted by spatializing the radar-station error (interpolation-based correction). The first approach is based on finding the statistical relations between the radar-station series of the three closet stations to the target centroid and applying the statistical correction (Copula or Cumulative Distribution Function (CDF) matching bias correction) to the precipitation series in the centroid cell. The result of the correction is a combination of the statistical relationships weighted according to a Triangular Irregular Network. The second technique focusses instead on the interpolation of the error (residuals) calculated as the difference between radar and rain-gauge values, which is subsequently added to the original radar raster. Two different interpolation techniques are used: Thin Plate Splines and Inverse Distance Weighting. All methods are evaluated through performance indices (KGE and RMSE) at the station locations by Leave One Out cross validation.

Point-based applications are cost-effective and require less computational effort than spatial interpolations. Preliminary results show that the point-based corrections through Copula and CDF have similar performances. In detail, the KGE increases from 0.18 to 0.52 and 0.55 for Copula and CDF, respectively. RMSE decreases from 0.78 mm to 0.53 mm (Copula) and 0.62 mm (CDF). Interpolation-based corrections are still ongoing, therefore there are no definite results regarding the comparative effectiveness of one type of correction over the other.

How to cite: Citrini, A., Lazoglou, G., Bruggeman, A., Zittis, G., Beretta, G. P., and Camera, C.: Correction of hourly radar precipitation data based on rain-gauges values: what is the most efficient method for hydrologic modeling purposes?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15902, https://doi.org/10.5194/egusphere-egu23-15902, 2023.

EGU23-15924 | ECS | PICO | HS7.1

Information-based approach for quantifying uncertainty in precipitation estimates from commercial microwave links 

Anna Špačková, Martin Fencl, and Vojtěch Bareš

Opportunistic sensors have great potential for rainfall monitoring, as the density of their networks can outperform standard rainfall monitoring networks. The commercial microwave link (CML) network enables indirect monitoring of path-averaged rainfall intensity. It is retrieved from signal attenuation caused by raindrops, which can be related to rainfall intensity by a simple power law. Quantitative precipitation estimates from CMLs are, however, affected by uncertainty, which is still challenging to estimate.

This study proposes, for the first time, to use information theory methods to quantify uncertainty in CML QPEs. This method enables measuring the firmness of relationships between different variables using discrete probability distributions and also estimates the uncertainty. The advantage resides also in the fact that it allows any type of data to be used. This approach was recently applied by Neuper and Ehret (2019) to evaluate quantitative precipitation estimates with weather radar.

Data from non-winter periods of 2014 – 2016 are used at a temporal resolution of 15 min. The target (reference) data are the rain gauge adjusted radar observation. The CML data (signal attenuation and its processing) from the Prague network and its hardware characteristics are used as predictors. Additionally, other predictors, e.g., temperature and synoptic types, are used as further predictors. First, the information content of individual predictors of the target rain gauge adjusted radar data is measured. Specifically, we tested how different combinations of predictors reduce uncertainty. Second, the effect of the sample size on uncertainty is investigated. Different sizes of random samples are selected from the dataset and their information content for the target is quantified.

Depending on the choice of the predictor(s), their abilities to estimate the target variable can be compared. Their predictive uncertainties are different, which results in a ranking of suitability of available predictors and their combinations.

 

References
Neuper, M. and Ehret, U. (2019) Quantitative precipitation estimation with weather radar using a data- and information-based approach, Hydrol. Earth Syst. Sci., 23, 3711–3733, https://doi.org/10.5194/hess-23-3711-2019.

 

This study is supported by the Student Grant Competition grant of Czech Technical University in Prague no. SGS22/045/OHK1/1T/11.

How to cite: Špačková, A., Fencl, M., and Bareš, V.: Information-based approach for quantifying uncertainty in precipitation estimates from commercial microwave links, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15924, https://doi.org/10.5194/egusphere-egu23-15924, 2023.

The polar mesospheric clouds (PMCs) obtained from Aeronomy of Ice in the Mesosphere (AIM)/Cloud Imaging and Particle Size (CIPS) and Himawari-8/Advanced Himawari Imager (AHI) observations are analyzed for the multi-year climatology and interannual variations. The PMCs dependence on mesospheric temperature and water vapor (H2O) are further investigated with data from Microwave Limb Sounder (MLS). Our analysis shows that PMCs onset date and occurrence rate are strongly dependent on the atmospheric environment, i.e. underlying seasonal behavior of temperature and water vapor. Upper-mesospheric dehydration by PMCs is evident in MLS water vapor observations, The spatial patterns of the depleted water vapor resemble the PMCs distribution over the Arctic and Antarctic region during the days after summer solstice. Year-to-year variabilities of the PMCs occurrence rate and onset date are highly correlated with the mesospheric temperature and H2O variations, particularly in the southern hemisphere (SH). The global increase of mesospheric H2O during the last decade may explain the increased PMCs occurrence in the northern hemisphere (NH). Although mesospheric temperature and H2O exhibits a strong 11-year variation, little solar cycle signature is found in the PMCs occurrence during 2005-2021.

How to cite: Lee, J. and Wu, D.: The Sensitivity of Polar Mesospheric Clouds to Mesospheric Temperature and Water Vapor, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-907, https://doi.org/10.5194/egusphere-egu23-907, 2023.

EGU23-1177 | ECS | Orals | ST3.5

Simultaneous observations of mesospheric bore and front over the Himalaya 

Subarna Mondal, Amitava Guharay, Sumanta Sarkhel, M. V. Sunil Krishna, and Martin G. Mlynczak

Interesting observational evidence of interaction between a mesospheric bore and a mesospheric front is found in O(1S) 557.7 nm airglow images over the western Himalayan region on 25 April 2022. The event is unique as it is the first report of a mesospheric bore interacting with a typical mesospheric front. The vertical profiles of temperature and Brunt Vaisala frequency indicate presence of a strong mesospheric inversion layer (MIL) which acts as a stable thermal duct for the propagation of the mesospheric bore. Analysis suggests that local chemical heating plays a significant role in sustaining a strong MIL/thermal duct. The bore front shows an anti-clockwise rotation, which is attributed to the differential phase speed of different regions of the bore due to variations in duct depth. The bore propagation above is observed to push the underlying OH layer downward, resulting in a maximum horizontal slope of the peak height of the OH volume emission rate (VER) on 25 April 2022. The results highlight the bore-front interaction, mesospheric background condition for bore propagation, and its effect on the altitudinal shift of adjacent airglow emission layers.

How to cite: Mondal, S., Guharay, A., Sarkhel, S., Krishna, M. V. S., and Mlynczak, M. G.: Simultaneous observations of mesospheric bore and front over the Himalaya, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1177, https://doi.org/10.5194/egusphere-egu23-1177, 2023.

Tektites are a naturally occurring form of cosmic impact ejecta, produced in ~ 2 or 3% of impact events from melted and mixed silicate sediments that are launched into space where they devolatilize and quench to solid glass.  Australasian tektites (AAT) make up the largest and most recent of the known tektite strewnfields, covering ~1/4 of Earth’s surface with 30 to 60 billion tons of melt glass.  In southeast Asia, the Indochinite sub-family of these glassy objects appear mainly as fractured and sometimes contorted fragments of formerly hollow spheroid predecessors.  Surface textures, bulk and detailed morphometrics of Indochinite fragment-form tektites record a tortured history that is not consistent with mere hypersonic atmospheric reentry into a standard atmospheric column.  The tektites show rapid bulk reheating and surface effects consistent with high-voltage arcing disruption.  The overall region where these fragment-form tektites fell has a surface that was laterized within hours of their arrival, pulsed with heat and moisture to the point of degrading the rocks and soil the tektites lie within.  Clear ablation signatures on symmetric ablated spheroid AAT of Australia and the Central Indian Ocean basin indicate their source as the N. American Great Lakes region.  The Marine Isotope Stage MIS20 epoch (deep ice age) of the event and Michigan Basin geology suggest several thousand cubic km of disrupted Laurentide Ice Sheet may have been injected across the exosphere via oblique ricochet impact, lingering as degenerate byproducts for a day or more.  High-potential E-field and regional disruption of the atmospheric column from exosphere to surface over southeast Asia is indicated.

How to cite: Harris, T.: Impact ejecta glass records atmospheric columnar disruption and strong E-field, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4027, https://doi.org/10.5194/egusphere-egu23-4027, 2023.

EGU23-4415 | ECS | Orals | ST3.5

On the Correlation between the sodium in the MLT and meteor radiant distribution 

Yanlin Li, Tai-Yin Huang, Julio Urbina, Fabio Vargas, and Wuhu Feng

The sodium layer in the mesosphere and lower thermosphere (MLT) region is originated from meteoroid mass deposits produced by its ablation. Understanding the correlation between the meteoroid material input and the concentration of the sodium layer is essential for many investigations that use sodium as a tracer to study the dynamics in the MLT. A new numerical sodium chemistry model has been developed to study such correlation, and the results are cross-compared to the meteoroid material input inferred from the recently revealed sporadic meteor radiant distribution derived from the data gathered by the Arecibo Observatory. The sodium chemistry model is computationally efficient, runs in high-time resolution, and the sodium-bearing species are equally treated in the continuity equation devoid of making any steady-state approximation. This work will also present the seasonal and latitudinal distribution of meteoroid injection rates derived from the aforementioned sporadic meteor radiant distribution.Our simulation results agreed with the general feature of the measurements obtained from the Colorado State University Lidar (CSU) and the Andes Lidar Observatory (ALO) but with variations three times smaller.

How to cite: Li, Y., Huang, T.-Y., Urbina, J., Vargas, F., and Feng, W.: On the Correlation between the sodium in the MLT and meteor radiant distribution, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4415, https://doi.org/10.5194/egusphere-egu23-4415, 2023.

EGU23-4518 | Posters on site | ST3.5

Understanding the Coupled OH Meinel and O2 Atmospheric Band Nightglow Emissions 

Konstantinos S. Kalogerakis

Nightglow emission signatures observed from space- and ground-based instruments are commonly used as proxies for atmospheric composition, especially for the altitude region around 100 km that cannot be easily studied in situ. Monitoring the intensity and temporal evolution of such proxies by remote sensing is often the method of choice to study a plethora of phenomena in this region of the atmosphere. Thus, the quantitative details relevant to the production and deactivation of excited atomic and molecular precursors responsible for prominent nightglow emissions are required to study atmospheric composition, radiative and energy balance, wave propagation and dissipation, as well as transport dynamics. Significant gaps and uncertainties exist in the understanding of the above processes and, as our recent studies on nightglow emissions revealed, substantial revisions of the relevant atmospheric models are warranted.

We will present a progress report on our efforts to advance the understanding of key mesospheric nightglow emissions by investigating the recently established coupling between the OH Meinel and the O2 Atmospheric band emissions, mediated by collisions of O atoms with vibrationally excited OH.

This work is supported by the U.S. National Science Foundation (NSF) under Grants AGS-2009960 and AGS-2113888.

How to cite: Kalogerakis, K. S.: Understanding the Coupled OH Meinel and O2 Atmospheric Band Nightglow Emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4518, https://doi.org/10.5194/egusphere-egu23-4518, 2023.

EGU23-5246 | Posters on site | ST3.5

Scientific Highlights from ROMIC 

Franz-Josef Lübken

The German Federal Ministry of Education and Research (Bundesministerium für Bildung und Forschung, BMBF) has launched a research initiative in 2013/2014 called ROMIC (Role of the Middle Atmosphere in Climate). The second phase of this project extends until 2024. The aim of ROMIC is to improve our understanding of long term variations in the stratosphere, mesosphere, and lower thermosphere and to investigate their potential role for
climate changes in the troposphere. This includes to study coupling mechanisms between various layers and the relative importance of anthropogenic and natural forcing, e.\ g., by the Sun. Scientists at a total of 13 research institutes in Germany are involved and cover a large range of experimental and theoretical topics relevant for ROMIC. Most projects are linked to international activities and cooperations. Some scientific highlightsfrom the research projects within ROMIC will be presented.

How to cite: Lübken, F.-J.: Scientific Highlights from ROMIC, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5246, https://doi.org/10.5194/egusphere-egu23-5246, 2023.

EGU23-5587 | Orals | ST3.5

Empirical modelling of SSUSI-derived auroral ionization rates 

Stefan Bender, Patrick Espy, and Larry Paxton

Solar, auroral, and radiation belt electrons enter the atmosphere at polar regions leading to ionization and affecting its chemistry. Climate models with interactive chemistry in the upper atmosphere, such as WACCM-X or EDITh, usually parametrize this ionization and calculate the related changes in chemistry based on satellite particle measurements. Widely used particle data are derived from the POES and GOES satellite measurements which provide electron and proton spectra. These satellites provide in-situ measurements of the particle populations at the satellite altitude, but require interpolation and modelling to infer the actual input into the upper atmosphere.

Here we use the electron energy and flux data products from the Special Sensor Ultraviolet Spectrographic Imager (SSUSI) instruments on board the Defense Meteorological Satellite Program (DMSP) satellites. This formation of currently three operating satellites observes both auroral zones in the far UV from (115--180 nm) with a 3000 km wide swath and 10 x 10 km (nadir) pixel resolution during each orbit. From the N2 LBH emissions, the precipitating electron energies and fluxes are inferred in the range from 2 keV to 20 keV. We use these observed electron energies and fluxes to calculate auroral ionization rates in the lower thermosphere (≈ 90–150 km), which have been validated previously against ground-based electron density measurements
from EISCAT. We present an empirical model of these ionization rates derived for the entire satellite operating time and sorted according to magnetic local time and geomagnetic latitude. The model is based on geomagnetic and solar flux indices, and the coefficients indicate where certain drivers have the largest influence. The model will be particularly targeted for use in climate models that include the upper atmosphere, such as the aforementioned WACCM-X or EDITh models, and we present an initial comparison to current implementations for ionization rates used in high-top whole-atmosphere models. Further applications include the derived conductances in the auroral region, as well as modelling and forecasting E-region disturbances related to Space Weather.

How to cite: Bender, S., Espy, P., and Paxton, L.: Empirical modelling of SSUSI-derived auroral ionization rates, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5587, https://doi.org/10.5194/egusphere-egu23-5587, 2023.

EGU23-7129 | Orals | ST3.5

The role of stratified turbulence in the cold summer mesopause region 

Victor Avsarkisov and Federico Conte

The primary physical mechanism behind the formation of the summer mesopause at middle and high latitudes is related to atmospheric gravity waves. An insight into this extreme thermal phenomenon can be gained from investigating the mesoscale energy spectrum. In this work, we decompose the frequency spectrum into divergent and rotational parts and find that their energy contributions are equipartitioned at high frequencies. This mesoscale energy equipartition indicates the effect of stratified turbulence. Analysis of the power spectra of observed and simulated horizontal winds at middle latitudes reveals the role of stratified turbulence in the formation of the summer mesopause region.

How to cite: Avsarkisov, V. and Conte, F.: The role of stratified turbulence in the cold summer mesopause region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7129, https://doi.org/10.5194/egusphere-egu23-7129, 2023.

Atmospheric gravity waves transport energy and momentum through the atmosphere and can travel large horizontal and vertical distances from the troposphere to the mesosphere and higher. They contribute to atmospheric dynamics and among others drive the meridional pole-to-pole circulation in the mesosphere. Thus, knowing about gravity waves, their spatio-temporal characteristics, their interaction with other waves and the atmospheric background is attracting more and more attention in order to further improve climate and even meteorological models.

In the upper mesosphere / lower thermosphere (UMLT) region around an altitude of 80km to 100km, OH airglow can be utilized for passive remote sensing and continuous nightly observations of atmospheric dynamics, especially of gravity waves. The OH airglow layer is a chemiluminescent layer with a strong emission in the short wave infrared spectral range (at about 1500nm) and is located at an altitude of about 86-87km with a layer halfwidth of about 4km. The OH airglow intensity is modulated by traversing atmospheric gravity waves which lead amongst others to a vertical transport of atomic oxygen. Observing the OH airglow with short-wave infrared imagers allows characterizing gravity waves. From these observations the horizontal wave parameters (horizontal wavelength, horizontal direction of propagation, etc.) can be derived.

In this study we present measurements of two ground-based FAIM (Fast Airglow IMager) systems, which are cameras sensitive in the short-wave infrared region observing the OH airglow layer with a high temporal resolution. The cameras are located at Oberpfaffenhofen, Germany and Otlica, Slovenia, about 300km apart from each other and are pointing to the same volume at about 87km located in the Alpine Region above Northern Italy. We developed a novel tomographic algorithm to allow for a three-dimensional reconstruction of the airglow layer by combining images from the two viewing angles. In order to solve the highly underdetermined equation system, prior knowledge of the OH airglow layer vertical profile is needed e.g. from multi-year observations of SABER on the TIMED satellite on a statistical basis, or Gaussian and Chapman basis functions. This allows us, among others, to derive the vertical wavelength of the waves, their three-dimensional propagation direction, and their three-dimensional structure. From that knowledge, further wave parameters but also the horizontal wind along the wave propagation can be estimated via the wave’s dispersion relation.

We will explain the tomographic reconstruction method, its capabilities and limits and will present a detailed case study showing a 3D-reconstructed gravity wave and the derivation of its parameters.

This work received funding from the Bavarian State Ministry of the Environment and Consumer Protection.

How to cite: Hannawald, P., Noll, S., Wüst, S., and Bittner, M.: 3D reconstruction of atmospheric gravity waves and derivation of vertical wave parameters with tomography applied to data from two ground-based cameras observing OH airglow, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7554, https://doi.org/10.5194/egusphere-egu23-7554, 2023.

EGU23-8477 | Posters on site | ST3.5

X-shooter-based climatologies of intensity, solar cycle effect, and residual variability for 298 OH lines 

Stefan Noll, Carsten Schmidt, Wolfgang Kausch, Michael Bittner, and Stefan Kimeswenger

The line emission from the various roto-vibrational bands of the OH radical is an important tracer of the chemistry and dynamics in the Earth's nocturnal mesopause region between about 80 and 100 km. As most studies have focused either on a few bright lines or integrated emission from relatively wide wavelength windows, there is still a lack of knowledge with respect to the variability of faint lines from high rotational levels as well as the change of the variability patterns depending on the line parameters, which influence the effective emission height. Thanks to a large data set of about 90,000 near-infrared X-shooter spectra taken at Cerro Paranal in Chile within a time interval of 10 years, we have been able to derive line-specific climatologies of intensity, solar cycle effect, and residual variability for local time and day of year based on a set of 298 OH lines. Our analysis of the derived climatologies involves different decomposition techniques, the study of the variance depending on the time scale of the perturbation, and the calculation of correlations for the line dependence of different properties. The considered effective line emission heights originate from the investigation of the propagation of a strong quasi-2-day wave in 2017 using the X-shooter and space-based SABER data. Our results for the entire X-shooter data set reveal the importance of the mixing of thermalised and non-thermalised rotational populations for the amplitude of a perturbation as well as a shift of the climatological variability patterns with local time depending on the emission height. The latter implies a strong influence of the migrating diurnal tide and causes significant line-dependent differences in the effective solar cycle effect, which mainly depends on the solar forcing in the austral winter.

How to cite: Noll, S., Schmidt, C., Kausch, W., Bittner, M., and Kimeswenger, S.: X-shooter-based climatologies of intensity, solar cycle effect, and residual variability for 298 OH lines, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8477, https://doi.org/10.5194/egusphere-egu23-8477, 2023.

EGU23-8579 | ECS | Posters on site | ST3.5

Long-term study of the summer wind variability in the mesosphere and lower thermosphere over nearly two decades at middle and high latitudes 

Juliana Jaen, Toralf Renkwitz, Jorge Chau, Huixin Liu, Christoph Jacobi, Masaki Tsutsumi, and Njål Gulbrandsen

Winds at the mesosphere and lower thermosphere have been measured by partial reflection radars and specular meteor radars for almost two decades (2004-2022) over Germany and Norway (i.e., middle and high latitudes, respectively). Continuous wind measurements during the mentioned period are important to understand their long-term behavior. The zonal mean wind climatology displays an eastward wind during the winter months and a westward summer jet below ~85km at middle latitudes (~90km at high latitudes). Above the mentioned height, an eastward wind jet is observed. In the meridional wind component, the southward summer wind displays amplitudes between 4 and 5 times less intense than the westward jet. We studied the intensity of the summer wind components, the long-term variability and the possible connection to external forcing (i.e. El Niño-Southern Oscillation, and quasi-biennial oscillation, solar activity and geomagnetic activity). Analyzing the summer winds for low and high geomagnetic activity classified with the Ap index, there is a significant difference between both cases suggesting disturbances in the wind due to high geomagnetic activity. The long-term study shows significant trends at middle latitudes in the monthly summer values of the westward summer jet. As a consequence of the increase in the westward wind, a decrease in the southward component is observed at the same latitudes. While at high latitudes the eastward jet shows a decreasing velocity during July.

How to cite: Jaen, J., Renkwitz, T., Chau, J., Liu, H., Jacobi, C., Tsutsumi, M., and Gulbrandsen, N.: Long-term study of the summer wind variability in the mesosphere and lower thermosphere over nearly two decades at middle and high latitudes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8579, https://doi.org/10.5194/egusphere-egu23-8579, 2023.

EGU23-11006 | ECS | Orals | ST3.5 | Highlight

One year of MLT dynamics over central and northern Peru from SIMONe systems 

Federico Conte, Jorge Chau, Erdal Yiğit, José Suclupe, Karim Kuyeng, and Rodolfo Rodríguez

One year of Spread spectrum Interferometric Multistatic meteor radar Observing Network (SIMONe) measurements are analyzed and compared for the first time between two low-latitude locations in Peru: Jicamarca (12°S, 77°W) and Piura (5°S, 80°W). Investigation of the mean horizontal winds and tides reveals that mesosphere and lower thermosphere (MLT) planetary-scale dynamics are similar between these two locations, although differences can be seen in some tidal components, e.g., the diurnal tide. On the other hand, monthly median values of the 4-hour, 4-km momentum fluxes indicate that the mesoscale dynamics differ significantly between Jicamarca and Piura. These differences are particularly evident during the (southern hemisphere’s) summertime in the zonal component, where a strong acceleration of the background wind by westward-propagating gravity waves (GWs) is observed at all altitudes (80-100 km) only over Piura. The latter finding observationally confirms the previous studies based on model simulations indicating that the directions of the GW drag and the background wind coincide in the low-latitude MLT [Yiğit & Medvedev, 2017].

How to cite: Conte, F., Chau, J., Yiğit, E., Suclupe, J., Kuyeng, K., and Rodríguez, R.: One year of MLT dynamics over central and northern Peru from SIMONe systems, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11006, https://doi.org/10.5194/egusphere-egu23-11006, 2023.

EGU23-13908 | ECS | Orals | ST3.5 | Highlight

Energetic Particle Precipitation reflected in the Global Secondary Ozone Distribution 

Jia Jia, Lisa E. Murberg, Tiril Løvset, Yvan J. Orsolini, Patrick J. Espy, Jude Salinas, Jae N. Lee, Dong Wu, and Jiarong Zhang

The secondary ozone layer is a global peak in ozone abundance in the upper mesosphere-lower thermosphere (UMLT) around 90-95 km. The effect of energetic particle precipitation (EPP) from geomagnetic processes on this UMLT ozone has not been well studied. In this research we investigated how the secondary ozone response to EPP from the Microwave Limb Sounder (MLS) and the Sounding of the Atmosphere using Broadband Emission Radiometry (SABER) instrument on the Aura and TIMED satellites, respectively. In addition, the Whole Atmosphere Community Climate Model with thermosphere and ionosphere extension and specified dynamics (SD-WACCM-X) was used to characterize the residual circulation during EPP events. By comparing ozone and circulation changes under High- and low-Ap conditions, we report regions of secondary ozone enhancement or deficit across low, mid and high latitudes as a result of circulation and transport changes induced by EPP.

How to cite: Jia, J., Murberg, L. E., Løvset, T., Orsolini, Y. J., Espy, P. J., Salinas, J., Lee, J. N., Wu, D., and Zhang, J.: Energetic Particle Precipitation reflected in the Global Secondary Ozone Distribution, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13908, https://doi.org/10.5194/egusphere-egu23-13908, 2023.

EGU23-13994 | Posters on site | ST3.5

The impact of extreme solar events on the atmosphere 

Thomas Reddmann, Monali Borthakur, Miriam Sinnhuber, Ilya Usoskin, Jan Maik Wissing, and Jan Maik Wissing

Besides the well-known 11 year solar cycle, the Sun occasionally produces strong eruptions on the Sun‘s surface and in the corona. They can first be seen as flare events in electromagnetic spectrum down to X ray wavelengths. Within these strong eruptions, particles in the solar plasma, mainly protons, are accelerated to high energies that hit the Earth within hours after the event. In addition, plasma clouds can be accelerated and ejected into the interplanetary space and, provided they are directed to the Earth, can cause severe geomagnetic disturbances. This results in a further energetic particle precipitation event a few days after the primary solar eruption. The strength of these events spans orders of magnitude, with the strongest having dramatic impact on the ionosphere and the middle atmosphere affecting even human activities. Here we study the chemical impact and dynamical of solar events on the middle atmosphere which are on the very extreme side but still within the range of a one per millennia event.

We first derive a reference example of an extreme solar event from historical records of solar proton events and from analyzed distributions of energy spectra for geomagnetic storms. We then take ionization rates calculated from strong observed events and scale them to represent the extreme events. Finally, we combine the solar proton event with the geomagnetic storm as both events typically impact different parts of the atmosphere. The ionization rates for the extreme event are then used in simulations in the KASIMA and EMAC model which both include energetic particle induced chemistry.In order to represent different dynamical situations in the middle atmosphere which are important for the vertical coupling between the mesosphere-lower thermosphere (MLT) region and the stratosphere we select specific periods of the ERA-Interim dataset with a special focus on sudden stratospheric warmings (SSW) and apply the event for those situations. The simplified production efficiency of NOx and HOx in the models is further compared to an ion chemistry model where the extreme ionization rates are applied. The case of a SSW which shows an elevated stratosphere synchronized with the extreme event is studied in detail as a kind of worst case scenario.

How to cite: Reddmann, T., Borthakur, M., Sinnhuber, M., Usoskin, I., Wissing, J. M., and Wissing, J. M.: The impact of extreme solar events on the atmosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13994, https://doi.org/10.5194/egusphere-egu23-13994, 2023.

Based on the hourly output from the 2000–2014 simulations of the National Center for Atmospheric Research’s vertically extended version of the Whole Atmosphere Community Climate Model in specified dynamics configuration, we examine the roles of planetary waves, gravity waves and atmospheric tides in driving the mean meridional circulation in the lower thermosphere and its response to the sudden stratospheric warming phenomenon with an elevated stratopause in the northern hemisphere. Sandwiched between the two summer-to-winter overturning circulations in the mesosphere and the upper thermosphere, the climatological lower thermosphere mean meridional circulation is a narrow gyre that is characterized by upwelling in the middle winter latitudes, equatorward flow near 120 km, and downwelling in the middle and high summer latitudes. Following the onset of the sudden stratospheric warmings, this gyre reverses its climatological direction, resulting in a “chimney-like” feature of un-interrupted polar descent from the altitude of 150 km down to the upper mesosphere. This reversal is driven by the westward-propagating planetary waves, which exert a brief but significant westward forcing between 70 and 125 km, exceeding gravity wave and tidal forcings in that altitude range. The attendant polar descent potentially leads to a short-lived enhanced transport of nitric oxide into the mesosphere (with excess in the order of 1. parts per million), while carbon dioxide is decreased.

How to cite: Orsolini, Y., Zhang, J., and Limpasuvan, V.: Abrupt Change in the Lower Thermospheric Mean Meridional Circulation during Sudden Stratospheric Warmings and its Impact on Trace Species, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14077, https://doi.org/10.5194/egusphere-egu23-14077, 2023.

EGU23-14102 | Posters on site | ST3.5 | Highlight

Dynamics and variability of the MLT represented by UA-ICON 

Claudia Stolle, Markus Kunze, Tarique Siddiqui, Chistoph Zülicke, Mozhgan Amiramjadi, Yosuke Yamazaki, Gerd Baumgarten, Sebastian Borchert, and Hauke Schmidt

The variability of the upper atmosphere is largely influenced by dynamical forcing from the lower and middle atmosphere. The Mesosphere and Lower Thermosphere (MLT) is the transition region between the middle atmosphere and the upper atmosphere, and it determines dynamical forcing to the upper atmosphere from below. It is thus of high importance to know, describe, and understand the dynamical processes within the MLT to quantify dynamics. Therein, General Circulation Models (GCMs) have been a significant tool to explain MLT processes.

However, developing the right parameterizations that allow to accurately model near-to-realistic states of the MLT by GCMs is challenging, which is reflected in a large diversity of results from different models in comparison to observations, e.g., of winds and temperatures at the MLT.

In recent years, the community model ICON (Icosahedral Nonhydrostatic Weather and Climate Model) has been expanded into altitudes up to 150 km, named the UA (Upper Atmosphere) branch. UA-ICON is increasingly being applied to model and to understand MLT processes and how they are controlled by the lower and middle atmosphere.

We present newly developed capabilities of UA-ICON. Examples are mesospheric cooling during stratospheric warming events, low summer mesopause temperatures through appropriate specification of gravity wave parameterizations and runs of high spatial resolution. Results are discussed in comparison with observations and with predictions by other GCMs.

How to cite: Stolle, C., Kunze, M., Siddiqui, T., Zülicke, C., Amiramjadi, M., Yamazaki, Y., Baumgarten, G., Borchert, S., and Schmidt, H.: Dynamics and variability of the MLT represented by UA-ICON, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14102, https://doi.org/10.5194/egusphere-egu23-14102, 2023.

EGU23-16759 | ECS | Posters virtual | ST3.5

Ionospheric Hole in the MLT Regions after Submarine Volcanic Eruptions 

Sovit Khadka, Cesar Valladares, and Andrew Gerrard

A gigantic submarine volcano erupted near Tonga Island on 15 January 2022 generating a tsunami and related atmospheric and oceanic waves across the globe. This violent volcano triggered extreme disturbances just above the volcanic center that reached near Earth’s stratosphere. This geophysical event generated acoustic-gravity waves to propagate upward and induce significant global perturbations and holes in the mesosphere and lower thermosphere (MLT) regions. Here, we study the MLT region’s response to the Tonga-induced perturbations using ground-based Global Positioning System (GPS)-total electron content (TEC) data from GPS receivers spread in the South American continent. The possible propagation mechanism of the Tonga-related ionospheric holes and perturbations mediated by neutral wind-driven dynamo fields, vertical drifts, and the contribution of geomagnetic conditions will also be discussed. 

How to cite: Khadka, S., Valladares, C., and Gerrard, A.: Ionospheric Hole in the MLT Regions after Submarine Volcanic Eruptions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16759, https://doi.org/10.5194/egusphere-egu23-16759, 2023.

EGU23-16826 | Orals | ST3.5 | Highlight

First light from the MATS satellite 

Ole Martin Christensen, Jörg Gumbel, Linda Megner, Donal Murtagh, Björn Linder, Jonas Hedin, Nickolay Ivchenko, and Jacek Stegman

Global three-dimensional data are a key to understanding gravity waves in the mesosphere and lower thermosphere. MATS is a small Swedish satellite that aims at providing such fields using tomographic measurements of oxygen A-band airglow and noctilucent clouds. MATS was successfully launched from Mahia, New Zealand, on November 4, 2022. Data collection started in December 2022, and MATS is projected to have collected over 3 million images of the MLT region by April 2023.

This presentation will provide an overview over first results from the MATS data. This includes analysis of in-flight performance of the instruments, an overview of data availability, and some examples of possible usage of the data. We will discuss data quality as well as possible biases and uncertainties that need to be considered when using this new and unique dataset for mesospheric studies.

How to cite: Christensen, O. M., Gumbel, J., Megner, L., Murtagh, D., Linder, B., Hedin, J., Ivchenko, N., and Stegman, J.: First light from the MATS satellite, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16826, https://doi.org/10.5194/egusphere-egu23-16826, 2023.

EGU23-1904 | Orals | AS1.29

Stratospheric wave reflection modulates North American cold spells 

Gabriele Messori, Marlene Kretschmer, Simon H. Lee, and Vivien Wendt

The proposed drivers of wintertime North American cold spells are multifarious, including modes of climate variability, planetary wave patterns and regional-to-continental-scale weather regimes. The Arctic stratospheric polar vortex has also been reported as a potential remote driver. One proposed coupling mechanism between the stratospheric polar vortex and the troposphere is upward-propagating planetary waves being reflected downward by the polar vortex. Here, we present a physically interpretable regional stratospheric wave reflection detection metric and identify the tropospheric circulation anomalies over North America associated with prolonged periods of wave reflection. The stratospheric reflection events show a systematic evolution from a Pacific Trough regime – associated on average with positive temperature anomalies and a near-complete absence of anomalously cold temperatures in North America – to an Alaskan Ridge regime, which favours low temperatures over much of the continent. The most striking feature of the stratospheric reflection events is thus a systematic shift in the tropospheric circulation in North America, associated with a rapid, continental-scale decrease in temperatures. These emerge as continental-scale cold spells by the end of the reflection events. Stratospheric reflection events are thus highly relevant in a tropospheric predictability perspective.

How to cite: Messori, G., Kretschmer, M., H. Lee, S., and Wendt, V.: Stratospheric wave reflection modulates North American cold spells, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1904, https://doi.org/10.5194/egusphere-egu23-1904, 2023.

EGU23-1961 | ECS | Posters on site | AS1.29

Comparison Of Northern And Southern Hemispheric SSW Using Reanalysis Data 

Sunil Kumar Ramatheerthan, Jan Laštovička, and Michal Kozubek

Sudden Stratospheric Warming (SSW) is an extreme dynamical event observed in the middle atmosphere. During this event, there will be changes in circulation behaviour in the middle atmosphere followed by a sudden warming in the polar stratosphere. The warming scenario is preceded by the polar vortex disruption due to the non-linear interaction of extra-tropical planetary waves from the troposphere with the mean flow. SSW affects both the upper and lower atmosphere, irrespective of latitude. It is known that warming events are more frequent in the northern hemisphere than in the southern hemisphere. The study investigates the evolution of warming events in both the northern and southern hemispheres. We use the reanalysis data to compare the 2013 - 2014 northern hemisphere and 2002 southern hemisphere SSW. To understand the forcing and responses in both hemispheres, we conducted meteorological and statistical analyses of SSW using temperature, zonal wind, meridional wind, and geopotential height. The factors that modulate the intensity of warming events in both hemispheres have been discussed in detail.

How to cite: Ramatheerthan, S. K., Laštovička, J., and Kozubek, M.: Comparison Of Northern And Southern Hemispheric SSW Using Reanalysis Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1961, https://doi.org/10.5194/egusphere-egu23-1961, 2023.

EGU23-2601 | ECS | Posters on site | AS1.29

Unravelling climate impacts of atmospheric internal gravity waves. 

Petr Šácha

Unresolved processes in climate models present a major source of uncertainty in future climate projections.
In this talk we will show the first results and introduce a newly founded five year project, which aims to re-examine the climate impacts of atmospheric internal gravity waves (GWs) using GW resolving simulations and to translate this knowledge to the development of modified GW parameterizations in climate models. Within the project, we will employ state-of-the-science high-resolution atmospheric datasets and theoretical methods for GW detection and wave-mean flow interaction to revisit and advance our understanding of GW effects on atmospheric dynamics, composition and coupling across atmospheric layers.

GWs exist on a variety of scales, but typically a significant portion of the GW spectrum remains unresolved in global weather prediction or climate models and the GW impacts need to be parameterized. Our knowledge on GW impacts ranging from regionality of precipitation to the evolution of the ozone layer has been so-far based on their predominantly parameterized effects. Analyzing the resolved GW effects will improve our understanding on the forcing of selected atmospheric phenomena, but will also put additional constraints on the current GW parameterizations by showing to what extent their effects (and our current understanding) are artificial. This will help us to modify GW parameterization schemes with an ultimate goal of alleviating the uncertainty in future climate projections.

How to cite: Šácha, P.: Unravelling climate impacts of atmospheric internal gravity waves., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2601, https://doi.org/10.5194/egusphere-egu23-2601, 2023.

EGU23-2905 | Orals | AS1.29

Stationary Waves Weaken and Delay the Near-Surface Response to Stratospheric Ozone Depletion 

Chaim Garfinkel, Ed Gerber, Ian White, Seok-Woo Son, and Martin Jucker

An intermediate-complexity moist general circulation model is used to investigate the factors controlling the magnitude of the surface impact from Southern Hemisphere springtime ozone depletion. In contrast to previous idealized studies, a model with full radiation is used; furthermore, the model can be run with a varied representation of the surface, from a zonally uniform aquaplanet to a configuration with realistic stationary waves. The model captures the observed summertime positive Southern Annular Mode response to stratospheric ozone depletion. While synoptic waves dominate the long-term poleward jet shift, the initial response includes changes in planetary waves that simultaneously moderate the polar cap cooling (i.e., a negative feedback) and also constitute nearly one-half of the initial momentum flux response that shifts the jet poleward. The net effect is that stationary waves weaken the circulation response to ozone depletion in both the stratosphere and troposphere and also delay the response until summer rather than spring when ozone depletion peaks. It is also found that Antarctic surface cooling in response to ozone depletion helps to strengthen the poleward shift; however, shortwave surface effects of ozone are not critical. These surface temperature and stationary wave feedbacks are strong enough to overwhelm the previously recognized jet latitude/persistence feedback, potentially explaining why some recent comprehensive models do not exhibit a clear relationship between jet latitude/persistence and the magnitude of the response to ozone. The jet response is shown to be linear with respect to the magnitude of the imposed stratospheric perturbation, demonstrating the usefulness of interannual variability in ozone depletion for subseasonal forecasting.

 

Garfinkel, C. I., White, I., Gerber, E. P., Son, S., & Jucker, M. (2023). Stationary Waves Weaken and Delay the Near-Surface Response to Stratospheric Ozone Depletion, Journal of Climate36(2), 565-583. 

How to cite: Garfinkel, C., Gerber, E., White, I., Son, S.-W., and Jucker, M.: Stationary Waves Weaken and Delay the Near-Surface Response to Stratospheric Ozone Depletion, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2905, https://doi.org/10.5194/egusphere-egu23-2905, 2023.

In addition to the well-known warming at high latitudes, sudden stratospheric warmings (SSWs) produce cooling and reduced static stability in the tropical lower stratosphere.  Based on 40 years of ERA5 reanalysis data and MJO amplitude data compiled at the U.S. National Oceanic and Atmospheric Administration, if these events occur in early winter (prior to ~ mid-January), the reduced static stability is sufficient to produce a statistically significant, lagged strengthening of the MJO peaking about 25 days after the SSW central date. Late winter SSWs produce no detectable strengthening.  This may be due to the timing of the SSW in early winter when tropical lower stratospheric temperatures and static stabilities are approaching their climatological minima.  This produces lower static stabilities than can occur following a late winter SSW when lower stratospheric temperatures are already higher and rising.  Positive feedbacks from MJO convection-induced temperature anomalies, cloud-radiative effects, and increased tropospheric Rossby wave amplitudes acting to further increase tropical upwelling rates, may further enhance MJO amplitudes.

The lagged strengthening of the MJO following early winter SSWs is also found in at least one climate model simulation in the CMIP6 archive (MRI-ESM-2.0).  We have so far analyzed in detail three full ensemble members (453 model years) of the 4xCO2 forcing version, which has relatively low climatological static stabilities in the tropical lower stratosphere.  Because of the large number of model years analyzed, the lagged strengthening is statistically robust but is weaker and occurs at a shorter time lag of 10-15 days than is estimated from the available observations.  Using the large number of available early winter SSWs, it is found that those SSWs that produce the largest reductions in static stability in the tropical lower stratosphere (70 to 100 hPa) also produce the largest lagged strengthenings of the MJO.  This supports a top-down static stability mechanism for producing the strengthening. Analyses of data from other climate models in the CMIP6 archive are in progress.

Because early winter SSWs occur primarily under easterly quasi-biennial oscillation (QBO) conditions and late winter SSWs occur most often under westerly QBO conditions, these results have implications for the origin of the observed modulation of the MJO by the stratospheric QBO.  Extratropical wave forcing events (including minor as well as major warmings) are typically stronger in early winter under easterly QBO conditions, as was originally reported by Holton and Tan (1980).  These events will reduce tropical lower stratospheric static stability primarily in boreal winter when the QBO-MJO connection is observed.  While most MJO convection extends only to lower altitudes in the troposphere, it is mainly the strongest MJO events that are modulated by the QBO.  These latter events may extend to higher altitudes and be more affected by stability conditions in the lowermost stratosphere.

How to cite: Hood, L. L., Trencham, N. E., Hoopes, C. A., and Galarneau, Jr., T. J.: Lagged Strengthening of the Tropical Madden-Julian Oscillation Following Early Winter Sudden Stratospheric Warmings:  Observational Analyses and CMIP6 Model Comparisons, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2935, https://doi.org/10.5194/egusphere-egu23-2935, 2023.

The ability of satellite instruments to accurately observe long-term changes in atmospheric temperature depends on many factors including the absolute accuracy of the measurement, the stability of the calibration of the instrument, the stability of the satellite orbit, and the stability of the numerical algorithm that produces the temperature data. We present an example of algorithm instability recently discovered in the temperature dataset from the SABER instrument on the NASA TIMED satellite. The instability resulted in derived temperatures that were substantially colder than anticipated from mid-December 2019 to mid-2022. This algorithm-induced change in temperature over one to two years corresponded to the expected change over several decades from increasing anthropogenic CO2. This paper highlights the importance of algorithm stability in developing Geospace Data Records (GDRs) for Earth’s mesosphere and lower thermosphere. A corrected version (Version 2.08) of the temperatures from SABER is described.

How to cite: Mlynczak, M.: Algorithm Stability and the Long-Term Geospace Data Record from TIMED/SABER, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2993, https://doi.org/10.5194/egusphere-egu23-2993, 2023.

EGU23-3526 | Orals | AS1.29

Sensitivity of EQBO’s boreal winter teleconnections and surface impacts to SSWs 

Amy Butler, Dillon Elsbury, Yannick Peings, and Gudrun Magnusdottir

The Quasi-Biennial Oscillation (QBO) is known to influence the boreal winter surface circulation. The QBO affects extratropical surface circulation and temperature over Asia as well as the North Atlantic and Europe. While these surface responses are undoubtedly associated with the QBO, it is less clear whether they arise solely due to modulations in the frequency of extreme stratospheric events such as sudden stratospheric warmings (SSWs) or due to other pathways of the QBO. SSWs rapidly evolve in the stratosphere but can initiate persistent hemispheric scale surface temperature and circulation responses and hence, may account for some of the surface response to the QBO. While not reproduced in climate models, reanalysis tends to show that the frequency of SSW is higher during easterly QBO (EQBO), which could suggest the SSW do in fact account for some of the EQBO surface response. However, the QBO has multiple pathways to influence boreal winter surface conditions and hence may affect surface conditions independently of SSWs.
Here, we study the teleconnections and extratropical surface responses to EQBO by prescribing EQBO in an ensemble of branched simulations derived from a control simulation run without a QBO. The EQBO branched simulations, which run with repeating annual cycles of sea surface temperatures and sea ice, reproduce many of the observed EQBO teleconnections and surface impacts. After subsampling the branched runs for members
with and without SSWs, it becomes clear that SSWs are necessary to fully realize both the polar and subtropical routes of EQBO influence. However, there are regions such as east Asia where the surface circulation is able to be modulated by the EQBO even in the absence of SSWs.

How to cite: Butler, A., Elsbury, D., Peings, Y., and Magnusdottir, G.: Sensitivity of EQBO’s boreal winter teleconnections and surface impacts to SSWs, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3526, https://doi.org/10.5194/egusphere-egu23-3526, 2023.

EGU23-3772 | ECS | Posters on site | AS1.29

Interpretable Deep Learning for the Identification of Sudden Stratospheric Warming Events 

Yi-Jhen Zeng and Yu-Chiao Liang

An advanced understanding of stratospheric variability and its coupling to the troposphere is critical to improving the prediction of near-surface fields at subseasonal-to-seasonal timescale. In the most extreme case, a stratospheric sudden warming (SSW) event occurs and substantially perturbs the stratospheric circulation and, subsequently, exerts profound surface impacts. Interpretable deep learning could be a powerful tool in recognizing SSW spatial details and better categorizing the type of disrupted vortices. Here we apply a deep learning approach to identify SSW events from nonSSW ones using a global climate model with large ensembles. We start with a 1-dimensional case by using the stratospheric zonal wind of SSW events along the 60°N latitude to train neural networks with different complexity: logistic regression network, shallow neural network, and deep neural network. All neural networks can identify SSW events with a fairly high accuracy. To address the interpretability of how these neural networks learn to distinguish SSW from nonSSW events, we mask out the zonal wind fields with varying longitudinal windows to test if the spatial structure of disrupted vortices is decisive for the network performance. Neither shallow nor deep neural networks show apparent spatial dependence when the masking window is short, while logistic regression network gives strong spatial dependence centering around 160°W, where small variation and negative mean value of zonal wind appear. The dependence of shallow and deep networks emerges as the window length increases. To further explore the 2-dimensional spatial dependence, we further train a convolutional neural network exploiting the two-dimensional zonal wind fields in the Northern Hemisphere. Similar tests are performed by systematically masking out the zonal wind fields by a rectangular region with varying size. The spatial dependence of 2-dimensional neural network is largely consistent with 1-dimensional networks, but the spatial extents expand wider to the north of south of 60°N. The results highlight the capability of interpretable deep learning tools in learning the SSW spatial information and revealing the spatial dependence, which may carry out important implications for the prediction of SSW genesis.

Key words: interpretable deep learning, stratospheric sudden warming

How to cite: Zeng, Y.-J. and Liang, Y.-C.: Interpretable Deep Learning for the Identification of Sudden Stratospheric Warming Events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3772, https://doi.org/10.5194/egusphere-egu23-3772, 2023.

EGU23-4011 | ECS | Orals | AS1.29

A dynamical separation of deep and shallow branches in the stratospheric circulation 

Rasul Baikhadzhaev, Felix Ploeger, Peter Preusse, Manfred Ern, and Thomas Birner

The Brewer-Dobson circulation is the wave driven meridional circulation of the stratosphere it plays an important role in determining the transport of trace gases and aerosols within the stratosphere, affecting the lifetimes of ozone depleting substances, and the global radiation budget. The overturning part of the circulation is usually split into a deep and a shallow branch. Here, we investigate the dynamical driving of these circulation branches, aiming for a dynamical separation of different circulation regimes.

For that purpose, we use data from fifth generation atmospheric reanalysis ERA5 by the European Centre for Medium-range Weather Forecasts (ECMWF) and apply the Transformed Eulerian Mean approach to estimate the overturning mass flux and the related wave forcing in the stratosphere. We find that reducing the horizontal resolution of the data from 0.3 to 1 degree does not affect results significantly. However, reducing temporal resolution from 1 to 6 hours has a significant effect on the structure of daily mean upwelling, but this effect is much less pronounced for monthly means. Eliassen-Palm flux divergence is used as a diagnostic to estimate the wave propagation in the stratosphere. Using Fourier transformation for spectral decomposition we estimate the contribution from different waves to the driving of the deep and shallow branches. In particular, it is found that the deep branch has a strong seasonality with maximum in winter, while the shallow branch is less affected by the change of seasons. On the one hand, we find a strong correlation between variability in residual circulation velocity along the deep branch and large scale waves with wavenumber 3 or smaller. On the other hand, variability of medium and small scale waves with wavenumber 4 or greater correlates strongly with variability in the shallow branch circulation velocities. The change between these two dynamical regimes happens at a level close to 37 hPa. These results were further tested by applying a downward control calculation, showing that indeed the large-scale, planetary waves (wavenumber less than 4) account for the largest part of deep branch variability, while smaller waves (wavenumber larger than 3) account for the largest part of shallow branch variability. Based on these results, we propose a physical definition of the different Brewer-Dobson circulation branches, with the deep branch defined as driven by planetary waves (wave numbers 1-3) and located above 35 hPa, whereas the shallow branch being located below that level and driven by smaller-scale waves (wave numbers 4 and greater).  

How to cite: Baikhadzhaev, R., Ploeger, F., Preusse, P., Ern, M., and Birner, T.: A dynamical separation of deep and shallow branches in the stratospheric circulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4011, https://doi.org/10.5194/egusphere-egu23-4011, 2023.

EGU23-4513 | ECS | Posters on site | AS1.29

The impact of structural changes in the middle atmosphere on the Brewer-Dobson circulation 

Radek Zajíček, Petr Šácha, Petr Pišoft, Roland Eichinger, Harald Rieder, and Aleš Kuchař

Changes in atmospheric composition affect surface climate and alter atmospheric structure, dynamics, and transport, which in turn further affect the composition. In the middle atmosphere, the composition is influenced by the Brewer-Dobson circulation (BDC), a global-scale interhemispheric meridional overturning circulation. Namely, the BDC controls the distribution and trends of radiatively important gases like ozone and water vapour. Another robust aspect of the changes in greenhouse gas concentrations is the changing structure of the atmosphere across layers. The troposphere is thermally expanding, the stratosphere is cooling and contracting and this is then reflected in the mesosphere and above as a downward shift of the height of pressure levels. Particularly, the tropospheric expansion and the stratospheric contraction has been shown to interfere with diagnosed BDC trends. We developed an analytical methodology that allows us to partition between the pure acceleration of the circulation and other kinematic factors (vertical shift, widening) contributing to the net advective mass flux changes and quantify their roles precisely. We apply this methodology to different datasets (ERA5, CMIP6, CCMI-1) to analyze the variability and trends of advective transport between different layers of the middle atmosphere. Finally, we discuss how the net advective transport and the individual kinematic mechanisms contributing to it respond to external forcings.

How to cite: Zajíček, R., Šácha, P., Pišoft, P., Eichinger, R., Rieder, H., and Kuchař, A.: The impact of structural changes in the middle atmosphere on the Brewer-Dobson circulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4513, https://doi.org/10.5194/egusphere-egu23-4513, 2023.

Recent studies have suggested that extreme stratospheric wave activity is connected to surface temperature anomalies, with a dynamical mechanism distinct from the canonical downward influence of stratospheric polar vortex events. However, some key processes regarding the underlying dynamics and timescales are not well understood. In this study, we show in observations that the stratospheric events featured by weaker-than-normal wave activity are associated with increased cold extreme risks over North America before and near the event onset, accompanied by less frequent atmospheric river (AR) events on the west coast of the U.S. Strong stratospheric wave events, on the other hand, exhibit a tropospheric weather regime transition. North American warm anomalies and increased AR frequency over the west coast are observed before strong wave events, while an increased risk of cold extremes over North America and north-shifted ARs over the Atlantic occurs after the events. Historical simulations from CMIP6 can capture the extreme stratospheric wave events and their overall tropospheric fingerprints, with evident uncertainties across different models.

These links between the stratosphere and troposphere are attributed to the vertical structure of wave coupling. Weak wave events are accompanied by a wave structure tilting westwards with increasing altitude, while strong wave events show a shift from westward tilt to eastward tilt during the life cycle of events. This wave phase shift indicates vertical wave coupling and likely regional planetary wave reflection. Further examination shows that models with a degraded representation of stratospheric wave structure exhibit biases in the troposphere during strong wave events. More specifically, models with a stratospheric ridge weaker than the reanalysis exhibit a weaker tropospheric signal. Our findings suggest that the vertical coupling of extreme stratospheric wave activity should be evaluated in the model representation of stratosphere-troposphere coupling. 

 

How to cite: Ding, X. and Chen, G.: Assessing Stratosphere-troposphere Coupling of Extreme Stratospheric Wave Activity in CMIP6 Models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4526, https://doi.org/10.5194/egusphere-egu23-4526, 2023.

EGU23-6234 | Orals | AS1.29

Revealing the statistics of extreme stratospheric sudden warming events hidden in short weather forecast data 

Edwin Gerber, Justin Finkel, Dorian Abbot, and Jonathon Weare

Climate change will be felt primarily through changes in extreme weather: intense storms, precipitation events, and temperature anomalies.  Extreme events in the stratosphere, namely Sudden Stratospheric Warmings (SSWs), are known to impact surface weather extremes, driving an equatorward shift of the storm tracks and associated jet streams.  Efforts to quantify potential changes in SSWs in response to anthropogenic forcing, both their frequency and their surface impact, however, have been hampered by the large uncertainty in the observational record.  The problem becomes more acute for the most extreme SSWs, which are known to have a stronger surface impact. A once-in-a-century event takes, on average, 100 years of observations or simulation time to appear just once.  This is far beyond the typical integration length of our most accurate weather models, which provide the best representation of stratosphere-troposphere coupling, so the task is often left to cheaper, but less accurate, low-resolution or statistical models.  One reduces the sampling error (aleatoric uncertainty) at the expense of increased model error (epistemic uncertainty).

In this work, we propose methods to extract climatological information from subseasonal forecast ensembles.  Despite being short in duration, weather forecast ensembles are produced multiple times a week, collectively, adding up to thousands of years of data.  Using ensemble hindcasts produced by the European Center for Medium-range Weather Forecasting (ECMWF) archived in the subseasonal-to-seasonal (S2S) database, we compute multi-centennial return times of extreme SSW events. Consistent results are found between alternative methods, including basic counting strategies and Markov state modeling. By combining different trajectories together in a statistically rigorous way, we obtain estimates of SSW frequencies and their seasonal distributions that are consistent with reanalysis-derived estimates for moderately rare events, but can be extended to events of unprecedented severity that have not yet been observed historically. The same methods hold potential for assessing extreme events throughout the climate system, beyond the example of stratospheric extremes presented here, and could be adopted in the context of climate change integrations to quantify the impact of anthropogenic forcing on extreme weather.

How to cite: Gerber, E., Finkel, J., Abbot, D., and Weare, J.: Revealing the statistics of extreme stratospheric sudden warming events hidden in short weather forecast data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6234, https://doi.org/10.5194/egusphere-egu23-6234, 2023.

EGU23-8908 | ECS | Orals | AS1.29

Stratosphere-troposphere coupling under the extreme conditions of the No-Montreal-Protocol scenario 

Timofei Sukhodolov, Franziska Zilker, Gabriel Chiodo, Tatiana Egorova, Marina Friedel, Eugene Rozanov, Jan Sedlacek, Svenja Seeber, and Thomas Peter

The Montreal Protocol and its amendments (MPA) have been a major success in preventing serious health damage from the destruction of the stratospheric ozone layer by chlorofluorocarbons (CFCs). Additionally, unabated CFC emissions would have significantly accelerated global warming and affected large-scale tropospheric circulation. CFC-induced ozone depletion would have contributed to global climate change through reduced absorption of UV radiation, resulting in weaker stratospheric circulation, affecting the dynamical coupling to the troposphere. With the Earth System Model SOCOLv4, we study an extreme condition where the MPA is absent to disentangle the radiative and chemical (i.e., ozone-mediated) effects of CFCs and their impacts on stratosphere-troposphere coupling. Our results show that at the end of the 21st century, unabated CFC emissions would have largely destroyed the global ozone layer, which would have strongly affected the large-scale stratospheric and tropospheric circulation. In the stratosphere, contrary to historical ozone destruction, the polar vortices severely weaken due to low-latitude ozone depletion. In the Northern Hemisphere (NH), the weakening of the vortex leads to a pronounced negative phase of the North Atlantic Oscillation (NAO) in boreal winter and spring due to the chemical CFC effect. Similarly, the stratosphere also affects the Southern Annular Mode (SAM) to be in a more negative phase in austral winter and spring. However, tropospheric warming from CFCs largely dominates the overall SAM response to be in a more positive phase, whereas in the NH it compensates for the NAO negative phase. Additionally to the circulation changes, uncontrolled CFC emissions would have led to around 2.5 K additional global surface warming, being partially compensated by a cooling of around 0.6 K due to ozone depletion, leading to an overall warming of around 1.9 K. Our study strongly emphasizes the importance of the MPA for our climate and its mitigation of stratospheric circulation changes and their effects on tropospheric variability.

How to cite: Sukhodolov, T., Zilker, F., Chiodo, G., Egorova, T., Friedel, M., Rozanov, E., Sedlacek, J., Seeber, S., and Peter, T.: Stratosphere-troposphere coupling under the extreme conditions of the No-Montreal-Protocol scenario, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8908, https://doi.org/10.5194/egusphere-egu23-8908, 2023.

EGU23-9027 | ECS | Orals | AS1.29

Reduced stratospheric variability following sudden stratospheric warming events 

Philip Rupp, Jonas Spaeth, Hella Garny, and Thomas Birner

Sudden stratospheric warming (SSW) events can form a window of forecast opportunity for polar vortex predictions on subseasonal-to-seasonal time scales. Analysing numerical ensemble simulations, we show that negative wind anomalies in the polar stratosphere following SSWs lead to a reduction in upward planetary wave propagation and hence a reduction in the dynamical variability of the polar vortex. Ensembles that predict an SSW show reduced ensemble spread in terms of polar vortex strength for several weeks to follow, as well as a corresponding reduction in forecast errors. The associated increase in predictability is particularly pronounced for strong SSWs and even occurs if not all ensemble members predict a major SSW. The decrease in upward wave fluxes and polar vortex variability following the event then manifests in a delay of the final warming during years that experience an SSW and potentially has further implications for the tropospheric or mesospheric circulation.

How to cite: Rupp, P., Spaeth, J., Garny, H., and Birner, T.: Reduced stratospheric variability following sudden stratospheric warming events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9027, https://doi.org/10.5194/egusphere-egu23-9027, 2023.

EGU23-9505 | Posters on site | AS1.29

Trends in stratospheric contraction under sulfate aerosol injection 

Juan Antonio Añel, Laura de la Torre, Juan Carlos Antuña-Marrero, and Petr Sácha

The change in the size and density of Earth’s atmospheric layers is a noticeable impact of human activity on climate. It is well known that the troposphere has been widening over the last decades, and a contraction of the stratosphere has been recently quantified. At stratospheric levels, the injection of sulphur dioxide into the stratosphere warms the stratospheric sulphur layer. One of its known side effects is a general decrease in ozone concentrations. However, the magnitude of global ozone depletion decreases with time, and results show that there is even an increase in the stratospheric ozone concentration after sulfate aerosol injection (SAI) has ceased.

Here we present some preliminary results from the Geoengineering Large Ensemble Project (GLENS) regarding stratospheric contraction that show that SAI enhances the stratopause descent caused by climate change. In contrast, for the tropopause height, SAI reverses the rising observed with climate change, in values similar to the existing rising but of the opposite sign.

How to cite: Añel, J. A., de la Torre, L., Antuña-Marrero, J. C., and Sácha, P.: Trends in stratospheric contraction under sulfate aerosol injection, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9505, https://doi.org/10.5194/egusphere-egu23-9505, 2023.

EGU23-9666 | Orals | AS1.29

Representation, evolution and validation of the stratopause and stratospheric contraction in reanalyses data 

Laura de la Torre, Juan Antonio Añel, Aleš Kuchař, and Petr Sacha

Recent work using models from the Chemistry-Climate Model Initiative shows that the stratopause is descending and that the stratosphere has contracted substantially over the last decades, being the increasing concentrations of greenhouse gases (GHGs) the main driver. This stratospheric contraction is not a mere response to stratospheric cooling, as changes in both tropopause and stratopause pressure contribute significantly to it.

Here we present the evolution over the last decades of the stratopause and stratospheric thickness in the main reanalyses datasets: MERRA-2, JRA-55, and ERA5.1. We compare them to model results with WACCM-X and satellite observations (GOMOS, MLS and SABER). For our computations, we consider the discontinuity problems in temperature at stratopause heights suitable to affect its structure and behaviour due to the assimilation of new observational data as they become available.

Our results show that there is high variability in the percentages of stratopauses and their height, a significant dependence on the latitude and dataset for the stratopause height and limitations of JRA-55 to represent elevated stratopause cases (probably linked to sudden stratospheric warnings) over the polar regions because of its low-top compared to other reanalyses.

How to cite: de la Torre, L., Añel, J. A., Kuchař, A., and Sacha, P.: Representation, evolution and validation of the stratopause and stratospheric contraction in reanalyses data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9666, https://doi.org/10.5194/egusphere-egu23-9666, 2023.

EGU23-10155 | Orals | AS1.29 | Highlight

Monitoring and understanding upper atmospheric long-term cooling 

Shun-Rong Zhang, Wenbin Wang, Ercha Aa, Phil Erickson, Liying Qian, and Larisa Goncharenko


Atmospheric climate change is characterized by global warming above the Earth’s surface associated with the increase of the greenhouse gas population since the start of the industrial era. In the upper atmosphere where both neutral and plasma gases are subject to substantial variability due to space and terrestrial weather, including low atmospheric forcing. Direct and long-term ionospheric observations with the incoherent scatter radar (ISR) technique provide an efficient way to quantify and understand the variation trend of the thermal status in the upper atmosphere. Since 2008, the ISRs have been providing some of the key evidence for the cooling in the ionosphere and thermosphere, particularly, its altitude dependence above 100 km. This cooling was increasing as a function of height and was initially interpreted as a greenhouse gas effect in the upper atmosphere which was also observed in satellite drag observations, however, almost all the ISR results suggested that the cooling appeared substantially large and therefore additional cooling processes beyond the greenhouse gases as a thermospheric cooling agent are needed. These include potential wave activity changes arising from climate change as well as secular changes in Earth’s main magnetic field. In this presentation, we provide an updated analysis of ISR-measured trends and discuss some progresses in understanding these results.

How to cite: Zhang, S.-R., Wang, W., Aa, E., Erickson, P., Qian, L., and Goncharenko, L.: Monitoring and understanding upper atmospheric long-term cooling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10155, https://doi.org/10.5194/egusphere-egu23-10155, 2023.

EGU23-10986 | ECS | Orals | AS1.29

Exploring the Sudden Stratospheric Warming Events in High-top and Low-top Climate Model Large Ensembles 

Yu-Chiao Liang, Yi Wang, Young-Oh Kwon, Claude Frankignoul, Lorenzo Polvani, and Lingling Suo

Sudden stratospheric warming (SSW) events, followed by a characteristic circulation regime in the lower troposphere, are crucial for the subseasonal weather prediction. What remains controversial is whether or not increasing the height of top layer in a climate model and the vertical resolution improve the representation of SSW events and the subsequent influences on the near-surface climate. In this study, we examine the SSW events simulated in a high-top climate model (the Whole Atmosphere Community Climate Model version6, WACCM6) and those simulated in a low-top model (Community Atmosphere Model version 6, CAM6) with 30 ensemble members. The two sets of experiments are forced by identical observational sea-surface temperature and sea-ice concentration, as well as the radiative forcings, during the 1979-2013 period. We find that WACCM6 produces about two times more SSWs than CAM6 (i.e., 759 v.s. 357 events), and, in terms of occurring frequency, SSWs in WACCM6 happen about 7 times per decade, closer to the SSW frequency in reanalysis datasets. Analyses on the thermodynamical and dynamical components of SSWs, including the sea-level pressure precursor, the preceding Eliassen-Palm fluxes into the stratosphere, the stratospheric temperature increases, and the downward propagation features, reveal that WACCM6 in general gives weaker signals than CAM6. This is likely attributed to the weaker mean stratospheric circulation in WACCM6. We also find that the WACCM6-CAM6 differences can be amplified during the years of El Niño and La Niña events. Finally, we perform the vortex moments diagnostics to gain further insights into the vortex structure and separate the splitting and displacement SSWs. The diagnostics shows that CAM6 generates more symmetric polar vortices than WACCM6, while the vortices from CAM6 deviate less often from the North Pole. However, the ratio of displacement and splitting SSWs in both model is about 70%, larger than about 60% in reanalysis datasets. Our study suggests that the high-top configuration leads to better performance of stratospheric circulation variability.

How to cite: Liang, Y.-C., Wang, Y., Kwon, Y.-O., Frankignoul, C., Polvani, L., and Suo, L.: Exploring the Sudden Stratospheric Warming Events in High-top and Low-top Climate Model Large Ensembles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10986, https://doi.org/10.5194/egusphere-egu23-10986, 2023.

EGU23-11805 | Posters on site | AS1.29

The influence of using ERA-5 instead of ERA-Interim on stratospheric chemistry and ozone in EMAC simulations 

Ole Kirner, Alexandra Laeng, and Patrick Jöckel

In 2019, the European Centre for Medium-Range Weather Forecasts (ECMWF) published the ERA-5 reanalysis dataset (Hersbach et al., 2020). These new reanalysis data set replaced ERA-Interim (Dee at al., 2011), which had been previously often used in nudged simulations.

ERA-5 provides hourly estimates of a large number of atmospheric, land and oceanic climate variables. It uses a horizontal resolution of T639 (approx. 31km) and resolves the atmosphere using 137 levels from the surface up to a height of 1 Pa (approx. 80km). ERA-Interim only used T255 (approx. 79 km) with 60 levels from the surface up to 10 Pa (approx. 60 km) with a 6-hourly output.

To investigate the impact of these two reanalyses on the results of chemistry-climate simulations with the ECHAM/MESSy Atmospheric Chemistry (EMAC) model system, we performed three nudged simulations from 1979 to present.

EMAC is a numerical chemistry and climate simulation system that includes submodels describing tropospheric and middle-atmospheric processes and their interaction with oceans, land and human influences (Jöckel et al., 2010). We used EMAC (ECHAM5 version 5.3.02, MESSy version 2.55) with a horizontal resolution of T42 (corresponding to a quadratic Gaussian grid of 2.8° x 2.8°) and with 90 levels up to 0.01 hPa (approx. 80 km). The applied model setup includes a comprehensive chemistry scheme with gas-phase reactions and heterogeneous reactions on polar stratospheric clouds (PSCs). We used a similar setup as in the REF-D1 simulations for the IGAC/SPARC Chemistry-Climate Model Initiative (CCMI) using boundary conditions for greenhouse gases from CMIP-6 (Eyring et al., 2016) and for ozone depleting substances mainly from WMO (2008). Surface pressure, temperature, vorticity and divergence were nudged above the boundary layer and below 1 hPa (approx. 50 km) using a Newtonian relaxation technique.

We performed three EMAC simulations all with the same model setup as described above, but used as reanalysis data set ERA-Interim in the first simulation (from 1979 to 201908), and ERA-5 in the second and third simulation (from 1979 to 2021). In the third simulation we used from 2000 to 2006 the ERA-5.1 data set instead of the ERA-5. ERA-5.1 is a rerun of ERA5 for the years 2000 to 2006 only, in which the cold bias in the lower stratosphere seen in ERA5 was improved.

In our presentation, we will compare these three EMAC simulations regarding temperature, dynamic and chemistry with focus of the influence of the different reanalysis data sets to the distribution and development of stratospheric ozone.

Additional we will present the comparisons of ozone fields of our three simulations with different satellite observations (in particular MIPAS and MLS) and access whether the use of ERA-5 leads to an improvement of the results of our EMAC simulations.

How to cite: Kirner, O., Laeng, A., and Jöckel, P.: The influence of using ERA-5 instead of ERA-Interim on stratospheric chemistry and ozone in EMAC simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11805, https://doi.org/10.5194/egusphere-egu23-11805, 2023.

EGU23-12607 | ECS | Posters on site | AS1.29

Implementation of sulfur hexafluoride (SF6) in the Belgian Assimilation System for Chemical ObsErvations (BASCOE) 

Sarah Vervalcke, Simon Chabrillat, Daniele Minganti, and Quentin Errera

Sulfur hexafluoride (SF6) is a greenhouse gas that is emitted at the surface because of its use as an insulator in electrical transmission equipment and electronic devices. Since its quasi-linear emission growth and its very long lifetime, SF6 can be used as a tracer for the Age of Air (AoA) to diagnose changes in the Brewer Dobson Circulation (BDC). The chemistry of SF6 has been implemented in the Chemistry Transport Model (CTM) of the Belgian Assimilation System for Chemical ObsErvations (BASCOE). Reaction rates were taken from previous studies while an electron density has been taken from WACCM-X-SD simulations.
In this contribution, BASCOE-CTM simulations driven by ERA5 and MERRA2 will be discussed considering SF6 with and without mesospheric sinks (i.e. passive SF6 in the latter case). During the course of the simulations, the computed mixing ratios have also been saved in the space of MIPAS observations to analyse the impact of the MIPAS sampling in its AoA derivation.

How to cite: Vervalcke, S., Chabrillat, S., Minganti, D., and Errera, Q.: Implementation of sulfur hexafluoride (SF6) in the Belgian Assimilation System for Chemical ObsErvations (BASCOE), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12607, https://doi.org/10.5194/egusphere-egu23-12607, 2023.

EGU23-12651 | ECS | Posters on site | AS1.29

Chemical and dynamical variability in the middle atmosphere related to energetic electron precipitation 

Antti Salminen, Timo Asikainen, and Kalevi Mursula

Energetic electron precipitation (EEP) directly influences the high-latitude thermosphere and mesosphere. Precipitating electrons originate from the Earth’s magnetosphere and their precipitation to the atmosphere is driven by the solar wind. EEP produces odd nitrogen (NOX) and odd hydrogen (HOX) oxides which catalytically destroy ozone. During the winter, EEP-NOX survives for months, which enables its descent to the polar stratosphere. Several studies, based on both observations and models, have shown that EEP-induced ozone destruction leads to changes in temperature and dynamics in the atmosphere which strengthen the stratospheric polar vortex, a westerly wind system surrounding the pole. However, most observational studies on EEP effects have relied on reanalysis datasets which are mainly limited to the stratospheric altitude. Thus, observations of EEP effects on the atmosphere are still partly incomplete. In this study we use the AURA/MLS satellite measurements of atmospheric variables and the POES/MEPED satellite measurements of precipitating electrons to study EEP-related interannual variability in chemical and dynamical properties of the northern winter mesosphere and stratosphere in 2004-2022. We confirm the earlier findings of EEP effects on ozone and temperature in the polar region and on the polar vortex in the stratosphere, and also examine the related variability in the northern winter mesosphere. Moreover, we confirm our recent results about the role of planetary waves in modulating the EEP effect on the polar vortex.

How to cite: Salminen, A., Asikainen, T., and Mursula, K.: Chemical and dynamical variability in the middle atmosphere related to energetic electron precipitation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12651, https://doi.org/10.5194/egusphere-egu23-12651, 2023.

EGU23-12717 | ECS | Orals | AS1.29

In situ chemical composition and density measurements of Earth’s thermosphere, exosphere, and ionosphere with CHESS 

Rico Fausch, Gregor Moeller, Aziz Belkhiria, Jean-Paul Kneib, and Peter Wurz

The Constellation of High-performance Exosphere Science Satellites (CHESS) mission is a dedicated CubeSat mission designed to analyse the upper atmosphere of Earth in situ. The status of this dynamic region is driven by external and internal forces, causing variations in temperature, the chemical composition, total number density, and their altitude profiles. Although such measurements are key for our understanding of the origin and evolution of the habitable atmosphere of Earth, the community lacks updated, local, detailed measurements. Recent technological advancements in instrumentation enable sensitive in situ measurements of the exosphere–thermosphere–ionosphere region with small satellites. On one hand, the miniaturisation of a high-performance mass spectrometer enables measurements of the chemical composition and density. On the other hand, a new generation of dual-frequency Global Navigation Satellite System (GNSS) receivers enable precise orbit determination. From the knowledge of the evolution of the orbits, the atmospheric drag and hence, the density can be derived complementary. Additionally, the GNSS receivers provide the dispersive line-of-sight total electron content from the linear combination of dual-frequency carrier phase measurements that can be converted into total column density between the spacecraft in low Earth orbit and the satellites of the GNSS in higher orbits. Thanks to the elliptic orbit of the spacecraft, the altitude profiles of these number density measurements of species can be converted into exospheric temperatures. Measuring with a constellation will allow for overcoming the space-time degeneracy to analyse the drivers and mechanisms including basic physics in detail. The CHESS mission is scheduled for launch in early 2026. Once available, the collected data will also be compared with atmospheric escape data on, for example, Venus and Mars to provide insights into the different evolution of these rocky, initially comparable planets.

How to cite: Fausch, R., Moeller, G., Belkhiria, A., Kneib, J.-P., and Wurz, P.: In situ chemical composition and density measurements of Earth’s thermosphere, exosphere, and ionosphere with CHESS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12717, https://doi.org/10.5194/egusphere-egu23-12717, 2023.

EGU23-13181 | Orals | AS1.29

Monitoring sudden stratospheric warmings under climate change since 1980 based on reanalysis data verified by radio occultation 

Ying Li, Gottfried Kirchengast, Marc Schwaerz, and Yunbin Yuan

We developed a new approach to monitor Sudden Stratospheric Warming (SSW) events under climate change since 1980 based on reanalysis data, verified by radio occultation data. We constructed gridded daily-mean temperature anomalies from the input fields at different vertical resolution (basic case full resolution; cross-check with reanalysis at 10 stratospheric standard pressure levels or 10 hPa and 50 hPa level only) and employed the concept of Threshold Exceedance Areas (TEAs), the geographic areas wherein the anomalies exceed predefined thresholds (such as 30 K) to monitor the phenomena.

We derived main-phase TEAs, representing combined middle and lower stratospheric warming, to monitor SSWs on a daily sampling basis. Based on the main-phase TEAs, three key metrics, including main-phase duration, area, and strength are estimated and used for the detection and classification of SSW events. An SSW is defined to be detected if the main-phase warming lasts at least 6 days. According to the strength, SSW events are classified into minor, major and extreme. An informative 42 winters’ SSW climatology 1980-2021 was developed, including the three key metrics as well as onset date, maximum-warming-anomaly location and other valuable SSW characterization information.

Detection and validation against previous studies underpins that the new method is robust for SSW detection and monitoring and that it can be applied to any quality-assured reanalysis, model, and observational temperature data that cover the polar region and winter timeframes of interest, either using high vertical resolution input data (preferable basic case), coarser standard-pressure-levels resolution or (at least) 10 hPa and 50 hPa pressure level data. Within the 42 winters, 43 SSW events were detected for the basic case, yielding a frequency of about one event per year. In the 1990s, where previous studies showed gaps, we detected several events. Over 95 % of event onset dates occurred in deep winter (Dec-Jan-Feb timeframe; about 50 % in January) and three quarters have their onset location over Northern Eurasia and the adjacent polar ocean.

Regarding long-term change, we found a statistically significant increase in the duration of SSW main-phase warmings, by about 5 days over the climate change period from the 1980s to the 2010s, raising the average duration by near 50 % from about 10 to 15 days and inducing an SSW strength increase by about 40 million km2 days, from about 100 to 140 million km2 days. The results are robust (consistent within uncertainties) across using different input data resolution. They can hence be used as a reference for further climate change-related studies and be a valuable basis for studying SSW impacts and links to other weather and climate phenomena, such as changes in polar vortex dynamics and in mid-latitude extreme weather.

How to cite: Li, Y., Kirchengast, G., Schwaerz, M., and Yuan, Y.: Monitoring sudden stratospheric warmings under climate change since 1980 based on reanalysis data verified by radio occultation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13181, https://doi.org/10.5194/egusphere-egu23-13181, 2023.

EGU23-13525 | ECS | Orals | AS1.29

Weakening of springtime Arctic ozone depletion with climate change 

Marina Friedel, Gabriel Chiodo, and Thomas Peter

Arctic ozone is subject to large interannual variability, and severe ozone minima can occur through chemical ozone depletion and dynamical variability. Such Arctic ozone minima have been shown to bear a great societal relevance due to their impacts on health and climate. Following the success of the Montreal Protocol, ozone depleting substances (ODSs) in the stratosphere are declining, implying an expected weakening of chemical ozone destruction. However, continuing greenhouse gas (GHG) emissions cool the stratosphere, which might lead to an enhanced formation of polar stratospheric clouds (PSCs) and thus more efficient chemical depletion of ozone. Due to these opposing processes, there is currently no consensus on the fate of Arctic ozone minima in future climate.

 

Here, we investigate the future evolution of Arctic ozone minima over the 21st century under different emission pathways in simulations conducted for the Chemistry-Climate Model Initiative (CCMI), CCMI-1 and CCMI-2022, and constrain these projections based on the models’ skill in reproducing present-day Arctic ozone variability. We find a large model discrepancy in the magnitude of ozone minima under present-day climate, caused by biases in the underlying model climatology. Models that simulate large ozone minima in present-day climate generally have a cold bias, and consequently large concentrations of active chlorine species (ClOx); these are the models that project the largest decline in the magnitude of ozone minima in the future. Conversely, models simulating weak Arctic ozone minima under present-day conditions generally have a warm bias and small ClOx concentrations; these are models with the smallest sensitivity of ozone minima to changes in ODS and GHG emissions. Consequently, inter-model spread in the magnitude of springtime Arctic ozone minima is projected to decline in the future. Through comparison with reanalysis, we identify the most realistic models. These models show a weakening in stratospheric ozone minima of about 1 DU/decade and with little sensitivity to the GHG emission scenario, which is deemed as the most likely projection. Taken together, these results indicate that Arctic ozone minima will likely become weaker in the future, largely due to the decline in ODS abundances, while stratospheric cooling due to GHGs is expected to play a secondary role.

How to cite: Friedel, M., Chiodo, G., and Peter, T.: Weakening of springtime Arctic ozone depletion with climate change, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13525, https://doi.org/10.5194/egusphere-egu23-13525, 2023.

EGU23-13741 | ECS | Orals | AS1.29

Non-Additivity of the Midlatitude Circulation Response to Regional Arctic Temperature Anomalies: The Role of the Stratosphere 

Bithi De, Yutian Wu, Lorenzo Polvani, and Gregory Elsaesser

Previous studies have documented the impact of the Arctic sea ice loss and associated warming on the midlatitude weather and climate, especially the influence of sea ice retreat over the Barents-Kara Sea on the North Atlantic and Europe regions. However, less attention has been given to other geographical locations over the Arctic, and to the linear additivity of the circulation response to regional Arctic sea ice loss and temperature anomalies. Using a simplified dry dynamical core model, we demonstrate that responses to regional Arctic temperature anomalies over the Barents-Kara Sea, Baffin Bay-Davis Strait-Labrador Sea, and East Siberia-Chukchi Sea, separately, cause similar equatorward shift of the tropospheric jet, but different stratospheric polar vortex responses. Furthermore, responses to regional Arctic temperature anomalies are not linearly additive, and the residual resembles a positive Northern Annular Mode-like structure. Additional targeted experiments highlight the stratospheric influence in the non-additivity of the midlatitude tropospheric response.

How to cite: De, B., Wu, Y., Polvani, L., and Elsaesser, G.: Non-Additivity of the Midlatitude Circulation Response to Regional Arctic Temperature Anomalies: The Role of the Stratosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13741, https://doi.org/10.5194/egusphere-egu23-13741, 2023.

EGU23-13881 | Posters on site | AS1.29

Montreal Protocol's impact on the ozone layer and climate 

Jan Sedlacek, Tania Egorova, Timofei Sukhodolov, Arseniy Karagodin-Doyennel, Franziska Zilker, and Eugene Rozanov

It is now recognized and confirmed that the ozone layer shields the biosphere from dangerous solar UV radiation and is also important for the global atmosphere and climate. The observed massive ozone depletion forced the introduction of limitations on the production of halogen-containing ozone-depleting substances (hODS) by the Montreal Protocol and its Amendments and adjustments (MPA). Further research was aimed at analyzing the role played by the Montreal Protocol to increase public awareness of its necessity. In this study, we evaluate the benefits of the Montreal Protocol on climate and ozone evolution using the Earth system model (ESM) SOCOLv4.0 which includes dynamic ocean, sea ice, interactive ozone, and stratospheric aerosol modules. Here, we analyze the results of the numerical experiments performed with and without limitations on the ozone-depleting substances emissions. In the experiments, we have used CMIP6 SSP2-4.5 and SSP5-8.5 scenarios for future forcing behavior. We confirm previous results regarding catastrophic ozone layer depletion in the case without MPA limitations. The climate effects of MPA consist of additional global mean warming by up to 2.5 K in 2100 caused by the direct radiative effect of the hODS. We also obtained dramatic changes in several essential climate variables such as regional surface air temperature, sea-ice cover, and precipitation fields. The warming rate without the MPA under the SSP2-4.5 scenario is comparable to the warming rate of the SSP5-8.5 scenario with MPA. Our research updates and complements previous modeling studies on the quantifying of MPA benefits for the terrestrial atmosphere and climate.

How to cite: Sedlacek, J., Egorova, T., Sukhodolov, T., Karagodin-Doyennel, A., Zilker, F., and Rozanov, E.: Montreal Protocol's impact on the ozone layer and climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13881, https://doi.org/10.5194/egusphere-egu23-13881, 2023.

EGU23-14758 | Orals | AS1.29

Sensitivity of ozone return dates to shared socioeconomic pathway in CMIP6 models 

James Keeble, Birgit Hassler, and Manuel Schlund

Following the success of the Montreal Protocol, stratospheric ozone is projected to recover over the coming decades as halogenated ozone depleting substances decline. However, future projections of stratospheric ozone recovery are also dependent on assumptions made about the emissions of other gases such as CO2, CH4, and N2O. As a result, the pathway of ozone recovery is sensitive to the choice of future emissions scenario. Here we explore ozone recovery under different Shared Socioeconomic Pathways (SSPs) in 6 CMIP6 models that include interactive chemistry schemes: CESM2-WACCM, CNRM-ESM2-1, GFDL-ESM4, GISS-E2-1-G, MRI-ESM2-0, UKESM1-O-LL. We explore the impact of different SSP scenarios on projections of ozone recovery, the date at which total column ozone returns to historic values, and the healing of the ozone hole. Additionally, we compare global mean return dates with regional return dates and explore the different processes affecting the timing of ozone recovery in these different regions.

How to cite: Keeble, J., Hassler, B., and Schlund, M.: Sensitivity of ozone return dates to shared socioeconomic pathway in CMIP6 models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14758, https://doi.org/10.5194/egusphere-egu23-14758, 2023.

EGU23-15173 | Orals | AS1.29

Characteristics of the Stratospheric Tropical Circulation of the Energy Exascale Earth System Model E3SMv2 

Christiane Jablonowski, Lisa Nguyen, Jean-Christophe Golaz, Nan Rosenbloom, and Gerald A. Meehl

The Energy Exascale Earth System Model version 2 (E3SMv2) was publicly released by the Department of Energy (DoE) in September 2021. An important component of the model validation were historical climate simulations that followed the protocols of the Coupled Model Intercomparison Project Phase 6 (CMIP6). In particular, five historical ensemble members were recently released, and 16 additional ensemble members will soon become available as part of an E3SMv2 Large Ensemble (LE). The paper sheds light on the characteristics of the E3SMv2 CMIP6 stratospheric circulation which has not yet been documented in the literature. Particular attention is paid to the tropical stratosphere which includes the so-called water vapor tape recorder and the Quasi-Biennial Oscillation. In addition, the general circulation and its variability are briefly described to reveal E3SMv2’s strengths and weaknesses. We compare E3SMv2’s circulation to observations and ERA5 reanalysis data. Furthermore, selected comparisons to the predecessor version E3SMv1 as well as other CMIP6 models are provided to put the results into context. The analysis informs the DoE Sandia National Laboratories project CLDERA which uses the Mt. Pinatubo volcanic eruption for climate attribution studies.

How to cite: Jablonowski, C., Nguyen, L., Golaz, J.-C., Rosenbloom, N., and Meehl, G. A.: Characteristics of the Stratospheric Tropical Circulation of the Energy Exascale Earth System Model E3SMv2, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15173, https://doi.org/10.5194/egusphere-egu23-15173, 2023.

EGU23-15552 | ECS | Posters on site | AS1.29 | Highlight

Ozone in a stratospheric aerosol injection scenario 

Andrin Jörimann, Gabriel Chiodo, Sandro Vattioni, Timofei Sukhodolov, Simone Tilmes, Daniele Visioni, David Plummer, and Olaf Morgenstern

Stratospheric aerosol injection (SAI) holds the potential to offset some of the future warming of the Earth’s surface. It comes with many potentially dangerous side effects, however, which are currently not well understood and poorly constrained. A major concern is the effect on stratospheric ozone, which could be weakened and delayed in its recovery, given that ozone-depleting substances will take decades to be completely removed. We are interested in ozone depletion and recovery in a scenario, where SAI is employed to keep the global surface temperature constant. Previous analyses have been conducted with models that have widely different treatments of aerosol microphysics and chemistry. To isolate and estimate the uncertainty of the chemical and dynamical effects in a multi-model context, CCMI-2022 proposed a new senD2-sai experiment, where the ocean is kept fixed and the elevated stratospheric aerosol burden, thus, only affects the middle atmospheric composition and temperature. Stratospheric aerosols are also uniformly prescribed for all participating models in order to minimize the uncertainty arising from the treatment of aerosol microphysics. In our work, we perform these experiments with our aerosol-chemistry-climate model SOCOLv4.0, and compare our results with other CCMI-2022 models, with a focus on the stratospheric ozone and temperature changes. We evaluate the role of individual processes, such as ozone destruction cycles and changes in large-scale transport. In addition, we discuss implementation issues related to imposing this aerosol forcing, as this will help in the interpretation of the main inter-model uncertainties. Finally, we discuss the implications of this work for our understanding of chemical feedbacks in future climate in the context of mitigation via SAI, and its relevance for future ozone assessments.

How to cite: Jörimann, A., Chiodo, G., Vattioni, S., Sukhodolov, T., Tilmes, S., Visioni, D., Plummer, D., and Morgenstern, O.: Ozone in a stratospheric aerosol injection scenario, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15552, https://doi.org/10.5194/egusphere-egu23-15552, 2023.

EGU23-17451 | Orals | AS1.29

Brewer Dobson Circulation trends from Age of Air in models 

Louis Rivoire, Marianna Linz, Jingyuan Li, and Marta Abalos

Given the couplings between the circulation of the stratosphere and its composition, tracking the evolution of both is crucial. At present however, much remains to be learned about long term trends in the composition of the stratosphere, and there is still little to no agreement between the modeled trends in the Brewer Dobson Circulation and their observational counterparts; while models indicate that the BDC is accelerating at a pace of 2-3 %/decade, observational estimates suggest that the BDC is slowing down. These shortcomings are attributable in part to the relatively short length of the historical record and in part to difficulty characterizing the BDC using observations.

To alleviate these shortcomings, we propose to re-visit historical and projected BDC trends using the metric time of emergence (ToE), defined as the length of record needed to separate long-term trends from internal variability with a chosen degree of statistical confidence. We use ToE as it enables the evaluation of current observational capabilities for the detection and validation of BDC trends predicted by models. ToE also provides tangible motivation for the continued monitoring of the composition of the stratosphere by space borne platforms, a topic recently brought to light by the planned decommissioning of the Aura satellite in the absence of a follow-up flight mission.

ToE is calculated using two methods, for which results are compared: a) classic bootstrapping based on a reference CMIP6 run (a pre-industrial run, or a run with fixed contemporary greenhouse gas concentrations), and b) an analytical method published by Li et al. (2017) that does not require a very long reference run. We focus the analysis on a comparison of ToE for trends in a) the diabatic circulation, taken as reference for the “true” BDC, and b) the BDC metric based on age of air developed by Linz et al. (2016), used as a proxy for observational trend estimates. The results shed light on how internal variability shapes our understanding of long term trends, and provide minimum requirements for the robust detection of trends in the BDC using observations. 

Li, J., Thompson, D.W., Barnes, E.A. and Solomon, S., 2017. Quantifying the lead time required for a linear trend to emerge from natural climate variability. J. of Climate.

Linz, M., Plumb, R.A., Gerber, E.P. and Sheshadri, A., 2016. The relationship between age of air and the diabatic circulation of the stratosphere. JAS.

How to cite: Rivoire, L., Linz, M., Li, J., and Abalos, M.: Brewer Dobson Circulation trends from Age of Air in models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17451, https://doi.org/10.5194/egusphere-egu23-17451, 2023.

EGU23-1246 | ECS | Orals | AS1.30 | Highlight

An ozone mini-hole associated with the record-breaking Australian bushfires 2019-2020: satellite observations and the modelled impact on surface ultraviolet radiation 

Redha Belhadji, Pasquale Sellitto, Maxim Eremenko, Silvia Bucci, Nguyet Minh, Gaëlle Dufour, and Bernard Legras

The Australian record-breaking bushfires around the turn of the year 2020 generated an unprecedented perturbation of thestratospheric composition through the injection of biomass burning material at relatively high altitudes in the upper-troposphere—lower-stratosphere. Associated with this event, a highly-stable smoke-charged anticyclonic vortex, with horizontal extent as large as about 1000 km, was observed. Due to the solar radiation absorption in this vortex, this structure was observed to rise from the initial ~15 km altitude to altitudes higher than ~35 km [Khaykin et al 2020]. This structure persisted in the stratosphere for about 3 months.

Here we present a detailed analysis of the vertically-resolved ozone fields based on the Infrared Atmospheric Sounding Interferometer (IASI) observations, supported by total column observations at relatively high horizontal resolution with Sentinel 5p TROPOMI (TROPospheric Ozone Monitoring Instrument), associated with the smoke-charged vortex due to the Australian bushfires. A marked ozone mini-hole is found, horizontally and vertically co-located with this smoke structure. The dynamical and/or chemical origin of this ozone mini-hole is briefly discussed. Then, ozone profile information is fed to the LibRadtran/UVSPEC radiative transfer model to estimate the impact of this ozone reduction on surface ultraviolet radiation and the results are critically discussed in terms of the possible impacts on the biosphere

Ref : Khaykin, S., Legras, B., Bucci, S., Sellitto P., Isaksen, L., Tencé, F., Bekki, S., Bourassa, A., Rieger, L., Zawada, D., Jumelet, J., and Godin-Beekmann, S.: The 2019/20 Aus- tralian wildfires generated a persistent smoke-charged vortex rising up to 35km altitude, Commun. Earth Environ. 1, 22, https://doi.org/10.1038/s43247-020-00022-5, 2020.

How to cite: Belhadji, R., Sellitto, P., Eremenko, M., Bucci, S., Minh, N., Dufour, G., and Legras, B.: An ozone mini-hole associated with the record-breaking Australian bushfires 2019-2020: satellite observations and the modelled impact on surface ultraviolet radiation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1246, https://doi.org/10.5194/egusphere-egu23-1246, 2023.

EGU23-1348 | Orals | AS1.30

Interhemispheric transport into the southern hemisphere polar stratosphere from the Asian monsoon region 

Xiaolu Yan, Paul Konopka, Felix Ploeger, and Aurélien Podglajen

The South-East Asian boundary layer has become one of the most polluted regions in recent years due to rapid
economic growth, which even affect the trace gas composition in the southern hemisphere by inter-hemispheric transport. We
study the transport from the boundary layer of the Asian summer monsoon (ASM) region [15N, 45N, 30E, 120E] into
the global upper troposphere and lower stratosphere (UTLS) using the Lagrangian chemistry transport model CLaMS driven
by the ERA5 reanalysis during 2010-2014. In particular, we quantify the inter-hemispheric transport contribution from the
ASM region to the southern hemisphere polar region (SP) [60S, 90S] and investigate the influence on pollution. Despite the
smaller size of ASM area compared to the southern hemisphere (SH) subtropics [15S, 45S] and tropics [15S, 15N], we
find that the air mass fractions (AMF) from the ASM to the SP are about 1.5 times larger than the corresponding contributions
from the SH subtropics and about two times smaller than those from the tropics. Transport from the ASM boundary layer to
the Southern polar vortex occurs largely above about 450 K and on timescales longer than 2 years, while transport timescales
to the Antarctic region below the vortex are shorter than about 2 years. The transport contribution from the ASM region to
the SP presents distinct inter-annual variability, which is strongly related to the strength of polar vortex. The relatively young
(less than two years) tracers originating from the ASM region show good correlations with CCl4, F12, and CH3Cl observations
from ACE-FTS in the antarctic UTLS. The reconstructed SF6 indicates that about 20% of SF6 in the SP stratosphere originates
from the ASM boundary layer, which is larger than the SF6 fraction of SH subtropical origin, while 50% of SF6 in the SP
stratosphere originates from the tropical boundary layer.

How to cite: Yan, X., Konopka, P., Ploeger, F., and Podglajen, A.: Interhemispheric transport into the southern hemisphere polar stratosphere from the Asian monsoon region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1348, https://doi.org/10.5194/egusphere-egu23-1348, 2023.

EGU23-1966 | Orals | AS1.30

Understanding the climate impacts of the Asian Summer Monsoon with in-situ observations of aerosol microphysical properties in the upper troposphere and lower stratosphere 

Christina Williamson, Dylan Simone, Charles Brock, Ming Lyu, Matthew Brown, Luke Ziemba, Joowan Kim, Teresa Campos, Kirk Ullmann, and Laura Pan

The Asian monsoon anticyclone transports aerosol and gas phase pollutants from the boundary layer to the upper troposphere and lower stratosphere, from whence they are transported out over the Western Pacific by eddy shedding. This significantly increases aerosol loading in the upper troposphere and maintains a layer of aerosol in the lowermost stratosphere with important implications for climate and stratospheric chemistry. Models show large spread in the spatial distribution and microphysical properties of aerosols transported by the Asian monsoon, and the chemical and radiative effects remain uncertain.

In August 2022 we measured aerosol size distributions in Asian summer monsoon outflow from two aircraft, the NCAR GV and NASA WB57, as part of the Asian Summer Monsoon Chemical Climate Impacts Project (ACCLIP). On both aircraft we operated a Nucleation Mode Aerosol Size Spectrometer (NMASS, a custom battery of 5 condensation particle counters) and a modified Ultra-High Sensitivity Aerosol Spectrometer (an optical particle counter from Droplet Measurement Technologies) to measure size distributions from 3 to 1500 nm at 1 Hz time resolution.

Here we use these data together with concurrently measured trace gases and reactive gases, and cloud properties, to quantify the transport of primary aerosol by the monsoon system, and the formation of secondary aerosol in the monsoon outflow. We show that new particle formation occurs in the upper troposphere in monsoon outflow and investigate its relation to lofting of condensable vapours and wet scavenging of larger aerosols by deep convection. We use data taken in the upper troposphere and lower stratosphere of the NASA Atmospheric Tomography Mission (ATom) to compare aerosol microphysical properties in the summer monsoon outflow with those in less anthropogenically influence air.

How to cite: Williamson, C., Simone, D., Brock, C., Lyu, M., Brown, M., Ziemba, L., Kim, J., Campos, T., Ullmann, K., and Pan, L.: Understanding the climate impacts of the Asian Summer Monsoon with in-situ observations of aerosol microphysical properties in the upper troposphere and lower stratosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1966, https://doi.org/10.5194/egusphere-egu23-1966, 2023.

EGU23-2049 | ECS | Posters on site | AS1.30

Global seasonal distribution of CH2Br2 and CHBr3 in the upper troposphere and lower stratosphere 

Markus Jesswein, Rafael P. Fernandez, Lucas Berná, Alfonso Saiz-Lopez, Jens-Uwe Grooß, Ryan Hossaini, Eric C. Apel, Rebecca S. Hornbrook, Elliot L. Atlas, Donald R. Blake, Stephen Montzka, Timo Keber, Tanja Schuck, Thomas Wagenhäuser, and Andreas Engel
Halogens from long-lived anthropogenic substances contribute to the depletion of stratospheric ozone. Besides these long-lived substances, chlorinated and brominated substances with lifetimes of less than 6 months are additional sources of stratospheric halogens. These substances, also known as very short-lived substances (VSLSs), have both natural and anthropogenic origins. The contribution of chlorinated VSLSs (Cl-VSLSs) to stratospheric chlorine is a few percent. In comparison, brominated VSLSs (Br-VSLS) contribute to about a quarter of the stratospheric bromine. The relative contribution of VSLSs to stratospheric halogen loading is expected to increase as the Montreal Protocol controlled substances progressively decrease. Due to their short lifetimes, VSLSs rapidly release their halogen content into the lowermost stratosphere, a region where changes in ozone have a relatively large impact on surface climate.

Here we present the global seasonal distribution of the two major Br-VSLSs CH2Brand CHBr3, which account for about 80 % of total organic Br-VSLS. Measurements from four High Altitude and Long Range Research Aircraft (HALO) missions, the HIAPER Pole-to-Pole Observations (HIPPO) mission, and the Atmospheric Tomography (ATom) mission were used for this purpose. Observational results show a similar seasonality of CH2Br2 in the free and upper troposphere of both hemispheres and less clear seasonality with larger variations for CHBr3. The distribution of CH2Brin the lowermost stratosphere suggests differences in hemispheric autumn, where the influx of tropospheric air seen in northern hemispheric summer to autumn is not evident in the Southern Hemisphere. However, the southern hemispheric database is insufficient to quantify this difference. The observed distributions were additionally compared to distributions based on model results of TOMCAT and CAM-Chem, both using the emission inventory of Ordóñez et al. (2012). Neither model was able to reproduce the seasonal distribution of CH2Br2 in the Southern Hemisphere. In contrast, both models show a pronounced seasonality of CHBr3 in both hemispheres, which is not confirmed by observations. The distributions of both substances in the lowermost stratosphere are overall well captured by the models, except for southern hemispheric autumn with considerably lower mixing ratios in the observations.

How to cite: Jesswein, M., Fernandez, R. P., Berná, L., Saiz-Lopez, A., Grooß, J.-U., Hossaini, R., Apel, E. C., Hornbrook, R. S., Atlas, E. L., Blake, D. R., Montzka, S., Keber, T., Schuck, T., Wagenhäuser, T., and Engel, A.: Global seasonal distribution of CH2Br2 and CHBr3 in the upper troposphere and lower stratosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2049, https://doi.org/10.5194/egusphere-egu23-2049, 2023.

We present our study on the sub-seasonal variability of UTLS aerosols and CO that is a result of the variability induced by the sub-seasonal variability of the Asian summer monsoon dynamics. We use the NASA global model GEOS simulations that incorporates emissions from anthropogenic, biomass burning, volcanic, and other natural sources to simulate CO, aerosols and related gases and the model experiments separating source types (anthropogenic, biomass burning, volcanic) and source locations (East Asia, South Asia). With model results and observations from recent aircraft measurements (StratoClim, ACCLIP) in the UTLS over the Asian summer monsoon regions, we will discuss (1) the sub-seasonal variability of transport pathways of surface-generated pollutants to reach UTLS, and (2) sub-seasonal variation of aerosol composition that is determined by the variability of source type originating in different locations.

How to cite: Chin, M., Bian, H., Colarco, P., Lait, L., and Chen, G.: Sub-seasonal variability of Asian summer monsoon transport of aerosols and CO to the UTLS in the context of recent aircraft observations in the Asia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2131, https://doi.org/10.5194/egusphere-egu23-2131, 2023.

EGU23-2417 | Orals | AS1.30 | Highlight

Stratospheric climate anomalies and ozone loss caused by the Hunga Tonga volcanic eruption 

William Randel, Xinyue Wang, Yunqian Zhu, and Simone Tilmes

The Hunga Tonga volcanic eruption in January 2022 injected extreme amounts of water vapor (H2O) and a moderate amount of aerosol precursor (SO2) into the Southern Hemisphere (SH) stratosphere. The H2O and aerosol perturbations have persisted and resulted in large-scale SH stratospheric cooling, equatorward shift of the Antarctic polar vortex, and slowing of the Brewer-Dobson circulation associated with a substantial ozone reduction in the SH winter midlatitudes. Chemistry-climate model simulations forced by realistic HTHH inputs of H2O and SO2 reproduce the observed stratospheric cooling, circulation changes and ozone loss, demonstrating the observed behavior is due to the volcanic influences. Furthermore, the combination of aerosol transport to polar latitudes and a cold polar vortex enhances springtime Antarctic ozone loss, consistent with observed polar ozone behavior in 2022.

How to cite: Randel, W., Wang, X., Zhu, Y., and Tilmes, S.: Stratospheric climate anomalies and ozone loss caused by the Hunga Tonga volcanic eruption, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2417, https://doi.org/10.5194/egusphere-egu23-2417, 2023.

EGU23-2552 | ECS | Posters on site | AS1.30

Assessment of variability and trends of the tropopause from reanalyses data 

Ling Zou and Lars Hoffmann

As the boundary between the troposphere and stratosphere, the tropopause plays a key role in regulating the entrance of air from the troposphere into the stratosphere and in controlling stratosphere-troposphere exchange. In the context of global warming, investigations of the climatological characteristics and trends of the tropopause are of particular interest. In this study, the long-term variability and trends of global tropopause characteristics from 1980 to 2021 are analyzed based on data derived from the ERA5, ERA-Interim, MERRA2, and NCEP reanalyses. We find a general increase in tropical tropopause geopotential height, which is on average about 0.05 km/decade$ during 1980-2021 for the WMO lapse rate tropopause and the cold point. Over the same time period, no significant trend in tropical tropopause temperature was detected in ERA5 and MERRA2. However, the tropical tropopause temperature experiences a decrease from 1980 to the early 21st century, then changes to an increasing trend (0.2 K/decade) from 2005 to 2021 in all reanalyses. Along with the increase of the tropical tropopause height, a widening of the tropics is observed from all reanalyses. The edges of the tropics are found to be extending poleward by about 0.2°/decade in the northern hemisphere and about 0.1°/decade in the southern hemisphere. Despite the multiple challenges involved in deriving the characteristics and trends of the tropopause from global reanalysis data, this study and our open data sets will help to better inform future assessments on stratosphere-troposphere exchange and chemistry and dynamics of the upper troposphere and lower stratosphere region.

 

How to cite: Zou, L. and Hoffmann, L.: Assessment of variability and trends of the tropopause from reanalyses data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2552, https://doi.org/10.5194/egusphere-egu23-2552, 2023.

EGU23-2643 | ECS | Orals | AS1.30

Model calculations of the contribution of tropospheric SO2 to the stratospheric aerosol layer 

Chiranjeevi Srinivasan Nalapalu, Ingo Wohltmann, Markus Rex, and Michael Höpfner

The stratospheric aerosol layer is important for stratospheric chemistry, climate change and in geo-engineering. Yet the processes governing the transport of sulfur to the stratosphere are poorly quantified. We present model calculations of the chemistry of sulfur dioxide (SO2) and its transport to the stratosphere and perform numerous sensitivity runs to assess the range of uncertainty of these calculations. The transport model is based on backward trajectories from the ATLAS model driven by ECMWF ERA 5. A simplified chemical box model constrained by CAMS data is used to calculate the SO2 chemistry. Sensitivity experiments explore the sensitivity to changes in OH, H2O2, DMS, cloud water, cloud pH value and in the driving analysis data. Input parameters were varied and their differences have been explored. The effect of El Nino and La Nina on SO2 transport was investigated. The SO2 reaching the stratosphere was quantified and the sources in the troposphere were determined. The model’s results were compared to POSIDON Aircraft measurements. 

How to cite: Nalapalu, C. S., Wohltmann, I., Rex, M., and Höpfner, M.: Model calculations of the contribution of tropospheric SO2 to the stratospheric aerosol layer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2643, https://doi.org/10.5194/egusphere-egu23-2643, 2023.

EGU23-2709 | ECS | Posters on site | AS1.30

Identification of source regions of the Asian Tropopause Aerosol Layer on the Indian subcontinent in August 2016 

Jan Clemens, Bärbel Vogel, Lars Hoffman, Sabine Griessbach, Nicole Thomas, Suvarna Fadnavis, Rolf Müller, Thomas Peter, and Felix Ploeger

The Asian tropopause aerosol layer (ATAL) is a distinct feature during the Asian summer monsoon season with an impact on the regional radiative balance of the Earth's atmosphere. However, the source regions and the detailed transport pathways of ATAL particles are still uncertain. In our study, we investigate transport pathways from different  regions at the model boundary (MB)  to the ATAL using the two Lagrangian transport models  CLaMS (Chemical Lagrangian Model of the Stratosphere) and MPTRAC (Massive-Parallel Trajectory Calculations), two reanalyses (ERA5 and ERA-Interim),  and balloon-borne measurements of the ATAL performed by the Compact Optical Backscatter Aerosol Detector (COBALD) above Nainital (India) in August 2016.  Trajectories are initialized at the location of the ATAL, as measured by COBALD in the Himalayas, and calculated 90 days backward in time to investigate the relation between the measured, daily averaged, aerosol backscatter ratio and different source regions at the MB. Nine source regions at the MB are distinguished, marking continental and maritime sources in the region of the Asian monsoon. Different simulation scenarios are performed, to find systematic differences as well as robust patterns, when the reanalysis data, the trajectory model, the vertical coordinate (kinematic and diabatic approach) or the convective parameterisation are varied.

While there are many robust features, the simulation scenarios also show some considerable differences between the air mass contributions of different source regions at the MB in the region of the Asian monsoon. The contribution to all air parcels from the MB varied between 5% and 40% for the Indo-Gangetic plain, the contribution from the Tibetan Plateau varied between 30% and 40% and contributions from oceans varied between 14% and 43% for different scenarios. However, the robust finding among all scenarios is that the largest continental air mass contributions originate from the Tibetan plateau and the India subcontinent (mostly the Indo-Gangetic plain), and largest maritime air mass contributions in Asia come from the Western Pacific (e.g. related to tropical cyclones such as typhoons).  Additionally, all simulation scenarios indicate that transport of maritime air from the Tropical Western Pacific to the region of the ATAL lowers the backscatter ratio (BSR) of the ATAL, while most scenarios indicate that transport of polluted air from the Indo-Gangetic plain increases the BSR. Therefore, while the results corroborate key findings from previous ERA-Interim based studies, they highlight the variability of the contributions of different MB regions to the ATAL depending on the meteorological input data, vertical velocities and in particular on the treatment of convection within the model calculations. 

 

How to cite: Clemens, J., Vogel, B., Hoffman, L., Griessbach, S., Thomas, N., Fadnavis, S., Müller, R., Peter, T., and Ploeger, F.: Identification of source regions of the Asian Tropopause Aerosol Layer on the Indian subcontinent in August 2016, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2709, https://doi.org/10.5194/egusphere-egu23-2709, 2023.

EGU23-2762 | ECS | Orals | AS1.30

Simulated mixing in the upper troposphere by small-scale turbulence 

Chun Hang Chau, Peter Hoor, and Holger Tost
Chemical composition in the upper troposphere/lower stratosphere (UTLS) plays an important role on the climate by affecting the radiation budget. Small-scale diabatic mixing like turbulence has a significant impact on the distribution of tracers which further affects the energy budget. Current models usually only have a higher resolution near the surface and a coarser resolution in the free atmosphere, which is too coarse to resolve the occurrence of small-scale turbulence in UTLS. In this work, we present enhanced vertical resolution (200 m in the UTLS) simulations focusing on the Scandinavian region using the state-of-the-art online coupled global/regional atmospheric chemistry model system MECO(n) (MESSy-fied ECHAM and COSMO models nested n times). We evaluated the basic meteorology (temperature and specific humidity) of the enhanced vertical resolution simulations with radiosonde data from the University of Wyoming and airborne in-situ measurements over northern Scandinavia. Additionally, we evaluated the ability of small-scale mixing in MECO(n) by comparing the model turbulence kinetic energy (TKE) with the calculated Ellrod Index and the impact of vertical diffusion in the COSMO instances in MECO(n) by releasing artificial passive tracer in the troposphere and stratosphere respectively. The results show that the enhanced vertical resolution simulations perform normally on basic meteorology. The simulations also show that the COSMO instances are able to resolve turbulence in UTLS with reasonable strength and the vertical diffusion in UTLS has a significant percentage impact on the tracer distribution.

How to cite: Chau, C. H., Hoor, P., and Tost, H.: Simulated mixing in the upper troposphere by small-scale turbulence, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2762, https://doi.org/10.5194/egusphere-egu23-2762, 2023.

EGU23-2828 | Orals | AS1.30

The 2022 Asian Summer Monsoon Transport and its Connection to the 2005-2021 Climatology as Illustrated by Carbon Monoxide 

Qing Liang, Huisheng Bian, Mian Chin, Laura Pan, Paul Newman, and Doug Kinnison

The Asian Summer Monsoon (ASM) provides one of the most effective transport pathways to deliver surface pollution into the stratosphere and impact stratospheric composition and climate. To better understand the impact of ASM, the Asian summer monsoon Chemical and Climate Impact Project (ACCLIP) took place in South Korea from July 29 – Sep 2, 2022.  During ACCLIP, in situ measurements of a wide range of trace gas, including carbon monoxide (CO), and aerosol species in the Upper Troposphere and Lower Stratosphere (UT/LS) were collected.

CO is a key pollutant emitted from anthropogenic emissions, as well as biogenic and biomass emissions, along with many other precursors for ozone and aerosol. In addition, its > 30-day atmospheric lifetime and linear chemical loss rate make it a key marker tracer for atmospheric pollution transport and ozone photochemistry. In this study, we use CO simulated by the NASA GEOS model to (1) analyze the ACCLIP-2022 observations, (2) examine surface-to-stratosphere transport in the Asian Summer Monsoon region during the summer of 2022, (3) assess how transport in 2022 is similar to or different from the 2005-2021 Climatology.  In addition, we use idealized tagged CO tracers that are used track pollution transport from a suite of source regions, e.g., within East Asia, South Asia, and Southeast Asia, to quantify the contribution of these target regions to CO and air mass abundance in the lower stratosphere over Asia and downwind regions.

How to cite: Liang, Q., Bian, H., Chin, M., Pan, L., Newman, P., and Kinnison, D.: The 2022 Asian Summer Monsoon Transport and its Connection to the 2005-2021 Climatology as Illustrated by Carbon Monoxide, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2828, https://doi.org/10.5194/egusphere-egu23-2828, 2023.

EGU23-2943 | ECS | Orals | AS1.30

An observational constraint on the uncertainty in stratospheric water vapour projections 

Peer Nowack, Paulo Ceppi, Sean Davis, Gabriel Chiodo, Will Ball, Mohamadou A. Diallo, Birgit Hassler, Yue Jia, James Keeble, and Manoj Joshi

Future increases in stratospheric water vapour (SWV) risk amplifying climate change and slowing down the recovery of the ozone layer. However, state-of-the-art climate models strongly disagree on the magnitude of these increases under global warming1,2. Uncertainty primarily arises from the challenges inherent in modelling the many complex processes leading to dehydration of air during its tropical ascent into the stratosphere3. Here we derive an observational constraint on this longstanding uncertainty factor in Earth's climate change response. Following a statistical learning approach4,5, we infer historical co-variations between the UTLS temperature structure and tropical lower SWV concentrations. For climate models, we demonstrate that these historically constrained relationships are also highly predictive of the SWV response under strong 4xCO2 forcing. By extension, we obtain an observationally constrained range for concentration changes per degree of global warming of 0.31±0.39 ppmv K-1 (90% confidence interval). Our constraint represents a 50% decrease in the 95th percentile of the climate model uncertainty distribution, which has major implications for surface warming, ozone recovery, and the tropospheric circulation response under climate change.

Across 61 climate models from the 5th and 6th phases of the Coupled Model Intercomparison Project (CMIP), we therefore find that a large fraction of future model projections is inconsistent with observational evidence. In particular, frequently projected strong increases (>1 ppmv K-1) are highly unlikely. We further demonstrate that our constraint on tropical lower SWV can be translated into also reduced uncertainty in the radiative SWV feedback (by 0.05 W m-2 K-1). This uncertainty reduction is comparable in size to the overall feedback responses in biogenic volatile organic compounds (BVOCs) or ozone6, and is thus of great relevance for policymakers.

References:

[1] Gettelman, A. et al. Multimodel assessment of the upper troposphere and lower stratosphere: Tropics and global trends. Journal of Geophysical Research 115, D00M08 (2010), https://doi.org/10.1029/2009JD013638.

[2] Keeble, J. et al. Evaluating stratospheric ozone and water vapour changes in CMIP6 models from 1850 to 2100. Atmospheric Chemistry and Physics 21, 5015–5061 (2021), https://doi.org/10.5194/acp-21-5015-2021.

[3] Fueglistaler, S. et al. Tropical tropopause layer. Reviews of Geophysics 47, RG1004 (2009), https://doi.org/10.1029/2008RG000267.

[4] Ceppi, P. and Nowack, P. Observational evidence that cloud feedback amplifies global warming. PNAS 118, e2026290118 (2021), https://doi.org/10.1073/pnas.2026290118.

[5] Nowack, P. et al. Using machine learning to build temperature-based ozone parameterizations for climate sensitivity simulations. Environmental Research Letters 13, 104016 (2018), https://doi.org/10.1088/1748-9326/aae2be.

[6] Szopa, S. et al. Short-lived climate forcers. In Climate Change 2021: The Physical Science Basis. Contribution of Working Group I to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change, Cambridge University Press, Cambridge, UK and New York, USA, 817–922 (2021).

 

How to cite: Nowack, P., Ceppi, P., Davis, S., Chiodo, G., Ball, W., Diallo, M. A., Hassler, B., Jia, Y., Keeble, J., and Joshi, M.: An observational constraint on the uncertainty in stratospheric water vapour projections, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2943, https://doi.org/10.5194/egusphere-egu23-2943, 2023.

EGU23-2948 | Orals | AS1.30 | Highlight

The Dynamical Background to the 2022 Asian Summer Monsoon Chemical and Climate Impacts Project (ACCLIP) 

Paul A. Newman, Laura Pan, Atlas Elliot, Randel William, Troy Thornberry, Owen Brian Toon, Rei Ueyama, Leslie Lait, and Eric Nash

The Asian summer monsoon Chemical and Climate Impact Project (ACCLIP) used the NSF/NCAR Gulfstream V (GV) research aircraft, the NASA WB-57f research aircraft, the Korean NARA King Air, and a broad set of balloon launches to investigate atmospheric processes that influence ozone depletion and climate in the Korea/Japan region.  The WB-57 and NSF GV part of the field campaign was flown from Osan Air Base, Republic of Korea during the July-August 2022 period.

This presentation will show some of the dynamical and transport aspects of the Asian summer monsoon anti-cyclone (ASMA) during the summer of 2022. In particular, the strength and flow aspects of the ASMA will be illustrated and shown in the context of an ASMA MERRA-2 climatology. Flight overviews against this flow field will be compared against detrainment events from the ASMA from Asia into the Pacific Ocean. Flight profiles will also show how ACCLIP made extensive sampling of the ASMA’s eastern flank – mapping of the vertical and horizontal structure in the upper troposphere and lower stratosphere.

How to cite: Newman, P. A., Pan, L., Elliot, A., William, R., Thornberry, T., Toon, O. B., Ueyama, R., Lait, L., and Nash, E.: The Dynamical Background to the 2022 Asian Summer Monsoon Chemical and Climate Impacts Project (ACCLIP), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2948, https://doi.org/10.5194/egusphere-egu23-2948, 2023.

EGU23-3280 | ECS | Orals | AS1.30

Gravity Waves in the Tropical UTLS: New Insights from Aeolus Wind Profiling Data 

Mathieu Ratynski, Sergey Khaykin, Alain Hauchecorne, and Joan Alexander

The European Space Agency's Aeolus satellite mission, launched in 2018, provides global wind profiling using a Doppler lidar instrument ALADIN. In this study, we examined ALADIN’s ability to capture and resolve internal gravity waves (IGWs) in the upper troposphere and lower stratosphere (UTLS). To derive the IGW-induced perturbations in the vertical profiles of ALADIN’s horizontal line-of-sight (HLOS) quasi-zonal wind velocity at ~1 km vertical resolution, we subtract the Aeolus-derived "background" wind profiles from the individual measurements. Through a spectral analysis of these data, we then derive the IGW kinetic energy and dominant vertical wavelength in the UTLS over the entire Aeolus mission lifespan. 

  This study represents the first attempt to reconstruct the global distribution of IGW activity using the global wind information exclusively provided by the Aeolus mission. The analysis reveals the well-known IGW sources such as orography, polar vortex dynamics and tropical convection. Here we focus on the tropical UTLS region, where ALADIN has an extended stratospheric coverage. The analysis reveals a previously undocumented spot of enhanced IGW activity in the UTLS, recurring above the Indian Ocean during Boreal Summer. The IGW activity spot is shown to slowly migrate from eastern Africa to the Pacific maritime continent during the June-December period. 

  The Aeolus-derived distribution and seasonal variation of IGW activity were cross-validated using the global temperature profiling by EUMETSAT radio-occultation (RO) satellites. The RO data were resampled to ALADIN resolution and spectrally analyzed in the same way as it was done for ALADIN wind data. The derived IGW potential energy data confirm the seasonal/zonal variation of IGW activity observed by ALADIN, in particular the eastward migration of the IGW activity hotspot, presumably linked to convection within the MJO (Madden-Julian Oscillation). The results suggest that the interannual variation of the IGW kinetic and potential energies in the UTLS is modulated by the Quasi-Biennial Oscillation, whereas the MJO-related waves can be characterized by shorter vertical wavelengths. 

  Another important finding enabled by the joint analysis of the Aeolus wind and RO temperature data is the evidence for a strong IGW generation by the Smoke-Charged Vortex (SCV) produced by the 2019/20 Australian megafires. Overall, with this study we point out the potential of Aeolus wind profiling to improve our understanding of atmospheric dynamics, particularly in the UTLS region.

How to cite: Ratynski, M., Khaykin, S., Hauchecorne, A., and Alexander, J.: Gravity Waves in the Tropical UTLS: New Insights from Aeolus Wind Profiling Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3280, https://doi.org/10.5194/egusphere-egu23-3280, 2023.

The tropical tropopause layer (TTL) is a sea of vertical motions. Convectively-generated gravity waves create vertical winds on scales of a few to 1000s of kilometers as they propagate in a stable atmosphere. Turbulence from gravity wave breaking, radiatively-driven convection and Kelvin-Helmholtz instabilities stirs up the TTL on the kilometer scale. TTL cirrus, which moderate the water vapor concentration in the TTL and stratosphere, form in the cold phases of large-scale (> 100 km) wave activity. It has been proposed in several modelling studies that small-scale (< 100 km) vertical motions control the ice crystal number concentration (NI) and the dehydration efficiency of TTL cirrus. Here, we present the first observational evidence for this.

We use 20 Hz data from the National Aeronautics and Space Administration (NASA) Airborne Tropical TRopopause Experiment (ATTREX) campaign to quantify small-scale vertical wind variability in the TTL and examine its influence on TTL cirrus microphysics. We develop an algorithm to classify turbulence, and long wavelength (5 km < λ < 100 km) and short wavelength (λ < 5 km) gravity wave activity, during level flight legs of at least 100 km. The most commonly sampled conditions are: 1) a quiescent atmosphere with negligible small-scale vertical wind variability, 2) long wavelength gravity wave activity (LWGWA), and 3) LWGWA with turbulence. Turbulence rarely occurs in the absence of gravity wave activity. Cirrus with NI exceeding 10 per liter are rare in a quiescent atmosphere, but about 25 times more likely when there is gravity wave activity and 50 times more likely when there is also turbulence, confirming the results of the aforementioned modeling studies.

Our observational analysis shows that small-scale gravity waves strongly influence NI within TTL cirrus. Global storm-resolving models have recently been run with horizontal grid spacings between 1 and 10 km, sufficient to resolve some small-scale gravity wave activity. We use ATTREX observations to evaluate simulated small-scale (10-100 km) vertical wind power spectra from four global-storm resolving simulations from DYnamics of the Atmospheric general circulation Modeled On Non-hydrostatic Domains (DYAMOND) that have horizontal grid spacings of 3–5 km. We find that all four models have too little resolved vertical wind at horizontal wavelengths less than 100 km, although the bias is much less pronounced in global SAM than in the other models. We expect that deficient small-scale gravity wave activity significantly limits the realism of simulated ice microphysics in these models.

How to cite: Atlas, R. and Bretherton, C.: Aircraft observations of gravity wave activity and turbulence in the tropical tropopause layer: prevalence, influence on cirrus and comparison with global-storm resolving models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3442, https://doi.org/10.5194/egusphere-egu23-3442, 2023.

EGU23-3544 | Orals | AS1.30

Massive ozone production from South American wild fires observed during SOUTHTRAC 

Peter Hoor, Daniel Kunkel, Lachnitt Hans-Christoph, Bozem Heiko, Bense Vera, Smoydzin Linda, Riese Martin, Zahn Andreas, and Ziereis Helmut

During the SOUTHTRAC mission, which took place in September and November 2019, the German
research aircraft HALO performed several cross sections from the equator to the southern tip of
south America. The flight legs were flown along the coast of Brazil at typical altitudes of 13-14 km.
During the northbound flight on October, 7th 2019 massive enhancements of pollutants were
observed at these altitudes. Notably, in-situ observations show continuously elevated CO values
exceeding 200 ppbv over a flight distance of more than 1000 km. These massive enhancements were
accompanied by strongly elevated NO and NOy as well as CO2 and could be attributed to the large fires
in South America during this time. These fires occurred in conjunction with convection over
Argentina and Brazil, which led to efficient vertical transport. Lagrangian and chemical model analysis
confirmed the potential impact of convection and biomass burning to the observed enhancements of
ozone and pollutants.
Comparing the tracer observations to previous flights in exactly the same region three weeks earlier,
we could estimate the ozone production due to the biomass burning. We
estimate an ozone production in the polluted air masses of almost 30%
of the observed ozone mixing ratio. Given the large extent of the polluted area over 15 degrees of
latitude this may have an impact on the local energy budget of the tropopause region.

How to cite: Hoor, P., Kunkel, D., Hans-Christoph, L., Heiko, B., Vera, B., Linda, S., Martin, R., Andreas, Z., and Helmut, Z.: Massive ozone production from South American wild fires observed during SOUTHTRAC, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3544, https://doi.org/10.5194/egusphere-egu23-3544, 2023.

EGU23-3654 | Orals | AS1.30 | Highlight

Highlights of the ACCLIP Campaign 2022: Operations and Science 

Laura Pan, Paul Newman, Elliot Atlas, Troy Thornberry, Bill Randel, and Brian Toon

The Asian summer monsoon Chemical and Climate Impacts Project (ACCLIP) is a large airborne field campaign conducted over the Western Pacific in summer 2022. The campaign deployed two research aircraft, the NCAR Gulfstream V (GV) and the NASA WB-57, both with extensive payload of chemistry and microphysics measurements for trace gas and aerosol content to investigate the Asian monsoon convective outflow at the UTLS levels. The campaign also included ground-based balloon soundings and extensive collaborative measurements in the region. Based from Osan, Republic of Korea, a total of 29 research fights were conducted covering the vertical range of 300 ft above sea level to ~70 hPa over a large domain of western Pacific (15°N-43°N, 125°E-155°). These measurements provide novel information on the role of Asian summer monsoon in altering atmospheric composition, serving as a distinct linkage between the weather and the climate through its impact on ozone chemistry and aerosol radiative effect. Observational highlights and initial indications of post campaign data analysis and modeling will be presented in this overview.

How to cite: Pan, L., Newman, P., Atlas, E., Thornberry, T., Randel, B., and Toon, B.: Highlights of the ACCLIP Campaign 2022: Operations and Science, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3654, https://doi.org/10.5194/egusphere-egu23-3654, 2023.

EGU23-3674 | ECS | Orals | AS1.30

Revisiting the stratospheric ozone response to global warming 

Aaron Match and Edwin Gerber

In response to global warming, ozone is predicted to increase aloft due to stratospheric cooling but decrease in the tropical lower stratosphere. The ozone reductions have been primarily attributed to a strengthening Brewer-Dobson circulation, which upwells ozone-poor air. Yet, we find that strengthening upwelling only explains part of the reduction. The reduction is also driven by tropospheric expansion under global warming, which erodes the ozone layer from below, the low ozone anomalies from which are advected upwards. Strengthening upwelling and tropospheric expansion are correlated under global warming, making it challenging to disentangle their relative contributions. Therefore, chemistry-climate model output is used to validate an idealized model of ozone photochemistry and transport with a tropopause lower boundary condition. In our idealized decomposition, strengthening upwelling and tropospheric expansion both contribute at leading order to reducing tropical ozone. Tropospheric expansion leads to an upward shift in the tropospheric destruction of ozone—not to an upward shift in ozone itself—implying that tropopause-following coordinates do not generally remove the effects of tropospheric expansion on ozone.

How to cite: Match, A. and Gerber, E.: Revisiting the stratospheric ozone response to global warming, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3674, https://doi.org/10.5194/egusphere-egu23-3674, 2023.

EGU23-4153 | ECS | Posters virtual | AS1.30

The stratosphere–troposphere exchange process during typhoon Molave (2020) 

Shujie Chang and Dong Huang

Typhoon is a significant source of deep convection which plays an important role in stratosphere–troposphere exchange (STE) in the Northwest Pacific Ocean. In this study, Typhoon Molave (2020) was simulated by using the Weather Research and Forecasting model (WRF) to examine the STE process and its detailed characteristics compared with the results from ERA5. The geopotential heights and wind field indicate existence of gravity waves (GWs) which transport large amounts of energy through the atmosphere. GWs also allow airmass exchanges between stratosphere and troposphere. A joint analysis of driving field reveals strong linkage between GWs and ozone variations over the region. A significant increasing response of the upper troposphere and lower stratosphere (UTLS) ozone to the gravity wave in areas near the typhoon path. The GW activity caused by typhoon Molave leads to turbulent flow, the mixing of momentum and air mass.

How to cite: Chang, S. and Huang, D.: The stratosphere–troposphere exchange process during typhoon Molave (2020), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4153, https://doi.org/10.5194/egusphere-egu23-4153, 2023.

EGU23-4449 | Orals | AS1.30

Impact of convection on trace gas composition during the summer monsoon season downwind of East Asia and over central North America 

Elliot Atlas, Kate Smith, Victoria Treadaway, Sue Schauffler, Roger Hendershot, Richard Lueb, Stephen Donnelly, Leslie Pope, Laura Pan, Troy Thornberry, Paul Newman, and Ken Bowman and the ACCLIP and DCOTSS Science Teams

Airborne research missions were conducted during the summer season over the Western Pacific downwind of the Asian summer monsoon (ACCLIP, Asian Summer Monsoon Chemical & CLimate Impact Project, Aug/Sept., 2022) and over central N. America (DCOTSS: Dynamics and Chemistry Of The Summer Stratosphere, July/Aug., 2021 and May/July, 2022).  A major objective of both of these missions was to characterize the impact of convective transport of trace gases on regional and hemispheric air quality and on ozone chemistry in the UT/LS.  The DCOTSS campaign focused on outflow from overshooting convection, and ACCLIP targeted outflow and eddy-shedding from the Asian summer monsoon anticyclone.  Whole air samples were collected from the three aircraft deployed during the missions (NSF GV, NASA WB-57, and NASA ER2), and a wide range of organic trace gases were measured that included NMHC, long and short-lived halocarbons and organic nitrates.   In-situ measurements of ozone and other trace gases were also included in the airborne instrument payloads.  Both campaigns showed cases of tropospheric transport into UT/LS region, with significantly larger amounts of certain trace gases (e.g., dichloromethane and others) found in the ACCLIP region.  This presentation will provide an overview of selected trace gas distributions and correlations from these campaigns to illustrate the role of the different monsoon regions on the chemistry of the UT/LS.

How to cite: Atlas, E., Smith, K., Treadaway, V., Schauffler, S., Hendershot, R., Lueb, R., Donnelly, S., Pope, L., Pan, L., Thornberry, T., Newman, P., and Bowman, K. and the ACCLIP and DCOTSS Science Teams: Impact of convection on trace gas composition during the summer monsoon season downwind of East Asia and over central North America, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4449, https://doi.org/10.5194/egusphere-egu23-4449, 2023.

EGU23-4532 | ECS | Posters on site | AS1.30

Impact of reduced aircraft emission on HOx Chemistry in the upper troposphere during BLUESKY Campaign 2020. 

Sreedev Sreekumar, Anywhere Tsokankunku, Daniel Marno, Roland Rohloff, Monica Martinez, Ivan Tadic, Zaneta Hamryszczak, Andrea Pozzer, Joachim Curtius, Horst Fischer, Birger Bohn, Florian Obersteiner, Jos Lelieveld, and Hartwig Harder

Hydroxyl radicals are the most predominant daytime initiator for atmospheric oxidation processes. Due to the COVID -19 pandemic, there was a considerable reduction in emissions from industry and all means of transportation during spring 2020. The main objective of the BLUESKY campaign is to understand the effect of these reduced emissions on atmospheric composition such as trace gases, aerosols, and cloud properties. OH and HO2 were measured with HORUS (HydrOxyl Radical measurement Unit based on fluorescence Spectroscopy), during eight research flights from the boundary layer up to 14 km.  Here we present the impact of reduced aircraft emissions and the meteorological situation on the HOx Chemistry in the upper troposphere over Europe during the COVID-19 lockdown. We contrast the findings during BLUESKY with results from previous campaigns and analyze the occurrence of HOx during daytime in the outflow of electrified and non-electrified convective systems.

How to cite: Sreekumar, S., Tsokankunku, A., Marno, D., Rohloff, R., Martinez, M., Tadic, I., Hamryszczak, Z., Pozzer, A., Curtius, J., Fischer, H., Bohn, B., Obersteiner, F., Lelieveld, J., and Harder, H.: Impact of reduced aircraft emission on HOx Chemistry in the upper troposphere during BLUESKY Campaign 2020., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4532, https://doi.org/10.5194/egusphere-egu23-4532, 2023.

EGU23-4565 | Orals | AS1.30

What does IASI see during the Asian Summer Monsoon over the west Pacific? 

Anne Boynard, Camille Viatte, Selviga Sinnathamby, Sarah Safieddine, Laura Pan, Shawn Honomichl, Warren Smith, Qing Liang, and Cathy Clerbaux

Several studies have found that the summertime Asian Summer Monsoon (ASM) anticyclone is linked to a persistent enhancement of carbon monoxide (CO) concentrations in the Upper Troposphere and Lower Stratosphere (UTLS).

In this study, more than 15 years (2008-2022) of satellite observations from Eumetsat’s Infrared Atmospheric Sounding Interferometer (IASI) are used to investigate the interannual, seasonal and sub-seasonal variability of CO in the UTLS during the ASM. To assess the ability of IASI CO data to characterize the UTLS monsoon circulation, we focus on the Asian Summer Monsoon Chemical & CLimate Impact Project (ACCLIP) campaign that took place in summer 2022 in Korea. Several case studies associated with the presence of eddy shedding features are presented. Simulations from the Goddard Earth Observing System (GEOS) model performed during the ACCLIP campaign period are also used to support the IASI data analysis and interpretation.

How to cite: Boynard, A., Viatte, C., Sinnathamby, S., Safieddine, S., Pan, L., Honomichl, S., Smith, W., Liang, Q., and Clerbaux, C.: What does IASI see during the Asian Summer Monsoon over the west Pacific?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4565, https://doi.org/10.5194/egusphere-egu23-4565, 2023.

EGU23-5894 | ECS | Posters on site | AS1.30

Measurements of nitrous acid (HONO), hydroxyl (OH), nitric oxide (NO), hydroperoxyl (HO2), and nitrogen dioxide (NO2) in the upper troposphere: is peroxynitrous acid (HOONO) a missing source of HONO? 

Benjamin Weyland, Flora Kluge, Klaus Pfeilsticker, Roland Rohloff, Hartwig Harder, Ivan Tadic, Horst Fischer, Raphael Doerich, John Crowley, Birger Bohn, Domenico Taraborrelli, Simon Rosanka, and Florian Obersteiner

Discrepancies between expected and observed NO-NO2 ratios in the upper troposphere suggest the presence of an unknown NOX reservoir. We report on airborne remote sensing limb observations from the mini-DOAS instrument on board the HALO (High Altitude Long Range) aircraft during the CAFÉ-Africa (Chemistry of the Atmosphere Field Experiment) campaign in 2018. Nitrous acid (HONO) slant column densities in limb scattered sunlight in the ultraviolet wavelength range retrieved by DOAS (Differential Optical Absorption Spectroscopy) are converted to volume mixing ratios using the O3 / O4 scaling method. Over the tropical Atlantic Ocean, in the cold upper troposphere, HONO is found in excess of what may be expected from known gas phase formation mechanisms or is predicted by the ECHAM/MESSy Atmospheric Chemistry (EMAC) model. At these altitudes (10-15 km), heterogeneous sources of the excess HONO are inefficient and thus unlikely. Therefore, we investigate the possibility of a gas phase HONO source, namely the oxidation of peroxynitrous acid (HOONO) formed in the reactions NO + HO2 and OH + NO2. Since there are no reported atmospheric measurements of HOONO, we use complementary, simultaneous in situ measurements of OH, NO, HO2, NO2, O3 and photolysis frequencies from onboard HALO to make steady state arguments and quantify reaction rate coefficients for both formation pathways and destruction of HOONO by O3, OH, and NO, the last of which may form HONO and NO2.

How to cite: Weyland, B., Kluge, F., Pfeilsticker, K., Rohloff, R., Harder, H., Tadic, I., Fischer, H., Doerich, R., Crowley, J., Bohn, B., Taraborrelli, D., Rosanka, S., and Obersteiner, F.: Measurements of nitrous acid (HONO), hydroxyl (OH), nitric oxide (NO), hydroperoxyl (HO2), and nitrogen dioxide (NO2) in the upper troposphere: is peroxynitrous acid (HOONO) a missing source of HONO?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5894, https://doi.org/10.5194/egusphere-egu23-5894, 2023.

EGU23-6021 | Orals | AS1.30 | Highlight

Self-lofting and dynamical confinement of the Raikoke volcanic plume 

Sergey Khaykin, A.T. Jos de Laat, Sophie Godin-Beekmann, Alain Hauchecorne, and Mathieu Ratynski

Recent research has provided evidence of the self-lofting capacity of smoke aerosols in the stratosphere and their self-confinement by persistent anticyclones (Smoke-Charged Vortices, SCV), prolonging the atmospheric residence time and radiative effects of wildfire emissions. By contrast, the volcanic aerosols - composed mostly of non-absorptive sulphuric acid droplets – were never reported to be subject of dynamical confinement. In this study, we use high-resolution satellite observations from various satellite instruments (TROPOMI, ALADIN, CALIPSO, OMPS-LP and EUMETSAT GNSS-RO) together with high-resolution ECMWF ERA5 reanalysis and meteorological radiosoundings to show that the eruption of Raikoke volcano in June 2019 produced a long-lived stratospheric anticyclone termed Vorticized Volcanic Plume (VVP). The primary VVP structure contained 24% of the total erupted mass of sulphur dioxide, circumnavigated the globe three times, and ascended diabatically by more than 13 km in three months through radiative heating of the confined aerosol plume. We argue that persistent anticyclonic formations act to maintain the volcanic plumes at high concentration thereby providing a high degree of radiative heating and upward thrust to volcanic plumes.

The mechanism of dynamical confinement has important implications for the planetary-scale transport of volcanic emissions, their stratospheric residence time, and atmospheric radiation balance. It also provides a challenge or “out of sample test” for weather and climate models that should be capable of reproducing such dynamical structures.

How to cite: Khaykin, S., de Laat, A. T. J., Godin-Beekmann, S., Hauchecorne, A., and Ratynski, M.: Self-lofting and dynamical confinement of the Raikoke volcanic plume, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6021, https://doi.org/10.5194/egusphere-egu23-6021, 2023.

EGU23-6439 | ECS | Orals | AS1.30

3D climatology of ice supersaturated regions over the North Atlantic 

Nils Brast, Yun Li, Susanne Rohs, Patrick Konjari, Christian Rolf, Martina Krämer, Andreas Petzold, Peter Spichtinger, and Philipp Reutter

Water vapor is an essential component for regulating the Earth's radiation budget. To realistically determine the global radiation budget, an accurate description of the water vapor distribution in the upper troposphere and lower stratosphere (UTLS) is therefore indispensable. For example, small changes in water vapor concentration can lead to significant changes in local radiative forcing, especially in the dry lower stratosphere. The change in this region can be even stronger if condensed water in the form of ice clouds is present instead of solely water vapor.

The formation and evolution of ice clouds is crucially determined by the saturation ratio over ice (Si). Ice crystals can only form (and grow) at supersaturated conditions (i.e. Si>1), i.e. in so-called ice supersaturated regions (ISSRs), which also constitute potential regions for the formation and existence of persistent aircraft contrails. Knowing and precisely forecasting the occurrence of ISSRs can help reducing the contribution of aviation to man-made climate change, as contrails usually have a warming effect on the climate.

Ice supersaturation is often observed in the UTLS. However, despite their importance, the large-scale three-dimensional structure of ISSRs is widely unknown. Therefore, we present a three-dimensional climatology of ice supersaturation in the UTLS over the North Atlantic for the years 2010 to 2019. This climatology is based on the recent ERA5 reanalysis data set of the European Center for Medium Weather Forecast (ECMWF), which explicitly allows ice supersaturation in cloud-free conditions. To quantify the quality of the ERA5 data set with respect to ice supersaturation, we use the long-term in-situ measurements of the European Research Infrastructure ’In-service Aircraft for a Global Observing System’ (IAGOS; www.iagos.org) (Petzold et al., 2015).

How to cite: Brast, N., Li, Y., Rohs, S., Konjari, P., Rolf, C., Krämer, M., Petzold, A., Spichtinger, P., and Reutter, P.: 3D climatology of ice supersaturated regions over the North Atlantic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6439, https://doi.org/10.5194/egusphere-egu23-6439, 2023.

EGU23-6586 | Posters on site | AS1.30

Tropopause inversion layer and its correlation with relative humidity 

Philipp Reutter, Daniel Köhler, and Peter Spichtinger

To better understand our climate and weather system, knowledge of the processes in the upper troposphere and lower stratosphere (UTLS) is crucial.

An important element in the UTLS region is the tropopause inversion layer (TIL). The TIL is a region of extraordinarily high or overshooting static stability just above the tropopause. Since its discovery, a couple of hypothesis were developed to explain the origin and formation of the TIL. In addition to dynamic mechanisms, such as baroclinic waves, a radiative forcing mechanism is considered, where ozone and water vapor are contributing to the TIL formation and persistence.

To investigate the latter mechanism further, we examine the correlation between the relative humidity with respect to ice, as a measure for water vapor in the UTLS region, and the TIL.

Based on high-resolution radiosonde data of the German Weather Service (DWD) from 2011 to 2019, we are investigating how TIL properties such as the height, strength or thickness of the TIL layer change with temperature and relative humidity over ice. We also investigate seasonal differences of the above-mentioned properties. Furthermore, the results are also compared with ERA5 reanalysis data. We can show that ERA5 can reproduce relevant properties of the TIL as compared to the radiosondes. Thus, ERA5 data can be used for extending the investigations to other geographical locations.

How to cite: Reutter, P., Köhler, D., and Spichtinger, P.: Tropopause inversion layer and its correlation with relative humidity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6586, https://doi.org/10.5194/egusphere-egu23-6586, 2023.

EGU23-6859 | Posters on site | AS1.30

SAGE III/ISS v5.3 Level 2 Data Product Changes and Improvements 

Carter Hulsey, Michael Pitts, David Flittner, Robert Damadeo, Robbie Manion, and Marsha Larosse

The Stratospheric Aerosol and Gas Experiment on the International Space Station (SAGE III/ISS) is an occultation instrument that acquires measurements of aerosols and gases within the Earth’s stratosphere and upper troposphere. SAGE III/ISS provides level 2 solar species products for aerosol extinction (9 channels), nitrogen dioxide (NO2), ozone (O3), and water vapor (H2O). The level 2 products currently provide three O3 profiles based on differing retrievals. The first O3 profile is based on measurements at short wavelengths within the Hartley-Huggins band (MesO3), the second O3 profile is based on measurements made at visible wavelengths within the Chappius band (MLR O3), and the final profile is found using a more SAGE II like approach (AO3). The SAGE III/ISS also provides level 2 lunar species products for ozone (O3), nitrogen dioxide (NO2), and nitrogen trioxide (NO3).

 

Version 5.3 of the SAGE III/ISS retrieval algorithm introduces improvements that affect the level 2 data products. The largest change to the solar algorithm is the implementation of disturbance monitoring package (DMP) corrections to improve pointing accuracy. The DMP is comprised of a miniature inertial measurement unit that measures rotation in inertial space using ring laser gyroscopes oriented about three orthogonal axes which can be used to correct pointing errors caused by mechanical disturbances. A major change common to solar and lunar algorithms is meteorological input from the coarser 42 level Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2) model data to the 72 level MERRA-2 model data. The final major change involves improving the automated quality assurance (QA) algorithm to recover events that were withheld from the public release because differences between the AO3 and MLR O3 for some events after the eruption of Tonga–Hunga Haʻapai. Other changes for v5.3 include minor bug fixes as well as restoration of some data quality flags that were removed in v5.21. This presentation presents the impacts of these changes as well as overall observations of interest from v5.3 level 2 data products.

How to cite: Hulsey, C., Pitts, M., Flittner, D., Damadeo, R., Manion, R., and Larosse, M.: SAGE III/ISS v5.3 Level 2 Data Product Changes and Improvements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6859, https://doi.org/10.5194/egusphere-egu23-6859, 2023.

EGU23-7965 | Posters on site | AS1.30

Organic trace gases collected using the Whole Air Sampler over North America (summer 2021, 2022), in the UTLS region, targeting deep convective regions 

Katie Smith, Elliot Atlas, Paul Bui, Bruce Daube, Stephen Donnelly, Fred Moore, Bradley Hall, Eric Hintsa, Roger Hendershot, Rich Lueb, Jasna Pittman, Leslie Pope, Sue Schauffler, Jessica Smith, Victoria Treadaway, and Steven Wofsy

Whole Air Samples (WAS) were collected as part of the Dynamics and Chemistry of the Summer Stratosphere (DCOTSS) field campaign in the Upper Troposphere-Lower Stratosphere (UTLS) region during Summer 2021 and 2022. Grid-Rad and satellite imagery were used to identify regions of overshooting convection, and areas with outflow from the overshooting were targeted by the DCOTSS aircraft using trajectory models and in-situ measurements. Because a wide range of trace gases with different atmospheric lifetimes and sources are measured, WAS can provide insight into the processes that influence trace gas composition of the UTLS over North America. We investigate the tropospheric tracer relationships within and around these deep convective regions to determine the extent of penetration of tropospheric gases into the lower stratosphere (LS). Compounds such as ethane and ethyne with short (< 6 months) tropospheric lifetimes do not reach the LS without rapid transport from deep convection, and we observe cases where these gases are elevated above stratospheric background, typically well correlated with other tropospheric tracers (e.g. CO).  However, the relationship between enhanced water vapor from overshooting convection and tropospheric tracers is more complex. Further, we show that ratios between different trace gas species can help identify and distinguish air mass types (e.g., biomass burning, oil and gas production, urban influence, etc.). Finally, we determine the Cl- and Br- halogen budgets for 2021 and 2022 stratosphere over N. America and the contribution of very-short-lived organic halogen species.

How to cite: Smith, K., Atlas, E., Bui, P., Daube, B., Donnelly, S., Moore, F., Hall, B., Hintsa, E., Hendershot, R., Lueb, R., Pittman, J., Pope, L., Schauffler, S., Smith, J., Treadaway, V., and Wofsy, S.: Organic trace gases collected using the Whole Air Sampler over North America (summer 2021, 2022), in the UTLS region, targeting deep convective regions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7965, https://doi.org/10.5194/egusphere-egu23-7965, 2023.

EGU23-7973 | ECS | Orals | AS1.30

Balloon-borne in situ profiles of aerosol, water vapor, and ozone within the Asian summer monsoon anticyclone during the ACCLIP 2022 

J. Douglas Goetz, Lars Kalnajs, Joowan Kim, Matthew Norgren, Bruce Kindel, Hyeong-Gyu Kim, and Hyungyu Kang

Balloon soundings within the Asian summer monsoon anticyclone (ASMA) were conducted from Osan, South Korea as part of the Asian Summer Monsoon Chemical and Climate Impact Project (ACCLIP) in August of 2022. Over 30 soundings in 12 days were accomplished with high resolution co-located in situ profiles of aerosol size distributions, water vapor, ozone, and state parameters from the surface to the lower stratosphere. Aerosol measurements included accumulation mode particle size and number concentrations with Printed Optical Particle Spectrometers (POPS), coarse mode measurements with LASP Optical Particle Counters (LOPC), and total aerosol between 20 nm and 10 µm with Stratospheric Total Aerosol Counters (STAC). The aerosol sondes observed a pervasive Asian Tropopause Aerosol Layer (ATAL) and temperature dependent microphysical trends that are consistent with the location of the cold-point tropopause and lapse rate minimum. Simultaneous flights with cryogenic frostpoint hygrometers (EN-SCI CFH) and ozonesondes (EN-SCI ECC) provided context on the UTLS mixing processes in the ASMA through tracer-tracer relationships. Model reanalysis products suggest that the soundings were within the ASMA domain and back trajectories indicate sampling of fresh and aged airmasses within the UTLS transported from the ASMA circulation. These measurements add to the limited record of aerosol and water vapor observations of the Asian UTLS during the summer monsoon and provide an understanding of the ATAL that can only be gathered from continuous vertical profiles.

 

How to cite: Goetz, J. D., Kalnajs, L., Kim, J., Norgren, M., Kindel, B., Kim, H.-G., and Kang, H.: Balloon-borne in situ profiles of aerosol, water vapor, and ozone within the Asian summer monsoon anticyclone during the ACCLIP 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7973, https://doi.org/10.5194/egusphere-egu23-7973, 2023.

EGU23-8021 | Orals | AS1.30

A long way of water vapor from the Asian Summer Monsoon into the stratosphere 

Paul Konopka, Christian Rolf, Marc von Hobe, Sergey M. Khaykin, Benjamin Clouser, Elizabeth Moyer, Fabrizio Ravegnani, Silvia Viciani, Armin Afchine, Martina Krämer, Fred Stroh, and Felix Ploeger

During the StraoClim Geophysica campaign, moist air with total water mixing ratios up to 200 ppmv was observed within the Asian Summer Monsoon anticyclone, above the local cold point tropopause (CPT). High ozone mixing ratios of up to 250 ppbv suggest substantial stratospheric moistening. We used 60-day back- and forward trajectories to classify the observations into two groups based on their distance to the Lagrangian dry point (LDP): those where the LDP has just occurred or is still expected to occur (type A, 0-3 days from LDP), and those where the LDP was passed 15-35 days before (type B). We applied a microphysical box model (CLaMS-Ice) and a simple freeze drying model (FDM) to simulate the evolution of ice mixing ratios along the trajectories. Type A air masses, with ice mixing ratios larger than 1 ppm, underwent multiple transitions between the solid and gas phase, in good agreement with CALIPSO ice and MLS water vapor observations of around 5 ppm. In contrast, type B air masses showed less agreement with CALIPSO ice and significantly overestimated MLS observations when CLaMS-Ice or FDM were applied. However, water vapor reconstructed from the LDP of the merged back- and forward trajectories agreed much better with MLS, indicating that the wet air masses of type B, observed up to 1.7 km above the CPT, are not representative of the large-scale water vapor distribution detected by MLS. Our results suggest that the full backward and forward evolution of the sampled air masses needs to be considered when inferring stratospheric moistening in the Asian monsoon region. Water vapor concentrations set by LDPs seem to be a better proxy for the stratospheric water vapor budget than rare observations of enhanced water mixing ratios above the local CPT. These observations call into question their applicability to quantify long-term stratospheric water vapor trends.

How to cite: Konopka, P., Rolf, C., von Hobe, M., Khaykin, S. M., Clouser, B., Moyer, E., Ravegnani, F., Viciani, S., Afchine, A., Krämer, M., Stroh, F., and Ploeger, F.: A long way of water vapor from the Asian Summer Monsoon into the stratosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8021, https://doi.org/10.5194/egusphere-egu23-8021, 2023.

EGU23-8406 | ECS | Orals | AS1.30

Relative Contributions of Anthropogenic and Lightning Nitrogen Sources in the Upper Troposphere during the Asian Summer Monsoon 

Jun Zhang, Douglas Kinnison, Simone Tilmes, Lousia Emmons, Warren Smith, Shawn Honomichl, Alessandro Franchin, Qing Liang, and Laura Pan

We examine the role of the Asian Summer Monsoon (ASM) in influencing the chemical composition of the upper troposphere and lower stratosphere (UTLS) using the Whole Atmosphere Community Climate Model, version 6 (WACCM6). This version of WACCM6 uses a Finite Volume dynamical core, with a horizontal resolution of ~1.0º and a vertical resolution of ~500m in the UTLS. For this study, the specified dynamics option is applied where the temperature, zonal and meridional winds are nudged towards MERRA-2 reanalysis fields from the NASA Goddard Earth Observing System version 5 (GEOS5). This model study examines the relative contribution of anthropogenic and lightning nitrogen oxide (NOx) sources in the UTLS during the Asian Summer Monsoon (ASM) using a tagged NOx mechanism (Emmons et al., Geosci. Model Dev., doi:10.5194/gmd-5-1531-2012). In this tagging mechanism, the NOx source regions in South and East Asia are examined separately. NOx sources from outside South and East Asia and the amount transported from the stratosphere are also derived. The model simulated NOx for the year 2022 is evaluated by comparing it to in situ measurements from the Asian summer monsoon Chemical and Climate Impact Project (ACCLIP). The model results suggest that the major contribution of NOx concentration within the ASM anticyclone is from South Asia lightning and South Asia anthropogenic sources, which contribute more than 55% to the upper troposphere NOx for the year 2022. In the shedding region, both South and East Asia anthropogenic emissions play an important role in the NOx budget. In addition, we also explore the hydroxyl radical (OH) and peroxyacetylnitrate (PAN) formation from different NOx sources, which are of importance to atmospheric compositions such as ozone and aerosols in the free troposphere.

How to cite: Zhang, J., Kinnison, D., Tilmes, S., Emmons, L., Smith, W., Honomichl, S., Franchin, A., Liang, Q., and Pan, L.: Relative Contributions of Anthropogenic and Lightning Nitrogen Sources in the Upper Troposphere during the Asian Summer Monsoon, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8406, https://doi.org/10.5194/egusphere-egu23-8406, 2023.

EGU23-9161 | ECS | Orals | AS1.30

Organic, inorganic and total bromine observations around the extratropical tropopause and lowermost stratosphere 

Meike Rotermund, Andreas Engel, Jens-Uwe Grooß, Peter Hoor, Markus Jesswein, Flora Kluge, Tanja Schuck, Bärbel Vogel, Thomas Wagenhäuser, Benjamin Weyland, Andreas Zahn, Siyuan Zheng, and Klaus Pleilsticker

Organic, inorganic and total bromine (Brtot) around the upper troposphere and lower stratosphere (UTLS) were measured over southern Argentina and the surrounding regions extending down to the Antarctic Peninsula in September and November of 2019. These observations were recorded from the German High Altitude and LOng range research aircraft (HALO) as part of the Transport and Composition of the Southern Hemisphere UTLS (SouthTRAC) research campaign. Total bromine (Brtot) is inferred from measured total organic bromine (Brorg) added to inorganic bromine (Bryinorg). Brorg is comprised of the bromine summed from CH3Br, the halons, and the major very short-lived brominated species measured onboard HALO by the University of Frankfurt, while the Bryinorg is evaluated from limb measured BrO and CLaMS photochemical transport modelling (FZ Jülich) accounting for the BrO/Bryinorg ratio. Air mass transport pathways into the UTLS and the likely origins of bromine-rich air masses reaching the Southern Hemisphere (SH) lower stratosphere are identified through distributions of in situ measured transport (CO and N­­2O) and air mass lag-time (SF6) tracers as well as Lagrangian transport modelling. Additionally, Brtot measured in the SH is compared with previous measurements observed in the Northern Hemisphere as part of the Wave-driven ISentropic Exchange (WISE) research campaign in fall 2017, as well as the long term trend in stratospheric bromine.

How to cite: Rotermund, M., Engel, A., Grooß, J.-U., Hoor, P., Jesswein, M., Kluge, F., Schuck, T., Vogel, B., Wagenhäuser, T., Weyland, B., Zahn, A., Zheng, S., and Pleilsticker, K.: Organic, inorganic and total bromine observations around the extratropical tropopause and lowermost stratosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9161, https://doi.org/10.5194/egusphere-egu23-9161, 2023.

EGU23-9166 | Orals | AS1.30

How much does new particle formation near the tropical tropopause contribute to stratospheric aerosol number concentration? 

Eric Jensen, Charles Brock, Christina Williamson, Luke Ziemba, and Matthew Brown

Nucleation of ultrafine aerosols near the tropical tropopause, followed by transport throughout the stratosphere by the Brewer-Dobson circulation, is thought to be the primary source of stratospheric aerosol number concentration.  However, depending on how rapidly the aerosols grow by condensation, many of the ultrafine particles generated by new particle formation (NPF) may be lost due to coagulation with accumulation-mode aerosols.  In this study, we use recent high-altitude aircraft measurements of aerosol size distribution, along with microphysical calculations, to investigate this issue.  Initial ultrafine and accumulation-mode size distributions are specified based on the aircraft measurements, and a bin microphysics model is used to simulate the evolution of the aerosol size distributions.  Coagulation and condensation of gases such as sulfuric acid, ammonia, and nitric acid are included.  Preliminary results indicate that for typical conditions, most of the ultrafine aerosols generated by NPF are removed by coagulation, resulting in a relatively small contribution to the total aerosol number concentration.  We have used the model to investigate the sensitivities of total number concentration evolution to aerosol size distributions and condensation rates.

How to cite: Jensen, E., Brock, C., Williamson, C., Ziemba, L., and Brown, M.: How much does new particle formation near the tropical tropopause contribute to stratospheric aerosol number concentration?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9166, https://doi.org/10.5194/egusphere-egu23-9166, 2023.

EGU23-9360 | ECS | Posters on site | AS1.30

An Examination of ACCLIP (2022) Airborne Observations in the Context of their Trajectory-derived Convective Influence 

Warren Smith, Laura Pan, Rei Ueyama, and Shawn Honomichl

The Asian summer monsoon (ASM) has long been known as a weather system, but only recently has its role in atmospheric composition come to be explored in detail.  During boreal summer, an anticyclone forms in the upper troposphere and lower stratosphere (UTLS) over Asia which is associated with a pronounced enhancement of chemical and aerosol species lofted from the boundary layer (BL) by ASM deep convection.  In this work, we explore the transport pathways and time scales associated with ASM anticyclone shedding events, which effectively redistribute air from the anticyclone into the global atmosphere.  In particular, we launch a series of kinematic backward trajectories using ERA5 reanalysis from the western Pacific UTLS, emphasizing a novel set of airborne in situ observations taken during the summer 2022 Asian summer monsoon Chemical and Climate Impact Project (ACCLIP).  Trajectories are integrated backward in time to their most recent encounters with a satellite-derived database of convective cloud top altitudes, as well as the top of the BL.  We find that there is a consistent story between observed pollution concentrations and their associated trajectory-derived transport histories, with enhanced concentrations of BL pollutants preferentially found in air masses with shorter transport times from their convective or BL sources.  We also find that air mass contributions from eastern Asia preferentially contain higher pollutant concentrations compared to those from southern Asia.  The results provide valuable context for the measurements taken during ACCLIP and provide new insight into the role of ASM transport in global atmospheric composition.   

How to cite: Smith, W., Pan, L., Ueyama, R., and Honomichl, S.: An Examination of ACCLIP (2022) Airborne Observations in the Context of their Trajectory-derived Convective Influence, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9360, https://doi.org/10.5194/egusphere-egu23-9360, 2023.

EGU23-9430 | Posters on site | AS1.30

CLaMS simulations of aerosol transport from the Asian monsoon anticyclone into the extratropical UTLS 

Ines Tritscher, Bärbel Vogel, and Rolf Müller

The Asian Tropopause Aerosol Layer (ATAL) in the Northern Hemisphere during summer was first discovered in satellite observation of aerosol particles in the Upper Troposphere / Lower Stratosphere (UTLS) by Vernier et al. (2011; 2015). It is related to the Asian monsoon anticyclonic circulation at UTLS altitudes. Motivated by the current lack of detailed understanding of the origin of ATAL particles and the transport of aerosols from the Asian monsoon anticyclone into the extratropical UTLS, we propose a model study based on simulations with the three-dimensional chemical transport model CLaMS. Simulations will be performed for the Asian summer monsoon 2017. In the framework of the StratoClim project, an aircraft measurement campaign was conducted in Kathmandu (Nepal) in summer 2017. A variety of trace gases and aerosol characteristics have been measured for the first time in the Asian monsoon anticyclone up to 20 km altitude. By using artificial tracers of air mass origin (Vogel et al., 2015; 2016; 2019), we plan to analyze the transport of aerosol particles into the extratropical UTLS with the help of the new ERA-5 reanalysis data from ECMWF.

How to cite: Tritscher, I., Vogel, B., and Müller, R.: CLaMS simulations of aerosol transport from the Asian monsoon anticyclone into the extratropical UTLS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9430, https://doi.org/10.5194/egusphere-egu23-9430, 2023.

EGU23-9439 | ECS | Orals | AS1.30

A Modern Approach to a Stability-Based Definition of the Tropopause 

Emily Tinney, Cameron Homeyer, Lexy Elizalde, Dale Hurst, Anne Thompson, Ryan Stauffer, Holger Vömel, and Henry Selkirk

Definition of the tropopause has remained a focus of atmospheric science since its discovery near the beginning of the twentieth century. An accurate identification of the tropopause is a vital component to upper troposphere and lower stratosphere research, especially for studies that seek to assess and quantify the two-way exchange of air across the tropopause, which in turn impacts our understanding and prediction of Earth’s radiation budget and climate. Few universal definitions (those that can be reliably applied globally and to both common observations and numerical model output) exist and many definitions with unique limitations have been developed over the years. The most commonly used universal definition of the tropopause is the temperature lapse-rate definition established by the World Meteorological Organization (WMO) in 1957 (the LRT). Despite its widespread use, there are recurrent situations where the LRT definition fails to reliably identify the tropopause. Motivated by increased availability of coincident observations of stability and composition, we reexamine the relationship between stability and composition change in the tropopause transition layer and identify areas for improvement in a stability-based definition of the tropopause. Six locations with long-term (up to 40+ years) balloon observations of temperature, ozone, and water vapor were selected for analysis to offer a variety of environments, including tropical, subtropical, extratropical, and polar environments. Data from these sites are then used to identify covariability between several metrics of atmospheric stability and composition. We show that the vertical gradient of potential temperature is a superior stability metric to identify the greatest composition change in the tropopause transition layer, which we use to propose a new universally applicable potential temperature gradient tropopause (PTGT) definition. A comparison of the PTGT and LRT applied to both observations and reanalysis output will be shown. Overall, our results reveal that the PTGT largely agrees with the LRT, but more reliably identifies tropopause-level composition change when the two definitions differ greatly.

How to cite: Tinney, E., Homeyer, C., Elizalde, L., Hurst, D., Thompson, A., Stauffer, R., Vömel, H., and Selkirk, H.: A Modern Approach to a Stability-Based Definition of the Tropopause, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9439, https://doi.org/10.5194/egusphere-egu23-9439, 2023.

EGU23-9693 | ECS | Orals | AS1.30

Detailed Examination of Upper Troposphere Lower Stratosphere Composition Change from In Situ Observations of Active Convection in the United States 

Andrea Gordon, Cameron Homeyer, Jessica Smith, T. Paul Bui, Jonathan Dean-Day, Thomas Hanisco, Reem Hannun, Jason St Clair, Steve Wofsy, Jasna Pittman, Bruce Daube, David Sayres, and Apoorva Pandey

Tropopause-overshooting convection in the midlatitudes provides a rapid transport pathway of air from the lower troposphere to the upper troposphere and lower stratosphere (UTLS), and can result in the formation of above-anvil cirrus plumes (AACPs).  Recent in situ observations from the Dynamics and Chemistry of the Summer Stratosphere (DCOTSS) field campaign are used to examine impacts from active overshooting convection on UTLS composition. There are little to no prior airborne observations of active overshooting convection, making observations from this flight valuable to interpreting and exploring processes seen in idealized modeling studies. DCOTSS research flight 13 on May 31st, 2022 sampled active overshooting convection over the state of Oklahoma for more than three hours with the NASA ER-2 high-altitude research aircraft. Additionally, an AACP was bisected during this flight, providing the first such extensive sampling of this phenomena. This study aims to provide a detailed understanding of changes in the UTLS composition from active overshooting convection and AACPs using the in-situ observations from this flight. The observations reveal multiple pronounced changes in air mass composition and stratospheric hydration. In agreement with prior modeling studies, maximum altitudes of water vapor enhancement were much higher than altitudes of mostly passive trace gas composition change. Stratospheric water vapor enhancements reached nearly a factor of four over background levels at a maximum altitude of 16.56 km and a potential temperature of 389.76 K. Carbon monoxide, a tracer of tropospheric origin, showed enhancements of a factor of two over background levels at a maximum altitude of 15.76 km and potential temperature of 363.6 K. There is a notable positive correlation between water vapor and ozone near the bisection of the AACP, which seems to be the result of horizontal mixing. It appears that the water vapor enhancement within the AACP was limited to the saturation mixing ratio of the low temperature environment.

How to cite: Gordon, A., Homeyer, C., Smith, J., Bui, T. P., Dean-Day, J., Hanisco, T., Hannun, R., St Clair, J., Wofsy, S., Pittman, J., Daube, B., Sayres, D., and Pandey, A.: Detailed Examination of Upper Troposphere Lower Stratosphere Composition Change from In Situ Observations of Active Convection in the United States, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9693, https://doi.org/10.5194/egusphere-egu23-9693, 2023.

The Asian Summer Monsoon Anticyclone (AMA) is known to bring ground-level pollutants up to the stratosphere. Aerosols in the AMA often form what is known as the Asian Tropopause Aerosol Layer (ATAL), with modelling studies suggesting that the ATAL can provide up to 15 % of the stratospheric aerosol in the Northern Hemisphere. In this work, we present single-particle mass spectrometry measurements of aerosol composition in the AMA outflow and in the North American upper troposphere/lower stratosphere (UTLS) during the same season. Measurements were taken by the Particle Analysis by Laser Mass Spectrometry (PALMS) instrument and made during the Asian Summer Monsoon Chemical & CLimate Impact Project (ACCLIP). We find that the dominant aerosol type found in the ATAL and those found in the UTLS over North America are chemically different. Despite high concentrations of ground-level gas phase pollutants, particles in the ATAL are dominated by secondary nitrate particles. The organic content of these particles is low, which precludes them from being organic-nitrate aerosol; thus, we believe that these particles are either nitric/sulfuric acid solutions, or they are mixtures of partially neutralized ammonium nitrate/sulfate. Finally, we present the mass concentrations of nitrate particles, dust, and sulfate-organic particles in the ATAL, and estimate each particle type’s influence on the aerosol composition over the North American continent.

How to cite: Schill, G., Murphy, D., Lawler, M., and Abou-Ghanem, M.: Single-Particle Aerosol Composition in the Asian Tropopause Aerosol Layer and in the North American Upper Troposphere/Lower Stratosphere during ACCLIP, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9792, https://doi.org/10.5194/egusphere-egu23-9792, 2023.

EGU23-9858 | Orals | AS1.30 | Highlight

A Case Study of the Highest Ever Altitude of In Situ Observations of Convective Hydration of the Stratosphere during the DCOTSS Field Campaign 

Cameron Homeyer, Jessica Smith, Thaopaul Bui, Jonathan Dean-Day, Thomas Hanisco, Reem Hannun, Jason St Clair, and Kristopher Bedka

On 24 June 2022, remnant outflow from a tornadic supercell storm that occurred in northern Kansas on the evening of 23 June 2022 was observed by the high-altitude NASA ER-2 aircraft during the Dynamics and Chemistry of the Summer Stratosphere (DCOTSS) field campaign. Namely, preliminary analysis indicates that stratospheric water vapor enhancements were observed at altitudes up to approximately 19.25 km (~1 km higher than any prior documented event), approximately 460 K potential temperature (~30 K higher than any prior documented event), and ozone mixing ratios of more than 1400 ppbv (more than double any prior documented event). The responsible storm was one of the most extreme events observed annually in the United States, within no more than 10 per year such high-reaching storms based on ground-based radar climatology. Here, we review the event using high-resolution ground-based radar volumes and satellite imagery and show that it reached altitudes exceeding 19 km for at least an hour. Linkages to the Kansas storm will be demonstrated via trajectory analyses initialized in the volumes impacted by the storm (as determined from radar and satellite observations). Broader evaluation of stratospheric composition impacts resulting from this event will also be presented. 

How to cite: Homeyer, C., Smith, J., Bui, T., Dean-Day, J., Hanisco, T., Hannun, R., St Clair, J., and Bedka, K.: A Case Study of the Highest Ever Altitude of In Situ Observations of Convective Hydration of the Stratosphere during the DCOTSS Field Campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9858, https://doi.org/10.5194/egusphere-egu23-9858, 2023.

EGU23-10056 | Orals | AS1.30

Dynamics of heated (or cooled) vortices in the stratosphere 

Bernard Legras, Aurélien Podglajen, Clair Duchamp, Pasquale Sellitto, Angela Limare, Zhaodong Niu, Paul Billant, Vladimir Zeitlin, Guillaume Lapeyre, and Riwal Plougonven

Recent extreme events associated with forest fires and large volcanic eruptions have demonstrated that dense aerosol clouds in the stratosphere often wraps up as persistent compact structures which rotate as anticyclones and also move vertically. One of these vortices has been observed over 3 months and experienced a 20 km rise. Such observations were made after the 2020 Australian wildfires, the 2017 British Columbia fire and more recently after the 2022 Tonga eruption and a few other cases. For all these events, the link was made with anomalous warming or cooling due to the composition of the clouds. This presentation will summarize the observed events and demonstrate the general characters of the stratospheric aerosol vortices. It will also discuss how they are detected by the weather assimilation systems through their signature in temperature, the conditions of their stability and how they can be reproduced experimentally with simple experimental models. Their impact on the transport of long-lived species will be discussed.

Such structures seem so far proper to the Earth stratosphere and have found analogies nowhere else.

Ref: DOIs: 10.1038/s43247-020-00022-5, 10.5194/acp-21-7113-2021, 10.5194/acp-22-14957-2022

How to cite: Legras, B., Podglajen, A., Duchamp, C., Sellitto, P., Limare, A., Niu, Z., Billant, P., Zeitlin, V., Lapeyre, G., and Plougonven, R.: Dynamics of heated (or cooled) vortices in the stratosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10056, https://doi.org/10.5194/egusphere-egu23-10056, 2023.

EGU23-10132 | ECS | Orals | AS1.30

Longitudinal Variations of Tropical Winds in the UTLS: Aeolus and Strateole measurements of Equatorial Waves and the Walker Circulation 

Timothy Banyard, Corwin Wright, Neil Hindley, and Martina Bramberger

Tropical atmospheric waves often have fine vertical scales that are difficult to resolve in models and cannot easily be observed using existing satellite or ground-based instruments. These waves are known to strongly influence the driving of the quasi-biennial oscillation (QBO), which is an important source of seasonal predictability in the lower stratosphere, and have important interactions with dynamical mechanisms such as the Walker Circulation. As the first Doppler wind lidar in space, Aeolus provides high resolution measurements of wind on a global scale, including in the hard-to-observe upper-troposphere lower-stratosphere (UTLS) region of the atmosphere. It is therefore a uniquely capable platform for studying these phenomena. Here, we sample ERA5 as Aeolus to produce like-for-like comparisons of resolved and observed wind structures, and co-locate measurements with stratospheric superpressure balloon observations from the Strateole-2 campaign. We analyse Kelvin waves and their interaction with the QBO, including the 2019/20 QBO disruption for which a special Aeolus scanning mode was implemented. We also compare our results with wave spectra from outgoing long-wave radiation (OLR) measurements, and highlight how Aeolus and future Doppler wind lidar satellites can deepen our understanding of the tropical UTLS more generally.

How to cite: Banyard, T., Wright, C., Hindley, N., and Bramberger, M.: Longitudinal Variations of Tropical Winds in the UTLS: Aeolus and Strateole measurements of Equatorial Waves and the Walker Circulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10132, https://doi.org/10.5194/egusphere-egu23-10132, 2023.

EGU23-10146 | ECS | Posters on site | AS1.30

High Altitude and Long-range Aircraft (HALO) measurements of carbon monoxide and methane to characterize dynamical transport processes in the tropical upper troposphere 

Linda Ort, Lenard Röder, Peter Michael Hoor, Jos Lelieveld, and Horst Fischer

The dynamics and transport processes in the upper troposphere are of great importance for the global long-term distribution of greenhouse gases and pollution tracers, and hence for the anthropogenic impact on the Earth climate. Especially in the tropics, large amounts of carbon monoxide (CO), carbon dioxide (CO2), methane (CH4) and nitrous oxide (N2O) are produced by e.g. biomass burning, anthropogenic and agricultural activities. These tracers are vertically transported by deep convective cells in the InterTropical Convergence Zone (ITCZ) into the Tropical Tropopause Layer (TTL). Long-range transport processes distribute the tracers globally, which have lifetimes of up to years and decades. It is crucial to understand the details of the transport processes and how the tracers are distributed throughout the upper troposphere and the lower stratosphere (UTLS).

During several aircraft campaigns (CAFE Brazil 2022/2023, SouthTrac 2019, CAFE Africa 2018, OMO 2015, ESMVal 2012) CO, CH4 and N2O have been measured nearly globally and especially in the tropics with quantum cascade laser absorption spectrometers deployed on the High Altitude and Long-range Aircraft (HALO). Combining these measurements, we can present a good overview of the large-scale distribution of the tracers in particular in the tropical troposphere up to altitudes of approx. 14 km.

The in-situ aircraft measurements will be used to study interhemispheric transport processes and regional trace gas budgets at the base of the TTL. Therefore, they will be further combined and investigated with modelling data and back trajectories. 

How to cite: Ort, L., Röder, L., Hoor, P. M., Lelieveld, J., and Fischer, H.: High Altitude and Long-range Aircraft (HALO) measurements of carbon monoxide and methane to characterize dynamical transport processes in the tropical upper troposphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10146, https://doi.org/10.5194/egusphere-egu23-10146, 2023.

EGU23-10355 | ECS | Orals | AS1.30

Hydroxyl radicals in the Amazon tropical troposphere measured during the CAFE-Brazil field campaign with HORUS 

Philip Holzbeck, Sreedev Sreekumar, Anywhere Tsokankunku, Daniel Marno, Roland Rohloff, Monica Martinez, Clara Nussbaumer, Horst Fischer, Joachim Curtius, Mira Pöhlker, Jos Lelieveld, and Hartwig Harder

The campaign Chemistry of the Atmosphere Field Experiment (CAFE) Brazil was conducted in the Amazon rainforest in December 2022 and January 2023 to study new particle formation in the outflow of convective systems over the Amazon rainforest. In the framework of this campaign, photochemical and aerosol processes in the tropical troposphere were investigated at different altitudes from the boundary layer up to 14 km using the High Altitude and Long Range Research Aircraft (HALO).

The HydrOxyl Radical measurement Unit based on fluorescence Spectroscopy (HORUS) measures the OH and HO2 abundances as a highly relevant tracer for photochemical and aerosol processes in the tropical troposphere and new particle formation. The Hydroxyl radical (OH) oxidizes trace gases transported by convective systems from the boundary layer into the upper troposphere, leading to the formation of condensable matter. Contrasting conditions were measured, from pristine rainforest to polluted biomass burning and pollution conditions, and the occurrence of HOx during the day and nighttime in the outflow of electrified and non-electrified convective systems.
The first results of these measurements will be presented, providing unique insights into the air chemistry and lifecycle of aerosols and clouds in the Amazon rainforest.

How to cite: Holzbeck, P., Sreekumar, S., Tsokankunku, A., Marno, D., Rohloff, R., Martinez, M., Nussbaumer, C., Fischer, H., Curtius, J., Pöhlker, M., Lelieveld, J., and Harder, H.: Hydroxyl radicals in the Amazon tropical troposphere measured during the CAFE-Brazil field campaign with HORUS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10355, https://doi.org/10.5194/egusphere-egu23-10355, 2023.

EGU23-10560 | ECS | Posters virtual | AS1.30

High-Alitutde Aircraft Measurements of NO and NO2 in the Upper Troposphere and Lower Stratosphere over South-East Asia 

Eleanor Waxman, Ru-Shan Gao, Richard McLaughlin, Troy Thornberry, and Andrew Rollins

Nitric oxide (NO) and nitrogen dioxide (NO2) are important trace gases in the upper troposphere and lower stratosphere (UTLS).  In the upper troposphere, NO is primarily formed by lightning and can react with other radicals to form a suite of reactive nitrogen (NOy) species and produce ozone.  In the lower stratosphere, NOx can be responsible for catalytic ozone destruction and can form halogen reservoirs such as ClNO2 and ClONO2.  Accurate measurements of NOx species are therefore important for understanding and diagnosing UTLS chemical regimes.  Further, understanding NO2 concentrations in the stratosphere and upper troposphere is critical for accurate satellite retrievals of tropospheric NO2

In-situ measurements of NOx species above 12-15 km are infrequent and challenging.  Where there are measurements of NOx species up to about 12 km, NO mixing ratios tend to be reasonably well-reproduced using global models.  However, NO2 measurements frequently agree well with models and photostationary state calculations up to about 8 km, but at higher altitudes routinely are significantly higher than expected relative to the measured NO.  Proposed sources of this discrepancy include measurement artifacts affecting the in-situ measurements, inaccuracies in rate constants at low temperatures, and missing chemistry.  The net result is significant uncertainty in the NO2 concentrations in the UTLS.

Here we present results from the recent high-altitude aircraft campaign Asian Summer Monsoon Chemistry and CLimate Impact Project (ACCLIP) over southeast Asia in summer 2022.  We show measurements from the recently-developed NOAA NO laser-induced fluorescence instrument up to altitudes of almost 20 km.  This instrument makes direct NO measurements with precision and accuracy sufficient for measurements below one ppt with one second of integration, making it ideal for aircraft campaigns.  In order to measure NO2 with this instrument, we have developed a photolysis inlet which converts NO2 to NO using an LED centered at 395 nm.  What is novel about this NO2 conversion is that it is done in an unpressurized pylon of the aircraft and thus the sample remains at the UTLS ambient temperatures until after photolysis.  This thus significantly reduces the potential interferences from NOy species that can thermally decompose to NO2 at room temperature, eliminating a potential source of major artifact.  Our data show good agreement with photostationary state calculations performed for these flights. 

How to cite: Waxman, E., Gao, R.-S., McLaughlin, R., Thornberry, T., and Rollins, A.: High-Alitutde Aircraft Measurements of NO and NO2 in the Upper Troposphere and Lower Stratosphere over South-East Asia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10560, https://doi.org/10.5194/egusphere-egu23-10560, 2023.

EGU23-11111 | ECS | Posters on site | AS1.30

Water vapor isotopic variations of the upper troposphere/ lower stratosphere in the N. American and Asian Summer Monsoons 

Carly KleinStern, Benjamin Clouser, Thaopaul Bui, Francesco D'Amato, Silvia Viciani, Giovanni Bianchini, Troy Thornberry, and Elisabeth Moyer

The 2022 ACCLIP (Asian summer monsoon Chemical and CLimate Impact Project) high-altitude aircraft campaign has provided a sampling of the diversity of processes that affect moisture transport in the upper troposphere / lower stratosphere (UT/LS). We report here on ACCLIP observations of water vapor isotopologues, which trace the origin and microphysical history of water vapor. Measurements with the Chicago Water Isotope Instrument (ChiWIS) show isotopic variations in the UT/LS that correlate with airmass history, and 100-150 ‰ variation even at the same water content. ACCLIP flights out of Osan, South Korea sampled monsoon anticyclone outflow with CO values over 200 ppb, recent local convection, extensive in-situ cirrus, and an overflight of tropical cyclone Hinnanmor showing strong isotopic depletion. Flights out of Houston, TX  sampled week-old remnants of sublimated ice from deep convection, producing enriched vapor, and possible mixing of convective overshoots with stratospheric air before sinking. We show through case studies from both Asia and North America that isotopologues provide a sensitive diagnostic of ice sublimation, and demonstrate how different meteorological contexts produce distinct isotopic signatures.

How to cite: KleinStern, C., Clouser, B., Bui, T., D'Amato, F., Viciani, S., Bianchini, G., Thornberry, T., and Moyer, E.: Water vapor isotopic variations of the upper troposphere/ lower stratosphere in the N. American and Asian Summer Monsoons, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11111, https://doi.org/10.5194/egusphere-egu23-11111, 2023.

EGU23-11537 | Posters on site | AS1.30

The influence of synoptic-scale processes on the paired H2O–O3 distribution in the UTLS: case study of a North Atlantic jet stream 

Andreas Schäfler, Michael Sprenger, Heini Wernli, Andreas Fix, and Martin Wirth

The distribution of H2O and O3 in the midlatitude UTLS is of key relevance for the Earth’s weather and climate. Tropospheric and stratospheric dynamical processes, acting on different time-scales, interact with chemistry and determine the composition of the UTLS and the extratropical transition layer (ExTL) therein. In this study, we investigate how strongly the fine-scale trace gas distribution in the UTLS/ExTL is related to interacting, tropospheric weather systems on synoptic time scales, which shape transport and mixing.

We present range-resolved, collocated lidar H2O and O3 measurements from a research flight during the Wave-driven ISentropic Exchange (WISE) campaign, which was conducted across a jet stream located over the eastern North Atlantic on 1 October 2017. The observations are combined with 10-day backward trajectories along which meteorological parameters and turbulence diagnostics are traced. The derived transport and mixing characteristics are projected to the vertical cross sections of the lidar measurements and to the H2O–O3 phase space (Tracer-Tracer space) to explore linkages with the evolution of synoptic-scale weather systems and their interaction.

We find that the formation of H2O and O3 filaments in the troposphere and stratosphere, the high variability of tropospheric H2O and the formation of the ExTL mixing layer can, to a large extent, be explained by transport and mixing associated with interacting tropical, midlatitude and arctic weather systems in the region of the jet stream on synoptic time scales. The mixed ExTL air exhibits a strong influence of turbulent mixing in the jet stream during the two days before the flight. The diagnosed non-local and transient character of mixing points to the complexity of the formation and interpretation of mixing lines in TT space.

 

The presented work is accepted for publication in ACP:

Schäfler, A., Sprenger, M., Wernli, H., Fix, A., and Wirth, M.: Case study on the influence of synoptic-scale processes on the paired H2O-O3 distribution in the UTLS across a North Atlantic jet stream, Atmos. Chem. Phys. Discuss. [preprint], https://doi.org/10.5194/acp-2022-692, accepted, 2022. 

How to cite: Schäfler, A., Sprenger, M., Wernli, H., Fix, A., and Wirth, M.: The influence of synoptic-scale processes on the paired H2O–O3 distribution in the UTLS: case study of a North Atlantic jet stream, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11537, https://doi.org/10.5194/egusphere-egu23-11537, 2023.

EGU23-11571 | Posters virtual | AS1.30

Very short-lived halogens amplify recent and future ozone depletion trends in the tropical lower stratosphere. 

Julián Villamayor, Fernando Iglesias-Suarez, Carlos A. Cuevas, Rafael P. Fernandez, Qinyi Li, Marta Abalos, Ryan Hossaini, Martyn P. Chipperfield, Douglas E. Kinnison, Simone Tilmes, Jean-François Lamarque, and Alfonso Saiz-Lopez

Recent observational evidences show ongoing net ozone depletion in the tropical lower stratosphere (LS) since the late 20th century, in contrast to the overall stratospheric ozone recovery following controls in the Montreal Protocol to limit the production of long-lived ozone depleting substances. Such behavior is currently thought to be driven by dynamical transport accelerated by global warming. In contrast, the role of chemistry, i.e., the enhanced ozone depletion due to emissions of halogenated ozone-depleting very short-lived substances (VSLS) has been considered to be unimportant. Here we employ a chemistry-climate model with a comprehensive chemical scheme to demonstrate that VSLS chemistry accounts for around a quarter of the observed tropical LS negative ozone trend in 1998-2018. We attribute such an effect to chemical reactions with VSLS from natural and anthropogenic emissions in concert. Future projections show the persistence of the currently unaccounted for contribution of VSLS to ozone loss throughout the 21st century in the tropical LS, the only region of the global stratosphere not projecting an ozone recovery by 2100. Our results show evidence for the need of mitigation strategies for regulating anthropogenic VSLS emissions to preserve the present and future ozone layer in low latitudes.

How to cite: Villamayor, J., Iglesias-Suarez, F., Cuevas, C. A., Fernandez, R. P., Li, Q., Abalos, M., Hossaini, R., Chipperfield, M. P., Kinnison, D. E., Tilmes, S., Lamarque, J.-F., and Saiz-Lopez, A.: Very short-lived halogens amplify recent and future ozone depletion trends in the tropical lower stratosphere., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11571, https://doi.org/10.5194/egusphere-egu23-11571, 2023.

EGU23-11640 | ECS | Orals | AS1.30

The Sensitivity of Moisture Fluxes into the Tropical Tropopause Layer to External Forcing 

Clarissa Kroll, Stephan Fueglistaler, Luis Kornblueh, Hauke Schmidt, and Claudia Timmreck

The very low temperatures in the tropical tropopause layer (TTL) restrict the moisture entering the stratosphere, leading to its dryness. Whereas the water vapor flux into the stratosphere can be described via the cold point temperatures, our knowledge on the contribution of frozen moisture to the total flux is incomplete. This raises concerns regarding the ability of General Circulation Models (GCMs) to accurately predict changes in total stratospheric moisture following perturbations in the radiative budget due to volcanic aerosol or stratospheric geoengineering, as GCMs  heavily rely on convective parameterizations. The emerging cloud-resolving simulations, however, offer the unprecedented possibility to gain insight into the sensitivity of a TTL, which is not strongly constrained by parameterized convection. Here we present the first results using global convection-resolving simulations to investigate the sensitivity of moisture fluxes within the TTL to an additional heating source. We address the question of how the partitioning of moisture fluxes into water vapor and frozen hydrometeors changes under perturbations. 
This study shows an exceptional resilience of the TTL, keeping the flux partitioning constant - even at an average cold-point warming exceeding 8 K. In the perturbed and unperturbed simulation, frozen moisture contributes around 20 % of the moisture flux into the stratosphere.

How to cite: Kroll, C., Fueglistaler, S., Kornblueh, L., Schmidt, H., and Timmreck, C.: The Sensitivity of Moisture Fluxes into the Tropical Tropopause Layer to External Forcing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11640, https://doi.org/10.5194/egusphere-egu23-11640, 2023.

EGU23-12081 | ECS | Orals | AS1.30

Chemical composition and processing of aerosol particles in the Asian Tropopause Aerosol Layer inferred from airborne measurements during the ACCLIP campaign 

Oliver Eppers, Franziska Köllner, Oliver Appel, Philipp Brauner, Fatih Ekinci, Sergej Molleker, Antonis Dragoneas, Andreas Hünig, Warren Smith, Rei Ueyama, Johannes Schneider, and Stephan Borrmann

The presence of aerosol particles in the upper troposphere/lower stratosphere (UTLS) region plays an important role for the Earth’s radiative balance and the formation of cirrus clouds. In recent years, a substantial amount of organic matter and ammonium nitrate have been found in the Asian upper troposphere (UT) associated with the Asian summer monsoon anticyclone (ASMA; Appel et al., 2022; Höpfner et al., 2019). These particles were observed at altitudes between 11 and 19 km (corresponding to potential temperatures between 355 and 420 K), known as the Asian Tropopause Aerosol Layer (ATAL).  However, the formation and aging processes of these particles remain unclear. In particular, the fate of aerosol particles in eastward eddy shedding events is poorly understood.

Here, we present the results of aircraft-based measurements in the eddy shedding region above the Western Pacific during the ACCLIP campaign in July/August 2022. Using the hybrid mass spectrometer ERICA (ERC instrument for chemical composition of aerosols; Hünig et al., 2022), the chemical composition of aerosol particles in the Asian UT was measured via a combination of two complementary aerosol mass spectrometry techniques: the desorption ionization technique (ERICA-LAMS) and the thermal desorption with subsequent electron impact ionization technique (ERICA-AMS). The detectable size range of ERICA extends from ~120 nm up to 3.5 µm.

Our ERICA-AMS measurements indicate that the ATAL above 360 K potential temperature exhibited enhanced concentrations of ammonium nitrate and organics with a growing fraction of sulfate towards higher altitudes. Additionally, measurements in aged ASMA air masses during eddy shedding events enabled the investigation of photochemical aging of particles originating from the ATAL. For this purpose, the degree of oxidation will be evaluated by the ratio of organic signals at m/z 43 and 44 from the ERICA-AMS. We will further combine the dataset from these observations with model results of the location and timing of recent convective influence. The determination of recent convective influence is based on kinematic backward trajectories and a satellite-derived database of convective cloud top altitudes to distinguish different source regions.

 

References:

Appel, O., Köllner, F., Dragoneas, A., et al.: Chemical analysis of the Asian tropopause aerosol layer (ATAL) with emphasis on secondary aerosol particles using aircraft-based in situ aerosol mass spectrometry, Atmos. Chem. Phys., 22, 13607–13630, https://doi.org/10.5194/acp-22-13607-2022, 2022.

Höpfner, M., Ungermann, J., Borrmann, S. et al.: Ammonium nitrate particles formed in upper troposphere from ground ammonia sources during Asian monsoons. Nat. Geosci., 12, 608–612, https://doi.org/10.1038/s41561-019-0385-8, 2019.

Hünig, A., Appel, O., Dragoneas, A., et al.: Design, characterization, and first field deployment of a novel aircraft-based aerosol mass spectrometer combining the laser ablation and flash vaporization techniques, Atmos. Meas. Tech., 15, 2889–2921, https://doi.org/10.5194/amt-15-2889-2022, 2022.

How to cite: Eppers, O., Köllner, F., Appel, O., Brauner, P., Ekinci, F., Molleker, S., Dragoneas, A., Hünig, A., Smith, W., Ueyama, R., Schneider, J., and Borrmann, S.: Chemical composition and processing of aerosol particles in the Asian Tropopause Aerosol Layer inferred from airborne measurements during the ACCLIP campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12081, https://doi.org/10.5194/egusphere-egu23-12081, 2023.

Deep convective storms represent the fastest vertical transport mechanism of both momentum and chemical species from the surface to the middle atmosphere, and these transports may potentially impact strongly the global atmospheric and climate processes. For example, the water vapor transported through the tropopause into LS may exert substantial radiative forcing due to its strong capability in intercepting terrestrial IR. Due to the difficulty in the in situ observation in the storm top region, most previous studies rely on remote sensing data whose interpretation can be ambiguous. Consequently, many details of the transport process remain unclear. On July 29, 2016, we encountered a line of convective storms along the coast of China from about Lat 35°N to Lat 22°N during a flight onboard of a commercial aircraft and made many photographic records of the storm tops that exhibited strong internal gravity wave (IGW) features. The visible satellite images of these coastal storms were retrieved from Himawari-8 archive and made into a loop. The simultaneous availability of both aircraft and satellite observations makes this episode a rare case for improving our understanding of the UTLS dynamics.

We performed WRF simulation of this case with a domain as illustrated in Fig. 1(a) and the results compare favorably with the satellite observations. We are analyzing the results to understand especially the vertical structure and the IGW, thermodynamics and mass transfer processes in the UTLS region (Fig. 1(b)). We will use the aircraft and satellite observations to substantiate the model interpretation of the storm top processes. The animations of model results and satellite loops provide a clear picture of deep convection dynamics in UTLS. We will also discuss the potential global impact of these processes.

How to cite: Wang, P. K., Chou, Y.-L., and Lindsey, D.: WRF modeling of the UTLS region of the July 29 2016 summer monsoon storms in China and comparison with aircraft and satellite observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12557, https://doi.org/10.5194/egusphere-egu23-12557, 2023.

EGU23-12992 | Orals | AS1.30 | Highlight

The Hunga Tonga-Hunga Ha’apai stratospheric eruption of 15th January 2022: a global warming volcanic plume? 

Pasquale Sellitto, Bernard Legras, Clair Duchamp, Redha Belhadji, Elisa Carboni, Richard Siddans, and Corinna Kloss

The underwater Hunga Tonga-Hunga Ha’apai volcano erupted in the early hours of 15th January 2022 and injected volcanic gases and aerosols to over 50 km altitude. In this talk, we synthesise satellite, ground-based, in situ and radiosonde observations of the eruption to investigate the emissions, the horizontal and vertical dispersion, and the strength of the stratospheric aerosol and water vapour perturbations in the initial six months after the eruption. The aerosol plume was initially formed of two clouds at 30 and 28  km, mostly composed of submicron-sized sulfate particles, without ash, which is washed out within the first day following the eruption. The large amount of injected water vapour led to a fast conversion of SO2 to sulphate aerosols. We find that the Hunga Tonga-Hunga Ha’apai eruption produced the largest global perturbation of stratospheric aerosols since the Pinatubo eruption in 1991 and the largest perturbation of stratospheric water vapour observed in the satellite era. Then, using offline radiative transfer calculations driven by aerosol and water vapour observations, we quantify the net radiative impact across the two species. Immediately after the eruption, water vapour radiative cooling dominated the local stratospheric heating/cooling rates, producing a spectacular radiatively-driven plume descent of several kilometres. At the top-of-the-atmosphere and surface, volcanic aerosol cooling dominated the radiative forcing during this first dispersion phase. However, after two weeks, due to dilution, water vapour heating started to dominate the top-of-the-atmosphere radiative forcing, leading to a net warming of the climate system. On a longer timescale, sulphate particles, undergoing hygroscopic growth and coagulation, sediment and gradually separate from the moisture anomaly entrained in the ascending branch Brewer–Dobson circulation. This is the first time a warming effect on the climate system has been linked to volcanic eruptions, which usually produce a transient cooling.

How to cite: Sellitto, P., Legras, B., Duchamp, C., Belhadji, R., Carboni, E., Siddans, R., and Kloss, C.: The Hunga Tonga-Hunga Ha’apai stratospheric eruption of 15th January 2022: a global warming volcanic plume?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12992, https://doi.org/10.5194/egusphere-egu23-12992, 2023.

EGU23-13057 | Posters on site | AS1.30

Vertical Ozone Profiles observed by Ozonesone at Pengjia Islet, Taiwan during ACCLIP 2022 

Wei-Nai Chen, Charles C.K. Chou, and RojaRaman Mekalathur

From Aug. 1st to Aug. 29th, 2022, 8 ozonesondes were successfully launched at Pengjia Islet, Taiwan (122°04’17” E, 25°37’46” N) to measure vertical ozone profiles up to 35 km. An ozone DIAL lidar was operated at Academia Sinica in Taipei City, Taiwan (25.040°N, 121.614°E, about 80 km southwest of Pengjia Islet) to continuously measure ozone profile up to 12 km. Ozonesondes launched by the CWB, Taiwan during 1992-2011 are also presented for comparison. The lowest ozone concentration usually occurred around cold point tropopause around 17.5km. The ozone concentration observed in Aug. 2022 in general was in the range of ozone observed during 1992-2011. And there is no significant ozone abundance observed in the UT/LS region. On Aug. 1st and 12th, significant low ozone episodes (about 0.5mPa and 0.8mPa) were found at 10km-16km and 9km-12km, respectively. These two ozone deficiencies might be owing to ozone quenching processes and HYSPLIT back-trajectory analysis indicated the air parcels passed northeast of the Philippines on 7/31 and south of Japan on 8/10, respectively. On the other hand, several weak ozone abundant/deficient episodes were noticed by ozonesonde and ozone DIAL measurements in the UTLS and the low troposphere regions. Ozone concentrations are also noticed to tend to be weakly negatively correlated with RH. HYSPLIT analysis shows most of the back-trajectory of air parcels nearby the south of Japan or northeast of the Philippines.

How to cite: Chen, W.-N., Chou, C. C. K., and Mekalathur, R.: Vertical Ozone Profiles observed by Ozonesone at Pengjia Islet, Taiwan during ACCLIP 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13057, https://doi.org/10.5194/egusphere-egu23-13057, 2023.

EGU23-13092 | ECS | Posters on site | AS1.30

Idealized modeling of anticyclonic plumes from wildfires and volcanic eruptions in the stratosphere 

Aurélien Podglajen, Bernard Legras, Guillaume Lapeyre, Riwal Plougonven, and Vladimir Zeitlin

Anticyclonically-trapped plumes were first discovered following the 2020 Australian fires. Since then, they have been reported after several extreme wildfires and volcanic eruptions, including the 2017 Canadian wildfires, the 2019 Raikoke and the 2022 Hunga Tonga-Hunga Ha’apai eruptions. They appear as coherent plumes of aerosols and combustion/volcanic compounds confined within mesoscale anticyclones (100s to 1000 km diameter), which for several months resist dispersion and dilution by the large-scale flow. Due to their unusual composition, large radiative forcing is prevailing inside the plumes, generating significant diabatic responses in terms of vertical motions and potential vorticity.

In this presentation, we propose a conceptual model of the anticyclonic plumes. We will explore ramifications through idealized numerical simulations and theoretical investigations. Particular focus will be put on the condition of their formation and the dynamics of their maintenance and diabatic motions in the stratosphere.

How to cite: Podglajen, A., Legras, B., Lapeyre, G., Plougonven, R., and Zeitlin, V.: Idealized modeling of anticyclonic plumes from wildfires and volcanic eruptions in the stratosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13092, https://doi.org/10.5194/egusphere-egu23-13092, 2023.

EGU23-13146 | Posters on site | AS1.30

Positive anomalies in Carbon Monoxide concentrations observed in the upper troposphere - lower stratosphere during the 2022 Asian summer monsoon season 

Silvia Viciani, Marco Barucci, Giovanni Bianchini, Teresa Campos, Francesco D'Amato, Caroline Dang, Levi Golstone, Colin Gurganus, Laura Iraci, Alessio Montori, Kristen Okorn, James Podolske, and Emma Yates

In the framework of the ACCLIP project (Asian summer monsoon Chemical and CLimate Impacts project), a measurement campaign was conducted during summer 2022 in the Western Pacific region, to investigate the impact of the Asian Summer Monsoon (ASM) on the composition of the upper troposphere and lower stratosphere (UTLS). Fifteen research flights were carried out by the NASA WB-57 stratospheric aircraft and 14 by the NCAR/NSF GV, with base in Osan (South Korea), covering a large region on the eastern edge of the ASM anticyclone.

We report on the Carbon Monoxide (CO) measurements performed by three different mid-infrared absorption spectrometers (COLD2, COMA and ACOS) installed onboard the WB-57 and by two different infrared absorption spectrometers (Aerodyne-CO and Picarro G2401) installed on the GV. Positive CO anomalies, never measured before in the UTLS outside direct biomass burning plumes, were collected by all sensors, showing a very good agreement. During the flight of the 19th of August, CO mixing ratio values higher than 250 ppb were registered at altitude around 14-15 km.

A comparison with the CO observations measured by the instrument COLD2 during the StratoClim (Stratospheric and upper tropospheric processes for better Climate predictions) campaign, conducted in summer 2017 from Kathmandu (Nepal), will be presented. Particular attention will be paid to the CO difference observed in the UTLS, by sampling the anticyclone directly from the Tibetan Plateau during StratoClim campaign or from the Western Pacific during ACCLIP.

How to cite: Viciani, S., Barucci, M., Bianchini, G., Campos, T., D'Amato, F., Dang, C., Golstone, L., Gurganus, C., Iraci, L., Montori, A., Okorn, K., Podolske, J., and Yates, E.: Positive anomalies in Carbon Monoxide concentrations observed in the upper troposphere - lower stratosphere during the 2022 Asian summer monsoon season, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13146, https://doi.org/10.5194/egusphere-egu23-13146, 2023.

EGU23-13151 | Posters on site | AS1.30

Inter-comparison of different sensors for in-situ airborne measurements of Carbon Monoxide during ACCLIP campaign 

Francesco D'Amato, Marco Barucci, Giovanni Bianchini, Teresa Campos, Caroline Dang, Levi Golston, Colin Gurganus, Laura Iraci, Alessio Montori, Kristen Okorn, James Podolske, Silvia Viciani, and Emma Yates

A series of in-situ Carbon Monoxide (CO) observations were recently performed in the Western Pacific region, during summer 2022, in the framework of the ACCLIP project (Asian summer monsoon Chemical and CLimate Impacts Project). During the ACCLIP measurements campaign, located in Osan (South Korea), two different research aircraft were employed with a set of sensors installed onboard. The NASA WB-57 aircraft carried out 15 research flights (reaching a maximum altitude of about 19 km), and the NSF/NCAR Gulfstream (GV) aircraft carried out 14 research flights (reaching a maximum altitude of about 15 km), covering a large region near Korea and Japan.

We report on the inter-comparison between five different instruments for in-situ CO mixing ratio measurements: three installed onboard WB-57 (ACOS, COLD2 and COMA), and two installed onboard GV (Aerodyne-CO and Picarro G2401-m). COLD2 (Carbon Oxide Laser Detector 2) [1] and Aerodyne-CO [2] are mid-infrared Quantum Cascade Laser spectrometers, based on direct absorption in combination with a multipass cell. ACOS (Carbonyl Sulfide Analyzer) [3] and COMA (Carbon mOnoxide Measurement from Ames) [4] are mid-infrared absorption spectrometers based on Off-Axis ICOS (Integrated Cavity Output Spectroscopy) technology. The Picarro sensor is a cavity ring down absorption spectrometer [5].

The in-flight CO mixing ratio values measured by the five spectrometers will be compared, with particular attention to both the accuracy of each instrument and the adopted or not-adopted calibration procedures, as, in principle, for many measurement environments the two sensors based on direct absorption do not need in-flight calibration. Laboratory measurements of common primary and secondary calibration standards made by the five CO measurement groups will be presented to increase confidence in method accuracy.

 

[1] Viciani S., Montori A., Chiarugi A., and D’Amato F.: "A Portable Quantum Cascade Laser Spectrometer for Atmospheric Measurements of Carbon Monoxide", Sensors, 18, 2380 -1-18 (2018).

[2] https://www.eol.ucar.edu/instruments/carbon-monoxide-co-and-nitrous-oxide-n%E2%82%82o-qcl-instrument

[3] https://ams.confex.com/ams/103ANNUAL/meetingapp.cgi/Paper/421824

[4] https://espo.nasa.gov/acclip/instrument/COMA

[5] https://www.eol.ucar.edu/instruments/airborne-carbon-dioxide-co2-methane-ch4-carbon-monoxide-co-and-water-vapor-h2o

How to cite: D'Amato, F., Barucci, M., Bianchini, G., Campos, T., Dang, C., Golston, L., Gurganus, C., Iraci, L., Montori, A., Okorn, K., Podolske, J., Viciani, S., and Yates, E.: Inter-comparison of different sensors for in-situ airborne measurements of Carbon Monoxide during ACCLIP campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13151, https://doi.org/10.5194/egusphere-egu23-13151, 2023.

EGU23-13364 | ECS | Posters on site | AS1.30

Estimation of dichloromethane emissions in East Asia using recent high-altitude aircraft observations and synthesis inversion 

Zihao Wang, Chris Wilson, Wuhu Feng, Ying Li, Ryan Hossaini, Elliot Atlas, Eric Apel, David Oram, Karina Adcock, Stephen Donnelly, Roger Hendershot, Alan Hills, Rebecca Hornbrook, Johannes Laube, Richard Lueb, Thomas Röckmann, Sue Schauffler, Katie Smith, Victoria Treadaway, and Martyn Chipperfield

Although the Montreal Protocol has been successful in reducing the emissions of long-lived ozone-depleting substances, certain unregulated, chlorinated very short-lived substances (VSLS, lifetimes < 6 months) are believed to be having an increasing impact on stratospheric ozone depletion. The major sources of the chlorinated VSLS are anthropogenic. Emissions of chlorinated VSLS have been reported to be increasing from both bottom-up estimates and observations in recent years, among which dichloromethane (DCM) is the most abundant. Emissions from East Asia have been identified as contributing significantly to this increase (Oram et al., 2017; Claxton et al., 2020; Adcock et al., 2021; An et al., 2021).

Here we use synthesis inversion to derive an estimation of DCM emissions with a focus on East Asia, with input from the TOMCAT/SLIMCAT 3-D offline chemical transport model (CTM), a gridded annual global emission estimate, and aircraft observations from three recent campaigns - POSIDON (2016, https://csl.noaa.gov/projects/posidon/), StratoClim (2017, http://www.stratoclim.org/), and ACCLIP (2021, https://www2.acom.ucar.edu/acclip). The CTM contains the production and loss of DCM and is driven by reanalysed meteorology (Chipperfield, 2006), with gridded emission field of DCM (Claxton et al., 2020). In the model we set up more source regions than previous studies based on prior information, transport pathways into stratosphere, and the distribution of major city clusters. The inversion is performed by finding the minimum of the cost function (Tarantola and Valette, 1982): xa = xb+ [GTR-1G + B-1]-1GTR-1[y - Gxb], where y has the observations, xb is the prior estimate, B and R are the error covariance matrix of the prior estimates and the observations respectively, and G is the sensitivity matrix, as an operator mapping the emissions onto the observations by the CTM. Then xa can be calculated as known as the posterior estimate. Coupling the model and observations, xa is considered the best estimate and reduces the errors in the prior estimate.

We will present our analysis of DCM emissions up to the present day and compare them with previously published values and longer-term trends.

References:

Adcock et al., 2021, JGR Atmos., https://doi.org/10.1029/2020JD033137.

An et al., 2021, Nat. Commun., https://doi.org/10.1038/s41467-021-27592-y.

Chipperfield, 2006, QJR Meteorol. Soc., https://doi.org/10.1256/qj.05.51.

Claxton et al., 2020, JGR Atmos., https://doi.org/10.1029/2019JD031818.

Oram et al., 2017, ACP, https://doi.org/10.5194/acp-17-11929-2017.

Tarantola and Valette,1982, Rev. Geophys., https://doi.org/10.1029/RG020i002p00219.

How to cite: Wang, Z., Wilson, C., Feng, W., Li, Y., Hossaini, R., Atlas, E., Apel, E., Oram, D., Adcock, K., Donnelly, S., Hendershot, R., Hills, A., Hornbrook, R., Laube, J., Lueb, R., Röckmann, T., Schauffler, S., Smith, K., Treadaway, V., and Chipperfield, M.: Estimation of dichloromethane emissions in East Asia using recent high-altitude aircraft observations and synthesis inversion, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13364, https://doi.org/10.5194/egusphere-egu23-13364, 2023.

EGU23-13722 | ECS | Posters on site | AS1.30

Chemical analysis of the 2017 ATAL measured during StratoClim – New insights into refractory aerosol components 

Franziska Köllner, Oliver Appel, Antonis Dragoneas, Andreas Hünig, Sergej Molleker, Martin Ebert, and Stephan Borrmann

The chemical nature of the Asian aerosol tropopause layer (ATAL) was controversially discussed in the past decade. Modeling studies show the importance of black carbon and mineral dust aerosol for the formation of the ATAL (e.g., Bossolasco et al., 2021).  However, in-situ measurements at these high altitudes are sparse. We present the first in-situ measurements of the ATAL chemical composition conducted during the aircraft-based campaign StratoClim in July/August 2017 out of Kathmandu. Our ERICA instrument combines the laser desorption ionization mass spectrometry and the thermal desorption with subsequent electron impact ionization techniques, allowing measurements of refractory and non-refractory aerosol components. The ERICA is able to detect particles in the size range from 120 nm to 3500 nm (dva, d50 cutoff; Hünig et al., 2022). In parallel, particle samples were also collected in-situ and examined a-posteriori using scanning electron microscopy (SEM) and X-ray microanalysis (EDX). Results of both methods will be shown and discussed.

In our recent publication, we demonstrated that a large fraction (up to 70 %) of the ATAL particles is of purely secondary origin (Appel et al., 2022). Nitrate and organics are the dominant non-refractory components. In contrast to the secondary particle type, we found that a non-negligible fraction (up to 50 % in the lower ATAL region) of the particles include refractory components. In regions above 400 K potential temperature, the aerosol can be attributed to meteoric material (Schneider et al., 2021). Below 400 K, we found that refractory components are mainly linked to the presence of potassium, internally mixed with nitrate, sulfate, and organics. However, the vertical profile of elemental carbon (EC) shows its presence within the ATAL, albeit with an abundance in the lower percentage range. Likewise, the abundance of iron, sodium, and calcium indicative for the transport from ground sources is in the lower percentage range. Nonetheless, we observed these refractory particles in the boundary layer above Kathmandu with a higher abundance as compared to that within the ATAL. We thus assume that the transport efficiency of refractory particles from ground sources to the UTLS is strongly limited by wet deposition.  

Appel, O., Köllner, F., Dragoneas, A., et al.: Chemical analysis of the Asian tropopause aerosol layer (ATAL) with emphasis on secondary aerosol particles using aircraft-based in situ aerosol mass spectrometry, Atmos. Chem. Phys., 22, 13607–13630, https://doi.org/10.5194/acp-22-13607-2022, 2022.

Bossolasco, A., Jegou, F., Sellitto, P., et al.: Global modeling  studies of composition and decadal trends of the Asian Tropopause Aerosol Layer, Atmos. Chem. Phys., 21, 2745–2764, https://doi.org/10.5194/acp-21-2745-2021, 2021

Hünig, A., Appel, O., Dragoneas, A., et al.: Design, characterization, and first field deployment of a novel aircraft-based aerosol mass spectrometer combining the laser ablation and flash vaporization techniques, Atmos. Meas. Tech., 15, 2889–2921, https://doi.org/10.5194/amt-15-2889-2022, 2022.

Schneider, J., Weigel, R., Klimach, T., et al.: Aircraft-based observation of meteoric material in lower-stratospheric aerosol particles between 15 and 68° N, Atmos. Chem. Phys., 21, 989–1013, https://doi.org/10.5194/acp-21-989-2021, 2021.

How to cite: Köllner, F., Appel, O., Dragoneas, A., Hünig, A., Molleker, S., Ebert, M., and Borrmann, S.: Chemical analysis of the 2017 ATAL measured during StratoClim – New insights into refractory aerosol components, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13722, https://doi.org/10.5194/egusphere-egu23-13722, 2023.

EGU23-13833 | Orals | AS1.30

A process based definition of the extratropical transition layer 

Thorsten Kaluza, Peter Hoor, and Daniel Kunkel

The existence of the extratropical transition layer (ExTL) still lacks a physical process based explanation. It is yet an empirical finding based on the observed gradient changes of species within the lowermost stratosphere (LMS). The trace gas distribution directly results from localized and transient dynamical processes in the tropopause region. However, up to this point a dynamic- or process based definition of the ExTL remains an open research question, to large parts due to limitations of the available model and measurement data and resulting uncertainties in the assessment of the relevance of individual processes.

 

We present a synopsis of a series of recent research studies, which provide strong indications that tropopause-based wind shear and resulting dynamic instability is the key process for the formation of the ExTL. For this we use a multitude of different model and observational data sets, thus addressing the formation and maintenance of the ExTL from the chemical view, the process based dynamical view as well as from the large scale synoptics:

  • Process studies identify dynamic instability and turbulent cross-tropopause mixing based on trace gas measurements within distinct mesoscale layers of exceptional wind shear at the tropopause.

  • The analysis of several years of ECMWF ERA5 reanalysis data shows that these vertically confined transient layers of intense shear are a frequently occurring global scale feature, which is forced by the underlying large scale tropospheric dynamics.

  • The significance of this wind shear layer as a persistent source for dynamic instability and turbulent breakdown of the flow at the tropopause is validated with several years of operational EDR turbulence measurements from commercial aircraft.

How to cite: Kaluza, T., Hoor, P., and Kunkel, D.: A process based definition of the extratropical transition layer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13833, https://doi.org/10.5194/egusphere-egu23-13833, 2023.

EGU23-14150 | ECS | Posters on site | AS1.30

Cirrus clouds in the tropical tropopause layer observed at Koror, Palau (7.34°N, 134.47°E)  

Xiaoyu Sun, Mathias Palm, Christoph Ritter, and Justus Notholt

A Compact Cloud and Aerosol LIDAR (ComCAL) is operated in Koror, Palau (7.34°N, 134.47°E) since 2018. Palau is located in the Pacific warm pool, which plays an important role in global stratosphere-troposphere exchange in the upper troposphere and the lower stratosphere (UTLS). ComCAL is operated during nighttime, carried out observations of atmospheric profiles of aerosols and clouds, and the lidar profile extends from 8 km to 30 km. Cirrus clouds were detected with very high occurrence in the upper troposphere (above 12 km). The subvisible clouds (with an optical thickness of less than 0.3) often occur in the higher region of the tropical tropopause layer (TTL) above about 16 km which is close to the cold point. The transport of air in this layer with thin cirrus and subvisible clouds was investigated by the TRACZILLA Lagrangian model, a variation of FLEXPART. The back-trajectory analysis gives insight into the origins of cirrus clouds in the TTL whether it is related to the convection or the in situ uplifting of the air masses.

How to cite: Sun, X., Palm, M., Ritter, C., and Notholt, J.: Cirrus clouds in the tropical tropopause layer observed at Koror, Palau (7.34°N, 134.47°E) , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14150, https://doi.org/10.5194/egusphere-egu23-14150, 2023.

EGU23-14405 | ECS | Orals | AS1.30

Microphysical Modeling of Water Isotopic Composition in the Asian Summer Monsoon 

Benjamin Clouser, Carly KleinStern, Sergey Khaykin, Clare Singer, Laszlo Sarkozy, Silvia Viciani, Giovanni Bianchini, Francesco D'Amato, Alexey Lykov, Alexey Ulanovsky, Frank WIenhold, Bernard Legras, Cameron Homeyer, Troy Thornberry, and Elisabeth Moyer

The summertime Asian Monsoon (AM) is the single most important contributor to water vapor in the UTLS and overworld stratosphere. Much of that water comes from sublimating ice, but the life cycle of the condensate lofted by overshooting convection is not well understood. We report here on insights into that life cycle derived from the first in-situ measurements of water vapor isotopic composition over the Asian Monsoon. The Chicago Water Isotope Spectrometer (ChiWIS) flew on high-altitude aircraft in the monsoon center during the StratoClim (2017) campaign out of Nepal, and in monsoon outflow during ACCLIP (2022) out of South Korea. Both campaigns sampled a broad range of convective and post-convective conditions, letting us trace how convective ice sublimates, reforms, and leaves behind characteristic isotopic signatures. We use the Bin Resolved Isotopic Microphysical Model (BRIMM), along with TRACZILLA backtrajectories and convective interactions derived from cloud-top products, to follow the evolving isotopic composition along flight paths in both campaigns. Results support the wide diversity of isotopic enhancements seen in both campaigns and show how temperature cycles downstream of convective events progressively modify environmental isotopic compositions.

How to cite: Clouser, B., KleinStern, C., Khaykin, S., Singer, C., Sarkozy, L., Viciani, S., Bianchini, G., D'Amato, F., Lykov, A., Ulanovsky, A., WIenhold, F., Legras, B., Homeyer, C., Thornberry, T., and Moyer, E.: Microphysical Modeling of Water Isotopic Composition in the Asian Summer Monsoon, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14405, https://doi.org/10.5194/egusphere-egu23-14405, 2023.

EGU23-15699 | Orals | AS1.30 | Highlight

The NOAA Stratospheric Aerosol processes, Budget and Radiative Effects (SABRE) Project 

Troy Thornberry and Eric Jensen

Stratospheric aerosols are an important component of Earth’s albedo, and therefore energy balance, and provide surface area for heterogeneous chemistry, which can lead to stratospheric ozone loss. Acquiring a comprehensive database of stratospheric aerosol, trace gas and dynamical observations to establish the baseline state and background variability of the stratosphere is essential to (1) developing a complete understanding of stratospheric dynamical and chemical processes that determine aerosol microphysics, radiative properties and heterogeneous chemistry, (2) evaluating the stratospheric response to natural and anthropogenic perturbations including climate change, volcanic eruptions, and potential climate intervention activities, and (3) strengthening the scientific foundation to inform policy decisions related to regulating global emissions that impact the stratosphere.

The NOAA Stratospheric Aerosol processes, Budget and Radiative Effects (SABRE) project is a multi-year, multi-deployment UTLS airborne science measurement program to study the microphysics, transport, chemistry and radiative properties of aerosols in the upper troposphere and lower stratosphere (UTLS).  The SABRE instrument payload and flight campaigns are designed to provide extensive, detailed measurements of aerosol size distributions, composition and radiative properties along with relevant trace gas species in different regions and seasons, which are critical for improving the ability of global models to accurately simulate the radiative, dynamical and chemical impacts of changes in stratospheric aerosol loading.

The first deployment of the SABRE project took place in February 2022, consisting of six flights from Ellington Field, Houston, TX. The flights provided an opportunity to field test several newly developed instruments that will be important for addressing SABRE science questions in subsequent deployments and sampled both the subtropical tropopause layer and midlatitude upper troposphere and lower stratosphere. The Realtime Air Quality Modeling System (RAQMS) was used for flight planning to target atmospheric dynamical features and species gradients. Complex structure was observed in trace gases and aerosol in the midlatitude UTLS, indicating significant stratosphere-troposphere exchange. Highlights from the deployment will be presented.

Subsequent SABRE deployments will target aspects of the stratospheric aerosol budget including high latitude processes with a deployment to Alaska in February-March 2023 and to the tropics to study Tropical Tropopause Layer (TTL) processes in 2024. Each deployment will also include flights from Houston, TX to investigate seasonal and interannual variability in the subtropical and midlatitude stratosphere.

How to cite: Thornberry, T. and Jensen, E.: The NOAA Stratospheric Aerosol processes, Budget and Radiative Effects (SABRE) Project, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15699, https://doi.org/10.5194/egusphere-egu23-15699, 2023.

EGU23-16187 | Posters on site | AS1.30

Study of clear air turbulence (detection, observation, generation) in the Tropical Upper Troposphere-Lower Stratosphere (UTLS) 

Clara Pitois, Richard Wilson, Aurélien Podglagen, Albert Hertzog, Milena Corcos, and Riwal Plougonven

The role played by turbulent mixing in the vertical transport of constituents in the UTLS is still poorly understood: there is a lack of knowledge of turbulence due to the limited number of observations in this region as well as to the limitations of current observation techniques.

The first part of the present work deals with the detection of small-scale turbulence in the tropical upper troposphere - lower stratosphere from in-situ meteorological measurements collected under super-pressure balloons (SPBs). Eight SPBs were launched during the first Strateole-2 campaign, from November 2019 to March 2020 and flying for several weeks (∼ 3 months). 

Turbulence detection methods relies on the quasi-periodic vertical oscillations (∼ ±15 m) of the SPBs around their equilibrium positions, such oscillations inducing large fluctuations of measured quantities (pressure, temperature, positions) and inferred quantities (density, potential temperature). A first method of detection is based on correlations between the increments of potential temperature δθ and the vertical displacements of the balloons (i.e. of the sensors) δz. Such correlations are expected to be null as ∂θ/∂z → 0 in case of turbulent mixing. A second method relies on the Richardson number criterion, Ri < 0.25. Ri is deduced from the vertical gradients of measured quantities (T , u, v), estimated from covariances between the increments of the considered quantities and the vertical displacements δz. 

Turbulence indexes (true of false) to describe the different states of the flow encountered by the SPBs during their flights (laminar or turbulent), are evaluated. These different indexes, based on independent measurements and on various methods, correlations or linear regressions, are found to be consistent: they differ for less than 3% of the cases. The flow is observed to be turbulent for about 5% of the time, with strong inhomogeneities along the longitude.

The second part of the present work aims to improve our understanding of turbulence, and its impacts, in the tropical UTLS by studying small- to meso-scale processes, i.e. atmospheric waves, deep convection and associated observed turbulence. These are all key processes of the dynamics of the equatorial UTLS. One can evaluate the probability of turbulence occurrences as a function of the distance to deep convection. Such a distance seems to be a good proxy of wave activity generated by deep convection. The occurrence frequency of turbulence is significantly larger when the distance to deep convection is small, i.e. smaller than ~ 200 km.

This research should contribute to a better parametrization of these processes in climate models, and to a better estimation of their impact to vertical transport in the tropical UTLS.

How to cite: Pitois, C., Wilson, R., Podglagen, A., Hertzog, A., Corcos, M., and Plougonven, R.: Study of clear air turbulence (detection, observation, generation) in the Tropical Upper Troposphere-Lower Stratosphere (UTLS), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16187, https://doi.org/10.5194/egusphere-egu23-16187, 2023.

A balloon-borne fiber optic distributed temperature sensing instrument named the Fiber-optic Laser Operated Atmospheric Temperature Sensor, or FLOATS, was used to retrieve continuous vertical temperature profiles spanning approximately 1.6 km within the tropical UTLS as part of the Stratéole 2 2021 balloon mission. In one isopycnic flight, flying at 18.5 km over the Indian Ocean and the Maritime continent, FLOATS retrieved nearly 22 days of temperature profiles with a sampling period of less than 10 minutes. The superpressure balloon flight demonstrated the applicability of distributed temperature sensing for ambient atmospheric temperature measurements and for analysis of dynamics within the UTLS. The temperature retrievals show good agreement with on-board reference sensors demonstrating the effectiveness of the in-flight calibration procedures. Comparisons to nearby meteorological soundings and COSMIC-2 temperature profiles were conducted for validation and to survey energy fluxes on the fiber optic cable including solar radiative heating and radiative cooling at night. Temperature perturbations retrieved from the FLOATS profiles are used to investigate small-scale and large-scale dynamics within the tropical tropopause layer.

How to cite: Kalnajs, L., Goetz, J. D., Alexander, M. J., and Bramberger, M.: Continuous temperature profiles within the tropical tropopause layer with fiber optic distributed temperature sensing aboard long duration constant altitude balloons in Stratéole 2, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17223, https://doi.org/10.5194/egusphere-egu23-17223, 2023.

EGU23-90 | Posters on site | HS7.8

Embracing Large-sample Data to Characterize Streamflow Extremes at a Global-scale 

Sai Kiran Kuntla and Manabendra Saharia

The recurrent and destructive nature of floods causes enormous economic damage and loss of human lives, leaving people in flood-prone areas fearful and insecure. It is essential to have a thorough knowledge of the factors that contribute to it. However, most catchment characterization studies are limited to case studies or regional domains. A detailed global characterization is currently unavailable due to the limitation in the holistic dataset that it demands. This study aims to fill this gap by utilizing multiple global datasets describing physiographic explanatory variables to characterize streamflow extremes. The role of catchment features such as landcover, geomorphology, climatology, lithology, etc., on spatial patterns and temporal changes of high streamflow extremes, was investigated in detail. Moreover, the multidimensional correlations between streamflow extremes and catchment features were modeled using a Random Forest approach and integrated with an interpretable machine learning framework to find the most dominating elements in different climate classes. The interpretation reveals that climatological variables are the most influential across all climates. However, the variables and their influences fluctuate between climates. Furthermore, distinct geomorphological variables dominate throughout climatic classes (such as basin relief in warm temperate and drainage texture in arid climates). Overall, the insights of this study would play a vital role in estimating the unit peak discharge at ungauged stations based on known watershed features. In addition, these findings can also help assess the nature of extremes in future climate scenarios, consequently implicating risk management methods.

How to cite: Kuntla, S. K. and Saharia, M.: Embracing Large-sample Data to Characterize Streamflow Extremes at a Global-scale, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-90, https://doi.org/10.5194/egusphere-egu23-90, 2023.

EGU23-230 | ECS | Orals | HS7.8

The role of spatial dependence in global-scale coastal flood risk assessment 

Huazhi Li, Toon Haer, Alejandra Enríquez, and Philip Ward

Coastal flooding is among the world’s deadliest and costliest natural hazards. The impacts caused by coastal flooding can be particularly high when an event affects a large spatial area, as witnessed during Hurricane Katrina and Cyclone Xaver. Current large-scale flood risk studies assume that the probabilities of water levels during such events do not vary in space. This failure to capture flood spatial dependence can lead to large misestimates of the hazard and risk at large spatial scales, and therefore potentially misinform the risk management community. In this contribution, we assess the effects of spatial dependence on coastal flood risk estimation at the global scale. To this end, we compare the assessments using two spatial dependence scenarios: i) complete dependence and ii) modelled dependence of water level return periods. For the complete dependence scenario, we use the existing risk information calculated by the GLOFRIS global risk modelling framework. To estimate the spatially-dependent risks, we use an event-based multivariate statistical approach and consider 10,000-year extreme coastal flood events derived from the global synthetic dataset of spatially-dependent extreme sea levels. The associated spatially coherent return periods of each event are then combined with the GLOFRIS spatially-constant inundation layers to create the spatially-dependent inundation map. These hazard maps, overlaid with exposure layers and vulnerability information, are further used to assess the coastal flood impacts. The flood risk is estimated using Weibull’s plotting formula and presented in terms of expected annual population and expected annual damage. This study will improve our understanding of flood spatial dependence and will provide improved risk estimation at the global scale. Such reliable estimates could lead to improved large-scale flood risk management through better wide-area planning decisions, more accurate insurance coverage, and better emergency response. 

How to cite: Li, H., Haer, T., Enríquez, A., and Ward, P.: The role of spatial dependence in global-scale coastal flood risk assessment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-230, https://doi.org/10.5194/egusphere-egu23-230, 2023.

EGU23-1384 | Orals | HS7.8

Estimating very rare floods at multiple sites in a large river basin with comprehensive hydrometeorological simulations 

Daniel Viviroli, Anna E. Sikorska-Senoner, Guillaume Evin, Maria Staudinger, Martina Kauzlaric, Jérémy Chardon, Anne-Catherine Favre, Benoit Hingray, Gilles Nicolet, Damien Raynaud, Jan Seibert, Rolf Weingartner, and Calvin Whealton

Rare to very rare floods (associated to return periods of 1'000–100'000 years) can cause extensive human and economic damage. Still, their estimation is limited by the comparatively short streamflow records available. Some of the limitations of commonly used estimation methods can be avoided by using continuous simulation (CS), which considers many simulated meteorological configurations and a conceptual representation of hydrological processes. CS also avoids assumptions about antecedent conditions and their spatial patterns.

We present an implementation of CS to estimate rare and very rare floods at multiple sites in a large river basin (19 locations in the Aare River basin, Switzerland; area: 17'700 km²), using exceedingly long simulations from a hydrometeorological model chain (Viviroli et al., 2022). The model chain consisted of three components: First, the multi-site stochastic weather generator GWEX provided 30 meteorological scenarios (precipitation and temperature) spanning 10'000 years each. Second, these weather generator simulations were used as input for the bucket-type hydrological model HBV, run at an hourly time step for 80 catchments covering the entire Aare River basin. Third, runoff simulations from the individual catchments were routed for a representation of the entire Aare River system using the routing system model RS Minerve, including a simplified representation of main river channels, major lakes and relevant floodplains. The final simulation outputs spanned about 300'000 years at hourly resolution and cover the Aare River outlet, critical points further upstream as well as the outlets of the hydrological catchments. The comprehensive evaluation over different temporal and spatial scales showed that the main features of the meteorological and hydrological observations were well represented. This implied that meaningful information on floods with low probability can be inferred. Although uncertainties were still considerable, the explicit consideration of important flood generating processes (snow accumulation, snowmelt, soil moisture storage) and routing (bank overflow, lake regulation, lake and floodplain retention) was a substantial advantage compared to common extrapolation of streamflow records.

The suggested approach allows for comprehensively exploring possible but unobserved spatial and temporal patterns of hydrometeorological behaviour. This is particularly valuable in a large river basin where the complex interaction of flows from individual tributaries and lake regulations are typically not well represented in the streamflow records. The framework is also suitable for estimating more common, i.e., more frequently occurring floods.

Reference

Viviroli D, Sikorska-Senoner AE, Evin G, Staudinger M, Kauzlaric M, Chardon J, Favre AC, Hingray B, Nicolet G, Raynaud D, Seibert J, Weingartner R, Whealton C, 2022. Comprehensive space-time hydrometeorological simulations for estimating very rare floods at multiple sites in a large river basin. Natural Hazards and Earth System Sciences, 22(9), 2891–2920, doi:10.5194/nhess-22-2891-2022

How to cite: Viviroli, D., Sikorska-Senoner, A. E., Evin, G., Staudinger, M., Kauzlaric, M., Chardon, J., Favre, A.-C., Hingray, B., Nicolet, G., Raynaud, D., Seibert, J., Weingartner, R., and Whealton, C.: Estimating very rare floods at multiple sites in a large river basin with comprehensive hydrometeorological simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1384, https://doi.org/10.5194/egusphere-egu23-1384, 2023.

EGU23-2129 | Posters on site | HS7.8

The Prevalence and Impact of Heavy Tails on Hydrologic Extremes and Other Statistics 

Richard Vogel, Jonathan Lamontagne, and Flannery Dolan

The prevalence of heavy tailed (HT) populations in hydrology is becoming increasingly commonplace due in part to the increasing need and use of high frequency and high-resolution data.   In addition to the impact of HT on extremes, HT populations can have a profound impact on a wide range of other hydrologic statistics and methods associated with planning,  management and design for  extremes.   We review the known impacts of HT populations on the instability and bias in a wide range of commonly used hydrologic statistics. Experiments reveal that HT distributions result in the degradation of many commonly used statistical methods including the bootstrap, probability plots, the central limit theorem, and the law of large numbers.     We document the gross instability of perhaps the best-behaved statistic of all, the sample mean (SM) when computed from HT distributions.  The SM is ubiquitous because it is a component of and related to a myriad of statistical methods, thus its unstable behavior provides a window into future challenges faced by the hydrologic community.  We outline many challenges associated with HT data, for example, upper product moments are often infinite for HT populations, yet upper L-moment always exist, so that the theory of L-moments is uniquely suited to HT distributions and data.  We introduce a magnification factor for evaluating the impact of HT distributions on the behavior of extreme quantiles

How to cite: Vogel, R., Lamontagne, J., and Dolan, F.: The Prevalence and Impact of Heavy Tails on Hydrologic Extremes and Other Statistics, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2129, https://doi.org/10.5194/egusphere-egu23-2129, 2023.

Extreme wildfires continue to be a significant cause of human death and biodiversity destruction across the globe, with recent worrying trends in their activity (i.e., occurrence and spread) suggesting that wildfires are likely to be highly impacted by climate change. In order to facilitate appropriate risk mitigation for extreme wildfires, it is imperative to identify their main drivers and assess their spatio-temporal trends, with a view to understanding the impacts of global warming on fire activity. To this end, we analyse monthly burnt area due to wildfires using a hybrid statistical deep-learning framework that exploits extreme value theory and quantile regression. Three study regions are considered: the contiguous U.S., Mediterranean Europe and Australia.

How to cite: Richards, J. and Huser, R.: Insights into the drivers and spatio-temporal trends of extreme wildfires with statistical deep-learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2332, https://doi.org/10.5194/egusphere-egu23-2332, 2023.

EGU23-2974 | ECS | Orals | HS7.8

Stochastic Generation of Snow Depth in Canada 

Hebatallah Abdelmoaty and Simon Papalexiou

Snow depth is a significant component in the hydrological cycle and global energy and water balances, contributing to climate change impacts. Weather stations with gauges for snow depth are scarce, especially in complex terrain regions, and require high accuracy for measurements. Advances in observational systems offer unconventional solutions yet are expensive. To bridge these gaps, stochastic generation methods offer a cost-effective solution to reproduce time series of hydrological variables, preserving their stochastic properties. Stochastic generation methods are well-established for total precipitation but lack snow depth generation. Here, we introduce a stochastic method to exclusively generate snow depth time series that preserve their distinct statistical properties on different time scales. We use 450 observed snow depth time series and 470 CMIP6 simulations to detect Canada's observed and physical statistical properties. The results indicate that snow depth has a light tail, and the distribution might change daily. The probability of zero snow depth shows a clear seasonal pattern. The synthetic snow depth time series can be an alternative to climate models’ outputs, offering a computationally effective solution to investigate the snow depth variability. This method advances the generation of stochastic time series of snow depth and can be applied to investigate catastrophes from snowmelt processes and avalanches that lead to severe damage and fatalities.

How to cite: Abdelmoaty, H. and Papalexiou, S.: Stochastic Generation of Snow Depth in Canada, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2974, https://doi.org/10.5194/egusphere-egu23-2974, 2023.

EGU23-3709 | Posters on site | HS7.8

Spatial and Temporal Evolution of Drought Events Using High-Resolution SPEI and Dynamic Drought Detection Algorithm 

Jiyoung Yoo, Jiyoung Kim, Hyun-Han Kwon, and Tae-Woong Kim

Drought is one of the world's major natural disasters. In order to monitor drought and reduce drought damage through preemptive response, it is important to understand the spatiotemporal evolutionary characteristics of drought. Droughts have a three-dimensional (3-D) space-time structure, typically spanning hundreds of kilometers and lasting months to years. In this study, a high-resolution(5 km) SPEI-HR(Standardized Precipitation Evaporation Index) dataset was used, considering climatic (typical temperate continental climate) and various geographic characteristics (mountainous terrain, lowland basin, desert, grassland, etc.). In addition, all large- and small-scale drought events that evolve spatiotemporally were extracted using the dynamic drought detection technique (DDDT) algorithm. These 3D-drought properties are important information to explain the spatiotemporal evolution of drought and are characterized by drought patches in dynamic drought maps. As a result, most of the trajectories of droughts in Central Asia during the period 1981 to 2018 tended to move laterally to the east and west (ENE, E, ESE, WNW, W, WSW). In addition, droughts in Central Asia are characterized by very strong correlations between indicators of duration, severity, area, and trajectory movement distance. These Central Asian drought characteristics are interpreted as meaning that there is consistency among various drought information in determining the most severe drought event. In addition, the dynamic drought map, which includes all 3D-drought properties, has the advantage of producing high-level drought information (temporal continuity of drought events and dynamic evolution characteristics, etc.) that are not found in general drought maps through various conditional drought monitoring.

Acknowledgements: This work was supported by the National Research Foundation of Korea (No. NRF-2020R1C1C1014636) and Korea Environment Industry & Technology Institute (KEITI) (No.2022003610001) funded by the Korean government (MSIT and MOE).

How to cite: Yoo, J., Kim, J., Kwon, H.-H., and Kim, T.-W.: Spatial and Temporal Evolution of Drought Events Using High-Resolution SPEI and Dynamic Drought Detection Algorithm, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3709, https://doi.org/10.5194/egusphere-egu23-3709, 2023.

EGU23-3851 | ECS | Posters on site | HS7.8

On the Projected Changes in the Seasonality and Magnitude of Precipitation Extremes 

Dario Treppiedi, Gabriele Villarini, Jens Bender, and Leonardo Noto

Heavy precipitation events are strongly affected by climate change and there is a high confidence that these extremes will become more frequent and more severe in the future. Moreover, potential changes in the seasonality of these events are important in terms of planning and preparation against these events. While efforts have been focused on changes in the magnitude and seasonality of extreme precipitation events, these studies have treated these two quantities separately.

In order to overcome to this limit, a different perspective is here used by modeling the seasonality and magnitude of extreme precipitation events together through circular-linear copulae. We perform analyses at the global scale and develop bivariate models for an historical dataset. The outputs provided from several global climate models from the sixth phase of the Coupled Model Intercomparison Project (CMIP6) and Shared Socioeconomic Pathways (SSPs) from 1-2.6 to 5-8.5 are then used to examine the joint projected changes in the seasonality and magnitude of extreme precipitation at the global scale.

How to cite: Treppiedi, D., Villarini, G., Bender, J., and Noto, L.: On the Projected Changes in the Seasonality and Magnitude of Precipitation Extremes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3851, https://doi.org/10.5194/egusphere-egu23-3851, 2023.

Spatially co-occurring floods pose a great threat to the resilience and the recovery potential of the communities. A timely forecasting of such events plays a crucial role for increasing the preparedness of public and private sectors and for limiting the associated losses. In this study we investigated the potential of dilated Convolutional Neural Networks (CNN) conditioned on a set of large-scale climatic indexes and antecedent precipitation for monthly forecast of widespread flooding severity in Germany using 63 years of streamflow observations. The severity of widespread flooding (i.e., spatially co-occurring floods) was estimated as simultaneous (within a given month) exceedance of an at-site two-year return period for streamflow peaks across 172 mesoscale catchments. The model was trained for the whole country and for the three diverse hydroclimatic regions individually to provide insights on spatial heterogeneity of model performance and drivers of flooding. Evaluation of the model skill for floods generated by different processes revealed the largest bias for events generated during dry conditions. The bias for rain-on-snow flood events was the lowest despite their higher severity indicating higher predictability of these events from large scale climatic indexes. Model-based feature attribution and independent wavelet coherence analyses both indicated considerable difference in the major drivers of widespread flooding in different regions. While the flooding in the North-Eastern region is strongly affected by the Baltic Sea (e.g., East Atlantic pattern), the North-Western region is affected more by global patterns associated with the El-Niño activity (e.g., Pacific North American pattern). In the Southern region in addition to the effect of the global patterns we also detect the effect of the Mediterranean Sea (Mediterranean Oscillation Index), while antecedent precipitation seems to play less important role in this region compared to the rest of the country. Our results indicate a considerable potential for forecasting widespread flood severity using dilated CNN especially as the length of the available time series for training increases.

How to cite: Tarasova, L., Ahrens, B., Hoff, A., and Lall, U.: Forecasting the monthly severity of widespread flooding in Germany using dilated convolutional neural networks conditioned by large-scale climatic indexes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4419, https://doi.org/10.5194/egusphere-egu23-4419, 2023.

EGU23-5298 | ECS | Posters on site | HS7.8

A spatial covariates model for storm surge extremes in the German Bight 

Gabriel Ditzinger, Henning Rust, Jens Möller, Tim Kruschke, Laura Schaffer, and Claudia Hinrichs

Storm surges and accompanying extreme water levels pose a major threat to coastal structures, urban and industrial areas and human life in general. In order to develop effective risk mitigation strategies, it is crucial to improve the understanding of these extreme events as well as their occurrence probabilities and quantiles, respectively.

The standard procedure to estimate extreme quantiles (return-levels) is to fit a suitable distribution to the observed extreme values on a site-by-site basis. However, this approach exhibits some disadvantages: 1) Estimates of extreme quantiles are only available at gauged locations. 2) The small amount of extreme events in tide gauge records makes these estimates highly uncertain.

We tackle both issues by pooling all available tide gauge records together through a covariates model that allows for smoothly varying distribution parameters in space. Using this approach, the model is not only able to reduce the uncertainty in quantile estimates, but also enables the interpolation of the distribution parameters at arbitrary ungauged locations, e.g. in between tide gauge locations.

Deploying our model for the German North Sea coast, we generate a probabilistic reanalysis of extreme water levels as well as associated probabilities for the period 2000 – 2019.

How to cite: Ditzinger, G., Rust, H., Möller, J., Kruschke, T., Schaffer, L., and Hinrichs, C.: A spatial covariates model for storm surge extremes in the German Bight, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5298, https://doi.org/10.5194/egusphere-egu23-5298, 2023.

Statistical dependency measures such as Kendall’s Tau or Spearman’s Rho are frequently used to analyse the coherence between time series in environmental data analyses. Autocorrelation of the data can however result in spurious cross correlations if not accounted for. Here, we present the asymptotic distribution of the estimators of Spearman’s Rho and Kendall’s Tau, which can be used for statistical hypothesis testing of cross-correlations between autocorrelated observations. The results are derived using U-statistics under the assumption of absolutely regular (or β-mixing) processes. These comprise many short-range dependent processes, such as ARMA-, GARCH- and some copula-based models relevant in the environmental sciences. We show that while the assumption of absolute regularity is required, the specific type of model does not have to be specified for the hypothesis test. Simulations show the improved performance of the modified hypothesis test for some common stochastic models and small to moderate sample sizes under autocorrelation. The methodology is applied to observed time series of flood discharges and temperatures in Europe and yields results that are consistent with the literature on flood regime changes in Europe. While the standard test results in spurious correlations between floods and temperatures, this is not the case for the proposed test, which is more consistent with the literature on flood regime changes in Europe.

How to cite: Lun, D., Fischer, S., Viglione, A., and Blöschl, G.: Attribution of flood changes with time series in the presence of autocorrelation: Modifications for Spearman‘s Rho and Kendall‘s Tau, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7352, https://doi.org/10.5194/egusphere-egu23-7352, 2023.

EGU23-7564 | ECS | Posters on site | HS7.8

Areal extremes from a different perspective: rainfall as 2D and 3D connected objects. 

Abbas El Hachem, Jochen Seidel, and András Bárdossy

Using the German weather radar data for the last 20 years with a high spatial and temporal resolution, the occurrence of rainfall extremes was analysed. By extracting and examining connected rainfall areas, several research questions were investigated: (1) How many extremes occur in a given area independent of their location? (2) To what extent is their occurrence in space a random and to what extent a structured process? (3) How are the connected volumes behaving in space and time? (4) How does the areal extent relate to event duration, rainfall volume, and discharge volume? The first two research questions were investigated for all of Germany, the last two by analysing rainfall and run-off data in several small and medium size headwater catchments in southern and western Germany.

The results show that the occurrence of events in space is related to their areal extent; there are regions where the frequency of occurrence of large spatially distributed events is greater than that of smaller ones. Moreover, there are interesting relationships between the spatial extent of an event, the event duration, and the event rainfall volumes. For high discharge values, not only does the rainfall intensity matter but also the event duration and spatial distribution of rainfall within a catchment. Many discharge peaks are not necessarily caused by high-intensity events (hourly or daily maxima) but by the accumulation of rainfall cells in space and time.

How to cite: El Hachem, A., Seidel, J., and Bárdossy, A.: Areal extremes from a different perspective: rainfall as 2D and 3D connected objects., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7564, https://doi.org/10.5194/egusphere-egu23-7564, 2023.

Alaba Boluwade*

School of Climate Change & Adaptation, University of Prince Edward Island, Charlottetown, Canada; aboluwade@upei.ca; abolu2013@gmail.com

*Correspondence: aboluwade@upei.ca

Abstract

Hydrological risk assessment, such as flood protection, requires estimates of variables (e.g., precipitation) measured from several weather stations. The spatial modeling of average rainfall estimates differs from extreme precipitation analysis. This is because extremes are focused on the tail of the probability distribution and the assumption of Gaussianity may not be suitable. Extreme Value Theory (EVT) application to univariate weather variables measured at weather stations has been well documented; however, extreme precipitation at closer stations tend to show trends and dependencies (similar values). It is, therefore, crucial to quantify the dependency structure and trend surface of weather stations in space. The max-stable process has been well documented to model spatial extremes. The objective of this study is to quantify the spatial dependency and trend of an annual maxima precipitation (annual highest daily precipitation, from 1970-2020) across selected weather stations in the Northern Great Plains (i.e., Nelson Churchill River Basin (NCRB)) of North America. The annual maxima data were extracted from the Global Historical Climatology Network Daily (GHCNd) and Environment and Climate Change Canada (ECCC). NCRB covers four states and four provinces in the United States and Canada. A heterogenous rainfall pattern characterizes NCRB. This is due to enormous quantities of orographic rainfall in the west and the convective precipitation in the Prairies (which is dominated by short-duration, sporadic, extreme rain), causing millions of dollars in damages. This study uses max-stable processes to examine spatial extremes of annual maxima precipitation.

The results show that topography, time, and geographical coordinates were important covariates in reproducing the stochastic extreme precipitation field using the spatial generalized extreme value (SPEV). Takeuchi’s information criterion (TIC) shows that the SPEV model with all the covariates above superseded the one without the covariates.   The inclusion of time as a covariate further confirms the impacts of climate change on extreme precipitation in the NCRB. The fitted Extremal-t max-stable model captured the spatial dependency and equally predicted the 50-year return period levels. Furthermore, ten realizations (equal probable) were simulated from the max-stable model. The study is relevant in quantifying the spatial trend and dependency of extreme precipitation in the Northern Great Plains. The result will help as a decision-support system in climate adaptation strategies in the United States and Canada.

 

Keywords: extreme events; Max-Stable processes; flood protection; maxima annual rainfall; flash flood protection; Canada, United States

How to cite: Boluwade, A.: Application of Max-Stable Process Model in Estimating the Spatial Trend & Dependency of Extremes in the Northern Great Plains, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9758, https://doi.org/10.5194/egusphere-egu23-9758, 2023.

EGU23-10538 | ECS | Orals | HS7.8

Improved data assimilation in regional frequency analysis of rainfall extremes across large and morphologically complex geographical areas 

Andrea Magnini, Michele Lombardi, Taha B. M. J. Ouarda, and Attilio Castellarin

In locations where measured timeseries are not available or not sufficiently long, reliable predictions of the rainfall depth associated with a given duration and exceedance probability may be obtained through regional frequency analysis (RFA). The scientific literature reports on a large number of different approaches to RFA of rainfall extremes, each one characterized by specific advantages and disadvantages. One of the most common drawbacks is that regional models specifically refer to a single duration or a single exceedance probability. Second, several approaches require the definition of a homogeneous region where the model is trained; this leads to higher accuracy, but also the applicability of the model is limited to those locations that are hydrologically similar to the homogeneous group used in the training. Moreover, most models require filtering the available gauged stations based on the length of the measured timeseries to perform reliable frequency analysis. These aspects lead to discard a significant amount of data, which could turn out to be detrimental to the accuracy of the regional prediction in some cases.

We set up a few alternative models aiming to investigate and discuss a different and innovative approach for RFA of rainfall extremes. We want to address three main research questions: (1) Can a single model represent the frequency of extreme rainfall events over a large, climatically, and morphologically complex geographical area? (2) Can a single RFA model handle all sub-daily  durations (i.e., from 1 to 24h)? (3) Is it possible to exploit all available annual maximum series, regardless of their length (i.e., very short ones too)? We select a large study area that is located in north-central Italy. We make use of more than 2300 Annual Maximum Series of rainfall depth for different time-aggregation intervals between 1 and 24 hours, that have been collected between 1928 and 2011 in the Italian Rainfall Extreme Dataset (I2-RED). For each gauged station, several morpho-climatic descriptors are retrieved (e.g., minimum distance to the coast, elevation of orographic barriers, aspect, terrain slope, etc.) and used as covariates for the prediction models. Our models are based on ensembles of unsupervised artificial neural networks (ANNs) and are able to predict parameters of a Gumbel distribution for any location and any duration in the 1-24 hours range based on the morphoclimatic descriptors. Through the analysis of results over 100 gauged validation stations, a profitable discussion is enabled on the potential and drawbacks of ensembles of unsupervised ANNs for regional frequency analysis of sub-daily rainfall extremes.

How to cite: Magnini, A., Lombardi, M., Ouarda, T. B. M. J., and Castellarin, A.: Improved data assimilation in regional frequency analysis of rainfall extremes across large and morphologically complex geographical areas, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10538, https://doi.org/10.5194/egusphere-egu23-10538, 2023.

EGU23-11332 | Posters on site | HS7.8

Interpolation of design rainfall at ungauged locations exploiting the potential of convection-permitting climate models. 

Giuseppe Formetta, Francesco Marra, Eleonora Dallan, and Marco Borga

Quantifying design rainfall events at varying durations is crucial for assessing flood risk and mitigating losses and damages. Yet, in a changing climate, they are fundamental tool for a reliable design of water related infrastructures, such as flood retention reservoirs, spillways, and urban drainage systems. Usually, design rainfall is quantified where rain gauges are located, and regionalization methods are used to provide estimates in ungauged locations. During the last years, convection-permitting climate models (CPM) are receiving increasing attention because, thanks to their high spatial resolution (~3km) and ability of explicitly resolving atmospheric convection, they allow for better estimating precipitation spatial patterns and extreme rainfall at multiple durations compared to coarser models.

In this work, we combine at-site rain gauge measurements with CPM simulations, within a non-asymptotic statistical framework for the analysis of extreme rainfall. We aim at quantifying the added value of the physics-based information provided by CPM simulations for the estimation of high quantiles of rainfall in ungauged locations.     

The performance of the new regionalization approach is compared with traditional interpolation methods (i.e. interpolation of distribution function parameters) using leave- one-out cross-validation as well as considering different rain gauge densities.

Preliminary results show that the proposed methodology based on CPM simulation provides: i) similar performances compared to traditional gauge-based regionalization methods for high station density scenarios and ii) improved performances for low station density scenarios.

How to cite: Formetta, G., Marra, F., Dallan, E., and Borga, M.: Interpolation of design rainfall at ungauged locations exploiting the potential of convection-permitting climate models., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11332, https://doi.org/10.5194/egusphere-egu23-11332, 2023.

EGU23-11828 | ECS | Posters on site | HS7.8

The Future of Extreme Event Risk Assessment: A Look at Multivariate Return Periods in More than Three Dimensions 

Diego Armando Urrea Méndez, Dina Vanesa Gómez Rave, and Manuel Del Jesus Peñil

The multivariate return period is a measure of the frequency with which simultaneous sets of variables are expected to occur in a given area. So far, most approaches to calculate the multivariate return period of various hydrological variables have used copulas in two and three dimensions. (Salvadori et al., 2011) proposed a methodology for calculating the return period based on Archimedean copulas and the Kendall measure in 2 and 3 dimensions. (Gräler et al., 2013) proposed the calculation of the trivariate return period based on Vine copulas and Kendall distribution functions to describe the characteristics of the design hydrogram, considering the annual maximum peak discharge, its volume and duration. (Tosunoglu et al., 2020) applied three-dimensional Archimedean, Elliptical and Vine copulas to study the characteristics of floods. These studies have shown that the use of copulas can improve the accuracy of the risk measure of extreme events compared to univariate approaches, that only consider one variable at a time.

One of the limitations in describing the occurrence of multivariate extreme involving more than three simultaneous variables is the complex mathematical model to be solved (highest probability density point of a hypersurface) and the high computational cost that this imposes. However, in some areas of hydrology, developing more robust analyses that consider more than three variables can further improve risk assessments. For example, considering multiple rainfall stations in a watershed may help to properly capture the spatial structure of extremes -instead of relying on other spatial distribution procedures-. This improvement can provide a more accurate measure of the return period in the design of critical infrastructure, flood prediction, risk plans, etc.

In this context, we present an application where an extreme characterization of 5 rain gauges is considered simultaneously, using vine copulas based on Kendall distribution functions. More specifically, we analyze which measures are suitable for explaining the spatial and temporal correlation of rain events in different locations within a network of stations; which families and structures of vine copulas can optimally capture the spatial dependence structure within a region; how to solve the complex mathematics that is imposed when expanding the dimensionality; what is a computationally reasonable alternative to improve the computational cost involved.; and how multivariate analysis can improve the precision of the extreme event risk measure compared to univariate approaches.

These questions are answered by applying the proposed methods to a pilot case, which is developed in a basin located in northern Spain. Multivariate modeling is becoming increasingly relevant in the field of hydrology due to its ability to model extreme stochastic events, which are key to mitigating the risk and damages caused by floods.

References

Gräler, B., Berg, M. J. van den, Vandenberghe, S., Petroselli, A., Grimaldi, S., De Baets, B. & Verhoest, N. E. C., 2013. Multivariate return periods in hydrology: a critical and practical review focusing on synthetic design hydrograph estimation. Hydrol. Earth Syst. Sci., 17(4), 1281–1296.

Salvadori, G., De Michele, C. & Durante, F., 2011. On the return period and design in a multivariate framework. Hydrol. Earth Syst. Sci., 15(11), 3293–3305.

How to cite: Urrea Méndez, D. A., Gómez Rave, D. V., and Del Jesus Peñil, M.: The Future of Extreme Event Risk Assessment: A Look at Multivariate Return Periods in More than Three Dimensions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11828, https://doi.org/10.5194/egusphere-egu23-11828, 2023.

EGU23-12249 | ECS | Posters on site | HS7.8

Space-time downscaling of extreme rainfall using stochastic simulations, intense runoff susceptibility modeling and remote sensing-based pluvial flood mapping 

Arnaud Cerbelaud, Etienne Leblois, Pascal Breil, Laure Roupioz, Raquel Rodriguez-Suquet, Gwendoline Blanchet, and Xavier Briottet

Accurate rainfall modeling is crucial to understand the way water is intercepted, infiltrates and flows through surfaces and rivers. In particular, it is paramount for the study of the influence of rainfall spatio-temporal distribution on basin hydrologic response and the structure of floods. Current weather radar products allow capturing the variability of rainfall extremes mainly at 1 km spatial resolution. In France, radar measurements are performed at a 5-minute time step, while gauge-based reanalysis are computed at hourly resolutions. During short-duration high-intensity precipitations, pluvial floods (PF, or flash floods) can occur outside the hydrographic network in runoff-prone areas, leading to various types of damages such as soil erosion, mud and debris flows, landslides, vegetation uprooting or sediment load deposits. Contrary to fluvial floods, PF are highly correlated to local rainfall. Depending on generic susceptibility linked to topography, soil texture and land use, specific precipitation patterns can trigger intense overland flow. Hence, after extreme weather events, precise reports on PF locations provide key information for rainfall reanalysis and downscaling at fine spatial resolution.

This work focuses on two extreme Mediterranean events (more than 300 mm of rainfall in 24 hours) that took place in the South of France between 2018 and 2020. Time series of hourly rainfall intensities from Comephore radar reanalysis data at 1 km resolution (Météo-France) are confronted to (i) maps of PF that occurred during the events and (ii) generic susceptibility maps to surface runoff. For (i), runoff-related impact maps of the events are produced using the remote sensing-based FuSVIPR algorithm (Cerbelaud et al., 2023) based on Sentinel-2 temporal change images and Pléiades satellite or airborne post event acquisitions. For (ii), the IRIP© method (Dehotin and Breil, 2011; Cerbelaud et al., 2022) is used to generate PF susceptibility maps. The model is run with the RGE Alti® 5 m DEM, the OSO French land cover dataset, and soil type susceptibility characteristics derived from both climatological information and the ESDAC database.

We primarily show that areas with higher IRIP levels are more likely to be impacted by PFs, and even more so where short-term precipitation was heavier. Additionally, rainfall intensities are negatively correlated with IRIP susceptibility scores in PF impacted areas. This corroborates that somewhat higher rainfall intensities are required for flash floods to occur in less susceptible areas. Similarly, comparatively smaller rainfall amounts can trigger PFs in locations where susceptibility is high. Then, the Comephore products are downscaled at 50 m resolution on both events using the SAMPO stochastic simulator (Leblois and Creutin, 2013). Among multiple scenarios, optimal ones are chosen based on the assumption that the negative correlation with the IRIP susceptibility levels in the affected areas should be equally or even more present in the downscaled rainfall time series. This study hence suggests an original way of selecting disaggregated extreme rainfall scenarios that are consistent with the observed consequences of intense runoff on the land surface using various tools such as a stochastic simulator, a hydrological risk mapping method and earth observation data.

How to cite: Cerbelaud, A., Leblois, E., Breil, P., Roupioz, L., Rodriguez-Suquet, R., Blanchet, G., and Briottet, X.: Space-time downscaling of extreme rainfall using stochastic simulations, intense runoff susceptibility modeling and remote sensing-based pluvial flood mapping, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12249, https://doi.org/10.5194/egusphere-egu23-12249, 2023.

EGU23-12736 | ECS | Posters on site | HS7.8

Multivariate Probability Analysis of Compound Flooding Dynamics. 

Dina Vanessa Gomez Rave, Diego Armando Urrea Méndez, and Manuel Del Jesus Peñil

Coastal cities are increasingly prone to compound flooding events. Particularly in estuaries, interactions between both freshwater fluxes (rainfall or discharge) and coastal water levels (tide, surge, waves, or combinations thereof) can strongly modulate flood hazard. These separate but physically connected processes can often occur simultaneously (but not necessarily in extreme conditions), resulting in compound events that may eventually have significant economic, environmental and social impacts. Conventional risk assessment mainly considers univariate-flooding drivers and does not include multivariate approaches; nevertheless, ignoring compound analysis may lead to a significant misestimation of flood risk.

In this respect, the complex interactions between coastal flooding drivers imply multidimensionality, nonlinearity and nonstationarity issues, and consequently, more relevant uncertainties. Copula-based frameworks are flexible alternatives to overcome limitations of traditional univariate approaches, and can incorporate the joint boundary conditions in riverine and coastal interactions in a statistically sound way (Harrison et al., 2021; Bevacqua et al., 2019; Couasnon et al., 2018, Moftakhari et al., 2017).  However, incorporations are often limited to the bivariate joint case. Trivariate (or higher dimensional) joint distribution are scarce, due to the convoluted and computationally expensive composition (Latif & Sinonovic, 2022). Notably, a need for robust and efficient approaches that help to characterize the nature of compound hazard remains (Moftakhari et al., 2021).

This study aims to improve copula-based methodologies that can adequately estimate the compound flood probability in estuarine regions, considering more than two variables, including more sources of uncertainty into the stochastic dependence analysis, raising the degree of accuracy to risk inference. This work develops a vine copula framework for the analysis of estuarine compound flooding risk, considering interactions and dependency structures between several oceanographic, hydrological, and meteorological processes and variables (rainfall, river discharge, waves, and storm tides). We show the potential of the framework in Santoña, a strategic estuarine ecosystem in Northern Spain. In order to yield proper design events, we focus here on estimating the multivariate joint and conditional joint return periods statistics, using the best-fitted model in the assessment of the extreme regime, based on Archimedean and Elliptical copula families. We also present the complexities of determining the ensemble of compound events corresponding to a given return period and compare these ensembles to the results of univariate extreme value analysis, to remark the importance of multivariate characterization of extremes.

References

Bevacqua, E., Maraun, D., Vousdoukas, M. I., Voukouvalas, E., Vrac, M., Mentaschi, L., & Widmann, M. (2019). Higher probability of compound flooding from precipitation and storm surge in Europe under anthropogenic climate change. Science advances, 5(9), eaaw5531.

Couasnon, A., Sebastian, A., & Morales-Nápoles, O. (2018). A copula-based Bayesian network for modeling compound flood hazard from riverine and coastal interactions at the catchment scale: An application to the Houston Ship Channel, Texas. Water, 10(9), 1190.

How to cite: Gomez Rave, D. V., Urrea Méndez, D. A., and Del Jesus Peñil, M.: Multivariate Probability Analysis of Compound Flooding Dynamics., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12736, https://doi.org/10.5194/egusphere-egu23-12736, 2023.

EGU23-13328 | ECS | Posters on site | HS7.8

Assessing daily precipitation tails over India under changing climate 

Neha Gupta and Sagar Chavan

Daily precipitation extremes are crucial in the hydrological design of major water control structures. The extremes are usually present in the upper part of the probability distribution of daily precipitation data, known as the tail. The distributions are bifurcated into heavy or light-tailed distributions depending on the tail. Heavy tails signify a higher frequency of occurrences of extreme precipitation events. Prediction of extreme precipitation depends on reliable modelling of the tail. Tail behaviour can be studied by graphical as well as threshold-based fitting approaches; however, each approach has associated shortcomings. In this work, we utilize a versatile and simple empirical index known as the “Obesity Index” (OB) to assess the tail of probability distributions of daily gridded precipitation data for India. This comprehensive regional analysis has been undertaken to quantify the tail heaviness of 4801 daily precipitation records over India for historical (1970–2019) and future (2020–2100) time periods. Future projections of daily precipitation are downscaled from the latest generation of climate models knowns as Coupled Model Intercomparison Project Phase 6 (CMIP6) under different emission scenarios. Finally, the application of the OB-based approach is extended to characterize daily precipitation in Indian Meteorological Subdivisions. Results indicate the applicability of heavy-tailed distributions in representing daily precipitation over India and establish the utility of the OB-based approach in diagnosing tail behaviour. Also, the spatial patterns of the tail heaviness are found to be matching with the Köppen–Geiger climate classification of India. The findings from this can be an input for the policymakers to develop adaptation strategies in response to the projected climate change impact.

Keywords: Extreme precipitation, Climate Change, India, Obesity index, Tail heaviness

 

How to cite: Gupta, N. and Chavan, S.: Assessing daily precipitation tails over India under changing climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13328, https://doi.org/10.5194/egusphere-egu23-13328, 2023.

EGU23-13386 | ECS | Posters on site | HS7.8

Use of high temporal resolution data to identify the key drivers and locations where walls of water occur in the UK 

Felipe Fileni, David Archer, Hayley Fowler, Fiona McLay, Elizabeth Lewis, and Longzhi Yang

Walls of water (WoW) are a subset of flash floods characterised by an extremely fast increase in the discharge rate of rivers. In the UK, WoWs, events where an almost instantaneous increase in river flow happens, are responsible for several deaths, even when the maximum peak flow of the said event is not as noticeable. Using a national 15-minute continuous dataset, this study identified WoWs for catchments in the UK. Next, the antecedent atmospheric conditions for these WoWs were extracted from gridded datasets. Furthermore, catchment descriptors such as catchment area, elevation, slope, land use, and permeability of every catchment were downloaded from the National River Flow Archive. Finally, with the use of machine learning algorithms, that is, tree regressions and neural networks, this study identified vulnerable catchments and key conditions for WoWs to occur. Early results indicate that WoWs are not solely driven by rainfall intensity and that larger catchments (>500km) with low permeability are the most vulnerable to these hazards. Further studies using additional atmospheric conditions, i.e., temperature and windspeed will allow a better understanding of the drivers of these events.

How to cite: Fileni, F., Archer, D., Fowler, H., McLay, F., Lewis, E., and Yang, L.: Use of high temporal resolution data to identify the key drivers and locations where walls of water occur in the UK, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13386, https://doi.org/10.5194/egusphere-egu23-13386, 2023.

EGU23-13732 | ECS | Posters on site | HS7.8

Simulation of extreme precipitation events over south-west France: the role of large-scale atmospheric circulation and atmospheric rivers 

Namendra Kumar Shahi, Olga Zolina, Sergey K. Gulev, Alexander Gavrikov, and Fatima Jomaa

South-western France has witnessed some of the most devastating extreme precipitation events that eventually lead to record-breaking severe flash flooding in the region and cause losses to human lives, urban transportation, agriculture, and infrastructure. In this study, two cases of deadly flash floods that occurred/reported in the Aude watershed in south-western France during 12-13 November 1999 and 14-15 October 2018 are studied using the WRF4.3.1 model simulations, with a particular emphasis on the model ability to capture these heavy precipitation events. We performed two simulations one with parameterized convection and one without the use of convection parameterizations for each case at gray-zone resolution (~9 km horizontal grid spacing) using the ERA5 reanalysis as the lateral boundary condition. In addition, attempts have been made to investigate the role of large-scale atmospheric circulation and atmospheric rivers in the production of these heavy precipitation events. The results from model simulations are compared quantitatively with available observations and reanalysis and found that the simulations at ~9 km gray-zone resolution capture the observed spatio-temporal distribution of precipitation characteristics during both extreme cases. The added value of gray-zone resolution simulations over driving coarse-scale ERA5 reanalysis datasets is observed in the representation of the precipitation characteristics. It has also been observed that the model simulation without the use of convection parameterization yields a reasonable and realistic representation of the precipitation characteristics during both extreme cases, and this suggests that at this “gray-zone” resolution the organized mesoscale convective systems/processes can be resolved explicitly by the model dynamics. The contribution of the large-scale atmospheric circulation and the atmospheric river (i.e., moisture transport) in the production of these flood events has also been observed.

How to cite: Shahi, N. K., Zolina, O., Gulev, S. K., Gavrikov, A., and Jomaa, F.: Simulation of extreme precipitation events over south-west France: the role of large-scale atmospheric circulation and atmospheric rivers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13732, https://doi.org/10.5194/egusphere-egu23-13732, 2023.

EGU23-14934 | ECS | Posters on site | HS7.8

Updating annual rainfall maxima statistics in a data-scarce region 

Angelo Avino, Luigi Cimorelli, Domenico Pianese, and Salvatore Manfreda

The growing number of extreme hydrological events observed has raised the level of attention toward the impact of climate change on rainfall process, which is difficult to quantify given its strong spatial and temporal heterogeneity. Therefore, the impact of the climate cannot be determined on the individual hydrological series but must be assessed on a regional and/or district scale. With this objective, the present work aims at identifying the trends and dynamics of extreme sub-daily rainfall in southern Italy in the period 1970-2020. The database of annual maxima was assembled using all available rainfall data (provided by the National Hydrographic and Mareographic Service - SIMN, and the Regional Civil Protection). However, due to the numerous changes (location, type of sensor, managing agencies) experienced by the national monitoring network, the time-series were found to be extremely uneven and fragmented. Since the spatio-temporal discontinuity could invalidate any statistical analysis, gap-filling techniques (deterministic and/or geostatistical [Teegavarapu, 2009]) were applied to reconstruct the missing data. In particular, the “Spatially-Constrained Ordinary Kriging” (SC-OK) method [Avino et al., 2021] was used, namely a mixed procedure that adopts the Ordinary Kriging (OK) approach with the spatial constraints of the Inverse Distance Weighting (IDW) method. The SC-OK method allows to reconstruct only missing data for stations selected by the IDW method (those with a sufficient number of functioning neighbouring rain gauges). Then, the reconstructed dataset has been used to explore trends and regional patterns in annual maxima highlighting, how rainfall are evolving in the most recent years.

REFERENCES

Avino, A., Manfreda, S., Cimorelli, L., and Pianese, D. (2021). Trend of annual maximum rainfall in Campania region (Southern Italy). Hydrological Processes, 35.

Teegavarapu, R.S.V. (2009). Estimation of Missing Precipitation Records Integrating Surface Interpolation Techniques and Spatio-temporal Association Rules. Journal of Hydroinformatics, 11(2).

How to cite: Avino, A., Cimorelli, L., Pianese, D., and Manfreda, S.: Updating annual rainfall maxima statistics in a data-scarce region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14934, https://doi.org/10.5194/egusphere-egu23-14934, 2023.

EGU23-15475 | Posters on site | HS7.8

A non-stationary gridded weather generator conditioned on large-scale weather circulation patterns for Central Europe 

Viet Dung Nguyen, Sergiy Vorogushyn, Katrin Nissen, and Bruno Merz

For many flood risk assessments at large spatial scales, long-term meteorological data (e.g. precipitation, temperature) with spatially coherent representation are needed. This is where a regional weather generator comes into play. Meteorological fields for a specific region are strongly dependent on weather circulation patterns (CP) at larger scales. Additionally, there is evidence that these fields covariate with the average regional surface temperature (ART). With future climate change, such changes in both CP and ART should be included in weather generators.

This study presents the development of such a non-stationary gridded weather generator conditioned on large-scale weather circulation patterns for Central Europe. The reanalysis dataset ERA5 (1o x 1o) is used for weather type classification. The E-OBS gridded observational dataset (0.25ox 0.25o) is used to parameterize the meteorological fields, such as precipitation and temperature (minimum, maximum, average). The spatial and temporal dependence is represented by the multivariate auto-regressive model. Daily precipitation amount is modelled by the extended generalized Pareto distribution and daily temperature is modelled by the transformed normal distribution. Both fields are conditioned on CP and allow to covariate with ART. In this way, the regional weather generator is capable of capturing “between-type” and “within-type” climate variability and can be used to generate long synthetic data for flood risk assessment in present and future periods.

How to cite: Nguyen, V. D., Vorogushyn, S., Nissen, K., and Merz, B.: A non-stationary gridded weather generator conditioned on large-scale weather circulation patterns for Central Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15475, https://doi.org/10.5194/egusphere-egu23-15475, 2023.

EGU23-16623 | ECS | Posters on site | HS7.8

Mapping Hazard to Extreme Temperature Events Over the Indian Subcontinent 

Anokha Shilin, Naveen Sudharsan, Arpita Mondal, Pradip Kalbar, and Subhankar Karmakar

The recent AR6 report of the Intergovernmental Panel on Climate Change (IPCC) explicitly shows that the observed change in hot extremes (including heatwaves) with high confidence in human contribution to the observed changes has highly increased in the South Asian (SAS) domain which comprises the Indian subcontinent. Extreme heat events are more frequent and intense across the globe since the 1950s and have adverse societal and economic impacts. Considering current warming trends and projections, heatwaves are becoming a serious problem in India. Exposure to extreme heat in the population is increasing due to climate change. Also, observed temperatures are increasing globally as well as regionally as an effect of global warming. As heat stress occurs when the human body cannot get rid of the excess heat, it can be considered a good proxy for the heatwave hazard. Heat stress results in heat stroke, exhaustion, cramps, or rashes. Exposure to extreme heat can result in occupational illnesses and injuries. An agrarian country like India will have large economic damage when climate-related heat stress increases the occurrence of droughts and exacerbate water scarcity for irrigation. Hence the impact of the heat stress hazard is spotted and largely discussed both in the academic and political domains. In this study, Universal Thermal Climate Index (UTCI) based hazard map is developed for India with a non-parametric multivariate approach. The prominent heat stress hazard areas are identified and mapped with reference to the UTCI assessment scale which is categorized based on thermal stress. The probability of occurrence is also mapped using the exceedance probability with the UTCI reference. Heat stress hazard map provides the basis for a wide range of applications in public and individual precautionary planning such as heatwave action plans, urban and regional planning, the tourism industry, and climate research. Hence a country-level extreme temperature hazard map is of dire necessity.

Keywords: Exceedance probability, hazard map, heat stress, multivariate approach, non-parametric method

How to cite: Shilin, A., Sudharsan, N., Mondal, A., Kalbar, P., and Karmakar, S.: Mapping Hazard to Extreme Temperature Events Over the Indian Subcontinent, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16623, https://doi.org/10.5194/egusphere-egu23-16623, 2023.

Humid heat extremes, taking account of both temperature and humidity, have adverse impacts on society, particularly on human health. It has been suggested that quasi-stationary waves (QSWs) with anomalously high amplitudes contribute to the occurrence of near-surface precipitation extremes and temperature extremes in the mid-latitudes of Northern Hemisphere. While little attention is paid to the linkages between amplified QSWs and humid heat extremes. Using the ERA5 dataset, we identify amplified QSWs of zonal wavenumbers 5-7 (Wave 5-7) in summer months from 1979 to 2020. These amplified QSWs show clear circumglobal wave patterns horizontally and nearly barotropic structure vertically. Linking amplified Wave 5-7 to wet-bulb temperature (WBT) extremes, we find that amplified QSWs preferentially induce prominently prolonged WBT extremes in specific regions: north-central North America for amplified Wave 5; western United States, south-central Asia, as well as eastern Asia for amplified Wave 6; western Europe and the Caspian Sea region for amplified Wave 7. Analyses of physical processes indicate that accompanied by the amplification of Wave 5-7, the changes in horizontal temperature advection, adiabatic heating, downward solar radiation, moisture transport and moisture flux convergence, and surface latent heat fluxes largely account for the increase in persistence of WBT extremes.

How to cite: Lin, Q. and Yuan, J.: Linkages between Amplified Quasi-stationary Waves and Humid Heat Extremes in Northern Hemisphere Midlatitudes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-78, https://doi.org/10.5194/egusphere-egu23-78, 2023.

EGU23-505 | ECS | Posters virtual | CL2.5

Investigating the Changing Heavy Rainfall Climatology of North East India 

Aniket Chakravorty, Shyam Sundar Kundu, and Shiv Prasad Aggarwal

The increase in the variability of rainfall as the climate of the world warms up is a concern for many regions. Studies in the past have associated this change in variability to rise in heavy rainfall events. Thus a regional analysis of heavy rainfall characteristics to evaluate its response to a changing climate becomes important. In this study, we are putting this focus on the North East Region (NER) of India, which boasts of being one of the wettest regions of the world. This study examines the heavy rainfall characteristics from 1901 till 2020 over NER using the IMD gridded daily rainfall product. The examination showed that although the annual and monsoonal rainfall over the NER has been decreasing, the intensity of heavy rainfall has increased by ~5mm over the decades. Singular Spectrum Analysis is used to identify the long-term trend, which showed a change in heavy rainfall characteristics around 1970 and hence further investigation is carried out over two time blocks (Pre-1970: 1901-1970 and Post-1970: 1971-2020). The investigation of the frequency of heavy rainfall events showed that its increasing trend, prior to 1970, transitions to a decreasing trend, post 1970. It also showed that the area under a negative trend of frequency has increased significantly after 1970. Furthermore, a non-parametric probability distribution approach has also been implemented to interpret the frequency and intensity relationship of heavy rainfall together. This showed that post 1970, the probability of occurrence of a very heavy or extreme rainfall events has increased. The increase in probability did show a spatial variability. The increase in probability is more for the pre-monsoon season compared to the monsoon. This finding corresponds to the fact that the contribution of pre-monsoon rainfall to annual rainfall has increased while that of the monsoon rainfall has decreased over the decades. To investigate the local causes of the observed changes, the 2m temperature (T2), 2m Dew-point temperature (TD2) are investigated using a cross-sample entropy analysis. Interestingly, both T2 and TD2 showed a significant increasing trend over NER. Coincidentally, locations with increasing heavy rainfall intensity and frequency are also the locations with increasing TD2. Also, the pre-monsoon show a stronger increase in TD2, i.e., more moisture is available for convection, compared to T2, which could explain the higher probability of heavy rainfall events. Thus, increasing intensity and decreasing frequency can be explained by the inter-relationship between T2, TD2 and the convective processes.

How to cite: Chakravorty, A., Kundu, S. S., and Aggarwal, S. P.: Investigating the Changing Heavy Rainfall Climatology of North East India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-505, https://doi.org/10.5194/egusphere-egu23-505, 2023.

Rainfall is an essential climatic parameter for any region, and it can have a significant socioeconomic impact on society. In this study, the trend analysis of rainfall data of the Ajay River Basin was performed for daily rainfall data from the APHRODITE dataset. It is a gridded dataset with a resolution of 0.25*0.25 degree latitude and longitude with 1951 to 2007 long time series for Asia. The non-parametric Mann-Kendall test was used to detect the monotonic trend in the rainfall time series and the Theil-Sen estimator to look at the magnitude of the change. The quantile perturbation method is used for extreme rainfall analysis. The study reveals that total annual rainfall and the monsoon period (June, July, August, September) have increased over the basin's southern part at a 5% significance level. In the pre-monsoon period (March, April, May) rainfall has increased all over the basin area at the 5% significance level. Extreme rainfall anomalies were found in most of the basin region, but some periods had very high perturbation. In the 1950-1960s, the northern area of the basin showed statistically significant negative anomalies, while the southern region showed significant positive anomalies. The 1970-1980s was the period of the highest significant positive anomalies, with up to 110% change. Significant negative anomalies dominated most of the southern basin from 1980 to 2000. The study concluded that although total rainfall has increased, extremes have decreased in the region.

How to cite: Mandraha, S. and Ray, S.: Trend analysis of total, seasonal and extreme rainfall data for Ajay River Basin, West Bengal., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-628, https://doi.org/10.5194/egusphere-egu23-628, 2023.

Three extreme cold events successively occurred across East Asia and North America in the 2020/21 winter. This study investigates the underlying mechanisms of these record-breaking persistent cold events from the isentropic mass circulation (IMC) perspective. Results show that the midlatitude cold surface temperature anomalies always co-occurred with the high-latitude warm anomalies, and this was closely related to the strengthening of the low-level equatorward cold air branch of the IMC, particularly along the climatological cold air routes over East Asia and North America. Specifically, the two cold surges over East Asia in early winter were results of intensification of cold air transport there, influenced by the Arctic sea ice loss in autumn. The weakened cold air transport over North America associated with warmer northeastern Pacific sea surface temperatures (SSTs) explained the concurrent anomalous warmth there. This enhanced a wavenumber-1 pattern and upward wave propagation, inducing a simultaneous and long-lasting stronger poleward warm air branch (WB) of the IMC in the stratosphere and hence a displacement-type Stratospheric Sudden Warming (SSW) event on 4 January. The WB-induced increase in the air mass transported into the polar stratosphere was followed by intensification of the equatorward cold branch, hence promoting the occurrence of two extreme cold events respectively over East Asia in the beginning of January and over North America in February. Results do not yield a robust direct linkage from La Niña to the SSW event, IMC changes, and cold events, though the extratropical warm SSTs are found to contribute to the February cold surge in North America.

How to cite: Yu, Y.: An Isentropic Mass Circulation View on the Extreme Cold Events in the 2020/21 Winter, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1192, https://doi.org/10.5194/egusphere-egu23-1192, 2023.

EGU23-1579 | ECS | Orals | CL2.5

Anthropogenic impact on the severity of compound extreme high temperature and drought/rainy events in China 

Wanling Li, Huijun Wang, Rufan Xue, Huixin Li, Mingkeng Duan, Xiaochun Luo, and Wenwen Ai

Extreme events seriously affect human health and natural environment. In the present study, several indexes that can describe the severity of compound extreme high temperature and drought/rainy events (CHTDE/CHTRE) are constructed based on copulas. According to observations, CHTDE and CHTRE have intensified in most areas of China during 1961–2014. The significant increase trend in the severity of CHTDE and CHTRE is basically consistent with simulations under historical anthropogenic forcing. This result proves that changes in CHTDE can be largely attributed to anthropogenic climate change. The historical greenhouse gas forcing is identified to be the dominant factor that affects the severity of CHTDE in China, particularly in the Tibetan Plateau and Northwest China. Moreover, the contribution of anthropogenic forcing to the linear change of the CHTRE severity in China is more than 90%. In addition, the ozone and land use signals also can be detected on change of CHTDE and CHTRE.

How to cite: Li, W., Wang, H., Xue, R., Li, H., Duan, M., Luo, X., and Ai, W.: Anthropogenic impact on the severity of compound extreme high temperature and drought/rainy events in China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1579, https://doi.org/10.5194/egusphere-egu23-1579, 2023.

EGU23-1580 | ECS | Orals | CL2.5 | Highlight

Future projections of meteorological, agricultural and hydrological droughts in China using the emergent constraint 

Rufan Xue, Wanling Li, Huixin Li, Xiaochun Luo, and Wenwen Ai

In the context of global warming, droughts occur more frequently and have caused great losses to human society. Therefore, understanding the potential changes in future droughts under climate change is of great scientific importance. In this paper, combining with climate models from CMIP6, the emergent constraint and the Model Goodness Index (MGI) are used to analyze the characteristics of meteorological, agricultural and hydrological droughts in China under four socioeconomic scenarios in the mid- and late 21st century. The results show that in the mid-21st century, there will be more frequent meteorological, agricultural and hydrological droughts in northern China. In the late 21st century, longer and more intense droughts are more likely to occur in China than in the mid-21st century. This indicates that drought events in China will gradually become more continuous and serious from the middle to the late 21st century. Additionally, northwestern and central China will be the main areas where the three types of drought areas and extreme droughts will increase in the future. In the mid-21st century, a higher socioeconomic scenario will suppress drought, which will enhance drought conversely in the late 21st century. These findings are of great significance for drought monitoring under climate change and can provide a basis for making a drought response plan.

How to cite: Xue, R., Li, W., Li, H., Luo, X., and Ai, W.: Future projections of meteorological, agricultural and hydrological droughts in China using the emergent constraint, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1580, https://doi.org/10.5194/egusphere-egu23-1580, 2023.

Southeastern South America (SESA), delimited between 38°S–25°S and 64°W–51°W, is characterized as one of the regions in the world with the highest frequency of occurrence of intense storms associated with deep convection, mainly during the spring and summer months (Zipser et al., 2006). These convective storm systems induce extreme precipitation events and produce most of the rain in the warm season (Rasmussen and Houze, 2016), generating significant damage (floods, intense winds, hail) and have a high impact on economic and social activities. Considering that the occurrence of extreme precipitation events in SESA is associated with the occurrence of certain synoptic patterns, the objective of this work was to detect the occurrence of extreme precipitation events from the synoptic patterns that induce these events, in spring (October to December, OND) and summer (January to March, JFM).

Daily data from the ERA5 reanalysis was used to detect recurring synoptic patterns associated with extreme precipitation events in the 1979-2013 calibration period. In order to identify a variety of precursor synoptic patterns of extreme precipitation events, the classification obtained from the principal component methodology (PCA) in orthogonally rotated T mode was used (Huth, 2000). To carry out the classification, the geopotential height was used at the 850 hPa level of the day prior to the occurrence of the extreme events (detected from the 95th percentile of the distribution of daily precipitation of the CPC Global Unified Gauge-Based Analysis of Daily Precipitation from the NOAA Climate Prediction Center). This classification resulted in two dominant synoptic situations for spring and summer. With the days obtained for each main component, compositions of the anomalies were made: the meridional component of the wind at the 850 hPa level, geopotential height at 850 and 500 hPa, and 200 hPa wind.

Based on the compositions made, an analog method was developed that was used to detect the occurrence of intense precipitation events in the verification period 2014-2021. In this methodology, two detection criteria were used, on the one hand, that the correlation coefficient between the fields of daily anomalies and the compositions are greater than a threshold and also that there is consistency between the sign of the daily meteorological variables with that of the compositions on certain grid points called hotspots regions.

For the evaluation of the analogue method, the F1 index developed by Gao et.al 2017 was used, which takes into account the number of true positives (TP), false positives (FP; type I error), and false negatives (FN; type II error).

How to cite: Martinez, D. and Solman, S.: Identification of extreme precipitation events in southeastern South America from their associated synoptic environment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1911, https://doi.org/10.5194/egusphere-egu23-1911, 2023.

EGU23-1945 | ECS | Orals | CL2.5

Explosive increase in convective Extreme El Niño events in the CO2 removal scenario 

Gayan Pathirana, Ji-Hoon Oh, Wenju Cai, Soon-Il An, Seung-Ki Min, Seo-Young Jo, Jongsoo Shin, and Jong-Seong Kug

Convective extreme El Niño (CEE) events, characterized by strong convective events in the eastern Pacific, are known to have a direct link to anomalous climate conditions worldwide, and it has been reported that CEE will occur more frequently under greenhouse warming. Here, using a set of CO2 ramp-up and –down ensemble experiments, we show that frequency and maximum intensity of CEE events increase further in the ramp-down period from the ramp-up period. Such changes in CEE are associated with the southward shift of the Intertropical Convergence Zone and intensified nonlinear rainfall response to SST change in the ramp-down period. The increasing frequency of CEE has substantial impacts on regional abnormal events and contributed considerably to regional mean climate changes to the CO2 forcings.

How to cite: Pathirana, G., Oh, J.-H., Cai, W., An, S.-I., Min, S.-K., Jo, S.-Y., Shin, J., and Kug, J.-S.: Explosive increase in convective Extreme El Niño events in the CO2 removal scenario, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1945, https://doi.org/10.5194/egusphere-egu23-1945, 2023.

Summer hot and dry extremes (defined as high air temperature and low atmospheric humidity) in monsoon (climatologically high-humidity) region, may cause severe disasters, such as flash droughts. However, it remains unclear whether hot (dry) extremes are amplified on dry (hot) days to warming temperature. Here, taking eastern monsoon China (EMC) as a typical monsoon region, we find a fastest positive (negative) response of air temperature (atmospheric humidity) on driest (hottest) days to per unit warming, indicating amplified warming (drying) of hot (dry) extremes on dry (hot) days (i.e. coupling hotter and drier extremes) especially in southern EMC.  The southern EMC is also a hotspot where the coupling of hot and dry extremes has become significantly stronger during the past six decades. The increasing hot-dry extremes in southern EMC is associated with anomalies in large-scale environmental conditions, such as reduced total cloud cover, abnormal anticyclone in upper atmosphere, intense descending motion, and strong moisture divergence over this region. Land-atmosphere feedbacks play another important role in enhancing the hot-dry coupling via increasing land surface dryness (described as decreasing evaporation fraction). The decreasing evaporation fraction is associated with drying surface soil moisture which is controlled by decreases in pre-summer 1-m soil moisture and summer-mean precipitation. Given hot extremes (atmospheric humidity) are (is) projected to increase (decrease) in the future, it is very likely to witness more hot-dry days in monsoon regions and associated disasters, which should be mitigated by adopting adaptive measures. 

How to cite: zhang, X. and Gu, X.: Coupling hotter and drier extremes under elevating air temperature over eastern monsoon China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1982, https://doi.org/10.5194/egusphere-egu23-1982, 2023.

The influence of moisture recycling and transport on major drought events is poorly understood, but essential to enhance our knowledge of the atmospheric water cycle. Here, we investigate this for two record-breaking droughts over the Mid-to-Lower Reaches of the Yangtze River (MLRYR), the winter-spring (WS) drought of 2011 and summer-autumn (SA) drought of 2019. Using a land–atmosphere water balance framework, we find the precipitation recycling ratio (the percentage of precipitation in a region derived from the same region’s evaporation) increased during both droughts, especially for the SA drought (from 14.5% to 22.9%). The WS drought was characterized by a 27.8% reduction in external advected moisture, originating principally from the northeast China and Bohai Sea (reduced by 22.3%) and from the northwest Pacific and South China Sea (25.7%). The SA drought was driven by a 43.8% reduction in external advected moisture, originating mainly from a southwesterly path, i.e. the Bay of Bengal and the South China Sea (reduced by 26.8%). From a regional viewpoint, moisture transportation from the Pacific Ocean (and South China Sea) decreased during the WS (SA) droughts, mainly resulting in moisture deficit over the MLRYR. Analyses reveal that this reduction was driven by strong negative convergence, which was unfavorable for precipitation formation and enhanced air flow out of the MLRYR. The weakened moisture transport was principally driven by seasonal mean flow rather than transient eddies. Changes in wind (i.e. dynamic processes), rather than specific humidity (i.e. thermodynamic processes) were dominant in regulating the seasonal mean moisture transport. Our study helps understand the atmospheric water cycle anomalies driving extreme drought events, and advances knowledge on moisture transportation and its controlling processes.

How to cite: Guan, Y. and Gu, X.: Tracing anomalies in moisture recycling and transport to two record-breaking droughts over the Mid-to-Lower Reaches of the Yangtze River, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2050, https://doi.org/10.5194/egusphere-egu23-2050, 2023.

Drylands play an essential role in Earth’s environment and human systems. Although dryland expansion has been widely investigated in previous studies, there is a lack of quantitative evidence supporting human-induced changes in dryland extent. Here, using multiple observational datasets and model simulations from phase 6 of the Coupled Model Intercomparison Project, we employ both correlation-based and optimal fingerprinting approaches to conduct quantitative detection and attribution of dryland expansion. Our results show that spatial changes in atmospheric aridity (i.e., the aridity index defined by the ratio of precipitation to potential evapotranspiration) between the recent period 1990–2014 and the past period 1950–74 are unlikely to have been caused by greenhouse gas (GHG) emissions. However, it is very likely (at least 95% confidence level) that dryland expansion at the global scale was driven principally by GHG emissions. Over the period 1950–2014, global drylands expanded by 3.67% according to observations, and the dryland expansion attributed to GHG emissions is estimated as ∼4.5%. Drylands are projected to continue expanding, and their populations to increase until global warming reaches ∼3.5℃ above preindustrial temperature under the middle- and high emission scenarios. If warming exceeds ∼3.5℃, a reduction in population density would drive a decrease in dryland population. Our results for the first time provide quantitative evidence for the dominant effects of GHG emissions on global dryland expansion, which is helpful for anthropogenic climate change adaptation in drylands.

How to cite: Shuyun, F. and Xihui, G.: Greenhouse gas emissions drive global dryland expansion but not spatial patterns of change in aridification, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2063, https://doi.org/10.5194/egusphere-egu23-2063, 2023.

Based on the precipitation and minimum temperature data observed at the stations from 1981 to 2020, two types of winter cold air activity events in the middle-lower reaches of the Yangtze River are identified, which are strong cooling events with precipitation and only strong cooling events without precipitation (referred to as “cold-wet” and “cold-dry” events), respectively. The atmospheric circulation differences and the characteristics of cold and warm air activities in the two type events, and their connection with the jet stream are also examined. The results show that the frequency of cold air activity events in the middle-lower reaches of the Yangtze River decreases year by year, among which the frequency of cold-dry events decreases and the frequency of cold-wet events increases significantly. In addition, the cooling amplitude of cold-wet events is greater than that with no precipitation. When cold-wet events occur, the upper-level subtropical jet moves northward and the polar front jet is weaker. There is a tilting ridge in the middle level and the subtropical high is located westward. In the lower-level, the Siberian high is strengthened and the warm and humid air flowing from the southwest converges and ascends in the middle-lower reaches of the Yangtze River. However, when cold-dry events occur, the subtropical jet in the upper level is weaker and the polar front jet is stronger. The trough and ridge in the middle level are weaker and the subtropical high is located eastward. In the lower level, the Siberian high is located southward and the dry air flowing from the north diverges and sinks in the middle-lower reaches of the Yangtze River. In addition, compared with cold-wet events, the jet stream intensity index and the meridional wind position index fluctuate more frequently during cold-dry events, and the cold air activity duration is shorter.

How to cite: Zhang, Y. and Zhu, X.: Circulation differences between two types of winter extreme cold air activity events in the middle-lower reaches of the Yangtze River and their relationship with the jet stream, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2192, https://doi.org/10.5194/egusphere-egu23-2192, 2023.

High temperatures and droughts pose a great threat to the human health, social economy and ecosystems. A large number of previous studies have focused on meteorological hot-dry events (based on temperature and precipitation), but there is a lack of comprehensive studies about hydrological hot-dry events (based on temperature and runoff). Here, using the ensemble empirical mode decomposition method and Copula function, we assess spatio-temporal evolution of global compound hot-dry events from temperature and runoff, and quantify their drivers based on monthly temperature and runoff data during 1902-2019. We find there is a significant warming at an unprecedented pace over the past 118 years, especially in the mid-latitudes of the Northern Hemisphere. However, changes in accumulated trends in precipitation and runoff show complex patterns globally. Probabilities of meteorological and hydrological hot-dry events both have been increasing significantly, but hydrological events are more likely to occur with higher spatial homogeneity, wider coverage and more severe damage. To analyze its underlying driving mechanism, we estimate quantitatively the contribution of high temperature, low runoff and the dependence between high temperature and low runoff to the compound event. High temperature plays a dominant role in the driving mechanism. In several regions, such as Australia, Europe and South America, hot-dry events could be considered as a potential hazard caused by increasing temperatures. Runoff deficit and dependence between the two, together with high temperature, exacerbate the occurrence of compound hot-dry events. Our findings provide a promising direction to predict joint probability of hot-dry events. Hydrological hot-dry events have seldom been considered, so far, in strategic policy formulation and risk assessment. Our results offer a powerful tool to improve planning and strategies to adapt to climate change.

How to cite: Min, R. and Gu, X.: Increasing likelihood of global compound hot-dry extremes from temperature and runoff during the past 120 years, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2299, https://doi.org/10.5194/egusphere-egu23-2299, 2023.

Abstract EGU General Meeting – April 2023

 

Abstract for session CL2.9: Atmospheric circulation in different spatial scales as one of the main climate variability factor

 

Precipitation extremes in the Ukraine: dynamical aspects, large-scale circulation and moisture sources

 

Ellina Agayar1,2, Franziska Aemisegger1, Moshe Armon1, Alexander Scherrmann1, and Heini Wernli1

 

1Institute for Atmospheric and Climate Science, ETH Zürich, Zürich, Switzerland

2Odessa State Environmental University, Odessa, Ukraine

 

 

 

Changes in the occurrence of large-scale circulation regimes link with changes in the global and regional climate and affect the frequency of occurrence and intensity of weather extremes, including extreme precipitation events (EPE). Understanding such natural hazards and their drivers is essential to mitigate related risks. In specific regions of the Ukraine, especially the Ukrainian Carpathians and the Crimean Mountains, precipitation can last for several days leading to floods. In this study, we investigate the dynamics of EPEs (≥ 100 mm day-1) over the territory of Ukraine in the recent decades (1979-2019). The EPEs are identified based on precipitation observations from 215 meteorological stations and posts in Ukraine. The atmospheric parameters for the categorization of the weather types (WTs) associated with the EPEs, as well as for composite studies and trajectory calculations were taken from ERA5 reanalyses. The identification of moisture sources contributing to extreme precipitation in Ukraine is based on the computation of kinematic backward trajectories and the subsequent application of a moisture source identification scheme based in the humidity mass budget along these trajectories.

By analysing the large-scale atmospheric circulation from reanalysis products, a four-class weather type (WT) classification of days with extreme precipitations in Ukraine is performed. The largest values of precipitation and greatest likelihood of EPEs occur in the WTs “Southerly cyclones and troughs” (45.1%) and “Easterly and South-Easterly cyclones and troughs” (23.2 %). The resulting WTs are assessed in terms of frequency of occurrence, seasonality, thermodynamic structure, and the spatial pattern of the large-scale flow, which allow identifying the main mechanisms for the formation of EPEs over Ukraine. Results show a clear spatial division in EPE occurrence, with summer and autumn being the seasons of highest EPE frequency in the western, south-western and eastern Ukraine. The last part of this study is dedicated to defining the origin, uptake characteristics, and transport pathways of moisture that precipitates during EPEs in Ukraine.

 

How to cite: Agayar, E.: Precipitation extremes in the Ukraine: dynamical aspects, large-scale circulation and moisture sources, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2647, https://doi.org/10.5194/egusphere-egu23-2647, 2023.

EGU23-2866 | ECS | Orals | CL2.5 | Highlight

Unravelling the origin of the atmospheric moisture deficit that leads to droughts 

Luis Gimeno-Sotelo, Rogert Sorí, Marta Vázquez, Raquel Nieto, Sergio M. Vicente-Serrano, and Luis Gimeno

Drought is the main natural hazard at the planetary scale and although this is a very complex phenomenon that involves many aspects of the hydrological cycle, there is always a deficit of precipitation compared to usual, understanding usual as climatological. This deficit can occur essentially for three reasons, either because there is less moisture available in the air column or because there is less atmospheric instability that forces air to rise, or for both reasons simultaneously. As the existing local humidity in the air column is mostly insufficient to justify precipitation, less humidity available for precipitation implies a deficit in the moisture which reaches the site in question. Therefore, on a global scale, moisture transport deficits lead to the occurrence of droughts.

In a first approximation, this humidity can have two origins, or comes directly from the ocean, or is subsequently recycled from the continents themselves. The processes that control the evaporation over oceans or the continents as well as the moisture transport are very different, and there is a variable relationship between the oceanic and terrestrial origin of precipitation both globally and regionally. In a second approximation, the main sources of humidity at a global level are those regions where evaporation greatly exceeds precipitation over them, which mainly occurs in the subtropical oceans, some inland seas, and the two continental areas known as green oceans, the Amazon and the Congo basins.

It is known where the humidity coming from the whole ocean or the whole continent precipitates, as well as the sinks of the humidity that comes from these large individual sources. It has also been studied how anomalous moisture transport affects droughts in specific regions, but the probability of occurrence of droughts at a planetary scale on continental areas given a deficit of the moisture transported from the global oceanic area, the global continental area, and each of these major sources has not been fully evaluated. Here we make use of a Lagrangian approach widely used and checked, which consists of estimating how much precipitation comes from the humidity arriving from a specific moisture source and enables to reveal the origin of the atmospheric moisture deficit underlying the occurrence of droughts. 

How to cite: Gimeno-Sotelo, L., Sorí, R., Vázquez, M., Nieto, R., Vicente-Serrano, S. M., and Gimeno, L.: Unravelling the origin of the atmospheric moisture deficit that leads to droughts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2866, https://doi.org/10.5194/egusphere-egu23-2866, 2023.

This study finds a significant negative correlation between the December–February mean surface temperature (Ts_DJF) and the following June–August mean surface temperature (Ts_JJA) in South Korea for the period 1991–2017. This indicates that colder winters tend to precede hotter summers with extreme seasonality, while mild winters generally precede mild summers. This winter-to-summer association can be attributed to persistent atmospheric circulation anomalies on the Eurasian continent during the preceding winter and spring characterized by cyclonic circulations in Europe and East Asia and anti-cyclonic circulation in the Arctic regions. Resembling a negative Arctic Oscillation (AO) pattern combined with a negative Polar/Eurasia (PE) pattern, these atmospheric patterns tend to cause colder winters in South Korea and to increase the springtime sea surface temperatures in the western tropical Pacific (WTP) and in the North Atlantic (tripole pattern, NATRI). High WTP and NATRI values induce summertime anti-cyclonic circulations and then hotter summers in Korea with different pathways, the former via northward Rossby wave propagation in response to strong convection over a warm Philippine Sea and the latter via both extratropical Rossby wave propagation from the North Atlantic to East Asia and tropical connections from the tropical Atlantic to the Indian Ocean and then increased summer precipitation in South Asia. Under the opposite conditions (e.g., positive AO and PE phases in winter and negative WTP and NATRI), mild summers are preceded by mild winters. Since the early 1990s, the aforementioned atmospheric circulation anomalies during winter have shown greater persistence, creating the negative correlation between Ts_DJF and Ts_JJA. These findings provide useful information for the long-lead prediction of summer temperatures and heat waves in South Korea.

How to cite: Myoung, B.: Recent Trend of Cold Winters Followed by Hot Summers in South Korea due to the Combined Effects of the Warm Western Tropical Pacific and North Atlantic in Spring, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2985, https://doi.org/10.5194/egusphere-egu23-2985, 2023.

Climate change can be reflected in terms of  shift in mean climatology as well as shift in the distribution of rainfall and temperature extremes over time. Southern Africa has distinct climate regimes that includes arid and semi-arid climates as well as relatively humid climate. This results in distinct spatio-temporal response of the region to climate change. In this study, major extreme climate indices for the region are derived from daily CHIRPS rainfall, ERA-Interim minimum, maximum and average temperatures to understand the spatio-temporal variability. The long term mean of the coldest annual day-time maximum temperature (90thpercentile) is observed over Lesotho highlands and adjoining areas in South Africa (21.0oC) whereas the warmest day-time temperature (37.4oC) is observed over areas bordering South Africa, southern Botswana and Namibia during the recent four decades. The trend in this indices shows warming (up to 1oC/decade) over southwestern South Africa, along coastal strips of South Africa, much of Mozambique, northwestern Zimbabwe, northern and western Zambia, eastern Angola and cooling over central Botswana. The annual night-time minimum temperature (10th percentile) is increasing northward in contrast to day-time maximum temperature which, in addition, exhibits zonal gradient. In terms of frequency, 10 to 12% of  the days in a year experienced maximum temperature above 90th percentile whereas 9 to 11 % of the days in a year observe night-time minimum temperature below 10th percentile. The annual heat wave duration indices show longest duration (8 days) over Southern Angola, northern Namibia, southern  Zambia, northern Zimbabwe and Botswana and decrease from here northward and southward. Annual number of days with rainfall  above 10 mm is about 10 days over western South Africa, Botswana, southern Zimbabwe, Namibia and southern Angola. In contrast,  it is in the range of 32 to 74 days over northern Angola, Zambia and Mozambique with increasing trend over Botswana, eastern parts of Zambia and Angola.  Similar trend in maximum 5 to 10 day total rainfall is observed over the same areas. Central part of the Southern Africa region exhibits the highest annual continuous dry days (147 to 254 days) whereas the southern and northern parts of the region has the lowest annual continuous dry days ( about 76 days). The long term mean of maximum annual continuous wet days increases northward from 3 days over western parts of South Africa and Namibia to 21 days over  Angola and northern Malawi. Besides secular trend, the rainfall extreme indices have coherent cyclic modes of variability with a period of 3.6 to 3.8 years accounting for 9 to 12 % of the total variance whereas the temperature extreme indices show periodicity of about 2.5 years accounting for 18 to 19% of the total variance. The periodicities are possibly associated with ENSO events that modulate interannual variability.

How to cite: Mengistu Tsidu, G.: Spatio-temporal variability of rainfall and temperature extremes over Southern Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3037, https://doi.org/10.5194/egusphere-egu23-3037, 2023.

Observations have shown sub-seasonal reversal of temperature anomalies between early and late winter over Eurasia, which is distinct from the seasonal mean condition. Based on the reanalysis data, the 1800-year control simulation and the 40-member ensemble simulations in 1920–2100 from the Community Earth System Model (CESM) Large Ensemble (CESM-LE), this study reveals that the reversal of surface air temperature (SAT) anomalies between early and late winter is one of the dominant and intrinsic features of the Arctic-Eurasian winter climate. Such a reversal is characterized by “colder Arctic, warmer Eurasia” in December (January–February) and ‘warmer Arctic, colder Eurasia’ in January–February (December). Robust climate dynamic processes associated with the reversal of SAT anomalies, including sub-seasonal reversals of anomalies in the Ural blocking, mid-latitude westerlies and stratospheric polar vortex, are found in both reanalysis data and CESM simulations, indicating the important role of internal atmospheric variability. Further analysis reveals that the reversal of Ural blocking anomalies in late December can be a potential precursor for the reversal of SAT anomalies in late winter. The reversal of mid-latitude westerly wind anomalies associated with the Ural blocking can affect upward propagation of planetary-scale waves especially with wavenumber 1, subsequently promoting the contribution of stratospheric polar vortex to the reversal of SAT anomalies in late winter over the Arctic-Eurasian regions. Such a troposphere-stratosphere pathway triggered by the perturbation of tropospheric circulations is confirmed by the CESM-LE simulations, and it may be useful for the prediction of sub-seasonal reversal of SAT anomalies.

How to cite: Xu, X.: Atmospheric contributions to the reversal of surface temperature anomalies between early and late winter over Eurasia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4395, https://doi.org/10.5194/egusphere-egu23-4395, 2023.

EGU23-4726 | Posters on site | CL2.5

Record-breaking High Temperature in July 2021 over East Sea and Possible Mechanism 

MinHo Kwon, Kang-Jin Lee, and Hyun-Woo Kang

As climate change due to global warming continues to be accelerated, various extreme events become more intense, more likely to occur and longer-lasting on a much larger scale. Recent studies show that global warming acts as the primary driver of extreme events and that heat-related extreme events should be attributed to anthropogenic global warming. Among them, both terrestrial and marine heat waves are great concerns for human beings as well as ecosystems. Taking place around the world, one of those events appeared over East Sea in July 2021 with record-breaking high temperature. Meanwhile, climate condition around East Sea was favorable for anomalous warming with less total cloud cover, more incoming solar radiation, and shorter period of Changma rainfall. According to the results of wave activity flux analysis, highly activated meridional mode of teleconnection that links western North Pacific to East Asia caused localized warming over East Sea to become stronger.

 

How to cite: Kwon, M., Lee, K.-J., and Kang, H.-W.: Record-breaking High Temperature in July 2021 over East Sea and Possible Mechanism, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4726, https://doi.org/10.5194/egusphere-egu23-4726, 2023.

EGU23-5494 | ECS | Posters on site | CL2.5 | Highlight

Understanding the Potential Changes in Causal-Physical Drivers of Extreme Mei-yu Precipitation and Potential Applications 

Kelvin S. Ng, Gregor C. Leckebusch, and Kevin I. Hodges

Accurate predictions of extreme Mei-yu precipitation (MYR) over China for near-term and long-term climate is crucial.  This is because such information is essential for decision and policy makers to develop optimal strategies to mitigate any negative socioeconomic impact which could be caused by changes in MYR. While the performance of climate models has improved substantially over the past few decades, accurate prediction of MYR remains an open challenge. On the other hand, climate models often have a better representation of the large-scale climate modes (LSCMs) and many studies have suggested some LSCMs and MYR are related. A recent study has demonstrated the representation of MYR in climate models can be improved by using causality-guided statistical models (CGSMs) based on LSCMs causally related to MYR as predictors. However, the potential changes in these causal-physical drivers on (multi-)decadal timescale has not previously been considered. In this presentation, we present the preliminary results on the potential changes in causal-physical drivers, which govern MYR, on (multi-)decadal timescales. A potential application of such information for decadal prediction systems is also discussed.

How to cite: Ng, K. S., Leckebusch, G. C., and Hodges, K. I.: Understanding the Potential Changes in Causal-Physical Drivers of Extreme Mei-yu Precipitation and Potential Applications, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5494, https://doi.org/10.5194/egusphere-egu23-5494, 2023.

EGU23-5554 | Posters on site | CL2.5 | Highlight

Changes in snow accumulation and snow depth in Slovakia in the 1921 – 2021 period 

Pavel Fasko, Ladislav Markovič, and Oliver Bochníček

Warming surface temperatures have driven a substantial reduction in the extent and duration of Northern Hemisphere snow cover. Analysis of the long-term snow cover data can provide an exact picture on the climate change induces changes. Slovak Hydrometeorological Institute maintains a network of 113 precipitation measuring stations with daily observations of the snow cover depth since 1921. This paper presents analysis of the cumulative snow cover depth in the territory of Slovakia in the period 1921 - 2021. Such an approach to processing can effectively point to changes in the seasonal development of the snow cover. The results show that, in general, we observe a decrease in the snow cover, which began to become more pronounced especially in the course of the 21st century. The magnitude and speed of the detected change is significantly influenced not only by the altitude of the precipitation gauge, but also by its geographical location.

How to cite: Fasko, P., Markovič, L., and Bochníček, O.: Changes in snow accumulation and snow depth in Slovakia in the 1921 – 2021 period, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5554, https://doi.org/10.5194/egusphere-egu23-5554, 2023.

EGU23-5767 | Posters on site | CL2.5

Dynamic and thermodynamic effects driving anomalous precipitation over Amazon 

Fernanda Cerqueira Vasconcellos and Laurent Li

Anomalous rainfall produces droughts and floods over the Amazon region, enhancing risks of forest fires, heatwaves and inundations, which affects the regional fauna, flora, and socioeconomic activities. In this study, the driest and wettest years of the Northern and Southern Amazon are investigated by analyzing the regional moisture and moist static energy budget. For the Northern and Southern Amazon, the dynamic effect, related to vertical movement changes, was the primary cause for the precipitation anomalies. The thermodynamic effect connected with moisture changes also contributed to the Northern Amazon precipitation anomalies. The anomalous vertical motion in the Northern Amazon was mainly caused by the horizontal advection of anomalous moist enthalpy through climatological wind, which alters the moist static energy in the region. Thus, a vertical movement is produced to compensate the energy changes, leading to changes in precipitation. Nonlinear terms and the horizontal advection of climatological moist enthalpy by the anomalous wind constrained the vertical motion in the driest years over Southern Amazon. For the wettest years over Southern Amazon, the anomalous ascending movement had contributions from all moist static equation terms, except the vertical advection of anomalous moist static energy by climatological wind, which had an opposite effect. The latent heat was the main contributor to anomalous moist enthalpy influencing the vertical movement. Further investigations indicated that the tropical Atlantic and Pacific SST anomalies could influence the vertical anomalies. In conclusion, although the dynamic effect (changes in the vertical motion) was the main driver for precipitation anomalies, the thermodynamic contribution related to latent heat anomalies is significant, mainly for Northern Amazon.

How to cite: Vasconcellos, F. C. and Li, L.: Dynamic and thermodynamic effects driving anomalous precipitation over Amazon, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5767, https://doi.org/10.5194/egusphere-egu23-5767, 2023.

Southeast Asia lies at the heart of heavy precipitation on Earth, and a large amount of latent heat released
here provides substantial energy for the global atmospheric circulation. Utilizing gauge-based daily precipitation and the
self-organizing map technique, the summertime extreme and total precipitation over Southeast Asia during 1979–2019 are
classified into three and five distinct patterns, respectively. The three extreme precipitation clusters are characterized by
southern dry and northern wet (C1_extreme), overall wet (C2_extreme), and northern dry and southern wet (C3_extreme)
structures. The frequencies of these patterns exhibit increasing trends during the analysis, although they are not statistically
significant for C1_extreme. The C1_extreme pattern is accompanied by an anomalous cyclone over the South China Sea in
response to negative Indian Ocean sea surface temperature anomalies (SSTAs). The C2_extreme and C3_extreme clusters
are characterized by a westward extension of the western Pacific subtropical high, regulated by cool SSTAs over the tropical
central-eastern Pacific that are induced by the tropical North Atlantic warming and the tropical Pacific and Atlantic
SSTAs, respectively. For total precipitation, the first and second clusters show overall dry distributions, which are mainly
composed of nonextreme precipitation. The spatial patterns and atmospheric and oceanic features associated with the
other three clusters of total precipitation bear large resemblances to those of C1_extreme, C2_extreme, and C3_extreme,
respectively, but their trends exhibit smaller similarities. Comparing the differences between extreme and total precipitation
over Southeast Asia could improve our understanding of their regional variabilities and relationships, and potentially
their global impacts.

How to cite: Xu, L.: Variations of Summer Extreme and Total Precipitation over Southeast Asia andAssociated Atmospheric and Oceanic Features, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5908, https://doi.org/10.5194/egusphere-egu23-5908, 2023.

EGU23-6124 | ECS | Posters on site | CL2.5 | Highlight

Trends in drought across Europe and their links to atmospheric circulation 

Zuzana Bešťáková, Jan Kyselý, Ondřej Lhotka, and Josef Eitzinger

We study trends in drought across the central latitude strip of Europe (defined as the region 47.5–52.5 °N and 2.5°W–32.5°E) during 1950–2019, and their links to atmospheric circulation. Drought characteristics are based on difference between potential evapotranspiration and precipitation in E–OBS data, and atmospheric circulation is characterized in terms of circulation types classified using daily sea level pressure patterns from the NCEP–NCAR reanalysis. Circulation types supporting drought in vegetation season (April–September) are identified, and we analyse changes in their occurrence since 1950, seasonal changes, and the connection with drought trends in individual European regions. We find that while in the early vegetation season, drought develops mainly in Central Europe, in the late vegetation season the most pronounced trends are shifted towards west. The circulation types supporting drought depend on regions and seasons, especially for directional types. The largest increase of the dry circulation types is observed in both seasons in Central Europe, and contributes to the pronounced drying.

How to cite: Bešťáková, Z., Kyselý, J., Lhotka, O., and Eitzinger, J.: Trends in drought across Europe and their links to atmospheric circulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6124, https://doi.org/10.5194/egusphere-egu23-6124, 2023.

EGU23-6127 | ECS | Orals | CL2.5

Comparison Analysis of the Climate Extreme in 2022 

Chaonan Ji, David Montero, Veronika Grupp, Karin Mora, and Miguel D. Mahecha

Extreme events are on the rise. The 2022 compound heatwave and drought event caused significant vegetation mortality and serious ecosystem destruction in Europe that urgently need to be investigated. In this study, we used climate data (ERA5-Land air temperature at 2 m and precipitation) and remote sensing products (kNDVI derived from MODIS and ESA CCI Land Cover product) to investigate the dynamics of the 2022 extreme events and vegetation responses. Furthermore, we compared the effects of this year to other normal as well as abnormal years in Europe. We propose a ranking-based approach that compares cumulative sums of climate variables and kNDVI over the growing season to determine extreme areas and compound intensity over the last 23 years.

The results show that the 2022 event is a widespread compound heatwave and drought event, with a similar spatial pattern to the 2018 extreme event, but less severe. Vegetational response differed among land cover classes, grassland was more affected while deciduous trees were barely affected in the 2022 event. In general, vegetation recovered relatively quickly after the 2022 event.

Our ranking-based approach enables an effective comparison and characterization of climate extremes and their effects on vegetation over different years. A more in-depth analysis of spatial and temporal patterns can contribute to the development of targeted measures and support decision-makers in responding to climate extremes.

How to cite: Ji, C., Montero, D., Grupp, V., Mora, K., and D. Mahecha, M.: Comparison Analysis of the Climate Extreme in 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6127, https://doi.org/10.5194/egusphere-egu23-6127, 2023.

Analyses of the standardized precipitation evaporation index (SPEI), using the season-reliant empirical orthogonal function (S-EOF) method, indicate that the second leading mode of drought over Northeast China features an in-phase variation from spring to summer. Such an in-phase change is closely connected to the persistence of geopotential height anomalies around Lake Baikal. The positive height anomalies around Lake Baikal, with an equivalent barotropic structure in the troposphere, can decrease water vapor transport into Northeast China and induce anomalous descending over Northeast China during both seasons, favoring precipitation deficit and high temperature in situ and hence resulting in the synchronous variations of spring and summer droughts. Further investigation reveals that the spring North Atlantic Oscillation (NAO) plays a notable role in the in-phase change of spring-summer droughts over Northeast China. The positive phase of spring NAO could induce spring drought over Northeast China directly through its influence on the above atmospheric circulations via a zonal wave train emanating from the North Atlantic. Meanwhile, it can also increase the soil moisture in Central Siberia by enhancing the local snow depth. The wetter soil moisture in the following summer, in turn, increases the meridional temperature gradient between the middle and high latitudes and then forces westerly anomalies around 60°N, consequently yielding positive height anomalies around Lake Baikal which favor the occurrence of summer drought over Northeast China. Therefore, the spring NAO is hypothesized to contribute to the in-phase variations of spring-summer droughts over Northeast China through the combined roles of zonal wave train and Central Siberian soil moisture.

How to cite: Hu, Y.: In-phase Variations of Spring and Summer Droughts over Northeast China and Their Relationship with the North Atlantic Oscillation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6270, https://doi.org/10.5194/egusphere-egu23-6270, 2023.

The South Asian High (SAH) experienced a decadal weakening in the late 1970s under global warming. Based on an evaluation of the historical runs from CMIP6 models, we quantitatively assessed the contributions of different external forcing using “good” models that reasonably simulated the decadal decline of the SAH. All-forcing runs yielded the weakened SAH after the late 1970s, albeit the decadal decline was underestimated by most models. Compared to the insignificant contributions of greenhouse gas and natural forcing, anthropogenic aerosol played a dominant role in the decadal decline of the SAH. The increased aerosol likely drove a cooling surface over the Tibetan Plateau and East China via its effect on radiation. Consequently, the weakened heat source over the Tibetan Plateau and associated thermodynamic effects over East China would have driven a cooling of eddy temperature and cyclonic anomalies in the upper troposphere, respectively, thereby causing the decline of the SAH.

How to cite: Zhang, D.: Contributions of External Forcing to the Decadal Decline of the South Asian High, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6331, https://doi.org/10.5194/egusphere-egu23-6331, 2023.

EGU23-6335 | ECS | Orals | CL2.5 | Highlight

The Arctic-Siberian Plain warming drives the heat waves in East Asia. 

Jeong-Hun Kim, Seong-Joong Kim, Joo-Hong Kim, Michiya Hayashi, and Maeng-Ki Kim

Generally, it is well known that the East Asian heatwaves are strongly affected by the Pacific-Japan pattern and circum-global teleconnection pattern. However, recent studies suggest that various teleconnection patterns also can contribute to the East Asian heat waves (e.g., Scandinavian pattern, Arctic Oscillation, El Nino-Southern Oscillation, etc.). However, the teleconnection between the Arctic-Siberian Plain (ASP) warming and East Asian heat waves has been unexplored. This study investigates the teleconnection mechanism between East Asian heatwaves and the warming over the ASP for the last 42 years (1979-2020). The results show that the enhanced surface radiative heating by the anticyclonic anomalies over the ASP region increases the air temperature and surface evaporation, amplifying the thermal high pressure via positive water vapor feedback. The Rossby wave, amplified by land-atmosphere interaction in the ASP, propagates to East Asia through the upper troposphere, causing favorable atmospheric patterns for the occurrence of the East Asian heatwaves.

How to cite: Kim, J.-H., Kim, S.-J., Kim, J.-H., Hayashi, M., and Kim, M.-K.: The Arctic-Siberian Plain warming drives the heat waves in East Asia., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6335, https://doi.org/10.5194/egusphere-egu23-6335, 2023.

Southwest China (SWC) is vulnerable to disasters caused by extreme precipitation. This study investigates the mechanisms of low-latitude intraseasonal oscillations affecting regional persistent extreme precipitation events (RPEPEs) over SWC during rainy seasons. Most of the RPEPEs over SWC are dominated by 7–20-day variability. The RPEPEs over SWC are preconditioned by two different types of 7–20-day Rossby waves with almost opposite phases over the western North Pacific (WNP). The two types of 7–20-day Rossby waves have direct (indirect) effects on Type 1 (2) RPEPEs, respectively. For Type 1, a coupled 7–20-day low-level anticyclone and suppressed convection originating from the tropical WNP propagate northwestward and cover the region from the South China Sea (SCS) to the Bay of Bengal before the RPEPEs. The anticyclone triggers ascending motion over SWC and transports more moisture to SWC, favoring the SWC RPEPEs. Before the Type 2 RPEPEs, a coupled 7–20-day low-level cyclone and enhanced convection propagates from the tropical WNP to the SCS. The enhanced convection over the SCS leads to the westward extension of the western Pacific subtropical high (WPSH) and the eastward shift of the South Asian high (SAH). The variations in the WPSH and the SAH directly cause SWC RPEPEs by inducing ascending motion and transporting moisture. The mechanisms for Type 2 RPEPEs tend to work under the background with a strong WPSH. Using a Lagrangian model, we found that both the 7–20-day oscillations and their background atmospheric circulations result in significant differences in moisture sources for the two types of RPEPEs. These findings benefit a better understanding of SWC extreme precipitation events.

How to cite: Nie, Y.: Regional Persistent Extreme Precipitation Events over Southwest China under Different Low-Latitude Intraseasonal Oscillations during Rainy Season, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6377, https://doi.org/10.5194/egusphere-egu23-6377, 2023.

EGU23-7451 | ECS | Orals | CL2.5

Evaluation of the main heatwave patterns in the northeast of the Iberian Peninsula using ERA5 and CORDEX models 

Sergi Ventura, Gara Villalba, Josep Ramon Miro, and Juan Carlos Peña

Heatwaves are expected to increase not only in intensity but also in frequency and duration in the next decades. Most of the studies are focused on the temperature variable, but little is known about their synoptic structure, which is especially important in mid-latitude regions.

In this study, we propose a Principal Sequence Pattern Analysis (PSPA) to classify the main synoptic patterns that define heatwaves in the northeast of the Iberian Peninsula. This is done by finding the most correlated input variables that represent the highest number of variance possible. The database used for this analysis comes from ERA5 reanalysis data covering the 1951-2020 period, in which we have selected three variables: mean sea level pressure (MSLP), geopotential height at 500 hPa (Z500) and maximum daily temperature at 2 meters (TMAX). Once the historical analysis is prepared, the same steps are repeated for CORDEX models (1951-2000) to discuss the performance of these models simulating heatwave periods.

The multivariate analysis has resulted in four synoptic patterns that explain more than 50% of the total variance. The four patterns are divided into two groups, stationary and dynamical. The HWs with highest temperatures in the Metropolitan Area of Barcelona are the prefrontal patters, which are dynamical and undulated at Z500 and undetermined at MSLP, with mean maximum temperatures around 35°C. However, the warmest pattern in inland areas is stationary and stable, generated at Z500 by intense anticyclonic ridges covering the Iberian Peninsula and at MSLP by deep thermal lows. The CORDEX models simulate similar patterns but less defined due to the lack of resolution. Z500 results in an overestimation of the anticyclonic ridges and MSLP shows an underestimation of pressure gradients, simulating more undetermined patterns. However, there are discrepancies between the models, which will result in different future projections in the climate change scenarios.

How to cite: Ventura, S., Villalba, G., Miro, J. R., and Peña, J. C.: Evaluation of the main heatwave patterns in the northeast of the Iberian Peninsula using ERA5 and CORDEX models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7451, https://doi.org/10.5194/egusphere-egu23-7451, 2023.

Concurrent heatwaves and droughts that occur over northeastern China (NEC) bring severe threats to human lives and crop productions. In the present study, a probability-based index that simultaneously considers precipitation deficiency and high temperature is calculated to represent concurrent heatwaves and droughts over NEC. Based on this index, the characteristics of concurrent heatwaves and droughts over NEC in summer are investigated using the year-to-year increment approach. The results indicate that the occurrence of concurrent heatwave and drought over NEC is closely related to the Polar-Eurasian teleconnection pattern and the Pacific-Japan teleconnection pattern. Further analyses indicate that the sea ice content in the Barents Sea in March (SICBS), the La Niña-like sea surface temperature (SST) in February (SST-PC1), and the northwestern Siberia soil moisture in April (SM) are coincidently linked to the two teleconnection patterns mentioned above. Based on their corresponding physical mechanisms, these three independent predictors are chosen to construct a physical-empirical prediction model for the prediction of concurrent heatwaves and droughts over NEC. Results suggest that this physical-empirical prediction model performs well with a high correlation coefficient and a low root mean squared error between the observed and predicted concurrent heatwaves and droughts over NEC for the period 1979–2018. Moreover, the cross-validation test and independent hindcasts both suggest that the physical-empirical model proposed in the present study with the three independent predictors has good prediction skills.

How to cite: Li, H.: Mechanisms and prediction of concurrent heatwaves and droughts in July–August over northeastern China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7631, https://doi.org/10.5194/egusphere-egu23-7631, 2023.

EGU23-7643 | ECS | Orals | CL2.5 | Highlight

The Role of Moisture and Heat Transport for Extreme Droughts in the Amazon Basin - a Lagrangian Perspective 

Katharina Baier and Andreas Stohl

In the last decade, tropical rainforests, e.g. the Amazon basin, have experienced events of extreme droughts. Such events have huge impacts on the forest, as trees are damaged. Therefore, it is relevant to gain deeper understanding on the main mechanisms causing such events, and further clarify the role of moisture recycling over the continent vs. moisture transport from oceanic regions.

We study the role of moisture- and heat transport for the Amazon basin, with special focus on drought events. We show how these extreme events differ from normal conditions, with special focus on the changes in atmospheric transport. We analyse the atmospheric transport with the particle dispersion model FLEXPART using meteorological input data from the ERA5 reanalysis. In this Lagrangian model, the atmosphere was filled homogeneously with particles, which were traced forward in time and represent the global atmospheric mass transport. From this Lagrangian reanalysis dataset, covering the years 1979-2021, air masses over the Amazon basin are selected and traced backward in time.

Based on that, we investigate the role of continental and oceanic moisture source areas, incorporating also information on soil moisture and burned areas. Thereby, we highlight the relevance of moisture recycling over continental - vs.  moisture transport from oceanic areas. For example, we found that for the northern parts of the Amazon basin the most important moisture source is the Atlantic Ocean, thus this area is less affected by deforestation in the southern areas.

How to cite: Baier, K. and Stohl, A.: The Role of Moisture and Heat Transport for Extreme Droughts in the Amazon Basin - a Lagrangian Perspective, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7643, https://doi.org/10.5194/egusphere-egu23-7643, 2023.

EGU23-8274 | ECS | Orals | CL2.5 | Highlight

Sources, propagation and sinks of Europe’s major heat waves; a complex network analysis of heat extremes 

Irene Garcia-Marti, Gerard van der Schrier, and Florian Polak

In the last few decades, Europe has seen many devastating heat waves; each one producing new all-time heat records and pushing the limits of climatic extremes. The quantification of the dynamical linkage, the evolution and propagation of such heatwaves is a start to understand these processes. This network structure and propagation characteristics for European heatwaves is analyzed using a complex network approach based on E-OBS, the gridded dataset based on in situ data from the European meteorological services.

Complex networks (CN) are data-driven methods suited to model natural non-linear dynamic systems (Dijkstra et al., 2019). CN are based on graph theory; hence a network is composed by two sets (nodes and vertices) conforming a network topology that can be subsequently explored. In this work, we process European-wide daily maximum temperature gridded layers to build up a CN capable of shedding light on interesting mechanisms underlying the heatwave propagation. We identify the source and sink regions primarily responsible for heatwave propagations and the strength of association between these regions. The network coefficients are derived to evaluate the extremal dependence, evolution, and spatial propagation of specific large scale heatwave events.

Enabling the tracking of climate extremes such as heatwaves might be a relevant resource to help evaluating climate attribution methodologies and expanding them further having this visual support. In addition, having a more realistic representation of a heatwave might help reduce uncertainties, hence better guiding the decision-making process. Both types of contributions might be of service at issuing weather warnings tailored to regions, therefore improving the social preparedness and response capacity when heatwaves hit a region (e.g. excess human mortality associated with heat stress).

References
Dijkstra, H. A., Hernandez-Garcia, E., Masoller, C., & Barreiro, M. (2019).
Networks in Climate. Cambridge: Cambridge University Press, Cambridge, UK and New York, NY, USA. 

How to cite: Garcia-Marti, I., van der Schrier, G., and Polak, F.: Sources, propagation and sinks of Europe’s major heat waves; a complex network analysis of heat extremes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8274, https://doi.org/10.5194/egusphere-egu23-8274, 2023.

EGU23-8502 | ECS | Orals | CL2.5 | Highlight

Trends and Variability in Extreme Precipitation over India 

Chaithra Sajeevan Thankamani and Krishna AchutaRao

The frequency, intensity and duration of weather and climate extremes have increased globally over the past several decades, and the trend is projected to continue. It is important to understand the changing nature of these extremes as it contributes to better monitoring and prediction, thereby reducing the risk to society. Changes in climate and associated weather extremes may be caused both by natural factors such as internal variability, volcanic eruptions, and solar variability as well as anthropogenic factors such as GHGs, aerosols and land use changes. It is essential to differentiate between the contributions of these drivers in order to take suitable measures to mitigate and adapt. Though the changes in temperature extremes are well-documented, rainfall extremes are significantly heterogeneous around the world.

This study analyses extreme precipitation indices over India (developed by the Expert Team on Climate Change Detection and Indices; ETCCDI) and their relationship with different modes of climate variability. The study examines the mean climatology, long-term trends and variability in extreme precipitation indices over India using the daily gridded rainfall data from the India Meteorological Department (IMD). The analysis is carried out over different homogeneous zones as well as custom-defined areas over India in different seasons. The study finds significant variability of extreme indices in the 2 to 4 year time scales and highlights the role of Indian Ocean Dipole (IOD) and El Niño-Southern Oscillation (ENSO) in modulating extreme precipitation. 

How to cite: Sajeevan Thankamani, C. and AchutaRao, K.: Trends and Variability in Extreme Precipitation over India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8502, https://doi.org/10.5194/egusphere-egu23-8502, 2023.

Marine Heat Waves (MHWs), persistent and anomalously sea water temperature warm events, are known to have significant impacts on marine ecosystems as well as on air-sea exchanges. As global ocean temperatures continue to rise, MHWs have become more widespread, threatening marine ecosystems and their services for food-provision, livelihoods and recreation. Detecting and predicting the occurrence, intensity and duration of these extreme events, and understanding their impacts on marine ecosystems is a key step towards developing science-based solutions for sustainable development.

The project “deteCtion and threAts of maRinE Heat waves – CAREHeat”, funded by ESA in the framework of the Ocean Health initiative, aims at improving the current MHW detection and characterization methodology, as well as advancing the understanding of the physical processes involved, and the corresponding ecological and biogeochemical changes.

This is being to be achieved following a multidisciplinary approach capitalizing on the large potential offered by satellite Earth observations, complemented with in situ field measurements, physical and biogeochemical ocean reanalyses, biogeochemical modelling and emerging machine learning technologies. In this presentation an overview of the CAREHeat Project activities and its preliminary results will be provided. In particular the assessment of the major gaps in scientific knowledge, existing products and tools in MHW detection will be discussed. A first version of the CAREHeat MHW Global Atlas covering the entire satellite era (1981-today) will be presented and analysed to investigate the year-to year MWH variability in spatial extension, intensity, duration and rate of evolution.

Specific work has also been done to investigate the impact of sea temperature trends and prominent climate modes, as El Nino Southern Oscillation (ENSO), in order to disentangle the slow-varying SST component and quasi-periodic oscillations from the abrupt changes that are characteristics of these extreme events.

A first preliminary analysis of the impact of MWHs on marine ecosystem will be presented.  

Up to date about the project research and results can be found visiting the  CAREHeat website (www.careheat.org) or on Twitter (@ careheat_)

How to cite: Santoleri, R. and the CAREheat team: Detection, characterization and trends of Marine Heat waves in the global worming scenario: the CAREHeat Project, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8961, https://doi.org/10.5194/egusphere-egu23-8961, 2023.

The effects of extreme temperature events depend critically on both the length and amplitude of the events. Here I review numerical evidence from a range of climate models - including complex Earth System Models and highly simplified aquaplanet models - that indicates robust changes in both temperature persistence and variance under climate change. The most robust changes are found over ocean areas and appear to arise from fundamental thermodynamic constraints on atmospheric water vapor concentrations, the moist atmospheric lapse rate, and longwave radiative cooling. It is argued that such constraints will drive robust changes in the persistence and amplitude of temperature variability over the next century that will be superposed on any other changes due to, say, land-surface processes or variations in the ENSO phenomenom.

How to cite: Thompson, D.: Thermodynamic constraints on changes in temperature persistence and variance under climate change, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10154, https://doi.org/10.5194/egusphere-egu23-10154, 2023.

Hourly gauge rainfall measurements and ERA5 reanalysis for the period 1980-2020 are used to identify typical synoptic weather patterns responsible for summer regional hourly extreme precipitation events over the lower Yangtze River basin. It turns out that the Meiyu front or cyclonic shear imbedded in the East Asian summer monsoon (EASM) and landfalling typhoons are the leading contributors. As the dominant synoptic pattern, the EASM accounts for ~93% occurrence of regional hourly rainfall extremes. The double peak diurnal occurrence (morning and late afternoon) of rainfall extremes corresponds to the Meiyu front and cyclonic shear driven by a strengthened and westward extended western North Pacific subtropical high and accelerated low-level southwesterly flow. During 1980-2020, there was a clear increasing trend in the occurrence of regional hourly rainfall extremes over the region. These findings are beneficial to the prediction and risk assessment of extreme rainfall events over the specific region. 

How to cite: Huang, A.: Typical Synoptic Weather Patterns Responsible for Summer regional Hourly Extreme Precipitation Events over the Lower Yangtze River Basin, China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10374, https://doi.org/10.5194/egusphere-egu23-10374, 2023.

This research evaluated the performance of 19 Coupled Model Intercomparison Project phase 6 (CMIP6) models in simulating the Arctic sea ice from the perspective of annual cycle, spatial pattern and temporal variation. Based on the evaluation, five models with better comprehensive performance capacity were optimized as the ensemble to project the response of the East Asian winter climate to the sea ice-free Arctic occurring under the SSP2-4.5 and SSP5-8.5 scenarios, respectively. The ensemble projections indicate that the sea ice-free Arctic is followed by a weakening of the East Asian winter monsoon, which is characterized with the shallower East Asian trough and weaker East Asian jet stream. Concurrently, the winter surface net radiation flux is projected to increase in the East Asian-western North Pacific region. These changes favour large-scale warming in the East Asian-western North Pacific region. Moreover, the warming is more pronounced under the sea ice-free Arctic of SSP2-4.5 than under that of SSP5-8.5. The winter precipitation tends to increase along the East Asian coast from South China to the Sea of Okhotsk. Such an increase is closely associated with the enhancement of low-level moisture. Due to larger enhancement of moisture, there appears greater increase of precipitation in the monsoon region from South China to Japan under the sea ice-free Arctic of SSP5-8.5 compare to that under SSP2-4.5. Substantial changes are also projected for the temperature and precipitation extremes, such as a general increase in warm days and warm nights and an overall intensification of extreme precipitation in the East Asian-western North Pacific region.

How to cite: Song, Z.: CMIP6 projected response of the East Asian winter climate to the sea ice-free Arctic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10470, https://doi.org/10.5194/egusphere-egu23-10470, 2023.

Devastating floods in July-August 2022 led to one-third of Pakistan being under water. The rainfall over Pakistan in these months was extreme—four to six times the 30-year average. We investigate the cause of this historically unprecedented flooding and extreme rainfall using station measurements and reanalysis datasets. In July-August 2022 there was an abnormal distribution of south Asian summer monsoon (SASM) precipitation characterized by more precipitation in Southern Pakistan and Central India but less precipitation in the south of the western Tibetan Plateau. The abnormal distribution of monsoon rainfall was dominated by the weakening of the 200-hPa northern westerly winds and SASM, and associated with anomalous westward moisture transport in the south of the Tibetan Plateau. Moreover, the temperature of the western Tibetan Plateau reaches its peak in 2022. The “heat pump effect” of the Tibetan Plateau led to positive geopotential height anomalies over Pakistan and the western Tibetan Plateau in the mid-to-upper troposphere. This blocked the 200-hPa northern westerly winds and shifted them northward. At the lower troposphere, the easterly winds are enhanced, and the SASM is suppressed. Furthermore, the Tibetan Plateau warming caused increased glaciers melt and large amounts of meltwater that feed the upper Indus River and worsened the floods. In the context of global warming, summers temperatures and melting will increase in the Tibetan Plateau. Our results indicate that this will cause massive flooding over Pakistan, such as in 2022, to become a common occurrence.

How to cite: Li, H.: Tibetan Plateau warming-induced abnormal distribution of south Asian monsoon precipitation contributes to Pakistan's fatal flood in 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10722, https://doi.org/10.5194/egusphere-egu23-10722, 2023.

EGU23-10759 | ECS | Orals | CL2.5

How Do Extreme Summer Precipitation Events Over Eastern China Subregions Change? 

Xin Hao, Linqiang He, Hua Li, and Tingting Han

Spatiotemporal features of summertime extreme precipitation occurrences (EPEs) over eastern China subregions were captured by using observations from the CN05.1 daily data set and K-means clustering from 1961 to 2018. Five subregions including South China (SC), the Yangtze River Basin (YRB), the HeTao Area (HTA), North China (NC), and Northeast China (NEC) are identified, which is distinct from previous studies. The accompanying evolution of synoptic development are discussed, including the high rates of EPEs transfer from the YRB-type to the SC-type (18%), the HTA-type to the YRB-type (16%), the HTA-type to the NC-type (22%), and the NC-type to the NEC-type (25%). Intrinsic relationships that exist within these types of regional EPEs have not been recorded by previous studies. The intraseasonal evolution of summer EPEs shows a northward migration of the rainbelt influenced by the East Asian summer monsoon system. Moreover, temporal variations of regional EPEs from interannual timescales to long-term trends are examined.

 

How to cite: Hao, X., He, L., Li, H., and Han, T.: How Do Extreme Summer Precipitation Events Over Eastern China Subregions Change?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10759, https://doi.org/10.5194/egusphere-egu23-10759, 2023.

EGU23-10834 | ECS | Orals | CL2.5

Cause of the cold condition over northeast Asia in April 2020 

Go-Un Kim, Hyoeun Oh, Yong Sun Kim, Jun-Hyeok Son, Jongmin Jeong, and Jin-Yong Jeong

Although northern Asia's temperature was the fourth highest on record, Northeast Asia was severely damaged agricultural and marine products due to the cold condition in April 2020. Previous studies have shown that the dipole atmospheric circulation over Siberia and the East Sea (also referred to as the Japan Sea) rendered this cold environment. Here we show that the atmospheric structure affecting the cold condition over northeast Asia was a mixed result of the East Atlantic/Western Russia (EAWR) pattern and blocking. The wave train was originated from the vorticity forcing of northwest/central Russia and propagated toward the southeast via the climatologically westerly and northerly flows. Furthermore, the blocking days over Siberia increased approximately ten times in April 2020 than climatology along with the easterly anomaly over Mongolia–northeast China. The blocking occurrence might be connected to wavy westerly at the high latitudes. The strong blocking and EAWR pattern led to the robust dipole atmospheric structure with the prevailing northerly wind in April 2020, thereby causing the cold over northeast Asia. Our results help to understand the cause of the cold condition in April over northeast Asia and its impact on the land and ocean ecosystems.

How to cite: Kim, G.-U., Oh, H., Kim, Y. S., Son, J.-H., Jeong, J., and Jeong, J.-Y.: Cause of the cold condition over northeast Asia in April 2020, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10834, https://doi.org/10.5194/egusphere-egu23-10834, 2023.

The summer extreme high temperature days (EHTDs) in the Northern Hemisphere have been frequently detected, posing a serious threat to the safety of human life, agricultural production, and the ecological environment of many countries. This study investigates the decadal variation of summer EHTDs in northern Eurasia (30°–70°N, 10°–130°E) during 1960–2018, using the EHTD index provided by Hadley Center and the atmospheric circulation and sea surface temperature (SST) data provided by NOAA. Statistical analysis shows that the first principal component of the EHTD index fluctuates slightly over a relatively low level during 1960–1994, while it increases significantly during 1995–2018. Moreover, Z-test and sliding t-test confirm that the decadal variations of the EHTD index in terms of trends and the climatological mean values change significantly around 1994/1995. Therefore, the total period is divided into two phases, i.e., fewer EHTDs and an insignificant trend during the period from 1960 to 1994, and more EHTDs with a significant increasing trend during the late period from 1995 to 2018. During 1960–1994 (1995–2018), low pressure and cyclonic (high pressure and anticyclonic) anomalies controlled Lake Baikal and the Caspian Sea, favoring more (less) cloud cover and precipitation, absent (sufficient) solar radiation and increased (decreased) EHTDs over there. Global warming and internal variability of the North Atlantic are both responsible for the decadal variations of EHTDs. On one hand, regression analysis shows that the global warming trend shows a significant influence on the positive pressure anomalies over the areas to the south of Lake Baikal. On the other hand, during 1995–2018, the anomalous Rossby wave activities induced by warmer than normal North Atlantic leads to high-pressure anomalies over the Caspian Sea, resulting in the significant anticyclonic anomaly over the area, which favors the more frequent occurrence of EHTDs than those during 1960–1994. Meanwhile, the Atlantic jet is located northward. The area around the Caspian Sea is to the right side of the jet stream exit. Under such a background, the negative vorticity advection at the upper-level troposphere would lead to the divergence anomaly and strengthen the sinking motion between lower- and higher- levels. Thus, the summer EHTD tends to be maintained over the Caspian Sea.

How to cite: Fan, Y.: Variations of summer extreme high temperatures in northern Eurasia during the recent decades, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10945, https://doi.org/10.5194/egusphere-egu23-10945, 2023.

Compared with daytime (occurring only in daytime) and nighttime (occurring only in nighttime) heat waves (HWs), daytime-nighttime compound HWs (occurring simultaneously in daytime and nighttime) are highlighted to exert much severer impacts especially on human health. However, the physical mechanisms underlying compound HWs are poorly understood. Based on the observed maximum and minimum temperatures and NCEP/ NCAR reanalysis data, this article addressed the physical processes for the occurrence of compound HWs in East China, where compound HWs occur most frequently across China. Comparisons with those related to daytime or nighttime HWs were also performed. The results indicate that the occurrences of three HW types are all associated with anticyclonic circulation anomalies from the upper troposphere to the lower troposphere, whereas their locations and intensities determine the configuration of atmospheric conditions for different categories of HWs. The resultant less (more) cloud cover and humidity as well as increased downward shortwave (longwave) radiation at the surface favor the warming of daytime (nighttime), conducive to the occurrence of daytime (nighttime) HWs. The combination of above conditions associated with daytime and nighttime HWs, which helps the persistence of high temperatures from daytime to nighttime, benefits the occurrence of compound HWs. In addition, nighttime and compound HWs occur with the northwestward extension of the western Pacific subtropical high (WPSH), while it stays in the climatological location for the occurrence of daytime HWs. Further investigation suggests that daytime (nighttime) HWs are accompanied with an upper-tropospheric meridional (zonal) wave train propagating downstream from western Siberia (the east to the Caspian Sea). In comparison, the wave train related to compound HWs shares the mixed features of daytime and nighttime HWs, characterized by a meridional wave propagation from the Scandinavian Peninsula to East China and then a zonal propagation toward the western Pacific.

How to cite: Xie, W.: On the atmospheric background for the occurrence of three heat wave types in East China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11002, https://doi.org/10.5194/egusphere-egu23-11002, 2023.

EGU23-11077 | ECS | Posters on site | CL2.5

Characteristics of Large-Scale and Localized Droughts in the Gangetic Plains 

Chamarthi Sarat Chandra, Veungopal Vuruputur, and Sekhar Muddu

The groundwater depletion over the past two decades in the Indo-Gangetic Plains has been extensively documented. On a smaller scale, the Bundelkhand sub-region (rectangular box in the Figure) has been experiencing an extended period of meteorological drought. In this region, as with a majority of the Gangetic Plains, the contribution of local evaporation is comparable to the moisture brought in from afar.  It is unclear whether the below-normal rainfall in this region is due to low-frequency climate variability or a result of a "negative" feedback loop in the regional hydrologic cycle where less rain leads to less soil wetness, which in turn leads to lower evaporation and less moisture available for rain. An analysis of this region's daily rainfall records from the past century shows that while most droughts in and around Bundelkhand coincide with larger-scale Indian monsoon droughts (Type-1 in the Figure), some appear to be localized (Type-2 in the Figure). In addition, our analysis shows that while north central India typically experiences a rainfall deficit in early July, western India often sees more than normal rainfall. We present our assessment of the causes of these droughts, including the role of local hydrology and potential large-scale drivers. 

How to cite: Chandra, C. S., Vuruputur, V., and Muddu, S.: Characteristics of Large-Scale and Localized Droughts in the Gangetic Plains, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11077, https://doi.org/10.5194/egusphere-egu23-11077, 2023.

The Yangtze River Valley (YRV) is the main rice-growing region in China and agriculture production in YRV plays a vital role in ensuring food security. Spring is the key season of plowing preparation and sowing, and drought during this period could cause serious threats to agricultural activity in YRV. As a basic feature of drought, consecutive dry days (CDDs), especially the extreme-CDDs with long duration, could directly reflect the drying degree and serve as a good indicator of drought. Therefore, knowledge of variations and mechanisms of spring extreme-CDDs has significant implications for a comprehensive view of spring drought in YRV. Based on daily station precipitation data, the variability of spring extreme-CDDs in YRV is investigated. It is found that the extreme-CDDs in YRV experienced a significant decadal increase around the early 2000s. Associated with this decadal change, the Mongolian high (MH) and western North Pacific anticyclone (WNPA) are significantly intensified and weakened, respectively. The intensified MH and weakened WNPA lead to anomalous northerlies and water vapor divergence over YRV, providing favorable atmospheric conditions for more extreme-CDDs over the region. Further mechanism analyses suggest that the transition of mega-El Niño/Southern Oscillation (mega-ENSO) from the negative-phase to positive-phase contributes to the decadal weakening of WNPA. And the phase transition of Atlantic Multidecadal Oscillation (AMO) and decadal decrease of sea ice over the Barents Sea lead to intensified MH through exciting atmospheric wave train. Multiple linear regression shows that there could be a synergistic role of mega-ENSO, AMO, and sea ice over the Barents Sea in the decadal change in YRV extreme-CDDs around the early 2000s. Analysis on the simulation of 14 models in the Atmospheric Model Intercomparison Project (AMIP) experiment from phase 6 of the Coupled Model Intercomparison Project (CMIP6) shows that the models can reproduce the observed decadal intensification of MH and weakening of WNPA around the early 2000s, indicating the contribution of mega-ENSO, AMO, and sea ice over the Barents Sea to the decadal changes in MH, WNPA and extreme-CDDs in YRV.

How to cite: Zeng, Z.: Decadal change of spring extreme consecutive dry days in the Yangtze River Valley around the early 2000s: Synergistic effect of mega-El Niño/Southern Oscillation, Atlantic Multidecadal Oscillation, and Arctic sea ice, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11219, https://doi.org/10.5194/egusphere-egu23-11219, 2023.

In this study, the variations in the extreme high-temperature event (EHE) over Northern Asia (NA) and the associated possible mechanisms are explored. On an interdecadal timescale, NA EHE frequency experienced a significant interdecadal increase around the mid-1990s, which could be associated with the phase shift of the Atlantic Multidecadal Oscillation. On an interannual timescale, the first two empirical orthogonal function modes of the NA EHE frequency exhibit meridional dipole pattern (EOF1) and diagonal tripolar pattern (EOF2), respectively. Further analysis reveals that the EOF1 mode is related to the Polar-Eurasian teleconnection pattern (POL), while the EOF2 mode is associated with North Atlantic Oscillation (NAO) and Pacific-Japan/East Asia-Pacific pattern (PJ/EAP). The fitted EHE frequency based on the atmospheric factors (POL, NAO and PJ/EAP) can explain the interannual variation in the regionally averaged EHE frequency by 33.8%. Furthermore, three anomalous sea surface temperature (SST) patterns over the North Atlantic-Mediterranean Sea region and around the Maritime Continent are associated with the two EHE modes by intensifying the pronounced atmospheric teleconnections. Analysis on the simulation of five models in the Atmospheric Model Intercomparison Project experiment further confirms the impact of the pronounced SST patterns on the POL, NAO and PJ/EAP. From a synoptic perspective, the atmospheric patterns responsible for the NA EHE are investigated. By applying a hybrid regionalization approach to the daily maximum temperature, three subregions of NA can be identified: western NA, central NA, and southeastern NA. To better understand the mechanism for the formation of EHE in each subregion of NA, the EHE-related synoptic circulation patterns over each subregion are further categorized into two types. These six synoptic circulation patterns influence the NA EHE occurrence through different radiation and advection processes. From the forecasting perspective, six wave train patterns are explored as the precursors of the six synoptic circulation patterns, separately. These wave train patterns appear over the upstream regions of NA subregions with at least three-day lead, and provide potential forecasting information for the NA EHEs. The results may deepen our understanding of the NA EHE formation and provide information for the prediction and forecast of NA EHE.

 

 

How to cite: Hong, H.: Variations in Summer Extreme High-temperature Events over Northern Asia and the Possible Mechanisms, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11276, https://doi.org/10.5194/egusphere-egu23-11276, 2023.

EGU23-11356 | ECS | Posters virtual | CL2.5 | Highlight

The Role of the Ocean for the Development of Heat Waves over Europe 

Sabine Bischof, Robin Pilch-Kedzierski, Martje Hänsch, and Katja Matthes

European heat waves are becoming more and more severe under global warming. The frequency and duration of heat waves are very likely to further increase under future climate conditions over most land areas. To improve the predictability of such extreme events, it is important to understand their driving mechanisms better.

Although earlier work hints at a connection between North Atlantic sea surface temperatures (SSTs) and the occurrence of European heat waves, the role of the ocean in shaping heat waves is still not fully understood. Here, we investigate the effect of the 2018 SST pattern, which was characterized by negative anomalies in the North Atlantic, on European heat wave characteristics.

Using the Flexible Ocean and Climate Infrastructure (FOCI) model we conducted two 100-year long AMIP-like model experiments: one that employs the observed global 2018 SST and sea ice patterns as a boundary forcing and another one that differs only in the North Atlantic SST field, for which we removed the cold SST anomaly. Comparing these two experimental settings, we find that cold North Atlantic SST anomalies can favor heat wave conditions especially over the most eastern part of the European continent.

How to cite: Bischof, S., Pilch-Kedzierski, R., Hänsch, M., and Matthes, K.: The Role of the Ocean for the Development of Heat Waves over Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11356, https://doi.org/10.5194/egusphere-egu23-11356, 2023.

EGU23-11753 | ECS | Orals | CL2.5

Assessing the role of thermodynamic drivers underlying extreme heat in a warming climate 

Dominik L. Schumacher, Mathias Hauser, and Sonia I. Seneviratne

In recent years, heatwaves around the globe have eclipsed long–term maximum temperature records. While a stronger warming over land than sea is both expected and observed, regional hot extremes are warming at an even faster pace. Modeling studies have suggested that soil moisture–temperature feedbacks drive this amplification in climate projections of the ongoing century, and there is solid observational evidence of a link between high temperatures and desiccating soils for individual events: dry soils invoke a shift in the surface energy partitioning toward sensible heating, thereby promoting higher air temperatures. A particularly notable heatwave unfolded in late June 2021 in the Pacific Northwest, baffling the scientific community with its high intensity. Using a combination of reanalysis data and factorial Earth System Model simulations, we show that heat released from condensation over the North Pacific and local soil moisture deficits strongly contributed to the extreme heat where the temperatures were most anomalous. Mediated by desiccating soils, our analysis also points to complex land–atmosphere interactions beyond intensified surface sensible heating. Since it remains unclear to what extent an enhanced thermodynamic potential — such as epitomized by this remarkable “black swan event” — is responsible for the observed exacerbation of heatwaves in recent decades, we we also investigate the link between summertime soil drought and hot extremes in our changing climate.

How to cite: Schumacher, D. L., Hauser, M., and Seneviratne, S. I.: Assessing the role of thermodynamic drivers underlying extreme heat in a warming climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11753, https://doi.org/10.5194/egusphere-egu23-11753, 2023.

EGU23-13740 | ECS | Orals | CL2.5

Detecting Extreme Temperature Events Using Gaussian Mixture Models 

Aytaç Paçal, Birgit Hassler, Katja Weigel, M. Levent Kurnaz, and Veronika Eyring

Extreme events are rare atmospheric phenomena that cause significant damage to humans and natural systems, but detecting extreme events in the future in a changing climate can be challenging. Traditionally, temperature distributions were assumed to follow a normal distribution and certain thresholds were used to define extreme events. However, the mean and the variance of temperatures are expected to change in a future climate, which might limit the application of traditional methods for detecting extreme events.

We found that daily maximum surface temperature data can be described accurately using a multimodal distribution. In this study, we therefore used a statistical method called Gaussian Mixture Models (GMM) to fit a multimodal distribution to daily near-surface maximum air temperature data from simulations participating in the Coupled Model Intercomparison Project Phase 6 (CMIP6) for 46 Intergovernmental Panel on Climate Change (IPCC) land regions. GMM allowed us to use the parameters from the Gaussian distribution fitted to the higher temperatures to define the thresholds for the return period of extreme events. We analysed the change in the return periods of extreme temperature events in study regions compared to the historical period (1980-2010) under future Global Warming Levels (GWL) of 1.5°C, 2°C, 3°C and 4°C for each Shared Socioeconomic Pathways (SSP) scenarios. 

How to cite: Paçal, A., Hassler, B., Weigel, K., Kurnaz, M. L., and Eyring, V.: Detecting Extreme Temperature Events Using Gaussian Mixture Models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13740, https://doi.org/10.5194/egusphere-egu23-13740, 2023.

EGU23-14462 | ECS | Posters on site | CL2.5

Analysis of rainfall generation process in east Asia by Summer Cold Wave 

Kwang-Hee Han, Ho-Young Ku, Jee-Hoon Jeong, and Baek-Min Kim

In August 2022, extremely heavy rainfall occurred in the central region of the Korean Peninsula. On August 8, Seoul received 381.5 mm of rain, the most in 115 years. Heavy rain is a phenomenon that accounts for the most significant portion of dangerous weather occurring in Korea, and many studies, including the mechanism of occurrence, have been done on this phenomenon. However, the synoptic pressure pattern that caused heavy rain in August 2022 differed from the rainfall pattern studied in general. The pressure system around the Korean Peninsula also showed a different pattern from the typical summer pressure characteristics. As a result, by reviewing the pressure system specificity of the Korean Peninsula and the Eurasian continent, this study investigated the mechanism and climatological factors of heavy rain in August 2022. In August 2022, strong high pressure developed over the Eurasian continent, the Kamchatka Peninsula, and the Ural Mountains. On August 8, a stationary front crossing the Korean Peninsula from east to west was located. To determine the specificity of the barometric pressure system, the air temperature and barometer of the ground and upper layers were analyzed using ECMWF's ERA-5 reanalysis data. At the surface level, high pressure intensified near the Ural Mountains and Lake Baikal in Siberia in early August. In the case of temperature, the advection of cold air below a -5°C anomaly from high latitudes to the northwest of the Korean Peninsula through Siberia following the flow of lower high pressure is analyzed. At 500 hPa, upper-level blocking was observed in the Ural Mountains and the Kamchatka Peninsula. The blocking over the Eurasian continent reduced zonal flow while increasing meridional flow. Cold air from the high latitudes was transported to East Asia by the increased meridional flow. The cold air that moved toward East Asia met the edge of the North Pacific high pressure and formed a stationary front, causing heavy rain. In this study, the development of a cold continental high pressure in summer affecting the mid-latitude region was defined as the "Summer Cold Wave" (SCW), and the development of the front by the SCW was defined as the "Summer Cold Front" (SCF). In addition, by analyzing cases where SCW occurred in the past, it was determined that the development of Ural blocking in summer influenced the occurrence of SCW, and it was determined that precipitation due to SCF increased in the Korean Peninsula when the North Pacific high pressure occurred strongly.

How to cite: Han, K.-H., Ku, H.-Y., Jeong, J.-H., and Kim, B.-M.: Analysis of rainfall generation process in east Asia by Summer Cold Wave, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14462, https://doi.org/10.5194/egusphere-egu23-14462, 2023.

EGU23-15195 | Orals | CL2.5

Extremely hot East Asia and flooding western South Asia in the summer of 2022 tied to reversed flow over Tibetan Plateau 

Chao He, Tianjun Zhou, Lixia Zhang, Xiaolong Chen, and Wenxia Zhang

In the summer (July and August) of 2022, unprecedented heat wave occurred along the Yangtze River Valley (YRV) over East Asia while unprecedented flood occurred over western South Asia (WSA), which are located on the eastern and western sides of Tibetan Plateau (TP). By analyzing the interannual variability based on observational and reanalysis data, we show evidences that these two extreme events are mutually connected, and the anomalous zonal flow over subtropical Tibetan Plateau (TP) explains a major fraction the extreme events occurred in 2022. In summer, there is a warm center in the atmosphere over TP, and the isentropic surfaces incline eastward (westward) with altitude on the eastern (western) side of the warm center over TP. As adiabatic flow move along isentropic surfaces, anomalous easterly (westerly) flow generates anomalous descent (ascent) on the eastern side of TP and anomalous ascent (descent) on the western side of TP via isentropic gliding. The anomalous easterly flow is extremely strong to reverse the climatological westerly flow over subtropical TP in 1994, 2006, 2013 and 2022. The easterly flow in 2022 is the strongest since 1979, and it generates unprecedented descent (ascent) anomaly on the eastern (western) side of TP, leading to extreme heat wave over YRV and extreme flood over WSA in 2022. The anomalously strong easterly flow over subtropical TP in 2022 is dominated by atmospheric internal variability related to mid-latitude wave train, while the cold sea surface temperature anomaly over the tropical Indian Ocean increases the probability of a reversed zonal flow over TP by reducing the meridional gradient of tropospheric temperature.

How to cite: He, C., Zhou, T., Zhang, L., Chen, X., and Zhang, W.: Extremely hot East Asia and flooding western South Asia in the summer of 2022 tied to reversed flow over Tibetan Plateau, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15195, https://doi.org/10.5194/egusphere-egu23-15195, 2023.

Atmospheric blockings have widespread, long-lasting, and severe consequences in a variety of regions, causing climate extremes such as drought, heavy rainfall, cold spells, and heatwaves. Depending on where the blocking occurs, climate anomalies caused by high-latitude Euro-Atlantic winter blockings, in particular, have a significant impact on Arctic sea ice export in the North Atlantic, and thus on the freshwater budget in deepwater formation regions, and also impact Greenland ice cap and Arctic sea ice recovery during the cold polar season. Understanding the evolution of future winter Euro-Atlantic blockings in the context of climate change is thus critical for accurately predicting future changes in cryosphere systems and ocean circulation. The future evolution of these blockings, however, remains highly uncertain because coupled climate models generally fail to reproduce their frequencies of occurrence and spatial locations in historical runs. Meanwhile, recent research has shown that historical atmospheric blockings are much better simulated in climate models with eddy-permitting ocean resolutions due to more accurately represented mean climate states and air-sea interactions. Here, we show that eddy-permitting climate models provide blocking projections with much lower uncertainties in terms of frequency and spatial extent by using an ensemble of more than a hundred of CMIP6 climate model simulations, both ran with and without eddying ocean models. Finally, we show from the set of model simulations with eddying ocean models that the frequency of blocking types leading to dryer and warmer winter conditions in North Atlantic-Arctic regions for the next three decades is likely to increase under strong warming scenarios. Such an evolution in blocking activity would trigger large sea ice export events in the North Atlantic and a low rate of recovery of Artic sea ice and the Greenland ice cap during winter, leading to quicker ice loss in general than for climate models with standard ocean grids resolutions.

How to cite: Michel, S. L. L., von der Heydt, A. S., and Dijkstra, H. A.: New projections of winter Euro-Atlantic atmospheric blocking activity under strong warming scenario and consequences for Arctic land and sea ice, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15205, https://doi.org/10.5194/egusphere-egu23-15205, 2023.

EGU23-16399 | Posters virtual | CL2.5

Spatial and temporal variability of compound drought heatwave events in the Northern Hemisphere 

Chan Diao, Liang Zhao, Xiuchen Wu, and Yang Li

Recent decades have witnessed a notable increase in the compound drought and heatwave events (CDHW) in many regions across the globe, which may have more complex and intense implications on terrestrial ecosystem stability than individual extreme events.  It is necessary to clarify the response of terrestrial ecosystems to compound drought-heatwave events. However, the research is remain poorly understood about this. Therefore, we used the Standardized Precipitation Index (SPI) and temperature data to extract the regions where occur compound drought and heatwave events in global. The results obtained in this study are as follows: Firstly, the majority of the regions that have experienced compound drought heatwaves have experienced only one such event, while only a small percentage have experienced two such events. Secondly, we found that the number of compound drought heatwave events in all years is generally more in drylands than in wetlands.

How to cite: Diao, C., Zhao, L., Wu, X., and Li, Y.: Spatial and temporal variability of compound drought heatwave events in the Northern Hemisphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16399, https://doi.org/10.5194/egusphere-egu23-16399, 2023.

Abstract

The empirical probability distribution of extreme precipitation in the eastern United States comprises heavy rainfall events stemming from the moisture held by the Atmospheric Rivers (ARs). In many sites, ARs trajectories can have varying impacts on the extreme precipitation seasonality based on the moisture source and tracks. Consequently, a characterization of location specific and regional patterns of timing of extreme precipitation caused by ARs and their non-stationarity has salience for both scientific and engineering concerns. To this end, analysis of annual maximum daily precipitation (AMP) at 581 long-term stations across the eastern United States was pursued in this study to evaluate the role of moisture sources and tracks in the seasonality of extreme rainfall-AR related events (AMP-AR) and their temporal changes over the 1950–2015 period. The key results from this study include: (a) spatio-temporal variation in the fraction of annual maximum precipitation events linked to ARs, and (b) a marked influence of moisture sources on the seasonality of AMP-AR related events. Results from this study have important bearing on the flood risk management and preparedness.

How to cite: Dhakal, N. and Aljoda, A.: Role of atmospheric moisture sources and pathways in the seasonality of extreme precipitation over the eastern United States, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16634, https://doi.org/10.5194/egusphere-egu23-16634, 2023.

EGU23-16862 | ECS | Posters on site | CL2.5

High Asia Refined analysis-based Monsoon precipitation characteristics over Indian Himalayas 

Rohtash Saini, Raju Attada, Nischal Sharma, and Sreehari Kizhuveettil

The Himalayas, known as the world's third pole, are extremely vulnerable to the ramifications of extreme precipitation events (EPEs), such as flash floods, landslides, and agricultural and infrastructural damages during the Indian summer monsoon (ISM). Complex terrain, high meteorological diversity and uncertainty in observations over this region, make it challenging to comprehend the precipitation disparities and predict the EPEs across the Western Himalayas (WH). Therefore, a better representation of ISM precipitation characteristics over the WH using high-resolution data is crucial for precisely understanding the precipitation variability and mechanisms of climate-triggered localised natural disasters. This study investigates the spatiotemporal variability of precipitation and EPEs using High Asia Refined analysis version 2 (HAR v2), during ISM. It is generated by dynamically downscaling global ERA5 reanalysis data, using Weather Research and Forecasting model (WRF). Before investigating the EPEs, we evaluated HAR v2's ability to represent general characteristics of ISM over the WH against reanalysis, satellite and observational datasets. Preliminary results indicate that, HAR v2 reanalysis better represented the spatiotemporal patterns of precipitation and EPEs across WH. The present study will also investigate the dynamic and thermodynamic processes, associated with EPEs over the study region. Overall, this study aims to provide scientific insights to investigate the potential impacts of climate change on extreme events, which in turn could help mitigate disasters in the Himalayan region. Detailed results of precipitation variability over the Himalayas, and mechanisms altering the atmospheric conditions attributed to the EREs will be discussed.

Keywords: Indian Summer Monsoon, Himalayas, HAR-V2 reanalysis, Extreme Precipitation Events

How to cite: Saini, R., Attada, R., Sharma, N., and Kizhuveettil, S.: High Asia Refined analysis-based Monsoon precipitation characteristics over Indian Himalayas, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16862, https://doi.org/10.5194/egusphere-egu23-16862, 2023.

EGU23-17028 | ECS | Posters on site | CL2.5

Diagnosis of Extreme Precipitation Events in the Yucatan Peninsula. 

Marta Paola Rodríguez González and Ruth Cerezo Mota

Given the impacts of human-induced global warming on the water cycle, it is relevant to pay attention to those impacts on water security as it is one of the UN's SDGs (sustainable development goals).

Many studies on future climate projections agree on a positive trend of extreme precipitation in various regions of the world. However, the process and causes of those events are not always clear and can change depending on local scales.

On the one hand, there is a dynamic mechanism due to atmospheric circulation, and on the other, there are local and thermodynamic effects from surface variables. In addition, the characteristics of the vegetation cover can influence the distribution and conservation of water in the system.

The Yucatan Peninsula - located in the southeastern part of Mexico- has a particular climate due to its morphological and hydrological characteristics (scarce orography and absence of rivers). Therefore, in this region, the recharge of the aquifer depends entirely on rainfall.

In this study, we first characterised the trend of precipitation in the last 30 years. Then we analysed the region's contribution to total annual precipitation by different hydrometeorological phenomena (e.g. tropical cyclones and cold fronts). Finally, simulations with RegCM4 were analysed to understand local mechanisms that favour the occurrence of extreme rainfall related to changes in vegetation and land use due to urbanization.

In general, the results show that the accumulated total annual precipitation has a negative trend, while the contribution of extreme events to total precipitation has increased. Moreover, under urban land use, precipitation would increase, especially in the spring months, and it would decrease during the summer.

Keywords: precipitation, extreme events, land use change, Yucatan, RegCM, urbanization.

How to cite: Rodríguez González, M. P. and Cerezo Mota, R.: Diagnosis of Extreme Precipitation Events in the Yucatan Peninsula., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17028, https://doi.org/10.5194/egusphere-egu23-17028, 2023.

EGU23-296 | ECS | Posters on site | CL2.4

Summer winds over the Iberian Peninsula related to thermal low conditions from COSMO-REA6 (1995-2018) high-resolution reanalysis 

María Ortega, Enrique Sánchez, Claudia Gutiérrez, Noelia López-Franca, Miguel Ángel Gaertner, and María Ofelia Molina

Thermal low pressure systems are typically generated over continental mid-latitudes and subtropical regions during summer, related to a strong heating over land caused by the long lasting solar radiation during this part of the year. They present a clear diurnal cycle, being more intense during the afternoon, and weakens at nighttime. In Europe, a thermal low forms frequently over the Iberian Peninsula. As strong pressure gradients are generated from the coastal regions to the interior of the Peninsula, wind characterization is a relevant feature to describe the Iberian thermal low. In particular, wind typically enters from the north (the Basque Country) and the east (the Mediterranean coast of Murcia and Valencia) through gaps between mountain ranges, and move respectively in a southwestward or westward direction. In the northern area, the wind flows into the regions of Burgos and Valladolid after channeling across the Duero valley, while in the southeast it reaches a large part of Castilla-La Mancha and even Extremadura. These winds are known in the Iberian Peninsula, for example, the regional wind from the Mediterranean to the Castilla-La Mancha plateau is typically named as Solano. Nevertheless, no systematic effort has been made to fully characterize and quantify its frequency or intensity, so no objective thresholds of wind speed, direction or spatial extension have been defined so far. A first effort to define such objective values is then proposed here. Hourly 10-m wind and 2-m specific humidity fields from COSMO-REA6 very high resolution (0.055º) reanalysis covering the 1995-2018 period are used. This high resolution, both temporal and spatial, will allow us to inspect the orographic aspects that seem to be relevant for these regional winds, together with its clear diurnal cycle and the moisture transport from coastal to inner regions. Humidity is a relevant variable for characterizing these flows, as there are marked differences between the moist air entering from the sea and the dry summer air characteristic of the inner regions of the Iberian Peninsula. The climatic perspective allows to study if interannual variability or trends are also relevant. First results indicate that these regional winds, with mean hourly speeds above 5 m/s for several hours per day, appear during most of the summer days, with important variations in spatial extension and strength. Strong moisture gradients are frequently observed during such episodes. Maximum speed and humidity jumps occur during the afternoon. This analysis is just a starting point, which will be followed by a deeper examination of these flows.

How to cite: Ortega, M., Sánchez, E., Gutiérrez, C., López-Franca, N., Gaertner, M. Á., and Molina, M. O.: Summer winds over the Iberian Peninsula related to thermal low conditions from COSMO-REA6 (1995-2018) high-resolution reanalysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-296, https://doi.org/10.5194/egusphere-egu23-296, 2023.

EGU23-615 | ECS | Posters on site | CL2.4

Convection-Permitting Future Climate Simulation Based on SSP3-7.0 Scenario Over the Black Sea Basin 

Mehmet Baris Kelebek and Barış Önol

The regional climate models are recently run at grid spacings of 4 km or less, so-called the convection-permitting scale, over different regions of the world. The previous studies highlighted the added value of the convection-permitting simulations, especially in representing the daily and sub-daily precipitation over complex topography. The Black Sea Basin, including the coastal areas of the Black Sea and a broad part of the Anatolian Peninsula, is one of the climate change hot-spots with its complex topographical features and where strong air-sea interactions occur. Previously, this region has become a subject of regional climate modelling studies at horizontal resolutions on the order of 10 km. In this study, we performed a decade-long convection-permitting climate simulation at 3 km horizontal resolution between 2061-2070 based on the SSP3-7.0 greenhouse gas emission scenario over the Black Sea Basin. To this end, we downscaled the last generation CMIP6 MPI-ESM1.2-HR outputs by using the WRF model. The results indicate that the daily 2m mean, minimum, and maximum air temperatures increase in the spring, summer, and autumn by about 3°C compared to the 2005-2014 reference period over the study area. Nevertheless, the increase in the cloud cover suppresses the warming in the winter. In terms of precipitation, the total precipitation amount decreases in spring and summer over the Black Sea Basin. On the other hand, the total precipitation amount increases significantly by about 3 mm/day in winter over the Eastern Black Sea region due to the positive change in evaporation of around 15%. The maximum daily precipitation amount reaches 350 mm over the northeast of Turkey and over the Caucasus. The intensification of the daily precipitation is most pronounced in the coastal subregions of the Black Sea Basin. Furthermore, the results highlight the intensification of sub-daily precipitation in these regions. In particular, the afternoon precipitation increases in autumn over the coastal regions of Turkey.

How to cite: Kelebek, M. B. and Önol, B.: Convection-Permitting Future Climate Simulation Based on SSP3-7.0 Scenario Over the Black Sea Basin, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-615, https://doi.org/10.5194/egusphere-egu23-615, 2023.

EGU23-2428 | Posters on site | CL2.4

The use of regional climate models for estimating past and future precipitable water vapor and extreme precipitation over Ethiopia 

Bert Van Schaeybroeck, Abdisa Kawo, Roeland Van Malderen, and Eric Pottiaux

There exist well known relations between Precipitable Water Vapor (PWV) and extreme rainfall which are of prominent importance in the context of climate change. These relations, however, are mostly established in mid-latitudes and for flat terrain. Ethiopia, however, is located in the tropics and features a complex orography, both of which may modulate these relations. We investigate PWV and extreme precipitation over Ethiopia by use of Regional Climate Models (RCMs) from the Coordinated Regional Climate Downscaling Experiment (CORDEX). We first evaluate the RCMs by comparing their annual PWV cycles with the ones obtained from Global Positioning System observations and reanalysis in the past. Additionally, we focus on the behaviour of PWV before and after a heavy-rainfall event. It is found that there are two characteristic timescales, both for the build-up and for the decline around the event of the heavy precipitation: a timescale of about 2 days and a longer timescale that extends beyond ten days which seems unreported in the literature. The RCMs are capable of reproducing the PWV annual cycle and the spatial variability. However, there is a predominantly dry bias that strongly increases with elevations. The RCMs reproduce well the spatial differences of the PWV anomaly peak during a heavy-rainfall event but overestimate the timescales of build-up and decline. Future PWV-changes scale linearly with the near-surface temperature changes at a rate of 7.7% per degree warming and locally increase up to 40% for the end-of-the-century RCP8.5 scenario. Changes in rainfall extremes, on the other hand, do not follow this trend especially in north-western Ethiopia, potentially caused by an overall decrease in rainfall in that region.

How to cite: Van Schaeybroeck, B., Kawo, A., Van Malderen, R., and Pottiaux, E.: The use of regional climate models for estimating past and future precipitable water vapor and extreme precipitation over Ethiopia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2428, https://doi.org/10.5194/egusphere-egu23-2428, 2023.

Abstract
Assessing agricultural drought is of great importance as it is viewed as the most serious problem in most
countries in terms of food security, economy, and social stability. Various drought indices have been
developed in order to describe the characteristics of drought such as severity, extent, frequency and
duration. These indices can be classified into two categories: ground-based and remotely-sensed indices.
Ground-based drought indices are more accurate but limited in coverage, while remote sensing drought
indices cover large areas but have poor precision. Therefore there is need to apply advanced data fusion
methods based on satellite data and ground-based drought indices to fill this gap. However there is a lag
time between drought events and the impacts they cause.
Due to the semi arid conditions of Botswana, the country is prone to the occurrence of droughts and has
a great influence on agriculture and economy of the country at large. In order to monitor droughts in
Botswana this paper proposes that it is necessary to link the pre meteorological observations and the
consequential vegetation drought. This is neededed for effective monitoring of agricultural drought and
early warning. In this study, MODIS reflectance data and data from recent satellites such as landsat OLI,
Sentinel will be used to discover relationships between vegetative drought and meteorological drought
using vegetation condition index (VCI) derived from NDVI and NDWI, and meteorological drought
derived from SPI and SPEI in Botswana. Dataset derived from Soil Moisture Active Passive (SMAP)
will be used to generate %soil moisture content. The %moisture content will be compared with
experimental results from the field. Pearson correlation analyses were performed between single remote
sensing drought indices and in-situ drought indices, NDVI and SPEI. Preliminary studies show that VCI
derived from NDWI (VCI-2) over Southern District of Botswana can be used as an approach to monitor
and provide early warnings. However, there is weak correlation SPEI and VCI-1 and VCI-2 ranging
from -1 to 0.2.

How to cite: Matsuokwane Manyothwane, T. and Mengistu Tsidu, G.: Dryland land crop yield sensitivity to drought in Botswana: Development ofstatistical tools based on satellite remote sensing, observation and climate models foruse in risk assessment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3481, https://doi.org/10.5194/egusphere-egu23-3481, 2023.

EGU23-3516 | Posters on site | CL2.4

Improved bias-adjustment methods for subdaily precipitation extremes 

Hans Van de Vyver, Bert Van Schaeybroeck, Lesley De Cruz, Rafiq Hamdi, and Piet Termonia

Extreme precipitation events are responsible for severe damage to various aspects of human society and ecosystems. Short-term extremes especially affect people in urban areas through flash floods. Extremely heavy precipitation is increasing in frequency and intensity due to global warming and Regional Climate Models (RCMs) of high-resolution are needed to estimate associated increased risks. However, even the RCMs that explicitly resolve deep convection are known to significantly underestimate subdaily precipitation extremes. Impact modellers and other users of climate projections therefore often use some form of bias correction. 

In this study, we propose bias adjustment methods especially designed for the estimation of future subdaily extreme precipitation return levels. These methods take into account the scaling intensity-duration-frequency (IDF) relationship between different levels of accumulation, and jointly estimate extreme rainfall over multiple rainfall durations (i.e. from hourly to multi-day extreme precipitation events). After comparison with established methods, we identify only one method that preserves the scaling IDF relationship, which is a necessary condition to have bias-adjusted return levels consistent among the different durations. A comparative analysis in a multi-model pseudo-reality setting shows that this method is superior to existing bias adjustment methods.

Finally, future projections of bias-adjusted subdaily precipitation return levels for Belgium are obtained in the form of an ensemble of 28 EURO-CORDEX simulations at 0.11° spatial resolution, under the RCM8.5 emission scenario.

How to cite: Van de Vyver, H., Van Schaeybroeck, B., De Cruz, L., Hamdi, R., and Termonia, P.: Improved bias-adjustment methods for subdaily precipitation extremes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3516, https://doi.org/10.5194/egusphere-egu23-3516, 2023.

EGU23-4462 | ECS | Posters on site | CL2.4

Lagrangian analysis of convective rainfall under different synoptic forcing 

Edmund P Meredith, Uwe Ulbrich, and Henning W Rust

Precipitation is commonly analysed from an Eulerian perspective, in which rainfall is considered at a fixed location. Lagrangian analysis of precipitation represents an alternative approach. Here, precipitation objects – for example, convective cells – are identified in a precipitation field and are then tracked through space and time, allowing object properties over the whole life of a convective cell to be collected. This approach offers additional insights into the mechanisms by which convective cells develop and behave across their lifecycle, which would not be evident from standard analysis methods.

In this study, we perform Lagrangian analysis of convective cells under different large-scale circulation regimes. Tracking is based on convection-permitting simulations with the COSMO-CLM at 0.025° resolution over central Europe. All identified precipitation objects are tracked through space and time, collecting cell characteristics for each object, e.g. cell area, intensity, distance travelled, etc. Here we associate precipitation objects with categorical synoptic-scale circulation patterns and compare the cell properties between the different categories.

How to cite: Meredith, E. P., Ulbrich, U., and Rust, H. W.: Lagrangian analysis of convective rainfall under different synoptic forcing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4462, https://doi.org/10.5194/egusphere-egu23-4462, 2023.

EGU23-5185 | ECS | Posters on site | CL2.4 | Highlight

Linking future Gulf Stream warming and increased European winter precipitation in an eddy-rich model 

Eduardo Moreno-Chamarro, Louis-Philippe Caron, Pablo Ortega, Saskia Loosveldt Tomas, Malcolm J. Roberts, Aude Carreric, Amanda Frigola, and Eneko Martín Martínez

This contribution discusses future changes in Gulf Stream temperatures, winter precipitation over northwestern Europe, and their connection. We compare HighResMIP historical and ssp5-8.5 scenario simulations generated with five different configurations of the global coupled model HadGEM3-GC3.1, including one at a pioneering 50-km-atmosphere–1/12°-ocean global resolution. The highest resolution model projects an increase in winter rainfall over Europe outside or to the extremes of multimodel ensembles, such as CMIP6 and HighResMIP, for which both the highest ocean and atmosphere resolutions are essential: on the one hand, only the eddy-rich ocean (1/12°) projects a progressive northward shift of the Gulf Stream and substantial surface warming of the region; on the other, only the 50-km atmosphere translates such warming into strengthened extratropical cyclone activity over the North Atlantic and, hence, increased rainfall over Europe. The results suggest that climate projections relying on traditional ~100-km-resolution models might underestimate climate changes in the North Atlantic and Europe, demonstrating the importance of improved Gulf Stream representation for robust uncertainty estimates of climate risk.

We also present the first results of the STREAM project, which aims to study the role of the ocean mesoscale in driving North Atlantic and European climate variability and predictability. We describe the results of the HighResMIP simulations generated with the EC-Earth global climate model at the T1270-ORCA12 resolution (about 15 km in both the atmosphere and the ocean) and explore the main model biases and response to climate change, as well as the variability in the North Atlantic circulation associated with subpolar oceanic deep mixing. 

How to cite: Moreno-Chamarro, E., Caron, L.-P., Ortega, P., Loosveldt Tomas, S., Roberts, M. J., Carreric, A., Frigola, A., and Martín Martínez, E.: Linking future Gulf Stream warming and increased European winter precipitation in an eddy-rich model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5185, https://doi.org/10.5194/egusphere-egu23-5185, 2023.

EGU23-6121 | Orals | CL2.4

Modeling present-day and future extreme events in the Lake Victoria Basin 

Nicole van Lipzig, Jonas Van de Walle, Matthias Demuzere, Andreas H. Fink, Patrick Ludwig, Grigory Nikulin, Joaquim Pinto, Andreas F. Prein, Dave Rowell, Minchao Wu, and Wim Thiery

The population in the Lake Victoria Basin (LVB) is affected by extreme weather both on land, where flooding regularly occurs and on the lake, where nightly storms often catch fishermen by surprise. The CORDEX Flagship Pilot Study ELVIC investigates how extreme weather events will evolve in this region of the world and to provide improved information for the climate impact community. Here we evaluate the performance of five regional climate models at convection-permitting resolution and present projections for the future using COSMO-CLM in a pseudo global warming approach. Most substantial systematic improvements were found in metrics related to deep convection in convection-permitting models compared to their coarser scale counterparts. For the future, extreme precipitation and wind gusts are expected to increase over the lake due to an thermodynamically induced increase in water vapor whereas the impacts of weaker meso-scale circulation over the lake and stronger thunderstorm dynamics compensate each other. More compound events are expected for the future during which both rainfall and wind gusts are intense. Interestingly, the mean precipitation is strongly affected by uncertainties in large-scale dynamics whereas thermodynamics dominate extreme precipitation. This might imply that uncertainties in future projected extremes are smaller than those in mean precipitation.

How to cite: van Lipzig, N., Van de Walle, J., Demuzere, M., Fink, A. H., Ludwig, P., Nikulin, G., Pinto, J., Prein, A. F., Rowell, D., Wu, M., and Thiery, W.: Modeling present-day and future extreme events in the Lake Victoria Basin, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6121, https://doi.org/10.5194/egusphere-egu23-6121, 2023.

EGU23-6228 | Posters on site | CL2.4

Pseudo-global-warming experiments for West Africa 

Beth Woodhams, Peter Knippertz, and Andreas Fink

With a rapidly growing population, West Africa is particularly vulnerable to the effects of climate change. While results from the Coupled Model Intercomparison Project (CMIP) experiments cannot agree on the sign of the end-of-century mean precipitation change over West Africa, there is consistent agreement that the most extreme precipitation events will become more intense. Indeed, an increase in the intensity of the most extreme events has already been observed in rain gauge and satellite datasets. These events are vital to understand since heavy rain can cause flooding as well as resulting property, infrastructure and crop damage, spread of disease and ultimately loss of life.

In West Africa, the majority of rainfall is delivered via Mesoscale Convective Systems (MCSs). Convection associated with the land–sea breeze circulation is also significant along the Guinea Coast. It is well understood that coarse climate models are unable to accurately represent systems on the meso- and local-scale and that high-resolution ‘convection-permitting’ models are required to represent the diurnal cycle, intensity, and organisation of convection. However, such models are expensive to run, especially for the long periods required for climate simulations. One solution is to run pseudo-global-warming (PGW) simulations, where 4D (x,y,z,t) climate ‘deltas’ from CMIP models are added to high-resolution reanalysis. The resulting dataset is then used as a boundary condition for high-resolution model runs of case study events in the future climate. In this work, the ERA5 reanalysis is used as the base, and the simulations are performed using the ICOsahedral Nonhydrostatic (ICON) model.

Initial results from bespoke PGW case studies for West Africa will be presented to show how the character of present-day extreme events might change if they were to occur in a future climate. In particular, the work will look at the thermodynamic and dynamic contributions to changes in intensity. Furthermore, changes in storm evolution, propagation and organisation will be analysed.

How to cite: Woodhams, B., Knippertz, P., and Fink, A.: Pseudo-global-warming experiments for West Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6228, https://doi.org/10.5194/egusphere-egu23-6228, 2023.

EGU23-6829 | ECS | Orals | CL2.4

Land-atmosphere coupling in km-scale climate modeling: effects of resolution vs. land-surface model sophistication 

Lorenzo Sangelantoni, Stefan Sobolowski, Rossella Ferretti, Gianluca Redaelli, Antonio Ricchi, and Enrico Scoccimarro

Recent studies exhibit a considerable reduction of summer season precipitation frequency in the new generation of convection-permitting (CP) climate simulations. This seems to over-correct non-CP wet biases with a knock-on effect on summer temperatures via soil moisture-atmosphere feedbacks. However, it is difficult to elucidate which part of the warmth/dryness in CP simulations can be ascribed to land-atmosphere coupling and/or "atmosphere-only" processes. Another layer of uncertainty belongs to the still crude representation of land surface/sub-surface processes that become especially relevant when approaching such high resolution.

In this study we explore the modulation of land-atmosphere coupling when moving from a non-CP to a CP-scale climate modeling, considering increasingly sophisticated land surface model configurations. We perform a two-step dynamical downscaling at ~15 km (convection-parameterized) and ~ 3km (convection-permitting) resolutions with the WRF-4.2.1 regional climate model driven by ECMWF-ERA5 reanalysis. The greater alpine region and the extended summer season (May to September) of 2003 are the spatial and temporal domains of interest. A mini multi-physics ensemble is generated with four Noah-MP land-surface model configurations to examine if, and how, including crucial land processes (e.g., vertical soil water transport) modifies hot-temperature forcing mechanisms in the two resolutions. Moreover, each ensemble member is run according to three different initial soil moisture levels, defining reference, anomalously dry- and wet-initialization experiments.

Preliminary results show an improved representation of precipitation statistics (seasonal cumulative, frequency, and 99th percentile) from CP simulations, particularly over complex orography. Generally, maximum temperature reproduction benefits from the CP scale. However, localized warm biases persist over flat terrains regardless of the land surface model configuration. Finally, the two resolutions show a substantially different decay of the initial soil moisture state. At CP scale all three runs converge to similar soil moisture at the end of the integration. Conversely, non-CP runs preserve large soil moisture differences until the end of the summer season, signaling longer soil moisture memory and different soil moisture-precipitation feedback.

These factors might significantly affect the reproduction and predictability of environmental and societal relevant hydroclimatic extremes on a wide-ranging temporal scale, from seasonal climate predictions to long-term climate projections.

How to cite: Sangelantoni, L., Sobolowski, S., Ferretti, R., Redaelli, G., Ricchi, A., and Scoccimarro, E.: Land-atmosphere coupling in km-scale climate modeling: effects of resolution vs. land-surface model sophistication, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6829, https://doi.org/10.5194/egusphere-egu23-6829, 2023.

EGU23-7501 | Orals | CL2.4 | Highlight

The Dutch heat wave of July 2019 in a warmer world: How much hotter could it get? 

Hylke de Vries, Geert Lenderink, Erik van Meijgaard, Wim de Rooij, and Bert van Ulft

Summertime heat waves are extreme meteorological events with a high impact. Three defining aspects are their intensity, duration and spatial extent. All three will change for the worse in a warming world. We illustrate how these changes could play out for the heat wave that produced the hottest day to date in the Netherlands (40.7C, Gilze-Rijen 25 July 2019, a record-shattering event of more than 2 degrees). This is done using a chain of hydrostatic and non-hydrostatic regional climate models of increasing horizontal resolution (12km-2.5km-500m-150m) in combination with the Pseudo Global Warming (PGW) approach. Various scenarios are explored using an ensemble approach to examine robustness. Results indicate that if the 2019 July heat wave were to occur in a +2K warmer world: (i) temperatures would likely reach 45C in many places; (ii) the cumulative heat-wave intensity sum would double; (iii) the time to “cool off” in between heat waves would reduce to a level where the total number of days spent in heat waves roughly equals the number of cool days (Tx<25C); (iv) the area where the 40C threshold is passed will increase strongly; (v) the heat wave will last longer as a simple consequence of the higher temperatures (i.e., an earlier start and a later end). Further persistence increases occur if large-scale circulation changes are supportive; (vi) the temperature response is between 1.5-2 degree per degree global warming, with higher values occurring in scenarios with a stronger future drying. (vii) Finally, during heat waves cities become ‘islands of heat’ where the daily maximum temperatures and the night-time minima are 1-5C higher than in nearby more rural areas. A first impression of these differences is obtained from experimental simulations with the convection permitting model HCLIM43 in ultra-high ‘resolution-of-the-future’ mode (500-150m).

How to cite: de Vries, H., Lenderink, G., van Meijgaard, E., de Rooij, W., and van Ulft, B.: The Dutch heat wave of July 2019 in a warmer world: How much hotter could it get?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7501, https://doi.org/10.5194/egusphere-egu23-7501, 2023.

The intensity of precipitation extremes across Europe is expected to increase through the 21st century under a warming climate . Current coarse-resolution global climate models broadly project increased variability of both wet and dry extremes; however, they rely on parametrizations schemes of crucial processes controlling extreme precipitation such as convection. These methods often introduce errors and thereby induced uncertainties in projections of extremes in the water cycle that are relevant for policy makers and infrastructure planning. The need for accurate extreme event information on such extremes became further evident after the July 2021 floods (Ibebuchi, 2022) and summer 2022 record-breaking heatwaves/drought across Western Europe.

The ongoing H2020 Next Generation Earth Modelling Systems (NextGEMS) project aims to address these issues with the development of fully-coupled storm-resolving Earth-System Models. Using some of the first runs of the Integrated Forecast System (IFS) from ECMWF and ICON from MPI-M at 4 km and 5 km horizontal resolution respectively, we examine individual extreme precipitation events across Europe and evaluate their representation against similar analogues in the Copernicus European Regional Reanalysis (CERRA) and observational datasets. The unprecedented high resolution of the fully-coupled Storm-Resolving Models and CERRA allows for an evaluation of precipitation characteristics in complex terrain like the Alps (Hughes et al., 2009) or complex coastlines. We first evaluate the spatial and temporal structure of the events, compare their representation to coarse-resolution GCMs and then examine the potential drivers such as atmospheric river using integrated moisture transport and vertical structure of the low-level jet (Swain et al., 2015).

Hughes, M., Hall, A., & Fovell, R. G. (2009). Blocking in Areas of Complex Topography, and Its Influence on Rainfall Distribution. Journal of the Atmospheric Sciences, 66(2), 508–518. https://doi.org/10.1175/2008JAS2689.1

Ibebuchi, C. C. (2022). Patterns of atmospheric circulation in Western Europe linked to heavy rainfall in Germany: preliminary analysis into the 2021 heavy rainfall episode. Theoretical and Applied Climatology, 148(1), 269–283. https://doi.org/10.1007/s00704-022-03945-5

Seneviratne, S.I., X. Zhang, M. Adnan, W. Badi, C. Dereczynski, A. Di Luca, S. Ghosh, I.

Iskandar, J. Kossin, S. Lewis, F. Otto, I. Pinto, M. Satoh, S.M. Vicente-Serrano, M. Wehner, and B. Zhou, 2021: Weather and Climate Extreme Events in a Changing Climate. In Climate Change 2021: The Physical Science Basis. Contribution of Working Group I to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change [Masson-Delmotte, V., P. Zhai, A. Pirani, S.L. Connors, C. Péan, S. Berger, N. Caud, Y. Chen, L. Goldfarb, M.I. Gomis, M. Huang, K. Leitzell, E. Lonnoy, J.B.R. Matthews, T.K. Maycock, T. Waterfield, O. Yelekçi, R. Yu, and B. Zhou (eds.)]. Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, pp. 1513–1766, doi:10.1017/9781009157896.013.

Swain, D. L., Lebassi-Habtezion, B., & Diffenbaugh, N. S. (2015). Evaluation of Nonhydrostatic Simulations of Northeast Pacific Atmospheric Rivers and Comparison to in Situ Observations. Monthly Weather Review, 143(9), 3556–3569. https://doi.org/10.1175/MWR-D-15-0079.1

How to cite: Wille, J. and Fischer, E.: Dynamical representation of extreme precipitation events in storm resolving global climate models within the NextGEMS project, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8455, https://doi.org/10.5194/egusphere-egu23-8455, 2023.

An abnormal episode of high rain or snow is classified as heavy precipitation; its extreme intensity and driver mechanisms can vary a lot depending on location and season. The most extreme events can turn into a severe impact at ground (in terms of flood or flash-flood, human casualties and injuries, ecosystem and economy damages and losses).

We have implemented a method to detect the most extreme precipitation events trough 10-year long dataset of high-resolution observations and built on a list of the most disastrous ones occurred between 2000 and 2009 within the so called great alpine region (1°–17° East, 40°–50° North).

The method is then applied to the models belonging to the coordinated experiment CORDEX-FPS dedicated to convection and the ensemble at the convection permitting  scale is able to represent the 70% of such kind of extreme events. The main drivers of the extreme precipitation are analysed and the factors affecting the model ability in correctly reproducing the unsuccessful cases are also investigated.

The same framework has been applied also to the model projections under the RCP8.5 scenario to study the sensitivity of such episodes and of their driving mechanisms to the climate change. The extreme events are projected to increase in frequency especially in the fall season over sub-regions with prevailing orographic forcing, whereas the events related to complex mesoscale interactions are projected to affect larger areas at the end of the century, posing the conditions of increased flood risk.

How to cite: Pichelli, E. and the CORDEX-FPSCONV Team: Detection of disastrous convective events in the great alpine region and analysis of their sensitivity to the climate change, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11196, https://doi.org/10.5194/egusphere-egu23-11196, 2023.

EGU23-12221 | ECS | Posters on site | CL2.4

Applying a scaling approach for extreme precipitation to disentangle thermodynamic and dynamic contributions to CORDEX-FPS simulations​ 

Nicole Ritzhaupt, Stefan P. Sobolowski, and Douglas Maraun and the the CORDEX Flagship Pilot Study on Convection over Europe and the Mediterranean – ensemble

The response of the hydrological cycle to global warming is one of the greatest concerns of climate change. Especially, extreme precipitation can lead to severe physical and economic impacts on human and natural systems. Though extreme precipitation is expected to increase over many land areas an important question remains: which factors drive the uncertainty in extreme precipitation? Answering this will help better understand, prepare for, and ultimately, predict future extreme precipitation. 

In this study, we use a scaling approach for extreme precipitation events developed by O’Gorman and Schneider (2009) to disentangle the thermodynamic and dynamic contributions to these events. Extreme precipitation is scaled by the vertical integral over the product of the vertical velocity (ω; dynamic contribution) and the derivation of the saturation specific humidity (; thermodynamic contribution):

We apply this scaling approach to a subset of the CORDEX-FPS ensemble and focus on change signals of seasonal extremes of daily precipitation for two 10-year periods (2090-2099 vs 1996-2005). By keeping either the first term or the second term in the formula constant over the entire time period we obtain the thermodynamic and dynamic signal, respectively. The thermodynamic signal is quite homogeneous over the domain, approximately in the order of Clausius-Clapeyron scaling (~ 7%/K), while the dynamic signal modifies the thermodynamic signal. Thus, the dynamic contribution, which is represented by vertical wind, is key in understanding differences between models and uncertainty in precipitation changes. The vertical wind profiles show, especially for summer, that the vertical winds during extreme events weaken in the future period compared to the historical period. This seemingly counterintuitive result could be due to more downdrafts leading to extreme precipitation in the future period instead of updrafts. However, a comprehensive interpretation is the subject of ongoing research.

How to cite: Ritzhaupt, N., Sobolowski, S. P., and Maraun, D. and the the CORDEX Flagship Pilot Study on Convection over Europe and the Mediterranean – ensemble: Applying a scaling approach for extreme precipitation to disentangle thermodynamic and dynamic contributions to CORDEX-FPS simulations​, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12221, https://doi.org/10.5194/egusphere-egu23-12221, 2023.

EGU23-13414 | ECS | Posters on site | CL2.4

Spatial and temporal patterns of tropical forest microclimate in Mount Kenya 

Jinlin Jia, Alice C. Hughes, Erone Ghizoni Santos, Petri K.E. Pellikka, and Eduardo Eiji Maeda

Tropical-mountane forests are global biodiversity hotspots, and also play important roles in regional hydrological systems. Yet, climate and especially microclimate in these areas, and how they vary spatially and temporally have been largely neglected. Due to the buffering effect of vegetation, microclimate (i.e. environmental conditions experienced by organisms inside the forest) can be substantially different from the conditions outside the forests. Additionally, sparse meteorological stations and satellite data cannot provide accurate climate estimates over tropical mountains, especially on microclimate under the canopy. Consequently, further research is needed to clarify the spatial and temporal patterns of environmental conditions in these regions.

In this study, we set 16 microclimate sensors on the southern and southeastern slopes of Mount Kenya, with an elevation range of 720 m (from 1730 m a.s.l. to 2450 m a.s.l) across the Lower Montane Wet Forest. The sensors measured understory air temperature and soil moisture every 15-minutes across a 2-year period.

We found that average soil moisture in the study area varied with monthly precipitation, synchronously increasing with the start of the rainy seasons, but decreasing with a approximate one month lag towards the dry seasons. Soil moisture did not have a linear relationship with altitude, presenting a local minimum at about 2050 m a.s.l.. The understory air temperature changed linearly with altitude, whereas the lapse rate varied across seasons. The seasonal variation of diurnal lapse rate was about three times larger than that during the night. For the intra-daily temperature, minimums occured simultaneouly (at 4:30 am) independently of altitude. Conversely, at higher altitudes, the maximum temperature occurred earlier. The lowest average daily temperature and smallest daily temperature range occurred between June and August, whilst the opposite phenomena occurred from January to March. Furthermore, Jan-Feb-Mar also presented the smallest lapse rate and low soil moisture, representing the main period of vegetation growth. Our results will contribute for clarifying the conditions sustaining the disproportionally high biodiversity and biomass observed in tropical mountain forests. Further research will investigate the drivers and biophysical feedbacks of microclimate, as well as their sensitivity to climate change.

How to cite: Jia, J., Hughes, A. C., Santos, E. G., Pellikka, P. K. E., and Maeda, E. E.: Spatial and temporal patterns of tropical forest microclimate in Mount Kenya, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13414, https://doi.org/10.5194/egusphere-egu23-13414, 2023.

EGU23-13843 | ECS | Posters on site | CL2.4

How does the assessment of extreme precipitation profit from convection permitting climate ensembles? 

Marie Hundhausen, Hendrik Feldmann, Regina Kohlhepp, and Joaquim G. Pinto

In response to global warming, an intensification of extreme precipitation has been observed, and models project this trend to continue. Since the return values of extreme precipitation events are regularly used in practice in the form of heavy rainfall hazard products, a reliable update of these products is required. Moreover, for resilient planning a projection of future conditions is urged by practice stakeholders.

A promising tool for projection are convection permitting climate simulations, which have been shown to better represent extreme precipitation events compared to coarser simulations and thus provide higher confidence in future extreme estimates. However, due to the large computation time of convection permitting simulations, evaluations are mostly based on single time slice experiments. Therefore, we explore the potential of an unique transient convection permitting (2.8 km) ensemble with COSMO-CLM regional simulations (1971-2100) over Germany, with four ensemble members driven by MPI-ESM-LR, EC-EARTH, CNRM-CM5, and HadGEM2-ES with the emission scenario RCP8.5. Extreme precipitation is derived over 30-year running time slices and the scales investigated span from hourly to 3-day event duration and return periods from 1 year to 100 years, representing the wide range of events considered for application.

Within the historical period (1971-2005) we found adequate agreement between the simulations and the observation data set KOSTRA with increasing bias with longer event duration. Furthermore, the climate change signal, derived as a relative value with regard to the historical period of the simulation, was found to increase with return period and for shorter durations. Strongest relative changes lie within the range of Clausius-Clapeyron-scaling with global warming. Analysis of the uncertainty revealed a substantial residual standard deviation of the linear approximation of the change signal over global warming, highlighting the benefit of a transient ensemble that enables a more robust estimation of the change signal of extreme events. Moreover, the results indicate an increased variance of future extreme precipitation.

How to cite: Hundhausen, M., Feldmann, H., Kohlhepp, R., and Pinto, J. G.: How does the assessment of extreme precipitation profit from convection permitting climate ensembles?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13843, https://doi.org/10.5194/egusphere-egu23-13843, 2023.

EGU23-13995 | Posters virtual | CL2.4

Climate change scenarios for IDF curves for mainland Portugal 

Cristina Andrade, Sandra Mourato, Rita Guimarães, and Claúdia Brandão

Rainwater drainage systems and other hydraulic infrastructure are scaled considering the intensity of precipitation and its probability of occurrence. The estimation of precipitation intensity through the analysis of the frequency of occurrence of extreme precipitation events is a key instrument for the dimensioning of hydraulic infrastructures and the associated risk of collapse. Sub- or over-estimated rainfall intensities can cause significant problems in various types of hydraulic infrastructures, including flood mitigation and support works due to flooding.

The aim of this study is to determine how climate change will influence extreme rainfall and, consequently, the future sizing of hydraulic systems, including rainwater drainage and hydraulic passages. Towards this aim, the Intensity-Duration-Frequency (IDF) curves were computed (durations between 24 and 72 hours), considering the historical period between 1950 and 2001, and for future precipitation projections (ensemble of biased-corrected Regional Climate Models, RCMs). The period 2041‒2070 under the RCP8.5 (Representative Concentration Pathways) and 2071‒2100 under the RCP4.5 and RCP8.5 emission scenarios were analyzed for 25 udometric stations studied in Brandão et al. (2001 and 2004) located in mainland Portugal.

Results show an increase in precipitation intensity, however, the differences between the projected IDF and those obtained with observed data (ERA5 dataset) for the 2, 5, 10, 20, 50, and 100 years return periods are not spatially uniform. The outcomes reveal North/South contrasts between the station’s IDFs, being also quite apparent in the influence of the orography.

Overall, this study is the first approach to the problem of extreme rainfall in a changing climate, due to the severe consequences of sudden floods and the resilience of territories and their hydraulic infrastructures to these extreme events. Therefore, planning of new policies and the dimensioning of new and existing infrastructures in the medium and long term is thus highly relevant.

Acknowledgment: This work was supported by National Funds by FCT - Portuguese Foundation for Science and Technology, under the project UIDB/04033/2020.

Keywords: Climate change, IDF curves, Hydraulic passages, Extreme precipitation, Drainage systems, Portugal.

How to cite: Andrade, C., Mourato, S., Guimarães, R., and Brandão, C.: Climate change scenarios for IDF curves for mainland Portugal, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13995, https://doi.org/10.5194/egusphere-egu23-13995, 2023.

EGU23-14134 | ECS | Posters on site | CL2.4

Impact of orography on sub-daily precipitation upper tail from convection-permitting climate model simulations: a multi-model ensemble perspective 

Nathalia Correa Sánchez, Eleonora Dallan, Francesco Marra, Giorgia Fosser, and Marco Borga

Understanding the impact of orography on the probability distribution of extreme precipitation at short (i.e., sub-daily) temporal scales, as well as on extreme-rainfall causative processes, is critical for managing risk from rainfall-triggered natural hazards in mountainous regions. High-resolution convection-permitting models (CPMs) are crucial for this type of analysis since they better represent convective processes key to short-duration extremes.

Here, we assess the ability of multi-model CPM ensemble CORDEX-FPS to represent the upper tail of sub-daily precipitation in a complex-orography region in the Eastern Italian Alps. In this area, different orographic impacts on sub-daily precipitation upper tail were reported at different event durations, and significant temporal trends in precipitation intensity were reported during the last few decades, making it a challenging and interesting test case for CPM simulations. An ensemble of six CPMs with a horizontal grid spacing of 2.2 km, driven by ERA-Interim reanalysis, are analysed and evaluated against 180 rain gauges. Since CPM simulations are too short (10 years) for analysing extremes using conventional methods, we use a non-asymptotic statistical approach (Simplified Metastatistical Extreme Value, SMEV), which was proven to provide reliable results even using short time records. We explore how the model spread vary with elevation and the ability of the multi-model mean to reproduce the distribution parameters and the extreme quantiles up to 100-year return period at different elevations.

How to cite: Correa Sánchez, N., Dallan, E., Marra, F., Fosser, G., and Borga, M.: Impact of orography on sub-daily precipitation upper tail from convection-permitting climate model simulations: a multi-model ensemble perspective, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14134, https://doi.org/10.5194/egusphere-egu23-14134, 2023.

Tropical-extratropical cloud bands are typical of the subtropical South American climate, occurring mainly during the rainy season and producing more than 60% of the seasonal precipitation. Thus, their correct representation in climate models is fundamental for the accuracy of simulated subtropical precipitation. Here, we investigate the occurrence of extreme precipitation during tropical-extratropical cloud band events, considering both observed and simulated events. We use outgoing longwave radiation (OLR) data from the National Oceanic and Atmospheric (NOAA) Climate Data Record (CDR) and precipitation from ERA5 reanalysis to identify the observed events. For simulated events, we use the UK Met Office Unified Model convective-permitting simulations considering two different configurations: a control run forced by a high-resolution global climate model (HadGEM3-GC3.1-n512) and a hindcast run forced by a reanalysis product (ERA-Interim) downscaled by an RCM. Both configurations have ten years of data at 4.5 km spatial resolution. The cloud bands are identified using an objective detection algorithm applied to OLR, as described by Zilli and Hart (2021). The convective-permitting simulations reproduce the location and seasonal cycle of observed cloud bands well. To select the extreme cloud band events, we choose the top 20% of events with (a) the most extensive land area with precipitation above a threshold; and (b) the largest average precipitation over the land areas with precipitation above a threshold. Cloud band events that fulfil both these extent and intensity criteria are considered extreme cloud band events. The precipitation threshold is defined as the precipitation rate with the largest fractional contribution to the cloud band's total precipitation over the land area. Extreme cloud band events are responsible for a significant fraction of the seasonal precipitation, with the largest precipitation rates occurring over subtropical latitudes. They occur throughout the cloud band season (NDJFM) but are more frequent during its onset (ND), particularly when considering only the transient ones (i.e., those events persisting less than three days). During persistent extreme cloud band events (i.e., those lasting for four or more days), the moisture anomalies are located mainly over Eastern Brazil and the adjacent tropical South Atlantic Ocean, with a similar but more intense than during all persistent events. On the other hand, transient extreme cloud band events are more dependent on the moisture from the western subtropical South Atlantic Ocean when compared to all transient events. The convective-permitting simulations adequately reproduce the ERA5 precipitation during the extreme cloud band events, despite biases in the intensity of the rain increasing the precipitation threshold values. Despite that, the convective-permitting simulations better represent the precipitation and extremes over subtropical latitudes, providing a valuable tool for improving the understanding and forecasting of cloud band-related extreme precipitation events. 

How to cite: Zilli, M. and Hart, N.: Extreme Precipitation during Tropical-Extratropical Cloud Bands over South America: comparing observations and Convective-Permitting Model simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15042, https://doi.org/10.5194/egusphere-egu23-15042, 2023.

EGU23-15059 | Orals | CL2.4

Evaluation of precipitation variability over the Sierra de Guadarrama 

Jesús Fidel González-Rouco, Emilio Greciano-Zamorano, Félix García-Pereira, Cristina Vegas-Cañas, Jorge Navarro-Montesinos, Elena García-Bustamante, Ernesto Rodríguez-Camino, and Esteban Rodríguez-Guisado

Heterogeneity in the occurrence, amount, and distribution of precipitation in mountainous areas is relevant for water resources and stresses the need for high-altitude observations and high-resolution modeling over complex terrain. However, the harsh weather conditions and the complex terrain associated with these environments hinder a continuous monitorization and pose challenges for regional climate models.

In this work, data from 37 stations located in the Sierra de Guadarrama and nearly lowlands, in Central Spain, and with altitudes ranging from 600 to 2200 m.a.s.l. have been studied. A few of the highest altitude sites belong to GuMNet facility (https://www.ucm.es/gumnet) and the rest to the Spanish Meteorological Agency (AEMET; https://www.aemet.es). These data have been compared to ERA5 reanalysis (https://confluence.ecmwf.int/display/CKB/ERA5) and to three different resolution (9, 3, and 1 km) outputs of a simulation of the regional climate model WRF (https://www.mmm.ucar.edu/WRF) during the period from 1990-2019. The comparison of the different data sources aims at characterizing the precipitation distribution over the area, assessing the goodness of ERA5, and the potential added value of the increasing resolution of WRF simulation in reproducing the observations.

Results show that the increase in WRF resolution from 9 to 3 km always produces a better representation of precipitation, whereas the step from 3 to 1 km shows a significant improvement at the highest altitudes, but an overestimation of precipitation at low plain areas. The lack of added value in the simulation at the highest resolution is discussed in relation to the parameterization of cumulus precipitation. Also, an altitudinal gradient of precipitation is observed and can be traced to large-scale precipitation.

How to cite: González-Rouco, J. F., Greciano-Zamorano, E., García-Pereira, F., Vegas-Cañas, C., Navarro-Montesinos, J., García-Bustamante, E., Rodríguez-Camino, E., and Rodríguez-Guisado, E.: Evaluation of precipitation variability over the Sierra de Guadarrama, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15059, https://doi.org/10.5194/egusphere-egu23-15059, 2023.

EGU23-16649 | ECS | Posters on site | CL2.4

Mountain climate: one of the multipronged challenges in Ethiopia’s Agriculture 

Emnet Negash, Bert Van Schaeybroeck, Piet Termonia, Michiel Van Ginderachter, Kwinten Van Weverberg, Maarten Podevyn, and Jan Nyssen

The Ethiopian highlands are home to more than 90% of the Ethiopian population and constitute for 90% of total area suitable for agriculture (Hurni et al., 2010). The livelihood of 66% of Ethiopia’s population depends on subsistence agriculture, mostly rainfed. Little rainfall variability can therefore cause massive economic loss for farmers reliant on rain-fed agriculture, making differences in wealth among farmers on different sides of the mountain. This study aims at understanding the sub daily distribution of summer rain over the Ethiopian highlands using the ALARO-0 regional climate model at convection-permitting resolution of 4 km. The dependence on factors such as leeward or windward conditions, and elevation are explored to categorize and relate the diurnal cycles of surface variables including precipitation, wind speed, humidity, and temperature. Rainfall occurrence in these mountains is mainly influenced by circulation patterns, orography, surface heating and convection, making its distribution very heterogeneous. Elevation is the most important determinant factor leading to increased average rainfall and rainfall per rainfall event towards higher elevations. Ethiopia’s summer rain exhibits a pronounced diurnal cycle with the highest rainfall occurring during the early afternoon hours (12:00–16:00) and the minimum occurring in the late night (04:00–11:00). Windward average rainfall and rainfall per rainfall event are on average 0.05mm h-1 and 0.08 mm hr-1 (respectively) larger than leeward events, except during peak hours when leeward events have 0.05 mm higher average rainfall and rainfall per rainfall event. In contrast to average rainfall events, extreme events in the afternoon are often followed by another peak rainfall event at night. Leeward wind speed features a weak diurnal variation as compared to the strong contrast between day and night for windward wind speed. The diurnal cycles of temperature and humidity start earlier in the morning and recede later than the cycles of wind speed and rainfall. Moreover, rainfall peaks occur earlier in the day at higher elevations, and at night in valleys and in Afar Triangle. The prevalence of windward over leeward event probability, the stark contrast in wind speed diurnal cycle between windward and leeward events, and the early peak hour of dewpoint and air temperature all point towards temperature-induced rather than wind-induced convection. Rainfall-temperature dependence, in other words Clausius-Clapeyron relationship, in the lowlands such as the Afar triangle is however at its lowest due to moisture deficit. These differences are very likely to determine hydrology and vegetation distribution, and farmers economy at large.

How to cite: Negash, E., Van Schaeybroeck, B., Termonia, P., Van Ginderachter, M., Van Weverberg, K., Podevyn, M., and Nyssen, J.: Mountain climate: one of the multipronged challenges in Ethiopia’s Agriculture, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16649, https://doi.org/10.5194/egusphere-egu23-16649, 2023.

EGU23-16986 | ECS | Posters virtual | CL2.4

The impact of climate change on fire danger over the contiguous United States 

Maria Klariza Madrazo, Huikyo Lee, Arezoo Khodayari, Weile Wang, Taejin Park, and Colin Raymond

Recent extreme heat events, especially those that have occurred in the Western United States (WUS), are fueling wildfires and funneling smoke at an unprecedented level, impacting air/water quality and leading to an increase in respiratory hospitalizations. Under greenhouse warming, extreme weather conditions that favor wildfire ignition are expected to occur more frequently over the contiguous United States (CONUS). Therefore, predicting wildfire danger under a changing climate is essential in managing future wildfires and protecting the welfare of people and the environment. In response to mitigating wildfire risks, the Canadian Fire Weather Index (FWI) was developed to provide a numeric rating representing the intensity of a spreading fire. In this work, we utilized fine-scale (0.25° x 0.25°) daily meteorological inputs from thirty-five general circulation models in NASA Earth Exchange Global Daily Downscaled Projections Coupled Model Intercomparison Project Phase 6 (NEX-GDDP-CMIP6) data to calculate the FWI. Using the daily maximum temperature, relative humidity, wind speed, and precipitation from NEX-GDDP-CMIP6, we calculated the FWI of historical and future simulations from the periods of 1950 to 2100 under different emission scenarios (Shared Socioeconomic Pathways 2-4.5 and 5-8.5). We have analyzed the FWI for the GISS-E2-1-G model, which indicates a 2-3% increase per decade in future fire danger under both emission-pathway-driven climate scenarios during the dry season in the Southwestern US. We have found that the FWI climatology in the Southwestern US during the Summer presents high to extreme fire danger (> 50) and higher FWI values in the future compared to historical observations. Moreover, we have explored the uncertainties across multiple models using NEX-GDDP-CMIP6 statistically downscaled data and found a significant spread of the FWI across the models for historical observations and future simulations. To correlate the link between the FWI and actual fire occurrence, we will calculate the FWI using reanalysis data (MERRA-2) and validate the FWI with actual fire occurrence data from Global Fire Emissions Database (GFED) with a special emphasis on the WUS. While supporting the US NCA and NASA’s Climate Adaptation Service Investigator (CASI), we will also try to contribute FWI to NASA’s FireSense, an initiative to bring an Earth systems approach to improving wildfire and wildland fire management.

How to cite: Madrazo, M. K., Lee, H., Khodayari, A., Wang, W., Park, T., and Raymond, C.: The impact of climate change on fire danger over the contiguous United States, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16986, https://doi.org/10.5194/egusphere-egu23-16986, 2023.

EGU23-428 | ECS | Posters on site | CL3.2.8

Is Argentina hotter? Understanding heatwaves temporal and spatial behavior using the ERA5-LAND dataset (1950-2022)  

Caterina Cimolai, Enric Aguilar, Benito Zaragozí, Jon Olano Pozo, and Anna Boqué Ciurana

Climate strongly impacts socio-ecologic systems. Increasing the intensity and frequency of heatwaves is one of its major consequences. Heatwaves are periods of consecutive days when temperatures are much hotter than normal. Cities are especially affected because their impact is usually aggravated by the Urban Heat Island (UHI), an intrinsic phenomenon that increases urban temperatures compared to surrounding rural areas. Extreme hot temperatures affect urban areas causing health problems, increasing energy requirements, and altering water supplies, among others.  

Heatwaves have been studied in Argentina but this has not been updated for the whole country recently. Due to these impacts on people’s well-being, infrastructure, and ecosystem functioning, this work proposes to study changes in spatial distribution and frequency of heatwaves in Argentina.  

We use the ERA5 LAND dataset and the HeatWaver R package to identify heatwaves over mainland Argentina. For the purpose of this study, we define heatwaves as periods where maximum and/or minimum temperatures are above the 90th percentile of the WMO standard reference period (1961-1990) during five or more consecutive days. We inspect the temporal and spatial extent of the phenome and monitor its changes over time. In agreement with global warming tendencies, heatwaves are more frequent, and a larger portion of the country has been under stress in recent years. We also inspect the heterogeneous impact over the territory and large cities.  

To understand the impact of heatwaves in cities, it is crucial to evaluate the risk, which is the conjunction of hazards, exposure and vulnerability. As a first step, this work studies heatwaves as hazards while those other aspects will be incorporated into future research. Our final objective is to reach an urban heatwave risk index, combining meteorological, environmental, urban, and social aspects. This indicator would liaise climate science with local and regional policies and offer information for adaptation and mitigation policies to face climate variability and change.  

Keywords: heatwaves, cities, climate change, Argentina. 

How to cite: Cimolai, C., Aguilar, E., Zaragozí, B., Olano Pozo, J., and Boqué Ciurana, A.: Is Argentina hotter? Understanding heatwaves temporal and spatial behavior using the ERA5-LAND dataset (1950-2022) , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-428, https://doi.org/10.5194/egusphere-egu23-428, 2023.

EGU23-862 | Posters on site | CL3.2.8

The hunter-gatherers of Abra del Toro rock shelter, northwestern Argentina, suffered the effects of the large 4.2 ka Cerro Blanco eruption 

Jose-Luis Fernandez-Turiel, Juan Pablo Carbonelli, and Carlos Belotti López de Medina

There is a dearth of information regarding prehistoric foraging societies from the intermontane longitudinal valleys of the South-Central Andes. Due to the intense anthropization of the landscape or the scarce research efforts on prehistoric populations of hunter-gatherers in the intermontane valleys of the Andes, occupation sites have been found on very few occasions. However, new perspectives in the Abra del Toro rock shelter in the Yocavil Valley (Catamarca province, Argentina) have opened up from recent and ongoing excavations. This rock shelter is the first archaeological case in which it is possible to analyze the relationship between a large-scale natural catastrophe and the prehistoric populations living in the Andean intermontane valleys of the southern Central Andes. This rock shelter's stratigraphy and archaeological remains contain the record of interactions between human communities and volcanism. The stratigraphic record of the rock shelter shows a 1-m-thick volcanic ash deposit formed by aeolian transport from primary outer ashfall deposits. Geomorphological and sedimentological context, texture, glass and mineral content, whole-rock chemical composition, and radiocarbon dating prove that the tephra was derived from the 4.2 ka BP eruption of the Cerro Blanco Volcanic Complex in southern Puna (NW Argentina). This volcanic eruption is the largest documented in the world in the last five thousand years and covered the surroundings of the archaeological site with an ash layer of approximately 1 meter thick. The stratigraphic sequence of the Abra del Toro rock shelter allows us to hypothesize that there were three main occupational moments: two hunter-gatherer moments, separated by the record of the large volcanic eruption, and a subsequent agro-pottery period (Carbonelli et al. 2022. J. Archaeol. Sci. Rep. 45, 103629). The rock shelter after the eruption remained in the memory of the hunter-gatherer groups. Good visibility, accessibility, and proximity to water were attributes of this space that made it possible for it to be re-occupied after the eruptive event. Our next objective is to reconstruct, using proxy analysis, how the paleoenvironment was in the intermontane valleys before and after the eruption. The evidence of this Mid-Holocene catastrophic volcanic event in the Abra del Toro rock shelter opens the possibility of knowing its impact on the contemporary hunter-gatherer community and drawing conclusions for similar future volcanic crises.

This work was supported by the National Scientific and Technical Research Council (Grant PIP 112-201301-00178), the University of Buenos Aires (Grant UBACyt 20020170100318BA) (University of Buenos Aires), the National Agency for the Promotion of Research, Technological Development and Innovation (Grant 2019-01229) and the QUECA Project (MINECO, Grant CGL2011-23307).

How to cite: Fernandez-Turiel, J.-L., Carbonelli, J. P., and Belotti López de Medina, C.: The hunter-gatherers of Abra del Toro rock shelter, northwestern Argentina, suffered the effects of the large 4.2 ka Cerro Blanco eruption, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-862, https://doi.org/10.5194/egusphere-egu23-862, 2023.

EGU23-1212 | Orals | CL3.2.8 | Highlight

Storylines of the impacts in the Netherlands of alternative realizations of the Western Europe July 2021 floods 

Bart Van Den Hurk, Karin de Bruijn, Kymo Slager, mark Hegnauer, and Guus Rongen

The 2021 summer flooding was an extremely rare event, driven by precipitation extremes that exceed Dutch design levels for flood protection in regions away from the main rivers and coastline. However, similar events in neighboring locations cannot be ruled out even in the near future. The implications of such extreme rainfall amounts will vary by region, subject to local topography, hydraulic flow patterns, water management, and societal exposure. We explore the geographic distribution of potential flood impacts induced by a similar event by constructing impact-oriented event storylines for different subregions in the Netherlands. The plausibility of the storylines is underlined by using physical evidence, proven impact-modelling concepts, and expert judgment successfully assessing the (sometimes unexpected) outcomes. The approach supports impact assessment for extraordinary events.

The presentation will illustrate the development of the storylines, and its uptake and interpretation by governing authorities responsible for water safety, civil protection and water management.

How to cite: Van Den Hurk, B., de Bruijn, K., Slager, K., Hegnauer, M., and Rongen, G.: Storylines of the impacts in the Netherlands of alternative realizations of the Western Europe July 2021 floods, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1212, https://doi.org/10.5194/egusphere-egu23-1212, 2023.

EGU23-2330 | ECS | Orals | CL3.2.8 | Highlight

Increasing chances of summer wildfires in the UK? 

Vikki Thompson, Dann Mitchell, Hannah Bloomfield, Nick Dunstone, and Gillian Kay

In the summer of 2022 unprecedented weather conditions in the UK lead to wildfires in many regions. Record breaking temperatures – above 40 °C for the first time - and prolonged dry conditions led to exceptional fire weather severity. On July 19th London Fire Brigade declared a major incident as firefighters battled several significant wildfires across the city. We investigate if climate change is enhancing summertime wildfire risk in the UK. 

We use reanalysis data from 1960 to the present day to analysis trends in the climatic indicators that influence the fire weather index. A large ensemble of initialised climate model simulations from the same time period are used to support the findings and identify as-yet-unrealised possible fire weather index situations in the UK. 

In the UK the term ‘wildfire’ is not limited to fires in wildland, but to any uncontrolled vegetation fire which requires action regarding suppression. Wildfires in the UK are considered a semi-natural hazard due to their close link with human activity. Though we investigate only meteorological influences, these are not the sole cause of wildfires – for example fuel availability plays a large role. 

Better understanding of the trends in the fire weather severity and chance of exceptional conditions for the UK will enable improved understanding of the risks. This information can feed into relevant policy and contingency planning, allowing society to become better prepared for the future as the planet continues to warm. 

How to cite: Thompson, V., Mitchell, D., Bloomfield, H., Dunstone, N., and Kay, G.: Increasing chances of summer wildfires in the UK?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2330, https://doi.org/10.5194/egusphere-egu23-2330, 2023.

EGU23-2376 | ECS | Orals | CL3.2.8

Advancing research on compound weather and climate events via large ensemble model simulations 

Emanuele Bevacqua, Laura Suarez-Gutierrez, Aglae Jezequel, Flavio Lehner, Mathieu Vrac, Pascal Yiou, Giuseppe Zappa, and Jakob Zscheischler

Societally relevant weather impacts typically result from compound events, which are rare combinations of weather and climate drivers. For example, compound hot-dry events frequently cause damage to human and natural systems, often exceeding separate impacts from heatwaves and droughts. Focussing on four event types arising from different combinations of climate variables across space and time, we illustrate that robust analyses of compound events – such as frequency and uncertainty analysis under present-day and future conditions, event attribution, and exploration of low-probability-high-impact events – require very large sample sizes. In particular, the required sample is much larger than that needed for routinely considered univariate extremes. We demonstrate how large ensemble simulations from multiple climate models are crucial for advancing our assessments of compound events and for constructing robust model projections. For example, among the case studies, we focus on compound hot-dry events and show that large ensemble model simulations allow for identifying plausible extremely dry climates that, if occurring in a warmer world, would be associated with high risk from compound hot-dry events. Overall, combining large ensemble simulations with an improved physical understanding of compound events will ultimately provide practitioners and stakeholders with the best available information on climate risks.

How to cite: Bevacqua, E., Suarez-Gutierrez, L., Jezequel, A., Lehner, F., Vrac, M., Yiou, P., Zappa, G., and Zscheischler, J.: Advancing research on compound weather and climate events via large ensemble model simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2376, https://doi.org/10.5194/egusphere-egu23-2376, 2023.

Historical extreme flooding events in Central European river catchments caused high socioeconomic impacts. Previous studies investigated single events in detail but did not focus on an analysis of the underlying extreme precipitation events in general as historical events are too rare for a robust assessment of their generic dynamical causes. This study attempts to fill this gap by analyzing a set of realistic daily 100-year large-scale precipitation events over five major European river catchments with the help of operational ensemble prediction data from the ECMWF. The dynamical conditions during such extreme events are investigated and compared to those of more moderate extreme events (20- to 50-year). 100-year precipitation events are generally associated with an upper-level cut-off low over Central Europe in combination with a surface cyclone southeast of the specific river catchment. The 24 hours before the event are decisive for the exact location of this surface cyclone, depending on the location and velocity of the upper-level low over Western Europe. The differences between 100-year and more moderate extreme events vary from catchment to catchment. Dynamical mechanisms such as an intensified upper-level cut-off low and surface cyclone are the main drivers distinguishing 100-year events in the Oder and Danube catchments, whereas thermodynamic mechanisms such as a higher moisture supply in the lower troposphere east of the specific river catchment are more relevant in the Elbe and Rhine catchments. For the Weser/Ems catchment, differences appear in both dynamical and thermodynamic mechanisms.

How to cite: Pfahl, S. and Ruff, F.: What distinguishes 100-year precipitation extremes over Central European river catchments from more moderate extreme events?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2390, https://doi.org/10.5194/egusphere-egu23-2390, 2023.

EGU23-3277 | ECS | Posters on site | CL3.2.8

Future socio-ecosystem productivity threatened by compound drought-heatwave events 

Jiabo Yin, Pierre Gentine, Louise Slater, Lei Gu, Yadu Pokhrel, and Shenglian Guo

Compound drought-heatwave (CDHW) events are one of the worst climatic stressors for global sustainable development. However, the physical mechanisms behind CDHW and their impacts on socio-ecosystem productivity remain poorly understood. Here, by combining satellite observations, field measurements and reanalysis, we show that terrestrial water storage and temperature are negatively coupled, likely driven by similar atmospheric conditions (e.g., water vapor deficit and energy demand). Using simulations from a large climate-hydrology model ensemble of 111 members, we demonstrate that the frequency of extreme CDHWs is projected to increase by ten-fold globally under the highest emissions scenario, along with a disproportionate negative impact on vegetation and socioeconomic productivity by the late 21st century. Limits on water availability are likely to play a more important role in constraining the terrestrial carbon sink than temperature extremes, and over 90% of the global population and GDP could be exposed to increasing CDHW risks in the future, with more severe impacts in poorer or rural areas. Our results provide crucial insights towards assessing and mitigating adverse effects of compound hazards on ecosystems and human well-being.

How to cite: Yin, J., Gentine, P., Slater, L., Gu, L., Pokhrel, Y., and Guo, S.: Future socio-ecosystem productivity threatened by compound drought-heatwave events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3277, https://doi.org/10.5194/egusphere-egu23-3277, 2023.

EGU23-3832 | ECS | Posters on site | CL3.2.8

Understanding the origins of climate anomalies during low-yield years in Australia’s largest breadbasket 

Hao Li, Jessica Keune, Qiqi Gou, Chiara Holgate, and Diego Miralles

Wheat yield in Australia is highly dependent on year-to-year climate variability. Prolonged droughts and anomalously high temperatures have been considered as causes of agricultural failures in recent years. However, the origins of these climate extremes and their impacts on yield remain under study. Here, we use a Lagrangian trajectory model driven by atmospheric reanalysis data to delineate the source regions of moisture and heat over Australia’s largest rainfed agricultural region. In particular, we focus on extreme crop failure years (1994, 2002, 2006) and analyze the impact of upwind droughts on heat and moisture imports into the region. Our results indicate that low-yield years are often associated with stable high-pressure systems that lead to a decreased import of moisture from the surrounding oceans. Within the breadbasket, however, this caused higher-than-usual surface sensible heating. Moreover, the analyzed low-yield years coincide with widespread droughts over the Australian continent. We find that upwind droughts can further influence moisture and heat imports to the region. During the initial phase of the Millennium Drought in 2002, crop failure over the breadbasket exceeded 50% and only around 9% of the precipitation over the region originated from (upwind) land — this constitutes a decrease of 5.0% compared to the climatological average. Simultaneously, the heat import from remote land regions increased from an average of 22.8% to 24.7% in 2002. While our findings suggest that upwind droughts played only a minor role for Australia's largest breadbasket due to the influence of oceanic contributions in the region, other agricultural areas that show a larger dependency on moisture and heat imports from the land would be more susceptible to upwind climate anomalies. 

How to cite: Li, H., Keune, J., Gou, Q., Holgate, C., and Miralles, D.: Understanding the origins of climate anomalies during low-yield years in Australia’s largest breadbasket, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3832, https://doi.org/10.5194/egusphere-egu23-3832, 2023.

The intensity and frequency of extreme storms have been increasing over time due to climate change, challenging sustainable stormwater management. This study examines the impacts of climate change on the precipitation patterns and extremes across the Cedar River Watershed in the Pacific Northwest under the Shared Socio-economic Scenario (SSP-585) obtained from CMIP6 models. Two global climate models (GCMs), namely MIROC6 and CMCC-ESM2, are considered in this study. Prior to generating future extreme storms for the selected GCMs and scenarios, the GCM simulated precipitation data was bias corrected relative to in-situ daily precipitation data. Precipitation data was bias corrected using three different statistical methods (please Named three method); among those Equidistant Quantile Mapping performed best. Bias corrected precipitation from the MIROC6 showed better performance compared to the CMCC-ESM2 in reproducing the observed precipitation statistics. Finally, the bias-corrected precipitation data from MIROC6 was used to develop non-stationary Intensity-Duration-Frequency curves (IDF) to identify the extreme storm events and their return periods. The results indicate that the storm intensities increase (ranging from 2.5% to 30%) over the future periods for all selected return periods, with relatively larger increase for higher return periods i.e., 50-year and 100-year storms. Further, we use the bias corrected precipitation projections and generate mean monthly perception maps of the Cedar River Watershed for the periods of 2020–2039 and 2040–2059.

 

How to cite: Salem, A. and Abduljaleel, Y.: Assessing the impact of climate change scenario for simulating nonstationary rainfall intensity and duration, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4309, https://doi.org/10.5194/egusphere-egu23-4309, 2023.

EGU23-4544 | Orals | CL3.2.8 | Highlight

Climate change contributes to the record-shattering 2022 Pakistan rainfall 

Yujia You and Mingfang Ting

From mid-June until the end of August 2022, a sequence of torrential rains and deluges pummeled Pakistan, displacing more than 30 million residents with a death toll of near 2000. The accumulated amount exceeds the centennial average of 126 mm by about 7 standard deviations (50 mm), reaching a value of 487 mm and breaking its record over a century. The extraordinary extremity underscores the urgency for understanding the physical drivers of the event and the relations with human-induced climate change.

Here, we find that distinctive from the historical floods which tend to occur over the relatively wet northern mountains, the 2022 rainfall took place over arid southern Pakistan. Unlike the floods over northern mountains which had closer associations with extratropical westerly troughs, the heavy downpours in 2022 were primarily initiated by the synoptic low-pressure systems (LPS). The longevity and intensity of LPS were sustained and enhanced by the cross-equatorial monsoon flow, which has trended upward since the 1970s and is at a historical high. In combination with the zonal inflow of moisture induced by La Niña, a corridor of heavy rainfall extending from the Bay of Bengal toward southern Pakistan formed.

The signal of greenhouse-gas-forced changes in the heavy rainfall over Pakistan and the cross-equatorial monsoon flow is detectable in climate models, confirming that the likelihood of such extreme events would increase under future warming.

How to cite: You, Y. and Ting, M.: Climate change contributes to the record-shattering 2022 Pakistan rainfall, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4544, https://doi.org/10.5194/egusphere-egu23-4544, 2023.

EGU23-4681 | Orals | CL3.2.8

Reduced moisture sources contributed to the 2017-2019 southeast Australian drought 

Andréa S. Taschetto, Milica Stojanovic, Chiara Holgate, Anita Drumond, Jason Evans, Luis Gimeno, and Raquel Nieto

The Murray Darling Basin, located in southeast Australia, is an agriculturally rich area, providing one-third of the country’ food supply. In 2017-2019 the region experienced one of its worst droughts since 1900. Rainfall in the Murray Darling Basin was consistently below average for three consecutive cool seasons, an unprecedented event on record. The drought set the extreme conditions that led later to the 2019-2020 Black Summer Bushfires. Previous studies suggest that the strong 2019 positive Indian Ocean Dipole intensified the conditions of the drought, however the state of the climate drivers cannot fully explain the onset and development of the Murray Darling Basin drought. In this study, we investigate processes other than remote climate drivers that may have triggered the drought. Using a Lagrangian model to backtrack moisture sources to southeast Australia, we show that local processes were crucial in explaining the onset and development of the drought. We identify the sources of moisture to the cool season precipitation over the Murray Darling Basin and show for the first time that the moisture supply from the Tasman Sea declined in 2017 and 2018. We further show that the expected moisture was instead transported northward by an anomalous anticyclonic circulation. Our results provide an explanation for the moisture and rainfall deficit that caused the 2017-19 drought. Understanding the processes that led to the 2017-2019 Murray Darling Basin drought is important for predicting and planning future multi-year droughts in Australia.

How to cite: Taschetto, A. S., Stojanovic, M., Holgate, C., Drumond, A., Evans, J., Gimeno, L., and Nieto, R.: Reduced moisture sources contributed to the 2017-2019 southeast Australian drought, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4681, https://doi.org/10.5194/egusphere-egu23-4681, 2023.

Under the context of global warming, climate and weather extremes (e.g., droughts, high temperature extremes) take a heavy toll on natural and human systems. It has been reported that the concurrence of droughts and hot extremes (CDHEs) in summer 2022 in the Northern Hemisphere (NH) have led to reduced water resources/crop yield and increased health risks. While assessments of droughts and heatwaves in summer 2022 have been noted, the assessment of these extremes from a compound event perspective is still limited. In this study, we analyzed the rarity of CDHEs in summer 2022 across the NH, detected anthropogenic influence on CDHEs area, and projected the likelihood under different warming levels based on observations from ERA5 and simulations from the Sixth Phase of the Coupled Model Intercomparison Project (CMIP6). Our results illustrate that severe CDHEs in summer 2022 across the NH mainly occur in central North America, Europe, and south China. Event attribution analysis shows that CDHEs area in summer 2022 in the NH would not have occurred without anthropogenic global warming. The CDHEs area like 2022 is projected to occur more likely, particularly under SSP585 in a 4°C warming world. This study provides useful insights for advancing our understanding of compound extremes during summer 2022 across the NH.

How to cite: Meng, Y. and Hao, Z.: Attribution and projection of the summer 2022 compound dry and hot extreme in the Northern Hemisphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4705, https://doi.org/10.5194/egusphere-egu23-4705, 2023.

EGU23-7134 | ECS | Posters on site | CL3.2.8

Developing storylines for unprecedented extreme events using ensemble boosting 

Luna Bloin-Wibe, Erich Fischer, and Reto Knutti

Recent extreme temperature and precipitation events such as the dry and heat events in summer 2022 in Europe and China, the New Year’s warm spell 2022/23 across Europe, the 2021 heavy rainfall extremes in northwestern Germany, Belgium and the Netherlands and the 2021 Pacific Northwest heatwave broke previous observed record levels by large margins. The probability of such unprecedented record-shattering extremes increases with the rapid rate of warming. Thus, there is a crucial need for analyzing the underlying processes leading to these events and quantifying potential intensities of events possible in the coming decades.

Here, we evaluate how ensemble boosting (Gessner et al. 2021 and Gessner et al. 2022) can help assess the tail of climate distributions and generate climate model-based storylines more resource-efficiently. In ensemble boosting the most extreme simulated events in an intermediate-size initial condition ensembles are re-initialized in targeted experiments in order to efficiently sample very extreme states of the model climatology. Here, we evaluate different ensemble design choices including lead time, ensemble size and potential iteration choices to most efficiently allocate computational resources to simulate events of very extreme intensity.

The resulting boosted events are analyzed through a storyline approach, thus helping to interpret the underlying mechanisms of each physically consistent unfolding extreme event and its consequences. The Pacific Northwest heatwave in June 2021 will be used as a starting point; but ensemble boosting and storylines can be powerful tools for understanding extremes beyond heat. We further discuss how ensemble boosting can also be applied to compound extremes and future climate scenarios.

How to cite: Bloin-Wibe, L., Fischer, E., and Knutti, R.: Developing storylines for unprecedented extreme events using ensemble boosting, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7134, https://doi.org/10.5194/egusphere-egu23-7134, 2023.

EGU23-7329 | ECS | Posters on site | CL3.2.8

Increases in Extreme Precipitation over the Northeast United States using High-resolution Climate Model Simulations 

Bor-Ting Jong, Thomas Delworth, and Hiroyuki Murakami

The Northeast United States (NEUS) has faced the most rapidly increasing occurrences of extreme precipitation within the US in the past few decades. Understanding the physics leading to long-term trends in regional extreme precipitation is essential to adaptation and mitigation planning. Simulating regional extreme precipitation, however, remains challenging, partially limited by climate models’ horizontal resolution. Our recent work shows that a model with 25 km horizontal resolution facilitates a much more realistic simulation of extreme precipitation than comparable models with 50 or 100 km resolution, including frequency, amplitude, and temporal variability, based on ensembles generated by GFDL (Geophysical Fluid Dynamics Laboratory) SPEAR (Seamless System for Prediction and EArth System Research) models. The 25-km GFDL-SPEAR ensemble also simulates the trend of NEUS extreme precipitation quantitatively consistent with observed trend over recent decades, as the observed trend is within the ensemble spread. We therefore leverage multiple ensembles and various simulations (with historical radiative forcing and projected forcing following the SSP2-4.5 and SSP5-8.5 scenarios) to detect and project the trend of extreme precipitation. The 10-ensemble member GFDL-SPEAR 25-km simulations project unprecedented rainfall events over the NEUS, driven by increasing anthropogenic radiative forcing and distinguishable from natural variability, by the mid-21st century. Furthermore, very extreme events (99.9th percentile events) may be six times more likely by 2100 than in the early 21st century.

 

We further conduct a process-oriented study, assessing the physical factors that have contributed to the increasing extreme precipitation over the NEUS. We categorize September to November extreme precipitation days based on daily cumulative precipitation over the NEUS into weather types, including atmospheric river (AR), tropical cyclone (TC), and others. In observations, the most precipitation days were AR days or/and TC days. The number of extreme precipitation days related to pure AR events (without any TC-related event in the vicinity) had increased slightly from 1959 to 2020. The greater contribution to the increasing extreme precipitation was caused by TC-related events, especially the influences from extratropical transitions. The extreme precipitation days related to extratropical transitions were 2.5 times more frequent for the 1990 to 2020 period compared to the 1959 to 1989 period. We apply the same analysis to the GFDL-SPEAR 25-km simulations. Similar to observations, the increasing extreme precipitation days were mainly caused by TC-related events, with a smaller influence from pure AR events. However, the increasing number of TC-related days was dominated by hurricane and tropical storm events, while the number of extratropical transitions near the NEUS changed very little from 1959 to 2020. These results are different from the observational results. Ongoing work focuses on the discrepancy between observations and SPEAR simulations. For example, we are assessing whether the prominent increasing extratropical transitions since the 1990s in observations were the results of limited sample size or caused by decadal variability.

How to cite: Jong, B.-T., Delworth, T., and Murakami, H.: Increases in Extreme Precipitation over the Northeast United States using High-resolution Climate Model Simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7329, https://doi.org/10.5194/egusphere-egu23-7329, 2023.

EGU23-9277 | Posters on site | CL3.2.8

Estimating compounding heat waves and rainfall extremes under projected climate change over the island of Sicily, Italy 

Armelle Remedio, Jeewanthi Sirisena, and Laurens Bouwer

According to the IPCC AR6 report, the frequency and intensity of high temperatures and precipitation extremes, such as heat waves, and extreme rainfall events that can lead to flash floods have increased in recent decades and are projected to keep increasing. These extreme events, which can occur in separate or as compound events can lead to droughts and flooding, causing severe economic and health impacts including loss of lives. Especially when such events occur shortly or directly in sequence, they can cause more severe impacts than in isolation. Understanding their compound behavior and timing in current and future climates can help to better estimate associated risks and require protection and adaptation planning.

In this study, the frequency and intensity of the compound events of heat waves and extreme precipitation over Sicily, Italy were analyzed and characterized for the present (1980-2010) and near future (2030-2050) periods. We used high resolution gridded datasets from observations (E-OBS) and from the EURO-CORDEX ensemble of regional climate change simulations. Heat waves were defined using a daily maximum temperature threshold persistent for at least three consecutive days while the extreme precipitation events were defined using the 95th percentile threshold of daily data. Results showed that the highest frequency of heat waves occured near the coastal regions of Sicily, while the extreme rainfalls were located in the west of Sicily.  We identified the areas where heat waves and extreme rainfall events have occurred in the past and we demonstrate how they are expected to change in the future, separately and as compound events. The results of this study will be used to develop a workflow for estimating climate risks in the region, which is part of the “risk workflow for CAScading and COmpounding hazards in COastal urban areas” (CASCO) project, and can be combined with other workflows on geophysical risks (earthquakes and tsunamis) to characterize overall natural hazard risks for the island of Sicily.

How to cite: Remedio, A., Sirisena, J., and Bouwer, L.: Estimating compounding heat waves and rainfall extremes under projected climate change over the island of Sicily, Italy, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9277, https://doi.org/10.5194/egusphere-egu23-9277, 2023.

EGU23-9290 | Orals | CL3.2.8 | Highlight

Quantifying windstorm risks by translating historical extreme events into the future 

Ed Hawkins, Philip Brohan, Samantha Burgess, Stephen Burt, Gilbert Compo, Suzanne Gray, Ivan Haigh, Hans Hersbach, Kiki Kuijjer, Oscar Martinez-Alvarado, Chesley McColl, Andrew Schurer, Laura Slivinski, and Joanne Williams

Extreme wind events are among the costliest natural disasters in Europe. Significant effort is dedicated to understanding the risk of such events, usually analysing observed storms in the modern era. However, it is likely that some historical windstorms were more extreme and/or followed different tracks from those in the modern era. Producing plausible reanalyses of such events would improve the quantification of current and future windstorm risks.

Billions of historical climatological observations remain unavailable to science as they exist only on paper, stored in numerous archives around the world. We demonstrate how the rescue of such paper observations has improved our understanding of an extreme windstorm that occurred in February 1903 and its significant impacts. By assimilating newly rescued atmospheric pressure observations into the 20th Century Reanalysis system, the storm is now credibly represented in an improved reanalysis of the event. In some locations this storm produced stronger winds than any event during the modern era. As a result, estimates of risk from severe storms, based on modern period data, may need to be revised. Simulations of the storm surge resulting from this storm show a large coastal surge of around 2.5m, comparing favourably with newly rescued tide gauge observations and increasing our confidence in the quality of the reconstruction.

In addition, we use novel reanalysis experiments to translate this windstorm into a warmer world to quantify how it might be different both in the present and in the future. We find that the same storm produces more intense rainfall and stronger winds in a warmer climate, providing a new approach to quantifying how extreme weather events will change as the world is warming.

How to cite: Hawkins, E., Brohan, P., Burgess, S., Burt, S., Compo, G., Gray, S., Haigh, I., Hersbach, H., Kuijjer, K., Martinez-Alvarado, O., McColl, C., Schurer, A., Slivinski, L., and Williams, J.: Quantifying windstorm risks by translating historical extreme events into the future, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9290, https://doi.org/10.5194/egusphere-egu23-9290, 2023.

EGU23-10709 | Orals | CL3.2.8

The Unprecedented Pacific Northwest Heatwave of June 2021: Causes and Impacts 

Rachel White, Sam Anderson, James F. Booth, Ginni Braich, Christina Draeger, Cuiyi Fei, Christopher D. G. Harley, Sarah B. Henderson, Matthias Jakob, Carie-Ann Lau, Lualawi Mareshet Admasu, Veeshan Narinesingh, Christopher Rodell, Eliott Roocroft, Kate R. Weinberger, and Greg West

In late June 2021 a heatwave of unprecedented magnitude impacted the Pacific Northwest (PNW) region of Canada and the United States. Many locations broke all-time maximum temperature records by more than 5°C, and the Canadian national temperature record was broken by 4.6°C, with the highest recorded temperature 49.6°C. Local records were broken by large margins, even when compared to local records broken during the infamous heatwaves in Europe 2003, and Russian in 2010. A region of high pressure that became stationary over the region (an atmospheric block) was the dominant cause of this heatwave; however, trajectory analysis finds that upstream diabatic heating played a key role in the magnitude of the temperature anomalies. Weather forecasts provided advanced notice of the event, while sub-seasonal forecasts showed an increased likelihood of a heat extreme with 10-20 day lead times, with an increased likelihood of a blocking event seen in forecasts initialized 3 weeks prior to the heatwave peak. The impacts of this event were catastrophic. We provide a summary of some of these impacts, including estimates of hundreds of attributable deaths across the PNW, mass-mortalities of marine life, reduced crop and fruit yields, river flooding from rapid snow and glacier melt, and a substantial increase in wildfires—the latter contributing to devastating landslides in the months following. These impacts provide examples we can learn from, and a vivid depiction of how climate change can be so devastating.

How to cite: White, R., Anderson, S., Booth, J. F., Braich, G., Draeger, C., Fei, C., Harley, C. D. G., Henderson, S. B., Jakob, M., Lau, C.-A., Mareshet Admasu, L., Narinesingh, V., Rodell, C., Roocroft, E., Weinberger, K. R., and West, G.: The Unprecedented Pacific Northwest Heatwave of June 2021: Causes and Impacts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10709, https://doi.org/10.5194/egusphere-egu23-10709, 2023.

EGU23-11435 | Posters on site | CL3.2.8 | Highlight

How to prepare for record-shattering hot events 

Lisette Klok, Timo Kelder, Elske van Vessem, and Laurens Severijn Hondema

The heat dome that Portland experienced in 2021 with temperatures up to 46 °C was unprecedented and unexpectedly severe, leading to the death of dozens of people. What if such an exceptional event were to occur somewhere else?  

The Netherlands seems to be sensitive to such 'record-shattering' hot events, but luckily has not yet experienced them. Here, we show how to qualitatively connect the increasing scientific understanding of plausible record-shattering hot events with potential impacts and necessary responses for the city of Amsterdam. The expected impacts and potential responses of record-shattering hot events are identified through expert judgement with professionals from various disciplines. 

We asked what could possibly happen in Amsterdam if the temperature rises to 45 degrees, in particular what kind of problems and bottlenecks are expected and what possible solutions are. The results of this exercise provided additional insights to heat plans based on lived experiences. As such, this case study may prove a useful example for governments and private sectors wishing to prepare for future exceptional heat waves.

How to cite: Klok, L., Kelder, T., van Vessem, E., and Hondema, L. S.: How to prepare for record-shattering hot events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11435, https://doi.org/10.5194/egusphere-egu23-11435, 2023.

EGU23-13309 | Orals | CL3.2.8

Variability in North Sea wind energy and the potential for prolonged winter wind drought 

Gillian Kay, Nick Dunstone, Anna Maidens, Adam Scaife, Doug Smith, Hazel Thornton, Laura Dawkins, and Stephen Belcher

The UK is committed to substantially increasing offshore wind capacity in its drive to decarbonise electricity production and achieve net zero. If low wind episodes – or “wind drought” events – occur during high energy demand periods, energy security may be threatened without alternative supply. To ensure resilience of the power system now and in the coming years as offshore wind generation grows, better understanding of the severity, frequency and duration of low wind episodes would be useful. Variability in winds is likely to dominate over trends in the next few decades, and hence having improved information on present day characteristics of wind drought is valuable.

Here we focus our attention on the North Sea as a centre of current and planned offshore wind resource for the UK and a number of other European countries, and on the winter season, given the occurrence of weather patterns that risk security of supply. We use a large ensemble of initialised climate model simulations to provide a synthetic but realistic event set that greatly increases the sample size of extreme events compared with that available from reanalysis data, and gives more robust information about their likelihood and properties. Using the basic unit of a week of low winds as the timescale of analysis, we report on the frequency and duration of wind drought events. In addition, we examine the wider conditions associated with wind drought events to investigate what remote factors may contribute to prolonged wind drought.

How to cite: Kay, G., Dunstone, N., Maidens, A., Scaife, A., Smith, D., Thornton, H., Dawkins, L., and Belcher, S.: Variability in North Sea wind energy and the potential for prolonged winter wind drought, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13309, https://doi.org/10.5194/egusphere-egu23-13309, 2023.

EGU23-14539 | ECS | Orals | CL3.2.8

Increasing probability of extreme records in heavy precipitation 

Iris de Vries, Sebastian Sippel, Erich Fischer, Joel Zeder, Vincent Humphrey, and Reto Knutti

It comes as no surprise that the future holds record-breaking weather and climate events. As global warming continues, temperature records will continue to be broken. Also heavy precipitation records are likely to be broken due to the increased water holding capacity of the atmosphere, in combination with changing atmospheric stability and circulation patterns. Improved estimates on the range of possible record-breaking precipitation events – now and in the future – are a first step to inform adequate adaptation policies for heavy precipitation. Of particular interest are events that break records by large margins – record-shattering events –, since these are likely to incur most damage and losses. 

In order to improve estimates of record shattering precipitation events in the present and future climate we use initial condition large ensemble simulation data (CESM2, SSP370) and statistical models. We evaluate record-shattering events in Rx1d (day with most precipitation per chosen time period (year or season)). In a stationary climate, the probability of Rx1d record-breaking is known to decrease with the number of data points since the start of measurements (inversely proportional). We find, however, that in our nonstationary climate, the decay in Rx1d record breaking and shattering probability is slowed down and even reversed in most world regions. Regional changes in record shattering probability are attributable to a changing underlying probability distribution of Rx1d, which also is region specific. We elucidate the contributions of changes in mean (distribution shift), and in variability (distribution widening/narrowing) to increasing record shattering probability by using a statistical model to create counterfactual realities representative of the regions of interest.

We focus on regions of a size relevant for national and cross-border policy that show differently driven changes in record shattering precipitation probabilities. For example, the annual probability of a record shattering precipitation event somewhere in the Benelux-Germany region which was hit by severe floods in summer 2021 increases from ~2% now to ~4.5% at the end of the century in CESM2. This increase results from a non-linear interaction between mean and variability increases, and is primarily driven by increasing variability. At lower latitudes, for example in Central America, the effect of variability is even stronger, where we find increasing record shattering probability despite a negative long-term trend in Rx1d levels.

Very unlikely events are, paradoxically, arguably the most important to know about, since their unimaginability often means that critical infrastructure is not sized to withstand these events. Our results may thus prove invaluable for regional policy. 

How to cite: de Vries, I., Sippel, S., Fischer, E., Zeder, J., Humphrey, V., and Knutti, R.: Increasing probability of extreme records in heavy precipitation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14539, https://doi.org/10.5194/egusphere-egu23-14539, 2023.

EGU23-14556 | ECS | Posters on site | CL3.2.8

A new Max Planck Institute-Grand Ensemble with CMIP6 forcing and high-frequency model output 

Dirk Olonscheck, Sebastian Brune, Laura Suarez-Gutierrez, Goratz Beobide-Arsuaga, Johanna Baehr, Friederike Fröb, Lara Hellmich, Tatiana Ilyina, Christopher Kadow, Daniel Krieger, Hongmei Li, Jochem Marotzke, Étienne Plésiat, Martin Schupfner, Fabian Wachsmann, Karl-Hermann Wieners, and Sebastian Milinski

We present the CMIP6 version of the Max Planck Institute-Grand Ensemble (MPI-GE CMIP6) with 30 realisations for the historical period and five emission scenarios. The power of MPI-GE CMIP6 goes beyond its predecessor ensemble MPI-GE by providing high-frequency model output, the full range of emission scenarios including the highly policy relevant scenarios SSP1-1.9 and SSP1-2.6, and the opportunity to compare the ensemble to high resolution simulations of the same model version. We demonstrate with six novel application examples how to use the power of MPI-GE CMIP6 to better quantify and understand present and future extreme events in the Earth system, to inform about uncertainty in approaching Paris Agreement global warming limits, and to combine large ensembles and artificial intelligence. For instance, MPI-GE CMIP6 allows us to show that the recently observed Siberian and Pacific North American heat waves are projected to occur every year in 2071-2100 in high-emission scenarios, that the storm activity in most tropical to mid-latitude oceans is projected to decrease, and that the ensemble is sufficiently large to be used for infilling surface temperature observations with artificial intelligence.

How to cite: Olonscheck, D., Brune, S., Suarez-Gutierrez, L., Beobide-Arsuaga, G., Baehr, J., Fröb, F., Hellmich, L., Ilyina, T., Kadow, C., Krieger, D., Li, H., Marotzke, J., Plésiat, É., Schupfner, M., Wachsmann, F., Wieners, K.-H., and Milinski, S.: A new Max Planck Institute-Grand Ensemble with CMIP6 forcing and high-frequency model output, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14556, https://doi.org/10.5194/egusphere-egu23-14556, 2023.

Managing extreme weather events of unprecedented magnitude is one of the main challenges facing climate risk management and climate adaptation. Because of the unprecedented nature of these events, some authors have questioned the use of probabilistic approaches in this context. As an alternative, they introduced the so-called climate storylines approach. Climate storylines do not aim at predicting system states; rather, their focus is on revealing plausible chains of events whose impact might undermine the performance of the system.

Conceptually, climate storylines relate to - but are separate from – downward counterfactual histories. Downward counterfactual histories are plausible alternative realizations of historical events that could have turned to the worse. By constructing downward counterfactual histories in a disaster risk reduction context, some authors showed that many disasters that took societies by surprise could have in fact been anticipated.

This talk will introduce a decision-support framework to build climate storylines based on downward counterfactual histories. The framework is event-oriented, it focuses on impact and it is designed to be applied in a participatory fashion. By following the framework, the user first constructs climate storylines based on an iterative analysis of what (combinations of) counterfactuals are deemed critical (i.e., downward). Then, the user analyzes the future impact of the constructed storylines under climatic and socio-economic scenarios. Finally, the user explores the effects on the estimated impacts of the value-laden choices involved in the construction of the storylines.

The framework is applied to study the impact of tropical cyclones hitting the European Union’s outermost regions on the stability of the European Union Solidarity Fund (EUSF), a public fund that provides financial relief to Member States affected by large disasters. Contrary to what historic evidence would suggest, it is found that extreme - yet plausible - tropical cyclones might deplete the EUSF capital if they happen concurrently with large events in mainland Europe, and that a substantial recapitalization of the fund might be required to cope with future climatic and socio-economic changes.

How to cite: Ciullo, A.: A decision-support framework to construct climate impact storylines using downward counterfactuals, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15450, https://doi.org/10.5194/egusphere-egu23-15450, 2023.

EGU23-16457 | Posters on site | CL3.2.8

Emulator-enhanced extreme event attribution for data scarce developing countries 

Fahad Saeed, Shruti Nath, Pierre Candela, Quentin Lejeune, Lukas Gudmundsson, Mathias Hauser, Dominik Schumacher, Sonia Seneviratne, and Carl Schleussner

Attribution of extreme events in developing countries poses a significant challenge. A primary hindrance is the lack of historical observations, which not only limits the appraisal of the extent of an extreme event, but also restricts benchmarking of climate models for the region. A secondary hindrance is that tropical climates, characteristic of developing countries, contain large uncertainties due to natural climate variability, which many climate models struggle to represent. As it is those countries and world regions where some of the most severe consequences of climate impacts emerge, addressing these challenges to robust climate attribution is critical to improve prospects of climate litigation in developing countries. In this study, we present a novel method for attribution using the Earth System Model (ESM) emulator for spatially resolved monthly temperatures, MESMER-M (Nath et al. 2022). We use a bootstrap method in calibrating MESMER-M, so as to also characterize its intrinsic parametric uncertainty. Attribution using MESMER-M is then demonstrated on the prolonged heat conditions of March/April 2022 over the Indo-Pakistani region. The outcomes of this study are twofold. Firstly, by calibrating MESMER-M on the BEST observational dataset, we are able to inflate observational records with observationally consistent natural climate variability estimates, enabling exploration of “possible pasts” and insofar characterization of the event and its likelihood under rising Global Mean Temperatures (GMTs). Secondly, by exploring the parametric uncertainty space of MESMER-M calibrated on both BEST and ESM data, we systematically disentangle the uncertainty surrounding the mean response of monthly temperatures to GMT from that surrounding the natural climate variability. Such allows robust appraisal of the uncertainty surrounding natural climate variability as present within ESMs/Observations for the region, so as to not over/understate the event’s likelihood under rising GMTs.

 

Nath, S., Lejeune, Q., Beusch, L., Seneviratne, S. I., & Schleussner, C. F. (2022) MESMER-M: an Earth system model emulator for spatially resolved monthly temperature. Earth System Dynamics, 13 (2), 851–877. doi: 10.5194/esd-13-851-2022

How to cite: Saeed, F., Nath, S., Candela, P., Lejeune, Q., Gudmundsson, L., Hauser, M., Schumacher, D., Seneviratne, S., and Schleussner, C.: Emulator-enhanced extreme event attribution for data scarce developing countries, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16457, https://doi.org/10.5194/egusphere-egu23-16457, 2023.

EGU23-17463 | ECS | Posters on site | CL3.2.8

Future Extreme Weather: a Data and AI driven approach to Understand Future Coastal Flooding 

Tudor Suciu, Emily Shuckburgh, and Nicholas Lane

Coastal flooding can be regarded as the most damaging extreme weather event. Careful
planning of mitigation and adaptation strategies requires a deep understanding of the event’s
likelihood and intensity.
This project provides a framework for assessing those changing statistics of coastal floods in
the future. We use historical records of coastal floods on the coasts of the UK historical
weather variables data (sea surface temperature, sea-level pressure, zonal and meridional
wind speeds and daily precipitations) from remote sensing sources, reanalysis data and
global climate models and future predictions of those weather variables from global climate
models. The method consists of using machine learning models to classify days as being
either ‘flooded’ (i.e. containing a coastal flood event) or ‘non-flooded’, at tide gauge
locations in the past 2 decades; both ‘out-of-the-box’ and more complex machine learning
models are trained on historical data. The models are then further used to assess the future
statistics of coastal flooding, by classifying days with or without flooding in the future
decades, from global climate models data. Currently, the method is showing promising
results on predicting the future number of ‘flooding days’, while the models used and trained
still show gradual improvement.
Using the same intensity scale as in the dataset of historical records of floods, it can be
assessed whether those events are becoming stronger or not. As well, the frequency, or the
return period, for the upcoming decades can be inferred from this project. This framework
produces an actionable set of information, that can be used by policy-makers, businesses,
governments and people, to plan accordingly for future floods.

How to cite: Suciu, T., Shuckburgh, E., and Lane, N.: Future Extreme Weather: a Data and AI driven approach to Understand Future Coastal Flooding, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17463, https://doi.org/10.5194/egusphere-egu23-17463, 2023.

EGU23-938 | ECS | Posters on site | AS1.37

The role of desert dust in the development of the Tropical Storm Rose 

Guillaume Feger, Thibaut Dauhut, and Jean-Pierre Chaboureau

Tropical storms, especially when they develop into hurricanes, are among the most destructive natural disasters. They are the subject of numerous studies, in particular to better understand their dynamics on meteorological scales in order to better predict them and reduce their impacts. We have been able to understand the role of African easterly waves in the formation of tropical storms in the Cape Verde region. However, the role of desert dust originating from the Sahara remains poorly understood due to their multiple and antagonistic effects in stabilizing the atmosphere by heating and reinvigorating convection through cloud icing as well as the lack of observation and limited simulation capabilities.

The CADDIWA (Clouds-Atmospheric Dynamics-Dust Interactions in West Africa) project aims to better understand the effects of desert dust on the atmospheric circulation off Senegal. The CADDIWA airborne campaign, took place from September 5 to 23, 2021 operating the SAFIRE Falcon 20 in the tropical environment of the Cape Verde Islands. During the campaign, the tropical storm Rose was observed on September 18 and 19, 2021. The goal of this PhD project is to exploit current very high resolution modeling capabilities combined with new observations to understand the dynamical and microphysical processes responsible for the development of Tropical Storm Rose. The first results of a large-eddy simulation of Tropical Storm Rose will be presented as well as its evaluation by comparison with available airborne and satellite observations.

How to cite: Feger, G., Dauhut, T., and Chaboureau, J.-P.: The role of desert dust in the development of the Tropical Storm Rose, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-938, https://doi.org/10.5194/egusphere-egu23-938, 2023.

EGU23-1087 | ECS | Posters on site | AS1.37

Development of Tropical Cyclones from African Easterly Waves : comparative study of three African Easterly Wave events during the CADDIWA campaign 

Tanguy Jonville, Cyrille Flamant, Christophe Lavaysse, Julien Delanoë, Pascal Richard, Sophie Bounissou, Quiterie Cazenave, Hélène Colomb, Christophe Caudoux, Philippe Peyrillé, and Erwan Cornillault

During the CADDIWA (Cloud-Atmospheric Dynamics-Dust Interaction in West Africa) airborne campaign that took place in September 2021, three tropical disturbances initiated from African Easterly Waves were sampled. Two of them reached the Tropical Storm state and were named Rose and Peter by the National Hurricane Center. The last one, later named Pierre-Henri, failed to develop. After a validation of reanalysis data for september 2021 against the data collected during the campaign, a comparative study of the three events will be conducted using ERA5, satellite and campaign data, with a focus on energy budgets. Several processes that may be catalysts or inhibiters for tropical cyclogenesis (AEW-Monsoon -, AEW-AEW -, dust-dynamics interaction ...) will especially be discussed. 

How to cite: Jonville, T., Flamant, C., Lavaysse, C., Delanoë, J., Richard, P., Bounissou, S., Cazenave, Q., Colomb, H., Caudoux, C., Peyrillé, P., and Cornillault, E.: Development of Tropical Cyclones from African Easterly Waves : comparative study of three African Easterly Wave events during the CADDIWA campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1087, https://doi.org/10.5194/egusphere-egu23-1087, 2023.

As support to the operational field campaign of the CADDIWA field experiment, the coupled regional model WRF-CHIMERE in forecast mode during the summer 2021. The simulation domain covers West Africa and the East Atlantic and allows the modeling of dust emissions and their transport to the Atlantic. On this route, we find Cape Verde which was used as a base for measurements during the CADDIWA campaign. The forecast consists of meteorological variables and mineral dust concentrations on a horizontal grid with a resolution of 30 km and from the surface to 200 hPa. Each day, the simulation starts the day before (D-1) and up to 4 days ahead (D+4). For each day, we thus have 6 different calculations, with logically a better precision the closer we get to the analysis (D-1). This presentation will show a quantification of the variability of the forecast of mineral dust according to the modelled lead. This quantification will also be done according to the interactions between clouds, aerosols and radiation.

How to cite: Menut, L.: Meteorology and mineral dust forecast variability during the CADDIWA campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1162, https://doi.org/10.5194/egusphere-egu23-1162, 2023.

EGU23-1355 | Orals | AS1.37

Validation of the Aeolus wind observations in the tropics using the ALADIN Airborne Demonstrator and 2-µm Doppler wind lidar 

Oliver Lux, Benjamin Witschas, Christian Lemmerz, Fabian Weiler, Uwe Marksteiner, Stephan Rahm, Alexander Geiß, Andreas Schäfler, Michael Rennie, and Oliver Reitebuch

The German Aerospace Center (Deutsches Zentrum für Luft- und Raumfahrt, DLR) conducted four airborne campaigns for the validation of the Aeolus L2B wind product during the first three years of ESA’s wind lidar mission between 2018 and 2021. After three campaigns in Europe, the Aeolus VAlidation Through Airborne LidaRs in the Tropics (AVATAR-T) campaign was performed around the Cabo Verde archipelago in September 2021 as part of the Joint Aeolus Tropical Atlantic Campaign (JATAC). AVATAR-T employed the DLR Falcon aircraft which carried two Doppler wind lidar (DWL) instruments: the heterodyne-detection 2-µm DWL acting as a high-accuracy reference and the ALADIN Airborne Demonstrator (A2D), representing a prototype of the direct-detection DWL on-board Aeolus with a high degree of commonality in terms of design and measurement principle.

In the framework of AVATAR-T, 11 coordinated flights along the Aeolus track were performed covering nearly 11,000 km of the satellite's measurement swath. The research flights yielded a comprehensive set of A2D and 2-µm DWL wind observations to validate the Aeolus wind product under the influence of the Saharan Air Layer (SAL), the African Easterly Jet, the Subtropical Jet and the Intertropical Convergence Zone. In particular, the campaign results give insight into the impact of atmospheric aerosols onto the operational Rayleigh-clear and Mie-cloudy horizontal line-of-sight (HLOS) winds regarding potential errors that arise from crosstalk between the two complementary receiver channels and their respective wind data coverage in the troposphere.

Validation of the Aeolus wind product based on 2-µm DWL data shows that the systematic error almost fulfills the mission requirement of being below 0.7 m/s (HLOS) for both Rayleigh-clear and Mie-cloudy winds. The random error, however, is larger than specified (2.5 m/s HLOS), being close to 3 m/s for Mie-cloudy winds and as high as 7 m/s for Rayleigh-clear winds. A more detailed investigation reveals that the Rayleigh-clear random error is increased at lower altitudes in case of signal extinction due to aerosols.

The collocated A2D wind observations provide valuable information on the potential optimization of the Aeolus wind retrieval and related quality control (QC) algorithms. For instance, the A2D, unlike ALADIN, delivered a broad vertical and horizontal coverage of Mie winds across the SAL, whereas A2D Rayleigh winds measured in this region, which are affected by Mie contamination through crosstalk and signal extinction, are effectively filtered out. Preliminary studies suggest that a refinement of the Aeolus wind retrieval may improve the Mie wind data coverage in aerosol regions.

In addition, we studied the influence of different QC schemes on the validation results and developed a two-step QC approach that ensures effective outlier removal and compliance with the Aeolus mission requirements document. The QC scheme also improves the comparability of different validation studies and thus helps to facilitate the consolidation of the Aeolus error evaluation from different Cal/Val teams.

The contribution presents comparative wind observations of Aeolus and the two DLR airborne wind lidar instruments from the JATAC with a focus on the error assessment and a potential improvement of the Aeolus wind data product.

How to cite: Lux, O., Witschas, B., Lemmerz, C., Weiler, F., Marksteiner, U., Rahm, S., Geiß, A., Schäfler, A., Rennie, M., and Reitebuch, O.: Validation of the Aeolus wind observations in the tropics using the ALADIN Airborne Demonstrator and 2-µm Doppler wind lidar, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1355, https://doi.org/10.5194/egusphere-egu23-1355, 2023.

EGU23-3398 | ECS | Posters on site | AS1.37

Lidar measurements of volcanic aerosol over Mindelo during the volcanic eruption at Las Palmas in autumn 2021 

Henriette Gebauer, Holger Baars, Athena Augusta Floutsi, Albert Ansmann, Kevin Ohneiser, and Cordula Zenk

From 19 September to 13 December 2021, a volcanic eruption took place at Las Palmas, Canary Islands. Thereby, fine ash and volatiles, like SO2, were emitted and transported over hundreds to thousand kilometers away from the island [1]. At the same time, continuous lidar observations with the multiwavelength-Raman-polarization lidar PollyXT were performed at the Ocean Science Center Mindelo (16.878°N, 24.995°W), Cabo Verde, in the frame of the JATAC-campaign 2021/2022. During autumn, typical aerosol conditions over Mindelo, as detected by the lidar, are a clean marine boundary layer up to approx. 1 km and a Saharan dust layer (up to 6 km) above. In the boundary layer, an extinction coefficient of less than 200 Mm-1 and a lidar ratio smaller than 40 sr is typically observed while a lidar ratio between 40 and 60 sr and a depolarization ratio between 20 and 30 % is typically found for the Saharan dust properties. Instead, during the time of the volcanic eruption, a strongly polluted planetary boundary layer (PBL) was observed beginning 23 of September, whereby the extinction coefficient and the lidar ratio increased up to 800 Mm-1 and 60 to 80 sr, respectively. On specific days, the aerosol optical depth, determined by an AERONET sun photometer, was as high as 1.0 (at 500 nm). Due to the small depolarization ratio around 0 % in the PBL and Hysplit trajectories indicating air masses coming from Canary Islands, the observed pollution over Mindelo can be attributed to sulfates emitted by the volcanic eruption at Las Palmas. No indications for volcanic ash over Mindelo were found, neither in the PBL nor in the lofted layer (mainly Saharan dust). This is furthermore supported by Hysplit trajectories, which show that air masses in higher altitudes come from the African continent and not from the Canary Islands. The potential of Aeolus to capture the volcanic plume on its way to Cabo Verde will also be assessed using the aerosol spin-off products (L2A) of the most recently available baseline.

 

References

[1] Carracedo, J. C., Troll, V. R., Day, J. M., Geiger, H., Aulinas, M., Soler, V., ... & Albert, H. (2022). The 2021 eruption of the Cumbre Vieja Volcanic Ridge on La Palma, Canary Islands. Geology Today, 38(3), 94-107.

How to cite: Gebauer, H., Baars, H., Floutsi, A. A., Ansmann, A., Ohneiser, K., and Zenk, C.: Lidar measurements of volcanic aerosol over Mindelo during the volcanic eruption at Las Palmas in autumn 2021, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3398, https://doi.org/10.5194/egusphere-egu23-3398, 2023.

EGU23-3490 | Orals | AS1.37 | Highlight

Aeolus: ESA’s wind mission. Status and future challenges 

Tommaso Parrinello, Denny Wernham, Thorsten Fehr, Jonas Von Bismarck, Viet Duc Tran, Massimo Romanazzo, Trismono Candra Krisna, Aditi Sathe, Peter Bickerton, Isabell Krisch, and Michael Rennie

The European Space Agency (ESA)’s wind mission, Aeolus, was launched on 22 August 2018. It is a member of the ESA Earth Explorer family and its main objective is to demonstrate the potential of Doppler wind Lidars in space for improving weather forecast and to understand the role of atmospheric dynamics in climate variability. Aeolus carries a single instrument called ALADIN: a high sophisticated spectral resolution Doppler wind Lidar which operates at 355 which is the first of its kind to be flown in space.

Aeolus provides profiles of single horizontal line-of-sight winds (primary product) in near-real-time (NRT), and profiles of atmospheric backscatter and extinction. The instrument samples the atmosphere from about 30 km down to the Earth’s surface, or down to optically thick clouds. The required precision of the wind observations is 1-2.5 m/s in the troposphere and 3-5 m/s in the stratosphere while the systematic error requirement be less than 0.7 m/s. The mission spin-off product includes information about aerosol and cloud layers. The satellite flies in a polar dusk/dawn orbit (6 am/pm local time), providing ~16 orbits per 24 hours with an orbit repeat cycle of 7 days. Global scientific payload data acquisition is guaranteed with the combined usage of Svalbard and Troll X-band receiving stations.

After almost five years in orbit and despite some performance issues related to its instrument ALADIN, Aeolus has achieved all its scientific objectives and gone beyond its original designed life-time in space. Positive impact on the weather forecast has been demonstrated by multiple NWP centres world-wide, with four European meteorological centres now are assimilating Aeolus winds operationally, paving the way to its successor: EPS-Aeolus. Aeolus data is being used with success over a number of innovative research streams with growing scientific impact on literature.

The status of the Aeolus mission will be presented including the last main challenge to re-enter the satellite from space with an assisted scenario instead of an uncontrolled one, as initially foreseen by design.

How to cite: Parrinello, T., Wernham, D., Fehr, T., Von Bismarck, J., Tran, V. D., Romanazzo, M., Candra Krisna, T., Sathe, A., Bickerton, P., Krisch, I., and Rennie, M.: Aeolus: ESA’s wind mission. Status and future challenges, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3490, https://doi.org/10.5194/egusphere-egu23-3490, 2023.

EGU23-4556 | Posters on site | AS1.37

Weather regime characterisation of the atmospheric environment leading to the development of tropical cyclones in the Northern Tropical Atlantic 

Marco Gaetani, Cyrille Flamant, Tanguy Jonville, Jean-Pierre Chaboureau, Christophe Lavaysse, Juan Cuesta, Laurent Menut, Natalia Castillo, and Formenti Formenti

At the end of the monsoonal season in West Africa, tropical cyclones (TCs) start to develop in the Northern Tropical Atlantic off shore Senegal, south of Cape Verde. TCs generally develop from low pressure disturbances travelling westward from West Africa embedded in the African easterly waves (AEWs), characterised by organised convection and high specific humidity. Some of these TCs eventually evolve into tropical storms and hurricanes. However, whereas there is overall agreement concerning the main necessary conditions, involving sea surface temperature (SST) and vertical wind shear, for a TC to evolve into a tropical storm or a hurricane, the elements concurring to the formation of TCs from easterly depressions are still unclear. Indeed, the environment where the transition occurs is characterised by complex interactions involving atmospheric dynamics and aerosol-cloud-radiation interactions not fully understood yet.

The purpose of this study is to contribute to enlighten the mechanisms leading an easterly African depression to evolve (or not) into a TC in the Northern Tropical Atlantic, by characterising the atmospheric environment off shore Senegal and south of Cape Verde, where TCs start to develop. To this aim, a weather regime (WR) classification of the atmospheric variability is first performed on a climatological time scale in a region including West Africa and Northern Tropical Atlantic. The WR classification is then used to characterise the relevant atmospheric variables involved in the TC development. In particular, the role of major outbreaks of mineral aerosols from the adjacent Sahara Desert is investigated. Data from ERA5 and CAMS reanalysis products are analysed for the period 1991-2020.

How to cite: Gaetani, M., Flamant, C., Jonville, T., Chaboureau, J.-P., Lavaysse, C., Cuesta, J., Menut, L., Castillo, N., and Formenti, F.: Weather regime characterisation of the atmospheric environment leading to the development of tropical cyclones in the Northern Tropical Atlantic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4556, https://doi.org/10.5194/egusphere-egu23-4556, 2023.

EGU23-5067 | Orals | AS1.37

Convective Processes Experiment – Aerosol and Winds (CPEX-AW): Virtual and Field Campaigns 

Shuyi Chen, Edoardo Mazza, Ajda Savarin, Brandon Kerns, Ed Zipser, Svetla Hristova-Veleva, Ousmane Sy, Simone Tanelli, Hu Su, Michael Kavaya, Amin Nehrir, Zhaoxia Pu, and Gail Skofronick-Jackson

Tropical convection is a key player in the global weather and climate. Observing and predicting convective initiation, growth, dissipation, and interactions with the environment over the tropical ocean remain a grand challenge. The science objectives of CPEX-AW are: 1) better understanding interactions of convective cloud systems and tropospheric winds as part of the joint NASA-ESA Aeolus Cal/Val - Joint Aeolus Tropical Atlantic Campaign (JATAC), 2) observing the vertical structure and variability of the marine boundary layer in relation to initiation and lifecycle of the convective cloud systems, convective processes (e.g., cold pools), and environmental conditions within and across the ITCZ, 3) investigating how the African easterly waves and dry air and dust associated with Sahara Air Layer control the convectively suppressed and active periods of the ITCZ, and 4) investigating interactions of wind, aerosol, clouds, and precipitation and effects on long range dust transport and air quality over the western Atlantic. The CPEX-AW science team and the NASA DC-8 aircraft were deployed to St. Croix, the US Virgin Islands, from 18 August–10 September 2021, to address the science objectives. DC-8 is equipped with the Doppler Aerosol Wind Lidar (DAWN), Airborne Precipitation and Cloud Radar 3rd Generation (APR-3), High Altitude Lidar Observatory (HALO) Water Vapor DIAL and HSRL, High Altitude Microwave Sounding Radiometer (HAMSR), and GPS dropsondes. This article provides a summary of CPEX-AW scientific discoveries with highlights from some key aspects: a unique virtual campaign during the COVID pandemic and outstanding airborne observations from the field campaign.

  • More than 120 researchers including graduate students and postdocs participated in CPEX-AW in St. Croix, Puerto Rico, and remotely.
  • We have flown seven research missions that collected unprecedented data from DAWN, HALO, APR-3, HAMSR, and dropsondes, in a wide arrange of conditions from strong dust outbreak events to tropical storms.
  • Underflown six Aeolus overpasses for a total of 5,836 km, which provide valuable data sets for Aeolus Cal/Val and studies of impact on weather forecasting.
  • Complex wind and convection in pre-Tropical Storm (TS) Ida and Ida over the Gulf of Mexico before the major Hurricane Ida made landfall, long lasting TS Kate and its interaction with dust and dry air over the central Atlantic, and dry air intrusion in Hurricane Larry.
  • Co-located boundary layer observations over saildrones that measure air-sea fluxes and ocean current data in collaboration with the NOAA field campaign.

How to cite: Chen, S., Mazza, E., Savarin, A., Kerns, B., Zipser, E., Hristova-Veleva, S., Sy, O., Tanelli, S., Su, H., Kavaya, M., Nehrir, A., Pu, Z., and Skofronick-Jackson, G.: Convective Processes Experiment – Aerosol and Winds (CPEX-AW): Virtual and Field Campaigns, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5067, https://doi.org/10.5194/egusphere-egu23-5067, 2023.

EGU23-5631 | Orals | AS1.37

Quality assessment of Aeolus L2A products at Cabo Verde during JATAC and beyond - validation with ground-based lidar observations 

Holger Baars, Henriette Gebauer, Athina Floutsi, Dimitri Trapon, Sebastian Bley, Dietrich Althausen, Ronny Engelmann, Annett Skupin, Martin Radenz, Albert Ansmann, Andi Klamt, Birgit Heese, Ulla Wandinger, Eder Silva, Elizandro Rodrigues, Pericles Silva, Cordula Zenk, Peristera Paschou, and Eleni Marinou

In the framework of the Joint Aeolus Tropical Atlantic Campaign (JATAC), a temporary ground-based ACTRIS aerosol remote sensing station has been setup by TROPOS at the Ocean Science Center Mindelo (OSCM) in June 2021. The instrumental capabilities for aerosol profiling at the OSCM comprise a multiwavelength-Raman-polarization lidar Polly XT and an AERONET sun photometer. Furthermore, a scanning HALO photonics Doppler lidar is utilized to study the dynamics near the observational site. Continuous 24/7 observations have been performed since June 2021, thus covering the four intensive observational periods of JATAC (July 2021, September 2021, June 2022, September 2022).

In this presentation, we want to discuss the capabilities of Aeolus to observe the aerosol conditions including the Saharan dust layer (SAL) above the Cabo Verdean islands. The time series of the ground-based PollyXT lidar from June 2021 until today has shown, that dust is omnipresent above the local boundary layer in the summer months. The maximum dust layer top height has been observed in July with 7 km. The SAL top height has then decreased to 3 km in November. Some rainy periods were observed in September/October, especially in the year 2022 for the fourth intensive JATAC campaign.

We will utilize the direct Aeolus overpasses over Mindelo each Friday during these four periods (and for other seasons) to make a long(er)-term assessment of the Aeolus aerosol capabilities (L2A) involving also products from the most recent algorithm versions (Baselines).  Due to the capabilities of the ground-based PollyXT lidar, we can directly compare the 2 main products of Aeolus: The extinction coefficient and the co-polar backscatter coefficient. Doing so, we can also quantify the influence of the missing polarization component in the Aeolus aerosol products which is important for the planning of the potential Aeolus follow-on mission, for which the polarization capabilities are still under discussion.

Finally, the lessons learnt from the current Aeolus Cal/Val on Cabo Verde can be also used for the upcoming EarthCARE mission as TROPOS has started to setup a permanent ACTRIS aerosol and cloud remote sensing supersite at Mindelo.

How to cite: Baars, H., Gebauer, H., Floutsi, A., Trapon, D., Bley, S., Althausen, D., Engelmann, R., Skupin, A., Radenz, M., Ansmann, A., Klamt, A., Heese, B., Wandinger, U., Silva, E., Rodrigues, E., Silva, P., Zenk, C., Paschou, P., and Marinou, E.: Quality assessment of Aeolus L2A products at Cabo Verde during JATAC and beyond - validation with ground-based lidar observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5631, https://doi.org/10.5194/egusphere-egu23-5631, 2023.

EGU23-7249 | Posters on site | AS1.37 | Highlight

The Joint Aeolus Tropical Atlantic Campaign 2021/2022 Overview– Atmospheric Science and Satellite Validation in the Tropics 

Thorsten Fehr, Will McCarthy, Vassilis Amiridis, Holger Baars, Jonas von Bismarck, Maurus Borne, Shuyi Chen, Cyrille Flamant, Franco Marenco, Peter Knipperz, Rob Koopman, Christian Lemmerz Lemmerz, Eleni Marinou, Griša Močnik, Tommaso Parrinello, Aaron Piña, Oliver Reitebuch, Gail Skofronick-Jackson, Jonathan Zawislak, and Cordula Zenk

ESA’s Aeolus satellite observations are expected to have the biggest impact for the improvement of numerical weather prediction in the Tropics. An important case relating to the predictability of tropical weather systems is the outflow of Saharan dust, its interaction with cloud microphysics and impact on the development of tropical storms over the Atlantic Ocean.

The Joint Aeolus Tropical Atlantic Campaign (JATAC) deployed on Cabo Verde (2021/2022) and the US Virgin Islands (2021) supported the validation and preparation of the ESA missions Aeolus, EarthCARE and WIVERN, and addressed science objectives regarding the Saharan Aerosol layer, African Easterly Waves and Jet, Tropical Easterly Jet, and the Intertropical Convergence Zone, as well as their relation to the formation of convective systems, and the long-range transport of dust and its impact on air quality.

JATAC started in July 2021 with the deployment of ground-based instruments in the frame of the ASKOS project at the Ocean Science Center Mindelo, including the eVe and PollyXT lidars, and a W-band Doppler cloud radar. By mid-August, the CPEX-AW campaign started operations from the US Virgin Islands with NASA’s DC-8 flying laboratory in the Western Tropical Atlantic and Caribbean carrying the Doppler Aerosol Wind Lidar (DAWN), Airborne Precipitation and Cloud Radar (APR-3), Water Vapor DIAL and HSRL (HALO), microwave sounder (HAMSR) and dropsondes. In September the DLR Falcon-20 aircraft, carrying the ALADIN Airborne Demonstrator (A2D) and the 2-µm Doppler wind lidar, and the Safire Falcon-20, carrying the high-spectral-resolution Doppler lidar (LNG), the RASTA Doppler cloud radar, in-situ cloud and aerosol instruments, and dropsondes, were deployed to Sal in the frame of the AVATAR-T and CADDIWA projects. The Aerovizija Advantic WT-10 light aircraft with optical particle spectrometers, filter-photometers and nephelometers for in-situ aerosol characterisation was operating in close coordination with the ground-based observations in the CAVA-AW project.

The activities continued in June 2022 when the ASKOS ground based observations were enhanced with UAV airborne in-situ aerosol measurements deployed by the Cyprus Institute, solar radiation measurements supported by PMOD/WRC, dust particle orientation measurements (WALL-E lidar), and radiosonde releases equipped with electric field-mills. NASA deployed the DC-8 aircraft all September to Sal with the 2021 payload in the framework of the CPEX-CV activity, including regular radiosonde launches. As in 2021, the Aerovizija aircraft took part with in-situ aerosol measurements during two weeks in September. JATAC was supported by dedicated numerical weather and dust simulations supporting forecasting efforts and addressing open science questions.

Around 60 scientific flights of four aircraft, with an additional 25 UAV flights, were performed during JATAC. 23 Aeolus orbits were underflown, many of them with simultaneous observations of multiple aircraft collocated with ground-based observations. In addition, the science objectives were fully covered through the large number of flights, ground based cloud and aerosol observations, regular radiosondes and dropsondes.

Overall, JATAC activities have resulted in a high-quality and comprehensive dataset supporting a wide range of tropical atmospheric research, the validation of Aeolus and other satellites, and have provided key reference data for the development future Earth Observation missions.

How to cite: Fehr, T., McCarthy, W., Amiridis, V., Baars, H., von Bismarck, J., Borne, M., Chen, S., Flamant, C., Marenco, F., Knipperz, P., Koopman, R., Lemmerz, C. L., Marinou, E., Močnik, G., Parrinello, T., Piña, A., Reitebuch, O., Skofronick-Jackson, G., Zawislak, J., and Zenk, C.: The Joint Aeolus Tropical Atlantic Campaign 2021/2022 Overview– Atmospheric Science and Satellite Validation in the Tropics, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7249, https://doi.org/10.5194/egusphere-egu23-7249, 2023.

EGU23-8956 | Posters on site | AS1.37 | Highlight

Overview of NASA’s Convective Processes Experiment – Cabo Verde (CPEX-CV) in the East Atlantic in September 2022 and Collaboration with the Joint Aeolus Tropical Atlantic Campaign (JATAC) 

Ed Nowottnick, Jon Zawislak, Amin Nehrir, Will McCarty, Aaron Piña, Jeff Reid, Shu-Hua Chen, Angela Rowe, Naoko Sakaeda, Shuyi Chen, Ed Zipser, Zhaoxia Pu, Claire Robinson, Rich Ferrare, Svetla Hristova-Veleva, Luke Ziemba, Lee Thornhill, Kris Bedka, Michael Kavaya, and Simone Tanelli and the CPEX-CV/JATAC Team

A continuation of the National Aeronautics and Space Administration’s (NASA) truncated Convective Processes Experiment – Aerosols and Winds (CPEX-AW) field program flown out of St. Croix, USVI, in the summer of 2021, CPEX – Cabo Verde (CPEX-CV) deployed NASA’s DC-8 from Sal Island, Cabo Verde in September 2022, equipped with a unique and comprehensive suite of active and passive remote sensing and in-situ capabilities that, in combination with the availability of similar spaceborne observations, allowed for the measurements of tropospheric aerosols, winds, temperature, water vapor, and clouds and precipitation. The tropical northern East Atlantic Ocean is a data sparse region that, in boreal summer, offers a unique location to study convective lifecycles and processes in a variety of thermodynamic, dynamic, and aerosol environments, such as within persistent (e.g., Intertropical Convergence Zone, ITCZ) and periodic (e.g., African easterly waves and tropical cyclones) large-scale forcing, local terrain effects (e.g., land-ocean transition off western Africa), and aerosol-cloud interactions (e.g., Saharan air layer). In addition to observing the interaction between large-scale environmental forcing and convective systems, the payload is uniquely capable of observing the smaller-scale processes within the near-environment of convection, including those within the marine boundary layer (e.g., cold pools), the inflow/outflow of the storm, and dust-cloud interactions, that affect convective initiation and lifecycle, as well as other poorly resolved/understood properties of these systems.

CPEX-AW and -CV were a part of a joint observing effort with the European Space Agency (ESA) and their partner laboratories and universities called the Joint Aeolus Tropical Atlantic Campaign (JATAC) out of Cabo Verde to validate ESA’s Aeolus satellite. As part of the CPEX-CV – JATAC collaboration in September 2022, the NASA DC-8 carried out coincident underpasses of the Aeolus satellite on four of the thirteen CPEX-CV research flights, performed four overpasses of the ASKOS ground site at Mindelo, and two coordinated flights with the Slovenian WT-10 in situ aircraft that also encompassed a coincident flight under Aeolus and over the Mindelo ground site. Here, we summarize the CPEX-CV science objectives, mission architecture, scientific targets observed on flights flown during the September 2022 campaign, and highlights of the data collected planned to be released to the community in early April 2023 with a focus on collaborative efforts between CPEX-CV and JATAC.

How to cite: Nowottnick, E., Zawislak, J., Nehrir, A., McCarty, W., Piña, A., Reid, J., Chen, S.-H., Rowe, A., Sakaeda, N., Chen, S., Zipser, E., Pu, Z., Robinson, C., Ferrare, R., Hristova-Veleva, S., Ziemba, L., Thornhill, L., Bedka, K., Kavaya, M., and Tanelli, S. and the CPEX-CV/JATAC Team: Overview of NASA’s Convective Processes Experiment – Cabo Verde (CPEX-CV) in the East Atlantic in September 2022 and Collaboration with the Joint Aeolus Tropical Atlantic Campaign (JATAC), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8956, https://doi.org/10.5194/egusphere-egu23-8956, 2023.

EGU23-9467 | ECS | Posters on site | AS1.37

Studying interactions between low clouds and wind profiles using ALADIN/AEOLUS data 

Zacharie Titus and Hélène Chepfer

Wind profiles in the lower troposphere influence the processes driving cloud formation and dissipation. For example, dendritic cumulus and linear sheets formations are governed by different factors including wind direction and velocity. Trade winds and local dynamic processes influence the formation of cumulus and stratocumulus.

Using multiple case studies where the ALADIN lidar observes the different cloud patterns mentioned above, we will see how AEOLUS retrieves winds and clouds and what are the links between them. This study will be backed by visible MODIS observations and Calipso-GOCCP data to confirm the presence of clouds and their types. The focus will be around the JATAC area (Cape Verde, June to September 2021 and 2022), especially in the boundary layer, where our knowledge about the interactions between the wind and clouds are yet to be improved.

How to cite: Titus, Z. and Chepfer, H.: Studying interactions between low clouds and wind profiles using ALADIN/AEOLUS data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9467, https://doi.org/10.5194/egusphere-egu23-9467, 2023.

EGU23-10020 | Orals | AS1.37

Three-dimensional pathways of Saharan dust export over the North Atlantic during the CADDIWA field campaign 

Juan Cuesta, Cyrille Flamant, Marco Gaetani, Julien Delanoë, Jean-Pierre Chaboureau, Laurent Menut, and Paola Formenti

Massive amounts of desert dust uplifted over the Sahara are exported over the North Atlantic. They play a major environmental role over this region, impacting the Earth radiative budget, atmospheric dynamics and thermodynamics, cloud properties, atmospheric composition, and biogeochemistry. These multiple impacts of Saharan dust can also affect the evolution of mesoscale convective systems (MCS) formed over West Africa that may lead to the formation of tropical cyclones over the North Atlantic. A better understanding of these aspects, also influenced by African Easterly waves, is the primary objective of the “Clouds-Atmospheric Dynamics-Dust Interactions in West Africa - CADDIWA ” field experiment that took place on September 2021.  

The current presentation will provide a comprehensive description of the three-dimensional (3D) distribution of Saharan dust and its pathways of export over the North Atlantic during CADDIWA. This will be analysed with respect to the location and evolution of the MCS travelling over the region. This characterisation will be done using a suite of observations which will be compared with dust simulations. The objective is to analyse the difference in terms of abundance and 3D distribution of dust between the cases where MCSs lead to cyclogenesis and those not evolving that way.

The ensemble of datasets describing the Saharan dust distribution will be inter-compared and their consistency verified. Twice-daily satellite thermal infrared hyperspectral measurements from IASI will be used to document the 3D distribution of desert dust for cloud-free conditions using the AEROIASI approach (Cuesta et al., 2015; 2020). Further details will be provided by nadir-pointing lidar measurements from AEOLUS and CALIOP space sensors, and from the RALI airborne instruments, in terms of transects of aerosol profiles and winds. In addition to aerosol backscatter profiles, AEOLUS and LNG-RALI will provide aerosol extinction profiles, provided their high spectral resolution capabilities. Observations from MODIS and VIIRS of aerosol optical depth will inform on the horizontal distribution of desert dust. Airborne in situ measurements of the size distribution and intensive optical properties of desert dust, such as the angstrom exponent, will be compared to those used as a priori properties of dust within the satellite dust retrievals (particularly for IASI). These satellite and airborne measurements will be confronted with simulations from the Meso-NH and WRF-CHIMERE, contributing with an all-sky and hourly 3D description.

How to cite: Cuesta, J., Flamant, C., Gaetani, M., Delanoë, J., Chaboureau, J.-P., Menut, L., and Formenti, P.: Three-dimensional pathways of Saharan dust export over the North Atlantic during the CADDIWA field campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10020, https://doi.org/10.5194/egusphere-egu23-10020, 2023.

EGU23-10983 | Posters on site | AS1.37

Investigating the evolution of a tropical wave observed during JATAC/CPEX-CV using the campaign data portal 

Svetla Hristova-Veleva, Angela Rowe, Edward Zipser, Jonathan Zawislak, P. Peggy Li, Brian Knosp, Quoc Vu, and Jason Eriksen

The Joint Aeolus Tropical Atlantic Campaigns (JATAC) 2021 and 2022 deployed on the US Virgin Islands and Cabo Verde, respectively, with science objectives related to the life cycle of convective systems, the long-range transport of dust and its impact on air quality, and the satellite calibration/validation of current and the preparation of future ESA and NASA missions (Aeolus, EarthCARE, AOS, WIVERN). The NASA components of JATAC, Convective Processes Experiment-Aerosols and Winds (CPEX-AW) and CPEX–Cabo Verde (CPEX-CV), included a focus on the complex multi-scale processes and interactions that lead to convective development and its upscale growth: Understanding the environmental conditions supporting the development of tropical cyclones (TCs) remains a research and operational challenge, owing in part to limited observations of the lifecycle of convective activity that eventually become TCs. In the Atlantic basin, early stages of TC development favor the region off the west coast of Africa as African Easterly Waves move offshore and provide, at times, favorable conditions for TC development. CPEX-CV provided airborne measurements in this region, with a total of 13 research flights throughout September 2022. The payload included a triple-frequency precipitation radar, Doppler wind lidar, and dropsondes, among other remote sensing and in situ instrumentation, offering a rare 4-D look at tropical oceanic convective systems and their environment.

 

To support the campaign goals, we developed the JPL CPEX-AW/CV portal (https://cpex-aw.jpl.nasa.gov), which integrates model forecasts with multi-parameter satellite and airborne observations from a variety of instruments. The portal provides an interactive system for multi-scale visualization and on-line analysis, allowing for the interrogation of a large number of variables for flight planning and execution and for post-campaign analysis, including the large-scale context of the detailed airborne observations. In this presentation, the portal will be used to provide an initial investigation into the evolution of a tropical wave observed during CPEX-CV. The 16 September 2022 flight targeted a growing convective system associated with a broad circulation, the wave structure itself, an Aeolus validation underflight, and dust over Mindelo in coordination with other JATAC measurements. While the wave was not forecasted to immediately develop into a TC downstream, the convection sampled on the western edge of the wave was intense with lightning, although did not grow upscale into a large organized mesoscale convective system during or immediately after the flight. A focus of this initial portal-based analysis is on gradients in environmental moisture, evolution of environmental wind shear in the vicinity of the precipitation, and the presence (or absence) of large-scale convergence as we suspect some combination of these factors limited the initial development of this convective system into a tropical cyclone. Potential later large-scale ties to the development of Hurricane Ian in the Caribbean will also be explored with the portal as it provided a useful tool for this purpose.

How to cite: Hristova-Veleva, S., Rowe, A., Zipser, E., Zawislak, J., Li, P. P., Knosp, B., Vu, Q., and Eriksen, J.: Investigating the evolution of a tropical wave observed during JATAC/CPEX-CV using the campaign data portal, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10983, https://doi.org/10.5194/egusphere-egu23-10983, 2023.

EGU23-13084 | ECS | Posters on site | AS1.37

Overview and first analysis of the in situ microphysical measurement dataset collected during the CADDIWA mission 

Pierre Coutris, Guy Febvre, Louis Jaffeux, Clément Bazantay, Clémantyne Aubry, Christophe Caudoux, Julien Delanoë, Alfons Schwarzenboeck, and Cyrille Flamant

In the frame of the Joint Aeolus Tropical Atlantic Campaigns, an airborne field campaign took place in Sal island of Cape-Verde from the 8th to 21st of September 2021, as part of the French CADDIWA mission. During this campaign, the SAFIRE F20 research aircraft equipped with in situ and remote sensing instruments performed nine 3 to 4 hour long flights sampling tropical environment underneath AEOLUS satellite tracks and performing exploration flights within the convective cloud systems of tropical disturbances. In this study, an overview of the available aerosol and cloud in situ dataset is given first, presenting the instrumental and methodological approaches relevant to the collection of data from a set of four instruments: the UHSAS (aerosol size range : 40 – 1000 nm,  Cai et al. 2008), the SPP-300 (aerosol 0.3 – 20 µm, Baumgardner 1992) and the CDP-2 (droplets 2-50 µm, Lance et al. 2010) scattering probes, and the 2D-S imager (10-1280 µm, Lawson et al. 2006). Then a detailed microphysical analysis is conducted on two case studies: a tropical perturbation referred to as Pierre-Henri in this study (unnamed/numbered by NOAA National Hurricane Center (NHC)), sampled during F20 flight #7/8, and the Tropical Storm Rose (# AL172021 according to NOAA NHC) sampled during flights #12/13. The analysis includes a discussion on the main microphysical properties such as Particle Size Distribution (PSD), Ice Water Content (IWC) retrieved at different locations in the cloud convective systems, complemented by 95GHz reflectivity and Doppler vertical velocity measured by the airborne cloud radar RASTA (Delanoe et al. 2013). The data supporting this study is illustrated in the figure below: the vertical velocity (derived from 3 Doppler non colinear measurements of the radar) and PSD time series are given on top of two samples ice crystal images taken by the 2DS imager at different location in the TS Rose. A newly developed image classification algorithm (Jaffeux et al. 2022) is applied to the 2D-S data to derive statistics on the ice particles morphological properties, yielding to a discussion on the microphysical ice growth processes occurring in these systems.

How to cite: Coutris, P., Febvre, G., Jaffeux, L., Bazantay, C., Aubry, C., Caudoux, C., Delanoë, J., Schwarzenboeck, A., and Flamant, C.: Overview and first analysis of the in situ microphysical measurement dataset collected during the CADDIWA mission, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13084, https://doi.org/10.5194/egusphere-egu23-13084, 2023.

EGU23-14445 | ECS | Posters on site | AS1.37

Validation of the Aeolus L2A products with the eVe lidar during ASKOS/JATAC campaign 

Peristera Paschou, Nikolaos Siomos, Eleni Marinou, Antonis Gkikas, Samira Moussa Idrissa, Daniel Tetteh Quaye, Désiré Dêgbé Fiogbe Attannon, Charoula Meleti, Jonas von Bismarck, Thorsten Fehr, and Vassilis Amiridis

Abstract. The Joint Aeolus Tropical Atlantic Campaign (JATAC) for the Calibration and Validation (Cal/Val) of the ESA’s Aeolus mission was held on summer and September 2021 and 2022 at the remote tropical islands of Cabo Verde. The JATAC campaign comprises airborne and ground-based instrumentation delivering reference measurements of wind profiles and aerosol/cloud optical properties for the validation of the Aeolus products, as well as supporting related research activities. The ground-based component of JATAC, ASKOS (https://askos.space.noa.gr/) was stationed at the Ocean Science Center in Mindelo (OSCM), São Vicente Island, where measurements from active and passive remote sensing sensors have been deployed for the validation of the Aeolus Level 2 aerosol and wind products.

The eVe lidar, which is the ESA’s ground reference lidar system, was deployed in ASKOS for the validation of the Aeolus Level 2A aerosol products. eVe lidar is a scanning system that can perform combined linear/circular polarization and Raman measurements that operates at 355 nm and retrieves the particle backscatter coefficient, the particle extinction coefficient, the lidar ratio, and the linear and circular depolarization ratios. The lidar is implemented in a dual-laser/dual-telescope configuration that allows eVe to simultaneously reproduce the operation of the ALADIN lidar onboard Aeolus, i.e. circularly polarized emission, as well as the operation of a traditional lidar system, i.e. with linearly polarized emission. Targeted measurements of eVe lidar for the Aeolus validation were performed every Friday evening during the nearest Aeolus overpass from Mindelo resulting to a dataset of fourteen collocations for the intensive ASKOS operation periods in 2021 and 2022. In this study, we present the results from the comparison of the particle backscatter and extinction coefficients, and the lidar ratio between eVe and Aeolus profiles.

 

Acknowledgements:

This research was supported by the European Space Agency project ASKOS (Grant agreement 4000131861/20/NL/IA) and the PANGEA4CalVal project (Grant Agreement 101079201) funded by European Union’s Horizon Widera 2021 Access program.

How to cite: Paschou, P., Siomos, N., Marinou, E., Gkikas, A., Moussa Idrissa, S., Tetteh Quaye, D., Dêgbé Fiogbe Attannon, D., Meleti, C., von Bismarck, J., Fehr, T., and Amiridis, V.: Validation of the Aeolus L2A products with the eVe lidar during ASKOS/JATAC campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14445, https://doi.org/10.5194/egusphere-egu23-14445, 2023.

EGU23-14575 | Posters on site | AS1.37

Dust orientation measurements 

Alexandra Tsekeri, Vasillis Amiridis, Spyros Metallinos, Peristera Paschou, Nikos Siomos, Ioanna Tsikoudi, Dimitra Kouklaki, and Eleni Marinou

Abstract. Dust orientation is an ongoing investigation in recent years (Ulanowski et al., 2007). Its potential proof will be a paradigm shift for dust remote sensing, invalidating the currently used simplifications of randomly-oriented particles. Vertically-resolved measurements of dust orientation can be acquired with the new polarization lidar “WALL-E”, designed to target the off-diagonal elements of the backscatter matrix which are non-zero only when the particles are oriented (Tsekeri et al., 2021). Herein, we present first measurements of oriented dust particles acquired during the ESA Aeolus Cal/Val Campaign “ASKOS” at Cabo Verde (June and September 2022).

 

Acknowledgments: This research was supported by D-TECT (Grant Agreement 725698) funded by the European Research Council (ERC) under the European Union's Horizon 2020 research and innovation program and PANGEA4CalVal (Grant Agreement 101079201) funded by European Union’s Horizon Widera 2021 Access program.

 

 

References:

Tsekeri, A., et al.: Polarization lidar for detecting dust orientation: system design and calibration, Atmos. Meas. Tech., 14, 7453–7474, 2021.

Ulanowski, Z., et al.: Alignment of atmospheric mineral dust due to electric field, Atmos. Chem. Phys., 7, 6161–6173, 2007.

How to cite: Tsekeri, A., Amiridis, V., Metallinos, S., Paschou, P., Siomos, N., Tsikoudi, I., Kouklaki, D., and Marinou, E.: Dust orientation measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14575, https://doi.org/10.5194/egusphere-egu23-14575, 2023.

EGU23-15338 | ECS | Posters on site | AS1.37

Dust aerosols’ mineralogy in the chemical transport model COSMO-MUSCAT during JATAC and comparison with lidar and in-situ data 

Sofía Gómez Maqueo Anaya, Dietrich Althausen, Kerstin Schepanski, Matthias Faust, Bernd Heinold, Ina Tegen, Holger Baars, Ronny Engelmann, Anett Skupin, Martin Radenz, Albert Ansmann, Birgit Hesse, Ulla Wandinger, Grisa Mocnik, Eder Silva, Elizandro Rodrigues, Pericles Silva, and Cordula Zenk

Mineral dust aerosols are composed from a complex assemblage of various minerals depending on the region they come from. Considering that minerals have their distinct physicochemical properties, differences on mineral dust aerosols climatic impact will arise as a consequence of distinct mineral content.

Chemical transport models typically assume that mineral dust aerosols have uniform composition, despite the known regional variations in the mineral components. This study adds mineralogical information to the mineral dust emission scheme used in the chemical transport model, COSMO-MUSCAT.

Here we show some steps of the inclusion of mineralogy to the emission scheme. Results of the simulated mineral dust aerosols are shown with their respective mineralogy from sources in Africa for an example case from the JATAC campaign in September 2021. The results of the simulated mineral dust aerosol are compared with lidar and in-situ data measured at Mindelo, Cape Verde. Furthermore, the comparison with the lidar retrieved vertical profiles at Mindelo, highlights a possible link between the mineral dust aerosol optical properties and the distinct minerals found within them.

How to cite: Gómez Maqueo Anaya, S., Althausen, D., Schepanski, K., Faust, M., Heinold, B., Tegen, I., Baars, H., Engelmann, R., Skupin, A., Radenz, M., Ansmann, A., Hesse, B., Wandinger, U., Mocnik, G., Silva, E., Rodrigues, E., Silva, P., and Zenk, C.: Dust aerosols’ mineralogy in the chemical transport model COSMO-MUSCAT during JATAC and comparison with lidar and in-situ data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15338, https://doi.org/10.5194/egusphere-egu23-15338, 2023.

EGU23-15901 | ECS | Orals | AS1.37

Airborne In-situ Measurements during JATAC/CAVA-AW 2021/2022 campaigns - First Climate-Relevant Results 

Jesús Yus Díez, Marija Bervida, Luka Drinovec, Blaž Žibert, Matevž Lenarčič, Eleni Marinou, Peristera Paschou, Nikolaos Siomos, Holger Baars, Ronny Engelmann, Annett Skupin, Cordula Zenk, Thorsten Fehr, and Griša Močnik

The JATAC campaign in September 2021 and September 2022 on and above Cape Verde Islands have resulted in a large dataset of in-situ and remote measurements. In addition to the calibration/validation of the ESA’s Aeolus ALADIN during the campaign, the campaign also featured secondary scientific objectives related to climate change. The atmosphere above the Atlantic Ocean off the coast of West Africa is ideal for the study of the Saharan Aerosol layer (SAL), the long-range transport of dust, and the regional influence of SAL aerosols on the climate.

We have instrumented a light aircraft (Advantic WT-10) with instrumentation for the in-situ aerosol characterization. Ten flights were conducted over the Atlantic Ocean up to over 3000 m above sea level during two intense dust transport events. PollyXT, and EvE lidars were deployed at the Ocean Science Center, measuring the vertical optical properties of aerosols and were also used to plan the flights.

The particle light absorption coefficient was determined at three different wavelengths with Continuous Light Absorption Photometers (CLAP). They were calibrated with the dual wavelength photo-thermal interferometric measurement of the aerosol light-absorption coefficient in the laboratory. The particle size distributions above 0.3 µm diameter were measured with two Grimm 11-D Optical Particle Size Spectrometers (OPSS). These measurements were conducted separately for the fine aerosol fraction and the enriched coarse fraction using an isokinetic inlet and a pseudo-virtual impactor, respectively.

The aerosol light scattering and backscattering coefficients were measured with an Ecotech Aurora 4000 nephelometer. The instrument used a separate isokinetic inlet and was calibrated prior to and its calibration validated after the campaign with CO2. We have measured the total and diffuse solar irradiance with a DeltaT SPN1 pyranometer. CO2 concentration, temperature, aircraft GPS position altitude, air and ground speed were also measured.

The in-situ single-scattering albedo Angstrom exponent and the lidar depolarization ratio will be compared as two independent parameters indicating the presence of Saharan dust. We will show differences between homogeneous Saharan dust layer in space (horizontally and vertically) and time and events featuring strong horizontal gradients in aerosol composition and concentration, and layering in the vertical direction. These layers often less than 100 m thick, separated by layers of air with no dust.

Complex mixtures of aerosols in the outflow of Saharan dust over the Atlantic Ocean in the tropics will be characterized. We will show the in-situ atmospheric heating/cooling rate and provide insight into the regional and local effects of this heating of the dust layers. These measurements will support of the research on evolution, dynamics, and predictability of tropical weather systems and provide input into and verification of the climate models.

How to cite: Yus Díez, J., Bervida, M., Drinovec, L., Žibert, B., Lenarčič, M., Marinou, E., Paschou, P., Siomos, N., Baars, H., Engelmann, R., Skupin, A., Zenk, C., Fehr, T., and Močnik, G.: Airborne In-situ Measurements during JATAC/CAVA-AW 2021/2022 campaigns - First Climate-Relevant Results, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15901, https://doi.org/10.5194/egusphere-egu23-15901, 2023.

EGU23-16530 | ECS | Orals | AS1.37

ASKOS Campaign 2021/2022: Overview of measurements and applications 

Eleni Marinou, Vassilis Amiridis, Peristera Paschou, Ioanna Tsikoudi, Alexandra Tsekeri, Vassiliki Daskalopoulou, Holger Baars, Athina Floutsi, Dimitra Kouklaki, Razvan Pirloaga, Franco Marenco, Maria Kazoudi, Ewan O Connor, Lukas Pfitzenmaier, Cordula Zenk, Claire Ryder, Jonas Von Bismarck, and Thorsten Fehr and the ASKOS team

In the framework of the Joint Aeolus Tropical Atlantic Campaign (JATAC), the ASKOS experiment was implemented in Cabo Verde during summer and autumn of 2021 and 2022. The main objective of ASKOS was the collection of an unprecedented dataset of synergistic measurements in the region, to be used to address a wide range of scientific objectives, namely the support of the validation of Aeolus mission’s products, the study of the processes affecting dessert dust transport (water vapor, giant particles, mixing with boundary layer dynamics), the characterization of the cloud microphysics, the effect of dust particles in the cloud formation over the region, the effect of the large dust particles on radiation and others.

During the ASKOS experiment, intense ground-based remote sensing and airborne in situ measurements took place on and above Mindelo on the island of São Vicente, Cabo Verde. At the Ocean Science Center in Mindelo (OSCM), a full ACTRIS remote sensing super site was set up in 2021, including a multiwavelength-Raman-polarization lidar PollyXT, an AERONET sun photometer, a Scanning Doppler wind lidar, a microwave radiometer and a cloud radar belonging to ESA fiducial reference network (FRM4Radar). Additionally, the ESA’s reference lidar system eVe, a combined linear/circular polarization lidar with Raman capabilities, was deployed. In 2022, the operations were enhanced with the deployment of airborne in-situ aerosol measurements on-board UAVs deployed by the Cyprus Institute, solar radiation measurements supported by PMOD/WRC, dust particle orientation measurements from the WALL-E lidar of National Observatory of Athens, and radiosonde releases equipped with additional electric field and electric charge measurements. The campaign was supported by dedicated numerical weather and dust simulations from CAMS and ECMWF, and tailored WRF simulations with nested domains above the campaign site.  

From the ASKOS dataset, three cases have been selected as "golden cases” where multiple JATAC airborne platforms and Aeolus satellite performed collocated measurements alongside with the ground-based instrumentation around the ASKOS operations site. Furthermore, multiple synergistic measurements with the JATAC airborne platforms were performed in the broader Cabo Verde region. Here, we quickly introduce ASKOS measurements and present first results. 

How to cite: Marinou, E., Amiridis, V., Paschou, P., Tsikoudi, I., Tsekeri, A., Daskalopoulou, V., Baars, H., Floutsi, A., Kouklaki, D., Pirloaga, R., Marenco, F., Kazoudi, M., O Connor, E., Pfitzenmaier, L., Zenk, C., Ryder, C., Von Bismarck, J., and Fehr, T. and the ASKOS team: ASKOS Campaign 2021/2022: Overview of measurements and applications, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16530, https://doi.org/10.5194/egusphere-egu23-16530, 2023.

EGU23-17089 | Posters on site | AS1.37

Unmanned Aerial Vehicles for the Joint Aeolus Tropical Atlantic Campaign 

Franco Marenco, Maria Kezoudi, Alkistis Papetta, Christos Keleshis, Claire Ryder, Natalie Ratcliffe, Konrad Kandler, Joe Girdwood, Chris Stopford, Frank Wienhold, Ru-Shan Gao, Eleni Marinou, Vassilis Amiridis, Holger Baars, Grisa Mocnik, and Jean Sciare

During June 2022, the Cyprus Institute (CyI) took part in the ASKOS experiment in Mindelo, Cape Verde, with several of Unmanned Aerial Vehicles (UAVs), fitted with a number of in-situ aerosol instruments able to profile the Saharan Air Layer between the surface and an altitude of 5,300 m. In addition to ASKOS objectives, transnational access project Diurnal vAriation of the vertically resolved siZe distribution in the Saharan Air Layer  (DAZSAL) was also carried out at the same time. The campaign aimed at validating the Aeolus L2A product in the presence of dust and marine aerosols, estimating the influence on Aeolus products of non-spherical particles, evaluating the impact of particle orientation, and study the diurnal cycle of the dust size-distribution at high altitude. In this presentation we will present and discuss the scientific objectives, the context, the Unmanned Aerial Systems (UASs) that we developed in-house, and the instruments used, together with their limitations, calibration methods, uncertainties, challenges and difficulties encountered. We will also discuss the logistical and planning challenges that such a campaign entails.

Operations took place from the Cesaria Evora International Airport. The instruments deployed on-board the UAVs permitted to evaluate the height-resolved particle size-distribution between 0.1 and 40 µm and detect cases of particle orientation, to complement the observations with ground-based remote sensing set out by NOA and TROPOS. Moreover, 24 high-altitude dust samples were collected on impactors, for further analysis by Scanning Electron Microscopy. In total, 25 scientific flights were performed on 12 flying days (almost half of which at night). Five flights were conducted during Aeolus overpasses. Weather has been a determining factor for both the ground-based remote sensing operations and the UAS operation, and airport traffic has been another constraint that needed to be accounted for, in the UAS operation.

How to cite: Marenco, F., Kezoudi, M., Papetta, A., Keleshis, C., Ryder, C., Ratcliffe, N., Kandler, K., Girdwood, J., Stopford, C., Wienhold, F., Gao, R.-S., Marinou, E., Amiridis, V., Baars, H., Mocnik, G., and Sciare, J.: Unmanned Aerial Vehicles for the Joint Aeolus Tropical Atlantic Campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17089, https://doi.org/10.5194/egusphere-egu23-17089, 2023.

EGU23-17090 | Orals | AS1.37

Profiling Saharan Airborne Dust with UAV-based in-situ Instrumentation during the ASKOS Experiment in Cape Verde 

Maria Kezoudi, Franco Marenco, Alkistis Papetta, Christos Keleshis, Claire Ryder, Konrad Kandler, Joe Girdwood, Chris Stopford, Frank Wienhold, Ru-Shan Gao, Eleni Marinou, Vassilis Amiridis, Grisa Mocnik, Holger Baars, and Jean Sciare

The ASKOS experimental campaign of European Space Agency (ESA) was organised by the National Observatory of Athens, and aimed at the calibration and validation of the Aeolus satellite aerosol/cloud product. Airborne observations were performed by the Climate and Atmosphere Research Centre (CARE-C) team of the Cyprus Institute at the Cesaria Evora International Airport of the island of São Vicente in Cape Verde between 10 and 30 June 2022. These in-situ aerosol measurements were conducted using the advanced Unmanned Aerial Vehicles (UAVs) of the Unmanned System Research Laboratory (USRL), equipped with specialised aerosol in-situ sensors, capturing the Saharan Air Layer (SAL) from ground up to 5.3 km Above Sea Level (ASL). The new custom-designed Composite Bird (CoBi) USRL and Skywalker UAVs (Kezoudi et al., 2021), were equipped with Optical Particle Counters (OPCs), samplers and backscatter sondes.

25 UAV vertical flights were performed in total, with 11 of them during night. The altitude of the Marine Boundary Layer (MBL) was mainly observed from ground up to about 1.0 km ASL, whereas during most of the flights, high concentrations of dust particles were found between 1.5 and 5.0 km ASL. Results obtained from OPCs show the presence of particles sizing up to 20 um within MBL and up to 40 um within SAL. Further information on morphology and mineralogy of observed particles will be given by the offline analysis of collected samples under Scanning Electron Microscope (SEM). COBALD observations alongside ground-based lidar measurements agree on the presence of non-spherical particles within dust layers.  

Ongoing exploitation of airborne observations along with coincident and collocated ground-based measurements will provide a complete picture for comparison with Aeolus data, particularly in relation to aerosols, where we have the most to learn.

How to cite: Kezoudi, M., Marenco, F., Papetta, A., Keleshis, C., Ryder, C., Kandler, K., Girdwood, J., Stopford, C., Wienhold, F., Gao, R.-S., Marinou, E., Amiridis, V., Mocnik, G., Baars, H., and Sciare, J.: Profiling Saharan Airborne Dust with UAV-based in-situ Instrumentation during the ASKOS Experiment in Cape Verde, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17090, https://doi.org/10.5194/egusphere-egu23-17090, 2023.

EGU23-17110 | Posters on site | AS1.37

Enhancing Aeolus L2A for depolarizing targets and impact on aerosol research and NWP 

Thanasis Georgiou, Emmanouil Proestakis, Antonis Gkikas, Konstantinos Rizos, Eleni Drakaki, Anna Kampouri, Athanasios Tsikerdekis, Holger Baars, Athena Augousta Floutsi, Angela Benedetti, and Vassilis Amiridis

Aeolus, ESA’s space mission, provides vertical profiles of the HLOS wind component in the troposphere and the lower stratosphere. In addition, ALADIN thanks to its HSLR configuration retrieves and provides profiles of extinction/backscatter coefficients of aerosols and clouds (known as spin-off or L2A products), at the ultraviolet region of the spectrum (355nm). However, ALADIN’s design enables the detection only of the returned co-polar component of the transmitted light. This inherent limitation hampers the ability of ALADIN to provide realistic optical products (i.e., underestimated backscatter coefficient profiles) when non-spherical particles (e.g., dust, volcanic ash, cirrus ice crystals) are probed, a deficiency for the case of Earth Observation of highly depolarizing targets with negative impacts on applications of Data Assimilation (DA) and Numerical Weather Prediction (NWP). 

The ESA L2A+ (Enhancing Aeolus L2A for depolarizing targets and impact on aerosol research and NWP) project kicked off in November 2022, with an overarching objective to develop a refined Aeolus L2A aerosol product (L2A+) and test its application for enhancing aerosol research. The generation of the refined L2A+ Aeolus aerosol optical product will be based, among others, on an integrated approach of novel algorithms (i.e., AEL-FM/AEL-PRO), model outputs (i.e., CAMS), advanced EO-based products (i.e., MSG, MODIS-MIDAS), existing climatologies (ESA-LIVAS), and AOD retrievals from Aeolus itself. The product will be thoroughly compared with L2A and validated against quality-assured measurements from the ESA-ASKOS/JATAC experiment in Cape Verde. 

With respect to the overarching objectives on aerosol research, L2A+ aims to (1) examine the impact of L2A and L2A+ on aerosol assimilation and dust transport models, (2) assess the impact of Aeolus on NWP, (3) highlight the benefit of the Aeolus joint aerosol and wind assimilation for simulating dust deposition fields, (4) assess the climatological value of L2A+ for aerosol databases such as the ESA-LIVAS long-term climate dataset, and (5) assess the impact of the novel L2A+ product on aerosol assimilation, towards improved dust transport modelling and for further enhancing NWP. 

The ESA-L2A+ project focuses on the broader the Western Sahara and the Tropical Atlantic Ocean, while due to the extensive wealth of available observational data collected in the framework of the European Space Agency (ESA) ASKOS Tropical Campaign in Cape Verde, which are needed for a complete and descriptive assessment analysis of the project outputs and the evaluation of the enhanced L2A+ product, the developments and experiments will be performed for September 2021. 

Preliminary results from the project will be presented. 

The L2A+ team acknowledges support by ESA in the framework of the "Enhancing Aeolus L2A for depolarizing targets and impact on aerosol research and NWP project (4000139424/22/I-NS). 

How to cite: Georgiou, T., Proestakis, E., Gkikas, A., Rizos, K., Drakaki, E., Kampouri, A., Tsikerdekis, A., Baars, H., Floutsi, A. A., Benedetti, A., and Amiridis, V.: Enhancing Aeolus L2A for depolarizing targets and impact on aerosol research and NWP, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17110, https://doi.org/10.5194/egusphere-egu23-17110, 2023.

EGU23-17250 | Orals | AS1.37

Overview of the High Altitude Lidar Observatory (HALO) water vapor DIAL and High Spectral Resolution Lidar observations during the summer 2022 CPEX-CV Campaign 

Amin Nehrir, Rich Ferrare, James Collins, Rory-Barton Grimley, Ewan Crosbie, and Eleni Marinou

The 2022 Convective Processes Experiment – Cabo Verde (CPEX-CV) collected observations using the NASA DC-8 to study dynamics and microphysics related to the Saharan Air Layer (SAL), African easterly waves and jets, and deep convection within the Intertropical Convergence Zone (ITCZ) in the tropical East Atlantic. CPEX-CV measurements also collected data to help calibrate and validate ESA’s Aeolus Doppler wind lidar.  CPEX-CV is part of combined effort with the European Space Agency (ESA) and their partner laboratories and universities called the Joint Aeolus Tropical Atlantic Campaign (JATAC) to validate ESA’s Aeolus satellite. As part of the CPEX-CV – JATAC collaboration from Cabo Verde in September 2022, the NASA DC-8, outfitted with a comprehensive suite of remote and in-situ sensors, coordinated with the ASKOS ground site at Mindelo and the Slovenian WT-10 aircraft to validate AEOLUS wind and aerosol products as well as to link quantitatve aerosol observations from multiple vantage points to better understand the role of the SAL in toprical dynamics.

During CPEX-CV the NASA DC-8 was outfitted with the Advanced Vertical Atmospheric Profiling System (AVAPS) dropsondes, Doppler Aerosol Wind Lidar (DAWN), High-Altitude Lidar Observatory (HALO), third generation Airborne Precipitation Radar (APR-3), High-Altitude Monolithic Microwave Integrated Circuit Sounding Radiometer (HAMSR), and the Cloud Aerosol and Precipitation Spectrometer.  This presentation will highlight the HALO water vapor DIAL and aerosol/cloud HSRL observations collected during CPEX-CV and discuss the synergies with the JATAC campaign.  HALO HSRL observations are compared and contrasted with those taken from the ground site at Mindelo to better understand the influence of orographic island effects on the transport of aerosols and better constrain aerosol processes such as aerosol electrification being studied by ASKOS.  Additionally, HALO aerosol backscatter, depolarization, and extinction products at 532 nm and 1064 nm are used to evaluate Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) aerosol retrievals at those same wavelengths and, after adjustment to 355 nm, are compared against Aeolus backscatter and extinction products.  Areas for future collaborative efforts will also be discussed including Aeolus and Earthcare validation.  

How to cite: Nehrir, A., Ferrare, R., Collins, J., Grimley, R.-B., Crosbie, E., and Marinou, E.: Overview of the High Altitude Lidar Observatory (HALO) water vapor DIAL and High Spectral Resolution Lidar observations during the summer 2022 CPEX-CV Campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17250, https://doi.org/10.5194/egusphere-egu23-17250, 2023.

EGU23-119 | ECS | Orals | CR7.3 | Highlight

Antarctic Atmospheric Rivers in the Past and Future Climates 

Michelle Maclennan, Andrew Winters, Christine Shields, Jonathan Wille, Rebecca Baiman, Léonard Barthelemy, and Vincent Favier

Atmospheric rivers (ARs) are long, narrow bands of warm and moist air that travel poleward from the midlatitudes. While Antarctic atmospheric rivers (ARs) occur only 1-3% of the time over the ice sheet, they are a significant contributor to Antarctic surface mass balance: they contribute 10% on average, and more than 20% locally, of Antarctic precipitation each year. Here we use an Antarctic-specific AR-detection algorithm to identify ARs in MERRA-2 and ERA5 reanalyses and the Community Earth System Model version 2 (CESM2). We use this algorithm to quantify the frequency, location, and precipitation attributed to Antarctic ARs for the period 1980-2014 and use these statistics to identify CESM2 biases relative to MERRA-2 and ERA5. We then apply the AR-detection algorithm to CESM2 for the future period (2015-2100) to examine how the frequency and intensity of ARs, AR-attributed total precipitation, and year-to-year variability in AR precipitation changes in the future under the SSP370 emissions scenario. Our results quantify past and future impacts of ARs on Antarctic annual precipitation, interannual variability, and trends, and ultimately provide an early assessment of future AR-driven changes in Antarctic surface mass balance.

How to cite: Maclennan, M., Winters, A., Shields, C., Wille, J., Baiman, R., Barthelemy, L., and Favier, V.: Antarctic Atmospheric Rivers in the Past and Future Climates, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-119, https://doi.org/10.5194/egusphere-egu23-119, 2023.

EGU23-814 | ECS | Orals | CR7.3 | Highlight

Evaluation of Greenland extreme snow melting patterns and their synoptic drivers 

Josep Bonsoms, Marc Oliva, and Juan Ignacio López-Moreno

 

Greenland Ice Sheet (GrIS) snow melting rates have drastically increased since the 1990s, with relevant implications in the entire ecosystem. According to climate projections, extreme weather events will potentially increase in the coming decades over the GrIS. Thus, it is necessary to analyze the past temporal evolution of GrIS extreme melting patterns, as well as their climate drivers. This work analyzes the GrIS summer extreme snow melting spatiotemporal evolution and trends (1990 to 2021). Further, we determine the contribution of synoptic weather types that drive extreme snow melting events. Results evidence that the frequency, magnitude, and the relative contribution of extreme snow melting to the total summer snow melting differs depending on the GrIS sector. Maximum extreme snow melting days per season are observed in western GrIS, whereas minimums are observed in northern sectors. The average extreme snow melting during summer is non-statistically significant increasing in the entire GrIS, which is consistent with the increase of the average snow melting for the same temporal period. Extreme snow melting days as well as the contribution of extreme snow melting to the total snow melting per season show an upward trend, except in the central and northern zones. The analysis of twenty summer circulation weather types reveals that extreme snow melting episodes for most of the GrIS sectors are mainly explained by a few synoptic systems; characterized by a high-pressure system located in central, southern, and eastern GrIS. During these synoptic episodes, stable weather conditions prevail, and the energy available for snow melting is mainly controlled by positive shortwave radiation heat fluxes leading to positive 850 hPa air temperature anomalies. Results presented in this work are relevant for a better understanding of extreme weather events over GrIS within a changing climate context.

How to cite: Bonsoms, J., Oliva, M., and López-Moreno, J. I.: Evaluation of Greenland extreme snow melting patterns and their synoptic drivers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-814, https://doi.org/10.5194/egusphere-egu23-814, 2023.

EGU23-2311 | ECS | Orals | CR7.3

The Atmospheric effects of Southern Ocean open-ocean polynyas onto coastal polynyas in EC-Earth3 

Jakob Gunnarsson, Lu Zhou, and Céline Heuzé

Polynyas are recurrent areas of open water or thin ice within the ice pack, which alter the local heat and moisture exchange and high-latitude atmosphere-ocean circulation interannual variability. They are differentiated as coastal (latent heat) or open-ocean (sensible heat) polynya according to their forming location. Especially, coastal polynyas are critical sources of dense water and the formation of Antarctic Bottom Water (AABW) following the brine enrichment of surface waters during sea-ice formation, and easily influenced by the local atmosphere conditions. However, few studies have examined the atmospheric response of open-ocean polynyas on the coastal polynyas given the fact that open-ocean polynyas have capability to re-adjust mesoscale atmosphere circulation. To better understand the surrounding impact of large open-ocean polynya events, output from CMIP6 historical experiment synoptic scale EC-Earth3 is adopted. Our results show an increasing coastal polynya frequency and extent accompanying with more active open-ocean polynya years in the Weddell Sea. The results are explained by near-surface wind speed differences in the coastal regions, which are found statistically significant between more and less active open-ocean polynya years. Furthermore, those intensifications of winds are found in days where easterly-dominated winds north-westerly to north-easterly and easterly to south-easterly cross the open-ocean polynya. Increased near-surface air temperatures as well as a deepening in sea level pressure are also observed during the years with more active open-ocean polynya events. The findings contribute to a better understanding of coastal polynya opening processes, as well as how we might expect to see the different type of polynya interact by their influence and dependence on surrounding atmospheric conditions.

How to cite: Gunnarsson, J., Zhou, L., and Heuzé, C.: The Atmospheric effects of Southern Ocean open-ocean polynyas onto coastal polynyas in EC-Earth3, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2311, https://doi.org/10.5194/egusphere-egu23-2311, 2023.

EGU23-3192 | ECS | Orals | CR7.3

Spatio-temporal variability of air temperature lapse rate in the glacierised catchment of the Chandra basin, western Himalaya using in-situ measurements 

Sunil N. Oulkar, Parmanand Sharma, Bhanu Pratap, Lavkush Patel, Sourav Laha, and Meloth Thamban

The air temperature lapse rate (TLR) plays an important role in estimating ice and snow melt in high mountain regions. The TLR can vary depending on several factors, including the topography of the catchments and the microclimate. TLR calculations are typically not precise in the Himalayan glacierised regions due to a lack of in-situ observation of meteorological parameters. Therefore, a dense in-situ monitoring network over a high altitudinal gradient is needed to estimate the TLR accurately. We have obtained in-situ measurements of air temperature data from five automatic weather stations (AWS) installed at the best possible locations in the Chandra basin catchment of the semi-arid zone of the western Himalaya from October 2019 to September 2022. The altitudinal range for air temperature measurement varied between ~4000 and 5000 m a.s.l. We utilise the air temperature data to estimate the TLR by regressing the temperature with the corresponding elevations.
Comparing all the estimated TLR, the mean annual value (4.9°C/km) was significantly lower than the standard environmental lapse rate (6.5 °C/km) with substantial seasonality. The maximum TLR (~6.8 °C/km) during the summer is likely due to the high-altitude range and thin air and the presence of cold air pools at higher altitudes. However, the significantly lower TLR (~1.9 °C/km) during winters is likely due to the low air temperature and high moisture content in the region due to western disturbance. Further, we observed strong diurnal variations of TLR, which was highest during the daytime and lowest at night. This study highlighted that the TLR was potentially influenced by the local topography, particularly with higher lapse rates at higher elevations. TLR vary topographically and temporally significantly in the Chandra basin, indicating that the air temperature in this region is more sensitive to climatic variations. The findings of this study will play an important role in glacio-hydrological models, where TLR is one of the essential inputs.

How to cite: Oulkar, S. N., Sharma, P., Pratap, B., Patel, L., Laha, S., and Thamban, M.: Spatio-temporal variability of air temperature lapse rate in the glacierised catchment of the Chandra basin, western Himalaya using in-situ measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3192, https://doi.org/10.5194/egusphere-egu23-3192, 2023.

The Arctic climate system has been suggested to be ‘en route’ to a new state with seasonally ice-free conditions expected within two-three decades under high-emissions scenarios. Here we show the prospect of its delayed emergence stemming from a consideration of observed and modelled Arctic cryosphere sensitivity to atmospheric circulation changes. While the observed Arctic warming contains a substantial contribution from large-scale circulation, it is not reflected in the modelled forced response. Numerical model simulations with the CESM2 with an active Greenland ice sheet model (CISM2), where model winds are nudged towards the observed state, advocate for the need to have a circulation-based model sensitivity evaluation metric. Hence a recalibration is proposed by matching the warming signals free of atmospheric circulation impacts in observations and models over 1979-2020. This constraint yields a ~decade delay in the projected timing of the first seasonally sea-ice free Arctic and widespread Greenland melting. Accounting for the role of large-scale atmospheric forcing in Arctic climate change offers new perspectives of estimating Arctic sea- and land-ice sensitivity to anthropogenic forcing and understanding the recently emerging issue of some CMIP6 climate models being ‘too hot’.

How to cite: Topal, D. and Ding, Q.: Atmospheric circulation-constrained model sensitivity recalibrates Arctic climate projections, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3971, https://doi.org/10.5194/egusphere-egu23-3971, 2023.

EGU23-5852 | ECS | Posters on site | CR7.3

CARRA-driven simulation of Greenland Ice Sheet surface mass balance at 2.5 km resolution 

Mathias Larsen, Ruth H. Mottram, and Peter L. Langen

Projections of present and future ice mass loss of the Greenland Ice Sheet are important for assessing its contribution to future sea-level rise. Critical for the total mass balance is the surface mass balance (SMB) which can be estimated from models, and improving these models can help to further constrain the uncertainties in future projections.

In this project, we use the CARRA reanalysis dataset generated from the HARMONIE-AROME weather forecast system to force an SMB model. The CARRA dataset is remarkable for its 2.5 km horizontal resolution providing unprecedented spatial detail. This is particularly important at the ice-sheet margins where both accumulation and ablation processes are impacted by strong topographic gradients. For example, the greater spatial detail is expected to provide more realistic profiles of accumulation and drying of airmasses from the coast toward the interior, in turn improving the SMB simulation.

The SMB model utilizes a subsurface scheme that consists of columns with 32 layers in the vertical. Driven by the atmospheric input, the SMB model computes all the interactions between the atmosphere and subsurface layers, such as accumulation, melting, percolation, refreezing and runoff. Using this SMB model, we performed a CARRA-driven simulation over the period 1991-2020 on the 2.5 km CARRA grid.

Our initial results show the CARRA-driven SMB model yielding somewhat higher SMB values compared to other published SMB products. The ice sheet-wide totals of accumulation and melt are comparable to other products. However, the location of maximum melt contributions is shifted further towards the interior of the ice sheet in the CARRA-driven simulation. This allows for larger refreezing and contributes significantly to the high SMB seen in the CARRA-driven simulation. Here, we evaluate the SMB model output and driving fluxes against PROMICE data and satellite observations and provide a new updated assessment of Greenland ice sheet SMB.

How to cite: Larsen, M., H. Mottram, R., and L. Langen, P.: CARRA-driven simulation of Greenland Ice Sheet surface mass balance at 2.5 km resolution, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5852, https://doi.org/10.5194/egusphere-egu23-5852, 2023.

EGU23-6243 | ECS | Posters on site | CR7.3

A systematic polar-induced signature in infrasound database highlithed by machine learning models 

Sentia Goursaud Oger, Alexandre Junqueira, and Mathilde Mougeot

Polar lows are intense but short duration maritime cyclones occurring in both hemispheres. In the northern pole, they are mainly located in the Barents and Norwegian seas, with significant damages for coastal populations. So far, a fully understanding of the physical processes at play is still lacking. This is due to the suddenness of such events, as well as a scarcity of meteorological observations in these areas. Infrasounds are sound waves with frequency ranges below the audible domain. It was shown that polar lows can be a source of infrasound. Only one study looked at the infrasound signature for two particular polar lows using data obtained from two stations, in Northern Norway and on Svalbard. Here we show the potentiality of a systematic polar low-induced signature in infrasound data.

Within the frame of the Comprehensive nuclear-test-ban treaty organization, infrasound stations were set up worldwide. One was settled in northern Norway (IS37NO) in 2003 and made fully operational since 2004. Its records consist in a timeseries of sub-daily pressure data, that are processed through a Progressive Multi Channel Cross Correlation method, resulting in variables such as the mean frequencies, azimuths and amplitudes of the detections, and covering 17 complete years (2004-2021). These variables were used to train statistical models to learn the occurrence of polar lows refered in a polar low database. Our models yield very good results, specially in term of precision and recall. They provide a basis for different research opportunities, such as the prediction of polar lows and a deeper comprehension of its climate controls.

How to cite: Goursaud Oger, S., Junqueira, A., and Mougeot, M.: A systematic polar-induced signature in infrasound database highlithed by machine learning models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6243, https://doi.org/10.5194/egusphere-egu23-6243, 2023.

EGU23-8805 | ECS | Orals | CR7.3

Extreme temperature events for the past 19 years in the McMurdo Dry Valleys, Antarctica linked to mesoscale meteorological variability 

Eva Bendix Nielsen, Marwan Katurji, Peyman Zawar-Reza, and Hanna Meyer

The McMurdo Dry Valleys (MDVs) in Antarctica have a unique environment classified as a hyper-arid desert with glacier runoff being the main source of liquid water. Previous studies have identified winds as the controlling factor of the climate in this region and especially the occurrence of foehn induced warming. Episodic foehn warming during the austral summer can contribute to above freezing temperatures sustained for multiple days. Years with extreme glacial runoff leading to flooding have been correlated with a higher occurrence of foehn induced warming events. Understanding the temporal availability of meltwater caused by extreme meteorological events is highly important since it is a dependant variable to the functioning of the area’s fragile ecosystem. Synoptic scale circulations in the surrounding Ross Sea Region are a driving factor for the occurrence of foehn warming in the MDVs with the local mesoscale meteorology modulating the spatiotemporal variability of the foehn-induced near-surface warming. AntAir ICE, a newly developed daily mean near surface air temperature dataset with a spatial grid resolution of 1 km2 has proven capable of capturing these mesoscale temperature variabilities for multiple seasons within the complex topography of the MDVs.

 

A case study on the 2nd of January 2020 where the maximum temperature measured in a Lake Vanda automatic weather station was above +9 degrees Celsius with multiple valleys experiencing foehn induced warming, displayed a clear warming signal for the MDVs in AntAir ICE. The atmospheric dynamic analysis from the numerical weather prediction model the Antarctic Mesoscale Prediction System (AMPS) indicated a clear foehn signature. This event was linked to a meso-low located in the Ross Sea which was detected in the climate re-analysis ERA5 mean sea level pressure dataset. By confidently identifying these warming events within the MDVs where there is a relatively high availability of Automatic Weather Stations and AMPS predictions, has allowed for further exploration of extreme sustained warming and potentially foehn induced warming along the terrestrial coastal margin of Antarctica. Using AntAir ICE, warming events during the austral summer season from November to February for the period 2003 to 2021 with sustained daily mean temperatures above freezing for multiple days have been identified for the Ross Sea Region. This study aims at capturing the mesoscale meteorological and climatological variability for multiple seasons within the Ross Sea Region, while linking these extreme warming events to larger scale circulation patterns can allow for understanding local extreme events in context of shifting large scale circulation drivers.

How to cite: Bendix Nielsen, E., Katurji, M., Zawar-Reza, P., and Meyer, H.: Extreme temperature events for the past 19 years in the McMurdo Dry Valleys, Antarctica linked to mesoscale meteorological variability, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8805, https://doi.org/10.5194/egusphere-egu23-8805, 2023.

EGU23-10042 | ECS | Orals | CR7.3 | Highlight

Global Sources of Moisture for Atmospheric Rivers over Antarctica 

Rajashree Datta, Adam Herrington, Luke Trusel, David Schneider, Jesse Nusbaumer, and Ziqi Yin

 

The quantity and characteristics of atmospheric rivers over Antarctica, which import heat and moisture towards the continent, are a major source of uncertainty in future sea level rise estimates. We employ a new variable-resolution grid over Antarctica, using CESM2 (VR-CESM2), which balances the extensibility of a GCM with the high computational costs of a high-resolution climate model. This setup uses observed sea surface temperature and sea ice concentration, implements moisture-tagging (linking precipitation to a moisture source region on the globe), and produces high spatial and temporal resolution atmosphere and ice sheet surface outputs, which can be used to detect atmospheric rivers and to estimate their impact.

As a baseline for experiments testing the relative importance of large-scale drivers, we first quantify, over an idealized 10-year period, the global sources of moisture and the portion of total precipitation that reaches the ice sheet during large-scale vs atmospheric river events (and their associated synoptic characteristics). Beyond this baseline, we will use this setup to perform initial test scenarios assessing the relative impact of reduced sea ice combined with enhanced ocean heat at lower latitudes.

How to cite: Datta, R., Herrington, A., Trusel, L., Schneider, D., Nusbaumer, J., and Yin, Z.: Global Sources of Moisture for Atmospheric Rivers over Antarctica, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10042, https://doi.org/10.5194/egusphere-egu23-10042, 2023.

The current period of Arctic amplification has been characterized by a pronounced reduction in high-latitude snow and ice cover that is reflective of rapidly changing thermodynamic environment. Given this change in the local background conditions, it is not surprising that the Greenland Ice Sheet (GrIS) has undergone drastic surface mass loss since the turn of the century; however, research has shown that the recent acceleration of runoff from the GrIS is strongly linked to a shift in the large-scale atmospheric circulation over the same period that has brought more frequent and intense bouts of summer Greenland blocking. While this atmospheric dynamical change may merely be a manifestation of internal variability, there is growing evidence that widespread changes in surface cover and near-surface thermal gradients under Arctic amplification may favor persistent extremes such as the episodes of Greenland blocking that have encouraged melt of the ice sheet.

Here, we explore whether the change in summer atmospheric circulation over Greenland may be a dynamical response to Arctic amplification and attendant snow cover loss. Our results suggests that low North American spring snow cover and a weakened meridional temperature gradient combine to encourage the high-amplitude Omega blocking patterns that we show to have driven the recent trend in summer Greenland blocking. We show that this delayed response to anomalous spring snow cover follows from the snow-hydrological effect, whereby low spring snow cover causes early depletion of soil moisture and anomalously warm surface temperature over eastern North America. The consequent stationary Rossby wave response enforces an anomalous anticyclone, centered over Baffin Bay, that resembles that of high-amplitude Omega blocks and the atmospheric conditions which have promoted melt of the northern GrIS. Together, these results provide evidence that Arctic amplification, and thus anthropogenic climate change, has contributed to recent atmospheric dynamical forcing of GrIS surface mass loss. However, regardless of how strong this link between climate change and atmospheric circulation over Greenland may be, the change in the local thermodynamic environment under Arctic amplification represents a far more robust climate change signal. We also examine the thermodynamic contribution to GrIS surface mass loss using the regional climate model, Modèle Atmosphérique Régional (MAR) associated with blocking circulation. MAR output of surface temperature, meltwater production, and runoff are used to assess the differential impact of blocking events across the ice sheet.

How to cite: Preece, J., Mote, T., and Wachowicz, L.: Examining Atmospheric Dynamical Forcing of Greenland Ice Sheet Surface Mass Loss Within the Context of Arctic Amplification, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10541, https://doi.org/10.5194/egusphere-egu23-10541, 2023.

EGU23-10672 | ECS | Posters on site | CR7.3

Comparing the response to meteorological drivers at Taylor and Commonwealth glacier, McMurdo Dry Valleys, Antarctica. 

Marte Hofsteenge, Nicolas Cullen, Jono Conway, Marwan Katurji, Carleen Reijmer, and Michiel van den Broeke

In the McMurdo Dry Valleys (MDV) of Antarctica thrives a unique ecosystem under extreme cold and dry conditions. The limited snowfall that falls on the valley floor quickly sublimates and therefore glacial melt is the most important input to the streams and ice-covered lakes that provide water for the ecosystem. Understanding what drives the variability and changes in glacial meltwater is therefore of great importance to foresee ecosystem changes in a warming world. To assess the temporal variability and meteorological drivers of glacial melt in Taylor Valley, a 22-year surface energy balance (SEB) record is constructed for Taylor and Commonwealth glacier. Automatic weather station observations from the Long-term Ecological Research (LTER) Program in the ablation zone of each glacier are gap filled and completed using locally-tuned parameterisations. The two SEB records are compared to understand the different response of two nearby glaciers (~30 km apart) to local and regional climate forcing. The more melt dominated Commonwealth glacier shows strong seasonal variability in ablation. The closer proximity of Commonwealth glacier to the ocean leads to more rapid changes in albedo as controlled by summer snowfall events. Not only does the presence of snow but also the larger variability in ice albedo compared to Taylor glacier explains much of the seasonal variability in melt. Another major driver of melt are the number of degree days above freezing for both glaciers, which is strongly linked to foehn wind events in Taylor Valley. The further inland Taylor glacier experiences drier and windier conditions and therefore sublimation dominates ablation and melt occurrence. Cloud cover and snowfall in summer switch off glacial melt in summer on both glaciers. We have also used ERA5 fields to study the moisture sources of the MDV precipitation and clouds. This will help us understand how changes in moisture and regional circulation patterns might impact the MDV glaciers and ecosystem in a warming climate.

How to cite: Hofsteenge, M., Cullen, N., Conway, J., Katurji, M., Reijmer, C., and van den Broeke, M.: Comparing the response to meteorological drivers at Taylor and Commonwealth glacier, McMurdo Dry Valleys, Antarctica., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10672, https://doi.org/10.5194/egusphere-egu23-10672, 2023.

EGU23-13291 | ECS | Orals | CR7.3

Spatial response of Greenland’s firn layer to NAO variability 

Max Brils, Peter Kuipers Munneke, and Michiel van den Broeke

Changes in the Greenland ice sheet (GrIS) firn layer may impact its ability to retain meltwater. These changes also need to be accounted for when converting measured ice sheet volume changes to mass changes. With a firn model (IMAU-FDM v1.2G) forced by a regional climate model (RACMO2.3p2), we investigate how the GrIS firn layer depth and pore space have evolved since 1958 in response to variability in the large-scale atmospheric circulation. On interannual timescales, the firn layer’s depth and pore space shows a spatially heterogeneous response to variability in the North Atlantic Oscillation (NAO). Notably, a stronger NAO following the record warm summer of 2012 led the firn layer in the south and east of the ice sheet to regain thickness and pore space after a period of thinning and reduced pore space. The main driving forces behind these changes vary between GrIS sectors: in the southwest, a decrease in melt dominates, whereas in the east an increase in snow accumulation dominates. However, these trends are not uniform across the GrIS, and over the same period, the firn in the northwest continued to lose pore space. The NAO is also stronger in winter than in summer and we observe that this impacts the seasonal cycle of the firn. In the wet southeastern GrIS, most of the snow accumulates during the winter, when firn compaction is slow, amplifying the seasonal cycle in firn depth and pore space. The opposite occurs in other regions, where snowfall peaks in summer or autumn, at the same time as densification and melt, damping the seasonal oscillations in the firn thickness and pore space.

How to cite: Brils, M., Kuipers Munneke, P., and van den Broeke, M.: Spatial response of Greenland’s firn layer to NAO variability, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13291, https://doi.org/10.5194/egusphere-egu23-13291, 2023.

EGU23-13345 | Posters on site | CR7.3

Three-decades of quality controlled Greenland Climate Network (GC-Net) weather station data 

Jason Box, Baptiste Vandecrux, Andreas Ahlstrøm, Robert Fausto, William Colgan, Nanna Karlsson, Signe Andersen, Patrick Wright, Derek Houtz, Daniel McGrath, Nicolas Cullen, Nicolas Bayou, and Konrad Steffen

The Greenland Climate Network (GC-Net) is a collection of automatic weather stations (AWS)  across the Greenland Ice Sheet. The first site was initiated in 1990, and the project has operated almost continuously since 1995, under the leadership of the late Pr. Konrad Steffen. The network consists of 19 long-running weather stations, and 14 AWS sites active under five years. As part of the continuation of the GC-Net by the Geological Survey of Denmark and Greenland (GEUS), the AWS data have recently undergone a reprocessing with new attention to erroneous data filtering, correction and derivation of additional variables: continuous surface height, instrument heights, turbulent heat fluxes.  This new augmented GC-Net level 1 (L1) AWS dataset is now available at https://doi.org/10.22008/FK2/VVXGUT and will continue to be refined. The processing scripts, the latest data and a data-user forum are available at https://github.com/GEUS-Glaciology-and-Climate/GC-Net-level-1-data-processing. In addition to the AWS data, a comprehensive compilation of valuable metadata is provided: maintenance reports, yearly pictures of the stations and the moving station positions through time. This unique dataset provides more than 320 station-years of weather data of improved quality and is made available in compliance under FAIR open data and code principles.

How to cite: Box, J., Vandecrux, B., Ahlstrøm, A., Fausto, R., Colgan, W., Karlsson, N., Andersen, S., Wright, P., Houtz, D., McGrath, D., Cullen, N., Bayou, N., and Steffen, K.: Three-decades of quality controlled Greenland Climate Network (GC-Net) weather station data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13345, https://doi.org/10.5194/egusphere-egu23-13345, 2023.

EGU23-13864 | ECS | Orals | CR7.3

New non-hydrostatic polar regional climate model HCLIM-AROME: analysis of the föhn event on 27 January 2011 over the Larsen C Ice Shelf, Antarctic Peninsula 

Kristiina Verro, Willem Jan van de Berg, Andrew Orr, Oskar Landgren, and Bert van Ulft

Recently, the climate version (HCLIM) of the regional numerical weather prediction model system ALADIN–HIRLAM of the ACCORD consortium, has been set up for the Arctic and Antarctic domains. Within the PolarRES project, HCLIM will be run, along with other regional climate models such as RACMO, MetUM, and MAR, to study the interactions between the atmosphere, oceans, and sea ice in the Arctic and Antarctic. For the Antarctic Peninsula, kilometre-scale horizontal resolution and non-hydrostatic model dynamics are essential to accurately resolve the complex topography and to capture small-scale processes such as the föhn winds that occur over ice shelves on the Antarctic Peninsula. 

Here, we present an analysis of the föhn event on 27 January 2011 over the Larsen C Ice Shelf, Antarctic Peninsula. The output of the non-hydrostatic HCLIM-AROME model, run at 2.5 km resolution, is evaluated against automatic weather station and radiosonde measurements and simulations of the non-hydrostatic regional climate model MetUM. We analyse the modelled air pressure, near-surface and tropospheric temperatures, wind speed and wind direction, and other atmospheric variables, demonstrating the strengths and weaknesses of the HCLIM-AROME model for this polar application. 

How to cite: Verro, K., van de Berg, W. J., Orr, A., Landgren, O., and van Ulft, B.: New non-hydrostatic polar regional climate model HCLIM-AROME: analysis of the föhn event on 27 January 2011 over the Larsen C Ice Shelf, Antarctic Peninsula, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13864, https://doi.org/10.5194/egusphere-egu23-13864, 2023.

EGU23-14194 | ECS | Posters on site | CR7.3

The microclimate and mass balance of Qaamarujup Sermia, West Greenland 1929-2022 

Florina Schalamon, Jakob Abermann, Sebastian Scher, Andreas Trügler, and Wolfgang Schöner

Understanding the interaction of the atmosphere and cryosphere is critical for predicting the consequences of the rapidly changing climate, particularly in the Arctic. To accurately represent feedback mechanisms between ice and climate in physical models, their thorough quantification at the local scale is required. This study analyses two high-resolution datasets from the Qaamarujup Sermia outlet glacier (West Greenland) that were collected 90 years apart (1929-1931 and 2022 onward). The first is a dataset from Alfred Wegener's last expedition 1929-31, including sub-daily atmospheric observations as well as monthly to (bi-)weekly mass balance measurements. An almost identical monitoring network was installed in 2022 with the goal of observing changes in microclimate and their impact on the glacier. Both periods cover far above-normal air temperatures. The newly installed monitoring network consists of two automatic weather stations (AWS), of which one is placed near the coast and the other one on the ice sheet in approx. 940 m a.s.l.. The station network is supplemented with three temperature and humidity sensors in 50, 270 and 950 m a.s.l. . Further, there are four autonomous ablations sensors and six ablation stakes to quantify the surface mass balance of the glacier. During the field campaign in 2022, 39 vertical drone flights were performed to investigate temperature and humidity profiles of the lowest 400 m of the atmosphere. Preliminary findings show that a surface-based temperature inversion above the glacier surface is present on all days investigated during the study period (2-10.7.2022). An elevated temperature inversion above the ice-free valley part is also present at 50% of the days, with one day reaching further inland than the glacier front. Both types of inversion occur in combination on three out of the eight study days. Comparison of the historic surface mass balance with data from a regional climate model shows reasonable agreement for locations 950 m a.s.l., while the complex topography in the valley is not represented sufficiently. Our results emphasize the value of validation data on a small spatial scale as well as the potential of short-term observations almost a century apart to investigate changing feedback mechanisms of the ice/climate interaction.  

How to cite: Schalamon, F., Abermann, J., Scher, S., Trügler, A., and Schöner, W.: The microclimate and mass balance of Qaamarujup Sermia, West Greenland 1929-2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14194, https://doi.org/10.5194/egusphere-egu23-14194, 2023.

EGU23-103 | ECS | Orals | CL4.7

Energetic Constraints on Baroclinic Eddy Heat Transport in a Rotating Annulus 

Cheng Qian, Peter Read, and David Marshall

We measure baroclinic eddy heat transport in a differentially heated rotating annulus laboratory experiment to test mesoscale ocean eddy parameterization frameworks. The differentially heated rotating annulus comprises a fluid placed between two upright coaxial cylinders which are maintained at different temperatures, usually with a cooled inner cylinder and a heated outer.  The annular tank is placed on a rotating table which provides conditions for baroclinic eddies to develop and equilibrate in different flow regimes, depending upon the imposed conditions. As the rotation speed is increased, the equilibrated flow changes from a steady or periodically varying low wavenumber pattern to a more complex, time-varying flow dominated by higher wavenumbers. With a topographic beta effect produced by conically sloping upper boundary, more complex flow regimes are observed combining zonal jets and eddies forming one or more parallel storm tracks. With this possibility to explore varied flow regimes, our experimental approach combines laboratory calorimetry and visualization measurements along with numerical simulations to derive the eddy heat transport properties. In the following, we focus on the visualisation measurement to test related assumptions and parametric dependencies for eddy transport. We first test the assumptions of a down-gradient temperature flux-gradient relationship, determining coefficients of the eddy transport tensor, and exploring scaling relations for the eddy coefficients. A clear statistical scaling is found between eddy heat fluxes and physical variables such as eddy energy, the beta effect, and the temperature contrast.

How to cite: Qian, C., Read, P., and Marshall, D.: Energetic Constraints on Baroclinic Eddy Heat Transport in a Rotating Annulus, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-103, https://doi.org/10.5194/egusphere-egu23-103, 2023.

EGU23-273 | ECS | Posters virtual | CL4.7

Understanding the variability and trend of the regional Hadley Cell over Asia-Pacific 

Pratiksha Priyam Baruah and Neena Joseph Mani

The zonal mean Hadley Cell (HC) has been reported to be expanding poleward in the last few decades. However, there has been no consensus on whether the zonal mean HC is strengthening or weakening. The features of longitudinally averaged HC are collectively modulated by various regional HCs, controlled by the regional differences in land-ocean distribution and topography. However, there have not been many studies exploring the variability and trend of regional HCs in a detailed manner. In this study, we examine the variability and long-term trend of the regional HC over the Asia-Pacific and explore the different factors contributing to the regional HC variability. Moist convection can regulate regional HCs on synoptic time scales through equatorial wave dynamics. The ocean–atmosphere coupled variability associated with the El Niño-Southern Oscillation (ENSO), and the modulation of tropical convection and equatorial waves are considered to exert a dominant control on the regional HC variability in the interannual timescale. In addition to the tropical forcing, the regional HC variability is also affected by fluxes transported by the midlatitude eddies from the subtropics to the tropics. In this study, we will be quantifying the relative role of these tropical and extratropical forcings in modulating the variability of regional HC over Asia-Pacific.

 

How to cite: Baruah, P. P. and Joseph Mani, N.: Understanding the variability and trend of the regional Hadley Cell over Asia-Pacific, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-273, https://doi.org/10.5194/egusphere-egu23-273, 2023.

EGU23-972 | ECS | Posters on site | CL4.7

Vanishing the El Niño-induced delay effect on the ice mass loss of West Antarctica under global warming 

Hyunju Lee, Emilia Kyung Jin, Byeong-Hoon Kim, and Won Sang Lee

West Antarctica has been losing their ice mass due to global warming, and the El Niño has delayed the ice mass loss by inducing weakening of the Amundsen Sea Low (ASL), encouraging of poleward moisture flux and consequent extreme precipitation. However, it is not yet revealed whether the delay effect will continue in the future. We analyzed future scenarios from the CMIP6 Earth system models (ESMs) to identify future change and identified that the El Niño-driven mass increase by precipitation will vanish in the high-emission future scenarios. Precipitation anomaly in response to El Niño starts to be negative from the 2050s in the SSP5-8.5 and from the 2060s in the SSP3-7.0, which means that the El Niño-driven delay effect disappears. It is because the moisture transport into West Antarctica is prevented due to east-equatorward migration of El Niño-induced ASL anomaly as global warming intensifies. The strengthened polar jet associated with positive Southern Annular Mode (SAM) trend moves the ASL anomaly east- and equatorward under global warming.

How to cite: Lee, H., Jin, E. K., Kim, B.-H., and Lee, W. S.: Vanishing the El Niño-induced delay effect on the ice mass loss of West Antarctica under global warming, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-972, https://doi.org/10.5194/egusphere-egu23-972, 2023.

 We show that the most prominent of the work theorems, the Jarzynski equality and the Crooks relation, can be applied to the momentum transfer at the air-sea interface using a hierarchy of local models. In the more idealized models, with and without a Coriolis force, the variability is provided from a Gaussian white-noise which modifies the shear between the atmosphere and the ocean. The dynamics is Gaussian and the Jarzynski equality and Crooks relation can be obtained analytically solving stochastic differential equations. The more involved model consists of interacting atmospheric and oceanic boundary-layers, where only the dependence on the vertical direction is resolved, the turbulence is modeled through standard turbulent models and the stochasticity comes from a randomized drag coefficient. It is integrated  numerically and can give rise to a non-Gaussian dynamics. Also in this case the Jarzynski equality allows for calculating a dynamic-beta ßD of the turbulent fluctuations (the equivalent of the thermodynamic-beta  ß=(kB T)-1 in thermal fluctuations). The Crooks relation gives the ßD as a function of the magnitude of the work fluctuations. It is well defined (constant) in the Gaussian models and can show a slight variation in the  more involved models. This demonstrates that recent concepts of stochastic thermodynamics used to study micro-systems subject to thermal fluctuations can further the understanding of geophysical fluid dynamics with turbulent fluctuations.

How to cite: Wirth, A.: Jarzynski equality and Crooks relation for local models of air-sea interaction, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1066, https://doi.org/10.5194/egusphere-egu23-1066, 2023.

The Arctic is warming at a rate faster than any other oceans, a phenomenon known as Arctic amplification that has widespread impact on the global climate. In contrast, the Southern Ocean (SO) and Antarctica have been cooling over the past decades. The projection of these regions under global warming has a non-negligible model spread. Here we show that under a strong warming scenario from 1950 to 2100, comparing a cutting-edge high-resolution climate model to a low-resolution model version, the increase of Arctic amplification is 3 °C more and the SO and Antarctica warming is 2°C less. Previously ice-covered Arctic Ocean will exhibit greater SST variability under future global warming. This is due to an increased SST increase in summer due to sea ice retreat. Extreme warming events in the Arctic and SO, known as marine heat waves (MHW) that influence the ecology, are largely unknown. We find that the MHWs in the Arctic and SO are twice as strong in the high-resolution model version, where the increasing intensity of MHWs in the Arctic corresponds to strong decline (<-6% per decade) of sea ice. In both the high-resolution and low-resolution models, the duration of MHWs in the Arctic and SO shows a declining trend under global warming. The much stronger MHWs in the high-resolution model could be caused by two orders of magnitude more ocean turbulent energy. For example, the spatial patterns of SO MHW intensity correspond to the pattern of SO EKE. We conclude that the Arctic amplification and MHWs at high latitudes might be underestimated by the current generation of climate models with low resolution, and the SO and Antarctica warming might be overestimated. Our eddy- and storm-resolving model is expected to open new frontiers on how the system responds to human activities in a high CO2 world by evaluating the impact on past and future climate and environmental extremes.

How to cite: Gou, R., Lohmann, G., and Wu, L.: Increase in Arctic amplification and high-latitude marine extremes in the 21st century as obtained from high-resolution modelling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1649, https://doi.org/10.5194/egusphere-egu23-1649, 2023.

EGU23-1773 | ECS | Posters on site | CL4.7

Tropical Instability Waves in a High-Resolution Oceanic and Coupled GCM 

Li Tianyan and Yu Yongqiang

Tropical instability waves (TIWs) are the dominant mesoscale variability in the eastern equatorial Pacific Ocean. TIWs have direct impacts on the local hydrology, biochemistry and atmospheric boundary layer, and feedback on ocean circulations and climate variability. In this study, the basic characteristics of Pacific Ocean TIWs simulated by an eddy-resolving ocean model and a coupled general circulation model are evaluated. The simulated TIW biases mainly result from the mean climatology state, as TIWs extract eddy energy from the mean potential and kinetic energy. Both the oceanic and coupled models reproduce the observed westward propagating large-scale Rossby waves between approximately 2-8N, but the simulated TIWs have shorter wavelengths than the observed waves due to the shallower thermocline. Meanwhile, the weak meridional shears of background zonal currents and the less-tilted pycnocline in these two models compared to the observations causes weak barotropic and baroclinic instability, which decreases the intensity of the simulated TIWs. We then contrast the TIWs from these two models and identify the roles of atmospheric feedback in modulating TIWs. The latent heat flux feedback is similar to observation in the coupled model but absent in the ocean model, contributing to the stronger standard deviation (STD) of the TIW SST in the ocean model. The ocean model is not able to capture realistic air-sea interaction processes when forced with prescribed atmospheric forcing. However, the misrepresented atmospheric feedback in the ocean model tends to decrease the sea surface height (SSH) variability, and the current feedback damping effect is stronger in the ocean model than in the coupled model. Combined with weaker barotropic conversion rate and baroclinic conversion rate in the ocean model than in the coupled model, the STD of the TIW SSH in the ocean model is weaker.

How to cite: Tianyan, L. and Yongqiang, Y.: Tropical Instability Waves in a High-Resolution Oceanic and Coupled GCM, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1773, https://doi.org/10.5194/egusphere-egu23-1773, 2023.

EGU23-1985 | ECS | Posters on site | CL4.7

Sensitivity of ocean heat content to atmospheric forcing in the period of global warming hiatus 

Chavely Albert Fernández, Armin Köhl, and Detlef Stammer

Between 1998 and 2012, there was a smaller rate of global warming, known as the "global warming hiatus". One of the suggested causes is that during this period additional heat sequestration occurs into the deep ocean layers such that deep layers warm at a greater rate than the upper layers. This research is focused on the origins of changes in ocean heat content during the hiatus period, defined in this case as the last 10 years of adjoint model run, where the cost function is defined. Adjoint sensitivities are used to determine the influence of atmospheric forcing (heat and freshwater fluxes and wind stress) on the ocean heat content.

The MIT General Circulation Model with a resolution of 2° x 2° is used over the period 1978-2008 to determine adjoint sensitivities of the globally and temporally (over the last 10 years, defined as hiatus period) integrated vertical heat fluxes across various depth levels. The contributions of different forcing components to the vertical heat flux anomalies are obtained from the scalar product between sensitivities and the anomalies of the atmospheric forcing.  For this, the atmospheric forcing anomalies are computed with respect to the climatology calculated over the period 1948-1968 when there was almost no change in the ocean heat content.

A more pronounced increase in ocean heat uptake during the hiatus period has been evidenced by the forward run of the model. Wind anomalies represent more than half of the contribution to the increase in heat flux across 300m, suggesting that the excess of heat stored by the ocean is transferred adiabatically to the deeper layers and that the zonal wind is one of the major drivers of ocean heat uptake. In the Southern Ocean, the sensitivities to the wind stress change from positive to negative when the hiatus starts. This indicates that, during the hiatus, the rate of change of ocean heat content is opposite to the one of the wind stress. The Southern Ocean presents smaller values of the computed amplitude weighted mean time, meaning that this region has the fastest response to changes in surface atmospheric forcing.

How to cite: Albert Fernández, C., Köhl, A., and Stammer, D.: Sensitivity of ocean heat content to atmospheric forcing in the period of global warming hiatus, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1985, https://doi.org/10.5194/egusphere-egu23-1985, 2023.

 Widespread observed and projected increases in warm extremes, along with decreases in cold extremes, have been confirmed as being consistent with global and regional warming. However, based on observational datasets and state-of-the-art CMIP6 model simulations, we disclose that the decadal variation in the frequency of the surface air temperature (SAT) extremes over mid- to high latitudes over Eurasia (MHEA) in winter is primarily dominated by the thermodynamical effect of the surface heat fluxes release over the midlatitude North Atlantic induced by Atlantic multidecadal oscillation (AMO), which even masks the dynamical large-scale Rossby wave propagation. Besides, the stronger Atlantic meridional overturning circulation (AMOC) gives rise to both warm and cold extremes through increasing the variance of winter SAT over MHEA due to thermodynamical heat release and enhanced dynamical Rossby wave propagation.

How to cite: Wang, H.: Frequency of winter temperature extremes over Eurasia dominated by variabilities over the Atlantic Ocean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3106, https://doi.org/10.5194/egusphere-egu23-3106, 2023.

EGU23-3282 | ECS | Posters on site | CL4.7

Physics of the Eddy Memory Kernel of a Baroclinic Midlatitude Atmosphere 

Elian Vanderborght, Jonathan Demeayer, Henk Dijkstra, Georgy Manucharyan, and Woosok Moon

In recent theory trying to explain the origin of low-frequency atmospheric variability, the concept of eddy-memory has been suggested. In this view, the effect of synoptic scale heat fluxes on the mean flow depends on the history of the mean meridional temperature gradient. Mathematically, this involves a convolution of an integral kernel with the mean meridional temperature gradient over past times. In atmospheric studies, it has been proposed that the shape of this integral kernel is linked to the baroclinic wave life cycle. However, this hypothesis has yet to be supported by numerical and observational evidence. In this study we use a low-order two layer quasi-geostrophic atmospheric model (Demaeyer et al., 2020). By perturbing the model with a known forcing, linear response theory can be used to estimate the shape of the integral kernel. Using this methodology, we find an integral kernel that resembles the shape of an exponentially decaying oscillation, different from the simple exponentially decaying integral kernel assumed in most previous studies. By computing the energies and performing a sensitivity analysis, we link the shape of the integral kernel to atmospheric dynamical processes.

References:

J. Demaeyer, L. De Cruz, and S. Vannitsem. qgs: A flexible python framework of reduced-order multiscale climate
models. Journal of Open Source Software, 5(56):2597, 2020.

How to cite: Vanderborght, E., Demeayer, J., Dijkstra, H., Manucharyan, G., and Moon, W.: Physics of the Eddy Memory Kernel of a Baroclinic Midlatitude Atmosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3282, https://doi.org/10.5194/egusphere-egu23-3282, 2023.

EGU23-3492 | Orals | CL4.7

Variability of summer-time Arctic sea ice: the drivers and the contribution to the sea ice trend and extremes 

Mehdi Pasha Karami, Torben Koenigk, and Bruno Tremblay

Understanding the variability of summer-time Arctic sea ice at interannual to multidecadal time scales in the midst of anthropogenically forced sea ice decline is crucial for better predictions of sea ice conditions in the future climate and rapid changes in sea ice. Here, we apply time-frequency analysis to study the modes of variability, extreme events and the trend in the September Arctic sea ice in 100–150 year datasets. We extract the non-linear trend for the sea ice area and provide an estimate for the anthropogenic-driven sea ice loss. For the used dataset, the anthropogenic-related sea ice loss is found to have a rate of ~-0.25 million km2 per decade in the 1980’s and accelerating to ~-0.47 million km2 per decade in 2010’s. By assuming the same rate of sea ice loss in the future, and without the contribution of the internal variability and feedbacks, we can approximate the occurrence of summer sea-ice free Arctic to be around 2060. Regarding the dominant modes of variability for the September sea ice, we find that they have periods of around 3, 6, 17, 28 and 55 years, and show what drives these modes and how they contribute to sea ice extreme events. The main atmospheric and oceanic drivers of sea ice modes include the Arctic oscillation and Arctic dipole anomaly for the 3-year mode, variability of sea surface temperature (SST) in Gulf Stream region for the 6-year mode, decadal SST variability in the northern North Atlantic Ocean for the 17-year mode, Pacific decadal oscillation (PDO) for the 28-year mode, and Atlantic multidecadal Oscillation (AMO) for the 55-year mode. Results show that changes in the sea ice due to internal variability can be as large as forced changes thus can slow down or accelerate the background anthropogenic-driven sea ice loss. By applying the same method, we also present modes of variability and trend of sea ice in the large ensemble global model simulations of EC-Earth model (SMHI-LENS) for the future climate projections and different climate scenarios.

How to cite: Karami, M. P., Koenigk, T., and Tremblay, B.: Variability of summer-time Arctic sea ice: the drivers and the contribution to the sea ice trend and extremes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3492, https://doi.org/10.5194/egusphere-egu23-3492, 2023.

Global circulation patterns are analysed using the mean meridional circulation (MMC) from ERA-Interim for the period of 1979 – 2017. The global isentropic MMC consists of a single overturning cell in each hemisphere with net heat transport from the equator to the pole. Six clusters are identified from daily data that are associated with one of four seasons. Two solstitial MMC clusters represent either stronger or weaker circulation in the winter hemisphere. We show that long-term trends do not reflect a gradual change in the atmospheric circulation, but rather a change in the frequency of preferred short-term circulation regimes. Before the late 1990s the clusters showing a stronger (weaker) winter circulation are becoming less (more) frequent; from around year 2000 the trends have paused. These trends are in close agreement with the change in the low-stratospheric Antarctic ozone trends reported by earlier studies. Our findings also reveal a strong coupling between Southern and Northern Hemispheres during boreal winter. Following Hartmann et al. (2022), we hypothesize that anomalous polar vortex over Antarctica leads to anomalies in the sea surface temperatures (SST) in the tropical Pacific that impact the circulation in both hemispheres. Furthermore, we show that consecutive solstice season demonstrates coherent anomalies in the frequency of circulation regimes. We discuss possible reasons for such relationship.

References:
Hartmann, D. L., Kang, S., Polvani, L. & Xie, S.-P. The Antarctic ozone hole and the pattern effect on climate sensitivity. (2022) doi:10.1073/pnas.

How to cite: Rudeva, I., Boschat, G., and Lucas, C.: How can atmospheric trends be explained by changes in frequency of short-term circulation regimes and what is the role of the Antarctic ozone?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4557, https://doi.org/10.5194/egusphere-egu23-4557, 2023.

EGU23-5305 | ECS | Orals | CL4.7

Linking ITCZ migrations to the AMOC and North Atlantic/Pacific SST decadal variability 

Eduardo Moreno-Chamarro, John Marshall, and Tom L. Delworth

This contribution discusses the link between migrations in the intertropical convergence zone (ITCZ) and changes in the Atlantic meridional overturning circulation (AMOC), Atlantic multidecadal variability (AMV), and Pacific decadal oscillation (PDO). We use a coupled climate model that allows us to integrate over climate noise and assess underlying mechanisms. We use an ensemble of ten 300-yr-long simulations forced by a 50-yr oscillatory North Atlantic Oscillation (NAO)-derived surface heat flux anomaly in the North Atlantic, and a 4000-yr-long preindustrial control simulation performed with GFDL CM2.1. In both setups, an AMV phase change induced by a change in the AMOC’s cross-equatorial heat transport forces an atmospheric interhemispheric energy imbalance that is compensated by a change in the cross-equatorial atmospheric heat transport due to a meridional ITCZ shift. Such linkages occur on decadal time scales in the ensemble driven by the imposed forcing, and internally on multicentennial time scales in the control. Regional precipitation anomalies differ between the ensemble and the control for a zonally averaged ITCZ shift of similar magnitude, which suggests a dependence on timescale. Our study supports observational evidence of an AMV–ITCZ link in the twentieth century and further links it to the AMOC, whose long-time-scale variability can influence the phasing of ITCZ migrations. In contrast to the AMV, our calculations suggest that the PDO does not drive ITCZ migrations, because the PDO does not modulate the interhemispheric energy balance.

How to cite: Moreno-Chamarro, E., Marshall, J., and Delworth, T. L.: Linking ITCZ migrations to the AMOC and North Atlantic/Pacific SST decadal variability, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5305, https://doi.org/10.5194/egusphere-egu23-5305, 2023.

EGU23-5962 | Orals | CL4.7

Tropical precipitation biases in nextGEMS storm-resolving Earth System Models 

Simona Bordoni, Roberta D'Agostino, and Adrian M. Tompkins

Global Earth System Models at storm-resolving resolutions (SR-ESM, with horizontal resolutions of ~4km) are being developed as part of the nextGEMS collaborative European EU’s Horizon 2020 programme. Through breakthroughs in simulation realism, these models will eventually allow us to understand and reliably quantify how the climate will change on a global and regional scale, and how the weather, including its extreme events, will look like in the future.

As part of the Storms & Ocean theme, we are exploring how resolving convective storms, ocean mesoscale eddies, and air-sea interaction on these scales influences the development of tropical SST anomalies and their influence on the mean climate (ITCZ and circulation biases) and its variability. Existing biases in the SR-ESM simulations in the first two development cycles are interpreted using the vertically integrated atmospheric energy budget to disentangle local and remote influences on tropical precipitation. More specifically, these biases are decomposed in hemispherically symmetric and antisymmetric components, which are linked, respectively, to biases in the atmospheric net energy input near the equator (tropical SST biases, low level clouds, etc) and to the cross-equatorial atmospheric energy flux (driven by inter-hemispheric contrast in net energy input, for instance biases in clouds in the southern ocean). We also explore the role that transient eddies, both of extratropical and tropical origin that are usually neglected in this framework, play in the global energetics and tropical precipitation patterns.

How to cite: Bordoni, S., D'Agostino, R., and Tompkins, A. M.: Tropical precipitation biases in nextGEMS storm-resolving Earth System Models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5962, https://doi.org/10.5194/egusphere-egu23-5962, 2023.

    Poleward atmospheric energy transport is determined by the overall equator-to-pole radiative imbalance. As this imbalance is projected to remain fairly constant in end-of-century greenhouse gas forcing scenarios, an increase in poleward latent heat transport must be accompanied by a reduction in dry static energy flux. Since midlatitude energy transport is dominated by the eddy component, changes in the energy budget go hand in hand with changes in cyclone characteristics. From a dynamical perspective, the enhanced condensation due to climate change promotes intensification, prolongs lifetime of cyclones, and can increase stationarity of anticyclones. However, it also tends to increase static stability and thereby reduce baroclinicity, which is another important driver of cyclone development. Additionally, baroclinicity is projected to increase at upper levels due to tropical amplification, to decrease at low levels as a result of Arctic amplification, and to be affected by land-sea temperature contrast changes. As these processes are at play simultaneously, isolating the role of moisture is rather complicated. Therefore, in addition to coupled climate model simulations we use idealized aquaplanet simulations to single out the effects of individual physical mechanisms and address the question: if the overall poleward energy transport remains largely unaffected by global warming, how do cyclone characteristics change in the presence of increased moisture in the atmosphere?

    For bridging the gap between the global energy flux and synoptic-scale features, we analyse the role of increasing moisture for shaping midlatitude storm tracks in present and future climates from both an Eulerian and a Lagrangian perspective. We apply the moist static energy (MSE) framework that allows partitioning atmospheric energy fluxes into eddy and mean, dry and moist components. Here, eddies are related to cyclones and anticyclones, while the mean energy flux is associated with planetary waves and the mean meridional overturning circulation. The goal is to relate the eddy MSE fluxes to feature-based results including extratropical cyclone number, lifetime, intensity, location, and tilt. By combining results from both global-scale eddy energy fluxes and synoptic-scale feature quantities, we aim to improve the understanding of the role of latent heating in shaping the mean properties of extratropical storm tracks. Therefore, a central question of this project is whether and how changes in cyclone quantities can be linked to changes in latent heat transport and release. Building on what we learn from bringing the two perspectives together, we will proceed to investigating the impact of increased latent heating on midlatitude storm tracks. 

How to cite: Zibell, J., Schemm, S., and Hermoso Verger, A.: Combining global-scale atmospheric heat transport and synoptic-scale extratropical cyclone characteristics to understand the role of latent heating for midlatitude storm tracks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7216, https://doi.org/10.5194/egusphere-egu23-7216, 2023.

EGU23-7348 | ECS | Orals | CL4.7

An Energy Transport View of ENSO Responses to Volcanic Forcing 

Shih-Wei Fang and Claudia Timmreck

El Niño-Southern Oscillation (ENSO) is one of the major climate phenomena impacting the globe. When a volcanic eruption happens, how ENSO will respond has still no consensus in proxy data though climate models tend to have an El Niño tendency. In this study, using 100 members of diverse (in locations and magnitude) idealized volcanic forcing ensembles, we found that the ENSO responses to north and south extra-tropical eruptions are related to the energy transport to the cooling hemisphere and involve direct and indirect responses through atmospheric and oceanic transport. The north extratropical forcing leads to more El Niño up to three years after eruptions, which is related to the direct atmospheric responses of the southward movement of ITCZ for transporting more energy to the north. The indirect oceanic transport then takes over afterward, leading to more La Niña due to more upwelling in the equatorial eastern Pacific. The south extra-tropical eruptions have less El Niño tendency due to the northward replacement of ITCZ. As the indirect oceanic transport also results in equatorial mean state changes, which may lead to distinct ENSO responses. The long-term ENSO responses from extra-tropical cooling will also be investigated through the simulations from the Extratropical-Tropical Interaction Model Intercomparison Project (ETIN-MIP) experiment.

How to cite: Fang, S.-W. and Timmreck, C.: An Energy Transport View of ENSO Responses to Volcanic Forcing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7348, https://doi.org/10.5194/egusphere-egu23-7348, 2023.

EGU23-9914 | Posters on site | CL4.7

Changes in river temperature, discharge and heat flux based on new observational data for Yenisei basin and modeling 

Alexander Shiklomanov, Richard Lammers, Alexander Prusevich, Irina Panyushkina, and David Meko

River temperature plays an important role in numerous biological and ecological processes within the Yenisei River basin and it is very sensitive to changes in climatic characteristics and anthropogenic disturbances. Water temperature and river discharge characterize heat or energy flux, which is important in northern latitudes for river freeze-up and ice break-up processes and thermal riverbank erosion. The changes in heat flux in river estuary can also significantly impact various biophysical processes in coastal ocean waters.

We use new water temperature data and river discharge records for 12 observational gauges in the Yenisei River basin to analyze changes in water temperature and heat flux from upstream to downstream over 1950-2018. Preliminary results show significant increases for most gauges in maximum annual water temperature as well as in 10-days mean water temperature during May-June and September-October. There were no significant changes in river temperature during July-August unless the gauges were impacted by reservoir regulations. The river heat flux has significantly increased in central and northern parts of the Yenisei basin and decreased in the south, mainly due to discharge variability.

The gridded hydrological Water Balance Model (WBM) developed at the University of New Hampshire, that takes into account various anthropogenic activities, was used to simulate river discharge and water temperature for entire Yenisei basin with a 5 minute spatial resolution river network using several climate reanalysis products (MERRA2, ERA5 and NCEP-NCAR).  The modeled results were verified with observational data and simulations using the MERRA2 climate drivers demonstrated the best match with observations (Nash-Sutcliffe model efficiencies coefficients were greater than 0.5 for both river temperature and discharge). Maps of modeled changes in runoff, river temperature and heat flux show the opposite changes in the southern and northern parts of Yenisei basin. The model simulations correspond well with observational data even for heavily disturbed river reaches. For example, they show unfrozen water with positive temperatures during the winter below large dams and reservoirs.       

The WBM was also applied to project changes in water temperature, discharge and heat flux up to 2100 for several SSPs and GCMs from CMIP6. In spite of heterogenous projected changes in these parameters across Yenisei basin, significant increases in discharge and heat flux to the Arctic Ocean are expected.

How to cite: Shiklomanov, A., Lammers, R., Prusevich, A., Panyushkina, I., and Meko, D.: Changes in river temperature, discharge and heat flux based on new observational data for Yenisei basin and modeling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9914, https://doi.org/10.5194/egusphere-egu23-9914, 2023.

EGU23-11159 | ECS | Orals | CL4.7

Causal model evaluation of Arctic-midlatitude process during the boreal cold season in CMIP6 

Evgenia Galytska, Katja Weigel, Dörthe Handorf, Ralf Jaiser, Raphael Köhler, Jakob Runge, and Veronika Eyring

Linked to increased sea ice loss, the Arctic region has warmed at least four times faster than the global average over the past 40 years. Mutual links between amplified Arctic warming with changes and variability in midlatitude weather have been discussed in several studies. Nevertheless, the lack of consistent conclusions between observations and model simulations obfuscates the interpretation behind the mechanisms of Arctic-midlatitude teleconnections. To contribute to the understanding of Arctic-midlatitude connections that occur in conditions of amplified Arctic warming, we applied causal discovery to analyse causal and contemporaneous links. Initially, we calculated causal dependencies for monthly mean ERA5 reanalysis data from the European Centre for Medium-Range Weather Forecasts (ECMWF) and Hadley Centre Sea Ice and Sea Surface Temperature among local and remote processes. Then, by comparing causal graphs detected in reanalyses data with a number of climate model historical simulations from the Coupled Model Intercomparison Project Phase 6 (CMIP6), we assessed the performance of climate models and evaluated the robustness of the observed Arctic-midlatitude connections in the current climate. By comparing causal graphs from the CMIP6 historical and Scenario Model Intercomparison Project (ScenarioMIP) we estimated future changes in Arctic-midlatitude teleconnections towards the end of the century. In this study, we focus on the differences in the mechanism of Arctic-midlatitude teleconnections that occur during the boreal cold season, i.e. early winter (October-November-December), winter (December-January-February), and late winter (January-February-March). In this study, we will present the major findings of Galytska et al., 2022 discussing how causal model evaluation helps to summarize major differences between causal interdependencies detected in observations and simulated by a number of climate models. Understanding these differences can be the basis for further improvement of the representation of Arctic-midlatitude teleconnections in climate models.

References. 

Evgenia Galytska, Katja Weigel, Dörthe Handorf, Ralf Jaiser, Raphael Köhler, Jakob Runge, and Veronika Eyring. Causal model evaluation of Arctic-midlatitude teleconnections in CMIP6. Authorea. October 06, 2022. DOI: 10.1002/essoar.10512569.1

 

How to cite: Galytska, E., Weigel, K., Handorf, D., Jaiser, R., Köhler, R., Runge, J., and Eyring, V.: Causal model evaluation of Arctic-midlatitude process during the boreal cold season in CMIP6, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11159, https://doi.org/10.5194/egusphere-egu23-11159, 2023.

EGU23-12377 | ECS | Posters on site | CL4.7

Thermodynamic assessment of simulations of the last deglaciation with an Earth system model of intermediate complexity 

Muriel Racky, Irene Trombini, Klaus Pfeilsticker, Nils Weitzel, and Kira Rehfeld

As we observe and expect severe changes in the Earth’ climate, the analyses of past climate state transitions is of major value for improving our Earth system understanding. Under this objective, the last deglaciation (~ 21 ka to 9 ka before present), the transition from the Last Glacial Maximum (LGM) to the Holocene, is an ideal case study. During this transition, the orbital configuration gradually changed and greenhouse gases have risen, which caused a sharp decline in northern hemisphere ice sheets and an increase in the global mean surface temperature.

We create an ensemble of deglaciation simulations with a modified version of the Planet Simulator, an Earth system model of intermediate complexity (EMIC). We produce single and combined forcing simulations for further investigation from a thermodynamic perspective. The response to the transiently changing radiative forcing is investigated in terms of energy and entropy budgets of the atmosphere. Here, we focus on the deglacial evolution of the material entropy production (MEP). Its contributions represent the strength of major climate features such as the kinetic energy generation rate, vertical and horizontal heat transport and the hydrological cycle. Preliminary results show an increase of the global mean MEP from the LGM to the Holocene because of a strengthening of the hydrological contribution. In contrast, the relative importance of kinetic energy dissipation and turbulent heat diffusion in the boundary layer decrease. Our work can provide the basis for investigating the MEP as a diagnostic quantity with other models and for other climate state transitions.

How to cite: Racky, M., Trombini, I., Pfeilsticker, K., Weitzel, N., and Rehfeld, K.: Thermodynamic assessment of simulations of the last deglaciation with an Earth system model of intermediate complexity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12377, https://doi.org/10.5194/egusphere-egu23-12377, 2023.

EGU23-12939 | Orals | CL4.7

The contribution of Arctic marine heatwaves to the minimum sea ice extent as compound events 

Armineh Barkhordarian, David Nielsen, and Johanna Baehr

On the global scale, the frequency of marine heatwaves (MHWs) is projected to increase further in the twenty-first Century. In our earlier study we demonstrate that the high-impact major marine heatwaves over the northeast Pacific are co-located with a systematically-forced long-term warming pool, which we attribute to forcing by elevated greenhouse gases levels (GHG), and the recent industrial aerosol-load decrease (Barkhordarian et al., 2022).  In current study we show that the magnitude of Arctic MHWs has significantly increased since 2006, and has exceeded the pre-industrial climate bounds since then. We here perform statistical attribution methodologies, and provide a quantitative assessment of whether GHG forcing was necessary for the Arctic MHWs to occur, and whether it is a sufficient cause for such events to continue to repeatedly occur in the future.

The probability of necessary causation of Arctic MHWs intensity, increases with increasing the severity of MHWs, and saturate to 1.0 by the time MHWs intensity exceeds the 2°C, indicating that any MHWs over the Arctic with an intensity higher than 2°C is entirely attributable to the inclusion of GHG forcing. These amplified extreme MHWs in the Arctic have each been accompanied by a record decline in Arctic Sea ice, in particular in the years 2007, 2012, 2016 and 2020. Over the last decade, MHWs occur in the Arctic where sea ice melt in June is 4 %/year faster, the ice-free season is ~3 months longer, the ocean heat-uptake is 50 W/m2 higher, and the sea surface temperature is ~2°C warmer, in comparison with the previous decade. In autumn surface evaporation rate is increasing, the increased low clouds favor more sea ice melt via emitting stronger longwave radiation. In summary, prolonged Arctic marine heatwaves, triggered by faster early summer sea ice melt, will accelerate Arctic warming, and cause Arctic Sea ice extent to shrink even faster in the near future.

Barkhordarian, A., Nielsen, D.M. & Baehr, J. Recent marine heatwaves in the North Pacific warming pool can be attributed to rising atmospheric levels of greenhouse gases. Nature Communications Earth & Environment, 3, 131 (2022). https://doi.org/10.1038/s43247-022-00461-2

 

How to cite: Barkhordarian, A., Nielsen, D., and Baehr, J.: The contribution of Arctic marine heatwaves to the minimum sea ice extent as compound events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12939, https://doi.org/10.5194/egusphere-egu23-12939, 2023.

EGU23-13091 | Posters on site | CL4.7

Emergent constraints on the future Arctic lapse-rate feedback 

Olivia Linke, Nicole Feldl, and Johannes Quaas

Arctic amplification (AA) is largely attributed to the effect of sea ice decline leading to greater surface solar absorption and further ice melt, and the vertical structure of the warming. The latter aspect evokes the positive lapse-rate feedback (LRF), which is commonly understood as an effect of stable stratification: The warming in the Arctic is particularly strong close to the surface, but muted aloft. This limits the outgoing long-wave radiative flux at the top-of-the-atmosphere (TOA) relative to vertically uniform warming.

We estimate the future Arctic LRF in 43 global climate models (GCMs) from the highest emission pathway SSP5 of CMIP6. The GCMs simulate a large spread of future AA (2-8 K above global warming) and Arctic LRF (1-4 K warming contribution) at the end of the century 2070-2099. Our work aims to identify emerging relationships between this spread and observable aspects of the current climate to ultimately narrow down the range of future Arctic climate predictions.

Previous studies have identified an emerging relationship for the surface-albedo feedback based on the observed seasonal cycle of Arctic sea ice. We similarly derive a positive relationship (r=0.70) between future and seasonal LRF, but due to its nature, no direct observation of the LRF exists. However, we find relationships between the future LRF and observable sea ice metrics, namely sea ice concentration, seasonality, extent and area. From these relationships, the sea ice concentration provides the strongest correlation (r=-0.76) for the area-averaged Arctic sea ice cover. This relationship implies a contribution of the LRF to future Arctic warming of approx. 2 K, which further relates to an AA of 4 K above global average at the end of the century.

We further emphasise the physical meaning behind our constraint: The negative emerging relationship implies that models with a lower Pan-Arctic sea ice concentration produce a larger LRF in the future. However, when dividing the entire sea ice area into regions of sea ice retreat (SIR) and persisting sea ice (PSI) in the future prediction, the relationship becomes positive over these two area-averaged regions. Thereby, the negative overall relationship is merely a result of the area-size distribution of SIR vs. PSI across the spread of model simulations. We conclude that while the Pan-Arctic perspective enables the emergent constraint, the physical meaning is hidden: A higher initial sea ice concentration produces a stronger positive Arctic LRF by setting the stage for greater sea ice retreat.

How to cite: Linke, O., Feldl, N., and Quaas, J.: Emergent constraints on the future Arctic lapse-rate feedback, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13091, https://doi.org/10.5194/egusphere-egu23-13091, 2023.

EGU23-14141 | Orals | CL4.7

Underestimation of Arctic warming trends in sub-seasonal forecasts 

Steffen Tietsche, Frederic Vitart, Michael Mayer, Antje Weisheimer, and Magdalena Balmaseda

The Arctic has warmed substantially over the last decades and will continue to do so owing to global warming in conjunction with polar amplification. The changing mean state poses many challenges to the construction, evaluation and calibration of subseasonal-to-seasonal forecasting systems, because it puts into question the representativeness of the system's retrospective forecasts (reforecasts). Furthermore, any inconsistencies with observed trends degrade the forecast skill and point to deficiencies in either the physical modelling or the initialization methods. Here, we assess the consistency of boreal winter trends of surface air temperature (SAT) in the Eurasian Arctic between the ERA5 reanalysis and ECMWF sub-seasonal reforecasts initialised from ERA5, for the 35-year period 1986-2021. We present methods to quantify robustness and importance of the observed trends, and to quantify the consistency of reforecast trends with these observed trends. We find that, in large parts of the marine Arctic, the reforecasts clearly underestimate the reanalsyis warming trend of about 1 K per decade at lead times beyond two weeks. For longer lead times, the reforecast trend is less than half of the reanalysis trend, with very high statistical significance. We present a series of numerical experiments to investigate potential reasons for the trend underestimation. These concern the sea-ice thermodynamic coupling to the atmosphere, impact of sea surface temperatures, and possible remote atmospheric influences from the North Atlantic and the Tropics. The outcome of these experiments provides guidance for future improvements in the physical forecast model and data assimilation methods needed to faithfully represent and predict Arctic climate variability and change.

How to cite: Tietsche, S., Vitart, F., Mayer, M., Weisheimer, A., and Balmaseda, M.: Underestimation of Arctic warming trends in sub-seasonal forecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14141, https://doi.org/10.5194/egusphere-egu23-14141, 2023.

EGU23-14470 | Posters on site | CL4.7

A first look at the new PolarRES ensemble of polar regional climate model storylines to 2100 

Ruth Mottram, Priscilla Mooney, and Jose Abraham Torres and the PolarRES Consortium

The Horizon 2020 project PolarRES is coordinating a large international consortium of regional climate modelling groups in building a new ensemble of regional climate projections out to 2100. The ensemble is built at very high resolution (~12km) and using common domains, and set-ups to give directly comparable model outputs. At the same time, all regional climate models have been upgraded to a next-generation set-up, producing an ensemble of unprecedented sophistication.

We use a storyline approach, focused on Arctic amplification and cyclones in the northern hemisphere and Southern Annular Mode variability in Antarctica, to select global climate models for forcing on the boundaries. Each regional climate modelling group will downscale ERA5 and multiple global climate models. The data produced from these simulations will be used to improve process understanding under present and future conditions as well as to identify impacts of climate change in the polar regions.

Here, we present the experimental protocol developed in PolarRES and give details of the different regional climate models used, their setup, processes and domains as well as an overview of the outputs and planned applications. We show preliminary analysis of hindcast outputs to assess the performance of the ensemble. We invite other regional climate modelling groups outside the PolarRES consortium to consider using the same CORDEX -compatible model set-up and we are happy to receive suggestions of further spin-off studies or requests for collaboration.

 

How to cite: Mottram, R., Mooney, P., and Torres, J. A. and the PolarRES Consortium: A first look at the new PolarRES ensemble of polar regional climate model storylines to 2100, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14470, https://doi.org/10.5194/egusphere-egu23-14470, 2023.

EGU23-15746 | Orals | CL4.7

Simulating oceanic mesoscale eddy dynamics: A comparison of novel parameterizations and energy diagnostics and their impact on the global ocean circulation 

Stephan Juricke, Sergey Danilov, Marcel Oliver, Anton Kutsenko, and Kai Bellinghausen

In this study, we present a variety of parameterizations for simulating ocean eddy dynamics including novel viscous and kinetic energy backscatter closures. Their effect is analyzed using new diagnostics that allow for application on unstructured meshes.

Ocean mesoscale eddy dynamics play a crucial role for large-scale ocean currents as well as for the variability in the ocean and climate. The interactions between eddies and the mean flow affect strength, position and variations of ocean currents. Mesoscale eddies have a substantial impact on oceanic heat transport and the coupling between the atmosphere and ocean. However, at so-called eddy-permitting model resolutions around ¼°, eddy kinetic energy and variability is often substantially underestimated due to excessive dissipation of energy. Despite ever-increasing model resolutions, eddy-permitting simulations will still be used in uncoupled and coupled climate and Earth system simulations for years to come.

To improve the presentation of eddy dynamics in such resolution regimes, we present and systematically compare a set of viscous and kinetic energy backscatter parameterization with different complexity. These schemes are implemented in the unstructured grid, finite volume ocean model FESOM2 and tested in both idealized channel and global ocean simulations. We show that kinetic energy backscatter and adjusted viscosity parameterizations can alleviate some of the substantial eddy related biases, for example biases in sea surface height variability, mean currents and in water mass properties. We then further analyze the effect of these schemes on energy and dissipation spectra using new diagnostics that can be extended to the unstructured grid used by FESOM2. The rigorous intercomparison allows to make informed decisions on which schemes are the most suitable for a given application, considering the complexity of the schemes, their computational costs, their adaptability to various model resolutions and any simulation improvements related to a specific scheme. We will show that novel viscous and kinetic energy backscatter schemes outperform previously used, classical viscous closures. Furthermore, when compared to higher resolution simulations, they are computationally less expensive but achieve similar results.

How to cite: Juricke, S., Danilov, S., Oliver, M., Kutsenko, A., and Bellinghausen, K.: Simulating oceanic mesoscale eddy dynamics: A comparison of novel parameterizations and energy diagnostics and their impact on the global ocean circulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15746, https://doi.org/10.5194/egusphere-egu23-15746, 2023.

EGU23-382 | ECS | Orals | NP1.2

Latent Dirichlet Allocation: a new machine learning tool to evaluate CMIP6 climate models atmospheric circulation and extremes 

Nemo Malhomme, Bérengère Podvin, Davide Faranda, and Lionel Mathelin

Climate models aim at representing as closely as possible the statistical properties of the climate components, including the extreme events. This is a fundamental requirement to correctly project changes in their dynamics due to anthropogenic forcing. In order to evaluate how closely models match observations, we need algorithms capable of selecting, processing and evaluating relevant dynamical features of the climate components. This has to be reiterated efficiently for large datasets such as those issued from the Coupled Model Intercomparison Project 6 (CMIP6). In this work, we use Latent Dirichlet Allocation (LDA), a statistical learning method initially designed for natural language processing, to extract synoptic patterns from sea-level pressure data and evaluate how close the dynamics of CMIP6 climate models are to the state-of-the-art reanalyses datasets such as ERA5 or NCEPv2, in general as well as in the case of extremes.

LDA allows for learning a basis of decomposition of maps into objects called "motifs". Applying it to sea-level pressure data, reanalysis or simulation, robustly yields motifs that are known relevant synoptic objects, i.e. cyclones or anticyclones. Furthermore, LDA provides their weight in each of the maps of the dataset, their most probable geographical position and their possible changes due to internal variability or external forcings. LDA decomposition is efficient and sparse, most of the information of a given sea-level pressure map is contained in few motifs, making it possible to decompose any map in a limited number of easy-to-interpret synoptic objects. This allows for a variety of new angles for statistical analysis.

We look at the dominant motifs and their distributions either on entire datasets or conditionally to particular extreme events, such as cold or heat waves, and compare results between reanalysis data and historical simulations. This enables us to assess which models can or cannot reproduce statistical properties of the observations, and whether or not there are properties that no model yet demonstrates. We find that models can capture the statistical synoptic composition of sea-level pressure data in general, but that some drawbacks still exist in the modelling of extreme events. LDA can also be applied separately to each dataset, and the two resulting synoptic bases can be compared. We find the sets of motifs from reanalysis and historical simulations are very similar, even if different spatial resolutions are used.

How to cite: Malhomme, N., Podvin, B., Faranda, D., and Mathelin, L.: Latent Dirichlet Allocation: a new machine learning tool to evaluate CMIP6 climate models atmospheric circulation and extremes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-382, https://doi.org/10.5194/egusphere-egu23-382, 2023.

EGU23-483 | ECS | Posters virtual | NP1.2

Characteristics of Medicanes using ERA-5 reanalysis 

Jesús Gutiérrez-Fernández, Mario Marcello Miglietta, Juan Jesús González-Alemán, and Miguel Ángel Gaertner

Several Medicanes, which have been previously analyzed in the literature, have been studied using ERA-5 reanalyses to identify the environment in which they develop and possibly distinguish tropical-like cyclones from warm seclusions. Initially, the cyclone phase space was analyzed to identify changes in the environmental characteristics. Subsequently, the temporal evolution of several parameters was considered, including sea surface fluxes, CAPE, coupling index, potential intensity, baroclinicity.

Although the results are not consistent for all cyclones, some general characteristics can be identified: cyclones develop in areas of moderate-to-high baroclinicity associated with intense jet streams, while in the mature stage the environment becomes less baroclinic. A general reduction in the horizontal extent of the cyclone can be observed as the cyclones begin to show a shallow warm core. In this phase a progressive reduction of the CAPE can be observed in proximity of the cyclone center. Finally, the wind speed appears strongly underestimated compared to the observations, raising some concerns about the applicability of ERA-5 for the detection of wind features.

How to cite: Gutiérrez-Fernández, J., Miglietta, M. M., González-Alemán, J. J., and Gaertner, M. Á.: Characteristics of Medicanes using ERA-5 reanalysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-483, https://doi.org/10.5194/egusphere-egu23-483, 2023.

EGU23-1388 | ECS | Orals | NP1.2

Extreme events in multiscale systems: theory and applications 

Tommaso Alberti

Many geophysical systems show emergent phenomena and extreme events at different scales, with signatures of chaos at large scales and an apparently random behavior at small scales. Despite the intrinsic morphological and/or physical difference between geophysical extremes, they all originate as temporary deviations from the typical trajectories of the large scale geophysical flows, resulting in dynamical patterns and structures. This motivated to bring together statistics (extreme value theory) and dynamics (dynamical system theory) to provide a new definition of extremes as rare recurrences in the phase space of physical systems. This means to explore the instantaneous properties of the geometrical object hosting the frequency and probability of all physical states attainable by the system, namely the so-called attractor, to inform us on the predictability, persistence and synchronization of physical states.

 

Here we present a recently proposed formalism to explore the active number of degrees of freedom and the predictability horizon of multiscale complex systems showing non-hyperbolic chaos, randomness, state-dependent persistence and predictability. We briefly discuss the newly introduced framework in comparison with classical approaches, based on generalized fractal dimensions, Lyapunov exponents, and Renyi entropies. Finally, we demonstrate the suitability of this novel formalism to trace the instantaneous scale-dependent and state-dependent features of climate and geophysical extremes, pointing out how the predictability horizon, the persistence and synchronization of geophysical systems’ states is a matter of scales.

How to cite: Alberti, T.: Extreme events in multiscale systems: theory and applications, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1388, https://doi.org/10.5194/egusphere-egu23-1388, 2023.

EGU23-1555 | ECS | Posters on site | NP1.2

Drought impact-based forecasting: Trade-offs between indicators and impacts 

Anastasiya Shyrokaya, Giuliano Di Baldassarre, Hannah Cloke, Gabriele Messori, Florian Pappenberger, and Ilias Pechlivanidis

Despite the progress in seasonal drought forecasting, it remains challenging to identify suitable drought indices for accurately predicting the impacts of a future drought event. In this study, we identified relationships across Europe between the forecasting skill of various drought indices and the estimated drought impacts. We calculated the indices over various accumulation periods, and assessed the forecasting skill of indices computed based on various seasonal prediction systems. An evaluation was performed by computing the same indices from the ERA5 reanalysis data and comparing them across various verification metrics. We further conducted a literature review of the studies assessing the performance of the indices in terms of estimating drought impacts across Europe. We finally performed a trade-off analysis and mapped the drought indices based on their drought forecasting and drought impact estimating skills.

Overall, this analysis is a step forward to detect the most suitable drought indices for predicting drought impacts across Europe. Here, not only we present a new approach for evaluating the relationship between drought indices and impacts, we also resolve the dilemma of choosing the indices to be incorporated in the impact functions. Such scientific advancements are setting significant contributions to the emerging field of operational impact-based forecasting and operational drought early warning services.

How to cite: Shyrokaya, A., Di Baldassarre, G., Cloke, H., Messori, G., Pappenberger, F., and Pechlivanidis, I.: Drought impact-based forecasting: Trade-offs between indicators and impacts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1555, https://doi.org/10.5194/egusphere-egu23-1555, 2023.

EGU23-2146 | ECS | Posters on site | NP1.2

Contrasting Deep and Shallow Arctic Warming Events on the Intraseasonal Time Scale in Boreal Winter 

Juncong Li, Xiaodan Chen, Yuanyuan Guo, and Zhiping Wen

The vertical structure of Arctic warming is of great importance and attracts increasing attention. This study defines two types of Arctic warming events (viz., deep versus shallow) according to their temperature profiles averaged over the Barents-Kara Seas (BKS), and thereupon compares their characteristics and examines their difference in generation through thermodynamic diagnoses. The deep Arctic warming event—characterized by significant bottom-heavy warming extending from the surface into the middle-to-upper troposphere—emanates from the east of Greenland and then moves downstream towards the BKS primarily through zonal temperature advection. The peak day of deep warming event lags that of the precipitation and resultant diabatic heating over Southeast Greenland by about four days, suggesting that the middle-to-high tropospheric BKS warming is likely triggered by the enhanced upstream convection at the North Atlantic high latitudes. In contrast, the shallow warming event—manifested by warming confined within the lower troposphere—is preceded by the meridional advection of warm air from inland Eurasia. These anomalous southerlies over Eurasian lands during shallow warming events are related to the eastward extension of deepened Icelandic Low. Whereas during deep warming events, the in-situ reinforcement of Icelandic Low favors abundant moisture transport interplaying with the Southeast Greenland terrain, leading to intense precipitation and latent heat release there. Both deep and shallow warming events are accompanied by Eurasian cooling, but the corresponding cooling of deep warming event is profoundly stronger. Further, intraseasonal deep Arctic warming events could explain nearly half of the winter-mean change in warm Arctic-cold Eurasia anomaly.

How to cite: Li, J., Chen, X., Guo, Y., and Wen, Z.: Contrasting Deep and Shallow Arctic Warming Events on the Intraseasonal Time Scale in Boreal Winter, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2146, https://doi.org/10.5194/egusphere-egu23-2146, 2023.

EGU23-2242 | ECS | Posters on site | NP1.2

A Quantile Generalised Additive Approach for Compound Climate Extremes: Pan-Atlantic Extremes as a Case Study 

Leonardo Olivetti, Gabriele Messori, and Shaobo Jin

We present an application of quantile generalised additive models (QGAMs) to study the rela-
tionship between spatially compounding climate extremes - namely extremes that occur (near-)
simultaneously in geographically remote regions. We take as example wintertime cold spells
in North America and co-occurring wet or windy surface weather extremes in Western Europe,
which we collectively term Pan-Atlantic compound extremes. QGAMS are largely novel in cli-
mate science applications and present three key advantages over conventional statistical models
of weather extremes:


1. they do not require a direct identification and parametrisation of the extremes themselves,
since they model all quantiles of the distributions of interest;
2. they do not require any a priori knowledge of the functional relationship between the predic-
tors and the dependent variable;
3. they make use of all information available, and not only of a small number of extreme values.


Here, we use QGAMs to both characterise the co-occurrence statistics and investigate possible
dynamical drivers of the Pan-Atlantic compound extremes. We find that recent cold spells in
North America are a useful predictor of upcoming near-surface extremes in Western Europe,
and that QGAMs can predict those extremes more accurately than conventional peak-over-
threshold models.

How to cite: Olivetti, L., Messori, G., and Jin, S.: A Quantile Generalised Additive Approach for Compound Climate Extremes: Pan-Atlantic Extremes as a Case Study, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2242, https://doi.org/10.5194/egusphere-egu23-2242, 2023.

EGU23-2644 | ECS | Posters on site | NP1.2

Investigating the typicality of the dynamics leading to extreme temperatures in the IPSL-CM6A-LR model 

Robin Noyelle, Pascal Yiou, and Davide Faranda

Understanding the physical mechanisms leading to extremes of quantities of interest in dynamical systems remains a challenge. Under mild hypothesis, the application of the theory of large deviations to dynamical systems predicts the convergence of trajectories leading to extremes towards a typical, i.e. most probable, one called the instanton. In this paper, we use a 2000 years long simulation of the IPSL-CM6A-LR model under a stationary pre-industrial climate to test this prediction. We investigate the convergence properties of trajectories leading to extreme temperatures at four locations in Europe for several variables. We show the convergence of trajectories for most physical variables, with some geographical and temporal discrepancies. Our results are coherent with the most probable path prediction and suggest that the instanton dynamics leading to extremes is a relevant feature of climate models.

How to cite: Noyelle, R., Yiou, P., and Faranda, D.: Investigating the typicality of the dynamics leading to extreme temperatures in the IPSL-CM6A-LR model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2644, https://doi.org/10.5194/egusphere-egu23-2644, 2023.

EGU23-3300 | Posters on site | NP1.2

Simulating the West Pacific Heatwave of 2021 with Analog Importance Samping 

Flavio Pons, Pascal Yiou, and Aglae Jezequel

During the summer of 2021, the North American Pacific Northwest was affected by an extreme heatwave that broke previous temperature records by several degrees and lasted almost two months after the initial peak. The event caused severe impacts on human life and ecosystems, and was associated with the superposition of concurrent extreme drivers, whose effects were amplified by climate change. We evaluate whether this record-breaking heatwave could be anticipated prior to 2021, and how climate change affects North American Pacific Northwest worst case heatwave scenarios. We use a stochastic weather generator  with empirical importance sampling. The generator simulates temperature sequences with realistic statistics using circulation analogues, chosen with an importance sampling based on the daily maximum temperature over the region that recorded the most extreme impacts. We show how some of the large-scale drivers of the event can be obtained form the circulation analogues, even if such information is not directly given to the stochastic weather generator.

How to cite: Pons, F., Yiou, P., and Jezequel, A.: Simulating the West Pacific Heatwave of 2021 with Analog Importance Samping, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3300, https://doi.org/10.5194/egusphere-egu23-3300, 2023.

EGU23-4216 | ECS | Orals | NP1.2

Large-scale perspective on the extreme near-surface winds in the central North Atlantic 

Aleksa Stanković, Rodrigo Caballero, and Gabriele Messori

This study investigates winter cyclones that cause extreme 10 m winds in the central North Atlantic region (30o to 60latitude, -50o to -10o longitude) in the ERA5 dataset. We employ a bottom-up approach consisting of selection of the extreme 10 m wind events and analysis of the cyclones that caused the extremes.

The 10 m wind extremes were ranked using the Klawa and Ulbrich (2003) destructiveness index, which takes into account wind exceedances over the local 98th percentiles. The top 1% of destructive events were chosen for further analysis. Cyclones were associated with the extreme winds by finding the closest sea-level pressure lows at the times of maximum wind speeds.

By analyzing various meteorological fields associated with the temporal evolution of the selected cyclones, we find an important role of interactions with other pre-existing cyclones that create suitable conditions for the development of the subsequent extreme windstorms.  

How to cite: Stanković, A., Caballero, R., and Messori, G.: Large-scale perspective on the extreme near-surface winds in the central North Atlantic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4216, https://doi.org/10.5194/egusphere-egu23-4216, 2023.

EGU23-5515 | ECS | Orals | NP1.2

Estimating non-linear persistence for impact assessment in European forests 

Tristan Williams, Miguel D. Mahecha, and Gustau Camps-Valls

Persistence is an important characteristic of many complex systems in nature and of the Earth system in particular. Relating this statistical concept to physical properties of ecosystems is rather elusive, but reflects how long the system remains at a certain state before changing to a different one and is measured via the memory and dependence of values on past states [1]. Characterizing persistence in the terrestrial biosphere is very relevant to understand intrinsic properties of the system such as legacy effects of extreme climate events [2]. Such memory effects are often highly non-linear and therefore challenging to detect in observational records and poorly represented in Earth system models. This study estimates long and short-term non-linear persistence in eddy-covariance flux measurements and remote sensing products in European forests and the corresponding hydro-meteorological data. Characterizing persistence in the data allows us to make inferences on the interaction between Drought-Heat events, forest dynamics, and ecosystem resilience [3]. The comparison of in-situ and Earth Observation (EO) data allows us to infer how meaningful EO data are for monitoring complex dynamics in ecosystems.

For short-term, spatio-temporal persistence, we use echo state networks using the technique suggested in [4] as an explainable AI (XAI) technique. In this context, the persistence of the system can be estimated by the model's response when the input fades abruptly. For the characterization of long-term persistence, we introduce a novel kernel extension of the well-established Detrended Fluctuation Analysis (DFA) [5], a method widely used in atmospheric sciences [1]. The DFA method is a scaling analysis that provides a simple quantitative parameter (the scaling exponent) to represent the correlation properties of a signal and a characteristic time of the event of interest. Unlike DFA, the proposed kernel DFA method can handle non-linear time-scales interactions. 

Estimating the non-linear persistence of forests and climate data allows us to relate characteristic times, crossover points between different scaling exponents, and short-term memory parameters with the duration and intensity of the events, as well as an indicator of change in the vegetation response to hydro-climatic conditions.

 

[1] Salcedo-Sanz, S., et al. “Persistence in complex systems”. Physics Reports 957, 1-73, (2022).

[2] Bastos, Ana, et al. “Direct and seasonal legacy effects of the 2018 heat wave and drought on European ecosystem productivity." Science advances 6.24 (2020)

[3] Scheffer, M., Carpenter, S. R., Dakos, V. & van Nes, E. H. Generic indicators of ecological resilience: inferring the chance of a critical transition. Annu. Rev. Ecol. Evol. Syst. 46, 145–167 (2015).

[4] Barredo Arrieta, A., Gil-Lopez, S., Laña, I. et al. On the post-hoc explainability of deep echo state networks for time series forecasting, image and video classification. Neural Comput & Applic 34, 10257–10277 (2022).

[5] Peng, C‐K., et al. "Quantification of scaling exponents and crossover phenomena in nonstationary heartbeat time series." Chaos: an interdisciplinary journal of nonlinear science 5.1 (1995): 82-87.

How to cite: Williams, T., Mahecha, M. D., and Camps-Valls, G.: Estimating non-linear persistence for impact assessment in European forests, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5515, https://doi.org/10.5194/egusphere-egu23-5515, 2023.

Atmospheric blocking can be described as a large-scale stationary or quasi-stationary circulation anomaly that blocks the mean westerlies. Blocking often triggers extreme temperature events like heat waves or cold spells. However, dynamical processes leading to the formation, maintenance, and decay mechanisms of blocking are still not well understood.

Moist processes have recently been proven to play a significant role in the formation and maintenance of blocking. However, it is unclear if moist processes generate special properties in the blocking life cycle that cannot be represented by dry dynamics or if they are just there to inject extra energy into the atmospheric disturbances. The following is the question we address in the present study: Is a dry dynamical model with climatology close to the observations capable of representing blocking characteristics correctly? The methodology relies on numerical experiments made with the new IPSL dynamical core called DYNAMICO, which enables high spatial resolutions. DYNAMICO is used here to analyze a long-term simulation in which the model forcing is designed to obtain a realistic climatology for a given season (perpetual winter in the present case). Blocking statistics like frequency of occurrence and duration are provided using two blocking detection algorithms and compared to the re-analysis dataset (ERA5). A focus is made on blocking onsets in the Euro-Atlantic sector. To highlight the differences in the processes leading to blocking onsets, backward Lagrangian trajectories seeded in the blocking regions are systematically computed and analyzed. Additional long-term simulations of the same dry model with the increased horizontal resolution are also analyzed following the same approach.

How to cite: Deshmukh, V., Rivière, G., and Fromang, S.: How are atmospheric blockings represented in a dry general circulation model with wave energy just as powerful as in the observations?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5671, https://doi.org/10.5194/egusphere-egu23-5671, 2023.

EGU23-6131 | ECS | Orals | NP1.2

Stochastic weather generator and deep learning approach for predicting and sampling extreme European heatwaves 

George Miloshevich, Dario Lucente, Freddy Bouchet, and Pascal Yiou

Sampling rare events such as extreme heatwaves whose return period is larger than the length of available observations requires developing and benchmarking new  simulation methods. There is growing interest in applying deep learning alongside already existing statistical approaches to better generate and predict rare events. Our goal is to benchmark Stochastic Weather Generator (SWG) [1] based on analogs of circulation, soil moisture and temperature as a tool for sampling tails of distribution as well as forecasting heatwaves in France and Scandinavia using data from General Circulation Model (GCM). Analog method has been successfully implemented in rare event algorithms for low dimensional climate models [2].

SWG is implemented using a Markov chain with hidden states (.e.g. geopotential height at 500 hPa) with Euclidean metric. When applying such methods to climate data two challenges emerge: a large number of degrees of freedom and the difficulty of including slow drivers such as soil moisture alongside circulation patterns. Consequently, we are going to discuss ways of adjusting the distance metric of the analog Markov chain and dimensionality reduction techniques such as EOFs and variational auto encoder. By choosing the correct combination of weighted variables in the Euclidean metric and using analogs of only 100 years and generating long synthetic sequences we are able to correctly estimate return times of order 7000 years, which is validated based on a 7200 year long control run. The teleconnection patterns generated thus also look reliable compared to the control run.

Next we compare SWG forecasts of heatwaves with a direct supervised approach based on a Convolutional Neural Network (CNN). Both CNN and SWG are trained and validated on exactly the same GCM runs which allows us to conclude that CNN performs better in both regions. One could consider SWG as a baseline approach for CNN for this task.

[1] Yiou, P. and Jézéquel, A., https://doi.org/10.5194/gmd-13-763-2020, 2020

[2] D. Lucente at al. https://10.1088/1742-5468/ac7aa7, 2022

[3] DP Kingma, M Welling - https://doi.org/10.48550/arXiv.1312.6114, 2013

[4] G. Miloshevich, at al - https://doi.org/10.48550/arXiv.2208.00971, 2022

How to cite: Miloshevich, G., Lucente, D., Bouchet, F., and Yiou, P.: Stochastic weather generator and deep learning approach for predicting and sampling extreme European heatwaves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6131, https://doi.org/10.5194/egusphere-egu23-6131, 2023.

EGU23-6507 | ECS | Posters on site | NP1.2

Simulation of future extreme rainfall events over Belgium with a focus on the Vesdre valley using the regional climate model MAR. 

Josip Brajkovic, Hans Van De Vyver, Sébastien Doutreloup, Nicolas Ghilain, and Xavier Fettweis

The rainfall in July 2021 that hit West Germany, Netherlands and Belgium was of unprecedented intensity. To assess the probability of such events ocuring in a near and far future (until 2100), the regional climate model MAR has been used to make simulations at a resolution of 7,5 km. To this end, the regional climate model MAR is linked to a set of Earth System models (ESMs) with 4 IPCC SSP scenarios over a domain that includes Belgium and Luxemburg. The analysis focused on the valley of the Vesdre which in Belgium was the most impacted by flooding in terms of damage to human infrastructures.

For some specific climatic conditions, MAR simulates events of similar intensity to those of the 2021-floods over the next 5 decades. To assess the statistic significance of the results, a Peaks Over Threshold analysis (POT) has been applied to MAR outputs for precipitation events of 1,2,3,4 and 5-days. Quantiles associated with high return periods have been calculated for the historical period of simulation (1980-2010) and for the 2011-2040, 2041-2070 an 2071-2100 periods. This shows that the frequency of such events in the periods 2011-2040 and 2041-2070 is likely to increase if climatic conditions are wet enough. For global warming levels above 3 to 4 °C, conditions appear too dry for such events to occur.

How to cite: Brajkovic, J., Van De Vyver, H., Doutreloup, S., Ghilain, N., and Fettweis, X.: Simulation of future extreme rainfall events over Belgium with a focus on the Vesdre valley using the regional climate model MAR., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6507, https://doi.org/10.5194/egusphere-egu23-6507, 2023.

EGU23-6732 | Posters on site | NP1.2

Deep learning techniques applied to an attribution study for heatwaves in the Iberian Peninsula 

Pablo G. Zaninelli, David Barriopedro-Cepero, Marie Drouard, José Manuel Garrido-Pérez, Jorge Pérez-Aracil, Dušan Fister, Ricardo García-Herrera, Sancho Salcedo-Sanz, and M. Carmen Alvarez-Castro

Extreme event attribution quantifies the influence of climate change on a particular extreme event (EE). Understanding the extent to which climate change is responsible for particular EE is of paramount importance because of the vulnerability of society and ecosystems to these events, especially when it comes to heatwaves that have become more frequent and intense in many parts of the world in recent decades. This led the scientific community to focus its efforts on attribution analysis and the implementation of new techniques for its study. Attribution studies of temperature EE using machine learning (ML) methods are scarce in the specialized literature. Most attribution studies perform statistical comparison between the probability of occurrence of an event today with its probability in the pre-industrial past, making it possible to determine how much more likely that event is due to climate change and how much severe it could be. However, some limitations of these classical methodologies are the difficulty in understanding the links between the physical processes responsible for the occurrence of extreme events and anthropogenic forcing and the impossibility of detecting new trends associated with this forcing. The CLImate INTelligent (CLINT) project aims, among its objectives, to design ML algorithms to improve classical attribution methodologies in some of the aforementioned limitations for three european hot-spots located in Spain, Italy and Netherlands. In this framework, this work presents a preliminary attribution analysis for summer heatwaves focused in Iberian Peninsula and based on deep learning tools such as anomaly detection with autoencoders. The autoencoder is an unsupervised method that comprises two neural networks, one to encode information and the other to decode it. The autoencoder is fed with pre-industrial realizations integrated in the framework of the Coupled Model Intercomparison Project in its sixth version (CMIP6) in such a way that it allows detecting variabilities and trends that are present in the historical run and not in the pre-industrial one. In addition, the influence of climate change for a particular temperature EE could be associated with the AE anomaly for this EE.

How to cite: Zaninelli, P. G., Barriopedro-Cepero, D., Drouard, M., Garrido-Pérez, J. M., Pérez-Aracil, J., Fister, D., García-Herrera, R., Salcedo-Sanz, S., and Alvarez-Castro, M. C.: Deep learning techniques applied to an attribution study for heatwaves in the Iberian Peninsula, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6732, https://doi.org/10.5194/egusphere-egu23-6732, 2023.

EGU23-7087 | Posters on site | NP1.2

A Temperature-Duration-Curve model for the real-time estimation of extreme river water temperatures at ungauged sites 

Taha Ouarda, Christian Charron, and André St-Hilaire

Water temperature is an important environmental variable that has impacts on the physical, chemical, and biological processes in streamflows. Extreme river water temperatures affect the spawning, development and survival of several fish species, and are considered as important indicators of the health of a river and essential variables in all habitat models. Unfortunately, river water temperature data is characterised by its limited availability: measurement sites are often scarce, and records are regularly very short when available. It is hence crucial to develop regional thermal data estimation models for ungauged and partially gauged locations. Very few studies in the literature focused on the estimation of extreme water temperatures at sites where thermal data are limited or inexistent. A Temperature-Duration-Curve (TDC) model is proposed in this work to provide real-time estimates of river water temperature at ungauged locations during extreme events. The TDCs are estimated at the ungauged locations using a Generalised Additive Model and are then used to provide continuous estimates of river water temperature at these sites based on a spatial interpolation model. The model is developed based on a data base of 126 river thermal stations from Canada. The performance of the method is compared to a simpler approach and results indicate that the developed TDC model is robust and useful in practice.

How to cite: Ouarda, T., Charron, C., and St-Hilaire, A.: A Temperature-Duration-Curve model for the real-time estimation of extreme river water temperatures at ungauged sites, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7087, https://doi.org/10.5194/egusphere-egu23-7087, 2023.

EGU23-7124 | ECS | Orals | NP1.2

Influence of the Atlantic Multidecadal Variability and of Soil Moisture on Extreme Heatwaves in Europe 

Valeria Mascolo, Clément Le Priol, Fabio d'Andrea, and Freddy Bouchet

Nowadays heat waves are a growing issue, causing detrimental effects on society, people’s health and environment in several parts of the world. Slow drivers such as spring soil moisture and sea surface temperature are known to impact the probability of occurrence of heatwaves in many areas of the globe. However, their influence remains still little understood and studied. Even fewer has been said on the cross effect and relative impact of both factors. 

Our work aims at analysing and comparing the effects of spring soil moisture deficit in Europe and sea surface temperature decadal variability in the North Atlantic (AMV) on the occurrence of typical and more extreme European heat waves. To do that, we use the outputs from three climate models, namely IPSL-CM6A-LR, EC-Earth3 and CNRM-CM6-1, in which North Atlantic sea surface temperatures are nudged to the observed AMV anomalies.

At a methodological level, previous studies mainly focused on typical heat waves. Our work goes beyond that and proposes a new methodology to study events with larger return times. By introducing return time maps we can study rare heatwaves with return time from 10 to 50 years. We find that the temperature and duration of typical and extreme heatwaves are influenced by the AMV and soil moisture. In general, the changes induced by typical AMV or soil moisture anomalies are of comparable amplitude. In many areas of Europe, the influence of AMV and soil moisture over duration or temperature of extreme heatwaves increases when the return time is longer and is statistically significant even for return times of 50 years. In general, the three models give consistent results. 

With positive AMV phase or low soil moisture, the temperature and duration of extreme heatwaves are changed according to regional patterns. As might be expected, positive AMV phase or low soil moisture often induce hotter and longer typical and extreme heatwaves. However, counter-intuitively, they also induce cooler and shorter heatwaves over part of Northern-Eastern Europe. For more extreme events, the impact of the AMV and soil moisture increases, according to rather similar regional patterns. However, the regions with decreased temperature or duration impact extend in size.

In this work, we have improved the study of extreme heat waves and better understood their slow drivers. Studying those drivers is important to enhance heat wave predictability. To move further in this direction, we need to improve the statistics of the events. In this context, developing and using new tools such as rare event simulations might be the right path to follow.

How to cite: Mascolo, V., Le Priol, C., d'Andrea, F., and Bouchet, F.: Influence of the Atlantic Multidecadal Variability and of Soil Moisture on Extreme Heatwaves in Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7124, https://doi.org/10.5194/egusphere-egu23-7124, 2023.

EGU23-7697 | ECS | Posters on site | NP1.2

Diagnosing atmospheric persistence for heatwaves and in extended range forecasts 

Emma Holmberg, Gabriele Messori, Rodrigo Caballero, Steffen Tietsche, and Davide Faranda

Extreme events can cause severe disruption to society on many levels, and the ability to forecast these events represents a significant step towards the ability to reduce their impacts. Anomalously persistent atmospheric configurations are typically regarded to be strongly linked with temperature extremes in Europe, however, traditional methods of analysing atmospheric persistence lack a mathematically well-grounded definition. Furthermore, we are not aware of a metric which allows for quantification of instantaneous atmospheric persistence for forecasts for either an individual ensemble member or a deterministic forecast. We aim to help refine the definition of atmospheric persistence by presenting a mathematically well-grounded definition of persistence, which can potentially also be applied in a forecasting environment. We examine the link between the extremal index, an indicator for atmospheric persistence based on dynamical systems theory, and warm temperature extremes in several regions of Europe. We then consider the applicability of this technique to forecast data, in particular ECMWF extended range reforecast data, discussing its potential value as an additional forecast evaluation metric.

How to cite: Holmberg, E., Messori, G., Caballero, R., Tietsche, S., and Faranda, D.: Diagnosing atmospheric persistence for heatwaves and in extended range forecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7697, https://doi.org/10.5194/egusphere-egu23-7697, 2023.

EGU23-7908 | ECS | Orals | NP1.2

Dynamical pathways for pan-Atlantic compound cold and windy extremes 

Jacopo Riboldi, Josh Dorrington, Richard Leeding, Antonio Segalini, and Gabriele Messori

North American cold spells tend to co-occur with extreme wind and precipitation events over Europe, but the physical mechanisms behind such “pan-Atlantic” compound extremes have not been fully clarified yet. Rather than proposing a single mechanism, we discuss how cold spells over a single North American region can be connected with wind extremes over different European regions through separate, physically consistent dynamical pathways. The first one involves the propagation of a Rossby wave train from the Pacific Ocean, and is associated with windstorms over north-western Europe in the 5-10 days after the cold spell peak. The second one is associated with a high-latitude anticyclone over the North Atlantic and an equatorward-shifted jet, leading to windstorms over south-western Europe already in the days preceding the cold spell peak.

The same dynamical pathways can be independently retrieved from a cluster analysis based on the temporal evolution of the North Atlantic circulation in the days preceding North American cold spells. Such an analysis highlights significantly different stratospheric circulation patterns between the two pathways, with cold spells of the second pathway tied to a weaker than usual stratospheric polar vortex, and an enhanced occurrence of sudden stratospheric warmings.

How to cite: Riboldi, J., Dorrington, J., Leeding, R., Segalini, A., and Messori, G.: Dynamical pathways for pan-Atlantic compound cold and windy extremes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7908, https://doi.org/10.5194/egusphere-egu23-7908, 2023.

EGU23-7954 | ECS | Orals | NP1.2

On the Response of North Atlantic Extratropical Cyclones to North America Cold Air Outbreaks 

Richard Leeding, Gabriele Messori, and Jacopo Riboldi

We examine the characteristics of North Atlantic extratropical cyclones in ERA5 data during cold air outbreaks over continental North America. Previous research has established a statistical link between occurrences of North American cold air outbreaks and an increased frequency of extreme wet and windy conditions over Europe. The theoretical understanding of cyclogenesis suggests that greater numbers of extratropical cyclones will be generated in the North Atlantic, resulting from an enhanced temperature difference between the North American continent and the Gulf Stream during cold air outbreaks. Our analysis finds that counts of extratropical cyclones in the North  Atlantic storm track are no greater, or even less than climatology during periods with cold air outbreaks. We instead find anomalous jet stream activity associated with the cold air outbreaks. The jet stream acts to focus extratropical cyclones to a specific region of the North  Atlantic, depending on the regional extent of the cold air outbreak, resulting in significantly higher extratropical cyclone counts for that specific region. The regions found to be experiencing higher counts of extratropical cyclones align with previously established geographical dependencies between co-occurrences of North American cold air outbreaks and wet and windy extremes over Europe. We also find that cold air outbreaks associated with an anomalously strengthened jet result in a general increase in the strength of the extratropical cyclones reaching Europe, whilst a more equatorward-displaced jet, with lower maximum speed, results in more persistent extratropical cyclones over southern Europe. 

How to cite: Leeding, R., Messori, G., and Riboldi, J.: On the Response of North Atlantic Extratropical Cyclones to North America Cold Air Outbreaks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7954, https://doi.org/10.5194/egusphere-egu23-7954, 2023.

EGU23-8138 | ECS | Orals | NP1.2

Return levels of extreme European windstorms, their dependency on the NAO, and potential future risks 

Matthew Priestley, David Stephenson, and Adam Scaife

European windstorms experience considerable interannual variability, which makes the quantification of extreme return periods challenging. Estimating 200-year return levels is also complicated by having only ~60 years of comprehensive observational data. Such estimations of return periods are often performed using ‘catastrophe models’, which use complex calibration and tuning processes.  We have developed a reliable statistical model to estimate extreme windstorm gust speed return levels from only a multi-year sample of windstorm footprints without the need for the complexities associated with catastrophe models.

 

We have also been able to include variations of the NAO in our estimates, allowing for the generation of NAO-dependent return levels. Positive phases of the NAO result in larger return levels across the northwest of Europe. Additionally, the NAO is shown to be especially important for modulating low return period gusts, with the most extreme gusts occurring due to further stochastic processes. Using plausible future states of the NAO we also show that return levels have the potential to increase significantly in the next 100 years to rise well above historical uncertainty levels.

How to cite: Priestley, M., Stephenson, D., and Scaife, A.: Return levels of extreme European windstorms, their dependency on the NAO, and potential future risks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8138, https://doi.org/10.5194/egusphere-egu23-8138, 2023.

EGU23-8224 | ECS | Orals | NP1.2

Severe windstorm projections for Europe 

Nicholas James Leach, Gabriele Messori, Alex Crawford, Ryota Wada, Sally Woodhouse, and Claire Burke

Extreme windstorms are of considerable interest due to their potential to cause significant socio-economic damages over very large areas of land. As a result, understanding how climate change may affect the characteristics of the most severe storms is an important question for adaptation planing. However, projections of how the hazard associated with windstorms will change in the future are highly uncertain.

Here, we use an efficient statistical approach that characterises individual windstorms in terms of their intensity and exposure to estimate the present-day risk from such storms. We then use a methodology used widely in detection and attribution of climate change to assess how such characteristics may change into the future. Using windstorms simulated by a diverse set of high-resolution regional climate model projections for Europe, the EURO-CORDEX ensemble, we provide projections of risk over a range of future climate scenarios. Finally, we explore how the variety of driving and regional models influence the associated uncertainties, and how considering the performance and independence of the models can improve the robustness of the projections.

How to cite: Leach, N. J., Messori, G., Crawford, A., Wada, R., Woodhouse, S., and Burke, C.: Severe windstorm projections for Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8224, https://doi.org/10.5194/egusphere-egu23-8224, 2023.

EGU23-8244 | ECS | Posters on site | NP1.2

Predictability of blocking and zonal flow regimes  in a reduced-order land atmosphere coupled model 

Anupama K Xavier, Jonathan Demaeyer, and Stéphane Vannitsem

Low-frequency variability (LFV) encompasses atmospheric and climate processes on time scales from a few weeks to decades.​ This includes atmospheric blockings, heat waves, cold spells, and at longer time scales long-term oscillations like the MJO, the NAO, ENSO….. Better understanding of LFV, could contribute to improved long term forecasts​. Identifying and evaluating LFVs in GCMs is computationally expensive, so in this study an idealised low order coupled model is used. They are climate models ‘stripped to the bone’,  which links theoretical understanding to the complexity of more realistic models, made by key ingredients and approximations​; which hence helps us to study a particular phenomenon by tweaking the parameters affecting them with less computational cost​. 

The Quasi Geostrophic land atmosphere coupled model is a python implementation of mid-latitude atmospheric model​ with two layer quasi geostrophic channel atmosphere on beta -plane​ coupled to a simple land portion.  The system exhibits blocking conditions at different time scales depending on the incoming solar radiation and also experiences transitions from blocking to zonal flow after applying different sets of parameters to the model. The predictability and persistence of these regimes is investigated by calculating the local lyapunov exponents at the specified transition points and around them.  The findings are discussed in the perspective of the current literature on the predictability of blocking.

How to cite: K Xavier, A., Demaeyer, J., and Vannitsem, S.: Predictability of blocking and zonal flow regimes  in a reduced-order land atmosphere coupled model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8244, https://doi.org/10.5194/egusphere-egu23-8244, 2023.

EGU23-9105 | Orals | NP1.2

Effect of anthropogenic climate change on explosive cyclogenesis cases in Europe 

Mireia Ginesta, Emmanouil Flaounas, Pascal Yiou, and Davide Faranda

Mid-latitude storms are essential features of atmospheric variability in the cold season. The subsequent damages are caused by high wind speeds and heavy precipitation. Among such events, explosive cyclones can lead to extreme impacts when they make landfall. Climate change is affecting the underlying characteristics of such types of extremes. Being able to understand the way it modifies their dynamics is of great importance. In this work, we assess the influence of anthropogenic climate change on observed explosive cyclones in an Extreme Event Attribution framework using a large ensemble dataset. We evaluate three storms that hit different parts of Europe: Xynthia in February 2010, Alex in October 2020, and Eunice in January 2022. 

We use three ensembles of 35 members of the Community Earth System Model (CESM). We compare two periods of 6-hourly data: present-day climate [1991-2001] and future climate [RCP8.5 scenario, 2091–2101]. We find analogues of the trajectories of the three storms before their highest intensity in both periods. We do that by tracking all cyclones in the dataset and selecting the cyclone tracks that have the minimum Euclidean distance in km from the trajectories of Xynthia, Alex, and Eunice. We explore the characteristics of the analogues of the trajectories in both periods such as frequency of explosive cyclogenesis and intensity to evaluate whether the dynamics of the storms have been affected by climate change. We further compare the analogues in terms of precipitation and low-level wind in the regions of impact.

How to cite: Ginesta, M., Flaounas, E., Yiou, P., and Faranda, D.: Effect of anthropogenic climate change on explosive cyclogenesis cases in Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9105, https://doi.org/10.5194/egusphere-egu23-9105, 2023.

EGU23-9123 | ECS | Posters on site | NP1.2

Modeling vegetation response to climate in Africa at fine resolution: EarthNet2023, a deep learning dataset and challenge. 

Claire Robin, Christian Requena-Mesa, Vitus Benson, Lazaro Alonso, Jeran Poehls, Nuno Carvalhais, and Markus Reichstein

Droughts are a major disaster in Africa, threatening livelihoods through their influence on crop yields but also by impacting and weakening ecosystems. Modeling the vegetation state can help anticipate and reduce the impact of droughts by predicting the vegetation response over time. Forecasting the state of vegetation is challenging: it depends on complex interactions between the plants and different environmental drivers, which can result in both instantaneous and time-lagged responses, as well as spatial effects. Furthermore, modeling these interactions at the fine resolution of landscape scale can only rely on remote sensing observations, as in-situ measurements are not global and weather models have a coarse grid. With the increasing availability of remote sensing data, deep learning methods are a promising avenue for these spatiotemporal tasks. Here, we introduce both a dataset and a baseline deep neural network, modeling the vegetation response to climate at landscape scale in Africa.

EarthNet2021 [1] introduced leveraging self-supervised learning for satellite imagery forecasting based on coarse-scale weather in Europe. Here, we introduce EarthNet2023 with a more narrow focus on drought impacts in Africa. It contains over 45,000 Spatio-temporal minicubes (each 1.28x1.28km) at representative locations over the whole African continent. Alongside Sentinel-2 reflectance, ERA5 weather, and topography, it also contains Sentinel-1 backscatter, soil properties, and a long-term Normalized Difference Vegetation Index (NDVI) climatology based on Landsat. The latter allows evaluating models on vegetation anomalies, thereby including modeling of drought impacts. EarthNet2023 is intended as an open benchmark challenge, allowing multiple research groups to develop their approaches to drought impact modeling in Africa. 

As a baseline for EarthNet2023, we train a  Convolutional Long Short-Term Memory (ConvLSTM) deep learning model. Previous work has shown it is suitable for spatiotemporal satellite imagery forecasting [2, 3, 4]. The ConvLSTM baseline captures the seasonal evolution of NDVI over a wide range of vegetation types. General spatial patterns are well-captured as well as a first indication of skill during weather extremes is seen, although the accuracy of the predictions is inconsistent, and the confidence in the model is therefore too low. This suggests, with further development, deep learning approaches are promising for modeling vegetation evolution in Africa, potentially even up to the degree to support anticipatory action with drought impact modeling.

 

[1] Requena-Mesa, C., Benson, V., Reichstein, M., Runge, J., & Denzler, J. (2021). EarthNet2021: A large-scale dataset and challenge for Earth surface forecasting as a guided video prediction task. In CVPR 2021 (pp. 1132-1142).

[2] Diaconu, C. A., Saha, S., Günnemann, S., & Zhu, X. X. (2022). Understanding the Role of Weather Data for Earth Surface Forecasting Using a ConvLSTM-Based Model. In CVPR 2022 (pp. 1362-1371).

[3] Kladny, K. R. W., Milanta, M., Mraz, O., Hufkens, K., & Stocker, B. D. (2022). Deep learning for satellite image forecasting of vegetation greenness. bioRxiv.

[4] Robin, C., Requena-Mesa, C., Benson, V., Alonso, L., Poehls, J., Carvalhais, N., & Reichstein, M. (2022). Learning to forecast vegetation greenness at fine resolution over Africa with ConvLSTMs. In Tackling Climate Change with Machine Learning: workshop at NeurIPS 2022. 

How to cite: Robin, C., Requena-Mesa, C., Benson, V., Alonso, L., Poehls, J., Carvalhais, N., and Reichstein, M.: Modeling vegetation response to climate in Africa at fine resolution: EarthNet2023, a deep learning dataset and challenge., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9123, https://doi.org/10.5194/egusphere-egu23-9123, 2023.

Loss and damage (L&D) has been on the international agenda for over 20 years, and recently gained significant headway at UNFCCC COP27. L&D has been a controversial aspect of the international climate negotiations. This is largely due to L&D being connected to responsibility and compensation for the impacts of climate change on vulnerable communities. Researchers and practitioners are beginning to ask how they can help with L&D while many remain unsure about what this may mean.

Loss and Damage (L&D) is associated with the adverse effects of climate change, including the effects that are related to extreme weather events, such as intense typhons, but also occur in slow events, such as at sea level rise. The paper sets out to synthesise three specific challenges to L&D: lack of a coherent definition of L&D, gaps in measuring disproportionate effects of loss and damage on people, including the non economic consequences of L&D events, who it affects, how and why, and on what scale, and finally, absence of coherent understanding of climate governance instruments to influence L&D in ways that do not undermine existing adaptation and development efforts.

How to cite: Boyd, E.: Recasting the disproportionate impacts of climate extremes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9492, https://doi.org/10.5194/egusphere-egu23-9492, 2023.

EGU23-9945 | Posters on site | NP1.2

Oceanic Maintenance of Atmospheric Blocking 

Jamie Mathews

In recent years the understanding of atmospheric blocking has changed from solely a dry phenomena to one that includes moist processes. The primary source of that moisture, the ocean, has, until recently, been neglected as a driver of this basin scale structure. Here, the connection between atmospheric blocking over the North Atlantic and the diabatic influence of the Gulf Stream was investigated using potential vorticity diagnostics. In line with previous research, the reliance atmospheric blocking has on latent heat fluxes over the Gulf Stream and its extension, for induction and maintenance, was shown to be significant. It was shown that not only is it more likely for a North Atlantic block to occur after significant surface latent heat fluxes over the Gulf Stream and its extension, but the resulting block is likely to be anchored on the western flank of the Atlantic, making it more stationary and hence, more impactful. Additionally, blocks that have a longer duration were highly associated with surface latent heat fluxes over the western boundary current, while shorter blocks were not, indicating a positive feedback from the oceanic mesoscale phenomena onto this basin scale structure. Finally, the frequency of the block was seen to correspond to the amount of surplus heat content in the western boundary currents prior to the blocking event which, in the North Atlantic, had leading order dependence on the heat transport via the Gulf Stream.

How to cite: Mathews, J.: Oceanic Maintenance of Atmospheric Blocking, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9945, https://doi.org/10.5194/egusphere-egu23-9945, 2023.

EGU23-11943 | Orals | NP1.2 | Highlight

Simulating worst case  heatwaves during the Paris 2024 Olympics 

Pascal Yiou, Camille Cadiou, Davide Faranda, Aglaé Jézéquel, Nemo Malhomme, George Miloshevich, Robin Noyelle, Flavio Pons, Yoann Robin, and Mathieu Vrac

The Summer Olympic Games in 2024 will take place during the apex of the temperature seasonal cycle in the Paris Area. The midlatitudes of the Northern hemisphere have witnessed a few intense heatwaves since the 2003 epitome event. Those heatwaves have had environmental and health impacts, which often came as surprises. In this paper, we search for the most extreme heatwaves in Ile-de-France that are physically plausible, under climate change scenarios, for the decades around 2024. We apply a rare event algorithm on CMIP6 data to evaluate the range of such extremes. We find that the 2003 record can be exceeded by more than 4°C in Ile-de-France before 2050, with a combination of prevailing anticyclonic conditions and cut-off lows. This study intends to build awareness on those unprecedented events, against which our societies are ill-prepared. Those results could be extended to other areas of the world.

How to cite: Yiou, P., Cadiou, C., Faranda, D., Jézéquel, A., Malhomme, N., Miloshevich, G., Noyelle, R., Pons, F., Robin, Y., and Vrac, M.: Simulating worst case  heatwaves during the Paris 2024 Olympics, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11943, https://doi.org/10.5194/egusphere-egu23-11943, 2023.

EGU23-12059 | ECS | Posters virtual | NP1.2

Present and projected humid heat exposure and precipitation extremes in Turkey 

Berkay Donmez, Kutay Donmez, Cemre Yuruk Sonuc, and Yurdanur Unal

Regional intensification of precipitation extremes and the emergence of humid heat stress conducive to periling vulnerable populations suggest the need for further nation-specific risk assessments. Here, we conduct the first analysis of present and projected population exposure to extreme wet-bulb temperature (Tw) values in Turkey and concurrently use the generalized extreme value (GEV) theory to model extreme precipitation based on multiple intensity, duration, and frequency metrics. Using simulations dynamically downscaled to 0.11-degree resolution via the COSMO-CLM model, we provide a nationwide picture of the trends in these metrics and derive the number of people exposed to Tw extremes based on the population estimates in the Shared Socioeconomic Pathways (SSPs) under the high-emission RCP 8.5 scenario. As part of the GEV analysis, our main goal is to show how precipitation extremes in Turkey evolve and transform due to the changing climate not only in stationary but also in non-stationary climate settings. Our results convey a detailed understanding of the potentially dangerous conditions across climatologically different regions of Turkey and are relevant for decision-makers.

How to cite: Donmez, B., Donmez, K., Yuruk Sonuc, C., and Unal, Y.: Present and projected humid heat exposure and precipitation extremes in Turkey, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12059, https://doi.org/10.5194/egusphere-egu23-12059, 2023.

EGU23-12095 | ECS | Posters on site | NP1.2

Weakened impact of the Atlantic equatorial mode of variability on the future Guinea Coast extreme rainfall indices 

Koffi Worou, Thierry Fichefet, and Hugues Goosse

The Atlantic equatorial mode (AEM) is an interannual oceanic internal mode of variability which impacts the tropical circulation during its active phases in the boreal summer. A positive phase of the AEM is characterized by above-normal sea surface temperature anomalies in the eastern equatorial Atlantic which lead to positive rainfall anomalies over the Guinea Coast, a region located in the southern part of West Africa. The AEM appears as the leading oceanic driver of the Guinea Coast rainfall (GCR) during the monsoon season, and the AEM-GCR relation during the last century is stationary.  Moreover, extreme rainfall events over the Guinea Coast are also enhanced by the AEM-positive phases.  Therefore, there is a need to study how the relationship between the AEM and extreme rainfall indices would change under future global warming. The present work assesses this relationship between the AEM and the Guinea Coast extreme rainfall indices in the historical simulations performed by 24 General Circulation Models (GCMs) participating in the sixth phase of the Coupled Models Intercomparison Project (CMIP6). Results indicate that the extreme rainfall responses to the AEM under present-day climate conditions are qualitatively well reproduced by the GCMs in the 1995-2014 period, although there are substantial biases in their magnitudes.  For the future changes, we consider the CMIP6 Shared Socio-economic pathway 5-8.5 (SSP5-8.5) simulations and three different periods: the near-term (2021-2040), the mid-term (2041-2060) and the long-term (2080-2099).  Relative to the present-day period, our results indicate an overall gradual increase with time in the mean and variability of the different extreme indices for the Guinea Coast. However, the future influence of the AEM on the extreme rainfall indices decreases with time, which is in line with the projected decrease in the future AEM variability.

How to cite: Worou, K., Fichefet, T., and Goosse, H.: Weakened impact of the Atlantic equatorial mode of variability on the future Guinea Coast extreme rainfall indices, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12095, https://doi.org/10.5194/egusphere-egu23-12095, 2023.

EGU23-12130 | ECS | Orals | NP1.2 | Highlight

A probabilistic assessment of extreme weather event impacts on crop yield in Germany 

Federico Stainoh, Julia Moemken, and Joaquim Pinto

The impacts of extreme weather on the agricultural sector are a global concern in a changing climate. In recent years, single and compound weather extremes have increased in frequency, intensity and duration and are expected to worsen in the upcoming decades. Therefore, it is necessary to have a better understanding of extreme weather-related crop yield shock to ensure food security in a growing worldwide population. In this study, we employed a logistic regression model to quantify the risk of major crop yield shocks associated with heat stress, extreme precipitation and frosts. We used reported sub-national level data from Germany and a percentile-based threshold to define yield shock. Climate extreme drivers were based on statistical thresholds over daily maximum temperature, minimum temperature and precipitation. In addition to this,  we investigated how the seasonal meteorological pre-conditions of temperature and precipitation can modulate extreme weather-related yield shock.

How to cite: Stainoh, F., Moemken, J., and Pinto, J.: A probabilistic assessment of extreme weather event impacts on crop yield in Germany, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12130, https://doi.org/10.5194/egusphere-egu23-12130, 2023.

EGU23-13507 | Orals | NP1.2

Using Artificial Intelligence to Reconstruct Missing Climate Data In Extreme Events Datasets 

Étienne Plésiat, Robert Dunn, Markus Donat, Colin Morice, Thomas Ludwig, Hannes Thiemann, and Christopher Kadow

Evaluating the trends of extreme indices (EI) is crucial to detect and attribute extreme events (EE) and establish adaptation and mitigation strategies to the current and future climate conditions. However, the observational climate data used for the calculation of these indices often contains many missing values and leads to incomplete and inaccurate EI. This problem is even greater as we go back in time due to the scarcity of the older measurements.

To tackle this problem, interpolation techniques such as the kriging method are often used to fill in the gaps. However, it has been shown that such techniques are inadequate to reconstruct specific climatic patterns [1]. Deep-learning based technologies give the possibility to surpass standard statistical methods by learning complex patterns and features in climate data.

In this work, we are using an inpainting technique based on a U-Net neural network made of partial convolutional layers and a loss function designed to produce semantically meaningful predictions [1]. Models are trained using vast amounts of climate model data and can be used to reconstruct large and irregular regions of missing data with few computational resources.

The efficiency of the method is well demonstrated through its application to the HadEX3 dataset [2]. This dataset contains gridded land surface EI, among which the TX90p index that measures the monthly (or annual) frequency of warm days (defined as a percentage of days where daily maximum temperature is above the 90th percentile). As for other EI, there is a lack of TX90p values in many regions of the world, even in recent years. It is particularly true when looking at an intermediate product of HadEX3 where the station-based indices have been combined without interpolation. This is illustrated by the left map of the figure where the gray pixels correspond to missing values. By training our model using data from the CMIP6 archive, we have been able to reconstruct the missing TX90p values for all the time steps of HadEX3 (see right map in the figure) and detect EE that were not included in the original dataset. The reconstructed dataset is being prepared for the community in the framework of the H2020 CLINT project [3] for further detection and attribution studies.

[1] Kadow C. et al., Nat. Geosci., 13, 408-413 (2020)
[2] Dunn R.J.H. et al., J. Geophys. Res. Atmos., 125, 1 (2020)
[3] https://climateintelligence.eu/

How to cite: Plésiat, É., Dunn, R., Donat, M., Morice, C., Ludwig, T., Thiemann, H., and Kadow, C.: Using Artificial Intelligence to Reconstruct Missing Climate Data In Extreme Events Datasets, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13507, https://doi.org/10.5194/egusphere-egu23-13507, 2023.

EGU23-14675 | ECS | Posters on site | NP1.2

Indirect and direct impacts of Typhoon In-Fa (2021) on heavy precipitation in inland and coastal areas of China: Synoptic-scale environments and return period analysis 

Liangyi Wang, Xihui Gu, Louise J. Slaster, Yangchen Lai, Xiang Zhang, Dongdong Kong, Jianyu Liu, and Jianfeng Li

Typhoon In-Fa in 2021 produced an indirect heavy precipitation event (HPE) in central China well over a thousand kilometers away from its center, as well as a direct HPE in eastern China near its eyewall, inner and outer spiral rainbands. Both indirect and direct HPEs of Typhoon In-Fa caused severe impacts on the society. However, the synoptic-scale environments and the impacts of return period estimations of these HPE events remain poorly understood. Here, we first evaluated the spatio-temporal evolution of the two HPEs indirectly and directly induced by Typhoon In-Fa, then examined the synoptic patterns during Typhoon In-Fa for both HPEs in central and eastern China, and finally analyzed how the Typhoon In-Fa-induced HPEs affected local return period estimations of precipitation extremes. Our results show that the remote HPE over central China ~2,200 km ahead of Typhoon In-Fa was a typical predecessor rain event (PRE). A low-level southeasterly jet conveyed abundant moisture from the vicinity of Typhoon In-Fa to central China. Abundant moisture experienced strong convergence and was forced ascent, which caused frontogenesis on the windward slope due to the impacts of orographic forcing, thereby the occurrence of PRE in central China. The PRE occurred beneath the equatorward entrance of the upper-level westerly jet. Meanwhile, Typhoon In-Fa and the PRE favored divergently and adiabatically driving outflow in the upper level, and thus intensified the upper-level westerly jet. In eastern China, the HPE occurred in areas situated less than 200 km from Typhoon In-Fa’s center and left of Typhoon In-Fa’s propagation. The persistent HPE was primarily due to the long duration and slow movement of Typhoon In-Fa. On the one hand, favorable thermodynamic and dynamic conditions, and abundant atmospheric moisture favored the maintenance of Typhoon In-Fa intensity. On the other hand, a saddle-shaped pressure field in the north of eastern China and peripheral weak steering flow impeded Typhoon In-Fa’s movement northward. From the perspective of hydrological impacts, indirect and direct HPEs induced by Typhoon In-Fa led to decreases in return period estimates of HPEs (especially in central China), indicating that such extreme HPEs might increase the failure risk of engineering operations. These results suggest that anomalous HPEs remotely triggered by TCs require improved early warnings, and that more attention should be paid to such HPEs when estimating the design values of hydraulic infrastructure.

How to cite: Wang, L., Gu, X., Slaster, L. J., Lai, Y., Zhang, X., Kong, D., Liu, J., and Li, J.: Indirect and direct impacts of Typhoon In-Fa (2021) on heavy precipitation in inland and coastal areas of China: Synoptic-scale environments and return period analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14675, https://doi.org/10.5194/egusphere-egu23-14675, 2023.

EGU23-14838 | Orals | NP1.2

Freva for ClimXtreme: an aid to get the bigger picture in analysis of extremes 

Etor E. Lucio-Eceiza, Christopher Kadow, Martin Bergemann, Andrej Fast, Hannes Thiemann, and Thomas Ludwig

 

The number of damaging events caused by natural disasters is increasing because of climate change. Projects of public interest such as ClimXtreme (Climate Change and Extreme Events [1, 2]), aim to improve our knowledge of extreme events, the influence of environmental changes and their societal impacts.

ClimXtreme focuses on an integral evaluation through a three-pronged approach, namely: the physical processes behind the extremes, the statistical assessment of them, and their impact. The success of such a project depends on a coordinate effort from many interdisciplinary groups down to the management of computational and data storage resources. The ever-growing amount of available data at the researcher’s disposal is a two-sided blade that craves for greater resources to host, access, and evaluate them efficiently through High Performance Computing (HPC) infrastructures. Additionally, these last years the community is demanding an easier reproducibility of evaluation workflows and data FAIRness [3]. Frameworks like Freva (Free Evaluation System Framework [4, 5]) offer an efficient solution to handle customizable evaluation systems of large research projects, institutes or universities in the Earth system community [6-8] over the HPC environment and in a centralized manner. Mainly written on python, Freva offers:

  • A centralized access. Freva can be accessed via command line interface, via web, and via python module (e.g. for jupyter notebooks) offering similar features.
  • A standardized data search. Freva allows for a quick and intuitive incorporation and search of several datasets stored centrally.
  • Flexible analysis. Freva provides a common interface for user defined data evaluation routines to plug them in to the system irrespective of the programming language. These plugins are able to search from and integrate own results back to Freva. This environment enables an ecosystem of plugins that fosters the interchange of results and ideas between researchers, and facilitates the portability to any other research project that uses a Freva instance.
  • Transparent and reproducible results. Every analysis run through Freva (including parameter configuration and plugin version information) is stored in a central database and can be consulted, shared, modified and re-run by anyone within the project. Freva optimizes the usage of computational and storage resources and paves the way of traceability in line with FAIR data principles.

Hosted at the DKRZ, ClimXtreme’s Freva instance (XCES [7]) offers quick access to more than 9 million datafiles of models (e.g. CMIP, CORDEX), observations (stations, gridded) and evaluation outputs. The ClimXtreme community has been actively contributing with plugins to XCES, its biggest asset, with close to 20 plugins of different disciplines at the disposal of everyone within the project, and more than 20,000 analysis run through the system. At present, any researcher can focus on a past, present or future period and a geographical region and run a series of evaluations ranging from coocurrence probabilities of extreme events, their impact on crops to wind tracking algorithms among many others. Freva facilitates comprehensive and exhaustive analysis of extreme events in an easy way.

 

References:

[1] https://www.fona.de/de/massnahmen/foerdermassnahmen/climxtreme.php

[2] https://www.climxtreme.net/index.php/en/

[3] https://www.go-fair.org/fair-principles/

[4] http://doi.org/10.5334/jors.253

[5] https://github.com/FREVA-CLINT/freva-deployment

[6] freva.met.fu-berlin.de

[7] https://www.xces.dkrz.de/

[8] www-regiklim.dkrz.de

 

How to cite: Lucio-Eceiza, E. E., Kadow, C., Bergemann, M., Fast, A., Thiemann, H., and Ludwig, T.: Freva for ClimXtreme: an aid to get the bigger picture in analysis of extremes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14838, https://doi.org/10.5194/egusphere-egu23-14838, 2023.

EGU23-14879 | ECS | Posters on site | NP1.2 | Highlight

Assessing recent trends in globally co-occurring hot, dry and wet events under climate change 

Bianca Biess, Lukas Gudmundsson, and Sonia I. Seneviratne

The spring-to-summer seasons in recent years were characterized by co-occurring hot, dry, and wet extremes around the globe, leading to questions about the contribution of human-induced global warming to the changing likelihoods of such extreme years.  Here we investigate recent trends in the fraction of global (and regional) land-area that is affected by hot days, wet days and dry months. Observed trends are put into context of Earth System Model (ESM) ensemble simulations accounting for present day and pre-industrial climate conditions in a detection and attribution setting. The analysis is applied to the global land area as well as to the regions defined in the sixth IPCC assessment report. Results show that on a global scale as well as on a regional level, observed trends of co-occurring hot, dry and wet events cannot be explained by internal climate variability, but are only captured by model simulations that account for anthropogenic changes in the composition of the atmosphere. Thus, the results show that recent global trends in spatially co-occuring hot and dry extremes are very likely linked to anthropogenic climate change.

How to cite: Biess, B., Gudmundsson, L., and Seneviratne, S. I.: Assessing recent trends in globally co-occurring hot, dry and wet events under climate change, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14879, https://doi.org/10.5194/egusphere-egu23-14879, 2023.

EGU23-15813 | ECS | Posters on site | NP1.2

Delayed Effects of ENSO and Indian Ocean Dipole on the ensuing-summer extreme precipitation over Yangtze River Valley 

Yucong Lin, Silvio Gualdi, and Enrico Scoccimarro

Yangtze River Valley (YRV) locates in Southeast China, is home to about a third of the population in China. Summer extreme precipitation in Yangtze River can lead to extensive social problems and loss of lives. Understanding the characteristics of extreme precipitation and identifying the possible driving factors can increase our ability to plan for, manage and respond to related extreme events over the YRV. This study applies ERA5 data during the period of 1950~2021 to examine the possible influence of ENSO and the sea surface temperature (SST) variability over the Indian Ocean domain on the interannual variability of the extreme precipitation over the YRV. The related physical processes that link the summer Yangtze River extreme precipitation, ENSO and Indian Ocean Dipole (IOD) are investigated.

Using composites analysis and Pearson correlation method, we found that both ENSO and IOD have delayed effects on summer extreme precipitation over the YRV, warm ENSO events and positive IOD phases are in favor of increased extreme precipitation in the subsequent summers, and vice versa. The anomalous anticyclone over the western Pacific Ocean (WNPAC) is the key factor in altering the inter-annual variability of extreme precipitation over the YRV. By comparing the extreme precipitation composites with different ENSO-IOD coupling events, we found that the signals of enhanced extreme precipitation are significant when El Niño occurs with a positive phase of IOD in the previous winter. The results based on the large circulation patterns also support that IOD plays an essential role in modulating the WNPAC. Our research highlights the need for a fundamental exploration into air-sea interactions over the tropical Pacific associate to ENSO-IOD coupling modes, our understanding in learning the impacts of these modes of variability on precipitation extremes over the YRV will contribute to improve the predictability of extreme events over this region.

Keywords:

Yangtze River Valley, extreme precipitation, ENSO, IOD, western North Pacific anomalous anticyclone 

How to cite: Lin, Y., Gualdi, S., and Scoccimarro, E.: Delayed Effects of ENSO and Indian Ocean Dipole on the ensuing-summer extreme precipitation over Yangtze River Valley, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15813, https://doi.org/10.5194/egusphere-egu23-15813, 2023.

The climate and weather over Europe and Asia are strongly influenced by the large-scale atmospheric circulation over the North Atlantic area. During the winter of 2009/10, the usually separate Atlantic and African jets merged into one zonal jet, resulting in unusually cold and wet conditions in Eurasian regions. During this winter the jet was unusually persistent, with characteristics more typical of the Pacific jet stream, which is a mixed thermally-eddy driven jet, suggesting the jet underwent a rare dynamical regime change.  Such a merging was only observed to occur for a whole winter during winters of 1968-69 and 1969-70. In this study, we apply GKTL rare event algorithm to produce an ensemble of PlaSim model runs of similar winter flow conditions, to study such merged jet (mixed thermally-eddy driven jet) transition and its dynamics. We try to understand how the initial conditions during the beginning of the winter could affect the jet to be in a persistent merged state. It is seen that there is a larger probability to continue in a merged jet state if there is a merged jet state at the beginning of winter. Similarly, there is a larger probability to continue in an eddy-driven jet state if there is an eddy-driven jet state at the beginning of winter. On comparing the ensemble of merged jet winter trajectories with the ensemble of eddy-driven jet winter trajectories there is a significant weakening of eddy heat fluxes over the west and central North Atlantic region. Also, the typically poleward-directed eddy momentum fluxes are significantly weaker during the winter merged jet state with small increases in the subtropics over the eastern North Atlantic due to the equatorward shift of the eddies.

How to cite: Suresan, S. and Harnik, N.: Computing and analyzing persistent merged jet state in climate model using rare event algorithm, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16917, https://doi.org/10.5194/egusphere-egu23-16917, 2023.

EGU23-271 | ECS | Orals | NH7.2 | Highlight

Impacts of climate variability and change on regional fire weather in heterogeneous landscapes of Central Europe 

Julia Miller, Andrea Böhnisch, Ralf Ludwig, and Manuela Brunner

Wildfires have reached an unprecedented scale in recent fire seasons of the Northern Hemisphere as demonstrated by the summers of 2021 and 2022. Severe fire seasons, characterized by heat, drought and windy conditions, might become even more frequent and will extend to more temperate regions in northern latitudes under global warming. Still, quantifying the effects of climate change on future fire danger is challenging because natural variability hides trends of increasing fire danger in climate model simulations in future potentially fire-prone areas. Single Model Initial-Condition Large Ensembles (SMILEs) help scientists to distinguish climate trends from natural variability. Here, we leverage the capabilities of SMILEs to assess future changes in fire weather conditions in a currently non-fire-prone area in Central Europe. The study area covers four heterogeneous landscapes, namely the Alps, the Alpine Foreland (southern parts), the lowlands of the Southern German Escarpment, and the eastern mountain ranges of the Bavarian Forest (northern parts). We use a SMILE of the Canadian regional climate model version 5 (CRCM5-LE) under the RCP 8.5 scenario from 1980 to 2099 to analyze trends in fire danger quantified by the globally applicable Canadian Fire Weather Index (FWI).

Our results show the strongest increases for the median (50th percentile) and extreme (90th percentile) FWI in the northern parts of the study area during the late summer months July, August and September. The southern, more alpine parts are affected less strongly and show high fire danger mostly in August by the end of the 21st century for the median FWI. Over the whole study area, we find that the extreme FWI in the present climate period will become much more frequent at the end of the century. In the South German Escarpment and Eastern Mountain Ranges, the climate change trend exceeds natural variability in the late 2040’s. Due to weaker variability, the time of emergence is reached in the Alps and Alpine Foreland in the early 2040's.

These results demonstrate that the CRCM5-LE is a suitable dataset to disentangle climate trends from natural variability in a multivariate fire danger metric. Our study emphasizes that regions with a low fire danger under current climate conditions will experience weather conditions facilitating the development of potentially uncontrollable wildfires in a warming climate.

How to cite: Miller, J., Böhnisch, A., Ludwig, R., and Brunner, M.: Impacts of climate variability and change on regional fire weather in heterogeneous landscapes of Central Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-271, https://doi.org/10.5194/egusphere-egu23-271, 2023.

EGU23-1004 | ECS | Posters virtual | NH7.2

Atmospheric Conditions Conducive to Forest Fire Events in the Greater Himalayan Region 

Anandu Prabhakaran, Piyush Srivastava, and Anand Pai

​​During the last decade, there has been a dramatic rise in Forest Fire incidents over the Indian Himalayan region, leading to a considerable loss of life and property. To mitigate and manage the impact of forest fires through a Forest Fire Early Warning System, a better understanding of both small and large-scale atmospheric processes conducive to the spread of forest fires is required. Although significant progress has been made in disseminating forest fire danger information, most of the operational methodologies in the Indian sub-continent still do not consider real-time weather forecasts from atmospheric numerical models as input to the fire module. The objective of this work is to systematically analyze the meteorological conditions during two major forest fire events that occurred over the Uttarakhand region in 2016 and 2020. Forest fire events in 2016 and 2020 coincide with El Nino, La-Nina and cycles of Indian Ocean Dipole (IOD). A detailed analysis of the 2016 and 2020 fire events shows an increased frequency of fire events and burnt areas in 2016, whereas the area burnt was considerably low in the 2020 event. A typical year without significant influences from ENSO and IOD shows relatively low spread of fires and burnt areas. Such an impenetrable correlation between atmospheric oscillations and fire events results in vast damage over the Indian Himalayan region. The inculcation of real-time weather forecasts with numerical weather prediction models could tackle this existing gap in the Forest Fire Early Warning System and possibly mitigate the further casualties caused by the increased acceleration of fire spread induced by atmospheric oscillation over the Indian Himalayan region.

How to cite: Prabhakaran, A., Srivastava, P., and Pai, A.: Atmospheric Conditions Conducive to Forest Fire Events in the Greater Himalayan Region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1004, https://doi.org/10.5194/egusphere-egu23-1004, 2023.

EGU23-1415 | ECS | Orals | NH7.2

Modelling of a wildfire in Portugal using a fully coupled atmosphere-fire spread modelling system 

Ricardo Vaz, Rui Silva, Susana Cardoso Pereira, Ana Carvalho, David Carvalho, and Alfredo Rocha

This work investigates the physical interactions and feedback between wildfires and the atmosphere using the coupled atmosphere-fire spread modelling system, WRF-SFIRE. The Figueira da Foz forest fire, occurred in Portugal in October 2017, which ocurred in association with hurricane Ophelia, was simulated under two different scenarios of fuel moisture settings, one static and one dynamic. Results show an underestimation of burnt area in the dynamic case, while static fuel moisture has shown a very high agreement. Pyrocumulus formed during late afternoon with a very dry base and more humid top, creating conditions favourable for the occurrence of downbursts, with very high Convective Available Potential Energy values. Lifted Condensation Level increased above the fire front as moisture was transported upwards, increasing surface temperature. Official reports show an overestimation of fuel moisture near the surface, leading to high CAPE values, compared to near zero values reported by vertical soundings. Relative Humidity values were higher by 30% when compared to weather station observations, and temperatures approximately 4ºC lower. Further model testing is needed to provide more accurate surface temperature and moisture simulations, to allow a more accurate fire progression representation and energy exchange, and improve the modelling of potential convective events. 

How to cite: Vaz, R., Silva, R., Cardoso Pereira, S., Carvalho, A., Carvalho, D., and Rocha, A.: Modelling of a wildfire in Portugal using a fully coupled atmosphere-fire spread modelling system, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1415, https://doi.org/10.5194/egusphere-egu23-1415, 2023.

EGU23-3274 | ECS | Posters on site | NH7.2

Meteorological variables controlling the forest fire over the Himalayas 

Leena Khadke and Subimal Ghosh

Forest fire is the main disturbance for the Himalayan ecosystems, which impacts the regional and global carbon cycle, climate, forest succession, and tree density. Forest fires can occur due to both natural processes and anthropogenic factors. The fires over the Himalayas are mostly observed in the summer and pre-monsoon season, with large interannual variability. The primary objective of the present study is to identify the main meteorological drivers controlling forest fires over the Himalayas from March to June. The study performed statistical analysis on the daily and monthly observed/reanalysis climate data between 2001-2016. We used precipitation (P), temperature (T), and soil moisture (SM) from the climate prediction center and Vapor Pressure Deficient (VPD) from ECMWF-ERA5. The three satellite-based datasets for the Burned Area (BA) are accessed from Global Fire Emissions Database version 4 (GFEDs), Collection 6 Moderate Resolution Imaging Spectroradiometer (MODIS C6), and the European Space Agency Fire Climate Change Initiative version 5.1 (FireCCI51 – CEDA archive). The preliminary results show that all three BA has significant spatial and temporal/interannual variability. Meteorological variables such as P, T, SM, and VPD indicate strong interannual variability with rising slopes throughout the study period. Among these, P and SM indicate a significant trend over the central and northeast parts of the Himalayas. The VPD has a maximum significant positive correlation with BA for all three datasets (highest for GFED). The daily climatology suggests that VPD drops with an increase in P and follows the peaks of increasing T. The VPD rises until the end of April and starts falling from May due to pre-monsoon showers. The study observed that the varying amount of BA follows the peaks of high VPD, high temperature, and dry days (PThreshold < 1mm). The northeast part of the Himalayas experiences major fires in March-April because of the substantial number of dry days and reduces in May-June due to pre-monsoon showers. In the northwest part, the amount of BA is high in May-June, despite having a smaller number of high VPD and dry days over the region. In the future, the study will focus on the impact of Himalayas forest fires on the atmospheric dust loading at a high temporal scale which can potentially trigger forest fires in adjacent regions.

How to cite: Khadke, L. and Ghosh, S.: Meteorological variables controlling the forest fire over the Himalayas, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3274, https://doi.org/10.5194/egusphere-egu23-3274, 2023.

EGU23-4547 | Posters on site | NH7.2

High-resolution modeling of historical forest fires in the Canton of Bern 

Renuka Prakash Shastri, Stefan Brönniman, and Daniel steinfeld

Forest fires are considered an important hazard in forested areas and a serious threat to forest ecosystem and buildings. The combination of drought, high temperatures, and wind increases the risk of forest fires. To better understand the fundamental causes and consequences of fire, we need to study the historical fire regimes. In this study, the meteorological conditions were simulated with the WRF model (Weather Research and Forecasting; Skamarock et al. 2008) for three historical forest fires, in the Canton of Bern, Switzerland (La Neuveville, April 1893, Simmenflueh, August 1911, Kirchberg, April 1915). In terms of area, these are the largest fires in the canton of Bern in the Swiss fire database. The "Twentieth Century Reanalysis" version 3 (20CRv3, Slivinski et al. 2019) was used as a boundary condition. 20CRv3 has a spatial resolution of about 75 km and a temporal resolution of three hours. Using WRF version 4.1.2 20CRv3 has now been gradually downscaled to a resolution of 1x1 km^2. Simulations suggest that the soil had dried out in the previous week and soil moisture had reached low values on the day the fire broke out. High-resolution fire weather indices are also calculated. A lack of precipitation and high temperatures led to high forest fire index values and a high to very high risk of forest fires.

 

References
[1] Slivinski, L. C.et al. (2019), Towards a more reliable historical reanalysis: Improvements to the
Twentieth Century Reanalysis system. , Q. J. Roy. Meteorol. Soc. 145, 2876-2908.
[2] Pfister, L. , S. Brönnimann, M. Schwander , FA Isotta , P. Horton, and C. Rohr, (2020) Statistical
Reconstruction of Daily Precipitation and Temperature Fields in Switzerland back to 1864, Clim.
past 16, 663-678.
[3] Skamarock, WC, et al. (2008) A Description of The Advanced Research WRF Version 3. NCAR
Technical Note.
[4] Van Wagner, C.E. (1987): Development and Structure of the Canadian Forest Fire Weather Index
System, Forestry Technical Report, Canadian Forestry Service Headquarters, Ottawa.

How to cite: Shastri, R. P., Brönniman, S., and steinfeld, D.: High-resolution modeling of historical forest fires in the Canton of Bern, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4547, https://doi.org/10.5194/egusphere-egu23-4547, 2023.

EGU23-8082 | Orals | NH7.2

Towards global prediction of fire risk in a changing climate 

James Brennan, Claire Burke, Graham Reveley, Sally Woodhouse, Hamish Mitchell, Nick Leach, and Laura Ramsamy

The identification of areas susceptible to fire is critical for planners, managers, and decision makers in developing effective mitigation strategies. At Climate X we are producing risk estimates to help businesses and communities mitigate and adapt for climate change related losses. Climate X provides risk scores and expected financial losses from a range of physical hazards.  The risks posed by wildfire are increasing in many regions and especially within the wildland–urban interface. We developed a machine learning model to predict changes in fire risk at 90m that can be applied globally. The approach combines meteorological drivers of fire weather utilising CORDEX regional climate models with local fire susceptibility modelling trained from Earth observation records of fire occurrence.  By 2100, we find an average 7% increase in fire risk across the US and western Europe under the rcp8.5 scenario. Our results demonstrate how the combined application of machine learning, climate and Earth observation data can provide time sensitive assessments of fire risk at global scale.

How to cite: Brennan, J., Burke, C., Reveley, G., Woodhouse, S., Mitchell, H., Leach, N., and Ramsamy, L.: Towards global prediction of fire risk in a changing climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8082, https://doi.org/10.5194/egusphere-egu23-8082, 2023.

EGU23-8967 | ECS | Orals | NH7.2

Modelling pyro-convective activity and the meteorological conditions leading to mega-fires 

Cátia Campos, Flavio T. Couto, Carolina Purificação, Jean-Baptiste Filippi, Roberta Baggio, and Rui Salgado

Mega-fires are wildfires that burn an area greater than 10.000 hectares. Despite being a minority in relation to the total number of fires, they are the one with the greatest negative impact on society and the environment. Associated with this wildfire type, the phenomenon of pyro-convection has been reported in several cases. Strong pyro-convective activity can lead to the formation of clouds within the smoke plume, also known as pyro-cumulus (PyroCu) or pyro-cumulonimbus (PyroCb). In 2017, Portugal recorded 11 mega-fires, of which 8 occurred on the 15th October. Since the photographic evidence of the formation of a PyroCu cloud, the chosen case study was the Quiaios mega-fire. The study aims to simulate the impact of a fire in the atmosphere, as well as the large-scale meteorological conditions that were affecting Portugal during the mega-fires. For this purpose, two numerical simulations were performed using the MesoNH atmospheric model: a coupled simulation with the ForeFire fire propagation model, with 3 nested domains with resolution of 2000m, 400m and 80m (300 by 300 grid points), and a large-scale non-coupled simulation, with a 15km resolution (300 by 250 grid points) to study the large-scale conditions. The coupled simulation allowed identifying the formation of a PyroCu cloud composed by different species of hydrometeors, namely graupel and rain droplets. The pyro-cloud developed inside the plume due the vertical transport of water vapor to higher levels. In the context of large scale, the simulation well represented the evolution of hurricane Ophelia, showing the change in wind direction from Southeast to Southwest in Portuguese territory, which created a favourable condition to the intensification of the active fires and the development of PyroCb clouds during the late afternoon. This study was funded by national funds through FCT-Foundation for Science and Technology, I.P. under the PyroC.pt project (Ref. PCIF/MPG/0175/2019).

 

How to cite: Campos, C., Couto, F. T., Purificação, C., Filippi, J.-B., Baggio, R., and Salgado, R.: Modelling pyro-convective activity and the meteorological conditions leading to mega-fires, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8967, https://doi.org/10.5194/egusphere-egu23-8967, 2023.

EGU23-9394 | Orals | NH7.2

Health impacts of wildfire smoke in the Arctic 

Ben Silver, Steve Arnold, Louisa Emmons, Carly Reddington, and Luke Conibear

Climate change has increased the vulnerability of boreal forests and grasslands to wildfires. An increase in high-latitude wildfires has resulted in the deterioration of air quality, particularly in Western Siberia, where PM2.5 levels have increased at >1 µg m-3 year-1 during 1998−2020. Arctic wildfire carbon emissions have doubled during the last 20 years, and in Siberia they have shifted northwards. Using fire air pollutant emissions data from the Quick Fire Emissions Dataset (QFED), we create two emissions scenarios for Arctic Council member nations, with and without wildfires. PM2.5 is simulated for the two scenarios using the Community Earth System Model, which we evaluate using in-situ measurement data, finding a large negative bias in wildfire plumes. To correct this underestimation we use a high resolution PM2.5 reanalysis dataset, improving agreement with observations. Bias-corrected scenarios are used to estimate air quality degradation and resulting health impacts due to Arctic Council nation wildfires across the Northern Hemisphere high- and mid-latitudes for the period 2001-2020. We use the Global Exposure Mortality Model to estimate the health impacts of chronic exposure to Arctic wildfire-attributed PM2.5­. We find that health impacts are highly variable, with 25,000−55,000 premature deaths yearly, with most of the health burden falling on nations outside the Arctic Council, particularly China, due to transboundary transport of Siberian wildfire PM2.5. Health impacts have decreased during our study period partly due to the northwards shift in wildfires.

How to cite: Silver, B., Arnold, S., Emmons, L., Reddington, C., and Conibear, L.: Health impacts of wildfire smoke in the Arctic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9394, https://doi.org/10.5194/egusphere-egu23-9394, 2023.

EGU23-10286 | Posters on site | NH7.2

Atmosphere and fire interactions from the New Zealand experimental burn campaigns 

Marwan Katurji, Jiawei Zhang, Andres Valencia, Dongqi Lin, Tara Strand, Grant Pearce, Mark Finney, Craig Clements, and Shana Gross

Wildfires are increasing in intensity, frequency, and occurring earlier and later than normal on the seasonal timeline. Coupled atmosphere-flame-fuel dynamics makes wildfire a difficult phenomenon to understand and predict across its temporal and spatial spectrum of scales. This is especially true at the turbulence scale where rapid fluctuations of near-surface wind velocity and temperature within the atmosphere-fire boundary layer can control fire spread rates and extreme fire behavior. Appropriate observations from wildfires suitable for process-based investigations of coupled atmosphere-fire boundary layer dynamics do not exist, instead experimentally controlled fire burns are usually carried out. These experiments rely on repeated short-term wind driven fires that are usually restricted to certain meteorological regimes. Experimental design remains a challenging endeavor, which still lacks spatially coherent ambient and fire-induced atmospheric observations for understanding coupled dynamics. We have carried out several experimental fire burns in New Zealand for short stubble wheat and more dense and higher gorse shrubs. Our observations covered fuel properties, atmospheric turbulence, and flaming zone behavior. We have used uncrewed aerial vehicles carrying high speed infrared and visible video cameras, along with in-situ eddy covariance towers for ambient and fire-induced turbulence heat and momentum measurements. Some methodological highlights include the combination of image processing techniques, fuel density maps from aerial Lidar, and atmospheric turbulence structure analysis. We present a synthesis of research findings over the last two observational campaigns and introduce our new objectives for the upcoming crown fire forest canopy fire experiments. In addition, we discuss large eddy simulations of carefully designed numerical experiments allowing for a better understanding of the fire-atmosphere energetics at the atmospheric boundary layer scales.

How to cite: Katurji, M., Zhang, J., Valencia, A., Lin, D., Strand, T., Pearce, G., Finney, M., Clements, C., and Gross, S.: Atmosphere and fire interactions from the New Zealand experimental burn campaigns, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10286, https://doi.org/10.5194/egusphere-egu23-10286, 2023.

EGU23-10618 | ECS | Orals | NH7.2

Impact of climate change on the fire weather in Indian forests 

Anasuya Barik and Somnath Baidya Roy

Forest fires strongly depend on local weather conditions. Weather conditions conducive for occurrence and growth of fires is known as “fire weather”. This work investigates how climate change can affect the future fire weather in Indian forests using the Canadian Forest Fire Danger Rating System – Fire Weather Index (CFFDRS-FWI), a well-known fire danger assessment system. To drive this model, we used a high-resolution dynamically downscaled climate projection DSCESM for a baseline (2006-2015) and an end-century (2091-2100) period to compute the metric ‘Fire Weather Index (FWI)’. We divided the forest areas of the country into 5 zones based on climate and forest types viz., Himalayan (HIM), Northeast (NE), Central India (CEN), Deccan (DEC) and Western Ghats (WG) zones. Then, we developed thresholds for five fire weather danger classes using the baseline FWI in conjunction with observed fire count from MODIS active fire data. The baseline and future FWI, fire weather danger, Seasonal Severity Ratings (SSR) and characteristics of the fire weather season were compared to estimate the effect of climate change on forest fire danger.

Results show that there is considerable heterogeneity in the baseline as well as future fire weather danger across, and even within, the different forest zones of India. Climate change is likely to have a strong effect on fire weather. Days exceeding the Very High FWI threshold are likely to increase by about 30-40 days by the end-century despite a modest increase of about 5% in annual FWI values. SSR analysis suggests a maximum increase in fire disturbances during the pre-monsoon months of March-April-May.  About 55% of forest area over India will experience increased fire danger in this season. The least effect will be in the post monsoon season in September-October-November. The fire season is also expected to lengthen up to 59 days depending upon the forest type. The forests which are most likely to be affected by fire disturbances by end-century are moist deciduous and evergreen forests in the northern WG, mixed dry deciduous forests in central and southern CEN, Pine and Sal forests in the HIM and the scrub forests in the DEC zone. Climate change is unlikely to affect the fire weather danger in the NE.

This study is one of the first attempts to quantify the effects of climate change on forest fire hazard in India. It has significant policy implications and can be valuable for fire management authorities for designing appropriate fire suppression and mitigating measures.

 

How to cite: Barik, A. and Baidya Roy, S.: Impact of climate change on the fire weather in Indian forests, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10618, https://doi.org/10.5194/egusphere-egu23-10618, 2023.

EGU23-10736 | ECS | Orals | NH7.2

Flammable Futures – A storyline of climatic and land-use change impacts on wildfire extremes in Indonesia 

Shelby Corning, Esther Boere, Andrey Krasovskiy, Andrey Lessa-Derci-Augustynczik, and Florian Kraxner

Wildfire events are driven by complex interactions of the climate and anthropogenic interventions. Predictions of future wildfire events, their extremity, and their impact on the environment and economy must account for the interactions between these drivers. Economic policy and land use decisions influence the susceptibility of an area to climate extremes, the probability of burning, and future decision making. To better understand how climate-driven drought events and adaptation efforts affect burned area, agricultural production losses, and land use decisions, we developed a storyline approach centered on Indonesia’s 2015 fire events, which saw significant production losses of palm oil – a product imported by the EU chiefly as a biofuel – surpassing 7%. We explored analogous events under three warming conditions and two palm oil sector adaptation scenarios using two storylines: ensemble mean climate and high aridity conditions. We employed a model chain consisting of IIASA's wildfire climate impacts and adaptation model (FLAM) and the partial equilibrium global biosphere management model (GLOBIOM) to predict burned area and assess resultant production losses in the oil palm sector in Indonesia. To quantify the changes in burned area, we applied a delta approach based on the different degrees of global warming that can be expected. To define fire-induced oil palm losses and associated economic impacts, we combined the burned areas from FLAM with land-use change and productivity estimates from GLOBIOM. We found that the total burned area and production loss increased across the projections and climate warming by up to 25%, with only minor differences between storylines. By varying characteristics of regional climate change features, we found that these results are spatially explicit and robust across projections. Our results highlight the importance of including future warming and drought conditions in predicting oil palm losses and land use decision making. They leave room to explore how climatic and economic impacts could be mitigated through economic and land use management policies affecting Indonesia and the EU.

How to cite: Corning, S., Boere, E., Krasovskiy, A., Lessa-Derci-Augustynczik, A., and Kraxner, F.: Flammable Futures – A storyline of climatic and land-use change impacts on wildfire extremes in Indonesia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10736, https://doi.org/10.5194/egusphere-egu23-10736, 2023.

EGU23-10866 | Posters on site | NH7.2

Wildfires in Warming Siberia: Trends, Transportation and Implications on Arctic Climate 

Sang-Woo Kim, Yeonsoo Cho, Jin-Ho Yoon, Baek-Min Kim, and Jee-Hoon Jeong

Wildfires in carbon-rich northern high latitudes, especially Siberia, is an important phenomenon because it can worsen the air quality and accelerate warming over the Pan-Arctic regions. We investigate the shift of wildfire regimes in northern high latitudes over the recent decades using Moderate Resolution Imaging Spectroradiometer (MODIS) active fire data. Northeast Siberia has experienced a significant increase in the number of wildfires (+11.04 % year-1) and the mean period of events (+0.16 days year-1). Strengthened anomalous anti-cyclonic circulation from the surface to the upper troposphere over Northeast Siberia under the Pan-Arctic warming is responsible for more active wildfires over the last decades. This causes strong and long-lasting warm and dry conditions conducive to the ignition and persistence of wildfire. Additionally, extreme wildfire events in Northeast Siberia show that biomass-burning aerosols and gases are transported into the Arctic Ocean, contributing to the rapid melting of sea ice and snow by altering the surface radiation budget. These results suggest that extended wildfire activities in Northeast Siberia are critical to predicting the future Arctic climate.

How to cite: Kim, S.-W., Cho, Y., Yoon, J.-H., Kim, B.-M., and Jeong, J.-H.: Wildfires in Warming Siberia: Trends, Transportation and Implications on Arctic Climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10866, https://doi.org/10.5194/egusphere-egu23-10866, 2023.

EGU23-10923 | ECS | Posters on site | NH7.2

Fire-atmosphere dynamics at a rural-urban interface using turbulence-resolving meteorological simulations 

Dongqi Lin, Marwan Katurji, Andres Valencia, and Fearghal Gill

Human settlements in many regions have suffered great damage due to the escalating impacts of wildfires in recent decades. Most human activities have taken place over urban areas and/or Rural-Urban Interfaces (RUI). These areas have their unique vegetative and built fuels and structures, microclimates, and local wind flow dynamics. Despite the significant impacts of wildfires in RUI, only a small number of studies have been done to investigate fire-atmosphere dynamics and wildfire risk at RUI. The parallelized large eddy simulation model (PALM) system 6.0 was used to conduct simulations for a real RUI at Bottle Lake Forest, Christchurch, New Zealand. The simulations contain over 3000 residential buildings spreading around a large pine forest with an area of over 7 km2. Fine-scale simulations (Δx = 9 m and Δz = 2 m) were run for the complex rural-urban environment by using initial conditions obtained from larger-scale weather simulations using the Weather Research and Forecasting (WRF) model. A novel experimental-based method allowing for realisation of forest fire heat forcing was developed and implemented into PALM. Heat sources to simulate a forest fire were prescribed at two separate locations for the assessment of the impact of fire locations on wildfire risk on the RUI. In addition, the simulations were performed with two weather scenarios for daytime and night-time conditions, respectively. We aim to investigate the sensitivity of fire-atmosphere dynamic behaviour to different fire ignition locations and weather conditions. Our work specifically focuses on the resulting development of wind gusts and implications for potential firebrand transport paths within the surrounding urban canopy. 

How to cite: Lin, D., Katurji, M., Valencia, A., and Gill, F.: Fire-atmosphere dynamics at a rural-urban interface using turbulence-resolving meteorological simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10923, https://doi.org/10.5194/egusphere-egu23-10923, 2023.

EGU23-11003 | ECS | Orals | NH7.2

Studying air pollution and weather feedbacks from wildfires over Greece using WRF-Chem 

Anastasios Rovithakis and Apostolos Voulgarakis

Wildfires are a major source of atmospheric aerosols and can have significant impacts on air quality and radiative forcing. In our work, we have utilized the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) to study the impact of wildfires on aerosol pollution and meteorological feedbacks, focusing on the geographical area of Greece as a test case. We focus on the summer season of 2021, during which intense wildfire activity occurred in the country. We have performed sensitivity experiments with and without emissions from fires as a way to quantify the impact of such emissions on atmospheric pollutants, AOD, radiative forcing and weather variables (temperature, humidity, winds). Our results show that wildfires can have a significant impact on AOD, with the magnitude of the effect depending on the size and intensity of the wildfire and the meteorological conditions. Our recent work has shown that fire prone areas determined using the FWI index seem to link closely with the areas in Greece with the highest burnt area. Since the emitted aerosols are an important parameter, we test how well the emissions correlate to the FWI. Overall, our work demonstrates the potential role of wildfires in the evolution of short-term weather conditions via fire pollution radiative forcing, and provides new insights into the mechanisms leading to such effects.

How to cite: Rovithakis, A. and Voulgarakis, A.: Studying air pollution and weather feedbacks from wildfires over Greece using WRF-Chem, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11003, https://doi.org/10.5194/egusphere-egu23-11003, 2023.

EGU23-11045 | Posters on site | NH7.2

Wildfire Effects on Air Quality: A Case Study of Wildfires in Korea in 2022 

Dong Yeong Chang and Sujong Jeong

In March 2022, an unprecedented largest forest fire occurred in South Korea, burning 22,477 ha of forest for two weeks. In this study, we studied the causes of these fires based on an analysis of all meteorological data available over 100 years and also investigated their effects on air quality data obtained from ground-based observations (AirKorea and Asian Initiative for Clean Air Networks (AICAN)) and satellite data. Analysis results of meteorological data reveal changes in the climate regime from cold and wet winter conditions to hot and dry conditions. The temperature has been increased by 4 °C and precipitation has decreased by 17 mm over 100 years. The resistance level of forest fires is drastically reduced in the past few years and eventually lead to large-scale wildfires. These devastating wildfires emitted large amounts of ultrafine biomass-burning aerosols that were composed mainly of small particle sizes with diameters less than 1.0 mm. It elevated the air pollution level by more than 20 folds than usual condition. Carbon monoxide (CO) was also emitted from biomass burning that was detected as smoke paths (from 373 ppb to 1181 ppb) by the Tropospheric Monitoring Instrument (TROPOMI). This study highlights that climate change can make forests more vulnerable to fires and their effects on air quality could be more severe than expected.

This work was supported by the National Research Foundation of Korea (NRF) grant funded by the Korea government (MSIT) (No. RS-2022-00155875).

How to cite: Chang, D. Y. and Jeong, S.: Wildfire Effects on Air Quality: A Case Study of Wildfires in Korea in 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11045, https://doi.org/10.5194/egusphere-egu23-11045, 2023.

EGU23-11112 | Posters virtual | NH7.2

Hydrological impacts of wildfires at a global scale 

Manolis Grillakis and Apostolos Voulgarakis

Wildfires can affect the hydrological regime of a watershed until vegetation is reestablished and the hydrological cycle returns to its previous state. Wildfire induced changes can lead to increased high flows due to vegetation destruction that affects rainfall interception, evapotranspiration, but also fire induced soil imperviousness. Floods or water cycle changes after wildfire events have been extensively studied at a fire event and basin level, or at regional scale, yet changes at a global scale have not been studied systematically. Based on a wide discharge observation inventory from 651 basins globally and MODIS burned area data between 2001 and 2018, we show that the average annual discharge tends to increase in the first two years after the wildfire event, but gradually tends to return to its previous state. Furthermore, it is also found that high flow events tend to increase with wildfire size. This work focuses to a better understanding of the hydrological impacts of wildfires, and hence contribute to the improved modeling representation of fire – hydrology processes.

How to cite: Grillakis, M. and Voulgarakis, A.: Hydrological impacts of wildfires at a global scale, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11112, https://doi.org/10.5194/egusphere-egu23-11112, 2023.

EGU23-12974 | ECS | Posters virtual | NH7.2

Unravelling wildland fire morphology and structure using image velocimetry 

Andres Valencia, Marwan Katurji, Dongqi Lin, Shana Gross, Jiawei Zhang, Grant Pearce, Mark Finney, and Tara Strand

Wildland fires have been increasing in size, frequency and intensity during recent decades, affecting entire ecosystems and societies even in regions historically not considered fire prone. Some of those fires display dynamics of extreme fire behaviour, which chaotic and large-scale nature make them challenging to study. Thus, there is a need of new methodologies for wildland fire analysis, capable of capturing spatiotemporal characteristics suitable for this application. This work presents two applications of the image velocimetry technique applied to wildland fires, offering new details on the morphology and structure of large-scale medium-intensity prescribed shrubland fires, as well as an outlook on new applications in more complex scenarios. Fire flow displacement vectors and streamlines were calculated and mapped from a high-resolution overhead visible-spectrum (RGB) video acquired during a four-hectare prescribed gorse fire. This method allowed for identification of spatially interleaved flow convergence and divergence regions, providing insight on the high-level structure of the fire front and flaming zone. The method was further expanded to identify what we refer to as “fire sweeps”, via the application of a 2D convolution operation on the displacement vector based upon a kernel carefully designed to highlight the characteristics highly divergent fire flows.

How to cite: Valencia, A., Katurji, M., Lin, D., Gross, S., Zhang, J., Pearce, G., Finney, M., and Strand, T.: Unravelling wildland fire morphology and structure using image velocimetry, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12974, https://doi.org/10.5194/egusphere-egu23-12974, 2023.

EGU23-13877 | ECS | Posters on site | NH7.2 | Highlight

The 2022 fire season over Europe 

Mafalda Canelas da Silva, Rita Durão, Ana Russo, and Célia Gouveia

Over the summer of 2022, Europe experienced exceptional wildfire activity, with fires occurring more frequently and intensively, mainly in Spain, France, and Portugal. Together these countries registered more than 470 000 hectares of the total 786 000 burnt area in the European Union, accordingly to the estimates of the European Forest Fire Information System (EFFIS) for this fire season. 

Southern Europe is a widely known climate change hotspot resulting in heatwaves, droughts, and wildfire activity (increase in the number and severity of fires, burnt area, and longer fire seasons) although severe droughts and heatwaves have been expanding and worsening in central and northern Europe, increasing fire risk.

This work aims to evaluate how extreme the 2022 fire season was when compared with the period 1979-2021 over Europe. The proposed methods comprise the analysis of fire-related products and atmospheric variables to evidence the fire-prone weather conditions. The European Centre for Medium-Range Weather Forecast (ECMWF) ERA5 reanalysis dataset of Fire Weather Index (FWI) and air temperature, relative humidity and wind products are used. FWI is part of a dataset from the Canadian Fire Weather Index System, and is defined as a numerical rating of the potential frontal fire intensity, that indicates fire intensity by combining the rate of fire spread with the amount of fuel being consumed. The Standardized Precipitation Evapotranspiration Index (SPEI) at time-scales of 1 to 6 months was used to assess drought conditions.

Results highlight the new fire dynamics in Europe since climate change effects are leading to new emergent hot spots (central and northern Europe), not so well known as the Mediterranean Basin. This is extremely important to allow the assessment of fire danger activity as well as the characteristics of wildfires and improve the monitoring, planning, and mitigation activities.

How to cite: Canelas da Silva, M., Durão, R., Russo, A., and Gouveia, C.: The 2022 fire season over Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13877, https://doi.org/10.5194/egusphere-egu23-13877, 2023.

EGU23-14223 | ECS | Orals | NH7.2

Modelling the atmospheric factors determining the evolution of the boundary layer during a wildfire event 

Carolina Purificação, Cátia Campos, Alice Henkes, and Flavio T. Couto

Over mountainous terrain, the atmospheric structure becomes much more complex than homogeneous terrain in terms of the Atmospheric Boundary Layer (ABL). In the context of interaction between fire and atmosphere, abrupt changes in the ABL wind often lead to erratic and turbulent flow in the fire environment and expose firefighters to dangerous conditions. The study aims to characterize the ABL conditions associated with the largest forest fire that occurred in Portugal in 2019. The fire event took place in Vila de Rei county, which is surrounded by hills and valleys with large differences in altitudes. In order to study the regional scale, a numerical simulation was performed using the Meso-NH atmospheric model, configured with 500 × 500 grid points at 2500 m horizontal resolution, between 19 July at 0000 UTC and 25 July 2019 at 0000 UTC. The simulation covered the Iberian Peninsula and corresponds to the period when the fire burned more than 9,000 hectares in Vila de Rei. Such a simulation helped to characterize the lower troposphere, which contributed to the evolution of the ABL height over the days. Results indicate that the simulated ABL evolution is characterized by the presence of a coastal low-level jet with a maximum wind speed of 10 meters per second at ~ 600 meters’ altitude (1800 UTC of 20 July).  ABL height calculated from Richardson number method depicted a growing in the morning that reached a peak height by mid-afternoon. The ABL height ranged from 500 to 900 m throughout the afternoon and evening during the entire study period. Besides the identification of the fire weather conditions, this study also highlights the factors that contributed to the lower values of the ABL height in the wildfire event. This study was funded by national funds through FCT-Foundation for Science and Technology, I.P. under the PyroC.pt project (Ref. PCIF/MPG/0175/2019).

How to cite: Purificação, C., Campos, C., Henkes, A., and Couto, F. T.: Modelling the atmospheric factors determining the evolution of the boundary layer during a wildfire event, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14223, https://doi.org/10.5194/egusphere-egu23-14223, 2023.

EGU23-15493 | ECS | Posters on site | NH7.2

Measuring the Carbon Footprint from Wildfires and Crop Burning Using Satellite Data 

Raunaq Jain, Mitchell Odhiambo, Nikita Kaushal, Abhilash Mishra, and Yash Gorana

Climate change and altered land use patterns have increased the risk and frequency of wildfires over the last decade. Today's estimates of the carbon impact of wildfires deploy a bottom-up approach to estimate the amount of carbon released into the atmosphere. Various parameters and variability in this approach make it difficult to make quick and accurate estimations of the carbon emissions from wildfires. We propose using satellite data from NASA’s OCO-2 and MODIS satellites to directly estimate the amount of CO2 released into the atmosphere from wildfires. A similar approach can be used to measure carbon emissions from crop-burning activities in the Gangetic plains- another significant source of carbon emissions. Direct measurements of carbon emissions can help policymakers and researchers make data-based decisions to prevent forests from becoming carbon sources instead of carbon sinks. 

In our presentation, we will present a new data platform to estimate carbon emissions from localized wildfires and crop-burning instances using publicly available satellite data. The platform has pre-built functions and pipelines, allowing researchers to perform data analysis without the need to write cumbersome code. The underlying data lake combines NASA’s Orbiting Carbon Observatory (OCO-2 and OCO-3) data with other data sources (e.g., MODIS-based fire data) that facilitate more accurate and complete modeling of the dynamics of biomass burning and the impact they have on their immediate geography and the planet’s climate system at large.

How to cite: Jain, R., Odhiambo, M., Kaushal, N., Mishra, A., and Gorana, Y.: Measuring the Carbon Footprint from Wildfires and Crop Burning Using Satellite Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15493, https://doi.org/10.5194/egusphere-egu23-15493, 2023.

EGU23-16190 | Orals | NH7.2

Modeling wildfire dynamics and future projections under climate change scenarios: the FLAM approach 

Andrey Krasovskiy, Shelby Corning, Esther Boere, Nikolay Khabarov, Reinis Cimdins, and Florian Kraxner

We will present approaches to modeling wildfire dynamics using the IIASA’s wildFire cLimate impacts and Adaptation Model (FLAM). FLAM operates with a daily time step and uses mechanistic algorithms to parametrize the impacts of climate, human activities, and fuel availability on wildfire probabilities, frequencies, and burned areas. Validation on historical data and future projections under climate change scenarios will be discussed at various scales and resolutions.  We will present results for the following case-studies: (i) projections of global burned areas driven by climate change scenarios until 2100; (ii) modeling burned areas and adaptation options in Europe; (iii) modeling burned areas and their feedback to land-use change in Indonesia with a particular emphasis on extreme fires due the impacts of El Niño southern oscillation using historical data and the delta approach for future scenarios; (iv) regional variability and driving forces behind forest fires in Sweden. Our results support international analyses that, irrespective of changes in management, it is evident that climate change is very likely to increase the frequency and impact of wildland fires in the coming decades.

How to cite: Krasovskiy, A., Corning, S., Boere, E., Khabarov, N., Cimdins, R., and Kraxner, F.: Modeling wildfire dynamics and future projections under climate change scenarios: the FLAM approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16190, https://doi.org/10.5194/egusphere-egu23-16190, 2023.

The Salish Sea is a semi-enclosed coastal sea between Vancouver Island and the coast of British Columbia and Washington State, invaluable from both an economic and ecologic perspective. Pacific inflow to the Sea is the main contributor of many biologically important constituents. The contribution of Pacific water masses to the flow through Juan de Fuca Strait (JdF), the Salish Sea’s primary connection to the Pacific Ocean, is explored. Quantitative Lagrangian particle tracking using Ariane was applied to two numerical ocean models (CIOPS-W in the shelf region, and SalishSeaCast in the Salish Sea) matched together within JdF. Water parcels seeded near the entrance of JdF were integrated forwards and backwards in time to assess water mass path (and properties while on this path) from the shelf region and once within the Salish Sea in more detail than previously possible. During summer upwelling, intermediate flow from the north shelf and offshore dominate inflow, while during winter downwelling, intermediate flow from the south shelf and surface flow from the Columbia River plume are the dominant sources. A weaker and less consistent estuarine flow regime in the winter led to less Pacific inflow overall and a smaller percentage of said inflow reaching the Salish Sea's inner basins than in the summer. Nevertheless, it was found that winter dynamics are the main driver of interannual variability, in part due to the strongly anti-correlated behaviour and distinct properties of the two dominant winter sources. This analysis extends the knowledge on the dynamics of Pacific inflow to the Salish Sea and highlights the importance of winter inflow to the interannual variability in biogeochemical conditions in the region.

How to cite: Beutel, B. and Allen, S.: Interannual and seasonal water mass analysis in the Salish Sea using Lagrangian particle tracking, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-316, https://doi.org/10.5194/egusphere-egu23-316, 2023.

EGU23-2725 | ECS | Posters on site | NP6.3

Lagrangian Spatiotemporal Fingerprints of Dissolved Inorganic Carbon in Eighteen Degree Water Formation 

Daan Reijnders, Dorothee Bakker, and Erik van Sebille

Mode waters are defined as thick, weakly stratified layers with homogeneous properties. They have the ability to store these properties, such as heat, carbon and nutrients, and exchange these with the surface or atmosphere during outcropping events or with other layers via mixing processes. Eighteen Degree Water (EDW) is the subtropical mode water of the western North Atlantic. Its yearly outcropping events in late winter makes it an important regulator of ocean heat, nutrients and carbon in the North Atlantic on annual timescales.

Previous studies have given insight into the formation and destruction of Eighteen Degree Water. These have largely focused on physical aspects such as EDW formation rates. Due to the importance of EDW formation in setting the biogeochemical environment in the North Atlantic, it is instructive to investigate how biogeochemical tracers are altered along EDW formation routes. This study investigates in particular how dissolved inorganic carbon (DIC) is altered along ocean water parcel trajectories as EDW is formed. To do so, we compute Lagrangian trajectories of subducted EDW backwards in time using a coupled hydrodynamic and biogeochemical model. By sampling biogeochemical tracer values along Lagrangian pathways, we construct timeseries which we use to map the dominant locations at which DIC concentrations are altered in space and time to identify the Lagrangian fingerprint of DIC in Eighteen Degree Water.

How to cite: Reijnders, D., Bakker, D., and van Sebille, E.: Lagrangian Spatiotemporal Fingerprints of Dissolved Inorganic Carbon in Eighteen Degree Water Formation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2725, https://doi.org/10.5194/egusphere-egu23-2725, 2023.

EGU23-3970 | ECS | Posters on site | NP6.3 | Highlight

Lagrangian trajectories to assess marine plastic pollution distribution in the Canary Islands 

Marcos Cividanes García, Borja Aguiar González, May Gómez Cabrera, Alicia Herrera Ulibarri, Ico Martínez Sánchez, Ángel Rodríguez Santana, and Francisco José Machín Jiménez

The increasing presence of plastics in the ocean is a harmful problem for marine ecosystems and the socio-economic sector. A recurrent type of debris gathered in waters of the Canary Islands are the identification tags employed at lobster traps deployed at the north-eastern coast of North America. Since 2016 to the present, these debris have been routinely collected and classified by the EOMAR group (MICROTROFIC Project) through coastal sampling focused on the eastern part of the Canary archipelago. In order to address this problem, a further understanding of the distribution and dynamics of these debris in the ocean is demanding. In this work, a pre-existing tool in Matlab has been upgraded to produce Lagrangian trajectories based on Marine Copernicus surface current velocity (GLORYS12V1). The main goal is to assess the trajectories that floating particles might follow in the North Atlantic subtropical gyre when released over a grid in the north-eastern coast of North America (Gulf of Maine). Our results provide a quantitative basis about the link between the North American north-eastern coast and the Canary Islands, where the presence of these and other debris is of increasing concern.

How to cite: Cividanes García, M., Aguiar González, B., Gómez Cabrera, M., Herrera Ulibarri, A., Martínez Sánchez, I., Rodríguez Santana, Á., and Machín Jiménez, F. J.: Lagrangian trajectories to assess marine plastic pollution distribution in the Canary Islands, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3970, https://doi.org/10.5194/egusphere-egu23-3970, 2023.

EGU23-4003 | ECS | Orals | NP6.3

Quasi-Objective Eddy Visualization from Sparse Drifter Data 

Alex Pablo Encinas Bartos, Nikolas O. Aksamit, and George Haller

Lagrangian eddies, generally referred to as elliptic Lagrangian coherent structures (LCS) in the dynamical systems literature, are material objects that trap and transport floating particles over large distances in the ocean in a coherent fashion. In order to expand our understanding of the transport of marine tracers, we need to accurately and reliably track the evolution of vortical flow structures. Drifter trajectories represent a valuable but sparse source of information for this purpose. We employ a recently developed single-trajectory Lagrangian diagnostic tool, the trajectory rotation average (TRA), to visualize oceanic vortices (or eddies) from sparse drifter data in a quasi-objective fashion. We apply the TRA to two drifter data sets that cover various oceanographic scales: the Grand Lagrangian Deployment (GLAD) and the Global Drifter Program (GDP). Based on the TRA, we develop a general algorithm that extracts approximate eddy boundaries. We find that the TRA outperforms other available single-trajectory-based eddy detection methodologies on sparse drifter data and identifies eddies on scales that are unresolved by satellite-altimetry.

How to cite: Encinas Bartos, A. P., O. Aksamit, N., and Haller, G.: Quasi-Objective Eddy Visualization from Sparse Drifter Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4003, https://doi.org/10.5194/egusphere-egu23-4003, 2023.

EGU23-6036 | Orals | NP6.3

A versatile Lagrangian-data aggregation framework for marine biological dispersal studies 

Willi Rath, Lara Schmittmann, Carola Trahms, Felix Kirch, Leon Mock, and Arne Biastoch

Lagrangian particle dispersal simulations are widely used for studying directed connectivity between different locations in the ocean. They are used, both, for the understanding of ocean physics and for interdisciplinary questions. One biological example is the dispersal of passively drifting marine organisms.

The typical modus operandi of such “bio-physical” studies is to design an underlying Lagrangian simulation in close synchronisation with a specific biological research question. This leads to a conflation of concerns between physical and biological aspects of the study. This conflation might result in repeated and slow development cycles of re-calculation for different scenarios and hence inhibit scientific progress.

We aim at improving the separation of concerns between biological and physical components for bio-physical Lagrangian studies, by aggregating physical Lagrangian data into directed multigraphs encoding locations as nodes and multiple parallel pathways as directed edges. Those graphs condense the physics-based information on directed oceanic relations and thus serve as a basis for simultaneously answering various biological questions on connectivity. As the proposed aggregation retains the distinction of different pathways between locations, it can, to some extent, also provide information of underway environmental conditions. This greatly enhances the range of applications of our approach over existing aggregations of Lagrangian data as connectivity probability graphs.

We present a specific set of biological case studies — the multi-year spreading of two oyster diseases in the North Sea — and develop a framework that facilitates efficiently and simultaneously testing multiple biological hypotheses for marine diseases of various species based on the same processed physical data set.

How to cite: Rath, W., Schmittmann, L., Trahms, C., Kirch, F., Mock, L., and Biastoch, A.: A versatile Lagrangian-data aggregation framework for marine biological dispersal studies, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6036, https://doi.org/10.5194/egusphere-egu23-6036, 2023.

EGU23-6537 | ECS | Orals | NP6.3

Forecast of Particle Spreading Using Machine Learning in a Complex Multiple-Inlet Coastal System 

Jeancarlo M. Fajardo-Urbina, Yang Liu, Ulf Gräwe, Sonja Georgievska, Meiert W. Grootes, Herman J.H. Clercx, Theo Gerkema, and Matias Duran-Matute

The implementation of continuous operational forecast systems using numerical models for coastal environments are scarce, computationally expensive, and difficult to maintain. As an alternative, computationally cheaper tools such as machine learning models can be employed. This is especially relevant when the time to produce a forecast is paramount like in oil spills, marine litter spread due to container-ship accidents, and search and rescue operations. Working in this direction, we tested the skill of an advanced deep learning model, namely a convolutional long short-term memory network (ConvLSTM), to predict the Lagrangian advection (the displacement vector of the center of mass) and the dispersion (the spread described by a covariance matrix) of patches of passive tracers. This model was trained with data from a realistic numerical simulation of the Dutch Wadden Sea: a multiple-inlet system of great ecological importance. Using the relevant drivers (wind, tidal amplitude, and atmospheric pressure), the model was set to learn the advection and dispersion after one tidal period of clouds of particles released on a 200 x 200 m grid, covering the entire DWS. Our results show that the model learned the system-wide temporal variability of both advection and dispersion, while the local spatial features were better reproduced for advection than for dispersion. We use the predicted advection and dispersion as inputs to a set of stochastic differential equations for the reconstruction of particle trajectories, as it is commonly done in particle tracking applications that employ diffusion instead of dispersion. We were able to predict the temporal evolution over several tidal periods of particle patches released from specific locations under contrasting cases like calm and stormy conditions. Our method was employed to predict only the horizontal spreading, but it can be extended to predict the 3D evolution of the particle clouds. Finally, our approach requires simulation data and relevant drivers (e.g. atmospheric forcing and tidal amplitudes) for training and the same drivers from any typical forecast systems for forecasting the evolution of particle patches, which makes it a promising operational tool.

How to cite: Fajardo-Urbina, J. M., Liu, Y., Gräwe, U., Georgievska, S., Grootes, M. W., Clercx, H. J. H., Gerkema, T., and Duran-Matute, M.: Forecast of Particle Spreading Using Machine Learning in a Complex Multiple-Inlet Coastal System, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6537, https://doi.org/10.5194/egusphere-egu23-6537, 2023.

EGU23-7212 | ECS | Orals | NP6.3

Lagrangian tracer spreading in surface ocean turbulence with ageostrophic dynamics 

Michael Maalouly, Gilmar Mompean, and Stefano Berti

Ocean submesoscales are characterized by horizontal scales smaller than approximately 10 km that evolve with timescales of O(1) day. Due to their small size and rapid temporal evolution, they are notoriously difficult to measure. In particular, the associated velocity field is not resolved in current satellite altimetry products. At these scales, surface ocean flows are populated by small eddies, and filaments linked with strong gradients of physical properties, such as temperature. Several recent studies indicate that submesoscale fronts are associated with important vertical velocities, thus playing a significant role in vertical transport. On that account, these fine-scale flows are key to the dynamical coupling between the interior and the surface of the ocean, as well as to plankton dynamics and marine ecology. In spite of their importance, the understanding of submesoscale ocean dynamics is still incomplete. In particular, a relevant open question concerns the role played by the ageostrophic components of the surface velocity field that manifest at these scales.

By means of numerical simulations, we investigate ocean submesoscale turbulence in the SQG+1 model, which accounts for ageostrophic motions generated at fronts, and which is obtained as a small-Rossby-number approximation of the primitive equations. In the limit of vanishing Rossby number, this system gives surface quasi-geostrophic (SQG) dynamics. In this study, we explore the effect of the ageostrophic flow components on the spreading process of Lagrangian tracer particles on the horizontal. We particularly focus on the characterization of pair-dispersion regimes and particle clustering, as a function of the Rossby number, using different indicators. The observed Lagrangian behaviours are further related to the structure of the underlying turbulent flow. We find that relative dispersion is essentially unaffected by the ageostrophic flow components. However, these components are found to be responsible for (temporary) particle aggregation in cyclonic frontal regions. These results appear interesting for the modelling of submesoscale dynamics and for comparison purposes with the new high-resolution surface current data that will be soon provided by the satellite SWOT.

How to cite: Maalouly, M., Mompean, G., and Berti, S.: Lagrangian tracer spreading in surface ocean turbulence with ageostrophic dynamics, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7212, https://doi.org/10.5194/egusphere-egu23-7212, 2023.

EGU23-7220 | ECS | Orals | NP6.3

Impact of Model Resolution on Mixing and Dispersion in the Gulf of Mexico 

Nektaria Ntaganou, Eric Chassignet, and Alexandra Bozec

We investigate the importance of model resolution in identifying the nature of mixing and dispersion in the Gulf of Mexico, by comparing two data-assimilative, high-resolution simulations, one of which is submesoscale-resolving. By employing both Eulerian and Lagrangian metrics, upper-ocean differences between the mesoscale- and submesoscale-resolving simulations are examined. Focusing on regions characterized by high submesoscale activity, we approach the notion of mixing by tracking the generation of Lagrangian Coherent Structures (LCSs) and transport barriers. Finite-time Lyapunov exponents (FTLE) fields reveal higher separation rates of fluid particles in the submesoscale-resolving case which indicates more vigorous mixing. Using probability density functions (PDFs), the extent of mixing homogeneity is also explored, with preliminary results suggesting that mixing is more homogeneous in the submesosclae-resolving case. Finally, we aim to identify regions of convergence in the areas of interest by advecting passive tracers that tend to organize themselves along attracting LCSs. Applications of passive tracer advection are then translated to extreme event situations, such as the Deepwater Horizon.  

How to cite: Ntaganou, N., Chassignet, E., and Bozec, A.: Impact of Model Resolution on Mixing and Dispersion in the Gulf of Mexico, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7220, https://doi.org/10.5194/egusphere-egu23-7220, 2023.

EGU23-8646 | Orals | NP6.3

Mixing and transport across the Atlantic Meridional Overturning Circulation: a 3D geometrical perspective 

Ana M. Mancho, Renzo Bruera, Jezabel Curbelo, and Guillermo Garcia-Sanchez

Vertical motions across the ocean are central to processes, like CO2 fixation, heat removal or pollutant transport, which are essential to the Earth’s climate. This presentation describes 3D conveyor routes across the Atlantic Meridional Overturning Circulation (AMOC), with the support of Lagrangian Coherent Structures. Our findings show the geometry of mixing structures in the upper and deep ocean layers. We identify among others, zones linked to vertical transport and characterize vertical transport time scales.

 

Acknowledgments: RB acknowledges support of a CSIC JAE intro fellowship.  AMM and GGS acknowledge the support of a CSIC PIE project Ref. 202250E001 and MICINN grants PID2021-123348OB-I00 and EIN2020-112235. AMM is an active member of the CSIC Interdisciplinary Thematic Platforms POLARCSIC. JC acknowledges the support of the RyC project RYC2018-025169, the Spanish grant PID2020-114043GB-I00 and the Catalan Grant No. 2017SGR1049 and the ``Beca Leonardo a Investigadores y Creadores Culturales 2022 de la Fundación BBVA''.

How to cite: Mancho, A. M., Bruera, R., Curbelo, J., and Garcia-Sanchez, G.: Mixing and transport across the Atlantic Meridional Overturning Circulation: a 3D geometrical perspective, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8646, https://doi.org/10.5194/egusphere-egu23-8646, 2023.

On 13 August 2021, the Fukutoku-Okanoba submarine volcano in the North Pacific Ocean was erupted. Satellites detected many pumice rafts that drifted westward to reach southern Japan in about two months. To cope with potential danger due to the pumice rafts, it is crucial to predict their trajectories. Using a Lagrangian particle tracking model, the trajectories of the rafts were investigated. The model results showed strong sensitivity to the windage coefficient of pumice rafts, which is uncertain and could cause large errors. By comparing the model results with satellite images using a skill score, the distance between a simulated particle and the nearest observed raft divided by the travel distance of the particle, an optimal windage coefficient was estimated. The optimal windage coefficients ranging between 2 to 3% produced pathways comparable to the obervation using satellites. The pumice rafts  moved from Fukutoku-Okanoba, toward the Ryukyu Islands for approximately two months before being pushed toward Taiwan by the intensified wind. The techniques presented here may become helpful in managing coastal hazards due to diverse marine debris.

How to cite: Park, Y.-G., Iskandar, M. R., kim, K., and Jin, H.: Tracking the pumice rafts from the recent eruption of the submarine volcano Fukutoku-Okanoba, Japan using Satellites and Lagrangian Particles tracking, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10296, https://doi.org/10.5194/egusphere-egu23-10296, 2023.

EGU23-11091 | Posters virtual | NP6.3

Detection of materially coherent eddies in the Bay of Bengal 

Lijin Jayan, Jishad Mandayi, Neeraj Agarwal, Rashmi Sharma, and Manikandan Mathur

Eddies are prominent features in the ocean and these energetic circulatory motions influence lateral and vertical transport of heat, mass and momentum. Ability of these eddies to coherently transport various scalar species is an important consideration in understanding freshwater transport, locating regions of harmful algal blooms, oxygen deficient zones and potential fishing zones. In this study, we present an implementation of Lagrangian Averaged Vorticity Deviation (LAVD) technique to detect materially coherent eddies from satellite derived sea surface currents in the Bay of Bengal (BoB). We also evaluate the efficacy of a Eulerian method based on sea surface height (SSH) in capturing materially coherent eddies in the BoB. Parameter values for robust detection of eddies are determined by performing a systematic sensitivity analysis in both the methods. Finite time material behaviour of eddies detected using both the methods are evaluated by numerical particle advection experiments. We then focus on material coherence of Sri Lanka Dome (SLD), an annually occurring cyclonic eddy of dynamical relevance in the BoB. SLD characteristics including its spatio-temporal evolution is discussed by analysing ocean surface currents data spanning 27 years from 1993 to 2019.

How to cite: Jayan, L., Mandayi, J., Agarwal, N., Sharma, R., and Mathur, M.: Detection of materially coherent eddies in the Bay of Bengal, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11091, https://doi.org/10.5194/egusphere-egu23-11091, 2023.

EGU23-13939 | ECS | Orals | NP6.3

Inertial effects on the transport of an anisotropic particle in surface gravity waves 

Himanshu Mishra and Anubhab Roy

We study the transportation and rotational dynamics of a finite-sized spheroidal particle in a linear monochromatic surface gravity wave to better understand the transport dynamics of microplastics in oceanic flows. A spheroidal particle, modeled as an anisotropic tracer, attains preferential alignment in a linear wavy flow. We analyze the drift of a finite-size anisotropic particle and find that the horizontal drift of such particles can either increase or decrease depending on the initial orientation and the ratio of the size of the particle to the wavelength of the background wave field. Next, we derive the finite-size modification to the preferred alignment of the spheroidal particle with the flow propagation direction of the wave. In most scenarios, particles in the ocean can have a wide range of densities and are classified into positively and negatively buoyant particles. Negatively buoyant particles settle in a wavy flow with complex trajectories. We study the effect of the orientation and size of such particles on settling and show that the aspect ratio of the particle could alter the trajectory in the wave propagation direction. We also obtain a non-zero vertical Stokes drift. Finally, we consider the effects of fluid and particle inertia in our coupled evolution equations and study the drift and the orientation of an anisotropic particle in a wavy flow field. We demonstrate that considering such an effect could provide a complete picture of the transport and dynamics of microplastics in the upper part of the ocean that can be described more accurately. 

How to cite: Mishra, H. and Roy, A.: Inertial effects on the transport of an anisotropic particle in surface gravity waves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13939, https://doi.org/10.5194/egusphere-egu23-13939, 2023.

EGU23-14947 | Posters on site | NP6.3

Small-scale Lagrangian modelling of air bubbles and oil droplets under breaking waves 

Tor Nordam and Arsalan Mostaani

Lagrangian transport modelling is commonly applied for marine environmental transport problems. When applied to problems on a timescale of days to weeks, such as marine oil spills, Lagrangian models are often forced with environmental data from operational models for atmosphere, waves and ocean currents. These models typically have a temporal resolution of around 1 hour. Effects that take place on shorter timescale, such as entrainment of oil droplets and air bubbles due to breaking waves, must therefore be parametereised.

On short timescales, the random flight approach is clearly more realistic than a random walk, since the particles have a well-defined and realistic velocity, regardless of the length of the timestep, and since particles in real turbulence do not instantaneously change their direction by arbitrarily large amounts. A consequence of this is that in random flight, particles exhibit superdiffusion on short timescales, and normal diffusion on long timescales, compared to the de-correlation time of the turbulent motion. Random walk methods, on the other hand, always behave as diffusion. Hence, random flight methods are expected to be more relevant for small-scale modelling of transport on short timescale under breaking waves.

Here, we consider small-scale modelling of oil droplet and air bubble entrainment, modelling the transport close to the surface, and at high temporal resolution. We use two different Lagrangian methods: random walk (AR0) and random flight (AR1), and compare the two modelling approaches to each other, as well as to pre-existing parameterisations of the average effects of entrainment. Input parameters to the Lagrangian models are informed by experimental turbulence measurements in a wave flume, and RANS-modelling of the breaking wave. Comparison of particle transport to observations in experimental flume work is ongoing.

How to cite: Nordam, T. and Mostaani, A.: Small-scale Lagrangian modelling of air bubbles and oil droplets under breaking waves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14947, https://doi.org/10.5194/egusphere-egu23-14947, 2023.

EGU23-15421 | ECS | Posters on site | NP6.3

Lagrangian dynamics of heavy inertial particles on vortical flows 

Anu Viswanathan Sreekumari Nath and Anubhab Roy

We study the dynamics of dust particles in various vortical flows which is relevant to geophysical context. The inertial particles are advected by the background vortex flow. The dynamics is tracked using the Maxey-Riley equation. The finite inertia of the particles make their dynamics different from passive fluid parcels, which is interesting. The dust particles may show periodic dynamics or chaotic diffusion depending on parametric variations. The result contradicts the earlier predictions that only density matched inertial particles can have chaotic dynamics, which we justify through our explanation. In addition, the heavy inertial particles in a self rotating vortex patch is observed to be attracted near the vortical region, which is contrary to the physics where they should ideally centrifuged out. The reason behind this phenomena also we explore in detail here.

How to cite: Viswanathan Sreekumari Nath, A. and Roy, A.: Lagrangian dynamics of heavy inertial particles on vortical flows, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15421, https://doi.org/10.5194/egusphere-egu23-15421, 2023.

EGU23-15441 | ECS | Posters on site | NP6.3

Measurements of bubble size distribution underneath breaking waves 

Arsalan Mostaani, Tor Nordam, and Emlyn Davies

Entrainment of particles by breaking waves are an important process for several applications. For example, entrainment of air bubbles is relevant for air-sea gas exchange, which in turn is relevant for climate modelling. Entrainment of oil droplets in a marine oil spill will have an effect on the fate of the oil, and help determine environmental effects. Hence, being able to measure and model these entrainment effects are important.

We are conducting experiments in a linear wave flume, with piston-type wave maker, looking at entrainment of air bubbles under breaking waves. Using a camera system with a uniform backlight and a telecentric lens, the SINTEF SilCam, we can image bubbles ranging in size from tens of micrometers, to cm scale. By accurately constraining the measurement volume, we can determine concentration of bubbles of different sizes. Taking images at high frequency, and repeating the same breaking wave many times, we are able to measure the time-development of the ensemble-average bubble size distribution.

In this poster, we describe the camera system and the image analysis pipeline, and we present some preliminary results and discuss some of the inherent challenges in measuring bubble size distributions close to the surface underneath breaking waves.

How to cite: Mostaani, A., Nordam, T., and Davies, E.: Measurements of bubble size distribution underneath breaking waves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15441, https://doi.org/10.5194/egusphere-egu23-15441, 2023.

EGU23-58 | ECS | Orals | NH1.5

Seasonal and regional distribution of lightning fraction over Indian Sub-continent 

Rakesh Ghosh, Sunil D Pawar, Anupam Hazra, and Jonathan Wilkinson

The three years of IITM LLN lightning observation data are used to determine the seasonal and spatial (over different geographical locations) distribution of the ratio of intra-cloud lightning (IC) to cloud-to-ground lightning (CG) in thunderstorms over the Indian sub-continent. The ratio is high (8-10) in the north-western parts and low (0.3-3) in the north-eastern parts. There is not a prominent latitudinal variation of IC and CG ratio, but a climatological seasonal variability exists all over the regions. In the Pre-monsoon (March to May), the mean ratio is observed at 3.87 with a standard deviation of 0.74, and during Monsoon (June to September), that is 3.01 with a standard deviation of 0.52. Pre-monsoon thunderstorm exhibits more IC discharge comparatively monsoonal thunderstorms; hence IC:CG ratio is also high in pre-monsoon. We have observed that CG lightning is approximately 20% of total lightning in pre-monsoon whereas 25% of total lightning in monsoon all over the Indian region. High CAPE associated with a stronger vertical updraft enhances the cold cloud depth and expands the mixed phase region, which can broaden and uplift the size of the upper positive charge center inside a thunderstorm while the middle negative charge center remains at the same temperature level. Therefore it enhances the occurrence of IC discharge between the upper positive charge center and middle negative charge center, hence increasing the IC:CG ratio of a thunderstorm. The implication of these observed results has the importance of separating CG lightning flash from total and can be used in the numerical model to give a proper prediction of CG lightning in hazard mitigation.

 

How to cite: Ghosh, R., Pawar, S. D., Hazra, A., and Wilkinson, J.: Seasonal and regional distribution of lightning fraction over Indian Sub-continent, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-58, https://doi.org/10.5194/egusphere-egu23-58, 2023.

EGU23-657 | ECS | Orals | NH1.5

Multi-station observation of periodic variations in long-term Schumann resonance records 

José Tacza, Tamás Bozóki, Gabriella Satori, József Bór, Anne Neska, Tero Raita, Ciaran Beggan, Mike Atkinson, Ashwini Kumar Sinha, and Rahul Rawat

Lightning has been declared as a new Essential Climate Variable by the World Meteorological Organization. Schumann resonance is a valuable parameter to monitor the global lightning activity, thus, the Atmospheric Observation Panel for Climate accepted Schumann resonance (SR) measurements as an emerging tool for studying lightning-related large-scale processes in the atmosphere. Previous studies showed a clear extraterrestrial influence on the SR parameters at different time scales (e.g., solar cycle). For all these reasons, a growing new interest arises in the scientific community to exploit the potential of SR better in gaining more information on electrodynamic coupling mechanisms taking place in the atmosphere. This has motivated the installation of new instruments worldwide to monitor SR measurements.

We performed a multi-station spectral analysis of the SR parameters (frequency and intensity) by using wavelet transformation. SR records from different monitoring sites around the globe were analyzed simultaneously for the first time: Hornsund (~12 years of data) and Belsk (~7 y.) managed by Poland, Rovaniemi and Ivalo in Finland (~16 y.), Eskdalemuir in Scotland (~10 y.), Nagycenk in Hungary (~22 y.), Boulder Creek in USA (~4 y.) and Shillong in India (~9 y.). For all SR sites, the periodicities of 0.5, 1, ~180 and 365-day appeared both in the frequency and the intensity of SR modes. Evidence was also found for the ~27- and ~45-day periods at specific time intervals. Cross-wavelet transform and wavelet coherence analyses were made between SR frequencies and the Kp index, and between SR intensities and Madden-Julian Oscillation index. Time periods of highly coherent 27-day as well as 45-day periodicities were found in the time series of these parameters intermittently. These preliminary results suggest that these periodicities are likely related to the solar rotation and Madden-Julian Oscillation, respectively. A detailed analysis about our findings will be presented and discussed.

How to cite: Tacza, J., Bozóki, T., Satori, G., Bór, J., Neska, A., Raita, T., Beggan, C., Atkinson, M., Kumar Sinha, A., and Rawat, R.: Multi-station observation of periodic variations in long-term Schumann resonance records, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-657, https://doi.org/10.5194/egusphere-egu23-657, 2023.

EGU23-795 | ECS | Orals | NH1.5

Changes in thunderstorm activity at high latitudes observed at WMO weather stations 

Daniel Kępski and Marek Kubicki

Knowledge about the occurrence of thunderstorms in polar regions is still limited. Lightning detection systems have varying detection efficiency over time and space, which makes climatological analysis difficult. This is especially problematic in areas where lightning strikes are relatively rare. Traditional observations carried out at weather stations are therefore still a very important source of information about the occurrence of thunderstorms in the polar and circumpolar regions. Scientific studies usually predict that these phenomena will be more frequent in high latitudes in a warmer world. To check whether the number of thunderstorms changes as projected, we summarize SYNOP data from manned World Meteorological Organization (WMO) stations operating in the years 2000-2019 located at latitudes above 60° of both hemispheres. According to this source, the changes in thunderstorm frequency are only visible in certain areas and mostly during the summer months. The regional Kendall test revealed a statistically significant increase in the number of thunderstorm days north of 60°N in Interior Alaska, northwestern Canada, much of Siberia and European Russia. However, a decrease in thunderstorm frequency has also been detected in some regions. This was the case on the shores of the southern Norwegian Sea and seasonally in spring in the northern Urals. The largest increase in thunderstorm days exceeded 5 per decade in the highly continental regions of central Siberia and interior Alaska. For the entire high-latitude area, the change in the number of days with thunderstorms was statistically insignificant. However, the statistically relevant increase in the number of thunderstorm days is visible for inland weather stations located 250 – 1,000 km from the coastline, where it was on average 1 day per decade.

How to cite: Kępski, D. and Kubicki, M.: Changes in thunderstorm activity at high latitudes observed at WMO weather stations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-795, https://doi.org/10.5194/egusphere-egu23-795, 2023.

The ground-level potential gradient atmospheric electric field, the air conductivity, and concentration of cloud condensation nuclei have been recorded at Stanislaw Kalinowski Geophysical Observatory in Świder, Poland (52°07' N, 21°14' E), for several decades. A new digitisation project of Świder atmospheric electric data published in the observatory year books provides an opportunity to review the results of studies of the long-term variation of the electric parameters. New results of an analysis of both short-term and long-term variations in the positive conductivity and related component of the air-Earth current density are presented, and implications for the Global Electric Circuit studies using the Świder dataset are discussed. This work is supported by Poland National Science Centre grant no 2021/41/B/ST10/04448.

How to cite: Odzimek, A., Pawlak, I., and Kępski, D.: Analysis of long-term variations in fair-weather PG, the positive air conductivity and conduction current density at Geophysical Observatory in Świder, Poland, and implications for the Global Electric Circuit, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-977, https://doi.org/10.5194/egusphere-egu23-977, 2023.

The ground-level atmospheric potential gradient (PG) has been measured with a radioactive collector method in Stanislaw Kalinowski Geophysical Observatory in Świder, Poland, for several decades. The observations have been previously analysed by Kubicki et al. (ICAE 2003, ICAE 2007) revealing rather typical behaviour in the diurnal and seasonal variations of the PG of a land station controlled by pollution. Electric field measurements at such station usually show a maximum at local winter months which are mostly affected by anthropogenic pollution. The whole series has been newly analysed to describe the Świder PG variations in greater detail, also in connection with an analysis of simultaneous measurements of cloud condensation nuclei. Fair-weather potential gradient course is calculated in different time scales (annual, seasonal and diurnal) with taking into account local meteorological and air pollution conditions. An attempt is made to calculate the diurnal and seasonal variations at very low cloud condensation nuclei counts. The work is supported by Poland National Science Centre grant no 2021/41/B/ST10/04448.

How to cite: Pawlak, I., Kępski, D., Tacza, J., and Odzimek, A.: New analysis of diurnal and seasonal variations in fair-weather atmospheric potential gradient and cloud condensation nuclei measured in S. Kalinowski Geophysical Observatory in Świder, Poland, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-978, https://doi.org/10.5194/egusphere-egu23-978, 2023.

EGU23-1480 | Orals | NH1.5

Employing Optical Lightning Data to identify lightning flashes associated to Terrestrial Gamma-ray Flashes 

Christoph Köhn, Matthias Heumesser, Olivier Chanrion, Victor Reglero, Nikolai Østgaard, Hugh Christian, Timothy Lang, Richard Blakeslee, and Torsten Neubert

Terrestrial gamma-ray flashes (TGFs) are bursts of energetic X- and gamma-rays emitted from thunderstorms and observed by the Atmosphere-Space Interactions Monitor (ASIM) mounted onto the International Space Station (ISS) detecting TGFs and optical signatures of lightning. ISS-LIS (Lightning Imaging Sensor) detects lightning flashes allowing for simultaneous measurements with ASIM. Whilst ASIM measures ~300-400 TGFs per year, ISS-LIS detects ~ 106 annual lightning flashes giving a disproportion of four orders of magnitude. Hence, based on the temporal evolution of lightning flashes and their spatial pattern, we present an algorithm to reduce the number of flashes potentially associated with TGFs by ~90%, and we use the ASIM TGF list to ensure that the resulting flashes are those associated with TGFs and thus benchmark our algorithm. We will compare how the radiance, footprint size and the global distribution of lightning flashes of the reduced set relates to the average of all measured lightning flashes. Finally, we will present a parameter study of our algorithm and discuss which parameters can be tweaked to maximize the reduction efficiency whilst keeping those flashes associated to TGFs. In the future, this algorithm will hence facilitate the search for TGFs in a reduced set of lightning flashes.

How to cite: Köhn, C., Heumesser, M., Chanrion, O., Reglero, V., Østgaard, N., Christian, H., Lang, T., Blakeslee, R., and Neubert, T.: Employing Optical Lightning Data to identify lightning flashes associated to Terrestrial Gamma-ray Flashes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1480, https://doi.org/10.5194/egusphere-egu23-1480, 2023.

EGU23-1492 | Posters on site | NH1.5

Measurements of PG during rain, hail, snow and lightning 

Konstantinos Kourtidis, Stergios Misios, Athanassios Karagioras, and Ioannis Kosmadakis

We present an analysis of the evolution of PG during the course of rain, hail and snow events at the Xanthi site, N. Greece. In particular, using data from eight rain events in 2021, four hail events in the period 2018-2021 and four snow events during the same period, we examine how the PG frequency distribution changes during the progression of these events and discuss potential implications for the charge of the hydrometeors and the clouds that produce them. We also present some first results from measurements of PG and lightning at the high altitude (2340 m ASL) site of Helmos Observatory, Peloponnese, Greece.

How to cite: Kourtidis, K., Misios, S., Karagioras, A., and Kosmadakis, I.: Measurements of PG during rain, hail, snow and lightning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1492, https://doi.org/10.5194/egusphere-egu23-1492, 2023.

EGU23-1742 | ECS | Orals | NH1.5 | Highlight

Experimental volcanic lightning under conditions relevant to the early Earth: Discharges as a possible prebiotic synthesis mechanism 

Christina Springsklee, Bettina Scheu, Christoph Seifert, Corrado Cimarelli, Damien Gaudin, Donald B. Dingwell, and Oliver Trapp

Far from being a recent development of the Earth System, volcanism has accompanied the Earth, terrestrial planets and countless exoplanets since their origins. Volcanism is a material mechanism whereby planets evolve to their differentiated states that are potentially capable of hosting life. Explosive volcanic eruptions are commonly accompanied by volcanic lightning, modulated by charging and discharging mechanisms within the eruption column. As discharges have been proposed as a potential prebiotic synthesis mechanism for forming first organic molecules, the behaviour of volcanic lightning at early Earth conditions could yield further insights into likely environments for the origin of life.

Earth´s atmosphere has changed significantly in composition and pressure since its early beginnings. Here, we would like to investigate how volcanic lightning might have operated and was influenced by changes in those environmental conditions. For this purpose, we have developed an experimental device, which consists of a gas-tight modification of a shock-tube apparatus, to investigate experimental discharges in decompressed jets of gas and volcanic ash particles under varying atmospheric conditions. The setup acts as a Faraday cage, capable of measuring discharges close to the vent. The gas inside the particle collector tank is sampled by crimp cap bottles and analysed by gas chromatography. We modified the enveloping atmospheric composition and pressure (200 mbar – 4 bar) and the transporting gas phase (argon and nitrogen).

We have tested atmospheres containing carbon dioxide, nitrogen and carbon monoxide to mimic early Earth conditions and obtained discharges with similar magnitude to those achieved in an air atmosphere. We have also varied the atmospheric pressure and observed that decreasing the atmospheric pressure results in less discharges. The results of the experiments demonstrate that it is the coupling between gas and ash particles which largely governs the occurrence and magnitude of discharges close to the jet nozzle. Nitrogen as transporting gas results in fewer discharges compared to argon, emphasizing the importance of the composition of the transporting gas phase in the jet charging and discharging mechanisms. The preliminary results point to active volcanic settings under varying atmospheric conditions as multivariate environment for the emergence of life and thus our experiments continue.  

How to cite: Springsklee, C., Scheu, B., Seifert, C., Cimarelli, C., Gaudin, D., Dingwell, D. B., and Trapp, O.: Experimental volcanic lightning under conditions relevant to the early Earth: Discharges as a possible prebiotic synthesis mechanism, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1742, https://doi.org/10.5194/egusphere-egu23-1742, 2023.

EGU23-1888 | Orals | NH1.5

Short term forecast and monitoring of thunderstorms - status and recent developments at DWD. 

Richard Müller, Axel Barleben, Stephane Haussler, and Matthias Jerg

During the last few years, DWD has developed a pioneering nowcasting procedure (NCS-A) for thunderstorms and strong convection based on  intelligent combination of lightning data, satellite information and Numerical Weather Prediction. The atmospheric motion vectors needed for the nowcasting are derived with the optical flow method TV-L1. Version 1 of the method NCS-A is operated 24/7 by DWD, covers the complete geostationary ring and has been very well received by aviation customers. The current developments of the nowcasting method focus on the analysis of life cycles in order to be able to improve the prediction of formation and decay of thunderstorms. This includes analysis of lightning activity. Further, work is also being done to seamlessly extend the forecast times by up to 6-8 hours through ensemble analysis of the Lightning Potential Index, provided by the DWD NWP model ICON. In addition to the mentioned developments of physical methods,  research is being also carried out on AI-based methods (neural networks) in cooperation with the University of Mainz. The presentation will start with an overview of the current 24/7 thunderstorm nowcasting. This will be followed by a presentation and discussion of the current developments at DWD aimed at providing accurate 6-8 hour forecasts of thunderstorms. Links for further readings and software will be provided as well.

References: 

Müller R, Haussler S, Jerg M. The Role of NWP Filter for the Satellite Based Detection of Cumulonimbus Clouds. Remote Sensing. 2018; 10(3):386. https://doi.org/10.3390/rs10030386

Urbich I, Bendix J, Müller R. Development of a Seamless Forecast for Solar Radiation Using ANAKLIM++. Remote Sensing. 2020; 12(21):3672. https://doi.org/10.3390/rs12213672.

Müller R, Haussler S, Jerg M, Heizenreder D. A Novel Approach for the Detection of Developing Thunderstorm Cells. Remote Sensing. 2019; 11(4):443. https://doi.org/10.3390/rs11040443

Zach, Christopher & Pock, Thomas & Bischof, Horst. (2007). A Duality Based Approach for Realtime TV-L1 Optical Flow. Pattern Recognition. 4713. 214-223. 10.1007/978-3-540-7

Müller, R.; Barleben, A.; Haussler, S.; Jerg, M. A Novel Approach for the Global Detection and Nowcasting of Deep Convection and Thunderstorms. Remote Sens. 2022, 14, 3372. https://doi.org/10.3390/rs14143372

Brodehl, S.; Müller, R.; Schömer, E.; Spichtinger, P.; Wand, M. End-to-End Prediction of Lightning Events from Geostationary Satellite Images. Remote Sens. 2022, 14, 3760. https://doi.org/10.3390/rs14153760 

 

How to cite: Müller, R., Barleben, A., Haussler, S., and Jerg, M.: Short term forecast and monitoring of thunderstorms - status and recent developments at DWD., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1888, https://doi.org/10.5194/egusphere-egu23-1888, 2023.

EGU23-2026 | Orals | NH1.5

Worldwide distributions and key properties of Blue LUminous Events (BLUEs) as detected by ASIM 

Francisco J. Gordillo-Vazquez, Sergio Soler, Francisco J. Pérez-Invernón, Alejandro Luque, Dongshuai Li, Torsten Neubert, Olivier Chanrion, Victor Reglero, Javier Pérez-Navarro, and Nikolai Ostgaard

The presence of transient corona discharges occurring in thunderclouds has been suspected for a long time. Thunderstorm coronas can be observed as Blue LUminous Events (BLUEs) formed by a large number of streamers characterized by their distinct 337 nm light flashes with negligible (or absent) 777.4 nm optical emission (typical of lightning leaders). The Modular Multispectral Imaging Array (MMIA) of the Atmosphere-Space Interaction Monitor (ASIM) has successfully allowed us to map and characterize BLUEs worldwide. The results presented here include a global analysis of key properties of BLUEs such as their characteristic rise times and duration, their depth with respect to cloud tops, vertical length and number of streamers. We present two different global annual average climatologies of BLUEs depending on considerations about the rise time and total duration of BLUEs worldwide [1-3].

We found that around 10 % of all detected BLUEs exhibit an impulsive single pulse 337 nm light curve shape. The rest of BLUEs are unclear (impulsive or not) single, multiple or with ambiguous pulse shapes. BLUEs exhibit two distinct populations with peak power density < 25 μWm−2 (common) and ≥ 25 μWm−2 (rare) with different rise times and durations. The altitude (and depth below cloud tops) zonal distribution of impulsive single pulse BLUEs indicate that they are commonly present between cloud tops and a depth of ≤ 4 km in the tropics and ≤ 1 km in mid and higher latitudes. Impulsive single pulse BLUEs in the tropics are the longest (up to about 4 km height) and have the largest number of streamers (up to approximately 3 × 109).

 

[1] S. Soler, F. J. Pérez-Invernón, F. J. Gordillo-Vázquez, A. Luque, D. Li, A. Malagón-Romero, T. Neubert, O. Chanrion, V. Reglero, J. Navarro-González, G. Lu, H. Zhang, A. Huang, N. Ostgaard.: "Blue optical observations of narrow bipolar events by ASIM suggest corona streamer activity in thunderstorms" (Editor's Hightlight), Journal of Geophysical Research - Atmospheres, vol. 125, 2020, doi: 10.1029/2020JD032708.

[2] S. Soler, F. J. Gordillo-Vázquez, F. J. Pérez-Invernón, A. Luque, D. Li, T. Neubert, O. Chanrion, V. Reglero, J. Navarro-González, N. Ostgaard.: "Global Frequency and Geographical Distribution of Nighttime Streamer Corona Discharges (BLUEs) in Thunderclouds", Geophysical Research Letters 2021, 48, doi: 10.1029/2021GL094657.

[3] S. Soler, F. J. Gordillo‐Vázquez, F. J. Pérez‐Invernón, A. Luque, D. Li, T. Neubert, O. Chanrion, V. Reglero, J. Navarro-González, N. Østgaard.: "Global distribution of key features of streamer corona discharges in thunderclouds". Journal of Geophysical Research: Atmospheres, vol. 127, 2022, doi: 10.1029/2022JD037535.

How to cite: Gordillo-Vazquez, F. J., Soler, S., Pérez-Invernón, F. J., Luque, A., Li, D., Neubert, T., Chanrion, O., Reglero, V., Pérez-Navarro, J., and Ostgaard, N.: Worldwide distributions and key properties of Blue LUminous Events (BLUEs) as detected by ASIM, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2026, https://doi.org/10.5194/egusphere-egu23-2026, 2023.

EGU23-3116 | Orals | NH1.5

The ALOFT mission: a flight campaign for TGF and gamma-ray glow observations over Central America and the Caribbean in July 2023 

Nikolai Ostgaard, Martino Marisaldi, Kjetil Ullaland, Shiming Yang, Bilal Hasan Qureshi, Jens Søndergaard, Andrey Mezentsev, David Sarria, Nikolai Lehtinen, Timothy Lang, Hugh Christian, Mason Quick, Richard Blakeslee, J. Eric Grove, and Daniel Shy

The Airborne Lighting Observatory for FEGS and TGFs (ALOFT)  is a field campaign focused on observing Terrestrial Gamma-ray Flashes (TGFs) and gamma-ray glows from thunderclouds. ALOFT will be flown on a NASA ER-2 research aircraft, flying at 20 km altitude, and the payload  includes:

1) Fly’s Eye GLM Simulator (FEGS), an array of imaging photometers as well as different wavelengths, and electric field change meters.
2) Lightning Instrument Package (LIP), giving three component electric field measurements.
3) Several gamma-ray detectors covering four orders of magnitude dynamic range in flux as well as the full energy range for TGF/gamma-ray glow detection.

ALOFT is scheduled for July 2023, with 50 flight hours based out of Florida.  Flying over thunderstorms in Central America and Caribbean, one of the most active TGF regions on the planet during the most optimal season, the ALOFT campaign will help us to answer the questions:

1) How and under what conditions are TGFs produced?
2) How extended in space and time are the gamma-ray glows?

To answer question 1), the ALOFT campaign will be supported by ground based radio measurements from different locations in Central America and Caribbean.

To answer question 2), with realtime downlink of data we will know when the ER-2 encounters gamma-ray glowing thunderclouds, and we will instruct the pilot to have the aircraft perform have repeated overflights over this cloud as long as the glow exists, to answer question 2).  This will also help us understand whether gamma-ray glows and TGFs are interrelated.

The full set of observational goals of ALOFT are:

1. Observe TGFs in one of the most TGF-intense regions on the planet.
2. Observe gamma-ray glows in thunderstorms and their relation to TGFs.
3. Perform International Space Station Lightning Imaging Sensor (ISS LIS) and Global Lightning Monitor (GLM) validation using improved suborbital instrumentation (including upgraded FEGS).
4. Evaluate new design concepts for next-generation spaceborne lightning mappers.
5. If relevant instrumentation is available, make measurements useful to advance convection science from a suborbital platform.

In this presentation we will give the status and plans for the ALOFT mission.

How to cite: Ostgaard, N., Marisaldi, M., Ullaland, K., Yang, S., Hasan Qureshi, B., Søndergaard, J., Mezentsev, A., Sarria, D., Lehtinen, N., Lang, T., Christian, H., Quick, M., Blakeslee, R., Grove, J. E., and Shy, D.: The ALOFT mission: a flight campaign for TGF and gamma-ray glow observations over Central America and the Caribbean in July 2023, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3116, https://doi.org/10.5194/egusphere-egu23-3116, 2023.

EGU23-3124 | Orals | NH1.5

Electrodynamic model of K-changes 

Petr Kaspar, Thomas Marshall, Maribeth Stolzenburg, Ivana Kolmasova, and Ondrej Santolik

K-changes are step-like electrostatic field changes, which occur during the final part of cloud flashes or between the return strokes in cloud-to-ground discharges. We numerically solve the full set of Maxwell’s equations coupled to the electrostatic Poisson’s equation for a given thundercloud charge structure to model the K-changes. We simulate the K-changes by a sequential increase of conductivity of the decayed vertical channel. This process creates a current pulse which attenuates as it propagates downward. We show how the modeled linear charge densities and electric potentials connected to K-changes evolve in time. We successfully compare our model with the electric field measured by a flat-plate E-change antenna with a sensor having a decay time constant of 1 s, a bandwidth of 0.16 Hz –2.6 MHz, and a sampling rate of 5 MS/s. The experimental data used for comparison with our model were obtained at KSC Florida in 2011.

How to cite: Kaspar, P., Marshall, T., Stolzenburg, M., Kolmasova, I., and Santolik, O.: Electrodynamic model of K-changes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3124, https://doi.org/10.5194/egusphere-egu23-3124, 2023.

EGU23-3281 | Posters on site | NH1.5

Library of simulated gamma-ray glows and application to previous airborne observations 

David Sarria, Nikolai Østgaard, Martino Marisaldi, Nikolai Lehtinen, and Andrey Mezentsev

Gamma-Ray Glows (GRGs) are bursts of high-energy radiation that are emitted by thunderclouds and have a duration of seconds to minutes. These radiation sources are extended over several to tens of square kilometers. GRGs have been observed from detectors on the ground, in aircraft, and on balloons. In this paper, we present a Monte-Carlo model that can be used to study the production and propagation of GRGs. We compare our model to one developed by Zhou et al. (2016) and find small differences between the two. We have also created a library of simulations that is available to the community. Using this library, we were able to reproduce five previous GRG observations from five airborne campaigns: balloons from Eack et al. (1996) and Eack et al. (2000), and aircraft from the ADELE (Kelley et al. 2015), ILDAS (Kochking et al. 2016), and ALOFT campaigns (Østgaard et al. 2019).

Our simulation results confirm that the flux of cosmic-ray secondary particles at a given altitude can be enhanced by several percent or even several orders of magnitude due to the effect of thunderstorms' electric fields. These results explain the five observations we studied and will be useful for the upcoming ALOFT-2023 campaign. While some GRGs can be explained solely by the MOS process, the strongest GRGs observed require electric fields significantly larger than the RREA threshold value (E_th). Some of the observations also came with in-situ electric field measurements that were always lower than E_th, but these measurements may not have been taken from the regions where the glows were produced. This study supports the idea that some thunderstorms must have electric fields with magnitudes of at least E_th on a kilometer scale.

 

References :

-Effect of near-earth thunderstorms electric field on the intensity of ground cosmic ray positrons/electrons in tibet. Zhou et al. (2016). https://doi.org/10.1016/j.astropartphys.2016.08.004

-Balloon-borne x-ray spectrometer for detection of x-rays produced by thunderstorms. Eack et al. 1996. https://doi.org/10.1063/1.1146959

-Gamma-ray emissions observed in a thunderstorm anvil. Eack et al. 2000. https://doi.org/10.1029/1999GL010849

-Relativistic electron avalanches as a thunderstorm discharge competing with lightning. Kelley et al. 2015. https://doi.org/10.1038/ncomms8845

-In-Flight Observation of Gamma Ray Glows by ILDAS. Kochkin et al. 2017. https://doi.org/10.1002/2017JD027405 -Gamma Ray Glow Observations at 20-km Altitude. Østgaard et al. 2019. https://doi.org/10.1029/2019JD030312

How to cite: Sarria, D., Østgaard, N., Marisaldi, M., Lehtinen, N., and Mezentsev, A.: Library of simulated gamma-ray glows and application to previous airborne observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3281, https://doi.org/10.5194/egusphere-egu23-3281, 2023.

EGU23-3432 | Posters on site | NH1.5

The effects of fog on the atmospheric electrical field close to the surface 

Yoav Yair, Roy Yaniv, and Colin Price

For almost a decade, ground-based measurements of the electric field (Ez) have been conducted continuously at Tel-Aviv University's Wise astronomical observatory, located in the Negev desert highland in southern Israel. The data enabled identifying the characteristics of Ez in fair weather, during dust storms, lightning activity and the passage of different cloud types overhead. We present new results of observations of the variability of the atmospheric electric field during several foggy days along with meteorological data of wind speed and relative humidity. The results show a substantial increase of the electric field (up to 400-650 V m-1) compared with the mean fair-weather values at the site (180-190 V m-1) during times of high values of relative humidity (>95%) and low wind speed (<3 m s-1). This increase is a consequence of the reduction in the conductivity at low levels due to the attachment of ions to fog droplets. We suggest that closely monitoring the electric field when there is a forecast for the occurrence of fog can offer a precise indication when fog begins and ends.

How to cite: Yair, Y., Yaniv, R., and Price, C.: The effects of fog on the atmospheric electrical field close to the surface, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3432, https://doi.org/10.5194/egusphere-egu23-3432, 2023.

EGU23-3546 | ECS | Posters on site | NH1.5

Lightning activity over central Europe in years 2017-2022 (analysis of ISS-LIS data) 

Andrea Kolínská, Ivana Kolmašová, Colin Price, and Ondřej Santolík

We analyze the lightning activity over central Europe from 2017 to 2022 using the optical data from the Lightning Imaging Sensor (LIS) on board the International Space Station (ISS). The area of interest covers a central European region limited by 54.5° N, 7.5° E and 44.5° N, 22.5° E. A total number of 68192 lightning flashes was detected during 1805 ISS orbital overpasses. This study compares the lightning activity in central Europe to the global lightning activity and investigates the impact of the COVID-19 pandemic. While there is a global reduction of the lightning activity during the lockdowns in 2020, no significant decrease is observed in central Europe.

On the territory of Czechia, the highest density of flashes was detected in the northwestern part of the country. We combine the ISS-LIS data with measurements of the Shielded Loop Antenna with Versatile Integrated Amplifier (SLAVIA) detectors located in this region. The measurements of the ISS-LIS and SLAVIA detectors are combined with data from the World Wide Lightning Location Network (WWLLN) or Global Lightning Dataset (GLD360) in order to understand the correlation between electromagnetic radiation from selected lightning flashes and their optical characteristics observed from space.

How to cite: Kolínská, A., Kolmašová, I., Price, C., and Santolík, O.: Lightning activity over central Europe in years 2017-2022 (analysis of ISS-LIS data), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3546, https://doi.org/10.5194/egusphere-egu23-3546, 2023.

EGU23-3801 | Orals | NH1.5

A strong pulsing nature of negative recoil leaders accompanied by regular trains of microsecond-scale pulses 

Ivana Kolmašová, Olaf Scholten, Ondřej Santolik, Brian M. Hare, Ningyu Y. Liu, Joseph R. Dwyer, and Radek Lán

A presence of regular sequences of microsecond-scale pulses has been occasionally reported in the lightning literature for more than forty years. Due to a fine time resolution of modern electromagnetic receivers, the properties of these pulse trains are now well described. Nevertheless, the conditions for their occurrence are still not understood, and the information needed for their proper modelling is not sufficient.  

To contribute to this effort, we report for the first time properties of negative recoil stepped leaders accompanied by regular trains of microsecond-scale pulses simultaneously seen by the broadband magnetic loop antenna SLAVIA (Shielded Loop Antenna with a Versatile Integrated Amplifier; 5 kHz-90 MHz), and the radio telescope LOFAR (Low Frequency Array; 30-80MHz). We investigate four pulse trains that occurred during complicated intracloud flashes on 18 June 2021, when heavy thunderstorms hit Netherlands.

The pulses within the trains are unipolar, a few microseconds wide with an inter-pulse interval of about ten microseconds. The pulse trains last from 100 µs to 800 µs. After a careful time alignment of both magnetic field and LOFAR time series, we found that the broadband pulses perfectly match with regularly distributed and relatively isolated bursts of VHF sources localized by the LOFAR impulsive imager. All trains were generated by negative recoil stepped leaders propagating downward (two events) or upward (two events) at altitudes between 5.5 km and 8.5 km. Their tracks were formed by positive leaders occurring within the same flash several hundreds of milliseconds previously. The peak powers of VHF sources seen by the LOFAR electric antennas closest to the investigated discharges were about one order of magnitude higher than the power of signals emitted by normal negative leaders. These stepped recoil leaders propagate at a relatively low speed of about 2-5x10^6 m/s, when similar recoil leaders often reach speeds of 10^7 m/s. The velocity and inter-pulse intervals decrease towards the end of trains.

We show that observed pulse trains are due to stepping recoil leaders. However, we consider this strong pulsing nature of the examined recoil leaders to be quite unusual. The physical mechanism giving rise to the energetic VHF bursts and accompanying regular microsecond-scale pulses remains unclear.

How to cite: Kolmašová, I., Scholten, O., Santolik, O., Hare, B. M., Liu, N. Y., Dwyer, J. R., and Lán, R.: A strong pulsing nature of negative recoil leaders accompanied by regular trains of microsecond-scale pulses, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3801, https://doi.org/10.5194/egusphere-egu23-3801, 2023.

EGU23-4086 | Posters on site | NH1.5 | Highlight

Effects of cloud-to-water lightning strokes on open sea fish cages during eastern Mediterranean winter thunderstorms 

Mustafa Asfur, Roy Lavie, Jacob Silverman, Colin Price, Menahem Korzets, and Yoav Yair

Based on data obtained by the Earth Networks Total Lightning Network (ENTLN) for 5 winter seasons (DJF, 2018-2022), the flash density of lightning striking the water surface of the eastern Mediterranean Sea up to 50 km from the Israeli coastline is on average 3 strokes/km2. Out of the total lightning that strike the sea surface in the said area, about 0.05% on are superbolts with peak current > 200 kA. Cloud-to-water strikes generate thunder and underwater acoustic noise that can propagate for a few km from the strike location. While anthropogenic noises have been shown to cause negative stress responses in the marine environment and specifically in aquaculture fish cages, no stress response of cultured fish due to lightning strikes have been recorded yet.  New areas in the Israeli territorial waters are allocated to fish farms. These commercial farms will be using net cages, with high fish density expecting large yields.

This research aims to find out how cultured fish respond to the acoustic noises generated by lightning strikes. This hypothesis meets a growing awareness in the aquaculture field to research fish stress that, in this case, stay trapped in the water body without the ability to effectively respond and flee lightning strikes. Continual stress of cultured fish can economically adversely affect the fish farm due to high mortality rates and decreased growth rates. By monitoring sea bream (Sparus aurata) cages, with cameras and hydrophone, during winter months of years 2021-2023, we have found several cases of stress related behavior. These cases were correlated with precise lightnings data, videos of surveillance cameras pointed toward the fish farm, audio records of underwater sound and indications of abnormal fish behavior (sudden dive or direction changes). We will present results from newly developed image processing algorithm that reads underwater fish videos files and automatically finds abnormal behavior events.

How to cite: Asfur, M., Lavie, R., Silverman, J., Price, C., Korzets, M., and Yair, Y.: Effects of cloud-to-water lightning strokes on open sea fish cages during eastern Mediterranean winter thunderstorms, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4086, https://doi.org/10.5194/egusphere-egu23-4086, 2023.

    Existing literature indicates that volcanic lightning occurs during a devastating volcano eruption. However, it is still limited to understanding the volcanic electrification mechanism in nature because of the rarity of the explosive volcano eruption and visible spectrum obstacles from plumes full of dirty ashes. The eruption of the Hunga Tonga–Hunga Haʻapai (HT-HH) submarine volcanoes in the Lau Basin, South Pacific, had an extremely violate surtseyan type eruption on January 15th and generated numerous volcanic lightning. This eruption event provides a great opportunity to explore the electrification and evolution of volcanic lightning. 

    In this work, more than 40,000 lightning events were detected by the World Wide Lightning Location Network (WWLLN) during the primary eruption on January 15th. At the first stage of the eruption, the geographic distribution of lightning strikes expanded rapidly and isotropically while the eruption column reached a specific altitude. Then a lightning tranquility period occurred subsequently, implying explosive erupting was intermittent. Several explosive sub-eruptions were detected from 04:00Z to 07:00Z, and sub-eruptions' timestamps are highly consistent with seismic data analysis from IRIS. Lightning footprint provided evidence that the HT-HH eruption was a surtseyan eruption unsteady with several quiescent phases separating the explosive stages.

    HT-HH is one of the most powerful eruptions of the 21st century and provides a favorable environment for volcanic lightning research. The result of this work can track the immediate eruption by using lightning activities. Moreover, volcanic lightning has a different charging mechanism than general tropospheric lightning. Therefore, many interesting issues can be discussed, such as the volcano eruption's contribution to global electrical circuits or whether volcanic lightning can generate other atmospheric electricity events like TLEs or TGFs.

How to cite: Lin, Y.-C. and Chen, A.: Characteristics of Volcanic Lightning Distribution Generated by Hunga Tonga–Hunga Haʻapai on January 15th, 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4714, https://doi.org/10.5194/egusphere-egu23-4714, 2023.

EGU23-5231 | ECS | Posters on site | NH1.5

Simultaneous detection of long continuing current lightning with space and ground-based detectors 

Pablo A. Camino-Faillace, Francisco J. Pérez-Invernón, Francisco J. Gordillo-Vázquez, Torsten Neubert, Víctor Reglero, and Nikolai Ostgaard

Long continuing current (LCC) lightning flashes contain a discharge in which a continuing electrical current flows for more than 40 ms. They represent about 10% of the total cloud-to-ground lightning flashes and have been associated with lightning-ignited wildfires. LCC flashes can be detected by different terrestrial- and space-based instruments. However, those instruments simultaneously detect all kinds of lightning across the globe, including those with long continuing current, which hinders the analysis of LCC-only events.

We present a method to match every single flash from the Geostationary Lightning Mapper (GLM), the Atmosphere-Space Interactions Monitor (ASIM) and the Earth Networks Total Lightning Network (ENTLN) by using a proximity index. In turn, we analyze the optical signal of LCC flashes simultaneously detected by GLM and ASIM.

According to preliminary results, we found an average of 15 LCC events per month in the continental United States simultaneously detected by the three mentioned sensors (GLM, ASIM and ENTLN). Moreover, this method can be used to match other atmospheric electricity phenomena simultaneously detected by different ground and/or space-based instruments.

How to cite: Camino-Faillace, P. A., Pérez-Invernón, F. J., Gordillo-Vázquez, F. J., Neubert, T., Reglero, V., and Ostgaard, N.: Simultaneous detection of long continuing current lightning with space and ground-based detectors, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5231, https://doi.org/10.5194/egusphere-egu23-5231, 2023.

EGU23-5302 | ECS | Orals | NH1.5

Global occurrence of continuing currents in lightning and lightning-ignited wildfires predicted for the next century 

Francisco J. Pérez-Invernón, Francisco J. Gordillo-Vázquez, Heidi Huntrieser, and Patrick Jöckel

Lightning flashes can produce a discharge in which a continuing electrical current flows for more than 40 ms. Such flashes have been proposed to be the main precursors of lightning-ignited wildfires.

In this work, we used lightning measurements provided by the Geostationary Lightning Mapper (GLM) over the continental United States of America during the summer of 2018 to confirm the role of lightning with continuing currents in the ignition of wildfires. We investigated projections in the occurrence of lightning with continuing currents and in the meteorological conditions that favor wildfires over the next century by applying a new parameterization of continuing currents based on the updraft strength. The simulations are performed by using the European Center HAMburg general circulation (ECHAM) / Modular Earth Submodel System (MESSy) Atmospheric Chemistry (EMAC) model [1]. We found a 41% increase in the occurrence of lightning with continuing currents worldwide. Increases are largest in South America, the western coast of Northern America, Central America, Australia, Southern and Eastern Asia, and Europe, while only regional variations are found in northern polar forests, where wildfires can affect permafrost soil carbon release.

We obtained a possible increase in the risk of lightning-ignited fires in Europe, Eastern Asia, North America, the Western coast of South America, Central Africa and Australia. In turn, the simulations suggest a decrease in the risk of lightning-ignited wildfires in polar regions of Eurasia and North America. Finally, projections do not show any clear tendency in the Amazon rainforest during the typical fire season.

[1] Pérez-Invernón, F. J., Huntrieser, H., Jöckel, P., and Gordillo-Vázquez, F. J.: A parameterization of long-continuing-current (LCC) lightning in the lightning submodel LNOX (version 3.0) of the Modular Earth Submodel System (MESSy, version 2.54), Geosci. Model Dev., 15, 1545–1565, https://doi.org/10.5194/gmd-15-1545-2022, 2022.

How to cite: Pérez-Invernón, F. J., Gordillo-Vázquez, F. J., Huntrieser, H., and Jöckel, P.: Global occurrence of continuing currents in lightning and lightning-ignited wildfires predicted for the next century, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5302, https://doi.org/10.5194/egusphere-egu23-5302, 2023.

Negative streamers play an important part in propagation of a negative stepped leader. They are emitted from the tip of a space stem or, as a streamer burst, from the tip of the space leader right after its attachment to the main leader.

In the laboratory conditions, it was shown that negative streamers need a significantly higher voltage for inception than positive streamers [e.g., Briels et al, 2008, doi:10.1088/0022-3727/41/23/234004]. The higher negative threshold is in agreement with the higher field measured inside streamer channels, namely 13±2 kV/cm for negative streamers versus 5 kV/cm for positive streamers.

We obtain the conditions for propagation of negative streamers using the Streamer Parameter Model (SPM) [Lehtinen, 2021, doi:10.1007/s11141-021-10108-5]. In this model, we calculate various streamer parameters from relationships between them, with the assumption of maximization of streamer velocity. This model, in the positive streamer case, was shown to agree well with both experimental measurements and hydrodynamic simulation results [Lehtinen and Marskar, 2021, doi:10.3390/atmos12121664]. In the negative streamer case, we show that the parameter equations have no solution below certain background electric fields. The threshold at which the negative streamer appears is around 12-14 kV/cm for 5-10 cm streamer length, which agrees with the experimental data. We also perform hydrodynamic simulations of negative streamers as another way to calculate the conditions for negative streamer propagation.

There is an important difference from positive streamers, for which the propagation threshold is determined by the rate of free electron removal from the streamer channel (i.e., attachment): namely, we find that the negative streamer threshold field is finite even in the absence of the electron removal.

How to cite: Lehtinen, N.: Conditions for inception and propagation of negative streamers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5529, https://doi.org/10.5194/egusphere-egu23-5529, 2023.

EGU23-6089 | Orals | NH1.5

Evolution of lightning activity observed during rapid intensity changes of tropical cyclones 

Kateřina Rosická, Ivana Kolmašová, and Ondřej Santolík

We study evolution of lightning activity accompanying rapid intensity changes of tropical cyclones worldwide. We use a dataset of 400 tropical cyclones occurring between 2012 and 2017. We use the cyclones tracks from the International Best Track Archive for Clime Stewardship. The lightning data are provided by the World Wide Lightning Location Network (WWLLN). We inspect the lightning activity and median stroke energies accompanying rapid intensifications (RI) of cyclones, defined as increases of the wind speed by more than 30 kt in 24 hours, and their rapid weakenings (RW), defined as decreases of the wind speed by more than 40 kt in 24 hours.

In an area of radial wind maximum (RWM), we observe a stroke density of 15.1 strokes/(100 km)2/hour for RI and 21.8 strokes/(100 km)2/hour for RW, respectively, which is much higher than average RWM density 7.9 strokes/(100 km)2/hour over the duration of the cyclone. A median stroke energy is 0.3 kJ during RI and 0.7 kJ during RW. It means that during rapid intensification of cyclones, there are less strokes with slightly higher energies and during rapid weakening there are more strokes with slightly lower energies. When analyzing the cyclones in both hemispheres separately, we obtain 0.3 kJ for RI and 0.6 kJ for RW in the northern hemisphere, and 0.8 kJ for RI and 0.9 kJ for RW in the southern hemisphere. The difference in the stroke density during RI and RW was observed larger in the northern hemisphere (19.7 vs 34.1 strokes/(100 km)2/hour), when in the southern hemisphere the stroke density is much lower and differs less (4.4 strokes/(100 km)2/hour for RI and 5.1 strokes/(100 km)2/hour for RW).

 

How to cite: Rosická, K., Kolmašová, I., and Santolík, O.: Evolution of lightning activity observed during rapid intensity changes of tropical cyclones, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6089, https://doi.org/10.5194/egusphere-egu23-6089, 2023.

EGU23-6099 | Posters on site | NH1.5

Analyses of thunderstorm structures using data of a Ka-band Doppler polarimetric vertical cloud profiler 

Zbyněk Sokol, Jana Popová, and Kateřina Skripniková

This study investigates the structure of strong convective storms to determine the difference between the structure of storms inducing or not lightning discharges. The structure of strong convective storms is investigated using a Ka-band Doppler polarimetric vertical cloud profiler operating at a frequency of 35 GHz. The profiler is located at the Milešovka meteorological observatory in Czechia (Central Europe). To study the structure of storms, we used the basic radar measurements of phase and power spectra of the co- and the cross-channel. We analysed the data from all the storms that occurred close to the Milešovka observatory during 2018-2022 and we performed statistical and correlation analyses of vertical profiles of phase and power spectra in the co- and the cross-channel in dependence on the distance of lightning discharges observed and recorded by the EUCLID lightning network.

How to cite: Sokol, Z., Popová, J., and Skripniková, K.: Analyses of thunderstorm structures using data of a Ka-band Doppler polarimetric vertical cloud profiler, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6099, https://doi.org/10.5194/egusphere-egu23-6099, 2023.

EGU23-6148 | Orals | NH1.5 | Highlight

Immediate effects of the Hunga Tonga - Hunga Ha’apai volcanic eruption on the AC and DC Global Electric Circuits 

József Bór, Tamás Bozóki, Gabriella Sátori, Earle R. Williams, Sonja Ann Behnke, Michael Rycroft, Attila Buzás, Hugo Gonçalves Silva, Marek Kubicki, Ryan Said, Chris Vagasky, Péter Steinbach, Karolina Szabone André, and Mike Atkinson

Observed responses of the AC and DC parts of the Global Electric Circuit (GEC) to the large eruption of the Hunga Tonga - Hunga Ha’apai (HT-HH) volcano on 15 January, 2022 are presented. The AC-related investigation is based on Schumann resonance (SR) measurements from the Nagycenk Geophysical Observatory (NCK), Hungary as well as from distant stations on the globe belonging to the HeartMath Institute (https://www.heartmath.org/gci/). The DC-related investigation is based on atmospheric electric potential gradient measurements (PG) from six recording stations in Europe and in the USA. The GLD360 and the WWLLN lightning detection networks were used to characterize lightning activity in the vicinity of the HT-HH island on the investigated day. The peak lightning stroke rate reached 80/s (5000/minute), whereas the average global rate is ~44/s. Lightning discharges occurred in rings around the vent of the volcano. Peak currents and the diameter of the ring of positive and negative polarity lightning strokes varied differently in the main phase of the eruption. At its peak, negative lightning dominated the electric activity in the volcanic cloud.

A global intensification of SR is apparent in connection with the enhanced lightning activity caused by the eruption. The SR data together with the global network observations indicate that the lightning activity in the eruption dominates the naturally occurring global activity for a period of at least one hour. The highly localized increase in lightning activity over HT-HH provides a unique point source of excitation for the SR.

In contrast with the dramatic response of the AC global circuit, the response of the DC GEC to this exceptional eruption is not readily unambiguous in the PG measurements. The observations suggest that impulse-like charging of the GEC by ~15% via -CG lightning strokes took place two times during the eruption. A time constant of 7 or 8 minutes has been inferred for near-surface electric field changes from these enhancements. This could be the first direct measurement of the time constant of the GEC near the Earth’s surface, as well as the first observation of the direct charging of the DC GEC by a single atmospheric electrified source.

How to cite: Bór, J., Bozóki, T., Sátori, G., Williams, E. R., Behnke, S. A., Rycroft, M., Buzás, A., Silva, H. G., Kubicki, M., Said, R., Vagasky, C., Steinbach, P., Szabone André, K., and Atkinson, M.: Immediate effects of the Hunga Tonga - Hunga Ha’apai volcanic eruption on the AC and DC Global Electric Circuits, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6148, https://doi.org/10.5194/egusphere-egu23-6148, 2023.

EGU23-6342 | ECS | Orals | NH1.5

Localization and quantification of the acoustical power of lightning flashes 

Damien Bestard, Thomas Farges, and François Coulouvrat

Lightning is a ubiquitous source of infrasound, and an essential climate variable. Acoustic measurements have been carried out by the CEA over the last ten years to characterize thunder within the framework of the HyMeX project. First, during the fall of 2012 in the south of France in the Cévennes region during the intensive measurement campaign (SOP1) and more recently, in the fall of 2018 in Corsica (France), as part of the EXAEDRE campaign. During both the SOP1 and EXAEDRE campaigns, mini-arrays (“AA” for “Acoustic Array”) of four microphones (respectively disposed on a 50m and a 30m-wide triangle) were used. Lightning information were available thanks to three kinds of electromagnetic detection systems. Firstly, classical Lightning Location Systems (LLS) measured the low frequency range (1-350 kHz), giving the flash emission time and location, as well as its peak current. Secondly, a network of 12 antennas, Lightning Mapping Array (LMA), detecting in the very high frequency range (60-66 MHz) was used. It measured the radiation from leaders and intracloud discharges, which occur mostly inside the thundercloud, providing the 3D location of these discharges. Thirdly, the Charge Moment Change (CMC) was provided by broadband Extremely Low Frequency (< 1.1 kHz) measurements.

Time delays between AA sensors inform on the direction of sound arrival, while the difference between emission time and sound arrival provides the source distance. Combining the two allows a geometrical reconstruction of individual lightning flashes, each viewed as a set of point sound sources. Co-localization of acoustic sources with in-cloud detections provided by the LMA and with ground impacts provided by the LLS shows the efficiency and precision of the method. The measured sound amplitude can also be back-propagated, compensating for absorption and density stratification. This allows to evaluate the acoustical power of each detected source, and then the total power of an individual flash.

In both campaigns, very heterogeneous geometrical distributions of source sound powers within a single flash are frequently observed. Most of the power is frequently located in only one portion of the lightning, most of the time in the return stroke, but also sometimes in the intracloud part. A few homogeneous cases are observed, especially in SOP1. The total acoustical power of the flashes turns out to be also extremely variable, extending over at least 4 orders of magnitude with a median value of 3 MW. It correlates quite good with the peak current or the CMC, and the nature of the correlation differs strongly with the category of lightning considered, either typical return strokes or very energetic positive flashes generating sprites. However, a high dispersion of the data is observed, so that it is not possible to correctly predict any electrical parameter using only the total acoustic power of an event, although a trend is statistically observed. This could be overcome by finding other variables to fully explain the relationship between acoustical and electrical parameters, and improving our propagation model to better account for acoustic variability.

How to cite: Bestard, D., Farges, T., and Coulouvrat, F.: Localization and quantification of the acoustical power of lightning flashes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6342, https://doi.org/10.5194/egusphere-egu23-6342, 2023.

Over the last few decades, lightning has been one of the fatal extreme weather phenomena in the Indian subcontinent. Aerosols which act as cloud condensation nuclei (CCN) and ice nuclei (IN) can modify the cloud properties and alter the thermodynamic processes within the deep convective clouds in a way that eventually affects the lightning flash rates associated with thunderstorms. Long-term satellite observations suggest that a maximum number of lightning strikes (40-45 flashes/km2) occur during the pre-monsoon (March-May) and monsoon (June-September) seasons over the Indian subcontinent. We analyzed the lightning data available from satellite observations over two distinctly different climatological regions namely, northeast India and western India. In this study, we evaluate the performance of a numerical weather research and forecasting model (WRF) in reproducing the lighting characteristics over these two regions and further try to understand the sensitivity of simulated lightning flash rates to aerosol characteristics and aerosol-cloud interactions considered in the model.

Two severe lightning episodes which occurred on 5-6 May 2013 and 16 April 2019 over northeast India and western India respectively are chosen as case studies for our model sensitivity experiments. We used Morrison, NSSL & SBM microphysics schemes to understand the capability of bulk and bin schemes in simulating these events. Our results show that SBM (bin) scheme affects lightning flash events more accurately than the other two bulk schemes. Increasing aerosol concentrations, increases the cloud droplet number concentrations, thus influences the collision-coalescence processes thereby increase lightning activity over both regions. To further understand the influence of aerosol size, we used a spectral bin microphysics method with a dry radius range of (0.7nm-12µm), which modified the cloud microphysical features. Changing the number concentration and default size of aerosols also influenced the meteorology and hence the deep convection and thunderstorms occurring over the two selected case study regions. More results with greater details will be presented.

How to cite: Ghoshal Chowdhury, S., Ganguly, D., and Dey, S.: A modeling study on the role of aerosols in modulating the lightning flash rates over two different climatological regions of India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6397, https://doi.org/10.5194/egusphere-egu23-6397, 2023.

The generation and variation of the atmospheric electric field (hereafter E-field), which exists under all meteorological conditions and drives the charge flow around the Earth globally, and many natural phenomena such as lightning, thunderstorms, and even earthquakes have been observed accompanied by surface E-field disturbances; therefore, E-field observations are also used in disaster warnings. Since 2021, a ground E-field network consisting of three stations using in-house electric field mills has been deployed in the Tainan area, covering two known seismic faults, to monitor the characteristics of the e-field variation caused by diurnal cycle, thunderstorms, and earthquake precursor.

The results indicated that the small-area E-field variation did not follow the Carnegie curve because local effects (aerosols, weather conditions, and environment) masked the variations of the global electrical circuit. In addition, the analysis of the disturbed E-field showed that more than 90% of the single-cell thunderstorms observed in the surface E-field could be classified as mature and dissipating stages. Each disturbance lasted approximately 34 minutes and was accompanied by an average of 1.4 times E-field phase reversals. Among them, the negative reversal of the surface electric field caused by the negative charge layer was relatively strong and frequent. Eventually, triangulation was used to reconstruct the charge structure of four distinctive single-cell thunderstorm events and restore the surface E-field responses during the passage of clouds. The correlation coefficients between the simulation and the observation were higher than 85%, and the trajectory and speed of the thunderclouds is also successfully reproduced by the recorded e-field data. Furthermore, some preliminary conclusions about earthquake precursors were drawn by analyzing the surface E-field.

How to cite: Chen, A. B.-C. and Chuang, C.-W.: The charge structure of thunderstorms revealed by the ground electric field monitoring network deployed in Tainan, Taiwan, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6527, https://doi.org/10.5194/egusphere-egu23-6527, 2023.

EGU23-6741 | ECS | Orals | NH1.5

Long-range Lightning Interferometry (A Simulation Study) 

Xue Bai and Martin Fullekrug

Traditional long-range lightning detection and location networks use Time-of-Arrival (TOA) differences, and a single timestamp to locate lightning events. For long propagation distances, the amplitude of ground waves decays faster with distance than sky waves as a result of the ground conductivity and the effects of Earth curvature (Caligaris et al., 2008, Cooray, 2009, Hou et al., 2018). This can lead the skywaves to interfere with their large amplitudes when locating lightning.

Coherency, which is short for phase coherency of the analytic signal, is used here, which exhibits lightning characteristics (Bai & Fullekrug, 2022). This work introduces a simulation study to lay the foundation for new lightning location concepts. A novel interferometric method using coherency is presented here, which expands the use of more data points of recorded lightning sferics to map the lightning into an area in a long-range network. In this map, each pixel corresponds to a lightning location with different coherency and time of arrival differences, simulated by shifting the complex lightning waveforms. In long-range networks, the coherency of the 1st skywave is larger than the ground wave, and it is difficult to distinguish them due to the short time delay between them. One solution is to use a small network so that the recorded waveforms are associated with short propagation distances which can eliminate the interferences caused by the first skywave. Another solution is to filter the data such that a lightning waveform is represented by an impulse. In this case, only one maximum coherency area exists for each event at the lightning occurrence time.

In the future, the data collected with a real-time lightning detection network will be analysed to map the lightning events using the complex interferometric method for use in long-range lightning location networks.

 

References

Bai, X., & Füllekrug, M. (2022). Coherency of Lightning Sferics. Radio Sci., 57(5), e2021RS007347. doi: 10.1029/2021rs007347

Caligaris, C., Delfino, F., & Procopio, R. (2008). Cooray–Rubinstein Formula for the Evaluation of Lightning Radial Electric Fields: Derivation and Implementation in the Time Domain. IEEE Trans. Electromagn. Compat., 50(1), 194-197. doi: 10.1109/temc .2007.913226

Cooray, V. (2009). Propagation Effects Due to Finitely Conducting Ground on Lightning-Generated Magnetic Fields Evaluated Using Sommerfeld’s Integrals. IEEE Trans. Elec-tromagn. Compat., 51(3), 526-531. doi: 10.1109/temc.2009.2019759

Hou, W., Zhang, Q., Zhang, J., Wang, L., & Shen, Y. (2018). A New Approximate Method for Lightning-Radiated ELF/VLF Ground Wave Propagation over Intermediate Ranges. Int. J. Antennas Propag., 2018(6), 1-10. doi: 10.1155/2018/9353294

How to cite: Bai, X. and Fullekrug, M.: Long-range Lightning Interferometry (A Simulation Study), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6741, https://doi.org/10.5194/egusphere-egu23-6741, 2023.

EGU23-7176 | Orals | NH1.5

Study of multiple ELVES at the Pierre Auger Observatory 

Adriana Vásquez Ramírez, Roberto Mussa, and Luis A. Núñez and the Pierre Auger Collaboration

ELVES are transient ring-shaped emissions occurring in the ionosphere above thunderstorms. Multi-ELVES are events consisting of two and up to four rings of light separated temporally by tens of microseconds. The Fluorescence Detector (FD) at the Pierre Auger Observatory has been detecting ELVES with a dedicated trigger since 2013. The high temporal resolution of 100 ns of the FD allows us to record the phototraces of the events in great detail. From the improved processing of the phototraces, we have observed ELVES with double and triple peaks. In fact, during the period 2014-20, about 27% of the events detected at Auger are multi-ELVES. The origin of multi-ELVES is still not fully understood, therefore in this work, we tested two models: the first one relates the temporal difference between two peaks (ΔT) to the rise (tr) and fall (tf) times of the current density pulse of the source beam; the second one relates the height of the intra-cloud lightning source (hb) to ΔT and is used to study events with three or more peaks. From the first model, we can obtain combinations of tr and tf where ΔT tends to zero, i.e. the origin of the simple ELVES can also be explained. For this analysis, we compare the ELVES parameters measured in Auger with the lightning properties detected by Earth Networks, i.e. the location, waveform, and height of these sources. 

How to cite: Vásquez Ramírez, A., Mussa, R., and Núñez, L. A. and the Pierre Auger Collaboration: Study of multiple ELVES at the Pierre Auger Observatory, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7176, https://doi.org/10.5194/egusphere-egu23-7176, 2023.

EGU23-7235 | ECS | Posters virtual | NH1.5

Towards a GPU based particle model for streamer discharges 

Elloïse Fangel-Lloyd, Saša Dujko, Sven Karlsson, Matthias Gammelmark, Anton Rydahl, Kenishi Nishikawa, and Christoph Köhn

Terrestrial gamma-ray flashes (TGFs), bursts of X- and gamma-rays, are emitted from thunderstorms and are produced through relativistic electrons through the Bremsstrahlung process. Despite recent progress through measurements and simulations, the specific mechanism of electron acceleration remains unknown. As the processes inside thunderclouds occur on a multiscale level, we need to develop models that cover a wide range of temporal and spatial scales. As a first step, we here present a GPU based Monte Carlo particle-in-cell code to simulate electron avalanches and streamers, benchmarked against existing particle models. We will present this benchmarking as well as details on the GPU-code implementation as well as first results of electron avalanches and streamers and compare runtimes with previous models. This code will form the basis for a fully hybrid code running on the newest generation of pre-exascale computers. In the future, such a code will allow us to gain insight on the mechanisms responsible for TGFs.

How to cite: Fangel-Lloyd, E., Dujko, S., Karlsson, S., Gammelmark, M., Rydahl, A., Nishikawa, K., and Köhn, C.: Towards a GPU based particle model for streamer discharges, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7235, https://doi.org/10.5194/egusphere-egu23-7235, 2023.

EGU23-9041 | ECS | Orals | NH1.5

Optical properties of the shallow and exposed lightning discharges observed by ASIM 

Dongshuai Li, Torsten Neubert, Olivier Chanrion, Lasse Skaaning Husbjerg, Alejandro Luque, Yanan Zhu, Nikolai Østgaard, and Víctor Reglero

The Atmosphere-Space Interactions Monitor (ASIM) on the International Space Station (ISS) observes lightning and Transient Luminous Events (TLEs) above the thunderstorm clouds. ASIM includes three photometers that sample at 100 kHz and two cameras that image at 12 frames per second. The photometers measure part of the far ultraviolet (FUV) and middle ultraviolet (MUV) band at 180 – 300 nm, a line of the second positive system of N2 at 337nm (blue) and an atomic oxygen line at 777.4 nm (red). The cameras measure in the blue and red bands of the photometers with a spatial resolution on the ground around 400 m × 400 m. When ASIM is in a nadir-viewing configuration, photometer signals in the blue and red are sometimes associated with coincident UV signals, indicating that the UV photons originated from lightning discharges at cloud altitudes and not from the TLEs at higher altitudes. Here, we analyse the optical properties of these events by combining data from ASIM, the global lightning network GLD360, Lightning Mapping Arrays (LMAs) and NEXRAD radars. Of the 12 cases identified with such data coverage, 5 are Cloud-to-Ground (CG) and 7 are Intra-Cloud (IC) lightnings. The lightning leaders are located nearby the cloud top boundaries or partly exposed outside the cloud. Both the CG and IC lightnings are associated with the exposed lightning leaders. The 5 CG lightnings are identified as the “bolts from the blue”, and the 7 IC lightnings are “cloud-to-air” lightning. The altitudes of the sources vary from 5 km to 7 km for the CG lightnings and from 7 km to 15 km for the IC lightnings. The optical properties for the events, such as their irradiance, rise time and duration in the different optical bands are summarized and discussed. The results provide information that allows to estimate the global occurrence of “bolts from the blue” and “cloud-to-air” lightning.

How to cite: Li, D., Neubert, T., Chanrion, O., Husbjerg, L. S., Luque, A., Zhu, Y., Østgaard, N., and Reglero, V.: Optical properties of the shallow and exposed lightning discharges observed by ASIM, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9041, https://doi.org/10.5194/egusphere-egu23-9041, 2023.

EGU23-9381 | Posters on site | NH1.5

The scientific payload of the ALOFT mission to chase Terrestrial Gamma-ray Flashes and gamma-ray glows 

Martino Marisaldi, Nikolai Østgaard, Kjetil Ullaland, Shiming Yang, B. Hasan Qureshi, Jens Søndergaard, Andrey Mezentsev, David Sarria, Nikolai Lehtinen, Timothy J. Lang, Hugh Christian, Mason Quick, Richard Blakeslee, J. Eric Grove, and Daniel Shy

ALOFT (Airborne Lightning Observatory for FEGS and TGFs) is a flight campaign designed to observe Terrestrial Gamma-ray Flashes (TGF) and gamma-ray glows close to their production source. The campaign consists of 50 flight hours of a NASA ER-2 research aircraft taking off from Florida and is scheduled for July 2023. The ER-2 cruise altitude of 20 km allows flying over active thunderstorms in the Gulf of Mexico and Caribbean region, one of the most TGF-active region on the planet. The main challenge for TGF detection at close distance is the large variability in the expected gamma-ray flux, spanning four orders of magnitude depending on the radial distance from the source. To cope with this challenge, the ALOFT gamma-ray payload consists of several detectors of different size, made of different materials and readout sensors, designed to cover 4 orders of magnitude dynamic range on the typical TGF/gamma-ray glow energy range (~100 keV - ~40 MeV). In addition, the payload includes the Fly’s Eye GLM Simulator (FEGS), an array of imaging photometers sensitive at different wavelengths, and electric field change meters, and the Lightning Instrument Package (LIP), giving three component electric field measurements. The synergy between airborne gamma-ray, optical and electric field measurements, combined with ground-based radio observations, will provide a unique set of observations to constrain the source properties and their physics. This presentation will focus on the ALOFT scientific payload and the system architecture.

How to cite: Marisaldi, M., Østgaard, N., Ullaland, K., Yang, S., Qureshi, B. H., Søndergaard, J., Mezentsev, A., Sarria, D., Lehtinen, N., Lang, T. J., Christian, H., Quick, M., Blakeslee, R., Grove, J. E., and Shy, D.: The scientific payload of the ALOFT mission to chase Terrestrial Gamma-ray Flashes and gamma-ray glows, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9381, https://doi.org/10.5194/egusphere-egu23-9381, 2023.

EGU23-9415 | ECS | Orals | NH1.5

Detections of high peak current lightning and observations of Elves 

Ingrid Bjørge-Engeland, Nikolai Østgaard, Martino Marisaldi, Alejandro Luque, Andrey Mezentsev, Nikolai Lehtinen, Olivier Chanrion, Torsten Neubert, and Victor Reglero

Elves are produced when electromagnetic pulses from lightning interact with the lower parts of the ionosphere and are observed from space as expanding rings of light in the UV and visible optical bands. Elves are known to be associated with high peak current lightning. Using data from the Modular Multi-spectral Imaging Array (MMIA) instrument of the Atmosphere-Space Interactions Monitor (ASIM) payload, we search for observations of Elves when high peak currents (>70 kA) are detected by the global ground-based lightning detection network GLD360. We identify two types of events; high peak current detections associated with Elves, and high peak current detections not associated with Elves. To understand why some high peak current discharges do not generate observable Elves, we explore the number of lightning discharges and their peak currents leading up to the events. Preliminary results indicate that for current pulses with peak currents below 100 kA we observe a significant number of Elves, but this quantity depends on the lightning activity within 5 minutes before. Current pulses with peak currents above 120 kA nearly always produce Elves, regardless of the preceding lightning activity.

 

How to cite: Bjørge-Engeland, I., Østgaard, N., Marisaldi, M., Luque, A., Mezentsev, A., Lehtinen, N., Chanrion, O., Neubert, T., and Reglero, V.: Detections of high peak current lightning and observations of Elves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9415, https://doi.org/10.5194/egusphere-egu23-9415, 2023.

EGU23-9459 | ECS | Posters on site | NH1.5

Characterization of Thunderstorm Cells Producing Observable Terrestrial Gamma Ray Flashes 

Lasse Husbjerg, Torsten Neubert, Olivier Chanrion, Martino Marisaldi, Martin Stendel, Eigil Kaas, Nikolai Østgaard, and Victor Reglero

We present the largest catalogue compiled to date of TGFs and associated lightning activity, geostationary satellite cloud images and ERA5 reanalysis data. The TGFs are observed from AGILE, ASIM, FERMI and RHESSI, and the lightning activity by the WWLLN and GLD360 networks. The 1582 TGF events identified are analysed and contextualized relative to lightning flashes. In our analysis, we consider the proportion of TGFs and lightning coming from overshooting tops, and the dependencies on Cloud Top Temperature (CTT) and the Convective Available Potential Energy (CAPE). We find that TGFs come from primarily higher cloud tops than lightning flashes, consistent with previous studies. We also find that CAPE is similar for TGF and lightning-producing cells, and that the proportion of TGF and lightning-producing cells in the overshooting phase are similar. We analyse the regional and seasonal differences between TGFs and lightning and see that regional meteorological effects dominate.

How to cite: Husbjerg, L., Neubert, T., Chanrion, O., Marisaldi, M., Stendel, M., Kaas, E., Østgaard, N., and Reglero, V.: Characterization of Thunderstorm Cells Producing Observable Terrestrial Gamma Ray Flashes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9459, https://doi.org/10.5194/egusphere-egu23-9459, 2023.

EGU23-9989 | Orals | NH1.5

The nonlinear interactions of whistlers in the ionospheric plasma during strong thunderstorms 

Jan Blecki, Roman Wronowski, and Paweł Jujeczko

  It is not new knowledge that whistler are always present in the ionosphere during the thunderstorms. The terrestrial ionosphere is mainly a plasma region which is very sensitive for different disturbances. A wide range of plasma instabilities can develop  in this region, which are often nonlinear processes and leading to the development of plasma turbulence.  Turbulence is one of the most universal events phenomena in nature. It plays a crucial role in the dynamics of the space plasma processes. The turbulence appears when some physical parameter exceeds a certain level. It can have place during strong thunderstorms. The ionosphere is sometimes treated as plasma physics laboratory with unique possibility to study fundamental plasma processes. The use of ionospheric satellite  gives the chance to perform insitu measurement of plasma parameters during dynamic processes. For our analysis we used set of selected data  of the electric and magnetic fields variations in ELF and VLF ranges originating from the all French microsatellite DEMETER which was operating on the circular orbit with inclination of about 800 at altitude of 660 km from July 2004 until December 2010.

The  Fourier, wavelet and bispectral analysis of these signals has been performed. The 3 waves processes has been identified during few very strong strokes. In some cases the nonlinear interactions of whistlers with VLF signals of ground based transmitters. The character of spectra suggests the presence of Richardson’s cascade. Our conclusion is that these results are related to whistler turbulence.

How to cite: Blecki, J., Wronowski, R., and Jujeczko, P.: The nonlinear interactions of whistlers in the ionospheric plasma during strong thunderstorms, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9989, https://doi.org/10.5194/egusphere-egu23-9989, 2023.

The use of very low frequency (VLF) radio waves for monitoring the lower part of ionosphere (D region) has contributed immensely to explore this unique domain as satellites and other ground-based instrumentations have not been able to physically assess and characterized it. Several deployed ground- and space-based observational techniques not only enhance a robust capability to monitor, model and predict processes in the atmosphere-ionosphere-magnetosphere coupled regions, but also act as key feature to perform scientific studies in geo-sciences related areas. Here, we present preliminary results from multi-dimensional analyses of LF broadband measurement conducted from Ariel University (AU), Israel, as a complementary useful data source to other available ground- and space- based observational tools, already deployed. The AU LF (0.50 – 470 kHz) observational site, receives electromagnetic waves from different worldwide VLF transmitters as well as other natural sources such as lightning discharges. The station data is mainly used for diagnostic probing of ionospheric irregularities, caused by space weather events such as gamma-ray burst and EUV radiation, along with additional atmospheric electricity measurements. Additionally, different Machine Learning (ML) are used to study spheric waveforms in order to infer their exact location along with different physical characteristics.

How to cite: Ajakaiye, M. P., Reuveni, Y., and Romano, B.: Multi-dimensional Analyses of the First Measurement from the Low Frequency (LF) Radio Waves Receiving Station at Ariel University, Israel, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10903, https://doi.org/10.5194/egusphere-egu23-10903, 2023.

EGU23-11467 | Posters virtual | NH1.5

Discerning TGF and Leader Current Pulse in ASIM Observation 

Andrey Mezentsev, Nikolai Østgaard, Martino Marisaldi, Torsten Neubert, Olivier Chanrion, and Victor Reglero

TGFs being the bursts of high energy photons shot from Earth’s atmosphere to space, are known to be produced during the initial upward propagation of the +IC lightning leader. VLF and LF radio sferics can often be found in association with the short duration TGFs. The Atmosphere-Space Interactions Monitor (ASIM) instrument provides synchronous X- and gamma-ray measurements with optical recordings in 180-240 nm, 337 nm and 777.4 nm wavelength. This allows for simultaneous detection for TGFs and the lightning processes associated with them.

ASIM TGF observations have shown that TGFs within the FOV of the optical instruments are always accompanied by the prominent optical pulse which starts the lightning flash. TGFs have a clear tendency to slightly precede the optical pulse, but the short duration of TGFs together with the optical delay of the lightning light propagating through the cloud do not allow to confidently resolve the true sequence of these events.

The same problem is present in radio measurements: radio signature from TGF current is usually mixed with lightning current in the recordings due to temporal proximity of the processes involved.

Here we report a remarkable, high fluence and long duration TGF, together with its associated optical recordings. This observation shows clear distinction between the TGF and the associated optical pulse: the optical pulse is subsequent to the TGF, as it starts after the TGF is terminated. This allows to conclude that strong current surges inside the leader channel are not responsible for the TGF generation, and, in turn, the current surge producing the optical pulse can be conditioned by the generated TGF, or even be responsible for TGF termination.

How to cite: Mezentsev, A., Østgaard, N., Marisaldi, M., Neubert, T., Chanrion, O., and Reglero, V.: Discerning TGF and Leader Current Pulse in ASIM Observation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11467, https://doi.org/10.5194/egusphere-egu23-11467, 2023.

EGU23-11504 | Orals | NH1.5

Searching for the VHF signature of the tip of an intra-cloud positive leader 

Olaf Scholten, Brian Hare, Joe Dwyer, Ningyu Liu, and Christopher Sterpka

We have used the LOw-Frequency ARray (LOFAR) to search for the growing tip of an intra-cloud (IC) positive leader. LOFAR is an extended astronomical radio telescope consisting of many (thousands antennas arranged is stations operating at very-high frequencies (VHF). For these lightning observations we have used about 170 dual polarized antennas in the Netherlands with baselines up to 100 km.  

Even with our most sensitive beamforming method, where we coherently add the signals of all 170 antenna pairs, we were not able to detect any emission from the tip of an IC positive leader. Instead, we put constraints on the emissivity of VHF radiation from the tip at 1 aJ/MHz at 60 MHz, well below the intensity of the galactic background.

We conclude that these IC positive leaders propagate in a continuous process which is in sharp contrast to what is seen to the step-wise propagation seen in some cloud-to-ground positive leaders and for negative leaders.

How to cite: Scholten, O., Hare, B., Dwyer, J., Liu, N., and Sterpka, C.: Searching for the VHF signature of the tip of an intra-cloud positive leader, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11504, https://doi.org/10.5194/egusphere-egu23-11504, 2023.

EGU23-12033 | ECS | Orals | NH1.5

CASPER: A Space Mission Concept to Investigate Transient Luminous Events and Terrestrial Gamma Ray Flashes 

Manuel Maurer, Louí Byrne, Ulrik Falk-Petersen, Ali Hamdoun, Gwendal Hénaff, Kilian Huber, Andreea Ilas, Nadja Reisinger, Jonas Sinjan, Crisel Suarez, András Szilágy-Sándor, Vertti Tarvus, Marialinda Tsindis, and Mikhail Vaganov

As part of the Alpbach Summer School, a collaboration between FFG, ESA and ISSI, a team of students developed the F-class CASPER mission concept to investigate Transient Luminous Events (TLEs) and Terrestrial Gamma Ray Flashes (TGFs). These lightning-related plasma phenomena, first detected on Earth in 1989, typically occur in the mesosphere at an altitude between 50-100 km. The UVS instrument onboard the JUNO mission detected several similar events on Jupiter, and they are expected to also occur on other planets.

The CASPER mission consists of two identical spacecraft, each of which will be equipped with three cameras in different wavelengths and four high speed sensors, the latter will function as triggers to start the data acquisition of higher resolution images. A system chosen to combat the transient characteristic of the events (lifetime < 300 ms). While three sensors will be taking measurements of photons, one will quantify the electron flux in order to constrain the role of TLEs and TGFs in the global electric circuit.

The second great area of interest is the vertical structure of TLEs as well as their global distribution and occurrence rates. To achieve this, data will be captured using a two-satellite train in a sun-synchronous low earth orbit. The orbit is inclined at 98° and the satellites are phased at an angle of 5.2° to observe these events from two points of view simultaneously. The operational mission lifetime is five years, with a possible extension.

How to cite: Maurer, M., Byrne, L., Falk-Petersen, U., Hamdoun, A., Hénaff, G., Huber, K., Ilas, A., Reisinger, N., Sinjan, J., Suarez, C., Szilágy-Sándor, A., Tarvus, V., Tsindis, M., and Vaganov, M.: CASPER: A Space Mission Concept to Investigate Transient Luminous Events and Terrestrial Gamma Ray Flashes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12033, https://doi.org/10.5194/egusphere-egu23-12033, 2023.

EGU23-12591 | Orals | NH1.5

The propagation and 3D VHF polarization properties of recoil leaders 

Brian Hare, Olaf Scholten, Stijn Buitink, Joseph Dwyer, Ningyu Liu, Chris Sterpka, and Sander ter Veen

Lightning dart and recoil leaders are difficult to understand, as they have a different (often smoother) propagation mode than stepped leaders, and re-ionize a previously ionized channel. In order to understand them better, we have imaged recoil leaders with the LOFAR radio telescope (30-80 MHz), and will present 3D polarization, speed, and intensity data from multiple recoil leaders. We will show that many recoil leaders with high VHF intensity have VHF polarization that is very parallel to the recoil leader channel, with an opening angle as small as 15 degrees. Recoil leaders with lower VHF intensity have larger polarization opening angles, but it is not clear if this is physical or instrumental. In addition, VHF emission from recoil leaders comes from a sub-meter thin channel. Finally, we will show that the propagation speed and VHF intensity are strongly correlated; almost following a power-law or exponential relationship. These results probe the streamer behavior of recoil leaders, and thus provide significant clues to how recoil and dart leaders propagate. The fact that recoil leaders are very VHF thin is consistent with small polarization opening angles, and demonstrates that recoil leaders have significant streamer activity in their core and their corona sheath is VHF silent. The power-law/exponential relationship between speed and VHF intensity, however, is very difficult to explain.

How to cite: Hare, B., Scholten, O., Buitink, S., Dwyer, J., Liu, N., Sterpka, C., and ter Veen, S.: The propagation and 3D VHF polarization properties of recoil leaders, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12591, https://doi.org/10.5194/egusphere-egu23-12591, 2023.

EGU23-13117 | Posters on site | NH1.5

Modelling of cloud electrification 

Jana Popová and Zbynek Sokol

We developed a cloud electrification model (CEM) which describes the evolution of the electric field in clouds, including electric discharges. Our CEM simulates evolution of charge of individual hydrometeors (cloud droplets, rain droplets, ice, snow, graupel) and models the distribution of positive and negative ions. Using this model, we compared the evolution of electric charge and electric field for selected winter and summer thunderstorms that occurred close to the Milešovka meteorological observatory. We analysed the dataset of thunderstorms using measurements of Ka-band cloud profiler and X-band weather radar, both located at the Milešovka observatory, and standard meteorological measurements. The analyses include a comparison of the structure of the modelled thunderstorms with the structure derived from radar and satellite observations. 

How to cite: Popová, J. and Sokol, Z.: Modelling of cloud electrification, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13117, https://doi.org/10.5194/egusphere-egu23-13117, 2023.

EGU23-13197 | ECS | Orals | NH1.5

The Role of Global Thunderstorm Activity in Modulating Global Cirrus Clouds 

Joydeb Saha, Colin Price, and Anirban Guha

Cirrus clouds provide a significant radiative forcing on the Earth's climate system. The net cloud radiative forcing for cirrus clouds results a warming of the climate.  More/less cirrus clouds result in more/less warming of the planet. The moisture for the formation of cirrus clouds in the upper atmosphere is transported there in large part via deep convective storms, many associated with lightning activity and hence defined as thunderstorms.  An increasing in cirrus clouds in a warmer atmosphere will amplify the initial warming. This paper looks at the connection in space and time between monthly mean lightning activity observed from the Lightning Imaging Sensor on board the International Space Station (LIS-ISS), and the global monthly mean cirrus cloud cover obtained from the MERRA-2 reanalysis product. The correlation coefficient between the global monthly mean cloud optical thickness (COT) of the cirrus clouds (clouds at altitudes above the 400hPa pressure levels) with the monthly mean lightning flash counts is 0.84, implying that monthly mean  lightning can explain 70% of monthly variability of the global high cloud optical thickness. In addition, lightning amount explains nearly 60% of the monthly mean global area coverage of cirrus clouds.  Given these statistically significant connections between lightning and cirrus clouds, we propose using global lightning data as an additional tool for monitoring monthly variability of cirrus clouds.

 

How to cite: Saha, J., Price, C., and Guha, A.: The Role of Global Thunderstorm Activity in Modulating Global Cirrus Clouds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13197, https://doi.org/10.5194/egusphere-egu23-13197, 2023.

EGU23-13985 | Posters virtual | NH1.5

Development and testing of a modernised Programmable Ion Mobility Spectrometer 

Karen Aplin, Alan Meaney, József Bór, and Attila Buzás

The atmosphere is made slightly electrically conductive by cosmic rays and natural radioactivity, which generate ions. Air conductivity is a key component of the global electric circuit and influences droplet and cloud charging [1]. Further, atmospheric ions may affect the radiative balance through particle formation and infra-red absorption [2], [3]. Both considerations motivate the need for accurate atmospheric ion measurements. The Programmable Ion Mobility Spectrometer (PIMS) is a computer-controlled instrument based on the Gerdien measurement principle in which a cylindrical capacitor, across which a voltage is applied, is aspirated to sample air ions [4]. Computer control of a switchable multimode electrometer [5] offers the capability to measure ions in two modes, offering self-calibration, which removes the difficulties with providing a well-characterised environment for calibration [6]. The PIMS can independently monitor internal leakage currents which can be a significant source of thermally dependent error, especially in outdoor use. First developed in the early 2000s, the PIMS has recently been modernised with a new electrometer and advanced microcontroller, leading to significantly miniaturised electronics and opportunities for more sophisticated interfacing. The modernised PIMS was tested at Nagycenk Geophysical Observatory (47.632°N,16.718°E), Hungary in summer 2022, alongside a full range of meteorological and atmospheric electrical measurements for comparison.

 

References

[1]      R. G. Harrison and K. A. Nicoll, “The electricity of extensive layer clouds,” Weather, vol. 77, no. 11, pp. 379–383, Nov. 2022, doi: 10.1002/wea.4307.

[2]      K. L. Aplin, “Composition and measurement of charged atmospheric clusters,” Space Sci Rev, vol. 137, no. 1–4, 2008, doi: 10.1007/s11214-008-9397-1.

[3]      K. L. Aplin and M. Lockwood, “Cosmic ray modulation of infra-red radiation in the atmosphere,” Environmental Research Letters, vol. 8, no. 1, 2013, doi: 10.1088/1748-9326/8/1/015026.

[4]      K. L. Aplin and R. G. Harrison, “A computer-controlled Gerdien atmospheric ion counter,” Review of Scientific Instruments, vol. 71, no. 8, 2000, doi: 10.1063/1.1305511.

[5]      R. G. Harrison and K. L. Aplin, “Multimode electrometer for atmospheric ion measurements,” Review of Scientific Instruments, vol. 71, no. 12, 2000, doi: 10.1063/1.1327303.

[6]      K. L. Aplin and R. G. Harrison, “A self-calibrating programable mobility spectrometer for atmospheric ion measurements,” Review of Scientific Instruments, vol. 72, no. 8, 2001, doi: 10.1063/1.1382634.

How to cite: Aplin, K., Meaney, A., Bór, J., and Buzás, A.: Development and testing of a modernised Programmable Ion Mobility Spectrometer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13985, https://doi.org/10.5194/egusphere-egu23-13985, 2023.

Being one of the natural hazards and an indicator of severe weather, studying and evaluating lightning activity has a well recognized role in scientific research. The detection of lightning activity with a good efficiency is crucial not only to the protection of human lives and minimizing economic losses, but to get a better understanding of Earth’s climate system as well.

There are several solutions for lightning detection implemented both on ground (e.g., Earth Networks, EUCLID, LINET, WWLLN, etc.) and in space (e.g., GLM, LIS, OTD) providing a big amount of reliable data. The BlitzOrtung (BO) is a dynamically developing and community-based lightning detection network (Wanke et al., 2014). By 2018, the BO had circa 2000 stations around the globe (Narita et al., 2018) and their data are used widely in Europe. However, there is a need to evaluate the detection efficiency and compare the parameters of the detected lightning strokes with the ones derived from other networks (Narita et al., 2018).

In this study, we aim at evaluating the performance of the BO network on a statistical basis. First, the detected lightning strokes are paired with those reported by the LINET and WWLLN systems using the time point and location information. Then the geographical distribution as well as the temporal stability of the number of detected events and the percentage of paired events are examined. The first results of a pilot analysis over Hungary (45.5°-49° N, 16°-23° E) in Central Europe will be presented. This project serves to establish a comparison-based method for the evaluation of the lightning climatology of a region.

 

Narita, T. et al. (2018): A study of lightning location system (Blitz) based on VLF sferics, 34th International Conference on Lightning Protection, 978-1-5386-6635-7/18/$31.00,

Wanke, E., Andersen, R., and Volgnandt, T. (2014): A World-Wide Low Cost Community-Based Time-Of-Arrival Lightning Detection and Lightning Location Network, http://www.blitzortung.org/Documents/TOA_Blitzortung_RED.pdf

How to cite: Buzás, A., Bozóki, T., and Bór, J.: Community-based lightning detection in Europe: studying the detection efficiency of the BlitzOrtung network - a case study concerning lightning climatology over Hungary, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14243, https://doi.org/10.5194/egusphere-egu23-14243, 2023.

EGU23-14440 | Orals | NH1.5

Removing local variability from Potential Gradient data – the Carnegie filter 

R.Giles Harrison, Keri Nicoll, Manoj Joshi, and Ed Hawkins

Measurements of atmospheric electricity have been made at many sites over a long time, with the vertical Potential Gradient (PG) the most commonly observed quantity. In general, the PG responds to local influences from weather, aerosol effects on charge exchange, and variability in the global atmospheric electric circuit. Different methods have been used to classify PG data, for example through identifying days when conditions were considered relatively undisturbed, or by using meteorological information to identify days on which weather-related variability was negligible. Nevertheless, local effects can persist, especially in data obtained at continental sites. Hence, if long term changes in the global atmospheric electric circuit are to be investigated, the local effects need first to be reduced or, ideally, removed.

Recent work has demonstrated a close relationship between the PG at some sites and ocean temperatures modulated by the El Niño Southern Oscillation, through the associated changes in the global atmospheric electric circuit ([1],[2], [3]). The expectation of such a relationship can be used to test methods of removing and reducing local effects in PG data. A method based on the Carnegie curve – the hourly variation known to be present in the global circuit – is discussed here. Through comparison of hourly PG data from a site with the Carnegie curve, outlier values lying beyond the usual range of global circuit changes can be identified and removed. The remaining data can then be used to construct new daily or monthly averages with reduced local variability, evaluated by comparison with global circuit changes associated with the El Niño Southern Oscillation.

 

References

[1] R.G. Harrison, K.A. Nicoll, M. Joshi, E. Hawkins: Empirical evidence for multidecadal scale Global Atmospheric Electric Circuit modulation by the El Niño-Southern Oscillation Environ Res Lett 17, 124048 (2022) https://iopscience.iop.org/article/10.1088/1748-9326/aca68c

[2] N.N. Slyunyaev, N.V.I lin, , E.A. Mareev,.G. Price: A new link between El Nino - Southern Oscillation and atmospheric electricity, Environ. Res. Lett., 16, (2021) https://doi.org/10.1088/1748-9326/abe908 

[3] R.G. Harrison, M. Joshi, K. Pascoe: Inferring convective responses to El Niño with atmospheric electricity measurements at Shetland Environ Res Lett 6 (2011) 044028  http://iopscience.iop.org/1748-9326/6/4/044028/ 

How to cite: Harrison, R. G., Nicoll, K., Joshi, M., and Hawkins, E.: Removing local variability from Potential Gradient data – the Carnegie filter, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14440, https://doi.org/10.5194/egusphere-egu23-14440, 2023.

EGU23-14579 | Orals | NH1.5

Increase in Lightning and Upper Tropospheric Water Vapour Over the Arctic Circle 

Anirban Guha, Joydeb Saha, and Colin Price

Sea ice in the Arctic grows during each hemisphere’s winter and it retreats in the summer. The highly reflective white surface of sea ice reflects solar energy, cooling the planet. When it melts, the darker ocean absorbs more heat, reinforcing the cycle of melting sea ice. Sea ice plays a critical role in regulating Earth’s climate, and it influences global weather patterns and ocean circulations. One essential feedback in the Arctic is the rise in upper tropospheric water vapor (UTWV) or the specific humidity (SH) that acts as an intense greenhouse gas trapping in additional heat released from the Earth's surface.   While temperature change is driven by increasing greenhouse gases, the interannual variability in sea ice can be explained by changes in the UTWV (ASO) at 400mb in the Arctic. Where is this increase in UTWV (400mb) coming from in the Arctic?  Thunderstorm activity appears to be increasing in the Arctic in the last decades, and could be a source of the increasing UTWV, and hence the decrease in Arctic sea ice.

How to cite: Guha, A., Saha, J., and Price, C.: Increase in Lightning and Upper Tropospheric Water Vapour Over the Arctic Circle, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14579, https://doi.org/10.5194/egusphere-egu23-14579, 2023.

EGU23-14736 | ECS | Posters on site | NH1.5

Validation of the ASIM MXGS performance using cosmic Gamma-Ray Bursts 

Andreas Ramsli, Martino Marisaldi, Anastasia Tsvetkova, Cristiano Guidorzi, David Sarria, Andrey Mezentsev, Anders Lindanger, Nikolai Østgaard, Torsten Neubert, Victor Reglero, Dmitry Svinkin, Alexandra Lysenko, and Dmitry Frederiks

The Atmosphere-Space Interactions Monitor (ASIM) is a mission of the European Space Agency launched in April 2018 and hosted onboard the International Space Station (ISS). ASIM is dedicated to study the physics of Transient Luminous Events (TLEs) and Terrestrial Gamma-ray Flashes (TGFs) and their relation to lightning. TGFs are X- and Gamma-ray flashes associated to lightning discharges, with average duration of few tens of microseconds and energies up to 40 MeV. ASIM detects TGFs by means of the Modular X- and Gamma-ray Sensor (MXGS). So far, the MXGS performance (efficiency, effective area) have been evaluated by Monte Carlo simulations only, while energy calibration is monitored using built-in radioactive sources and background lines. TGFs are local events, very rarely observed by more then one spacecraft simultaneously, therefore it is difficult to use them to validate the MXGS performance. Goal of this study is to use cosmic Gamma-ray Bursts (GRBs) simultaneously detected by ASIM and other spacecraft as calibration sources to validate the spectral performance of MXGS. GRBs are the brightest explosions in the universe, associated to the collapse of massive stars or the merger of compact objects, involving at least one neutron star, at cosmological distances. During the period from June 2018 to December 2021, 12 GRBs were detected by ASIM and by one or more other spacecraft. Here we use data from the Konus-WIND mission and from the Fermi Gamma Burst Monitor (GBM), both considered as benchmarks in the field of GRB analysis. We cross-correlate the light curves of the three instruments, and we perform simultaneous spectral analysis using the forward-folding approach. In some cases, we find good consistency between the detectors, indicating an overall validation of the MXGS performance. In other cases, we identified discrepancies, possibly due to absorption from structures of the ISS, currently under investigation. In this presentation, we show our data sample, the methodology used and the preliminary joint spectral analysis results. This work is relevant because it will provide an independent assessment of the MXGS performance, with clear implications for ASIM TGF results.

How to cite: Ramsli, A., Marisaldi, M., Tsvetkova, A., Guidorzi, C., Sarria, D., Mezentsev, A., Lindanger, A., Østgaard, N., Neubert, T., Reglero, V., Svinkin, D., Lysenko, A., and Frederiks, D.: Validation of the ASIM MXGS performance using cosmic Gamma-Ray Bursts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14736, https://doi.org/10.5194/egusphere-egu23-14736, 2023.

EGU23-15378 | Orals | NH1.5

Studying downward TGFs with the largest ground array of gamma-ray detectors 

Roberta Colalillo, Joseph Dwyer, David M. Smith, and John Ortberg and the Pierre Auger Collaboration

The Pierre Auger Observatory, the largest cosmic-ray detector in the world, has been
observing peculiar events which are very likely downward TGFs. Their experimental
signature and their time evolution are very different from those of a shower produced
by an ultra high energy cosmic ray. The TGF-like events happen in coincidence with
lightning and low clouds and their deposited energy at the ground is compatible with
that of a standard downward TGF with the source at few kilometers above the
ground. The surface detector (SD) of the Auger Observatory consists of 1660 water-
Cherenkov detectors (WCDs) spread over 3000 km2 in the Argentinian pampa. The
WCD height of 1.2 m makes them highly sensitive to gamma rays and the large area
covered with SD allows us to sample the TGF beam from different points. The
timing shape of WCD signals can be very important to constrain different TGF source
models. Cold runaway from the high fields near the leader tips or relativistic
feedback produce the same energy spectrum but predict a different rise and fall of the
counts versus time, and they could produce a different angular distribution.
Comparisons between simulations and data will be shown.
Moreover, first results from a preliminary analysis of the available meteorological
data at the time of Auger TGF-like events will be presented. Little is known about the
TGF-producing storms. The characteristics of these thunderstorms are being
investigated by studying meteorological data in coincidence with upward TGFs. A
similar analysis is important to better understand downward TGF production
mechanisms and investigate if are the same as those producing upward TGFs.

How to cite: Colalillo, R., Dwyer, J., Smith, D. M., and Ortberg, J. and the Pierre Auger Collaboration: Studying downward TGFs with the largest ground array of gamma-ray detectors, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15378, https://doi.org/10.5194/egusphere-egu23-15378, 2023.

EGU23-15873 | Posters on site | NH1.5

THOR-DAVIS: A neuromorphic camera to observe thunderstorms from inboard ISS. 

Olivier Chanrion, Nicolas Pedersen, Andreas Stokholm, Benjamin Hauptmann, and Torsten Neubert

The technical purpose of THOR-DAVIS is to test a new camera concept in space for observations of thunderclouds and their electrical activity at up to a resolution of 10 µs. The scientific purpose is to conduct video camera observations of thunderclouds and their electrical activity. The focus is on altitude-resolved measurements of activity at the top of the clouds and the stratosphere above. The camera type is a so-called neuromorphic camera (or event camera) where pixels are read out asynchronously when the pixel illumination changes. The goal is to understand, under realistic conditions, the use of such a camera for future use in space for observations of processes in severe electrical storms. The camera has a high temporal resolution 100.000 equivalent frame per second and a huge dynamic range of about 120 dB and is particularly well suited for this kind of observations. The camera weights about 200g and consumes about 1.5A in operation and is particularly well suited for space applications.

In this presentation we will give the status of the development of the THOR-DAVIS experiment to be conducted by the Danish astronaut Andreas Mogensen during his upcoming ESA mission Huggin onboard the International Space Station (ISS). We’ll present the design of the payload based on a Davis 346 neuromorphic camera mounted on top of a Nikon D5 camera for handheld operation. The 2 cameras are controlled by an AstroPi unit based on a Raspberry Pi computer board.

Finally, we’ll give preliminary results of laboratory measurements made with the flight model.

 

How to cite: Chanrion, O., Pedersen, N., Stokholm, A., Hauptmann, B., and Neubert, T.: THOR-DAVIS: A neuromorphic camera to observe thunderstorms from inboard ISS., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15873, https://doi.org/10.5194/egusphere-egu23-15873, 2023.

EGU23-15876 | Orals | NH1.5

TGFs - "Storm Activity" relationship  

Javier Navarro-González, Paul Connell, Chris Eyles, Víctor Reglero, Jesús Alberto López, Joan Montanyà, Martino Marisaldi, Andrey Mezentzev, Anders Lindanger, David Sarria, Nikolai Østgaard, Olivier Chanrion, Freddy Christiansen, and Torsten Neubert

In the first two years of ASIM operations from June 2018 till the end of 2019 486 TGFs have been observed, with a TGF rate of 0.84 per day. Their geographical distribution is consistent with the three main lightning chimneys Central America, Central Africa, and South East of Asia. Figure 1 displays the ISS footprint positions when the TGFs were detected.

Figure 1: ISS position for the 2018-2019 ASIM TGFs. Red circles marked those within 4 minutes of the previous TGF detected.

If the TGF occurrence follows a stochastic process (each TGF is not related to the next one), the time-difference distribution between a TGF detection and the next one should fit an exponential distribution. For a Δt < 4 minutes the number of TGFs following the exponential distribution is 16. Opposite we got 85 in groups of 2-3 TGFs displayed in Figure 1 in red circles. Analyzing the apparent strong discrepancy in the number of detection in less than 4 minutes (Figure 2) and the number derived from the exponential distribution is one of the motivations of this study.

We build a grid of variable dimension cell size to keep the same ISS observing time for each cell in a Monte Carlo code to simulate the TGF generation that has into account the frequency and the anisotropy distribution of the TGFs over the earth.

To preserve the total number of TGF observed in Δt < 4 minutes we need to add a parameter related to the “Storm Activity” defined as the time in a cell available to generate a TGF. The model fits observations when this parameter is 7%±1%. The good correlation between model/observation is displayed in Figure 2.

Figure 2: The predicted distribution of the TGF pairs (Orange) in 15s bins fits the observations (Blue).

The scope of this work is to check the adopted “Storm Activity” value using WWLLN sferics database as a good indicator of storm activity.

 

 

 

 

 

 

 

How to cite: Navarro-González, J., Connell, P., Eyles, C., Reglero, V., López, J. A., Montanyà, J., Marisaldi, M., Mezentzev, A., Lindanger, A., Sarria, D., Østgaard, N., Chanrion, O., Christiansen, F., and Neubert, T.: TGFs - "Storm Activity" relationship , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15876, https://doi.org/10.5194/egusphere-egu23-15876, 2023.

EGU23-16046 | Orals | NH1.5

Investigating ELVE photometric waveforms with elementary electromagnetics 

Alejandro Luque Estepa, Ingrid Bjørge-Engeland, Dongshuai Li, Nikolai Østgaard, and Martino Marisaldi

ELVEs are quickly expanding rings of light emissions excited in the lower ionosphere by the electromagnetic pulse of an electric discharge in a thundercloud. They are commonly observed from space platforms and have been reported in conjunction with other atmospheric-electricity events. One motivation to investigate ELVEs is that their signal may provide insight into the discharge that created them. Until now the modeling of ELVES has either relied on strong simplifications or on the Finite-Difference Time-Domain (FDTD) method to directly solve the Maxwell equations. One limitation of the latter is that non-axisymmetrical discharges (with a slanted channel or a non-vertical magnetic field for example) require computationally expensive, fully three-dimensional meshes, which makes parametric studies of the ELVE features slow and cumbersome.  We show here that elementary electromagnetic theory allows one to model ELVEs, even non-axisymmetrical ones, with sufficient accuracy at little computational cost. We then apply our methods to the parametric study of ELVE photometric waveforms as recorded by space-based instruments.

How to cite: Luque Estepa, A., Bjørge-Engeland, I., Li, D., Østgaard, N., and Marisaldi, M.: Investigating ELVE photometric waveforms with elementary electromagnetics, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16046, https://doi.org/10.5194/egusphere-egu23-16046, 2023.

EGU23-16868 | ECS | Posters on site | NH1.5

Project JetNet: Hemispheric-scale gigantic jet detection network 

Levi Boggs, Jeffrey Smith, Douglas Mach, Steve Cummer, John Trostel, Jeffery Burke, and Jessica Losego

In this presentation we will provide an overview and present preliminary results from a multi-institutional collaborative project, which seeks to detect gigantic jets over hemispheric scales using a combination orbital and ground-based sensors and machine learning. Gigantic jets are a type of transient luminous event (TLE, Pasko 2010, doi: 10.1029/2009JA014860) that escape the cloud top of a thunderstorm and propagate up to the lower ionosphere (80-100 km altitude), transferring tens to hundreds of Coulombs of charge. Our detection methodology primarily uses the Geostationary Lightning Mapper (GLM), which is a staring optical imager in geostationary orbit that detects the 777.4 nm (OI) triplet commonly emitted by lightning (Goodman et al. 2013, doi: 10.1016/j.atmosres.2013.01.006).  Gigantic jets have been shown to have unique signatures in the GLM data from past studies (Boggs et al. 2019, doi: 10.1029/2019GL082278; Boggs et al. 2022, doi: 10.1126/sciadv.abl8731). Thus far, we have built a preliminary, supervised machine learning model that detects potential gigantic jets using GLM, and begun development on a series of vetting techniques to confirm the detections as real gigantic jets. The vetting techniques use a combination of low frequency (LF) and extremely low frequency (ELF) sferic data, in combination with stereo GLM measurements. When our detection methodology grows in maturity, we will deploy it to all past GLM data (2018-present), with the potential to detect thousands of events each year, allowing correlation with other meteorological and atmospheric measurements. We will share the database of gigantic jet detections publicly during and at project conclusion (2025), allowing other researchers to use this data for their own research.

How to cite: Boggs, L., Smith, J., Mach, D., Cummer, S., Trostel, J., Burke, J., and Losego, J.: Project JetNet: Hemispheric-scale gigantic jet detection network, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16868, https://doi.org/10.5194/egusphere-egu23-16868, 2023.

EGU23-16886 | ECS | Orals | NH1.5

Earth Networks Lightning System Update 

Elizabeth DiGangi, Jeff Lapierre, Yanan Zhu, and Michael Stock

Global lightning location data has long been a critical tool for lightning research and safety. The Earth Networks Total Lightning Network (TLN) incorporates advanced lightning location technology delivering competitive lightning detection efficiency, location accuracy, and classification (intracloud vs cloud-to-ground). It consists of over 1800 wideband sensors deployed in 40+ countries to detect lightning and generate real-time localized storm alerts. TLN is constantly evolving through network expansion, as well as hardware and software development. In this presentation, we will cover some of the recent advances to the TLN hardware and processor. The new TLN sensor has been redesigned to use a dipole sensing element to help reduce the requirements of a strong ground. These new sensors are currently being used operationally and produce comparable waveforms to the previous monopole antenna. New upgrades to the lightning location algorithm have increased the detection efficiency, location accuracy, and classification accuracy of the network. Globally, TLN is locating approximately 50% more pulses than it was before. In moderately remote regions of the world, performance gains can be higher. TLN continues to use data from the World Wide Lightning Location Network (WWLLN), enhanced via raw signals from approximately 200 TLN sensors, to locate lightning in extremely remote regions like the deep oceans. However, how WWLLN data is incorporated into the TLN feed has changed, leading to significantly reduced false alarm rates in some regions. Location accuracy was improved by developing a new propagation model for signals produced by lightning, resulting in a reduction in location error by as much as a factor of 2. As a result of the improved location accuracy, as well as enhancements to the false alarms rates, there is improved clustering of lightning, which directly impacts downstream products such as lightning alerting and Dangerous Thunderstorm Alerts.

How to cite: DiGangi, E., Lapierre, J., Zhu, Y., and Stock, M.: Earth Networks Lightning System Update, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16886, https://doi.org/10.5194/egusphere-egu23-16886, 2023.

EGU23-17102 | ECS | Orals | NH1.5

ELF-transients detected in the broadband recordings at the Hylaty station in Poland 

Tamas Bozoki, Janusz Młynarczyk, Jozsef Bor, Jerzy Kubisz, Istvan Bozso, Andras Horvath, Lukacs Kuslits, and Mate Timko

Lightning acts as a natural antenna radiating electromagnetic (EM) waves in a wide frequency range. In the extremely low frequency (ELF) band (3 Hz - 3 kHz), lightning-induced EM waves suffer very weak attenuation while they propagate in the waveguide formed by the Earth’s surface and the lowest part of the ionosphere. These EM waves can travel around the Earth several times before losing most of their energy. This allows ELF-transients generated by powerful lightning discharges from around the globe to be detected at any observation site. We developed an algorithm that identifies ELF-transients in the broadband recordings at Hylaty, Poland (sampling frequency: 3004.81 Hz, antenna bandwidth: 0.02 Hz to 1.1 kHz) and finds their most probable source lightning discharge in the lightning database of the Word Wide Lightning Location Network (WWLLN) based on the technique described by Bór et al. (2022).

Between July 2020 and April 2021 about 270,000 ELF-transients were found in the records from Hylaty. The most probable source of 160,000 transients  was identified in the WWLLN database. Using this data set, we show that the propagation speed of broadband ELF-transients differ significantly when the propagation path is on the dayside or on the nightside of the Earth. It is also demonstrated that for lightning discharges close to Hylaty (d<2Mm), the timing and location accuracy of WWLLN has a large impact on the identification of the lightning source and on the inferred propagation speed. A convolutional neural network, trained with ELF-transients of known source location, was used to determine the distance to the lightning source in cases where the source lightning discharge could not be found in the WWLLN database. The average accuracy of the distance provided by the neural network is 700 km. No significant difference can be seen between the distribution of distances obtained by matching the source lightning stroke in the WWLLN database and that obtained using the neural network-based approach.

 

Reference:

Bór, J., Szabóné André, K., Bozóki, T., Mlynarczyk, J., Steinbach, P., Novák, A., and Lemperger, I. (2022): Estimating the Attenuation of ELF-Band Radio Waves in the Earth’s Crust by Q-Bursts. IEEE Transactions on Antennas and Propagation, 70, 8. https://doi.org/10.1109/TAP.2022.3161504

How to cite: Bozoki, T., Młynarczyk, J., Bor, J., Kubisz, J., Bozso, I., Horvath, A., Kuslits, L., and Timko, M.: ELF-transients detected in the broadband recordings at the Hylaty station in Poland, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17102, https://doi.org/10.5194/egusphere-egu23-17102, 2023.

AS2 – Boundary Layer Processes

EGU23-350 | ECS | Posters virtual | AS2.1

Atmospheric Boundary Layer and the Vertical Distribution of Black Carbon over Plain and Hilly Terrain of North East India using In Situ Measurements 

Manasi Gogoi, Arup Borgohain, Arundhati Kundu, Shyam S. Kundu, Pradip K. Bhuyan, Binita Pathak, Kalyan Bhuyan, Nilamoni Barman, Trisanu Banik, Abhishek Charri, Aniket Chakravorty, Praveen Kumar, Rajdeep Chanda, Penumetcha L.N. Raju, Abhay Srivastava, Rekha B. Gogoi, and Shiv P. Aggarwal

The Atmospheric Boundary Layer (ABL) has always played a critical role in determining global aerosol dispersion and distribution in the atmosphere. Absorbing aerosols constituting of black carbon (BC) influences our atmosphere in several ways which includes absorption of the incoming solar radiation. There have been several studies on the spatio – temporal heterogeneity of aerosols over the North Eastern Region (NER) of India but very few studies exist on the vertical distribution of aerosols till date. To fill this gap, Microaethalometer (MA), Optical Particle Counter (OPC) and Dr. Pisharoty Radiosonde (sonde) has been deployed using tethered balloon up to 1 kilometre altitude on campaign mode for the first time in NER of India for characterization of airborne aerosols and meteorological parameters. The experiment was conducted successfully over a high altitude station in Meghalaya, Umiam (25.67 oN, 91.91o E, 1040 m amsl) during winter, pre monsoon and post monsoon seasons of the year 2019 and over 3 stations viz., Dhubri (26.02° N, 89.97° E, 31 metres), Guwahati (26.10° N, 91.60° E, 55 metres), and Dibrugarh (27.47° N, 94.91° E, 108 metres) along the Brahmaputra valley in Assam, India during the winter and pre monsoon seasons of the year 2021. Meteorological balloons were also launched simultaneously 4-5 times per day in each of these 3 stations for one day during the time of tethered balloon launch. Distinct diurnal variability has been observed in the vertical profiles of BC and meteorological parameters throughout the day. In the absence of incoming solar radiation or weak turbulence i.e. during the morning, evening and night time the ABL height (ABLH) measured by sonde varied from 75 – 200 m, 50 – 150 m, 100 – 275 m and 50 – 225 m during winter season over Umiam, Dhubri, Guwahati and Dibrugarh respectively. While during pre monsoon season, ABLH varied from 50 – 200 m, 75 – 250 m, 125 – 250 m and 50 to 250 m respectively over the 4 stations. Near surface BC concentration (BCC) was found to be high within the ABL during morning, evening and night time over all the stations. During winter and pre monsoon, maximum BCC reached up to approximately 9 µg/m3, 30.98 µg/m3, 22.16 µg/m3, 13.01 µg/m3 and 5 µg/m3, 9.65 µg/m3, 13.6 µg/m3, 6.4 µg/m3 respectively over Umiam, Dhubri, Guwahati and Dibrugarh near to the surface. ABLH goes above 1 km during day time, where the rapid development of a well mixed vertical profile of BC was observed during the day over the study sites. The vertical profiles of BC also showed multiple elevated layers in some stations which closely followed the vertical profiles of the meteorological parameters.

How to cite: Gogoi, M., Borgohain, A., Kundu, A., Kundu, S. S., Bhuyan, P. K., Pathak, B., Bhuyan, K., Barman, N., Banik, T., Charri, A., Chakravorty, A., Kumar, P., Chanda, R., Raju, P. L. N., Srivastava, A., Gogoi, R. B., and Aggarwal, S. P.: Atmospheric Boundary Layer and the Vertical Distribution of Black Carbon over Plain and Hilly Terrain of North East India using In Situ Measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-350, https://doi.org/10.5194/egusphere-egu23-350, 2023.

Vertical temperature profile close to the ground controls many micrometeorological processes. These include development of inversion layer, occurrence of fog, pollution dispersion and vertical transport of heat and moisture.  We here present results from an extensive field study, conducted at the observation site next to the north runway at the Kempegowda International Airport, Bengaluru, India (13.208°N, 77.704°E). At the site, we have deployed a HATPRO microwave radiometer, a Windcube Lidar, a set of 4-component radiative flux sensors, a weather station, a 2m mast carrying humidity and temperature sensors for monitoring temperature and humidity, along with a soil temperature profiler and two soil heat flux sensors. With this arrangement at the site, we continuously monitor the vertical profile of temperature, relative and absolute humidity from surface to 10 km height.

Evening transition of the atmospheric boundary layer (ABL) observed during and after the sunset (under calm and clear sky conditions) indicates the development of Lifted Temperature Minimum (LTM) type vertical temperature profiles at the site. Boundary layer cooling observed after the sunset extends more than 200 m from the surface. Cooling is strong near the ground. This leads to formation of penetrative-convection layer close to the ground. Above this unstable convective layer, a stable inversion layer develops that extends to several hundred meters in height.

We will present results from the numerical simulation of the ABL, by initializing from the radiometer observed vertical profile of temperature before sunset. Numerical simulations are based on a high-resolution, one-dimensional radiation model, coupled with ground temperature with and without aerosols' presence. LTM height, intensity, and its evolution with time observed from the field experiments and simulations have been compared and analyzed regarding radiation budget, aerosol property, number density, and soil emissivity. Results presented here indicate that the observed temperature profile in the field experiments matches closely with the simulations only when the presence of aerosols is considered in the numerical simulations. A high concentration of the aerosol in the surface layer, close to the ground enhances the radiative cooling and leads to the formation of the LTM profile.

How to cite: Singh, S. P. and Sreenivas, K.: Role of Aerosol-Induced Radiative Cooling on the Evening Transitions Observed in the Atmospheric Boundary Layer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-395, https://doi.org/10.5194/egusphere-egu23-395, 2023.

EGU23-1267 | Orals | AS2.1

PBL-Aerosol-Interactions and Impact on Turbulent Entrainment 

Zhanqing Li and Tianning Su

Aerosol-boundary layer interactions play an important role in affecting atmospheric thermodynamics and air pollution. As a key factor in dictating the development of the boundary layer, the entrainment process in the context of aerosol-boundary layer interactions is still poorly understood. Using comprehensive field observations made at a superstation in Beijing, we gain insight into the response of the entrainment process to aerosols. We found that high aerosol loading can significantly suppress the entrainment rate, breaking the conventional linear relationship between sensible heat fluxes and entrainment fluxes. Related to aerosol vertical distributions, aerosol heating effects can alter vertical heat fluxes, leading to a strong interaction between aerosols and the entrainment process in the upper boundary layer. Such aerosol-entrainment coupling can inhibit boundary layer development and explains the great sensitivity of observed entrainment rates to aerosols than can traditional calculations. The notable impact of aerosols on the entrainment process raises holistic thinking about the dynamic framework of the boundary layer in a polluted atmosphere, which may have a significant bearing on the dispersion of air pollutants and the land-atmosphere coupling

How to cite: Li, Z. and Su, T.: PBL-Aerosol-Interactions and Impact on Turbulent Entrainment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1267, https://doi.org/10.5194/egusphere-egu23-1267, 2023.

EGU23-1425 | ECS | Posters on site | AS2.1

Towards numerical simulation of a wind machine during spring frost calibrated with field measurements 

Clara Le Cap, Johan Carlier, Marwan Katurji, Dongqi Lin, Hervé Quénol, Philippe Georgeault, Emmanuel Buisson, and Dominique Heitz

Spring frost has been recognized as the most harmful weather hazard for agriculture. One way to fight it back is using a wind machine - a 6-m diameter blowing fan atop a 10-m mast. It rotates on itself in approximately 4min30s and blows a slightly positive air using the strength of the nocturnal thermal inversion to mix cold air near the ground with warmer air above. Previous studies have focused on the protection area of the wind machine under different weather conditions or propeller designs. However, while weather conditions are undergone and field measurements are sparse, effects like the topography, the synergy between devices, or the addition of a burner are hard to catch and separate and are, therefore, not yet well understood.

In this study, we present field measurements dedicated to the future calibration of a computational fluid dynamics model (PALM) involving an actuator disk to simulate a wind machine operating during radiative frost conditions. This numerical model will aim to understand better such tower's external effects, for which field measurements are challenging to implement.

To characterize the jet of the propeller at the onset, vertical profiles were measured with a 3D sonic anemometer at high frequency (100Hz) 10 m away from the wind machine every meter between 3 and 15 m heights. Mass flow and momentum rates of about 500m3/s and 5000N were deduced for some different designs of wind machines.

To characterize how the jet interacts with the ground regarding the distance from its source, 2D sonic anemometers were placed in a row in front of the wind machine. Results highlight three different zones where the jet behaved distinctively:

  • A dead zone, where the jet passed over the ground (0 to 30 m away from the WM);
  • An impact zone where the jet directly hit the ground with maximum velocity (40 to 60m away from the WM);
  • A spreading zone where the protection mixing was due to eddies spreading in the inter-rows and breaking into smaller eddies in contact with posts and vine plants (70m away from the WM and beyond). As the distance from the machine increased, the jet velocity decreased before vanishing.

From these results about the onset condition and development of the jet, it will be possible to tune the rotating actuator disk to reproduce with PALM (an LES meteorological-oriented modeling system) an acceptable behavior of the flows (gust and weather interacting with the ground) despite several simplifications of the underlying physics.

While calibrations are still ongoing, the first results are encouraging, whether it be on a wind machine in a free environment or with the reproduction of a radiative night situation. The primary analysis will focus on the animation of state variables to assist in analyzing statistical results on field measurements. As little knowledge is available about the combined use of a burner with a wind machine, several strategies for a burner location will be tested in order to initiate a research topic that the authors believe is currently unexplored.

How to cite: Le Cap, C., Carlier, J., Katurji, M., Lin, D., Quénol, H., Georgeault, P., Buisson, E., and Heitz, D.: Towards numerical simulation of a wind machine during spring frost calibrated with field measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1425, https://doi.org/10.5194/egusphere-egu23-1425, 2023.

A series of discrepancies between field observations and the traditional thermal energy balance derived from the 1st law of thermodynamics are investigated. Intrigued by some historically known puzzles such as surface energy imbalance, failed potential temperature conservation, and dissimilarity between temperature and humidity, the investigation focuses on physical processes in the atmospheric boundary layer that are uniquely controlled by the diurnal variation of surface heating/cooling. Examination of temperature changes is extended to air-temperature-related variables such as turbulent heat fluxes and temperature variances. Inconsistency between field observations and the traditional thermal energy balance is found not only in their magnitudes but also in their diurnal cycles. Inability of the traditional thermal energy equation for explaining all the observations that are distinctively related to air temperature changes challenges validity of the traditional thermal energy balance theory. 

 

 

The research is supported by NSF AGS-2203248.

How to cite: Sun, J.: Discrepancies between Boundary-layer Observations and the Traditional Thermal Energy Balance, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1681, https://doi.org/10.5194/egusphere-egu23-1681, 2023.

The center of Israel presents relatively simple vertical topographical cross-section: The eastern Mediterranean coast on the west, Judea and Samaria mountain in the center and the deep steep Jordan valley on the east.

To the best of our knowledge, the variability of the boundary layer height (BLH) over Israel during the non-summer period was not investigated. This work presents climatological examination of the daytime BLH variability during non-summer months according to WRF simulations with 3 km horizontal resolution during 5 years. The monthly average BLH above the mountain peak and its easterly slope is found to be lower than that over the coastal area (1-2.5 .vs. 2-3 km) during the winter months, November-February, while during the rest of the year (except March) the situation is reversed.

In order to track the mechanism responsible for the reduction of the BLH over the mountain peak area during winter, an examination of the BLH variability during 10-13 UTC was performed. Accordingly, events with relatively weak pressure gradients and weak (< 5 m/s) easterly flow were found to be responsible for minimal BLH (< 350 m). The synoptic pressure during these events is characterized by ridge from the south in the middle troposphere (500 hPa) and central Red Sea Trough or high to the east or to the north of Israel next to the surface. Fohn winds which locally reduce the humidity and enhance the temperature due to subsidence flow over the eastern slope of the valley and the western slope of the mountain. In such cases, the mild synoptic pressure gradients are responsible for the maintenance of the local cooling over the mountain peak. The advection of hot air to the mountain peak is limited and therefore relatively stable thermal stability is obtained over the mountain peak and its eastern slope.

How to cite: Berkovic, S.: Theoretical examination of non-summer daytime boundary layer height variability over coastal-mountain-valley topography: the case of central Israel, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2014, https://doi.org/10.5194/egusphere-egu23-2014, 2023.

EGU23-3500 | ECS | Posters on site | AS2.1

Can we measure evaporation using commercial microwave links? 

Luuk van der Valk, Oscar Hartogensis, Miriam Coenders-Gerrits, Rolf Hut, Bas Walraven, and Remko Uijlenhoet

The aim of this study is to investigate whether it is feasible to obtain evaporation estimates from commercial microwave links, which are normally used for telecommunication. These commercial microwave links are already used to monitor path-averaged precipitation by determining the rain-induced attenuation along the link path. The signal transmitted by these microwave links is also perturbed by turbulence during dry periods, which consists of diffraction of the emitted beam by turbulent eddies. This is known as the scintillation effect and special microwave links, called scintillometers, have been designed to measure the full spectral range of the signal intensity fluctuations caused by the scintillation effect and link these fluctuations to the turbulent heat fluxes. However, commercial microwave links are usually sampled at too low temporal resolution to directly capture all the relevant scintillation fluctuations (typically between 0.1 – 100 s). Currently, the links are most often sampled at a temporal resolution of 15 minutes with a recording of the minimum and maximum values, while more recently also “active” forms of sampling with possible intervals up to 1 s have been set up. We intend to investigate what kind of sampling is required to obtain the structure parameter of the refractive index, Cnn, from commercial microwave link data. We will use high resolution sampling rates, which we resample to mimic various commercial sampling strategies. Subsequently, we aim to compute evaporation through deriving the structure parameters for temperature, Ctt, and humidity, Cqq, through a combination with auxiliary data. For this research, we will use data from a dual-beam scintillometer setup, a RPG-MWSC 160 GHz and a Large-Aperture Scintillometer with a 15 cm diameter over a 850 m path over the Ruisdael Observatory at Cabauw, the Netherlands. Additionally, we will install a Nokia Flexihopper 38 GHz, formerly part of a telecom network in the Netherlands, serving as our commercial microwave link. On the measurement site, many other relevant meteorological measurements for studying evaporation (e.g. temperature, humidity, turbulence and energy fluxes) are performed, which we will use as auxiliary and reference data. During this poster session, we would like to present our research plans and invite fellow session participants to join the discussion and give feedback on our ideas.

How to cite: van der Valk, L., Hartogensis, O., Coenders-Gerrits, M., Hut, R., Walraven, B., and Uijlenhoet, R.: Can we measure evaporation using commercial microwave links?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3500, https://doi.org/10.5194/egusphere-egu23-3500, 2023.

EGU23-4115 | ECS | Posters virtual | AS2.1

Atmospheric Turbulent Characteristics under Summer Shamal in Coastal Qatar 

Yuan Li and Reza Sadr

Summer Shamal, a strong low-level northwesterly wind in the Middle Eastern region, is the major trigger for dust storm activity with a broad impact on regional transport and human safety. Due to the scarcity of high-frequency data, near-ground turbulent mixing analyses under Shamal are still rare. The current study investigates the near-surface turbulence characteristics of the atmospheric boundary layer (ABL) in the coastal region of Qatar under summer Shamal conditions (26.08 N, 51.36 E). The results show that, in the absence of monsoon, Shamal prevents the development of summer sea breezes in the Persian Gulf. Compared to non-Shamal days (NSD), Shamal days (SD) are characterized by higher sensible heat flux magnitude and turbulent kinetic energy (TKE) with lower humidity, especially around noon time. Turbulence stability analysis indicates the probability of different dust activities during summer SD and NSD. Wind velocity spectra are investigated to evaluate the TKE dissipation rate. A Weibull distribution is observed for PDFs of TKE dissipation rate under SD for both stable and unstable conditions.

How to cite: Li, Y. and Sadr, R.: Atmospheric Turbulent Characteristics under Summer Shamal in Coastal Qatar, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4115, https://doi.org/10.5194/egusphere-egu23-4115, 2023.

The atmospheric stability condition in the coastal region of Qatar are analyzed using the measurements conducted on the shoreline (26.08N, 51.36E). The micrometeorological data are collected, from August 2015 to September 2016, using sonic anemometers (20 Hz) at three heights and a weather station on the top of a 9 m tower. Two different atmospheric daily stability patterns, ‘orderly’ and ‘disheveled’, are identified based on the wind conditions. A day is classified as ‘orderly’ if the amount of wind from the sea lasts less than 10% of the day. Otherwise, a day with an onshore wind of more than 10% is considered ‘disheveled’. The orderly stability pattern shows a daily descending and ascending trend during the sunrise and sunset periods, respectively, while the disheveled days follow a random pattern with no clear order. The probability distribution of the stability parameter shows a narrower distribution for the ‘orderly’ days, containing fewer unstable periods than the ‘disheveled’ days. The chaotic trend during disheveled days could be caused by the inhomogeneity of the roughness between the land and the sea (1000 times). The integral length scales are further investigated to clarify the influence of the local thermally forced flow to the disheveled patterns.

How to cite: Sadr, R. and Li, Y.: Two daily stability patterns in the atmospheric surface layer of the coast of Qatar, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4130, https://doi.org/10.5194/egusphere-egu23-4130, 2023.

EGU23-5566 | Posters on site | AS2.1

Scalar turbulent flux observations in the entrainment layer and assessment of current parametrizations 

Fabien Gibert, Dimitri Edouart, Paul Monnier, Julie Collignan, Julio Lopez, and Claire Cénac

The entrainment zone (EZ) capping the convective boundary layer (CBL) is documented using lidar turbulent-scale observations. Sensible and latent heat fluxes have been measured during one hundred hours in CBL temperate and arid regions in free-cloud meteorological conditions. The EZ fluxes have been confronted with scalar gradients, integral scales of turbulence, wind shear, and surface sensible heat flux.  In agreement with former observations in stratified surface layer or with EZ large eddy-simulation (LES) studies, Lidar observations show that the buoyant oscillation period associated to the vertical velocity variance are found to be universal relevant parameters for EZ scalar fluxes and gradients. Attempts to introduce non-local CBL scales like the turbulent vertical velocity scale and height, the scalar interfacial layer jumps and the surface sensible heat flux globally increases the scatter of the data. Non-local parametrization particularly failed for EZ latent heat flux compared to sensible heat flux and for weak surface heat flux as it is usually the case in temperate region. Investigating a possible non-local parametrization of EZ vertical velocity variance, it was found that EZ wind shear and then EZ gradient Richardson number play a negligible role. Rather, observations often showed an excess of EZ vertical velocity variance with respect to CBL similarity law that may be explained by a significant contribution of wave-turbulence interaction in the entrainment layer.

How to cite: Gibert, F., Edouart, D., Monnier, P., Collignan, J., Lopez, J., and Cénac, C.: Scalar turbulent flux observations in the entrainment layer and assessment of current parametrizations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5566, https://doi.org/10.5194/egusphere-egu23-5566, 2023.

EGU23-5664 | ECS | Posters on site | AS2.1

Influence of the extraordinary Filomena snowstorm on the surface energy balance and its relationship with the subsequent very-low surface temperatures 

Pablo Fernández-Castillo, Carlos Román-Cascón, and Carlos Yagüe

Filomena snowstorm impacted a large part of the Iberian Peninsula during January 2021, especially affecting the central part of Spain, and covering the Madrid region with up to 50 cm of snow.

In this work, we analyse data from a micrometeorological station (GuMNet-Herrería) placed in a rural environment in the northwest of the Community of Madrid. The objective is to determine the influence of the microscale on the extremely low temperatures reached after Filomena's passage, as well as to better understand the physical processes associated with these extreme conditions.

Although the snowfall lasted only for 2 days, the snow was present on the surface for more than 10 days, already with stable synoptic conditions, accompanied by a weak turbulent transfer between the surface and the lower part of the atmospheric boundary layer. These days after, extremely low temperatures were recorded, reaching minima of up to -26.5 ºC in the central part of the Iberian Peninsula. The presence of snow on the surface modified significantly the components of the surface energy balance (SEB). This included a reduction in the available net radiation at the surface as result of increased albedo and emissivity of the surface, compared to standard conditions (previous period to Filomena), as well as in the turbulent fluxes, contributing to some records of minimum temperatures. The persistence of the snow cover also affected the soil temperatures, keeping the ground heat flux practically constant.

How to cite: Fernández-Castillo, P., Román-Cascón, C., and Yagüe, C.: Influence of the extraordinary Filomena snowstorm on the surface energy balance and its relationship with the subsequent very-low surface temperatures, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5664, https://doi.org/10.5194/egusphere-egu23-5664, 2023.

EGU23-6095 | ECS | Posters on site | AS2.1

Dynamics and scaling of moist, internally cooled convection 

Lokahith Agasthya and Caroline Jane Muller

Idealised models of convection such as Rayleigh-Bénard convection, horizontal convection etc. have been widely used to study the behaviour of natural fluid systems including but not limited to the atmosphere, the oceans and the flow of lava in the earth's core in a simplified setting 1,2. While such idealised models include only a small subset of the physical processes occurring in nature, their simplified dynamics allows for easier interpretation and study of the interactions of individual physical processes. 

In this numerical study, we consider the case of an idealised moist convecting thermal system, with various Dirichlet and Neumann boundary conditions for the temperature and water vapour mixing ratio. The model includes a vertical temperature lapse-rate, the release of latent heat due to the condensation of water vapour and a constant bulk-cooling term to simulate moist convection accompanied by radiative cooling in the earth's atmosphere. This study follows previous studies which have used similar idealised scenarios to understand dry 3 as well as as moist 4 atmospheric convection. 

The model is studied for its dynamical response and scaling for varying boundary conditions and input parameters such as the strength of the radiative cooling, the steepness of the lapse rate and the latent heat of condensation to better understand the interaction between moist convection and radiative cooling in the atmosphere. We also compare the convective organisation in our simplified model with more complex cloud-resolving atmospheric simulations 5

References:

1. G. Ahlers, S. Grossmann, and D. Lohse, “Heat transfer and large scale dynamics in turbulent Rayleigh-Bénard convection,” Reviews of modern physics, vol. 81, no. 2, p. 503, 2009.

2. G. O. Hughes and R. W. Griffiths, “Horizontal convection,” Annu. Rev. Fluid Mech., vol. 40, pp. 185–208, 2008.

3. M. Berlengiero, K. Emanuel, J. Von Hardenberg, A. Provenzale, and E. Spiegel, “Internally cooled convection: a fillip for philip,” Communications in Nonlinear Science and Numerical Simulation, vol. 17, no. 5, pp. 1998–2007, 2012

4. G. K. Vallis, D. J. Parker, and S. M. Tobias, “A simple system for moist convection: the rainy–bénard model,” Journal of Fluid Mechanics, vol. 862, pp. 162–199, 2019

5. C. J. Muller and I. M. Held, “Detailed investigation of the self-aggregation of convection in cloud-resolving simulations,” Journal of the Atmospheric Sciences, vol. 69, no. 8, pp. 2551– 2565, 2012.

Acknowledgement - This project has received funding from the European Union's Horizon 2020 research and innovation programme under the Marie Sklodowska-Curie grant agreement No. 101034413.

How to cite: Agasthya, L. and Muller, C. J.: Dynamics and scaling of moist, internally cooled convection, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6095, https://doi.org/10.5194/egusphere-egu23-6095, 2023.

EGU23-6371 | ECS | Posters on site | AS2.1

Influence of gross primary production in energy partitioning in three different forest ecosystems based on Eddy Covariance time series analysis 

Victor Cicuéndez, Javier Litago, Victor Sánchez-Girón, Carlos Román-Cascón, Laura Recuero, César Saénz, Carlos Yagüe, and Alicia Palacios-Orueta

Ecosystems plays a key role on the interaction between the land surface and the atmospheric processes being responsible for strong feedback processes that affect the climate by modifying the relative contribution of the latent and sensible heat to the total energy of the atmospheric air, i.e., the energy partitioning processes. The mechanisms and consequences of this feedback are uncertain and must be studied to evaluate their influence on global climate change.

In this study, our overall objective was to assess the Gross Primary Production (GPP) dynamics and the energy partitioning patterns in three different European forest ecosystems through time series analysis of eddy covariance data. The three contrasted forest types in terms of functioning and climate were an Evergreen Needleleaf Forest in Finland (ENF_FI), a Deciduous Broadleaf Forest in Denmark (DBF_DK), and a Mediterranean Savanna Forest in Spain (SAV_SP). In each site there was and eddy covariance flux tower from which meteorological data, carbon and energy fluxes were analyzed. Firstly, a univariable time series analysis of all variables was made by means of the Buys-Ballot tables, i.e., average year, to study the intra-annual dynamics and then, through the use of the autocorrelation function the interannual dynamics were assessed.  Finally, causality of GPP and energy fluxes was studied with Granger causality tests.

Results show that temperature and solar radiation were the main limiting factors in the Northern ecosystems while water availability was determinant for growth in the Mediterranean ecosystem. The autocorrelation function showed that GPP and the meteorological variables in the SAV_SP were more irregular and show lower memory at the long term than at the short one. In addition, this ecosystem presented higher radiation and a larger amount of H+LE, showing the highest Bowen ratio and a lower primary production efficiency in terms of total energy (GPP/(H+LE)). On the contrary, both northern ecosystems showed similar production efficiencies in terms of total energy. However, the DBF_DK showed lower Bowen ratio related to a larger amount of latent heat in relation to sensible heat in associated to the larger plant activity in this forest. Finally, the Granger causality tests showed that the vegetation feedback to the atmosphere was more noticeable in the ENF_FI and the DBF_DK at the short term, influencing latent and sensible heat fluxes.

In conclusion, the impact of the vegetation on the atmosphere influences the energy partitioning in a different way depending on the vegetation type, which makes essential the study of the vegetation dynamics at the local scale to parameterize with more detail these processes and build improved global models.

How to cite: Cicuéndez, V., Litago, J., Sánchez-Girón, V., Román-Cascón, C., Recuero, L., Saénz, C., Yagüe, C., and Palacios-Orueta, A.: Influence of gross primary production in energy partitioning in three different forest ecosystems based on Eddy Covariance time series analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6371, https://doi.org/10.5194/egusphere-egu23-6371, 2023.

Surface-layer stability is important in many processes, such as the surface energy budget, atmospheric pollution, and boundary-layer parametrization. Most previous studies on stability, however, conducted either theoretical or observational investigations at specific sites, thus leaving a gap with regard to the large-scale pattern. Here, wind speed and temperature observations at multiple heights from the wind-tower network of China are used to estimate the stability during the 2009–2016 period. A series of data-quality-control procedures are conducted and data from 170 wind towers with more than 2 years’ worth of valid observations are selected. The degree of stability is classified by the Obukhov length, which is derived from the wind speed and temperature at 10 m and 70 m above ground level, combined with information regarding the roughness length. Overall, the occurrence frequency of surface-layer instability exhibits significant temporal and spatial variability, being particularly larger in spring and summer than in autumn and winter. The maximum frequency of summertime instability occurs in the time period 1000–1200 local solar time, approximately 2 h earlier than in autumn. Geographically, the peak instability frequency occurs much earlier in the day in north-west China than in other regions, likely owing to the arid and semi-arid land cover. Also noteworthy is the steady increase in instability frequency observed during the period analyzed here, likely resulting from the reduction in the vertical gradient of wind speed. Our findings call for explicit consideration of stability variability in the wind-energy industry and in fundamental boundary-layer investigations in China.

How to cite: Li, J.: Assessing the Surface-Layer Stability over China Using Long-Term Wind-TowerNetwork Observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6812, https://doi.org/10.5194/egusphere-egu23-6812, 2023.

EGU23-7255 | ECS | Orals | AS2.1

Modelling momentum transport in climate simulations of boundary-layer winds with a higher order parameterization scheme 

Emanuele Silvio Gentile, Ming Zhao, Vince Larson, and Colin Zarzycki

Accurate modelling of sub-grid momentum flux is crucial for reliable climate simulations of the boundary-layer wind. While first-order momentum flux parametrizations often employed in leading climate models are crude, consisting in a downgradient diffusion scheme with a separate cumulus momentum transport scheme, higher-order turbulence parametrizations which directly prognose the momentum flux are more flexible and general, adhering more closely to the governing equations.

Here, we present the results of studying the sensitivity of the AM4-GFDL global climate simulations of the boundary-layer wind to a first-order, diagnostic, and a higher-order, prognostic, sub-grid momentum flux parametrization. Moreover, we demonstrate how the boundary-layer wind turning angle can be effectively used as a metric to evaluate the impact of changing the sub-grid momentum flux parametrization on the boundary-layer wind structure. 

How to cite: Gentile, E. S., Zhao, M., Larson, V., and Zarzycki, C.: Modelling momentum transport in climate simulations of boundary-layer winds with a higher order parameterization scheme, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7255, https://doi.org/10.5194/egusphere-egu23-7255, 2023.

The horizontal resolution of numerical weather prediction models (NWP) keeps decreasing towards the hectometric range. However, although topography, land-use, and other static parameters might be better resolved, the performance of physical parameterizations also has to be evaluated and assessed.
One of the most challenging environments for modern NWP models is mountainous topography - namely because, among other issues, turbulence parameterizations were developed for horizontally homogeneous and flat terrain. This assumption is clearly violated in complex terrain, leading to the underestimation of the turbulence kinetic energy and an unrealistic representation of the mountain boundary layer.
In this study, we perform limited-area simulations with the state-of-the-art NWP model ICON (Icosahedral Nonhydrostatic Model) across resolutions (1km, 500m, 250m, 125m) in the Inn Valley, Austria for a day where boundary-layer processes dominate. A thermally-induced valley wind circulation forms on this day, typical for wide valleys. The model is evaluated with observations from the CROSSINN measurement campaign, providing besides the usual meteorological parameters also measurements from LIDAR systems, radiosondes, turbulence eddy-covariance towers, and scintillometers. This data pool of observations allows us to evaluate the current turbulence parameterizations of ICON, starting with the (pre-)operational NWP resolution (1km) across the turbulence grey zone towards large-eddy simulation resolutions (125m). Both the one-dimensional (1D, Mellor-Yamamda type) and the three-dimensional (3D, Smagorinsky closure) turbulence schemes of the model compared with the observations across the grid resolutions to identify the resolution at which the 3D scheme starts to add value over the 1D scheme. Finally, we can check whether further improvements in the turbulence schemes are necessary for the turbulence grey zone.

How to cite: Goger, B. and Dipankar, A.: Evaluating the Turbulence Representation in a Numerical Weather Prediction Model over Mountainous Terrain, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7270, https://doi.org/10.5194/egusphere-egu23-7270, 2023.

EGU23-7640 | ECS | Posters on site | AS2.1

Contribution of wavelets to decrease gap filling in turbulent surface fluxes measurements 

Pedro Henrique Herig Coimbra, Benjamin Loubet, Olivier Laurent, Pauline Buysse, Jérémie Depuydt, Daniel Berveiller, Nicolas Delpierre, and Matthias Mauder

There is an urgent need to provide data for greenhouse gases (GHG) monitoring. Flux towers currently represent the most direct approach to provide continuous datasets of surface exchange of these gases. Typically, the flux is derived from the EC method over 30 minutes averaging periods. However, technical and meteorological conditions create gaps with missing or non-reliable data which can represent from 20 % to 60 % of the total period. To compute annual GHG balances, one needs to fill these gaps. Studies on benchmark forest datasets show that gap-filling methods, such as the marginal distribution sampling (MDS), have a good performance on hourly and daily data as well as on annual budgets. This overall setup (EC and MDS gap-filling) is the standard for consolidated datasets over FLUXNET and most flux networks (e.g. Warm Winter 2020 available at www.icos-cp.eu/).

Direct observations are the base of the gap-filling itself and should be praised over gap-filling techniques. More so, the flux community nowadays faces new challenges by moving towards less ideal sites (e.g. European PAUL-ICOS-Cities project to monitor city GHG fluxes), and facing increasing extremes conditions (e.g. Drought-2018, available at www.icos-cp.eu/). In these less conventional frameworks, gap-filling techniques need to be evaluated. Among flux processing techniques, wavelets (WV) can reliably measure non-stationary periods and thus retain more data than standard EC. It does that by resolving flux calculation at sampling rate. For flux measurements it has been most notably used for airborne measurement as it allows computing a flux over short enough periods to attribute the measured flux to a limiter land area.

Here we analyse the CO2 flux over the three consecutive years (2019, 2020 and 2021) in two ICOS sites: FR-Gri, a crop site and FR-Fon a mixed deciduous forest site, both near Paris, France. Results show that from 52 606 data points in FR-Fon, around 50% needed to be gap filled, this includes 11% of missing data and 22% of periods with developed turbulence but non-stationary. Preliminary results for 2019 in FR-Gri show similar ranges. By not requiring stationarity, WV method avoid close to half of the gap filling compared to EC. Comparing 30-minutes-averaged fluxes derived from EC and WV shows good correlation (R²=0.99 for observed data and 0.94 for gap filled data), low root mean square error (RMSE=1.12  for observed data and 1.95 for gap filling). The extra data also decreased continuous gaps, which is expected to improve the performance of gap filling methods. More so, during summer 2019 heatwaves stroke Europe and in particularly French ecosystems. On the flux data, daytime observations during elevated temperatures in 2019 show a WV derived CO2 fluxes closer to zero, suggesting the expected response of stomatal closure during these events. The gap-filled EC data, however, showed relatively unchanged photosynthesis. This study shows the usefulness of using WV computed CO2 fluxes, a result expected to remain valid for longer time series and for other ecosystems and meteorological conditions.

How to cite: Herig Coimbra, P. H., Loubet, B., Laurent, O., Buysse, P., Depuydt, J., Berveiller, D., Delpierre, N., and Mauder, M.: Contribution of wavelets to decrease gap filling in turbulent surface fluxes measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7640, https://doi.org/10.5194/egusphere-egu23-7640, 2023.

EGU23-7929 | ECS | Posters on site | AS2.1

Attenuation of mountain-valley winds on wintertime PM2.5 change over the western Sichuan Basin, Southwest China 

Yuqing Zhang, Tianliang Zhao, Zhuozhi Shu, Yan Zhu, Weikang Fu, and Dingyuan Liang

The Sichuan Basin (SCB) with complex mountain-basin topography, located immediately to the east of the Tibetan Plateau (TP) in southwest China, is identified as a region with severe PM2.5 pollution over China. To comprehensively understand the SCB terrain effect on the atmospheric environment change, we investigated the effect degree and meteorological mechanism of mountain-valley winds on wintertime PM2.5 in the western SCB, thermally driven mountain-valley winds between the mountains of eastern TP and the western edge of SCB based on near-surface observations of PM2.5 and the ERA5 reanalysis data of meteorology. The results show that the western SCB exhibits a significant diurnal change of mountain-valley winds, shifting between daytime easterly flows and nighttime westerly flows over the western edge of SCB. The frequency of the mountain-valley winds was accounted for 39% of the study’s duration, with the valley and mountain wind-controlling periods being from 2:00 pm to 5:00 pm and 01:00 am to 05:00 am in local time, respectively, and the remaining time being the transition period. Notably, a reduction of 4.5~20.7μg m-3 in near-surface PM2.5 concentrations averaged over the western edge of SCB, decreasing 6~74% in the PM2.5 pollution during the days of mountain-valley winds, which indicates that the mountain-valley winds could alleviate wintertime near-surface PM2.5 in improving air quality over the western SCB. The easterly wind speed was uplifted by 18% during the valley wind-controlling period, corresponding to a 22% reduction in the near-surface PM2.5 levels driven by the mountain-valley winds. The westerly wind speed increased by 50% at the mountain wind-controlling period with a 20% reduction in PM2.5, reflecting the attenuating effect of the favorable atmospheric diffusion conditions on PM2.5 pollution over the western SCB. The daytime noticeably enhanced easterly wind and the strong updraft flows over the eastern slope of TP promoted the dilution and diffusion of air pollutants over the western edge of SCB, and the nocturnal downhill flows along the slope in the westerly winds on the western edge of SCB brought clean TP air to the polluted SCB region in southwest China.

How to cite: Zhang, Y., Zhao, T., Shu, Z., Zhu, Y., Fu, W., and Liang, D.: Attenuation of mountain-valley winds on wintertime PM2.5 change over the western Sichuan Basin, Southwest China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7929, https://doi.org/10.5194/egusphere-egu23-7929, 2023.

EGU23-8231 | Orals | AS2.1

Law-of-the wall adjustments above the Amazon Forest via Cospectral Budget Model 

Luca Mortarini, Gabriel Katul, Daniela Cava, Cleo Quaresma Dias-Junior, and Marcelo Chamecki

Measurements collected at two experimental sites, the Amazon Tall Tower Observatory (ATTO) and the tower at the Cuieiras Biological Reserve (ZF2) that was part of the GoAmazon experiment, were considered to study deviations from the law-of-the wall for the roughness sublayer (RSL) above the Amazon Forest. A plethora of physical, chemical, and biological processes are influenced by the flow structure in the RSL. Further, above tall and dense canopies the handshake between the land and the atmosphere in numerical Weather Predictions and Earth Systems Models occurs in the RSL. For the mean velocity, the RSL effects are operationally accommodated using a dimensionless roughness sublayer correction function (φ) to the law-of-the wall. For dense canopies the mixing-layer analogy is assumed, and the correction function φ depends on the vorticity thickness, Ls. φ measures the ratio of the eddy viscosity from attached eddies to a zero-plane displacement (d) and the actual eddy viscosity in the RSL at (z-d), for (z-d)/Ls>>1, φ∼1. However, this formulation remains only plausible for dense forested canopies and its extension to sparse and urban canopies difficult at the least. In the Amazon the experimental determination and modeling of φ may also be challenging for the forest topography that introduce z-dependent mean pressure gradients that then lead to variability in second-order flow velocity statistics with z.  In this work an original formulation of φ is proposed based on a scale-wise co-spectral budget model that balances mechanical production to pressure-decorrelation terms in the co-spectral budget. Because the turbulent kinetic energy dissipation rate (ε) is conserved across the vertical velocity spectrum, the co-spectral budget model reveals a novel link between φ and a macro-scale dissipation length, Ld=u*3/ε.The friction velocity, u*, is interpreted from the moving-equilibrium hypothesis to be appropriately defined at the canopy top. The analysis shows that the estimation of φ with the new formulation agrees with independent estimates of φ using measured turbulent momentum flux and mean velocity gradient. Further, Ld emerges as a key length scale in the RSL, being more efficient than the vorticity thickness in the estimation of the peaks of the wind vertical velocity spectra.

How to cite: Mortarini, L., Katul, G., Cava, D., Quaresma Dias-Junior, C., and Chamecki, M.: Law-of-the wall adjustments above the Amazon Forest via Cospectral Budget Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8231, https://doi.org/10.5194/egusphere-egu23-8231, 2023.

EGU23-8468 | ECS | Orals | AS2.1

Vertical momentum in the boundary layer and its consequences for transport of greenhouse gases 

Jesús Abril-Gago and Andrew S. Kowalski

Like mass and energy, momentum is an extensive quantity and so the momentum of a system is equal to the sum of the momenta of its components. Considering boundary-layer air in the surface-normal ("vertical") direction, its components have momentum in different directions. That of carbon dioxide is downward due to photosynthetic uptake by ecosystems, while those of oxygen and water vapor are upward due to photosynthetic and evaporative sources, respectively. And so on. Importantly, evaporation is several orders of magnitude greater than any other form of surface exchange, and therefore the vertical momentum of air can be precisely approximated by that of water vapor. This allows estimation of the vertical velocity as simply the ratio of the evaporative flux density to the air density, and has important consequences for many aspects of boundary-layer meteorology.

We analyzed atmospheric data from numerous flux towers over a range of climatological and ecological contexts to characterize the vertical velocity and consequent magnitudes of non-diffusive greenhouse gas transport. Our results invalidate long-standing and intuitive attribution of diffusion of some greenhouse gas directly to its sources and sinks, which has neglected the key role of water vapor in diluting the components of dry air.

This work was supported by the project PID2020-117825GB-C21 and PID2020-117825GB-C22 (INTEGRATYON3) funded by MCIN/AEI/10.13039/501100011033, and by projects BRNM-60-UGR20 (OLEAGEIs) and P18-RT-3629 (ICAERSA) including European Union ERDF funds.

How to cite: Abril-Gago, J. and Kowalski, A. S.: Vertical momentum in the boundary layer and its consequences for transport of greenhouse gases, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8468, https://doi.org/10.5194/egusphere-egu23-8468, 2023.

Identifying turbulence regimes in the stable boundary layer (SBL) is not only important for advancing our fundamental understanding of turbulent mixing but is also needed for model-observation intercomparisons and to build meaningful Earth system science models for predicting future climate change in regions subject to weak winds and significant radiative cooling. As a common regime classification, the classic hockey stick curve (Sun et al., 2012) relates the turbulence kinetic energy to the mean horizontal wind speed and differentiates between (1) weak turbulence driven by local shear and (2) strong turbulence driven by the bulk shear separated by a height-dependent threshold. A third (3) intermittent regime marks transitions between the former. However, the effect of thermal stratification on the surface heat fluxes is not directly included in this metric. Here, we explore the recently proposed decoupling metric Ω = LB (z√2)-1  (Peltola et al., 2021) to overcome this limitation as the buoyancy length scale LB ∝ NBV-1 directly incorporates the stratification through the bulk Brunt-Vaisala frequency. Analyzing multi-level observations in persistent polar SBLs, short-lived SBLs over snow and topographically sheltered nocturnal SBLs we found that Ω versus wind speed exhibits an even more clearly pronounced hockey stick behavior with a sudden regime change from (1) to (2), but without the intermittent (3). In contrast to the classic hockey stick metrics, heat fluxes were largest for an intermediate Ω within the strong regime (2) but above the critical threshold velocity. In the SBL, heat fluxes vanished for either very small stratification and, hence, weak gradients, leading to large Ω > 1 in (2), or in (1) as vertical transport is suppressed by the strong stratification. The observations satisfied a simple linear model to predict the threshold Ωcrit from height-dependent wind speed. The latter resembled a classic neutral boundary layer profile with meaningful friction velocities and surface roughness length, suggesting that turbulent transport is coupled to the local surface throughout regime (2). The height-dependence of Ωcrit,however, suggests that z is not the most appropriate vertical length scale in the SBL even for the strong turbulence regime.

References:

Peltola, O., Lapo, K., & Thomas, C. K. (2021). A Physics-Based Universal Indicator for Vertical Decoupling and Mixing Across Canopies Architectures and Dynamic Stabilities. Geophysical Research Letters, 48(5), e2020GL091615. https://doi.org/https://doi.org/10.1029/2020GL091615;

Sun, J., Mahrt, L., Banta, R. M., & Pichugina, Y. L. (2012). Turbulence Regimes and Turbulence Intermittency in the Stable Boundary Layer during CASES-99. Journal of the Atmospheric Sciences, 69(1), 338–351. https://doi.org/10.1175/JAS-D-11-082.1

How to cite: Thomas, C. and Huss, J.-M.: Revisiting the hockey stick curve: exploring an alternative metric for incorporating the role of stratification in distinguishing turbulence regimes in the stable boundary layer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8626, https://doi.org/10.5194/egusphere-egu23-8626, 2023.

EGU23-8816 | ECS | Orals | AS2.1

Midday Boundary-Layer collapse in the Altiplano Desert: the combined effect of Advection and Subsidence 

Francisca Aguirre Correa, Jordi Vilà-Guerau de Arellano, Reinder Ronda, Felipe Lobos Roco, Francisco Suárez, and Oscar Hartogensis

Observations in the Altiplano region of the Atacama Desert show that the atmospheric boundary layer (ABL) suddenly collapses at noon. This behavior departs from the typical convective ABL normally reproduced by weather and climate models. The collapse occurs simultaneously to the entrance of a thermally driven and topographically enhanced regional flow, characterized by strong winds that produce mechanical turbulence and advect cold air. To identify the main drivers that cause such ABL collapse and the impact on the potential temperature diurnal variability, we use a land-atmosphere coupled model, observations from a comprehensive field campaign, and the Weather and Research Forecasting regional model. We also address the question of how local (surface-atmosphere interactions) and non-local processes (entrainment/ advection/ subsidence) contribute to the surface and ABL dynamics in the region.

A suite of numerical experiments were performed to disentangle the boundary-layer collapse by increasing the level of complexity: from only considering local land-atmosphere interactions to systematically including the non-local contributions of mass advection, cold air advection, and subsidence. Our results show that during the morning the local surface-atmosphere interactions are the dominant contributions and lead to increase the heat exchange that, together with the entrainment processes, warm the atmosphere and allow the ABL to grow. However, this regime abruptly changes at noon and turns into a boundary-layer regime mainly controlled by non-local phenomena. Two interconnected processes lead to a strong decrease of the ABL height (h ): the advection of a shallower boundary layer (~ -250 m h−1 at noon) that causes an immediate decrease of h at midday, and the arrival of a cold air mass which reaches a strength of ~ -3 K h−1 at 1400 LT, strong enough to stop the ABL growth by counteracting the large turbulence levels driven by the high surface fluxes. These two external forcings become dominant over entrainment and surface processes that warm the atmosphere and increase h. As a consequence, the ABL growth is capped during the afternoon. Finally, a wind divergence of ~ 8 x 10−5 s−1 contributes to the collapse by causing subsidence motions that provide additional downward push over the ABL from 1200 LT onward. Without these non-local processes, the ABL would be continuously growing to 3.5 km by the end of the afternoon. Our findings show the relevance of treating large and small processes as a continuum to be able to understand the ABL dynamics and reproduce them adequately in weather and climate models.

How to cite: Aguirre Correa, F., Vilà-Guerau de Arellano, J., Ronda, R., Lobos Roco, F., Suárez, F., and Hartogensis, O.: Midday Boundary-Layer collapse in the Altiplano Desert: the combined effect of Advection and Subsidence, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8816, https://doi.org/10.5194/egusphere-egu23-8816, 2023.

EGU23-8867 | Orals | AS2.1

First results of applying the updated two-energies turbulence scheme over complex terrain 

Juerg Schmidli, Ivan Bastak Duran, Julian Quimbayo-Duarte, Mirjana Sakradzija, and Shweta Singh

The unified parameterization of turbulence and clouds in the atmospheric boundary layer is one of the challenges in current weather and climate models. The updated two-energy turbulence scheme is able to successfully model both stratocumulus cases and shallow convection without the need of an additional parameterization for non-local fluxes. The update includes the introduction of the entropy potential temperature to distinguish between a shallow convection and a stratocumulus regime. In addition, the two-energy scheme is coupled to a simplified assumed PDF method in order to achieve a more universal representation of the cloudy regimes. The updated turbulence scheme has been tuned based on several idealized cases and is now evaluated for several real cases in the ICON modeling framework. These cases include cloud streets over relatively flat terrain and stable boundary layers including fog over complex terrain. The performance of the updated scheme is comparable to or better than the operational setup, and can be thus used instead of the operational turbulence and shallow convection scheme in ICON.

How to cite: Schmidli, J., Bastak Duran, I., Quimbayo-Duarte, J., Sakradzija, M., and Singh, S.: First results of applying the updated two-energies turbulence scheme over complex terrain, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8867, https://doi.org/10.5194/egusphere-egu23-8867, 2023.

EGU23-9116 | ECS | Orals | AS2.1

Numerical simulation and analysis of transient Ekman boundary layers using a stochastic turbulence model 

Marten Klein, Mark Simon Schöps, Juan Alí Medina Méndez, and Heiko Schmidt

Atmospheric boundary layers (ABLs) govern the atmosphere–surface coupling and are therefore of fundamental relevance for Earth’s weather and climate system. Key challenges in modeling and simulation of ABLs arise from the emerging spatio-temporal variability that manifests itself by fluctuating transport processes and intermittency on multiple scales (e.g. [1,2]). Observed flow features are the result of interacting inertial, Coriolis, buoyancy, and viscous forces, acting on all relevant scales of the turbulent flow. Small-scale processes, even if nonuniversal in nature, are usually not resolved due to cost constraints but modeled based on justified physical or empirical relations with the resolved scales, neglecting expensive backscatter (e.g. [3]). This issue is addressed here by a stochastic forward model, the so-called one-dimensional turbulence (ODT) model [4], which allows to preserve small-scale information in a feasible manner. In the ABL, ODT autonomously evolves flow profiles for prescribed initial and boundary conditions. Turbulent advection is modeled by a stochastically sampled sequence of mapping events that punctuate the deterministic advancement of molecular-diffusive processes and Coriolis forces. The model aims to reproduce turbulent cascade phenomenology, resolved along a notional vertically oriented line-of-sight, respecting fundamental physical conservation principles. The dynamical complexity of the model arises from a physically based feedback of the evolving flow state on the stochastic sampling procedure.

In this study, ODT is utilized as standalone tool for the numerical simulation of fluctuating wind velocity and temperature profiles in temporally developing neutral and stably stratified ABLs [5]. Comparison with available reference data shows that the model is able to reasonably reproduce conventional low-order but also detailed flow statistics for fixed model parameters. The model exhibits scale-selective buoyancy damping, but is unable to completely capture the relaminarization under prescribed, but developing, very stable conditions. This can be attributed to the model’s resistance against leaving the fully developed turbulent state. Forthcoming research addresses fluctuations and intermittency effects. For the latter, an event-based clustering approach is presented that aims to identify turbulent cascade events across flow regimes, yielding new possibilities for the analysis and prediction of turbulent time series.

References

[1] L. Mahrt. Annu. Rev. Fluid Mech. 46:23–45, 2014.
[2] V. Boyko, and N. Vercauteren. Boundary-Layer Meteorol. 179:43–72, 2021.
[3] S. S. Zilitinkevich, T. Elperin, N. Kleeorin, I. Rogachevskii, and I. Esau. Boundary-Layer Meteorol. 146:341–373, 2013.
[4] A. R. Kerstein, and S. Wunsch. Boundary-Layer Meteorol. 118:325–356, 2006.
[5] M. Klein, and H. Schmidt. Adv. Sci. Res. 19:117–136, 2022.

How to cite: Klein, M., Schöps, M. S., Medina Méndez, J. A., and Schmidt, H.: Numerical simulation and analysis of transient Ekman boundary layers using a stochastic turbulence model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9116, https://doi.org/10.5194/egusphere-egu23-9116, 2023.

EGU23-9568 | ECS | Posters virtual | AS2.1

Patterns of PBL hight during 1989-2019 over Romania, Moldavia Region using ERA5 data and correlation with NAO index. 

Apetroaie Cosmina, Bostan Diana-Corina, Timofte Adrian, Miclăuș Ingrid-Mihaela, and Cazacu Marius-Mihai

The evolution of the Planetary Boundary Layer Height (PBLH) is a very important meteorological parameter because most of the population carries out their socio-economic activities inside this layer and because it has a significant impact on weather events and air quality. This parameter is influenced by energy and mass exchanges between the land surface and the atmosphere. In our study, hourly PBLH data were used over a period of 30 years (1989-2018), for the warm season (May, June, July, August and September). The data we used comes from the ECMWF (European Centre for Medium-Range Weather Forecasts) database, ERA5. By means of Open GrADS (The Grid Analysis and Display System), the PBLH deviations were graphically represented and interpreted. On the other hand, the NAO (The North Atlantic Oscillation) has influences over the climate variability and weather worldwide. It is well known that NAO exhibits considerable variability throughout a season and during a year, as well, and prolonged periods (for a few months) of both positive and negative phases of the pattern are ordinary. Both the PBLH variations and the NAO index can have an impact on the weather and climate conditions. In this study we will present the patterns of PBLH during 1989-2019 and correlations between the NAO index and the variability of the monthly summer PBLH in Moldavia Region, Romania.

How to cite: Cosmina, A., Diana-Corina, B., Adrian, T., Ingrid-Mihaela, M., and Marius-Mihai, C.: Patterns of PBL hight during 1989-2019 over Romania, Moldavia Region using ERA5 data and correlation with NAO index., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9568, https://doi.org/10.5194/egusphere-egu23-9568, 2023.

EGU23-10792 | Orals | AS2.1

A multi-approach to study and communicate on the effect of highway infrastructures on the dispersion of traffic-related air pollutants. 

Pierre Camps, Thierry Poidras, Patrick Nicol, Marc-Antoine Vittori, Sarah Letaïef, and Margaux Lefevre

In this work, we will present 4 different approaches to study and visualize the effects of motorway infrastructures such as precast noise barriers or vegetated flat-top earth berms on the dispersion of traffic-related pollutants. The micrometeorological characteristics that directly affect the dispersion of pollutants in the atmosphere were first computed with a pseudo-3-dimensional CFD model by means of the openFoam toolbox. The strengths of this model based on the Reynolds-Averaged Navier–Stokes (RANS) equations with K-ε first-order closure model is to consider the traffic-induced momentum and turbulence (Letaïef et al., 2020). A second approach was to directly visualize the microturbulence from a 1/100 scale model of the motorway cross-section in a wind tunnel. To this end, we refracted the beam of a laser light with a glass rod to observe eddies along a thin plane through a fog generated by a fog machine. Simple shots with a camera can reveal coherent patterns in the chaos. To complete these two models, we conducted two types of field measurements of fine particle concentrations on the studied motorway sector. Direct and indirect measurements were carried out with low-cost microsensors and with environmental magnetism tools applied on dust depositions on accumulating surfaces (Hofman et al., 2017), respectively.

These four approaches indicates similar results. A large recirculation wake region formed on the leeward side of the wall that brings back to the wall the pollutant generated by the traffic is evidenced. On the contrary, flat-top earth berms favor the dispersion of pollutants in the atmosphere. These 4 different approaches allowed us not only to establish these conclusions but also to communicate with all the actors concerned by this study site: scientists specialized in the metrology of atmospheric pollutants, the persons in charge of the motorway company, the elected representatives and the inhabitants of the city where the study site is located. 

References:

Hofman, J., Maher, B. A., Muxworthy, A. R., Wuyts, K., Castanheiro, A., and Samson, R.: Biomagnetic Monitoring of Atmospheric Pollution: A Review of Magnetic Signatures from Biological Sensors, Environ Sci Technol, 51, 6648–6664, https://doi.org/10.1021/acs.est.7b00832, 2017.

Letaïef, S., Camps, P., Poidras, T., Nicol, P., Bosch, D., and Pradeau, R.: Biomagnetic monitoring vs. CFD modeling: A real case study of near-source depositions of traffic-related particulate matter along a motorway, Atmosphere, 11, 1–23, https://doi.org/10.3390/atmos11121285, 2020.

How to cite: Camps, P., Poidras, T., Nicol, P., Vittori, M.-A., Letaïef, S., and Lefevre, M.: A multi-approach to study and communicate on the effect of highway infrastructures on the dispersion of traffic-related air pollutants., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10792, https://doi.org/10.5194/egusphere-egu23-10792, 2023.

EGU23-11368 | Orals | AS2.1 | Highlight

Studies of land-atmosphere feedback with a new synergy of observing systems 

Volker Wulfmeyer

In this presentation, a series of projects is presented and discussed to study land-atmosphere (L-A) interaction entirely based on measurements. The first effort, where a suitable sensor synergy was deployed for studying mainly the atmospheric leg, was the Land Atmosphere Feedback Experiment (LAFE) performed in August 2017 at the ARM SGP site. During this campaign, new tools where developed to derive turbulence and flux profiles, investigate flux-gradient relationship, retrieve surface fluxes using machine learning, measure feedback metrics using remote sensing instruments, and compare the observations with nested model simulations down to the turbulent scales. LAFE also demonstrated the importance of advection to investigate local and non-local feedback processes.

The successful performance of LAFE led to the establishment of the Land-Atmosphere Feedback Observatory (LAFO, see https://lafo.uni-hohenheim.de/en) at the University of Hohenheim, Stuttgart, Germany. Here, the LAFE observations are realized operationally so that larger data sets and their statistics can be evaluated. First results on feedback metrics over the heterogeneous agricultural landscape of LAFO will be presented.

These activities culminated in the GEWEX Land-Atmosphere Feedback Observatory (GLAFO), which is one of the projects of the Global Land-Atmosphere System Studies (GLASS) Panel (see https://www.gewex.org/panels/global-landatmosphere-system-study-panel/glass-projects). The GLAFO will observe mass, energy, water, and momentum transport with unprecedented spatial and temporal resolutions, from bedrock to the lower troposphere encompassing the atmospheric boundary layer (ABL). The vision of GLAFO is to establish LAFOs in different climate zones over the Earth in order to study L-A feedback from the diurnal cycle, via seasonal/annual to ideally climatological time scales.

How to cite: Wulfmeyer, V.: Studies of land-atmosphere feedback with a new synergy of observing systems, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11368, https://doi.org/10.5194/egusphere-egu23-11368, 2023.

EGU23-11526 | Posters on site | AS2.1

Do cold pools generated by convective downdrafts allow the development of low-level jets? 

Eduardo Weide Luiz and Stephanie Fiedler

Despite the importance of low-level jets (LLJ), their driving mechanisms are not well understood largely due to a shortage of suitable observational data. The classical description for LLJ follows the concept of inertial oscillations at night (NLLJ). Their development is associated with the nocturnal decoupling of winds from the surface friction due to the formation of a near-surface temperature inversion. However, LLJs have also been connected to convectively generated Cold Pools (CP) in kilometre-scale model. CPs are mesoscale areas of cool and dense air formed through convective downdrafts underneath precipitating clouds. Data from the Field Experiment on Submesoscale Spatio-Temporal Variability (FESSTVal) gave us the unique opportunity to test the hypothesis that LLJ formation is also connected to CP passages. We used measurements from three Doppler LIDAR instruments located about 6 km apart from each other, a microwave radiometer and radiosondes for atmospheric profiling, and a large and dense network of surface measurements for the CP detection. During the three-month long field experiment, about 4.7% of all identified LLJ profiles were connected to a CP event (CPLLJ). The average length of CPLLJs was almost two hours. The core of CPLLJ had a mean wind speed of 7 ms−1 and a mean height of 207 m. Using Doppler LIDAR also allowed us to look at wind gusts in the core of the CPLLJs. We measured wind gust of up to 17.5 ms−1 in their core, which exceeds the maximum gust of 15 ms−1 in NLLJs. Close to the surface, the wind speed differences between CPLLJs and NLLJs were even larger than in the core. Most measured CPLLJs appeared at the time of the passage of the CP front and lasted not long after the front has passed, with an interesting exception of a six-hour long CPLLJ during daytime on 29 June 2022. In wind and temperature profiles, we clearly see density currents reaching the experiment site paired with the appearance of strong LLJ profiles. After the passage of the CP front, relatively weaker LLJ profiles were seen. The measurements show that the CP favoured the development of a stably stratified near-surface layer. In a first moment, when the CP front reached the site, there was a mean cooling between the surface up to at least 400 m a.g.l.. After that, the layers bellow 200 m a.g.l. continued to cool, forming a temperature inversion, similar to what one would expect from nocturnal radiative cooling. Radiosondes indicate the typical daytime unstable conditions at the surface and a neutral stratification in the well-mixed boundary layer before the CP arrived. At the time of the CP passage, unstable stratification was seen over a deeper layer followed by the development of a stable stratification in the two hours after the front passed. These conditions led to the formation of a strong and long-lived CPLLJ during daytime. The observations from the FESSTVaL campaign gave first robust evidence that CPs can favour reduced frictional coupling of the wind field to the surface as a prerequisite for generating LLJs.

How to cite: Weide Luiz, E. and Fiedler, S.: Do cold pools generated by convective downdrafts allow the development of low-level jets?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11526, https://doi.org/10.5194/egusphere-egu23-11526, 2023.

EGU23-11552 | Orals | AS2.1 | Highlight

Evapotranspiration: spatial variability in semiarid terrain at the sub-daily scale 

Joan Cuxart, Aaron Boone, Jeremy Price, Jannis Groh, and Daniel Martínez-Villagrasa

An experimental campaign was organised in summer 2021 in the Eastern Ebro basin, in the frame of the LIAISE Initiative (Land surface Interactions with the Atmosphere over the Iberian Semi-arid Environment). Amongst other measurements, the surface energy budget were obtained over different surfaces, including irrigated crops and orchards, rainfed areas and a lake, all them within a radius of 10 km.

For dry weather conditions, the values of the latent heat flux (or Evapotranspiration, ET) were very different depending on the surface, varying from more than 500 W/m2 over an irrigated corn field to less than 30 W/m2 over dry bare soil. These different values implied also different sensible heat fluxes, with the irrigated surfaces showing thermal stable stratification in the afternoon well before sunset due to the cooling effect of evaporation.

The contrast between the irrigated and the rainfed areas is very well-marked induced mesoscale circulations and local transport of humidity, which were overruled by the sea breeze arrival in the afternoon. Over the semi-arid rainfed areas, ET proceeded very irregularly in time and challenged the fundamental hypotesis of stationarity for the computation of the turbulent fluxes. Over all the well-watered surfaces, classical estimates of Potential ET, such as Penman-Monteith or Priestley-Taylor, overestimated the observed values.

How to cite: Cuxart, J., Boone, A., Price, J., Groh, J., and Martínez-Villagrasa, D.: Evapotranspiration: spatial variability in semiarid terrain at the sub-daily scale, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11552, https://doi.org/10.5194/egusphere-egu23-11552, 2023.

EGU23-11730 | ECS | Posters on site | AS2.1

Sensitivity study of the PALM model system to different driving conditions 

Jelena Radovic, Michal Belda, Jaroslav Resler, Pavel Krč, Kryštof Eben, Martin Bureš, and Jan Geletič

The LES-based PALM model system 6.0 is a state-of-the-art atmospheric numerical model widely used among scientists for urban boundary layer and urban climate studies. Despite being subjected to many validation and sensitivity studies which tested the model’s accuracy and applicability to urban environments, a major step is needed to test its sensitivity to different driving conditions.

In this study, we performed a series of PALM model simulations for a given domain and two selected episodes during the year 2019. Each simulation lasts 72 h, and all of them were performed for an 8 km x 8 km domain in 10 m resolution encompassing a real built-up residential area in the southeast part of the city of Prague, Czech Republic. The simulation setups are identical apart from  the initial and boundary conditions imposed. For that purpose we utilized the mesoscale WRF model and created an ensemble consisting of several members with different parameterization schemes.

This study's findings are serving to better understand how different initial and boundary conditions affect the PALM model simulations. In addition, we present the process, complexity, and challenges one can encounter while trying to find the optimal set of initial and boundary conditions for a given PALM model simulation. Moreover, the performed simulations have shown that most of the variance in the ensemble comes from the driving conditions. 

How to cite: Radovic, J., Belda, M., Resler, J., Krč, P., Eben, K., Bureš, M., and Geletič, J.: Sensitivity study of the PALM model system to different driving conditions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11730, https://doi.org/10.5194/egusphere-egu23-11730, 2023.

EGU23-12270 | ECS | Posters on site | AS2.1

Sensitivity of boundary layer parameterization to the critical bulk Richardson number in a climate model over India and its adjoining regions 

Prabhakar Namdev, Maithili Sharan, and Saroj Kanta Mishra

The planetary boundary layer (PBL) scheme is required in almost all numerical weather prediction and general circulation models to parameterize the vertical diffusion of mass, moisture and momentum, in which the critical bulk Richardson number (Ricr) is a crucial component. This study investigates the sensitivity of the Holtslag and Boville (HB) PBL scheme to the Ricr in the National Centre for Atmospheric Research Community Atmosphere Model version 5 (NCAR-CAM5) over India and its adjoining regions. According to the HB PBL scheme, turbulent motion in the PBL is caused by surface heating because of incoming solar radiation. The simulations were conducted using various values of Ricr (0.19, 0.25, 0.35, and 0.5) as well as the default scheme (Ricr = 0.30) at a horizontal resolution of 1o. A total of five sets of simulations have been conducted, each for six years; the first year was discarded as spin-up time, and the last five years of simulations are considered for the analysis. The study spans DJF (December–January), MAM (March–May), JJA (June–August), and SON (September–November) seasons over the study domain. The study shows that the HB PBL is highly sensitive to the value of Ricr employed in the simulation. The results demonstrate that over the whole study domain (20S-40N, 40E-140E), as well as just over land and ocean, the mean planetary boundary layer height (PBLH) increases nearly linearly with increasing Ricr during all four seasons. The surface sensible and latent heat fluxes exhibit opposite behaviour towards the increment in the values of Ricr. The 2-m temperature, wind, and specific humidity changes are marginal and insignificant during all seasons. Moreover, the total precipitation averaged over the whole domain also shows increasing behaviour as Ricr increases during all four seasons.

Keywords: PBL parameterization, Critical bulk Richardson number, Climate model, Surface turbulent fluxes, Precipitation

How to cite: Namdev, P., Sharan, M., and Mishra, S. K.: Sensitivity of boundary layer parameterization to the critical bulk Richardson number in a climate model over India and its adjoining regions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12270, https://doi.org/10.5194/egusphere-egu23-12270, 2023.

EGU23-12568 | ECS | Posters on site | AS2.1

Effects of near-surface atmospheric stability and turbulence on air pollution levels in Madrid 

Pablo Ortiz-Corral, Carlos Román-Cascón, Encarna Serrano, Mariano Sastre, Gregorio Maqueda, and Carlos Yagüe

Air pollution is one of the main hazards for human health worldwide, especially in cities. Surface emissions are the main responsible for the presence of pollutants in the near atmosphere, but meteorological conditions typically play a fundamental role in their accumulation or dispersion. In this work, we focus on the near-surface atmospheric stability and turbulence, for which data from four field campaigns with meteorological and pollutant measurements belonging to the AIRTEC-CM project(*) have been analysed. Available data correspond to the winter and summer seasons of 2020 and 2021 at two public sites located in the city centre of Madrid: a University (ETSII) and a Hospital (HCSC). The evolution of turbulence and stability and their relationships with pollutants such as NO2, PM2,5 and PM10 are investigated. To study turbulence, an analysis of friction velocity and turbulent kinetic velocity is carried out, while the stability parameter (Obukhov length) and the Richardson number obtained by means of the simplified universal similarity functions have been considered for the analysis of the stability. Through the analysis of the mean daily cycle of pollutants, it has been observed how its evolution shows two maxima centered on the morning and evening transitions. The results obtained indicate that pollutant concentrations are strongly influenced by the daily cycle of stability and turbulence, marked by the presence of a maximum of turbulence in the central hours of the day (when the sensible heat flux is greater) and a strong decay of this in the day-night transitions, which in the case of the afternoon transition coincides with the shift from the convective to the stable boundary layer. In addition, the time when this turbulence decay occurs modulates the pollutant concentration values reached, added to the intensity of the stability itself.

 

(*) AIRTEC-CM research project (S2018/EMT-4329) is funded by The Regional Government of Madrid (Spain) and the European Union.

How to cite: Ortiz-Corral, P., Román-Cascón, C., Serrano, E., Sastre, M., Maqueda, G., and Yagüe, C.: Effects of near-surface atmospheric stability and turbulence on air pollution levels in Madrid, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12568, https://doi.org/10.5194/egusphere-egu23-12568, 2023.

EGU23-12826 | Posters on site | AS2.1

Coastal winds in the Gulf of Cádiz (southwestern Iberian Peninsula): insights from observations and models 

Carlos Román-Cascón, Tina Brnas, Pablo Ortiz-Corral, Gert-Jan Steeneveld, Águeda Vázquez, Miguel Bruno, Alfredo Izquierdo, Julio Reyes, Jeanette Romero, José Antonio Adame, Jielun Sun, and Carlos Yagüe

Winds in coastal areas are particularly complex due to the drastic change of roughness and thermal properties between the sea and the land areas. Besides, the coastal topography, the shoreline irregularities, the surface state (land cover/use, soil moisture, sea surface temperature (SST), wind waves), and the interactions with the upper parts of the atmospheric boundary layer (ABL) add more complexity to the final characteristics of the surface winds of these regions.

Among coastal winds, coastal breezes are especially common thermally driven flows formed in mid-latitude regions under fair-weather synoptic conditions. Under these situations, the thermal gradient between the sea and the ocean becomes more important, generating pressure gradient forces that lead to onshore winds during the daytime and offshore during the night. The impacts of these winds are broad and varied: they transport humidity, pollutants, and other physical properties in these regions; they can initiate convection (and even trigger the formation of storms), and they also drive the surface coastal currents, among others. From a societal point of view, the coastal breezes are crucial for the wind power industry, air-quality forecasts, maritime sports, and simply for the refreshing impact they cause, an aspect especially important in some areas commonly affected by extreme maximum temperatures and heat waves. Therefore, a correct understanding of the physical characteristics of the coastal breezes is a needed step to correctly forecast them and to be able to investigate their future trends.

In this work, we present an observational analysis of the coastal breezes observed in the Gulf of Cádiz. We highlight some differences found between the breezes formed at the sea and at the land areas from observational measurements. Besides, we use the mesoscale Weather Research and Forecasting (WRF) model to simulate key case studies, showing how the interaction with the background synoptic wind is very important for the final characteristics that the breezes have. Related to this, we have observed how the effect of the changes in the surface (SST, soil moisture) on the breeze’s characteristics depend on the wind vertical profile (background wind). That is, surface changes impact the ABL mixing and the momentum transfer from higher levels, which seems to be the main mechanism that impact the breezes at lower levels, even more than the surface thermal gradient effect.

How to cite: Román-Cascón, C., Brnas, T., Ortiz-Corral, P., Steeneveld, G.-J., Vázquez, Á., Bruno, M., Izquierdo, A., Reyes, J., Romero, J., Adame, J. A., Sun, J., and Yagüe, C.: Coastal winds in the Gulf of Cádiz (southwestern Iberian Peninsula): insights from observations and models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12826, https://doi.org/10.5194/egusphere-egu23-12826, 2023.

EGU23-12869 | Orals | AS2.1

Neutral and stratified turbulent boundary layer flow over low mountains 

Francois Lott, Lucile Pauget, and Anton Beljaars

A uniform approximation of flow over gentle hills with a turbulent closure based on mixing length theory is derived. It permits to  describe the transition from neutral to stratified flow in the production of mountain drag. Our results corroborate previous studies showing that the transition from the form drag associated to the mountain induced changes in boundary layer friction  to the mountain gravity waves drag can be captured by theory. We also confirm that the first is associated with downstream sheltering with relative acceleration at the hill top, the second with upstream blocking with strong downslope winds.  We also show that the downslope winds penetrate well into the inner layer. The theory show that the altitude at which the incident flow need to be taken to calculate the drag is related to the inner layer depth at which dissipative effects equilibrate disturbance advection. We also show that the parameter that capture the transition, which in our case is a Richardson number, is directly related to the altitude of the turning levels of the gravity waves with respect to the mountain length. Our uniform solutions are also used to describe the wave field aloft and the distribution of the Reynolds stress in the vertical. Some directions to combine neutral and stratified effects in the parameterization of subgrid scale orographies in large scale models are given.

How to cite: Lott, F., Pauget, L., and Beljaars, A.: Neutral and stratified turbulent boundary layer flow over low mountains, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12869, https://doi.org/10.5194/egusphere-egu23-12869, 2023.

EGU23-13532 | ECS | Orals | AS2.1

Climatology of boundary layer wind patterns from clear air radar echoes in Germany 

Sebastian Buschow and Petra Friederichs

Long term observations of shallow convection in the atmospheric boundary layer are rare and difficult to obtain, making it hard to evaluate the capabilities of weather models to accurately represent such features. In this study, we demonstrate that clear air radar reflectivities from insects can be exploited to visualize the horizontal structure of convective cells and rolls over Germany. The patterns observed over a 7 year period are analyzed in terms of their spatial scale, orientation and anisotropy using a two-dimensional wavelet transform. Comparable characteristics can be computed from the near-surface windfields of the convection-permitting regional reanalysis COSMO-REA2. We show that, despite the proximity to the gray zone of turbulence, the reanalysis reproduces a surprisingly realistic diurnal cycle in the spatial patterns and may thus give hints on the wind structures during the unobserved part of the timeseries.

How to cite: Buschow, S. and Friederichs, P.: Climatology of boundary layer wind patterns from clear air radar echoes in Germany, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13532, https://doi.org/10.5194/egusphere-egu23-13532, 2023.

EGU23-13685 | ECS | Posters on site | AS2.1

Unveiling the turbulence scale couplings in fluctuating time series during EUREC4A 

Edouard Gauvrit, Marie-Noelle Bouin, Jean-Marc Delouis, and François Boulanger

Inside the Marine Atmospheric Boundary Layer (MABL) turbulence drives a large amount of physical processes through a dynamical coupling. Understanding this coupling is a key issue in weather and climate modeling, but an adapted statistical representation is still lacking. A strong limitation comes from the non-Gaussianities existing inside the MABL. We seek an approach to describe statistically the couplings across scales, which is poorly measured by the power spectrum. Recent developments in data science provide new tools as the Wavelet Scattering Transform (WST), which gives a low-variance statistical description of non-Gaussian processes and offers to go beyond the power spectrum representation.

We proposes to apply WST technique on turbulent moments recorded during the EUREC4A campaign in trade-wind cloud regimes. Using WST analysis on both fluctuating time series and realistic Large-Eddy Simulations (LES), we study how the different scales in turbulent flows interact between each other in the MABL. Are the turbulent flows organised or purely random in the MABL ? Do the couplings change for different cloud organisations ? Do the models show evidence of such scale couplings ?

In this presentation, we first look at the expected WST coefficients law for turbulent flows in the inertial subrange. Second, we present what are the WST coefficients for the measured turbulent moments and how they evolve for different cloud organizations.

How to cite: Gauvrit, E., Bouin, M.-N., Delouis, J.-M., and Boulanger, F.: Unveiling the turbulence scale couplings in fluctuating time series during EUREC4A, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13685, https://doi.org/10.5194/egusphere-egu23-13685, 2023.

EGU23-14855 | ECS | Posters on site | AS2.1

Large-eddy simulations analyzing the impact of RV Polarstern on surrounding measurements during MOSAiC 

Robert Rauterkus and Björn Maronga

The Arctic atmospheric boundary layer (ABL) is a driver of current and future Arctic warming. Yet, the Arctic ABL provides many distinct and nearly idealized cases for investigation. The contrast between polar day and night and the lack of a diurnal cycle and complex topography promotes the formation and observation of persistent ABL states that are usually only short-term in lower latitudes. In 2019 and 2020, the yearlong MOSAiC expedition [1] took place to inject our understanding of the reasons and consequences of current rapid Arctic warming. Its tailor-made combination of atmospheric measurements gathered by the research vessel Polarstern, aircraft, drones, radiosondes, balloons, and various surface-based and remote sensing systems provides us with vast data to analyze.

To ensure MOSAiC data quality and support future data analysis, we apply large-eddy simulations (LESs) for selected weather conditions during MOSAiC, using the PALM model [2] and resolutions of up to less than a meter. Such fine grid spacings allow us to resolve the ship's envelope as an obstacle to the flow and sufficiently represent stably stratified ABLs. PALM's virtual measurement module enables our LESs to create synthetic perturbed and unperturbed observational data. Thus, analysis of their difference and the ship-induced wakes provides an insight into the ship's effects on surrounding in-situ measurements, which is a central aspect for interpreting corresponding data.

Our simulations reveal that effects are not only tied directly to the ship's wake within the turbulent flow. They indicate that ship-induced gravity waves also bear the potential to influence surrounding measurements notably (i. e. their accuracy exceeding). We present and analyze:

  • how influences from both sources rely on atmospheric conditions, the measurement positioning, and the considered atmospheric quantity
  • that effects notably perturb performed measurements frequently up to more than a kilometer distance
  • the underlying mechanisms causing the observed perturbations
  • mitigation and interpretation strategies to work with corresponding data

[1] Shupe, M. D. et al. (2022): Overview of the MOSAiC expedition: Atmosphere. Elementa: Science of the Anthropocene. DOI: 10.1525/elementa.2021.00060.
[2] Maronga, B., et al. (2020): Overview of the PALM model system 6.0, Geoscientific Model Development. DOI: 10.5194/gmd-13-1335-2020.

How to cite: Rauterkus, R. and Maronga, B.: Large-eddy simulations analyzing the impact of RV Polarstern on surrounding measurements during MOSAiC, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14855, https://doi.org/10.5194/egusphere-egu23-14855, 2023.

EGU23-14885 | ECS | Posters virtual | AS2.1

Fog formed by stratus lowering: an observational and modeling case study from the SOFOG3D field campaign 

Maroua Fathalli, Christine Lac, and Frederic Burnet

Fog is a difficult meteorological phenomenon to predict due to its high spatial and temporal variability and the complexity of physical processes and their interplay. In this context, the SOFOG3D field campaign, which took place during winter 2019/2020 over the Landes region in the South-West of France, provides a 3D mapping of the boundary layer during fog events. It aims to advance our understanding of fog processes in order to improve forecasts of fog events by numerical weather prediction (NWP) models.

 

The present study focuses on three days between 28 and 30 December 2019 characterized by different fog life cycles between two sites about 100 km apart. In situ and remote sensing measurements, such as microwave radiometer and cloud radar, show that on the supersite a radiative fog that occurred the first night lifted into a stratus in the morning remained all day long, and lowered in the afternoon to form a new fog by stratus lowering. In contrast at the Agen site, the stratus completely dissipated and a radiative fog formed the second night. The widespread radiative fog over the entire domain during the first night developed due to cold air advection from the East. We conduct data analysis to study why the stratus lowering is generalized over the northern part of the domain, while the stratus completely dissipates over the southern part of the domain.

 

This analysis is complemented by a 3D numerical simulation performed with the Meso-NH model applied at 100 m resolution with a downscaling approach from the operational AROME model, using the LIMA 2-moment microphysical scheme with a prognostic representation of a multimodal aerosol population. Preliminary results show that for the second night, the simulation well reproduces the contrasting fog life cycle for both sites with radiative fog on Agen and stratus lowering on the supersite but forming earlier fog on the former.

 

A budget analysis is conducted to investigate the spatial heterogeneity of this fog event at the regional scale and to study the physical mechanisms involved in fog formed by stratus lowering that remains especially difficult to forecast by NWP models.

 

How to cite: Fathalli, M., Lac, C., and Burnet, F.: Fog formed by stratus lowering: an observational and modeling case study from the SOFOG3D field campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14885, https://doi.org/10.5194/egusphere-egu23-14885, 2023.

EGU23-15143 | Orals | AS2.1

Investigation of Concentration Fluctuations for continuous point sources by high resolution Large Eddy Simulation and Stochastic Modeling 

Massimo Cassiani, Hamidreza Ardeshiri, Ignacio Pisso, Pietro Salizzoni, Massimo Marro, Andreas Stohl, Kerstin Stebel, and Soon-Young Park

Concentration fluctuations from continuous small sources in a neutral boundary layer were investigated by mean of high-resolution Large Eddy Simulation (LES). The data set includes concentration moments up to the fourth order and shows the range of validity of the Gamma probability density function (PDF) model for the concentration fluctuations and the transition to a  Gaussian PDF for ground sources. We also investigated systematically the off-center line peaks in the concentration variance showing that they are persistent for ground level sources while they disappear according to theoretical arguments for elevated sources. The analysis includes a thorough investigation of the distribution of the most energetic components in the frequency domain by using spectral analysis of the LES results and a stochastic model based on simple theoretical arguments. This analysis supports the picture that the peak in concentration variance frequency distribution is related to both the plume dispersion geometry and the turbulent flow. The results also confirm the recent literature findings that for an elevated source the peak in the concentration variance frequency distribution is almost independent from the crosswind location for a given downwind distance from the source. To our knowledge no previous LES or wind tunnel study had the completeness of the current study.

How to cite: Cassiani, M., Ardeshiri, H., Pisso, I., Salizzoni, P., Marro, M., Stohl, A., Stebel, K., and Park, S.-Y.: Investigation of Concentration Fluctuations for continuous point sources by high resolution Large Eddy Simulation and Stochastic Modeling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15143, https://doi.org/10.5194/egusphere-egu23-15143, 2023.

EGU23-16243 | Posters on site | AS2.1

Turbulent dispersion of artificial SO2 puffs in the PBL from tomographic reconstructions of the concentration 

Ignacio Pisso, Massimo Cassiani, Arve Kylling, Kerstin Stebel, Norbert Schmidbauer, Andreas Stohl, Anna Solvejg Dinger, Hamidreza Ardeshiri, and Soon-Young Park

Tomographic 3D reconstructions of artificial puff releases of SO2 were obtained from 2D images taken with UV cameras.  These novel 3D reconstructions provide information on the distribution of concentration from a unique experimaental campaign dataset collected in Rena, Norway. The numerical solutions of the inverse problem of obtaining 3D reconstruction form 2D images were addressed with algebraic methods. Preliminary turbulence analysis of the puff concentration pdf, spatial moments, and 2-point statistics are presented. The experimentally obtained concentration pdf of a puff can be compared with different statistical models found in the literature. The time series of the puff spatial moments are obtained from the 3D concentration field directly in relative coordinates from observations. The distance-neighbour function can also be estimated directly from the 3d puff concentrations. The time series of 3D reconstructions of puffs entail promising posibilities for improving physical parametrizations in numerical dispersion models.

How to cite: Pisso, I., Cassiani, M., Kylling, A., Stebel, K., Schmidbauer, N., Stohl, A., Dinger, A. S., Ardeshiri, H., and Park, S.-Y.: Turbulent dispersion of artificial SO2 puffs in the PBL from tomographic reconstructions of the concentration, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16243, https://doi.org/10.5194/egusphere-egu23-16243, 2023.

EGU23-16390 | ECS | Posters on site | AS2.1

Atmospheric turbulence structure above urban heterogeneous surface 

Ilya Drozd, Alexander Gavrikov, Victor Stepanenko, Irina Repina, Arseniy Artamonov, and Artem Pashkin

The main exchange of energy and mass between the atmosphere and the surface occurs through the means of turbulent processes in the boundary layer of the atmosphere. A modern atmospheric dynamics models use simplified schemes for calculating energy exchange with the surface, based on the Monin-Obukhov similarity theory (MOST). The main requirement of MOST is the uniformity of the underlying surface. This simplification reduces the accuracy of the forecast, especially in regions with complex (heterogeneous) orography, such as in urban conditions. The obtained regularities in the future may allow us to choose the most accurate parameterization for better use of MOST in conditions of a geometrically complex surface and increasing the accuracy of the forecast for urbanized territories.

This paper presents the result of the analysis of the data series for period from 2020 to 2022 obtained from the eddy covariance tower installed in the Meteorological observatory of Moscow State University. Acoustic anemometers with a frequency of 20 Hz record three components of wind speed  and acoustic temperature at altitudes of 2.2 m, 11.1 m and 18.8 m. For processing high-frequency mast data and calculating the static characteristics of turbulence, a set of programs implemented by the authors is used. Gaps are filled by a new algorithm proposed in [3].

Based on a long series of measurements, the seasonal and daily variability of heat and momentum fluxes over an urbanized surface was analyzed. The detailed statistical analysis of the influence of eddy structures was carried out on the formation of turbulent fluxes in the city. The method proposed in [2] was used to identify coherent vortices. The method is based on the hypothesis of the relationship of third and second moments, described by the ratio:

where C∼1 is non-dimensional constant, and Sw is skewness of vertical velocity [1]. The compliance of third moments with theoretical values was established for various stratification conditions in 80% of cases. The result indicates a significant contribution of coherent structures to the formation of vertical fluxes over a geometrically complex surface, which is consistent with the estimates received earlier [2, 4].

References

  • [1] Abdella K. et al. A new second-order turbulence closure scheme for the planetary boundary layer //Journal of the atmospheric sciences. – 1997. – Т. 54. – №. 14. – С. 1850-1867.
  • [2] Barskov K.V. et al. Two regimes of turbulent fluxes above a frozen small lake surrounded by forest //Boundary-Layer Meteorology. – 2019. – Т. 173. – №. 3. – С. 311-320.
  • [3] Drozd I.D. et al. Comparative characteristics of gap filling methods in high-frequency data of micrometeorological measurements //IOP Conference Series: Earth and Environmental Science. – IOP Publishing, 2022. – Т. 1023. – №. 1. – С. 012009.
  • [4] Pashkin A.D. et al. An experimental study of atmospheric turbulence characteristics in an urban canyon //IOP Conference Series: Earth and Environmental Science. – IOP Publishing, 2019. – Т. 386. – №. 1. – С. 012035.

How to cite: Drozd, I., Gavrikov, A., Stepanenko, V., Repina, I., Artamonov, A., and Pashkin, A.: Atmospheric turbulence structure above urban heterogeneous surface, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16390, https://doi.org/10.5194/egusphere-egu23-16390, 2023.

EGU23-17257 | ECS | Orals | AS2.1

Study of atmospheric dispersion under low wind conditions in an urban environment 

Hanane Bounouas, Pierre Roupsard, Eric Dupont, Yannick Lefranc, Aurélien Faucheux, Didier Hebert, Olivier Connan, Philippe Languionie, and Yelva Roustan

Impact studies of industrial sites for air pollutant emissions must consider all representative meteorological conditions. For low wind conditions, the impact evaluations present large uncertainties. Dispersion mechanisms and turbulence properties in these situations are modified and favor the stagnation of emitted pollutants in the atmosphere. The improvement of the understanding and modeling of these situations is hampered by a lack of data at the international level, particularly for the built environment.

The objectives of this study are to present and analyze experimental data of dispersion of a tracer gas (Helium) under low winds in urban environment, as well as analyze the meteorological conditions corresponding to these situations to characterize the processes dominating the dispersion (especially meandering).

Two measurement campaigns were realized in 2020 and 2022 respectively on the SIRTA (Site Instrumental de Recherche par Télédétection Atmosphérique). This built area is located near Paris in a peri-urban environment. The height of the buildings varies between 5 and 30 m. Helium concentrations are measured using air samples and mass spectrometers in real time, in the near field of the emission point (<300m). Wind and turbulence conditions are measured by ultrasonic anemometers positioned at different heights in the surface layer and in the canopy layer.  Atmospheric Transfer Coefficients (ATC) are determined to quantify plume dispersion.

Data processing consists in establishing atmospheric turbulence parameters of each experiment (friction velocity, heat flux, Monin-Obukhov Length), in analyzing the spatial distribution of Helium concentrations in the built environment, especially searching correlation between the variations of the concentrations and of the wind directions and making spectral and autocorrelation analysis of the wind speed components to characterize the flow meandering.

The meandering is characterized by an oscillating behavior of the Eulerian autocorrelation function with the presence of a negative loop for the horizontal components u and v of the wind speed. The autocorrelation function of the vertical component w presents a classical exponential curve. The periods of this process vary between 20 and 60 min in the first experimental campaign. The meandering disperses the plume over a wide angular range. The analysis of the time series shows the oscillation of the wind direction in low wind.

The meandering modifies the low frequencies part of the spectrum of the wind speed horizontal components. The impact of the urban environment on this phenomenon is shown using comparisons between spectrum and autocorrelation functions measured at 3 m (inside the buildings canopy) and 30 m heights (above the buildings). The next step is to link the dispersion and meandering processes by performing  cospectrum of ATC and wind direction, in order to have information on the frequency dependence of the covariance of these two variables.

How to cite: Bounouas, H., Roupsard, P., Dupont, E., Lefranc, Y., Faucheux, A., Hebert, D., Connan, O., Languionie, P., and Roustan, Y.: Study of atmospheric dispersion under low wind conditions in an urban environment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17257, https://doi.org/10.5194/egusphere-egu23-17257, 2023.

EGU23-17284 | Posters on site | AS2.1

Perturbed Roughness Sublayer affecting the law of thewall modeled by a "co-spectral link" 

Yardena Bohbot-Raviv and Gabriel George Katul

 

Fully developed turbulent flows near walls, regardless of their roughness, are commonly studied based on the law of the wall originally proposed by Prandtl and von Karman in the early part of the 20th century. The derivation of the law of the wall has traditionally been based on theoretical and scaling arguments, under which a balance between dissipation and production (negligible advection terms) of turbulent kinetic energy and a nearly constant shear stress with distance from the wall are assumed in a thin layer of fluid, accommodating about 10% of the boundary layer (i.e., separation of scales). One of the hallmarks of this theory is the von-Karman constant (=0.4) valid across many wall-roughness and boundary layer flow configurations. In many situations, however, the separation of scales required to observe a log-layer is hardly realizable, especially in tall and fully rough canopy flows as in submerged aquatic vegetation and urban centres under certain atmospheric conditions. In recent years, several spectral- and co-spectral -based theories have revealed a "link" between the law of the wall and the energy spectrum of turbulent eddies. This link is exploited here to examine the roughness sublayer of a rough canopy boundary layer. A simplified co- spectral model and data collected from wind tunnel experiments allows to examine the roughness sublayer correction to the law of the wall and test the effect of finite Reynolds number and intermittency on the von-Karman constant, from which the scales dominating the law of the wall in the roughness sublayer are revealed.

How to cite: Bohbot-Raviv, Y. and Katul, G. G.: Perturbed Roughness Sublayer affecting the law of thewall modeled by a "co-spectral link", EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17284, https://doi.org/10.5194/egusphere-egu23-17284, 2023.

EGU23-17377 | Orals | AS2.1

Using Mixing Diagrams to Evaluate the Evolution of theConvective Boundary Layer in NWP Models 

David D. Turner, Timothy Wagner, Thijs Heus, Tessa Rosenberger, and Siwei He

Land-atmosphere feedbacks can play a critical role in daytime convective boundary layer (CBL) evolution. Mixing diagrams provide a framework for disentangling the relative contributions of entrainment, advection, and surface fluxes in the evolution of the CBL moisture and energy budgets. Entrainment is particularly difficult to observe with operational ground-based sensors, and mixing diagrams provide a way to quantify this contribution to the CBL.

We use this framework to evaluate the evolution of the CBL as represented by the Rapid Refresh (which has 13-km grid) and the High-Resolution Rapid Refresh (which has a 3-km grid) numerical weather prediction models.  We have identified 30 cases in a three-month period between May and July 2019 at the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) site in north-central Oklahoma; over this period of time the land surface transitioned from a moist soil with green vegetation to a relatively dry soil with harvested crops.  A key instrument in this analysis is an infrared spectrometer (IRS), from which profiles of temperature and humidity can be retrieved at 5-min resolution.  At this ARM site, a network of IRS and Doppler lidars surround the central facility, from which we are able to derive the advective fluxes of temperature and water vapor.  Our analysis focused on how well the two modeling systems represent the relative contributions from entrainment, surface fluxes, and advection over this three-month period.

How to cite: Turner, D. D., Wagner, T., Heus, T., Rosenberger, T., and He, S.: Using Mixing Diagrams to Evaluate the Evolution of theConvective Boundary Layer in NWP Models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17377, https://doi.org/10.5194/egusphere-egu23-17377, 2023.

Measurements of the atmospheric boundary layer (ABL) structure were performed for three years (October 2017–August 2020) at the Russian observatory “Ice Base Cape Baranova” (79.280° N, 101.620° E) using SODAR (Sound Detection And Ranging). These measurements were part of the YOPP (Year of Polar Prediction) project “Boundary layer measurements in the high Arctic” (CATS_BL). ABL measurements and near-surface observations were used for verification of the regional climate model COSMO-CLM (CCLM) with a 5 km resolution for 2017–2020. The SODAR showed a topographical channeling effect for the wind field in the lowest 100 m. The verification of the CCLM with near-surface data of the observatory showed good agreement. The comparison with SODAR data showed a positive bias for the wind speed of about 1.0-1.5 m/s. The CCLM data showed the frequent presence of low-level jets (LLJs) associated with the topographic channeling. Although SODAR wind profiles are limited in range and have a lot of gaps, they represent a valuable data set for model verification. However, a full picture of the ABL structure and the climatology of channeling events could be obtained only with the model data. LLJs were detected in 37% of all profiles and most LLJs were associated with channeling, particularly LLJs with a jet speed ≥15 m/s (which were 29% of all LLJs). The analysis of the simulated 10m wind field showed that the 99%-tile of the wind speed reached 18 m/s and clearly showed a dipole structure of channeled wind at both exits of Shokalsky Strait. The climatology of channeling events showed that this dipole structure was caused by the frequent occurrence of channeling at both exits. Channeling events lasting at least 12 h occurred on about 62 days per year at both exits.

How to cite: Heinemann, G., Drüe, C., and Makshtas, A.: SODAR observations and model simulations of the wind field structure in the atmospheric boundary layer at Severnaya Zemlya (Siberia) during YOPP, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2112, https://doi.org/10.5194/egusphere-egu23-2112, 2023.

EGU23-3690 | PICO | AS2.2 | Highlight

Atmospheric Rivers and Surface Melt Events Over the Greenland Ice Sheet 

William Neff, Mathew Shupe, Christopher Cox, and Michael Gallagher

In the summer of 2012, nearly the entire Greenland Ice Sheet (GIS) melted  as warm air and thin clouds moved over the GIS in association with an Atmospheric River (AR) (Bennartz et al. 2013, Neff et al. 2014).  More recently surface melt as well as rainfall have been observed at Summit Station Greenland.  While these events garner much media attention, systematic mass loss in the ablation zones around the ice sheet (particularly along the southwest coast), in the transition to the accumulation zone and vulnerable glacier systems (Mattingly et al. 2021) is important to forecast sea level rise.  In this analysis, we use a simple detection method to identify ARs along the Greenland west coast using reanalysis data at two points (60N/310W and 65N/305W) at 850 hPa, namely wind speed and direction and total integrated water vapor.  We show a comparison between ERA5, NCEP/NCAR, and the Twentieth Century Reanalysis to show the efficacy of this approach and the ability to track ARs over the past hundred years. The approach exploits the barrier effect of the GIS, which extends to about 700 hPa.
This use of reanalysis data is then coupled with the calculation of the fraction of melt in a series of latitude-longitude boxes at various locations around the ice sheet using the MEaSURES data set (Mote 2016) for the period 2000-2012. We then develop composite synoptic maps for geopotential height, total column water vapor, and Omega (for vertical velocity) for each class of event (e.g. strong ARs) and their subsequent evolution over 3 to 5 days. A key finding is that ARs that first impact the west coast later transport moisture to the SE coast leaving a residue of moisture along the west coast as the associated blocking high moves to the east.  In addition, we show how strong ARs along the west coast reflect geopotential height patterns very similar to those presented in (Gallagher et al. 2018) that are also associated with warmer temperature and increased opaque cloudiness at Summit Station.  Finally, we examine how various extreme events fit into this picture and affect the meteorology at Summit Station, including dramatic changes in boundary layer structure.

References

Bennartz, R., M. D. Shupe, D. D. Turner, V. P. Walden, K. Steffen, C. J. Cox, M. S. Kulie, N. B. Miller and C. Pettersen (2013). Nature 496(7443): 83-86.Gallagher, M. R., M. D. Shupe and N. B. Miller (2018. Journal of Climate."  31(21): 8895-8915.

Mattingly, K. S., T. L. Mote and X. Fettweis (2018). Journal of Geophysical Research: Atmospheres.

Mote, T. L. (2016). MEaSUREs Greenland Surface Melt Daily 25 km EASE-Grid 2.0, version 1. https://doi.org/10.5067/MEASURES/CRYOSPHERE/nsidc-0533.001.

Neff, W., G. P. Compo, F. M. Ralph and M. D. Shupe (2014). Journal of Geophysical Research-Atmospheres 119(11): 6520-6536.

Mattingly et al., EGU General Assembly 2021

How to cite: Neff, W., Shupe, M., Cox, C., and Gallagher, M.: Atmospheric Rivers and Surface Melt Events Over the Greenland Ice Sheet, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3690, https://doi.org/10.5194/egusphere-egu23-3690, 2023.

EGU23-4112 | PICO | AS2.2

New source mechanism for airborne particulate mercury in the central Arctic 

Julia Schmale, Helene Angot, Benjamin Heutte, Nora Bergner, Stephen Archer, Ludovic Bariteau, Ivo Beck, Byron Blomquist, Matthew Boyer, Markus Frey, Detlev Helmig, Dean Howard, Hans-Werner Jacobi, Tuija Jokinen, Tiia Laurila, Jakob Pernov, Kevin Posman, Kerri Pratt, and Lauriane Quelever

Understanding the mercury cycle in the Arctic is important due to the harmful bioaccumulation of its toxic form, methylmercury, in wildlife and ultimately Arctic residents. Gaseous elemental mercury (Hg(0)) is relatively well-mixed across the northern hemisphere atmosphere due to its long atmospheric lifetime. Hg(0) can be oxidized, especially in the Arctic spring during halogen-driven depletion events. The resulting gaseous oxidized mercury (Hg(II)) is relatively quickly deposited onto snow, either directly or via condensing onto particles, forming particulate mercury (PHg). It is generally understood that a large fraction of the deposited Hg(II) and PHg is photoreduced to Hg(0) and re-emitted to the atmosphere. However, mercury remaining in the snowpack till melt can become bioavailable through entering the ocean.

There is a severe lack of Hg(II) and PHg observations in the central Arctic, particularly over sea ice, limiting our understanding of the mercury cycle in that region and inhibiting us from quantifying mercury budgets in all environmental compartments and particularly where it unfolds its harmful neurotoxic effects. Moreover, most of the observational efforts aiming at creating process understanding focused on spring during mercury depletion events or the snow melt period, leaving large knowledge gaps for fall and winter.

Here, we show atmospheric observations of PHg during MOSAiC, measured with an aerosol mass spectrometer in fall and spring over the central Arctic pack ice. In both seasons, PHg concentrations correlate strongly with wind speed and chloride, suggesting a mechanical (wind-driven) process behind atmospheric PHg related partly to blowing snow. In addition, there are significant differences between fall and spring observations (e.g. no atmospheric mercury depletion events in fall), suggesting that various processes are at play.

This wind-driven process has hitherto not been reported and is different from observations at land-based stations as well as previous measurements over sea ice that ascribed the formation of PHg to adsorption of Hg(II) onto pre-existing aerosols or diamond dust rather than aerosolization from the snow pack. We hypothesize, based on snow chemical analyzes and literature, that the elevated halide content in snow on sea ice creates complexes of PHg, which are much harder to photoreduce than Hg(II), leading to a larger PHg content in snow. These processes of forming PHg and wind-driven aerosolization have implications for the mercury content of snow and the distances over which PHg is re-deposited after atmospheric transport given that the lifetime of PHg is about one order of magnitude larger than that of Hg(II) in the atmosphere. 

How to cite: Schmale, J., Angot, H., Heutte, B., Bergner, N., Archer, S., Bariteau, L., Beck, I., Blomquist, B., Boyer, M., Frey, M., Helmig, D., Howard, D., Jacobi, H.-W., Jokinen, T., Laurila, T., Pernov, J., Posman, K., Pratt, K., and Quelever, L.: New source mechanism for airborne particulate mercury in the central Arctic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4112, https://doi.org/10.5194/egusphere-egu23-4112, 2023.

EGU23-5469 | ECS | PICO | AS2.2

Snowpack nitrate photolysis drives the summertime atmospheric nitrous acid (HONO) budget in coastal Antarctica 

Amelia M. H. Bond, Markus M. Frey, Jan Kaiser, Jörg Kleffmann, Anna E. Jones, and Freya A. Squires

In the polar regions, the usual OH radical formation pathway (ozone photolysis and reaction of O(1D) with H2O) is limited by the low water vapour concentration. However, gases emitted from the snowpack can be pre-cursors of HOx radicals and ozone, thereby controlling the oxidising capacity of the lower atmosphere above remote snow-covered regions.

Snowpack photolysis of nitrate and the resulting emissions of the reactive nitrogen species NOx and HONO can lead to OH production through rapid cycling of RO2 → HO2 → OH and photolysis of HONO. Research into reactive nitrogen species in polar environments has focused on NOx, with far fewer investigations into HONO. Previous studies of HONO in the polar boundary layer and snowpack interstitial air suggest a photolytic snowpack source but the exact mechanism for HONO production is poorly understood; photochemical models of HONO sources and sinks often cannot be reconciled with the measured HONO concentrations.

A LOng Path Absorption Photometer (LOPAP) was used to investigate the net HONO flux density above snow in the Clean Air Sector at Halley VI Research Station in coastal Antarctica during Austral summer 2021/22. We present amount fraction measurements of HONO in ambient air, as well as measurements of the HONO flux density between the snow and atmosphere by the flux-gradient method. The potential snowpack reactions driving this HONO release are discussed, as well as the implications of these measurements for the HOx budget. These findings help further our understanding of the atmospheric budget of reactive nitrogen and highlight the significant effects snow surfaces can have on the atmospheric chemistry in the boundary layer above.

How to cite: Bond, A. M. H., Frey, M. M., Kaiser, J., Kleffmann, J., Jones, A. E., and Squires, F. A.: Snowpack nitrate photolysis drives the summertime atmospheric nitrous acid (HONO) budget in coastal Antarctica, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5469, https://doi.org/10.5194/egusphere-egu23-5469, 2023.

EGU23-5706 | PICO | AS2.2

Vertical profiles of pollutants in Fairbanks, Alaska during the ALPACA 2022 field campaign 

Brice Barret, Natalie Brett, Roman Pohorsky, Andrea Baccarini, Julia Schmale, Gianluca Pappacogli, Federico Scoto, Stefano Decesari, Antonio Donateo, Gilberto J. Fochesatto, William Simpson, Meeta Cesler-Maloney, Jinqiu Mao, Elsa Dieudoné, Slimane Bekki, Stephen Arnold, Barbara d'Anna, Patrice Medina, Maurizio Busetto, and Kathy S. Law

The ALPACA (Alaskan Layered Pollution and Chemical Analysis) field campaign (January-February 2022) aimed to collect new data to document Arctic wintertime air pollution. State of the art instrumentation was deployed in Fairbanks, Alaska to characterise inorganic/organic aerosols, vertical layering and mixing of aerosols and precursors, and meteorology at sites influenced by local anthropogenic emissions and background Arctic Haze.

Vertical profiles of the boundary layer composition were collected from an instrumented tethered ballon (helikite) deployed at the UAF-Farm site in West Fairbanks. The Helikite payload included instruments dedicated to the characterisation of particles (concentration, composition, size distribution) and to measurement of trace gases with dedicated analysers for O3, CO and CO2 and a MICROMEGAS instrument. MICROMEGAS is a light-weight package based on low-cost Alphasense electrochemical sensors for trace gases (CO/O3/NO/NO2). This instrument was also deployed on the ground close to reference-grade trace gas analysers at the CTC measurement site in downtown Fairbanks, and onboard a vehicle for 2D-mapping of pollution within and around Fairbanks.

Low-cost electrochemical sensors are sensitive to temperature and humidity and require careful calibration and validation. We first introduce the calibration method based on multi-linear regression with the collocated CTC reference measurements. The performance (biases, correlation coefficients, RMSDs) of the calibrated data are then evaluated against CTC observations not used for the calibration. Cases of vertical helikite profiles with polluted layers related to specific dynamical conditions (temperature inversions, wind regimes…) are investigated. Tracer-tracer relationships (CO, NO, NO2 versus CO2 ; NOx versus Ox) together with meteorological observations are used to examine air mass origins (domestic combustion, vehicles, power plants), as well as dilution and chemical transformation of the sampled pollution plumes.

How to cite: Barret, B., Brett, N., Pohorsky, R., Baccarini, A., Schmale, J., Pappacogli, G., Scoto, F., Decesari, S., Donateo, A., Fochesatto, G. J., Simpson, W., Cesler-Maloney, M., Mao, J., Dieudoné, E., Bekki, S., Arnold, S., d'Anna, B., Medina, P., Busetto, M., and Law, K. S.: Vertical profiles of pollutants in Fairbanks, Alaska during the ALPACA 2022 field campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5706, https://doi.org/10.5194/egusphere-egu23-5706, 2023.

Ice is one of the most common matters on earth and regarded as active reaction media in the environment. Recently, it was reported that several chemical reactions in frozen state proceed unexpected pathway and markedly accelerated compared to those in aqueous phase. The freeze concentration of reactants, protons, and gases in ice grain boundaries between ice crystals is regarded as main driving force for the intrinsic chemical processes in ice. Iodine plays important roles on ozone depletion event, oxidation of gaseous elemental mercury (Hg0) to Hg(II), oxidizing capacity in atmosphere, control of HOx and NOx ratio in marine boundary layer, and the formation of ultrafine aerosol particles as cloud condensation nuclei(CCN). Furthermore, iodine is also proposed to be a potential proxy for past sea ice variability. However, the chemical behavior of iodine compounds during transport and after deposition is not well understood. Although the intensive investigations on chemical behavior of iodine species such as theoretical studies, laboratory experiments, and field observations, the clear pathway and mechanism of iodine formation in polar regions are still uncovered. In this presentation, I want to introduce several unique chemical processes in ice related to iodine compounds such as 1) redox reactions of iodide (I-), iodate (IO3-), periodate (IO4-) in ice, 2) interaction between iodine and metal oxides, 3) degradation and removal of pollutants with iodine species for the better understanding of fate of iodine species in polar environment. The detailed experimental conditions and mechanism will be discussed in the presentation

How to cite: Kim, K.: Abiotic transformation of iodine species in ice and its environmental implications, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5906, https://doi.org/10.5194/egusphere-egu23-5906, 2023.

EGU23-6258 | ECS | PICO | AS2.2

Investigating the relative contributions of power plant and surface emissions to air pollution in Fairbanks, Alaska during the wintertime ALPACA 2022 campaign 

Natalie Brett, Kathy S. Law, Stephen R. Arnold, Brice Barret, Elsa Dieudonné, Gilberto J. Fochesatto, Robert Gilliam, Tatsuo Onishi, Slimane Bekki, Julia Schmale, Roman Pohorsky, Andrea Baccarini, Barbara D'Anna, Brice Temime-Roussel, Stefano Decesari, Gianluca Pappaccogli, Antonio Donateo, Federico Scoto, Meeta Cesler-Maloney, and Deanna Huff and the UAF & EPA Continued

Local air pollution sources in the Arctic lead to poor air quality in Arctic cities, particularly during the winter months. Fairbanks in central Alaska, is a prime example of such an Arctic city which suffers from acute wintertime pollution episodes. The topography of Fairbanks (situated in a basin), coupled with strong surface-based temperature inversions, contributes to stable meteorological conditions that hinder the dispersion of pollutants and surface temperatures reaching -40 °C. These harsh winter conditions result in enhanced domestic and power plant combustion emissions. Stable meteorological regimes are frequently interspersed with less stable episodes, resulting in vertical mixing between surface and elevated inversion layers. However, there are many uncertainties in our understanding about pollution sources and secondary aerosol formation under cold, dark winter conditions, where photochemistry is limited. These issues were addressed through the collection of comprehensive datasets on atmospheric composition and meteorology in Fairbanks, during the international ALPACA (Alaskan Layered Pollution and Chemical Analysis) field campaign in January and February 2022. Data were collected at the surface and vertical profiles were collected using a tethered balloon (EPFL Helikite).

Here, we examine the relative contributions and distributions of power plant emissions, emitted above the surface, and surface emission sources to pollution levels in the Fairbanks region. The FLEXPART-Weather Research and Forecasting (WRF) Lagrangian particle dispersion model, driven by meteorological fields from WRF-Environmental Protection Agency (EPA, Alaska) simulations is deployed. Firstly, model runs are used to evaluate the transport and dispersion of emissions from power plants at several altitudes in and around Fairbanks. Surface-based and elevated temperature inversions, characteristic of the winter boundary layer in Fairbanks, are considered in a parameterisation of power plant plume injection heights, and temporal variations in these emissions is also taken into account. Secondly, the extent to which power plant emissions are contributing to surface pollution is investigated using power plant (point source) and sector-based surface EPA emissions at 1.3km resolution at hourly time resolution during the 2022 campaign period. Model results are evaluated against available vertical profile and ground-based observations from ALPACA 2022. Power plant plumes are simulated aloft at several ALPACA measurement sites, as validated by vertical profile observations. The simulations indicate that power plant emissions are mixed down towards the surface in some cases. These results also provide insights into relative source contributions from each power plant in Fairbanks within the vertical profile of the lower atmospheric boundary layer, which could be used as tool for source apportionment studies.

How to cite: Brett, N., Law, K. S., Arnold, S. R., Barret, B., Dieudonné, E., Fochesatto, G. J., Gilliam, R., Onishi, T., Bekki, S., Schmale, J., Pohorsky, R., Baccarini, A., D'Anna, B., Temime-Roussel, B., Decesari, S., Pappaccogli, G., Donateo, A., Scoto, F., Cesler-Maloney, M., and Huff, D. and the UAF & EPA Continued: Investigating the relative contributions of power plant and surface emissions to air pollution in Fairbanks, Alaska during the wintertime ALPACA 2022 campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6258, https://doi.org/10.5194/egusphere-egu23-6258, 2023.

EGU23-6320 | ECS | PICO | AS2.2

Freezing-induced bromate reduction through iodide and its implications 

Quoc Anh Nguyen and Kitae Kim

Freezing, which is the naturally facile process in the cold climate regions, has been extensively investigated as a non-contamination and effective cost method in the environmental treatment. The reactive halogens chemistry has a huge impact on the global environment, especially polar regions. Here, we elucidated the generation of iodine (I2), tri-iodide (I3-), and bromide (Br-) through the bromate (BrO3-) reduction by iodide (I-) in the unfrozen solution of ice while it did not take place in aqueous solution. This appreciably enhanced transformation was attributed majorly to the freeze concentration effect of BrO3-, I-, and protons (H+) in the liquid boundary of ice. The ice grain boundary regions created as well as the consumption of BrO3- in the BrO3-/I-/freezing systemin those regions during freezing were visualized with the confocal Raman microscope. pH decrease (the accumulation of H+) during freezing was measured quantitatively by the UV-Vis absorption spectra of cresol red (as the acid-base indicator). Also, the freeze concentration effect of I- on the BrO3- transformation was verified in the differently experimental conditions of pH and/ or I- concentration. The study on the acceleration of BrO3-/I-/freezing system provides not only an unknown production pathway of bromine and iodine speciation in the polar environment but also the environmentally friendly insight into BrO3- treatment (known as the disinfection byproduct during ozonation in water treatment). 

How to cite: Nguyen, Q. A. and Kim, K.: Freezing-induced bromate reduction through iodide and its implications, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6320, https://doi.org/10.5194/egusphere-egu23-6320, 2023.

EGU23-6988 | ECS | PICO | AS2.2

Modelling sea salt aerosol flux from blowing snow over a changing sea ice environment 

Ananth Ranjithkumar, Eliza Duncan, Xin Yang, Daniel Partridge, and Markus Frey

A quantitative understanding of climate change in the polar regions being more extreme than at lower latitudes requires monitoring and modelling of key climate variables in these regions. Climate models disagree with observational datasets on the magnitude of the rate of Arctic amplification, and the representation of the chemistry and microphysics of aerosol particles in models is one of the contributing factors to the uncertainty in predicting polar climate. Aerosols represents one of the key model uncertainties through its impact on the surface energy balance via the scattering and absorption of solar radiation, and by its ability to influence cloud microphysics. Sea salt aerosol originating from the sublimation of blowing snow is a newly discovered source of aerosol particles above sea ice during winter and spring, and the hypothesised formation mechanism has been validated recently in the Antarctic. However, the lack of observations over a wide range of sea ice conditions including sub-micron sized particles has been a barrier towards accurately quantifying the mechanism of formation of SSA and the resulting SSA mass flux. Moreover, current blowing snow model parameterisations do not consider the spatial and temporal variability of sea ice and atmospheric state, which has a strong impact on the strength of the particle source from blowing snow across individual storms. In this study, we use observations from the MOSAIC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition (Oct 2019 to Sept 2020) and N-ICE2015 (Feb-June 2015) in the Arctic, and Weddell Sea measurements (June-October 2013) in the Antarctic to better constrain the blowing snow sea salt flux. We consider snow particle size distribution and snow salinity, which are both sensitive model parameters that govern the sea salt aerosol flux over sea ice. A gamma distribution fit is used to characterise the snow particle size distribution as a function of the 10-meter wind speed (ranging from the threshold wind speed (~5ms-1) to 15ms-1). Using the observations, we were able to better constrain the shape parameter of the gamma distribution, alpha, when compared to past studies.  We discuss the relationship between snow salinity and snow depth, to capture the influence of the changing sea ice and snowfall on blowing snow aerosol source. We implement these parametrisations derived from point measurements into a chemistry transport model (p-TOMCAT) to better capture the spatially and temporally variable blowing snow source across polar regions, which helps to accurately simulate the aerosol number and mass concentration, and sodium concentration in polar regions.

How to cite: Ranjithkumar, A., Duncan, E., Yang, X., Partridge, D., and Frey, M.: Modelling sea salt aerosol flux from blowing snow over a changing sea ice environment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6988, https://doi.org/10.5194/egusphere-egu23-6988, 2023.

EGU23-8027 | ECS | PICO | AS2.2

Linking Sea Spray, Bioaerosols and Ice-Nucleation Proteins in Arctic Marine Environments 

Christian DF Castenschiold, Claudia Mignani, Sigurd Christiansen, Malin Alsved, Sylvie Tesson, Jacob Löndahl, Merete Bilde, Kai Finster, and Tina Šantl-Temkiv

Clouds have one of the most profound effects on Earth’s climate, yet they are still responsible for some of the biggest uncertainties in climate models. Cloud formation, radiative properties, thickness and lifetime are tightly interlinked with the presence of atmospheric particles (aerosols) and the formation of ice. Biological aerosols (bioaerosols) such as ice-nucleation proteins (INpro) produced by microorganisms are most efficient catalysts in the formation of ice and can trigger heterogenous freezing between -1°C and -15°C. Several studies have demonstrated that Arctic environments are a source of airborne INpro. Sea spray is one of the major sources of aerosols, which aside of the sea salt contain large amounts of organic material. These are ejected into the atmosphere through the process of wave breaking and bubble bursting of small bubbles, which eject drops from the sea surface microlayer (SML) to the atmosphere. Here, we present results derived from droplet freezing assays and amplicon sequencing combined with quantitative PCR, targeting the 16S rRNA gene from sea and aerosol samples collected along a transect from sub- to high Arctic Greenland (Baffin Bay). We demonstrate a positive correlation between INpro concentration and higher latitudes in sea bulk water (SBW) and SML. Additionally, we try to link specific taxonomic groups from the microbial communities to INpro production. Last, we aim to investigate if partitioning of specific taxonomic groups can be observed from SBW to SML and from SML to the atmosphere. Finally, we performed laboratorial sea-spray experiments simulating turbulent sea conditions. This study has the potential to help closing the current knowledge gap in understanding the partitioning of microorganisms from the sea to the atmosphere and unravel which microbes are the major contributors to atmospheric INpro and hence cloud formation.

How to cite: Castenschiold, C. D., Mignani, C., Christiansen, S., Alsved, M., Tesson, S., Löndahl, J., Bilde, M., Finster, K., and Šantl-Temkiv, T.: Linking Sea Spray, Bioaerosols and Ice-Nucleation Proteins in Arctic Marine Environments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8027, https://doi.org/10.5194/egusphere-egu23-8027, 2023.

EGU23-8076 | ECS | PICO | AS2.2

Can thawing permafrost alter the general circulation of the atmosphere? 

Mark Schlutow, Tom Doerffel, Martin Heimann, and Mathias Goeckede

Thawing Arctic permafrost has been assigned increasing importance as a key element in the global climate system over the past decades. One quarter of land surface of the northern hemisphere are permafrost regions, containing about 50% of the global below-ground carbon pool. Permafrost degradation and the associated climate feedback pose a potential tipping element that might be reached even within 1.5 °C global warming. Besides the potential release of additional carbon, permafrost degradation also holds the potential to significantly alter the surface characteristics of affected landscapes, resulting in further feedback processes that are poorly understood so far.

In the presented study, we investigate the impact of permafrost degradation onto the structure of the atmospheric boundary layer (ABL) as a first feedback link to the global circulation. High-resolution Large Eddy Simulations (LES) are used to quantify the role of surface heterogeneity as a particular driver for boundary layer characteristics. Our virtual experiments simulate the structural changes of the ABL linked to long-term enhanced permafrost thaw, including e.g. the formation of new ponds and lakes, or increased spatial heterogeneity in vegetation structure with the establishment of different grass and shrubs species. Such changes may result in shifted fingerprints of heat and momentum fluxes into the atmosphere. Through this connection, ongoing climate change may lead to permanently altered influences of thawed permafrost on temperature and moisture profiles within the Arctic atmosphere, including changes in the boundary layer height. A particular focus of our study will be placed on the potential loss of water being drained away from the ecosystem after permafrost degradation, where the dried out soil not only changes the carbon cycle processes but also exhibits new surface characteristics. We quantify how the ABL reacts to those changes in idealized LES experiments, and investigate how atmospheric changes may further affect permafrost degradation.

How to cite: Schlutow, M., Doerffel, T., Heimann, M., and Goeckede, M.: Can thawing permafrost alter the general circulation of the atmosphere?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8076, https://doi.org/10.5194/egusphere-egu23-8076, 2023.

EGU23-8833 | PICO | AS2.2

Turbulent heat exchange over polar leads – an LES study 

Micha Gryschka and Zakaria Mostafa

Leads are Chanel-like openings in the sea-ice through which heat of several 100 Watt/m2 is transferred from the ocean into the atmosphere. Even though leads account only for a view percent to the total ice coverage in polar regions, they modify the polar boundary layer significantly. Therefore, leads need to be considered in numerical weather and climate models. Since, generally leads are not explicitly resolved in these models it is important to understand the overall effect of leads of different sizes onto the boundary layer for different meteorological conditions.

With numerous Large-Eddy simulations, we investigated the dependency of the lead averaged surface heat flux on the lead width in a range between a few meters to several kilometers for different meteorological and surface conditions. Generally, we found under same temperature differences between ice and water and same meteorological conditions for small leads a decrease of lead averaged surface heat flux with lead width (as often observed in experimental studies), but for wider leads a significant increase.

We like to give some brief explanations of the possible causes for this behavior as well as to oppose these results to other former studies in this field, which might disagree to these in some points.

How to cite: Gryschka, M. and Mostafa, Z.: Turbulent heat exchange over polar leads – an LES study, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8833, https://doi.org/10.5194/egusphere-egu23-8833, 2023.

EGU23-9024 | PICO | AS2.2

Sea salt aerosol and ice nucleating particles (INP) in the Central Arctic during winter/spring – a discussion of a source from blowing snow above sea ice 

Markus M. Frey, Amélie Kirchgäßner, Floor van den Heuvel, Thomas Lachlan-Cope, Frank Stratmann, Heike Wex, Amy R. Macfarlane, Jessica Mirrielees, Kerri Pratt, Ivo Beck, Julia Schmale, Kouichi Nishimura, and Ian Brooks

Arctic clouds are poorly represented in climate models partly due to a lack of understanding of their source and nucleating capability of natural aerosol in the high Arctic. Recent field campaigns provided evidence of a source of sea salt aerosol (SSA) from blowing snow above sea ice, which can account for SSA winter/spring maxima observed in the polar regions. SSA emissions from sea ice sources can potentially influence regional climate via the indirect radiative effect, but contributions to cloud-forming particles, in particular, ice-nucleating particles (INP), are unknown. Here we report the first online spring-time observations of INPs in the Central Arctic. INP concentrations were on the order of a few tens [particle m-3] activating between -38 and -15°C and were often associated with high wind speeds. Initial offline droplet assay analysis of snow on sea ice indicates the presence of potential INPs in winter/spring activating at -29 to -25°C. This is evidence that snow on sea ice represents a viable reservoir of INPs, which can be physically released via the blowing snow mechanism to the air above. We discuss sea ice sources of coarse SSA and INPs and their role in the lower atmosphere with a focus on blowing snow. To do this, we consider the comprehensive set of MOSAiC observations, including aerosol size and composition, airborne snow particles, and chemical and physical properties of both aerosol and snow on sea ice.

How to cite: Frey, M. M., Kirchgäßner, A., van den Heuvel, F., Lachlan-Cope, T., Stratmann, F., Wex, H., Macfarlane, A. R., Mirrielees, J., Pratt, K., Beck, I., Schmale, J., Nishimura, K., and Brooks, I.: Sea salt aerosol and ice nucleating particles (INP) in the Central Arctic during winter/spring – a discussion of a source from blowing snow above sea ice, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9024, https://doi.org/10.5194/egusphere-egu23-9024, 2023.

EGU23-10564 | ECS | PICO | AS2.2

Evidence of Ocean and Permafrost as Sources of Bioaerosols in the Alaskan Arctic Boundary Layer 

Marina Nieto-Caballero, Thomas C. J. Hill, Kevin R. Barry, Christina S. McCluskey, Thomas A. Douglas, Paul J. DeMott, Sonia M. Kreidenweis, and Jessie M. Creamean

As a result of Arctic air temperatures rising at four times the global rate, the cryosphere is rapidly thawing, releasing greenhouse gas reservoirs and metabolically active greenhouse gas-producing microorganisms. In addition, thawing cryosphere elements, such as permafrost (i.e., ground that is frozen for at least two consecutive years) and ice wedges (i.e., frozen water accumulated in ground cracks due to expansion and contraction of permafrost), can be introduced into water systems by different mechanisms. These mechanisms can include thermokarst lake formation (i.e., ice-rich permafrost areas that thaw and create surface depressions that are filled with thawed ice) and the increasingly common permafrost landslides.

 

One of the hypotheses proposed in the multidisciplinary ARCSPIN (ARCtic Study of Permafrost Ice Nucleation) project is that microorganisms from thawed permafrost and ice wedges are discharged into water bodies in the Arctic region, and are ultimately released to the atmosphere through mechanisms such as thermokarst lake greenhouse gas bubble-bursting, and bubble-bursting due to higher wind-induced wave action on lakes, lagoons, and the open ocean. Additionally, these airborne biological particles can be a potential source of ice nucleating particles (INPs) active at warm temperatures (≥ -10oC), potentially altering cloud properties in Arctic regions. Arctic clouds have strong effects on regional and global energy budgets, with cloud phase (i.e., liquid or ice) being a key modulator of their interactions with radiation. Arctic mixed-phase clouds (AMPCs) are prevalent and are key in the ocean-ice-atmosphere system affected by the delicate energy balance over frozen surfaces. Ice formation in AMPCs is highly sensitive to the quantity and effects of aerosols serving as INPs.

 

Here, we present results from a broad range of environmental samples collected during the ARCSPIN campaign in the Summer of 2021 in Northern Alaska (Utqiaġvik region), including air, water (i.e., sea, river, lagoon, and thermokarst lake), terrestrial (i.e., active layer, permafrost, ice wedge, and sediment), and vegetation samples. These samples were processed for 16S rRNA gene sequencing to identify and track microorganisms, showing for the first time how bioaerosols in Northern Alaska are influenced by terrestrial and water sources of the region. We additionally include results from published microbiome studies to perform source tracking analysis (Sourcetracker2), showing the potential long-range influence of ocean microorganisms, in particular, as bioaerosol sources in the Arctic. The obtained microbiome results are linked to meteorological conditions and air back trajectories calculated with NOAA’s HYSPLIT model.

 

Data generated from the ARCSPIN study in combination with the Community Earth System Model (CESM) will be used for parameterization development and to investigate potential impacts of this unique INP source on Arctic clouds, helping to understand sources and impacts of bioaerosols in the Arctic. 



How to cite: Nieto-Caballero, M., Hill, T. C. J., Barry, K. R., McCluskey, C. S., Douglas, T. A., DeMott, P. J., Kreidenweis, S. M., and Creamean, J. M.: Evidence of Ocean and Permafrost as Sources of Bioaerosols in the Alaskan Arctic Boundary Layer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10564, https://doi.org/10.5194/egusphere-egu23-10564, 2023.

EGU23-11181 | ECS | PICO | AS2.2

The long-term observation of black carbon and CO concentration in Alaska: Effect of forest fire emissions 

Takeshi Kinase, Masayuki Takigawa, Fumikazu Taketani, Hideki Kobayashi, Chunmao Zhu, Yongwon Kim, and Yugo Kanaya

The climate change in the Arctic region seriously accelerated compared to the entire globe. Black carbon (BC) aerosol particles, which are one of the SLCFs (short-lived climate forcers) emitted from incomplete combustion processes, absorb solar radiation and have a large impact on the climate. In addition, deposited BC on snow and ice surface decreases surface albedo and contributes to snow melting and Arctic warming. However, a large spread among model estimations for BC in the Arctic remains because of the lack of observation as a constraint and differences among emission inventories.

Alaska in northern America has a large boreal forest. Forest fires in Alaska represent an important BC source for the Arctic and surrounding regions, especially for interior Alaska during the summer season. However, observation of BC in interior Alaska is not sufficient. In this presentation, we introduce our five-year-long observations of BC and CO in interior Alaska and our findings on the relationship between the BC/∆CO ratio and the forest fire intensity.

BC and CO monitoring at Poker Flat Research Range (PFRR; 65.12 N, 147.43 W) started in April 2016. PFRR is located in the centre of Alaska and is surrounded by evergreen needle-leave forests. Forest fires occur occasionally in the summer season and strongly affect BC and CO concentrations in PFRR. Median BC mass concentration through the observation period was 15.2 ng/m3 and did not show a clear seasonal variation. However, sporadically significant increases in BC were observed during summer. Comparing BC concentrations observed at PFRR with those at Denali (63.72 N, 149.0 W), Trapper creek (62.32 W, 153.15 W), and Barrow (71.32 N, 156.61 W), we found a weak correlation only for Denali (r2 =0.3), indicating different air mass transport patterns as strong separated by high mountains particularly large differences between the interior and coastal regions in Alaska were noticed. On the other hand, the CO mixing ratio showed clear seasonal variation patterns, i.e. high in spring and low in summer. The median value of the CO mixing ratio was 124.7 ppb and significant increases were observed in the same period as BC, indicating the influences from the common emission sources. The median BC/∆CO ratio was 1.6 ng/m3/ppb and did not show clear seasonal variations. Furthermore, we quantitatively estimated the source contributions of BC using FLEXPART-WRF based on GFEDv4.1 inventory. As a result, FLEXPART-WRF represented high BC concentration periods with a relatively good correlation (r2 =0.54) but underestimated approximately 17 %. Source estimation by FLEXPART-WRF indicated a strong contribution of forest fires from surrounding areas during the high BC concentration periods. We compared BC/∆CO and Fire Radiative Power observed in Alaska by MODIS. As a result, we found a positive relationship between these two values, indicating the increase of BC/∆CO with forest fire intensity. Our result suggests that the dependency of the BC and CO emission factors on the combustion intensity of forest fires should be taken into account to elaborate emission estimations from boreal forest fires.

How to cite: Kinase, T., Takigawa, M., Taketani, F., Kobayashi, H., Zhu, C., Kim, Y., and Kanaya, Y.: The long-term observation of black carbon and CO concentration in Alaska: Effect of forest fire emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11181, https://doi.org/10.5194/egusphere-egu23-11181, 2023.

EGU23-11403 | ECS | PICO | AS2.2

Wintertime vertical distribution of air pollution in suburban Fairbanks during the ALPACA 2022 field campaign 

Roman Pohorsky, Andrea Baccarini, Brice Barret, Natalie Brett, Gianluca Pappaccogli, Federico Scoto, Antonio Donateo, Maurizio Busetto, Slimane Bekki, Kathy Law, Stefano Decesari, Steve Arnold, Javier Fochesatto, William Simpson, and Julia Schmale

The Alaskan Layered Pollution and Chemical Analysis (ALPACA) field campaign investigated the sources and processing of wintertime urban pollution in Fairbanks, Alaska in January and February 2022. Several sites located around the city of Fairbanks collected data to study the underexplored cold and dark wintertime dynamical, physical and chemical processes driving air pollution, both outdoors and indoors. We deployed a tethered balloon system at a farm field site near the University of Alaska (UAF) to specifically investigate the vertical layering of pollution and influence of different emission altitudes on surface pollution levels.

The study site is located in a suburban area, west of downtown Fairbanks. Observational efforts there focused mainly on surface exchanges and the vertical distribution of pollutants in relation to the boundary layer structure, specifically under stable (inversion) conditions. Instruments at the UAF-farm provided continuous ground measurements of aerosol physical, optical and chemical properties, trace gases (O3, CO, N2O) and meteorology. The newly designed Modular Multiplatform Air Compatible Measurement System (MoMuCAMS) was deployed with a tethered-balloon (helikite) to sample air up to 350 m above ground level, providing information on the vertical distribution and mixing processes of atmospheric pollutants. Instruments onboard MoMuCAMS provided information on aerosol characteristics (particle number concentration, size distribution, absorption coefficient and chemical composition), trace gases (CO2, O3, CO, N2O, NOx), and meteorology. MoMuCAMS performed 21 flights between January 26 and February 25, 2021, collecting roughly 140 individual profiles of varying altitude under different boundary layer conditions, intercepting pollution plumes at different heights and of different composition. Given the suburban location of  the study site, we measured the influence of polluted air from the city and “cleaner” air from more remote origins.

We will show how the vertical structure of the atmosphere and the frequently occurring temperature inversions affect transport and dispersion of pollution at different heights and how different meteorological conditions affect local air circulation and pollution at the study site. 

How to cite: Pohorsky, R., Baccarini, A., Barret, B., Brett, N., Pappaccogli, G., Scoto, F., Donateo, A., Busetto, M., Bekki, S., Law, K., Decesari, S., Arnold, S., Fochesatto, J., Simpson, W., and Schmale, J.: Wintertime vertical distribution of air pollution in suburban Fairbanks during the ALPACA 2022 field campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11403, https://doi.org/10.5194/egusphere-egu23-11403, 2023.

EGU23-11513 | ECS | PICO | AS2.2

Spatial Variability and Composition of Ice Nucleating Particles over the Southern Ocean 

Kathryn Moore, Thomas Hill, Christina McCluskey, Bryan Rainwater, Darin Toohey, Cynthia Twohy, Jorgen Jensen, Sonia Kreidenweis, and Paul DeMott

Supercooled liquid clouds are ubiquitous over the Southern Ocean (SO), even down to temperatures of -25 °C, and comprise a large fraction of the marine boundary layer clouds. Many Earth System Models and reanalysis products overestimate the occurrence of ice and have insufficient liquid cloud cover in the region, while recent simulations have found that the microphysical representation of ice nucleation and growth has a large impact on these properties. However, measurements of SO ice nucleating particles (INPs) to validate simulated ice nucleation are sparse, and many previous observations were limited to fairly warm temperatures (-15 or -20 °C). Observations of INPs are presented here from two simultaneous field campaigns in the SO during January-March 2018: the Clouds, Aerosols, Precipitation Radiation and atmospherIc Composition Over the southeRN ocean II (CAPRICORN-2) study on the CSIRO R/V Investigator, and the Southern Ocean Cloud Radiation Aerosol Transport Experimental Study (SOCRATES) on the NSF/NCAR G-V aircraft. The SOCRATES campaign is noteworthy for collecting the first in-situ observations in and above cloud in the SO. Measurements of INPs active in the immersion freezing mode were made during both projects in real time with Colorado State University (CSU) Continuous Flow Diffusion Chambers (CFDCs) at temperatures below -25 ℃, and via offline analyses of aerosol filter and seawater samples using the CSU Ice Spectrometers from -10 to -30 ℃. INP concentrations were at the lower bound of those from other ocean regions, and much lower than historical measurements in the SO collected prior to the early 1970s. Chemical treatments performed on the filter suspensions were used to infer the fraction of biological, organic, and mineral INPs, which varies with latitude and height, and indicate a variety of sources, including local marine aerosol and dust. Data from G-V overflights of the R/V Investigator were used to investigate the vertical structure of INPs in this region. Electron microscopy analyses of INPs collected from the CFDCs, along with back trajectories and aerosol measurements, provide additional information on INP composition and possible sources.

How to cite: Moore, K., Hill, T., McCluskey, C., Rainwater, B., Toohey, D., Twohy, C., Jensen, J., Kreidenweis, S., and DeMott, P.: Spatial Variability and Composition of Ice Nucleating Particles over the Southern Ocean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11513, https://doi.org/10.5194/egusphere-egu23-11513, 2023.

EGU23-12241 | ECS | PICO | AS2.2

The Partitioning Processes of Sea Ice Associated Marine Ice Nucleation Particles Impacting the Arctic Clouds 

Lasse Jensen, Eva Kjærgaard, Maria Cifarelli, Rosella Di Pompeo, Martina D'Agostino, Jennie Schmidt, Jane Skønager, Dorte Søgaard, Bernadette Rosati, Merete Bilde, Lars Lund-Hansen, Kai Finster, and Tina Šantl-Temkiv

The Arctic is a region that is particularly vulnerable to the impacts of climate change, as it is warming at a faster rate than the rest of the world. This warming causes a decline in multiyear sea ice cover, which results in an increasing open-ocean surface with a much lower albedo therefore leading to positive feedback and enhanced warming. Another factor that plays a role in regulating the temperature in the Arctic is the type and extent of cloud cover. Aerosols that can serve as cloud condensation nuclei or ice nucleating particles (INPs) are key for cloud formation. Some microorganisms are known to produce INPs, but it is not well understood which microorganisms are responsible, which environments they inhabit, and how active they are. In this study, we set out to investigate the partitioning of INPs between the Arctic marine and atmospheric environment by combining in situ measurements with laboratory experiments.

First, we wanted to determine if sea ice acts as a reservoir for INPs and, if so, whether the INPs are partitioned into the sea ice during its formation or produced by microorganisms within the sea ice. We used a modified ice-finger to grow sea ice using natural samples from West Greenland and found that INPs concentrate into the ice fraction during sea-ice formation, and that these INPs typically are associated with microorganisms.

Next, we wanted to understand the temporal and spatial dynamics of INPs in Arctic sea ice. We collected sea ice cores from the Arctic before and during the spring sea ice phytoplankton bloom and analysed them using cold-stage INP measurements, flow-cytometry, and amplicon sequencing. The results showed that there are between <105 · L-1 (at the top) and >106 · L-1  (at the bottom of the sea ice) INP-10 present in the Arctic sea ice.  

Finally, we wanted to determine the potential contribution of sea ice to the atmospheric INP pool in the Arctic. We introduced natural samples of bulk water and sea ice from Nuuk and Station Nord into a temperature-controlled sea spray simulation chamber and quantified the microorganisms and INPs present in the bulk water, surface microlayer and air before and after aerosolization. The results showed that the highly active INPs are efficiently aerosolized into the atmosphere during bubble-bursting where they may contribute to the formation of ice in clouds.

Overall, this study provides new insight into the role of Arctic sea ice as a reservoir for INPs and the microorganisms that produce them, as well as the mechanisms by which INPs are released into the Arctic atmosphere. This information is important for understanding the impact of climate change on the Arctic region and the potential consequences for the rest of the world.

How to cite: Jensen, L., Kjærgaard, E., Cifarelli, M., Di Pompeo, R., D'Agostino, M., Schmidt, J., Skønager, J., Søgaard, D., Rosati, B., Bilde, M., Lund-Hansen, L., Finster, K., and Šantl-Temkiv, T.: The Partitioning Processes of Sea Ice Associated Marine Ice Nucleation Particles Impacting the Arctic Clouds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12241, https://doi.org/10.5194/egusphere-egu23-12241, 2023.

EGU23-14269 | ECS | PICO | AS2.2

Characterization of size-segregated particles turbulent fluxes in an Arctic city (Fairbanks, Alaska) 

Gianluca Pappaccogli, Antonio Donateo, Federico Scoto, Maurizio Busetto, Roman Pohorsky, Andrea Baccarini, Julia Schmale, Brice Barret, Slimane Bekki, Natalie Brett, Kathy S. Law, Elsa Dieudonné, Gilberto J. Fochesatto, William Simpson, Barbara D'Anna, Brice Temime-Roussel, and Stefano Decesari

Wintertime air pollution affects air quality of Arctic and sub-Arctic urban areas, because of the coupling between strong local emissions for residential heating and energy production and poor atmospheric dispersion associated with a stratified planetary boundary layer. Aerosols represent priority pollutants in such environments, and their behaviour in the Arctic wintertime boundary layer not only impacts air quality but also determines deposition on snow or ice surfaces, leading to chemical and physical modifications in the snowpack. The interactions between boundary layer meteorology and air pollution were the focus of the international ALPACA (Alaskan Layered Pollution and Chemical Analysis) field campaign held in January and February 2022 in Fairbanks (AK, USA). The aim of the present work is to analyse the fluxes of atmospheric particles in at a urban background site in Fairbanks, based on continuous observations of aerosol concentration, size distributions, and size-segregated deposition velocities. The EC system was installed at the suburban site of UAF (University of Alaska Farm), located nearby the foothills bordering the city basin. The main micrometeorological parameters and fluxes (wind field, friction velocity, turbulent kinetic energy, and sensible heat flux) were characterized in terms of boundary layer conditions (occurrence of thermal inversions, dynamic stratifications, vertical wind shear, slope currents, coherent turbulence structures). The aerosol eddy covariance system was based on a condensation particle counter (CPC) - able to measure particles down to 5 nm in diameter - and an Optical Particle Counter Optical Particle Counter (OPC) for evaluating particle fluxes in the accumulation mode (0.25 < dp < 0.8 μm) and quasi-coarse mode (0.8 < dp < 3 μm). The median number concentration was 13 E+3 cm−3, 76 cm−3 and 0.3 cm−3 for ultrafine, accumulation and quasi-coarse particles mode, with higher concentrations found at low wind speeds. The particle fluxes showed a net emission pattern for the ultrafine, accumulation and quasi-coarse dimensional mode, especially in daytime, with average values of 203, 0.3, and 0.02 cm-2 s-1 respectively. Deposition periods were observed most frequently for air masses from the city located to the east, while local emission sources due to traffic lead emission fluxes, especially in the accumulation mode. We discuss the particle flux measurements in the context of parallel aerosol and gaseous pollutants determined by fixed and mobile platforms (a tethered balloon and a car) as well as of determinations of depositions in the snow pack across the Fairbanks area.

How to cite: Pappaccogli, G., Donateo, A., Scoto, F., Busetto, M., Pohorsky, R., Baccarini, A., Schmale, J., Barret, B., Bekki, S., Brett, N., Law, K. S., Dieudonné, E., Fochesatto, G. J., Simpson, W., D'Anna, B., Temime-Roussel, B., and Decesari, S.: Characterization of size-segregated particles turbulent fluxes in an Arctic city (Fairbanks, Alaska), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14269, https://doi.org/10.5194/egusphere-egu23-14269, 2023.

EGU23-14320 | ECS | PICO | AS2.2 | Highlight

Aerosol source identification in the spring and summertime central Arctic Ocean using high-resolution mass spectrometry during MOSAiC. 

Benjamin Heutte, Lubna Dada, Hélène Angot, Imad El Haddad, Gang Chen, Kaspar R. Dällenbach, Jakob B. Pernov, Ivo Beck, Lauriane Quéléver, Tiia Laurila, Tuija Jokinen, and Julia Schmale

The Arctic region is undergoing considerable changes and is warming at a rate three to four times as fast as the rest of the world. Aerosols, which can originate from natural or anthropogenic sources, both of which can be locally emitted or long-range transported, play a crucial role in the Arctic radiative balance by directly absorbing or scattering incoming solar radiation or indirectly by changing cloud properties and modulating cloud formation mechanisms. Here, we investigate the sources of anthropogenic and natural aerosols in the central Arctic Ocean, using data collected during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition with a high-resolution time-of-flight aerosol mass spectrometer. Using positive matrix factorization on the organic fraction of aerosols during spring and summertime (March – July), we identified six distinct chemical sources of organic aerosols (OA): a hydrocarbon-like factor, a Haze factor, two factors related to two extreme events of warm and moist air mass intrusions (WAMI) in mid-April, an Arctic oxygenated factor, and a Marine factor. We also describe the geographical origin of these factors, inferred from a potential source contribution function applied on 3-hourly back-trajectories. Together, these results suggest that OA from Eurasian anthropogenic origin (including the two extreme WAMI events in mid-April) dominate the central Arctic OA budget until at least the month of May, where episodic spikes in naturally-sourced marine OA, originating from the Fram Strait marginal ice-zone start to become important through June and July. We also highlight a hitherto unreported highly-oxygenated organic factor, whose temporal variability is closely related to that of particulate ammonium (maximum concentration in May) and whose geographical origin, in the Canadian archipelagoes, could indicate a co-emission mechanism of organic aerosols and ammonia from Arctic seabird colonies.

How to cite: Heutte, B., Dada, L., Angot, H., El Haddad, I., Chen, G., Dällenbach, K. R., B. Pernov, J., Beck, I., Quéléver, L., Laurila, T., Jokinen, T., and Schmale, J.: Aerosol source identification in the spring and summertime central Arctic Ocean using high-resolution mass spectrometry during MOSAiC., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14320, https://doi.org/10.5194/egusphere-egu23-14320, 2023.

EGU23-14641 | ECS | PICO | AS2.2

Characterization of blowing snow aerosol events in the central Arctic 

Nora Bergner, Ivo Beck, Kerri Pratt, Jessica Mirrielees, Jessie Creamean, Markus Frey, Benjamin Heutte, Hélène Angot, Steve Arnold, Janek Uin, Stephen Springston, Sergey Matrosov, Tiia Laurila, Tuija Jokinen, Lauriane Quéléver, Jakob Pernov, Xianda Gong, Jian Wang, and Julia Schmale

Sea salt aerosols play a critical role in aerosol-radiation and aerosol-cloud interactions. Salty blowing snow has been hypothesized as an important source of sea salt aerosol in polar regions. The snow over sea ice can become salty by upward brine migration or deposition of sea spray produced from leads or transported from the ice edge. Wind-driven resuspension and sublimation of the snow is hypothesized to leave salty aerosol particles behind. Our understanding of aerosol emissions from blowing snow is based mainly on modeling studies, and direct observations to validate this process are sparse. The year-long Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition, with its integrated measurements and sampling of frequent winter storms, is well suited to enhance our understanding of coupled Arctic system processes. Here, we focus on the impact of blowing snow and high wind speed events on aerosol number concentrations, size distributions, optical properties and cloud condensation nuclei (CCN) concentrations. Total aerosol number concentrations were significantly enhanced during high-wind speed periods, also concurrent with increased scattering aerosol coefficients and CCN concentrations. We further present a process-based characterization of the blowing snow events during MOSAiC and identify the influence of environmental variables on aerosol emissions. Our observations provide new insights into wind-driven aerosol in the central Arctic and may help to validate modelling studies and inform parameterization improvement particularly with respect to aerosol direct and indirect radiative forcing.

How to cite: Bergner, N., Beck, I., Pratt, K., Mirrielees, J., Creamean, J., Frey, M., Heutte, B., Angot, H., Arnold, S., Uin, J., Springston, S., Matrosov, S., Laurila, T., Jokinen, T., Quéléver, L., Pernov, J., Gong, X., Wang, J., and Schmale, J.: Characterization of blowing snow aerosol events in the central Arctic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14641, https://doi.org/10.5194/egusphere-egu23-14641, 2023.

EGU23-15174 | ECS | PICO | AS2.2

Estimation of moisture fluxes in East Antarctica and their impact on the isotopic composition of the snow surface 

Inès Ollivier, Hans Christian Steen-Larsen, Barbara Stenni, Mathieu Casado, and Amaëlle Landais

The ability to infer past temperatures from ice core records has in the past relied on the assumption that after precipitation, the stable water isotopic composition of the snow surface layer is not modified before being buried deeper into the snowpack and transformed into ice. However, in extremely dry environments, such as the East Antarctic plateau, the precipitation is so sparse that the surface is exposed to the atmosphere for significant time before burial. During that exposure, several processes have been recently identified as impacting the snow isotopic composition after snowfall: (1) exchanges with the atmosphere (i.e. sublimation/condensation cycles), (2) wind effects (i.e. redistribution and pumping) and (3) exchanges with the firn below (i.e. metamorphism and diffusion).

Here we present the data over several seasons and years of the atmospheric water vapor and snow surface isotopic composition at Dome C, East Antarctica. To understand the link between these two elements, we investigate the moisture fluxes at the surface of the ice sheet, at the snow-air interface. No eddy-covariance measurements are available for the recent years, we therefore make use of the available primary meteorological parameters measured continuously on site to estimate the surface moisture fluxes using the bulk method. We estimate that the cumulative effect of the moisture fluxes is positive: about 12% of the mean annual accumulation is sublimated away. Alongside, we see an enrichment in d18O in the snow surface during the summer months, when most of the moisture fluxes are taking place. The snow d-excess is also affected and evolving in anti-phase with d18O. This indicates occurrence of fractionation during sublimation in line with previous field and laboratory studies. The moisture fluxes could be a key driver of changes in the snow isotopic composition between precipitation events influencing the climate signal stored in the isotopic record of ice cores.

How to cite: Ollivier, I., Steen-Larsen, H. C., Stenni, B., Casado, M., and Landais, A.: Estimation of moisture fluxes in East Antarctica and their impact on the isotopic composition of the snow surface, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15174, https://doi.org/10.5194/egusphere-egu23-15174, 2023.

EGU23-15867 | ECS | PICO | AS2.2

Invaluable insights into the dynamics and water-vapor isotopes of the planetary boundary layer above the Greenland Ice Sheet from fixed-wing uncrewed aircraft samplings. 

Laura Dietrich, Kevin Rozmiarek, Tyler Jones, Valerie Morris, Chloe Brashear, Hayley Bennett, Bruce Vaughn, Michael Town, Martin Werner, Xavier Fettweis, and Hans Christian Steen-Larsen

The chemistry and aerosols in ice core records are used as proxy data for the past climate. Traditional interpretation of this recorded climate signal is that during formation snow captures a snapshot of the atmosphere. In recent years, observations have documented that the snow surface’s chemistry and isotopic composition change during the post-depositional interaction with the surface-near atmosphere. To more accurately interpret the climate signal in ice cores it is necessary to understand thesource of the water vapor in the planetary boundary layer (PBL), as well as the vertical mixing and transportation in the polar atmosphere. However, the dynamics in the polar PBL are poorly constrained in most climate models due to a lack of observations.

 

Here we present insights from the first Arctic in-situ water-vapor isotope record both within and above the PBL up to 1500 meters above the Greenland Ice Sheet (GrIS) from the EastGRIP ice core camp 2022 field campaign. Flights were performed with a fixed-wing uncrewed aircraft recording high resolution atmospheric profiles. Moreover, air is sampled in glass flasks and brought to the surface for determination of δ18O and δDof water vapor. The observational set-up has been proven to guarantee reliable measurements of the isotopic composition of the atmospheric water vapor in remote locations and under extremely cold temperatures. Based on 105 observed temperature, humidity and isotopic profiles we identify different types of atmospheric structure above the GrIS. We evaluate the vertical atmospheric representation of the polar regional climate model MAR and the isotope-enabled global climate model ECHAM-wiso. Finally, from observations we estimate the height up to which the surface-near δ18O and δD isotopic values are affected by the atmosphere above.

How to cite: Dietrich, L., Rozmiarek, K., Jones, T., Morris, V., Brashear, C., Bennett, H., Vaughn, B., Town, M., Werner, M., Fettweis, X., and Steen-Larsen, H. C.: Invaluable insights into the dynamics and water-vapor isotopes of the planetary boundary layer above the Greenland Ice Sheet from fixed-wing uncrewed aircraft samplings., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15867, https://doi.org/10.5194/egusphere-egu23-15867, 2023.

EGU23-16059 | ECS | PICO | AS2.2

Understanding the Abundance, Variability and Sources of Ice NucleatingParticles (INPs) over the Kara and Laptev Seas in the Eurasian Arctic 

Guangyu Li, André Welti, Arianna Rocchi, German Pérez, Iris Thurnherr, Manuel Dall’Osto, and Zamin A. Kanji

The Arctic region is sensitive to climate change, experiencing accelerated warming. Cloud radiative properties and related feedback mechanisms on Arctic climate are highly uncertain and dependent on the cloud phase. Primary ice formation in Arctic mixed-phase clouds is initiated by INPs. So far, little is known regarding the abundance, variability, and potential sources of INPs in the Arctic owing to the scarcity of data, particularly in the marine environment. We study the INP-cloud interactions to improve the understanding of the abundance and sources of INPs in this region.  We present results from a cruise-based Arctic Century Expedition, which took place from 5 August to 6 September 2021 in the previously uncharted Kara and Laptev Sea in the Eurasian Arctic. Ship-borne INP concentrations (immersion mode) and their spatiotemporal variabilities will be presented and linked to the physicochemical properties of ambient aerosols, including particle size distribution, heat lability, chemical compositions, and biological activities. Additionally, geographical variability of INPs along the ship track are investigated to assess the influence from different origins, e.g., sea ice, marine or terrestrial origins. Ultimately, we will report the results from the in-situ aerosol generator experiments to reveal the phase partitioning of INPs at the sea-air interface highlighting the importance of the aerosolization mechanisms to the production of marine INPs.

How to cite: Li, G., Welti, A., Rocchi, A., Pérez, G., Thurnherr, I., Dall’Osto, M., and A. Kanji, Z.: Understanding the Abundance, Variability and Sources of Ice NucleatingParticles (INPs) over the Kara and Laptev Seas in the Eurasian Arctic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16059, https://doi.org/10.5194/egusphere-egu23-16059, 2023.

EGU23-17118 | PICO | AS2.2

The Effects of the Large Scale Synoptic fields in the High Latitude PBL states. 

Gilberto Javier Fochesatto, Douglas Keller, Elsa Dieudonné, Natalie Brett, Kathy Law, Slimane Bekki, David Atkinson, Ellsworth Wellton, and Eric Peterson

Polar and sub-polar winters represent outstanding opportunities to study the PBL state in connection to the synoptic meteorological fields. In the high latitudes, the absence of a diurnal cycle combined with the presence of an anticyclone feature promotes surface radiative cooling resulting in the formation of a surface based temperature inversion (stably-stratified structure). Under such meteorological conditions, large scale subsidence promotes adiabatic compression (i.e., warming in upper levels) promoting the formation of elevated temperature inversions layers. This multilayered configuration represents a significant challenge for micro-scale/mesoscale modeling and air pollution dispersion as well as for the transport of the local contamination to the global arctic air shed. However, this structure is fragile and can be disrupted by dynamic and radiative effects caused by synoptic variability affecting the PBL state. Thus, significant changes in the PBL state are verified when synoptic situation changes (i.e, warm air advections and more mesoscale frontogenesis).

In this contribution, we describe the state of the PBL linked to the synoptic large scale variability using the high resolution thermodynamic profiling datasets from the 2022 ALPACA field experiment in Fairbanks, Alaska. High resolution synoptic scale reanalysis datasets are used to detail dynamic processes coupled to atmospheric dynamics in the PBL state.-

 

How to cite: Fochesatto, G. J., Keller, D., Dieudonné, E., Brett, N., Law, K., Bekki, S., Atkinson, D., Wellton, E., and Peterson, E.: The Effects of the Large Scale Synoptic fields in the High Latitude PBL states., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17118, https://doi.org/10.5194/egusphere-egu23-17118, 2023.

EGU23-17554 | PICO | AS2.2

Arctic Cyclone Cloud and Boundary-Layer Features Producing Thermodynamic and Dynamic Impacts on Arctic Sea Ice During MOSAiC 

Ola Persson, Christopher Cox, Michael Gallagher, Matthew Shupe, Jennifer Hutchings, Daniel Watkins, and Donald Perovich

MOSAiC was a rare opportunity to obtain observational data on Arctic cyclones (ACs), with at least 22 ACs sampled during four of the five legs.  This presentation will illustrate how some of the AC cloud and boundary-layer characteristics produce both thermodynamic and dynamic impacts on the sea ice in the non-melt seasons.  Deep clouds associated with the ACs enhanced the downwelling radiation, with the surface radiation dependent on cloud height, temperature, and liquid water layers.  Underneath the warm fronts ahead of the ACs, this effect directly warmed the surface, sometimes to the extent of destabilizing the near-surface boundary layer.  Synoptically induced low-level jets (LLJs) found within AC warm sectors between the surface warm front and cold front often also provided warm-air advection down to a few hundred meters above the surface, which, in many cases, produced a stable lower boundary layer and enhanced downward sensible heat flux in these AC regions.  These effects in some mid-winter ACs produced near-surface temperature increases of 20° C or more compared to the surface temperatures prior to the ACs, with some, but not all, winter cases also producing strong thermal waves penetrating through the snow and ice and reducing sea-ice growth. 

In some ACs, a quasi-axisymmetric LLJ near the top of the boundary layer in the warm sector and then wrapping around the low center as a “bent-back” feature produces the appearance of two successive LLJs with greatly differing wind directions at the MOSAiC site.  The rapid change in wind speed and direction between these LLJ pairs produces a rapid change in the surface stress vector and imparts strong forcing on the sea ice.  During MOSAiC, strong ice deformation, lead formation, etc., was observed during the time periods between the two LLJs.  Hence, these LLJs not only play a role in the atmospheric thermal impacts on sea ice from ACs, but also on the dynamic impacts.

The broad relevance of Arctic Cyclone mesoscale features, such as low-level jets, warm-sector warm-air advection, and cloud macro and microstructure, to the sea-ice thermodynamic and dynamic environment during the MOSAiC field program will be illustrated with MOSAiC case-study observations, including basic meteorological measurements, rawinsondes, ARM remote sensors, surface energy budget measurements, and ice motion measurements.

How to cite: Persson, O., Cox, C., Gallagher, M., Shupe, M., Hutchings, J., Watkins, D., and Perovich, D.: Arctic Cyclone Cloud and Boundary-Layer Features Producing Thermodynamic and Dynamic Impacts on Arctic Sea Ice During MOSAiC, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17554, https://doi.org/10.5194/egusphere-egu23-17554, 2023.

EGU23-314 | ECS | Posters on site | OS1.2

Current feedback in an anticyclonic eddy during the passage of cold frontal systems over the Gulf of Mexico 

Ivonne García Martínez and Julio Sheinbaum Pardo

In autumn and winter, the dynamics and thermodynamics of the anticyclonic eddies detached from the Loop Current in the Gulf of Mexico are strongly influenced by the passage of cold fronts and Northerly winds. In turn, the interaction between the wind and these anticyclonic eddies modulates vertical nutrient fluxes, biomass, and phytoplankton community distribution at mesoscale and sub-mesoscale. In this work, the physical mechanisms of eddy-cold front interactions are analysed based on high-resolution (3 km) numerical simulations of the NEMO (Nucleous for European Modeling of the Ocean) model, contrasting simulations that partially include or not the effect of ocean currents on the wind stress (the so-called current feedback). This analysis is part of a work in progress focused on developing and implementing a high-resolution ocean-atmosphere coupled model for the Gulf of Mexico.

How to cite: García Martínez, I. and Sheinbaum Pardo, J.: Current feedback in an anticyclonic eddy during the passage of cold frontal systems over the Gulf of Mexico, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-314, https://doi.org/10.5194/egusphere-egu23-314, 2023.

EGU23-514 | ECS | Orals | OS1.2

Impact of Bay of Bengal mesoscale eddies on Indian Summer Monsoon Rainfall 

Kiran Vg, Suryachandra A Rao, and Prasanth A Pillai

The northern Indian Ocean serves as an ideal space to study the interaction between Ocean and atmosphere as it accommodates unique and versatile oceanic conditions and the largest monsoonal circulation in the world. The South Asian Monsoon System, the largest of its kind, directly impacts the lives and livelihoods of billions of people living in the Indian Subcontinent. Various factors that influence its strength and characteristics have been studied extensively throughout the years. But, owing to its complex and dynamic nature, a comprehensive understanding and accurate monsoon prediction remain a work in progress. Several Oceanic components that play a part in monsoon processes have been identified. Our study focuses on the Bay of Bengal, distinguished from other oceans due to its highly stratified upper layers. Through this study, we aim to understand the Impact of mesoscale eddies in the Bay of Bengal on the Indian Summer monsoon.

 

The influence of oceanic mesoscale eddies on the circulation and precipitation directly over them has been addressed through different studies after the advent of high-resolution satellite data. The current research focuses on the large-scale influence of the eddies in the Bay of Bengal on the seasonal rainfall during the Indian summer monsoon(ISM). Indices were created using the Okubo Weiss parameter to understand the inter-annual variation of eddies (classified according to polarities and regions of occurrence). These indices correlated with the ISM system suggested that Anticyclonic eddies in the  Western Bay of Bengal strongly influenced wind and rainfall patterns over the monsoon region. The Anticyclonic Eddy activity that peaked during the El Nino years countered the suppression of rainfall by El Nino through enhanced synoptic activity in BoB. The low-pressure system formation and propagation in BoB were found to be stronger in the years having more anticyclonic eddies. The warming created by the warm-core Anticyclonic eddies initiates an Anticyclonic(Clockwise) circulation around the region, which feeds back into the existing oceanic conditions. This coupled Ocean-Atmospheric system mediated through the mesoscale eddies needs to be further analyzed through stand-alone and coupled modeling experiments. Improving the representation of the mesoscale processes in the Northern Indian Ocean can serve as a crucial step in improving the monsoon prediction systems.

How to cite: Vg, K., A Rao, S., and A Pillai, P.: Impact of Bay of Bengal mesoscale eddies on Indian Summer Monsoon Rainfall, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-514, https://doi.org/10.5194/egusphere-egu23-514, 2023.

The Bay of Bengal is a unique tropical ocean basin because of seasonally reversing monsoon
winds; copious freshwater discharge from nearby continental rivers helps barrier layer formation. 
Again, due to its capacity to keep warm SST beyond 28oC, the bay is prone to tropical cyclones
during the transition between two monsoons. Geographically, the basin is land bounded on three 
sides and connected to global oceans through its southern boundary. Vicinity to the equatorial 
The Indian Ocean facilitates the propagation of Kelvin waves through its rim as coastally trapped 
waves. Hence, local and remote forcings make the bay an active basin for brewing mesoscale 
features like eddies. Eddies play a vital role in the bay's upper ocean mesoscale dynamics (O[100s 
Km]). Surface intensified eddies are well studied, but very little is known about subsurface 
circulations. Limited literature reports active subsurface eddy fields in the basin. Observations by 
a RAMA buoy at 90oE, 15oN from 2007 to 2020 shows a thermocline bulge. For about a month, 
this peculiar subsurface feature is characterized by the doming (denting) of the seasonal 
thermocline's upper (lower) part. The bulge is a regular seasonal feature during the winter 
monsoon as denoted by time series analysis of D26 (depth of 26oC isotherm) – D12 (depth of 
26oC isotherm) from RAMA temperature. This research, using a suite of in-situ moored buoy 
observations, satellite altimetry, OSCAR surface current, near-surface ASCAT wind and HYCOM 
re-analysis data, suggests a possible mechanism for the formation of thermocline bulge. Usually, 
it isn't easy to detect a subsurface feature from the sea surface variables like SST or SLA. But 
eddy-wind interactions can lead to the local generation of lens-shaped features in the 
thermocline of a pre-existing surface-intensified anti-cyclonic eddy. Observations show the 
simultaneous development of a surface anti-cyclone off the Irrawaddy delta (hereafter referred 
to as ICAE) and upwelling-favourable winter monsoon winds in the background. The interaction 
of background wind stress with the IACE facilitates the formation of a bulge by doming the 
seasonal thermocline at the eddy core. The thermocline bulge starts its westward journey along 
with the parent eddy due to Rossby wave forcing in December and crosses the RAMA buoy in 
mid-January. Three factors are responsible for a bulged IACE off the Myanmar coast: 1. the arrival 
of coastal Kelvin waves due to intense remote equatorial forcing by Wrytki jets, 2. eddy 
separation from the coast, and 3. Ekman suction (or upwelling) at the centre of IACE due to local 
"eddy-wind" interaction during late fall to winter. The IACE that wraps a bulged thermocline in 
its core is an example of seasonal mode-water ACE or intra-thermocline eddy during the winter, 
typical in higher latitudes but only recently observed in tropical basins like the Bay of Bengal.

How to cite: Kalita, B. K. and Vinayachandran, P.: Role of coastally trapped waves of remote origin and local eddy-wind interaction in the formation of seasonal thermocline bulge in the Bay of Bengal, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-713, https://doi.org/10.5194/egusphere-egu23-713, 2023.

In this study, two years (2021-2022) of High Frequency Radar (HFR) sea surface current data (30 min time resolution) and modelled near-bottom wind data (1 h time resolution) in the Gulf of Trieste (Northern Adriatic Sea) are analysed through a superstatistical (a superposition of different statistics) approach.
 
Three distinct main wind forcing regimes are present in the Gulf of Trieste: Bora, Sirocco and low wind. Bora and Sirocco are strong winds whose characteristics are different: the Bora is a cold wind that blows in gusts from the East-North-East with a short fetch, the Sirocco is a warm wind that blows from the South with a fetch along the entire Adriatic.
 
The currents in the Gulf of Trieste are forced and highly dependent on such variable wind conditions. It results in a succession of different sea current dynamics on different time scales, asking for a superstatistical analysis of the sea surface current data. From the oceanic signal it is possible to extract two different time scales: a relaxation time τ, the time the system spends to reach the local equilibrium and a larger timescale T, the time for which the signal is locally gaussian. This permits extracting a slowly varying β(t) strictly connected to the original time series’ local variance σ2-1. Neither β nor σ2 show well known PDFs and have algebraic tails. Contrary to what one might expect, they show a universal behaviour with respect to the different wind regimes blowing over the Gulf of Trieste.

How to cite: Flora, S., Ursella, L., and Wirth, A.: Superstatistical analysis of sea surface currents in the Gulf of Trieste, measured by HF Radar, and its relation to wind regimes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1063, https://doi.org/10.5194/egusphere-egu23-1063, 2023.

EGU23-1996 | ECS | Posters on site | OS1.2

Resolution sensitivity of tropical turbulent fluxes and precipitation in NorESM models 

Fangxing Tian, Noel Keenlyside, Ingo Bethke, Shunya Koseki, and Fei Li

We evaluated the ¼° model NorESM1.3 in which the well-known “double-ITCZ problem” in the Pacific is mitigated. However, excessive precipitation is produced in the northern branch of the ITCZ. The excessive precipitation is consistent with overevaluated latent heat flux in the tropical ocean. Further analysis shows that in NorESM1.3, the latent heat flux is too sensitive to the surface wind. The increased sensitivity in the ¼° model is partly contributed by small-scale air-sea interaction. The sensitivity of latent heat flux to surface wind, with the scale finer than 2.5°, is up to 40 (Wm-2 / ms-1), which is almost twice of that with scale coarser than 2.5°. This study helps to understand extra air-sea interaction resolved by higher-resolution models, and helps to tune and correct the related model bias.  

How to cite: Tian, F., Keenlyside, N., Bethke, I., Koseki, S., and Li, F.: Resolution sensitivity of tropical turbulent fluxes and precipitation in NorESM models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1996, https://doi.org/10.5194/egusphere-egu23-1996, 2023.

EGU23-2108 | ECS | Posters on site | OS1.2

Impact of Diurnal Warm Layers on Atmospheric Convection 

Radomyra Shevchenko, Cathy Hohenegger, and Mira Schmitt

The phenomenon of sea surface temperature (SST) anomalies created by oceanic diurnal warm layers has been extensively studied for the last decades, but the assessment of its importance for atmospheric convection has come within reach only very recently, thanks to the development of kilometre-scale simulations. We use the output of a global coupled simulation with a 5km horizontal grid spacing and near-surface ocean layers of order O(0.5m) to explicitly resolve both atmospheric convection and diurnal warm layers. As expected, the simulations produce daily SST fluctuations of up to several degrees. The increase of SST during the day causes an abrupt afternoon increase of atmospheric moisture due to enhanced latent heat flux. This increase is followed by an increase in cloud cover and cloud liquid water content. However, although the daily SST amplitude is exaggerated in comparison to reanalysis, the impact on cloud cover and cloud liquid water content only lasts for 5-6 hours. Moreover, the global daily average of these quantities is not influenced by their increase. All in all, we conclude that the global short-timescale impact of diurnal warm layers is negligible.

How to cite: Shevchenko, R., Hohenegger, C., and Schmitt, M.: Impact of Diurnal Warm Layers on Atmospheric Convection, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2108, https://doi.org/10.5194/egusphere-egu23-2108, 2023.

EGU23-2957 | Orals | OS1.2 | Highlight

Extreme air-sea turbulent heat fluxes over the global oceans: determination, implications and mechanisms 

Sergey Gulev, Konstantin Belyaev, and Natalia Tilinina

Extreme surface turbulent heat fluxes affecting convective processes in subpolar ocean regions may amount to 1000-3000 W/m2. Their quantitative estimation is critically important for many oceanographic and meteorological applications. Extreme turbulent fluxes are largely responsible for the vertical mixing in the ocean, especially in the subpolar latitudes where deep convection forms intermediate waters. Over western boundary currents and their extension regions very strong turbulent heat fluxes may result in local responses in the lower atmosphere on time scales from several hours to days and spatial scales from several kilometers to several tens of kilometers. Accurate estimation of extreme turbulent fluxes also strongly relates to the sampling problem especially for the poorly and irregularly sampled regions. Estimation of extreme turbulent fluxes is thus requires knowledge of probability distribution of fluxes. We suggest a concept for determination of extreme surface turbulent heat fluxes based upon theoretical probability distributions, which allow for accurate estimation of extreme fluxes. In this concept the absolute extremeness of surface turbulent fluxes is quantified from the Modified Fisher-Tippett (MFT) distribution. Further we extend MFT distribution to a fractional distribution, quantifying the so-called relative extremeness, representing the fraction of surface flux accumulated during continuous time (e.g. months, season) due to most intense surface fluxes (e.g. the strongest 1% of flux events). We provide explicit form of the fractional distribution and effective algorithms for parameter estimation.

Further we demonstrate applications of the concept for the global ocean using reanalyses and Voluntary Observing Ship (VOS) data for the period 1979 onwards. Global climatologies reveal that the regions with the strongest relative extremeness are not collocated with the strongest mean fluxes. Moreover, interannual variability of the absolute and relative flux extremes is not necessarily correlated with variability of mean fluxes. Growing mean flux may result in both increase and decrease of absolute and relative extremes that has implications for estimates of linear trends which may have different signs for mean fluxes, absolute and relative flux extremes – the situations found for the western boundary currents and major convections sites. Suggested concept has also profound implications for comparative assessments of surface turbulent fluxes from reanalyses (ERA5, ERA-Interim, CFSR, MERRA2, NCEP-DOE, JRA55) and satellite (IFREMER, J-OFURO, HOAPS, SEAFLUX) products. High mean fluxes in some products are not necessarily associated with the strongest absolute and relative extremeness in the same products and vice versa. Also a new concept allows for accurate estimation and minimization of sampling biases in VOS and satellite flux products. Finally, we analyzed the mechanisms responsible for forming extreme surface turbulent fluxes associated with cold air outbreaks in the rear parts of midlatitudinal cyclones under locally high winds and strong air-sea temperature gradients.

How to cite: Gulev, S., Belyaev, K., and Tilinina, N.: Extreme air-sea turbulent heat fluxes over the global oceans: determination, implications and mechanisms, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2957, https://doi.org/10.5194/egusphere-egu23-2957, 2023.

EGU23-3127 | ECS | Orals | OS1.2

Develop an ocean-atmosphere-wave regional coupled model Windwave version 1.0 for predicting wind and wave conditions of the Northwest Pacific Ocean 

Shu Fu, Wenyu Huang, Runqing Lv, Zifan Yang, Tianpei Qiu, Danyi Sun, Jingjia Luo, Xiaomeng Huang, Haohuan Fu, Yong Luo, and Bin Wang

A new ocean-atmosphere-wave regional coupled model named Windwave version 1.0 for simulating and predicting winds and waves has been developed for the Northwest Pacific Ocean. In particular, the global-to-regional nesting technique is adopted for the ocean component to alleviate the bias due to the inconsistency in the lateral boundary. This paper is devoted to describing the coupling details of Windwave and the initialization scheme and assessing its basic performance, especially in predicting surface winds and significant wave heights (SWH) on the weather timescale. The control experiment set contains 31 experiments for August 2020, with seven typhoons passing through the Northwest Pacific. Each experiment starts at 0:00 am UTC of each day and runs for three days. Experiment results show that the new coupled model performs well in predicting surface winds, SWH, surface air temperature, and sea surface temperature on the weather timescale. In particular, the Root Mean Square Errors (RMSEs) of surface winds at 10 m height over the Northwest Pacific of the control experiment are 1.82 m s-1, 2.22 m s-1, and 2.59 m s-1, respectively, at lead times of 24 h, 48 h, and 72 h. Meanwhile, the RMSEs of SWH at lead times of 24 h, 48 h, and 72 h are 0.39 m, 0.43 m, and 0.51 m. In addition, we have explored the impacts of the different sea surface aerodynamic roughness parameterization schemes on predicting surface winds and SWH. In total, five different sea surface aerodynamic roughness parameterization schemes are adopted, corresponding to one control set and four sensitivity sets of experiments. Under normal conditions, the sea surface aerodynamic roughness parameterization scheme considering the effects of wind-wave direction tends to perform better for winds and waves, while that depending on wave age and SWH tends to perform worse. Under extreme wind and wave conditions, the schemes considering the effects of wind-wave direction and that considering wave age and peak wave length have better performance. These findings can provide new insights for developing a more advanced sea surface aerodynamic roughness parameterization scheme.

How to cite: Fu, S., Huang, W., Lv, R., Yang, Z., Qiu, T., Sun, D., Luo, J., Huang, X., Fu, H., Luo, Y., and Wang, B.: Develop an ocean-atmosphere-wave regional coupled model Windwave version 1.0 for predicting wind and wave conditions of the Northwest Pacific Ocean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3127, https://doi.org/10.5194/egusphere-egu23-3127, 2023.

EGU23-3608 | Orals | OS1.2 | Highlight

Lessons learned from the EUREC4A-OA experiment on the impact of ocean small scales on air-sea interactions in the Northwest Tropical Atlantic 

Sabrina Speich, Johannes Karstensen, Gilles Reverdin, Léa Olivier, Pablo Fernandez, Pierre L'Hégaret, Solange Coadou, Rémi Laxenaire, Dongxiao Zhang, Chelle Gentemann, Peter Landschutzer, Jacqueline Boutin, Hugo Bellenger, Claudia Pasquero, Agostino Meroni, Matteo Borgnino, Claudia Acquistapace, and Laurent Bopp

EUREC4A-OA is a large international project, connecting experts of ocean and atmosphere observations and modelling to enhance the understanding of key ocean and air-sea processes at the and to improve the skill of forecasts and future projections.

The core of EUREC4A-OA has been a one-month (Jan/Feb 2020) field study in the western tropical North Atlantic Ocean where high-resolution, synchronized observational data have been collected using cutting-edge technology on ships, airplanes and autonomous vehicles. EUREC4A-OA investigates heat, momentum, water and CO2 transport within the ocean and exchanges across the air/sea interface using innovative high-resolution ocean observations and a hierarchy of numerical simulations. EUREC4A-OA focuses on ocean dynamics at the small-scale (0.1–100 km) and related atmospheric boundary layer processes. EUREC4A-OA is centered on the tropics where the primary external time scale affecting air-sea exchange is the diurnal cycle. However, the internal ocean and atmosphere dynamics convolute the diurnal, synoptic, seasonal and longer time scales to climate variability.

The talk will present some of the results we obtained so far from the observations collected during the field experiment and from numerical simulations. The analyses carried out revealed with unprecedented detail the particular characteristics of the ocean small-scale dynamics, enlightening that such scales are also very active in the tropical regions and not only over the mid and higher latitudes ocean.  Observations and models also unveil that the ocean small scales is important in contributing to the exchanges of heat, freshwater and CO2 between the ocean and the atmosphere. Moreover, the evaluation of the intensity of the coupling between the ocean and the atmosphere assessed from data and high-resolution simulations show that they are very important and intimately linked with the 3D structure of the small-scale ocean dynamics. The project has also provided preliminary results in terms of parametrization of different processes influencing the ocean and atmosphere exchanges that have been uncovered by the EUREC4A-OA field experiment. Notably a better representation of the small-scale freshwater patches due to precipitation has been introduced in the French Earth-System model that improves the overall simulations of air-sea interactions and clouds. A similar parametrization is now been introduced to take into account these physical processes in air-sea fluxes of CO2.

How to cite: Speich, S., Karstensen, J., Reverdin, G., Olivier, L., Fernandez, P., L'Hégaret, P., Coadou, S., Laxenaire, R., Zhang, D., Gentemann, C., Landschutzer, P., Boutin, J., Bellenger, H., Pasquero, C., Meroni, A., Borgnino, M., Acquistapace, C., and Bopp, L.: Lessons learned from the EUREC4A-OA experiment on the impact of ocean small scales on air-sea interactions in the Northwest Tropical Atlantic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3608, https://doi.org/10.5194/egusphere-egu23-3608, 2023.

EGU23-3693 | Orals | OS1.2

Seasonal buildup and downward transfer of Warm Pool heat content by wind-driven ocean mixing 

Noel Gutierrez Brizuela, Yi Xia, Shang-Ping Xie, Matthew Alford, and James Moum

Ocean heat stored in the Western Pacific Warm Pool (WPWP) helps drive some of the foremost modes of weather and climate variability including ENSO, Intraseasonal Oscillations, and tropical cyclones. To understand the associated coupled mechanisms that regulate ocean temperature, we use reanalysis and a novel moored microstructure dataset yielding estimates of the turbulent ocean heat flux (Jq(z)) to describe how WPWP mixing is regulated by seasonal, intraseasonal, and synoptic-scale atmospheric disturbances. It is argued that observed variations in Jq(z) impact seasonal-to-synoptic trends in SST and mixed-layer depth. Jq(z) is weakest during Spring (dry season), when heat fluxes into the ocean (Qnet > 0) create a shallow mixed layer (ML) of warm water that lays undisturbed atop the seasonal thermocline. In the Summer, westerly winds associated with the Asian Monsoon create favorable conditions for tropical depression-like (TD-like) storms, which in turn cause episodic spikes in Jq(z) that gradually deepen the ML and momentarily cool sea surface temperature (SST) while the background SST continues to rise. Towards the end of the summer, SST at our mooring was greater than 30.7 °C but rapidly dropped and stabilized below 29.5 °C after a strong pulse of the Madden-Julian Oscillation (MJO) cooled the upper ocean and deepened the ML for almost 15 days in a row. Enhanced upper ocean mixing continued to be episodic throughout the Fall as TD-like storms and intraseasonal disturbances moved over the mooring site. Mixing remained high throughout the Winter, when cold outbreaks forced the upper ocean at high frequencies and mean convective cooling (Qnet < 0) further contributed to mixing. A similar seasonality is observed at the thermocline level, where Jq(z) is enhanced by storm-driven near-inertial internal waves (NIWs) whose power peaks between Fall and Winter. While intraseasonal wind bursts had the greatest impact on near-surface mixing, synoptic disturbances generated greater-amplitude NIWs and thus had a greater potential to mix temperature gradients in the permanent thermocline. Lastly, we use reanalysis data to argue that storm-driven mixing shapes interannual relations between SST, storm activity, and the Asian Monsoon. 

How to cite: Gutierrez Brizuela, N., Xia, Y., Xie, S.-P., Alford, M., and Moum, J.: Seasonal buildup and downward transfer of Warm Pool heat content by wind-driven ocean mixing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3693, https://doi.org/10.5194/egusphere-egu23-3693, 2023.

Reanalysis and current generation global coupled climate models have shown a dominant role of atmospheric forcing for the ocean such as stronger winds that increase turbulent heat flux and consequently cools sea surface temperatures (SSTs) . While satellite observations and eddy-resolving global coupled climate models have additionally shown clear imprints of mesoscale ocean forcing on the atmosphere, such as warm SST anomalies that can destabilise the overlying atmosphere and enhance surface winds by transferring momentum from aloft to the surface (vertical mixing mechanism; VMM). With winds blowing along downwind or crosswind SST gradients, this can subsequently induce wind stress divergence or curl respectively, particularly over mesoscale ocean features. The dominance of forcing from either atmosphere or ocean indicate a spatial scale dependency for the coupling variability of air-sea interactions.
 
Using a global coupled 5-km ICON-ESM simulation, we derive a global distribution map of the air-sea coupling associated with the VMM, and investigate the spatial and temporal scale dependency of the vertical mixing mechanism. Choosing various regions over the ocean, we evaluate the frequency-wavenumber cross-spectra between downwind SST gradients and windstress divergence in order to identify the dominant temporal and spatial scales between them. For example, we found that over the tropical Pacific, such interactions are prevalent on spatial scales of about 300-3000km and longer than 10-days timescale, while over the Gulf stream region, they are dominant at scales of roughly 100-1000km and longer than 5-days timescale. This is the first time that the dominant spatial and temporal scales for the vertical mixing mechanism in various regions of the world's ocean is quantified. 

How to cite: Putrasahan, D. and von Storch, J.-S.: Geographical distribution and spatio-temporal scale dependence of air-sea coupling via the vertical mixing mechanism, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4685, https://doi.org/10.5194/egusphere-egu23-4685, 2023.

EGU23-4800 | ECS | Posters on site | OS1.2

Intense atmospheric frontogenesis by air-sea interaction captured at Ieodo Ocean Research Station during Typhoon Lingling (2019) 

Sinil Yang, Il-Ju Moon, Hyo-Jun Bae, Baek-Min Kim, Do-Seong Byun, and Hwa-Young Lee

The Ieodo Ocean Research Station (Ieodo ORS) is a fixed marine observation platform at the boundary of the Yellow and East China Seas. In 2019, a Category 4 Typhoon Lingling passed by the Ieodo ORS very closely. At that time, the Ieodo ORS observed Sea Surface Temperature (SST) cooling of 4.5°C by vertical mixing and negative turbulent heat flux (i.e., the sum of sensible and latent heat fluxes) due to the SST cooling. In this study, uncoupled and coupled simulations were conducted to examine the role of air-sea interactions in changes in atmospheric frontogenesis around the typhoon passage. In the coupled simulation, SST cooling up to 6°C occurred over the dangerous semicircle due to vertical mixing induced by wind stress. Strong wind stress also enhanced the SST gradient and, therefore, contributed to the formation of a steeper atmospheric frontal zone. Moreover, the comparison with reliable datasets supports the physical linkage between SST cooling and atmospheric frontogenesis by utilizing the meridional theta-e gradient and moisture convergence zone. Therefore, we hope to improve our understanding of atmospheric frontogenesis by air-sea coupling processes in developing a coupled atmosphere-ocean modeling system from the simulation results.

How to cite: Yang, S., Moon, I.-J., Bae, H.-J., Kim, B.-M., Byun, D.-S., and Lee, H.-Y.: Intense atmospheric frontogenesis by air-sea interaction captured at Ieodo Ocean Research Station during Typhoon Lingling (2019), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4800, https://doi.org/10.5194/egusphere-egu23-4800, 2023.

EGU23-4940 | Orals | OS1.2

The rate of information transfer as a measure of ocean-atmosphere interactions 

David Docquier, Stéphane Vannitsem, Alessio Bellucci, and Claude Frankignoul

Exchanges of momentum, energy and mass between the ocean and atmosphere are of large importance in regulating the climate system. Here we apply the Liang-Kleeman rate of information transfer to quantify interactions between the upper ocean and lower atmosphere over the period 1988-2017 at monthly time scale in two different case studies. In the first case study, we investigate dynamical dependencies between sea-surface temperature (SST), SST tendency and turbulent heat flux in satellite observations. We find a strong two-way influence between SST or SST tendency and turbulent heat flux in many regions of the world, with largest values in eastern tropical Pacific and Atlantic oceans, as well as in western boundary currents. The total number of regions with a significant influence of turbulent heat flux on SST and SST tendency is reduced when considering the three variables, suggesting an overall stronger ocean influence compared to the atmosphere. In the second case study, we focus on the influence of ocean heat transport convergence (dynamical influence) and net surface heat flux (thermodynamical influence) on upper ocean heat content tendency in three global climate models with at least two different ocean resolutions. We find that low-resolution model configurations (1° in the ocean) show a much larger number of regions with a significant dynamical influence compared to high-resolution model configurations. The reason for the large difference in dynamical influence between low and high resolutions partly comes from the spatial distribution of ocean velocity field, which displays a larger spatial variability at high resolution.

How to cite: Docquier, D., Vannitsem, S., Bellucci, A., and Frankignoul, C.: The rate of information transfer as a measure of ocean-atmosphere interactions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4940, https://doi.org/10.5194/egusphere-egu23-4940, 2023.

EGU23-5161 | ECS | Orals | OS1.2

Partial control of the Gulf of Mexico dynamics by the current feedback to the atmosphere 

Marco Larrañaga, Lionel Renault, and Julien Jouanno

The feedback of ocean surface currents to the atmosphere (CFB) has been shown to correct long-lasting biases in the representation of ocean dynamics by providing an unambiguous energy sink mechanism. However, CFB effects on the Gulf of Mexico oceanic circulation, mainly dominated by the Loop Current and large anticyclonic eddies that shed from it), remain unknown. Here, twin ocean-atmosphere eddy-rich coupled simulations, with and without CFB, are performed over 24 years (1993-2016) to assess to which extent CFB modulates the dynamics of the Gulf of Mexico. We show that CFB damps the mesoscale activity by roughly 20% over the Gulf of Mexico through the eddy killing mechanism and the associated transfer of momentum from mesoscale currents to the atmosphere, but also by modifying the production of eddy kinetic energy via barotropic and baroclinic instabilities. This energy adjustment results in increasing the mean Loop Current penetration into the Gulf of Mexico and plays a key role in determining the shedding of Loop Current Eddy and their subsequent preferential trajectories and properties.

How to cite: Larrañaga, M., Renault, L., and Jouanno, J.: Partial control of the Gulf of Mexico dynamics by the current feedback to the atmosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5161, https://doi.org/10.5194/egusphere-egu23-5161, 2023.

EGU23-7362 | ECS | Orals | OS1.2

A Preliminary Forecast Study of the North Indian Ocean Tropical Cyclones Using a Coupled Atmosphere-Ocean Model 

Aref Farhangmehr, Sarmad Ghader, Abbas Ali Ali Akbar Bidokhti, and Zahra Ranji

Tropical cyclones (TCs) are severe weather marvels, occur in warm tropical waters. These phenomena are among the most influential atmospheric-oceanic events in subtropics regions as the northern part of the Indian Ocean, affecting the Arabian Sea and the Oman Sea, which often cause severe damage to the coastal areas. The interaction between the atmosphere and the upper ocean plays an important role in the structure of TCs, in which successful connections between ocean circulations and the intensity and track of TCs have been identified. TCs derive their energy primarily from the release of latent heat through evaporation and sea spraying in the atmosphere boundary layer. This implies that the presence of a moisture source, with sufficiently warm sea surface temperature (frequently above 26°C) is required to sustain the flux of moisture from the ocean to the atmosphere. The most visible effect of TC passage is the cooling of the sea surface temperature (SST) as the response of the ocean mixed layer (OML) temperature. This decrease in SST has a negative feedback on the intensity of TCs, as it suppresses the heat exchange flux between the atmosphere and the ocean, consequently it can affect the TC track.

To investigate the effect of the temperature field on TCs structure, TC Shaheen (2021) with unusual track and entry into the Gulf of Oman is studied. In this regard, Weather Research and Forecasting (WRF) model was used with two different configurations. First, WRF was ran standalone and SST field was only adopted from global models as initial conditions and were not updated during the simulation. Then, as the second configuration, WRF model was coupled with an ocean finite volume model and the SST field was updated online during the simulation. The initial conditions of the ocean temperature, salinity and velocity field were taken from GOFS 3.1 global reanalysis product from the HYCOM Consortium. Primary result for the selected event implies that SST correction during TC simulation with WRF improves air-sea heat flux and has a pronounced effect on the TCs’ intensity and track predictions. Cold wake underside of the TC led to a remarkable heat flux loss from ocean surface into the storm. Hence, the TC size is reduced and the maximum wind speed of the storm is intensified.

How to cite: Farhangmehr, A., Ghader, S., Ali Akbar Bidokhti, A. A., and Ranji, Z.: A Preliminary Forecast Study of the North Indian Ocean Tropical Cyclones Using a Coupled Atmosphere-Ocean Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7362, https://doi.org/10.5194/egusphere-egu23-7362, 2023.

EGU23-8166 | Orals | OS1.2

Observing the Air-Sea Transition Zone using Combined Uncrewed Systems and Other Conventional Platforms 

Chidong Zhang and the Saildrone Hurricane Observations Mission Team

Full understanding of air-sea interaction requires observations not only at the air-sea interface but also through the entire air-sea transition zone (the upper ocean, air-sea interface, and marine atmospheric boundary layer as a single identity). Our capabilities of observing collocated and simultaneous profiles through the entire column of the air-sea transition zone are currently limited. This study explores the feasibility of using combined uncrewed robotic systems in conjunction with conventional platforms to provide such collocated and simultaneous profiles of the air-sea transition zone. An introduction is given to experimental deployments of uncrewed surface vehicles (saildrones), underwater vehicles (gliders), aerial vehicles in coordination with profiling floats, surface drifters, airborne dropsondes, and moored buoys to observe the air-sea transition zone. Based on the preliminary results and lessons learned, a vision of potential capabilities of observing the air-sea transition zone in the future using combined uncrewed systems is offered.

How to cite: Zhang, C. and the Saildrone Hurricane Observations Mission Team: Observing the Air-Sea Transition Zone using Combined Uncrewed Systems and Other Conventional Platforms, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8166, https://doi.org/10.5194/egusphere-egu23-8166, 2023.

EGU23-8293 | Orals | OS1.2

Beyond Mesoscale off Mauretania 

Heiner Dietze, Ulrike Löptien, Robinson Hordoir, and Matthias Renz

Hitherto unresolved oceanic sub-mesoscale variability may retard air-sea exchange of heat and carbon in contemporary IPCC-type model projections. Here, we set out to put this hypothesis to the test in the Atlantic in a region off Mauretania that is renown for its complex coastal dynamics. Results from a suite of coupled ocean-circulation biogeochemical models suggest that the oceanic bottleneck between the atmosphere and the vast abyssal stocks of heat and carbon is relatively insensitive in the range from mesoscale and to sub-mesoscale resolution. More specifically we find that the sensitivity of effective vertical mixing to changes in spatial resolution is comparable to infamous uncertainties associated with contemporary numerical algorithms.

How to cite: Dietze, H., Löptien, U., Hordoir, R., and Renz, M.: Beyond Mesoscale off Mauretania, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8293, https://doi.org/10.5194/egusphere-egu23-8293, 2023.

EGU23-10356 | ECS | Posters on site | OS1.2 | Highlight

The Competing Forces of Hurricane-Induced Ocean Cooling 

Lev Looney and Gregory Foltz

It is known that oceanic conditions can play a crucial role in the intensification of tropical cyclones (TCs) when atmospheric conditions are conducive. However, the relative roles of ocean temperature and salinity stratification on ocean mixing and TC-induced sea surface temperature (SST) cooling are unclear. Temperature stratification has competing effects on cooling from ocean mixing: stronger stratification leads to cooler water near the surface which can enhance SST cooling (thermodynamic effect), yet it also leads to resistance to vertical mixing due to a stronger density gradient and increased static stability (mixing effect). In contrast, salinity stratification almost always acts to reduce mixing and cooling. To investigate the mechanisms that control the amount of ocean cooling under a storm, we use a one-dimensional mixed layer model, initialized with different oceanic profiles and forced with cyclones of various intensities, translation speeds, and sizes. We then compare output from the mixed layer model with observations. Results consistently show that the thermodynamic effect (changes in vertical temperature gradient with density gradient held constant) is 2-3 times that of the mixing effect (changes in density stratification with temperature stratification held constant). Furthermore, we find that translation speed and storm size are the two most important factors for SST cooling, followed by temperature stratification, maximum wind speed, and mixed layer depth, respectively. These results emphasize the importance of temperature stratification over most of the tropical cyclone basins and the often overlooked role of storm size.

How to cite: Looney, L. and Foltz, G.: The Competing Forces of Hurricane-Induced Ocean Cooling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10356, https://doi.org/10.5194/egusphere-egu23-10356, 2023.

EGU23-11795 | ECS | Orals | OS1.2

Atmospheric and Oceanic Responses to Surface Current Coupling near the Kuroshio Current 

Ajin Cho, Hajoon Song, and Hyodae Seo

The so-called frontal-scale air-sea interaction describing the atmospheric responses to oceanic fronts has been mainly discussed in the context of interactions between sea surface temperature and surface winds. The ocean current also influences the surface winds, which can significantly affect the atmosphere, especially in regions of energetic ocean currents and mesoscale activities as in the western boundary current systems. This study uses an atmosphere-ocean coupled model to analyze how the Kuroshio Current affects the momentum and turbulent heat fluxes and the atmospheric boundary layer and how these responses feed back to the ocean and atmosphere in this region. The ocean current coupling influences the path of Kuroshio extension and the eddy activities by mechanical and thermal current feedbacks. Mechanical current feedback reduces momentum flux and damps eddy kinetic energy (EKE) by reducing wind work as expected. On the other hand, the thermal current feedback associated with turbulent heat fluxes injects EKE by baroclinic energy conversion. Overall, the shift of Kuroshio Current and the change of eddy activities impact the region of strong turbulent heat release to the atmosphere, which can eventually trigger changes in weather systems.

How to cite: Cho, A., Song, H., and Seo, H.: Atmospheric and Oceanic Responses to Surface Current Coupling near the Kuroshio Current, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11795, https://doi.org/10.5194/egusphere-egu23-11795, 2023.

EGU23-13039 | ECS | Orals | OS1.2

Mesoscale and Submesoscale air-sea interactions in the lower North Atlantic trades 

Carlos Conejero, Lionel Renault, and Hervé Giordani

In the past decades, numerous studies have shown that oceanic mesoscale activity, over scales of O(50–250) km, has a strong influence on the atmosphere through both the Thermal FeedBack (TFB) and the Current FeedBack (CFB). However, at the submesoscale, over scales of O(1–10) km, both TFB and CFB are not well understood, mainly due to technical barriers (observation and simulation). Here, a realistic high-resolution coupled oceanic model (dx = 1 km), including tidal forcing and river discharge, and atmospheric (dx = 2 km) model in the lower North Atlantic trades region over a period of 1-year (from July 2019 to June 2020) is used to assess the atmospheric response to submesoscale processes. We used classic coupling coefcients between the ocean and the atmosphere to quantify spatial and temporal variabilities of the TFB and CFB coupling.

Our results show that, similar to oceanic mesoscale activity, at the submesoscale, both TFB and CFB have an imprint on the low-level wind, surface stress and turbulent heat fluxes. On the one hand, the linear relationship between surface wind (stress) curl and surface current vorticity existing at the mesoscale regime is also supported at the submesoscale. At submesoscale, CFB, as at the mesoscale, is acting as a sink of energy from the ocean to the atmosphere, acting as an submesoscale eddy killer. Furthermore, the magnitude of surface stress curl introduced by submesoscale processes is greater by ~17 % than that presented by mesoscale processes, which is explained by a reduction of the wind response by ~55 %. On the other hand, the linear relationship between wind stress magnitude, or latent heat flux, and sea surface temperature (SST) anomalies, widely present at the mesoscale, is also found at the submesoscale. Similar results are found when considering wind stress curl/divergence and crosswind/downwind SST gradients coupling coefficients. However, the magnitude of the corresponding TFB coupling at submesoscale is reduced by ~30 % with respect to those at mesoscale.

Overall, our results emphasize the significant impact of both oceanic currents and strong SST fronts on the local wind/stress and latent heat flux response at the submesoscale regime.

How to cite: Conejero, C., Renault, L., and Giordani, H.: Mesoscale and Submesoscale air-sea interactions in the lower North Atlantic trades, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13039, https://doi.org/10.5194/egusphere-egu23-13039, 2023.

EGU23-14929 | ECS | Posters on site | OS1.2

Overview of aerosol observations from the Marion Dufresne Atmospheric Program – Indian Ocean (MAP-IO) program 

Meredith Dournaux, Pierre Tulet, Joris Pianezze, Karine Sellegri, and Jérôme Brioude

The study of marine aerosols size distribution and cloud condensation nuclei (CCN) properties is of major interest as they influence clouds life and clouds radiative properties, particularly in the remote ocean which remains poorly documented. Several short campaigns focusing on specific regions as phytoplankton bloom regions, pristine regions or remote areas influenced by continental air masses took place to address this issue. However, long sampling periods targeting different in-situ conditions had not been realized.

In this context, the MAP-IO program was launched with the aim of providing a large new set of marine aerosol observations (size distribution from 10 nm to 10 µm and CCN properties) on different sea state and meteorological conditions. Thus, the Marion Dufresne vessel has been equipped with a set of various instruments described in Tulet et al. (in preparation) or on the website www.mapio.re. Two years after the launch of the program, we now have aerosol observations (about 200 days) over an area covering 50 ° of latitudes and extending from the Tropics to the upper Southern Ocean. 

These measurements were first used to investigate the size distribution and CCN variability of marine aerosols according to local conditions (sea states and wind speed).The results highlight that at the lowest latitudes (south of 50 °S) the minimum concentration of CCN tends to increase when the wind speed exceeds approximately 12 m s-1, which is consistent with the literature as sea salt  emissions are mechanically driven by local conditions and tend to be predominant from 10 m s-1. .When analyzing the size distributions of aerosols according to the wind speed during a 5-day storm that occurred in the Southern Ocean, we found that: (1) the number of particles with a diameter less than 500 nm is predominant and stable over the full range of wind speeds (4 to 33 m s-1), (2) the number of aerosols with diameter greater than 500 nm remains low under 10 m s-1 and increases from 10 m s-1 to 33 m s-1 to finally reach the concentration of the particles with diameter less than 500 nm at 33 m s-1. 

Taking this first analysis into account, further work will focus on average size distributions per region, season, origin of air masses (from simulated FLEXPART back trajectories) and wind speed conditions. Analysis of these distributions is unique due to the size of the database, the variability of regions encountered and knowing that the measurements were carried out with the same experimental device. 

 Finally, to deepen the study, the activation diameter of marine aerosols will be determined and the hygroscopicity parameter Kappa-Köhler will be calculated (Petters and Kreidenweis, 2007) in this case to distinguish sea salts (Kappa~1.2) from organic matter (0.01<Kappa<0.5).

How to cite: Dournaux, M., Tulet, P., Pianezze, J., Sellegri, K., and Brioude, J.: Overview of aerosol observations from the Marion Dufresne Atmospheric Program – Indian Ocean (MAP-IO) program, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14929, https://doi.org/10.5194/egusphere-egu23-14929, 2023.

EGU23-15444 | ECS | Posters virtual | OS1.2

Surface attached vortices as a proxy for gas transfer in free-surface turbulent flow 

Omer Babiker, Ivar Bjerkebæk, Anqing Xuan, Lian Shen, and Simen A Ellingsen

Gas transfer between ocean and atmosphere is largely governed by the turbulence in the topmost centimetres beneath the free surface. It has been frequently observed that areas of strong positive divergence of the surface-tangential velocity field correspond to efficient surface renewal and consequently increased transfer of gas across the interface. Patches of strong positive surface divergence occur in the form of intermittent upwelling events visible as ``boils'' on the surface.

It has been qualitatively observed that surface-attached ``bathtub'' vortices tend to appear at the edges of upwelling boils, hence a correlation between the density of these long-lived vortices and average surface divergence might be expected. Surface-attached vortices leave imprints on the surface which are particularly simple to detect: they live for a long time compared to turbulence turn-over, and their imprints are in the form of nearly circular dimples.

From direct numerical simulations, we show that a very high correlation exists between the time-dependent number of surface-attached vortices and the mean square of the surface divergence. A correlation coefficient of over 0.9 is found, where peaks in the number of vortices occur a little time after the peak in surface divergence, approximately half of the integral timescale of the bulk turbulence.

We use a newly developed method whereby the surface-attached vortices are identified with high precision and accuracy from their surface imprint only. Thus, observation of surface dimples can act as a proxy for surface divergence, with the prospect of remote sensing of gas transfer rate.

How to cite: Babiker, O., Bjerkebæk, I., Xuan, A., Shen, L., and Ellingsen, S. A.: Surface attached vortices as a proxy for gas transfer in free-surface turbulent flow, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15444, https://doi.org/10.5194/egusphere-egu23-15444, 2023.

EGU23-16033 | Posters on site | OS1.2

Investigating the Impact of Sea Waves on Offshore Wind Simulation: A Study Using the WRF Model 

Mohammadreza Mohammadpour Penchah, Mostafa Bakhoday Paskyabi, and Hai Bui

Previous studies showed that interaction between the atmosphere and sea is very important for simulating offshore wind, due to the effects of sea waves on momentum, mass and energy exchanges. In numerical weather prediction models, this effect is typically represented by a parameter known as roughness length. However, many atmospheric models do not take into account the impact of waves on roughness length over the sea.

In this study, we aimed to investigate the effects of waves on offshore wind simulation by applying some new roughness length formula in Weather Research and Forecasting (WRF) to consider wave characteristics in roughness length calculation. The simulations were compared with observations during some cases of misalignment and alignment of wind and wave directions at FINO1 station. We compared wind speed and wind power density of the simulated and observed data using met mast and lidar data.

How to cite: Mohammadpour Penchah, M., Bakhoday Paskyabi, M., and Bui, H.: Investigating the Impact of Sea Waves on Offshore Wind Simulation: A Study Using the WRF Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16033, https://doi.org/10.5194/egusphere-egu23-16033, 2023.

EGU23-16379 | Posters on site | OS1.2

The diurnal warm layer and its consequences for the upper ocean: from EUREC4A-OA observations and the global coupled ICON-ESM 

Florian Schuette, Diego Lange, Dian Putrasahan, Ruben Carrasco, Pierre L'Herguet, Dongxiao Zhang, Sabrina Speich, Jin-Song von Storch, and Johannes Karstensen

The uppermost 0-20m depth of the ocean within the mixed layer (ML) were investigated on diurnal scales using data collected during the EUREC4A campaign in the western tropical Atlantic. The results are compared against data from the global coupled Earth System model ICON. In both datasets is the diurnal impulse generator the penetrating shortwave solar radiation, heating the first meters of the ocean. During day on top of the ML a stably stratified near-surface layer, called the diurnal warm layer (DWL), can be formed. Depending on the wind conditions or the amount of incoming solar radiation the depth of such a DWL can reach from several centimeters to tens of meters. Associated to the stable stratification (and the wind) shear is produced which propagates down with time. At that point, the model and the observations start to differ. Using high-resolution current measurements of ADCP’s mounted on saildrones the detailed structure of the descending shear layer is observed. The cycle of shear instability leads the diurnal mixing cycle, typically by 2–3 h, consistent with the time needed for instabilities to grow and break (observed by microstructure measurements). In the morning, the turbulence decays and the upper ocean restratifies. At this point, wind accelerates the near-surface flow to form a new unstable shear layer, and the cycle begins again. Since the study area is located around 15°N, the excited layers are affected by the Coriolis force, which causes the descending shear layer to rotate around the inertial frequency of 1.8 days. Compared to the global coupled earth system model, these processes cannot be represented in such detail here. This leads to lower shear (and also mixing) at the different time and depth. Different model configurations show that even small differences in the upper 20m of the ocean, such as those observed, can lead to quite large changes in the model, e.g., a different strength of the ocean current system down to 1000m depth.

How to cite: Schuette, F., Lange, D., Putrasahan, D., Carrasco, R., L'Herguet, P., Zhang, D., Speich, S., von Storch, J.-S., and Karstensen, J.: The diurnal warm layer and its consequences for the upper ocean: from EUREC4A-OA observations and the global coupled ICON-ESM, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16379, https://doi.org/10.5194/egusphere-egu23-16379, 2023.

EGU23-16810 | ECS | Posters on site | OS1.2

Comparison of ECMWF-ERA5 turbulent Air-Sea Fluxes and related environmental variables to data from to the OCARINA wave following platforms 

Saïd Benjeddou, Denis Denis Bourras, Boris Dewitte, Christopher Luneau, and Philippe Fraunié

The ECMWF-ERA5 reanalysis is amongst the best products to access the hourly state and trend of the global Atmosphere, Wave field, and Ocean over several decades, for many scientists and in many studies. In the proposed presentation, we will compare the turbulent momentum and heat exchange flux values output from the reanalysis to corresponding estimates that were not assimilated in the model. Those estimates were computed from data collected with a wave following platform that was deployed in several basins since 2012, including the Chile-Peru upwelling region in 2014. Not only the fluxes and the bulk variables will be statistically compared, but the focus will also be laid on the sensitivity of the results to the surface current, to the proximity of coast and, where it applies, to the direction of the wind (onshore, offshore and parallel to the coast).

How to cite: Benjeddou, S., Denis Bourras, D., Dewitte, B., Luneau, C., and Fraunié, P.: Comparison of ECMWF-ERA5 turbulent Air-Sea Fluxes and related environmental variables to data from to the OCARINA wave following platforms, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16810, https://doi.org/10.5194/egusphere-egu23-16810, 2023.

EGU23-16883 * | ECS | Orals | OS1.2 | Highlight

Identifying an Evaporative Thermal Refugium for the Preservation of Coral Reefs in a Warming World—The Gulf of Eilat (Aqaba) 

Shai Abir, Hamish A. McGowan, Yonathan Shaked, and Nadav Lensky

Coral bleaching events are more frequent and severe as global temperatures rise and marine heat waves are more frequent. However, quantifying the surface energy fluxes in coral reefs at various geoclimatic regions and the mechanisms by which the air-water interactions regulate water temperature is rare. We measure surface energy fluxes over coral reefs using Eddy Covariance towers in two contrasting geo-climatic regions: The typical setup of humid/tropical coral reefs (Heron Reef, Great Barrier Reef, Australia) and the rarer desert coral reef (Golf of Eilat, Israel). We analyze how the surface heat fluxes regulate the temperature of shallow coral reef environments. We show that in the desert reefs, the dry air overlying the shallow coral reef results in extremely high evaporation rates which in turn results in extensive cooling of the water. In humid/tropical reefs, evaporation is suppressed by humidity and is limited in the ability to offset the heating of the water. The extreme difference in evaporative cooling in desert versus tropical reefs is key in the response to marine heat waves. Marine heat waves which impose thermal stress on corals are a result of synoptic-scale circulation variations which suppress evaporation and increase heating. The most severe marine heatwave ever measured at the Gulf of Eilat (August 2021) was found to be caused by low evaporation rates, which resulted from synoptic circulation with weak winds and high humidity. After the onset of water temperature rise and the return of the dry winds, evaporation instantly cooled the water overlying the corals- relieving potential stress. Whereas, at the humid/tropical Heron Reef (Great Barrier Reef, Australia) evaporation solely is unable to reduce the high water temperature and therefore coral heat induce stress events are inevitably longer and more frequent. We conclude that evaporative cooling is a key mechanism protecting coral reefs located in deserts from extreme high-water temperatures, thereby representing possible thermal refugium for corals against background global warming.

How to cite: Abir, S., McGowan, H. A., Shaked, Y., and Lensky, N.: Identifying an Evaporative Thermal Refugium for the Preservation of Coral Reefs in a Warming World—The Gulf of Eilat (Aqaba), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16883, https://doi.org/10.5194/egusphere-egu23-16883, 2023.

EGU23-791 | ECS | Posters virtual | AS2.4

Response of the atmospheric boundary layer to cold pools of thunderstorms at rural location, Gadanki 

Donali Gogoi and T.Narayana Rao

The thunderstorms produce cold pools that spread horizontally few kms from the location of cumulonimbus clouds. They are often seen during the noon-evening period. The atmosphere and several surface meteorological parameters show a sudden change during the passage of these cold pools. An earlier study has noted that 85% of gust events observed at Gadanki, India are associated with these cold pools (and thunderstorms). Cold Pools are mainly found to occur in the months of April, May and June during 11 years’ time from 2010 -2021 over Gadanki. A total of 84 cases of cold pools were seen during this period with highest number of cold pools occurring in the noon-evening time 3 pm- 4 pm, followed by the time intervals of 2 pm- 3 pm and 4 pm- 5 pm. The atmospheric variables (temperature, wind speed, pressure and humidity) are used to determine the onset of a cold pool using meteorological tower data. It is interesting to note that we have observed cold pools with heavy rainfall and cold pool events with drastic changes in all these parameters but no rainfall. Wind profiler data shall provide a better understanding of these cold pools.

How to cite: Gogoi, D. and Rao, T. N.: Response of the atmospheric boundary layer to cold pools of thunderstorms at rural location, Gadanki, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-791, https://doi.org/10.5194/egusphere-egu23-791, 2023.

EGU23-1527 | ECS | Posters on site | AS2.4

Intercomparison of lower-cost and conventional eddy covariance systems for CO2 and H2O flux measurements above cropland monoculture and agroforestry 

José Ángel Callejas Rodelas, Justus van Ramshorst, Alexander Knohl, and Christian Markwitz

Agroforestry (AF) systems are recognized as a more sustainable agricultural practice compared to conventional agriculture due to its potential for increase carbon sequestration, among others. Short Rotation Alley Cropping (SRAC) is an AF practice in Central Europe in which trees and crops are cultivated in alternating rows.

The amount of carbon sequestered by a SRAC system can be estimated by the eddy covariance (EC) technique, the standard method for the continuous assessment of energy, momentum and trace gas exchanges above terrestrial ecosystems. As SRAC systems are heterogeneous, using only one EC set-up might limit the spatial representativity and, hence, the statistical power of measured fluxes. Increasing the number of EC set-ups could increase the statistical power, which is, however, cost intensive.

Therefore, the aim of this study was to test (i) the performance of a lower-cost EC (LC-EC) set-up for CO2- and H2O-flux measurements above SRAC and monocropping (MC) agriculture and (ii) if the sensor-to-sensor differences in fluxes are lower than differences between ecosystems (SRAC and MC).

We performed CO2 and H2O flux measurements above a MC system with three lower-cost and one conventional EC set-up from March to August 2022. In addition, CO2 and H2O fluxes were also measured with a LC-EC set-up located in a SRAC system at 520 m distance from the MC site.

The CO2 and latent heat (LE) fluxes of the three LC-EC set-ups showed similar results compared to the conventional EC setup. The linear regression between the conventional and the LC systems showed R2 coefficients in the range of 0.8-0.9 for CO2 and 0.7-0.9 for LE, and slopes in the range of 0.9-1.0 for CO2 and 0.8-1.0 for LE. The energy balance was consistent for all the systems, providing an average 70% closure. The total cumulative C uptake over the entire campaign was similar among the 3 LC-EC set-ups, but they underestimated the C uptake compared to the conventional EC set-up by 18% on average. The C uptake measured by the LC-EC systems at the end of the measuring campaign was 74 g C·m-2 at the MC (mean across all the 3 LC-EC set-ups) and 111 g C·m-2 at the SRAC. The C uptake of the conventional EC system at the MC was 90 g C·m-2. Hence, the SRAC system had a larger C uptake than the MC system throughout the measurement campaign.

We conclude that the LC-EC provided satisfying results compared to conventional EC, with the potential to improve the spatial replication of EC measurements. Furthermore, the difference between the 3 LC-EC set-ups in the MC was much lower compared to the difference between the MC and the SRAC.

How to cite: Callejas Rodelas, J. Á., van Ramshorst, J., Knohl, A., and Markwitz, C.: Intercomparison of lower-cost and conventional eddy covariance systems for CO2 and H2O flux measurements above cropland monoculture and agroforestry, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1527, https://doi.org/10.5194/egusphere-egu23-1527, 2023.

EGU23-1565 | Orals | AS2.4 | Highlight

Isoprene and monoterpene emission response to the El Niño-Southern Oscillation 

Ryan Vella, Andrea Pozzer, Jos Lelieveld, Matthew Forrest, and Holger Tost

Isoprene and monoterpene emissions from the terrestrial biosphere play a significant role in major atmospheric processes. Such emissions account for 90% of the total volatile organic compound (VOC) emissions and exert a significant influence on the atmosphere's oxidation capacity, aerosol formation and in turn, clouds and climate. Emissions depend on the vegetation response to atmospheric conditions (primarily temperature and light), as well as other stresses e.g. from droughts and herbivory. The El Niño-Southern Oscillation (ENSO) is a natural cycle, arising from sea surface temperature (SST) anomalies in the tropical Pacific, which perturbs the natural seasonality of weather systems on both global and regional scales. Several studies evaluated the sensitivity of BVOC fluxes during ENSO events using transient simulations. While these studies employ realistic scenarios, it is difficult to assess the individual impact of ENSO given multiple forcing on the climate system (e.g. from CO2, aerosol, etc.). In this work, simulations from a global atmospheric chemistry-climate model with enabled interactive vegetation are used to assess changes in vegetation (net primary production (NPP) and leaf area index (LAI)), meteorology (surface temperature, surface radiation, and precipitation), and consequently, isoprene and monoterpene emission changes attributed to ENSO. Global isoprene emissions could increase by 4% during strong El Niño events with substantial regional changes e.g. + 20% over Amazonia. Changes in isoprene and monoterpene emissions are evaluated in response to meteorological and vegetational variability.

How to cite: Vella, R., Pozzer, A., Lelieveld, J., Forrest, M., and Tost, H.: Isoprene and monoterpene emission response to the El Niño-Southern Oscillation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1565, https://doi.org/10.5194/egusphere-egu23-1565, 2023.

EGU23-1901 | ECS | Posters on site | AS2.4

A new 24/7 operational workflow in agro-meteorology, based on the coupled WRF/SEBAL models 

Amirhossein Nikfal, Mohammadamin Karimi, Salar Pashapour, Majid Vazifedoust, Masoumeh Khorani, Amirmahdi Khosravi Tabrizi, Hamideh Noory, Mohammad Rezvani, and Zahra Toofaninejad

Water scarcity is regarded as a primary issue in many dry climates, with significant impacts on food security and national developments. Since agricultural irrigation accounts for most of water consumption worldwide, providing a water management system is critical to cope with water stress and its challenges. Agricultural water management is an interdisciplinary task, dealing with meteorological and environmental factors. In this work, we have established a 24/7 operational system to simulate those land surface variables, associated with evapotranspiration, biomass growth, and water deficit, using the Surface Energy Balance Algorithm for Land (SEBAL). SEBAL simulates the energy balance, using satellite data in shortwave and thermal bands, as well as soil and meteorological data (wind speed, humidity, etc).

This workflow consists of 3 interconnected units: WRF model, Python implementation of the SEBAL model (pySEBAL), and a web-based management panel for the visualization, reanalysis, and publishing the results. The WRF model is run in a daily basis for 36 hours, starting from 12:00 UTC, to provide the meteorological data for the next day. At the next stage, the simulated WRF data after some required processing (converting formats and units of files and
variables, etc.) will be incorporated as input data into the SEBAL model. The key data for the SEBAL model is the “Visible Infrared Imaging Radiometer
Suite” (VIIRS) real-time data over the Suomi satellite, which is received automatically after tracking the satellite and picking the appropriate data files for download. SEBAL outputs include some of the variables with key role in agricultural water management, such as actual and potential evapotranspiration, biomass production and deficit, albedo, NDVI, etc, with a resolution of 375m over Iran.

The third section of the operational system is a web-based panel, consisting of an open-source server to share and edit the SEBAL outputs. An open-source database management system for the client- based analysis of the SEBAL outputs, and an open-source JavaScript library for displaying the maps of the SEBAL outputs in web browsers.

How to cite: Nikfal, A., Karimi, M., Pashapour, S., Vazifedoust, M., Khorani, M., Khosravi Tabrizi, A., Noory, H., Rezvani, M., and Toofaninejad, Z.: A new 24/7 operational workflow in agro-meteorology, based on the coupled WRF/SEBAL models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1901, https://doi.org/10.5194/egusphere-egu23-1901, 2023.

Irrigation is still widely neglected in land surface models which are used for numerical weather prediction. However, with the general improvement of coupled surface-atmosphere models and the evolution towards kilometer or hectometer grids, this omission is beginning to be reconsidered. Better understanding the links between the strong surface heterogeneity and local meteorology is one of the objectives of the LIAISE (Land surface Interactions with the Atmosphere In Semi-Arid Environment) project. The work presented here focuses on two clear and warm days of the special observation period of the LIAISE campaign that took place during the summer of 2021 in northeastern Spain. The coupled surface-atmosphere model Surfex-MesoNH is used to model two days of interest with and without an irrigation parameterization. The model outputs are then compared to multiple surface-based and airborne observational data. A clear improvement is provided by the irrigation representation. In particular, the modeled sensible and latent heat fluxes are reconciled with the observations, the temperature biases at 2m are corrected up to 5°C, and the specific humidity is increased by about 50% around noon near the surface. It is also shown that irrigation leads to changes in the structure and height of the atmospheric boundary layer. A breeze-like, non-classical mesoscale circulation induced by the surface contrasts between the irrigated area and the surrounding semi-arid area is highlighted.

How to cite: Lunel, T., Boone, A., and Le Moigne, P.: Influence of irrigation on land-surface interactions and the atmospheric boundary layer in a semi-arid region – Results from the LIAISE campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2253, https://doi.org/10.5194/egusphere-egu23-2253, 2023.

EGU23-3338 | ECS | Orals | AS2.4

Effects of spatial heterogeneity within the eddy covariance (EC) footprint on up-scaled methane fluxes across multiple wetland sites 

Tiia Määttä and Avni Malhotra and the FLUXNET-CH4 EC-chamber working group

Methane (CH4) is a strong greenhouse gas that is produced in anoxic soil conditions. Wetlands are the largest natural source of CH4 globally because their anoxic soils provide suitable habitats for CH4-producing Archaea. Both global and regional wetland CH4 budgets remain unconstrained due to large uncertainties in wetland extent and high spatio-temporal variability in CH4 dynamics that are in part driven by wetland spatial heterogeneity. High wetland spatial heterogeneity often results from the variability in microtopography, soil hydrological and chemical properties, and vegetation and microbial composition. Intertwined together, the different abiotic and biotic variables further contribute to the ratio between CH4 production, consumption and transport processes in wetland soil, resulting in either net CH4 emission or uptake. However, the contribution of different abiotic and biotic factors to CH4 flux variability in wetlands remains unclear, increasing uncertainties in up-scaling CH4 emissions from plot to ecosystem and regional scales. Therefore, including well-defined spatial heterogeneity into wetland CH4 bottom-up estimates can help improve the regional and global CH4 budget calculations.

This study investigates the effect of spatial heterogeneity on observed CH4 emissions in ten different wetland sites with varying climatic conditions. Our approach will include up-scaling chamber measurements from different land cover classes to the level of the eddy covariance (EC) footprint. The compiled chamber datasets include both manual (n=5) and automatic (n=5) measurements that have been combined with EC measurements (FLUXNET-CH4 database) based on matching timestamps. First, the chamber observations will be compared to the corresponding EC measurements without accounting for spatial heterogeneity. Then, various remotely sensed environmental variables, such as leaf area index (LAI) and topographic wetness index (TWI), in high spatial resolution will be used to create land cover classes and combined with a modeled footprint to include spatial heterogeneity in the up-scaling of point-level measurements in all sites. 

Preliminary results suggest that the chamber and EC observations differ significantly in magnitude between seasons and sites. In general, chamber observations had a larger range than EC, which we expected, given that chambers capture finer spatial heterogeneity than EC. However, no consistent trends emerged in the difference in magnitude between chamber and EC. We expect that the inclusion of spatial heterogeneity into the footprint model will decrease the differences  between up-scaled chamber and EC observations for all sites. Notably, we expect that the inclusion of proxies for soil moisture, plant functional type (PFT) and aerenchyma  will improve footprint-level comparisons to chamber-level data. We will present updated comparisons of EC and chamber data with and without inclusion of spatial heterogeneity. Altogether, this study will establish a workflow for combining wetland CH4 data from different measurement types (EC and chamber) and will allow global syntheses to use more of the available data to constrain CH4 budgets. 

How to cite: Määttä, T. and Malhotra, A. and the FLUXNET-CH4 EC-chamber working group: Effects of spatial heterogeneity within the eddy covariance (EC) footprint on up-scaled methane fluxes across multiple wetland sites, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3338, https://doi.org/10.5194/egusphere-egu23-3338, 2023.

Land-atmosphere energy and moisture exchange can strongly influence local and regional climate changes. However, high uncertainties exist in the representation of land-atmosphere interactions in numerical models and the coupling strength between land and atmosphere is largely overestimated, in which the determination of surface exchange coefficient is one of the main problems. Here, we show the improvements from a dynamic vegetation-type-dependent exchange scheme in the offline Noah land surface model with multi-parameterization options and the Weather Research and Forecasting model when applied to China. Compared to the default schemes, the dynamic exchange scheme significantly reduces land-atmosphere coupling strength overestimations, and comparisons to flux tower observations reveal its capability to better match observed surface energy and water variations. In particular, the above remarkable improvements produced by the dynamic exchange scheme primarily occur in areas covered with short vegetation. The improved version benefits from the treatment of the roughness length for heat. Further, land-surface processes play significant roles in cloud formation and precipitation generation by affecting local planetary boundary layer profiles. The dynamical exchange scheme could narrow the positive discrepancies in the simulated precipitation. Using 3-km-resolution convection-permitting models for three heavy precipitation cases, the dynamic coupling simulations could achieve the closest agreement with the field observations, especially the intensity and location of the heaviest rainfall during the precipitation process. Overall, our findings highlight the applicability of the dynamic scheme as a better physical alternative to the current treatment of surface exchange processes in atmosphere coupling models and could help achieve more accurate simulations.

How to cite: Zhang, X., Chen, L., and Ma, Z.: Improvement of surface exchange coefficient parameterization and its application to regional numerical simulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3423, https://doi.org/10.5194/egusphere-egu23-3423, 2023.

EGU23-3707 | Posters on site | AS2.4

From soils to clouds - An integrated atmospheric boundary layer observatory in a temperate forest of eastern Canada 

Manuel Helbig, Nickerson Nick, Mengering Deklan, Rudaitis Lukas, Ryan Jillian, Benítez-Valenzuela Lidia, Creelman Chance, and Taylor Mara

Temperate forests have been shown to substantially impact near-surface climate and atmospheric boundary layer dynamics through a range of complex land-atmosphere feedback mechanisms. For example, forests can reduce water loss to the atmosphere during periods of high vapour pressure deficit, thereby preventing or delaying severe drought impacts. Reducing water loss during periods of high atmospheric water demand comes at the expense of reduced forest productivity and may contribute to additional warming of near-surface air temperatures through increased partitioning of energy to sensible heat. Understanding how land-atmosphere interactions in forested landscapes modify regional and local climate is thus crucial for the design of efficient national and international climate mitigation and adaptation strategies.

To better understand complex land-atmosphere interactions in a typical forested landscape of eastern Canada, we have established an integrated atmospheric boundary layer observatory in a temperate forest in New Brunswick, Canada. Observations will be used to quantify environmental, plant physiological, and atmospheric feedbacks and their impacts on near-surface climate. Here, we present the instrumental setup and preliminary results from the integrated observatory. Forest soils are monitored using soil temperature, volumetric soil moisture, soil water potential, and snow depth measurements and are complemented by soil CO2 efflux measurements using forced diffusion chamber systems. Detailed vertical profiles of air temperature and humidity, wind speed and direction, and light are measured from the forest floor to a height of 28 m (i.e., 18 m above the forest canopy) using six weather stations. At the top of the flux tower at 28 m above ground, net ecosystem CO2 exchange and evapotranspiration of the forested landscape is measured using the eddy covariance technique along with longwave and shortwave radiation fluxes. A ceilometer will be added to the observatory in spring 2023 to continuously observe cloud base height and atmospheric boundary layer height. The integrated measurements will produce datasets that can be used to diagnose complex land-atmosphere interactions, to characterise forest microclimate, and to validate coupled land-atmosphere models.

How to cite: Helbig, M., Nick, N., Deklan, M., Lukas, R., Jillian, R., Lidia, B.-V., Chance, C., and Mara, T.: From soils to clouds - An integrated atmospheric boundary layer observatory in a temperate forest of eastern Canada, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3707, https://doi.org/10.5194/egusphere-egu23-3707, 2023.

EGU23-3987 | Posters on site | AS2.4 | Highlight

Improvements in infrared gas analyzers for measuring atmospheric gases on moving platforms 

Ivan Bogoev, Douglas Vandemark, Marc Emond, Scott Miller, Shawn Shellito, and Jason Covert

Accurate observations of atmospheric composition and exchange of greenhouse gases between the ecosystems and the atmosphere are critical for constraining climate models. Infrared gas analyzers (IRGA) using either broad band non-dispersive or narrow band tunable laser technologies are widely used for this purpose. Typically, such analyzers are installed on stationary meteorological towers over land; but an increasing number of systems are being deployed on mobile platforms and buoys to extend the spatial coverage and include measurements over water.  One technological challenge is that the motion of the platform influences the gas concentration measurements. Empirical correction methods have been proposed, but their universality is limited because the source of these sensor-related effects and their underlining mechanisms have not been understood. In this study we identified the dominant source of the error: orientation-dependent temperature stabilization of the thermoelectrically cooled infrared detector. To further investigate this hypothesis and gain insights to a solution, a new prototype closed-path IRGA with an improved infrared detector was developed. In the study, we compared the performance of the prototype to standard models of commercially available IRGA measuring CO2 and H2O.  Tilt experiments with side-by-side mounted IRGAs were first conducted on a controlled laboratory platform with independent pitch and roll axes. Over the ±30° range of angular position, the orientation-correlated errors were reduced by a factor of 4 to 10 on CO2 and a factor of 2 to 8 on H2O. Subsequent testing was performed duplicating realistic buoy motion in a deep-water tank with typical at-sea combined pitch and roll motion. In these tests, improvements in the measurement errors were similar to the laboratory experiments. Implications for the correction of past field measurements and insights for further sensor optimization and system improvements are discussed.

How to cite: Bogoev, I., Vandemark, D., Emond, M., Miller, S., Shellito, S., and Covert, J.: Improvements in infrared gas analyzers for measuring atmospheric gases on moving platforms, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3987, https://doi.org/10.5194/egusphere-egu23-3987, 2023.

The near-surface humidity is a crucial variable in many atmospheric processes, mostly in those related to development of clouds and rain. The humidity at the height of a few tens of meters above surface is highly influenced by the surface characteristics. In many cases the land-cover (LC) is responsible for the spatial variation of the surface humidity field, therefore, it is a major factor in determining the conditions for rainfall. Cities are one of the primary LCs which have a substantial impact on the humidity field. Large urban areas are expanding, causing a significant change in the near-surface humidity field. Measuring the near-surface humidity in high resolution, where most of the humidity’s sinks and sources are, is challenging with the common tools available today. Current measurement tools do not satisfactorily assess the cities’ effects on the humidity field. A new approach for measuring the humidity, based on the cellular network, provides high resolution information on the near-surface humidity. Therefore, we can examine the land-cover effect on the humidity in the low atmosphere in fine scale. In this study, the humidity field around Tel Aviv was retrieved from the cellular network during the summer of 2017. The results show a well-noticed impact of the city and other LC types on the humidity field over the Tel Aviv metropolitan area. The method presented here can offer an improved description of the humidity field at the city-canopy level and therefore provide a better assessment of the urban/LC effects on the environment, atmospheric modeling, and particularly on clouds/rain development.

How to cite: Rubin, Y., Sohn, S., and Alpert, P.: Urban moisture based on commercial microwave links (CML) data and relation to land-cover – case of Tel- Aviv metropolitan area, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4355, https://doi.org/10.5194/egusphere-egu23-4355, 2023.

It has been well-recognised that the horizontal advection can modulate the downwind footprint of the urban heat island (UHI). However, limited studies have considered the urban heat advection (UHA) generated from this boundary-layer process, mainly due to the lack of a dense network of sensor to sufficiently resolve the local climate in a city. For the first time, this study explores the possible influence of the horizontal advection on the nocturnal surface urban heat island sensed by the MODIS satellite (sUHA) over a ten-year period. Results show that the heat transport from urban to downwind areas can be observed by the satellite instrument. A significant warming up to 0.5 ºC and 1.7 ºC were found at city (Birmingham) and regional scale (West Midlands area), respectively. The amplification of the sUHA at regional scale was largely attributed to the topography effects according to the significant correlation between sUHA and a topography index (i.e. R2=0.53). An approximate 0.5 ºC can be corrected for sUHA after minimising the topography impact by applying a statistical method. Overall, this study highlighted the value of the satellite instrument to investigate the UHA at both city and regional scale. However, more importantly, the topography was found to have considerable influences on regulating the heat transfer from urban to its downwind areas, which provides further implications for urban planning and risk management with respect to the UHI.

How to cite: Feng, J., Wang, Y., Cai, X., and Chapman, L.: The Effect of Horizontal Advection on the Nocturnal Surface Urban Heat Island Using MODIS Satellite over Birmingham and the West Midlands, United Kingdom, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4605, https://doi.org/10.5194/egusphere-egu23-4605, 2023.

EGU23-4877 | Orals | AS2.4

Addressing forest canopy decoupling on a global scale 

Georg Jocher

The eddy covariance (EC) method, nowadays the standard method for determining forest ecosystem-atmosphere turbulent exchange, faces a major threat in its application: the air masses below the canopy are regularly decoupled from the air masses above the canopy. Consequently, the EC measurements above the canopy like e.g. H2O and particularly CO2 fluxes can be biased due to missing signals from below-canopy processes. This decoupling is strongly site dependent and influenced by meteorological conditions, canopy properties and tower-surrounding topography. It can be verified and addressed by subsequent EC measurements below and above the canopy. Specifically, the correlation of σw below and above the canopy gives information about the coupling state as this correlation is linear during periods of full coupling.

The current study aims to address the decoupling issue on a global scale. For this purpose, approximately 30 forest sites from around the world will be analyzed in a standard way with regards to decoupling. The study sites cover manifold vegetation types and climate zones, all sites are equipped with concurrent below and above canopy EC measurements. Preliminary results highlight the dependence of decoupling on meteorological conditions, canopy properties and tower surrounding topography. Nevertheless, the final goal of this action is to derive global relations between these influence factors and decoupling which will be applicable in a general way on each forest site worldwide. Highest quality turbulent fluxes will be the outcome and the accuracy of EC derived forest water and carbon budgets will improve.

How to cite: Jocher, G.: Addressing forest canopy decoupling on a global scale, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4877, https://doi.org/10.5194/egusphere-egu23-4877, 2023.

EGU23-5762 | ECS | Orals | AS2.4

Cloud-driven patterns of surface solar irradiance as seen by a spatial network of radiometers 

Wouter Mol, Bert Heusinkveld, Oscar Hartogensis, and Chiel van Heerwaarden

Surface solar irradiance varies on scales down to seconds or meters due to clouds. This highly variable nature of irradiance is not resolved by atmospheric models, yet heterogeneity in surface irradiance impacts the overlying cloud field. The inability to resolve irradiance variability, aside from insufficient model resolution, is explained by our limited understanding of cloud-driven solar irradiance variability at short spatiotemporal scales and the lack of high resolution spatial observational data. Cloud resolving models utilizing ray tracing techniques are a useful research tool, but ultimately require validation against observations.

In 2021, we gathered new observational data with a network of radiometers, specifically designed to gather data on cloud-driven surface patterns of irradiance. I will present results on various kinds of surface patterns in relation to cloud type and atmospheric conditions, based on these observations. Our radiometers sample surface solar irradiance at 10 Hz for 18 wavelengths, which we deployed in different setups in the FESSTVaL (Germany) and LIAISE (Spain) field campaigns. Our results highlight the complexity and wide range of regimes in spatiotemporal irradiance variability, but also provide insights into its driving mechanisms. These insights help guide the development of improved radiative transfer calculations, in order to move towards models that can accurately resolve irradiance variability in an operational setting.

How to cite: Mol, W., Heusinkveld, B., Hartogensis, O., and van Heerwaarden, C.: Cloud-driven patterns of surface solar irradiance as seen by a spatial network of radiometers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5762, https://doi.org/10.5194/egusphere-egu23-5762, 2023.

EGU23-5832 | ECS | Posters on site | AS2.4

Water and carbon fluxes along a land use gradient in the tropical mountain dry forest of South Ecuador 

Charuta Murkute, Franz Pucha Cofrep, Volker Raffelsbauer, Sebastian Scholz, Oliver Limberger, Galo Carillo-Rojas, Jörg Bendix, and Katja Trachte

Ecosystems play an important role in controlling the exchange of energy, water and carbon between the land surface and the atmosphere, which contributes to the regulation of the climate through biogeochemical process. Changes in vegetation or biomass impacts the microclimatological conditions of the landscapes with feedbacks to the heat and water budgets. Knowledge about the dynamics and driving factors of the exchange processes contributes to our understanding of the land surface – atmosphere interactions as drivers of the Earth’s surface energy budget.

In the Tumbesian mountain dry forest (MDF) in the Laipuna reserve on the western escarpment of the Andes mountains in South Ecuador two eddy-covariance measurement stations have been installed over natural forest and an anthropogenic replacement system to observe atmospheric water and carbon fluxes. The MDF is characterized by a distinct seasonality, which can be divided into a dry (May - December) and wet (November - May) season following the inter-hemispherical shift of the ITCZ. Mean monthly precipitation totals ranges between 50 and 400mm with an annual amount of 650mm, while the temperature varies between 21 – 26°C. The forest ecosystem is dominated by deciduous trees and hold a clear annual cycle in the water budget and carbon sequestration. In the scope of global climate change such water limited landscapes are strongly vulnerable to climatic stress situations which lead to changes in the phenological cycles in the ecosystem associated with feedbacks to the water and carbon cycle. The aim is thus, to investigate the energy, water and carbon dynamics along a land use gradient in order to estimate the impact of deforestation on net-ecosystem exchange and evapotranspiration in the MDF region. The study shows first results of microclimatological conditions, such as radiative fluxes, moisture and soil conditions of both sites as well as water and carbon fluxes.

How to cite: Murkute, C., Cofrep, F. P., Raffelsbauer, V., Scholz, S., Limberger, O., Carillo-Rojas, G., Bendix, J., and Trachte, K.: Water and carbon fluxes along a land use gradient in the tropical mountain dry forest of South Ecuador, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5832, https://doi.org/10.5194/egusphere-egu23-5832, 2023.

EGU23-5833 | ECS | Orals | AS2.4

A conceptual system for identifying and distinguishing different non-rainfall water fractions in agroecosystems 

Jannis Groh, Thomas Pütz, Daniel Beysens, Harry Vereecken, and Wulf Amelung

Most of the water input to the ecosystem comes from rainfall. However, depending on the local climatic conditions a considerable amount of water can also be produced by different fractions of non-rainfall water inputs (NRWIs), namely dew, hoarfrost, rime, fog, and the adsorption of water vapour in the soil. Such NRWIs are often neglected because they are typically small compared to rainfall on the daily scale. Nevertheless, these NRWIs provide our ecosystems with additional water, which is important for the survival of the fauna and flora in the ecosystem, especially during dry periods. 

In the past different devices were used to determine some of these fractions, based on artificial surfaces (e.g., dew or fog collector). We will present a conceptual measurement set-up that allows us to determine each non-rainfall water (NRW) component for natural surfaces of agricultural ecosystems. The method is based on precise weighable lysimeter measurement to determine the incoming water fluxes of NRW. The partitioning between the NRW components will be done based on parallel observations on the surface and air temperature, humidity, rain gauge, and dust collector. Based on this conceptual system, we will compare the temporal development and occurrence of different NRW components for eight different agroecosystems under similar climatic conditions.

How to cite: Groh, J., Pütz, T., Beysens, D., Vereecken, H., and Amelung, W.: A conceptual system for identifying and distinguishing different non-rainfall water fractions in agroecosystems, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5833, https://doi.org/10.5194/egusphere-egu23-5833, 2023.

EGU23-5854 | Posters on site | AS2.4

Application of a bi-directional ammonia exchange model for optimization of input parameters at a fertilized crop system; validation by flux measurements 

László Horváth, Helga Huszár, Zoltán Nagy, Krisztina Pintér, Anna Szabó, Tünde Takács, Péter Torma, Eszter Tóth, Tamás Weidinger, and Zoltán Bozóki

In parameterization of the bi-directional ammonia exchange models over vegetated surfaces there are three most crucial parameters: (1) the stomatal (χs) and (2) the soil (χg) compensation point concentrations as the function of Γ=[NH4+]/[H+] in the apoplast and soil, as well as (3) the cuticular resistance Rw. These factors determine the direction and magnitude of the ammonia flux. Moreover, in the sophisticated models the soil (Fg) and litter (Fl) fluxes must be distinguished as well. Furthermore, the recapture of ammonia volatilized from the ground in the lower layer of the canopy should also be considered.

            For partitioning the measured ammonia flux into stomatal, cuticular and ground parts two-layer, bi-directional exchange models are generally used. However, the parameterization mostly based on empirical relationships involves uncertainties, resulting in disagreements among the applied models in the estimation of the stomatal/soil flux ratio.  

            The main reasons of the deviations may be the following: 

  • a) Overestimation of the soil compensation-point (χg).The Γg calculated from the ammonium content of the soil and the pH of the soil solution is overestimated, because part of the ammonium content in the soil is bound in the solid phase hence Henry's law for the liquid phase cannot be applied for this fraction.
  • b) Neglecting of the part of soil derived ammonia recaptured by leaves. For this reason, soil emissions may be underestimated.
  • c) Uncertainty or lack of bioassay measurement for Γs and difficulties with the Γs determined by indirect way. Instead of complicated bioassay measurements, the models generally use empirical approximations to calculate the stomatal compensation point concentration or infer it from the bulk ammonium content of the leaf tissue. Both methods can be a source of error.
  • d) Inaccurate or rough estimate of cuticular resistance. Beside the temperature and humidity, the ratio of acidic air components and ammonia determines the Rw. Models often consider a constant site-specific average for this parameter, even though the ratio of acidic substances to ammonia varies from day to day.

            Due to these uncertainties, the estimation of the share of fluxes controlled by soil and vegetation is often uncertain. Furthermore, the uncertainty of the parameterization limits the applicability of the model and reduces its robustness.

            As a conception, we are aiming the use of the following measurement and parameterisation protocol:

  • a) Measurement of the flux above bare soil and above the litter covered soil separately, by soil chambers using the PICARRO-G2103 NH3 Hence, the Fg and Fl and the ratio of compensation point concentrations (χg/χl) can be estimated separately. Comparison of the χg calculated from soil NH4+ and pH with the measured values.
  • b) Calculation of the recaptured ammonia by the model as the residual term among soil-cuticular-stomatal exchange.
  • c) Performing bioassay measurements.
  • d) Use of daily acid/base gas ratio from the nearby regional background air pollution station.

            Model conception based on previously developed models. Bulk fluxes above the canopy will be measured by the relaxed eddy accumulation technique (REA) with a newly designed photoacoustic system using a QCL as light source. 

How to cite: Horváth, L., Huszár, H., Nagy, Z., Pintér, K., Szabó, A., Takács, T., Torma, P., Tóth, E., Weidinger, T., and Bozóki, Z.: Application of a bi-directional ammonia exchange model for optimization of input parameters at a fertilized crop system; validation by flux measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5854, https://doi.org/10.5194/egusphere-egu23-5854, 2023.

EGU23-6854 | ECS | Orals | AS2.4

High-resolution satellite-based cloud detection for the analysis of land surface effects on boundary layer clouds 

Julia Fuchs, Hendrik Andersen, Jan Cermak, Eva Pauli, and Rob Roebeling

In this study, geostationary satellite observations are used to develop and validate two high-resolution cloud-masking approaches for the region of Paris to show and improve applicability for analyses of urban effects on clouds. 

Firstly, the Local Empirical Cloud Detection Approach (LECDA) uses an optimised threshold to separate the distribution of visible reflectances into cloudy and clear sky for each individual pixel accounting for its locally specific brightness. Secondly, the Regional Empirical Cloud Detection Approach (RECDA) uses visible reflectance thresholds that are independent of surface reflection at the observed location.

Results show that

  • A decrease of cloud cover during typical fog or low-stratus conditions over the urban area of Paris for the month of November is likely a result of urban effects on cloud dissipation.
  • The regional approach, RECDA, is a more appropriate choice for the high-resolution satellite-based analysis of cloud cover modifications over different surface types than LECDA with regional biases of ±5 %.

This approach can provide comprehensive insights into spatiotemporal patterns of land-surface-driven modification of cloud occurrence and locally induced cloud processes, such as the diurnal variation of the occurrence of fog holes and cloud enhancements attributed to the impact of the urban heat island. Further, it is potentially transferable to other regions and temporal scales for analysing long-term natural and anthropogenic impacts of land cover changes on clouds.

How to cite: Fuchs, J., Andersen, H., Cermak, J., Pauli, E., and Roebeling, R.: High-resolution satellite-based cloud detection for the analysis of land surface effects on boundary layer clouds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6854, https://doi.org/10.5194/egusphere-egu23-6854, 2023.

EGU23-7132 | ECS | Posters on site | AS2.4

Comparison of the energy fluxes inferred from eddy covariance and optical scintillometer at the agricultural field during different parts of the season 

Matěj Orság, Milan Fischer, Gabriela Pozníková, Josef Eitzinger, and Miroslav Trnka

This study summarizes seasonal monitoring of turbulent energy fluxes from eddy covariance (EC) and large aperture optical scintillometer, measuring in parallel. The site (agricultural field of app. 16.5 ha) is located in north-eastern Austria, Danube river lowland (48.21N, 16.622E); in 2019 covered subsequently by a winter wheat field, straw, and bare soil. The EC together with ancillary measurement was located at the 2.7 m height at the center of the field. The radiation balance components measurements consist of a 4-channel net radiometer for net radiation (Rn) installed at 3.5 m and three soil heat flux plates for soil heat flux (G) monitoring (0.05 m below surface), including thermocouples for quantification of the heat storage above the soil heat flux plates. The scintillometer transmitter and receiver units were fixed at 4 m height masts, facing towards each other from the NW and SE corners of the field, with a measurement path length of 570 m diagonally across the field. The EC method enables the determination of fluxes within a footprint centered around the point of measurement in the middle of the field, whereas the scintillometer provides an estimation of sensible heat flux (HSC), derived from air refractive index fluctuation integrated over the measurement path length. The scintillometer-based latent heat (LESC) is calculated as a residuum from available energy (Rn-G) and HSC, provided by the scintillometer. As the EC method provides direct measurements of sensible heat (HEC) and latent heat (LEEC) fluxes we use it as a reference method. During the period March to June (green canopy) the comparison of the EC-based turbulent fluxes (HEC+LEEC) and the available energy (Rn-G) showed a very good agreement, resulting in the energy balance closure of 0.97 (R2 = 0.94). This suggests the ability of the EC method to capture all scales of eddies responsible for energy transport at this site as well as the good accuracy and robustness of the measurement setup. During the period March to June (green canopy), the HEC, LEEC, HSC, and G fluxes accounted for 23 % (R2 = 0.55), 60 % (R2 = 0.72), 32 % (R2 = 0.56), and 12 % (R2 = 0.62) of the Rn flux, respectively. The comparison of methods indicates that HSC overestimated HEC by 20 % (R2 = 0.78). However, during the latter part of the season (straw and bare soil) we found that under highly unstable atmospheric stratification, HSC is even more overestimating HEC and sometimes is even exceeding the available energy. The main reason for such behavior can be the choice of the universal stability function in the computation of HSC. Recommendations for universal functions that are correcting this artifact in HSC will be discussed.

Acknowledgment: This study was supported by SustES - Adaptation strategies for sustainable ecosystem services and food security under adverse environmental conditions (CZ.02.1.01/0.0/0.0/16_019/0000797).

How to cite: Orság, M., Fischer, M., Pozníková, G., Eitzinger, J., and Trnka, M.: Comparison of the energy fluxes inferred from eddy covariance and optical scintillometer at the agricultural field during different parts of the season, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7132, https://doi.org/10.5194/egusphere-egu23-7132, 2023.

Micrometeorological measurements, and greenhouse-gas monitoring, performed by on-site sensors or remote sensing are not exclusively influenced by the terrain beneath the sensor position or at the optically aimed spot, sometimes they are not even influenced by it at all. The footprint function (or so-called source area) provides a description of the actual “field of view”, namely the 2D spatial distribution of the weighing function applied on the sources and sinks to yield the signal value. Given a scalar of interest, different distributions are obtained depending on whether the considered quantity is the concentration or the flux of this scalar.

Footprints derived from fully analytical models are restricted due to the following hypotheses: homogeneous flow (i.e. in terms of soil-atmosphere interactions, e.g. roughness length, thermal sources driving the turbulence), the eddy diffusivity and the mean wind speed are power-law functions of height. Despite these restrictions, they are often used due to their ease and speed. The footprint functions are expressed in terms of the inverse Gamma distribution whose parameters depend on the power-law parameters. These parameters must be identified from the actual wind speed and diffusivity profiles, which are generally assimilated to profiles parameterized according to the Monin-Obukov theory. The scope of the analytical approach can be broadened by relaxing the power-law constraint regarding the profiles. In this perspective a new semi-analytical model was developed which is based on a graded multi-layer approach. A Liouville transformation is first applied which introduces a new independent variable, the Diffusion-Ascent-Associated Advection Distance (DAAAD, in place of height) and a new advection-diffusion parameter, the atmosphere inertivity, which describes the atmosphere inertia to state change at the considered position. The graded multi-layer method allows approximating the real inertivity profile by a piecewise function, with continuously joined sublayers, hence allowing a close fitting with a minimal number of sub-layers.

As an example, Monin-Obukhov profiles based on the Businger-Högström parameterization, from unstable to stable, were considered and the footprint functions were computed for a large range of height. It was shown that the corresponding concentration and flux footprints are very accurately approximated (to less than 1-1.2% RMS error) by the functions mentioned before based on the inverse Gamma distribution. The optimal values of the two or three parameters involved therein were computed to provide a database depending on the two ratios zm/z0 and z0/L. Furthermore, an analytical parameterization of the two parameters intervening in the flux footprint has been proposed with only a slight reduction of the performance as compared to the highly accurate semi-analytical multi-layer model.

A comparison to the classical Kormann & Meixner, and Hsieh et al. models, which otherwise share the same hypotheses, is finally presented. With a negligibly small increased effort in the computation of the parameterization functions, a much better rendering of the Monin-Obukhov footprints is achieved. Moreover, the Monin-Obukhov profiles are just an example, the graded multi-layer method can be applied to any pair of profiles inasmuch the K-theory can be considered valid in the studied context.

How to cite: Krapez, J.-C.: Footprint parameterization derived from a graded multilayer semi-analytical model valid in homogeneously driven boundary layers described by Monin-Obukhov theory, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7164, https://doi.org/10.5194/egusphere-egu23-7164, 2023.

EGU23-7420 | ECS | Posters on site | AS2.4

Partitioning the urban carbon budget with carbonyl sulfide (COS) flux measurements conducted in a high-latitude city 

Jesse Soininen, Pekka Rantala, Liisa Kulmala, and Leena Järvi

Globally, cities correspond to most of the direct anthropogenic carbon emissions, and due to the global mega-trend of urbanization, their importance will only increase. The carbon budget of an area is often given as a net ecosystem exchange (NEE), which describes net CO2 fluxes measured with eddy covariance (EC) method. However, these measurements alone cannot partition anthropogenic and biogenic carbon sources and sinks. Earlier studies on vegetated ecosystems have defined leaf-scale relative uptake (LRU) of carbonyl sulfide (COS) and CO2 to partition the biogenic uptake, namely gross primary production (GPP).

In this research, the aim was to examine the suitability of using COS flux measurements to partition GPP from urban NEE, to better understand the effect of urban green areas on the carbon balance of cities. EC fluxes of CO2 and COS were measured at ICOS Associated Ecosystem Station FI-Kmp station in Helsinki, Finland, during Winter 2020-2021 and July 2022. Urban LRU is estimated for a footprint dominated by urban parks. Then, GPP is estimated from the measured COS flux, using three methods with varying complexity, for more heterogeneous footprints with more pronounced anthropogenic influence. Estimates are compared with a more common carbon balance partitioning method where only ecosystem respiration is considered.

Preliminary results showed how LRU over urban park has similar behavior as forest LRU, and the values are same order of magnitude. COS flux can be used as a tracer for carbon uptake by photosynthesis also in urban areas. Two out of the three methods showed the daily dynamics of GPP qualitatively right, with more complex underestimating and simpler overestimating the GPP, respectively. When using COS as a proxy for GPP in a heterogeneous urban environment, errors arise due to anthropogenic emissions of COS, which are not expected in the original context of using the compound as a biogenic activity tracer. In the future, more focus will be put to adapt methods to determine anthropogenic influence.

How to cite: Soininen, J., Rantala, P., Kulmala, L., and Järvi, L.: Partitioning the urban carbon budget with carbonyl sulfide (COS) flux measurements conducted in a high-latitude city, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7420, https://doi.org/10.5194/egusphere-egu23-7420, 2023.

Absorption, transformation and release of incoming solar radiation as turbulent heat into the atmosphere is critical for earth's energy balance. However, there is a lack of knowledge of the governing factors of the associated turbulent fluxes. Especially the influence of land surface heterogeneities is uncertain, as often only one-dimensional measurements are available. Finding an interrelation of the surrounding terrain to the turbulent fluxes is therefore not possible. This might be the explanation for why measured fluxes often cannot be reproduced with common calculation methods.

Thus, the objective of our study is to investigate the impact of surface heterogeneities on turbulent surface fluxes by performing idealized Large Eddy Simulations of a convective boundary layer over heterogeneous land surfaces under varying conditions. The simulations are run with the Parallelized Large-Eddy Simulation Model (PALM), covering a 10 km x 10 km domain with cyclic boundary conditions. The horizontal resolution is 5 m, the vertical resolution is 2 m near the surface and is increasing with height. The simulation period is one day. The scenarios differ in initial wind profiles, radiation, soil moisture and the type of surface heterogeneities. Output variables are averaged over 5 minutes.

By means of these highly resolved simulations, an encompassing three-dimensional analysis of the turbulent surface fluxes and their governing factors could be carried out, enabling the development of improved methods for calculating turbulent fluxes.

How to cite: Koerner, B.: High resolution Large Eddy Simulations of the convective boundary layer over idealized land surface heterogeneities, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7621, https://doi.org/10.5194/egusphere-egu23-7621, 2023.

EGU23-7666 | ECS | Orals | AS2.4

Interpretability of negative latent heat fluxes from Eddy Covariance measurements during dry conditions 

Sinikka Jasmin Paulus, Tarek Sebastian El-Madany, Rene Orth, Anke Hildebrandt, Markus Reichstein, Jacob A. Nelson, Arnaud Carrara, Gerardo Moreno, Matthias Mauder, Jannis Groh, Sung-Ching Lee, and Mirco Migliavacca

Non-rainfall water can play a critical role in many ecosystems, but is understudied in most regions due to a lack of continuous, specialized measurements. One of the most commonly used techniques to quantify in situ ecosystem water fluxes is Eddy Covariance (EC). However, its use for the quantification of the two most famous non-rainfall water sources, dew and (radiation) fog, is limited because they often occur under humid conditions and nighttime stable stratification, making EC measurements particularly uncertain or non-valid.

Here we describe how a non-rainfall water input observed under dry conditions, namely water vapor adsorption by soil particles (VWA), can be monitored using existing eddy covariance datasets, giving insight into this little-studied soil water source. Unlike dew and radiation fog, atmospheric stability is not a prerequisite for WVA. Instead, WVA is driven by a highly negative soil matric potential inducing water vapor to condensate already at relative humidity < 100 %. Therefore, EC measurements may be more suitable to detect and quantify this flux than for dew and fog.

In this study, we test EC measurements for inferring WVA by comparing them to observations from large-weighing lysimeters, where the latter can be considered as a reference system for the measurement of WVA. Our aim is to explore the potential and limitations of the EC technique to detect and quantify WVA. We assess the quantitative and qualitative agreement between WVA estimated with the lysimeters and negative (downward) LE fluxes from EC. Our analysis uses four years of observations from a semi-arid tree-grass ecosystem and one year of a temperate agricultural ecosystem during the 2018 drought.

Our results show that during dry conditions the water vapor gradient between the relatively humid atmosphere and the dry soil pores leads to WVA in both ecosystems. We find a decent agreement between the timing of fluxes detected as WVA with lysimeters and with EC instruments, but the magnitudes (i.e. the amount of flux) differ. Furthermore, we aim to characterize the conditions under which negative LE fluxes from EC measurements can and should be interpreted as WVA. This way, our study expands the possibilities to investigate the relevance of WVA as a non-rainfall water source and, more generally, sheds light on a mostly overlooked aspect of land-atmosphere interaction during dry conditions in different ecosystems.

How to cite: Paulus, S. J., El-Madany, T. S., Orth, R., Hildebrandt, A., Reichstein, M., Nelson, J. A., Carrara, A., Moreno, G., Mauder, M., Groh, J., Lee, S.-C., and Migliavacca, M.: Interpretability of negative latent heat fluxes from Eddy Covariance measurements during dry conditions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7666, https://doi.org/10.5194/egusphere-egu23-7666, 2023.

EGU23-7803 | Orals | AS2.4

Simultaneous eddy flux monitoring of 10 greenhouse gases and air pollutants with a single instrument 

Morten Hundt, Marco Brunner, and Oleg Aseev

Monitoring of trace gas fluxes and greenhouse gas fluxes is key to understand the interaction between atmosphere, plants, and soil and therefore to improving our understanding of the climate system in general.

The complex flux systems require measurement of many different inert and reactive trace gases and greenhouse gases simultaneously to obtain a complete budget. This is especially the case in urban environments where both biogenic and anthropogenic sources and sinks play a role.

The eddy covariance (eddy flux) technique is often used to determine fluxes of the gases in question. Until recently, however, the monitoring was usually limited to only a few gases per measurement device making the technique complex and expensive but providing only a limited picture. MIRO Analytical has developed a novel multicompound gas analyzer that can monitor up to 10 air pollutants (CO, NO, NO2, O3, SO2 and NH3) and greenhouse gases (CO2, N2O, H2O and CH4) simultaneously with the high time resolution necessary for eddy-covariance flux measurements. The compact system combines several mid-infrared lasers (QCLs) providing outstanding precision, selectivity and accuracy for the gas measurements.

In our contribution we will introduce the measurement technique and will demonstrate application examples of this all-in-one atmospheric flux monitor. The system will be compared to alternative devices in parallel measurements and results of long-term observations and shorter campaigns will be presented.

How to cite: Hundt, M., Brunner, M., and Aseev, O.: Simultaneous eddy flux monitoring of 10 greenhouse gases and air pollutants with a single instrument, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7803, https://doi.org/10.5194/egusphere-egu23-7803, 2023.

EGU23-9744 | Orals | AS2.4

Evaluating and bridging the flux-variance and surface renewal methods 

Milan Fischer, Gabriel Katul, Asko Noormets, Gabriela Pozníková, Jean-Christophe Domec, Matěj Orság, Miroslav Trnka, and John S. King

Two micrometeorological methods that utilize high frequency sampling of air temperature were tested against eddy covariance (EC) sensible heat flux (H) measurements at three sites representing agricultural, agro-forestry and forestry systems. The two methods encompass conventional and newly proposed forms of the flux-variance (FV) and surface renewal (SR) schemes.  In terms of measurement setup, the sites represent surface, roughness and roughness to surface transitional layers, respectively. After the selection of the most reliable approaches, regression analyses against EC showed that both methods can estimate H with slopes within ±10 % from unity, and coefficient of determination R2 >0.9 across all three sites. The best performance, of both FV and SR, was at the agricultural field, where the measurements were within the surface layer.  The worst performance occurred in the tall, relatively heterogeneous forest, where the measurements were taken in the roughness sublayer, the depth of which (with its inherent uncertainty) needs to be taken into account in the calculations. In addition to the evaluation of the FV and SR forms, an alternative perspective relating ramp-like structures to the vertical temperature gradients in the surface boundary layer is introduced here. Ramp-like structures carry much of the heat flux and temperature variance, representing opportunities to constrain the coefficients of the two methods. As a corollary, we introduce a novel approach emerging from bridging FV and SR methods that combines information about the coherent structures with the overall variance to obtain heat fluxes in a turbulent atmosphere. The proposed approach yields reliable H estimates without the need for site-specific calibration and instrumentation other than a single fast thermocouple.

 

Acknowledgement: This study was conducted with support of SustES - Adaptation strategies for sustainable ecosystem services and food security under adverse environmental conditions (CZ.02.1.01/0.0/0.0/16_019/0000797) and USDA NIFA-AFRI Sustainable Bioenergy Program, 2011-67009-20089, Loblolly pine-switch grass intercropping for sustainable timber and biofuels production in the Southeastern United States.  Funding for AmeriFlux core site US-NC4 (natural forested wetland) was provided by the USDA NIFA (Multi-agency A.5 Carbon Cycle Science Program) award 2014-67003-22068. Additional funding was provided by the DOE NICCR award 08-SC-NICCR-1072, the USDA Forest Service award 13-JV-11330110-081, and the DOE LBNL award DE-AC02-05CH11231. 

How to cite: Fischer, M., Katul, G., Noormets, A., Pozníková, G., Domec, J.-C., Orság, M., Trnka, M., and King, J. S.: Evaluating and bridging the flux-variance and surface renewal methods, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9744, https://doi.org/10.5194/egusphere-egu23-9744, 2023.

EGU23-9884 | Orals | AS2.4 | Highlight

ICOS pilot observatories to monitor greenhouse gas emissions from three different-size European cities 

Andreas Christen, Lukas Emmenegger, Samuel Hammer, Werner Kutsch, Claudio D’Onofrio, Jia Chen, Markus Eritt, Martial Haeffelin, Leena Järvi, Natascha Kljun, Thomas Lauvaux, Benjamin Loubet, Matthias Mauder, Amewu A. Mensah, Dario Papale, Leonard Rivier, Stavros Stagakis, and Alex Vermeulen and the ICOS Cities Team

By continuously monitoring greenhouse gas emissions from densely populated urban areas, we can independently assess and monitor emission reduction efforts at a policy-relevant scale. The EU-funded project PAUL (Pilot Application in Urban Landscapes - Towards integrated city observatories for greenhouse gases) develops, evaluates, and refines innovative greenhouse gas monitoring technologies including observational strategies for urban areas that enhance the capabilities of the Integrated Carbon Observation System at urban scales (ICOS Cities). In 2022, three pilot observatories have been set up to test, refine and optimize approaches for monitoring emissions from a metropolitan area (Paris, France), a large isolated city (Munich, Germany) and a mid-size city (Zurich, Switzerland). The three observatories have been developed in a co-design approach and integrated different observational technologies in support of inverse and inventory modelling. The pilot observatories focus on carbon dioxide (CO2) emitted from fossil-fuel sources.

The three observatories operate for a pilot phase of two years and collect comparative data across cities with a multitude of instrument networks that serve three main goals: (1) to assess the input for inverse models of CO2 at city-scale and attribute inferred CO2 emissions to sub-city scale and emission sectors; (2) to refine spatial, temporal, and sectoral attribution of emissions in emission inventories and parametrize process models that separate urban fossil-fuel and biogenic fluxes; and (3) as independent validation datasets to evaluate estimated emission products.

In all three cities, CO2 concentrations and selected co-emitted species are continuously sampled on tall towers, on top of high buildings and/or at street level. In the Paris metropolitan area, 10 tall tower sites and 30 roof-top sites continuously measure high-precision CO2 and co-emitted species in the boundary layer upwind, over and downwind of the city. The Munich and Zurich observatories feature a combination of roof-top and street-level sensor networks placed closer to sources and sinks, with a stronger signal strength that is more forgiving in terms of the sensitivity, hence allowing the deployment of mid- and low-cost sensors. In Paris and Munich, additionally, total column observations of CO2 are performed upwind, over and downwind of the main urban emission sources using concurrent ground-based FTIR spectrometers. Three new tall-tower eddy-covariance (EC) systems have been established in central Paris, Munich and Zurich. The EC-towers provide total CO2 fluxes for defined sub-areas of each city and their characteristic diurnal, weekly and seasonal cycles. Further, the three EC-towers provide sector-specific emission ratios and fossil-fuel CO2 fluxes based on differences of measured CO2-fluxes, six co-emitted species and radiocarbon fluxes. Finally, all cities have observational systems in place that monitor biogenic fluxes, vegetation dynamics and meteorological conditions, including lidars for wind and mixed layer determination for an improved quantitative description of atmospheric transport and vertical mixing.

We highlight design considerations for the three observatories and exemplarily show how multi-scale systems can efficiently complement and constrain fossil-fuel emissions in urban areas. Knowledge and experience from these observations will feed into the establishment of guidelines for operational greenhouse gas monitoring systems in European cities on their way to climate neutrality.

How to cite: Christen, A., Emmenegger, L., Hammer, S., Kutsch, W., D’Onofrio, C., Chen, J., Eritt, M., Haeffelin, M., Järvi, L., Kljun, N., Lauvaux, T., Loubet, B., Mauder, M., Mensah, A. A., Papale, D., Rivier, L., Stagakis, S., and Vermeulen, A. and the ICOS Cities Team: ICOS pilot observatories to monitor greenhouse gas emissions from three different-size European cities, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9884, https://doi.org/10.5194/egusphere-egu23-9884, 2023.

EGU23-9974 | Orals | AS2.4

How much additional improvements in measurements and data filtering can help to close the energy balance at eddy covariance stations 

Dario Papale, Giacomo Nicolini, Maarten Op de Beeck, Simone Sabbatini, Marta Galvagno, and Bert Gielen and the ICOS Ecosystem Stations PIs

The non-closed energy balance is still an unsolved problem of eddy covariance measurements: when the net radiation budget is compared with all the different energy exchange components measured at the flux station there is a general systematic imbalance, highlighting that one or more  energy components are either underestimated or not measured. Different hypotheses have been stated and many analyses into potential causes have been performed in the past years, ranging from methodological problems (water vapour flux underestimation due to condensation or unaccounted spectral damping in the analyser tube, underestimation of the vertical wind speed component due to transducers shadowing in the sonic anemometers), to components not fully monitored (e.g. the heat stored in the vegetation) different sensor footprints and field of views, to large scale motions particularly relevant in heterogeneous and fragmented landscapes. All these aspects are important and probably the issue of the energy balance non-closure is due to a combination of all the factors.

The ICOS Ecosystem network consists of a set of eddy covariance stations equipped with high-level and quality standardized instrumentation, whose data are processed centrally. The availability of these data (freely accessible through the ICOS Carbon Portal) allows for a systematic analysis of the importance of the different measured energy components (soil heat flux and the soil storage above the soil heat flux plates, air mass storage of sensible and latent heat measured with sensors along vertical profiles) in relation to various data quality filtering steps applied (raw data screening, low turbulence conditions etc.). The results show that improving the measurement and the quality control of the energy components, leads to an average 10% increase of the energy balance closure. This is not yet sufficient to obtain a perfect closure of the balance and further investigation is needed but helps to identify the magnitude of the real imbalance to be explained. Analysis of data collected under different environments and conditions helps also to identify and better understand the main possible causes of the energy balance non-closure.

How to cite: Papale, D., Nicolini, G., Op de Beeck, M., Sabbatini, S., Galvagno, M., and Gielen, B. and the ICOS Ecosystem Stations PIs: How much additional improvements in measurements and data filtering can help to close the energy balance at eddy covariance stations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9974, https://doi.org/10.5194/egusphere-egu23-9974, 2023.

EGU23-10032 | ECS | Orals | AS2.4

Parameterizing surface conductance of different urban vegetation types for the urban land surface model SUEWS with evaluation in two mid-latitude cities 

Hei Shing Lee, Minttu Havu, Anni Karvonen, Joyson Ahongshangbam, Jesse Soininen, Helen C. Ward, Joseph P. McFadden, Annalea Lohila, Stephan Weber, and Leena Järvi

As cities are taking actions to reduce and offset part of their anthropogenic carbon dioxide (CO2) emissions, urban vegetation has become vitally important in pursuing carbon neutrality and climate mitigation. Its effectiveness in carbon sequestration, however, has large uncertainties due to the complex urban environment comprising both natural and artificial elements. By considering seven interacting land surface covers (buildings, pavement, evergreen trees, deciduous trees, grass, soil and water) within each model grid, the Surface Urban Energy and Water balance Scheme (SUEWS) is an urban land surface model that can simulate energy, water and CO2 exchanges in cities. For SUEWS to simulate the CO2 fluxes in urban green spaces, it requires information of maximum photosynthesis and surface conductance of specific urban vegetation as well as the response of surface conductance to environmental conditions. To derive these parameters, it is necessary to utilize on-site measurements conducted over urban green spaces for an accurate description of the surface processes and variables.

To our knowledge, only the mixed vegetation type and street trees in Helsinki have been parameterized in SUEWS so far. In order to extend the flexibility and usability of SUEWS modelling across different cities and for specific urban vegetation, this research aims to (1) derive surface conductance and photosynthesis parameters from eddy covariance and chamber measurements conducted over several urban sites corresponding to different urban vegetation types, such as non-irrigated lawn, turf grass, park trees, urban fields, green roof and urban forests (evergreen and mixed-leaf); and (2) evaluate the impact of selected surface conductance and photosynthesis parameters on SUEWS model performance in two mid-latitude cities: Swindon, UK and Minneapolis-Saint Paul, USA.

The surface conductance and photosynthesis parameters for specific urban vegetation are derived by fitting measurements to an empirical canopy-level photosynthesis model where the effect of the local conditions (i.e. meteorology and ecology) is considered. Using the bootstrapping method to randomly select seven-eighths of the available measurements for 100 times, the fitted maximum photosynthesis rates range from 5.27 μmol m-2 s-1 over an non-irrigated lawn to 10.72 μmol m-2 s-1 over an evergreen forest with the dependencies on the local environmental response functions such as air temperature, incoming shortwave radiation, specific humidity deficit and soil moisture deficit. As a following step, the choice of model parameters in SUEWS simulations will be examined in the two cities along with on-site measurements. 

This research improves SUEWS simulations over urban areas by deriving new surface conductance and photosynthesis parameters specific to different urban vegetation types and provides a more accurate quantification of their biogenic CO2 flux in a complex urban environment. The results also provide a better understanding on the carbon sequestration potential of urban vegetation, which will be useful in planning urban green spaces to maximize natural carbon sinks and in setting climate mitigation strategies.

How to cite: Lee, H. S., Havu, M., Karvonen, A., Ahongshangbam, J., Soininen, J., Ward, H. C., McFadden, J. P., Lohila, A., Weber, S., and Järvi, L.: Parameterizing surface conductance of different urban vegetation types for the urban land surface model SUEWS with evaluation in two mid-latitude cities, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10032, https://doi.org/10.5194/egusphere-egu23-10032, 2023.

EGU23-10175 | Posters on site | AS2.4

Mapping of traffic emissions from a busy road in a rural village using gaseous perfluorocarbon tracers 

James Matthews, Anwar Khan, and Dudley Shallcross

The exposure of populations to toxic traffic emissions is an important concern and significant research effort has been put into measuring and modelling exposure to traffic related pollutants within urban areas. It is also the case that busy trunk roads can pass through villages and towns subjecting those populations to both particulates and pollutant gases. Often, smaller villages in urban areas have complex topographies and provide a different environment to cities with regard to pollutant dynamics. Perfluorocarbon (PFC) trace gases are useful to measure the flow of gases within an area [1]. PFCs are inert, non-depositing and non-toxic and can be detected at low levels using sufficiently sensitive mass spectrometers and preconcentration devices [2]. To understand the passage of gaseous pollutants from a busy road passing through a rural village in Southern England, PFCs were released from a fixed and a moving source and sampled in several locations downwind.

Eight experiments occurred over three different measurement periods, three in June 2021, two in February 2022 and two in May 2022, covering different times of day and meteorological and road conditions. In each experiment, perfluoromethylcyclohexane was released from a fixed position approximately 400 m downwind of the road (July, Feb) or on the road west of the village (May) for 15 minutes, while 1,3-perfluorodimethylcyclohexane was released from the passenger side of a moving vehicle travelling with the flow of traffic through the village. 30-minute Tedlar bag samples were collected in up to 10 locations, some of these locations also measured PM10, PM2.5 and PM1 using an Alphasense N3 optical particle sensor. Bag samples were stored separately from release equipment and transported to Bristol University School of Chemistry for analysis using the methodology described in [3].

Wind directions during the experiments were south westerly and westerly. The highest tracer concentrations from the moving source were often measured within a bus stop roadside in the centre of the village, whereas the static release was highest at a residential roadside sample on the western side of the village. Two samples were taken roadside in a church yard and at the top of the spire, the moving release was consistently higher at ground level, but from the stationary release the tracer was predominantly higher in concentration at roof height.  

[1] Shallcross, D. E. et al. 2009. Atmospheric Science Letters, 10(2), 59-65.

[2] Simmonds, P. G. et al .1995. Analytical Chemistry, 67(4), 717-723.

[3] Matthews, J. C. et al. 2020. Boundary-Layer Meteorology, 175(1), 113-134.

How to cite: Matthews, J., Khan, A., and Shallcross, D.: Mapping of traffic emissions from a busy road in a rural village using gaseous perfluorocarbon tracers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10175, https://doi.org/10.5194/egusphere-egu23-10175, 2023.

EGU23-10397 | ECS | Orals | AS2.4

On the impact of leaf-level processes on the water and carbon canopy-turbulent fluxes 

Raquel González Armas, Jordi Vilà-Guerau de Arellano, Hugo de Boer, Oscar Hartogensis, Mary Rose Mangan, and Fabien Gibert

Representing the diurnal variability of state meteorological variables, including carbon dioxide, is still an open challenge as shown by the large discrepancies with observations and weather and climate models. These discrepancies translate into different diurnal exchanges of heat, water and carbon dioxide between the canopy and atmosphere. These sub-diurnal differences can propagate to larger temporal and spatial scales.

With a systematic approach, we investigate the diurnal gas exchange of both water and carbon dioxide for an irrigated crop. Our investigation is based on a comprehensive observational dataset that ranges from scales covering from the leaf level to the canopy level  to the atmospheric boundary layer gathered at the LIAISE campaign. This campaign took place over two weeks in summer of 2021 in a region of the Ebro basin located in Catalonia, Spain. We focus specially on one of the “supersites” of the campaign: La Cendrosa, which is an irrigated alfalfa field surrounded by a very dry region.

Our observational approach is bottom-up in which we first analyze the leaf, second the canopy and third the interactions with the atmosphere at a local field scale. Among the observations, we analyzed leaf gas exchange measurements, turbulent surface fluxes and vertical profiles of driving environmental variables such as radiation, wind, temperature, and specific humidity. To support the observational analysis, we use a land-atmospheric interactive model (CLASS model). This model allows the representation at each of the three levels mentioned: (1) leaf, (2) canopy and (3) field.

Our observations show an asymmetry in the diurnal variability of the stomatal conductance, which indicates a larger opening of the stomata during the morning than during the afternoon. To attribute processes to the causality in the stomatal opening, we derive new expressions of the tendency of the stomatal aperture as a function of the mean meteorological drivers including radiation, temperature, atmospheric CO2 concentration, and water vapor deficit. The asymmetry is only simulated by models once specific characteristics of the crop are considered. It is also observed that dynamics at the leaf level such as a closure of the stomata during the midday can cause a dip in the evapotranspiration and enhance the sensible heat flux. Our results open the debate on the circumstances under which it is important to constrain the leaf gas exchange.

How to cite: González Armas, R., Vilà-Guerau de Arellano, J., de Boer, H., Hartogensis, O., Mangan, M. R., and Gibert, F.: On the impact of leaf-level processes on the water and carbon canopy-turbulent fluxes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10397, https://doi.org/10.5194/egusphere-egu23-10397, 2023.

EGU23-10938 | ECS | Orals | AS2.4

Parameterizing the Large Scale Impact of Land Surface Heterogeneity Induced Circulations on Convective Cloud Development 

Tyler Waterman, Andrew Bragg, Finley Hay-Chapman, Paul Dirmeyer, Meg Fowler, and Nathaniel Chaney

Understanding the role of surface heterogeneity of surface fluxes in the development of convection is a critical topic in land-atmosphere interactions. This is especially relevant in the context of Earth System Models (ESMs), where simulated sub-grid surface heterogeneity over the land surface is mostly ignored by the overlying modeled atmosphere. Indeed, previous studies using Large Eddy Simulation (LES) have shown that heterogeneities in the surface field below ESM spatial resolution (~100 km) can cause appreciable secondary circulations and, at times, a significant increase in convective cloud development. These large scale changes initiated by small scale heterogeneity have yet to be adequately parameterized in ESMs. To address this particular weakness, this presentation presents a parameterization scheme for a near surface density driven circulation between two lower atmosphere columns with variable surface heating for use within ESMs.

The secondary circulation parameterization is fit to data from 184 LES runs over 92 days, one run each day with a homogeneous surface and one run each day with a heterogeneous surface derived from land surface model output, over a 100 km square domain centered around the ARM site in the US Southern Great Plains (SGP) in Oklahoma. It is then tested over those 92 simulation days at the SGP site, as well as shallow convective days over four heterogeneous sites where differential heating is common: Wisconsin (lake-land), Florida (ocean-land), Missouri (urban-rural) and Appalachia (elevation). 

To test the circulation scheme, we use standalone columns of Cloud Layers Unified by Binormals (CLUBB) a boundary layer, cloud and shallow convection scheme used in multiple modern ESMs. CLUBB is run for three cases on each simulation day at each site: 1) as a single homogeneous column model over the domain, 2) as two separate columns over high and low sensible heat portions of the domain, and 3) following 2) with the addition of the circulation parameterization scheme. The homogeneous CLUBB simulations and those with secondary circulations are compared to evaluate the impact of the secondary circulation on cloud development, turbulent kinetic energy, and profiles of the means and variances of heat and moisture. Results over the SGP site show that the parameterized circulation yields similar changes in cloud development and profiles of heat and moisture to LES.

How to cite: Waterman, T., Bragg, A., Hay-Chapman, F., Dirmeyer, P., Fowler, M., and Chaney, N.: Parameterizing the Large Scale Impact of Land Surface Heterogeneity Induced Circulations on Convective Cloud Development, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10938, https://doi.org/10.5194/egusphere-egu23-10938, 2023.

EGU23-11031 | ECS | Orals | AS2.4

Towards reducing uncertainties of global evapotranspiration due to the energy balance closure gap in flux tower data 

Weijie Zhang, Jacob A. Nelson, Diego G. Miralles, Rafeal Poyatos, Markus Reichstein, and Martin Jung

Accurate quantification of evapotranspiration (ET) is crucial for understanding variability in the global water cycle, yet state-of-the-art estimates of ET derived from models and remote sensing products contain large uncertainties. Taking the advantage of extensive eddy covariance measurements and machine learning algorithms, ET can be upscaled from globally distributed in-situ observations by combining them with global meteorological and satellite data (e.g., FLUXCOM ensembles, Jung et al., 2019). However, eddy covariance measurements suffer from well-known energy balance non-closure problems, and those uncertainties are further propagated to the global ET estimates. Here, we first estimate the energy balance non-closure within dynamic sliding windows for flux tower site, then we compute correction factors for ET measurements following different hypothesis (that assign errors to latent and/or sensible heat fluxes) according to insights from large eddy simulation studies. Then energy balance closure corrected ET data are used in FLUXCOM to estimate global ET. The upscaled ET then is evaluated by comparison with water-balance-drived ET at the catchment level. This comparison helps to determine the most consistent correction of ET for different regions and conditions. By providing improved global ET estimates, water-related studies can be further facilitated, and model parameterizations can be further optimized to address the challenges posed by climate change on ecosystems and water resources.

How to cite: Zhang, W., Nelson, J. A., Miralles, D. G., Poyatos, R., Reichstein, M., and Jung, M.: Towards reducing uncertainties of global evapotranspiration due to the energy balance closure gap in flux tower data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11031, https://doi.org/10.5194/egusphere-egu23-11031, 2023.

EGU23-11370 | Orals | AS2.4

An implementation of the advanced footprint analysis for UAV-based BVOC measurements 

Dmitrii Krasnov, Valentina Zolotarjova, Alisa Krasnova, Kaia Kask, Ülo Niinemets, and Steffen Noe

Biogenic volatile organic compounds (BVOCs) are emitted into the atmosphere by plants and other living organisms and play a significant role in various plant functions, such as growth, reproduction, and defense. BVOCs are also an essential part of many chemical reactions in the atmosphere and contribute to the formation of ozone and secondary organic aerosols and affect the radiation balance.

Investigating the atmospheric vertical profile concentrations of BVOCs has become an important focus for understanding these processes. There are various methods that can be used to study the atmospheric vertical profile, including towers, balloons, aircraft, and unmanned aerial vehicles (UAVs). Among these methods, UAVs offer greater flexibility for local air sampling by hovering over a target area and can reach altitudes of up to 1000m, making them ideal for permanent BVOCs monitoring that requires repeated measurements in a specific spatial and temporal domain. However, the source contribution area of the obtained BVOCs concentrations is often not identified, potentially leading to inaccurate conclusions about the exchange between the surface, vegetation, and atmosphere above the target area.

In this study, the vertical profile of BVOCs concentrations was obtained at SMEAR Estonia (Station for Measuring Ecosystem Atmosphere Relations) to analyze the composition and distribution of these compounds in the near-surface layer. The vertical samples were collected in 2020-2021 using a commercially available pump equipped with cartridges filled with adsorbents and mounted on a UAV. The UAV was used to collect samples from heights between 0 m and 90 m.

To address the issue of space-time representativeness related to the source signal, a footprint analysis was conducted. Micrometeorological data for four target areas were obtained from three SMEAR Estonia flux towers. The Flux Footprint Prediction model (Kljun et al., 2015) was used for the footprint calculation. We determined temporal and spatial changes in roughness length (z0) and zero-displacement height (zd) for each day when BVOCs measurements were carried out using meteorological and geospatial data on land cover types and corresponding canopy heights. Due to the presence of surface heterogeneity, z0 and zd varied significantly for each wind sector. Therefore, we ran the spin-up of the FFP model with updated input parameters at each step. For the measurement results interpretation, we also evaluated the representativeness of the obtained footprints over the target areas in the space-time domain and analysed the land cover composition and vegetation characteristics.

In this work, we show how the source contribution area of BVOCs concentrations can vary in size and shape depending on atmospheric conditions, and spatial and temporal variation and thus have an effect on the obtained species composition of BVOCs.  Based on the presented findings we discuss the potential implementation of this approach for similar research and its future development.

How to cite: Krasnov, D., Zolotarjova, V., Krasnova, A., Kask, K., Niinemets, Ü., and Noe, S.: An implementation of the advanced footprint analysis for UAV-based BVOC measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11370, https://doi.org/10.5194/egusphere-egu23-11370, 2023.

EGU23-11585 | Orals | AS2.4 | Highlight

Impact of a large isolated city on the mixed layer height during different weather conditions 

Daniel Fenner, Andreas Christen, Nektarios Chrysoulakis, Sue Grimmond, Melania Van Hove, Simone Kotthaus, Fred Meier, William Morrison, and Matthias Zeeman

Understanding how cities impact the atmospheric boundary layer is crucial for many processes such as air-pollution dispersion and concentrations, and is therefore important as part of weather and climate modelling. To improve modelling of those dynamic processes observation are critical as they inform development and evaluation of models, and enhance delivery of services to citizens and the management of urban infrastructure, which is vulnerable to different strengths of heat and pollutant exposure.

During a year-long field campaign from Autumn 2021 to Autumn 2022 a comprehensive set of ground-based remote sensing observations were gathered in Berlin, Germany. These allow us to explore the impact of a large city on the regional atmospheric boundary layer. The campaign, undertaken within the European Research Council funded urbisphere project, involved a grid-like network of instruments in the densely built-up city centre, with ground-based remote sensing (e.g. automatic lidars and ceilometers ALC, Doppler-wind lidars) for mixed/mixing layer height (MLH) detection. Additional instruments were located along two perpendicular rural-urban-rural transects, with existing instruments in the city and surrounding region complementing the network. During Intensive Observation Periods (IOP) in spring and summer 2022 radiosonde releases within and outside the city during selected days allow air temperature, humidity and wind-distribution profiles in the atmospheric boundary layer to be investigated.

This contribution showcases how an urban environment modifies the dynamics and convective cloud properties under varying regional-scale weather conditions. We focus on case studies for different synoptic conditions to show the extent of impact of a large city on the MLH within and beyond the urban area, including urban-rural contrasts, upwind-downwind effects, and intra-urban variability of MLH.

How to cite: Fenner, D., Christen, A., Chrysoulakis, N., Grimmond, S., Van Hove, M., Kotthaus, S., Meier, F., Morrison, W., and Zeeman, M.: Impact of a large isolated city on the mixed layer height during different weather conditions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11585, https://doi.org/10.5194/egusphere-egu23-11585, 2023.

EGU23-12035 | Posters on site | AS2.4

A comparison of methods for gap-filling sensible and latent heat fluxes in different climatic conditions 

Erkka Rinne, Henriikka Vekuri, Juha-Pekka Tuovinen, and Mika Aurela

Eddy covariance flux measurements need to be gap-filled when utilising the data for the calculation of annual balances. The measurement technique itself is prone to errors and technical failures may also lead to gaps of various lengths. Gap-filling of the flux time series is typically based on estimating statistically representative values based on various environmental variables through linear regression, lookup tables or machine learning methods.

A large number of methods for the imputation of energy fluxes have been applied and compared in recent literature (Zhu et al. 2022; Mahabbati 2022; Khan, Jeon, and Jeong 2021; Foltýnová, Fischer, and McGloin 2019). Both latent and sensible heat fluxes are strongly driven by the incoming solar radiation, and it is usually used as an independent variable in gap-filling models. Vekuri et al. showed that a widely used method for gap-filling carbon dioxide fluxes creates a systematic bias in northern ecosystems, where the distribution of incoming radiation is highly skewed.

Here, we assess if a similar bias error emerges for sensible and latent heat fluxes after gap-filling with the standard methods or suggested alternatives. We use global data from openly available flux measurement databases and compare the bias and other metrics between different latitudes. We assume that the errors in total energy balances are not as significant as in carbon budgets, but the results could still indicate which methods should be preferred when complete time series of energy flux data are needed.

 

References

Foltýnová, L., M. Fischer, and R.P. McGloin, ‘Recommendations for Gap-Filling Eddy Covariance Latent Heat Flux Measurements Using Marginal Distribution Sampling’, Theoretical and Applied Climatology, Vol. 139, No. 1–2, September 11, 2019, pp. 677–688.

Khan, M.S., S.B. Jeon, and M.-H. Jeong, ‘Gap-Filling Eddy Covariance Latent Heat Flux: Inter-Comparison of Four Machine Learning Model Predictions and Uncertainties in Forest Ecosystem’, Remote Sensing, Vol. 13, No. 24, January 2021, p. 4976.

Mahabbati, A., ‘Investigating the Application of Machine Learning Models to Improve the Eddy Covariance Data Gap- Filling’, The University of Western Australia, 2022.

Vekuri, H., J.-P. Tuovinen, L. Kulmala, D. Papale, P. Kolari, M. Aurela, T. Laurila, J. Liski, and A. Lohila, ‘A Widely-Used Eddy Covariance Gap-Filling Method Creates Systematic Bias in Carbon Balance Estimates’, Scientific Reports, forthcomig.

Zhu, S., R. Clement, J. McCalmont, C.A. Davies, and T. Hill, ‘Stable Gap-Filling for Longer Eddy Covariance Data Gaps: A Globally Validated Machine-Learning Approach for Carbon Dioxide, Water, and Energy Fluxes’, Agricultural and Forest Meteorology, Vol. 314, March 1, 2022, p. 108777.

How to cite: Rinne, E., Vekuri, H., Tuovinen, J.-P., and Aurela, M.: A comparison of methods for gap-filling sensible and latent heat fluxes in different climatic conditions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12035, https://doi.org/10.5194/egusphere-egu23-12035, 2023.

EGU23-12068 | Orals | AS2.4

Evapotranspiration dynamics and partitioning from concurrent above and below canopy flux measurements in a Montane Sierra Nevada Forest 

Sebastian Wolf, Eugenie Paul-Limoges, Dan Sayler, and James W. Kirchner

Evapotranspiration (ET) from the land surface to the atmosphere consists of transpiration (T) from plants and evaporation (E) from soil and vegetated surfaces. These biological and physical component fluxes respond differently to changes in temperature, water availability and atmospheric composition. ET can be measured directly at the ecosystem scale with the eddy covariance (EC) method but similar measurements are not currently available for the component fluxes E and T. Concurrent EC measurements above and below forest canopies provide a promising approach to partition ET into T and E. However, our understanding of the performance of such measurements is still very limited. To address these challenges, we measured and partitioned ET with three concurrent EC towers (1 above & 2 below canopy) in a montane forest at Sagehen Creek in the Sierra Nevada, California from late June 2017 to September 2020. We observed a total forest ET of 606 mm yr-1 with 275 mm yr-1 measured in the understory and a tree transpiration of 331 mm yr-1. Below-canopy measurements replicated at two locations within the above-canopy footprint indicated only small spatial variability for understory ET near the creek at Sagehen. Interannual variability in ET above and below canopy was small during the water years 2018 to 2020, despite large variability in precipitation totals. Accordingly, vegetation water use was relatively stable across years and the P–ET water balance was mainly driven by variations in water supply. Partitioning the components of total forest ET at Sagehen with concurrent EC measurements showed that on average 67–74% originated from T (47% from trees and 20–27% from understory grasses), while 26–33% were from E (mostly from the understory). Our results demonstrate the strength of concurrent above- and below-canopy EC measurements for the partitioning of ET.

How to cite: Wolf, S., Paul-Limoges, E., Sayler, D., and Kirchner, J. W.: Evapotranspiration dynamics and partitioning from concurrent above and below canopy flux measurements in a Montane Sierra Nevada Forest, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12068, https://doi.org/10.5194/egusphere-egu23-12068, 2023.

EGU23-12230 | Posters on site | AS2.4

Effect of thinning on turbulence structure, energy and gas exchange in a boreal forest 

Ivan Mammarella, Abin Thomas, Toprak Aslan, Juho Aalto, Jaana Back, Pasi Kolari, Samuli Launiainen, Olli Peltola, and Timo Vesala

Thinning is performed primarily to manage between-tree competition and allocate growth-limiting resources (e.g. light, water, nutrients) to the remaining trees and to increase their growth rate and vitality. From biophysical point of view, thinning changes tree spacing, number, and size distribution. Our hypothesis is that altered stand structure and decreased foliage density cause modifications of the microclimate, radiation budget and turbulence characteristics within the canopy. Jointly, these physical constraints change the dynamics of biogeochemical cycles and affect mass and energy exchange between soil and vegetation components and the atmosphere.

Here, we investigate the short-term response (i.e. one-two years post thinning) to the thinning done at Hyytiälä forest located in southern Finland. We present results using eddy covariance (EC) fluxes of NEE and ET at both ecosystem level (i.e. above canopy EC) and ground vegetation level (i.e. sub-canopy EC). We found that the forest became a source of carbon during the first post thinning year (+55 gC m-2), while in the second post-thinning year (2021), the ecosystem has only partly recovered showing annual NEE value of -152 gC m-2 which is somehow far from the long-term net uptake measured at the site (-252 gC m-2). Preliminary results show that the thinning had less impacts on ET fluxes. We also report the effect of thinning on ecosystem surface fluxes of carbonyl sulfide (COS), carbon monoxide (CO) and ozone (O3). Here, we hypothesize an increase of CO biogenic emission, due to an increase of amount of litter and light on the forest floor, and a decrease of COS and O3 deposition rates, related to foliage removal.

Finally, the functional response of the flux components are analysed by using clustering and modelling approaches in order to disentangle the roles of thinning and weather on measured fluxes and budgets.

How to cite: Mammarella, I., Thomas, A., Aslan, T., Aalto, J., Back, J., Kolari, P., Launiainen, S., Peltola, O., and Vesala, T.: Effect of thinning on turbulence structure, energy and gas exchange in a boreal forest, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12230, https://doi.org/10.5194/egusphere-egu23-12230, 2023.

EGU23-12898 | ECS | Orals | AS2.4

Application of open photoacoustic cell in an eddy covariance system for water vapor flux measurement 

Péter Torma, Tamás Weidinger, Viktor Juhász, Bence Molnár, László Horváth, Helga Huszár, and Zoltán Bozóki

Water vapor flux plays a crucial role in surface-atmosphere exchange processes as evapotranspiration regulates the energy balance of the surface. Moreover, it transfers water vapor into the atmosphere and, as a result, shapes the hydrological cycle. The eddy-covariance (EC) technique is the most commonly applied method to directly measure water vapor flux over a wide variety of surfaces. An EC arrangement consists of a 3D sonic anemometer and a gas analyzer. To derive surface fluxes, wind components and the gas concentration (e.g. water vapor) have to be recorded with high-frequency (at least at 10 Hz). In the case of open-path (sampling-free) EC systems, infrared (IR) gas analyzers are used dominantly, which are still quite large so that e.g. they cannot be easily mounted on drones. In contrast, small and light sonic anemometers are available for flux measurements.

In this study, we present the application of a sampling-free photoacoustic (PA) sensor for water vapor flux measurement employing the EC technique. The fast response PA sensor records the water vapor concentration through an open cylindrical chamber having an overall size of less than 1 dm3. On the one hand, a previous first test showed that the vertical covariance functions obtained by the PA cell follow closely to those resulting from an accepted IR sensor. On the other hand, the PA system showed some underestimation at higher frequencies based on the analysis of co-spectra.  

To comprehensively test and evaluate the PA cell for flux measurements, a seven-week-long field measurement was performed over a plain grassland when a calibrated EC150 IR sensor (Campbell Sci.) was used as a reference gas analyzer. We analyze the accuracy of the PA system: (i) depending on the orientation of the cell or i.e. the wind direction, and (ii) for a broad range of meteorological conditions, such as different wind speeds and atmospheric stability. Furthermore, to overcome the high-frequency attenuation, we establish and apply empirical spectral transfer functions following the literature and standard EC postprocessing procedures. The characteristic response time of the PA sensor is also assessed.

How to cite: Torma, P., Weidinger, T., Juhász, V., Molnár, B., Horváth, L., Huszár, H., and Bozóki, Z.: Application of open photoacoustic cell in an eddy covariance system for water vapor flux measurement, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12898, https://doi.org/10.5194/egusphere-egu23-12898, 2023.

EGU23-15305 | ECS | Posters on site | AS2.4

Turbulent energy fluxes and surface energy balance closure of a coniferous forest at the complex-terrain site of Renon (Italian Alps) 

Nadia Vendrame, Martina Destro, Mirco Rodeghiero, Leonardo Montagnani, and Dino Zardi

Exchanges of mass and energy between a subalpine coniferous forest and the atmosphere have been continuously monitored since few decades at Renon (Bolzano, Italy) applying the eddy covariance (EC) technique. The station is part of the Integrated Carbon Observation System (ICOS) EU Research Infrastructure. The area surrounding the site is characterized by complex topography, with a mean slope angle of about 11° and a Southward aspect. In this study, we focused on the analysis of turbulent energy fluxes (sensible and latent heat) and the energy budget closure of the forest during a period of about three months (August-October 2021), when a below-canopy EC system was additionally deployed to better understand the dynamics of turbulent exchanges. The energy balance closure was assessed for periods characterized by distinct wind circulation patterns (thermally-driven slope winds vs.  synoptic winds) and turbulent energy fluxes were processed applying different coordinate rotation methods (double rotation and planar fit). We found significant differences in the magnitude of sensible and latent heat fluxes computed with double rotation or planar fit. These differences were more marked during periods characterized by slope winds, suggesting a connection with local advection performed by these winds.

How to cite: Vendrame, N., Destro, M., Rodeghiero, M., Montagnani, L., and Zardi, D.: Turbulent energy fluxes and surface energy balance closure of a coniferous forest at the complex-terrain site of Renon (Italian Alps), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15305, https://doi.org/10.5194/egusphere-egu23-15305, 2023.

EGU23-15468 | Posters on site | AS2.4

Some forests like it cold 

Albin Hammerle, Felix Spielmann, Katharina Scholz, Walter Oberhuber, and Georg Wohlfahrt

Forests cover roughly one third of the global land area and currently remove around one quarter of anthropogenic CO2 emissions, thus slowing down the increase in atmospheric CO2 concentrations. Forests account for approximately 90% of all terrestrial biomass, which corresponds to about 400 Gt C.

However, the ratio of carbon uptake to release is a very fragile one and is determined by many factors such as water and nutrient availability, the amount and quality of light or stand age. In addition to the factors mentioned above, temperature is one of the most important factors that determine this ratio. Both fluxes determining the net ecosystem exchange (NEE), the gross uptake of CO2 by photosynthesis (GPP) and ecosystem respiration (Reco) are sensitive to temperature. Thus, we investigated the temperature sensitivity of NEE at a newly established pine forest field site in Austria at 960 m a.s.l. Applying an understory and an ecosystem scale eddy covariance system we were able to disentangle temperature effects on understory and tree crown CO2 exchange.

We found a clear temperature optimum for CO2 uptake on ecosystem scale at around 20°C and a decrease in uptake on higher temperatures. This decrease was caused by (i) the understory turning from a slight sink for CO2 into a source of CO2 at higher temperatures, and (ii) a reduction of CO2 uptake in the tree canopy layer. Furthermore, we compared carbon flux data with continuous tree growth data from dendrometer measurements.

How to cite: Hammerle, A., Spielmann, F., Scholz, K., Oberhuber, W., and Wohlfahrt, G.: Some forests like it cold, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15468, https://doi.org/10.5194/egusphere-egu23-15468, 2023.

EGU23-15533 | ECS | Orals | AS2.4

Reducing the effects of weather on the sampling bias in tall tower eddy covariance flux measurements 

Konstantinos Kissas, Charlotte Scheutz, and Andreas Ibrom

Tall tower eddy covariance (TTEC) flux measurements are employed to estimate turbulent matter and energy fluxes at landscape scales (e.g. within 1 to 5 km radius around a tower). Virtually all landscapes feature horizontal surface heterogeneity. One main complication for the interpretation of TTEC is the sampling bias by the varying local meteorological conditions. While the wind direction bias can only be considered by the choice of the location of the TTEC, we examine here how the effects of atmospheric stability can be alleviated by sampling from different measurement heights (zm). The objective is to define an optimal set of measurement heights to minimize sampling bias from variation in atmospheric stratification for TTEC long-term flux observation. To our knowledge, this problem has not yet been addressed in the scientific literature.

We used a two years’ dataset from the 122 m tall tower at Risø (Denmark, 55°41'39.15" N, 12°5'17.93" E) and two flux footprint models to develop an objective statistical approach for the definition of a set of measurement heights for optimal sampling of the landscape heterogeneity. The tower is equipped with 3D ultrasonic anemometers in five different heights. The evaluations concern the Eastern sector, which is comprised of a mosaic of land uses, small settlements and comparably sparse road infrastructures.

We define the criteria for optimal landscape flux sampling from the distributions of the source weights (contribution to the measured flux per unit area) sampled in a number of stability classes relative to a frequent unstable stability class as reference. The upper sampling height is set a priory to match measurements and the targeted area; here zm equal to 120 m for the 70% cumulated footprint to stay within a 5 km radius around the tower.

Theoretical analysis with the footprint model shows the limitation of the attempt to compensate for lateral footprint extension at different stabilities, while the longitudinal sampling of the landscape heterogeneity can be maintained more homogeneously by the systematic choice of the measurement height according to atmospheric stability and wind speed.

The results rely on the accuracy of the footprint estimation, which is generally an essential criterion for the interpretation of TTEC measurements in heterogeneous landscapes.

How to cite: Kissas, K., Scheutz, C., and Ibrom, A.: Reducing the effects of weather on the sampling bias in tall tower eddy covariance flux measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15533, https://doi.org/10.5194/egusphere-egu23-15533, 2023.

EGU23-15992 | ECS | Orals | AS2.4

Can fiber-optic distributed sensing be used to resolve temperature turbulence values over time and space? 

Gijs Vis, Oscar Hartogensis, Marie-Claire ten Veldhuis, and Miriam Coenders

Turbulence is essential for land atmosphere interactions; however, it is difficult to quantify because of its statistical nature. Typically, turbulence is determined using time series data, on which Taylor’s hypothesis is applied to obtain turbulent data over a length scale. Taylor’s frozen turbulence hypothesis is an assumption in the core of turbulence research, however currently turbulence measurements are limited to either time series (e.g., sonic anemometers) or integrated spatial measurements (e.g., scintillometers). Therefore, the spatiotemporal nature of turbulence cannot be independently assessed. In this study we use fiber-optic distributed sensing (FODS) to measure turbulence over both time and space.

The turbulence parameter used is the structure parameter of temperature, CT2, which quantifies the intensity of temperature fluctuations over a certain scale. The structure parameter can be determined using temperature series directly, using its definition. Alternatively, the inertial range of the turbulent temperature spectrum can be used to obtain structure parameter through the Kolmogorov -5/3 power law.

A FODS experiment was conducted in the LIAISE (Land surface Interactions with the Atmosphere over the Iberian Semi-arid Environment) field campaign during 15-30 July 2021 in the north-east of Spain. A set-up was installed with a horizontal extent of 70 m, measuring at four heights between 0.40 m and 2.05 m. A thin 0.5 mm cable was used in an effort to obtain the fastest possible time response. Measurements were made at 1 Hz and 12.7 cm resolution, however the actual sampling frequency appeared to be 0.15 Hz in the temperature spectrum, likely because of the long response time of the cable.               

Despite the limited 0.15 Hz sampling rate it was possible to obtain turbulence information through the use of the structure parameter of temperature. This parameter indicates the intensity of temperature fluctuations and was calculated over time, as is conventional. In a novel approach, it was also calculated over space. The spatial structure parameter obtained through the definition method was found to have the best correlation with a sonic anemometer reference, with a correlation coefficient of 0.88.

The temporal structure parameter lacks the structure that is shown in the spatial method, which is likely due to the use of 30-min averaged data for horizontal wind speed from the sonic anemometer or to Taylor's frozen turbulence hypothesis not being a suitable assumption within the dimensions of this research. Determining structure parameters through the turbulent spectrum was successful for limited data points for the time seriess and is currently inconclusive for the spatial series. This work provides a first step towards using FODS in capturing turbulent information along spatial temperature series.

How to cite: Vis, G., Hartogensis, O., ten Veldhuis, M.-C., and Coenders, M.: Can fiber-optic distributed sensing be used to resolve temperature turbulence values over time and space?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15992, https://doi.org/10.5194/egusphere-egu23-15992, 2023.

EGU23-16002 | ECS | Posters virtual | AS2.4

A comparison of two approaches of dust deposition for Parabolic Trough Collector Mirrors 

Athanasios Voukelatos, Aggeliki Anastasiou, Johannes Christoph Sattler, Spiros Alexopoulos, Siddharth Dutta, and Ioannis Kioutsioukis

Abstract

This study presents a soiling forecasting (SF) tool developed by the University of Patras in order to predict the deposition of dust on Parabolic Trough Collector (PTC) mirrors. The SF estimation is occurred from the ADTM models. Dust accumulation from sedimentation, Brownian motion and impaction are considered in the estimation of deposition velocity. Moreover, the impact of rainfall is also considered. The computational procedure was divided into the laminar flow regime and the turbulence flow regime in order to estimate the rate at which dust particles can accumulate on the surface of a PTC mirror.

The meteorological data used in the model's training were taken from a weather station at the company KEAN Soft Drinks Ltd. in Limassol, Cyprus (PTC location), and the particle concentrations were obtained from CAMS global atmospheric forecasts [1]. Two variants of the model were used. The first model uses PM2.5 and PM10 (kg/m3). The second model uses a wider distribution of aerosols. Specifically, dust aerosol mixing ratio in the bins 0.03-0.55 μm, 0.55-0.9 μm and 0.9-20 μm were used.

The reflectivity estimations from both models were compared with the available PTC mirror reflectivity measurements to confirm the effectiveness of the SF tool [2]. The validation measurement campaign was conducted from June 3rd to June 7th, 2019. A major soiling event occurs within the first three days which increases gradually until June 5th and then recedes. For the chosen validation period, both models accurately captured the phasing and magnitude of reflectivity. Figure 1 illustrates the soiling mechanisms for the first model and the Figure 2 for the second model respectively. The wind speed during the 4-day period was below 6.8 m/s (laminar flow threshold). The larger particles included in the second model and the corresponding deposition velocity of the coarse particles resulted at higher values for Sedimentation and Brownian motion while Impaction had the same range between the two models (because the wind is the dominant factor of this mechanism). Therefore, the coarser particles resulted in increased influence of sedimentation over impaction in model 2. In both models, the impact of Brownian deposition was the least among the mechanisms. Moreover, the sedimentation had the highest influence, at most hours, in the modelled deposition velocity with occasional outbursts of impaction. The process of calibrating the models with data covering various atmospheric conditions is ongoing.

Fig. 1: Input data, soiling mechanisms and reflectivity for model 1.

 

Fig. 2: Input data, soiling mechanisms and reflectivity for model 2.

 

Acknowledgements

Smart Solar System (S3) project is supported under the umbrella of SOLAR-ERA.NET Cofund by Projektträger Jülich – Forschungszentrum Jülich GmbH – Energie-Technologie-Nachhaltigkeit (ETN 1) and General Secretariat of Research and Innovation (GSRI). SOLAR-ERA.NET is supported by the European Commission within the EU Framework Programme for Research and Innovation HORIZON 2020 (Cofund ERA-NET Action, N° 691664).

 References

[1] CAMS, https://atmosphere.copernicus.eu

[2] P. K. Ktistis, R. A. Agathokleous, and S. A. Kalogirou, “Experimental performance of a parabolic trough collector system for an industrial process heat application,” Energy, doi: 10.1016/j.energy.2020.119288.

How to cite: Voukelatos, A., Anastasiou, A., Sattler, J. C., Alexopoulos, S., Dutta, S., and Kioutsioukis, I.: A comparison of two approaches of dust deposition for Parabolic Trough Collector Mirrors, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16002, https://doi.org/10.5194/egusphere-egu23-16002, 2023.

EGU23-16012 | ECS | Orals | AS2.4

Five-year inter-annual variation in the net landscape carbon balance of a managed boreal forest landscape in Sweden 

Jinshu Chi, Anne Klosterhalfen, Mats Nilsson, Hjalmar Laudon, Anders Lindroth, Natascha Kljun, Jörgen Wallerman, Johan Fransson, Tomas Lundmark, and Matthias Peichl

The boreal biome exchanges large amounts of carbon (C) with the atmosphere and thus significantly affects the global climate. A managed boreal landscape typically consists of various sinks and sources of carbon dioxide (CO2), methane (CH4), and dissolved organic and inorganic carbon (DOC and DIC) across forests with different stand ages, mires, lakes, and streams. Due to the spatial heterogeneity, a full understanding of the landscape-scale C balance requires capturing all C fluxes. Here, we investigate the five-year interannual variability in the net landscape carbon balance (NLCB) by compiling terrestrial and aquatic fluxes of CO2, CH4, DOC, DIC, and harvested C obtained from 2016 to 2020. For that purpose, we applied tall-tower eddy covariance measurements, stream monitoring, and remote sensing of biomass stocks (i.e. harvested C via clearcutting) to estimate the landscape-scale C fluxes across the land-water-atmosphere continuum for an entire boreal catchment (~68 km2) in Sweden. Our results show that this managed boreal forest landscape was a net C sink during 2016-2020 (123 ± 63 g C m-2 yr-1) with the lowest and highest sink-strength occurring during a wet year 2017 (16 g C m-2 yr-1) and a drought year 2019 (182 g C m-2 yr-1), respectively. The net landscape-atmosphere CO2exchange was the dominant component of NLCB, followed by the C export via harvest and streams. We further found that global radiation and vapor pressure deficit regulated the inter-annual variations of NLCB, whereas forest biomass and source area contribution of mires determined its spatial variability. Overall, our multi-year NLCB investigations provide a holistic understanding of the inter-annual variations in NLCB of managed boreal forest landscapes to better evaluate their potential for mitigating climate change.

How to cite: Chi, J., Klosterhalfen, A., Nilsson, M., Laudon, H., Lindroth, A., Kljun, N., Wallerman, J., Fransson, J., Lundmark, T., and Peichl, M.: Five-year inter-annual variation in the net landscape carbon balance of a managed boreal forest landscape in Sweden, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16012, https://doi.org/10.5194/egusphere-egu23-16012, 2023.

Kolkata, one of the oldest and largest urban centres in Asia echoes all the major characteristics of cities from developing countries experiencing rapid urbanization and unplanned development. This study focuses on understanding the impact of intra-urban variations within a morphologically complex metropolis and its capability to modify the enveloping atmospheric conditions at the meso to micro-scale. The Weather Research and Forecasting (WRF) model was configured using a 3-tier nested domain to conduct high-resolution simulations incorporating improved land surface and urban parameterization and appropriate physical parameterization. Local Climate Zone (LCZ) map representing the land use land cover (LULC) was prepared for the innermost domain covering the city and surroundings using Planet-Scope datasets for 2019, adopting Artificial Neural Network (ANN) approach and validated using ground information. This was then integrated into the model with redefined values of specific urban parameters for a better representation of the city’s morphology. It was observed that LCZ-2 (Compact Mid-rise) and LCZ-3 (Compact Low-rise) cover almost the entire core city and around 70 % of the total built-up extent of the study area, which also consists of LCZ-5 (Open Mid-Rise) and LCZ-6 (Open Low-Rise) regions. Thus, the model was calibrated according to the surface and atmospheric conditions of the region and its performance was evaluated in comparison with ground observations. Simulations were conducted at hourly intervals for a 10-day period (August 2019) during the peak summers coinciding with the south-west monsoon period receiving heavy rain spells, to analyse the impact of heterogenous urban form on the micro-climatic variations within the city as well as its surroundings. The modelled results obtained for 2m air temperature (Tair), surface temperature (Tskin), 10m Wind Speed (WS) and Rainfall (RF) indicated a significant influence of the different LCZ classes and their spatial variations over the city. The average daytime Tair and Tskin values in the LCZ-2 is about 1℃ and 1.5℃ higher than LCZ-3, which is again 0.7℃ and 1.5℃ higher compared to the other urban LULC classes where the internal variation is relatively less. Further, the average temperature differences between the compact and open built-up structures increase significantly during night (2℃ – 3.5℃), further increasing when compared to the peri-urban (around 5℃). The inter-urban heterogeneity however, has a reverse effect on the average WS even during the typical monsoon period, with lowest speed observed in the compact core (2ms-1 – 5ms-1) due to highest surface drag (d), increasing (3ms-1 – 7ms-1) along LCZ-5 and LCZ-6 with reduction in d; which further increases substantially in the peri-urban areas (10ms-1 – 15ms-1) with lowest value of d. The variations in total RF received from the complex towards peripheral urban also depicts a similar pattern, as average RF intensity is the lowest within LCZ-2 and LCZ-3 (7mm/hr – 15 mm/hr), moderate in LCZ-5 and LCZ-6 (10mm/hr – 20mm/hr) and highest along the peri-urban areas (15mm/hr – 35 mm/hr). Thus, urban structural and morphological complexity can have a substantial effect on the local-scale climatic variations even along small horizontal distances within a city.

How to cite: Bhattacharjee, S. and Bharti, R.: Intra-urban morphological heterogeneity and its impact on the micro-climatic variations in the Kolkata Metropolitan region of India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16058, https://doi.org/10.5194/egusphere-egu23-16058, 2023.

EGU23-17499 | ECS | Posters on site | AS2.4

Studying the Atmospheric Boundary Layer influence on the Surface EnergyBalance Closure combining eddy covariance and Doppler lidar 

Sergio David Aguirre García, Juana Andújar-Maqueda, Jesús Abril-Gago, Sergio Aranda- Barranco, Daniel Agea-Plaza, Pablo Ortiz-Amezcua, Enrique P. Sánchez-Cañete, Andrew-S. Kowalski, Penélope Serrano-Ortiz, and Juan-Luis Guerrero-Rascado

The eddy covariance technique (EC) is used worldwide to measure surface fluxes of greenhouse
gases and energy balance components. Nevertheless, in the scientific community it is well-known
that EC presents an imbalance of the energy components. In this regard, the atmospheric boundary
layer (ABL) directly influences the mass and energy transfer between surface and atmosphere.
Thus, knowledge and characterization of the ABL might be essential to disentangling the drivers
causing the imbalance of the energy components measured by EC. This work aims to relate ABL
characteristics to the accuracy of the surface energy balance closure (SEBC) obtained by EC.

The study was carried out in an irrigated olive orchard (Olea europaea var. europaea L.) in the
Southeastern Iberian Peninsula (37.9427º N, 3.3002º W and 370 m asl) during the intensive
BLOOM (turBulence and oLea pOllen prOperties experiMent) campaign, from May 19th to June
20th 2022. In order to characterise ABL dynamics, remote sensing techniques are commonly used.
One of them is via Doppler lidar, which provides measurements of wind components and
turbulence-related products at high spatial and temporal resolutions. In particular, a Doppler lidar
Stream Line (HALO photonics) with a temporal resolution of 2 seconds and 10 minutes (for vertical
and scanning measurements, respectively) and 30 m of vertical spatial resolution was used to
retrieve the turbulent kinetic energy dissipation rate (ε) and wind shear (sh) with a common
resolution of 3 minutes as indicators of convective and mechanical sources of turbulence,
respectively. To assess the SEBC, we used (1) a three-axis sonic anemometer (CSAT-3, Campbell
Scientific, Logan, UT, USA) and an enclosed path infrared gas analyser (IRGA, Li-Cor 7200;
Lincoln, NE, USA) on a tower 9 m tall to measure latent heat (λE) and sensible heat (H) fluxes; (2)
an incoming and outgoing short- and long-wave 4-component radiometer (CNR-4, Kipp & Zonen,
Delft, Netherlands) to measure net radiation (Rn); and (3) two each: soil moisture probes (CS616,
CSI), thermocouples (TCAV, CSI) and heat flux plates (HFP01, Hukseflux, Delft, the Netherlands)
at 0.10 m, 0.04 m and 0.08 m depth, respectively to calculate the soil heat flux (G).

Preliminary results show that SEBC enhances under turbulent conditions (slope and R2 from 0.49
and 0.92 to 0.81 and 0.94, respectively). However, when the source of turbulence is mechanical the
SEBC is less accurate (slope and R2 from 0.82 and 0.94 to 0.77 and 0.9, respectively). A more
detailed study based on principal component analysis of the ABL height, skewness of the vertical
wind velocity and vertical profile of horizontal wind, together with ε and sh, among other Dopplerlidar-
derived products is expected to offer reliable information that is highly relevant regarding the
influence of the ABL on the SEBC.

ACKNOWLEDGMENTS: This work was supported by the
Spanish Ministry of Science and Innovation through project PID2020-117825GB-C21
(INTEGRATYON3), the Andalusian regional Development through the projects B-RNM-60-
UGR20 (OLEAGEIs) and P18-RT-3629 (ICAERSA), including European Union ERDF funds.

How to cite: Aguirre García, S. D., Andújar-Maqueda, J., Abril-Gago, J., Aranda- Barranco, S., Agea-Plaza, D., Ortiz-Amezcua, P., Sánchez-Cañete, E. P., Kowalski, A.-S., Serrano-Ortiz, P., and Guerrero-Rascado, J.-L.: Studying the Atmospheric Boundary Layer influence on the Surface EnergyBalance Closure combining eddy covariance and Doppler lidar, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17499, https://doi.org/10.5194/egusphere-egu23-17499, 2023.

Flux partitions between surface water and energy terms are essentially important to the climate system. They can potentially affect assessments of climate risk projections in the future. However, the characterization of surface flux partitioning in numerical models is rarely evaluated due to the absence of large-scale observational evidence. Here, we use long-term satellite datasets and observational meteorological records to evaluate the flux partitioning regime presented in four widely-used Land surface models (LSMs) over two study regions (i.e., China and Continental U.S.). We show that the regime in LSMs differs significantly from satellite-based estimations, which can be due to unrealistic representations of land surface characteristics. The biases in models’ flux partitioning regime may lead to the underestimated potential for climate risks, especially over regions with typical land surface characteristics. The results highlight that particular attention should be paid to the calibration of surface flux partitioning regimes in LSMs. Large model spreads in surface flux partitioning strength and climate risk maps are also reported.

How to cite: He, Q., Lu, H., and Yang, K.: Observation-based assessments of surface flux partitioning regimes in 4 commonly-used land surface models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-333, https://doi.org/10.5194/egusphere-egu23-333, 2023.

In recent years, drought has become an increasing problem in agricultural production in many places where these problems did not exist in the past. The frequency and intensity of agricultural droughts are increasing, so it is very important to detect temporal and spatial variability of drought. This study analyzed the properties of agricultural drought (duration and intensity) in Bărăgan region (Romania) and Prekmurje region (Slovenia) between 1991-2020 based on the Standardized Precipitation Index (SPI) and the Standardized Precipitation Evapotranspiration Index (SPEI) at different time scales. The reasons for comparing the two regions are similar climatic conditions, the importance of maize cultivation for food security, and repeated droughts in the recent period in these regions. The meteorological data for Romania were provided from ROCADA database, and for Slovenia from SLOCLIM database. Furthermore, relationships between drought-sensitive phenological stages of maize (germination, formation of the first 2 leaves, and flowering), growing season length, thermal time above threshold 10 °C, standardized yields, and calculated drought indicators were calculated. Based on our analysis, we expect to be able to evaluate whether SPI and SPEI can be used to monitor conditions on a variety of time scales and to provide indicators at regional scales on the likely occurrence of drought during critical phenological phases of maize, as well as the differences and similarities between the two regions will be discussed.

How to cite: Kobulniczky, B., Holobâcă, I.-H., Črepinšek, Z., Pogačar, T., Jiman, A.-M., and Žnidaršič, Z.: Comparison of Standardized Precipitation Index (SPI) and Standardized Potential Evapotranspiration Index (SPEI) applicability for drought assessment during the maize growing period between Bărăgan (Romania) and Prekmurje (Slovenia) regions (1991, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-499, https://doi.org/10.5194/egusphere-egu23-499, 2023.

The surface-air temperature difference (Ts-Ta) is the main contributor to the sensible heat flux, and also an important indicator for land degradation. However, as the main influencing factor, the effect of soil moisture (SM) on Ts-Ta at the global scale has not been well articulated. Here, based on the ERA5-land reanalysis data from 1981 to 2019, the impacts of SM on Ts-Ta were studied. It was found that Ts-Ta over 54% of the global land increased, and SM across 70.7% of the world land decreased. In the increased SM areas, the increased soil evaporation weakened the increasing trend of Ts resulting in smaller Ts-Ta. In the decreased SM areas, the latent heat flux increased with soil evaporation and Ts-Ta decreased when SM was relatively high, and the larger sensible heat flux due to decreased soil evaporation aggravated Ts-Ta when SM was relatively low. The effect of SM on Ts-Ta presented nonlinear relationship due to the different background value of SM and temperature. The variation of SM at low SM or low temperature areas had an amplification effect on Ts-Ta. These findings will provide new insights into the different regional characteristics of global changing climate and the improvement of land degradation assessment indicators.

How to cite: jiang, K.: Influence patterns of soil moisture change on surface-air temperaturedifference under different climatic background, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-557, https://doi.org/10.5194/egusphere-egu23-557, 2023.

EGU23-799 | ECS | Posters on site | CL4.1

The role of atmospheric humidity in controlling land-atmosphere feedbacks over forest: regional and global-scale analyses 

Shulin Zhang, Weiguang Wang, and Adriaan J. Teuling

Abstract:

The interaction of land cover and atmosphere can affect the climate patterns via biogeochemical and biogeophysical process. The afforestation contributes to increase the biogeochemical cycles like carbon sequestration. Meanwhile, the landcover change modify the biogeophysical parameters perturbs the energy and water fluxes. The latter will be the most direct process to affect the atmosphere and its effects from landcover change outweigh radiative forcing triggered off by CO2 emissions.

After the “Grain to Green Program”, the Loess Plateau (LP) has experienced a widespread forest expansion. Up to 2012, the extension of forest area in the central LP (Ningxia, Shanxi, and Shaanxi) accounted for 11.2 % of the area of the three provinces. The greening trend has changed the energy and water cycle, hence to a climate variability. The moist heat stress (a combined climate metric) has been recently investigated because it is directly related to human health. However, the affection of afforestation to moist heat stress is still unclear in LP.

In a recent study, we used the Weather Research and Forecasting (WRF) model to simulate the modulation of moist heat in LP caused by the afforestation. The result demonstrates that the intensive revegetation in LP shows a cooling effect on regional average near surface air temperature, especially in central LP. In addition, an increase of relative humidity caused by afforestation is detected. Driving by the near-surface temperature, sensible heat flux, and the subsidence of the planetary boundary layer the moist heat stress has obvious change after afforestation. The average moist heat stress decreases in central LP. While the decrease rate of moist heat stress is slower than near-surface temperature. It is worth noting that, an increased signal occurs in the maximum moist heat stress which might expose humans to the risk of moist heat stress. Our sensitivity results imply that the moist heat stress should be accounted for in climate change adaptation.

In ongoing work, we study the role of atmospheric VPD on mitigating land-atmosphere feedbacks over forest and non-forest land cover based on a global analysis of FLUXNET data. Preliminary results show a strong climate control on the effect of VPD on land-atmosphere exchange, in particular during heatwaves.

Reference: Zhang, S., Wang, W., Teuling, A. J., Liu, G., Ayantobo, O. O., Fu, J., & Dong, Q. (2022). The effect of afforestation on moist heat stress in Loess Plateau, China. Journal of Hydrology: Regional Studies, 44, 101209

How to cite: Zhang, S., Wang, W., and Teuling, A. J.: The role of atmospheric humidity in controlling land-atmosphere feedbacks over forest: regional and global-scale analyses, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-799, https://doi.org/10.5194/egusphere-egu23-799, 2023.

The EC-Earth earth system model is characterized by biases in various aspects of the simulated climate. Biases in precipitation result in biases in soil moisture, while biases in temperature and precipitation contribute to biases in vegetation. In this study, the extent to which the biases in soil moisture and vegetation contribute to the biases in the surface energy fluxes (which, in turn, lead to near-surface climate biases) in EC-Earth through interactions with the atmosphere is investigated.

The study is based on two simulations for the recent period 19719-2017: an offline simulation with the land-surface component of EC-Earth, combining the HTESSEL land surface model and the LPJ-GUESS dynamical vegetation model forced, by the meteorological conditions from the ERA5 re-analyses, and a simulation with the atmospheric version of EC-Earth, where the land-surface conditions, i.e., soil moisture and vegetation, are prescribed from the offline simulation.

The purpose of the study is twofold: By comparing the offline simulation with the land-surface component of EC-Earth with observational estimates of the surface energy fluxes, it is investigated to which extent the land-surface component, combing HTESSEL and LPJ-GUESS, is capable to simulate the surface energy fluxes under “perfect” climate conditions. And by comparing the simulation with the atmospheric component of EC-Earth with the offline simulation, the effects of the land-surface atmosphere interactions on the biases of the surface energy fluxes in EC-Earth are assessed. These effects are, to a large extent, related to climate biases in the atmospheric component of EC-Earth, e.g., the radiative fluxes, precipitation or the near-surface climate conditions.

How to cite: May, W.: The role of land-surface interactions for the surface energy fluxes in the EC-Earth earth system model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1067, https://doi.org/10.5194/egusphere-egu23-1067, 2023.

EGU23-1689 | ECS | Posters on site | CL4.1

Contrasting influences of biogeophysical and biogeochemical impacts of historical land use on global economic inequality 

Shu Liu, Yong Wang, Guang Zhang, Linyi Wei, Bin Wang, and Le Yu

Climate change has significant implications for macro-economic growth. The impacts of greenhouse gases and anthropogenic aerosols on economies via altered annual mean temperature (AMT) have been studied. However, the economic impact of land-use and land-cover change (LULCC) is still unknown because it has both biogeochemical and biogeophysical impacts on temperature and the latter differs in latitudes and disturbed land surface types. In this work, based on multi-model simulations from the Coupled Model Intercomparison Project Phase 6, contrasting influences of biogeochemical and biogeophysical impacts of historical (1850–2014) LULCC on economies are found. Their combined effects on AMT result in warming in most countries, which harms developing economies in warm climates but benefits developed economies in cold climates. Thus, global economic inequality is increased. Besides the increased AMT by the combined effects, day-to-day temperature variability is enhanced in developing economies but reduced in developed economies, which further deteriorates global economic inequality.

How to cite: Liu, S., Wang, Y., Zhang, G., Wei, L., Wang, B., and Yu, L.: Contrasting influences of biogeophysical and biogeochemical impacts of historical land use on global economic inequality, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1689, https://doi.org/10.5194/egusphere-egu23-1689, 2023.

Heavy precipitation (HP) events can be preceded by moist heatwaves (HWs; i.e., hot and humid weather), and both can be intensified by urbanization. However, the effect of moist HWs on increasing urban HP remains unknown. Based on statistical analyses of daily weather observations and ERA5 reanalysis data, we investigate the effect of moist HWs on urban-intensified HP by dividing summer HP events into NoHW- and HW-preceded events in the Yangtze River delta (YRD) urban agglomeration of China. During the period 1961–2019, the YRD has experienced more frequent, longer-lasting, and stronger intense HP events in the summer season (i.e., June–August), and urbanization has contributed to these increases (by 22.66%–37.50%). In contrast, urban effects on HP are almost absent if we remove HW-preceded HP events from all HP events. Our results show that urbanization-induced increases in HP are associated with, and magnified by, moist HWs in urban areas of the YRD region. Moist HWs are conducive to an unstable atmosphere and stormy weather, and they also enhance urban heat island intensity, driving increases in HP over urban areas.

How to cite: Gu, X., Li, C., and Slater, L.: Urbanization-Induced Increases in Heavy Precipitation are Magnified by Moist Heatwaves in an Urban Agglomeration of East China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1814, https://doi.org/10.5194/egusphere-egu23-1814, 2023.

EGU23-2064 | ECS | Posters virtual | CL4.1

Hot weather amplifies the urban dry island effect, especially in wetter climates 

Sijia Luo and Xihui Gu

Atmospheric humidity is usually drier in cities than the surrounding rural areas, a phenomenon known as the urban dry island (UDI) effect. However, the response of atmospheric humidity to hot weather in urban versus rural settings remains unknown. Using long-term summer (June-August) observations at 1658 stations over 1961-2020, we find that China is dominated by drying trends in atmospheric humidity (i.e., increasing vapor pressure deficit [VPD]). These drying trends are aggravated on hot days and amplified by urbanization, i.e., the UDI effect is stronger in hot weather. This amplification of the UDI effect on hot days is more prominent in humid than in arid regions. Attributions show that the stronger VPD-based UDI effect on hot days is explained by increased contribution of air temperature in southeastern China, and specific humidity in North China. We suggest that adaptations are required to mitigate adverse combined effects of urban heatwaves and UDIs.

How to cite: Luo, S. and Gu, X.: Hot weather amplifies the urban dry island effect, especially in wetter climates, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2064, https://doi.org/10.5194/egusphere-egu23-2064, 2023.

EGU23-2078 | Posters on site | CL4.1

A new satellite-based product for studying land-atmosphere interactions 

Jian Peng and Almudena García-García

Information about the energy and water exchanges between the land surface and the lower atmosphere (i.e. land-atmosphere interactions) is necessary for example to improve our understanding of the effect of land-atmosphere interactions on the exacerbation of temperature and precipitation extremes. Observations of energy and water fluxes at the land surface usually rely on the eddy covariance method. There is a wide network of these measurements providing data over all continents but with large spatial gaps in Africa, Asia, South America and Oceania. Additionally, other problems are associated with these observational methods such as the energy and water balance non-closure. To improve the spatial coverage of land-atmosphere interactions data considering the energy and water balance closure, we explore the combination of remote sensing data and a physical-based model. The High resOlution Land Atmosphere Parameters from Space (HOLAPS) framework is a one dimensional modelling framework that solves the energy and water balance at the land surface using remote sensing data and reanalysis products as forcings. Preliminary results from the evaluation ofHOLAPS outputs over Europe at 5 km resolution show an improvement in the simulation of latent heat flux when using remote sensing data in comparison with results using only reanalysis data as forcing. Additionally, we see a moderate improvement in HOLAPS latent heat flux estimates against energy-balance corrected eddy covariance measurements in comparison with other products that solve the energy and water balance equations, such as the ERA5Land product. The new HOLAPS product is available at hourly resolution for the period 2001 to 2016 and these estimates can be useful for agriculture and forest management activities and to evaluate the representation of land-atmosphere feedbacks in weather and climate models.

How to cite: Peng, J. and García-García, A.: A new satellite-based product for studying land-atmosphere interactions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2078, https://doi.org/10.5194/egusphere-egu23-2078, 2023.

EGU23-3211 | ECS | Orals | CL4.1

Characterisation and interpretation of local climate evolution in the South-West of France 

Marine Lanet, Laurent Li, and Hervé Le Treut

Summer 2022 has been the second hottest summer after 2003 in France since 1900, with 33 cumulative days of heatwaves. It has also been one of the 10 driest summers in France since 1959. The average precipitation deficit reached 20% compared to the 1991-2020 period, exceeding 60% in some regions, even though June 2022 broke the monthly record of storm occurrences.

These extreme climate conditions led to water restrictions and fostered the development of many wildfires. In particular, so called “megafires” burnt more than 28,000 hectares of the Landes forest in the Nouvelle-Aquitaine region, in the South-West of France.

Starting from the 18th century, this swampy region has been dried out by planting maritime pines and digging ditches to drain away excess water. Due to recent events, these land management practices are questioned : the record-breaking soil dryness of summer 2022 enabled fire to propagate underground and resurface further away, making firemen’s work extremely difficult.

By controlling ditch drainage, is it possible to reduce soil dryness and thus fire risk in summer, as well as mitigate heavy precipitation impacts in this flood prone area ? To answer this question, this work first aims at characterizing and interpreting local climate evolution during the last decades, in terms of trends, changes in the seasonal cycle and extreme events, using  ERA 5 reanalysis, the E-Obs dataset, and MODIS satellite observations. CORDEX regional climate projections are also analysed. Nouvelle-Aquitaine will experience both more frequent and intense heatwaves and droughts and an increase in heavy precipitations. Landes forest management thus has to be adapted.

The perspective of this work is to develop a conceptual ditch drainage model and quantify the drought and flood risk reduction potential using storylines based on plausible short and long term climate conditions in Nouvelle-Aquitaine.

In a broader perspective, the objective of this work is to develop a methodology replicable in other regions of the world to analyse the impacts of climate change at a local scale and explore how climate science can provide quantitative information to help decision making.

How to cite: Lanet, M., Li, L., and Le Treut, H.: Characterisation and interpretation of local climate evolution in the South-West of France, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3211, https://doi.org/10.5194/egusphere-egu23-3211, 2023.

EGU23-3549 | ECS | Posters virtual | CL4.1

The incorporation of 250 m soil grid textural layers in the NOAH-MP land surface models and its effects on soil hydrothermal regimes 

Kazeem Ishola, Ankur Sati, Matthias Demuzere, Gerald Mills, and Rowan Fealy

Effective representation of soil heterogeneity in land surface models is crucial for accurate weather and climate simulations. The NOAH-MP land surface model uses dominant soil texture from State Soil Geographic (STATSGO)/Food and Agriculture Organization (FAO) datasets, considerably introducing uncertainty in the simulation of soil hydrothermal changes and terrestrial water and energy fluxes, at a fine scale. This study investigates the likely added value of incorporating an alternative high resolution soil grid data at different depths, for a better representation of soil hydrothermal dynamics in NOAH-MP v4.3. The model is set up at 1 km grid space over all Ireland domain and soil layer thicknesses of 0.07, 0.21, 0.72 and 1.55 m, with a cummulative soil depth of 2.55 m. The thicknesses are selected to match the layers of initial soil input fields. Model experiments are carried out based on two soil data options namely, (1) the STATSGO/FAO dominant soil texture and (2) the 250 m global soil grid textural compositions from the International Soil Reference and Information Centre (ISRIC), in combination with PedoTransfer Functions (PTFs). The current model integration is applied within the high resolution land data assimilation (HRLDAS) framework to simulate soil temperature and soil liquid water, and evaluated for wet and dry periods using observations from the newly established Terrain-AI data platforms (terrainai.com). Ultimately, the study highlights the importance of using realistic dynamic soil information, which could provide insightful scientific contributions to better monitor surface climate and the influences on land use and land management under climate change.

How to cite: Ishola, K., Sati, A., Demuzere, M., Mills, G., and Fealy, R.: The incorporation of 250 m soil grid textural layers in the NOAH-MP land surface models and its effects on soil hydrothermal regimes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3549, https://doi.org/10.5194/egusphere-egu23-3549, 2023.

EGU23-3780 | ECS | Orals | CL4.1

Greening vegetation alleviates hot extremes in the semiarid region of China 

Yipeng Cao, Weidong Guo, Jun Ge, Yu Liu, Chaorong Chen, Xing Luo, and Limei Yang

China has shown a world-leading vegetation greening trend since 2000, which may exert biophysical effects on near-surface air temperature (SAT). However, such effects remain largely unknown because prior studies either focus on land surface temperature, which differs from SAT, or rely on simulations, which are limited by model uncertainties. As a widely used metric in climate and extremes research, SAT is more relevant to human health and terrestrial ecosystem functions. Therefore, it is necessary to explore impacts of greening on SAT and extremes based on observations. Here, we investigate the greening effects on SAT and subsequent extremes over 2003–2014 in China based on high-resolution SAT observations combined with satellite datasets. We find that greening can cause cooling effects on the mean SAT and more pronounced cooling effects on SAT extremes over semiarid regions. Such cooling effects are attributed to enhanced evapotranspiration caused by greening and strong coupling between evapotranspiration and SAT in semiarid regions. Semiarid regions in China are the transitional zone of both climate and ecosystem and deeply influenced by human agricultural and pastoral activities. These factors make the ecosystem of these regions fragile and extremely vulnerable to climate change. Our results reveal a considerable climate benefit of greening to natural and human systems in semiarid regions, and have significant implications for on-going revegetation programs implemented in these regions of China.

How to cite: Cao, Y., Guo, W., Ge, J., Liu, Y., Chen, C., Luo, X., and Yang, L.: Greening vegetation alleviates hot extremes in the semiarid region of China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3780, https://doi.org/10.5194/egusphere-egu23-3780, 2023.

EGU23-4818 | ECS | Posters on site | CL4.1

Simulating regional inter-annual crop yield variability over multiple decades with the Community Land Model (CLM5) 

Theresa Boas, Heye Bogena, Dongryeol Ryu, Harry Vereecken, Andrew Western, and Harrie-Jan Hendricks-Franssen

Global climate change with a predicted increase in weather extremes entails vulnerability and new challenges to regional agriculture. While the general impacts of climate change on global food security are a much studied topic, the implications for regional inter-annual yield variability remain unclear. In this study, we analysed the effects of weather trends on regional crop productivity within two agriculturally managed regions in different climate zones, simulated with the latest version of the Community Land Model (version 5.0) over two decades (1999-2019). We evaluated the models’ potential to represent the inter-annual variability of crop yield in comparison to recorded yield variability and different weather indicators, e.g., drought index and growing season length and evaluated which variables (i.e., temperature, precipitation, initial soil moisture content) dominantly drive changes in CLM5-predicted yield variability. The simulation results were able to reproduce the sign of crop yield anomalies, and thus provide a basis on which to study the effects of different weather patterns on inter-annual yield variability. However, the simulations showed limitations in correctly capturing inter-annual differences of crop yield in terms of total magnitudes (up to 10 times lower than in official records). Our results indicate that these limitation arise mainly from uncertainties in the representation of the subsurface soil moisture regime and a corresponding lack of sensitivity towards drought stress. Insights from this work were used to summarize implications for future analysis of CLM5-BGC simulation results over agriculturally managed land and allowed us to discuss and investigate possible technical model improvements.

How to cite: Boas, T., Bogena, H., Ryu, D., Vereecken, H., Western, A., and Hendricks-Franssen, H.-J.: Simulating regional inter-annual crop yield variability over multiple decades with the Community Land Model (CLM5), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4818, https://doi.org/10.5194/egusphere-egu23-4818, 2023.

EGU23-5624 | ECS | Orals | CL4.1

Abrupt late 1980s surface climate warming effects on drought risk over main french crop production basins 

Léa Laurent, Albin Ullmann, and Thierry Castel

Since late 1980s, warming trend intensifies strongly over Western Europe, resulting in an abrupt shift in air surface temperature over France (Sutton & Dong 2012; Reid et al., 2016). This rapid warming has modified the hydrological cycle with especially a significant decrease in runoff between January and July (Brulebois et al., 2015). As cumulative annual liquid precipitation didn’t significantly evolve after 1987/1988, evapotranspiration might be the main driver of the water cycle evolution.

Along with this abrupt warming, stagnation of crop yields is observed since the 1990s over France, especially for bread wheat (Schauberger et al., 2018). In addition to maize and grapevine, the impact of climate hazard and agro-climatic risk linked to water cycle on the evolution of bread wheat yields is a major issue for agricultural insurance companies (Fusco et al., 2018). In this context, two major concerns need to be assessed: what are the patterns of water balance responses to abrupt changes in temperature? How did this abrupt warming impact drought risk over crops of interest main production basins?

SIM (Safran-Isba-Modcou) dataset of reanalyzed surface meteorological observations offers the opportunity to address the complexity of processes leading to changes in local water cycle (Soubeyroux et al., 2008). Daily liquid precipitation and potential evapotranspiration on an 8km spatial resolution from 1959 to 2021 are used to quantify the evolution of climate hazard linked to water cycle on a continuous time-scale and over the entire French territory. A simplified two reservoirs water balance model is also used to compute daily water balance using agronomic parameters of crops of interest, taking into account crop cover stage (Jacquart & Choisnel, 1995). The evolution of frequency and intensity of drought risk is analyzed using Tweedie distributions (Dunn, 2004).

Our results suggest that the abrupt warming in air temperature in 1987/1988 had strong influence on water balance evolution. Potential evapotranspiration significantly increases after 1987/1988 over the whole French territory especially in spring and summer. The evolution of annual and seasonal cumulative liquid precipitation differs in space and time and is less pronounced, leading to an intensification of water cycle. Water balance displays various evolutions depending on the crop and the production basin studied. The exceeding of water stress threshold is more frequent or more pronounced, leading to modifications of intensity and/or duration of drought events that significantly modify the risk. Risk evolution depends on the crop cover and main production basin.

Evolving climate hazard linked to water cycle impacts agro-climatic risks, identified as one of the main factor affecting the evolution of crop yields. Both mean conditions changes and modifications of the spatio-temporal variability of water balance affect the probability to overcome risk threshold. This is of major concern for the agricultural sector, especially insurance companies, and may lead to adaptation process from managers.

How to cite: Laurent, L., Ullmann, A., and Castel, T.: Abrupt late 1980s surface climate warming effects on drought risk over main french crop production basins, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5624, https://doi.org/10.5194/egusphere-egu23-5624, 2023.

EGU23-5726 | ECS | Posters on site | CL4.1

Ground surface temperature linked to remote sensing land surface temperature in mountain environments 

Raul-David Șerban, Paulina Bartkowiak, Mariapina Castelli, and Giacomo Bertoldi

Ground surface temperature (GST), measured at approximately 5 cm into the ground is a key parameter controlling all the subsurface biophysical processes at the land-atmosphere boundary. Despite the GST significant importance, the current observational network for GST is sparse, particularly in mountain regions. This work exploits the relationship between the GST and satellite-based land surface temperature (LST) derived from MODerate resolution Imaging Spectroradiometer (MODIS). The GST and LST were compared at 14 weather stations in Mazia Valley, North-eastern Italian Alps. The 1-km MODIS LST was downscaled to a spatial resolution of 250-m using the random forest algorithm. The LST dataset covers the years 2014-2017 during the phenological cycle, between April and October. The in-situ GST measurements were recorded using Campbell Scientific CS655 data loggers. LSTs were usually larger than GSTs with temperature differences ranging from 0.1 to 22 °C and an average of 7.9 °C. The lowest and largest average difference was 4.49 °C (1823 m, pasture, south slope) and 10.27 °C (1778 m, forest, north slope), respectively. GST was positively correlated with LST with an R2 ranging from 0.24 to 0.52 and was above 0.45 for 57 % of the stations. The RMSE ranged between 6.05 and 11.05 °C, while for 71 % of the stations was below 9.3 °C. The statistics were influenced by the number of available pairwise for comparison that were ranging from 110 to 377 due to cloud contamination or logger malfunction. Although the RMSE was relatively high, the LST closely followed the pattern of the GST variability suggesting the possibility of linking GST to LST products.

How to cite: Șerban, R.-D., Bartkowiak, P., Castelli, M., and Bertoldi, G.: Ground surface temperature linked to remote sensing land surface temperature in mountain environments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5726, https://doi.org/10.5194/egusphere-egu23-5726, 2023.

EGU23-5961 | ECS | Orals | CL4.1 | Highlight

Soil Hot Extremes are Increasing Faster than Air Hot Extremes Regionally 

Almudena García-García, Francisco José Cuesta-Valero, Diego G. Miralles, Miguel D. Mahecha, Johannes Quaas, Markus Reichstein, Jakob Zscheischler, and Jian Peng

Hot temperature extremes are changing in intensity and frequency. Quantifying these changes is key for developing adaptation and mitigation strategies. The conventional approach to study changes in hot extremes is based on air temperatures. However, many biogeochemical processes, i.e. decomposition of organic material and release of CO2, are triggered by soil temperature and it remains unclear whether it changes as does air temperature. Here, we demonstrate that soil hot extremes are intensifying and becoming even more frequent faster than air hot extremes over central eastern and western Europe. Based on existing model simulations, we also show that the increase in hot soil extremes could amplify or spread future heat waves by releasing sensible heat during hot days. We find an increase of 3 (7) % in the number of hot days with a contribution of heat from the soil under a warming level of 2.0 (3.0) °C than under a warming level of 1.5 °C. Furthermore, defining intensity and frequency extreme indices based on soil and air temperatures leads to a difference of more than 1 °C in intensity and 10% in frequency regionally during the last decades of the 21st century under the SPP5 8.5 emission scenario. In light of these results, maximum soil temperatures should be included in ecological risk studies as a complementary perspective to the conventional approach using extreme indices based on air temperatures.

 

How to cite: García-García, A., Cuesta-Valero, F. J., Miralles, D. G., Mahecha, M. D., Quaas, J., Reichstein, M., Zscheischler, J., and Peng, J.: Soil Hot Extremes are Increasing Faster than Air Hot Extremes Regionally, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5961, https://doi.org/10.5194/egusphere-egu23-5961, 2023.

EGU23-6528 | ECS | Posters on site | CL4.1

Improving the temporal and spatial vegetation variability in land surface models based on satellite observations  

Fransje van Oorschot, Ruud van der Ent, Markus Hrachowitz, Emanuele di Carlo, Franco Catalano, Souhail Boussetta, Gianpaolo Balsamo, and Andrea Alessandri

Land-atmosphere interactions are largely controlled by vegetation, which is dynamic across spatial and temporal scales. Most state-of-the-art land surface models do not adequately represent the temporal and spatial variability of vegetation, which results in weaknesses in the associated variability of modelled surface water and energy states and fluxes. The objective of this work is to evaluate the effects of integrating spatially and temporally varying vegetation characteristics derived from satellite observations on modelled evaporation and soil moisture in the land surface model HTESSEL. Specifically, model fixed land cover was replaced by annually varying land cover, and model seasonally varying Leaf Area Index (LAI) was replaced by seasonally and inter-annually varying LAI. Additionally, satellite data of Fraction of green vegetation Cover (FCover) was used to formulate and integrate a spatially and temporally varying model effective vegetation cover parameterization. The effects of these three implementations on model evaporation and soil moisture were analysed using historical offline (land-only) model experiments at a global scale, and compared to reference datasets.

The enhanced vegetation variability lead to considerable improvements in correlation of anomaly evaporation and surface soil moisture in semiarid regions during the dry season. These improvements are related to the adequate representation of vegetation-evaporation-soil moisture feedback mechanisms during water-stress periods in the model, when integrating spatially and temporally varying vegetation. These findings emphasize the importance of vegetation variability for modelling land surface-atmosphere interactions, and specifically droughts. This research contributes to the understanding and development of land surface models, and shows that satellite observational products are a powerful tool to represent vegetation variability.

How to cite: van Oorschot, F., van der Ent, R., Hrachowitz, M., di Carlo, E., Catalano, F., Boussetta, S., Balsamo, G., and Alessandri, A.: Improving the temporal and spatial vegetation variability in land surface models based on satellite observations , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6528, https://doi.org/10.5194/egusphere-egu23-6528, 2023.

The diurnal air temperature range (DTR) is strongly shaped by solar radiation but is modulated by hydrologic cycling through changes in atmospheric (clouds) and land-surface (evaporation) characteristics. Here, we aim to determine the distinct patterns in DTR over dry and wet periods and identify their respective controls. To do this, we develop a simple energy balance model that constrains the land-atmosphere exchange using the thermodynamic limit of maximum power. In this framework, we explicitly account for changes in radiative conditions due to clouds and changes in boundary layer heat storage associated with surface water limitation, both of which affect the maximum power limit. Using observations of radiative forcings and surface evaporation, our model predicts DTR reasonably well across 81 FLUXNET sites in North America, Europe, and Australia. We show that DTR is primarily shaped by the trade-off between the heat gain due to solar absorption and heat lost at the surface due to evaporation. Radiation remains a primary control on DTR over very dry and wet conditions where evaporation is either close to zero or limited by available energy. Over these regions, changes in DTR are strongly modulated by clouds which alters the radiative conditions. DTR becomes coupled to the land surface during the transition regime where changes in surface water availability directly control the evaporation rates. Over these regions, increased soil moisture results in more evaporation and reduced DTR. These responses were consistent in both, observations and maximum power estimates. We then apply our framework to quantify the response of DTR to global warming. Our model projects a decrease in DTR by 0.18K for a 1K rise in global temperature, which is consistent with the current observed response. Our findings imply that the predominant controls on DTR are set by clouds and evaporation as they directly modulate the diurnal heating of the lower atmosphere and can be further altered by increased greenhouse forcing.

How to cite: Ghausi, S. A., McColl, K., and Kleidon, A.: Determining the radiative and hydrologic controls on the diurnal air-temperature range using the thermodynamic limit of maximum power, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7721, https://doi.org/10.5194/egusphere-egu23-7721, 2023.

EGU23-9421 | ECS | Orals | CL4.1

An emergent constraint exposes widespread underestimation of drought impacts by Earth System Models 

Julia K. Green, Yao Zhang, Xiangzhong Luo, and Trevor Keenan

The response of vegetation canopy conductance (gc) to changes in moisture availability gc) during drought is a major source of uncertainty in climate projections. Representing ϒgc accurately in Earth System Models (ESMs) is particularly problematic because no regional scale gc observations exist with which to evaluate it. Here, we overcome this challenge by deriving an emergent constraint on ϒgc across ESMs from Phase 6 of the Coupled Model Intercomparison Project (CMIP6). We leverage an ensemble of satellite, reanalysis and station-based estimates of surface temperatures, which are physically and statistically linked to ϒgc due to the local cooling effect of gc. We find that models systemically underestimate ϒgc by ~50%, particularly in semi-arid grasslands, croplands, and savannas. Based on the mediating effect of gc on carbon, water and energy fluxes through land-atmosphere interactions, the underestimation of modeled ϒgc in these regions contributes to biases in temperature, transpiration and gross primary production. Our results provide a novel benchmark to improve model representation of vegetation dynamics and land-atmosphere feedbacks in these regions, thus improving forecasting ability of climate extremes under future climate change scenarios.

How to cite: Green, J. K., Zhang, Y., Luo, X., and Keenan, T.: An emergent constraint exposes widespread underestimation of drought impacts by Earth System Models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9421, https://doi.org/10.5194/egusphere-egu23-9421, 2023.

EGU23-9767 | ECS | Posters on site | CL4.1

Diagnosing above- and below-canopy temperature impacts of forest in the Netherlands during heatwaves 

Jingwei Zhou, Adriaan J. Teuling, and Michiel K. van der Molen

Heatwaves have significant effects on ecosystems and human populations. Human habitability is impacted severely as human exposure to heatwaves is projected to increase. Future risk of heatwaves has demonstrated the need of effective measures for adaptation to persistent hot temperature extremes and ambitious mitigation to limit further increases in heatwave severity.

At local scales, forest management could be a potential approach of modifying surface energy budget and in this way alleviating heatwave impacts. In this study,  open-site, below-canopy, and above-canopy climatic conditions from 4 different sites during the time period 1997-2020 in the Netherlands were compared to investigate canopy functions of affecting above-canopy macroclimate and as a thermal insulator to regulate understory microclimate and land surface ecology. Using high-resolution sub-daily data sets from Loobos, in which water vapor and heat fluxes were measured every half an hour by a combination of eddy covariance flux measurements and a profile system, we analysed temperatures at three levels of Loobos (23.5m, 7.5m, and soil litter layer) of the same profile and compared them with those measured at open sites in De bilt and Deleen.

Heatwave periods are defined as a sequence of at least five days during which the daily maximum temperature exceeds the climatological mean over the reference period 1997-2010 by at least 5 °C. During heatwave periods, the cooling effects of the canopy on surface temperatures are stronger compared to normal periods while the canopy may aggravate the temperature above it during certain hours. By contrast, temperature differences are higher during normal times than heatwave periods when considering temperature buffer effects of canopy on understory climate (7.5m).

Further study on heat fluxes, Bowen ratio, and canopy effects on heat stress during normal conditions and heatwaves will be conducted as well. Relative humidity will be incorporated in measuring heat stress to reflect real conditions living bodies experience.

How to cite: Zhou, J., Teuling, A. J., and van der Molen, M. K.: Diagnosing above- and below-canopy temperature impacts of forest in the Netherlands during heatwaves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9767, https://doi.org/10.5194/egusphere-egu23-9767, 2023.

EGU23-9777 | Orals | CL4.1

Leaves, land-atmosphere interactions and extremes 

Gregory Duveiller

Leaves are the main interface between terrestrial ecosystems and the atmosphere. They govern the exchange of carbon, water and energy between vegetation and the atmospheric boundary layer. They are the surface designed to capture light and transform it to sugars via photosynthesis, but they also regulate how much water they transpire through their stomata. Their colour, density and orientation will affect their albedo, which determines how much energy is reflected back to the atmosphere, while their overall configuration within the canopy structure can affect the roughness length of the surface.

When we manage landscapes, be it by planting crops or cutting down forests, we are typically changing the quantity and type of leaves covering the surface of the land. By doing so, we can modify the land-atmosphere interactions and thereby have an effect on the climate. For instance, a substantial local cooling effect could be attained by using cover crops in winter, especially with highly reflective chlorophyll deficient mutants. Increasing forest cover appears to lead to more cloud cover, which itself could affect albedo at the top of the atmosphere. But the amount of leaves in the landscape can further affect extremes.

Here I will illustrate how leaves affect land-atmosphere interactions in the context of extreme events with two studies. The first study looks at the known biophysical effect of land use change on local surface temperature, but extends it to explore its sensitivity across the globe during the extremes observed in 20 years of satellite remote sensing records. The second study shows how much getting leaves right matters within the reanalysis records of ERA5 and ERA5-Land, where prescribed seasonal cycles of leaf area index (LAI) lead to biases in modelling land surface temperature (LST), thereby underestimating the intensity of heat waves over Europe.

How to cite: Duveiller, G.: Leaves, land-atmosphere interactions and extremes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9777, https://doi.org/10.5194/egusphere-egu23-9777, 2023.

EGU23-9838 | ECS | Orals | CL4.1

Vegetation-climate coupling and vegetation sensitivity to climate extremes in growing seasons 

Minchao Wu, Gabriele Messori, Giulia Vico, Stefano Manzoni, Zhanzhang Cai, Jing Tang, Torbern Tagesson, and Zheng Duan

Terrestrial vegetation is largely mediated by vegetation-climate coupling. Growing conditions control vegetation growth, which in turn feeds back to climate through changes in biophysical and biogeochemical properties and processes, such as canopy structure and carbon and water exchanges. The vegetation-climate coupling is thus highly variable in space and time. However, little is known on how the large-scale vegetation-climate coupling varies within growing season, and how vegetation responds to climate extremes. In this contribution, we present some recent findings on seasonal and intra-seasonal vegetation-climate coupling and vegetation sensitivity to droughts using multiple remote sensing products including MODIS EVI, GIMMS3g NDVI and VIP EVI2. We account for the differences in phenological stages of growing seasons affected by both climate and landscape heterogeneity. Based on a novel analytical framework incorporating meteorological and vegetation conditions to locally defined vegetation growing seasons, we analyse vegetation-climate couplings using both local climate conditions and teleconnection indices (e.g., Jet Latitude Index). In addition, vegetation sensitivity to droughts and post-drought vegetation changes are assessed. Our results highlight the importance of considering vegetation phenology in understanding sub-seasonal land-atmosphere interaction and vegetation dynamics. The developed analytical framework is suggested to be an effective approach for evaluating vegetation and climate dynamics simulated by Earth System Models.

How to cite: Wu, M., Messori, G., Vico, G., Manzoni, S., Cai, Z., Tang, J., Tagesson, T., and Duan, Z.: Vegetation-climate coupling and vegetation sensitivity to climate extremes in growing seasons, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9838, https://doi.org/10.5194/egusphere-egu23-9838, 2023.

EGU23-9920 | ECS | Posters on site | CL4.1

Diurnal to interannual variability in Cabauw simulated by the ECLand land surface model 

Luís Fróis, Pedro M. A. Miranda, and Emanuel Dutra

Land surface plays a fundamental role in the earth system, mediating the water, energy and carbon fluxes between the land and the atmosphere. The land surface physical and biophysical processes act on time scales ranging from sub-daily to decades with relevant impacts from weather forecasts to climate change. However, there are very few available in-situ observations of land surface state and fluxes extending for several years to decades, limiting an integrated validation of the models on the different time scales. The long time series of Cabauw (Netherlands) observations provides a unique opportunity to evaluate land surface processes and their representation in land surface model at time scales ranging from sub-diurnal to interannual. In this study, we take advantage of the uniqueness of Cabauw observational record to investigate the performance of the ECMWF land surface model ECLand for the period 2001-2020 (20 years). Emphasis is given to the summer season and to evaporation and evaporative fraction. An idealized simulation without canopy resistance is performed along with other model configurations with changes to the constraints of canopy resistance (soil moisture availability and atmospheric humidity deficit) and the vertical discretization of the soil layers.

Observational uncertainties impact the surface energy budget closure. For example, the model shows a large overestimation of the ground heat flux diurnal cycle. However, part of this can be attributed to observational uncertainties associated with the sinking of the temperature sensors.  The default configuration of ECLand shows an underestimation of latent heat and evaporative fraction, which can be partially attributed to the model’s representation of canopy resistance. The increased vertical discretization of the soil layers has a neutral impact on the simulated turbulent fluxes, showing an improved representation of near-surface soil temperature. Our results show limitations in the representation of the summer interannual variability of the turbulent fluxes. These are associated with the representation of extreme events (droughts) and are not fully addressed in any of the model configurations tested. These results suggest that other processes relevant to the representation of evaporation in dryness stress conditions need to be further investigated.

This work was developed in the framework of the project NextGEMS funded through the European Union’s Horizon 2020 research and innovation program under the grant agreement number 101003470. Luis Frois was funded by the FCT Grant 2020.08478.BD. The authors also acknowledge the financial support of the Portuguese Fundação para a Ciência e a Tecnologia (FCT) I.P./MCTES through national funds (PIDDAC) – UIDB/50019/2020- IDL.

How to cite: Fróis, L., Miranda, P. M. A., and Dutra, E.: Diurnal to interannual variability in Cabauw simulated by the ECLand land surface model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9920, https://doi.org/10.5194/egusphere-egu23-9920, 2023.

EGU23-10118 | ECS | Orals | CL4.1

Mechanistic patterns of land hydroclimate changes in a changing climate 

Suqin Duan, Kirsten Findell, and Stephan Fueglistaler

Climate model predictions of land hydroclimate changes show large geographic heterogeneity, and differences between models are large. We introduce a new process-oriented phase space that reduces the dimensionality of the problem but preserves (and emphasizes) the mechanistic relations between variables. This transform from geographical space to climatological aridity index (AI) and daily soil moisture (SM) percentiles allows for interpretation of local, daily mechanistic relations between the key hydroclimatic variables in the context of time-mean and/or global-mean energetic constraints and the wet-get-wetter/dry-get-drier paradigm. Focusing on the tropics (30S-30N), we show that simulations from 16 different CMIP models exhibit coherent patterns of change in the AI/SM phase space that are aligned with the established soil-moisture/evapotranspiration regimes. Results indicate the need to introduce an active-rain regime as a special case of the energy-limited regime. In response to CO2-induced warming, rainfall only increases in this regime, and this temporal rainfall repartitioning is reflected in an overall decrease in soil moisture. Consequently, the regimes where SM constrains evapotranspiration become more frequently occupied, and hydroclimatic changes align with the position of the critical soil moisture value in the AI/SM phase space. Analysis of land hydroclimate changes in CMIP6 historical simulations in the AI/SM phase space reveal the very different impact of CO2 forcing and aerosol forcing. CESM2 Single Forcing Large Ensemble Experiments are used to understand their roles.

How to cite: Duan, S., Findell, K., and Fueglistaler, S.: Mechanistic patterns of land hydroclimate changes in a changing climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10118, https://doi.org/10.5194/egusphere-egu23-10118, 2023.

EGU23-11343 | ECS | Posters on site | CL4.1

The relevance of coupled climate model WRF-CTSM for land-atmosphere interactions analysis 

Iris Mužić, Øivind Hodnebrog, Terje Koren Berntsen, Yeliz Yilmaz, Jana Sillmann, David Lawrence, Sean Swenson, and Negin Sobhani

A credible assessment of spatial and temporal variability of the water and energy budget is of viable importance for the quantification of the observed changes and prediction of extremes in a changing climate. However, an accurate representation of feedback mechanisms between the land surface and the atmosphere is a key source of uncertainty in climate models.

WRF-CTSM (Weather Research and Forecasting model, WRF, and Community Terrestrial Systems Model, CTSM) is a state-of-the-art modelling tool that represents the forefront in the climate modelling community and unifies the recent model development activities across weather, climate, water and ecosystem research. This study is the first to provide a systematic regional scale assessment of the WRF-CTSM coupled climate model performance in the European context - in the high-latitude region encompassing Norway, Sweden and Finland.

A 10-year-long regional WRF-CTSM simulation (2010-2020) using meteorological boundary conditions from the ERA5 reanalysis is performed on a 10.5 km horizontal resolution to evaluate the representation of hydroclimatic variables through comparison against ERA5 and a range of observational datasets. Changes in boundary layer variables such as soil and near-surface air temperature, soil moisture and snowpack are essential for the assessment of the land-atmosphere feedbacks in this region and are thus selected as central for the analysis of the model skill. Besides the WRF-CTSM simulations using default CTSM settings, this study investigates the added value of including the recently developed Hillslope Hydrology model in WRF-CTSM runs that has the potential to improve the understanding of the role of topography and hydrology on the soil moisture and snowpack variability.

Preliminary results indicate the capacity of WRF-CTSM to identify the high-temperature susceptible areas in Norway, Sweden and Finland and reproduce the interannual variability and spatial patterns of hydroclimatic variables in the respective region.

How to cite: Mužić, I., Hodnebrog, Ø., Berntsen, T. K., Yilmaz, Y., Sillmann, J., Lawrence, D., Swenson, S., and Sobhani, N.: The relevance of coupled climate model WRF-CTSM for land-atmosphere interactions analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11343, https://doi.org/10.5194/egusphere-egu23-11343, 2023.

EGU23-11538 | Orals | CL4.1

Mesoscale Gradients in Soil Moisture over South America Lead to Enhanced Convection 

Francina Dominguez, Divyansh Chug, Christopher Taylor, Cornelia Klein, and Stephen Nesbitt

This work presents the first observationally-based study over subtropical South America linking the spatial location of convection and drier soil patches of the order of tens of kilometers, as well as observational evidence of the control of background flow on the sign of SM-PPT feedbacks at convective scales. Using satellite data from multiple infrared and microwave radiometers, we track nascent, daytime convective clouds over subtropical South America and quantify the underlying, antecedent (morning), SM heterogeneity. We find that convection initiates preferentially on the dry side of strong dry-wet SM boundaries that are associated with spatially drier and warmer patches of tens of kilometers scale consistent with findings in other parts of the world. This preference maximizes during weak background low-level wind, high convective available potential energy, low convective inhibition and low vegetation density when analyzing surface gradients of 30 km length scale. On the other hand, surface gradients of 100 km length scale are significantly associated with afternoon convection during convectively unfavorable synoptic conditions and strong background flow, unlike previous studies. The location of the precipitation maxima following CI onset is most sensitive to the lower tropospheric background flow at the time of CI. The wind profile during weak background flow does not support propagation of convective features away from the dry regions and rainfall accumulates over the dry patch. Convection during strong background flow leads to greater rainfall hundreds of kilometers away from the CI location. 

 

 

How to cite: Dominguez, F., Chug, D., Taylor, C., Klein, C., and Nesbitt, S.: Mesoscale Gradients in Soil Moisture over South America Lead to Enhanced Convection, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11538, https://doi.org/10.5194/egusphere-egu23-11538, 2023.

EGU23-12925 | ECS | Orals | CL4.1

Interannual Variation of Land-Atmosphere Interactions and their Connection with Extremes over Europe 

Lisa Jach, Thomas Schwitalla, Volker Wulfmeyer, and Kirsten Warrach-Sagi

The land surface supplies heat and moisture to the atmosphere influencing the regional climate during the convective season. Availability of soil moisture for evapotranspiration, vegetation phenology and atmospheric conditions influence the strength of the land surface impact on the atmosphere, and the mechanisms predominating the heat and moisture exchange. As both the synoptic conditions as well as the vegetation state vary on sub-seasonal to interannual time scales, the strength of land-atmosphere (L-A) interaction is expected to fluctuate on these time scales.

Up to now, research typically either focuses on case studies to understand the mechanisms of how land surface and atmosphere interact, or on climatic time scales to quantify co-variances in the climate system based on a sufficient sample size. Timescales in between remain rarely considered in land-atmosphere feedback studies.

In our study, we applied various L-A coupling measures to evaluate land surface impacts on the atmosphere and quantify interactions associated with the triggering of convective precipitation and droughts for all summers between 1991 and 2022 over Europe based on ERA5 data.

Our results highlight that differently strong L-A interactions evolve in dependence of atmospheric wetness, temperature, and the circulation pattern, as well as the root zone soil moisture and vegetation cover. Under warm and dry conditions such as in 2003, 2018 and 2022, soil moisture availability imposed limits for evapotranspiration not only in Southern Europe, but also in Central and Eastern Europe, interfering with vegetation growth and atmospheric moisture supply. Limited moisture and excessive heat supply amplified the already high temperatures and low near-surface moisture, which finally aggravated the unfavorable conditions for local precipitation and caused extreme drought conditions. On the contrary, warm and wet conditions such as in 2021 provided well-suited conditions for vegetation growth, which enhanced the moisture supply to the atmosphere. Together with stronger atmospheric instability, this provided more favorable preconditions for convective precipitation. Generally, most L-A interactions perform as an intensifier of persisting anomalies, particularly under warm and dry atmospheric conditions over Europe.

How to cite: Jach, L., Schwitalla, T., Wulfmeyer, V., and Warrach-Sagi, K.: Interannual Variation of Land-Atmosphere Interactions and their Connection with Extremes over Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12925, https://doi.org/10.5194/egusphere-egu23-12925, 2023.

EGU23-13277 | ECS | Posters on site | CL4.1

Earth observation time series for the monitoring of droughts in Cyprus: Patterns and drivers of vegetation dynamics 

Soner Uereyen, Christina Eisfelder, Ursula Gessner, Sophie Reinermann, Sarah Asam, Constantinos F. Panagiotou, Marinos Eliades, Ioannis Varvaris, Eleni Loulli, Zampela Pittaki, Diofantos Hadjimitsis, Claudia Kuenzer, and Felix Bachofer

With amplified climate warming, climate extremes over Europe become more frequent. Since the 2000’s, many years have been characterized by extreme events such as droughts and heat waves. For example, in Central Europe, extreme droughts and heat waves took place in the years 2003 and 2018. In comparison, Cyprus experienced strong droughts during 2003 and 2016-2018. Such extreme climate events can have severe impacts on agricultural yields, the productivity of natural vegetation, and on water resources. In this regard, long-term Earth observation (EO) time series are essential to quantitatively assess and analyse changes on the land surface, including vegetation condition. In this study, a joint analysis of geoscientific time series over the last two decades, including EO-based MODIS vegetation indices and meteorological variables is performed to assess drought events and analyse trends as well as potential drivers of vegetation dynamics in Cyprus. The analysis of drought events and vegetation trends is based on the full archive of MODIS imagery at 250 m spatial resolution covering the period 2000-2022. In detail, climate-related effects on vegetation were analysed by means of the deviations of MODIS 16-day vegetation index composites from their long-term mean. Next, trends of the MODIS vegetation index were calculated to evaluate spatial patterns of vegetation change over the investigated period. These analyses were additionally performed for geographically stratified regions, including diverse vegetation classes such as cropland and grassland. Furthermore, the application of a causal discovery algorithm reveals linkages within a multivariate feature space, in particular between vegetation greenness and climatic drivers. Preliminary analyses showed that drought patterns differ with respect to seasons and the investigated vegetation class. For example, the strong drought year 2008 is clearly reflected in the results, whereas forest areas appear to be least affected by the drought during the spring months. Moreover, considering the significant trends over the last two decades, an increase in vegetation greenness could be observed.

How to cite: Uereyen, S., Eisfelder, C., Gessner, U., Reinermann, S., Asam, S., Panagiotou, C. F., Eliades, M., Varvaris, I., Loulli, E., Pittaki, Z., Hadjimitsis, D., Kuenzer, C., and Bachofer, F.: Earth observation time series for the monitoring of droughts in Cyprus: Patterns and drivers of vegetation dynamics, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13277, https://doi.org/10.5194/egusphere-egu23-13277, 2023.

EGU23-13932 | Posters on site | CL4.1

The Impact of Recent European Droughts and Heatwaves on Trace Gas Surface Fluxes: Insights from Land Surface Data Assimilation 

Paul Hamer, Heidi Trimmel, Jean-Christophe Calvet, Bertrand Bonan, Catherine Meurey, Islen Vallejo, Sabine Eckhardt, Gabriela Sousa-Santos, Virginie Marecal, and Leonor Tarrason

Heatwave and drought extremes can have significant impacts on vegetation, which can in turn lead to important effects on reactive trace gas fluxes at the land-atmosphere interface that can ultimately alter atmospheric composition. We present results from the EU-funded Sentinel EO-based Emission and Deposition Service (SEEDS) project, which aimed at developing upgrades to the existing Copernicus Atmospheric Monitoring Service (CAMS) component on European air quality. In this work, we used land surface modelling (SURFEX – Surface Externalisée) combined with data assimilation (Extended Kalman Filter - EKF) of satellite leaf area index (LAI) to deliver improved estimation of the land surface state. The land surface model is coupled with an online model for dry deposition and an offline model (MEGANv3.1) for biogenic volatile organic compounds (BVOCs) to estimate trace gas losses and emissions, respectively. This approach exploits methods at the forefront of land surface modelling (dynamic vegetation simulation and data assimilation) and combines them with the latest algorithms to estimate trace gas fluxes at the surface. We present findings from two extreme events in Europe: the 2018 drought and the 2019 June/July heat waves. SURFEX was forced using ECMWF meteorology at 0.1° × 0.1° resolution that captured both events. Both extreme events provoked strong responses in the models for dry deposition velocity and BVOC emissions. The 2018 drought began in spring and endured through summer, during which dry deposition velocities declined steadily beyond seasonal norms due to increased stomatal resistance forced by the vegetation response to drought. Over continental Europe, BVOCs initially increased in the early phase of the drought, but then sharply declined into July in the worst-affected regions in Germany, Denmark, and Poland. Meanwhile, BVOCs increased in Scandinavia relative to seasonal norms due to the warmer-than-average conditions. The first episode of severe heat in 2019 arrived in late June, which initially caused a large increase in BVOC emissions compared to seasonal norms. Then drought set in during July and despite a second large heat wave BVOC emissions were lower overall compared to seasonal norms. In fact, the European-wide BVOC emissions were higher in June compared to July due to the drought effects that commenced later in the heat wave cycle. This reverses the normal seasonal cycle in BVOC emissions, and drought impacts on vegetation were the primary driver behind this. Dry deposition velocities are reduced during both heat waves, but we see a larger decline in the second heat wave in July when drought conditions are more severe.

Our findings suggest that these impacts on trace gas surface fluxes would have a strong effect on atmospheric composition, and on photochemical ozone formation. We, therefore, conclude that these effects likely played a contributory role to the ozone pollution episodes that occurred coincidentally in time with the heat wave events in both 2018 and 2019. The project aim within SEEDS is to eventually test the BVOC emissions and dry deposition velocities within a chemical transport model participating within the CAMS regional ensemble (MOCAGE) and to therefore evaluate the impact on ozone.

How to cite: Hamer, P., Trimmel, H., Calvet, J.-C., Bonan, B., Meurey, C., Vallejo, I., Eckhardt, S., Sousa-Santos, G., Marecal, V., and Tarrason, L.: The Impact of Recent European Droughts and Heatwaves on Trace Gas Surface Fluxes: Insights from Land Surface Data Assimilation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13932, https://doi.org/10.5194/egusphere-egu23-13932, 2023.

EGU23-14104 | ECS | Orals | CL4.1

Transpiration in forest ecosystems based on deep learning and sap flow observations 

Marco Hannemann, Almudena García-García, and Jian Peng

Transpiration (T), the component of evaporation (E) controlled by vegetation, dominates terrestrial Evaporation, but measurements are highly uncertain. In the light of the importance of evaporation for studying the terrestrial water cycle, hydro-climatic extremes such as droughts and heatwaves and land-atmospheric interactions, there is a strong demand on novel approaches to reliably estimate T. Currently available approaches to estimate T mostly rely on its relationship with photosynthesis, but parameterizing this relationship is difficult and estimates of T strongly disagree among each other in terms of magnitude. Moreover, in-situ measurements are scarce and and evaporation cannot be measured directly from space.

We developed a hybrid Priestley-Taylor (PT) model using Deep Learning to learn the relationship between T and state variables such as soil moisture, vapor pressure deficit and the fraction of photosynthetic active radiation for different plant functional types (PFTs). We use globally available variables from reanalysis and remote sensing data as forcing to train an artificial neural network on the PT-coefficient α obtained by inverting the PT model on sap flow based ecosystem T. In this way, we can predict Transpiration at local scales independently from hard-to-obtain fluxes like E or vegetation parameters such as stomatal conductance. We evaluate our algorithm against T estimates from flux partitioning methods based on water use efficiency at eddy covariance sites for different PFTs and regions. Also, we compare our estimates with other available products of transpiration like GLEAM, PML-V2 and ERA5-Land. Preliminary results of this research showed that the developed model can learn the relationship between T and few influencing variables, without incorporating variables such as net radiation or GPP. Our findings contribute to dissolving the scarcity of T estimates in forest ecosystems based on actual observations. Future work is needed to apply our method to the larger scale for studying spatial patterns of T, e.g. across the European continent.

How to cite: Hannemann, M., García-García, A., and Peng, J.: Transpiration in forest ecosystems based on deep learning and sap flow observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14104, https://doi.org/10.5194/egusphere-egu23-14104, 2023.

EGU23-14158 | Posters on site | CL4.1

Continuous observations of CO2 and CH4 exchange from East-African rangelands 

Lutz Merbold, Vincent Odongo, Thomas Dowling, Francesco Fava, Ilona Glücks, Anton Vrieling, Martin Wooster, and Sonja Leitner

Semi-arid rangelands in Sub-Saharan Africa (SSA) are an important source of food security and nutrition but are under increased anthropogenic pressure by a growing population. These rangelands are characterized by nutrient poor soils and distinct wet and dry season(s). Due to the soil and climate combination, conventional crop agriculture is rarely feasible without irrigation and mineral fertilizer amendments, which in turn are limited by prohibitively high fertilizer prices and lack of water. Instead, pastoral livestock keeping is a valuable option to use these marginal lands and – under the right management – can be a sustainable form of food production and biodiversity protection given that most of these landscapes have co-evolved with megafauna over millennia. Despite the global role of livestock systems on climate change, there is still limited understanding on the role of SSA rangelands. At the same time, livestock systems emit greenhouse gases (GHG) and can promote global warming. But despite the impact of livestock systems on climate change, our understanding of the role of SSA rangelands is limited. To date, a thorough assessment that includes continuous GHG exchange measurement in combined wildlife-livestock systems on the African continent has not been undertaken. Here we provide the first eddy covariance (EC) measurements of CO2/CH4/H2O fluxes from the ILRI Kapiti Wildlife Conservancy - a benchmark rangeland site in East Africa that is grazed by livestock and wildlife. Our results show continuous ecosystem CO2 uptake from the wet to dry seasons with considerable CO2 emission pulses following precipitation events after long dry periods that turn the landscape into short-term net CO2 emitters. In contrast to CO2, CH4 fluxes are highly variable and depend particularly on wildlife and/or livestock being present in the fetch of the EC tower. In addition to EC measurements and given the need for scaling of our results, we relate CO2 and CH4 fluxes to simple remote sensing measurements of vegetation greenness derived from phenological cameras. Our results show good agreement between the two approaches. Yet, more observations across a climatic gradient and along varying management intensities are needed to reduce existing uncertainties in the effect of SSA rangelands on climate change. To build a complete GHG budget, hot spots of greenhouse gas emissions such as from livestock enclosures or water bodies as well as soil carbon sequestration have yet to be accounted for.

How to cite: Merbold, L., Odongo, V., Dowling, T., Fava, F., Glücks, I., Vrieling, A., Wooster, M., and Leitner, S.: Continuous observations of CO2 and CH4 exchange from East-African rangelands, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14158, https://doi.org/10.5194/egusphere-egu23-14158, 2023.

EGU23-14377 | Posters on site | CL4.1

Sensitivity to soil moisture initialization in the simulation of Indian pre-monsoon season, using a regional climate numerical model 

Arjun Vasukuttan, Lorenzo Sangelantoni, Ka Shateesan, and Gianluca Redaelli

Soil moisture content is crucial for the representation and predictability of hydroclimatic extremes of different spatial/temporal scales such as heavy rainfall, droughts and heatwaves. In order to include these effects and the relevant feedback with the atmosphere in a regional climate model, the soil moisture initialization has to be adequate.

This study explores the soil moisture precipitation (SM-P) feedback, the soil moisture temperature (SM-T) feedback and the heat fluxes over the entire domain and 3 smaller regions of interest. A hydrostatic version of the Regional Climate Model  4.7 (RegCM4.7) with Arakawa B grid is used to run the simulations. The simulations  are performed for the months February to May during the years 2008, 2009 and 2010 with a spatial resolution of 12 km and temporal resolution of 3 hours. The initial and boundary conditions(ICBC)  are derived from the ERA5 data.  We examine results from simulations initiated using three different soil moisture datasets, namely, the control, dry and wet datasets. The soil moisture data from the ERA5-Land reanalysis is used for the control simulation. A dry/wet simulation is run using dry/wet datasets derived from the ERA5-Land data. This is done by halving/doubling the soil moisture values from ERA5-Land data, giving rise to new soil moisture values with lower/higher soil moisture as compared to the control dataset (ERA5-Land). CMORPH (Climate Prediction Center (CPC) Morphing Technique (MORPH)) and CRU (Climate Research Unit) datasets are used as reference to evaluate the precipitation and temperature values resulting from the control simulation.

The results display the mean changes in the dry/wet simulation results with respect to the control simulation. Plots showing the vertical profile changes in relative humidity and air temperature, and changes in lower tropospheric wind and specific humidity, indicates the build-up of the observed precipitation events and temperature patterns induced by the initial soil moisture perturbation. Interestingly the simulation results show negative SM-P feedback.  In other words, the average precipitation seemed to increase/decrease for the dry/wet cases with respect to the control simulation. This is contrary to the general expectation that dry/wet soil moisture decreases/increases precipitation. The possible reasons for the negative SM-P feedback and its distribution over the region include the proximity to the ocean, topography, and the pre-monsoon dryline. The SM-T and the heat fluxes on the other hand display expected behaviour with few exceptions in some regions in the dry simulation case.

How to cite: Vasukuttan, A., Sangelantoni, L., Shateesan, K., and Redaelli, G.: Sensitivity to soil moisture initialization in the simulation of Indian pre-monsoon season, using a regional climate numerical model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14377, https://doi.org/10.5194/egusphere-egu23-14377, 2023.

Numerous cyclones develop in the Bay of Bengal during the pre-monsoon and post-monsoon seasons. The heavy rain associated with these cyclones causes devastating damage to life and property during landfall. The modern numerical weather prediction models and high temporal satellite observation data have significantly increased the accuracy of cyclone prediction in recent years. However, accurately predicting rainfall intensity and its dissipation after landfall is still challenging. Previous studies have indicated that land-based evapotranspiration plays an essential role in determining the intensity and decay of cyclones post-landfall. In this study, we quantify the contribution of land-based evapotranspiration to the rainfall associated with cyclones and the impact of land conditions on the speed and track of cyclones originating in the Bay of Bengal. For this purpose, we employed the Weather Research Forecasting (WRF) model upgraded with Eulerian water tagging capabilities to track evapotranspiration from land. The tagging model will tag the evapotranspiration originating on land and track it throughout the atmosphere till it precipitates or moves out of the domain. We simulated six cyclones of varying intensities, with three during the pre and three during the post-monsoon seasons. We conducted sensitivity experiments with dry and wet initial soil moisture conditions to determine the impact of perturbed soil moisture on TC. To account for the model's internal variability, we simulated an ensemble with four members for the control simulation. The ensemble is created by changing each member's model initialization time by six hours. This ensemble helped identify the magnitude of the model's internal variability, which was less than the variability due to soil moisture changes. The study revealed that soil moisture conditions prior to TC formation have an impact on its evolution. By analyzing the latent heat, temperature, and wind pattern, we found that the initial soil moisture during the pre and post-monsoon seasons alters the synoptic features over the Indian subcontinent, resulting in variations in the TC evolution. The relatively low-intensity TC tracks are more sensitive to the initial soil moisture conditions. The rainfall originating from land-based evapotranspiration is more significant as the cyclone approaches land. Therefore, land-based evapotranspiration plays a crucial role in the end phase of the cyclone (from just before landfall till its decay). For post-monsoon cyclones, the rainfall from land-based evapotranspiration is as high as 20% to 30% after landfall, whereas, for pre-monsoon cyclones, the land contribution is around 5% to 10%. In addition to soil moisture, factors such as proximity to land, track length over land, and TC intensity also have a role in determining the quantity of precipitation originating from the land for a TC.

How to cite: Lanka, K. and Navale, A.: Influence of Soil Moisture on the Evolution of Landfalling Tropical Cyclones during pre and post-monsoon seasons, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15299, https://doi.org/10.5194/egusphere-egu23-15299, 2023.

EGU23-15403 | Orals | CL4.1 | Highlight

Global observations highlight regions where vegetation can enhance S2S predictability 

Christopher Taylor and Bethan Harris

The land surface is a key source of predictability for forecasts at the subseasonal-to-seasonal (S2S; 2 weeks to 2 months) timescale, since variables such as root zone soil moisture and leaf area vary more slowly than the atmospheric state. Previous work has mostly focused on the predictability gained from realistic soil moisture initialisations. Considering observable land surface variables, vegetation shows more persistent changes than surface soil moisture following subseasonal rainfall events, and therefore has the potential to provide predictability at longer lead times. We therefore perform the first investigation of vegetation feedbacks onto near-surface air temperatures using global daily data, to ascertain in which regions and seasons these feedbacks can provide S2S predictability. We use daily datasets of Vegetation Optical Depth (VOD, from the VODCA X-band product) and 2m temperature (from ERA5) at 0.25° horizontal resolution, and compute lagged correlations to identify where spatial structures in VOD anomalies are associated with similar structure in 2m temperature anomalies. Using daily data allows us to investigate how the correlations decay as a function of lead time within the S2S timescale. At zero lag, water-limited regions exhibit negative correlations, indicating that an increase in vegetation water content is associated with increased evapotranspiration and reduced sensible heat, leading to cooler near-surface air temperatures. We find extensive regions in the semi-arid tropics and sub-tropics where at certain times of year VOD anomaly patterns are anti-correlated with temperature patterns 2 weeks ahead. These periods tend to occur outside of the wettest time of year. In some regions, e.g. southern Africa in MAM,  predictability of temperature from VOD anomalies extends to lags of 30 days, suggesting that incorporating vegetation variability can improve S2S forecasting. We develop a model for the strength and persistence of vegetation feedbacks to near-surface temperatures based on seasonal cycles of rainfall and vegetation.

How to cite: Taylor, C. and Harris, B.: Global observations highlight regions where vegetation can enhance S2S predictability, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15403, https://doi.org/10.5194/egusphere-egu23-15403, 2023.

EGU23-16444 | ECS | Orals | CL4.1

Exploring deep root water uptake, soil moisture, and land surface fluxes in the Amazon 

Carolina Bieri, Francina Dominguez, Gonzalo Miguez-Macho, and Ying Fan

Plant roots act as critical pathways of moisture from subsurface sources to the atmosphere. Moreover, deep plant roots allow vegetation to meet water demand during seasonally dry periods by taking up moisture from accessible groundwater. This is an important resilience mechanism in the Amazon, a hydrologically and ecologically significant region. However, most regional land-atmosphere computational models do not adequately capture the link between deep roots and groundwater. This study details the implementation of a dynamic rooting scheme in the Noah-Multiparameterization (Noah-MP) land surface model, a widely used tool for studying the exchange of energy and moisture between the land and atmosphere. The rooting scheme is a first-order representation of dynamic rooting depth based on the soil water profile and includes quantification of deep root water uptake (RWU). The scheme is easily scalable and ideal for regional or continental-scale climate simulations. It is used in conjunction with a groundwater scheme which captures high-resolution spatial groundwater variations, allowing us to capture the critical link between deep roots and groundwater. We perform 10-year simulations with and without the root scheme for a test region in the Amazon to validate the enhanced model. We analyze time series of soil moisture, RWU, and evapotranspiration for points with differing vegetation cover and elevation. This allows us to demonstrate functionality of the root scheme and ensure it behaves properly for varying conditions. Representation of deep RWU is critical for realistic simulation of the soil-plant-atmosphere system. As the land surface is an important component of atmospheric predictability, inclusion of deep RWU can contribute to improved prediction of atmospheric variables such as precipitation.

 

How to cite: Bieri, C., Dominguez, F., Miguez-Macho, G., and Fan, Y.: Exploring deep root water uptake, soil moisture, and land surface fluxes in the Amazon, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16444, https://doi.org/10.5194/egusphere-egu23-16444, 2023.

EGU23-1134 | Orals | AS2.6

Transparent exopolymer particles (TEP) in the tropical oligotrophic Atlantic Ocean: Sea-to-air transfer and atmospheric in situ formation 

Manuela van Pinxteren, Tiera-Brandy Robinson, Sebastian Zeppenfeld, Oliver Wurl, Heike Wex, Anja Engel, and Hartmut Herrmann

Transparent exopolymer particles (TEP) exhibit the properties of gels and are ubiquitously found in the world oceans. Here we demonstrate that TEP may enter the atmosphere as part of sea spray aerosol and likely influence cloud properties. We show number concentrations of TEP with a diameter > 4.5 µm, hence covering a part of the supermicron particle range measured in ambient aerosol and cloud water samples from the tropical Atlantic Ocean. Furthermore, TEP were analysed in generated aerosol particles using a plunging waterfall tank that was filled with the ambient seawater.

Based on Na+ concentrations in seawater and the atmosphere, the enrichment of TEP in the tank generated aerosol particles was well in-line with another study. The TEP enrichments in the ambient atmosphere were, however, up to two orders of magnitude higher compared to the tank study and such high values are thus far not reported for supermicron aerosol particles. We propose that the high enrichment of TEP in the particles and in cloud water result from a combination of enrichment during bubble-bursting transfer from the ocean and secondary in-situ atmospheric formation. We suggest that similar (biotic and abiotic) formation mechanism reported for TEP formation in the (sea)water might take place in the atmosphere as well, as the required conditions (e.g. high concentrations of dissolved TEP precursors such as polysaccharides, presence of bacteria in the cloud water) were given.

TEP concentrations in the atmosphere were two orders of magnitude higher than INP concentrations in the aerosol particles and cloud water, respectively. However, only a part of the TEP population, assumingly the one colonized by bacteria, might contribute to INP population, and are worth further studies.

The study contributes to the international SOLAS program.

Ref. : van Pinxteren, M., Robinson, T.-B., Zeppenfeld, S., Gong, X., Bahlmann, E., Fomba, K. W., Triesch, N., Stratmann, F., Wurl, O., Engel, A., Wex, H., and Herrmann, H.: High number concentrations of transparent exopolymer particles in ambient aerosol particles and cloud water – a case study at the tropical Atlantic Ocean, Atmos. Chem. Phys., 22, 5725–5742, https://doi.org/10.5194/acp-22-5725-2022, 2022.

 

How to cite: van Pinxteren, M., Robinson, T.-B., Zeppenfeld, S., Wurl, O., Wex, H., Engel, A., and Herrmann, H.: Transparent exopolymer particles (TEP) in the tropical oligotrophic Atlantic Ocean: Sea-to-air transfer and atmospheric in situ formation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1134, https://doi.org/10.5194/egusphere-egu23-1134, 2023.

EGU23-1513 | Posters on site | AS2.6

Contribution of metal production to bioaccessible Fe deposition into Southern Indian Ocean 

Akinori Ito and Takuma Miyakawa

Atmospheric iron (Fe) from anthropogenic, lithogenic, and pyrogenic sources contributes to ocean fertilization, climate change, and human health risk. However, significant uncertainties remain in the source apportionment, due to a lack of source-specific evaluation of Fe-laden aerosols. Here, the large uncertainties in the model estimates are investigated using different Fe emissions from metal production.  The anthropogenic and lithogenic factors are evaluated by using high-time-resolution measurements of Fe-laden species in fine particulate matter at Fukue observational site in downstream region of East Asian outflow. The better agreement in anthropogenic factor of aerosol Fe concentrations with the field data is obtained with the low estimate of smelting Fe emission. Our simulation with the low estimate of smelting Fe emission confirms that anthropogenic aerosols play dominant roles in bioaccessible Fe deposition to the northwestern Pacific, compared to lithogenic sources. Aerosol Fe co-emitted with sulfur dioxide from metal production predominantly contributes to atmospheric bioaccessible Fe input to the Southern Indian Ocean. Our simulation with different estimates of smelting Fe emission reveals that accurate representation of aerosol Fe from metal production is a key to reduce large uncertainties in bioaccessible Fe deposition to the Southern Ocean.

How to cite: Ito, A. and Miyakawa, T.: Contribution of metal production to bioaccessible Fe deposition into Southern Indian Ocean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1513, https://doi.org/10.5194/egusphere-egu23-1513, 2023.

While plastics are indispensable to our lives, they are known to emit harmful chemicals which can cause devastating effects to the environmental and human health. With the increasing concerns for global air pollution and climate change, the potential contributions of volatile organic compounds (VOCs) released from plastics have also been receiving increasing attention in recent years. Here, we developed and optimized a method for characterization of VOCs emitted from plastics. Using a selected-ion flow tube mass spectrometry (SIFT-MS), VOCs emissions were measured in real-time and data interpretations were performed using multivariate analysis. Expanded polystyrene (EPS), polypropylene (PP), high- and low-density polyethylene (HDPE and LDPE) and polyethylene terephthalate (PET) pellets were selected by their dominance as marine plastic debris. Emission characteristics of VOCs from selected polymers were monitored according to temperatures from 30℃ to 80℃. The emission of VOCs significantly increased with increasing temperatures for all plastic types, but varied in the order of LDPE, HDPE, PP, EPS, and PET. Partial least squares (PLS) analysis showed significant differences in compound group types, especially for compounds with relatively high molecular weight when heated at 80℃. The less-distinct differences in clustering of VOCs emitted at temperatures below 80℃, especially 60℃, were likely represented by additives and residuals during plastic production while VOCs emitted with temperatures above 80℃ were likely due to thermal degradation of polymers. The emitted compounds showed the highest mass concentrations with hydrocarbons such as alkane and alkene followed by monomers of each plastic type. These results suggested that the temperature threshold for VOCs emissions from residual materials and thermal degradations needs to be considered as one of the main factors for the analysis of VOCs from plastic debris.

How to cite: Choi, N., An, J., Kim, D., Loh, A., and Yim, U.: Optimization of analytical method for volatile organic compounds released from plastics and their emission characteristics by selected-ion flow tube mass spectrometry., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2508, https://doi.org/10.5194/egusphere-egu23-2508, 2023.

EGU23-4826 | ECS | Posters on site | AS2.6

Impacts of wildfire aerosol on carbon uptake and sea-ice in the East Siberian Sea 

Min-Woo Seok, Young Ho Ko, and Tae-Wook Kim

The frequency of wildfires has increased in the Siberian region. Wildfire plumes carrying black carbon and biologically important elements may have impacts on downwind ocean regions including Arctic seas such as the East Siberian Sea (ESS). However, the responses of marine environments to the wildfire plume introduced to the ESS are not well known. In this study, we tried to identify changes in ocean phytoplankton and sea-ice associated with wildfire activities by utilizing satellite-based and reanalysis data. The amount of carbon produced by wildfires in Boreal Asia coincides with the concentration of black carbon, indicating that wildfires are responsible for the majority of the black carbon in the atmosphere. In addition, we could detect wildfire plume-derived significant increases in ocean carbon uptake from satellite-based bio-optical variables (phytoplankton growth and biomass concentration). Summertime black carbon deposition has more than doubled over the last decade, and black carbon deposition was highly correlated with sea-ice melting rate, implying a contribution of black carbon deposition on sea-ice melting, which may increase ocean productivity by enhancing light availability in the upper ESS.   

How to cite: Seok, M.-W., Ko, Y. H., and Kim, T.-W.: Impacts of wildfire aerosol on carbon uptake and sea-ice in the East Siberian Sea, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4826, https://doi.org/10.5194/egusphere-egu23-4826, 2023.

EGU23-6011 | ECS | Orals | AS2.6

What happens to biomass burning-emitted particles in the Ocean? A laboratory experimental approach based on their tracers 

Juan Miguel González-Sánchez, Christos Panagiotopoulos, Candice Antich, France Van Wambeke, and Benjamin Misson

Biomass burning is a major contributor to the emission of particle matter in the atmosphere (up to 90 % of primary organic aerosol) and thus has an impact on climate, human health, and ecosystems. Once emitted, biomass burning-derived organic aerosol can be transported to the oceans. However, the impact and fate of this particulate matter and its major components in the marine biological carbon pump and the trophic chain are largely unknown. Understanding these processes is of paramount importance to better asses the carbon cycle. This work presents the first attempt to investigate the bioavailability of two biomass-burning tracers (i.e., levoglucosan and galactosan) in seawater inoculated with marine microorganisms. To do so, a novel method was developed to extract the anhydrosugar from their salty matrix and monitor their evolution for 44 days under controlled conditions. Along with the anhydrosugar concentration, multiple parameters (dissolved organic carbon, inorganic nutrient concentrations, prokaryotic production, heterotrophic prokaryotes abundance, and prokaryotic diversity) were monitored to achieve a complete picture of their fate in seawater. Furthermore, two control experiments (glucose- and non-amended) were run in parallel for comparison purposes. The results show that both levoglucosan and galactosan can be biodegraded at slow rates as their concentrations dropped from 2.5 ± 0.6 and 2.4 ± 0.3 μM to 0.1 ± 0.1 and 1.5 ± 0.7 μM, respectively, over a period of 44 days. The decrease in the levoglucosan and galactosan concentrations was accompanied by an increase in both prokaryotic production (up to 40 and 5 times greater, respectively, when compared to the non-amended experiment) and heterotrophic prokaryotes abundance (for levoglucosan, up to one order of magnitude greater than the non-amended experiment). While glucose was assimilated by heterotrophic prokaryotes within 1.7 days, levoglucosan and galactosan biodegradation did not start until at least 8.7 days after the experiments were set. These delays suggest that the chemical structure of these anhydrosugars can only be tackled by specific enzymatic abilities regulated by slow-growing heterotrophic prokaryotes. Prokaryotic diversity analyses revealed the predominance of a few bacterial genera from the Roseobacter clade that were specifically selected by the addition of the anhydrosugars. These results raise questions about the enzymatic capabilities of this widespread marine bacterial clade and the processing of semi-labile compounds accumulating in surface ocean waters. This work shows that biomass-burning organic compounds have the potential to be biodegraded by prokaryotic bacteria and thus contribute to the trophic chain and the production of CO2

How to cite: González-Sánchez, J. M., Panagiotopoulos, C., Antich, C., Van Wambeke, F., and Misson, B.: What happens to biomass burning-emitted particles in the Ocean? A laboratory experimental approach based on their tracers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6011, https://doi.org/10.5194/egusphere-egu23-6011, 2023.

EGU23-7047 | Orals | AS2.6

Development, intercomparison and evaluation of an improved mechanism for the oxidation of dimethyl sulfide 

Alexander Archibald, Ben Cala, Scott Archer-Nicholls, N. Luke Abraham, Paul Griffiths, Lorrie Jacob, Matthew Shin, Laura Revell, and Matthew Woodhouse

Dimethyl sulfide (DMS) is an important trace gas emitted from the ocean. The oxidation of DMS is important for global climate through the role DMS plays in setting the sulfate aerosol background in the troposphere. However, the mechanisms of DMS oxidation are very complex and have proved elusive to accurately determine in spite of decades of research. As a result the representation of DMS oxidation in global chemistry-climate models is often greatly simplified. Recent field observations and laboratory studies have prompted renewed efforts in constraining the uncertainty in the oxidation mechanism of DMS as incorporated in global chemistry-climate models. Here we build on recent laboratory and observational evidence and develop a new DMS mechanism for inclusion in the UKCA chemistry-climate model. We compare our new mechanism to the existing UKCA mechanism and to a range of recently developed mechanisms reported in the literature through a series of global and box model experiments. Our box model experiments highlight that there is significant variance in simulated secondary oxidation products of DMS across mechanisms used in the literature, with divergence in the sensitivity of these products to temperature exhibited. Our global model studies show that our updated and improved DMS scheme performs better than the current scheme when compared against observations. However, sensitivity studies underscore the need for further laboratory and observational constraints.

How to cite: Archibald, A., Cala, B., Archer-Nicholls, S., Abraham, N. L., Griffiths, P., Jacob, L., Shin, M., Revell, L., and Woodhouse, M.: Development, intercomparison and evaluation of an improved mechanism for the oxidation of dimethyl sulfide, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7047, https://doi.org/10.5194/egusphere-egu23-7047, 2023.

EGU23-8058 | ECS | Orals | AS2.6

Nighttime atmospheric nucleation driven by marine microorganisms 

Guillaume Chamba, Maija Peltola, Theresa Barthelmeß, Matti Rissanen, Clémence Rose, Siddharth Iyer, Alexia Saint-Macary, Alfonso Saiz-Lopez, Manon Rocco, Karl Safi, Stacy Deppeler, Neil Barr, Mike Harvey, Anja Engel, Erin Dunne, Cliff Law, and Karine Sellegri

Understanding ocean-cloud interactions and their effect on climate requires that atmospheric new particle formation is characterized. Yet, the process of particle formation from marine biogenic gaz-phase emissions has not been evidenced in the open ocean lower atmosphere, partly due to the naturally low concentrations of these particles in remote oceanic places. Here we show, using new ship-borne air-sea interface enclosures, that new particles are formed in relation to marine micro-biology present in the seawater. The chemical analysis of newly formed clusters with API-ToF-MS shows unexpected results, implicating nucleating coumpounds and pathways that are usually not taken into account in nucleation processes.

How to cite: Chamba, G., Peltola, M., Barthelmeß, T., Rissanen, M., Rose, C., Iyer, S., Saint-Macary, A., Saiz-Lopez, A., Rocco, M., Safi, K., Deppeler, S., Barr, N., Harvey, M., Engel, A., Dunne, E., Law, C., and Sellegri, K.: Nighttime atmospheric nucleation driven by marine microorganisms, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8058, https://doi.org/10.5194/egusphere-egu23-8058, 2023.

Atmospheric transport and deposition of dust aerosol is very efficient in supplying iron to large part of global oceans. In this study, an Earth system model with ocean biogeochemistry component is used to explore how dust deposition can impact vertical distribution of dissolved iron (DFe) and phosphate in the upper 1000 m of the global oceans by impacting phytoplankton growth.  Although large areas of the global oceans show positive chlorophyll response following dust deposition, some regions (those having high levels of background DFe from continental shelf sediments and high atmospheric DFe input) experience net scavenging losses of DFe following dust depositions. Such regions experience a reduction in chlorophyll concentrations along with reduction in particulate organic carbon (POC) production and fluxes following dust deposition. While positive chlorophyll response is associated with low levels of background DFe and low atmospheric DFe input compared to regions experiencing negative chlorophyll response, the magnitude of chlorophyll increase depends on the background nitrate-to-iron ratio. With increase in the magnitude of positive chlorophyll response to atmospheric DFe deposition, an increase in POC production and resulting fluxes are encountered. Such an increase in POC flux can play the dual role of increase in scavenging removal of DFe as well as increase in PFe remineralization. The net result is that variation in NREG (Net REGeneration, taken as difference between PFe remineralization and DFe scavenging) in the upper 1000 m of the ocean has significant positive correlation with variation in POC fluxes, indicating that sinking organic matter following positive chlorophyll response to atmospheric iron deposition is the main driver of net DFe regeneration. Furthermore, a depth-wise difference between the impact of sinking POC and PFe fluxes on NREG is also evident. In the upper 150 m, high POC fluxes drive NREG while at deeper depths, PFe fluxes become important in driving NREG due to slow desorption release of iron from sinking PFe mass. As a result, with increase in POC fluxes, the depth of maximum NREG becomes shallower due to the shorter remineralization length scale of POC compared to lithogenic particles. On the contrary, with increases in the magnitude of atmospheric DFe , the depth of maximum NREG increases due to high dust deposition driving increased scavenging. Furthermore, increase in POC fluxes also leads to regeneration of phosphate at shallower depths. In this manner, the magnitude of chlorophyll response to atmospheric iron can significantly control the patterns of nutrient limitations.

How to cite: Banerjee, P.: Variable role of dust deposition on upper ocean nutrient distribution, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8622, https://doi.org/10.5194/egusphere-egu23-8622, 2023.

EGU23-9032 | Posters on site | AS2.6

Linking production of carbonyl sulphide to the composition of the marine dissolved organic matter pool 

Heike Simon, Marc von Hobe, Thorsten Dittmar, and Sinikka Tina Lennartz

Sulfur containing trace gases impact Earth’s climate, and the ocean is a major natural source for the most abundant sulfur gas in the atmosphere, carbonyl sulfide (COS). Understanding and quantifying COS oceanic emissions is relevant for closing the gap in the atmospheric COS budget, which currently impedes conclusions about trends in stratospheric aerosol formation and gross primary production on a global level. The main production process of COS in surface seawater, photochemical production, remains one of the largest uncertainties in quantifying marine COS emissions. Precursors of COS are dissolved organic molecules, which form an enormously diverse mixture. How the composition of this diverse pool influences COS production has not yet been fully understood.

Here we present continuously measured COS concentrations in seawater and the marine boundary layer to quantify the relationship between photochemical production of COS in various marine regions: Along a North-South Atlantic transect from Bremerhaven to Cape Town and at two stations in the North Sea, one located in the open sea area close to Heligoland, one in the Wadden Sea area close to Spiekeroog Island. Samples of dissolved organic matter (DOM) were taken twice daily for subsequent analysis of the molecular composition and optical properties of the large precursor pool for COS photo- and dark production. Concentrations of COS in surface seawater showed distinct diurnal cycles with considerable day-to-day variations. The marine DOM pool differed with respect to sulfur containing molecules mainly between locations, and less along diurnal cycles. Our results will help to improve mechanistic models of marine COS cycling, especially with regard to the currently existing uncertainties in the global emission estimate of COS.

How to cite: Simon, H., von Hobe, M., Dittmar, T., and Lennartz, S. T.: Linking production of carbonyl sulphide to the composition of the marine dissolved organic matter pool, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9032, https://doi.org/10.5194/egusphere-egu23-9032, 2023.

EGU23-9269 | ECS | Orals | AS2.6

Carbon disulphide in the spotlight: UV-dependent production and consumption processes in seawater and their impact on oceanic emissions 

Sinikka Lennartz, Heike Simon, Dennis Booge, Li Zhou, Thorsten Dittmar, and Christa Marandino

Carbon disulfide (CS2) is one of the most important precursors for atmospheric carbonyl sulphide (OCS), a climate relevant trace gas that can serve as a proxy to quantify terrestrial gross primary production. Currently, limited understanding of the production and consumption processes of CS2 in seawater preclude quantifying its marine emissions, which pose major uncertainties in the atmospheric budget of both OCS and CS2. Here we present controlled incubation experiments with natural dissolved organic matter (DOM) from three different oceanic locations, with and without UV light treatment. We show for the first time that in addition to its photochemical production, CS2 is also naturally degraded by UV light. CS2 is also produced in the dark: while the mechanism of this light independent production process is currently unknown, we show that dark production rates scale with the amount of organic sulphur present in DOM. Our results help to disentangle production and consumption processes of CS2 in seawater, in order to facilitate the interpretation of field measurements and ultimately enable modelling approaches.

How to cite: Lennartz, S., Simon, H., Booge, D., Zhou, L., Dittmar, T., and Marandino, C.: Carbon disulphide in the spotlight: UV-dependent production and consumption processes in seawater and their impact on oceanic emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9269, https://doi.org/10.5194/egusphere-egu23-9269, 2023.

EGU23-10224 | Posters on site | AS2.6

Assessing Air-sea CO2 Flux Products with Constraints from Atmospheric Inverse Analyses 

Parv Suntharalingam, Zhaohui Chen, Jamie Shutler, and Andrew Watson

Oceanic uptake of atmospheric CO2 has been estimated to remove ~25% of  global anthropogenic emissions in recent decades (1990-2020), and this flux displays significant decadal variability (Global Carbon Budget: Friedlingstein et al. 2022). Key contributors to this ocean CO2 flux estimate are data products derived from interpolated surface ocean pCO2 measurements combined with air-sea gas-exchange parameterizations.  Although derived from a common surface ocean CO2 database (Surface Ocean CO2 Atlas (SOCAT), Bakker et al. 2016), these data products display variations on regional and global scales due to differences in their underlying construction methodologies. Here we assess three widely cited air-sea CO2 flux products, namely, Landschutzer et al. (2016), Roedenbeck et al. (2014) and Watson et al. (2020).  Our assessment uses the GEOSChem-LETKF data assimilation system (Chen et al. 2020), together with atmospheric CO2 observations from the NOAA-ESRL global network of surface sites (Obspack_CO2_Globalviewplus, 2020).  The individual air-sea flux products are implemented as alternative representations of the ocean prior flux, and we derive optimized estimates of surface CO2 fluxes in a set of atmospheric inverse analyses with the GEOSChem-LETKF system. We assess the performance of the individual ocean flux products on regional and global scales using a range of metrics derived from the atmospheric inversions including model concentration bias, CO2 flux error reduction, and comparison to independent atmospheric measurements from surface sites and aircraft. We also compare the derived posterior ocean fluxes to estimates from global ocean biogeochemistry models and discuss the implications for closure of the global carbon budget.

How to cite: Suntharalingam, P., Chen, Z., Shutler, J., and Watson, A.: Assessing Air-sea CO2 Flux Products with Constraints from Atmospheric Inverse Analyses, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10224, https://doi.org/10.5194/egusphere-egu23-10224, 2023.

EGU23-10739 | Posters on site | AS2.6

Ocean-air trace gas (N2O) fluxes derived from open-path FTIR atmospheric concentration gradient measurements 

Aldona Wiacek, Martin Hellmich, and Thomas Flesch

Open-Path Fourier Transform Infrared (OP-FTIR) spectroscopy is a well-established technique used to measure path-average trace gas concentrations [ppbv] in the atmospheric boundary layer.  Recently, the technique has been applied to derive trace gas fluxes from soils using the flux-gradient (FG) approach. We describe the novel application of OP-FTIR-FG to derive ocean-air fluxes of N2O [kg N2O ha-1 h-1] at a coastal site in the northwest Atlantic (2018, 2020-2021).  Details of OP-FTIR system deployment across Halifax Harbour (Nova Scotia, Canada) are presented and we describe the application of co-located 3-D sonic anemometer measurements to gas flux calculations.  Finally, we present a full error characterization of N2O flux and a case study of episodic negative (into ocean) flux.  This high frequency (30 min) and spatially averaging (560 m) method is well suited to coastal monitoring of ocean-air N2O fluxes and complementary to ocean-side measurements of N2O in complex circulation and microbial environments.  The possibility of other gas flux detection by this technique will be discussed.

How to cite: Wiacek, A., Hellmich, M., and Flesch, T.: Ocean-air trace gas (N2O) fluxes derived from open-path FTIR atmospheric concentration gradient measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10739, https://doi.org/10.5194/egusphere-egu23-10739, 2023.

EGU23-14624 | ECS | Orals | AS2.6

Insights to the short-term atmospheric deposition impacts on the biology and chemistry of the sea surface microlayer in the Adriatic Sea coastal region 

Andrea Milinković, Abra Penezić, Ana Cvitešić Kušan, Saranda Bakija Alempijević, Valentina Gluščić, Silva Žužul, Ivana Jakovljević, Sanda Skejić, Danijela Šantić, Ranka Godec, Gordana Pehnec, Carola Lehners, Maren Striebel, Jutta Niggemann, Anja Engel, Jelena Godrijan, Blaženka Gašparović, Mariana Ribas Ribas, Oliver Wurl, and Sanja Frka

The Mediterranean basin continuously receives anthropogenic aerosols from industrial and domestic activities from the European region, as well as high rates of aeolian material in the form of mineral dust from northern Africa. Moreover, combustion dominates over natural dust, whereas vegetation fires frequently burn throughout the Mediterranean coastal zone, especially during hot and dry summers. Once in the atmosphere, aerosols become an important external source of nutrients but also of toxins to the marine ecosystem through atmospheric deposition (AD), affecting the quality and quantity of organic matter (OM) produced by phytoplankton in the photic zone, and altering the CO2 uptake. AD onto sea surface cannot be completely understood without considering the interfacial processes within the sea surface microlayer (SML). As the uppermost millimeter of the sea surface, the SML represents the natural interface of the major environmental importance. It could serve as the first indicator of increasing human impact and climate change due to fast response of its biological and physico-chemical properties. However, surprisingly little research assessed the impact of AD on surface plankton communities, distinguishing between the SML and the water column bellow.

This work is designed to assess the magnitude and temporal variability of atmospheric concentrations and deposition fluxes of nutrients and trace metals, and to gain insight into the AD impacts on the nature of enrichments of organic compounds within surface layers in a typical Mediterranean coastal environment. The field campaign was conducted during the period of retrieval of sea surface oligotrophic conditions (February-July 2019) at the Adriatic coastal area. On-line black carbon (BC) concentrations were measured while the aerosol particles (PM10), wet and total deposition samples as well as the SML and underlying water (ULW; 0.5 m depth) samples were collected simultaneously. The first comprehensive insight into concentration levels of macro nutrients (N, P) and trace metals (e.g. Cu, Pb, Cd, Ni, Zn, Co) in atmospheric samples, their transport history, source apportionment and deposition fluxes to the coastal Adriatic area will be presented. The temporal dynamics of SML biology as well as concentrations of inorganic and organic constituents enabled the assessment of their sources and the nature of the enrichments taking place within the SML. Due to their significance throughout the Mediterranean coastal area, open-fire episodes and Saharan dust inputs were especially considered. In order to better understand the impacts of ambient AD from diverse sources on the physiology and biomass of the natural plankton population and consequently on the chemistry of the surface layers (SML and ULW), we further conducted the first in situ bioassay incubation experiment of its kind at the Adriatic Sea. We experimentally examined the impact of locally collected anthropogenic aerosols, that had different levels of biologically important nutrients, trace metals and organic pollutants, in contrast to the material mimicking biomass burning events.

Acknowledgment: This work has been supported by the Croatian Science Foundation under the IP-2018-01-3105 project: Biochemical responses of oligotrophic Adriatic surface ecosystems to atmospheric deposition inputs.

How to cite: Milinković, A., Penezić, A., Cvitešić Kušan, A., Bakija Alempijević, S., Gluščić, V., Žužul, S., Jakovljević, I., Skejić, S., Šantić, D., Godec, R., Pehnec, G., Lehners, C., Striebel, M., Niggemann, J., Engel, A., Godrijan, J., Gašparović, B., Ribas Ribas, M., Wurl, O., and Frka, S.: Insights to the short-term atmospheric deposition impacts on the biology and chemistry of the sea surface microlayer in the Adriatic Sea coastal region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14624, https://doi.org/10.5194/egusphere-egu23-14624, 2023.

EGU23-15168 | Orals | AS2.6

Seasonal DMSP production dynamics in temperate waters driven by significant contributions from both eukaryotic and prokaryotic autotrophs 

Frances Hopkins, Ruth Airs, Beth Williams, Qianyao Ma, Xiaoyu Zhu, and Jonathan Todd

The influence of dimethyl sulfide (DMS) on climate is potentially large but highly uncertain. Some of this uncertainty results from the over-simplification of biological drivers of marine DMS production within predictive models. The available models rely on chlorophyll (chl) as the sole biological parameter and often fail to replicate observations, particularly during highly productive events with elevated seawater DMS concentrations. The major precursor for DMS is dimethylsulfoniopropionate (DMSP), an abundant compatible solute produced by many marine eukaryotes and prokaryotes. Despite its importance, knowledge of how, why and by what DMSP is produced is limited. For example, haptophytes and dinoflagellates typically produce 50-100 times more DMSP per unit chl than diatoms and prochlorophytes - yet the relevant enzymes have until recently been poorly characterised, limiting our understanding. Furthermore, although the DMSP synthesis genes and their transcripts are widespread in surface ocean bacterial communities, the contribution by this group of organisms to total DMSP production is so far unquantified.

Here, we explore the diversity and expression of functional DMSP synthesis and lyase genes alongside DMS/P biogeochemical states and rates over a spring-summer time series (March – July 2021) at an established time series station in temperate shelf sea waters, to characterise the biological drivers of DMSP and DMS production.

DMSP concentrations ranged from <5 nmol L-1 to 160 nmol L-1, with peaks in mid April and late June. The April peak coincided with significant increases in the transcription of eukaryotic DMSP biosynthesis genes. As the season progressed, the eukaryotic transcripts fell dramatically, whilst an increase in transcription of prokaryotic (cyanobacterial) DMSP biosynthesis genes was observed. DMS concentrations in the spring/summer productive period were characterised by three sharp peaks in early May (27 nmol L‑1), early June (13 nmol L-1) and late June (20 nmol L-1),interspersed with lower concentrations of ~2 - 6nmol L-1. Each peak was associated with distinct prokaryotic community composition. Some relationships were observed between the DMS peaks and the transcription of eukaryotic DMS production genes and prokaryotic DMS degradation genes, demonstrating the fine balance of processes which determine net DMS production in the surface ocean.  Overall, we observed that both eukaryotic and prokaryotic autotrophs significantly contributed to seasonal variation in DMSP production in these temperate waters.

How to cite: Hopkins, F., Airs, R., Williams, B., Ma, Q., Zhu, X., and Todd, J.: Seasonal DMSP production dynamics in temperate waters driven by significant contributions from both eukaryotic and prokaryotic autotrophs, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15168, https://doi.org/10.5194/egusphere-egu23-15168, 2023.

EGU23-15506 | ECS | Orals | AS2.6

Physicochemical Properties of Nascent vs. Aged Sea Spray Aerosols in the Eastern North Atlantic 

Sneha Aggarwal, Olga Garmash, Delaney Kilgour, Chris Jernigan, Julika Zinke, Xianda Gong, Shengqian Zhou, Jiaoshi Zhang, Gabriel Freitas, Bruno Cunha, Tercio Silva, Jian Wang, Timothy Bertram, Joel Thornton, Matthew Salter, Paul Zieger, and Claudia Mohr

Sea spray aerosols (SSA) represent one of the largest sources of atmospheric particles since over two-thirds of the Earth’s surface is covered by oceans. They play an important role in climate and atmospheric chemistry, however, despite this a series of knowledge gaps hinder us from constraining their relevance. One critical question is why the physicochemical properties of nascent particles generated in the laboratory are so different from those measured in the ambient marine atmosphere. For example, a series of studies have highlighted that SSA generated in the laboratory exhibit essentially the same ability to act as cloud condensation nuclei as inorganic sea salt, regardless of the amounts of organic substances present in the seawater from which they were generated (e.g., Collins et al., 2016). This is in stark contrast to observations of ambient marine aerosols - their ability to act as cloud condensation nuclei is often significantly reduced in comparison (Swietlicki et al., 2000).

To address this discrepancy, we prepared a novel experimental setup in which we deployed a chemical ionisation mass spectrometer (CIMS) with an Aim inlet in a setup together with a sea spray simulation chamber, an oxidative flow reactor (OFR), and a differential mobility particle sizer (DMPS) at Graciosa Island, Azores, in the eastern north Atlantic Ocean during summer 2022 as a part of the AGENA campaign.

We used freshly-sampled ocean water to generate SSA that were aged in an OFR for an equivalent period of 3 to 3.5 days in the atmosphere. We recorded the gas-phase chemical composition of nascent and aged aerosols using the AIM-CIMS with multiple reagent ions, collected filter samples for offline analysis of the particle-phase chemical composition, and used a DMPS to compare the particle size distribution and concentration.

The first results of our study show that the volatile organic compounds released from the sampled ocean water considerably nucleate when they are oxidized in the OFR. Furthermore, the chemical analysis of these gases reveals an increase in the concentration of DMS oxidation products, such as methane sulfonic acid, when the nascent SSAs along with the gases in the tank headspace are exposed to oxidants in the OFR. However, we did not observe any substantial differences in the concentration and size distribution of the accumulation and larger-mode particles for primary and aged SSA. This could be attributed to extensive nucleation taking place in the OFR. It is possible that in the real world, these VOCs would rather condense on the primary SSA than form new particles.

In this presentation we will compare the properties of ambient SSA particles in the Eastern North Atlantic and those generated and aged with our experimental setup using real seawater in an attempt to address the discrepancy.

Collins, D. B., et al.Geophys. Res. Lett. 2016, 43 (18), 9975-9983.

Swietlicki, E., et al.Tellus B: Chemical and Physical Meteorology 2000, 52 (2), 201-227

How to cite: Aggarwal, S., Garmash, O., Kilgour, D., Jernigan, C., Zinke, J., Gong, X., Zhou, S., Zhang, J., Freitas, G., Cunha, B., Silva, T., Wang, J., Bertram, T., Thornton, J., Salter, M., Zieger, P., and Mohr, C.: Physicochemical Properties of Nascent vs. Aged Sea Spray Aerosols in the Eastern North Atlantic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15506, https://doi.org/10.5194/egusphere-egu23-15506, 2023.

EGU23-15599 | Orals | AS2.6

Evaluation of model-simulated glyoxal in the remote marine atmosphere and dependencies sea-air exchange processes 

Steve Arnold, Natalie Brett, Siyuan Wang, Louisa Emmons, Wuhu Feng, Hannah Walker, Dwayne Heard, Daniel Stone, and Emily Kelly

Reactive volatile organic compounds (VOCs) in the remote marine atmosphere have impacts on climate through affecting atmospheric oxidation capacity (with subsequent effects on methane lifetime), and through affecting remote aerosol abundances, where they may modify cloud condensation nuclei (CCN) concentrations in regions of low CCN abundance. An improved understanding of aerosol and trace gas budgets in the remote marine atmosphere may aid in reducing uncertainties in the extent of anthropogenic warming and cooling contributions to radiative forcing of climate, since they are key components of the background natural atmospheric composition upon which anthropogenic influences are added. Glyoxal (CHOCHO) is a highly reactive oxygenated VOC, which observations have shown is ubiquitous throughout the global troposphere. In the remote marine atmosphere, glyoxal has the potential to act as a source of secondary organic aerosol and to modify the atmospheric oxidising capacity through impacts on radical photochemistry. In our recent work, we demonstrated the potential for acetaldehyde as a source of glyoxal in the remote atmosphere, via a minor oxidation pathway which dominates in-situ glyoxal production in clean marine air masses.

Here we present the first evaluation of global model-simulated glyoxal abundances in the remote marine atmosphere using high temporal (hourly) in situ measurements, and a collection of glyoxal observations synthesised from the literature. Measurements made using a sensitive laser-induced phosphorescence instrument at the Cape Verde Atmospheric Observatory in the tropical Atlantic  over two 4-week campaigns are compared with CAM-chem, a component of the Community Earth System Model (CESM) v2.2 including the MOZART-TS1 tropospheric chemistry mechanism. We show that the global model is capable of reproducing the magnitude of the in situ glyoxal observations from the tropical Atlantic marine boundary layer only when accounting for both the production of glyoxal from acetaldehyde oxidation, and the two-way sea-air exchange of acetaldehyde over the oceans. These model processes also improve the model-simulated glyoxal compared with remote sensing measurements in the tropical Pacific, but with a larger remaining bias. The model is not capable of reproducing observed nighttime glyoxal abundances at Cape Verde, with a large model underestimate. We show that the inclusion of a sea-air emission source of glyoxal, as a proxy for a potential source from the sea surface microlayer, allows the model to reproduce the observed magnitude of nighttime glyoxal. Our results demonstrate that an unconstrained global model is capable of reproducing observed daytime glyoxal abundances in the remote tropical Atlantic atmosphere, and further imply a coupling between acetaldehyde and glyoxal in the remote troposphere. The model results support the potential for a net sea surface to atmosphere source in sustaining nighttime glyoxal concentrations in this region.  

 

How to cite: Arnold, S., Brett, N., Wang, S., Emmons, L., Feng, W., Walker, H., Heard, D., Stone, D., and Kelly, E.: Evaluation of model-simulated glyoxal in the remote marine atmosphere and dependencies sea-air exchange processes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15599, https://doi.org/10.5194/egusphere-egu23-15599, 2023.

EGU23-16526 | Posters on site | AS2.6

Marine methane fluxes to the atmosphere in the Western Black Sea: comparing eddy covariance and diffusive fluxes 

Jean-Daniel Paris, Martin Goxe, Mathis Lozano, Roberto Grilli, Livio Ruffine, Marc Delmotte, Sylvain Bermell, Stéphanie Dupré, and Vincent Riboulot

The global ocean is a net source of CH4 to the atmosphere. Large uncertainties remain on marine emissions that deserves effort to improve current estimates, and eventually predict their trajectories in a changing climate. Ocean CH4 emissions can either be CH4 emanating from seafloor sediments or in situ production in surface water linked to primary productivity. Sediment input into the water column can be either CH4 emanating from hydrate dissociation or free gas rising through the sediment. Ultimately, CH4 enters the atmosphere across the sea-air interface either from bubbles rising from the seafloor or by diffusion from dissolved gas. Estimates of global marine emissions diverge widely due to very large uncertainties linked to limited data coverage, methodological differences and the difficulty to capture the environmental factors that lead to high variability of the emissions.
As the world’s largest natural anoxic waterbody, the semi-enclosed Black Sea (BS) is characterized by widespread seafloor CH4 emissions from the shallow coast to the deep basin. The evolution of the anoxic properties of the BS is strongly linked to the amount of CH4 discharged and the supply of organic matter from the connected large rivers. Therefore, it is crucial to estimate the BS CH4 budget and understand the transfer mechanism to the atmosphere to better understand the impact of climate change. 
During the GHASS2 (Gas Hydrates, fluid Activities and Sediment deformations in the black Sea) cruise in September 2021, CH4 transfer to the atmosphere has been investigated at water depths ranging from 60 m to 1200m in the Western sector of the BS. CH4 partial pressures were measured in the surface water and in the atmosphere using optical spectrometers, respectively the SubOcean membrane inlet laser spectrometer (Grilli et al., 2021, https://doi.org/10.3389/feart.2021.626372) and an ICOS-calibrated commercial analyzer (Picarro model G2401). We report eddy covariance measurements using  an open-path CH4 analyzer Li-7700 and a H2O-CO2 analyzer 7200RS from LiCor, a Gill 3D sonic anemometer, and an inertial navigation sensor (Lord). 
We compare flux estimates obtained from partial pressure gradient by the diffusive method under various schemes with the experimental eddy covariance set-up, applying available corrections for ship movement and interference with airflow. We also compare our results with previous reports for the area and conclude on the respective challenges and relative basin-scale representativity of the various measurement techniques.

How to cite: Paris, J.-D., Goxe, M., Lozano, M., Grilli, R., Ruffine, L., Delmotte, M., Bermell, S., Dupré, S., and Riboulot, V.: Marine methane fluxes to the atmosphere in the Western Black Sea: comparing eddy covariance and diffusive fluxes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16526, https://doi.org/10.5194/egusphere-egu23-16526, 2023.

AS3 – Atmospheric Composition, Chemistry and Aerosols

EGU23-253 | ECS | Posters on site | AS3.1

Phase state of PM2.5 in Seoul and Beijing and its effect on particle size distribution 

Daeun Kim, Rani Jeong, Yanting Qui, Xiangxinyue Meng, Zhijun Wu, Andreas Zuend, Yoonkyeong Ha, Changhyuk Kim, Haeri Kim, Sanjit Gaikwad, Kyoung-Soon Jang, Jiyi Lee, Joonyoung Ahn, and Mijung Song

A phase state of ambient aerosols is a key parameter to understand physicochemical properties of aerosols such as growth rate, size distribution, and mass concentration that affect climate and human health. However, only limited information of real aerosol phase states has been obtained. Herein, to explore phase states of fine particulate matter (PM2.5) in megacities, we collected daily PM2.5 filter samples during December 2020 – January 2021 in Seoul and Beijing. Optical microscopy and a poke-and-flow technique were used to observe the morphologies and phase states of the PM2.5. Results showed that the average phase states of the PM2.5 were significantly different in the two megacities. The PM2.5 existed as a liquid state to a semisolid in Seoul while it existed as a semisolid to a solid in Beijing. These differences were governed by the chemical composition of PM2.5 and aerosol liquid water content. Furthermore, the phase state of PM2.5 in two megacities was correlated with particle size distribution. Our findings can provide an understanding of the phase states of real-world aerosols and how the phase state is linked to chemical compositions, ALWC, and size distributions of PM2.5.

How to cite: Kim, D., Jeong, R., Qui, Y., Meng, X., Wu, Z., Zuend, A., Ha, Y., Kim, C., Kim, H., Gaikwad, S., Jang, K.-S., Lee, J., Ahn, J., and Song, M.: Phase state of PM2.5 in Seoul and Beijing and its effect on particle size distribution, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-253, https://doi.org/10.5194/egusphere-egu23-253, 2023.

EGU23-325 | ECS | Posters on site | AS3.1

Understanding the role of forest fires in urban pollution in São Paulo, Brazil 

Maria Oliveira and Regina Maura Miranda

The air quality in the Metropolitan Area of São Paulo (MASP) is influenced by local sources of pollution, mainly from vehicles and industries, but there is a concern about the role of remote sources in the concentration of particulate matter, such as biomass burning plumes, which occur mainly in the interior regions of Brazil. During the dry period (mainly between July and October), the central region of Brazil suffers from biomass burning, which releases large quantities of gases and particles into the atmosphere and not only affects nearby cities, but also regions hundreds of kilometers away, as is the case of the city of São Paulo.This study aimed to evaluate the concentration of PM10, PM2.5and Aerosol Optical Depth (AOD) between 2005 and 2022, identifying seasonal variations, spatial distribution, frequency, meteorological influences, and the main sources of the aerosol, including understanding and quantifying the impact of burning events on air quality in the MASP.The surface pollutant data, meteorological data, and AOD data were provided, respectively, by: São Paulo Environmental Company (CETESB; https://cetesb.sp.gov.br/ar/qualar/),Institute of Astronomy, Geophysics andAtmospheric Sciences (IAG/USP; http://www.estacao.iag.usp.br/)and Aerosol Robotic Network (AERONET;https://aeronet.gsfc.nasa.gov/).The results indicate a downward trend for aerosol, since several public policies were implemented in the period, but the values are still far above the standards recommended by the World Health Organization (WHO), especially in the winter months (June-September), due to meteorological conditions. Burning events that affect the MASP (more frequent in September) contribute to the increase of particle concentrations at the surface,as well as to the increase of AOD, related to the frequency of northwest wind direction in these eventsandalsoto the number of fire spots in the country.

How to cite: Oliveira, M. and Miranda, R. M.: Understanding the role of forest fires in urban pollution in São Paulo, Brazil, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-325, https://doi.org/10.5194/egusphere-egu23-325, 2023.

EGU23-563 | ECS | Orals | AS3.1

Characteristics of cluster mode particle number concentrations in India 

Mathew Sebastian and Vijay P Kanawade

The dynamics of atmospheric aerosols is governed by the spatio-temporal variability in the particle number size distributions. Atmospheric new particle formation begins with the formation of the cluster mode (sub-3nm) particle number concentrations followed by their growth to large sizes in the atmosphere. Here, we used three years (2019-2022) particle number size distribution measurements in the size range from 1 to 3 nm from nano Condensation Nucleus Counter (nCNC) in Hyderabad, India. The distinct seasonal variation was observed in size-segregated cluster mode particle number concentrations, with the highest concentrations in spring (March-May) and the lowest concentrations in winter (December-February). The seasonal variability is strongly linked to the factors affecting cluster mode formation such as planetary boundary layer evolution, temperature (oxidation extent), pre-existing particles (coagulation sink), etc. The calculated sulfuric acid proxy is strongly correlated with cluster mode particle number concentrations and formation rates, indicating the important role of sulfuric acid in aerosol nucleation. The formation rate and growth rate of cluster mode particles were also the highest during spring than winter. Our analysis further revealed that cluster mode number concentrations were the highest at low particulate matter less than 2.5 µm (PM2.5) while it was the lowest at high PM2.5 levels, indicative of the efficient scavenging of cluster mode particles by large-size pre-existing particles. We have also used PARticle Growth And Nucleation (PARGAN) inversion model to estimate the formation rate and growth rate from particle size distribution measurements in the size range from 10 nm to 560 nm. We found that the estimated formation and growth rates from PARGAN model were compared with the measured formation and growth rates from nCNC, within the uncertainty levels. This underlines the applicability of PARGAN inversion model for estimating cluster mode formation and growth rates where such measurements are not available, particularly in India.

How to cite: Sebastian, M. and Kanawade, V. P.: Characteristics of cluster mode particle number concentrations in India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-563, https://doi.org/10.5194/egusphere-egu23-563, 2023.

EGU23-585 | ECS | Orals | AS3.1

Comparison of real-time NMVOCs measurements using PTR-TOF-MS in two cities of IGB region, India: Sources identification and influence on SOA formation 

Vaishali Jain, Sachchida N. Tripathi, Nidhi Tripathi, Mansi Gupta, Lokesh K. Sahu, Vishnu Murari, Sreenivas Gaddamidi, Ashutosh K. Shukla, and Andre S.H. Prevot

Non-methane volatile organic compounds (NMVOCs) are emitted from various anthropogenic and biogenic sources. They act as precursors for the formation of tropospheric ozone and secondary organic aerosols (SOA) in the presence of sunlight and oxidizing radicals (OH, Cl, NO3). The measurements of NMVOCs are essential to understand the formation of new gas-to-particle aerosols, leading to high air pollution episodes. The Indo-Gangetic Basin (IGB) of India, one of the world’s most polluted areas, has been experiencing high aerosols and NMVOCs loadings throughout the year. Delhi and Lucknow are the two main cities in the IGB region selected for the study. The main aim of this study is to compare the contributions of different source factors to NMVOCs concentrations and their role in SOA formation. A proton-transfer-reaction time-of-flight mass spectrometer (PTR-TOF-MS) was deployed to perform real-time chemical characterisation of NMVOCs during two different campaigns in Delhi (2019) and Lucknow (2020-2021), respectively. The High-resolution Time of Flight Mass Spectrometer (HR-ToF-MS), Aethalometer and other instruments were also deployed at both sites. A receptor modelling approach, positive matrix factorisation (PMF), was used with a robust multilinear engine (ME-2) for source apportionment analysis. The present study is a novel attempt to perform PMF over mass spectra of ~90 and ~170 NMVOCs in Delhi and Lucknow, respectively, for different seasons. Their associations with secondary organic aerosol formation using SOA yields were also analyzed. For Delhi, 8-factor solution was selected and resolved into two traffic-related factors: solid-fuel combustions (SFC), secondary VOCs (SVOCs), biogenic factor and solvent-use factor based on statistical parameters. Similarly, for Lucknow, a 6-factor solution was selected with traffic, 2 SVOC factors, 2 SFC factors and one volatile chemical products-related factor. The traffic factor has the presence of aromatics, non-aromatics and oxygenates, while the biogenic factor is marked by isoprene and its fragment (methyl vinyl ketone). The first, second, and third-order oxygenates show peaks in the SVOCs factor, while phenols, furans, and n-containing compounds are found in the SFC factor. It is observed that vehicular emissions (30%) contributed highest to NMVOCs concentrations in Delhi, while the SFC (28%) was a prominent factor in Lucknow. Interestingly, SFC factors contribute the highest to SOA formation at both cities. It is inferred that the agricultural residue burning episodes in neighbouring states, trash burning and solid fuel burning for cooking within and around the cities contributed to the emissions of NMVOCs and the formation of SOA during winter and post-monsoon periods.

How to cite: Jain, V., Tripathi, S. N., Tripathi, N., Gupta, M., Sahu, L. K., Murari, V., Gaddamidi, S., Shukla, A. K., and Prevot, A. S. H.: Comparison of real-time NMVOCs measurements using PTR-TOF-MS in two cities of IGB region, India: Sources identification and influence on SOA formation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-585, https://doi.org/10.5194/egusphere-egu23-585, 2023.

More than 50% of the population in the Indian subcontinent still depends on solid fuel for cooking purposes, and around 0.5 million yearly deaths are attributed to household air pollution. Despite the poor indoor air quality, especially in the rural spheres of the country, there is a lack of comprehensive field-based understanding of exposure to toxic chemical components such as polycyclic aromatic hydrocarbons (PAHs) associated with particulate matter (PM). This study attempts to quantify and assess the exposure to and inhalation health risk from 16 US EPA priority PAHs in size-segregated PM collected from relatively unexplored rural kitchens of northeastern India. A total of 44 sets of samples (5 from kitchens using liquefied petroleum gas (LPG), 18 using firewood (FW), 18 using a mixture of biomass (MB), and 3 non-cooking blanks) were collected and characterized from 6 locations. The sum of PM10-associated 16 priority PAHs (∑16 PAHs) was observed to be 258, 745, and 2554 ng m-3 for LPG, MB, and FW using kitchens, respectively. Size fraction-wise, the highest concentration of ∑16 PAHs was observed in PM0.25 and the least in PM1-10 across kitchen categories, with PM1 associated ∑16 PAHs comprising 80-92% of the total. ∑16 PAHs in kitchen settings were enriched by factors of 1.7-16.5 in comparison to the non-cooking background. Fuel-wise, stark differences were observed between kitchen categories. Within biomass using kitchens, the type of biomass and combustion (flaming vs smoldering) influenced the PAHs concentration and composition, e.g., ∑16 PAHs were enriched by factors of 3.4 for smoldering combustion of FW compared to flaming combustion of MB. Composition-wise, 2-3 ring PAHs dominated the total PAHs concentration in LPG kitchens (82%), while it constituted 43 and 25% in MB and FW using kitchens, respectively. In contrast, 5-6 ring PAHs showed dominance in FW using kitchens (52%), followed by MB (40%). This suggested a greater release of high molecular weight PAHs during biomass combustion with an increased contribution during the smoldering phase. Estimation of the total BaP equivalent concentration (BaPeq) revealed a similar profile as ∑16 PAHs with the lowest values in LPG using kitchens (29 ng m-3) followed by MB (235 ng m-3), and the highest in FW (856 ng m-3). Incremental lifetime cancer risk (ILCR) estimation via the inhalation pathway showed values above the acceptable risk for LPG (3.2×10-5), and much above tolerance levels for biomass using kitchens (MB: 2.6×10-4; FW: 9.4×10-4). Overall, these findings warrant immediate intervention into the cooking practices prevalent in northeastern India, with an emphasis on biomass-dependent households, in order to alleviate health risks.

How to cite: Sharma, B. and Sarkar, S.: Human exposure to size-segregated particulate polycyclic aromatic hydrocarbons during residential cooking in northeastern India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-616, https://doi.org/10.5194/egusphere-egu23-616, 2023.

EGU23-916 | ECS | Orals | AS3.1

Organic aerosol sources and their water-solubility in Delhi NCR: Insights from offline Aerosol mass spectrometric technique. 

Himadri Bhowmik, Neeraj Rastogi, André Prévôt, and Sachchida Nand Tripathi

A major fraction of organic aerosol (OA) is water-soluble. The water-soluble organic aerosol (WSOA) significantly impacts aerosol hygroscopicity and cloud condensation nuclei (CCN) formation, and adversely affects human health. In this study, characterization of WSOA in PM2.5 was done for the samples collected at two sites (Hauz Khas and Pusa) in Delhi NCR, one of the most polluted cities in the world, during the agricultural crop-residue burning period (October-November, 2019) and winter (December, 2019) using offline aerosol mass spectrometry (AMS) technique and compared with co-located real-time AMS measurements. Offline AMS provides quantitative separation of OA factors that can be primary or secondary. Offline AMS analysis showed that approximately 68% and 64% of OA are water-soluble in Hauz Khas and Pusa, respectively, which was corroborated by the filter-based measurements of water-soluble organic carbon (WSOC) and organic carbon (OC) using a TOC-L analyzer and OCEC analyzer, respectively. Three primary factors, including traffic, biomass burning, and solid fuel combustion, and two secondary factors (or sources) were resolved with Positive Matrix Factorization (PMF) analysis on the WSOA data from offline AMS. The results showed that secondary factors dominated the WSOA (~41%), followed by biomass-burning organic aerosol (BBOA) (30-34%).  In addition, the recoveries of the organic factors from several sources, including traffic, biomass burning, solid fuel combustion, and secondary organic aerosol are discussed. More oxidized organic aerosol (MO-OOA) is highly water soluble (88-92%), representing highly oxidized compounds generated from aqueous-phase reactions. The relatively small contribution of hydrocarbon-like organic aerosol (HOA) to WSOA was most likely due to their low water solubility. Overall, this study improves the understanding of the OA sources and their water solubility over the study region.

How to cite: Bhowmik, H., Rastogi, N., Prévôt, A., and Tripathi, S. N.: Organic aerosol sources and their water-solubility in Delhi NCR: Insights from offline Aerosol mass spectrometric technique., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-916, https://doi.org/10.5194/egusphere-egu23-916, 2023.

EGU23-995 | Posters on site | AS3.1

Viscosity and physical state of sucrose/ammonium sulfate/H2O droplets 

Mijung Song, Rani Jeong, Joseph Lilek, Andreas Zuend, Rongshuang Xu, and Mannin Chan

To explore aerosol chemistry and climate change, information of the physical state of aerosol particles is essential. Herein, we measured viscosities of binary mixtures of sucrose/H2O and ammonium sulfate (AS)/H2O, and ternary mixtures of sucrose/AS/H2O with different organic-to-inorganic dry mass ratios. For sucrose droplets, the viscosity gradually enhanced from ~4 × 10-1 to > ~1 × 108 Pa‧s as the relative humidity (RH) decreased from ~81% to ~24%. This corresponds from liquid to semisolid or solid state. For AS droplets, the viscosity dramatically enhanced at ~ 50% RH upon dehydration; to be < 102 Pa‧s for RH > ~50% (liquid state), and > ~1 × 1012 Pa‧s for RH ≤ ~50% (solid state). In case of the ternary mixtures, remarkable enhancement in viscosity was observed as the inorganic ratio increased at a given RH. All particles studied in this work were observed to exist as a liquid, semi-solid or solid depending on the organic-to-inorganic dry mass ratios and RH. Moreover, the measured viscosities of the binary and ternary mixtures were compared with the calculated viscosities using the Aerosol Inorganic–Organic Mixtures Functional groups Activity Coefficients Viscosity model (AIOMFAC-VISC) predictions with the Zdanovskii–Stokes–Robinson (ZSR)-style organic–inorganic mixing model. It showed excellent model–measurement agreement. The result will be discussed.

How to cite: Song, M., Jeong, R., Lilek, J., Zuend, A., Xu, R., and Chan, M.: Viscosity and physical state of sucrose/ammonium sulfate/H2O droplets, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-995, https://doi.org/10.5194/egusphere-egu23-995, 2023.

EGU23-1108 | ECS | Orals | AS3.1

Southern Ocean Emissions of DMS 

Yusuf Bhatti, Laura Revell, Schuddeboom Alex, McDonald Adrian, Archibald Alex, Willaims Jonny, and Behrens Erik

The biogeochemical behaviour of the Southern Ocean is extremely complex and dynamic. The processes that effect this behaviour in the Southern Ocean are highly dependent on radiative (e.g. sunlight), chemical (e.g. nutrient availability) and biological (e.g. phytoplankton) constraints. We aim to assess how the Southern Ocean DMS emissions change when the underlying biological constraints on the production of DMS are altered across time and space.

Using a nudged configuration of the atmosphere-only Earth System Model, UKESM1-AMIP, we performed two sets of four different 10-year simulations from 2009 – 2018. One set tested four different seawater DMS data sets (Anderson et al. 2001, Hulswar et al. 2022, Lana et al. 2011, ), while the other set tested four different DMS sea-to-air flux parameterisations (Goddijn-Murphy et al. 2016, Liss and Merlivat 1986, Nightingale et al. 2000, Wanninkhof 2014). Our goal is to evaluate the variability in each stage for atmospheric DMS formation using four sea-to-air parameterizations and four oceanic DMS sources.

Using a quadratic sea-to-air flux (Wanninkhof (2014) and Nightingale et al. (2000)) provides high transfer velocities in DMS, creating a positive bias across most areas of the Southern Ocean, except for biologically productive areas, such as the high latitude regions. Although the Southern Ocean atmospheric DMS average corresponds well to observations using quadratic formulas, large areas of the Southern Ocean have lower measured atmospheric DMS than model simulations. Linear relationships between wind and flux are shown to be more realistic. We find that there is a greater range of outcomes from the different sea-to-air flux parameterizations (2.84 TgS Yr-1 to 7.44 TgS Yr-1) than from the different oceanic DMS datasets (3.37 TgS Yr-1 to 7.29 TgS Yr-1). This work highlights the need for Earth System Models to include a sea-to-air parameterization that is more appropriate for DMS, and for oceanic DMS datasets to capture the time-varying nature of biological activity. Such improvements would help provide more accurate and realistic simulations of DMS in the Southern Ocean.

How to cite: Bhatti, Y., Revell, L., Alex, S., Adrian, M., Alex, A., Jonny, W., and Erik, B.: Southern Ocean Emissions of DMS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1108, https://doi.org/10.5194/egusphere-egu23-1108, 2023.

EGU23-1301 | ECS | Orals | AS3.1

Investigation of the aqueous oxidation of terpenoic alcohols by OH as a potential source of secondary organic aerosols 

Priyanka Jain, Bartłomiej Witkowski, Agata Kołodziejczyk, and Tomasz Gierczak

      The oxygenated volatile organic compounds, including terpenoic alcohols (TAs) are emitted into the atmosphere mainly from vegetation; from plant resins, and to communicate with neighbouring plants and insects. Furthermore, biogenic alcohols, including menthol, borneol, fenchol, pinanediol and camphanediol are widely utilized in industries. Consequently, terpenoic alcohols are present in all environmental compartments: air, surface and cloud water, fog, and atmospheric particulate matter. Therefore, water provides an important reaction medium for the environmental processing of  terpenoic alcohols.

     Hydroxyl radical (OH) is the most important daytime atmospheric oxidant, and plays a fundamental role in the advanced oxidation processes in the gas phase as well as in the atmospheric waters. In the atmosphere, TAs partition into the clouds and fog droplets, where they can undergo aqueous oxidation by free radicals, mainly OH, which yields low-volatility products. These low-volatility, highly-oxygenated molecules contribute to secondary organic aerosols (SOA) and tropospheric ozone following their aqueous and multiphase oxidation. Hence, terpenoic alcohols are the potential precursors of aqueous SOAs (aqSOAs). Atmospheric aerosols are important climate forcing agents and also have a negative impact on human health. According to recent estimates, SOAs, including aqSOAs, contribute significantly to the global budget for fine particulate matter (PM).

     The goal of this work is to investigate kinetics and mechanism of the aqueous phase oxidation of menthol, borneol, fenchol, pinanediol and camphanediol by the OH radicals. The rate coefficients measurements for reaction of TAs with OH radicals were carried out in the custom-designed aqueous photoreactor using relative rate method approach. The mechanism of the oxidation reactions under investigation were studied with gas and liquid chromatography coupled with the mass spectrometry. Such an approach provided detailed insights into the molecular structures and distribution of products, including neutral molecules (alcohols, carbonyls) and functionalized carboxylic acids. Yields of formation of the major products were also measured using a commercially available and synthesized standards (terpenoic acids). The detailed reaction mechanism of the OH-initiated reaction for five TA was proposed using the experimental data acquired. Subsequently, a box-model for the aqueous OH oxidation of the five terpenoic alcohols was developed and compared to the experimental data; the reaction channels and branching ratios of the major detected by-products were proposed. Atmospheric implications of the results obtained are discussed in the connection with the possible in-cloud formation following the OH oxidation of menthol, borneol, fenchol, pinanediol and camphanediol. Additionally, the rate coefficients and reaction mechanism information for TA reaction with OH radicals in water could be utilized for wastewater treatment.

How to cite: Jain, P., Witkowski, B., Kołodziejczyk, A., and Gierczak, T.: Investigation of the aqueous oxidation of terpenoic alcohols by OH as a potential source of secondary organic aerosols, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1301, https://doi.org/10.5194/egusphere-egu23-1301, 2023.

EGU23-1608 | Posters on site | AS3.1

Source apportionment of water-soluble and water-insoluble metal content of coarse and fine PM in central Los Angeles 

Constantinos Sioutas, Mohammad Mahdi Badami, Ramin Tohidi, and Vahid Jalali Farahani

In this study, principal component analysis (PCA) was utilized to identify the sources of water-soluble and water-insoluble metal content of coarse and fine PM in the air. The sampling campaign was conducted in winter (December 2021-February 2022) at the University of Southern California Particle Instrumentation Unit (PIU) in central Los Angeles. Ambient PM2.5 and coarse PM samples were collected on Teflon filters and chemically analyzed to quantify their water-soluble and total metal content. The Multiple Linear Regression (MLR) model was employed to investigate the contribution of each found factor by PCA to the total metal. The most abundant elements in the fine size range were Na, S, Fe, Al, and Ca, while in the coarse range, they were Na, Fe, Ca, Al, and Mg. Ca, Na, and Zn exhibited the highest solubility levels in both size ranges, while Ti, Fe, and Al showed the lowest solubility. Most metals had higher solubility in the fine size fraction. The PCA results indicated that the tire and brake wear source factor contributed significantly to the water-soluble fraction of metals in both size ranges, whereas the soil and re-suspended road dust source factor had the most contribution to the water-insoluble fraction of metals. The primary source of fine water-soluble metal was metal-dominated abrasion due to its higher water-soluble content, typically corresponding to a greater impact of anthropogenic than crustal sources. MLR results confirmed that tire and brake wear are major sources of metal in the water-soluble fractions of both size ranges, while soil and re-suspended road dust are major sources in the water-insoluble portion.

How to cite: Sioutas, C., Badami, M. M., Tohidi, R., and Jalali Farahani, V.: Source apportionment of water-soluble and water-insoluble metal content of coarse and fine PM in central Los Angeles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1608, https://doi.org/10.5194/egusphere-egu23-1608, 2023.

EGU23-1782 | Orals | AS3.1

How to derive regional/global averages from sparsely sampled data 

Nick Schutgens and the AEROCOM modellers & AEROSAT retrieval specialists

Aerosol observations always suffer from limited sampling, be they in-situ or remote sensing measurements. This introduces representation errors when using these observations to derive regional estimates, or when using them to evaluate models. In the latter case, one can collocate the model data with the observations to alleviate the problem. The downside is that only part of the model data (the collocated part) can be compared to observations).

We present a technique to homogenize observations (i.e. "remove" their limited sampling). In essence, this is possible because aerosol exhibits spatial and temporal correlations. In practice, we use models to provide this information. Here the technique is applied to satellite data.

First we use synthetic observations to show that remaining representation errors due to this homogenization technique are below 10%. Next, we show that after applying this homogenization technique, estimates of regional AOD (or AAOD) from 14 (or 5) different observational datasets are far better in agreement than without homogenziation. Lastly, we present evidence that remaining differences in homogenzied (A)AOD in these daatsets is dominated by retrieval error.

We also discuss the evaluation of AEROCOM models with these homogenized data. In particular, we highlight existing biases in modelled AAOD.

Although we have not tried it yet, the technique should also be applicable to in-situ data.

How to cite: Schutgens, N. and the AEROCOM modellers & AEROSAT retrieval specialists: How to derive regional/global averages from sparsely sampled data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1782, https://doi.org/10.5194/egusphere-egu23-1782, 2023.

EGU23-1923 | ECS | Orals | AS3.1

Not all types of secondary organic aerosol mix: two phases observed when mixing different secondary organic aerosol types 

Fabian Mahrt, Long Peng, Julia Zaks, Paul E. Ohno, Natalie R. Smith, Florence K. A. Gregson, Yi Ming Qin, Celia L. Faiola, Sergey A. Nizkorodov, Markus Ammann, Scot T. Martin, and Allan K. Bertram

Atmospheric aerosol particles play an important role for air quality and climate. Secondary organic aerosol (SOA) make up a significant mass fraction of these particles. SOA particles mostly forms from oxidation of gases, followed by gas-particle conversion of the oxidation products. Due to the variety of precursors and oxidation pathways involved in SOA formation, atmospheric SOA rank among the least understood aerosol types. To assess the impacts of SOA particles on air pollution and climate, knowledge of the number of phases in internal mixtures of different SOA types is critical. For example, gas-particle partitioning of organic species, and thus ultimately ambient SOA mass concentration, strongly depend on the number of phases in SOA particles. Atmospheric models traditionally assumed that different SOA types form a single condensed organic phase when internally mixed in individual particles. In case of mixed SOA particles with a single condensed phase uptake of semi-volatile vapors are enhanced, due to a lowering of the activities in the organic aerosol phase, and hence a lowering of the equilibrium partial pressure. By contrast, the equilibrium partial pressure is greater if the different SOA types form separate phases due to repulsive intermolecular forces between immiscible organic molecules. Consequently, enhancement of vapor uptake and ambient SOA mass concentrations will be smaller or absent in the case of phase-separated SOA particles.

Here, using fluorescence microscopy, we directly observed the number of phase in individual particles containing mixtures of different SOA types. A total of 6 different SOA types were generated in environmental chambers from oxidation of single precursors. This included both biogenic and anthropogenic SOA types, having elemental oxygen-to-carbon (O/C) ratios between 0.34 and 1.05, covering values characteristic for aged and fresh atmospheric SOA. The number of phases of all possible internal mixtures of two different SOA types, termed SOA+SOA particles, was investigated as a function of humidity between 90% and 0% relative humidity (RH). We found that the number of phases was independent of RH within the range investigated and that 6 out of 15 SOA+SOA mixtures resulted in particles with two condensed organic phases. The observation of phase separated SOA+SOA particles challenges the approach of assuming a single condensed organic phase when representing SOA formation in atmospheric models. Specifically, we demonstrate that the difference in the average O/C ratio between the two SOA types of a mixture (ΔO/C) is a good predictor of the number of phases in particles that are internal mixtures of different SOA types: two-phase SOA+SOA particles formed for ΔO/C ≥ 0.47, while one-phase SOA+SOA particles formed for ΔO/C < 0.47. This threshold ΔO/C provides a simple, yet powerful parameter to predict whether mixtures of fresh and aged SOA particles form one- or two-phase particles in models.

How to cite: Mahrt, F., Peng, L., Zaks, J., Ohno, P. E., Smith, N. R., Gregson, F. K. A., Qin, Y. M., Faiola, C. L., Nizkorodov, S. A., Ammann, M., Martin, S. T., and Bertram, A. K.: Not all types of secondary organic aerosol mix: two phases observed when mixing different secondary organic aerosol types, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1923, https://doi.org/10.5194/egusphere-egu23-1923, 2023.

EGU23-1939 | Orals | AS3.1

Semi-and intermediate- volatility organic compounds from Chinese domestic cooking emissions and their contribution to secondary organic aerosols 

Song Guo, Kai Song, Yuanzheng Gong, Daqi Lv, Yuan Zhang, Zichao Wan, Tianyu li, Wenfei Zhu, Hui Wang, Ying Yu, Rui Tan, Ruizhe Shen, Sihua Lu, Yunfa Chen, and Min Hu

To elucidate the molecular chemical compositions, volatility-polarity distributions, as well as influencing factors of Chinese cooking emissions, a comprehensive cooking emission experiment was conducted. Volatile organic compounds (VOCs), intermediate volatility, and semi-volatile organic compounds (I/SVOCs) from cooking fumes were analyzed by a thermal desorption comprehensive two-dimensional gas chromatography coupled with quadrupole mass spectrometer (TD-GC×GC-qMS). Emissions from four typical Chinese dishes, i.e., fried chicken, Kung Pao chicken, pan-fried tofu, and stir-fried cabbage were investigated to illustrate the impact of cooking style and material. Fumes of chicken fried with corn, peanut, soybean, and sunflower oils were investigated to demonstrate the influence of cooking oil. A total of 201 chemicals were quantified. Kung Pao chicken emitted more pollutants than other dishes due to its rather intense cooking method. Aromatics and oxygenated compounds were extensively detected among meat-related cooking fumes, while a vegetable-related profile was observed in the emissions of stir-fried cabbage. Ozone formation potential (OFP) was dominated by chemicals in the VOC range. 10.2% - 32.0% of the SOA estimation could be explained by S/IVOCs. Pixel-based partial least squares-discriminant analysis (PLS-DA) and multiway principal component analysis (MPCA) were utilized for sample classification and component identification. The results indicated that the oil factor explained more variance of chemical compositions than the cooking style factor. MPCA results emphasize the importance of the unsaturated fatty acid-alkadienal-volatile products mechanism (oil autooxidation) accelerated by the cooking and heating procedure.

How to cite: Guo, S., Song, K., Gong, Y., Lv, D., Zhang, Y., Wan, Z., li, T., Zhu, W., Wang, H., Yu, Y., Tan, R., Shen, R., Lu, S., Chen, Y., and Hu, M.: Semi-and intermediate- volatility organic compounds from Chinese domestic cooking emissions and their contribution to secondary organic aerosols, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1939, https://doi.org/10.5194/egusphere-egu23-1939, 2023.

EGU23-2058 | ECS | Orals | AS3.1

Aerosol hygroscopic growth study from synergy between Mie-Raman-Fluorescence Lidar and Microwave Radiometer 

Robin Miri, Philippe Goloub, Olivier Pujol, Qiaoyun Hu, Igor Veselovskii, Thiery Podvin, and Fabrice Ducos

This study focuses on the characterization of aerosol hygroscopicity using remote sensing techniques. A Mie-Raman-Fluorescence lidar, developed at the Laboratoire d’Optique Atmosphérique in Lille, France, in combination with a Microwave radiometer, allow to monitor continuously both aerosols and water vapor. Hygroscopic growth cases can be identified when an aerosol layer presents an increase in both aerosol backscattering coefficient and relative humidity. Looking at the class of the aerosol among the layer, determined from clustering methods, and the fluorescence backscattering coefficient, which is expected to be unaffected by the presence of water, it is possible to verify that the aerosol layer is homogeneous. Therefore, the change in the backscattering coefficient is then only due to water uptake. The Hänel theory describes the evolution of the backscattering coefficient with relative humidity and introduces a hygroscopic coefficient, γ which depends on the aerosol type and the relative humidity threshold of the dry condition. One case study has been identified on 10 March 2021 for a smoke aerosol layer. For this case, γ was determined at  for . This value is consistent with other values found in the literature for smoke particles. Other cases have been analyzed and this set of example illustrates the potentiality of the methodology presented here.

How to cite: Miri, R., Goloub, P., Pujol, O., Hu, Q., Veselovskii, I., Podvin, T., and Ducos, F.: Aerosol hygroscopic growth study from synergy between Mie-Raman-Fluorescence Lidar and Microwave Radiometer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2058, https://doi.org/10.5194/egusphere-egu23-2058, 2023.

EGU23-2213 | ECS | Orals | AS3.1

Deriving the hygroscopicity of ambient particles using low-cost optical particle counters 

Wei-Chieh Huang, Wei-Chun Hwang, and Hui-Ming Hung

The chemical composition and physical properties of aerosols significantly affect human health, cloud physics, and local climate. Hygroscopicity, a crucial physical property, represents the ability of aerosol to absorb moisture from the surrounding atmosphere and act as cloud condensation nuclei. In this study, we applied two home-built Air Quality Box (AQB) systems co-locating with Taiwan EPA Nanzi station (22°44’12” N, 120°19’42” E) in Kaohsiung, Taiwan, from 4 to 19 February 2021. AQB is composed of low-cost sensors to monitor the ambient gaseous pollutants (CO, CO2, NO, NO2, O3, SO2, and Non-Methane Hydrocarbons), aerosol particles (number size distribution between the diameter of 0.38-17 μm), and the meteorological parameters (T, RH, and P). As to PM (Particulate matter), EPA station monitors PM concentration at the dry state by controlling the measurement at less than 50% while the optical particle counter (OPC) in AQB reflects the ambient PM directly. The difference between the two values represents the amount of absorbed liquid water in the ambient condition. With the consideration of OPC sensitivity and aerosol hygroscopicity, OPC sensitivity and k-Köhler equation are applied to derive the hygroscopicity parameter (k) for PM2.5 (fine particles) and PM2.5-10 (coarse particles with a diameter in the range of 2.5 to 10 µm). In our preliminary results, OPC sensitivity is different between fine and coarse particles at RH<50%, suggesting the requirement of sensitivity adjustment for simple OPC at different particle ranges. The derived k ranges from 0.15 to 0.29, and 0.05 to 0.13 for fine and coarse particles, respectively. The results are consistent with those derived from collected samples analyzed using ion chromatography in our previous Kaohsiung winter campaign. The developed method provides a comprehensive way to determine the hygroscopicity of ambient aerosols, which can be helpful for atmospheric models to compare the results for further efficiency evaluation of aerosol acting as cloud condensation nuclei and radiation calculation. Furthermore, the application of this method for the low-cost sensors applied widely nearby EPA stations is under analysis to evaluate the performance of low-cost OPC sensors and to retrieve the enhanced temporal and spatial aerosol hygroscopicity.

How to cite: Huang, W.-C., Hwang, W.-C., and Hung, H.-M.: Deriving the hygroscopicity of ambient particles using low-cost optical particle counters, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2213, https://doi.org/10.5194/egusphere-egu23-2213, 2023.

Light-absorbing organic aerosols, often referred to as brown carbon (BrC), significantly contribute to atmospheric brown clouds and are a major climate forcing agent over South Asia. In addition to direct emissions in the form of fine mode aerosol, BrC forms secondarily in the atmosphere via homogeneous and heterogeneous chemical reactions involving anthropogenic and biogenic precursor gases, thereby enhancing the complexity of its molecular composition. Detailed molecular characterization and identification of potential BrC chromophores are essential to facilitate a proper understanding of BrC source profiles, atmospheric transformation processes and resultant climate effects. However, owing to its relatively short atmospheric lifetime and large spatial variability, molecular-level characterization of BrC aerosol is challenging. Here we report the first insights into molecular profile of aqueous BrC in the Indian subcontinent, specifically, the eastern Indo-Gangetic Plains (IGP) with a distinct heterogeneity of BrC sources, on a diurnal and seasonal basis. To this end, daytime and nighttime PM2.5 samples collected during 2019-2020 at a rural receptor location in the eastern IGP were extracted for the aqueous BrC fraction and subsequently analyzed using high-performance liquid chromatography coupled with a diode array detector and a time-of-flight mass spectrometer (HPLC-DAD-ToF-ESI-MS).

In total, around 3000 chemical formulas of organic compounds were determined in the positive and negative modes, which were classified into four major groups: CHO, CHON, CHONS and CHOS. In the negative mode, CHO- (36-48%) was the most abundant group, followed by CHON- (23-31%) and S-containing groups (CHONS- (7-19%) and CHOS- (11-32%)) whereas CHON+ (47-58%) showed the highest abundance in the positive mode followed by CHO+ (21-29%) and S-containing groups (CHONS+ (11-18%) and CHOS+ (3-11%)). The reaction between ammonia and carbonyls could lead to the formation of abundant CHON+ compounds with reduced N-containing groups (averaged O/C: 0.2, H/C: 1.7), while CHON- consisted of oxidized N-containing groups (averaged O/C: 0.5, H/C: 1.1). Daytime samples were enriched with CHO- and CHOS- compounds as compared to nighttime samples throughout the seasons, potentially suggesting photochemical formation of these multifunctional compounds. On the contrary, N-containing compounds such as CHON- and CHONS- showed higher abundance during nighttime, suggesting the importance of dark-phase NO3- chemistry. The higher double-bond equivalent (DBE) value of the CHON- group in post-monsoon and winter (7-8) indicated the presence of unsaturated compounds possibly emitted from agricultural residue burning or via secondary formation through NOx reactions. In contrast, the higher DBE value of the CHOS- group during summer (~6) suggested the emission of S-containing compounds from diesel vehicles, coal combustion or secondary formation via photochemical reaction pathways. The enrichment of water-soluble nitroaromatic chromophores (C6H5NO3, C7H7NO4, C9H7NO4, etc.) during post-monsoon and winter was consistent with the dominant presence of a biomass burning source, echoing our previous findings based on multiple independent lines of evidence. Overall, these results provide the first insights into the linkage between BrC chemical and optical properties in the Indian context.

How to cite: Dey, S. and Sarkar, S.: Molecular characteristics of aqueous brown carbon in the eastern Indo-Gangetic Plains: Insights from a high resolution mass spectrometry approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2275, https://doi.org/10.5194/egusphere-egu23-2275, 2023.

EGU23-2334 | Orals | AS3.1

Regional transport and formation of air pollutants between sea and land under the monsoon climate 

Min Hu, Qingfeng Guo, Dongjie Shang, Zhijun Wu, Sihua Lu, and Song Guo

Reactive air pollutants and their secondary products are related to air quality and climate. The growing human activities (fossil fuel combustion, biomass burning, fertilizer use, and industrial activity) result in increasing negative impacts on ocean biota and marine resources. Aerosols in the marine atmosphere are episodically & dramatically influenced by long distance transport from continental regions. Monsoon climate, high population density and strong anthropogenic emissions in East Asia and Southeast Asia cause interaction of air pollutants between sea and land to affect air quality and climate change.

Our study based on two intensive measurements by ground sites, ship cruise, and aircraft in eastern of China in 2011 and southern and southwest of China in 2015.

The ship cruise measurements in the eastern coast of China indicated that the decline of the organic indicators for continental anthropogenic sources and the decline of PM and its major chemical compositions with longitude. The influence of Asian continental outflow during monsoon season was analyzed by identification of BC source regions at a receptor site of eastern coast of China. The variability in the relationship between BC and CO found BC aging during transport.

Two Mt. background sites and aircraft measurements to explore the influence of biomass burning (BB) in the South Asia to air quality in southern and southwest of China. The aloft BB transport was captured by aircraft observations to demonstrate impacts of springtime BB in Southeast Asia on atmospheric carbonaceous components over the Gulf of Beibu in China. Intensive BB activities in the South Asia were detected by fire maps. The long-range transport of BB pollutants can increase the accumulation mode particles in the background atmosphere at Mt. Yulong (3410 m). CCN concentration was 2-8 times higher during BB periods than during clean periods.

How to cite: Hu, M., Guo, Q., Shang, D., Wu, Z., Lu, S., and Guo, S.: Regional transport and formation of air pollutants between sea and land under the monsoon climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2334, https://doi.org/10.5194/egusphere-egu23-2334, 2023.

EGU23-2421 | ECS | Orals | AS3.1

Secondary organic aerosol formation during the oxidation of large aromatic and other cyclic anthropogenic volatile organic compounds 

Damianos Pavlidis, Andrea Simonati, Kalliopi Florou, Christina Ν. Vasilakopoulou, Angeliki Matrali, Christos Kaltsonoudis, and Spyros Ν. Pandis

Volatile (VOCs) and intermediate volatility organic compounds (IVOCs) can undergo atmospheric oxidation, forming secondary organic aerosol (SOA) as their low volatility oxidation products condense in the particulate phase. Recent research has suggested that IVOCs, which have been neglected for decades, may have an important role in atmospheric SOA formation (Tkacik et al., 2012). Most of the work until now, has focused on SOA formation from VOCs with 5 to 10 carbon atoms.

The main goal of this work is to study the SOA production from the reactions of individual anthropogenic large VOCs and IVOCs with hydroxyl radicals (OH), under high NOx conditions often encountered in urban areas. The organic compounds that were studied include cyclic alkanes of increasing size (amylcyclohexane, hexylcyclohexane, nonylcyclohexane and decylcyclohexane) and also aromatic compounds (1,3,5-trimethylbenzene, 1,3,5-triethylbenzene and 1,3,5-tri tri-tert-butylbenzene). The effects of the structure of the compound (alkylic cycle and aromatic ring) and the size of the molecule on the SOA yields is also investigated.

Photo-oxidation experiments were carried out in the atmospheric simulation chamber of the Foundation for Research and Technology-Hellas (FORTH-ASC). The instrumentation used included a scanning mobility particle sizer (SMPS) to measure the particle size distribution, a high-resolution aerosol mass spectrometer (AMS) to quantify the particle mass concentration and composition, and a proton transfer reaction mass spectrometer (PTR-MS) to monitor the organic vapor concentrations. Thermal desorption gas chromatography was also used for offline analysis of the gas-phase products of the reactions. The volatility distribution of the produced SOA was quantified combining thermodenuder and isothermal dilution measurements with the SOA yields.

In each experiment the basic procedure was to fill the chamber, which is a 10 m3 Teflon reactor, with dry, clean air, introduce dry ammonium sulfate particles, inject d9-butanol and the VOC, add the nitrous acid (HONO) and turn on the UV lights to initiate the SOA formation. The injection of the cyclic alkanes demanded heating the injection lines. Because the 1,3,5-tri-tert-butylbenzene is solid at room temperature, it was introduced with a vaporizer. Before each experiment the chamber was cleaned with dry, clean air for a full day.

The total SOA concentration in the chamber was calculated after the data were corrected for particle losses to the chamber walls. The AMS measurements were corrected also for the collection efficiency (CE) that was estimated in each experiment using the algorithm of Kostenidou et al. (2007). From the same algorithm the density of SOA was also estimated.

All the compounds were found to form a considerable amount of SOA. The cyclohexanes were found to have higher yields than the aromatic compounds. Our experiments indicated that aromatic precursors produce a more oxidized SOA than the cyclohexanes. The results of this study can be used in atmospheric chemical transport models for more accurate simulation of anthropogenic SOA formation.

 

REFERENCES

Kostenidou, E., Pandis, S. N., Pathak, R. K., Pandis, S. N., Kostenidou, E., and Pandis, S. N. (2007). Aerosol Science and Technology, 41, 1002–1010.

Tkacik, D. S., Presto, A. A., Donahue, N. M., and Robinson, A. L. (2012). Environmental Science and Technology, 46, 8773–8781.

How to cite: Pavlidis, D., Simonati, A., Florou, K., Vasilakopoulou, C. Ν., Matrali, A., Kaltsonoudis, C., and Pandis, S. Ν.: Secondary organic aerosol formation during the oxidation of large aromatic and other cyclic anthropogenic volatile organic compounds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2421, https://doi.org/10.5194/egusphere-egu23-2421, 2023.

Aerosols have drawn great scientific interests in the past decades dur to their essential roles in the nucleation of ice, clouds, radiation budget and climate change. Light-absorbing carbonaceous particles (LACs), including black carbon (BC) and brown carbon (BrC), are important radiatively-active aerosols in the atmosphere. In this research, we will present the emissions and physicochemical properties of BC and BrC particles. We will try to figure out the contribution of BC and BrC respectively, by combining results from instrument measurement (photoacoustic extinctiometer and aethalometer) and the analysis of aerosol samples collected on filters (UV/vis spectrometry and LC-TOF-MS). In the end, we would like to show the impacts of LACs in cold-climate sites, comparing with warm-climate sites. 

How to cite: Li, H. and Ariya, P.: The Emission and Physicochemical Properties of Light-Absorbing Carbonaceous Particles at A Cold-Climate Site, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2936, https://doi.org/10.5194/egusphere-egu23-2936, 2023.

Humic-like substances (HULIS) are complex macromolecular components of light-absorbing water-soluble organic carbon (brown carbon; BrCaq) consisting of polyacidic and monocyclic/polycyclic structures. HULIS contribute to climate forcing via strong absorption at UV and near-visible wavelengths, and by facilitating the formation of cloud condensation nuclei. Consequently, characterization of the HULIS fractions of BrC is critical to develop a robust understanding of its sources, atmospheric processing and optical effects. To address this issue, we report HULIS fractionation from bulk BrCaq by pH-based multi-step solid phase extraction (hydrophobic fraction at pH=7: neutral HULIS (H-n); hydrophilic fraction at pH=2: acidic HULIS (H-a)) and corresponding optical (UV-Vis and 3D-fluorescence) and chemical properties (1H NMR and FT-IR) on a diurnal and seasonal basis. The study was conducted on PM2.5 samples collected in the eastern part of the Indo-Gangetic Plain (IGP), which is dominantly affected by marine airmasses mixed with fossil fuel emissions during summer, and biomass burning emissions in the IGP outflow during post-monsoon and winter.

Distinct diurnal and seasonal variations were observed for optical and chemical signatures of bulk BrCaq and HULIS fractions. At 365 nm, daytime absorption of BrCaq, H-n and H-a was 3-13 times higher in post-monsoon and 2-8 times higher in winter as compared to summer while that for nighttime samples were enhanced by factors of 2-7 and 3-13, respectively. These possibly point towards greater emission intensity and/or enhanced dark-phase formation of soluble chromophores of BrCaq and H-n during nighttime and an enhanced presence of conjugated aromatics during post-monsoon and winter. On the other hand, enrichment of H-a during daytime might be due to increased polarity of oxidation products via photochemical processing. Excitation-emission matrix fluorescence coupled with the parallel factor analysis (PARAFAC) model identified two types of HULIS (condensation and degradation) and combinations of tryptophan and tyrosine type protein-like substances (PRLIS) in BrCaq across seasons, with higher PRLIS abundance (78%) in summer associated with marine biogenic emissions and higher HULIS abundance in post-monsoon (62%) and winter (67%) linked to regional biomass burning. H-n showed greater humification during nighttime as compared to day (0.74-1.92 vs. 0.67-1.15) while H-a was more humified during daytime (0.62-1.54 vs. 0.57-1.34), suggesting that the degree of unsaturation in H-a was associated with the atmospheric ageing process. Aliphatics (H-C) were the most abundant group among BrCaq, H-n and H-a, accounting for about 35-51% of total organic hydrogen throughout the seasons. An increased contribution of H-Ar was observed in H-a (8-24%), followed by H-n (2-19%) and BrCaq (7-14%) suggesting dominance of conjugated aromatics in the HULIS fractions. In BrCaq, aliphatic groups (O-H, N-H, C-H) were dominant in summer, consistent with transported fossil fuel emissions, while biomass burning-derived aromatic signatures (phenolic O-H, C=O, C=C) were prominent during post-monsoon and winter. In contrast, HULIS fractions showed aliphatic signatures of O-H and –COOH- throughout the seasons. Overall, these findings provide the first insights into the source- and atmospheric processing-dependent chromophoric composition of BrC over the IGP.

How to cite: Sarkar, S. and Dey, S.: Polarity-based chemical characterization of humic-like substances (HULIS) in the Indo-Gangetic Plain (IGP) and linkage with optical signatures of aqueous brown carbon, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3022, https://doi.org/10.5194/egusphere-egu23-3022, 2023.

EGU23-3072 | ECS | Posters on site | AS3.1

Analysis of Mass Extinction Efficiency variation according to relative humidity using lidar and visibility data in Seoul 

sohee Joo, Juhyeon Sim, Jawon Kim, Yuseon Lee, and Youngmin Noh

The mass extinction efficiency(MEE), which indicates the degree of aerosol extinction(scatter and absorption) per unit PM mass concentration, is an important factor in converting optical concentration into mass concentration. Because its value varies depending on the particles' size and composition, which are particles' characteristics. In this study, the extinction coefficients of coarse and fine particles were calculated using the LiDAR data of Seoul observed by NIES(Japan's National Institute of Environmental Studies) and the visibility data of Seoul observed by the Korea Meteorological Administration. In the case of lidar data, two wavelengths (532nm, 1064nm) measured by lidar were used to calculate extinction coefficients, and the wavelength of 532 nm (532P and 532S) were used to classify extinction coefficients into coarse particles(PM10-2.5) and fine particles(PM2.5). In the case of visibility data, the PM10 and PM2.5 extinction coefficients were calculated using the equation of Koschmieder (1924) and Cheng et al. (2017). The PM10, PM10-2.5, and PM2.5 respective MEE were calculated using Seoul data of PM10 and PM2.5 at the same time provided by the Korea Environment Corporation. The relative humidity data provided by the Korea Meteorological Administration were divided into seven sections less than 40%, 40~49%, 50~59%, 60~69%, 70~79%, 80~89%, and 90~100%. According to relative humidity, this study examined the change of the calculated MEE. This study analyzes the effect of relative humidity on the Hygroscopic Growth of PM10, PM10-2.5, and PM2.5.

 

How to cite: Joo, S., Sim, J., Kim, J., Lee, Y., and Noh, Y.: Analysis of Mass Extinction Efficiency variation according to relative humidity using lidar and visibility data in Seoul, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3072, https://doi.org/10.5194/egusphere-egu23-3072, 2023.

The synoptic meteorological field plays an important role in the daily-scale PM2.5 variability in East Asia. Since East Asia is located on the eastern boundary of the Eurasian continent, the expansion and contraction of the Siberian high-pressure system act as an essential mechanism for determining surface PM2.5 concentrations in the winter season. Here, we select four climate indices representing the variability of the Siberian high-pressure system and analyze the correlation with the daily variability of the observed winter PM2.5 concentrations in China and South Korea over the past six years. Siberian High Intensity and East Asian Winter Monsoon indices showed a more pronounced correlation with the daily surface PM2.5 concentration changes, and the daily surface PM2.5 concentrations in North China Plain showed a maximum change of ±40 μg m-3 after exceeding the threshold (+1 or −1). The climate indices associated with the Siberian high-pressure system can effectively predict daily PM2.5 concentrations in East Asia within a week.

How to cite: Jeong, J. and Park, R.: Prediction of PM2.5 concentrations during winter in East Asia using climate indices, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3150, https://doi.org/10.5194/egusphere-egu23-3150, 2023.

EGU23-3886 | Posters virtual | AS3.1

Sand flux in a desert site of Mongolia 

Erdenebayar Munkhtsetseg, Masato Shinoda, John Gillies, and Yaping Shao

Mongolia experiences frequent dust and sand storms, particularly in the spring. As a result, this country losses a huge amount of top soils, which triggers land degradation and desertification. We measured sand flux of 2 consecutive dust storm cases occured in 2011 using BSNE (Big Spring Number Eight) sand traps installed at the Bulgan meteorological station in the Gobi area .

Vertical gradients for the sand mass (flux) demonstrated 3 typical patterns:

  • a) sand flux increases with height when there is a transported sand from the areas distanced away from the study site
  • b) sand flux is constant vertically in the days following dust sand storm (DSS)
  • c) sand flux declines exponentially with the height when DSS occur at the site.

Among these three typical patterns, we investigated the c) pattern to quantify the amount of eroded soil during the on-site dust emissions of dust storm event (DSS) at the site. The DSS was largely associated with the increased friction velocity excluding some cases those are related to a short time-span of rainfall even though underlain by dry soil surface etc. Furthermore, we estimated a saltation height, Zq, which was much greater (30 cm) than the other reported findings (3-10 cm).

Keywords: sand flux patterns, saltation height, sand traps, Mongolia

How to cite: Munkhtsetseg, E., Shinoda, M., Gillies, J., and Shao, Y.: Sand flux in a desert site of Mongolia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3886, https://doi.org/10.5194/egusphere-egu23-3886, 2023.

EGU23-3943 | ECS | Orals | AS3.1

Significant spatial gradients in new particle formation frequency in Greece during summer 

Andreas Aktypis, Christos Kaltsonoudis, Angeliki Matrali, Christina N. Vasilakopoulou, Nikolaos Mihalopoulos, Panayiotis Kalkavouras, Aikaterini Bougiatioti, Nikos Kalivitis, Konstantinos Eleftheriadis, Stergios Vratolis, Maria I. Gini, Athanasios Kouras, Mihalis Lazaridis, Sofia Eirini Chatoutsidou, Athanasios Nenes, and Spyros N. Pandis

Homogeneous nucleation is an important source of new particles in the atmosphere worldwide. The resulting newly formed stable nuclei can grow to larger sizes and affect air quality and climate. Unexpected significant spatial variability of the nucleation frequency has been observed in Greece in the only previous relative study: very high frequency in Thessaloniki, intermediate in Eastern Crete and low in Patras (Patoulias et al., 2018). Our hypothesis is that Greece may be an excellent natural laboratory to investigate the factors affecting nucleation and to understand the reasons behind this surprising variability.

Extensive continuous aerosol size distribution measurements took place during two summers (2020 and 2021) as part of the PANACEA project in 11 different locations: Patras, Xanthi, Ioannina, Finokalia, Athens, Thessaloniki, Sifnos, Chania, Costa Navarino (NEO), Lesvos and Mt. Helmos. The instrumentation used included a number of scanning mobility particle sizers (SMPS) for the measurement of the particles and a suite of gas monitors for measuring SO2, NOx, NH3 and CO in selected sites. A particle size magnifier (PSM) was deployed in the Patras site during the 2021 campaign, providing valuable information regarding nanoparticles with diameter down to 1 nm.

The observations suggest that indeed the nucleation frequency during summer in Greece varies from close to zero in the southwestern parts of the country to more than 70% in the northern central and eastern regions. The analysis of the measurements in the various sites shows that the proximity to coal-fired power plants is a major factor affecting the nucleation frequency. North-eastern and northern airmasses passing over such locations in the Balkans and Western Turkey where strongly associated with nucleation. Also, the emissions of ammonia during summer, suggest that it exhibits similar spatial gradients with the observed nucleation frequency and may be controlling nucleation in Greece. The corresponding measurements in each site, were also used to estimate the corresponding particle growth and formation rates and the condensation and coagulation sinks.

The detailed analysis of the measurements in Patras, Western Greece, suggests that nucleation was infrequent in this location (12%), but particles that were formed a few hours earlier over central Greece are often transported to this area after they have grown to sizes of 20-30 nm. The air mass history suggested that new particle formation often took place in the vicinity of an area 100-150 km northeast of Patras, with significant agricultural activity and therefore, high emissions of ammonia and amines. The relatively high emissions of biogenic volatile organic compounds in Western Greece where Patras is located, did not appear to assist in the local formation of new particles.

How to cite: Aktypis, A., Kaltsonoudis, C., Matrali, A., Vasilakopoulou, C. N., Mihalopoulos, N., Kalkavouras, P., Bougiatioti, A., Kalivitis, N., Eleftheriadis, K., Vratolis, S., Gini, M. I., Kouras, A., Lazaridis, M., Chatoutsidou, S. E., Nenes, A., and Pandis, S. N.: Significant spatial gradients in new particle formation frequency in Greece during summer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3943, https://doi.org/10.5194/egusphere-egu23-3943, 2023.

Atmospheric aerosols are of great concern due to their impacts on human health, visibility, and climate. Sub-3 nanometer particles are initially formed through gas-to-particle conversion with a typical size of 1-3 nm, which is crucial for understanding the steps of new particle formation and sources of aerosol particles in the atmosphere. In this study, sub-3 nm particle concentration was measured from 2018 to 2020 at SORPES station in the Yangtze River Delta, China by particle size magnifier (PSM). Based on three years’ measurement, a high number concentration of sub-3 nm particles was observed all year round. Sub-3 nm particle concentration in polluted urban environments is two orders of magnitude higher than that in clean environments, e.g., Hyytiälä. Moreover, formation rates and growth rates of sub-3 nm particles were calculated in these 3 years. The formation rate in anthropogenic pollution regions is much higher than that in the clean environment, while the growth rate is similar to other field observations. Besides the secondary formation of sub-3 nm particles via new particle formation, we found traffic primary emission is a neglectable source of sub-3 nm particles in the urban area. We estimated the contribution of traffic emission and new particle formation on sub-3 nm particle concentration using sulfuric acid and NOx concentration as tracers. During the daytime, the contribution of traffic emissions can be over 50% on non-NPF-event days, and the contribution even comes to 13% on NPF-event days. During the nighttime, the contribution of traffic emissions can be up to 70%. Furthermore, in some conditions, synergistic effects of traffic emission and new particle formation can happen in the daytime, which causes an extremely high concentration of sub-3 nm particles. Our study also suggests that regional and global air quality models should consider traffic emissions as a primary source of sub-3 nm particles in anthropogenic pollution areas.

How to cite: Chen, L.: High Number Concentration of Atmospheric Sub-3 nm Particles in Polluted Environment of East China: three-year Observation at SORPES Station, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3958, https://doi.org/10.5194/egusphere-egu23-3958, 2023.

EGU23-4572 | Posters virtual | AS3.1

Estimation on the refractive index of ambient aerosols as fine- and coarse-mode volume size distribution 

Juseon Shin, Juhyeon Sim, Dukhyeon Kim, and Youngmin Noh

The refractive index (RI) of aerosol is an important parameter that reflects the scattering and absorption capacity of aerosol and is widely used in atmospheric models and remote sensing studies. It depends on several properties such as chemical species, moisture content, etc. RI is usually obtained by the chemical method using a volume mixing ratio of known chemicals and by the optical method based on extinction, scattering and/or absorption coefficient using Mie theory. However, these methods are complicated and are mainly for singular particles. In this study, we tried to make a simple method to estimate RI by measuring the extinction coefficient from camera images and size distribution from the optical particle counter (OPC). We used the wavelength of Red-Green-Blue color as 597, 534, and 459 nm to calculate the extinction coefficient and the number size distribution to retrieve the volume size distribution obtained by OPC. The volume size distribution is expressed by six parameters of two gaussian graphs for fine and coarse-mode particles. We got the volume, median radius, and standard deviation of fine and coarse aerosol peaks. The measurement site was the port area in Busan, Korea. We sometimes discovered the emission of particles but mainly measured for clear days. We effectively retrieved six parameters determining the volume size distribution of ambient aerosols and tried to inverse RI as total, fine, and coarse particles using the nonlinear optimization method. We mainly considered the scattering effects of ambient aerosols, so we focused on the real part of RI. The retrieved RI was from 1.27 to 1.50 and showed different values on fine- and coarse-mode size particles. The results were lower than other RI measurement studies, so we need to validate more. However, we identified the possibility of retrieving the RI of aerosols using the known size distribution retrieved from OPC and the three-color extinctions from the camera.

How to cite: Shin, J., Sim, J., Kim, D., and Noh, Y.: Estimation on the refractive index of ambient aerosols as fine- and coarse-mode volume size distribution, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4572, https://doi.org/10.5194/egusphere-egu23-4572, 2023.

EGU23-4702 | ECS | Posters on site | AS3.1

Relationship of aerosol optical properties and particle types from SPARTAN and AERONET data in South Korea 

Sujin Eom, Jhoon Kim, Seoyoung Lee, Yeseul Cho, and Sang Seo Park

SPARTAN (Surface Particulate Matter Network) is a network of Particulate Matter (PM) samplers that analyze aerosol samples for PM mass concentration and chemical composition. Two aerosol samplers were installed at two sites in Korea: Yonsei University at Seoul and UNIST (Ulsan Institute of Science and Technology) at Ulsan. These SPARTAN filter samplers and additional nephelometers provide the PM2.5 mass concentration and reconstructed chemical speciation data (May, 2019~ Nov, 2021). In most SPARTAN PM2.5 cases, both sites showed time series patterns similar to data from the Korean regional observation network (Airkorea). In the case of high-loading fine dust, the daily value was relatively well matched with Airkorea data. The co-location of these SPARTAN samplers with AERONET (Aerosol Robotic Network) sun photometer presents the possibility of analyzing aerosol optical depth, aerosol surface mass concentration, and aerosol speciation data together. If the fraction of a particular component is high, the optical properties may vary. When the mass concentration of sulfate was relatively high, AERONET data displayed a large distribution of non-absorbing small particles. Similar to the previous analysis, we also show a detailed analysis of the relationship between other chemical components and optical properties.

How to cite: Eom, S., Kim, J., Lee, S., Cho, Y., and Park, S. S.: Relationship of aerosol optical properties and particle types from SPARTAN and AERONET data in South Korea, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4702, https://doi.org/10.5194/egusphere-egu23-4702, 2023.

EGU23-4891 | Posters on site | AS3.1

Oxidative potential and chemical characterization of PM2.5 in a medium-sized residential city of South Korea. 

Sung-Won Park, Youngj-Ji Han, Ji-Won Jeon, Jin-Hyuk Hong, Hyo-Won Lee, Se-in Hong, Ji-Hyeon Koo, and Young-Kyu Kim

PM2.5, defined as particulate matter less than 2.5 μm, is derived from a variety of natural and anthropogenic sources. Studies have shown that PM2.5 adversely affects human health, causing various respiratory and cardiovascular diseases. One of the methods to assess the potential health impacts of PM2.5 is to measure its oxidative potential, which refers to the ability of the particles to generate reactive oxygen species when inhaled into the lungs. In this study, antioxidants including ascorbic acid (AA) and reduced glutathione (GSH) as well as dithiothreitol (DTT) were used to measure the oxidative potential of PM2.5 collected in Chuncheon, a medium-sized residential city of South Korea. The degree of oxidation of antioxidants and DTT were measured using a spectrophotometric assay. In addition, a detailed PM2.5 compositions including NO3-, SO42-, NH4+, organic carbon (OC), elemental carbon (EC), metallic elements, and individual organic substances were measured to identify the characteristics of high PM2.5 concentration episodes (HCE) and to determine the association between chemical components with oxidative potential.

PM2.5 concentrations were generally higher in fall than in summer, and OC was the biggest contributor to PM2.5 mass. Among organic matters, sugar compounds, the marker species of biomass burning, were prominent while dicarboxylic acids, predominantly secondarily formed in atmosphere, were important in summer. For HCEs, NO3- and dicarboxylic acids increased the most among PM2.5 components, suggesting that secondary formation was important to enhance PM2.5 concentration. Nitrogen oxidation ratio (NOR) also increased during HCEs, and there was statistically significant correlation between NO2 and NO3-, possibly indicating that in situ oxidation of NO2 and/or gas-aerosol partitioning for HNO3 and NO3- occurred. Average OP measured by depletion of AA (OPAA), GSH (OPGSH), and DTT (OPDTT) were 4.5 ± 1.1, 4.9 ± 1.3, and 17.7 ± 5.9 pmol min-1 mg-1, respectively, during summer. All three OPs were especially low for the sample obtained when Asian dust event occurred. PM2.5 mass concentration was successfully reconstructed by EC, ∑n-Alkane, Ca2+, SO42–, and OC from multiple linear regression while oxidative burden by GSH (OBGSH) was explained by EC and ∑PAHs. These different results between PM2.5 mass and OP suggest that the PM2.5 concentration alone is not sufficient to explain the association with health effects.

How to cite: Park, S.-W., Han, Y.-J., Jeon, J.-W., Hong, J.-H., Lee, H.-W., Hong, S., Koo, J.-H., and Kim, Y.-K.: Oxidative potential and chemical characterization of PM2.5 in a medium-sized residential city of South Korea., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4891, https://doi.org/10.5194/egusphere-egu23-4891, 2023.

EGU23-5085 | ECS | Posters on site | AS3.1

Origin and transformation of organic aerosol at three background sites in Central Europe 

Radek Lhotka, Petra Pokorná, Petr Vodička, Naděžda Zíková, Jakub Ondráček, Saliou Mbengue, Shubhi Arora, Laurent Poulain, Hartmut Herrmann, Jaroslav Schwarz, and Vladimír Ždímal

The source apportionment of organic aerosols (OA) in background locations is one of the important issues in contemporary air quality protection. A better understanding of the atmospheric aerosols origin and their source apportionment in different locations is essential for improving air quality.

Measurements of non-refractory PM1 (NR-PM1) were simultaneously performed during winter (1st February – 10th March) and summer (1st July – 20th August)  2021 at three background sites, National Atmospheric Observatory Košetice (N 49°35′, E 15°05′; 534 m a.s.l.) and Frýdlant (N 50°94′, E 15°07′; 366 m a.s.l.) in Czech Republic, and Melpitz (N 51°32', E 12°56'; 86 m a.s.l.) in Germany. Each site was equipped with an Aerosol Mass Spectrometer: a ToF- Aerosol Chemical Speciation Monitor (ToF-ACSM) at Košetice, a Compact Time-of-Flight Aerosol Mass Spectrometer C-ToF-AMS) at Frýdlant, and a High-Resolution Time-of-Flight Aerosol Mass Spectrometer (HR-ToF-AMS) at Melpitz.

A Positive Matrix Factorization (PMF) with multi-linear engine (ME-2) using Source Finder (SoFi) (Canonaco et al., 2013) was applied to OA data sets to separate OA into different factors in terms of their mass spectra and time series. Four sources of OA were identified for the winter season. Three of these sources, hydrocarbon-like organic aerosol (HOA), biomass burning organic aerosol (BBOA), and coal combustion organic aerosol (CCOA), belong to the primary sources. The last factor, designated oxidised organic aerosol (OOA), belongs to the secondary sources. Four sources of OA have also been identified for the summer season. Two of these sources were designated as primary sources (HOA and BBOA) and two as secondary sources, more oxidized organic aerosol (MO-OOA) and less oxidized organic aerosol (LO-OOA).

 

Acknowledgements:

This work was supported within a German-Czech cooperation in the TRACE project funded by the GACR under grant 20-08304J and by DFG under grant 431895563, also by the MEYS of the Czech Republic under grants ACTRIS-CZ LM2018122 and ACTRIS-CZ RI (CZ.02.1 .01 / 0.0 / 0.0 / 16_013 / 0001315), and European Union's Horizon 2020 research and innovation program ACTRIS IMP (871115).

 

Reference:

Canonaco, F., Crippa, M., Slowik, J. G., Baltensperger, U., Prévôt, A. S.: SoFi, an IGOR-based interface for the efficient use of the generalized multilinear engine (ME-2) for the source apportionment: ME-2 application to aerosol mass spectrometer data, Atmos. Measur. Tech., 6(12), 3649-3661, 2013.

How to cite: Lhotka, R., Pokorná, P., Vodička, P., Zíková, N., Ondráček, J., Mbengue, S., Arora, S., Poulain, L., Herrmann, H., Schwarz, J., and Ždímal, V.: Origin and transformation of organic aerosol at three background sites in Central Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5085, https://doi.org/10.5194/egusphere-egu23-5085, 2023.

EGU23-5289 | ECS | Posters on site | AS3.1

New insights into submicron particles impact on visibility 

Ewa Anioł, Grzegorz Majewski, Wioletta Rogula-Kozłowska, Bartosz Szeląg, Patrycja Rogula-Kopiec, Andrzej Brandyk, Agata Walczak, and Maja Radziemska

The aim of the study was to analyze the impact of very fine atmospheric particles (submicron particulate matter; PM1) on visibility deterioration. Taking into consideration not only their entirely different physio-chemical properties in comparison to a well-recognized PM10 but also the origin and a growing environmental awareness of PM1, the main research problem has been solved in few steps. At first, the chemical composition of PM1 was determined in two selected urban areas in Poland. Measurements of meteorological parameters, i.e., air temperature and humidity, precipitation, atmospheric pressure, wind speed, and visibility, were also conducted. The next step of the work was the analysis of (1) seasonal changes of the concentration of PM1 and its main components, (2) the influence of chemical components of PM1 on light extinction, and (3) the influence of PM1 and humidity on visibility. Hierarchical cluster analysis, correlation matrixes and a heat map, and classification and regression tree analysis were used. The light extinction coefficient is influenced mainly by coarse mass of PM, and PM1-bound ammonium nitrate, organic matter, and by Rayleigh scattering. The less important in the light extinction coefficient shaping has PM1-bound ammonium sulfate, elemental carbon, and soil. In this way, the secondary origin PM1 components were proved to most significantly influence the visibility. The obtained results confirmed the possibility of the use of statistical agglomeration techniques to identify ranges of variation of visibility, including independent variables adopted to analyses (meteorological conditions, chemical composition of PM1, etc.).

How to cite: Anioł, E., Majewski, G., Rogula-Kozłowska, W., Szeląg, B., Rogula-Kopiec, P., Brandyk, A., Walczak, A., and Radziemska, M.: New insights into submicron particles impact on visibility, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5289, https://doi.org/10.5194/egusphere-egu23-5289, 2023.

The physical and chemical characteristics of atmospheric aerosol particles are complex in urban areas. It is of great significance to clarify the influence of different emission sources on atmospheric chemical components for tracing and fine control of air pollution. In this study, passive aerosol samplers were used to collect samples in urban area and steel industrial area in Rizhao, a typical coastal city in eastern China, the collected samples were analyzed by intelligent scanning electron microscope environmental particle analysis system (IntelliSEM-EPAS), which is based on computer-controlled scanning electron microscopy technology. The results show that the atmospheric particulates in Rizhao city are mainly composed of irregular carbonaceous particles, sulfur-containing particles and mineral particles, the number contribution of C-rich particles in urban samples is 53.5%, which is 2.5 times higher than that in steel industrial area samples, the number contribution of particles greater than 1 μm was 9.0%, which is 1.7 times that of the samples in steel industrial area, urban dwellers' activities and industrial processes are the main sources of atmospheric particulate matter in urban area. In steel industrial area, the number contribution of sulfur-containing particles is 72.9%, the mass contribution of sulfur-containing particles is 30.9%, and the mass contribution of iron rich particles is 5.3%, which are 1.8 times, 3.6 times and 2.9 times higher than that of urban samples, respectively. These results indicated that primary pollutants emitted by iron and steel enterprises and secondary formation are the main sources of atmospheric particles in steel industrial area, which has a significant impact on the composition of regional atmospheric particulates.

How to cite: Yao, W. and Pan, X.: Study on physical and chemical characteristics and source of atmospheric Single particulate matter in Rizhao city based on EPAS technology, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5435, https://doi.org/10.5194/egusphere-egu23-5435, 2023.

EGU23-5521 | Orals | AS3.1

A Machine Learning approach to aerosol thermodynamics embedded in aglobal chemistry-climate model 

Holger Tost, Sarah Bruening, Stefan Niebler, and Peter Spichtinger

The chemical composition of the aerosol phase is still a major uncertainty in global chemistry climate models. One the one hand, aerosol thermodynamics  calculations are needed to determine the chemical composition of the inorganic fraction of the aerosol particles, on the other hand these calculations are computationally expensive. However, to properly describe the combined gas and aerosol phase composition, e.g., the reactive nitrogen budget including HNO3 or chlorine displacement from sea-salt aerosol, it is mandatory to have a reasonable description of the aerosol thermodynamics. To overcome the computational costs, but to still obtain a reasonable degree of proper process description, a machine learning  approach for the aerosol thermodynamics might offer opportunities in CCM modelling.
In this study, we embed a machine learning approach for the description of aerosol thermodynamics in the chemistry climate model EMAC to reduce computational load (compared to explicit thermodynamics calculations) and show the capabilities of a modern computing approach, implemented in a multi-modal aerosol scheme.
The new aerosol thermodynamics scheme is formulated as a machine learning neural network, which has been trained with the help of an explicit inorganic aerosol thermodynamics box model, i.e. ISORROPIA-2.

This study presents first results of global 3D simulations using the ML approach and compares the results to explicit calculations in terms of the spatio-temporal distribution of the aerosol chemical composition as well as the effective performance of the modelling system.

How to cite: Tost, H., Bruening, S., Niebler, S., and Spichtinger, P.: A Machine Learning approach to aerosol thermodynamics embedded in aglobal chemistry-climate model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5521, https://doi.org/10.5194/egusphere-egu23-5521, 2023.

EGU23-6145 | Orals | AS3.1

Source apportionment of fine aerosol at a rural background site in Central Europe based on seasonal distributions of dicarboxylic acids, sugars and related compounds 

Petr Vodička, Kimitaka Kawamura, Dhananjay K. Deshmukh, Petra Pokorná, Jaroslav Schwarz, and Vladimír Ždímal

Water-soluble dicarboxylic acids (hereafter diacids) and sugars are an important part of the atmospheric water-soluble organic aerosol. Here, we studied diacids and other compounds in fine aerosol particles (PM1) collected at a rural background site National Atmospheric Observatory Košetice (NAOK), Czech Republic, Central Europe. Aerosol samples were collected every second day for 24 h from September 2013 to August 2014 (n=146). Based on receptor modeling (PMF), we identified PM1 organic compounds that are more typical to anthropogenic and to biogenic sources. We have apportioned two anthropogenic sources especially evident during the heating season from mid-October to mid-April: (i) biomass burning (BB) (main contribution of levoglucosan and methylsuccinic, maleic, methylmaleic and azelaic acids) and (ii) fossil fuel combustion (FF) (represented by phthalic, terephthalic and ketomalonic acids). Furthermore, we identified two sources of biogenic aerosols: (iii) summer factor was largely characterized by compounds with three and seven carbons (malonic, 4-ketopimelic, oxoheptanoic, methylmalonic acids) while (iv) spring biogenic factor was characterized mostly by primary sugars, normal chain diacids and their precursors (oxalic, malonic, succinic, glutaric, ketomalonic, 4-oxobutanoic and 5-oxopentanoic acids). Last but not least, we distinguished (v) background factor mainly represented by less oxidized diacids precursors such as glyoxal, methylglyoxal, glyoxylic and pyruvic acids, but also by aromatic diacids, which may originate from traffic emissions; a stable and year-round source.

Acknowledgement: This conference contribution was supported by the Ministry of Education, Youth and Sports of the Czech Republic under the project ACTRIS-CZ-LM2018122, by the Czech Science Foundation grant No. 20–08304J and by the Japan Society for the Promotion of Science (JSPS) through Grant-in-Aid No. 24221001. We appreciate the financial support of JSPS fellowship to P. Vodička (P16760) in Japan.

Reference: Vodička, P., Kawamura, K., Deshmukh, D.K., Pokorná, P., Schwarz, J., Ždímal, V.: Anthropogenic and biogenic tracers of fine aerosol based on seasonal distributions of dicarboxylic acids, sugars and related compounds at a rural background site in Central Europe, Atmos. Environ., submitted, 2023.

How to cite: Vodička, P., Kawamura, K., Deshmukh, D. K., Pokorná, P., Schwarz, J., and Ždímal, V.: Source apportionment of fine aerosol at a rural background site in Central Europe based on seasonal distributions of dicarboxylic acids, sugars and related compounds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6145, https://doi.org/10.5194/egusphere-egu23-6145, 2023.

EGU23-6340 | ECS | Posters on site | AS3.1

Vertical distribution of black carbon and its mixing state in urban boundary layer in summer 

Hang Liu, Xiaole Pan, Yele Sun, and Zifa Wang

The vertical distribution of black carbon (BC) as well as its mixing state is of great concern due to BC’s strong regional climatic and environmental effects. In this study, vertical measurements were conducted through a moveable container based on a meteorology tower in an urban area. A total of 112 vertical profiles (0-240 m), including the concentrations of BC, O3, NOx and the optical properties of aerosols, were obtained. Based on BC concentration, the vertical profiles could be classified into four categories: uniform, gradual decrease, sharp decrease, and sudden increase. The uniform type indicates strong vertical mixing with similar pollutant concentrations along the vertical direction. The gradual/sharp decrease types indicate stable vertical conditions with higher pollutant concentrations on the ground and lower concentrations at higher altitudes. Due to the strong radiation in summer, the vertical profiles exhibited a clear diurnal variation in which ~80% of profiles were uniform during the daytime and ~40%-90% of profiles were gradual/sharp decrease types at night. O3 is an exception, and its concentration generally increases with height even under strong vertical mixing conditions. The size distribution of BC core varied slightly along the vertical direction, and the coating thickness of BC increased with height under stable conditions. However, the vertical variation in BC concentration is much more significant than BC coating thickness and plays a more critical role in the determination of BC absorption ability vertical distribution. In addition, O3 and Dp/Dc occasionally increased during 6:00-8:00 but remained stable during 8:00-10:00. Vertical mixing and transportation from upper heights, such as the residual layer, could significantly influence the pollutant properties on the surface during early mornings. This study exhibits a continuous vertical picture of BC and its mixing state in urban areas, which would be helpful for understanding BC’s regional environmental effect.

How to cite: Liu, H., Pan, X., Sun, Y., and Wang, Z.: Vertical distribution of black carbon and its mixing state in urban boundary layer in summer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6340, https://doi.org/10.5194/egusphere-egu23-6340, 2023.

EGU23-6415 | ECS | Posters on site | AS3.1

Deep learning based classification of biological aerosols 

Hao Zhang, David Topping, Ian Crawford, Martin Gallagher, Man Nin Chan, Hing Bun Martin Lee, Sinan Xing, Tsin Hung Ng, and Amos Tai

Biological aerosols mainly include viruses, bacteria, fungal and pollen, which can significantly affect the human health and environments. Accurate classification of biological aerosols contributes to further understand the implications of these aerosols in different domains. In this work, we collected the real-time fluorescence intensity, size and scattering images data of bioaerosols over a six-month period in Hong Kong by using Rapid-E particle identifier. To clustering the different types of bioaerosols, two deep leaning methods: autoencoder neural network (AE) and bidirectional long short-term memory neural network (Bilstms) were designed to extract the main features of bioaerosol fluorescence intensity and scattering images. The results showed that both AE and Bilstms could reconstruct the input bioaerosol data quite well, which illustrated that the main features they exacted were accurate. Then two clustering methods: K-means, and genie clustering were used to assign the extracted main features of bioaerosol into different clusters respectively. According to the aerosol number distribution in different clusters, the K-means clustering always presented a more uniform aerosol number distribution than genie clustering, especially for bioaerosol features extracted by Bilstms, genie believed that no matter how the number of clusters and the type of bioaerosol data changed, most aerosols were only distributed in one or two clusters. In order to assess the accuracy of clustering and obtain the species of bioaerosol in different clusters, different clusters were identified by analyzing their diurnal variation, average scattering images pattern and the relationship to the meteorological variables temperature, relative humidity, wind speed and wind direction. Based on the identification results, the accuracy of different combinations of two deep learning methods and two clustering methods in bioaerosol classification was evaluated. We believed that this work could provide the potential aid in aerosol classification methods development to achieve the easy and accurate bioaerosol identification.

How to cite: Zhang, H., Topping, D., Crawford, I., Gallagher, M., Chan, M. N., Lee, H. B. M., Xing, S., Ng, T. H., and Tai, A.: Deep learning based classification of biological aerosols, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6415, https://doi.org/10.5194/egusphere-egu23-6415, 2023.

Redox reactions transition metal ions (TMI), such as iron and copper, affect the concentrations of reactive oxygen species (ROS) in atmospheric cloud droplets and aqueous aerosol particles. Copper and iron have distinct emission sources resulting in only a small number fraction of cloud condensation nuclei and droplets that contain these metals. The fact that TMI reactions only occur in a small subset of particles and droplets is not taken into account in current multiphase chemistry models that are usually initialized with TMI concentrations derived from bulk sampling.

Our previous model studies have shown that model predictions based on bulk iron concentrations may significantly underestimate total OH and HO2 budgets if iron is assumed in all cloud (Ervens, 2022; Khaled et al., 2022). We extend this approach to copper reactions and to reactions between copper and iron ions. We use a multiphase chemistry box model to investigate the importance of the number fraction of TMI-containing particles and droplets and show under which atmospheric conditions detailed information on this parameter is most important. The aim of our study is to identify the impacts of the copper and iron distributions in cloud droplets and aqueous aerosol particles on the total gas and aqueous budgets of OH, HO2, H2O2 and O3 in the multiphase system. Our model results give guidance for measurement needs to further constrain the ROS budgets in the atmosphere.

How to cite: Aregahegn, K. and Ervens, B.: The impact of copper and iron distribution on reactive oxygen species concentrations in the atmospheric multiphase system, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6704, https://doi.org/10.5194/egusphere-egu23-6704, 2023.

EGU23-6917 | ECS | Posters on site | AS3.1

Insights into Aqueous Glyoxal Chemistry via Glass Transition Measurements 

Jan-Hendrik Peters, Hans Peter Dette, and Thomas Koop

Atmospheric aerosols affect the Earth’s radiative budget directly by scattering, reflecting, and absorbing light and also indirectly by acting as nuclei for the formation of liquid water and ice clouds. Many of these effects are directly related to the chemical and physical properties of the aerosol particles, e.g. their phase state, which is unknown for many atmospherically relevant compounds.

Glyoxal is one of the most abundant organic species in the atmosphere with a production rate of about 45 teragram per year.1 Despite being a simple gaseous dialdehyde in the absence of water, glyoxal exhibits a complex chemistry in aqueous solutions.2 Upon drying such solutions, glyoxal does not evaporate completely, but remains in the condensed phase due to the formation of water adducts and oligomeric species.3

In our work, we present differential scanning calorimetry (DSC) experiments on dried aerosolized as well as bulk aqueous glyoxal solutions. We studied the effect of the drying rate, of the concentration of the initial glyoxal solution, of temperature, and of the addition of atmospherically relevant ammonium salts on the glass transition temperature (Tg) of the glyoxal solutions. During fast and very slow drying, highly viscous or even glassy phase states were detected via DSC measurements, and we report the corresponding glass transition temperatures of such systems. After diluting the aqueous solutions with water, mimicking atmospheric water uptake in the atmosphere, Tg of the dried solution varies with time until a new chemical equilibrium is established. Considering their temperature dependence, the time scale of these processes can range from hours to days. We use the measured time-dependent glass transition temperatures to infer dependencies of the aqueous phase equilibria between monomer, dimer, and trimer glyoxal species and their water adducts and support these by infrared spectroscopy.4 We show that glass transition measurements can be used to infer information on the aqueous chemistry of organic molecules in solution in slowly equilibrating systems.

 

References:

(1) Fu, T.-M.; Jacob, D. J.; Wittrock, F.; Burrows, J. P.; Vrekoussis, M.; Henze, D. K. Global budgets of atmospheric glyoxal and methylglyoxal, and implications for formation of secondary organic aerosols. J. Geophys. Res. 2008, 113 (D15). DOI: 10.1029/2007JD009505.

(2) Ervens, B.; Volkamer, R. Glyoxal processing by aerosol multiphase chemistry: towards a kinetic modeling framework of secondary organic aerosol formation in aqueous particles. Atmos. Chem. Phys. 2010, 10 (17), 8219–8244. DOI: 10.5194/acp-10-8219-2010.

(3) Loeffler, K. W.; Koehler, C. A.; Paul, N. M.; De Haan, D. O. Oligomer formation in evaporating aqueous glyoxal and methyl glyoxal solutions. Environmental Science & Technology 2006, 40 (20), 6318–6323. DOI: 10.1021/es060810w.

(4) Peters, J.-H.; Dette, H. P.; Koop, T. Glyoxal as a Potential Source of Highly Viscous Aerosol Particles. ACS Earth Space Chem. 2021, 5 (12), 3324–3337. DOI: 10.1021/acsearthspacechem.1c00245.

How to cite: Peters, J.-H., Dette, H. P., and Koop, T.: Insights into Aqueous Glyoxal Chemistry via Glass Transition Measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6917, https://doi.org/10.5194/egusphere-egu23-6917, 2023.

EGU23-7486 | ECS | Posters on site | AS3.1

Glass Transition Temperature Prediction via Machine Learning 

Gianluca Armeli, Jan-Hendrik Peters, and Thomas Koop

Knowledge of the glass transition temperature of molecular compounds in atmospheric aerosol particles is important for estimating their viscosity, which directly influences chemical reaction kinetics and phase state. While there is a great diversity of organic compounds present in aerosol particles, experimental glass transition temperatures are known of only a minor fraction of them. Therefore, we have developed a machine learning model in Python designed to predict the glass transition temperature of organic molecular compounds based on molecule-derived input variables. The extremely randomized trees (extra trees) procedure was chosen for this objective. Two approaches using different sets of input variables were followed. The first one uses the number of predefined functional groups present in the compound, while the second one generates descriptors from a SMILES (Simplified Molecular Input Line Entry System) string. For improved results both approaches can be combined with the melting temperature of the compound as an additional input variable, if known. The results show that the SMILES-based predictions had a slightly lower mean absolute error (MAE), but both approaches had a similar MAE of about 12-13 K. Furthermore, we also show that its performance exceeds that of previous parametrizations developed of this purpose and performs better than existing machine learning models. We believe that this model is a powerful tool for many applications in atmospheric aerosol science and material science.

How to cite: Armeli, G., Peters, J.-H., and Koop, T.: Glass Transition Temperature Prediction via Machine Learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7486, https://doi.org/10.5194/egusphere-egu23-7486, 2023.

EGU23-7737 | ECS | Orals | AS3.1

The efflorescence-deliquescence behavior of saliva droplets and its implication for viability of airborne microorganisms 

Yue Meng, Thomas Dresch, Denis Duft, Alexei Kiselev, and Thomas Leisner

The aerosol-based transport of viruses and bacteria through the transmission of aerosolized expiratory secretions is one of the main routes for the spreading of infectious diseases such as SARS-CoV-2. A number of studies have confirmed that environmental factors such as temperature and relative humidity can affect the inactivation and transmission of respiratory pathogens. However, there remain significant uncertainties in understanding aerosol micro-physics occurring under different environmental conditions to quantify the survival of microorganisms carried by aerosols. Here we study the size and phase changes of levitated saliva droplets composed of various salts and mucin under well-defined atmospheric conditions. An electrodynamic balance (EDB) is utilized for recording the evaporation and condensation kinetics of single, levitated saliva droplets with a time resolution of seconds. Efflorescence and deliquescence behaviors of droplets are monitored using light scattering and Mie theory. Compared with pure water droplets, a saliva droplet remains stably levitated for hours when the droplet approaches crystallization having reached a final size during evaporation. The morphology of crystallized particles will be imaged using a scanning electron microscope (SEM). The organic-based phase is expected to shield pathogens from inactivation by forming a solid or semisolid shell hindering the diffusion of solutes. This work highlights the importance of accounting for changes in the micro-environment of aerosols undergoing evaporation and condensation in a realistic environment which is needed to study the viability of airborne viruses and other microorganisms.

How to cite: Meng, Y., Dresch, T., Duft, D., Kiselev, A., and Leisner, T.: The efflorescence-deliquescence behavior of saliva droplets and its implication for viability of airborne microorganisms, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7737, https://doi.org/10.5194/egusphere-egu23-7737, 2023.

EGU23-9624 | Orals | AS3.1

Air pollution health inequalities in a low-carbon future 

Carly Reddington, Steven Turnock, Luke Conibear, Stephen Arnold, Lea Berrang Ford, Charlotte Weaver, Piers Forster, and Jason Lowe

Understanding the health co-benefits of climate change mitigation and how they manifest across different socioeconomic groups is crucial to justify and prioritise future decarbonisation pathways to achieve net zero. In this work, we quantify future worldwide air quality and public health co-benefits of decarbonisation to limit end-of-century warming to either 2ºC (scenario SSP1-2.6) or 1.5ºC (scenario SSP1-1.9), relative to the middle-of-the-road pathway with a medium long-term radiative forcing target of 4.5 W m-2 (scenario SSP2-4.5). We use simulated ambient fine particulate matter (PM2.5) concentrations for the period 2015-2100 from the Coupled Model Intercomparison Project (CMIP6) experiments. We estimate the mortality burden attributable to exposure to ambient PM2.5 using population attributable fractions of relative risk, incorporating projected changes in population demographics and per-capita GDP. We find that following a future decarbonisation pathway could produce substantial global reductions in population exposure to PM2.5 pollution and associated premature mortality across all socioeconomic groups, with maximum health benefits achieved for middle-income populations (predominantly in Asia) around mid-century. Overall, the more moderate 2ºC-compliant mitigation scenario (SSP1-2.6) could reduce the global PM2.5-attributable mortality burden by 24% in 2050 relative to SSP2-4.5, averting ~2.5M (95% uncertainty interval (UI): 2.1-2.8M) annual deaths worldwide. The more stringent 1.5ºC scenario (SSP1-1.9) could reduce the PM2.5 mortality burden by 29% in 2050, averting ~2.9M (UI: 2.5-3.4M) annual deaths. The magnitude of the air quality and health benefits of reduced PM2.5 pollution through decarbonisation vary with the socioeconomic status of the exposed population, with greater reductions in the PM2.5 mortality burden in middle- and high-income regions (22%) than in the low-income region (15%). Overall, the disparity in PM2.5 exposure between low- and high-income populations is predicted to reduce by 2100 under all three future scenarios. However, the global PM2.5 exposure disparity is projected to increase up to mid-century under the SSP2-4.5 scenario, thus, immediate reduction in the disparity in the near term, is only achieved under a decarbonisation scenario. Despite overall reductions in global PM2.5 exposure inequalities by the end of the century, the disparity in PM2.5 exposure remains around 30%, with the low- and lower-middle-income populations continuing to experience PM2.5 exposures that are over three times the WHO Air Quality Guideline.

How to cite: Reddington, C., Turnock, S., Conibear, L., Arnold, S., Berrang Ford, L., Weaver, C., Forster, P., and Lowe, J.: Air pollution health inequalities in a low-carbon future, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9624, https://doi.org/10.5194/egusphere-egu23-9624, 2023.

Brown carbon (BrC) is the light-absorbing fraction of organic aerosols that can affect atmospheric photochemistry and influence regional and global climate. BrC can be emitted directly from incomplete combustion or formed through multiphase reactions. BrC consists of both water-soluble and methanol-soluble fractions (Me-BrC), with the Me-BrC fraction exhibiting greater absorption compared to the aqueous fraction owing to greater extraction potential. It is important to characterize the molecular composition of BrC to gain a better understanding of the link between BrC chromophores and their light absorption properties. In this study, proton nuclear magnetic resonance (1H NMR) and high-performance liquid chromatography (HPLC) coupled with a diode array detector (DAD) and a time-of-flight mass spectrometer (TOF-MS) with an electrospray ionisation (ESI) source are used to comment on the molecular composition of Me-BrC. For this purpose, daytime and nighttime PM2.5 samples collected from April 2019 to February 2020 in a rural area in the eastern Indo-Gangetic Plain (IGP) were used.  

Both ESI- and ESI+ modes were utilized due to their respective affinity towards acidic and basic functional groups and about 500-2000 molecules were classified into four major compound classes: CHO, CHON, CHONS and CHOS. Among these, CHO- (25-32%) was the most abundant group followed by CHONS- (25-30%), CHON- (21-28%) and CHOS- (13-17%) in the negative mode whereas CHON+ (42-50%) showed the highest abundance in the positive mode followed by CHONS+ (30-38%) and CHO+ (6-14%) and CHOS+ (5-13%). 1H-NMR showed dominance of saturated oxygenated compounds (H-C-O) for all seasons, which is consistent with the high O/C ratio and OSc (oxidation state), with increasing Ar-H and hence double bond equipment (DBE) towards winter. Higher O/C (>0.3) and lower DBE of CHON+ and CHONS+ showed their significant contribution towards H-C-O type of BrC along with CHO-. CHON species can be formed by atmospheric reactions involving NOx (oxidised N-containing groups (O/C: 0.4, H/C: 1.5)) or NH3 (reduced N-containing groups (O/C: 0.2, H/C: 1.9)) with CHON- containing more organic nitrate moieties (−(O)NO2); (O/N >3)). Lower CHON towards the night time cross all seasons corresponds to the lower relative percentage of the H–C–C= type in NMR. High CHONS+ suggest presence of nitroxy organo-sulfate (formed via photooxidation of BVOCs under high NOx) or come from coal combustion. CHOS+ showed greater fraction of high‐molecular weight organosulfate compounds (low DBE or high H/C) which increased towards the winter. Also CHOS+ with high DBE (>4) with O/C (<0.4) suggests presence of reduced S‐containing compounds which are more likely to be originated from primary emissions. These findings provide the first insights into the chromophoric composition of the Indo-Gangetic Plain outflow. 

 

How to cite: Rana, A. and Sarkar, S.: Molecular characterization of methanol-soluble BrC using 1H NMR fingerprinting and high-resolution mass spectrometry., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10478, https://doi.org/10.5194/egusphere-egu23-10478, 2023.

EGU23-10785 | ECS | Posters on site | AS3.1

Humic-like substances in residential biofuel use emissions from the northwestern Himalayan region, India 

Prashant Rawat, Sebastien Bau, and Sayantan Sarkar

Indoor biofuel use for cooking/heating purposes is potentially a significant source of fine-mode aerosols in the Indian Himalayan region, with important implications for ambient atmospheric processes. Incomplete combustion of biofuels leads to emission of absorbing aerosols such as elemental carbon (EC), brown carbon (BrC) and humic-like substances (HULIS), which can affect climate via direct as well as indirect forcing.  However, profiles of these aerosols in indoor microenvironments are poorly studied, especially from the Indian Himalayan region. Here, we report size-segregated light absorption properties (absorption coefficient; babs_aq) of aqueous brown carbon (BrCaq) for cow dung cake (CDC), firewood (WD), charcoal (CC), kerosene (KS) and liquified petroleum gas (LPG) combustion in indoor settings from two northwest Himalayan states (Uttarakhand and Himachal Pradesh). We further characterize BrC composition using excitation emission matrix (EEM) fluorescence spectroscopy coupled with parallel factor (PARAFAC) analysis. Size-segregated samples (>2.5 µm, 2.5-1 µm, 1-0.5 µm, 0.5-0.25 µm and <0.25 µm) were collected during indoor cooking activities which showed PM levels exceeding Indian ambient PM2.5 standard by 8-460 times, with CDC showing the highest PM concentration in all size ranges. Size distribution profile of the fuels showed trimodal distributions with one peak in the Aitken nuclei mode (0.05 μm for CDC, WD and LPG; 0.06 μm for CC and KS) and the other two in the accumulation mode (0.22 and 2.03 μm for CDC, 0.21 μm and 2.1 μm for WD, 0.24 and 1.91 μm for KS, and 0.17 and 0.83 μm for CC). PM size distribution across kitchen and fuel types was characterized by more than 50% concentration in the Greenfield Gap region (0.1-2 μm)., CDC showed highest babs_365 for all size ranges combined (2245±357 Mm-1) compared to other fuels while LPG showed the lowest (190±46 Mm-1). BrCaq in the lowest size fraction showed greater babs compared to other size ranges in all fuels except KS. High values of babs ratio (>5) for300-400 nm (babs_300_400) to 400-500 nm (babs_400_500) wavelength range suggested the presence of HULIS in CDC and WD samples while other fuels exhibited values below 2.6. The lower size fractions (<0.5 µm) of CDC and WD were characterized by higher babs_300_400/babs_400_500 values (6.9±1.6 for CDC and 7.4±2.8 for WD) than upper size ranges (3.2±0.8 for CDC and 2.3±0.5 for WD), indicating a dominance of HULIS components in finer aerosol. Upon analysis of EEMs coupled with PARAGAC, three major chromophoric categories in BrCaq of CDC and WD samples were observed: two types of HULIS components with varying degree of conjugation and one type of protein-like substances (PRLIS). HULIS was the dominant chromophore type in lower size fractions (<0.5 µm) of CDC and WD samples (70±4% for CDC and 61±6% for WD) while for upper size fractions its contribution was relatively lower (50±10% for CDC and 36±9% for WD). Finally, BrCaq from CDC and WD emissions exhibited direct climate forcing potential equivalent to EC (relative radiative forcing (RRF): 91-98%), confirming that indoor biofuel emissions are indeed significant sources of climate forcing agents in the Indian Himalayan context.

How to cite: Rawat, P., Bau, S., and Sarkar, S.: Humic-like substances in residential biofuel use emissions from the northwestern Himalayan region, India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10785, https://doi.org/10.5194/egusphere-egu23-10785, 2023.

EGU23-10787 | ECS | Orals | AS3.1

Deposition and mineralogy of atmospheric dust at Sierra Nevada and Granada (Andalusia, SE Spain): A single particle perspective 

Aryasree Sudharaj, Jose A.G. Orza, Pedro J. Gomez-Cascales, Victor M.E. Suarez, Abel Milena-Perez, Maria.A. Ferro-Garcia, and Konrad Kandler

The transport of Saharan dust to the mountain range of Sierra Nevada occurs recurrently as well as episodically and represents an important source of nutrients for its ecosystem. At the same time, the mountain range is also vulnerable to the radiative effects, changing albedo and reduced snow covers attributed to the deposited particles from various natural and anthropogenic sources. A two-year campaign was conducted from June 2018 to August 2019 in the Sierra Nevada at 2500 m MSL (site: Albergue Universitario de Sierra Nevada) and simultaneously samples were also taken from Granada, a city lying in the foothills of Sierra Nevada (site: Faculty of Sciences, University of Granada, 670m MSL). The aim was to deduce the various sources acting over two distinct environments within a short-range distance (22 km). Deposition samples were collected on a carbon substrate using a flat plate sampler (passive method) with a sampling period of 40-72 hours. An average of 10 samples were collected per month from both sites and the current study focuses mainly on the summer months of June, July, and August when episodic dust events were observed. Along with the dust episodes, control days samples were also taken when no rain event or dust event occurred.

Single particle microscopy coupled with energy-dispersive X-ray analysis was utilized to get the chemical information on approx. 100,000 single particles over the size range of 0.5- 50 µm projected area diameter. The particles were classified according to a definite set of rules, and the main chemical classes as dust-like, sulphates, and salts-like and their mixtures were derived. Particles which didn’t fit into any of these classes were named ‘other’ classes. The focus of the results includes the relative abundance of these classes and their particle morphology (size and shape) over the two locations affected by different aerosol sources. Furthermore, the characteristics of iron-rich particles and iron content in the other dust particles were also studied given their importance in absorption properties and bioavailability for ecosystems. During the dust event days, the relative number abundance of chemical composition at Sierra Nevada showed >98 % of dust particles enriched in silicate type in the particle size range >1 µm while the <1 µm had a significant percentage in sulphates (>20%). Meanwhile at Granada, even though the dust events had an influence on the composition with higher dust content (>90%) for diameter >5µm modes, the lower size range presented higher fractions of anthropogenic particles consisting of sulphates and other particle types.

How to cite: Sudharaj, A., Orza, J. A. G., Gomez-Cascales, P. J., Suarez, V. M. E., Milena-Perez, A., Ferro-Garcia, M. A., and Kandler, K.: Deposition and mineralogy of atmospheric dust at Sierra Nevada and Granada (Andalusia, SE Spain): A single particle perspective, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10787, https://doi.org/10.5194/egusphere-egu23-10787, 2023.

EGU23-10852 | ECS | Orals | AS3.1

Dark aging of iron containing alpha-pinene secondary organic aerosol 

Natasha Garner, Jens Top, Fabian Mahrt, Imad El Haddad, Markus Ammann, and David Bell

Secondary organic aerosol (SOA) can undergo atmospheric aging processes that alter their impact on climate, air quality and human health. Transition metals, such as iron, can age SOA particles through catalytic chemical reactions within the condensed phase. Iron-containing particles originating from e.g., mineral dust, often become internally mixed with SOA, forming iron-containing SOA particles through various atmospheric processes, such as coagulation, condensation or cloud processing. When acidic organic vapors condense on iron-containing mineral dust particles, they can cause dissolution of minerals followed by iron-organic complex formation. Iron-organic complexes are common in atmospheric particles and can generate reactive oxygen species within a particle through dark peroxide and photochemical reactions (i.e., Fenton chemistry), leading to further aging of the particles by functionalization or fragmentation of organic species. Such particle-phase aging processes can considerably change the particle chemical composition. However, detailed understanding of these compositional changes is lacking to date, and hence considerable uncertainties still exist regarding the impact aged particles have on air quality and climate.

Here, we present detailed information on the chemical composition of iron-containing SOA particles and how it evolves over time. Particles were produced by forming SOA via α-pinene ozonolysis on both ammonium sulfate or iron-containing seed particles in an atmospheric simulation chamber under dark conditions. This allowed us to probe the impacts of iron on dark e.g., peroxide reactions and aerosol aging in the absence of photochemical driven Fenton chemistry, i.e., simulating nocturnal aging processes. Experiments were also conducted under both wet (relative humidity (RH) >80%) and dry (RH <10%) conditions. Aerosol bulk composition was determined using extractive electro-spray ionization mass spectrometry, allowing for high chemical and temporal identification of oxidation products, i.e., monomers and dimers, present within the particles. Under dry conditions, particles (both with and without iron) were found to contain a higher fraction of monomers, compared to dimers. Whereas under wet conditions the monomer/dimer ratio was smaller when iron was present. This suggests that iron-catalyzed functionalization reactions are favoured under wet conditions. Furthermore, when iron was present in the seed particles the lifetimes of monomers and dimers varied greatly, where the signal for some organic species (e.g., C19s and C20s) was observed to decrease rapidly (t1/2 ~ 25 min.) following SOA formation under wet conditions, while only slow decay was observed under dry conditions (t1/2 ~ 110 min.). This suggests that iron-catalyzed reactions are limited by diffusion of organic molecules under dry conditions. Overall, our results elucidate the key role of transition metals, such as iron, in altering the chemical composition of SOA particles during atmospheric transport. Such effects need to be considered to correctly reflect atmospheric aging of ambient SOA particles that are internally mixed with e.g., mineral dust, when predicting their role for air pollution and climate in atmospheric models.

How to cite: Garner, N., Top, J., Mahrt, F., El Haddad, I., Ammann, M., and Bell, D.: Dark aging of iron containing alpha-pinene secondary organic aerosol, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10852, https://doi.org/10.5194/egusphere-egu23-10852, 2023.

EGU23-10921 | Orals | AS3.1

Aerosol mixing state evolution in the atmosphere: A synthesis of measurements and models 

Nicole Riemer, Jeff Curtis, Jessica Gasparik, and Matthew West

Quantifying aerosol impacts on climate is an inherently multiscale problem since macro-scale impacts are determined by processes on the micro-scale. This poses unique modeling challenges, since these microscale processes lead to a continuously evolving aerosol mixing state, which is difficult to represent in large-scale models. This presentation will show how high-detail particle-resolved simulations can be used to predict the evolving aerosol mixing state on the regional scale. In contrast to traditional aerosol models that use bins or modes to represent the aerosol, the particle-resolved approach uses individual computational particles that evolve in size and composition as the particles undergo aging processes in the atmosphere. This approach is therefore not limited by assumptions about particle composition within a given size range and can represent the full aerosol mixing state without simplifying assumptions. I will show results that illustrate the spatio-temporal evolution of aerosol mixing state, going beyond the traditional definitions of “externally” or “internally” mixed populations. I will conclude with a framework to synthesize a picture of the ambient aerosol from models and observations. This focuses on suitable metrics to quantify mixing state and sampling strategies to determine these metrics that are accessible for both models and observations. Together, these provide a unique opportunity for “getting the right answer for the right reasons”.

 

How to cite: Riemer, N., Curtis, J., Gasparik, J., and West, M.: Aerosol mixing state evolution in the atmosphere: A synthesis of measurements and models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10921, https://doi.org/10.5194/egusphere-egu23-10921, 2023.

EGU23-10987 | Posters on site | AS3.1

Air quality deterioration episode associated with typhoon over the complex topographic environment in central Taiwan 

Chuan-Yao Lin, Yang-Fang Sheng, Wan-Chin Chen, Charles, C.K. Chou, Yi-Yun Chien, and Wen-Mei Chen

 Air pollution is typically at its lowest in Taiwan during summer. The mean concentrations of PM10, PM2.5, and daytime ozone (08:00–17:00 LST) during summer (June–August) over central Taiwan are 35–40 µg m-3, 18–22 µg m-3, and 30–42 ppb, respectively, between 2004 and 2019. Sampling analysis revealed that the contribution of organic carbon (OC) in PM2.5 could exceed 30% in urban and inland mountain sites during July in 2017 and 2018. Frequent episodes of air quality deterioration occur over the western plains of Taiwan when an easterly typhoon circulation interacts with the complex topographic structure of the island. We explored an episode of air quality deterioration that was associated with a typhoon between 15 and 17 July 2018, using the Weather Research Forecasting with Chemistry (WRF-Chem) model. The results indicated that the continual formation of low-pressure systems or typhoons in the area between Taiwan and Luzon island in the Philippines provided a strong easterly ambient flow, which lasted for an extended period between 15 and 17 July. The interaction between the easterly flow and Taiwan’s Central Mountain Range (CMR) resulted in stable weather conditions and weak wind speed in western Taiwan during the study period. Numerical modeling also indicated that a lee side vortex easily formation and the wind direction could be changed from southwesterly to northwesterly over central Taiwan because of the interaction between the typhoon circulation and the CMR. The northwesterly wind coupled with a sea breeze was conducive to the transport of air pollutants, from the coastal upstream industrial and urban areas to the inland area. The dynamic process for the wind direction changed given a reasonable explanation why the observed SO42- became the major contributor to PM2.5 during the episode. SO42- contribution proportions (%) to PM2.5 at the coastal, urban, and mountain sites were 9.4 µg m-3 (30.5%), 12.1 µg m-3 (29.9%), and 11.6 µg m-3 (29.7%), respectively. Moreover, the variation of the boundary layer height had a strong effect on the concentration level of both PM2.5 and ozone. The combination of the lee vortex and land-sea breeze, as well as the boundary layer development, were the key mechanisms in air pollutants accumulation and transport. As typhoons frequently occur around Taiwan during summer and fall, and their effect on the island’s air quality merits further research attention.

How to cite: Lin, C.-Y., Sheng, Y.-F., Chen, W.-C., Chou, C. C. K., Chien, Y.-Y., and Chen, W.-M.: Air quality deterioration episode associated with typhoon over the complex topographic environment in central Taiwan, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10987, https://doi.org/10.5194/egusphere-egu23-10987, 2023.

EGU23-11259 | ECS | Orals | AS3.1

Understanding the aerosol-cloud interactions in ship-dominated and cleaner environments in the Celtic Sea. 

Navaneeth Meena Thamban, Huihui Wu, Thomas Choularton, Hugh Coe, Keith Bower, Emily Matthews, Thomas Bannan, Nicholas Marsden, James Lee, Dominika Pasternak, Ming-Xi Yang, Stephanie Batten, Thomas Bell, Loren Temple, and Stéphane Bauguitte

Aerosol-cloud interaction contributes to one of the highest uncertainties in radiative forcing estimations. Aerosols from ship emissions alter the cloud properties and have become an important source of anthropogenic air pollution in recent decades.  We have measured the size distributions and number concentrations of aerosols in the cloud and outside clouds using various onboard instruments such as cloud droplet probe (CDP; DMT), passive cavity aerosol spectrometer (PCASP, DMT), Scanning Mobility Particle Sizer (SMPS) and Single Particle Soot Photometer (SP2; DMT). The measurements were performed in the ship emission-dominated environments and relatively cleaner regions of the Celtic Sea.  We discuss the difference in the characteristics of in-cloud and out-cloud measurements in these relatively contrasting environments. The measurements were made between 29th September and 12th October 2021 using the Facility for Airborne Atmospheric Measurements (FAAM) research aircraft as a part of the Atmospheric Composition and Radiative forcing changes due to UN International Ship Emissions regulations (ACRUISE) Project.

How to cite: Thamban, N. M., Wu, H., Choularton, T., Coe, H., Bower, K., Matthews, E., Bannan, T., Marsden, N., Lee, J., Pasternak, D., Yang, M.-X., Batten, S., Bell, T., Temple, L., and Bauguitte, S.: Understanding the aerosol-cloud interactions in ship-dominated and cleaner environments in the Celtic Sea., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11259, https://doi.org/10.5194/egusphere-egu23-11259, 2023.

EGU23-12438 | ECS | Orals | AS3.1

Spontaneous Formation of OH Radicals in the Air-Water Interface of Water Droplets 

Maria Angelaki, Yoan Carreira Mendes Da Silva, and Christian George

Water covers about 71 percent of the Earth’s surface (i.e., oceans, glaciers) and it is crucial for all the biological systems. Although bulk water is inert, water microdroplets provide a favourable environment for chemical processes. The investigation and the understanding of the physico-chemical processes that occur in the atmospheric aerosols is of great importance, while aerosols is well-known that have an adverse effect in air-quality, climate and public health. In the air-water interface the presence of a strong electric field can lead to the acceleration of chemical reactions and initiate spontaneous reduction of organic compounds. Our study is focusing on the spontaneous H2O2 production at the interface of water droplets, which occurs via the recombination of the hydroxyl radicals that are formed via the dissociation of hydroxyl ions, while other pathways cannot be excluded.  H2O2 may play a key role in the oxidation of atmospheric aerosols and therefore, it may alter the oxidation capacity by increasing the production of radicals.

Within this framework, a thorough laboratory study, using state-of-the-art instrumentation has been carried out. Two different types of experiments were performed, where the H2O2 and thus the OH production was measured either directly or indirectly by using sensitive water-soluble fluorescent probes. Aqueous microdroplets, in a range of diameter 0.1 to 10 µm were generated by nebulizing salted solutions inside a glass reactor. These particles were then collected after 4 hours reaction time and the liquid phase H2O2 was measured by using an H2O2 analyser. During our experiments, an Optical Particle Counter was connected in order to monitor the size distribution and the number of the particles. To extend our understanding in the processes that occur at the interface, different types of salts were selected (NH4Cl, Na2SO4 and CaSO4) in order to investigate the way that different ions of different valence affect the H2O2 production. A correlation between the size distribution and the hydrogen peroxide concentration was also performed. In order to verify the OH production, salted solutions containing terephalic acid (TA) were also nebulised inside the reactor. The collected droplets were analysed via fluorescent spectroscopy where the 2-hydroxyterephthalic acid (TAOH), product of the reaction of TA with OH radicals, was observed. TAOH was also observed in the particle phase in a size range of 1–5 µm.

All the experiments provide evidence that H2O2 is produced in the air-water interface of microdroplets at a range of (1–7)×10-2 µM, which depends on the size distribution, the concentration of the solution and the type of salt. Results from this study are expected to significantly improve our insight on the processes that occur in atmospheric droplets and to assess the contribution of this OH radical source in total atmospheric budget.

How to cite: Angelaki, M., Carreira Mendes Da Silva, Y., and George, C.: Spontaneous Formation of OH Radicals in the Air-Water Interface of Water Droplets, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12438, https://doi.org/10.5194/egusphere-egu23-12438, 2023.

EGU23-12455 | ECS | Orals | AS3.1

Biogenic volatile organic compounds concentrations and their conversion to oxidized VOCs and secondary organic aerosol particles 

Yanxia Li, Feng Jiang, Hengheng Zhang, Yuxuan Bian, and Harald Saathoff

Biogenic volatile organic compounds (BVOC) are key precursors for the formation of secondary organic aerosol (SOA) and strongly impact air quality and climate change. To assess the role of BVOC and their transformation to SOA, we studied BVOC sources, concentrations, and their oxidation to SOA in an urban area in southwest Germany during a summertime heatwave episode. State-of-the-art mass spectrometers including a proton-transfer-reaction time-of-flight mass spectrometer (PTR-TOF-MS) coupled with a new particle inlet chemical analysis of aerosol online (CHARON) and an aerosol mass spectrometer (AMS) were utilized to measure compositions and concentrations of particles and trace gases.  By combining meteorological parameters (temperature, relative humidity, wind direction, wind speed, and radiation), potential sources of BVOC and SOA in this characteristic urban area during the summer heatwave of 2022 were identified. Potential sources as well as the influence of temperature on BVOC to SOA conversion will be discussed.

How to cite: Li, Y., Jiang, F., Zhang, H., Bian, Y., and Saathoff, H.: Biogenic volatile organic compounds concentrations and their conversion to oxidized VOCs and secondary organic aerosol particles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12455, https://doi.org/10.5194/egusphere-egu23-12455, 2023.

EGU23-12594 | ECS | Orals | AS3.1

Roles of peroxy radicals and Criegee intermediates in β-pinene ozonolysis at different temperatures 

Yiwei Gong, Harald Saathoff, Feng Jiang, Yanxia Li, and Thomas Leisner

Organic peroxy radicals (RO2) and stabilized Criegee intermediates (SCIs), as important reactive species in the atmosphere, are critical in oxidation processes and secondary organic aerosol (SOA) formation. However, the influence of temperature on these reactive intermediates and the corresponding reaction mechanisms in SOA formation is still not well defined. In this study, through utilizing SCIs scavengers and regulating [HO2]/[RO2] from ~0.3 to ~1.9, the roles of RO2 and SCIs in SOA formation were investigated at 298 K, 273 K, and 248 K, respectively, particularly for dimers formation in β-pinene ozonolysis. It was found that the dependence of the SOA yields on temperature was not monotonic. With the temperature decreasing from 298 K to 273 K, the SOA formation was promoted by the gas-particle partitioning of semi- and low-volatility products. However, when the temperature further decreased to 248 K, the SOA yields were lower due to the temperature effect on chemical reactions. The addition of SCIs scavengers showed that SCIs reactions accounted for more than 40% of both dimers and aerosol formation under all temperature conditions. The SCIs reactions predominantly contributed to the formation of C18 and C19 dimers. Increasing the [HO2]/[RO2] ratio suppressed SOA and dimers formation at all temperatures, indicating that in β-pinene ozonolysis RO2+RO2 reactions generate products of lower volatility, while RO2+HO2 reactions tend to form products of higher volatility. The lower RO2 concentrations and suppressed RO2+RO2 reactions could partly explain the reduced SOA yield at 248 K. Additionally, it was found that the sensitivity of dimers formation on [HO2]/[RO2] was higher at lower temperatures. Even though the impact of temperature on the reaction coefficients of peroxy radicals was considered, the dimers formation at different [HO2]/[RO2] ratios could not be explained well at 273 K and 248 K. This suggests that SCIs reactions with RO2 radicals may become more important at lower temperatures due to slower isomerization and decomposition of SCIs.

How to cite: Gong, Y., Saathoff, H., Jiang, F., Li, Y., and Leisner, T.: Roles of peroxy radicals and Criegee intermediates in β-pinene ozonolysis at different temperatures, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12594, https://doi.org/10.5194/egusphere-egu23-12594, 2023.

EGU23-12650 | ECS | Orals | AS3.1

Numerical simulation and evaluation of global ultrafine particle concentrations 

Matthias Kohl, Sourangsu Chowdhury, Disha Sharma, Yafang Cheng, Sachchida Nand Tripathi, Mathew Sebastian, Govindan Pandithurai, Hongli Wang, Jos Lelieveld, and Andrea Pozzer

Ultrafine particles (UFP), i.e. particles with an aerodynamic diameter below 100 nm, have a significant impact on public health and the hydrological cycle. Recent studies showed that their ability to penetrate more deeply into the lungs and potentially into the blood stream may cause an increased incidence of cardiovascular and cerebrovascular diseases. Additionally, UFPs significantly contribute to cloud condensation nuclei concentrations. However, knowledge on global distributions of UFPs is scarce.

We present a global simulation of UFP concentrations using the ECHAM/MESSy Atmospheric Chemistry Model (EMAC), including tropospheric and middle-atmospheric processes, and the modal aerosol microphysics submodel GMXe. Due to the high sensitivity of UFP concentrations to the size distribution of emitted particles, we derived emission median diameter for primary emissions from various sectors and species based on existing literature. We show the importance of primary emissions and nucleation on UFP concentrations as well as their composition, seasonality and vertical distributions.

Model results were evaluated over Europe, the United States, India and China, using particle size distribution and particle number concentration measurements from available datasets and the literature. We obtain reasonable agreement between the model results and observations. However, the highest values of observed, street-level UFP concentrations are systematically underestimated, whereas in rural environments close to urban areas they are generally overestimated by the model. As the relatively coarse global model does not resolve concentration gradients in urban centres and local UFP hotspots, high-resolution data of anthropogenic emissions is used to account for such differences in each model grid box. This downscaling further improves the agreement with observations, decreasing the root mean squared logarithmic error and removing discrepancies associated with air quality and population density gradients within the model grid boxes.

How to cite: Kohl, M., Chowdhury, S., Sharma, D., Cheng, Y., Tripathi, S. N., Sebastian, M., Pandithurai, G., Wang, H., Lelieveld, J., and Pozzer, A.: Numerical simulation and evaluation of global ultrafine particle concentrations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12650, https://doi.org/10.5194/egusphere-egu23-12650, 2023.

EGU23-13194 | ECS | Posters on site | AS3.1

MultilayerPy: a tool for creating and optimising multi-layer models of aerosol and film processes 

Adam Milsom, Amy Lees, Adam Squires, and Christian Pfrang

Heterogeneous processes such as aerosol-gas chemical reactions and vapour uptake are key to understanding the behaviour of aerosols in our environment. They contribute to their ability to take up water to form cloud droplets and determine the persistence of harmful particle-bound compounds, impacting the climate and human health.

Kinetic multi-layer models such as the kinetic multi-layer model for aerosol surface and bulk chemistry (KM-SUB) and gas-particle interactions (KM-GAP) are state-of-the-art models used to describe these processes on the particle and film level (Shiraiwa et al., 2010, 2012). KM-SUB and KM-GAP-based models have been used to determine the oxidative potential of particulate matter, the impact of surfactant self-organisation on aerosol chemical lifetimes, and the impact of aerosol phase state on the long-range transport of toxic chemicals. These models are useful but cumbersome to write and there is a need for an open-source tool to assist researchers in creating and optimising them.

We have developed MultilayerPy (Milsom et al., 2022), an open-source Python package which facilitates the creation and optimisation of kinetic multi-layer models. This software is written such that the user uses building blocks (i.e. reaction scheme, bulk diffusion parameterisations, and model components) to automatically generate model code which can then be ran and the output presented in a reproducible manner. This reduces the time needed to develop model descriptions of aerosol processes and allows the user to focus on the scientific issues rather than coding the models. I will present recent use cases of the software looking at the chemical lifetime of real aerosol material in the atmosphere, along with ongoing work extending the base package.

References:

Milsom, A., Lees, A., Squires, A. M. and Pfrang, C.: MultilayerPy (v1.0): a Python-based framework for building, running and optimising kinetic multi-layer models of aerosols and films, Geosci. Model Dev., 15(18), 7139–7151, doi:10.5194/gmd-15-7139-2022, 2022.

Shiraiwa, M., Pfrang, C. and Pöschl, U.: Kinetic multi-layer model of aerosol surface and bulk chemistry (KM-SUB): The influence of interfacial transport and bulk diffusion on the oxidation of oleic acid by ozone, Atmos. Chem. Phys., 10, 3673–3691, doi:10.5194/acp-10-3673-2010, 2010.

Shiraiwa, M., Pfrang, C., Koop, T. and Pöschl, U.: Kinetic multi-layer model of gas-particle interactions in aerosols and clouds (KM-GAP): Linking condensation, evaporation and chemical reactions of organics, oxidants and water, Atmos. Chem. Phys., 12(5), 2777–2794, doi:10.5194/acp-12-2777-2012, 2012.

How to cite: Milsom, A., Lees, A., Squires, A., and Pfrang, C.: MultilayerPy: a tool for creating and optimising multi-layer models of aerosol and film processes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13194, https://doi.org/10.5194/egusphere-egu23-13194, 2023.

EGU23-13967 | Orals | AS3.1

Molecular composition and volatility of secondary organic compounds from nitrate radical oxidation of biogenic volatile organic compounds – from lab to field 

Cheng Wu, Emelie L. Graham, David M. Bell, Amelie Bertrand, Urs Baltensperger, Imad El Haddad, Chieko Fujimura, Yvette Gramlich, Sophie L. Haslett, Radovan Krejci, Epameinondas Tsiligiannis, Mattias Hallquist, Ilona Riipinen, and Claudia Mohr

Night-time reactions of biogenic volatile organic compounds (BVOCs) and nitrate radicals (NO3) can lead to the formation of secondary organic aerosol (BSOANO3). Here we firstly present the chemical composition and volatility of BSOANO3 formed in the dark from three precursors (isoprene, α-pinene, and β-caryophyllene) in atmospheric simulation chamber experiments (Wu et al., 2021; Bell et al., 2022; Graham et al., 2022). The chemical composition of particle-phase compounds was measured with a chemical ionization mass spectrometer with a filter inlet for gases and aerosols (FIGAERO-CIMS) and an extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF). The volatility information of BSOANO3 was derived from isothermal evaporation chambers, temperature-dependent evaporation in a volatility tandem differential mobility analyzer (VTDMA), and thermal desorption in the FIGAERO-CIMS. In addition, the molecular composition of particulate compounds was used in volatility parametrizations to calculate the compounds’ saturation vapor pressures and to establish volatility basis sets (VBS, Donahue et al., 2011) for the bulk aerosol. Four different parametrizations were tested for reproducing the observed evaporation in a kinetic modeling framework (Riipinen et al., 2010). Here, we compare the different methods for particle volatility determination and discuss the limitation of the parameterizations.

Our results suggest the BSOANO3 from α-pinene and isoprene be dominated by low-volatility organic compounds (LVOC) and semi-volatile organic compounds (SVOC), while the corresponding BSOANO3 from β-caryophyllene consists primarily of extremely low-volatility organic compounds (ELVOC) and LVOC. The parameterizations yielded variable results in terms of reproducing the observed evaporation, and generally the comparisons pointed to a need for re-evaluating the treatment of the nitrate group in such parameterizations.

Furthermore, we link the lab experiments to field observations of secondary organic aerosols and organic nitrates from a boreal forest (ICOS Norunda, Sweden), which is dominated by monoterpene emissions and includes also isoprene and sesquiterpene emissions. We will show the chemical composition and volatility of the particles detected with a FIGAERO-CIMS, compare them to the lab results, and discuss how nitrate-initiated nighttime oxidation of different precursors contribute to the total particle formation and growth.

 

References:

Wu, C. et al., Atmos. Chem. Phys., 21, 14907–14925, 2021

Bell, D. et al., Atmos. Chem. Phys., 22, 13167–13182, 2022

Graham, E. and Wu, C. et al, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2022-1043, 2022

Donahue, N. M. et al., Atmos. Chem. Phys., 11, 3303–3318, 2011

Riipinen, I. et al., Atmos. Environ., 44-5, 597-607, 2010

 

How to cite: Wu, C., Graham, E. L., Bell, D. M., Bertrand, A., Baltensperger, U., El Haddad, I., Fujimura, C., Gramlich, Y., Haslett, S. L., Krejci, R., Tsiligiannis, E., Hallquist, M., Riipinen, I., and Mohr, C.: Molecular composition and volatility of secondary organic compounds from nitrate radical oxidation of biogenic volatile organic compounds – from lab to field, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13967, https://doi.org/10.5194/egusphere-egu23-13967, 2023.

EGU23-14075 | ECS | Orals | AS3.1

Formation of secondary organic aerosol from sitka spruce emissions 

Hayley Furnell, Julien Kammer, Astrid Wingler, Kieran Kilcawley, David Mannion, and John Wenger

Biogenic volatile organic compounds (BVOCs) emitted from a wide range of trees and plants undergo oxidation reactions in the atmosphere to produce secondary organic aerosol (SOA), which has direct and indirect effects on climate, and is accountable for a large proportion of climate uncertainties. The composition and yield of SOA is determined by the precursor BVOCs, which depends on the emission profile of the plant. In Ireland forestry is dominated by Sitka spruce (Picea Sitchensis), the emissions of which are not well characterised. The goal of this study is to identify the BVOC emissions from Sitka spruce, and to assess their SOA formation potential.

To characterise the emission profile of Sitka spruce, 4-year old trees were housed in a plant growth chamber under controlled environmental conditions and the emissions monitored on-line with a time-of-flight chemical ionisation mass spectrometer (ToF-CIMS), and off-line with thermal desorption gas chromatography mass spectrometry. The atmospheric reactions of the VOCs emitted by the Sitka spruce were investigated by oxidising them with hydroxyl (OH) radicals in an atmospheric simulation chamber. BVOC oxidation and gas-phase product formation was monitored by ToF-CIMS. A scanning mobility particle sizer (SMPS) was used to track particle formation and growth, and the SOA composition was determined with the use of a filter inlet for gas and aerosols (FIGAERO) fitted to the ToF-CIMS.

Over 60 different BVOCs were identified in the Sitka spruce emissions, with oxygenated species accounting for over 50% of them. The most abundant compound identified was piperitone, C10H16O an oxygenated monoterpene. Other compounds prevalent in the emissions included isoprene and monoterpenes, such as myrcene and β-phellandrene. During oxidation experiments the decay of the Sitka spruce emissions was observed with the ToF-CIMS in C6H6+ mode, while the formation of oxidised gas products was observed in I- mode. The most prevalent gas-phase product was C5H6O3. Analysis of the gas-phase oxidation products indicated that the oxidation of multiple BVOCs led to their formation. Particle formation and growth commenced quickly after the OH reaction was initiated. The composition of the SOA showed C6H8O6 as the dominant species, but the majority of the products had formulas in the range #C7 – 15 and #O5 - 8. Analysis of both gas and particle phase chemistry has been performed to determine the SOA formation potential of Sitka spruce BVOC emissions.

 

How to cite: Furnell, H., Kammer, J., Wingler, A., Kilcawley, K., Mannion, D., and Wenger, J.: Formation of secondary organic aerosol from sitka spruce emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14075, https://doi.org/10.5194/egusphere-egu23-14075, 2023.

EGU23-14862 | ECS | Posters virtual | AS3.1

Key Role of Equilibrium HONO Concentration over Soil in Quantifying Soil-Atmosphere HONO Fluxes 

Fengxia Bao, Yafang Cheng, Uwe Kuhn, Guo Li, Wenjie Wang, Alexandra Kratz, Jens Weber, Bettina Weber, Ulrich Pöschl, and Hang Su

Nitrous acid (HONO) is an important component of the nitrogen cycle in the atmosphere. Photolysis of HONO generates hydroxyl (OH) radicals and significantly influences the atmospheric oxidative capacity. Early laboratory work discovered that soil nitrite, produced via biological nitrification or denitrification, can be an important HONO source. However, the laboratory-determined chamber HONO fluxes can largely deviate from those in the real world for the same soil sample. Therefore, quantification of soil fluxes of HONO in the atmosphere remains challenging. [HONO]*, the equilibrium gas-phase concentration over the aqueous solution of nitrous acid in the soil, has been suggested as a key parameter for quantifying soil fluxes of HONO; but it has not yet been well-validated and quantified. In this project, we present a method to retrieve [HONO]* by conducting controlled dynamic chamber experiments with soil samples and validate the existence of [HONO]* over the soil. We show that [HONO]* is a soil characteristic, independent of HONO concentrations in the chamber. Therefore, it is reliable to use [HONO]* to quantify soil fluxes of HONO. [HONO]* performs as an indicator of the potential of soil to be a source or a sink for atmospheric HONO and helps to better quantify the role of HONO fluxes of soil in the HONO budget and its implications on the oxidizing capacity in the atmosphere. 

How to cite: Bao, F., Cheng, Y., Kuhn, U., Li, G., Wang, W., Kratz, A., Weber, J., Weber, B., Pöschl, U., and Su, H.: Key Role of Equilibrium HONO Concentration over Soil in Quantifying Soil-Atmosphere HONO Fluxes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14862, https://doi.org/10.5194/egusphere-egu23-14862, 2023.

EGU23-15074 | ECS | Posters on site | AS3.1

Elemental characterization of PM2.5 at an urban traffic site in Central Europe 

Laurence Windell, Petra Pokorna, Jakub Ondracek, Jaroslav Schwarz, Radek Lhotka, and Vladimir Zdimal

Metal content in traffic emissions is often overlooked during regulation and policy making. Exhaust and non-exhaust traffic emissions, including tire, brake wear and re-suspended dust, contribute greatly to particulate matter and pose significant health effects to humans in urban areas (Johansson et al., 2009). The current lack of strict regulations on these metal emissions draws attention to the need for controls and monitoring, as reflected in the recent Euro 7 standards proposal for research on traffic emissions. This work aims to quantify metal emissions from traffic at an urban traffic site in Prague, Czech Republic, identify key tracers of emissions, and investigate exhaust and non-exhaust emissions observable in fine particulate matter (PM2.5). This project signifies the first high-time resolution metal analysis in Prague.

Two one-month long measurement campaigns were conducted from February to March and November to December 2020 at an urban traffic site in Prague. Elemental data were obtained from the Xact625i Ambient Metals Monitor (analytical method nondestructive energy dispersive X-ray fluorescence – EDXRF) equipped with a PM2.5 head at a two-hour time resolution. Enrichment factors were calculated, and correlations of key tracers (e.g. Cu, Ba, Zn, Mn) were identified. Source apportionment will be carried out using Positive Matrix Factorization (US EPA PMF 5.0) as well as a human risk assessment for potentially carcinogenic elements. Metallic elemental concentrations were observed in decreasing order: Fe > Zn > Cu > Ti > Mn > Ba > Cr > As > Cd > Ni. The most abundant metal, Fe, was found in the range of 10 – 2933 ng/m3, followed by Zn (1 – 144 ng/m3), Cu (1 – 104 ng/m3), Ba (0.1 – 41 ng/m3) and Cr (0.2 – 16 ng/m3). Enrichment factors of Cr, Mn, Cu and Zn were found to be up to 113, 71, 1937 and 1066, respectively.

Acknowledgement:

This conference contribution was supported by the Ministry of Education, Youth and Sports of the Czech Republic under grants ACTRIS-CZ LM2018122,  ACTRIS-CZ RI (CZ.02.1 .01 / 0.0 / 0.0 / 16_013 / 0001315) and LTAUSA19006.

References:

JOHANSSON, C., NORMAN, M. & BURMAN, L. 2009. Road traffic emission factors for heavy metals. Atmospheric Environment - ATMOS ENVIRON, 43, 4681-4688.

 

How to cite: Windell, L., Pokorna, P., Ondracek, J., Schwarz, J., Lhotka, R., and Zdimal, V.: Elemental characterization of PM2.5 at an urban traffic site in Central Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15074, https://doi.org/10.5194/egusphere-egu23-15074, 2023.

EGU23-15676 | Orals | AS3.1

Aerosol source and processes in the Arctic 

Mao Du and Zongbo Shi

Arctic earth system is highly sensitive environmental change. Arctic warms up by 2-4 times faster than the rest of the world. Environmental changes in Arctic has a profound impact on the regional and global climate. Aerosol particles play an important role in Arctic climate system. Predicting how Arctic atmosphere will change in a warming world requires a better understanding of the state of aerosols now, as a baseline from which any predictions can be made. Motivated by this, we carried out field observations in the Arctic region during a research cruise and at ground stations. The overall aim is to improve our understanding on the sources and aerosol particles and their impact on the climate and clouds.

This presentation will show preliminary results from the DY151 research cruise (May-June 2022) to the Labrador Sea and the Davis Strait. The main objectives of the cruise include:

  • Sources and processes of aerosol particles, cloud condensation nuclei and ice nuclei
  • Source and processes of gaseous pollutants
  • Formation and growth mechanism of new particles
  • Improve modelling of aerosol sources and processes in the Arctic and predict the impact of potential increase in Arctic shipping on the clouds and climate in the future

Operations onboard included the measurement of atmospheric and oceanic parameters, including:

  • size distributions of particles from 1 nm to 20 µm;
  • gaseous pollutants such as volatile organic compounds, nitrogen oxides, HONO, HCHO, carbon monoxide, and sulphur dioxide;
  • molecular clusters and highly oxygenated organic compounds that contribute to the formation and growth of new particles;
  • chemical composition of aerosol particles including both organic tracers and inorganic species, and black carbon;
  • particle mass concentrations;
  • cloud condensation nuclei and ice nuclei concentrations;
  • optical observations of atmospheric particles and radiation; and
  • surface ocean chlorophyll a concentrations and routinely measured parameters onboard such as salinity.

These comprehensive observations will allow to better understand (1) the emissions, sources, and oxidation of key gaseous pollutants, (2) formation and growth of new particles, (3) contribution of newly formed particles to cloud condensation nuclei, and (4) sources of aerosol particles, cloud condensation nuclei and ice nuclei.

How to cite: Du, M. and Shi, Z.: Aerosol source and processes in the Arctic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15676, https://doi.org/10.5194/egusphere-egu23-15676, 2023.

EGU23-15685 | ECS | Posters on site | AS3.1

Expanding volatility calibration range of FIGAERO-ToF-CIMS 

Arttu Ylisirniö, Noora Hyttinen, Zijun Li, Mitchell Alton, Iida Pullinen, Taina Yli-Juuti, and Siegfried Schobesberger

Filter Inlet for Gases and Aerosols (FIGAERO) inlet coupled with Time-of-Flight Chemical Ionization Mass Spectrometers (ToF-CIMS) have been successfully employed in numerous studies during past years (Thornton et. al., 2020). The instrument can be used to study both gas-phase and particle-phase chemical compounds over a broad range of chemical functionalities. The inbuilt controlled thermal desorption mechanism also allows for the investigation of volatility of the compounds present in the particle phase. Such a particle volatility measurement using FIGAERO-ToF-CIMS relies on accurate identification of the Tmax for individual compounds, i.e. the temperatures at which highest respective signals are observed. These Tmax values can be converted to saturation vapor pressure Psat and saturation mass concentration C* values with a reliable calibration (Ylisirniö et. al., 2021). 

However, due to a lack of calibration compounds with known Psat at the low end of the volatility range (Psat <10-9 (Pa) / C* < -10-4 (μg/m3)), the current calibration procedure can only cover the desorption temperature range up to ~80-100 ˚C, while desorption temperatures of FIGAERO-ToF-CIMS can reach 200 ˚C and Tmax values are routinely identified up to 160 ˚C. In this study we aim to extend the FIGAERO-ToF-CIMS calibration values to cover lower Psatvalues by utilizing a range of different approaches to increase the accuracy of the volatility measurement.

Methods

Tmax values of Polyethylene Glycols (PEG’s) from PEG 5 to 15 were measured with FIGAERO-CIMS and corresponding C* values were either measured (for PEG 5-9) with isothermal evaporation experiments or estimated (PEG 5-15) with several different methods. Used estimation methods were quantum chemical modelling (COSMOtherm), desorption modelling (Schobesberger et. al., 2018), and parametrizations including Modified Grain Model, EVAPORATION, SIMPOL, and by Li et. al., 2016, Stolzenburg et. al., 2018 and Mohr et. al., 2019. Additionally, a parametrization equation according to Li et. al. 2016 was fitted to PEG 4-9 literature data and C* values of PEG 10-15 were estimated with this fit.                   

Results

Figure 1 shows the measured and estimated C*(298 K) values as function of the measured Tmaxvalues. The spread of results with different models is increasingly larger especially at the higher order PEG’s, with over 10 orders of magnitude difference between models. Two independent measurement methods agree with each other within one order of magnitude. Best agreement with measurements is with desorption model, Modified Grain Model and COSMOTherm.

Figure 1. Tmax vs. C*. Results from different measurements or estimates are shown in the figure legend. Note that some markers are very close to each other.

 

This work was supported by Academy of Finland Flagship funding (grant no. 337550)

 

Li et. al., 2016, Atmos. Chem. Phys., 16, 3327-3344.

Krieger et. al., 2018, Atmos. Meas. Tech., 11(1), 49–63.

Mohr et. al., 2019, Nat. Comm. 10, Article number: 4442.

Schobesberger et. al., 2018, Atmos. Chem. Phys., 18(20), 14757–14785.

Stolzenburg et. al., 2018, PNAS, 115 (37) 9122-9127.

Thornton et. al., 2020, Acc. Chem. Res., 53(8), 1415–1426.

Ylisirniö et. al., 2021, Atmos. Meas. Tech., 14(1), 355–367.

How to cite: Ylisirniö, A., Hyttinen, N., Li, Z., Alton, M., Pullinen, I., Yli-Juuti, T., and Schobesberger, S.: Expanding volatility calibration range of FIGAERO-ToF-CIMS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15685, https://doi.org/10.5194/egusphere-egu23-15685, 2023.

EGU23-15768 | ECS | Orals | AS3.1

Molecular rearrangement of bicyclic peroxy radicals: key route to aerosol from toluene 

Siddharth Iyer, Avinash Kumar, Anni Savolainen, Shawon Barua, Olga Garmash, Prasenjit Seal, and Matti Rissanen

Aromatic compounds contribute significantly to the formation of secondary organic aerosol (SOA) that have implications on health and on climate. Toluene is the most abundant aromatic compound in the atmosphere and is emitted through anthropogenic activities such as incomplete combustion and industrial processes. To form SOA, participating vapors such as toluene need to have sufficiently low volatility, which in practice implies molecules with multiple oxygen containing polar functional groups called highly oxygenated organic molecules (HOMs). The oxidation of toluene by OH can lead first to bicyclic peroxy radicals (BPR), and then to HOM. While the formation of HOM has been shown to be efficient, the underlying molecular level mechanism has been challenging to accurately elucidate because of the sheer number of potential pathways. This leads to a major gap in the understanding of the formation of SOA from toluene in the atmosphere. In this work, we conclusively demonstrate for the first time that the toluene derived BPR is unstable under atmospheric conditions and undergoes spontaneous molecular rearrangement to lead to completely ring broken RO2s at rates competitive with bimolecular reactions with NO even under polluted conditions. Intriguingly, several of the closed shell products deriving from the BPR are likewise unstable and decompose in finite timescales. This is relevant for those aromatic compounds that lead to BPRs that are otherwise stable against rearrangement reactions, providing, e.g., a long-range transport vehicle for NOx similar to peroxyacyl nitrates (PAN). Using quantum chemical calculations and master equation simulations that account for energy non-accommodation, we elucidate the molecular level mechanism of the subsequent autoxidation of the ring broken RO2s that leads rapidly to the HOM O9-RO2. Furthermore, using targeted flow reactor experiments of the OH reaction of toluene and partially deuterated toluene with nitrate chemical ionization mass spectrometry (CIMS) detection, we corroborate the proposed new mechanism. This is the only unambiguous reaction pathway to toluene derived HOM reported to date, and it has implications on the aerosol and ozone forming potential of toluene.

How to cite: Iyer, S., Kumar, A., Savolainen, A., Barua, S., Garmash, O., Seal, P., and Rissanen, M.: Molecular rearrangement of bicyclic peroxy radicals: key route to aerosol from toluene, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15768, https://doi.org/10.5194/egusphere-egu23-15768, 2023.

EGU23-15897 | ECS | Posters on site | AS3.1

Risks and benefits of stratospheric solid particle injection for climate intervention 

Sandro Vattioni, Rahel Weber, Oliver Klaus, Beiping Luo, John Dykema, Andrea Stenke, Aryehe Feinberg, Max Döbeli, Christof Vockenhuber, Ulrich Kreiger, Uwe Weers, Luca Artiglia, Huanyu Yang, Luca Longetti, Jerome Gabathuler, Markus Ammann, Frank Keutsch, Thomas Peter, and Gabriel Chiodo

Recent studies have suggested that injection of solid particles such as alumina (Al2O3) and calcite (CaCO3) instead of SO2 for stratospheric aerosol intervention could reduce some of the adverse side effects of SAI such as ozone depletion, stratospheric heating, and changes in diffuse radiation. However, the expected improvements from alteration of stratospheric chemistry are subject to large uncertainties. We constrain some of these uncertainties by experimental work on calcite particles using elastic recoil detection analysis (ERDA) and in-situ experiments using X-ray photoelectron spectroscopy (XPS). Subsequently, we use a global aerosol-chemistry climate model that, for the first time, interactively couples microphysical and chemical processes of solid calcite and alumina particles as well as liquid sulfuric acid aerosols with model radiation and transport. Notably, SAI by solid particles only leads to more effective radiative forcing per aerosol burden compared to sulfuric acid aerosols, not per injected mass. However, reduced stratospheric warming remains a major advantage of solid particles. Furthermore, different assumptions on the heterogeneous chemistry of solid particles, based on the available experimental data, result in drastically different impacts on stratospheric composition, in particular, ozone. For alumina particles, which are thought to not undergo chemical aging during their stratospheric residence time we present a sensitivity analysis for heterogenous reactions to quantify uncertainty. For the alkaline calcite particles, which are thought to undergo chemical aging in the stratosphere via reaction with acids (e.g., HCl, HNO3, H2SO4) we find even larger uncertainties due to unknown reaction pathways and highly uncertain rates under stratospheric conditions. The large uncertainty in predicted stratospheric ozone changes can only be reduced via substantial additional laboratory experiments under stratospheric conditions, i.e., partial pressures of relevant gases (e.g., HCl, HNO3, H2SO4), temperatures < 220 K, relative humidity < 1% and realistic UV irradiance. From the present perspective, sulfur-based SAI has significantly lower uncertainty than injection of solid particles, which have significantly reduced stratospheric heating but very large uncertainties in impacts on stratospheric composition.

How to cite: Vattioni, S., Weber, R., Klaus, O., Luo, B., Dykema, J., Stenke, A., Feinberg, A., Döbeli, M., Vockenhuber, C., Kreiger, U., Weers, U., Artiglia, L., Yang, H., Longetti, L., Gabathuler, J., Ammann, M., Keutsch, F., Peter, T., and Chiodo, G.: Risks and benefits of stratospheric solid particle injection for climate intervention, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15897, https://doi.org/10.5194/egusphere-egu23-15897, 2023.

Over the past few decades, adequate evidence has confirmed the adverse effects of short-term PM2.5 exposure on asthma exacerbation, whereas the effects of long-term exposure on asthma morbidity and mortality, especially in adults, are still under debate. Benefiting from the recent explosion of relevant epidemiological studies, we comprehensively explored the impact of long-term ambient PM2.5 exposure on both childhood and adult asthma in light of the emerging evidence by combining multiple state-of-the-art approaches.

First, we explored the association between long-term PM2.5 exposure and risk of asthma by conducting a systematic review and meta-analysis. Through the systematic review, we identified a total of 3187 unique literatures, and found 32 on childhood asthma and 17 on adult asthma meeting the full eligibility criteria. According to the random-effects meta-analyses covering 10,519,588 children and 9,876,107 adults, we find that every 2 µg/m3 increment in PM2.5 is associated with a 3.8% (95% CI: 1.6%–6.1%) and a 1.1% (95% CI: 0.1%–2.2%) increase in risk of childhood asthma and adult asthma, respectively.

We then explored the exposure-response effect of asthma at different exposure levels—i.e., estimated the exposure-response curves for asthma, by constructing exposure-response functions (ERFs) based on the data extracted from the systematic review. We find that risk of childhood asthma increases almost linearly with exposure concentrations, while the risk of adult asthma increases sub-linearly. We also find that the risk of childhood asthma is much higher than that of adult asthma at any given exposure level.

After confirming by the meta-analysis and exposure-response analysis that PM2.5 exposure is statistically significantly associated with increased risk of asthma, we estimated the global burden of asthma attributable to long-term PM2.5 exposure by applying the ERFs in an epidemiological model. We find that PM2.5 exposure is responsible for 11.2 (95% CI: 7.4–14.1) million new cases of asthma and 58.3 (95% CI: 37.3–74.7) million prevalent cases in 2015, and children present majority of these cases.

Our study provides additional evidence on the effects of long-term PM2.5 exposure on asthma by concluding a statistically significantly positive association between PM2.5 exposure and the increased risk of asthma both in children and adults. Moreover, the substantial PM2.5-attributable burden of asthma assessed in this study suggests a large impact of PM2.5 on public health through asthma—i.e., the overall disease burden caused by PM2.5 is much higher than previously thought. In light of these findings, we call for more attention to the effects of PM2.5 exposure on asthma and for more stringent legislation to be designated sooner to improve air quality. In addition, the exposure-response curves established in our study—which incorporating evidence on high exposure levels that covering most of the worldwide exposure ranges—could be applied to assess the city to global scale asthma-related health benefits obtained from air pollutant reduction associated with policy scenarios.

How to cite: Ni, R., Su, H., and Cheng, Y.: Effects of long-term ambient fine particulate matter exposure on asthma: Evidence both for children and adults, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16213, https://doi.org/10.5194/egusphere-egu23-16213, 2023.

EGU23-16364 | Posters on site | AS3.1

DRAGON J-ALPS: study of aerosol properties in Japanese Alps and valley region 

Itaru Sano, Sonoyo Mukai, Nakata Makiko, Brent Holben, and Teruya Maki

A field campaign, AERONET DRAGON J-ALPS (joint research on aerosol process studies), is planned to is planned to study the influence of mountain topography on aerosol transport, the aerosol life cycle, and aerosol properties in a narrow valley. DRAGON/J-ALPS was planned to start in March 2020, with 12 AERONET Cimel sun/sky radiometers deployed in the central valley surrounded by the Japanese Alps. Some instruments were also placed in the mountains to study aerosols transported through the higher layers. In April 2020, however, observations were discontinued due to the COVID-V2; they resumed in the fall of 2020 and were extended until the spring of 2021. Some sites also operated until fall 2021.

The initial results of DRAGON/J-ALPS are presented in terms of aerosol characteristics from ground and satellite observations, with particular focus on regional background aerosols and long-range transboundary aerosols (biomass burning smoke, Asian dust, and volcanic smoke) across the Japanese Alps. Results of regional model simulations will also be presented.

How to cite: Sano, I., Mukai, S., Makiko, N., Holben, B., and Maki, T.: DRAGON J-ALPS: study of aerosol properties in Japanese Alps and valley region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16364, https://doi.org/10.5194/egusphere-egu23-16364, 2023.

EGU23-16598 | Orals | AS3.1

From volatile to non-volatile in sub second time-scales: rapid HOM formation in seemingly disparate chemical systems 

Matti Rissanen, Avinash Kumar, Shawon Barua, and Siddharth Iyer

During the recent decade our molecular level understanding of  secondary aerosol generation in the atmosphere has progressed tremendously. The old paradigm that ambient aerosol pre-stage formation necessitates long processing times with scarce oxidants in the atmosphere has been found flawed, and we are continuously learning how the increase in molecular oxygen content, and the corresponding decrease in vapour pressure, happen far faster than presumed. We are steadily approaching a situation where the classical “single compound, single SOA yield” type of a thinking becomes obsolete, and the mechanistic description at a molecular level is required to tackle the rapid formation of ambient secondary aerosol mass.

In the current work we have performed laboratory flow reactor experiments of monoterpene and aromatic compound (auto-)oxidation applying chemical ionization mass spectrometry (CIMS) for product detection. The experiments were complemented by high-level quantum chemical computations of the important mechanistic steps, and the energy non-accommodation was accounted for in the formation of the important intermediates (i.e., we investigated the role of excess reaction energy for the product formation). It has been learned that even in seemingly very disparate chemical systems the formation of condensable products occurs fast, often in sub-second time-scales.

How to cite: Rissanen, M., Kumar, A., Barua, S., and Iyer, S.: From volatile to non-volatile in sub second time-scales: rapid HOM formation in seemingly disparate chemical systems, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16598, https://doi.org/10.5194/egusphere-egu23-16598, 2023.

EGU23-16841 | Orals | AS3.1

Seasonal changes of sources, volatility, and aging of organic aerosols in eastern Europe reflected in the stable isotopic composition 

Ulrike Dusek, Agne Masalaite, Peng Yao, Noni van Ettinger, Vidmantas Remeikis, and Dipayan Paul

The stable carbon isotope 13C has the potential to give insights into sources and processing of organic aerosol. We use a method to measure d13C in OC desorbed from filter samples at three different temperature steps: 200 °C, 350°C and 650°C. The results give a rough indication of aerosol volatility, as more volatile compounds usually desorb at lower temperatures.

We demonstrate with an extensive source study that in Lithuania and likely other Eastern European regions, the main anthropogenic primary sources for organic carbon (OC) have distinct isotopic signatures. d13C values of vehicular emissions show the most negative values around - 29 ‰, emissions from combustion of the most common wood types are more enriched with values around -26 to -27 ‰, and coal burning is around -25‰. For source samples, d13C values at the three desorption temperature steps usually do not differ more than 1 ‰.

In the ambient samples, OC had more negative δ13C values in summer than in winter, which can be explained by the contribution of biomass/coal burning sources in winter. At the urban site δ13C of OC did not change much with increasing desorption temperature in winter, which is typical for primary sources. In the summer δ13C of OC was clearly more negative for lower desorption temperatures at all three sites. This is likely due to the influence of secondary organic aerosol formation in summer, which should have depleted (more negative) isotopic signature and contributes strongly to the more volatile fraction.A higher fraction of more refractory OC in summer compared to winter-time suggests active photochemical processing of the primary organic aerosol as an important process at all three sites.

This is consistent with our laboratory studies, where we age source samples in a small reactor under UV light. Photolysis causes mainly mass loss in OC that desorbs at 200 °C. At the same time, 13C becomes more enriched in OC desorbed at the higher temperature steps, leading to a bigger difference in d13C between OC200 and OC350, as observed in the ambient atmosphere.

In summary, analyzing stable isotopes of OC at different desorption temperature steps gives a powerful tool for diagnosing aging processes.

How to cite: Dusek, U., Masalaite, A., Yao, P., van Ettinger, N., Remeikis, V., and Paul, D.: Seasonal changes of sources, volatility, and aging of organic aerosols in eastern Europe reflected in the stable isotopic composition, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16841, https://doi.org/10.5194/egusphere-egu23-16841, 2023.

EGU23-396 | ECS | Orals | AS3.2

Closure and parameterization of sub-micron aerosols’ hygroscopicity and it’s seasonal variability over the Western Ghats, India 

Avishek Ray, Govindan Pandithurai, Subrata Mukherjee, Anil V Kumar, and Anupam Hazra

Hygroscopicity of atmospheric aerosol primarily depends on the size and chemical composition of the particle and is important for estimating anthropogenic aerosol radiative forcing. Hygroscopicity is highly related to the activation of aerosols to Cloud Condensation Nuclei (CCN), and hence plays a crucial role in cloud formation and modulating its properties. However, due to limitations of measurement techniques, seasonal variation in size segregated aerosol hygroscopicity (k) is not available over the Indian region.  This study presents ‘k’ as derived from a Humidified Tandem Differential Mobility Analyzer (HTDMA) over the High Altitude Cloud Physics Laboratory (HACPL) in the Western Ghats, India for more than a year (from May 2019 to May 2020).  The average hygroscopicity values of aerosol particles of diameters 32, 50, 75, 110, 150, 210, and 260 nm at 90% RH conditions are 0.189, 0.177, 0.163, 0.170, 0.183, 0.199, 0.207 respectively during the entire observation period.  k was observed to decrease with an increase in size in the Aitken mode regime (32-75 nm) and an increase in the accumulation mode (110-260 nm).  Seasonal variation of hygroscopicity for a wide range of particle diameters is reported which is highly demanding as there is a change in the air mass flow pattern in each of the seasons.  The diurnal cycle of hygroscopicity showed a prominent peak during the midnight to early morning hours followed by a decrease in the forenoon hours and a secondary peak in the afternoon hours.  k is found to be higher in pre-monsoon as compared to the winter season as Chl is approximately 3% higher in pre-monsoon and NH4Cl is highly hygroscopic among the assumed chemical composition.  Assuming the internal and external mixing of aerosols, the closure study yields chemically derived hygroscopicity (kchem) overestimates as compared to kHTDMA though the assumption of external mixing of aerosols improved the values of predicted k. CCN derived hygroscopicity (kccn) underestimates as compared to hygroscopicity derived from HTDMA measurements. Both kchem and kccn are found to follow the similar diurnal variation of kHTDMA. Thus, the kchem and   can be used as a proxy of  in the absence of direct HTDMA measurements. Using kchem and  in numerical models will propagate systematic bias in aerosol to CCN activation processes so a parameterization of hygroscopicity with dry diameter of sub-micron particles is developed and that could be used for a closer real-atmospheric value of hygroscopicity.

Keywords: Hygroscopicity, Parameterization, sub-micron aerosols

How to cite: Ray, A., Pandithurai, G., Mukherjee, S., Kumar, A. V., and Hazra, A.: Closure and parameterization of sub-micron aerosols’ hygroscopicity and it’s seasonal variability over the Western Ghats, India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-396, https://doi.org/10.5194/egusphere-egu23-396, 2023.

EGU23-462 | ECS | Orals | AS3.2

Simulation chamber study of the spectral mass absorption, scattering, and extinction cross-sections (MAC, MSC, MEC) of fresh and aged combustion aerosols 

Johannes Heuser, Claudia Di Biagio, Laura Renzi, Angela Marinoni, Jermone Yon, Marco Zanatta, Chenjie Yu, Antonin Bergé, Mathieu Cazaunau, Servanne Chevaillier, Paolo Laj, Dario Massabo, Gael Noyalet, Eduoard Pangui, Paolo Prati, Brice Temime-Roussell, Roberta Vecchi, Vera Bernardoni, Virginia Vernocchi, and Jean-Francois Doussin

Carbonaceous soot particles are formed during incomplete combustion of fossil fuels, biofuels or biomass and are considered to be a significant proportion of aerosol emission, especially in polluted areas, and to contain light-absorbing carbon fractions. The light-absorbing carbon components make these particles exhibit positive radiative forcing and thus they contribute to atmospheric warming processes. The exact contribution to this process however still has significant uncertainties. One of the sources of uncertainty is related to the capacity to accurately describe soot spectral optical properties (MAC/MSC/MEC - mass absorption/scattering/extinction cross-sections in m2g-1; CRI - complex refractive index), due to significant uncertainties for key measurements like the absorption coefficient or absorbing mass fraction. A second source is considered to be the change of the optical properties with the variable physico-chemical state of soot (e.g. chemical composition, morphology, primary particle size, aggregate size distribution, coating and mixing state) which depends on (i) the combustion conditions/sources  and is (ii) known to change during atmospheric lifetime due to ageing and mixing processes.

The present work aims at providing new measurements of soot spectral optical properties and investigating their dependence on particles’ physico-chemical state and the role of measurement uncertainties. For this, a set of original experiments was performed in the 4.3m3 CESAM atmospheric simulation chamber (https://cesam.cnrs.fr/) on soot aerosols generated by a commercial propane diffusion flame soot generator (miniCAST model 6204 TYPE C, JING). In these experiments, the variability of soot properties due to (i) generation and (ii) atmospheric ageing was explored. Different combustion conditions going from fuel–leaner to fuel-richer were set to produce soot aerosol with different effective densities, EC/TC-ratios ranging from 0.8 ± 0.1 to 0.0 ± 0.1 and size distributions with median diameters between 30 and 120 nm. Selected aerosols were subjected to ageing in a N2/O2 atmosphere under simulated atmospheric conditions (humid, with/without illumination, up to 26 hours lifetime). In these conditions, physical and chemical ageing, under the presence of different gaseous phases (O3, SO2) and addition of a second aerosol phase produced by photo-oxidation of SO2 or the ozonolysis of α-pinene, led to changes in the physico-chemical properties of the soot.

State-of-the-art techniques were used to generate an extensive dataset of physico-chemical parameters (mass concentration, morphology, effective density, composition, size distribution) and spectral optical properties (absorption, scattering, extinction coefficients) for different soot aerosols and different ageing states of these. The absorption coefficient in particular was measured by both filter-based (AE - Aethalometer, MAAP - Multi-Angle Absorption Photometer, MWAA – Multi-Wavelength Absorbance Analyzer, PP_UniMI - Polar Photometer by University of Milano) and extinction minus scattering techniques. The MAC, MSC and MEC datasets, retrieved by combining these measurements, will be presented for the ensemble of chamber experiments and the variability of these parameters in link with variations in the particles’ physico-chemical properties will be discussed together with key relevant uncertainties.

How to cite: Heuser, J., Di Biagio, C., Renzi, L., Marinoni, A., Yon, J., Zanatta, M., Yu, C., Bergé, A., Cazaunau, M., Chevaillier, S., Laj, P., Massabo, D., Noyalet, G., Pangui, E., Prati, P., Temime-Roussell, B., Vecchi, R., Bernardoni, V., Vernocchi, V., and Doussin, J.-F.: Simulation chamber study of the spectral mass absorption, scattering, and extinction cross-sections (MAC, MSC, MEC) of fresh and aged combustion aerosols, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-462, https://doi.org/10.5194/egusphere-egu23-462, 2023.

EGU23-465 | ECS | Posters on site | AS3.2

New observations of climate-relevant properties of atmospheric aerosols in Namibia, southern Africa. 

François Hemeret, Paola Formenti, Claudia Di-Biagio, Brigitte Language, Servanne Chevaillier, Anaïs Féron, Mathieu Cazaunau, Raquel Torres-Sánchez, Stuart Piketh, François Engelbrecht, Raeesa Moolla, Ulrich Bezuidenhoudt, Brendan Luyanda, Eugene Marais, and Gillian Maggs-Kölling

Southern Africa, and in particular its western part, Namibia, is considered a climate change hotspot by the IPCC and is at risk of severe temperature-related changes. As examples, models projections suggest by the end of the century: 1) Increase of surface temperature of +4 to +7°C; 2) destruction of the stratocumulus cloud deck along the western coast; and 3) decrease of the fog inland. The role of aerosols in this context is still not completely quantified, due to their high spatial and temporal variability, the many sources responsible for the complex mixture and the lack of continuous observations. Most of the past regional climate modelling (RCM) and intensive field campaigns focussed primarily on constraining the radiative effects of the seasonal biomass burning aerosols generally occurring in the end of the austral winter (August to October). However, the aerosol spectral optical properties, aerosol optical depth and the organic fractions are not studied enough to provide a firm understanding of regional aerosol load, interaction with radiation and interplays in relation to particle chemistry.

In this work, we present the first analysis of new long-term ground-based aerosol observations conducted since april 2022 at Gobabeb Namib Research Institue (23°33’40‘’S, 15°02’24’’E) in Namibia. Gobabeb is located in the hyperarid Namib desert and it is under the influence of different air masses, transporting maritime and biomass burning aerosols, amongst others. The measurements of optical and physical properties of the aerosol mixtures are analysed to provide with the aerosol single scattering albedo and mass absorption, scattering and extinction efficiencies which are needed to evaluate the first Africa-based Earth system model by the Global Change Institute at the University of Witwatersrand in South Africa. The in situ surface data are complemented by the analysis of pre-existing observations such as those from the AERONET sunphotometers.

How to cite: Hemeret, F., Formenti, P., Di-Biagio, C., Language, B., Chevaillier, S., Féron, A., Cazaunau, M., Torres-Sánchez, R., Piketh, S., Engelbrecht, F., Moolla, R., Bezuidenhoudt, U., Luyanda, B., Marais, E., and Maggs-Kölling, G.: New observations of climate-relevant properties of atmospheric aerosols in Namibia, southern Africa., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-465, https://doi.org/10.5194/egusphere-egu23-465, 2023.

EGU23-909 | ECS | Orals | AS3.2 | Highlight

A Geostationary View of a Liquid water Path Adjustment dependence on Cloud Regime 

Kevin Smalley and Mathew Lebsock

Aerosol-cloud-interactions remain a large climate uncertainty; especially uncertain is the liquid water path (LWP) adjustment to varying aerosol concentrations in stratocumulus (StCu). Large-eddy simulations (LES) have found that the LWP response of StCu to aerosol can be either positive or negative depending on the cloud regime, whereas climate models simulate uniformly positive correlations. Observations of the real-world evolution of LWP in varying aerosol environments are needed to resolve the nature of the correlation between LWP and aerosol. We address this by analyzing a large ensemble of parcel trajectories over the southeast Pacific within the GOES-16 field of regard. Preliminary results are consistent with LES, showing consistent regime dependent evolution of the LWP depending on the initial cloud state, with LWP generally decreasing with varying number concentrations (N). However, LWP generally increases at low N, potentially supporting LES conclusions showing a cloud-regime dependence. To investigate this further, we will further condition observations by MERRA-2 large-scale environmental variables (e.g. estimated inversion strength, moisture, and boundary-layer decoupling). We expect environmental differences will correlate with the differences between changes in LWP at low and high N.

How to cite: Smalley, K. and Lebsock, M.: A Geostationary View of a Liquid water Path Adjustment dependence on Cloud Regime, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-909, https://doi.org/10.5194/egusphere-egu23-909, 2023.

EGU23-1413 | ECS | Posters on site | AS3.2 | Highlight

Understanding sources of contrail cirrus radiative forcing uncertainty using a new diagnostic contrail scheme for the UK Earth System Model 

Weiyu Zhang, Alexandru Rap, Kwinten Van Weverberg, Kalli Furtado, Wuhu Feng, Cyril Morcrette, Piers Forster, and Timmy Francis

Condensation trails (contrails) are aircraft-induced line-shaped high clouds, which may persist and grow to form contrail cirrus in ice supersaturated regions. Contrail cirrus is the largest known component of aviation radiative forcing, with a large uncertainty associated with troposphere water budgets and contrail radiative properties. In addition, due to the limited number of climate models able to simulate contrail cirrus, the uncertainty in the global contrail cirrus radiative forcing cannot be estimated statistically.

The aim of this work is to implement a contrail cirrus parameterisation in the UK Earth System Model, therefore providing a new independent estimate of the contrail cirrus radiative forcing to be used in future assessments of aviation climate impacts. The new diagnostic scheme is based on the processes governing contrail formation (Schmidt-Appleman Criteria) and persistence (ice supersaturation). Persistent contrails are then added to the model cloud fields, where they interact with and evolve alongside natural clouds.

We use ensemble runs of both nudged and free running model experiments to estimate the contrail cirrus cover and effective radiative forcing. Comparisons with a similar contrail scheme implemented in the NCAR Community Atmospheric Model (CAM) indicate the importance of the host climate model via (i) the host’s cloud microphysics scheme (e.g. single vs. double moment) and (ii) its ability to simulate realistic ice supersaturated regions. By providing a new independent assessment of the contrail cirrus radiative forcing, our work contributes to improving our understanding of aviation climate impacts and therefore potential mitigation strategies for current and future generation aircraft. 

How to cite: Zhang, W., Rap, A., Van Weverberg, K., Furtado, K., Feng, W., Morcrette, C., Forster, P., and Francis, T.: Understanding sources of contrail cirrus radiative forcing uncertainty using a new diagnostic contrail scheme for the UK Earth System Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1413, https://doi.org/10.5194/egusphere-egu23-1413, 2023.

EGU23-1440 | ECS | Orals | AS3.2 | Highlight

Simplifying cloud microphysical process representation to reduce climate model complexity 

Ulrike Proske, Sylvaine Ferrachat, and Ulrike Lohmann

Earth's climate system is complex. Thus, trying to represent this system as the sum of its parts, climate models have grown increasingly complex as well (Shackley et al., 1998). However, this makes the model results and behaviour difficult to interpret, and increases simulations' computational costs.

Building onto Proske et al. (2022), who demonstrated the potential for simplification in the two moment cloud microphysics (CMP) scheme of the global aerosol climate model ECHAM-HAM, we implement such simplifications for the CMP and activation scheme in ECHAM-HAM. For the CMP the sensitivity of the model to a specific process determines whether it is simplifiable. For example, heterogeneous freezing and secondary ice production in their present implementation can be removed without strong deviations in results. Replacing the sublimation and self-collection of ice with a constant rate, or replacing melting of ice crystals with a climatology has similarly small effects. The deviations that simplifications of other processes such as riming produce are larger, but all simplifications are robust to changing climate states.
For aerosol activation into cloud condensation nuclei, using a climatology of CCN diagnosed from a previous run gives satisfactory results. From the perspective of the CMP this simplification eliminates the need for the whole aerosol module HAM, associated with large computational time savings (for aerosol optical effects, the representation of at least anthropogenic aerosols with a simplified climatology has already been demonstrated successfully (Stevens et al., 2017)).

Of course, the value of simplifications and the evaluation standard for their results depends on one's modelling purpose (Parker, 2009). However, our results show that ECHAM-HAM contains redundancy in model detail and thus question the value of complexity in model representation as a normative principle (Shackley et al., 1998).

 

 


Parker, W. S. “Confirmation and Adequacy-for-Purpose in Climate Modelling.” Aristot. Soc. Suppl. Vol. 83, no. 1 (2009): 233–49. https://doi.org/10.1111/j.1467-8349.2009.00180.x.

Proske, U., S. Ferrachat, D. Neubauer, M. Staab, and U. Lohmann. “Assessing the Potential for Simplification in Global Climate Model Cloud Microphysics.” Atmos. Chem. Phys. 22, no. 7 (April 12, 2022): 4737–62. https://doi.org/10.5194/acp-22-4737-2022.

Shackley, S., P. Young, S. Parkinson, and B. Wynne. “Uncertainty, Complexity and Concepts of Good Science in Climate Change Modelling: Are GCMs the Best Tools?” Clim. Change 38, no. 2 (1998): 159–205. https://doi.org/10.1023/A:1005310109968.

Stevens, B., S. Fiedler, S. Kinne, K. Peters, S. Rast, J. Müsse, S. J. Smith, and T. Mauritsen. “MACv2-SP: A Parameterization of Anthropogenic Aerosol Optical Properties and an Associated Twomey Effect for Use in CMIP6.” Geosci. Model Dev. 10, no. 1 (2017): 433–52. https://doi.org/10.5194/gmd-10-433-2017.

How to cite: Proske, U., Ferrachat, S., and Lohmann, U.: Simplifying cloud microphysical process representation to reduce climate model complexity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1440, https://doi.org/10.5194/egusphere-egu23-1440, 2023.

EGU23-1448 | ECS | Orals | AS3.2 | Highlight

Past trends in Australian rainfall: internally generated or human-caused? 

Nora Fahrenbach, Massimo Bollasina, Bjorn Samset, Tim Cowan, and Annica Ekman

The expectations of the public and policymakers for accurate climate projections have grown with improvements in climate models. Internal variability, however, poses an inherent limit on climate predictability and, thus, accurate future climate projections of temperature and precipitation. This challenge is further amplified at a regional scale where internal variability can even dominate over forced anthropogenic climate change.

 

In this study, we focused on the contribution of decadal climate variability and anthropogenic forcing (greenhouse gases and aerosols) on past precipitation changes over Australia since the 1970s. Using observational data, we find that the variance explained on decadal to multi-decadal timescales is comparable to that on sub-decadal scales across Australia, underlining the importance of examining Australian trends in the context of variability. While decadal and longer precipitation trends over Australia’s east coast are dominated by internal variability, significant drying trends in the austral winter (June to August) over southwest Western Australia and wettening trends in summer (December to February) over northwest Australia are evident. We further disentangle the influence of internal variability from that of different anthropogenic forcing agents on these trends using simulations from the CESM2 Large Ensemble and idealised anthropogenic aerosol simulations from PDRMIP (Precipitation Driver Response Model Intercomparison Project). Our findings provide additional evidence for the significant role of internal variability on regional climate change and also underline the importance of a focused dialogue between scientists, policymakers and the public to ensure realistic expectations for regional future climate projections.

How to cite: Fahrenbach, N., Bollasina, M., Samset, B., Cowan, T., and Ekman, A.: Past trends in Australian rainfall: internally generated or human-caused?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1448, https://doi.org/10.5194/egusphere-egu23-1448, 2023.

EGU23-1699 | ECS | Orals | AS3.2 | Highlight

Assessing effective radiative forcing from aerosol-cloud interactions over the global ocean 

Casey Wall, Joel Norris, Anna Possner, Daniel McCoy, Isabel McCoy, and Nicholas Lutsko

How clouds respond to anthropogenic sulfate aerosols is one of the largest sources of uncertainty in the radiative forcing of climate over the industrial era. This uncertainty limits our ability to predict equilibrium climate sensitivity (ECS) – the equilibrium global warming following a doubling of atmospheric CO2. Here we use satellite observations to quantify relationships between sulfate aerosols and low-level clouds while carefully controlling for meteorology. We then combine the relationships with estimates of the change in sulfate concentration since about 1850 to constrain the associated radiative forcing. We estimate that the cloud-mediated radiative forcing from anthropogenic sulfate aerosols is −1.11 ± 0.43 W m-2 over the global ocean (95% confidence). This constraint implies that ECS is likely between 2.9 and 4.5 K (66% confidence). Our results indicate that aerosol forcing is less uncertain and ECS is probably larger than the ranges proposed by recent climate assessments.

How to cite: Wall, C., Norris, J., Possner, A., McCoy, D., McCoy, I., and Lutsko, N.: Assessing effective radiative forcing from aerosol-cloud interactions over the global ocean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1699, https://doi.org/10.5194/egusphere-egu23-1699, 2023.

EGU23-1907 | ECS | Orals | AS3.2

A causal approach to disentangle fast and slow stratocumulus adjustments to aerosol perturbations 

Emilie Fons, Jakob Runge, David Neubauer, and Ulrike Lohmann

A large part of the uncertainty around future global warming is due to the cooling effect of aerosol-liquid cloud interactions, and in particular to the elusive sign of liquid water path (LWP) adjustments to aerosol perturbations. We quantify this adjustment with a novel causal approach that combines physical knowledge in the form of a causal graph with geostationary satellite observations of stratocumulus clouds. This allows us to remove confounding from large-scale meteorology and to disentangle counteracting physical processes such as cloud-top entrainment enhancement and precipitation suppression due to aerosol perturbations. The resulting LWP adjustment is time-dependent, with positive initial values due to fast precipitation suppression and negative values after entrainment enhancement has fully developed. We also use the causal framework as a diagnosis tool to detect potential issues with precipitation retrievals, which might cause precipitation-related influences on the LWP to be underestimated. These results suggest that time-aware causal analyses are key to reconcile conflicting studies concerning the sign of LWP adjustments across different data sources.

How to cite: Fons, E., Runge, J., Neubauer, D., and Lohmann, U.: A causal approach to disentangle fast and slow stratocumulus adjustments to aerosol perturbations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1907, https://doi.org/10.5194/egusphere-egu23-1907, 2023.

EGU23-1946 | Posters virtual | AS3.2

A study on morphology and microphysics of clouds during southwest monsoon over Western Ghats, India, using multi-platform observations 

Parakkatt Parambil Leena, Mercy Varghese, Jithin .S.Kumar, Vasudevan Anil Kumar, Govindan Pandithurai, Rohit .D.Patil, Eruthiparambil Ayyappan Resmi, and Thara .V.Prabha

Clouds play a significant role in the dynamics and thermodynamics of the atmosphere. To understand the impact of clouds on climate and for better representation of these in the global models, accurate information about the temporal, spatial and vertical distribution of cloud properties such as microphysical, morphological and types are essential. In the present work, vertical structure and microphysics of clouds during southwest (SW) monsoon has been studied from a high altitude site (Mahabaleshwar (17.92°N, 73.66°E, and 1348 m above mean sea level (MSL)) and within ± 0.1 degrees) over Western Ghats, India. Vertical structure of the clouds has been detailed using radiosonde observations. Warm cloud microphysics was investigated using in-situ ground and aircraft cloud measurements. Radiosonde profiles showed the presence of single and multi-layered clouds over the observational site. Higher occurrence frequency for cloud layers below 2 km and above 6 km altitude compared to mid-level clouds (2 to 6 km) during SW monsoon were noticed. Higher occurrences of single layer clouds during June and September (transition period) were noticed whereas frequency of two-layer was higher in July and August (core period). Low (~30%) and high-level (~60%) clouds were dominantly seen compared to mid-level clouds over the observational site during SW monsoon. Warm cloud microphysics was investigated using collocated ground and airborne in situ measurements. Cloud microphysical properties such as cloud droplet number concentration (CDNC), liquid water content (LWC), droplet effective diameter (ED), droplet mean radius (Rm) respectively were analyzed. The cloud liquid water content and the effective droplet diameter showed increase with altitude. Analyzed cloud droplet size distribution (DSD) showed a steep decrease in number concentration of droplets above 25 µm diameters at altitudes above 1800 m, suggesting active collision-coalescence. This is the first such report combining in situ observations from two different platforms to study the vertical structure of monsoon clouds over a complex terrain like the Western Ghats in India.  

How to cite: Leena, P. P., Varghese, M., .S.Kumar, J., Kumar, V. A., Pandithurai, G., .D.Patil, R., Resmi, E. A., and .V.Prabha, T.: A study on morphology and microphysics of clouds during southwest monsoon over Western Ghats, India, using multi-platform observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1946, https://doi.org/10.5194/egusphere-egu23-1946, 2023.

EGU23-2082 | ECS | Posters on site | AS3.2

A reduced complexity aerosol model for km-scale climate models 

Philipp Weiss, Ross Herbert, and Philip Stier

Despite their small size, aerosols strongly influence Earth's climate. Aerosols scatter and absorb radiation referred to as aerosol-radiation interactions but also modify the properties of clouds, as cloud droplets form on aerosol particles, referred to as aerosol-cloud interactions. Kilometer-scale simulations allow us to examine long-standing questions related to these interactions. Such simulations resolve atmospheric motions on scales of a few kilometers and represent important atmospheric processes like convective updrafts that were parameterized previously. Regional simulations revealed significant effects of aerosols on convective clouds and provided insights into the underlying processes and drivers. 

To examine these interactions with the climate model ICON, we developed the simple aerosol model HAMlite based on and fully traceable to the complex aerosol model HAM. HAMlite represents aerosols as an ensemble of log-normal modes. To reduce the computational and physical complexity, aerosol microphysics are discarded and aerosol sizes and compositions are prescribed. The selection of modes is flexible and can include the Aitken, accumulation, and coarse modes. The calculation of aerosol properties and thermodynamics remains fully consistent with HAM. HAMlite is linked to the atmospheric processes of ICON. Aerosols are transported as tracers in the dynamical core and coupled to the radiation, turbulence, and cloud microphysics schemes.

We present first results from global simulations with ICON-HAMlite. The atmosphere is governed by non-hydrostatic conservation equations, the land is represented with the dynamic vegetation model JSBACH, and the sea surface temperature and sea ice are prescribed with the AMIP database. The horizontal resolution is about 5 km and time period is about 40 days. First, we evaluate the global distributions of the different aerosol modes. And second, we investigate how aerosols influence the diurnal cycle and deep convection in the tropics. In contrast to regional simulations, global simulations include the large-scale circulation and in particular the budgetary constraints on precipitation due to the conservation of water and energy.

How to cite: Weiss, P., Herbert, R., and Stier, P.: A reduced complexity aerosol model for km-scale climate models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2082, https://doi.org/10.5194/egusphere-egu23-2082, 2023.

EGU23-2345 | ECS | Orals | AS3.2

By how much can co-condensation of semi-volatile compounds alter clouds? 

Yu Wang, David Neubauer, Ying Chen, Pengfei Liu, Beiping Luo, Ulrike Proske, Sylvaine Ferrachat, Claudia Marcolli, and Ulrike Lohmann

Semi-volatile compounds (organics, nitrate, chloride) are ubiquitous in atmospheric aerosols and usually contribute over 50 % to particulate matter worldwide (Jimenez et al., 2009). Co-condensation of semi-volatiles and water vapour can enhance aerosol particle growth and facilitate their activation to cloud droplets, affecting cloud properties and thus the Earth's radiation balance.

Yet, the effect of co-condensation on aerosol hygroscopic growth is not well constrained as the loss of semi-volatiles during drying and heating in traditional aerosol sampling devices (e.g., by HTDMA, CCN counter) is poorly understood. Here, we developed a novel method to derive aerosol hygroscopic growth by considering the co-condensation effect, from open-access data including visibility, PM2.5 mass concentration and meteorological parameters (Wang and Chen, 2019). By applying our visibility method and thermodynamic modelling in Delhi (India), we found that the co-condensation of HCl with water vapour can largely enhance aerosol hygroscopicity by doubling the light extinction coefficient of wetted particles and halving the critical supersaturation needed for cloud droplet activation (as shown in Fig. 1 a-b, Gunthe et al., 2021). Our recent results showed that the co-condensation effect in Chinese megacities (Beijing, Guangzhou, and Shanghai) is as significant as in Delhi, but acts via co-condensation of HNO3.

The next question is how significant the co-condensation effect is globally and how much it can alter clouds and the radiation balance. Here, we combine novel field observation, a cloud parcel model, and an aerosol-climate model to disentangle this question. The particle and gas composition, particle size distribution, and air parcel cooling rate are essential factors for the co-condensation effect in a rising air parcel.

Our preliminary sensitivity study (doubling hygroscopicity) in a climate model showed that the co-condensation effect plays only a minor role in clouds formation globally, but significantly increases cloud droplet number concentration and liquid cloud cover in regions with large anthropogenic emissions, e.g. East/Southeast Asia, India, Europe, East US. Consistently, parcel model calculations confirm that for a given cooling rate, co-condensation increases the number of activated cloud nuclei. Our study will help to develop a parameterization for aerosol-climate models to include the co-condensation effect on cloud formation.

References

Gunthe, S. S., et al. (2021), Enhanced aerosol particle growth sustained by high continental chlorine emission in India, Nature Geoscience.

Jimenez, J. L., et al. (2009), Evolution of Organic Aerosols in the Atmosphere, Science, 326(5959), 1525-1529.

Wang, Y., and Y. Chen (2019), Significant Climate Impact of Highly Hygroscopic Atmospheric Aerosols in Delhi, India, Geophysical Research Letters, 46(10), 5535-5545.

How to cite: Wang, Y., Neubauer, D., Chen, Y., Liu, P., Luo, B., Proske, U., Ferrachat, S., Marcolli, C., and Lohmann, U.: By how much can co-condensation of semi-volatile compounds alter clouds?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2345, https://doi.org/10.5194/egusphere-egu23-2345, 2023.

Global warming potential (GWP) has been used as an indicator to compare with the greenhouse effect of different gases. Utilized gases, especially, in semiconductor and display manufacturing processes are greenhouse gas with high GWP values. Accordingly, countries and relevant companies are trying to synthesize the alternative gases expressed with low GWP values along with a lot of interest. But GWP values of these hasn’t been presented at any other thesis. Hence it is inevitable to measure GWP of newly gases to compare with climate effect between conventionally used gases and newly gases.

Therefore, this study proposes a measurement method of GWP based on various papers using instrument such as fourier-transform infrared spectroscopy (FT-IR), time of flight- mass spectroscopy (TOF-MS) equipped with the proton transfer reaction (PTR) as a detector and so on. Equation is used in IPCC fifth assessment report to calculate the GWP.

  • Calculating absorbed cross-sectional area by measuring infrared absorption spectra using FT-IR and by applying to lambert-beer’s law
  • Applying original pinnock curve (Pinnock et al., 1995) and final pinnock curve using the line-by-line model (Myhre et al., 2006) to calculate the radiative forcing by integrating the calculated absorbed cross-sectional area from first step
  • Measuring the rate constant when they react with the hydroxyl radical using PTR-MS equipped with the PTR and calculating the atmospheric lifetime based on the constant and tropospheric lifetime of CH3CCl3 as a reference material proposed by WMO (2014)
  • In accordance with the IPCC fifth assessment report (2013), calculating GWP using the radiative forcing and atmospheric lifetime induced by second and third step, respectively

Acknowledgment:

This work was supported by Korea Environment Industry & Technology Institute (KEITI) through Climate Change R&D Project for New Climate Regime Program, funded by Korea Ministry of Environment (MOE) ( 2022003560008 ).

How to cite: Lee, B. J. and Park, S. H.: The measurement method of global warming potential based on the infrared absorption spectra and rate constant with the hydroxyl radical, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2489, https://doi.org/10.5194/egusphere-egu23-2489, 2023.

EGU23-2490 | ECS | Posters on site | AS3.2

Black carbon-climate interactions regulate dust burdens over India revealed during COVID-19 

Linyi Wei, Yong Wang, Zheng Lu, and Xiaohong Liu

India as a hotspot for air pollution has heavy black carbon (BC) and dust (DU) loadings. BC has been identified to significantly impact the Indian climate. However, whether BC-climate interactions regulate Indian DU during the premonsoon season is unclear. Here, using long-term Reanalysis data, we show that Indian DU is positively correlated to northern Indian BC while negatively correlated to southern Indian BC. We further identify the mechanism of BC-dust-climate interactions revealed during COVID-19. BC reduction in northern India due to lockdown decreases solar heating in the atmosphere and increases surface albedo of the Tibetan Plateau (TP), inducing a descending atmospheric motion. Colder air from the TP together with warmer southern Indian air heated by biomass burning BC results in easterly wind anomalies, which reduces dust transport from the Middle East and Sahara and local dust emissions. The premonsoon aerosol-climate interactions delay the outbreak of the subsequent Indian summer monsoon.

How to cite: Wei, L., Wang, Y., Lu, Z., and Liu, X.: Black carbon-climate interactions regulate dust burdens over India revealed during COVID-19, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2490, https://doi.org/10.5194/egusphere-egu23-2490, 2023.

EGU23-2765 | Orals | AS3.2

Cloud and aerosol observations from DSCOVR satellite 

Alexander Marshak

Earth sensors NIST Advanced Radiometer (NISTAR) and Earth Polychromatic Imaging Camera (EPIC) of the Deep Space Climate Observatory (DSCOVR) measure outgoing radiative fluxes of the entire sunlit Earth and key spectral characteristics at 10 km resolution, respectively.  The unique near backscatter angular perspective of DSCOVR is used to measure ozone, sulfur dioxide, aerosols, clouds, ocean surface photosynthetically available radiation (PAR), vegetation, sun glints, and to obtain UV radiation estimates.  In the presentation I will focus on clouds and aerosol EPIC products: cloud mask, cloud height and optical thickness, aerosol optical depth and aerosol height, single scattering albedo, their correlation and daytime variability.

How to cite: Marshak, A.: Cloud and aerosol observations from DSCOVR satellite, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2765, https://doi.org/10.5194/egusphere-egu23-2765, 2023.

EGU23-3152 | Orals | AS3.2 | Highlight

Near-term precipitation change highly sensitive to black carbon emissions 

Bjorn H. Samset, Laura J. Wilcox, Marianne T. Lund, Carley Iles, Camilla W. Stjern, and Kalle Nordling
Changes in mean and extreme precipitation are arguably the most impactful aspects of climate change. Detailed and accurate projections are therefore crucial for climate risk assessments and adaptation strategies. Generally, global mean precipitation increases with surface warming, with a global mean hydrological sensitivty of around 1 to 2 %/K, and stronger increases in rates or extreme precipitation events. Local variations are however very large, and model projections are much more uncertain than for temperature. 
 
Absorbing aerosols, notably black carbon (BC), brown carbon (BrC) and mineral dust, are an exception to the rule. Their absorption of shortwave radiation inhibits precipitation formation, through rapid adjstments that overwhelm their influence on surface temperature. The hydrological sensitivty to black carbon emissions is therefore around -4 %/K, again with large regional variations, and with a very high spread between models ( -1 to -7 %/K)
 
In this talk, we discuss the near-term (2015-2045) dependence of precipitation change on the evolution of absorbing aerosols. We show the transient hydrological sensitivty in CMIP6, globally and regionally, and how it is affected by air quality policy (i.e. scenario choice) and model treatment of BC, BrC and dust. We confirm that, globally, while black carbon emissions have a modest impact on surface temperature, their influence on precipitation is outsized, causing a factor of 2 difference in hydrological sensitivty beween future scenarios with strict (SSP126) and weak (SSP370) air quality control measures. 
 
Further, for highly populated regions close to, or downwind from, major emission sources - notably India, China and northern Brazil - we find very high sensitivity of precipitation evolution to the levels of absorbing aerosol emissions. Several of these regions are therefore set for a "double whammy" of precipitation increase from global warming and a removal of short wave absorbing air pollution. We also discuss the rates of change of extreme precipitation events, and how they relate to absorbing aerosols in different regions. 
 
Our key message is that changes in absorbing aerosols over the coming decades is a key uncertainty in near term precipitation and extreme event evolution, and therefore a burning knowledge gap for the aerosol-climate community. 

How to cite: Samset, B. H., Wilcox, L. J., Lund, M. T., Iles, C., Stjern, C. W., and Nordling, K.: Near-term precipitation change highly sensitive to black carbon emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3152, https://doi.org/10.5194/egusphere-egu23-3152, 2023.

EGU23-3557 | ECS | Orals | AS3.2

Model simulation of the aerosol perturbation on the Tibetan Plateau convective precipitation 

Mengjiao Jiang, Yaoting Li, Weiji Hu, Yinshan Yang, and Guy Brasseur

The Tibetan Plateau (TP) is important for weather and climate. Relatively clean aerosol conditions over the Plateau makes the study on the aerosol-cloud-precipitation interactions in this region distinctive. A convective event with precipitation observed on 24 July 2014 in Naqu was selected to explore the influence of aerosols on the onset and intensity of precipitation. We use the Modern-Era Retrospective analysis for Research and Applications Version 2 (MERRA-2) reanalysis to derive the cloud condensation nuclei (CCN), which can be regarded as the real-time background. These values are adopted to initialize the regional WRF 4.0 meteorological model and to simulate the onset of convective events and the formation of precipitation. Four sets of experiments were adopted for our simulations. A detailed analysis of microphysical processes shows that, with the increase in the aerosol number concentration, the conversion rate of cloud water to rain in clouds is enhanced at first. Under polluted situation, the conversion process of cloud water to rain is suppressed; however, the transformation of cloud water to graupel and the development of convective clouds are favored. As a result, the onset of the precipitation is delayed and cold-rain intensity increases.

How to cite: Jiang, M., Li, Y., Hu, W., Yang, Y., and Brasseur, G.: Model simulation of the aerosol perturbation on the Tibetan Plateau convective precipitation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3557, https://doi.org/10.5194/egusphere-egu23-3557, 2023.

EGU23-3816 | ECS | Orals | AS3.2

Influence of mixed air pollution on surface micro-meteorological characteristics in autumn and winter in Nanjing area 

Jiaze Wang, Xiaolu Ling, Xinsheng Zhu, Weidong Guo, Jun Zou, and Jianning Sun

Abstract: This work used the Multi-element observation data from the Station for Observing Regional Processes of the Earth System (SORPES) from November 27 to December 3, 2018. It quantitatively analyzed the influence of mixed air pollution conditions on the surface micrometeorological elements and energy balance characteristics under the combined effects of long-distance sand and dust and local emission pollution. On this basis, the response characteristics of surface meteorological elements and energy distribution under different pollution conditions in autumn and winter in Nanjing are compared by synthetic analysis. The results showed that the daytime temperature on polluted days was about 1°C lower than that on clean days, and the night temperature was about 2°C higher. Both downward/upward shortwave radiation flux decreased on polluted days, and the long-wave radiation flux at night increased. On clean days, the net radiation budget during the day was 45.6% higher than that of polluted days and the surface sensible heat flux was 75.5% higher than that of polluted days. The average Bowen ratio at night on polluted days was higher than that on clean days, indicating that the nighttime sensible heat exchange was stronger. The results help to deeply understand the influence process and mechanism of air pollution from different sources and different properties on surface energy balance and local meteorological elements in the urban agglomerations of the Yangtze River Delta, and the results also provide a verification basis for the interaction between air pollution and meteorological conditions, air quality prediction and corresponding countermeasures.

How to cite: Wang, J., Ling, X., Zhu, X., Guo, W., Zou, J., and Sun, J.: Influence of mixed air pollution on surface micro-meteorological characteristics in autumn and winter in Nanjing area, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3816, https://doi.org/10.5194/egusphere-egu23-3816, 2023.

EGU23-4129 | ECS | Orals | AS3.2

Anthropogenic aerosols turn liquid cloud droplets into ice crystals, produce snow and eat holes in the clouds 

Velle Toll, Jorma Rahu, Hannes Keernik, Heido Trofimov, Tanel Voormansik, Peter Manshausen, Emma Hung, Daniel Michelson, Matthew Christensen, Piia Post, Heikki Junninen, Ulrike Lohmann, Duncan Watson-Parris, Philip Stier, Norman Donaldson, Trude Storelvmo, Markku Kulmala, and Nicolas Bellouin

Living downwind of a cement-producing or a metallurgical plant could mean you get more snow, fewer clouds and more sunshine compared to nearby areas. We use satellite observations to reveal the glaciation of supercooled stratiform liquid-phase clouds by anthropogenic aerosols acting as ice-nucleating particles. There are strong indications that glaciation is caused by aerosols emitted from oil refineries, coal-fired power plants, cement, metal smelting and processing, chemical plants, and other anthropogenic air pollution sources in Europe, Asia, North America and Australia. Heavily polluted areas derived by simulating aerosol dispersion from strong anthropogenic aerosol point sources overlap with the areas of glaciation, snowfall, and decreased cloud cover strikingly well. Moreover, the polluted areas with decreased cloud cover are plume-shaped, with a distinctive head pointing towards the pollution source, similar to aerosol-polluted cloud tracks in liquid-water clouds (Toll et al 2019 Nature https://doi.org/10.1038/s41586-019-1423-9).

Glaciation-induced snowfall downwind of aerosol sources is observed using ground-based precipitation radars, and tracks of snow are also seen on the ground in satellite imagery. Aerosol-induced glaciation and snowfall lead to reduced cloud cover. At multiple aerosol sources, glaciation events are more frequent than polluted tracks in liquid-phase clouds. Thus, at least locally at some aerosol sources in the middle and high latitudes, the warming effect induced by aerosols acting as ice-nucleating particles likely exceeds the cooling effect induced by aerosols acting as cloud condensation nuclei. Further research is needed to quantify the global radiative forcing by anthropogenic ice nucleating particles.

How to cite: Toll, V., Rahu, J., Keernik, H., Trofimov, H., Voormansik, T., Manshausen, P., Hung, E., Michelson, D., Christensen, M., Post, P., Junninen, H., Lohmann, U., Watson-Parris, D., Stier, P., Donaldson, N., Storelvmo, T., Kulmala, M., and Bellouin, N.: Anthropogenic aerosols turn liquid cloud droplets into ice crystals, produce snow and eat holes in the clouds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4129, https://doi.org/10.5194/egusphere-egu23-4129, 2023.

EGU23-4266 | ECS | Posters virtual | AS3.2

Changes in low clouds optical characteristics in the atmosphere of two different urban sites in Romania 

Genica Liliana Saftoiu Golea, Sabina Stefan, Bogdan Antonescu, and Gabriela Iorga

The aerosol particles that become condensation nuclei affect the formation and evolution of clouds, their cycle lifetime, and their optical properties, having thus a major impact on the atmosphere, the radiative balance and leading therefore to climate changes. The aim of the study is to investigate the second indirect aerosol effect and the relationship between cloud droplet effective radius and cloud albedo for cleaner and polluted clouds over two sites in Romania (Bucharest and Cluj-Napoca), using satellite data collected from March 2000 to March 2022. Present study is the first one over sites in Romania. A series of physical parameters (albedo, cloud cover fraction, cloud optical depth, liquid water path and cloud water radius) were extracted from the Clouds and the Earth's Radiant Energy System (CERES) database for Bucharest, as a high polluted city, and for Cluj - Napoca, as a cleaner city in Romania. The time series for albedo and low cloud characteristics contained 193.584 hourly profiles. In addition, based on the optical depth from CERES, we calculated low cloud albedo using a parameterization currently used in the climate models. The study was also focused on the life cycle of the low clouds and on the cloud cover fraction over the two sites. The annual and seasonal variations of the cloud physical parameters were investigated and compared for both sites. We highlight how the cloud droplet effective radius modifies differently the cloud albedo for polluted clouds over Bucharest (presence of more and smaller cloud droplets and thus, a higher cloud albedo and less drizzle size drops) than for the cleaner clouds over Cluj-Napoca (presence of fewer and larger cloud droplets, and therefore a lower cloud albedo). The results also shows comparatively the frecqueny of occurence of this type of clouds over both sites and the temporal trend of analyzed physical characteristics. Modifications and variations of cloud characteristics at a city scale help us to better understand the second indirect aerosol effect, life cycle and the climatology of low clouds.

Acknowledgment

GLSG, SS and GI acknowledge the support from NO Grants 2014-2021, under contract no 31/01.09.2020, Project EEA-RO-NO-2019-0423. GLSG work was also supported by the University of Bucharest, PhD research grant and by the Romanian Nucleu Programme.

 

How to cite: Saftoiu Golea, G. L., Stefan, S., Antonescu, B., and Iorga, G.: Changes in low clouds optical characteristics in the atmosphere of two different urban sites in Romania, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4266, https://doi.org/10.5194/egusphere-egu23-4266, 2023.

EGU23-4331 | ECS | Orals | AS3.2

Evaluate parameterizations of cloud droplet spectral dispersion by using worldwide aircraft data 

Hengqi Wang, Yiran Peng, Chunsong Lu, and Johannes Quaas

Increased aerosol potentially impacts the cloud droplet spectrum, which in turn affects the aerosol-cloud interaction (ACI), known as the dispersion effect (DE). To consider DE in general circulation models (GCMs), many parameterizations have been proposed, but there are relatively few quantitative and global evaluations due to lacking suitable data and methodology. Additionally, both observations and numerical simulations confirmed that DE has opposite effects on ACI in aerosol- and updraft-limited regimes, but whether this effect can be reproduced by parameterizations has no clear conclusion until now. In this study, we used a liquid water content (LWC) binning method and worldwide data (China, Canada, Brazil, and Chile) to evaluate six dispersion parameterizations, namely Martin94, RLiu03, PengL03, Liu08, LiuLi15, and Zhang22. The LWC binning method ensures the difference between ACI values calculated by the cloud droplet number concentration and the effective radius is mainly caused by DE, which makes the quantitative calculation of DE possible. The results show that 1). DE has a weakening effect on ACI in the aerosol-limited regime, but an enhanced effect in the updraft-limited regime; 2). empirical parameterizations (Martin94, RLiu03, PengL03, and Liu08) can only show the weakening effect of DE on ACI, leading to an underestimation (-29% ~ -42%) for calculated ACI, especially for the updraft-limited regime; 3). both LiuLi15 and Zhang22 can reproduce the opposite effects of DE on ACI in different regimes, so we recommend giving priority to the LiuLi15 and the Zhang22 schemes when calculating DE in GCMs.

How to cite: Wang, H., Peng, Y., Lu, C., and Quaas, J.: Evaluate parameterizations of cloud droplet spectral dispersion by using worldwide aircraft data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4331, https://doi.org/10.5194/egusphere-egu23-4331, 2023.

EGU23-5203 | Orals | AS3.2

A recent assessment of the state of global cloudiness in the satellite-based climate data records 

Abhay Devasthale and Karl-Göran Karlsson

 

Four decades of satellite-based observations of clouds are now available and there are currently four different global cloud climate data records (CDRs) available providing 35+ years of data from the passive imagers, namely CLARA-A3, ESA Cloud CCI, ISCCP and PATMOS-X. This contribution presents a comprehensive assessment of the latest versions of these four long-term cloud CDRs. Given the fact that clouds cover nearly 70% of our planet and exert strong control on the radiation budget through their effects on radiation, precipitation, circulation and through their susceptibility to aerosols, such a periodic observational assessment of their global state is necessary from the climate perspective. CLARA-A3, PATMOS-X and ISCCP have been improved considerably in the recent years, thanks mainly to improved calibration, better training, algorithm developments, and rigorous validations.

This contribution will focus on three main areas:

1) Presenting the state-of-the-art global climatologies of cloud properties from the said CDRs, while highlighting the agreements and disagreements among them.

2) Evaluating the decadal stability of cloudiness in these CDRs using CALIPSO and MODIS as the references in light of the stringent requirements set by the WMO Global Climate Observing Systems (GCOS).

3) Investigating the robust trends in global cloudiness and their commonalities across the CDRs.

 

How to cite: Devasthale, A. and Karlsson, K.-G.: A recent assessment of the state of global cloudiness in the satellite-based climate data records, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5203, https://doi.org/10.5194/egusphere-egu23-5203, 2023.

EGU23-5374 | Orals | AS3.2

Trends in subtropical marine low-level cloud cover from 2007 to 2021 

Matthias Tesche and Sina Bruder

Marine low-level clouds play an important role in the Earth's energy budget. They reflect large amounts of incoming solar radiation that would otherwise heat the Earth's surface. Areas of persistent low-level stratocumulus clouds cover the subtropical eastern oceans where lower-tropospheric stability is high. Based on spaceborne lidar measurements, which allow to precisely identify clouds at different altitudes, we find that low-level cloud cover of Peruvian, Namibian, and Californian stratocumulus decreased by between 0.05 and 0.10 per decade between 2007 and 2021. A seasonally resolved analysis gives even stronger trends for those seasons in which low-level cloud cover is highest. No trend is found for Australian and Canarian stratocumulus. The decrease in low-level cloud cover is strongly tied to increasing sea-surface temperatures. Our analysis suggests statistical significant reductions in albedo for Namibian and Californian stratocumulus of 0.11 and 0.05, respectively, per 0.10 decrease in low-level cloud cover. Such changes will have a direct impact in the Earth's energy budget by reducing the cooling effect of major marine stratocumulus sheets.

How to cite: Tesche, M. and Bruder, S.: Trends in subtropical marine low-level cloud cover from 2007 to 2021, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5374, https://doi.org/10.5194/egusphere-egu23-5374, 2023.

EGU23-5377 | ECS | Orals | AS3.2

Large Eddy Simulations of aerosol-cirrus interactions 

Jhaswantsing Purseed and Nicolas Bellouin

The climate impacts of global aviation include CO2 effects and their so-called non-CO2 effects. Among
those non-CO2 effects, the effects of aerosol-cirrus interactions are the least understood and the latest
assessment of aviation radiative forcing could not give a best estimate and an uncertainty range [1]. Previous
studies [2, 3] have shown that a perturbation to the ice crystal number leads to a change in cirrus lifetime
and ice water path. In this talk, we investigate whether aerosol perturbations to ice nucleation can produce
large perturbations to cirrus ice crystal number.
We study these interactions using the 3D Met-Office NERC Cloud model (MONC). MONC is a Large Eddy
Simulation model coupled to the cloud micro-physics scheme, CASIM. We simulate two types of cirrus namely
the Gravity Wave cirrus (GW) and the Warm Conveyor Belt cirrus (WCB). The GW cirrus is thicker with
a higher ice crystal number concentration (ICNC) compared to the WCB cirrus, which is consistent with
aircraft observations [4]. We find that perturbing the formation stage of the cirrus cloud by injecting soluble
aerosols leads to an increase in ice crystal number and a decrease in the initial crystal size. Furthermore,
the ice clouds created in the presence of the injected soluble aerosols tend to have a higher ice water content
and an increased lifetime. Both GW and WCB cirrus clouds behave similarly to perturbation by soluble
aerosols at the formation stage.
In contrast, perturbing a pre-existing cirrus with soluble and insoluble aerosols does not change the properties
of the ice cloud. Ice crystal growth by vapour deposition uses available water vapour during the lifetime of
the cirrus [5, 6], which we find comes at the expense of activating aerosols that would lead to an increase
in the ICNC. Hence, although cirrus clouds would be sensitive to a perturbation in their ice crystal number
concentration, it is difficult to obtain such perturbations by injecting aerosols at cloud level, for example from
commercial aircraft exhaust. Furthermore, even though these results do not completely preclude large cirrus
perturbations from aviation aerosols in specific cases, they suggest that the corresponding global radiative
forcing is small.


References
[1] Lee et al. Atmospheric Environment. (2021). 
[2] Verma & Burkhardt. Atmospheric Chemistry and Physics. (2022).
[3] Gilbert et al. In preparation. (2022).
[4] Li et al. Atmospheric Chemistry and Physics Discussions. (2022).
[5] Hill et al. Quarterly Journal of the Royal Meteorological Society. (2014).
[6] Lohmann & Feichter. Atmospheric Chemistry and Physics. (2005).

How to cite: Purseed, J. and Bellouin, N.: Large Eddy Simulations of aerosol-cirrus interactions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5377, https://doi.org/10.5194/egusphere-egu23-5377, 2023.

EGU23-5520 | Orals | AS3.2 | Highlight

The climate impact of contrails from hydrogen combustion and fuel cell aircraft 

Alexandru Rap, Wuhu Feng, Piers Forster, Daniel Marsh, and Benjamin Murray

Aviation has been under increasing pressure in recent years to substantially cut its impact on climate. The International Air Transport Association (IATA) committed in October 2021 to achieve net-zero carbon emissions by 2050. Other similar ambitious targets have been set for aviation, all relying strongly on alternative fuel aircraft such as hydrogen combustion or fuel cells. A significant (i.e. 60%) proportion of the current aviation contribution to global warming is caused by non-CO2 effects, with contrail cirrus the largest of these effects. Here we perform and analyse the first calculation of the contrail cirrus effective radiative forcing (ERF) for fuel cell powered aircraft and one of the first calculations for liquid hydrogen combustion aircraft, comparing them with estimates for kerosene and sustainable aviation fuel (SAF).

The exhaust mix of the hydrogen combustion in an aircraft gas turbine or hydrogen fuel cell aircraft is different to that of the current hydrocarbon fuels. This leads to a potential climate penalty due to the significant increase in associated water vapour emissions. We find that for liquid hydrogen combustion and fuel cell powered planes, the area of the globe covered by contrails is set to increase substantially (~70%) due to their additional water vapour emissions leading to more regions of the atmosphere becoming susceptible to contrail formation. However, the expected cleaner exhaust and corresponding increase in average contrail particle sizes lead to changes in contrail radiative properties. These changes result in a reduction in contrail cirrus ERF for liquid hydrogen combustion (~25%) and fuel cell (~20%) powered planes, compared to kerosene planes. SAF planes are expected to lead to a slight (~5%) increase in contrail cover, but a decrease (~20%) contrail cirrus ERF, compared to kerosene planes.

In general, our analysis finds that changes in contrail cirrus ERF are relatively modest between fuel types, compared to the overall uncertainty in the ERF estimate itself. Some of this uncertainty stems from our representation of physical processes in contrails and further work is needed to look at the effects of alternative fuels on contrail ice crystal sizes, contrail lifetimes and aerosol-cloud interactions. 

How to cite: Rap, A., Feng, W., Forster, P., Marsh, D., and Murray, B.: The climate impact of contrails from hydrogen combustion and fuel cell aircraft, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5520, https://doi.org/10.5194/egusphere-egu23-5520, 2023.

EGU23-6166 | ECS | Posters on site | AS3.2

Measuring spontaneous charging of single aerosol particles 

Andrea Stoellner, Isaac Lenton, Caroline Muller, and Scott Waitukaitis

            Charge accumulation on aerosol particles (including water droplets) plays a critical role in a variety of natural and industrial processes. It gives rise to lightning in thunder- and sandstorms, influences particle transport and interactions in the atmosphere and can lead to dangerous dust explosions during industrial processing [1]. Shavlov et al. [2] suggest that the hydroxide ions and protons formed by the dissociation of water molecules are sufficient to cause charging during evaporation and condensation of droplets or surface-adsorbed water on solid particles. This hypothesis is backed up by Moreira et al. [3] who find that liquid evaporation leads to charge buildup on dielectric surfaces.

            By levitating individual aerosol particles in an optical trap we can characterize and manipulate the particle without losing information to ensemble averages or external interference from other particles or substrates [4, 5]. Our setup allows for trapping of various types of solid and liquid particles in the micrometer size range, like silica spheres, water droplets or droplets with solid nuclei inside. Figure 1 shows an illustration of the measurement principle. The particle’s charge is measured by applying a sinusoidal electric field and observing the resulting particle motion. The Mie scattering pattern of the particle furthermore gives information about the particle’s size and refractive index, both at equilibrium and during evaporation and condensation. The experiment allows us to control the relative humidity and air ion concentration around as well as air flow across the particle.

Ultimately we hope to contribute to a better understanding of the microphysical processes involved in thundercloud electrification and adjacent electrical phenomena in the atmosphere.  

FIGURE 1. Optical tweezers (λ = 532 nm) holding a solid or liquid aerosol particle. A sinusoidal electric field is applied between the two electrodes and the resulting particle motion as well as the particle’s Mie scattering pattern are recorded.

Acknowledgments

This project has received funding from the European Research Council (ERC) under the European Union’s Starting Grant (No. 949120).

References

  • Zhang L., et al. (2016) Indoor Built Environ 25 (3) 437-440.
  • Shavlov A. et al. (2018) J Aerosol Sci. 123 17-26.
  • Moreira K. S., et al. (2020) Mater. Interfaces 7(18) 202000884.
  • Reich O., et al. (2020) Phys. 3(1).
  • Ricci F., et al. (2022) ACS Nano 6 (16) 8677–8683.

How to cite: Stoellner, A., Lenton, I., Muller, C., and Waitukaitis, S.: Measuring spontaneous charging of single aerosol particles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6166, https://doi.org/10.5194/egusphere-egu23-6166, 2023.

EGU23-6429 | Orals | AS3.2

Do aerosols increase or decrease precipitation? 

Paul Field and Kalli Furtado

The observed variety of aerosol effects on precipitation at different spatial and time scales means that no simple answer to this question has so far been discovered.  However, although aerosol effects are many, it remains possible that there are universal constraints on the number of degrees of freedom needed to represent them.  We use convective-scale simulations to reveal a self-similar probability density function that underpins surface rainfall statistics. This function is independent of cloud-droplet number concentration and is unchanged by aerosol perturbations. It therefore represents an invariant property of our model with respect to cloud–aerosol interactions. For a given aerosol concentration, if at least one moment of the rainfall distribution on cloud-droplet number is a known input parameter, then this can be combined with the self-similar function to reconstruct the entire rainfall distribution to a useful degree of accuracy. We will demonstrate this using simulations from convective permitting, aerosol interacting simulations over China.

How to cite: Field, P. and Furtado, K.: Do aerosols increase or decrease precipitation?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6429, https://doi.org/10.5194/egusphere-egu23-6429, 2023.

EGU23-6535 | Orals | AS3.2

Cloud parameters from reanalysis datasets – a comparison with satellite data 

Axel Lauer, Lisa Bock, and Birgit Hassler

Clouds are a key component of the hydrological cycle and play an important role in weather and climate. Feedbacks between clouds and climate have important implications for climate sensitivity and thus on amplitude and pace of future climate change. In this study, as part of the SPARC Reanalysis Intercomparison Project (S-RIP) phase 2, we compare the cloud parameters from different reanalysis datasets, including the most widely used reanalyses ERA5, MERRA2 and JRA-55, with satellite observations. The study focuses on tropospheric clouds on monthly to seasonal and multi-year time scales. Means and variability of cloud parameters from the reanalyses such as cloud fraction, cloud liquid and ice water content as well as cloud radiative effects are compared to satellite observations for specific cloud regimes and regions. In addition to evaluating the performance of the different reanalysis products, we investigate whether the multi-reanalysis mean is in closer agreement with the observations than the individual reanalyses.

The analyses are performed with the Earth System Model Evaluation Tool (ESMValTool), a community developed open-source software tool. The tool provides common operations such as interpolating data on the same grid, calculating multi-reanalysis means, common data masking, area extraction, and basic statistics such as seasonal means, annual means, area means, etc. which facilitates a fair comparison with observations. Uncertainties are estimated using multi-product observational reference datasets.

How to cite: Lauer, A., Bock, L., and Hassler, B.: Cloud parameters from reanalysis datasets – a comparison with satellite data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6535, https://doi.org/10.5194/egusphere-egu23-6535, 2023.

The accurate representation of clouds and their phase is crucial to enable a correct representation of the Earth’s radiation balance. This has been demonstrated by large radiative errors in global models over the Southern Ocean mainly caused by an incorrect representation of supercooled liquid lowlevel clouds. In contrast to lowlevel clouds, midlevel clouds are rarely investigated. To fill this gap, this study investigates active satellite observations of midlevel clouds over the Southern Ocean and the Arctic Ocean from 2007 and 2008 with a comprehensive comparison to observations of lowlevel clouds. Midlevel and lowlevel clouds are distinguished by cloud base height. The DARDAR dataset provides a detailed phase categorization based on CloudSat and CALIPSO measurements. We have analyzed the cloud phase partitioning as a function of cloud top temperature, vertical cloud thickness, and the horizontal cloud extent. A local minimum in the mean liquid fraction within a cloud column can be observed for a cloud top temperature of -15 °C. An exception to this observation occurs for lowlevel clouds over the Arctic Ocean, which feature a plateau instead of a minimum. This hints at processes producing ice at these temperatures, which could be habit dependent vapor growth, secondary ice production, or a combination of both processes, as already discussed in other studies. Furthermore, daily sea ice concentrations from a passive microwave instrument are collocated to investigate their correlation with the cloud phase. At equal cloud top temperature, lowlevel clouds over the Southern Ocean and the Arctic Ocean have a higher liquid fraction, if they occur over sea ice. Midlevel clouds over the Southern Ocean show the same behaviour, while midlevel clouds over the Arctic Ocean show no significant phase dependence on the sea ice concentration. In addition, collocated CAMS reanalysis data are used to investigate the influence of different concentrations of various aerosol types such as sea salt, dust, black carbon, or organic matter on the cloud phase. Preliminary results show a stronger influence of the mixing ratio of sea salt on the phase of lowlevel clouds, but also the phase of midlevel clouds over the Southern Ocean seems to be influenced. Future work will further investigate the influence of different parameters, such as sea ice concentration, aerosol concentration, and cloud top temperature on the cloud phase by applying a machine learning model and exploring the relative importance of these parameters for the cloud phase, as well as their interactions and synergies.

How to cite: Dietel, B., Sourdeval, O., and Hoose, C.: The phase of midlevel and lowlevel clouds over the Southern Ocean and the Arctic Ocean and their dependence on cloud top temperature, sea ice, and aerosol concentrations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6713, https://doi.org/10.5194/egusphere-egu23-6713, 2023.

With global storm-resolving models (SRMs) a new type of global high-resolution models is now becoming available that explicitly resolves the main drivers of the atmospheric flow of matter and energy on the kilometer scale. In these models, arguably two poorly constrained physical processes remain unresolved  - microphysics and turbulence - but are at least fundamentally linked to their controlling factors, i.e., the circulation. In this study, we use a global SRM with two different microphysical schemes and do several sensitivity runs, where we vary one parameter of the applied microphysics scheme in its range of uncertainty. We find that the two microphysics schemes have distinct signatures (e.g., in how condensate is partitioned in ice and snow) but their mean cloud cover and total condensate is rather robust. Perturbing single parameters of each scheme also affects the condensate distributions and causes several 10s W/m2 variations in radiative fluxes. Changes in radiative properties of cloudy points dominate changes in the radiative balance at the top of the atmosphere. Overall, microphysical sensitivities in global SRMs are substantial and resemble inter-model differences of a multi-model ensemble.

How to cite: Naumann, A. K.: Microphysical controls on condensate distributions and the tropical energy budget in global storm-resolving models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6739, https://doi.org/10.5194/egusphere-egu23-6739, 2023.

EGU23-7097 | ECS | Orals | AS3.2

Threefold reduction of modeled uncertainty in direct radiative effects by constraining absorbing aerosols over biomass burning regions 

Qirui Zhong, Nick Schutgens, and Guido van der Werf and the AeroCom modelers

Absorbing aerosols emitted from biomass burning play an essential role in affecting the radiation balance, cloudiness, and atmospheric circulation over tropical regions. Assessments of these impacts rely heavily on the modeled aerosol absorption from poorly constrained global models and thus exhibit large uncertainties. By combining the AeroCom global model ensemble with satellite and in situ observations, we provide new constraints on the aerosol absorption optical depth (AAOD) over the Amazon and Africa. Our approach enables identifying, for each model, error contributions from emission, lifetime, and MAC (mass absorption coefficient), with emission and MAC dominating the modeled AAOD errors. In addition to primary emissions, we quantify substantial formation of secondary organic aerosols over the Amazon but not over Africa, which potentially contributes to the modeled AAOD errors. Furthermore, we find that discrepancies in the direct aerosol radiative effects between models decrease by threefold after correcting for the identified errors. This demonstrates that our work can significantly reduce the uncertainty in aerosols, which are considered the most uncertain radiative forcing agent.

How to cite: Zhong, Q., Schutgens, N., and van der Werf, G. and the AeroCom modelers: Threefold reduction of modeled uncertainty in direct radiative effects by constraining absorbing aerosols over biomass burning regions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7097, https://doi.org/10.5194/egusphere-egu23-7097, 2023.

EGU23-7104 | ECS | Posters on site | AS3.2

Effect of aerosols on the properties of low-level liquid clouds over the Southern Great Plains, USA 

Kanika Taneja, Harri Kokkola, Sami Romakkaniemi, Antti Arola, Seethala Chellappan, and Tero Mielonen

One of the largest uncertainties in estimating the anthropogenic radiative forcing is related to the impact of atmospheric aerosols on cloud properties. This uncertainty originates mainly from the complicated nature of aerosol-cloud interaction as it is much stronger and more difficult to observe than the aerosol-radiation interaction. The estimates of radiative forcing due to changes in cloud properties vary significantly between different global climate models, highlighting the need for constraining this forcing by using observations. Moreover, it is challenging to determine the impact of aerosols on clouds from satellite observations only. In this study, we aim to improve that by combining the in-situ observations with satellite retrievals, in order to reduce uncertainties in the anthropogenic impact on clouds and the climate. The study is performed for the low-level liquid clouds over the Southern Great Plains (SGP), Oklahoma. The in-situ data on particle number concentration, large enough to act as cloud condensation nuclei (CCN), with diameter larger than 100 nm (N100) were collected for a 5-year period from the Atmospheric Radiation Measurement (ARM) observatory at SGP site. In this analysis, the level-2 collection-6 MODIS cloud property dataset (MYD06_L2) with a 1x1 km resolution was used, where only liquid, single-layer clouds with a cloud top warmer than 268 K were included. It was observed that both CER and COT increased with increasing CWP. However, at a same level of CWP, the CER was smaller, and COT was larger at high N100 concentrations, as compared to the lower N100 concentrations. This result is consistent with the hypothesis of enhanced aerosol load increasing the number concentration of CCN, which in turn leads to smaller cloud droplets.

How to cite: Taneja, K., Kokkola, H., Romakkaniemi, S., Arola, A., Chellappan, S., and Mielonen, T.: Effect of aerosols on the properties of low-level liquid clouds over the Southern Great Plains, USA, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7104, https://doi.org/10.5194/egusphere-egu23-7104, 2023.

EGU23-7402 | ECS | Posters on site | AS3.2

Preliminary results from global modelling of Cirrus Cloud Thinning in the Geoengineering Model Intercomparison Project 

William Smith, Daniele Visioni, and Hugh Hunt

Cirrus clouds have a net positive radiative forcing effect on the climate, leading to the suggestion of cirrus cloud thinning (CCT) as a means to ameliorate global warming. By deliberately thinning cirrus clouds, more longwave radiation is able to escape the Earth system into space, cooling the planet. CCT has been modelled as part of the Geoengineering Model Intercomparison project in the G7cirrus experiment. Given the complexities of cirrus cloud modeling, to obtain similar results across different models this experiment simulates CCT by increasing the fall seed of ice crystals in cirrus clouds. This is carried out against a SSP5-8.5 scenario background, beginning in 2020 and ending in 2100. So far, G7cirrus has been run in two Earth System Models: UKESM1 and IPSL. Here, we look at some preliminary results from this experiment, such as analysing the intervention’s effective radiative forcing and its impact on different climate variables such as air temperature and precipitation.

How to cite: Smith, W., Visioni, D., and Hunt, H.: Preliminary results from global modelling of Cirrus Cloud Thinning in the Geoengineering Model Intercomparison Project, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7402, https://doi.org/10.5194/egusphere-egu23-7402, 2023.

EGU23-7634 | ECS | Orals | AS3.2

Identification of fog Particle Size Distributions by inverting the radiative transfer equation 

Ali Krayem, Fréderic Bernardin, and Arnaud Munch

            Degraded meteorological conditions, including fog, limit the performance of optical sensors used in various fields of application (avionics, intelligent road vehicles, etc.). Cerema, the French research and expertise center under the supervision of the Ecological Transition Ministry, conducts evaluations of these sensors under artificial and controlled fog conditions in the dedicated PAVIN Fog&Rain platform.  In order to perform a digital twin of the platform, it is necessary to develop robust modeling of the propagation of electromagnetic waves in fog. Propagation is governed by the phenomena of scattering and absorption of photons in contact with fog droplets. The fog Droplet Size Distribution (DSD) is a key parameter of the propagation models.

In the present work, we investigate the DSD identification from spectral radiation measurements by inverting the stationary radiative transfer equation (RTE). This distribution together with Lorenz-Mie scattering theory allow to compute the optical properties (scattering coefficient, absorption coefficient, and phase function). First, we prove the well-posedness of the underlying inverse problem, then we perform some numerical experiments using synthetic data. The numerical results suggest that the method allows to identify the DSD.

We present some numerical results obtained by using various models describing
the particle size distribution (e.g. Shettle and Fenn models) and some experimental distribution measured in the Cerema platform. Afterwards, the identification of the DSDs is carried out using the radiative transfer equation with the collision term (multiple scattering) and by performing direct scattering and backscattering measurements. The robustness of the reconstruction was studied numerically by introducing several noise levels to the measurements.

 

 

How to cite: Krayem, A., Bernardin, F., and Munch, A.: Identification of fog Particle Size Distributions by inverting the radiative transfer equation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7634, https://doi.org/10.5194/egusphere-egu23-7634, 2023.

EGU23-7846 | ECS | Posters on site | AS3.2

Combining geostationary and polar-orbiting satellite observations for studying the effect of INP on cold clouds 

Fani Alexandri, Felix Mueller, Torsten Seelig, and Matthias Tesche

Aerosol particles play a key role on Earth’s radiation budget and indirectly affect climate due to aerosol-cloud interactions (ACI), by acting as ice nucleating particles (INP) during the phase change in mixed-phased clouds. The forcing associated with the modification of cloud optical properties due to aerosol is yet insufficiently understood and represents a large uncertainty in future climate projections. Spaceborne remote sensing is a promising technique for quantifying ACI at a global scale and improving the performance of climate models.

Height-resolved measurements of aerosol optical properties from the Cloud Aerosol Lidar with Orthogonal Polarization (CALIOP) onboard the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite are used to estimate the vertical distributions of INP concentrations. Individually tracked clouds from geostationary observations are then matched with the aforementioned concentrations in the vicinity of those clouds. Hence, a bottom-up data set of cold clouds is formed that can be stratified according to different aerosol and cloud properties to investigate the INP effects on ice-containing clouds.

How to cite: Alexandri, F., Mueller, F., Seelig, T., and Tesche, M.: Combining geostationary and polar-orbiting satellite observations for studying the effect of INP on cold clouds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7846, https://doi.org/10.5194/egusphere-egu23-7846, 2023.

EGU23-8087 | ECS | Orals | AS3.2

The supercooled cloud fraction in the mixed-phase clouds from Himawari-8 observations 

Ziming Wang, Husi Letu, Huazhe Shang, Luca Bugliaro, and Christiane Voigt

The determination of supercooled cloud fraction (SCF) based on satellite remote sensing is important for research fields including estimation of global radiative energy balance, artificial weather modification, and prevention of aircraft ice accretion. However, nearly all retrieval algorithms for passive instruments provide binary phase information - ice, supercooled or liquid - making it difficult to retrieve mixed-phase cloud properties and understand the transition from supercooled water droplets to ice crystals. Motivated by these questions, we proposed a method to evaluate the ice partitioning of single-layer thermodynamic cloud top phase, under the assumption of the shape of ice crystals.

In order to retrieve optical properties of SCF, we use a droxtal habit model to investigate the scattering properties of frozen supercooled water particles. We compare the single scattering phase functions between droxtals and spherical particles at different wavelengths. Furthermore, the difference of satellite observed radiance reflected by supercooled water clouds and ice clouds are discussed. The difference between cloud ice water path of these two categories of clouds and observations from the same satellite channel can be used to evaluate the SCF in single-layer cloud top mixed phase clouds. Taking the ice-to-liquid ratio in the GCM (global climate model)-Oriented CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) Cloud Product (CALIPSO-GOCCP) as the criteria to validate our retrieved SCF, the average deviation, root mean square error and correlation coefficient are 6.98%, 9.62%, and 0.78, respectively. As a future work, we plan to adjust ice particle habits regarding ambient temperature to represent frozen supercooled water particles.

Our method could be applied to the to be launched EarthCARE (Cloud, Aerosol and Radiation Explorer) satellite in 2023 as it boards one multi-spectral imager and one atmospheric lidar simultaneously. This study is also of interest for related researches on assessing the climate impacts of supercooled and mixed-phase clouds and validating the associated global model simulations.

How to cite: Wang, Z., Letu, H., Shang, H., Bugliaro, L., and Voigt, C.: The supercooled cloud fraction in the mixed-phase clouds from Himawari-8 observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8087, https://doi.org/10.5194/egusphere-egu23-8087, 2023.

EGU23-9124 | Orals | AS3.2 | Highlight

Investigating ice crystal formation and growth in wintertime stratus clouds over the Swiss Plateau (CLOUDLAB project) 

Ulrike Lohmann, Jan Henneberger, Fabiola Ramelli, Robert Spirig, Christopher Fuchs, Anna Miller, Nadja Omanovic, Huiying Zhang, Johannes Bühl, Tom Gaudek, Kevin Ohneiser, Martin Radenz, Patric Seifert, Philipp Baettig, Maxime Hervo, and Daniel Leuenberger

Wintertime stratus clouds over the Swiss Plateau can last for days.  They dissipate either due to airmass changes, absorption of solar radiation during the day, or after glaciation when a sufficiently large number of cloud droplets freezes. After formation, the ice crystals grow in an ice-supersaturated environment via vapor deposition until they are large enough to sediment from the cloud as drizzle or freezing drizzle.

To better understand how quickly ice crystals of various habits grow in real clouds with turbulence, we conduct glaciogenic seeding experiments in wintertime stratus clouds over the Swiss Plateau in our project CLOUDLAB[1]. During these experiments, a drone releases silver iodide (AgI) particles into the cloud, upwind of our measurement site, and we use various ground-based remote sensing and in-situ cloud and aerosol instruments to detect the microphysical changes induced by seeding. Preliminary results from the first CLOUDLAB field campaign proved that our method successfully allows us to detect the seeding signal in the cloud radar. In addition to our field measurements, we conduct numerical model simulations with ICON at different horizontal resolutions and different seeding particle concentrations to understand which seeding AgI concentration is theoretically needed for partial or full glaciation of the cloud, i.e. how fast the ice crystals grow at the expense of the evaporating cloud droplets due to the Wegener-Bergeron-Findeisen process.

First results will be presented in this talk.


[1] https://cloudlab.ethz.ch/

How to cite: Lohmann, U., Henneberger, J., Ramelli, F., Spirig, R., Fuchs, C., Miller, A., Omanovic, N., Zhang, H., Bühl, J., Gaudek, T., Ohneiser, K., Radenz, M., Seifert, P., Baettig, P., Hervo, M., and Leuenberger, D.: Investigating ice crystal formation and growth in wintertime stratus clouds over the Swiss Plateau (CLOUDLAB project), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9124, https://doi.org/10.5194/egusphere-egu23-9124, 2023.

EGU23-9212 | ECS | Orals | AS3.2

Investigation of cloud response to the 2014 Holuhraun and the 2021 La Soufrière eruptions using the ICON-ART model 

Fatemeh Zarei, Corinna Hoose, Julia Bruckert, and Gholam Ali Hoshyaripour

Aerosols act as cloud condensation nuclei (CCN) and ice nuclei (IN) within cloud droplets, therefore they influence the microphysical features of clouds. Although many numerical and observational studies have investigated aerosol-cloud interaction, the extent and quality of aerosol impact on cloud formation and precipitation processes are not clear yet. Volcanic eruptions, which are rich sources of various chemical compounds in the atmosphere, can help to improve the understanding of aerosol effects on clouds by providing natural laboratories with locally high aerosol conditions adjacent to an unperturbed environment.

In the present study, we selected two volcanoes that emitted different aerosols and trace gases into the atmosphere to investigate their impact on the cloud microphysical processes: the 2014 Holuhraun and the 2021 La Soufrière eruption. The first one is an Icelandic volcano that mostly emitted sulfur dioxide (SO2), which forms sulfate particles serving as CCN. The second one is located on the Caribbean island of Saint Vincent and is an ash-rich eruption, so it is an appropriate case to study heterogeneous ice nucleation since ash particles serve as IN.

We simulated the initial phases of these eruptions using the ICOsahedral Nonhydrostatic model with Aerosols and Reactive Trace gases (ICON-ART) and performed different sensitivity experiments. For each case, we conducted two different simulations, in one of which the volcanic emission is considered, while in the other one, it is not (termed ‘Plume’ and ‘No-plume’).  For more detailed analysis, we divided the simulated area into two areas inside and outside of the plume using these criteria, column abundance of SO2>1 DU for Holuhraun and mass concentration of ash>10-4 gm-3 for La Soufrière.

For the Holuhraun case, the results showed a pronounced effect of volcanic aerosols on the different hydrometeors and process rates. Furthermore, the range and distribution of the liquid water path (LWP) have a good agreement with MODIS-Aqua satellite retrievals. In the Plume simulation, an increase in the number of cloud droplets but with smaller sizes was observed while we saw a reduction of graupel mass concentration in this simulation. These results confirmed our expectations, since in the Plume case the aerosol number concentration increases, resulting in an enhancement of the cloud droplet number concentration but with a smaller droplet size. In addition, the riming rate which highly depends on the cloud droplet sizes was reduced in the Plume simulation and led to the reduction of graupel mass that is mostly created by riming.

For the La Soufrière case, we mostly concentrated on heterogeneous ice nucleation as this case was an ash-rich eruption. Our preliminary results showed that the enhancement of ash particles reduced the ice crystal number concentration although the number of heterogeneously nucleated particles increased. To explain this behavior, we refer to the fact that additional heterogeneous freezing suppresses homogeneous freezing so that the total number of ice crystals is reduced. 

Keywords: Aerosol, Cloud, ICON-ART Model, volcanic aerosols, aerosol-cloud interactions, Holuhraun eruption, La Soufrière eruption

How to cite: Zarei, F., Hoose, C., Bruckert, J., and Hoshyaripour, G. A.: Investigation of cloud response to the 2014 Holuhraun and the 2021 La Soufrière eruptions using the ICON-ART model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9212, https://doi.org/10.5194/egusphere-egu23-9212, 2023.

EGU23-9516 | ECS | Posters on site | AS3.2

Constraints on cloud fraction adjustment to aerosols using explainable machine learning 

Yichen Jia, Hendrik Andersen, and Jan Cermak

This study applies explainable machine learning to near-global daily satellite and reanalysis data. We quantify and analyse the sensitivities of cloud fraction (CLF) to aerosol changes and their dependence on meteorological parameters.

Aerosol-cloud interactions have prolonged influences on the Earth’s radiation budget but remain one of the most substantial uncertainties in the climate system. Marine boundary layer clouds (MBLCs) are particularly important since they cover a large portion of the Earth’s surface. One of the biggest challenges in quantifying aerosol-cloud interactions from observations lies in isolating the CLF adjustments due to aerosol perturbations from the covariability of local meteorology and quantifying the influences of meteorology on the aerosol-CLF relationship. In this study, 10 years (2011-2020) of near-global daily satellite cloud products are used in combination with reanalysis data of meteorological confounders. Using cloud droplet number concentration (CDNC) as a proxy for aerosol, MBLC CLF is predicted by region-specific gradient boosting machine learning models. By means of SHapley Additive exPlanation (SHAP) regression values, the predictions are explained by quantifying the sensitivities of CLF to the predictors. Furthermore, the meteorological influences on the CLF adjustments are analysed with SHAP interaction values to define an interaction index (IAI). Globally, the regional ML models are able to capture on average 32% and up to around 71% of the variability of CLF. Global patterns of CLF sensitivities show that CLF is positively associated with CDNC and lower tropospheric stability (LTS), strongest in low-cloud regions. Increased sea surface temperature (SST) on the other hand will lead to reduced CLF, probably by increasing the vertical moisture gradient. The CDNC-CLF sensitivities are especially strong in stratocumulus-to-cumulus transition regions. Negative CLF sensitivities to the u wind component at 700 hPa are found for most regions which may indicate an influence of facilitated turbulence at the cloud top. In terms of the interactive effects of meteorological parameters, a significant dependence of the CDNC-CLF relationship on LTS and SST is found in low-cloud regions, and the patterns coincide with sensitivities. Positive IAIs are shown globally for SST and LTS, indicating that the CDCN-CLF sensitivity is stronger with high SST/LTS values.

The ongoing work shows that CDNC-CLF sensitivity is positive globally after accounting for meteorological covariations. Globally, SST and LTS can influence the positive CDNC-CLF relationship significantly, which is especially the case in stratocumulus regions. Detailed investigations will be carried out for not only SST/LTS but also other predictors to dig out the physics and causality behind the statistics.

 
 

How to cite: Jia, Y., Andersen, H., and Cermak, J.: Constraints on cloud fraction adjustment to aerosols using explainable machine learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9516, https://doi.org/10.5194/egusphere-egu23-9516, 2023.

EGU23-10174 | ECS | Posters on site | AS3.2

Dust impacts on storm development in the Eastern Mediterranean 

Ioannis Chaniotis, Athanasios Nenes, and Helena Flocas

Suspended particles of mineral dust are known to have a strong impact on the evolution of clouds and precipitation from meteorological to climate timescales. The ability to understand and predict the impacts of dust outbreaks on storm development and evolution would strongly benefit water management, food security, agriculture, and flood early warning systems. This is especially true for the Eastern Mediterranean, being a region heavily impacted by climate extremes and events (drought, floods) and frequent dust transportation from the Saharan desert throughout the year. To investigate the impact of mineral dust on the characteristics of storm development in the E. Mediterranean, several cases studies were examined with the aid of the Integrated Community Limited Area Modeling System (ICLAMS), a version of the Regional Atmospheric Modeling System (RAMS) augmented to include various parameterizations and numerical schemes of the complex microphysical processes of the forementioned aerosol particles. All cases involved storms developed in frontal systems with considerable vertical development and potential for deep convective clouds characterized by strong wind gusts, high rainfall and hailfall rates. In the simulations, dust emissions were allowed to provide particles that act as cloud condensation nuclei (CCN) and ice nuclei (IN). From the simulations we investigate how different descriptions of primary ice formation may affect results regarding cloud and precipitation characteristics, as well as the potential role of ice multiplication processes and the impact of enhanced cloud glaciation on convective invigoration of the storm clouds. In all cases considered (without any effects of ice multiplication and enhanced glaciation from it), precipitation patterns were spatially shifted under the influence of dust, maximum cloud updrafts were significantly increased, and the extreme conditions of rain and hail rates were enhanced considerably (up to 45% and 100% respectively).

How to cite: Chaniotis, I., Nenes, A., and Flocas, H.: Dust impacts on storm development in the Eastern Mediterranean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10174, https://doi.org/10.5194/egusphere-egu23-10174, 2023.

EGU23-10250 | Orals | AS3.2

Formation of secondary organic aerosols under various UV light intensities in a smog chamber 

Jae Young Lee, Hyun Kim, Jungdo Kim, and Heon Young Jung

The presence of anthropogenic organic compounds in aerosols can affect climate by altering the hygroscopicity of the aerosols and their behaviors as cloud condensation nuclei. Due to their importance, characteristics of atmospheric organic aerosols and their mixtures have been studied.

Among atmospheric organic aerosols, secondary organic aerosols (SOA) have not been well known. However, understanding on the chemical and photochemical properties of SOA is necessary to forecast the concentration of ultrafine particles more accurately. One of the important factors affecting the formation of SOA is the intensity of light. The stronger the intensity of light, the more the photochemical reactions, and thus the more the SOA formation. Thus, in this study, we examined how the formation of secondary organic aerosols can be changed under various UV light intensity.  

For this study, we used a smog chamber (1mm1.7m) with a Teflon or Tedlar bag used as a reactor. To provide ozone and clean air into the chamber, zero air generator (8301 LC, EcoTech, Australia) and gas dilution calibrator (Serinus CAL, EcoTech, Australia) were used. To detect ozone, NOx and particulate matters, ozone analyzer (Serinus 10, EcoTech, Australia), NOx analyzer (Serinus 40, EcoTech, Australia) and scanning mobility particle sizer (3938 Series, TSI, USA) were used, respectively. Input gas wasa mixture of NO, NO2, ozone and toluene, and set temperature varies from 25 to 26 C. 22 lamps (Philps TL-40W) were used for UV light sources, and the intensity was set by controlling 22 lamps. 

According to our investigations, the concentration of SOA with the strongest UV lights was more than three times higher than that without UV lights. As a result of the SOA formation, the concentration of NOx was decreased while the concentration of ozone was increased. We also found that the ratio of NOx and toluene affects the concentrations of SOA in the chamber experiments.

Acknowledgments

This study was supported by the National Research Foundation of Korea (grant number NRF-2021R1C1C1013350).

How to cite: Lee, J. Y., Kim, H., Kim, J., and Jung, H. Y.: Formation of secondary organic aerosols under various UV light intensities in a smog chamber, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10250, https://doi.org/10.5194/egusphere-egu23-10250, 2023.

Understanding co-variability between particulate matter (PM) concentration and meteorological conditions could provide insight into how the former varies under given weather conditions and eventually improve its prediction skill. However, relatively short data length of observed PM2.5 is a challenging issue not limited to Korea. Therefore, in such an analysis PM10, which has reliable observation for more than 30 years, has been widely used as a proxy of fine particles. Also, there are two stations in Seoul, Korea have relatively long-term observed PM2.5 in the period of 2000-current. As a result, more reliable analysis on the daily variation of PM2.5 in comparison with PM10 and meteorological conditions is feasible. First, the winter-mean of both PM10 and PM2.5 showed significant decreasing trends in the period of 2000-2020. Interestingly, decreasing trends of these weakened in the last 10 years with a different rate, resulting in a nearly flat trend of PM2.5 yet a relatively consistent decreasing trend of PM10 in the period of 2010-2020, suggesting a potential discrepancy in the variability of PM2.5 and that of PM10. Second, unlike the previously noted difference in long-term trends of seasonal mean values, PM2.5 and PM10 shared significantly similar daily variabilities if Asian dust cases were removed. In other words, the aforementioned discrepancy in the long-term trend of seasonal mean values of PM2.5 and PM10 does not affect their daily variation. The covarying patterns of PM2.5 and meteorological conditions were denoted as a migratory synoptic system. In particular, a migratory anticyclone from northwest China had significant positive correlation patterns with PM2.5 from two days before and remained stagnant over Korea after two days due to blocking by low pressure over the Northern Pacific. Along with this system, warm temperature anomalies and weak northerlies in the low troposphere were present over Korea, which is a conducive condition for high PM2.5. On the contrary, Asian dust cases were accompanied by cyclone that extended from arid regions of northern China with corresponding negative temperature anomalies and strengthened northerlies. In short, a migratory synoptic system over Korea is tightly correlated with PM2.5 daily variations as well as PM10. But once again, Asian dust events could be an important mechanism to differentiate daily variations of PM2.5 and PM10.

How to cite: Jang, W. and Yoon, J.-H.: Daily variation of PM2.5 and covarying meteorological conditions during wintertime using long-term observation in Seoul, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10407, https://doi.org/10.5194/egusphere-egu23-10407, 2023.

EGU23-10469 | ECS | Posters on site | AS3.2

PHIPS-HALO Radiative Measurement Applications to Atmospheric Bullet Rosette Ice Crystals 

Shawn Wagner, Martin Schnaiter, Guanglang Xu, Franziska Nehlert, and Emma Järvinen

Cirrus clouds provide a substantial amount of coverage in the earth’s atmosphere, resulting in a major impact on the global radiative budget. The extent of the radiative impact is determined by the aspherical ice crystal composition within the cirrus. Thus, a proper understanding of ice crystal single scattering properties is necessary for accurate climatological modeling and forecasting. One of the most relevant cirrus ice crystal habits is a polycrystalline bullet rosette, where individual bullets are radiating from the same nucleation point. Comprehensive studies on the dependencies of ice crystal habit formation have shown that bullet rosettes grow at a range of ice supersaturations with temperatures below -40 °C; environmental conditions frequently found within high altitude cirrus clouds. The Particle Habit Imaging Polar Scattering (PHIPS-HALO) probe is a unique aircraft mounted instrument which simultaneously acquires high-resolution stereo images and single scattering properties of individual cloud ice crystals. The ability to combine observed angular scattering functions with detailed images of their related crystals allows for in-depth analysis of the radiative effects of specific habits in critical atmospheric systems such as cirrus clouds. Here, a detailed explanation of the PHIPS-HALO performance and capabilities is provided with an investigation of single scattering properties of atmospheric bullet rosettes. Bullet rosette stereo-images were taken during a range of flights from the CIRRUS-HL campaign and were analyzed for their maximum dimensions as well as for crystal complexity and visually inspected for number of bullets per rosette, individual bullet aspect ratios and bullet hollowness. These bullet rosette microphysical properties were then associated with environmental conditions and with the simultaneously measured angular light scattering function and resulting asymmetry parameter. Angular scattering functions and asymmetry parameters are discussed for bullet rosettes grouped into subsets by complexity parameter. Results indicate that much lower asymmetry parameters represent real atmospheric bullet rosette crystals than what is expected by theoretical studies assuming smooth surfaces.

How to cite: Wagner, S., Schnaiter, M., Xu, G., Nehlert, F., and Järvinen, E.: PHIPS-HALO Radiative Measurement Applications to Atmospheric Bullet Rosette Ice Crystals, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10469, https://doi.org/10.5194/egusphere-egu23-10469, 2023.

EGU23-10839 | Orals | AS3.2 | Highlight

What is the aerosol state in the ambient atmosphere? Or: Multiscale modeling to tackle structural uncertainty in aerosol models 

Nicole Riemer, Jeff Curtis, Joseph Ching, Yu Yao, Zhonghua Zheng, and Matthew West

The diversity in particle composition within the atmospheric aerosol is well-documented in field observations, but usually grossly oversimplified in chemistry transport models or earth system model. This is for good reasons--- to save computational cost---but comes with the trade-off of introducing considerable and difficult-to-quantify structural uncertainty in our predictions of aerosol composition, and by extension, of aerosol interactions with clouds and radiation. This presentation will illustrate how targeted particle-resolved simulations can be used to quantify structural uncertainty in more approximate aerosol models (i.e., sectional or modal models). The particle-resolved approach resolves the aerosol using individual computational particles that evolve in size and composition during their simulated lifetime in the atmosphere. I will present our model development of WRF-PartMC, a stochastic particle-resolved model embedded into the Weather Research and Forecasting Model (WRF) for explicit simulation of aerosol mixing state on the regional scale. The novel computational methods developed for this purpose include a particle-resolved emission inventory and stochastic transport algorithms. With its fully-resolved aerosol mixing state representation, WRF-PartMC allows for direct inter-model comparisons with traditional aerosol schemes used in regional and climate models. We used this modeling approach to quantify the extent to which simplifying the diversity of aerosol composition introduces errors in our estimates of cloud condensation nuclei concentration and aerosol optical properties. I’ll conclude the presentation by demonstrating how machine learning can leverage particle-resolved simulation data to efficiently bridge to the global scale.

 

 

How to cite: Riemer, N., Curtis, J., Ching, J., Yao, Y., Zheng, Z., and West, M.: What is the aerosol state in the ambient atmosphere? Or: Multiscale modeling to tackle structural uncertainty in aerosol models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10839, https://doi.org/10.5194/egusphere-egu23-10839, 2023.

Near-cloud aerosols have distinct direct radiative effects (DRE) compared to aerosols far from clouds due to aerosol hygroscopic growth and cloud-related processes. Since near-cloud regions cover approximately 20-30% of the globe, DRE from these regions must be understood and better quantified. However, retrieving aerosol properties in the vicinity of clouds is challenging, mainly because the adjacent three-dimensional (3D) cloud radiative effects obscure aerosol scattering signals. In this paper, we will first introduce a new method for retrieving aerosol properties in the vicinity of clouds, capitalizing on machine-learning techniques that allow us to incorporate 3D radiative effects directly. Using this retrieval capability, we will show how DRE varies with cloud organizations such as Sugar, Fish, Gravel, and Flowers, which are commonly observed in the trade-wind regimes. More importantly, we will discuss the implications for near-cloud aerosol DRE under a warmer climate.

How to cite: Yang, C. K. and Chiu, J. C.: Investigating the Near-cloud Aerosol Direct Radiative Effects Under Cloud Organizations of Sugar, Fish, Gravel, and Flowers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11022, https://doi.org/10.5194/egusphere-egu23-11022, 2023.

EGU23-11310 | Orals | AS3.2

Projected changes in cloud properties in low/medium/high ECS models from CMIP5 and CMIP6 

Lisa Bock, Axel Lauer, and Veronika Eyring

Since the release of the first CMIP6 simulations one of the most discussed topics is the higher effective climate sensitivity (ECS) of some of the models resulting in an increased range of ECS values in CMIP6 compared to previous CMIP phases. An important contribution to ECS is the cloud climate feedback. Although climate models have continuously been developed and improved over the last decades, a realistic representation of clouds remains challenging. As projected changes in cloud properties and cloud feedbacks also depend on the simulated present-day fields, this contributes to the large uncertainties in modelled ECS.

In this study, we investigate the representation of both, cloud physical and radiative properties from CMIP5 and CMIP6 models grouped by ECS. Model results from historical simulations are compared to observations and projected changes of cloud properties in future scenario simulations are analysed by ECS group. For consistent processing of all datasets, the Earth System Model Evaluation Tool (ESMValTool) is applied to CMIP5 and CMIP6 simulations alongside with satellite observations.

Our results show that there are significant differences in simulated cloud properties and cloud radiative effects among the low/medium/high ECS groups with the high ECS models typically showing a better agreement with observations than the two other groups. Further analysis also shows differences in the projected changes in cloud properties among the different ECS groups related to cloud cover, cloud ice and cloud liquid water content. For example, a decrease in TOA net cloud radiative effect with increasing temperature is found in the tropics in the high ECS models whereas there is an increase in TOA net cloud radiative effect in medium and low ECS models.

How to cite: Bock, L., Lauer, A., and Eyring, V.: Projected changes in cloud properties in low/medium/high ECS models from CMIP5 and CMIP6, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11310, https://doi.org/10.5194/egusphere-egu23-11310, 2023.

EGU23-11374 | ECS | Orals | AS3.2

Aerosol-cloud interactions derived from the 2014 Holuhraun volcanic eruption 

Amy Peace, Jim Haywood, Ying Chen, George Jordan, Florent Malavelle, Daniel Partridge, and Ellie Duncan

Aerosol effective radiative forcing (ERF) has persisted as the most uncertain aspect of anthropogenic forcing over the industrial period, limiting our ability to constrain estimates of climate sensitivity and the accuracy of climate projections. Aerosol-cloud interactions are the most uncertain component of aerosol ERF. The 2014 Holuhraun volcanic eruption acted as large source of sulfur dioxide, providing a natural experiment for testing aerosol-cloud interaction hypotheses at a climatically relevant scale. Our study builds on previous aerosol-cloud interaction analyses of the eruption. We evaluate the observed aerosol perturbation to cloud properties inside the volcanic plume in the weeks following the eruption. As expected, on most days, we find an in-plume shift to increased cloud droplet concentration and decreased effective radius. The sign and magnitude of an in-plume shift in liquid water path varies in the weeks following the eruption. We probe this variation in the observed in-plume cloud perturbations to elucidate the aerosol-cloud interaction mechanisms following the Holuhraun eruption.

How to cite: Peace, A., Haywood, J., Chen, Y., Jordan, G., Malavelle, F., Partridge, D., and Duncan, E.: Aerosol-cloud interactions derived from the 2014 Holuhraun volcanic eruption, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11374, https://doi.org/10.5194/egusphere-egu23-11374, 2023.

EGU23-11682 | ECS | Posters on site | AS3.2

WRF-PMCAMx: a mesoscale model for cloud-aerosol interaction studies 

Georgia Sotiropoulou, David Patoulias, Spyros Pandis, and Athanasios Nenes

Cloud-aerosol interactions constitute the largest source of uncertainty in predictions of the global climate. In this study we present WRF-PMCAMx, a powerful tool for detailed cloud-aerosol investigations. This consists of the Weather Research and Forecasting model (WRF; Skamarock et al., 2008) coupled with PMCAMx-UF (Patoulias et al. 2022). PMCAMx-UF is a three-dimensional chemical transport model with a high-resolution sectional bin aerosol approach. The aerosol fields predicted by PMCAMx-UF are used to update the cloud droplet and ice number predictions in the Morrison et al. (2005) microphysics scheme in the WRF atmospheric component. To evaluate the impact of this coupling, we compare the cloud, precipitation and radiation patterns predicted by WRF-PMCAMx over Europe to the diagnostic fields produced by the standard Morrison scheme in the open-source WRF code.

REFERENCES:

Morrison, H., Curry, J.A., and Khvorostyanov, V.I.: A New Double-Moment Microphysics Parameterization for Application in Cloud and Climate Models. Part I: Description, Atmos. Sci., 62, 3683-3704 62, 2005 

Patoulias, D. and Pandis, S. N.: Simulation of the effects of low-volatility organic compounds on aerosol number concentrations in Europe. Atmos, Chem Phys., 22, 1689-1706, 2022.

Skamarock, W. C., Klemp, J. B., Dudhia, J., Gill, D. O., Barker, D., Duda, M. G., … Powers, J. G.: A Description of the Advanced Research WRF Version 3 (No. NCAR/TN-475+STR). University Corporation for Atmospheric Research. doi:10.5065/D68S4MVH, 2008

* This study is supported by the H2020-EU.1.3.- EXCELLENT SCIENCE - Marie-Skłodowska-Curie Actions project SIMPHAC (ID 8985685)

 

How to cite: Sotiropoulou, G., Patoulias, D., Pandis, S., and Nenes, A.: WRF-PMCAMx: a mesoscale model for cloud-aerosol interaction studies, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11682, https://doi.org/10.5194/egusphere-egu23-11682, 2023.

EGU23-11727 | ECS | Posters on site | AS3.2

A model study on aerosol impact on extreme precipitation 

Birthe Steensen and Kari Alterskjær

Observations and model results show an increase in extreme precipitation with global warming since the 1950s. During the last decades there have also been strong trends in anthropogenic aerosol concentration, aerosols that may affect cloud and precipitation processes that develop these extreme events. As human activities are the source of anthropogenic aerosols, they tend to be concentrated over highly populated regions where the potential cost and impact of extreme precipitation is high. In this study we investigate the link between extreme precipitation and aerosol particles in the atmosphere by using the cloud resolving WRF model. The model is set up with an aerosol-dependent cloud microphysics scheme that include processes such as; the increase in smaller droplets in aerosol rich clouds, the change in cloud reflective properties that can reduce surface evapotranspiration as well as a deepening of convective clouds and possible an increase in precipitation intensity. The model is run over several years in a stable climate to distinguish how these processes influence extreme precipitation separately from the extreme precipitation increase due to global warming. 

How to cite: Steensen, B. and Alterskjær, K.: A model study on aerosol impact on extreme precipitation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11727, https://doi.org/10.5194/egusphere-egu23-11727, 2023.

EGU23-11754 | ECS | Posters on site | AS3.2

Identifying and analyzing fog and low stratus life cycle regimes over central Europe 

Eva Pauli, Jan Cermak, and Hendrik Andersen

This contribution presents spatially distinct fog and low stratus (FLS) formation and dissipation regimes derived from satellite and reanalysis data and their sensitivities to meteorological and land surface conditions over central Europe.
FLS formation and dissipation processes are strongly governed by meteorological and land-surface conditions and vary geographically and across seasons. The timing of FLS formation and dissipation further has implications for traffic and solar energy production. While climatological analyses of FLS formation and dissipation exist, the influence of meteorological and land surface conditions on specific FLS formation and dissipation regimes is not clear yet.
In this study, satellite-derived fog and low stratus life cycle information is explicitly linked to land surface and meteorology in Europe. Pixel-based correlations of FLS formation and dissipation times with environmental conditions were analyzed in a hierarchical clustering approach. Spatially distinct regimes of FLS formation and dissipation can be identified, and a dependency on the background geography and climate is apparent. FLS formation and dissipation regimes are analyzed on multiple hierarchy levels, i.e. various cluster numbers are explored, to investigate the spatial division of larger regional regimes to smaller sub-regional and local regimes. Monthly mean sensitivities for selected sub-regional regimes suggest a dependency of those sensitivities on FLS type. A case study of a regime covering the Po valley in northern Italy is used to showcase the quantification of FLS drivers regionally using explainable machine learning. Future work will expand this approach to analyze and compare FLS drivers in regional regimes with different background geography and climate.

How to cite: Pauli, E., Cermak, J., and Andersen, H.: Identifying and analyzing fog and low stratus life cycle regimes over central Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11754, https://doi.org/10.5194/egusphere-egu23-11754, 2023.

EGU23-11909 | Posters virtual | AS3.2

Change of tropospheric aerosol over the ocean in the Arctic observed from space 

Linlu Mei, John Burrows, Marco Vountas, and Hartmut Bösch

Aerosols play a critical role in climate change over the polar regions. The impacts of aerosol on Arctic Amplification is not well understood. In this talk, satellite observations from different instruments are used to understand the spatial and temporal changes of aerosol properties in the troposphere over the ocean in the Arctic in the past four decades. The model simulations are also used to identify the change of aerosol components. The change of Arctic haze due to anthropogenic source is well identified from both satellite observations and model simulations. However, the change of marine aerosol source in the Arctic, especially for the period with strong sea ice melting, is only being observed from satellite observations.

How to cite: Mei, L., Burrows, J., Vountas, M., and Bösch, H.: Change of tropospheric aerosol over the ocean in the Arctic observed from space, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11909, https://doi.org/10.5194/egusphere-egu23-11909, 2023.

EGU23-12131 | ECS | Posters on site | AS3.2

Controls of cloud radiative effects: a data-driven observation-based quantification 

Hendrik Andersen, Jan Cermak, Alyson Douglas, Philip Stier, and Casey Wall

In this contribution, a statistical learning technique is used to quantify the response of cloud radiative effects to changes in a large number of environmental factors in spatial observation data.

Clouds play a key role for the Earth’s energy balance; however, their response to climatic and anthropogenic aerosol emission changes is not clear, yet. Here, 20 years of satellite observations of cloud radiative effects (CRE) are analysed together with reanalysis data sets in a (regularised) ridge regression framework to quantitatively link the variability of observed CREs to changes in environmental factors, or cloud-controlling factors (CCFs). In the literature the meteorological kernels of such CCF analyses are typically established in regime-specific regression frameworks based on a low (2-8) number of CCFs. In our data-driven approach, the capabilities of the regularised regression to deal with collinearities in a large number of predictors are exploited to establish a regime-independent CCF framework based on a large number of CCFs. Using a reference 7-CCF framework, we show that ridge regression produces nearly identical patterns of CCF sensitivities when compared to the traditional regression. In the data-driven framework, however, the traditional regression fails at producing consistent results due to overfitting. The data-driven analysis reveals distinct regional patterns of CCF importance for shortwave and longwave CRE: 

  • Sea surface temperatures and inversion strength are important for shortwave CRE in stratocumulus regions, in agreement with existing studies. However, zonal wind speeds in the free troposphere and surface fluxes are also shown to be important.
  • Free tropospheric meridional winds are important drivers of CRE in the subtropical belts (20°-40°) in both hemispheres, likely capturing aspects of Rossby Wave-related CRE variability. 
  • Aerosols are shown to be most important for shortwave CRE in the regions of stratocumulus to cumulus transition. 

While the multivariate method aims at limiting the influence of confounding factors on the estimated sensitivities, particularly the aerosol-CRE sensitivity may still be confounded to a degree. Future analyses of interactions between different CCFs and comparisons to global climate models are outlined.

How to cite: Andersen, H., Cermak, J., Douglas, A., Stier, P., and Wall, C.: Controls of cloud radiative effects: a data-driven observation-based quantification, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12131, https://doi.org/10.5194/egusphere-egu23-12131, 2023.

EGU23-12466 | ECS | Orals | AS3.2

Modeling global radiative responses and aerosol composition changes in EC-Earth3 from detailed new-particle formation predictions 

Carl Svenhag, Moa Sporre, Pontus Roldin, Lars Nieradzik, Daniel Yazgi, and Tinja Olenius

Representing detailed atmospheric aerosol processes in global climate models has proven challenging from both a computational and a parameterization perspective. A recent study on different Earth System Models (ESM) responses to small changes in the precursors to new aerosol particle formation (NPF) showed that two different models can produce opposite radiative outcomes in response to the removal of isoprene emissions (atmospheric cooling versus warming; Sporre et al., 2020).

Here, we examine and test particle formation rate schemes and the sensitivity of the ESM EC-Earth3 applied in the work by Sporre et al. 2020. We have replaced the formation rate scheme based on Riccobono et al. (2014), derived exclusively from the relationship between organics vapors and sulfuric acid (H2SO4), with a more detailed molecular-model-based formation rate look-up table approach. This new scheme was created utilizing the Atmospheric Cluster Dynamics Code (ACDC) and currently applies tables of NPF from H2SO4 and ammonia. The tables include the effects of atmospheric H2SO4 and ammonia concentrations, temperature, ion-pair production, and cluster scavenging sink in the NPF process. We compare our model simulation results with ambient spring-time measurements of aerosol formation. We focus on boreal conditions and compare the performance of the new scheme to the previous model configuration to assess the simulations of local NPF events. For benchmarking, we also couple M7 with a one-dimensional high-resolution trajectory model ADCHEM with a more complex representation of aerosol chemistry. This enables us to compare observations of aerosol size distribution data from SMEAR II, a boreal measurement station in Finland (61.85°N, 24.28°E) with our ESM model results and with the detailed ADCHEM model results.

Keywords: global modeling, new particle formation, aerosols, clouds, radiative effects, EC-Earth.

 

Sporre, M. K., …, R., & Berntsen, T. K. (2020). Large difference in aerosol radiative effects from BVOC-SOA treatment in three Earth system models, Atmos. Chem. Phys., 20, 8953–8973. https://doi.org/10.5194/acp-20-8953-2020.

Riccobono F., Schobesberger S., Scott C. E., et al. (2014) Oxidation products of biogenic emissions contribute to nucleation of atmospheric particles. Science. 344, 717–721, doi:10.1126/science.1243527.

Session: AS3.2

Consent: The presenting author is acting on behalf and with the consent of all authors of this contribution.

How to cite: Svenhag, C., Sporre, M., Roldin, P., Nieradzik, L., Yazgi, D., and Olenius, T.: Modeling global radiative responses and aerosol composition changes in EC-Earth3 from detailed new-particle formation predictions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12466, https://doi.org/10.5194/egusphere-egu23-12466, 2023.

Biogenic volatile organic compounds (BVOCs) and their oxidation products are known to facilitate the formation and growth of secondary aerosol particles in the ambient atmosphere. Some originate from the ocean, emitted by plankton or bacteria, while others stem from vegetation over the continents. Both marine and continental processes leading to aerosol formation or growth has been researched extensively and described in numerous publications. Their interactions however are yet to be examined. We seek to understand how marine precursors such as dimethyl sulfide (DMS) affects new particle formation over the boreal forest, and how highly oxygenated organic molecules (HOM) originating from monoterpenes grows said particles into the cloud condensation nuclei (CCN) size range.

We have utilised the Lagrangian chemistry transport model ADCHEM in reproducing observations from the SMEARII station (61°51' N, 24°17' E) located
in Hyytiala, Finland, during the year of 2018. The model operates along trajectories generated by HYSPLIT, using meteorology data from GDAS and incorporating emission inputs from CAMS. The atmospheric cluster dynamics code (ACDC) is coupled to the model in order to consider ion mediated new particle formation from sulphuric acid and ammonia.

We demonstrate how ADCHEM captures the gas-phase concentrations of key species including sulfuric acid (SA), HOM monomers and HOM dimers along with new particle formation and growth as observed by CI-APi-TOF and SMPS instrumentation, respectively. By running the model without anthropogenic influence, we show how DMS-derived SA and ammonia emitted from the ocean is transported inland in quantities sufficient to initiate
NPF over the boreal forest. The newly formed particles grow by condensation of HOM to reach the CCN size range. Our model results also indicate gas-phase concentrations of iodic acid (IA) at approximately 105 molecules cm-3, originating from marine emissions of methyl iodide (MeI). While ADCHEM does not consider the effect of IA on NPF, studies have claimed that IA may be able to cluster is the presence of SA and ammonia. This could increase the marine impact on continental NPF and will become the focus of future work with ADCHEM.

We theorise that the interactive marine and continental aerosol formation may act as a key element in the hydrological cycle. Marine air masses not only transport water vapour inland from the ocean but also SA, ammonia and halogens that under the influence of HOM formed over the boreal forest initiates the formation and growth of aerosol particles (without anthropogenic influence) ultimately reaching the CCN size range. These particles in turn can influence the formation, lifetime and precipitation patterns of clouds.

Figure (1). Measured and modelled aerosol particle number concentrations at the SMEARII station. The bottom panel
illustrates ADCHEM model results without the influence of DMS.

How to cite: Wollesen de Jonge, R. and Roldin, P.: Maritime-continental air-mass exchanges of biogenic marine volatile compounds boost inorganic new particle formation and production of cloud condensation nuclei over the boreal forest, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12511, https://doi.org/10.5194/egusphere-egu23-12511, 2023.

EGU23-12641 | Orals | AS3.2

Investigation of rainfall precursors using in-situ and remote sensing techniques in the southeast of the Iberian Peninsula 

Francisco Navas Guzmán, Wenyue Wang, Klemens Hocke, Leonardo Nania, Alberto Cazorla, Gloria Titos, Renaud Matthey, and Lucas Alados Arboledas

Rainfall prediction is one of the most challenging and uncertain tasks in weather forecasting, which has a significant impact on human society. Detection of heavy rainfall trends may be masked or amplified by natural variability, and numerical weather prediction (NWP) models have difficulty to predict them accurately. Therefore, understanding of rainfall effects with the evolution of atmospheric parameters and seeking atmospheric precursors of rainfall for nowcasting or prediction become an urgent need.

To date, most related studies have analyzed only a limited number of rain events or lacked long-term observations. This is likely to have a weak robustness. A multi-instrument and multi-parameter atmospheric monitoring system to detect precipitation precursors can improve the existing nowcasting system. AGORA (Andalusian Global ObseRvatory of the Atmosphere) is an ACTRIS facility located in the southeast of the Iberian Peninsula which offers unique infrastructure for the study of aerosol, clouds and precipitation. AGORA consists of two stations, an urban station located in the city of Granada (680 m asl) and a high-mountain station located in the National Park of Sierra Nevada (2580 m asl), separated by a horizontal distance of 20 km only. This infrastructure comprises state-of-the-art instrumentation covering active and passive remote sensing and in-situ techniques, including lidars, cloud radars, microwave radiometer, and weather stations. These instruments can obtain multiple atmospheric parameters (atmospheric water, aerosol, temperature, wind, etc.), including their vertical profiles.

In this study, we investigate the potential of different atmospheric parameters from ground-based microwave radiometer, ceilometer, nephelometer, absorption photometer and weather stations for the nowcasting of rainfall. We use 694 rain events identified by microwave radiometer in the southeast of Iberian Peninsula to identify conditions favorable to trigger rainfall over 10 years, and to analyze how they are related to observed changes in water vapor and aerosol load and properties. The composite analysis is carried out in a long time interval of 8 hours before and 16 hours after rain, with the onset of rain serving as the time marker for this method. The aim of our study is to show the typical behavior of rainfall, to reveal the interaction of rainfall with atmospheric parameters, and to explore the precursors of rainfall.

How to cite: Navas Guzmán, F., Wang, W., Hocke, K., Nania, L., Cazorla, A., Titos, G., Matthey, R., and Alados Arboledas, L.: Investigation of rainfall precursors using in-situ and remote sensing techniques in the southeast of the Iberian Peninsula, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12641, https://doi.org/10.5194/egusphere-egu23-12641, 2023.

It is unclear to what extent the cooling effect of anthropogenic air pollution particles, known as aerosols, counteract the warming effect of greenhouse gases. In particular, it is uncertain how strong the cooling effect caused by aerosol-induced changes in cloud properties is. Clouds and precipitation can form in the Earth's atmosphere thanks to aerosols. However, cloud thickness, coverage, and lifetime may be perturbed when anthropogenic activities add additional aerosols to clouds, leading to the formation of more numerous, but smaller droplets. We show that it is possible to quantify these perturbations by comparing the properties of polluted clouds at air pollution hotspots with those of nearby unpolluted clouds. There are large-scale polluted cloud areas around the world that are hundreds of kilometres in size, yet surrounded by distinctively less polluted cloud areas. We show that such strong anthropogenic cloud perturbations occur intermittently and only under favourable meteorological conditions. We challenge the assumption of a unidirectional increase in cloud thickness in current climate models and show that, on average, cloud thickness does not increase in response to aerosols. This suggests that the cooling effect of anthropogenic aerosols on Earth's climate may not be as strong as previously thought. Our results will ultimately lead to more reliable climate projections.

How to cite: Trofimov, H. and Toll, V.: Polluted clouds at air pollution hot spots help to better understand anthropogenic impacts on Earth’s climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12707, https://doi.org/10.5194/egusphere-egu23-12707, 2023.

EGU23-12715 | Posters on site | AS3.2

Ground-based remote sensing observations of aerosols and clouds above a coastal site in the Central Mediterranean 

Marco Rosoldi, Ilaria Gandolfi, Donato Summa, Benedetto De Rosa, Bojan Cvetkovic, Slobodan Nickovic, and Fabio Madonna

Aerosol particles, acting as condensation nuclei, affect the cloud microphysical and radiative properties as well as the precipitation processes. Aerosol-cloud interactions are not well understood and quantified yet. With the aim to contribute to their understanding, quantify the role of dust and marine aerosol in the cold and warm cloud formation, and for testing model parameterization, the MESSA-DIN (MEditerranean Sea Salt And Dust Ice Nuclei) measurement campaign was organized and carried out by the CNR-IMAA Atmospheric Observatory (CIAO), part of the Italian component of the European research infrastructure ACTRIS (Aerosol Clouds Trace gases Research InfraStructure). The measurements were performed at the coastal site of Soverato (10 m asl, 38.69 N, 16.54 E), on the South-Eastern coast of Italy, in the Central Mediterranean, from June to November 2021. Different types of remote sensing instruments were deployed and operated at the measurement site, including a polarization Raman lidar, a ceilometer, a Doppler lidar, a cloud Doppler radar, a microwave radiometer, a sun photometer and a sky-imager.

The synergy processing of the measurements from part of these instruments, using the ACTRIS algorithms, allows to distinguish between the aerosol and the different types of hydrometeors forming clouds and precipitations, as well as to retrieve aerosol geometrical and optical properties together with cloud geometrical and microphysical properties through the troposphere. The profiles of aerosol optical properties may allow to identify aerosol types and to retrieve their concentration profiles, using or adapting existing algorithms such as POLIPHON (Polarization Lidar Photometer Networking). Aerosol-type specific concentration profiles are used in models’ aerosol-type specific parameterizations for estimating cloud-relevant aerosol microphysical parameters, which are the concentration profiles of cloud condensation nuclei (CCN) and ice nucleating particles (INP). The above information and retrievals are investigated in synergy with air masses vertical and horizontal velocities through the troposphere, estimated from the Doppler lidar, and with column-integrated aerosol optical and microphysical properties, retrieved by the sun photometer using the AERONET (Aerosol Robotic Network) algorithms.

Case studies related to the formation of warm and cold clouds in presence of dust, marine aerosol and their mixture are discussed. Moreover, for cold clouds, the observational products are compared with the results of a DREAM-based aerosol transport model with included parameterizations for INP originating from both dust and marine aerosols, developed by the Republic Hydrometeorological Service of Serbia. Finally, correlations between clouds formation and properties and aerosol type and properties are also investigated, considering the role of vertical and horizontal wind profiles and other thermodynamic variables derived from observations or models.

How to cite: Rosoldi, M., Gandolfi, I., Summa, D., De Rosa, B., Cvetkovic, B., Nickovic, S., and Madonna, F.: Ground-based remote sensing observations of aerosols and clouds above a coastal site in the Central Mediterranean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12715, https://doi.org/10.5194/egusphere-egu23-12715, 2023.

EGU23-13005 | ECS | Posters on site | AS3.2

An investigation of fog and low cloud life cycles and their interaction with biomass burning aerosols in the Namib 

Alexandre Mass, Hendrik Andersen, and Jan Cermak

This contribution presents early results on the effects of biomass burning aerosols (BBA) on fog and low clouds (FLC) in the Namib, using data from multiple satellite platforms and station measurements.

Fog, which is the most relevant non-rainfall water source for plants and animals in the coastal parts of the Namib Desert, may become increasingly important for local ecosystems as regional climate simulations predict a warmer and drier climate for southern Africa in the future. Previous studies showed the role of BBA on cloud development over the ocean off the Namibian coast. The same processes are likely to influence Namib-region FLC formation and persistence as well. However, the potential effects of aerosols on FLC in the Namib Desert, a direct extension of the South-East Atlantic cloud system, have yet to be investigated.

A clear seasonal cycle of FLC dissipation is found in a satellite-based product of FLC formation and dissipation times, with longer FLC persistence during the BBA season. Using a BBA reanalysis product in combination with the satellite data, it is found that during this season, FLC dissipation times are positively correlated to BBA loading (higher aerosol loading coinciding with later FLC dissipation). It is assumed that semi-direct and indirect BBA effects contribute to this pattern, with further analyses aimed at isolating aerosol effects from possible confounders.

These findings are a first step in a better understanding of the Namib-region FLC system and will help in the development of a statistical model to quantify the sensitivities of FLC lifetime in the region in the next step of the project.

How to cite: Mass, A., Andersen, H., and Cermak, J.: An investigation of fog and low cloud life cycles and their interaction with biomass burning aerosols in the Namib, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13005, https://doi.org/10.5194/egusphere-egu23-13005, 2023.

EGU23-13559 | ECS | Posters on site | AS3.2

Online calculation of aerosol optics in atmospheric models with machine learning 

Pankaj Kumar and Gholam Ali Hoshyaripour

Aerosols affect weather and climate by absorbing and scattering radiation. Such effects strongly depend on the optical properties of aerosols that are mainly controlled by their other characteristics like size distribution, morphology and chemical composition. Chemistry and aerosol microphysics constantly modify these characteristics causing a large spatial and temporal variability. Most atmospheric models cannot account for this variability as they rely on look-up table to treat aerosol optics. This simplification can lead to large errors in weather and climate models when it comes to aerosol radiative impacts.  

This study presents a novel and computationally inexpensive machine learning approach for online representation of the aerosol optical properties. These properties are fully coupled with the chemical and microphysical variability of particles. Aerosol composition is considered with two ternary systems for solid (dust, soot and sea salt) and liquid (water, sulfate and organics) mixtures. Then Mie calculations are performed based on these aerosol compositions assuming core-shell and volume-average mixing states. The output of the Mie code is then used to train an artificial neural network. The results show that neural network model is able to predict the aerosol optical properties (extinction coefficient, single scattering albedo and asymmetry parameter) by R2 >0.90 and O(103 ) lower computational cost compared to Mie calculations. Potential applications of this approach for ICON-ART modeling system is discussed.

How to cite: Kumar, P. and Hoshyaripour, G. A.: Online calculation of aerosol optics in atmospheric models with machine learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13559, https://doi.org/10.5194/egusphere-egu23-13559, 2023.

EGU23-14021 | ECS | Posters on site | AS3.2

Collision efficiency of poly-dispersed charged spheres settling in a quiescent environment 

Pijush Patra and Anubhab Roy

We study the gravity-induced collisions of charged spheres of dielectric materials dispersed in a gaseous medium. When the gap thickness between the surfaces of two spheres is shorter than the mean free path of the surrounding fluid medium, continuum assumptions for the hydrodynamics interactions are no longer valid, and the non-continuum lubrication interactions result in surface-to-surface contact in finite time. Two like-charged dielectric spheres attract each other at close separations for a wide range of size and charge ratio values. We use trajectory analysis to calculate the collision rate and, thus, explore the role of electrostatic interactions on the collision dynamics of a pair of like-charged dielectric spheres. We present the modifications of pair trajectories due to electrostatic forces and show how collision efficiencies vary with the non-dimensional parameter capturing the relative strength of the electrostatic force to gravity as well as the charge ratio and size ratio.

How to cite: Patra, P. and Roy, A.: Collision efficiency of poly-dispersed charged spheres settling in a quiescent environment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14021, https://doi.org/10.5194/egusphere-egu23-14021, 2023.

EGU23-14380 | Orals | AS3.2

Impacts of aerosol-cloud-radiation interactions on photovoltaic generation: case of Saharan dust outbreaks in March 2021 

Gholam Ali Hoshyaripour, Kilian Hermes, Axel Seifert, Vanessa Bachmann, Florian Filipitsch, Jochen Foerstner, Christian Grams, Corinna Hoose, Julian Quinting, Anika Rohde, Heike Vogel, and Bernhard Vogel

Aerosols interact with radiation and clouds and thereby disturb radiative budget and temperature structure in the atmosphere. To account for these effects, numerical weather prediction models rely on climatological mean concentrations. This simplification may lead to large errors in the forecasted cloud cover and radiative fluxes especially during major aerosol events. For example, Saharan dust events often coincide with significant errors in shortwave radiation and thus, day-ahead photovoltaic forecasts in Europe. In this study we investigate errors in the short-range forecasts during Saharan dust outbreaks in March 2021, analyze possible causes and explore the solutions. We use the data from pre-operational forecasts performed with the ICOsahedral Nonhydrostatic model with Aerosols and Reactive Trace gases (ICON-ART) based on two experiments: without dust effects and with direct dust effect only. We compare model data with the measurements from satellite and in-situ instruments. The results reveal that the inclusion of direct radiative effects from prognostic dust improves the forecast in surface radiation during clear-sky conditions. However, dusty Cirrus clouds are strongly underestimated, pointing to the importance of representing indirect effects. To fill this gap, we develop and test corresponding sub-grid parameterization for dusty Cirrus in the ICON-ART model. Only with help of this parameterization ICON-ART is able to simulate the formation of the dusty cirrus, which leads to substantial improvements in cloud cover and radiative fluxes compared to simulations without this parameterization. This study confirms that a reliable photovoltaic forecast requires explicit treatment of aerosol-cloud-radiation in numerical weather forecast systems.

How to cite: Hoshyaripour, G. A., Hermes, K., Seifert, A., Bachmann, V., Filipitsch, F., Foerstner, J., Grams, C., Hoose, C., Quinting, J., Rohde, A., Vogel, H., and Vogel, B.: Impacts of aerosol-cloud-radiation interactions on photovoltaic generation: case of Saharan dust outbreaks in March 2021, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14380, https://doi.org/10.5194/egusphere-egu23-14380, 2023.

EGU23-14509 | ECS | Orals | AS3.2

Response of atmospheric rivers to aerosols treatment in regional climate simulations 

Eloisa Raluy-López, Leandro Segado-Moreno, Francisco Sánchez-Jiménez, Ester García-Fernández, Pedro Jiménez-Guerrero, and Juan Pedro Montávez

Atmospheric rivers (ARs) play an essential role in extreme precipitation phenomena. To predict
such events, a correct simulation of ARs becomes crucial. Since most of the regional climate models
do not take aerosols into account in an interactive way, the main objective pursued in this work was to
analyse the role of aerosols in the intensity and behaviour of ARs on the regional scale. The identifi-
cation of ARs has always been carried out in global climate simulations applying detection algorithms
that may not be suitable in regional climate models, due to the presence of boundaries in the spatial
domain.

This work presents a new ARs identification algorithm for regional climate simulations (AIRA).
The implemented algorithm has proved to be able to properly identify the vapour structures associated
with ARs. AIRA was applied to a set of hourly data from three regional simulations (BASE, ARI and
ARCI), covering a period of 20 years. In BASE, aerosols were prescribed, while the model incorporates
aerosols dynamically in both ARI and ARCI. In ARI, aerosols are only incorporated interactively in
aerosol-radiation interactions. In ARCI, they are also included in the microphysical processes.

AIRA has identified about 250 ARs in the three simulations. Spring and autumn ARs were the
most frequent, intense and long-lasting, while they were less frequent, shorter and weaker in summer.
The identified ARs explain up to a 30% of the total precipitation in some areas of the Iberian Penin-
sula. The differences between the three simulations are significant in the spatial distribution of the
precipitation and in the trajectory and intensity of some ARs. Although the number of detected ARs
is similar, the temporal steps with ARs common to the three simulations represent only a 37% of the
total BASE steps containing ARs. This indicates that the sensitivity to the inclusion of aerosols is
relevant. The common ARs events showed that the BASE and ARI simulations generally present sim-
ilar trajectoriesk. However, important differences appear regarding ARCI, specially
when ARs are not quite intense.

A cluster analysis of the thickness field between 1000 and 850 hPa in ARI identifies three main
patterns. The comparison between the centroids in ARI and ARCI, reveals that the differences between
ARs in both simulations are mainly related to the aerosols type and concentration. The main
mechanism behind this behaviour is related to the modification of the temperature field due
to aerosol-cloud interactions (indirect effect) while aerosol-radiation effects are less relevant. 

How to cite: Raluy-López, E., Segado-Moreno, L., Sánchez-Jiménez, F., García-Fernández, E., Jiménez-Guerrero, P., and Montávez, J. P.: Response of atmospheric rivers to aerosols treatment in regional climate simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14509, https://doi.org/10.5194/egusphere-egu23-14509, 2023.

EGU23-14608 | ECS | Posters on site | AS3.2

Following the Plume: Evaluation of UKESM1 simulation of 2014 Holuhraun eruption in a Lagrangian Framework. 

Eliza Duncan, George Jordan, Florent Malavelle, Paul Kim, Andy Jones, Duncan Watson-Parris, Alistair Sellar, James Haywood, Amy Peace, João Teixeira, Zak Kipling, and Daniel Partridge

Volcanic eruptions provide invaluable natural experiments to evaluate the transport, evolution, and potential impact of sulphate aerosol on clouds in global climate models (GCMs). The 2014 fissure eruption in Holuhraun, Iceland had an emission rate greater than a third of daily global sulphur dioxide emissions at its peak, resulting in significant perturbations to cloud radiative properties across vast swathes on the North Atlantic. Probing the GCM representation of aerosol lifecycle during transport in the volcanic plume, offers a unique insight to improve aerosol source and sink process understanding, which is essential to reducing one of the largest sources of uncertainty in climate modelling - aerosol-cloud-interactions.

Using rural aerosol measurement sites with climatologically relevant time series, we first perform a Eulerian evaluation of the UK Met Office Earth System Model (UKESM1) simulation of the volcanic eruption. Both in-situ observations and UKESM1 demonstrate a significant increase in aerosol concentration during the volcanic eruption compared to the climatology (2008-2013). However, the ‘standard’ version of the model fails to replicate the significant growth events associated with new particle formation seen in the observations during the volcanic eruption. A second simulation of UKESM1 with the addition of boundary layer nucleation, which is not included in the standard configuration, accurately reproduces the timing of nucleation events seen during the eruption period. Finally, we utilise a Lagrangian framework, in which HYSPLIT trajectories are calculated for both GCMs and reanalysis data, to analyse the relevant aerosol source and sink processes during transport that drive the differences between modelled and observed aerosol at the measurement sites. 

How to cite: Duncan, E., Jordan, G., Malavelle, F., Kim, P., Jones, A., Watson-Parris, D., Sellar, A., Haywood, J., Peace, A., Teixeira, J., Kipling, Z., and Partridge, D.: Following the Plume: Evaluation of UKESM1 simulation of 2014 Holuhraun eruption in a Lagrangian Framework., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14608, https://doi.org/10.5194/egusphere-egu23-14608, 2023.

This study investigates the top of atmosphere (TOA) solar radiative forcing induced by the transport of the biomass burning (BB) absorbing aerosol from the African continent over the south-eastern Atlantic Stratocumulus (Sc) region during the longer fire seasons, i.e., the 4 months of June through September.

The evolution, since 2002, of the BB aerosol and the Sc cloud properties from MODIS satellite data, as well as the evolution of the TOA outgoing solar radiative flux in clear and all skies from CERES (Clouds and the Earth’s Radiant Energy System) satellite data are presented and discussed. In clear skies, CERES shows an increasing trend in TOA outgoing shortwave flux (negative TOA forcing) associated to an increasing trend in MODIS aerosol optical thickness (direct effect) over the southeastern Atlantic Sc region. While in the presence of clouds, CERES shows that the negative TOA forcing by BB aerosol in clear skies is converted into a positive forcing, consistent with previous studies.

Further statistical analyzes are performed to determine whether this positive TOA forcing is primarily attributed to the increase in BB aerosols above Sc clouds or to the negative trend in cloud cover and liquid water path observed by MODIS data.

How to cite: Jouan, C. and Myhre, G.: Investigating Solar Radiative Forcing by Biomass Burning Aerosols within Clouds Over Southwest Africa Using Satellite Data., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14888, https://doi.org/10.5194/egusphere-egu23-14888, 2023.

EGU23-14906 | ECS | Orals | AS3.2

Changes in cloud activity of ship exhaust particles: Potential effects on Arctic mixed-phase clouds 

Luis Santos, Kent Salo, Hannah Frostenberg, Xiangrui Kong, Jun Noda, Thomas Kristensen, Takuji Ohigashi, Annica Ekman, Luisa Ickes, and Erik Thomson

Maritime shipping remains a large source of anthropogenic airborne pollutants, including exhaust particles that can act as cloud condensation nuclei (CCN). The International Maritime Organization (IMO) imposed global fuel sulfur content (FSC) limits on marine fuels in order to target ship exhaust sulfur oxides and particulate matter emissions, but has allowed competing pathways to regulatory compliance; i.e., low FSC fuels versus exhaust after-treatment. Laboratory experiments revealed that these compliance measures have secondary effects on physicochemical properties of exhaust particles, affecting their CCN activity (Santos et al., 2022a; 2022b). We observe that combustion of low FSC fuels results in emissions of highly hydrophobic particles, causing significant reductions in CCN emissions, whereas wet scrubbing leads to an increase in CCN activity.

One area of focus is the Arctic region, which has been shown to be particularly susceptible to the effects of climate warming. A steady decrease in observed sea ice cover amplifies the regional warming (Screen and Simmonds, 2010), but also opens the region to increased ship traffic which may result in further climate feedbacks (Stephenson et al., 2018). It is of particular interest to identify how increased ship exhaust particle emissions may affect cloud processes; for example, by facilitating liquid droplet formation and thus, potentially changing the radiative properties of the aerosol and clouds.

Here, we investigate how increased shipping activity potentially influences the properties of Arctic mixed-phase clouds. In our study the experimentally observed characteristics of marine particle emissions and their liquid droplet forming potential have been implemented in large eddy simulations. We use the MIMICA model (MISU/MIT Cloud-Aerosol model) (Savre et al., 2014) to simulate a stable stratiform mixed-phase cloud based on the Arctic Summer Cloud Ocean Study (ASCOS) (Tjernström et al., 2014). A range of input parameters for ship aerosol, including size distributions, number concentrations, vertical distributions and hygroscopicities, has been studied to assess the potential impact on cloud properties and regional climate.

Santos et al. (2022a). Environ. Sci.: Processes Impacts, 24:1769-1781

Santos et al. (2022b). Environ. Sci.: Atmos., Advance Article

Savre et al. (2014). J. Adv. Model. Earth Syst., 6:630-649

Screen and Simmonds (2010). Nature, 464(7293):1334–1337

Stephenson et al. (2018). Geophys. Res. Lett., 45:9898–9908

Tjernström et al. (2014). Atmos. Chem. Phys., 14:2823-2869

How to cite: Santos, L., Salo, K., Frostenberg, H., Kong, X., Noda, J., Kristensen, T., Ohigashi, T., Ekman, A., Ickes, L., and Thomson, E.: Changes in cloud activity of ship exhaust particles: Potential effects on Arctic mixed-phase clouds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14906, https://doi.org/10.5194/egusphere-egu23-14906, 2023.

EGU23-15030 | ECS | Posters on site | AS3.2

Using causal inference to investigate anthropogenic aerosol impacts on the diurnal temperature range 

Carla Roesch, Andrew Ballinger, Jakob Runge, and Gabriele Hegerl

Near surface air temperature is a primary variable to track global climate change. While mean temperature is often used to quantify global warming, the diurnal temperature range (DTR) - defined as the difference of daily minimum and maximum temperature - can provide additional information on changes to the diurnal cycle and temperature extrema, which is important for impacts of climate change. Different to increasing global mean temperature, observations have shown a decrease of global mean DTR over recent decades. This trend has been attributed to human emissions of greenhouse gases (GHG) which increase daily minimum temperature (Tmin), usually measured at night, more than daily maximum temperature (Tmax), observed during the day, by trapping outgoing longwave radiation. Aerosol radiative forcing has been associated with absorbing and scattering incoming (solar) shortwave radiation; thus, aerosols are assumed to reduce Tmax more than Tmin, decreasing the DTR. However, historical single and ALL forcing simulations from models that are part of phase 6 of the Coupled Model Intercomparison Project (CMIP6) model a decrease of the DTR for GHG and ALL forcings but show an increase in the DTR for anthropogenic aerosols due to a larger reduction of Tmin than Tmax. 

We investigate this discrepancy in aerosol contributions to changes in the DTR by applying causal inference methods to quantify the impact aerosols have on the DTR in Europe. To address the various effects aerosols have on the climate system, by interacting with both radiation and clouds, we include Tmin, Tmax, aerosol optical depth (AOD), cloud cover, cloud height, incoming shortwave radiation (SW) and outgoing longwave radiation using observational satellite and gridded station data for the past decade in our analysis. First results agree with the cooling effect of aerosols on Tmax by reducing SW radiation and show a positive effect of AOD on low cloud cover. They further suggest that a decrease of Tmax causes a decrease in Tmin, possibly explaining the CMIP6 model results.  

How to cite: Roesch, C., Ballinger, A., Runge, J., and Hegerl, G.: Using causal inference to investigate anthropogenic aerosol impacts on the diurnal temperature range, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15030, https://doi.org/10.5194/egusphere-egu23-15030, 2023.

EGU23-15360 | Orals | AS3.2 | Highlight

The Role of Anthropogenic Aerosols in Recent North Atlantic Climate Change: A Synthesis of Findings from the UK ACSIS Programme 

Laura Wilcox, Rowan Sutton, Jon Robson, Buwen Dong, Paul Griffiths, Daniel Grosvenor, Daniel Hodson, James Keeble, Steven Rumbold, Alex Archibald, Ken Carslaw, Andrea Dittus, Ben Harvey, and Bablu Sinha

Evidence from model simulations has suggested that anthropogenic aerosols may have forced multidecadal variability in a range of North Atlantic variables including sea surface temperatures, ocean circulation, and sea ice. However, many questions remain concerning the importance of anthropogenic aerosols in driving past changes in the North Atlantic climate system. The pathways via which changes in aerosol and aerosol precursor emissions, and oxidant levels, influence climate are complex. They involve both chemical and physical processes, and likely include changes in clouds, radiation, surface temperatures, atmospheric and oceanic circulation, and Arctic sea ice. This complexity is an important factor in the large uncertainty surrounding the role of anthropogenic aerosol in North Atlantic climate change, and was one of the major motivations for the UK’s North Atlantic Climate System Integrated Study (ACSIS). ACSIS was a multidisciplinary research programme conducted over the period 2016-2022, delivered by a consortium of seven UK institutions. This presentation draws together findings from the programme to provide an overall synthesis of what was learned in ACSIS about the role of anthropogenic aerosol in North Atlantic climate change. Remaining uncertainties, the potential for observational constraints, and opportunities for future work will also be discussed.

 

ACSIS made extensive use of simulations conducted for CMIP6, particularly historical simulations, and attribution experiments included in AerChemMIP and DAMIP. Additional sensitivity experiments with HadGEM3-GC3.1 and UKESM1 were used to quantify the effects of uncertainty in aerosol forcing in the absence of the additional uncertainty associated with model differences, to decompose the aerosol forcing, and to better illustrate the role of aerosol in recent changes.

 

As aerosol emissions increased (1850-1985), North Atlantic CDNC increased. Emissions of ozone precursors, and resulting changes in OH, contributed to this trend. This led to downwelling surface shortwave decreases across the North Atlantic, which drove colder surface temperatures, increased sea ice extent, and increased mean sea level pressure. In contrast, the eastern subpolar gyre warmed, likely due to increased ocean heat convergence due to the increase in the AMOC.

 

As local aerosol emissions fell (1986-2014) much of the reverse occurred. Downwelling surface shortwave increased across the North Atlantic, predominantly over land, driving warmer surface temperatures and reduced sea ice extent. The eastern subpolar gyre cooled. However, the role of aerosol in this later period is less clear due to a dominance of temperature-mediated cloud feedbacks over aerosol forcing, AMOC related feedbacks, and a changing aerosol forcing pattern.

How to cite: Wilcox, L., Sutton, R., Robson, J., Dong, B., Griffiths, P., Grosvenor, D., Hodson, D., Keeble, J., Rumbold, S., Archibald, A., Carslaw, K., Dittus, A., Harvey, B., and Sinha, B.: The Role of Anthropogenic Aerosols in Recent North Atlantic Climate Change: A Synthesis of Findings from the UK ACSIS Programme, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15360, https://doi.org/10.5194/egusphere-egu23-15360, 2023.

There are two types of activation of aerosols to become cloud-droplets.   First, clouds with liquid have a base at the level of water saturation where the first cloud-droplets form during ascent.  In the first 10 m or so above the base, the supersaturation rises to a peak value and aerosols activate to become cloud-droplets (“cloud base activation”).  The supersaturation then relaxes to an equilibrium.  Second, if the supersaturation becomes high enough during ascent into the interior of the cloud aloft, then there can be “in-cloud activation” as an extra source of cloud droplets.  A possible cause of in-cloud activation is entrainment of aerosols from the environment that are large enough to activate.  Another cause can be an increase with height of the supersaturation, causing it to exceed the peak value at cloud-base.

In-cloud activation is often overlooked in cloud-microphysics schemes of atmospheric models and is challenging to represent.  In deep convective updrafts, simulations of storms have shown it can generate most of the droplets at subzero levels aloft.  In-cloud activation of aerosols to become droplets can even generate most of the ice crystals in the anvil cirriform anvils by their homogeneous freezing near -36 degC. 

This presentation provides a theoretical analysis of microphysical feedbacks controlling sustained in-cloud activation and precipitation production.  A parcel model with 3 evolution equations for cloud mass, precipitation mass and cloud-particle number is created, during ascent for a cloud of a single phase, liquid or ice.   The theory predicts how in-cloud activation is most likely to be triggered by the onset of precipitation during sufficient ascent, with the ascent only needing to approach almost twice the cloud-base updraft speed aloft.  The initial state of no precipitation is unstable with respect to a perturbation. In the 2D phase space of cloud mass and precipitation mass, a neutral line is elucidated. Unstable growth of precipitation mass occurs by a positive feedback, driving the microphysical system to cross the line into a regime of stability.  A stable equilibrium, namely an attractor, is approached where precipitation mass is balanced by accretion of cloud mass (source) and its fallout (sink).

The cloud-particle number concentration attains a stable equilibrium involving in-cloud activation.  A source of droplets from the inexorably increasing supersaturation, caused by the vertical acceleration, is balanced against losses from accretion of cloud droplets by precipitation. Formulae for novel dimensionless numbers, characterizing the microphysical equilibria and their stability, are derived analytically.  These include a ‘condensation–precipitation efficiency’ and an ‘in-cloud activation efficiency’.  

The theory explains the orders of magnitude of liquid water content commonly seen in convective and stratiform clouds.  Sensitivity tests are performed by altering the loading of cloud condensation nucleus (CCN) aerosols and the updraft speed.  Microphysical equilibria are sensitive to the assumed ascent but are insensitive to CCN aerosol concentrations.  Nevertheless, higher aerosol concentrations cause more extreme oscillations of the mass fields during the approach to equilibrium.   This theory of in-cloud activation applies to both ice-only and liquid-only cloud.   More details are available in a recent published paper.

How to cite: Phillips, V.: In-Cloud Activation of Aerosols and Microphysical Quasi-Equilibrium with Precipitation in Deep Cloudy Ascent: a New Theory, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15789, https://doi.org/10.5194/egusphere-egu23-15789, 2023.

EGU23-15921 | ECS | Orals | AS3.2

Assessing cloud sensitivity to shipping aerosol across large emissions ranges 

Peter Manshausen, Duncan Watson-Parris, Matthew W Christensen, Jukka-Pekka Jalkanen, and Philip Stier

Aerosol-cloud interactions remain a large source of uncertainty in anthropogenic climate forcing. One of the reasons for this uncertainty is the confounding role of meteorology, influencing both aerosols and cloud properties. To untangle these variables, ship tracks, the clouds polluted by shipping emissions, have been widely studied. Recently, the use of shipping emissions locations and amounts, combined with reanalysis winds, has allowed us to study polluted clouds by following ship emissions to the locations they are advected to by the time of a satellite measurement of clouds. This is possible even when no visible tracks appear in satellite images. Here, we additionally use emission amounts data and investigate their effect on key cloud characteristics like droplet numbers and liquid water. This per-ship emissions data is valuable as it allows us to investigate cloud property changes stratified by region or meteorology. Between the ships with the lowest and highest emissions, droplet number anomalies increase by an order of magnitude from 0.25% to 2.5%, but the effect saturates at high emissions. We furthermore present evidence that increases of liquid water are insensitive to the amount of aerosol increases. Crossing data with a set of machine-learning detected ship tracks, we show that emissions amount has a similarly saturating effect on the formation of visible tracks as on droplet number, increasing roughly linearly for a large range of emissions before saturating (and even declining) at high emissions. The saturation of cloud responses at relatively high emissions could indicate that clouds react strongly to reductions in aerosol emissions.

 

How to cite: Manshausen, P., Watson-Parris, D., Christensen, M. W., Jalkanen, J.-P., and Stier, P.: Assessing cloud sensitivity to shipping aerosol across large emissions ranges, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15921, https://doi.org/10.5194/egusphere-egu23-15921, 2023.

EGU23-16028 | Orals | AS3.2

High-altitude aerosol characterization and PMF analysis of PM1 at the Helmos Mt station during the CALISHTO campaign 

Konstantinos Eleftheriadis, Olga Zografou, Maria Gini, Prodromos Fetfatzis, Konstantinos Granakis, Evangelia Diapouli, Manousos Ioannis Manousakas, Romanos Foskinis, Alexandros Papayannis, and Athanasios Nenes

This study presents part of the results of the CALISHTO campaign (Cloud-AerosoL InteractionS in the Helmos Background TropOsphere) that took place in autumn 2021 at the free-troposphere high-altitude Helmos station (2314 m a.s.l.). A Time-of-Flight Aerosol Chemical Speciation Monitor (ToF-ACSM, Aerodyne) was deployed among other instruments (AE31, PVM-100, SMPS, EC/OC analyzer) in the framework of the campaign. The chemical characterization of the non-refractory PM1 (NR-PM1), the influence from the Boundary Layer / Free Troposphere, the origin of the incoming masses and the influence of clouds were studied. The sources of PM1 including the non-refractory species of ACSM (organics and inorganics) combined with the equivalent black carbon were also investigated by applying the PMF model to the combined dataset. The results showed that there is a great variability of aerosol characteristics depending on the height of the PBL and the origin of the air masses. During September the station was exposed to PBL emissions, and thus displayed much higher mass concentrations of NR-PM1 than October and November. Concerning the sources of PM1, different types were identified with ammonium sulphate and oxygenated organics being predominant, as expected for aged aerosol with the degree of ageing investigated against air mass origin and microphysical parameters.  

How to cite: Eleftheriadis, K., Zografou, O., Gini, M., Fetfatzis, P., Granakis, K., Diapouli, E., Manousakas, M. I., Foskinis, R., Papayannis, A., and Nenes, A.: High-altitude aerosol characterization and PMF analysis of PM1 at the Helmos Mt station during the CALISHTO campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16028, https://doi.org/10.5194/egusphere-egu23-16028, 2023.

EGU23-16095 | ECS | Posters on site | AS3.2

Retrieving cloud sensitivity to aerosol using ship emissions 

Rodrigo Quilelli Correa Rocha Ribeiro, Edward Gryspeerdt, and Maarten Van Reeuwijk

Aerosol-cloud interactions are one of the key uncertainties in understanding future climate change. A commonly used method for constraining these interactions is using ship tracks. Aerosol-containing plumes from ships can develop into linearly shaped clouds identifiable in satellite images, isolating the aerosol impact on clouds. Previous studies have shown that ship tracks form more commonly in clean conditions, but even accounting for this, many ships that might be expected to form ship tracks do not. This leads to uncertainties in aerosol-cloud interactions and their climate impact.  

Ship track formation depends on the aerosol-containing plumes from the ship being sufficiently concentrated upon reaching the cloud. The cloud must also be sensitive to aerosol. In focus are updraft-limited clouds: smaller updrafts promote slower cooling as a cloud parcel rises, higher critical supersaturation values and lower aerosol activation fractions. It is not clear which of these are more important, but it is vital to understand them if we are using ship tracks to retrieve cloud sensitivity to aerosol.    

We develop a plume-parcel model to address these issues to estimate cloud droplet enhancements in ship tracks. Ship aerosol concentrations at the cloud height were modelled as plumes, simulating the shorter timescales of injection. Droplet number concentration enhancements were estimated using Köhler theory for over one hundred thousand ships off the coast of California.  

Using a constant updraft, the model was able to achieve reasonable enhancements (r2 ranging between (0.32, 0.4)). These enhancements were shown to be significantly sensitive to the choice of the updraft. In order to examine the hypothetical updraft values required for activation, an optimisation algorithm was developed to fit updrafts to cloud enhancement observations; a 1-1 correlation was achieved between observed and parameterised enhancements. Updrafts consistent with Köhler theory are considerably smaller than cloud-top radiative cooling-based estimates, suggesting that these clouds are less sensitive to aerosol than current estimates suggest. 

How to cite: Quilelli Correa Rocha Ribeiro, R., Gryspeerdt, E., and Van Reeuwijk, M.: Retrieving cloud sensitivity to aerosol using ship emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16095, https://doi.org/10.5194/egusphere-egu23-16095, 2023.

EGU23-16289 | Orals | AS3.2

Evaluating cloud-aerosol interaction parameterizations in the WRF-Chem model against cloud observations during a large volcanic eruption 

Louis Marelle, Jean-Christophe raut, Gunnar Myhre, and Jennie Thomas

In 2014/2015, the intense eruption of the Holuhraun/Bárðarbunga volcano in Iceland emitted extreme amounts of SO2, far above the anthropogenic or natural background. This event had major impacts on cloud properties observed by satellite in the Northern Atlantic. Malavelle et al. (2017) showed that many climate models struggled to reproduce these observed impacts on clouds, indicating potential serious issues in the cloud-aerosol interaction frameworks currently used in models. These issues could explain part of the very large uncertainty remaining in current estimates of the radiative effect of aerosol-cloud interactions.

Here, we use MODIS observations of cloud properties during the eruption to evaluate 3 different cloud-aerosol interaction approaches of decreasing complexity in the WRF-Chem 4 regional atmospheric model: First, the default model setup, using the Abdul-Razzak and Ghan (2000) parameterization (AR2000), coupling MOSAIC-4bin aerosols to the Morrison-2-moment microphysics. Second, the Thompson & Eidhammer (2014) aerosol-aware microphysics (TE2014), coupled for this study to MOSAIC-4bin aerosols. Third, the default version of TE2014 in WRF 4 using forced offline aerosols, where we replaced the original static aerosol climatology with 3D time-varying aerosols during the eruption. This last simplified approach does not require simulating fully interactive aerosols, and could be used to investigate regional cloud-aerosol processes and radiative forcing at high resolutions and climate time scales at a lower computational cost.

In addition, we compare how these 3 cloud-aerosol approaches impact the detailed cloud response during the eruption in terms of cloud microphysical and optical properties, radiative fluxes, and precipitation.

How to cite: Marelle, L., raut, J.-C., Myhre, G., and Thomas, J.: Evaluating cloud-aerosol interaction parameterizations in the WRF-Chem model against cloud observations during a large volcanic eruption, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16289, https://doi.org/10.5194/egusphere-egu23-16289, 2023.

EGU23-16295 | ECS | Posters virtual | AS3.2

Seasonal dust aerosol optical depth patterns using MODIS Deepblue aerosol product and MERRA-2 aerosol reanalysis 

Yahui Che, Bofu Yu, and Katherine Parsons

Dust storm as one of severe natural disasters occur frequently in central Australia. Ground-based networks with visibility and PM observation instruments are more often used for dust storm monitoring and research. With the development of satellite remote sensing and general circulation models (GCM), dust storm research has been with larger spatial coverage, especially where ground-based stations cannot be installed. The Deepblue (DB) aerosol product from the Moderate Resolution Imaging Spectroradiometer (MODIS) and the Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2) provide long-term aerosol records over 20 years from 2000 to the present. In this study, a dust AOD dataset was produced using MODIS DB and MERRA-2 aerosol reanalysis. The comparison of the dust AOD with AERONET data shows that 71% of collocated data points are within an EE of . The dust AOD dataset was then used to study seasonal dust distribution in Australia. Results show that dust storms occur more frequently in eastern Australia than the western part. In the northern part of eastern Australia, dust storm intensity reached the peak in the spring while in the southern part dust storm occur more frequently in the summer. Additionally, dust storms obtained from MODIS differs from those from traditional site observations, which reveals that our understanding on dust storm over regions without observations might be with large uncertainty.

How to cite: Che, Y., Yu, B., and Parsons, K.: Seasonal dust aerosol optical depth patterns using MODIS Deepblue aerosol product and MERRA-2 aerosol reanalysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16295, https://doi.org/10.5194/egusphere-egu23-16295, 2023.

EGU23-16589 | Posters on site | AS3.2

Uncertainty in aerosol-cloud radiative forcing is driven by clean conditions 

Edward Gryspeerdt, Adam C. Povey, Roy G. Grainger, Otto Hasekamp, N. Christina Hsu, Jane P. Mulcahy, Andrew M. Sayer, and Armin Sorooshian

Atmospheric aerosols and their interaction with clouds are the largest uncertainty in the human forcing of the climate system. Anthropogenic emissions have increased aerosol concentrations, increasing the concentration of cloud droplets and leading to reductions in droplet size and increases in cloud reflectivity (a negative radiative forcing). Central to this climate impact is the susceptibility of cloud droplet number to aerosol. This susceptibility varies widely with the method and data used to estimate it and within global climate models, explaining much of the variation in estimates of the radiative forcing from aerosol-cloud interactions (RFaci). Better constraints on the susceptibility have been a key target for recent observation-based constraints on the aerosol forcing.          
                                                                                                                                       
Previous work has shown that the aerosol burden of the clean, pre-industrial atmosphere has been demonstrated as a key uncertainty for the aerosol forcing. Here we show that the behaviour of clouds under these clean conditions is of equal importance for understanding the spread in radiative forcing estimates between models and observations. This means that the uncertainty in the aerosol impact on clouds is, counterintuitively, driven by situations with little aerosol. Removing these clean conditions from observational estimates of the susceptibility produces a close agreement between different model and observational estimates of the cloud response to aerosol, but does not provide a strong constraint on the RFaci. If we are to produce tighter constraints on the radiative forcing from aerosol-cloud interactions, better constraints on the behaviour of cloud in keen conditions are vital.

How to cite: Gryspeerdt, E., Povey, A. C., Grainger, R. G., Hasekamp, O., Hsu, N. C., Mulcahy, J. P., Sayer, A. M., and Sorooshian, A.: Uncertainty in aerosol-cloud radiative forcing is driven by clean conditions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16589, https://doi.org/10.5194/egusphere-egu23-16589, 2023.

EGU23-17581 | Posters on site | AS3.2

Idealised studies of aerosol effects on precipitation – from aqua-planets to global km-scale models 

Philip Stier, Andrew Williams, Ross Herbert, Philipp Weiss, Guy Dagan, and Duncan Watson-Parris

Aerosol effects on precipitation can be broadly categorized into radiatively and microphysically mediated effects – all of which remain highly uncertain. Their assessment in atmospheric models generally relies on the simulation of a complex chain of microphysical process growing aerosols into radiatively active size ranges and into size ranges suitable to act as cloud condensation nuclei, subsequently perturbing radiative fluxes, diabatic heating, cloud microphysical processes and ultimately precipitation formation.  The associated uncertainties along each step in these complex process chains remain significant and make it difficult to disentangle uncertainties in aerosol and cloud processes. 

Here we present results from a hierarchy of highly idealised model simulations in which aerosols are prescribed as fixed plumes of radiative properties, with an optional associated semi-empirical scaling of droplet number perturbations. These idealised simulations provide fascinating insights into the physical processes underlying aerosol effects on precipitation and into the interaction of local perturbations with the larger scale dynamics. 

Idealised aqua-planet general circulation model simulations reveal that the response of regional precipitation to idealised and realistic aerosol radiative perturbations can be well explained in an energetic framework (because associated changes in the net diabatic heating needs to be balanced by latent heat release, surface or top-of-atmosphere fluxes or compensated for by energy divergence/convergence). Extending this framework by adding land and realistic sea surface temperatures in an AMIP setup, we probe the regional sensitivity of precipitation changes to absorbing aerosol perturbations across the globe. Our results confirm the findings from the aqua-planet studies that that the local precipitation response to aerosol absorption is opposite in sign between the tropics and the extratropics and we show that this contrasting response can be understood in terms of different mechanisms by which the large-scale circulation responds to heating in the extratropics and in the tropics. Finally, we apply our framework in cloud resolving km-scale model simulations regionally and globally, which highlights the importance of radiative perturbations as well as a complex interplay of aerosol effects with the diurnal cycle of precipitation. 

How to cite: Stier, P., Williams, A., Herbert, R., Weiss, P., Dagan, G., and Watson-Parris, D.: Idealised studies of aerosol effects on precipitation – from aqua-planets to global km-scale models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17581, https://doi.org/10.5194/egusphere-egu23-17581, 2023.

The present study attempts to investigate the climatic impacts of PBAPs using the GISS-E2.1 Earth system model with the newly built PBAP emission model recently introduced to GISS-E2.1 to calculate the terrestrial and marine fluxes of PBAPs and estimate their transport and sinks. The current version of the PBAPs emission model accounts for different tracers of PBAPs including bacteria, fungal spores, and marine PBAPs (MPBAPs). The new PBAP tracers are allowed to interact with the radiation and to affect the liquid cloud droplet number concentration (CDNC).

Primary biological aerosol particles (PBAPs) can play a key role in cloud formation and phase regionally and locally by acting as cloud condensation nuclei (CCN), and ice nucleating particles (INP) at high sub-zero temperatures. Earlier studies suggested that the climatic impacts of PBAPs are negligible due to their globally small contribution to the total observed aerosol loads compared to other aerosols such as dust. However, PBAPs emissions are not yet well constrained. According to the IPCC AR5 report, the terrestrial emission flux of PBAPs was estimated in the range of 50-1000 Tg/yr, while AR6 neither updated the earlier estimates nor mentioned PBAPs at all. Recent observations proposed that the PBAPs' concentrations have likely been underestimated in earlier modelling studies. This suggests that PBAPs emission together with their climatic impacts and feedback remain highly uncertain, and thus, require a deeper investigation.

The study involves several scenarios where the emission fluxes of PBAPs were varied and different climatic diagnostics including, precipitation, cloud parameters, and direct and indirect radiative forcing resulting from these runs were compared with the ones from the control run of GISS-E2.1 with no PBAPs. We further investigated whether these differences were statistically significant. In this context, we present the results of the impact of changing the PBAPs' number fluxes on emission mass fluxes, burdens, number and mass concentrations, and atmospheric lifetime. For bacteria and when using the best estimate of number fluxes for bacteria cell diameter of 1 mm, the global average of emission, burden, and atmospheric lifetime was estimated to be 0.79 Tg/yr, 7.5 Gg, and 3.5 days, respectively. Those values are comparable with what has been reported by Burrows et al. (2009). For fungal spores, we estimated 2.55 Tg/yr, 19.5 Gg, and 2.8 days, which were comparable with Janssen et al. (2021). We further found that PBAPs have an overall negative/cooling direct forcing (NDF), however, the global average of the NDF was an order of magnitude smaller than the NDF of other aerosols, e.g., seasalt and OC. Nevertheless, regionally, the higher the emission of PBAPs (over vegetated surfaces), the cooling can be evidenced, which cannot be negligible (values up to ~ -0.4 W/m2). Moreover, adding PBAPs contributed to more global negative/cooling indirect forcing (NIF) (-28.8 w/m2) than the NIF from the control run (-27.1 W/m2).   

 

References

    Burrows, S. M. et al., ACP 2009, 9(23), 9281, doi: 10.5194/acp-9-9281-2009.

    Huang, S. et al., Environment International 2021, 146., doi: 10.1016/j.envint.2020.106197

    Janssen et al., ACP 2021, 21(6), 4381., doi: 10.5194/acp-21-4381-2021

How to cite: Sahyoun, M., Tsigaridis, K., and Im, U.: Predicting the Climatic impacts of Primary Biological Aerosol Particles; Sensitivity study using GISS-E2.1 Earth system model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17582, https://doi.org/10.5194/egusphere-egu23-17582, 2023.

EGU23-2 | Posters on site | CL2.1

State of a challenge – Third annual review 

Miklos Zagoni

We announced a public challenge at the EGU 2020 General Assembly against CMIP6 models predicting an increase of downward longwave radiation (DLR) in the range of 10 – 40 Wm-2 during the 21st century as a result of human greenhouse gas emissions. We based our challenge on observed facts, supported by long-known but rarely referred theoretical constraints. 22 years of CERES data show +0.11 Wm-2/decade increase in DLR, equivalent to +0.36 Wm-2 increase (+0.06 °K) until 2050 (in contrast to IPCC AR6, predicting +2 Wm-2/decade).

Supporting our prediction, we repeat here the deduction of the constraint equations, and control them on the recently available data sets. — Our best tool the compute the transfer of radiation in the atmosphere is Schwarzschild’s (1914) equation; its early, two-stream form is given in Schwarzschild (1906, Eq. 11), appropriate for global-mean energy flow computations. The equation consists of three terms; the difference of the second and first terms gives the net radiation at the surface as constrained to half of the outgoing longwave radiation (OLR), independently of the optical depth.  In the literature it was observed early (Emden 1913) that there is a discontinuity at the surface in radiative equilibrium, balanced by the turbulent fluxes in radiative-convective equilibrium. The formula for this net radiation is given for example in the textbook of Goody (1964, Atmospheric radiation: theoretical basis); repeated by Houghton (1977, Eq. 2.13), graphically represented in Chamberlain (1979, Fig. 1.4); and verified by the data (without explicitly describing the equation) of Hartmann (1994, pp. 61-63) within 0.3 Wm-2. The equation is verified by the CERES EBAF Ed2.8 (16 years of clear-sky global mean data) within 0.6 Wm-2. We use the second term of Schwarzschild (1906, Eq.11) with a particular optical depth of τ = 2 to compute the total energy absorption (and emission) at the surface, verified by the same satellite data product within the same difference (0.6 Wm-2) in the clear-sky annual global mean. — We created the all-sky versions of these two equations by introducing longwave cloud radiative effect (LWCRE), and justified the four individual equations on the most recent 22 years of CERES EBAF Edition 4.1 global mean data within ±3 Wm-2; while the mean bias of the four equations together is 0.0007 Wm-2. These equations form the boundary conditions of every valid climate prediction.

Reference:
Zagoni, M.: Challenging CMIP6 model predictions, EGU General Assembly 2020, Online, 4–8 May 2020, EGU2020-1, https://doi.org/10.5194/egusphere-egu2020-1

 

How to cite: Zagoni, M.: State of a challenge – Third annual review, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2, https://doi.org/10.5194/egusphere-egu23-2, 2023.

EGU23-6 | Posters on site | CL2.1

Nitrous Oxide and Climate 

William van Wijngaarden, Cornelis de Lange, James Ferguson, and Will Happer

Higher concentrations of atmospheric nitrous oxide are expected to slightly warm Earth's surface because of an increase in radiative forcing.  For current concentrations of greenhouse gases, the radiative forcing per added N2O molecule, is about 230 times larger than the forcing per added carbon dioxide molecule.  This is due to the heavy saturation of the absorption band of the relatively abundant greenhouse gas, CO2, compared to the much smaller saturation of the absorption bands of the trace greenhosue gas N2O.  But the rate of increase of CO2 molecules, about 2.5 ppm/year is about 3000 times larger than the rate of increase of N2O molecules, which has held steady at around 0.85 ppb/year since 1985.  So the contribution of nitrous oxide to the annual increase in forcing is 230/3000 or about 1/13 that of CO2.  If the main greenhouse gases, CO2, CH4 and N2O have contributed about 0.1 K/decade of the warming observed over the past few decades, this would correspond to about 0.00064 K per year or 0.064 K per century of warming from N2O.  This rather small warming does not support placing harsh restrictions on nitrous oxide emissions, which could seriously jeopardize world food supplies.

How to cite: van Wijngaarden, W., de Lange, C., Ferguson, J., and Happer, W.: Nitrous Oxide and Climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6, https://doi.org/10.5194/egusphere-egu23-6, 2023.

EGU23-12 | Orals | CL2.1

Evidence for Hemispheric Spectral Albedo Inequality 

William Collins and Daniel Feldman

In this study, we examine whether the interhemispheric symmetry observed
in broadband shortwave albedos also applies to the
hemispheric-mean visible and near-infrared albedos.  While
several recent exploratory studies have examined this question
using climate models, we explore this
question using direct observations of the visible and
near-infrared albedos collected by the Nimbus-7 satellite. This
study builds upon earlier intercomparisons of cloud spectral
albedos from Nimbus-7 and from climate models using the same
combinations of Nimbus-7 measurements used here (Collins, 1998).

We find that the hemispheric-mean spectral partitioning of albedo is
consistently and statistically significantly different between the two
hemispheres.  Consistent with prior studies, the origin of these
differences is due to interhemispheric differences in cloud cover.
Over oceans, the regional daily-mean differences between visible and
near-IR albedos are closely correlated with cloud amount.  The
relative differences are maximized for clear-sky conditions and
minimized for overcast conditions.

Background: The shortwave broadband albedo is a weighted sum of the albedos
in the visible and near-infrared bands.  Under condensate-free
conditions, the interactions of solar insolation in these bands
with the atmosphere and surface are quite different.  To an
excellent approximation, the condensate-free atmosphere is a
conservative Rayleigh-scattering medium in the visible.  Solar
radiation that is not reflected back to space is, to leading
order, transmitted to the surface.  In the near-infrared, the
interactions of sunlight with the atmosphere are dominated by
absorption, primarily with water vapor.  Additional absorption is
contributed by well-mixed greenhouse gases, oxygen, and other
gaseous constituents. The solar radiation
reaching the surface has therefore been reduced both by
reflection to space (from atmospheric condensates and the surface
albedo) and by absorption in the atmosphere. Hence, the relative
partitioning of net TOA insolation between the visible and
near-infrared bands will affect the relative partitioning between
atmospheric absorption and transmission to the surface.

 

How to cite: Collins, W. and Feldman, D.: Evidence for Hemispheric Spectral Albedo Inequality, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12, https://doi.org/10.5194/egusphere-egu23-12, 2023.

EGU23-1015 | Orals | CL2.1

State Dependence of CO2 Forcing and Its Implications for Climate Sensitivity 

Brian Soden, Haohe He, Ryan Kramer, and Nadir Jeevanjee

Instantaneous radiative forcing (IRF) is a fundamental metric for measuring the extent to which anthropogenic activities and natural events perturb the Earth's energy balance. This perturbation initiates all other forced climate responses. Among all the anthropogenic forcing agents, CO2 is the dominant driver of warming over the past century and the defining forcing variable for quantifying climate sensitivity. When evaluating the effect of CO2 changes on the earth’s climate, it is universally assumed that the IRF from a doubling of a given CO2 concentration (IRF2×CO2) is constant and that variances in climate sensitivity arise from differences in radiative feedbacks, or a dependence of these feedbacks on the climatological base-state. In this paper, we show that the IRF2×CO2 is not constant, but also depends on the climatological base-state, increasing by ~25% for every doubling of CO2, and has increased by ~10% since the pre-industrial era, implying a proportionate increase in climate sensitivity. This base-state dependence also explains about half of the intermodel spread in IRF2×CO2, a problem that has persisted among climate models for nearly three decades. It may also have important implications for elucidating the causes and consequences of deep-time paleoclimates, where changes in the climatological base-state can strongly modulate the magnitude of the CO2 IRF.

How to cite: Soden, B., He, H., Kramer, R., and Jeevanjee, N.: State Dependence of CO2 Forcing and Its Implications for Climate Sensitivity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1015, https://doi.org/10.5194/egusphere-egu23-1015, 2023.

The slope of the quasi-linear relation between planetary outgoing longwave radiation (OLR) and surface temperature (TS) is an important parameter measuring the sensitivity of the Earth climate system. The main goal of this study is to seek a general explanation for the quasi-linear OLR-TS relation that does not require the narrowing of “atmospheric window” of planetary thermal radiation. The physical understanding on the quasi-linear OLR-TS relation and its slope is gained from observation analysis, climate simulations with radiative-convective equilibrium and general circulation models, and a series of online feedback suppression experiments.

The observed quasi-linear OLR-TS relation manifests a climate footprint of radiative (such as greenhouse effect) and non-radiative processes (poleward energy transport). The former acts to increase the meridional gradient of surface temperature and the latter decreases the meridional gradient of atmospheric temperatures, causing the flattening of the meridional profile of the OLR. Radiative processes alone can lead to a quasi-linear OLR-TS relation that is more steeply sloped. The atmospheric poleward energy transport alone can also lead to a quasi-linear OLR-TS relation by rerouting part of the OLR to be emitted from the warmer place to colder place. The combined effects of radiative and non-radiative processes make the quasi-linear OLR-TS relation less sloped with a higher degree of linearity. In response to anthropogenic radiative forcing, the slope of the quasi-linear OLR-TS relation would be further reduced via stronger water vapor feedback and enhanced poleward energy transport.

How to cite: Cai, M., Sun, J., Ding, F., Kang, W., and Hu, X.: The quasi-linear relation between planetary outgoing long wave radiation and surface temperature: a climate footprint of radiative and non-radiative processes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1078, https://doi.org/10.5194/egusphere-egu23-1078, 2023.

EGU23-1130 | ECS | Posters on site | CL2.1

Analyzing Spatio-temporal variability of clouds over the Arabian Sea using ERA5 reanalysis dataset 

Jaswant Moher, Vimlesh Pant, and Sagnik Dey

Clouds cover 67% of the earth's surface hence they play an essential role in governing the energy balance of the earth. The combined effect of two properties, i.e., emissivity and albedo of clouds, defines the net radiative effect and their relative importance changes from day to night. In this study, we analyze four decades (1979-2018) of high-resolution (0.25°×0.25°) hourly cloud data from ECMWF fifth-generation reanalysis ERA5 dataset to study the long-term changes in Spatio-temporal variability of clouds over the Arabian Sea. The rationale behind choosing the ERA5 data is that, unlike any other climate variables, the long-term ground truth data for clouds do not exist, and satellite datasets have discrepancies. Ship-observation compiled Extended Edited Synoptic Cloud Reports Archive (EECRA) is a multidecadal data but has a coarse resolution (10°×10°) and suffers from human observational error. In this study, we used a combination of wind speed, air temperature, sea surface temperature (SST), and cloud cover data from ERA5  to explain the observed diurnal behavior and long-term changes in diurnal amplitude and local time of maximum clouds. The clouds over the Arabian Sea show two distinct diurnal peaks during June - August (JJA), but a single diurnal peak is found during the rest of the year. The seasonal and spatial variability in the diurnal behavior of clouds can be characterized in terms of the local thermodynamics of the Arabian Sea. The diurnal amplitude and local time of a maximum of low, mid, and high-level clouds have changed from 1979 to 2018, and the changes are spatially heterogeneous across all seasons. The diurnal amplitude of high-level clouds has increased through all seasons except during JJA. During the JJA season, the entire Arabian Sea shows a decrease in the diurnal amplitude of high-level clouds, with the largest decrease, observed in the eastern Arabian Sea along the west coast of India.

How to cite: Moher, J., Pant, V., and Dey, S.: Analyzing Spatio-temporal variability of clouds over the Arabian Sea using ERA5 reanalysis dataset, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1130, https://doi.org/10.5194/egusphere-egu23-1130, 2023.

Fossil-fuel combustion now outweighs solar variations in driving climate change (Higgs 2022, GSA, www.researchgate.net/publication/362103181). Remarkably, land (near-surface-air) warming is three times faster than ocean-surface warming, and Northern Hemisphere (NH; land-ocean average) three times Southern. This aberrant behavior began abruptly in 1985 (contrast pre-1985 lockstep warming-cooling; data.giss.nasa.gov/gistemp/graphs_v4). Moreover, over land and over the NH, warming is significantly slower at altitude (UAH satellite-measured lower-troposphere average temperature).

These strong lateral- and vertical warming gradients incriminate airborne soot (warms atmosphere by absorbing solar radiation). Soot’s poor dispersal causes strong concentration gradients, both (A) laterally, toward its main sources, which are predominantly on-land and NH (diesel engines, cooking woodfires, coal-fired powerplants/industries), e.g. over intensely industrialized nations (USA, Europe, China, etc.), average atmospheric soot concentration is ~1000% (i.e. 10 times) greater than over adjacent oceans (NASA 2011 global black carbon video https://svs.gsfc.nasa.gov/3844), starkly contrasting with CO2’s 1% difference (NASA global CO2 video); and (B) vertically, e.g. year-round average soot concentration above rural Siberia is ~500% higher at 0.5km than at 3km (doi: 10.3390/atmos12030351), far exceeding CO2’s 4% difference above Tokyo (10.3390/s18114064).

Two further observations implicate diesel- and coal-sourced soot specifically. Firstly, 25 years (y) before the 1985 decouplings (above), world annual oil consumption tripled in 1960, then remained high almost continuously (OurWorldinData, GlobalPrimaryEnergyConsumptionBySource graph). Secondly, coal’s distinctively stepwise growth (same graph) is mimicked, with a similar time-lag (10-20y), by stepwise land-air warming (data.giss.nasa.gov/gistemp/graphs_v4): COAL GROWTH fast 1974-1989 (tripled in 1974, due to 1973 oil crisis), nil 1989-1999, fast 1999-2014 (mainly China; OurWorldinData, CoalConsumptionByRegion graph); LAND WARMING fast 1994-2005, nil 2005-2011 (famed ‘hiatus’), fast since 2011.

CO2 cannot explain the observed strong lateral and vertical warming gradients, because its efficient dispersal produces near-homogenous atmospheric concentration. Even heavily industrial regions barely (<0.5%) exceed the global average (10.1038/s41598-019-53513-7). Furthermore, no leap in CO2 concentration occurred ~1985 or any other time; instead, CO2 grew by gradual acceleration, not stepwise (keelingcurve.ucsd.edu). Evidently, CO2 has negligible effect on climate, implying that its greenhouse effect is nullified by unknown and/or underestimated feedbacks (e.g. 10.1007/978-94-007-6606-8_17). If so, hyper-expensive CO2 capture is misconceived, besides counter-productive (today’s 420ppm is well below ~1,000ppm optimum for crop- and forest growth).

In the literature, the global-warming contribution of soot (‘black carbon’) is very uncertain. According to an influential review (10.1002/jgrd.50171; italic emphasis added here): “The best estimate of industrial-era climate forcing of black carbon ... is +1.1 W m-2 with 90% uncertainty bounds of +0.17 to +2.1 W m-2 (sic) ... We estimate that black carbon ... is the second most important human emission in terms of its climate forcing”. Black carbon’s warming effect was estimated to be 70% as strong as CO2. Recent IPCC estimates are 35% and 12% (2013, Physical Science Basis, Summary for Policymakers, fig.SPM.5; 2021, ditto, fig.SPM.2c). On the contrary, the data presented above suggest black carbon is overwhelmingly the dominant anthropogenic-warming agent. Helping to explain previous underestimates, two additional soot-induced warming mechanisms, via its effects on clouds, were recently recognised (10.1038/s41561-020-0631-0). Moreover, developing-world powerplants possibly emit far more soot (10.1029/1999JD900187) than the review assumed.

How to cite: Higgs, R.: Global land-surface warming much faster than ocean surface, and Northern Hemisphere faster than Southern: incriminates soot from burning oil and coal, exonerates CO2, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1416, https://doi.org/10.5194/egusphere-egu23-1416, 2023.

EGU23-2384 | ECS | Orals | CL2.1

Optimising water vapour retrievals by exploiting sensitivity within the far-infrared: A study in support of the ESA FORUM mission. 

Sanjeevani Panditharatne, Helen Brindley, Caroline Cox, and Richard Siddans

Theoretical models suggest that ∼55% of the outgoing longwave radiation from Earth is within the far-infrared region, 100-666 cm−1. Nevertheless, the top-of-atmosphere radiation spectrum in this region has never been measured, something that will change with ESA’s Far-infrared Outgoing Radiation Understanding and Monitoring (FORUM) mission, launching in 2027. Studies have indicated that absorption within this region is dominated by tropospheric water vapour, significantly impacting Earth’s radiation budget. Quantifying these concentrations plays a vital role in estimating its radiative effects and associated feedbacks.

The Infrared and Microwave Sounding (IMS) retrieval scheme developed at RAL Space is an optimal estimation scheme currently using channels within the mid- and near-infrared as well as the microwave region to obtain simultaneous retrievals of the vertical atmospheric profile and cloud properties. Current retrievals using this scheme have been performed on observations from Infrared Atmospheric Sounding Interferometer (IASI), Microwave Humidity Sounder (MHS) and the Advanced Microwave Sounding Unit (AMSU) onboard the MetOp satellites. Temperature and water vapour retrievals using this framework have been validated against radiosonde data with biases within 1 K and 10% of the reference respectively.

This work seeks to extend IMS into the far-infrared and exploit the known sensitivity of upwelling radiation within this region to improve current retrievals of water vapour. This would enhance our understanding of the spatial and temporal variations of water vapour within the atmosphere, and its role in Earth's radiation budget. Unique clear-sky airborne measurements will be used to analyse channel sensitivity within this region and maximise the information content for the retrieval. This retrieval capability would be the first of its kind to be thoroughly validated in this way and would be available for use on FORUM observations.

How to cite: Panditharatne, S., Brindley, H., Cox, C., and Siddans, R.: Optimising water vapour retrievals by exploiting sensitivity within the far-infrared: A study in support of the ESA FORUM mission., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2384, https://doi.org/10.5194/egusphere-egu23-2384, 2023.

EGU23-2448 | ECS | Orals | CL2.1

Including Ice-Cloud Longwave Scattering and Surface Spectral Emissivities in Climate Models Leads to More Impacts on Mean-State Climate than Climate Feedbacks 

Chongxing Fan, Yi-Hsuan Chen, Xiuhong Chen, Wuyin Lin, Xianglei Huang, and Ping Yang

Climate models often ignore cloud scattering and surface emissivity in the longwave (LW) for computational efficiency. Such approximations can cause biases in radiative fluxes and affect simulated climate, especially in the Arctic because of its large sensitivity to perturbations. We implemented treatments to both physics into the Energy Exascale Earth System Model (E3SM) version 2 by DoE and assessed their impacts on the simulated mean-state global climate as well as climate feedback and sensitivity.

By turning on and off the switches in the modified E3SMv2 model, we studied the changes in mean-state climate due to cloud LW scattering and surface emissivity effects by comparing four 35-year fully-coupled simulations. Cloud LW scattering warms the entire global troposphere by ~0.4 K on average; the warming is stronger in the Arctic (~0.8 K) than in the tropics, which is a manifestation of the polar amplification phenomenon. When realistic emissivity is incorporated into the model, the surface skin temperature increases by 0.36 K instantaneously on a global average, especially in the Sahara Desert (~0.7 K) where the surface emissivity is low. Surface skin temperature, as well as surface air temperature and tropospheric temperature, further increases by 0.19 K due to the inclusion of surface spectral emissivity. The mean-state climate changes due to both effects are linearly additive. The latitudinal and seasonal pattern of surface air temperature warming resulting from both effects is very similar to the response due to CO2 increase in the standard E3SMv2 model.

We also carried out four 35-year simulations under the abrupt 4xCO2 scenario, with cloud LW scattering and/or surface emissivity effects on and off. Based on standard radiative kernel analysis, we found that total global-mean climate feedback does not change significantly after including either or both physics. Nevertheless, lapse rate feedback, water vapor feedback, and cloud feedbacks in the tropics have changes by up to 10%. They are primarily associated with high cloud fraction response in the upper troposphere. Our study suggests that both the cloud LW scattering effect and the surface spectral emissivity effect should be included in climate models for a faithful representation of the radiative process in the atmosphere, especially at regional scales.

How to cite: Fan, C., Chen, Y.-H., Chen, X., Lin, W., Huang, X., and Yang, P.: Including Ice-Cloud Longwave Scattering and Surface Spectral Emissivities in Climate Models Leads to More Impacts on Mean-State Climate than Climate Feedbacks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2448, https://doi.org/10.5194/egusphere-egu23-2448, 2023.

The incoming surface solar radiation is an essential climate variable as defined by GCOS. Long term monitoring of this part of the earth’s energy budget is required to gain insights on the state and variability of the climate system. In addition, climate data sets of surface solar radiation have received increased attention over the recent years as an important source of information for solar energy assessments, for crop modeling, and for the validation of climate and weather models.

Gridded regional and global data records of the surface irradiance are available based on satellite measurements as well as derived from numerical models, e.g., reanalysis systems. For climatological analyses, long-term data records, covering about multiple decades, are required. Recently generated satellite-based climate data records from the EUMETSAT Satellite Application Facility on Climate Monitoring (CM SAF), i.e., SARAH-3 and CLARA-A3, as well as the GEWEX SRB data set, fulfill this requirement. Corresponding reanalysis data are also available, i.e., ERA-5, MERRA-2.

Here we will assess the quality of these satellite-based and reanalysis-derived climate data records of the surface irradiance by comparison with monthly surface reference data from the Global Energy Balance Archive (GEBA). The quality assessment will include the accuracy of the gridded data as well as their ability to realistically reproduce the anomalies and temporal trends as derived from the surface observations. The inter-comparison of the gridded data records allows to identify regions of high / low confidence in our knowledge of the surface irradiance and the surface radiation budget.  

How to cite: Trentmann, J. and Pfeifroth, U.: Assessing the quality of gridded Climate Data Records of the Surface Irradiance using global Reference Data Sets, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2563, https://doi.org/10.5194/egusphere-egu23-2563, 2023.

EGU23-2608 | ECS | Orals | CL2.1

Global ground heat flux from remote sensing data: preliminary results and evaluation 

Francisco José Cuesta-Valero and Jian Peng

Ground heat flux constitutes the conductive component of the surface energy budget. Quantifying this energy component is important to close the surface energy balance and to understand the energy exchanges between the lower atmosphere and the shallow subsurface. Furthermore, ground heat storage accounts for approximately 90 % of the continental heat storage, and 4-5 % of the total Earth heat storage. Therefore, monitoring changes in ground heat flux at global scale is of critical importance to quantify and understand the evolution of the Earth heat inventory, and thus climate change. However, the main sources of information about past and present ground heat flux are measurements of subsurface temperature profiles and micrometeorological observations, which are incomplete records biased towards northern extratropical latitudes.

Here, we present preliminary estimates of global ground heat flux derived from remote sensing products from the European Space Agency (ESA) Climate Change Initiative (CCI). Estimates from four land surface temperature (LST) products (MODIS-Terra, MODIS-Aqua, ENVISAT-AATSR, and SSMI-SSMIS) are evaluated against FLUXNET observations, obtaining a range of root mean squared errors from 3.8 to 5.2 W m-2 at monthly resolution. Nevertheless, there are some spatial inconsistencies among estimates from different LST products, as well as in long-term trends during the period 2003-2013. Several factors affecting the estimated ground heat flux are analyzed, with soil water and land cover having the largest effect on the retrieved values. These results suggest that land surface temperature from satellite observations may be able to provide global long-term ground heat flux estimates, although some issues still need to be solved.

How to cite: Cuesta-Valero, F. J. and Peng, J.: Global ground heat flux from remote sensing data: preliminary results and evaluation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2608, https://doi.org/10.5194/egusphere-egu23-2608, 2023.

EGU23-2796 | ECS | Orals | CL2.1

A novel approach for assessing regionally differentiated ocean contributions to Earth Energy Imbalance from GRACE(-FO) and multi-mission altimetry 

Bernd Uebbing, Kristin Vielberg, Bene Aschenneller, Roelof Rietbroek, Armin Köhl, and Jürgen Kusche

Earth Energy Imbalance (EEI) results from a net positive radiative flux at the top of atmosphere. Over 90% of this excess energy is stored as heat in the ocean causing present day ocean heat content (OHC) change. This in turn leads to volumetric or steric expansion of the water column and sea level rise. Utilizing observed bias-corrected short- and long-wave energy fluxes from the CERES project, it is possible to estimate EEI at the top of atmosphere. However, bias corrections rely on reanalysis OHC, potentially resulting in overestimation of ocean heat uptake (OHU).

Combining GRACE(-FO) and altimetry observations and constructing global sea level budgets allows to derive (thermo-)steric sea level change and convert this to OHU; the latter is generally achieved considering a literatute-based ocean-mean expansion efficiency of 0.52 [W/m^2 / mm/yr]. Nonetheless, this approach is valid for global mean steric sea level change only and it is unclear to what extent one can use it for investigating regional OHU.

Here, we develop a novel approach for deriving global and regional observation based OHC and OHU, which consists of three steps. (1) Fitting mass and steric spatial patterns, so called fingerprints, to GRACE(-FO) and altimetry data in a joint least-squares inversion. (2) Projecting reanalysis OHC onto the same spatial patterns that we use to explain steric variability. (3) Rescaling reanalysis OHC based on the observed steric sea level changes and reconstruction of spatial maps of OHC. These can then be further analyzed in order to derive global and regional OHU.

Based on preliminary results for years 2005-01 till 2015-12, we find ~1.2 mm/yr (thermo-)steric sea level change. Global-mean OHU of 0.62 [W/m^2] can be derived from the literature expansion efficiency above, while we find 0.63 [W/m^2] from the novel rescaling approach and 0.87 [W/m^2] based on ORAS5 ocean model data only. Regionally analyzing these results regarding individual ocean contributions reveals that the ocean model seems to significantly overestimate the uptake of the Atlantic and Pacific oceans, while slightly underestimating the Indian ocean contribution.

How to cite: Uebbing, B., Vielberg, K., Aschenneller, B., Rietbroek, R., Köhl, A., and Kusche, J.: A novel approach for assessing regionally differentiated ocean contributions to Earth Energy Imbalance from GRACE(-FO) and multi-mission altimetry, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2796, https://doi.org/10.5194/egusphere-egu23-2796, 2023.

EGU23-2962 | Orals | CL2.1 | Highlight

Observational Assessment of Changes in Earth’s Energy Imbalance Since 2000 

Norman Loeb, Tyler Thorsen, Sueng-Hee Ham, Fred Rose, and Seiji Kato

Observations from the Clouds and the Earth’s Radiant Energy System (CERES) show a marked increase in Earth’s energy imbalance (EEI) since 2000. At the same time, we’ve seen marked changes in numerous geophysical variables that influence EEI. While observations alone cannot quantify the anthropogenic and natural contributions to changes in these quantities, they can provide insight into how changes in different components of the climate system have led to the observed EEI trend. Using additional data from MODIS, CALIPSO, Cloudsat, and reanalysis, we find the increase in EEI to be due to decreased reflection by clouds and sea-ice, which cause a pronounced increase absorbed solar radiation (ASR), and a decrease in outgoing longwave radiation (OLR) due to increases in trace gases and water vapor. The ASR increases are largest over the subtropics and mid-latitudes in regions with decreases in low and middle cloud fraction, which likely occur in response to observed increases in sea-surface temperature (SST) in those locations. We diagnose the SST changes by performing an ocean mixed layer energy budget analysis at regional, hemispheric, and global scales using TOA and surface radiation observations from CERES, SST and temperature/humidity fields from ERA-5, and ocean mixed layer depth from ocean reanalysis. This analysis suggests that heating of the mixed layer and the subsequent increase in SST stems from ocean mixing/advection rather than from surface forcing. 

How to cite: Loeb, N., Thorsen, T., Ham, S.-H., Rose, F., and Kato, S.: Observational Assessment of Changes in Earth’s Energy Imbalance Since 2000, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2962, https://doi.org/10.5194/egusphere-egu23-2962, 2023.

EGU23-3268 | Orals | CL2.1

Aerosol Radiative Forcing 

Steven Dewitte

The long term global temperature rise caused by increased greenhouse gas radiative forcing is partially masked by temporary aerosol radiative cooling, which remains poorly known.

I present a new purely observation based estimate of Aerosol Radiative Forcing (ARF) due solely to the direct radiative effect of aerosols over clear sky ocean, and its time variation over the period 2003-20204 from combined MODIS and CERES aerosol, cloud, and radiation measurements. The resulting mean 2003-2020 ARF is -1.16 +/- 0.39 W/m2 , with no significant trend within an uncertainty of +/- 0.025 W/m2dec.

Combining this ARF with the best estimate of the greenhouse gas and solar radiative forcing, and the most likely value of the Equilibrium Climate Sensitivity, produces a plausible Earth Energy Imbalance as a residual of the energy balance equation at the top of the atmosphere.

How to cite: Dewitte, S.: Aerosol Radiative Forcing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3268, https://doi.org/10.5194/egusphere-egu23-3268, 2023.

EGU23-3896 | ECS | Orals | CL2.1

Constraining the tropical anvil cloud "iris" feedback 

Brett McKim, Sandrine Bony, Marion Saint-Lu, and Jean-Louis Dufresne

An outstanding question in climate science is how much the change in tropical anvil cloud clover with warming influences Earth's climate sensitivity. Here, we construct a simple model of cloud radiative effects to obtain an analytical equation for the tropical anvil area “iris” feedback. Our equation shows how the feedback is constrained by the fractional change in anvil cloud area, the anvil cloud radiative effect, and the radiative masking of low clouds that live beneath anvils.  We then look at satellite observations to diagnose these quantities. We find that the inferred values of anvil cloud radiative effect and low cloud masking effects sum to 1 Wm-2. Owing to this small radiative effect, the observed changes in anvil cloud cover in interannual variability implies an iris feedback that is wholly insufficient to strongly influence climate sensitivity. We then extend our equation to address whether anvil clouds might affect climate sensitivity through their masking of other forcings  or feedbacks.

How to cite: McKim, B., Bony, S., Saint-Lu, M., and Dufresne, J.-L.: Constraining the tropical anvil cloud "iris" feedback, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3896, https://doi.org/10.5194/egusphere-egu23-3896, 2023.

EGU23-4469 | ECS | Orals | CL2.1

Impacts of the Ocean Modes on the Surface Solar Radiation decadal variability over the western Pacific 

Lucas Ferreira Correa, Doris Folini, Boriana Chtirkova, and Martin Wild

Sea Surface Temperature (SST) plays a major role in the unforced variability of the climate system on decadal scales via the interplay between ocean and atmosphere, and associated changes in cloud cover and water vapor. The ocean modes, such as El Nino Southern Oscillation (ENSO) and Interdecadal Pacific Oscillation (IPO), are major coherent manifestations of SST variability. This means that the impacts of the ocean modes might be reflected in several components of the climate system, such as the energy budget. At the surface, this can be observed in the decadal trends in surface solar radiation (SSR). In this study we investigated the impacts of IPO and ENSO and associated cloud cover and water vapor variability on the decadal trends in SSR at 6 island stations scattered in the western Pacific (two stations in Fiji, one in New Caledonia, Nauru, Papua New Guinea and Marshall Islands). We combined between 15 and 40 years of daily SSR observations (depending on the station) with cloud cover from ERA5 reanalysis, aerosol optical depth (AOD) from CAMS reanalysis, and time series of IPO and ENSO. The comparison between clear-sky and all-sky SSR trends show that the all-sky trends strongly dominate in 5 out of the 6 stations. The exception is New Caledonia, where the clear-sky seems to also play an important role in the overall trend. This is the least cloudy station, and also the closest station to eastern Australia, an important source of aerosols in the region. Maps of cloud cover trends show two distinct regions which can be approximately separated by the average climatological position of the South Pacific Convergence Zone (SPCZ): one where cloud cover trends follow the phase of the IPO (positive IPO phase = positive cloud cover trend; N-NE of the SPCZ) and one where the opposite happens (positive IPO phase = negative cloud cover trend; S-SW of the SPCZ). The direct comparison between annual time series of all-sky SSR and IPO shows correlations stronger than 0.5 at two stations in Fiji and the one in New Caledonia (SW of the SPCZ). At the station in Nauru (North of the SPCZ) there is a negative correlation stronger than -0.5. When comparing annual all-sky SSR to the ENSO index, significant negative correlations are found at Momote-Papua New Guinea (-0.41) and at Nauru (-0.96), both located in the Western Pacific Warm Pool, near the Equator. In all cases strong negative correlations (<-0.7) between SSR and cloud cover using both annual and 11-year moving means time series support the hypothesis of strong cloud control over SSR interannual and decadal variability. The results indicate that IPO and ENSO play a major role in the SSR variability over the Western Pacific by controlling different cloud cover regimes in the region. This reveals a real world case of the importance of unforced internal variability to the SSR decadal and sub decadal changes.

How to cite: Ferreira Correa, L., Folini, D., Chtirkova, B., and Wild, M.: Impacts of the Ocean Modes on the Surface Solar Radiation decadal variability over the western Pacific, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4469, https://doi.org/10.5194/egusphere-egu23-4469, 2023.

EGU23-5155 | ECS | Orals | CL2.1

Low-frequency modes in internal variability of surface solar radiation 

Boriana Chtirkova, Doris Folini, Lucas Ferreira Correa, and Martin Wild

We investigate potential reasons for decadal-scale internal variability of surface solar radiation (SSR) using model data from the Coupled Model Intercomparison Project - Phase 6. We compare unforced coupled atmosphere-ocean (piControl) to atmosphere-only (piClim) simulations with prescribed climatological sea surface temperatures (SSTs) to access the relevance of SSTs for unforced SSR inter-annual variability. Further, the connection between SSTs and known climate modes of variability is exploited. We focus on coupled and ocean-only modes of variability such as El Niño–Southern Oscillation (ENSO), Pacific Decadal Oscillation (PDO) and Atlantic Multidecadal Oscillation (AMO). Using the climate indices which describe these modes, we relate the SST field to SSR trends in different regions and we find a relationship between periods with strongly changing SSTs and decadal SSR depending on the regions. Unforced clear-sky SSR trends appear to mimic the SST trend pattern, while all-sky trends show a complex spatial structure with trends opposite in sign in different regions. These results are based only on pre-industrial control simulations (CMIP6 piControl) and can be used to infer in which direction internal variability has affected SSR in the historical period and whether it has enhanced or suppressed the anthropogenic signal from aerosols.

How to cite: Chtirkova, B., Folini, D., Ferreira Correa, L., and Wild, M.: Low-frequency modes in internal variability of surface solar radiation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5155, https://doi.org/10.5194/egusphere-egu23-5155, 2023.

EGU23-5372 | ECS | Orals | CL2.1

Direct observation of Earth’s spectral longwave feedback parameter 

Florian E. Roemer, Stefan A. Buehler, Manfred Brath, Lukas Kluft, and Viju O. John

The spectral longwave feedback parameter λν represents how Earth’s outgoing longwave radiation adjusts to temperature changes and is thus the detailed fingerprint of all longwave feedbacks, directly impacting Earth’s climate sensitivity. Most research so far has focused on the spectral integral of λν. Spectrally resolving λν permits inferring information about the vertical distribution of longwave feedbacks, thus gaining a better understanding of the underlying processes. However, investigations of λν have so far been largely limited to model studies, and no observational study we are aware of has inferred the global all-sky λν.

Here we show that it is possible to directly observe the global all-sky λν using satellite observations of seasonal and interannual variability taken by the Infrared Atmospheric Sounding Interferometer (IASI). We find that spectral bands subject to strong water vapour absorption exhibit a substantial stabilising net feedback. We demonstrate that this stabilising feedback is partly caused by changes in relative humidity with warming, the radiative fingerprints of which can be directly observed. Therefore, our findings emphasise the importance of better understanding processes affecting future trends in relative humidity. This first observational constraint on the global all-sky λν can be used as a powerful tool to evaluate the representation of longwave feedbacks in global climate models and to better constrain Earth’s climate sensitivity.

How to cite: Roemer, F. E., Buehler, S. A., Brath, M., Kluft, L., and John, V. O.: Direct observation of Earth’s spectral longwave feedback parameter, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5372, https://doi.org/10.5194/egusphere-egu23-5372, 2023.

EGU23-5727 | ECS | Orals | CL2.1

Aerosol Radiative Forcing Over Indian Subcontinent for 2000-2021 using satellite observations 

Shreya Srivastava, Sushovan Ghosh, and Sagnik Dey

Aerosols directly affect Earth’s radiation budget by scattering and absorbing incoming solar radiation and outgoing terrestrial radiation. While the uncertainty in aerosol radiative forcing (ARF) has decreased over the years, it is still higher than that of greenhouse gas forcing, particularly in the South Asian region, due to high heterogeneity in aerosols’ chemical properties. India has been identified as an aerosol hotspot. Understanding the Spatiotemporal heterogeneity of aerosol composition is critical in improving ARF estimation.                            

In this study, we have taken aerosol data from Multi-angle Imaging Spectro-Radiometer (MISR) level-2 version 23 aerosol products retrieved at 4.4 km and radiation data from Clouds and the Earth’s Radiant Energy System (CERES, spatial resolution=1ox1o), for 21 years (2000-2021) over the Indian subcontinent. MISR aerosol product includes size and shapes segregated aerosol optical depth (AOD), Angstrom exponent (AE), and single scattering albedo (SSA). Additionally, 74 aerosol mixtures included in version 23 data are used for aerosol speciation. In addition, we have used CERES radiation data in four different atmospheric conditions: all-sky (AS), clear-sky (CS), pristine (PR) and no aerosol (NAER), for estimating aerosol radiative forcing in different aerosol-cloud conditions.

We have seasonally mapped aerosol optical and microphysical properties from MISR for India at quarter degrees resolution. Results show strong Spatio-temporal variability, with a constant higher value of AOD for the Indo-Gangetic Plain (IGP). The fractional contribution of small-size particles to AOD is higher (>0.4) throughout the year, spatially during post-monsoon and winter seasons (October to February). SSA is found to be overestimated by MISR, where absorbing particles are present. The climatological map of short wave (SW) ARF at the top of the atmosphere (TOA) shows a strong cooling except in only a few places (values ranging from +2.5W/m2 to -22.5 W/m2). Cooling due to aerosols is higher in the absence of clouds. Higher aerosol cooling is found over the IGP region, given the high aerosol concentration over the region. Aerosols are causing a surface cooling effect over our study domain, which is higher in clear conditions. The results strongly correlate with AOD from MISR and ARF from CERES. 

How to cite: Srivastava, S., Ghosh, S., and Dey, S.: Aerosol Radiative Forcing Over Indian Subcontinent for 2000-2021 using satellite observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5727, https://doi.org/10.5194/egusphere-egu23-5727, 2023.

EGU23-6217 | Orals | CL2.1

Concept and validation of a Meteosat based dataset for Surface Radiative Balance 

Quentin Bourgeois, Anke Tetzlaff, Reto Stöckli, Nicolas Christen, John Viju, William Moutier, Nicolas Clerbaux, Françoise Gellens-Meulenberghs, Jörg Trentmann, and Isabel Trigo

During the Third Continuous Development and Operations Phase (CDOP-3) of EUMETSAT, the Satellite Application Facility (SAF) on Climate Monitoring (CM SAF) extends its product portfolio with a Thematic Climate Data Record (TCDR) of Regional Land Fluxes based on two sensors of the Meteosat suite of geostationary satellites: the Meteosat Visible and InfraRed Imager (MVIRI) and the Spinning Enhanced Visible and InfraRed Imager (SEVIRI). The Regional Land Fluxes TCDR will provide various parameters depicting the surface states and radiation fluxes, including the Surface Radiative Balance (SRB), the Cloud Fractional Cover (CFC), the Land Surface Temperature (LST), the Evapotranspiration (ET) and the Latent (LE) and Sensible (H) Heat Fluxes. The TCDR is achieved by consolidating and unifying previously separated developments in CM SAF, LSA SAF and the EUMETSAT Secretariat, and running them in a joint retrieval using the Meteosat Fundamental Climate Data Record. This unique concept ensures consistency among the TCDR parameters.

We focus here on the SRB product of the Regional Land Flux TCDR. All components of the SRB - including the Surface Incoming Solar radiation (SIS, or solar irradiance), the Surface Albedo (SAL), the Surface Outgoing Longwave radiation (SOL) and the Surface Downward Longwave radiation (SDL) - are jointly retrieved using the CM SAF software “GeoSatClim” over the period 1983-2020. The SRB data record covers area up to 65°N/S and 65°W/E. The TCDR consists in hourly, daily and monthly means with a spatial resolution of 0.05 degree.

In this presentation, we show the detailed concept of the SRB algorithm. The SRB product and its single components are validated with BSRN, GEBA, ASRB and SwissMetNet ground based stations and they are compared with other global SRB products such as ERA5-Land, ISCCP-FH and CLARA. Overall, the SRB monthly mean absolute bias reaches the target accuracy of 15 W.m-2, and the SRB stability falls below the requirement of 2 W/m2/decade.

How to cite: Bourgeois, Q., Tetzlaff, A., Stöckli, R., Christen, N., Viju, J., Moutier, W., Clerbaux, N., Gellens-Meulenberghs, F., Trentmann, J., and Trigo, I.: Concept and validation of a Meteosat based dataset for Surface Radiative Balance, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6217, https://doi.org/10.5194/egusphere-egu23-6217, 2023.

EGU23-6759 | Posters on site | CL2.1

The Global Energy Balance as represented in CMIP6 climate models 

Martin Wild, Doris Folini, and Donghao Li

A plausible simulation of the global energy balance is a first-order requirement for a credible climate model. Therefore we investigate the representation of the global energy balance in the latest generation of global climate models (CMIP6). In the multi-model global mean, the magnitudes of the energy balance components of the CMIP6 models are often in better agreement with our reference estimates (Wild et al. 2015, 2019 Clim Dyn) as well as those from CERES/EBAF and NASA/NEWS than in earlier model generations (Wild 2020). However, the inter-model spread in the representation of many of the components remains substantial, often on the order of 10-20 Wm-2 globally, except for the shortwave clear-sky budgets, which are now more consistently simulated by the CMIP6 models. The substantial inter-model spread in the simulated global mean latent heat fluxes in the CMIP6 models, exceeding 20% (18 Wm-2), further implies also large discrepancies in their representation of the global water balance. From a historic perspective of model development over the past decades, the largest adjustments in the magnitudes of the simulated present-day global mean energy balance components occurred in the shortwave atmospheric clear-sky absorption and the surface downward longwave radiation. Both components were gradually adjusted upwards over several model generations, on the order of 10 Wm-2, to reach 73 and 344 Wm-2, respectively in the CMIP6 multi-model means. Thereby, CMIP6 has become the first model generation that largely remediates long-standing model deficiencies related to an overestimation in surface downward shortwave and compensational underestimation in downward longwave radiation in its global multi-model mean. There are also indications for an overall improvement in the representation of the energy budgets in the CMIP6 models compared to CMIP5 on regional scales (regions considered here as defined by the NASA/NEWS project). Still substantial spreads between the energy balance components of individual CMIP6 models appear also on regional scales (Li et al. 2022).

 

Related references:

Wild, M., 2020: The global energy balance as represented in CMIP6 climate models. Clim Dyn., 55, 553–577

Li, D., Folini D., Wild, M., 2022: Assessment of regional energy budgets in CMIP6 models, submitted

 

 

How to cite: Wild, M., Folini, D., and Li, D.: The Global Energy Balance as represented in CMIP6 climate models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6759, https://doi.org/10.5194/egusphere-egu23-6759, 2023.

EGU23-7024 | ECS | Posters on site | CL2.1

Assessment of land energy uptake in the industrial period from observation and simulation-based products 

Félix García-Pereira, Jesús Fidel González-Rouco, Norman Julius Steinert, Camilo Melo-Aguilar, Philipp de Vrese, Johann Jungclaus, Stephan Lorenz, Stefan Hagemann, and Elena García-Bustamante

Under increased warming from ongoing anthropogenic climate change, the land acts as an energy sink for the climate system, interacting with the atmosphere at a wide range of time scales. Based on CMIP multi-model comparisons, the latest estimates of the global energy budget quantify the land contribution to be 2% in the last six decades, whereas other studies based on borehole temperature profiles scale it up to 5%. This discrepancy is suspected to stem from state-of-the-art CMIP land surface models using a shallow zero flux bottom boundary condition placement (BBCP) that severely constrains land energy storage by halting ground heat flux penetration at the BBCP depth and biasing subsurface thermal structure. A 2000-year-long (past2k) forced simulation using a version of the Max Planck Institute (MPI) Earth System Model (ESM) with a deep BBCP (1417 m) was performed to assess the behavior of subsurface temperature and energy storage at long-term scales. Results show that land energy uptake is 4 times higher in a coupled MPI-ESM simulation with a deep version of the land component compared to standard shallow (~10m) simulations. These estimates are well above those provided by CMIP6 models and are much closer to observations, underlining the importance of BBCP-depth in correctly representing the role of the land component in the global energy budget. The results of the analysis of the past2k simulation also allow for deriving reliable estimates of land energy uptake from other observational and reanalysis products as well as providing corrected estimates for the shallow LSM CMIP6 historical and scenario simulations. Land energy uptake estimates rendered from this new approach are much closer to previous BTP-based estimates and agree with the value derived from MPI-ESM deep simulation.

How to cite: García-Pereira, F., González-Rouco, J. F., Steinert, N. J., Melo-Aguilar, C., de Vrese, P., Jungclaus, J., Lorenz, S., Hagemann, S., and García-Bustamante, E.: Assessment of land energy uptake in the industrial period from observation and simulation-based products, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7024, https://doi.org/10.5194/egusphere-egu23-7024, 2023.

Anthropogenic aerosol particles affect clouds by serving as cloud condensation nuclei, thus significantly influencing Earth’s energy balance. The magnitude of aerosol-induced changes in cloud properties is still uncertain. This is primarily due to the meteorological covariability between aerosols and clouds, which hinders inferring causal relationships. Industrial air pollution sources serve as natural experiments to study strong anthropogenic cloud perturbations (Toll et al. 2019 Nature https://doi.org/10.1038/s41586-019-1423-9) and allow us to infer causal relationships between aerosols and clouds.

 

We use geostationary satellite observations to study the temporal evolution of polluted clouds. Polluted clouds are usually thinner than nearby unpolluted clouds. But in some cases, the polluted clouds grow much thicker in the afternoon than the nearby unpolluted clouds. We find that continental polluted cloud tracks are relatively long-lived, with a median lifetime of 18 hours. Moreover, there are many cases where polluted cloud tracks are visible for multiple consecutive days. This means polluted cloud tracks live long enough for clouds to fully adjust to aerosol-increased cloud droplet numbers. Future work is needed to combine geostationary and polar orbiting satellite observations of polluted cloud tracks to develop stronger observational constraints for aerosol-cloud interactions.

How to cite: Rahu, J. and Toll, V.: Novel insights into aerosol-cloud interactions enabled by analysing the temporal evolution of strong anthropogenic cloud perturbations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7090, https://doi.org/10.5194/egusphere-egu23-7090, 2023.

Multidecadal dimming and brightening of solar radiation at Earth’s surface has been shown to occur over all continents. Trends have been especially well documented over the Northern Hemisphere (NH) with dimming from the 1950s through the middle 1980s followed by brightening through the first decade of the 2000s in the United States, Europe, and parts of Asia. Trends in Europe and China have been attributed to both aerosols and clouds, but in the U.S. cloud variability has been dominant. A recent analysis shows that U.S. brightening of 7.4 Wm-2/decade peaked in 2012 and then dramatically dropped to near normal values in 2013. Since then, surface solar radiation in the U.S. has remained within 1 Wm-2 of the long-term average. However, in Europe surface solar radiation has remained high, at least through 2017.

 

It has been shown that the direct effect of aerosols cannot account for the magnitude of the latest brightening in the U.S. It has also been shown that the second indirect effect of aerosols may explain brightening into the first decade of the 2000s, but is in opposition to the observed dimming after 2012. High aerosol content does explain perpetual dimming in India and industrial parts of China, but, given that the magnitude and period of dimming and brightening trends from the 1950s through the first decade of the 2000s are similar over North America, Europe, and parts of Asia, I speculate the primary cause is meteorological. A recent study documents a strong association between multidecadal surface solar radiation trends over NH continents and long-term North Pacific and North Atlantic sea surface temperature (SST) patterns. For example, the reversal of the Pacific Decadal Oscillation (PDO) index in the mid-1980s is nearly simultaneous with the change from dimming to brightening over NH continents. A similar association is shown between Atlantic SST patterns and continental surface solar radiation trends but with a decade lag. Using reanalysis and observed SST patterns it is demonstrated that persistent warm SST anomalies support overlying semipermanent geopotential height ridges at tropospheric mid-levels that dynamically induce persistent troughs downstream over adjacent continents, if positioning is favorable. Semipermanent troughs over the continents cause greater than average cloud cover and dimming. Conversely, long-term cool SSTs produce the opposite scenario and yield less clouds and brightening downstream over the continents. Further, marine heat waves on either side of North America are shown to be associated with the recent dimming in the midcontinent from 2013 to the present, and warm SSTs in the Mediterranean and North Seas in the last decade are likely responsible for a persistent midlevel geopotential ridge pattern and continued high surface solar radiation there. Recent studies present evidence that the observed increase in frequency and variability of marine heat waves in the past few decades may be associated with global warming, possibly linking warming to trends in surface solar radiation.

How to cite: Augustine, J.: Contributors to multidecadal dimming and brightening of surface solar radiation over Northern Hemisphere continents, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8365, https://doi.org/10.5194/egusphere-egu23-8365, 2023.

EGU23-8463 | ECS | Orals | CL2.1

Global energy budget changes from underestimated land heat uptake in CMIP6 models 

Norman Julius Steinert, Jesús Fidel González-Rouco, Philipp de Vrese, Francisco José Cuesta-Valero, Félix García Pereira, and Camilo Andrés Melo Aguilar

Under current climate-change conditions, the energy imbalance at the top of the atmosphere results in an uptake of energy by the Earth system. Previous efforts have identified the magnitude and proportions of this energy excess and how it is distributed among the different components of the climate system. However, the bulk of the Earth System Models (ESMs) participating in CMIP5/6 deliver Earth energy inventory estimates that differ substantially from recent observations. Particularly for the land component, there is a significant underestimation of simulated continental energy uptake, which was hypothesized to be caused by too shallow land surface model components in current-generation ESMs. Support for the latter was given by previous modeling estimates based on analytical heat conduction models and standalone land surface model simulations. Here we use a suite of current-generation fully-coupled CMIP6 ESMs and a version of the MPI-ESM that includes a deep land model component, accommodating the required space for increased terrestrial energy storage. The simulations show that a sufficiently deep land model leads to more realistic subsurface energy storage - correlating with model depth rather than climate sensitivity, and an adjusted estimate of energy uptake ratios among the Earth system components compared to observational estimates. However, the impact of changes in the land energy budget from the perspective of the entire Earth system appears to have only a marginal influence due to its relatively small fraction of the Earth energy inventory.

How to cite: Steinert, N. J., González-Rouco, J. F., de Vrese, P., Cuesta-Valero, F. J., García Pereira, F., and Melo Aguilar, C. A.: Global energy budget changes from underestimated land heat uptake in CMIP6 models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8463, https://doi.org/10.5194/egusphere-egu23-8463, 2023.

EGU23-8983 | Orals | CL2.1

Aerosol Radiative Forcing time development in the CMIP6 historical experiment 

Ragnhild Bieltvedt Skeie and Gunnar Myhre

In this study, radiative forcing time series on a component basis from the historical experiment in CMIP6 are presented. For each aerosol component (sulphate, black carbon, organic aerosols, nitrate) aerosol radiative forcing for aerosol-radiation interaction (RFari) is calculated from 1850 to 2014 using a radiative kernel and modelled changes in aerosol mass. The radiative kernel has been generated using the DISORT radiative transfer model. Aerosol radiative forcing for aerosol-cloud interaction (RFaci) is calculated offline based on the monthly fields from CMIP6 and simulate changes in the effective radius. For the individual models the time development of total aerosol radiative forcing is compared to aerosol effective radiative forcing (ERF) time series calculated within RFMIP, that take into account the adjustments. The radiative forcing trend will be presented on a global and a regional scale. The calculations are also done for the AeroCom phase III historical experiment. Both the AeroCom phase III and CMIP6 historical experiment use the CMIP6 CEDS emissions. These emissions are recently updated and extended. Using results from a chemistry transport model (OsloCTM3) we show how the updated emissions have changed the radiative forcing trends in the model. The emissions used to drive the models play an important role for determining the time development of the aerosol radiative forcing. At the end we will discuss uncertainties in the trend based on available historical global emission inventories for aerosol and aerosol precursors.

How to cite: Skeie, R. B. and Myhre, G.: Aerosol Radiative Forcing time development in the CMIP6 historical experiment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8983, https://doi.org/10.5194/egusphere-egu23-8983, 2023.

EGU23-9084 | ECS | Posters on site | CL2.1

Determining Earth’s outgoing radiative flux from a Moon-Based Wide Field-of-view Radiometer 

yuan zhang, Shengshan Bi, and Steven Dewitte

Observing the Earth radiation budget (ERB) at top of the atmosphere (TOA) from space is crucial for monitoring and understanding Earth’s climate. The accurate estimation of Earth’s outgoing radiative flux is of critical importance to studying ERB at TOA. The Moon-based wide field-of-view radiometer (MWFVR) can provide long-term, continuous full-disk broadband irradiance measurements, which provides an important data source for studying the ERB. Within this context, the lunar surface site 0° E 0° N is selected as the position of the Moon-based wide field-view radiometer, and based on the radiation transfer function, the entrance pupil irradiances time series are obtained by utilization of the CER_SYN1deg-1Hour_Edition4 data products and ERBE ADMs, which is used as the substitute for the truth of the measurements. In this work, the Earth outgoing radiative flux estimating model from the MWFVR measurements is established, and according to the framework, the entrance pupil irradiances are converted to full-disk LW and daytime SW outgoing radiative fluxes. By comparing the results from Moon-based radiometer measurements with those from NISTAR data and CERES SYN1deg data, the results show the moon-based data a much better agreement with those from the satellite data. Besides, The Moon-based SW fluxes oscillate around 194 and 205 W∙m-2, and the range of LW fluxes is 251 ~ 287 Wm−2. Therefore, the complementary advantages and cooperative work of platforms at different altitudes will be an important way for future research on the ERB.

 

 

How to cite: zhang, Y., Bi, S., and Dewitte, S.: Determining Earth’s outgoing radiative flux from a Moon-Based Wide Field-of-view Radiometer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9084, https://doi.org/10.5194/egusphere-egu23-9084, 2023.

EGU23-10334 | ECS | Posters on site | CL2.1

Using Brutsaert’s Equation to Understand the Spatiotemporal Variations of Downwelling Longwave Radiation 

Yinglin Tian, Axel Kleidon, Sarosh Alam Ghausi, Deyu Zhong, and Guangqian Wang

Downwelling longwave radiation (Rld) is a dominant term in the surface energy balance and is central to global warming. It is influenced by the radiative properties in the whole atmospheric column, particularly greenhouse gases, water vapor, clouds, and atmospheric heat storage. To reveal the leading terms responsible for the spatiotemporal climatological variations in Rld, we use the semi-empirical equation derived by Brutsaert (1975, “B75”), which only needs near-surface observations of air temperature and humidity. We first evaluated B75 and its extension by Crawford and Duchon (1999, "C&D99") with FLUXNET observations, NASA-CERES satellite data, and ERA5 reanalysis. We found a strong agreement, with R2 being 0.87, 0.97, and 0.99, respectively. We then used the equations to show that diurnal and seasonal variations in Rld are predominantly controlled by changes in atmospheric heat storage. Variations in atmospheric emissivity form a secondary contribution to the variation of Rld, and are mostly controlled by anomalies in cloud cover. We also found that with increased aridity, the contributions by changes in atmospheric heat storage and emissivity acted to compensate each other (20~30 W/m2 and ~-40 W/m2, respectively), thus explaining the relatively little variation in Rld with aridity (-20~-10 W/m2). The equations further indicate that under global warming, the amplification of water vapor is stronger in arid regions because clear-sky conditions are more sensitive to an increase in greenhouse gases. These equations thus provide a firm, physical basis to understand the spatiotemporal variability of downwelling longwave radiation at the surface. This should be helpful to better understand and interpret climatological changes, for instance those associated with global warming and extreme events.

How to cite: Tian, Y., Kleidon, A., Alam Ghausi, S., Zhong, D., and Wang, G.: Using Brutsaert’s Equation to Understand the Spatiotemporal Variations of Downwelling Longwave Radiation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10334, https://doi.org/10.5194/egusphere-egu23-10334, 2023.

The outgoing longwave radiation (OLR) at the top of the atmosphere is a critical component of the Earth's radiation energy budget. A substantial portion of the OLR energy lies in the far-infrared (FIR) spectrum, which has not been directly measured for understanding weather and climate variations. Several satellite projects under development, including the Thin Ice Cloud in Far Infrared Experiment (TICFIRE, Blanchet et al. 2011) funded by the Canadian Space Agency, the Polar Radiant Energy in the Far Infrared Experiment (PREFIRE, L’Ecuyer et al., 2021) of U.S. NASA, and the Far-Infrared Outgoing Radiation Understanding and Monitoring (FORUM, Palchetti et al., 2020) of the European Space Agency, are being developed to fill this observation gap. Given that the FIR observation data is not available yet, we use simulations to acquire prior knowledge of the climatological mean distribution of the OLR in FIR, by using a rapid radiative transfer model, RRTMG, to simulate spectrally decomposed OLR in different spectral bands from global instantaneous atmospheric profiles of the fifth generation European Centre for Medium-Range Weather Forecasts atmospheric reanalysis (ERA5). Based on the radiative transfer equation, we dissect the OLR by attributing its distribution and variation to spectrally and vertically decomposed contributions of the atmosphere and Earth surface. Our results disclose that the relatively higher far-infrared fraction of the OLR in polar region is due to stronger surface contribution and identify a minimum atmospheric contribution layer around the tropopause. On the other hand, the variability of the spectrally decomposed OLR field is dissected with the aid of a new set of radiative sensitivity kernels. This analysis discovers that the non-cloud longwave climate feedback, as well as its inter-climate model discrepancy, mainly results from the upper tropospheric thermodynamic fields (temperature and water vapor) and their effects on the FIR radiation.

How to cite: Huang, H. and Huang, Y.: The spectrally and vertically decomposed outgoing longwave radiation and its climate trends in the far-infrared, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10455, https://doi.org/10.5194/egusphere-egu23-10455, 2023.

EGU23-10502 | Posters virtual | CL2.1

From Quantum Mechanics to Climate Change: Global Warming From First Principles 

Robin Wordsworth, Jacob Seeley, and Keith Shine

Although the scientific principles of anthropogenic climate change are now extremely well-established, all existing descriptions of the physics of global warming are either partly empirical or rely on the results of complex numerical models. Here, we present a description of radiative forcing and climate sensitivity that begins from the basic quantum properties of the CO2 molecule. The shape of the CO2 15 micron band, which is so critical to the strength of CO2 radiative forcing, can be understood in terms of vibrational-rotational states and a quantum resonance effect (Fermi resonance). We discuss how classical analogy to the coupled pendulum experiment can be used to understand the nature of this phenomenon in simple terms. We finish by deriving a new analytic equation for CO2 radiative forcing expressed in terms of basic molecular properties such as bond strength and atomic mass. Our aim is for this analysis to elucidate the fundamental physics of climate change for both climate scientists and for physicists working in other fields.

How to cite: Wordsworth, R., Seeley, J., and Shine, K.: From Quantum Mechanics to Climate Change: Global Warming From First Principles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10502, https://doi.org/10.5194/egusphere-egu23-10502, 2023.

EGU23-11280 | ECS | Orals | CL2.1

Contribution of cloudy/clear-sky partitions and aerosol variability to the solar irradiance measured over 2010-2020 in Northern France 

Gabriel Chesnoiu, Nicolas Ferlay, Frédérique Auriol, Maxime Catalfamo, Isabelle Jankowiak, and Isabelle Chiapello

The absorption and scattering by aerosols and clouds greatly affect surface solar irradiance and the Earth's energy budget. Large uncertainties still remain on the current estimates of these radiative effects because of an incomplete knowledge of their spatial and temporal variabilities.

 

We analyze coincident daytime ground-based measurements of aerosol optical properties from AERONET photometer and of direct and diffuse horizontal surface irradiances from a set of pyrheliometer and pyranometer routinely performed at the ATOLL (Atmospheric Observations in LiLle) platform in north of France over the period 2010-2020. The site is located in a highly populated area greatly influenced by clouds and aerosol pollution. In order to isolate the radiative effect of aerosols from that of cloud occurences, a separation between cloudy-sun, clear-sun with surrounding clouds and clear-sky moments is performed using two cloud detection algorithms at 1-min resolution. The measurements are further analyzed using a radiative transfer code to simulate the spectrally integrated solar global horizontal irradiance and its components in clear-sky conditions with and without aerosols (pristine like conditions).

 

Our analysis shows that on average in ATOLL over the period 2010-2020, the sky is cloudy 89% of the time with around 67% of cloudy-sun situations and 22% of clear-sun with clouds moments. The proportion of clear-sky conditions is relatively low (11%) with a minimum in winter (6%) and a maximum in spring (15%).

 

In summer, we observe over the period a robust increasing trend in measured total irradiances in all-sky conditions of +5.2 ± 1.8 W/m²/year. This evolution is mainly explained by a positive trend in the occurrence of clear-sky situations (+0.7 ± 0.3% per year) to the detriment of cloudy-sun moments.

 

In spring, we highlight a high variability of cloud occurences and mean solar irradiances. Indeed, the mean proportion of clear-sky moments varies more than fourfold between 2013 (8%) and 2020 (35%), leading to corresponding all-sky irradiance extrema of 285 and 389 W/m² respectively. Moreover, in clear-sky conditions, an important variability is observed between the maximum of seasonal global irradiance of spring 2018 (522 W/m²) and the minimum of spring 2014 (435 W/m²). The latter variability is emphasised by a significative positive trend in direct irradiances observed for springtime clear-sky conditions of +5.3 ± 2.3 W/m²/year. A sensitivity analysis based on our radiative simulations shows that it is partly explained by a significant decrease in measured AOD440 nm (-0.006 ± 0.002 per year) and a change in the proportion of high aerosol loads over 2010-2020. This is also consistent with a negative trend of the diffuse component (-1.2 ± 0.4 W/m²/year) observed for clear-sky conditions in spring.

 

Finally, besides showing the highest proportion of clear-sky moments, spring is also the most polluted season in aerosol, with more than 80% of AOD440 nm higher than 0.1. This translates to an average seasonal maximum of aerosol direct radiative effect in spring of -22.6 W/m² (-6.1%), with a loss of -69.3 W/m² (-19.2%) of direct irradiance partially compensated by an increase of the diffuse radiation of +46.6 W/m² (101.0%).

How to cite: Chesnoiu, G., Ferlay, N., Auriol, F., Catalfamo, M., Jankowiak, I., and Chiapello, I.: Contribution of cloudy/clear-sky partitions and aerosol variability to the solar irradiance measured over 2010-2020 in Northern France, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11280, https://doi.org/10.5194/egusphere-egu23-11280, 2023.

Downwelling longwave irradiance (LW) is challenging and expensive to measure and is often estimated indirectly with parametric modeling of routinely measured surface-level meteorological variables.  Modeling LW under all-sky conditions typically involves “correcting” a clear- (or non-overcast) sky model estimate using solar-irradiance-based proxies of cloud cover in lieu of actual cloud cover given uncertainties and measurement challenges of the latter.  While such approaches are deemed sound, their application in time and space is inherently limited.  Here, we present a correction model free of cloud variables applicable at the true daily (24-hr.) and global scale that – irrespective of the underlying clear-sky model – yields errors over land that are lower than those from stand-alone models and on par with daytime errors from the prevailing solar-based cloud proxy corrections (rRMSD = ~7%; rMAD = ~5.5%).  We document and critically assess its performance over land and ocean independently, as well as in high elevation and cold environments representing two notoriously challenging conditions.  The cloud-free correction is found to perform better than stand-alone approaches at all subsets; however, within-subset performance differences were evident and attributable to the underlying clear-sky model, reinforcing previous findings surrounding performance thresholds of parametric models with globally-tuned parameters. 

How to cite: Bright, R. and Eisner, S.: Modeling downwelling longwave irradiance at daily resolution under all skies:  A cloud-free approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11494, https://doi.org/10.5194/egusphere-egu23-11494, 2023.

EGU23-11930 | Orals | CL2.1 | Highlight

Fingerprint of CO2 and other gases on the greenhouse effect from direct satellite observation 

Chris Rentsch and Gunnar Myhre

We use 19 years of continuous near-global land and ocean direct AIRS satellite measurements combined with detailed atmospheric radiative transfer modelling to demonstrate strong strengthening in the greenhouse effect caused by CO2 and detectable, but comparatively smaller strengthening, by CH4 and N2O. An increase in the outgoing longwave radiation is found in the 800-1000 cm−1 atmospheric window resulting from the Planck response to surface heating. The combined use of satellite measurements and the radiative transfer model also demonstrate that reductions in concentrations of prohibited ozone depleting substances have weakened the greenhouse effect in the spectral region where these gases absorb thermal infrared radiation. The strong greenhouse effect strengthening signal in the satellite data in the spectral region 710-720 cm−1 is a fingerprint of CO2 increase since we demonstrate that other factors could not cause such a robust spectral feature. We show how the spectral clear sky instantaneous change in TOA flux relates to the greenhouse gas radiative forcing over the 19-year period.

How to cite: Rentsch, C. and Myhre, G.: Fingerprint of CO2 and other gases on the greenhouse effect from direct satellite observation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11930, https://doi.org/10.5194/egusphere-egu23-11930, 2023.

EGU23-12198 | Posters on site | CL2.1

Advances in ISCCP-based Surface Fluxes at Higher Spatial Resolution from the Surface Radiation Budget Project 

Paul Stackhouse, Stephen Cox, J. Colleen Mikovitz, and Taiping Zhang

The NASA Langley Research Center (LaRC) Surface Radiation Budget (SRB) project produced 3-hourly shortwave and longwave surface and top of atmosphere radiative fluxes for the 1983-2017 in its most recent version, Release 4 Integrated Product (IP) in collaboration with other GEWEX collaborators (Kummerow et al., 2019, Stackhouse et al., 2020, ATBD). This version uses the newly recalibrated and processed ISCCP HXS product as its primary input for cloud and radiance data, replacing ISCCP DX with a ninefold increase in pixel count (10 km instead of 30 km).  Previous work showed comparisons to BSRN and to ocean buoy measurements showed ensemble agreement for monthly averaged shortwave (SW or solar) wavelengths to be ~1 W m-2 bias with an RMS of 14.7 W m-2 RMS and longwave (LW or thermal infrared) ~+1 W m-2 bias with a 15.9 W m-2 RMS.  However, we also found that utilizing the Tselioudis (2020) weather state analysis with ISCCP to partition fluxes by cloud state over the BSRN sites showed that particular cloud states, such as the convective cloud state, showed much larger biases, particularly in the SW.

To address such issues, and to better resolve surface radiative flux spatial variability, this talk describes advances to the SRB inputs and algorithms towards the next release, referred to as LaRC SRB future Release 5. Since the resolution of ISCCP HXS is 10 km (excluding pixels within 25 km of coast lines), the ISCCP data products have enough sampling to grid cloud properties at the 0.5°x0.5°on a global basis.  In the shortwave, the Pinker-Laszlo lookup table approach with a forward call to the Fu-Liou radiative transfer model as modified by the CERES team (Rose et al., 2006).  In addition to being a proven radiation code, Fu-Liou allows the calculation of fluxes at different atmospheric levels and spectral bands, which will provide more insight into the surface radiation budget, its variability and attribution.  Updates to various inputs are described such as surface spectral albedos, emissivities, surface skin and near-surface temperatures, atmospheric profiles, and aerosols optical properties.  

This talk presents the results of early versions of the new products from grid boxes containing BSRN and ocean buoy measurement sites and compare these surface fluxes to the previous version and also to other prominent available data products in the literature.  Key regional differences over oceans and land are assessed to evaluate the changes in the resolving the flux variability.  Although the Tselioudis “weather states” are classified for a 1°x1° resolution, an initial flux partitioning is made at both full and a degraded 1°x1° resolution to assess the new algorithms under different cloud state conditions. The newer algorithms rely on the Fu-Liou based radiative transfer for both the SW and LW providing fluxes within the atmosphere and at the surface and for spectral band fluxes. 

How to cite: Stackhouse, P., Cox, S., Mikovitz, J. C., and Zhang, T.: Advances in ISCCP-based Surface Fluxes at Higher Spatial Resolution from the Surface Radiation Budget Project, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12198, https://doi.org/10.5194/egusphere-egu23-12198, 2023.

EGU23-12792 | ECS | Posters on site | CL2.1

Investigating the role of 3D radiative effects in contrail cirrus and ice clouds. 

Julie Carles, Jean-Louis Dufresne, and Nicolas Bellouin

The aviation sector contributes to anthropogenic radiative forcing via impacts from well-known CO2 effects and more uncertain non-CO2 effects. The largest contributor to aviation radiative forcing is one of the non-CO2 effects: induced cirrus cloudiness evolved from contrails generated by aircrafts that persist in the atmosphere. The latest assessment of the impacts of aviation on climate attributes a forcing of 149.1 (90% confidence range: 70, 229) mW/m² to global aviation, including 111.4 (33, 189) mW/m² from contrail cirrus (Lee et al, 2021). Those estimations are based on results from global climate models which use approximations for the description of clouds and radiative transfer, resulting in uncertainties of about 70% in aviation induced cloudiness radiative forcing. As of today, the 3D nature of clouds and the corresponding 3D radiative effects are neglected in climate models, as well as the size and shape of ice crystals in contrails.

In this poster, we present work aimed at improving the estimation of the radiative effect of ice clouds and contrail cirrus by studying its dependence on cloud geometry and size. This work uses a Monte Carlo radiative transfer code that takes into account the full 3D interactions between clouds and radiation (Villefranque et al 2019). Results are compared to a 1D, plane parallel calculation, which is the common assumption in climate models used to estimate radiative forcing.

Results show that 3D effects play a substantial role in the radiative effect of cirrus clouds. The plane parallel calculations always under-estimate cloud radiative effect compared to Monte Carlo calculations when the Sun is at zenith. We discuss the dependence of the results to solar angle. We find that the optical depth of the contrail is not the only driver of its radiative forcing, contrary to behavior in plane parallel calculations. This work contributes to reducing uncertainty in the radiative forcing of aviation, and may over ways to correct estimates of contrail cirrus radiative forcing and high clouds radiative effect in climate models.

How to cite: Carles, J., Dufresne, J.-L., and Bellouin, N.: Investigating the role of 3D radiative effects in contrail cirrus and ice clouds., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12792, https://doi.org/10.5194/egusphere-egu23-12792, 2023.

EGU23-13064 | ECS | Orals | CL2.1

The Global Dimming & Brightening based on FORTH radiative transfer model during 1984-2018 and its evaluation against GEBA & BSRN ground-based networks 

Michael Stamatis, Nikolaos Hatzianastassiou, Marios Bruno Korras Carraca, Christos Matsoukas, Martin Wild, and Ilias Vardavas

The Earth’s energy balance and radiation budget, which play a key role in the Earth’s climate system, are driven by the incident solar radiation at surface (surface solar radiation, SSR). Over the past few decades, changes in the SSR (ΔSSR) have been observed that are dependent on the transparency of the terrestrial atmosphere. This phenomenon, called global dimming and brightening (GDB), is a significant factor in climate change and modulates global warming. This study examines the interdecadal variability of SSR based on computations of the FORTH radiative transfer model, using as input data cloud optical properties taken from the International Satellite Cloud Climatology Project H Series (ISCCP-H) and aerosol optical properties and meteorological data taken from the Modern-Era Retrospective analysis for Research and Applications, version 2 (MERRA-2) Reanalysis. Ground-based measurements of SSR from the Global Energy Balance Archive (GEBA) and Baseline Surface Radiation Network (BSRN) networks are utilized to evaluate the FORTH’S SSR fluxes and GDB. The FORTH RTM computations are made on a monthly basis from 01/1984 - 12/2018 at 51 atmospheric levels and a spatial horizontal resolution of 0.5°×0.625° (with a conversion of the original input data to the same spatio-temporal resolution). Firstly, the FORTH SSR fluxes are evaluated against ground measurements from GEBA and BSRN. This comparison reveals a general underestimation of the FORTH SSR fluxes, with a satisfactory evaluation metrics, such as the relative bias, which is equal to –2.9% and –7.7% against GEBA and BSRN, respectively or the correlation coefficient values, computed using deseasonalized SSR anomalies, being equal to 0.72 and 0.8 against GEBA and BSRN, respectively. Then, the SSR changes (or GDB) for each pixel, also calculated using deseasonalized SSR anomalies, were compared with the GDB from the corresponding GEBA/BSRN station, lying in that pixel, for their common time period. This comparison reveals an agreement between the sign of the FORTH’s pixels and the corresponding stations’ GDB equal to 63.5% for the GEBA and 54.5% for the BSRN sites. Finally, the GDB was also calculated on global (land & ocean), hemispherical and regional scales, either for the entire period and for sub-periods too. The computed GDB for the period 01/1984-12/2018 is equal to –2.22 ± 0.38 W/m2 for the Globe, -0.48 ± 0.39 W/m2 for the Northern Hemisphere and -2.73 ± 0.54 W/m2 for the Southern Hemisphere. Larger GDB values are estimated over oceans than land (-2.56 ± 0.44 versus -1.04 ± 0.47 W/m2, respectively), suggesting that the atmosphere over oceans got less transparent than over continents during the 35-year study period. During this period, a brightening has taken place over Europe, Middle East, Mexico against a dimming over India, Maritime Continent, Australia and Southern Ocean.

How to cite: Stamatis, M., Hatzianastassiou, N., Korras Carraca, M. B., Matsoukas, C., Wild, M., and Vardavas, I.: The Global Dimming & Brightening based on FORTH radiative transfer model during 1984-2018 and its evaluation against GEBA & BSRN ground-based networks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13064, https://doi.org/10.5194/egusphere-egu23-13064, 2023.

EGU23-13198 | Posters on site | CL2.1

Spectral Aerosol Radiative Forcing and Efficiency of the La Palma Volcanic Plume over the Izaña Observatory 

Omaira García, Rosa Delia García, Emilio Cuevas-Agulló, África Barreto, Victoria Eugenia Cachorro, Carlos Marrero, Fernando Almansa, Ramón Ramos, Óscar Álvarez, and Mario Pó

By injecting aerosols and gases into the atmosphere, volcanoes significantly affect global climate, force changes in atmospheric dynamics, and influence many distinct cycles such as hydrological, carbon, and biogeochemical cycles. However, the irregular temporal and spatial distributions of volcanic processes and their effects are still poorly characterised. The volcanic eruption on La Palma (Canary Islands, Spain), which occurred in the autumn of 2021, presented an outstanding opportunity to improve the current understanding of these natural phenomena. The special conditions at the Izaña Observatory (IZO, Tenerife) and its proximity to La Palma (∼140 km) make it a strategic site for the comprehensive study of the almost unperturbed volcanic plume including the climate effects.

In this context, the present work deals with the experimental estimation of the solar spectral direct radiative forcing (ΔF) and efficiency (ΔFEff) during the volcanic eruption based on radiation measurements performed with an EKO MS-711 grating spectroradiometer during three events characterised by the presence of different types of aerosols: fresh volcanic aerosols, Saharan mineral dust, and a mixture of volcanic and Saharan dust aerosols. Three case studies were identified using ground-based (lidar) data, satellite-based (Sentinel-5P Tropospheric Monitoring Instrument, TROPOMI) data, reanalysis data (Modern-Era Retrospective Analysis for Research and Applications, version 2, MERRA-2), and backward trajectories (Flexible Trajectories, FLEXTRA), and subsequently characterised in terms of optical and micro-physical properties using ground-based sun-photometry measurements. Despite the ΔF of the volcanic aerosols being greater than that of the dust events (associated with the larger aerosol load present), the ΔFEff was found to be lower. The spectral ΔFEff values at 440 nm ranged between −1.9 and −2.6 Wm−2nm−1AOD−1 for the mineral dust and mixed volcanic and dust particles, and between −1.6 and −3.3 Wm−2nm−1AOD−1 for the volcanic aerosols, considering solar zenith angles between 30 and 70, respectively.

How to cite: García, O., García, R. D., Cuevas-Agulló, E., Barreto, Á., Cachorro, V. E., Marrero, C., Almansa, F., Ramos, R., Álvarez, Ó., and Pó, M.: Spectral Aerosol Radiative Forcing and Efficiency of the La Palma Volcanic Plume over the Izaña Observatory, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13198, https://doi.org/10.5194/egusphere-egu23-13198, 2023.

EGU23-14330 | Orals | CL2.1 | Highlight

Earth’s energy imbalance trend strengthened by recent aerosol emission reductions 

Øivind Hodnebrog, Gunnar Myhre, Hailing Jia, Johannes Quaas, Caroline Jouan, and Piers M. Forster

The Earth’s energy imbalance (EEI) is the difference in the net solar radiative flux and outgoing longwave radiative flux at the top-of-atmosphere. It has been shown that the positive EEI trend in the previous two decades is unexplained by internal variability and caused by anthropogenic forcing and response, such as that resulting from anthropogenic CO2 emissions. In this work we apply two state-of-the-art global climate models, the CESM2 and ICON-HAM, forced with observed (evolving) sea-surface temperature fields for the period 2000-2019 and with multiple ensemble members, to explore causes for the positive trend in EEI. Both models are able to reproduce the observed EEI trend from the CERES satellite product relatively well. Sensitivity simulations with aerosol emissions kept constant at year 2000 values indicate a relatively strong influence of recent aerosol emission reductions on the EEI trend. Preliminary results further indicate a considerable effect of using the latest CEDS emission version, as opposed to the CMIP6 CEDS version, on the EEI trend.

How to cite: Hodnebrog, Ø., Myhre, G., Jia, H., Quaas, J., Jouan, C., and Forster, P. M.: Earth’s energy imbalance trend strengthened by recent aerosol emission reductions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14330, https://doi.org/10.5194/egusphere-egu23-14330, 2023.

Aerosols are known to play an important role in regulating the Earth’s energy budget, by directly interacting with solar and terrestrial radiation and modifying the cloud properties. Radiative forcing is commonly used as an index for quantifying such imbalances in the Earth’s radiation budget by any factor. Quantifying aerosol radiative forcing is an initial step towards understanding the response of the Earth’s climate system to changes in emissions of aerosols from anthropogenic sources from pre-industrial (year 1850) to present day.

Our present study is designed to understand implications of changing emissions of aerosols over the historical period (1985-2014) on the evolution of aerosol and cloud radiative forcing using a state of art global chemistry-climate model named CAM6. The estimates of evolution of aerosol radiative forcing and its decomposition into direct radiative forcing (DRF or ERFARI), cloud radiative forcing (CRF or ERFACI) and surface albedo radiative forcing (SARF) on a global scale with special emphasis over the Indian region is being investigated. For this purpose, simulations are performed by CAM6 model for the 30-year period from 1985 to 2014 with model meteorology nudged towards the ERA5 reanalysis data using CMIP6 global emission inventory. We are trying to understand the implications of changing emissions of aerosols on the estimates of ERFARI, ERFACI and SARF to understand the contribution of each pathway through which changes in emissions of aerosols from PI to PD perturb the radiation budget of the earth-atmosphere system. We follow the methodology of Ghan et al. (2012) and use various combinations of additional radiative diagnostics with neglected absorption and scattering of aerosols and clouds along with all sky fluxes of shortwave (SW) and longwave (LW) radiation at top of the atmosphere (TOA) to decompose the total aerosol radiative forcing into ERFARI, ERFACI, and SARF.

Our results show that although the overall effect of changing emissions aerosols and their precursors from anthropogenic sources is to produce a negative radiative forcing at the top of atmosphere (TOA) thereby resulting in cooling over the south Asian region, we find that the aerosol-radiation interaction (ari) leads to warming while aerosol-cloud interaction (aci) results in cooling over the same region. The results from our CAM6 simulations show that the annual mean shortwave aerosol direct radiative forcing (DRF or ERFARI) averaged across the Indian land mass due to major aerosol species has increased from 0.46 W/m2 to 0.76 W/m2 during the 30-year period from 1985 to 2014. More results with greater details on the contribution of individual aerosol towards the temporal evolution of ERFARI and ERFACI will be presented.

 

Keywords: aerosols, Radiative forcing, ARI, ACI, CAM6

 

How to cite: Sharma, A. K. and Ganguly, D.: Temporal evolution of the aerosol radiative forcing due to changing emissions of individual aerosol species and their precursors over the Indian region as estimated using a global climate model CAM6., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14393, https://doi.org/10.5194/egusphere-egu23-14393, 2023.

EGU23-14718 | ECS | Orals | CL2.1

Low opaque clouds formed over Baffin Sea enhances Greenland's west coast surface cloud warming 

Jean Lac, Hélène Chepfer, Michael R. Gallagher, and Assia Arouf

Greenland Ice Sheet (GrIS) melt plays a major role in the global sea level rise. Surface melting is driven by changes in the radiative budget at the surface which is modulated by clouds. However, relatively little is known on the influence of local atmospheric processes on the fragile GrIS coast. Here we used space based lidar cloud profile observations with complementary data to show that low clouds formed in response to the Arctic sea ice retreat in September are transported over the GrIS west coast and warm radiatively the GrIS surface. Previous works have shown that low liquid clouds are formed in response to arctic sea ice retreat in September. We first showed the existence of continuous stratiform low liquid clouds between the Baffin Sea and the GrIS west coast in September using 12 years space lidar data at full resolution (instantaneous time scale and less than 500m spatial scale). Secondly, we analyzed wind profiles from re-analyis and from recent Doppler wind space lidar data and found that westerlies transport these stratiform clouds from the Baffin Sea to the GrIS west coast. Then, we used Surface LongWave Cloud Radiative Effect data derived from space-based active sensors for days that correspond to these specific situations where clouds are transported from the Baffin Sea, to quantify how much they warm radiatively the GrIS coast. We found that clouds coming from the Baffin Sea warm radiatively the GrIS west coast surface by +80W/m2 during the month of September. This contributes to an increase of +10W/m2 of cloud surface warming in average between July and September on the GrIS west coast. Overall, this study suggests that processes independent from large-scale circulation also influence the GrIS mass balance. 

How to cite: Lac, J., Chepfer, H., Gallagher, M. R., and Arouf, A.: Low opaque clouds formed over Baffin Sea enhances Greenland's west coast surface cloud warming, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14718, https://doi.org/10.5194/egusphere-egu23-14718, 2023.

EGU23-14872 | Posters on site | CL2.1

Changes in cloudiness cause a changing seasonality in the Baltic Sea region 

Piia Post and Margit Aun

In the Baltic Sea region, a significant decrease and subsequent increase in solar radiation have been detected during the past half-century. But the rise in shortwave irradiance is not seen for all seasons; significant changes appear in the seasonality of the cumulative sum of daily shortwave irradiance and the sea surface temperature of the Baltic Sea. Kahru et al. (2016) show that the accumulated surface incoming shortwave (SIS) energy has decreased in winter and increases during the spring and summer. The cumulative thresholds of surface incoming shortwave irradiance up to 1000 W/m2 are reached later in the season, but higher thresholds are reached earlier. The shift from later towards earlier cumulative thresholds occurs in spring, around March 15.

Changes in shortwave irradiance are associated with atmospheric transparency and cloudiness parameters like cloud fraction and albedo. The more substantial factor here is cloudiness, and therefore, we concentrate on reasons for changes in cloud properties. One of the most important reasons here is the synoptic-scale atmospheric circulation. The satellite-based cloud climate data record CLARA-A2 has been used to analyse regional time series and trends in the Baltic Sea region, from 1982-2019. The investigated cloud parameters were total fractional cloud cover (CFC) and SIS.

In March the interannual variability in CFC is high. The Increasing trend in incoming shortwave radiation could be explained by the decrease in CFC. The decrease in CFC is due to a smaller number of overcast days, that vary in the same rhythm with “cloudy” circulation patterns. This shows, that the shift in seasons that is connected to the earlier accumulated sums of SIS is at least partly explained by the changes in synoptic-scale atmospheric circulation.

 

How to cite: Post, P. and Aun, M.: Changes in cloudiness cause a changing seasonality in the Baltic Sea region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14872, https://doi.org/10.5194/egusphere-egu23-14872, 2023.

EGU23-15351 | Orals | CL2.1 | Highlight

Unmasking the Effects of Aerosols on Greenhouse Warming Over Europe 

Paul Glantz

Unmasking the Effects of Aerosols on Greenhouse Warming Over Europe

P. Glantz1, O. G. Fawole2, J. Ström1, M. Wild3 and K. J. Noone1

1Department of Environmental Science, Stockholm University, Stockholm, Sweden

2Dept. of Physics and Engineering Physics, Obafemi Awolowo University, Ile-Ife, Nigeria

3Institute for Atmospheric and Climate Science, ETH Zurich, Zurich, Switzerland

 

This work with corresponding publication in Journal of Geophysical Research: Atmospheres, 127, e2021JD035889. https://doi.org/10.1029/2021JD035889 is supported by FORMAS, grant 2018-01291.

 

Aerosol optical thickness (AOT) has decreased substantially in Europe in the summer half year (April–September) since 1980, with almost a 50% reduction in Central and Eastern Europe, according to Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2) reanalysis. At the same time, strong positive trends in ERA5 reanalysis surface solar radiation downward for all-sky and clear-sky conditions (SSRD and SSRDc, respectively) and temperature at 2 m are found for Europe in summer during the period 1979–2020. The Global Energy Balance Archive (GEBA) observations show as well strong increases in SSRD during the latest four decades. Estimations of changes in SSRDc, using the Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART) model, show similarly strong increases when fed by MERRA-2 AOT. The estimates of warming in this study, caused by increases in SSRD and SSRDc, are based on energy budget approximations and the Stefan Boltzmann law. The increases in near surface temperature, estimated both for clear-sky and all-sky conditions, are up to about 1°C for Central and Eastern Europe. The total warming over large parts of this region for clear-sky conditions is however nearly double the global mean temperature increase of 1.1°C, while somewhat less for all-sky conditions. Although the largest effects from aerosols on the radiation balance occurred in the 1980s and 1990s, the total warming has continued to increase more or less at the same rates during the latest four decades over large parts of Europe, considering both all-sky and clear-sky situations. Thus, decline in aerosols can certainly not explain all warming observed and particularly not considering the southern Iberian Peninsula where the aerosol effects on warming are weaker compared to countries further north. The largest increases in sensible heat flux at the expense of latent heat flux have occurred in Iberian Peninsula, which is probably a result of drier surface conditions. This means a positive feedback associated with reduced evaporate cooling and warming of the lowest air layers. Decline in water vapor in combination with the warming may have contributed to decreased cloud cover, which is found for large parts of Europe in the summer half year during the latest four decades. Anthropogenic aerosols over large parts of Europe have thus temporarily masked, until around 1980, parts of rapid warming from increases in greenhouse gases. CO2 from fossil fuels is of particularly serious concern, since it can continue to affect climate for thousand years.

How to cite: Glantz, P.: Unmasking the Effects of Aerosols on Greenhouse Warming Over Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15351, https://doi.org/10.5194/egusphere-egu23-15351, 2023.

Addressing the cause of intermodel spread in carbon dioxide (CO2) radiative forcing is essential for reducing uncertainty in estimates of climate sensitivity. Recent studies demonstrate that a large proportion of this spread arises from variance in model base state climatology, particularly the specification of stratospheric temperature, which itself plays a dominant role in determining the magnitude of CO2 forcing.

Here we investigate the significance of intermodel differences in stratospheric ozone (O3) as a cause of intermodel differences in stratospheric temperature, and hence its role as a contributing factor to intermodel spread in CO2 radiative forcing. We use the Community Earth System Model 2 and the Norwegian Earth System Model 2 to analyse the impact of systematic increases/decreases in stratospheric O3 on the magnitude of 2xCO2 and 4xCO2 effective radiative forcing (ERF). Corresponding rapid adjustments and instantaneous radiative forcing (IRF) are diagnosed using radiative kernels and the Parallel Offline Radiative Transfer code, respectively.

We demonstrate that differences in base state stratospheric O3 lead to significant differences in base state stratospheric temperature, ranging from +6 K to -8 K given a 50% increase and decrease in stratospheric O3 concentration. However, this does not result in a correspondingly large spread in CO2 IRF and ERF due to the compensating greenhouse effect of CO2 and O3. Intermodel differences in stratospheric O3 concentration are therefore not predominantly responsible for intermodel spread in CO2 IRF and ERF.

How to cite: Byrom, R. and Myhre, G.: Investigating the relationship between stratospheric temperature and intermodel CO2 radiative forcing spread, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15880, https://doi.org/10.5194/egusphere-egu23-15880, 2023.

EGU23-16873 | Posters on site | CL2.1

Understanding Water Temperature Regulating of Lakes Through the Energy Balance Approach: Direct Observations (Agamon Hula, Israel) and Analytical Solutions 

Guy Tau, Yehouda Enzel, Hamish McGowan, Vladimir Lyakhovsky, and Nadav Lensky

Air-water interactions regulate lake-water temperature by balancing the rate of change of water temperature (stored heat) with the incoming and outgoing heat fluxes, which are functions of water temperature and external forcing. Yet, there is a large knowledge gap in quantifying the thermoregulation of a lake, and especially managed lakes, which is hypothesized to be related to both external environmental forcing and management decisions on the lake depth and water discharge. Here we explore the thermoregulation of a restored and managed Mediterranean lake (Agamon Hula, Israel), by direct measurements of all major heat fluxes and interpret the results with a rigorous analysis of the energy balance equation. We provide general solutions of (i) the steady-state water temperature under given constant external conditions and show that it is unrelated to water depth, (ii) the time response of the lake’s temperature to reach a steady-state following an abrupt change in various environmental conditions and show its relation to water depth and thermal properties of water, and (iii) the response of the lake’s temperature to a pre-defined oscillations of the environmental forcing (diurnal, seasonal or other cycles). The amplitude of water temperature fluctuations, and the time delay from steady-state are functions of the environmental conditions oscillations and the ratio of the forcing’s time period over the thermal response time of the lake. The summertime measured CO2 fluxes of Agamon Hula revealed the lake acts as a CO2 source to the atmosphere, overpassing similar water bodies from different climates.

How to cite: Tau, G., Enzel, Y., McGowan, H., Lyakhovsky, V., and Lensky, N.: Understanding Water Temperature Regulating of Lakes Through the Energy Balance Approach: Direct Observations (Agamon Hula, Israel) and Analytical Solutions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16873, https://doi.org/10.5194/egusphere-egu23-16873, 2023.

The Libera Mission, named for the daughter of Ceres in Roman mythology, will provide continuity of the Clouds and the Earth’s Radiant Energy System (CERES) Earth radiation budget (ERB) observations from space. Libera’s attributes enable a seamless extension of the current 23-year ERB climate data record from CERES. Libera will acquire spectrally integrated radiance over the CERES FM6-heritage broad spectral bands in the shortwave (0.3 – 5 μm), longwave (5 – 50 μm) and total (0.3 – beyond 100 μm) and adds a split-shortwave band (0.7 – 5 μm) to provide deeper insight into shortwave energy deposition. Libera leverages advanced detector technologies using vertically aligned black-carbon nanotubes with closed-loop electrical substitution radiometry to achieve radiometric uncertainty of approximately 0.2%. Libera will also employ a wide field-of-view camera to provide scene context and accelerate the development of the split-shortwave angular distribution models.

Libera’s stewardship of the ERB record begins in the latter part of this decade, at an important juncture in the monitoring of climate trends. Libera is currently slated for a launch aboard JPSS-3 in December 2027, when the probability of a CERES data gap will be approaching 50%. The Libera science objectives associated with continuity and extension of the ERB data record are to identify and quantify processes responsible for ERB variability on various times scales. Beyond data continuity, Libera’s new and enhanced observational capabilities will advance our understanding of spatiotemporal variations of radiative energy flow in the visible and near-infrared spectral regions in addition to facilitating the rapid development of new angular distribution models for near-infrared and visible radiance-to-irradiance conversion.

This talk provides an overview of the Libera’s observational strategy, its measurements, science goals and objectives. We discuss the importance of climate data record continuity in the context of the current climate state and anticipated changes over the next decade and beyond.

How to cite: Pilewskie, P., Hakuba, M., and Stephens, G.: The Future of Earth Radiation Budget Observations Beyond CERES: Libera and Continuity of the ERB Climate Data Record, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17097, https://doi.org/10.5194/egusphere-egu23-17097, 2023.

On March 10th 2020, COVID-19 was categorised as a global pandemic by the World Health Organisation (WHO), concerned both by the alarming levels of spread and severity across 114 countries. On account of this, India announced the first nationwide lockdown on 25th March 2020. The present study examines the impact of the lockdown period on the atmospheric levels of overall aerosols (PM2.5) and on individual aerosol species (Black Carbon (BC), Organic Matter (OM), Sulphate (SO42-), Nitrate (NO3-) and Ammonium (NH4+) over the Indian subcontinent using a chemical transport model, CHIMERE. In this study, CHIMERE is forced externally by Weather Research and Forecasting (WRF) model as a meteorological driver in offline mode. The model was run for usual and pandemic lockdown scenarios to estimate the reductions in aerosol species concentration during the lockdown period. The cessation of industrial and transportation activity caused a significant drop in PM2.5 concentration of 20–30% over India, and notably 48% over Delhi. In-land regions saw a sharp decline in PM2.5 concentration (39–48% at Delhi, Bengaluru, and Raipur) compared to coastal locations (11–24% decrease at Kolkata, Mumbai, Chennai, Ahmedabad, and Bhubaneswar), which is explained by the marine influence at those coastal locations. The decrease in measured PM2.5 concentration is very well reproduced by the model for the agricultural state of Telangana, where agricultural residue burning is prominent as a major source of anthropogenic emissions. The elimination of traffic and industrial emissions during the lockdown period resulted in a significant decrease of aerosol species concentration (BC (10-40%), OM (3-10%), SO42- (30-80%), NO3- (70-90%) and NH4+ (60-80%)) over the subcontinent. The study also aims to understand the effect of lockdown on the aerosol optical property and found a reduction of 10-40% in the aerosol optical depth (AOD) over the Indian region. The reductions in the simulated mass concentration of PM2.5 are in eminent agreement (bias ≤ 40%) with the available measurements, rendering the model to be effective for simulating low emission scenarios over India.

How to cite: Dubey, K. and Verma, Dr. S.: Ambient aerosol variation in India during the COVID-19 lockdown : Simulations from high resolution chemical transport model (CHIMERE), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-91, https://doi.org/10.5194/egusphere-egu23-91, 2023.

EGU23-423 | ECS | Posters on site | AS3.5

The role of sulfur oxidation on cloud and aerosol properties in UKESM1 CMIP6 historical experiments 

Vichawan Sakulsupich, Paul T. Griffiths, and Alexander T. Archibald

Understanding the link between anthropogenic emissions and radiative forcing remains a grand challenge in the field of climate research. Linkages arise between emissions, atmospheric chemistry and climate through the formation of secondary aerosols such as sulfate, nitrate and organic aerosols. Sulfur dioxide (SO2) is an important aerosol precursor with the largest sources coming from anthropogenic activity. Unlike well-mixed greenhouse gases, anthropogenic aerosols are heterogeneously distributed because of localised emissions and the short atmospheric residence time. Thus SO2 conversion to aerosol is dictated by its emission location and the locally available oxidants; both of which are changing rapidly and disparately with time.

This work uses the UKESM1 to investigate the modelled response of sulfate aerosol properties and cloud properties to emissions increases and oxidant changes over the period 1850-2014. We compare modelled hydrogen peroxide, which is important for SO2 oxidation, with observations. From an analysis of the CMIP6 and AerChemMIP experiments, we show that there have been significant changes in the atmospheric oxidation processes of SO2 over this period with consequences for the calculated radiative forcing. 

In UKESM1 historical experiments, the gas-phase reaction with hydroxyl radicals dominates the oxidation pathways in most regions. This channel is the most sensitive to oxidant changes and contributes to new aerosol particle formation. In contrast, in the aqueous-phase reaction, the oxidation of SO2 by ozone decreased in the European region in 1980 and oxidation by hydrogen peroxide increased in Eastern Asia in 2014. We present an analysis of the impacts of these sulfur oxidation changes on cloud properties and radiative forcing. Ultimately, this work contributes to the improvement of our process-level understanding of Earth system models that interactively simulate aerosol from precursors and aims to improve the accuracy of aerosol radiative forcing predictions.

How to cite: Sakulsupich, V., Griffiths, P. T., and Archibald, A. T.: The role of sulfur oxidation on cloud and aerosol properties in UKESM1 CMIP6 historical experiments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-423, https://doi.org/10.5194/egusphere-egu23-423, 2023.

EGU23-1291 | ECS | Orals | AS3.5

Regional impacts of CO and NOx mitigation in a methane emissions-driven model 

Zosia Staniaszek, Paul T Griffiths, Gerd A Folberth, Fiona M O'Connor, and Alexander T Archibald

Methane plays a central role in the atmosphere, affecting the atmospheric oxidising capacity through its reaction with OH, air quality through its role as an ozone precursor, and climate through its greenhouse gas properties.  

Methane emissions-driven models provide an opportunity to study the Earth system within a global model that features the most accurate representation of the methane cycle. Here we use the methane emissions-driven configuration of the UK Earth System Model, UKESM1-CH4. 

Previously we explored a zero anthropogenic methane scenario, which focused on attributing the composition, air quality and climate impacts of future anthropogenic methane emissions. Here, we study the potential co-benefits of methane mitigation: reducing NOx and CO emissions. We use SSP1-2.6 emissions pathways for CO and NO in these scenarios. 

The complex interactions between methane, CO, OH and NOx are represented more completely in the emissions-driven model. We calculate the sensitivity of ozone and OH to the CO and NO emissions changes, and their dependence on the methane burden. We also show the impacts on other near-term climate forcers such as aerosols and ozone. 

Global reductions in CO and NO emissions have disproportionate effects in different regions. We present analysis of the regional differences in ozone and OH response, based on the HTAP regions. We demonstrate much greater effects in South and East Asia than in the Europe and North America.

How to cite: Staniaszek, Z., Griffiths, P. T., Folberth, G. A., O'Connor, F. M., and Archibald, A. T.: Regional impacts of CO and NOx mitigation in a methane emissions-driven model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1291, https://doi.org/10.5194/egusphere-egu23-1291, 2023.

EGU23-1597 | Orals | AS3.5

Quantifying effects of Indian aerosol emissions on regional aerosol abundances, energy balance, and health impacts, using a novel national emission inventory 

Marianne T. Lund, Saroj K. Sahu, Poonam Mangaraj, Bjørn H. Samset, Sourangsu Chowdhury, Gunnar Myhre, and Ane N. Johansen

After years of rapid growth, India has become a hotspot for emissions of aerosols and their precursors, recently surpassing China in terms of magnitude of SO2 emissions. The resulting high air pollution levels influence climate through interactions with solar radiation, clouds, and the hydrological cycle, and pose one of the greatest environmental threats to public health. Model estimates of these impacts are influenced by the substantial spread that exists between current emission inventories, in terms of both trend and magnitude. Activity and fuel data is heterogeneous and can be challenging to compile, and many emission sources are highly region specific. Hence, inventories need to be based on up-to-date national statistics and detailed sectoral information.

Here we use one such inventory for Indian anthropogenic emissions, the recently developed, bottom up SNEII (Sabe National Emission Inventory for India) dataset to simulate and evaluate regional air pollution levels for 2018. SNEII includes a more detailed spatial allocation of point sources of emissions and sectoral disaggregation than many global inventories. The results are compared to estimates using the Community Emission Data System (CEDS) emissions, version 2021, also placing them in the context of the trend over the past decades. For most species, SNEII estimates higher emissions, and we explore the resulting impact of these differences on simulated aerosol abundances, as well as implications for radiative forcing and premature mortality. Finally, we quantify the sectoral contribution to air pollution with a finer breakdown than previously provided, including sectors unique for Indian/South Asian region.  

How to cite: Lund, M. T., Sahu, S. K., Mangaraj, P., Samset, B. H., Chowdhury, S., Myhre, G., and Johansen, A. N.: Quantifying effects of Indian aerosol emissions on regional aerosol abundances, energy balance, and health impacts, using a novel national emission inventory, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1597, https://doi.org/10.5194/egusphere-egu23-1597, 2023.

EGU23-1836 | ECS | Orals | AS3.5

Change in daily weather variability due to warming and regional aerosols. 

Kalle Nordling, Bjørn Samset, and Nora Fahrenbach

The world has changed: You can feel it in the air as temperatures rise, you can feel it in the water as precipitation patterns change. Much of what has once been our daily weather is lost. It began with humankind emitting greenhouse gases and aerosols. However, there is a growing resistance that wants to limit theses emissions. 

Daily variability can be described by probability density functions (PDF). Change can manifest as changes of the mean properties of weather-related variables, and/or changes in the chape of their PDFs. In this study, we examine how regional PDF shapes change due to increasing temperature, driven primarily by greenhouse gas emissions, and due to emissions of different aerosols species (black carbon and sulfate). Our main questions are: (1) How do shapes of regional daily PDFs evolve with global warming? (2) How do these changes differ in response to aerosol and greenhouse gas emissions? (3) And which aerosol-related teleconnections induce these changes in PDF shapes?  As changes in shape affect low and high extremes differently, we aim to link changes in PDF shape to changes in extreme events of daily temperature and precipitation by using parameters describing PDF width and asymmetry.

We use data from PDRMIP single forcer climate model simulations to examine how changes in regional and global aerosol concentrations change the PDF shapes. We also use three CMIP6 large ensembles (MPI-ESM1-2-LR, CanESM5 and ACCESS-ESM1-5) to examine changes in PDF shape at five different levels of global warming, from 1°C to 4 °C. Our main questions are how the shapes of regional daily PDFs evolve with globalwarming, how their changes differ between aerosol and greenhouse gas induced changes, and what teleconnections due to regional aerosol changes induce in PDF shapes.

For the time will soon come when aerosols will shape the near future of our weather.

How to cite: Nordling, K., Samset, B., and Fahrenbach, N.: Change in daily weather variability due to warming and regional aerosols., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1836, https://doi.org/10.5194/egusphere-egu23-1836, 2023.

Near-term climate forcers (NTCF) are a group of chemically and radiatively active constituents that have a relatively short lifetime in the atmosphere (<20 years). They can exert effects on the climate, important for the future rate of climate warming, and in elevated concentrations at the lowest most levels of the atmosphere can lead to poor air quality and detrimental impacts on human health. Two important NTCFs that are considered in this study are tropospheric O3 and fine particulate matter (with a diameter less than 2.5 microns – PM2.5). Future climate mitigation scenarios that seek to limit future temperature increases, and include reductions in air pollutant emissions, need to consider the impact on climate, air quality and human health from changes in NTCFs. Here we use results from UKESM1 (an Earth system model with interactive chemistry and aerosols) in different future sensitivity scenarios that consider air pollutant emission mitigation, future climate change and land-use change, conducted as part of the Aerosol and Chemistry Model Intercomparison Project (AerChemMIP). We assess the impact on climate (in terms of effective radiative forcing), air pollutants (in terms of change in ambient surface concentrations) and human health (in terms of long-term adult mortality from exposure to ambient air pollutants) by comparing the results from these sensitivity scenarios to the future reference scenario ssp370, a scenario that involves low mitigation of climate and air pollutants.

Scenarios that involve combined strong mitigation of aerosols and O3 precursors, including large reductions in global CH4 concentrations, produce the largest benefits to climate (an ERF of -1.2 Wm-2), air quality (10-25% reduction in O3 and PM2.5 concentrations) and human health (>25% reduction in the rate of long-term premature mortality). Benefits to health are largest across Asia for these scenarios (a 44% reduction in the mortality rate). If global CH4 concentrations are not reduced or aerosol precursors emissions are reduced in isolation, then there is a detrimental impact to future climate but there are still improvements to future air quality and a reduction in the long-term air pollutant health burden. If climate and air quality mitigation measures are not enacted on top of ssp370 then there is a penalty to global climate, a detrimental impact on air pollutant concentrations and an increase in the long-term air pollutant health burden across certain regions (e.g. by 20% over Africa). Considering only the impacts from climate change show increases in air pollutant concentrations over some continental regions and also an increase in the long-term rate of premature mortality by more than 10% over Europe and parts of Asia, offsetting some of the benefits achieved from emission mitigation measures. Quantifying co-benefits and trade-offs between climate, air quality, and human health together in this way, enables policy makers to understand the outcomes of different mitigation strategies and to identify pathways with maximum benefits across all three axes.

How to cite: Turnock, S., Reddington, C., and O'Connor, F.: The Climate, Air Quality and Health co-benefits and trade-offs from different future mitigation scenarios involving Near-Term Climate Forcers in UKESM1, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2685, https://doi.org/10.5194/egusphere-egu23-2685, 2023.

The Asian summer monsoons are globally significant meteorological features, creating a strongly seasonal pattern of precipitation, with the majority of the annual precipitation falling between June and September. The stability of such a strongly seasonal hydrological cycle is of extreme importance for a vast range of ecosystems and for the livelihoods of a large share of the world’s population.

 

Simulations are performed with an intermediate complexity climate model, PLASIM, in order to assess the future response of the Asian monsoons to changing concentrations of aerosols and greenhouse gases. The radiative forcing associated with aerosol loading consists of a mid-tropospheric warming and a compensating surface cooling, which is applied to India, Southeast Asia and East China, both concurrently and independently. The primary effect of increased aerosol loading is a decrease in summer precipitation in the vicinity of the applied forcing, although the regional responses vary significantly. The decrease in precipitation is only partially ascribable to a decrease in the precipitable water, and instead derives from a reduction of the precipitation efficiency, due to changes in the stratification of the atmosphere.

 

When the aerosol loading is added in all regions simultaneously, precipitation in East China is most strongly affected, with a quite distinct transition to a low precipitation regime as the radiative forcing increases beyond 60 W/m2. The response is less abrupt as we move westward, with precipitation in South India being least affected. By applying the aerosol loading to each region individually, we are able to explain the mechanism behind the lower sensitivity observed in India, and attribute it to aerosol forcing over East China. Additionally, we note that the effect on precipitation is approximately linear with the forcing.

 

The impact of doubling carbon dioxide levels is to increase precipitation over the region, whilst simultaneously weakening the circulation. When the carbon dioxide and aerosol forcings are applied at the same time, the carbon dioxide forcing partially offsets the surface cooling and reduction in precipitation associated with the aerosol response.

How to cite: Reccchia, L. and Lucarini, V.: Modelling the effect of aerosol and greenhouse gas forcing on the Asian monsoons with an intermediate complexity climate model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3339, https://doi.org/10.5194/egusphere-egu23-3339, 2023.

EGU23-3715 | ECS | Posters on site | AS3.5

How would shifting manufacturing from China to Indonesia or India impact human health and social economy? 

Qi Ran, Shao-Yi Lee, Duofan Zheng, Han Chen, Shili Yang, John Moore, and Wenjie Dong

The COVID-19 pandemic is reshaping the global trade and supply chains, and some developed countries may consider relocating strategic manufacturing operations out of China, providing new opportunities for some South and Southeast Asian countries. Since the shift of manufacturing is accompanied by redistribution of emission sources of air pollutants, the impacts on environment and human health of the countries directly involved and their neighbors, should be considered. We used the Community Earth System Model, the Integrated Exposure-Response (IER) model and Willingness To Pay (WTP) method, to simulate fine particulate matter (PM2.5) and the socio-economic responses to shifting manufacturing from China to Indonesia or India. Our results show that significant effects on PM2.5 related mortality and economic cost for these deaths were seen in many East, Southeast and South Asian countries, particularly those immediately downwind of these three countries. Transferring all of export-related manufacturing to Indonesia resulted in significant mortality decreases in China and South Korea by around 78k (5 per 100k) and 1k (2 per 100k) respectively, while Indonesia’s mortality significantly increased (73.7k; 29 per 100k), as well as India, Pakistan and Nepal. When manufacturing was transferred to India, mortality rates in East Asia show similar responses to the Indonesian scenario, while mortalities in India increased dramatically by 87.9k (6 per 100k), and mortalities in many neighbors of India also severely increased. Shifting manufacturing to India in our simulations led to more Asian countries showing significant changes in PM2.5 related deaths and economic costs than an equivalent shift to Indonesia. This is because of the maritime Indonesian setting as well as patterns of surface winds. Nevertheless, the economic costs for these deaths were much smaller than national GDP changes in China (0.9% of GDP vs. 18.3% of GDP), India (2.7% of GDP vs. 84.3% of GDP) or Indonesia (9.4% of GDP vs. 337% of GDP) due to shifting all of export-related production lines from China to India or Indonesia. Perhaps the most concerning aspect of this study is the damage to “innocent” victims of any manufacturing shifts in third countries that do not see any domestic economic gains. Morally, part of the benefits of economic activity should be used to compensate the neighboring communities where mortality increases occur.

How to cite: Ran, Q., Lee, S.-Y., Zheng, D., Chen, H., Yang, S., Moore, J., and Dong, W.: How would shifting manufacturing from China to Indonesia or India impact human health and social economy?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3715, https://doi.org/10.5194/egusphere-egu23-3715, 2023.

EGU23-4217 | ECS | Orals | AS3.5

High Resolution Simulations of European Air Quality in 2050 Following Different CMIP6 Climate Change Mitigation Pathways 

Connor J. Clayton, James B. McQuaid, Daniel R. Marsh, Steven T. Turnock, Ailish M. Graham, Kirsty J. Pringle, and Rajesh Kumar

Air quality co-benefits are expected to occur with greater climate mitigation, however climate mitigation is not expected to occur in isolation of other socio-economic changes. Although modelling studies investigating these co-benefits are common, limited work uses the recently developed “Shared Socioeconomic Pathways” which factor in the different patterns of climate mitigation, socioeconomic development and pollution control. Additionally, as the SSPs were designed for climate model ensembles, such as CMIP6, existing work usually uses global climate or earth system models with interactive chemistry simulated at relatively coarse horizontal resolution. These computational trade-offs may impact how effectively they model air quality at human exposure-relevant scales and may miss differing trends seen only at subregional scales.

We have used the anthropogenic emissions inputs from different SSPs which have different mitigation patterns applied to climate change and air pollution in 2050 to drive a specialised Atmospheric Chemistry model (WRF-Chemv4.2) at 30km resolution over Europe. We compare these to a 2014 control simulation. We present the validation of this model setup, which suggests an overestimation of surface PM2.5 concentrations, largely driven by overestimated NO3 aerosol, but good agreement with O3 observations. We find that while significant potential for air quality co-benefits exists, these effects are non-linear, with both PM2.5 and O3 worsening in some locations and scenarios despite increased pollution control compared to the present. We also find notable spatial heterogeneity in the change of PM2.5 and O3 across Europe in some scenarios.  Overall, however the results show that across Europe, scenarios with greater mitigation of climate change and air pollution show improvements in air quality that could lead to benefits to human health. 

How to cite: Clayton, C. J., McQuaid, J. B., Marsh, D. R., Turnock, S. T., Graham, A. M., Pringle, K. J., and Kumar, R.: High Resolution Simulations of European Air Quality in 2050 Following Different CMIP6 Climate Change Mitigation Pathways, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4217, https://doi.org/10.5194/egusphere-egu23-4217, 2023.

EGU23-4612 | ECS | Posters on site | AS3.5

Relationship between synoptic weather pattern and surface Particulate Matter (PM) during winter and spring seasons over South Korea 

Dasom Lee, Hyun Cheol Kim, Kwanchul Kim, Sung Bum Yun, Jae-Hoon Yang, and Dae-Hwan Kim

Regional air quality over East Asia, including South Korea, has been a center of public attention recently because of a few episodes in which very high particulate matter (PM) concentrations have been observed. Predicting PM variation with lead time of a few hours up to days is one of the key areas that the governments are working on because it can benefit from early warning system to short-term mitigation effort. In this study, the influence of synoptic weather conditions on regional air quality was investigated with the occurrence frequencies of PM episodes as a function of various synoptic weather patterns during winter and spring. (1) During winter, dry moderate (DM) types occur frequently alongside high PM cases (24-h mean PM10 concentration > ). The composite weather map showed a weak northwesterly wind field as a potential cause. On the contrary, it is interesting to note that dry polar (DP) types can be associated with low PM cases (24-h mean PM10 concentration < ) as well as high PM depending on near-surface wind speed. (2) Furthermore, during spring, DM and dry tropical (DT) types were found to be highly correlated with high (much higher) PM concentrations, likely because of the enhanced static stability in the lower troposphere. It should be noted that PM concentration depends on the lower atmospheric stability. The close relationship between synoptic weather patterns and PM concentration suggests that synoptic weather can play an important role in regional air quality.

How to cite: Lee, D., Kim, H. C., Kim, K., Yun, S. B., Yang, J.-H., and Kim, D.-H.: Relationship between synoptic weather pattern and surface Particulate Matter (PM) during winter and spring seasons over South Korea, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4612, https://doi.org/10.5194/egusphere-egu23-4612, 2023.

EGU23-5642 | Orals | AS3.5

Future projection of ozone-related mortality under SSP3-7.0 scenario based on CMIP6 simulations 

Dimitris Akritidis, Sara Bacer, Prodromos Zanis, Aristeidis K. Georgoulias, Larry W. Horowitz, Vaishali Naik, Fiona M. O'Connor, James Keeble, Philippe Le Sager, Twan van Noije, Putian Zhou, and Andrea Pozzer

Long-term exposure to ambient ozone is linked with respiratory-related mortality, while the emerging climate change is projected to pose double-edged challenges for ozone air quality. Here, we calculate the impact of emissions- and climate-change under SSP3-7.0 scenario on ozone-related mortality on a global scale, using historical (experiment histSST) and future simulations (experiments ssp370SST and ssp370pdSST) from three CMIP6 Earth System Models (ESMs) (GFDL-ESM4, EC-Earth3-AerChem, and UKESM1-0-LL). The ssp370SST experiment follows time-varying SSTs, while the SSP370pdSST follows a present-day climatology for SSTs. The chronic obstructive pulmonary disease mortality attributable to ozone pollution is estimated following the Global Burden Disease (GBD) 2019 approach, by using the ozone season daily maximum 8-hour mixing ratio (OSDMA8), the baseline mortality rate (from the GBD), and the SSP3-7.0 present and future gridded population. An increase in ozone-related mortality of approximately 2.5 million people per year globally is projected at the end of the century (2090) with respect to 2000 due to emissions and population changes. The climate-change footprint on ozone-related mortality exhibits large variability among the ESMs; yet, over India and China all ESMs project an increase of ozone-related mortality in the future, highlighting the importance of the ozone penalty due to global warming in regions with strong anthropogenic sources.

How to cite: Akritidis, D., Bacer, S., Zanis, P., Georgoulias, A. K., Horowitz, L. W., Naik, V., O'Connor, F. M., Keeble, J., Le Sager, P., van Noije, T., Zhou, P., and Pozzer, A.: Future projection of ozone-related mortality under SSP3-7.0 scenario based on CMIP6 simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5642, https://doi.org/10.5194/egusphere-egu23-5642, 2023.

EGU23-5883 | ECS | Orals | AS3.5

Effects of marine biology and air-mass trajectories on cloud brightness 

Eszter Kovacs, Daniel Grosvenor, Ken Carslaw, Jane Mulcahy, and Thomas Lachlan-Cope

The role of marine phytoplankton emissions in aerosol-cloud interactions is still a cause of large uncertainties in climate modelling. We investigate the effects of DMS and sea spray aerosol, which are both affected by marine phytoplankton, on the droplet concentrations of liquid clouds. To do this we examine MODIS satellite data for an area of liquid clouds in the Southern Ocean during the southern hemispheric summer. Backwards trajectories of air masses from the clouds were simulated with the FLEXPART Lagrangian particle dispersion model for a duration of 9 days.

Clouds whose trajectories were not influenced by continental air masses could be split into two groups based on their trajectory history in the two days before encountering cloud: group 1 spent most of their time in the free troposphere, whereas group 2 spent their last two days within the boundary layer. 

Group 1 cloud droplet concentrations were positively correlated with exposure to sea surface chlorophyll that took place prior to them entering the free troposphere (i.e., at least 2 days before encountering their clouds), whereas droplet concentrations were negatively correlated with wind speed in the last day before encountering clouds. Group 2 clouds did not show the same correlations. Instead, wind speeds in the last two days before a cloud encounter were positively correlated with cloud droplet number concentration, with the relationship between the two having a steeper slope for higher chlorophyll values.

These results give an insight into the factors controlling the changes in Southern Ocean cloud properties with associated climate impacts via cloud brightening effects.

How to cite: Kovacs, E., Grosvenor, D., Carslaw, K., Mulcahy, J., and Lachlan-Cope, T.: Effects of marine biology and air-mass trajectories on cloud brightness, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5883, https://doi.org/10.5194/egusphere-egu23-5883, 2023.

EGU23-6263 | ECS | Posters on site | AS3.5

Estimating the impact of the radiative feedback from atmospheric methane on climate sensitivity 

Laura Stecher, Franziska Winterstein, Martin Dameris, Patrick Jöckel, and Michael Ponater

Methane (CH4), the second most important greenhouse gas directly emitted by human activity, is removed from the atmosphere via chemical degradation.

In this study we assess the radiative feedback from atmospheric CH4 resulting from changes in its chemical sink, which is mainly the oxidation with the hydroxyl radical (OH) and, which is influenced by temperature and the chemical composition of the atmosphere.

We present results from numerical simulations with the chemistry-climate model EMAC perturbed by either CO2 or CH4 increase.

The essential innovation in the simulation set-up is the use of CH4 emission fluxes instead of prescribed CH4 concentrations at the lower boundary. This means that changes in the chemical sink can feed back on the atmospheric CH4 concentration without constraints.

For both forcing agents, CO2 and CH4, we explore so called rapid radiative adjustments in simulations with prescribed sea surface temperatures, as well as slow radiative feedbacks and the climate sensitivity in respective simulations using an interactive oceanic mixed layer.

To quantify individual physical and chemical radiative adjustments and feedbacks we use the partial radiative perturbation method in offline simulations with a radiative transfer model consistent with the one used in the online simulations.

First results show a negative feedback of atmospheric CH4 in a warming and moistening troposphere. As water vapour is a precursor of OH, increased humidity leads to increasing OH mixing ratios. This leads in turn to a shortening of the CH4 lifetime and a reduction of the CH4 mixing ratios accordingly. This decrease in CH4 also affects the response of tropospheric ozone (O3) leading to a less pronounced increase of O3 in the tropical upper troposphere compared to previous studies of the O3 response following a CO2 perturbation (Dietmüller et al., 2014;Nowack et al., 2015;Marsh et al., 2016).

How to cite: Stecher, L., Winterstein, F., Dameris, M., Jöckel, P., and Ponater, M.: Estimating the impact of the radiative feedback from atmospheric methane on climate sensitivity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6263, https://doi.org/10.5194/egusphere-egu23-6263, 2023.

EGU23-6282 | ECS | Posters on site | AS3.5

Potential impacts of wildfire on Southern Ocean clouds 

Saisai Ding

Wildfires produce serious and long-lasting effects on weather and climate by large dust and aerosol emissions. However, its remote impacts on clouds over the Southern Ocean (SO) and polar regions remain unxplored. Based on ship observations conducted during MARCUS feild campaign from November, 2017 to March, 2018, a fire index (FI) is defined along the ship track by a lagrangian particle dispersion model (FLEXPART) combined with a daily high-resolution wildfire burned area dataset. Correaltions between this fire index and observed aerosol and CCN concentrations are analyzed to explore potential impacts of wildfire on SO clouds and its latitudinal variations. Our results show that the correlations between FI and aerosol concentrations are significant over the SO, which means the Autralia wildfire could affect the SO clouds reaching far to 70°S. The most significant positive correlations are found in the range of 40°S-55°S between FI and aerosol and CCN concentrations, with correlation coefficients of 0.65 and 0.88 respectively.

How to cite: Ding, S.: Potential impacts of wildfire on Southern Ocean clouds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6282, https://doi.org/10.5194/egusphere-egu23-6282, 2023.

EGU23-7319 | Orals | AS3.5

Climate influences of Asian anthropogenic aerosols decomposed using a Reduced Complexity Model 

Camilla Weum Stjern, Bjørn Halvard Samset, Laura Wilcox, and Manoj Joshi

Aerosol emissions have a wide range of impacts on the climate both near to and far from emission sources. Impacts span from local changes in surface solar warming to large-scale modifications of atmospheric circulation patterns and monsoonal precipitation. They have also been found to have an outsized near-term influence on extreme events in recent climate model studies. Consequently, future aerosol emission changes are likely to contribute to climate related risk in many highly populated regions, some of which are particularly vulnerable, for instance, to shifts in precipitation patterns or timing with respect to growing seasons. However, aerosol climate impacts generally follow patterns and time evolutions that are markedly different to those from greenhouse gas driven global surface warming, and our understanding of them is still plagued by high scientific uncertainty.

Given the urgent need for improved knowledge about the near-term influences of changes in aerosol emissions, we here introduce SyRAP-FORTE – a tool for understanding and decomposing the local and remote climate effects of regional aerosol emissions. SyRAP – a set of Systematic Regional Aerosol Perturbations – is developed using FORTE2.0, a Reduced Complexity (RC) climate model developed in the UK. Current and expected future aerosol emission changes are particularly strong in East and South Asia, where high population densities imply high potential climate risk. In the initial version of SyRAP, presented here, we therefore perturb absorbing and scattering aerosols, separately, over India and East China, to assess their separate influence on local responses in a range of climate parameters.

We document and validate the climate responses in FORTE to the regional aerosol perturbations, showing for instance that removing emissions of absorbing aerosols over both East China and will cause a local drying, but a range of more widespread effects. We find that SyRAP is able to reproduce the overall aerosol responses documented in the literature, and also that it allows us to decompose the influences of different aerosol species from the two regions on the climate near to, and far from, the emission sources.

Finally, we show how SyRAP can be used as input to emulators and tunable simple climate models, and as a ready-made tool for projecting the effects of near-term changes in Asian aerosol emissions.

How to cite: Stjern, C. W., Samset, B. H., Wilcox, L., and Joshi, M.: Climate influences of Asian anthropogenic aerosols decomposed using a Reduced Complexity Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7319, https://doi.org/10.5194/egusphere-egu23-7319, 2023.

EGU23-7364 | Posters on site | AS3.5

Tropospheric ozone budget in AerChemMIP experiments 

Paul Griffiths, Youngsub Shin, James Keeble, and Alexander Archibald

A grand challenge in the field of chemistry-climate modelling is to understand the connection between anthropogenic emissions, atmospheric composition and the radiative forcing of trace gases and aerosols.  The AerChemMIP model intercomparison project, part of CMIP6, aims to understand the role of near-term climate forcers, aerosol and chemistry and includes experiments focused on tropospheric ozone.

We present an analysis of the trends in tropospheric ozone budget in the UKESM1 and other models for which diagnostic data is available from CMIP6 experiments. We focus on the historical period, and evaluate trends in ozone budget terms of chemical production and loss of ozone as well as physical processes such as transport and deposition.  We include AerChemMIP attribution experiments such as histSST-piCH4, to quantify the effect of individual emissions and forcing changes on the historical ozone burden and budget.  We include a comparison of ozone budget over ocean basins with data from recent ATom field campaigns.

How to cite: Griffiths, P., Shin, Y., Keeble, J., and Archibald, A.: Tropospheric ozone budget in AerChemMIP experiments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7364, https://doi.org/10.5194/egusphere-egu23-7364, 2023.

EGU23-7597 | ECS | Posters on site | AS3.5

Radiative Effects of Recent Changes in PM2.5 Pollution over China and Local and Remote Climate Impacts 

Yue Chen, Steve R. Arnold, and Steven T. Turnock

The large reduction in anthropogenic aerosol emissions across China in recent years has improved China’s air quality but also caused changes in radiative forcing. Some studies confirmed the reduction of aerosols over China cause a positive radiative forcing locally and play an important role in Arctic warming. However, few studies have differentiated and quantified the radiative forcing of different aerosol components including BC and sulphate. Here, we aim to understand the reduction of black carbon (BC) and SO2 emissions over China from 2008 to 2016 under a series of policies enacted by the Chinese government and to determine the change in radiative forcing both locally and remotely. We use the Evaluating the Climate and Air Quality Impacts of Short-Lived Pollutants (ECLIPSE) emission inventory to represent China's emissions of the two pollutants during this period and use the United Kingdom Earth System Model (UKESM) v-1 to calculate the individual radiative forcing due to changes in all anthropogenic aerosols, China BC only, and China SO2 only between 2008 and 2016. Finally, we use the temperature coefficients of individual pollutants at different latitude bands to calculate the temperature responses. Our results show the largest reduction of BC over China was from the residential and energy sectors, while the reduction in SO2 emissions from energy and industrial sources were significant. Compared with other inventories, ECLIPSE overestimates the reduction of emissions but shows the same trend. The aerosol radiative forcing over China locally due to the large Chinese emission reductions of BC and SO2 are -0.30±0.01Wm-2 and 1.03±0.07 Wm-2, respectively, which jointly accounts for more than 80% of the total aerosol radiative forcing calculated by the model from all anthropogenic aerosol emission sources. In addition, changes in BC and SO2 over China together contributed to a positive radiative forcing of 0.18 Wm-2 across the North Pacific. However, BC and sulphate are not major contributors to changes in Arctic radiative forcing. The temperature response due to BC (-0.008 ℃) and sulphate (0.060 ℃) is most pronounced locally in the mid-latitudes, while the temperature response in the low and high latitudes is small. This study bridges the gap on changes in radiative forcing due to anthropogenic emissions reductions in China and quantifies the contributions of BC and sulphate aerosols to better understand the impact of air pollution emission control policies on climate.

How to cite: Chen, Y., R. Arnold, S., and T. Turnock, S.: Radiative Effects of Recent Changes in PM2.5 Pollution over China and Local and Remote Climate Impacts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7597, https://doi.org/10.5194/egusphere-egu23-7597, 2023.

EGU23-8236 | ECS | Orals | AS3.5

Chemistry-albedo feedbacks from reforestation partially offset CO2 removal benefits 

James Weber, James A. King, N. Luke Abraham, Daniel P. Grosvenor, David J. Beerling, Peter Lawrence, and Maria Val Martin

Reforestation is widely proposed for carbon dioxide (CO2) removal but the impact on climate, via atmospheric composition and surface albedo changes, remains relatively unexplored. Using two Earth System models, UKESM1 and CESM2, we compare scenarios where existing forests expand to a near biophysical limit (with croplands fixed at 2015 to preserve food production) with SSP1-2.6 and SSP3-7.0 at 2050 and 2095.  

In the reforestation scenario, global BVOC emissions are 18% (35%) higher than SSP3-7.0 at 2050 (2095) and 8% (12%) higher than SSP1-2.6. The resulting increases to secondary organic aerosols and aerosol scattering, from BVOC emission changes, drive a negative radiative forcing (RF). However, this is outweighed by the positive RF from increases to methane and ozone and decreases to surface albedo.

The net RF is equivalent to CO2 increases of 13 (32) ppm relative to SSP3-7.0 at 2050 (2095) and 3 (8) ppm relative to SSP1-2.6. These indirect factors offset ~25% of the additional CO2 removal arising from reforestation relative to SSP3-7.0 and ~10% relative to SSP1-2.6. This highlights the importance of assessing the full response of the Earth System to reforestation, rather than just the potential CO2 removal.  



How to cite: Weber, J., King, J. A., Abraham, N. L., Grosvenor, D. P., Beerling, D. J., Lawrence, P., and Val Martin, M.: Chemistry-albedo feedbacks from reforestation partially offset CO2 removal benefits, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8236, https://doi.org/10.5194/egusphere-egu23-8236, 2023.

EGU23-8532 | Posters on site | AS3.5

The role of an interactive methane cycle in climate sensitivity and climate feedbacks 

Fiona O'Connor, Gerd Folberth, Nicola Gedney, and Chris Jones

Despite methane’s importance as a greenhouse gas, the Earth System Models that contributed to Phase 6 of the Coupled Model Intercomparison Project (CMIP6) typically prescribe surface methane concentrations - following either historical observations or specified future shared socioeconomic pathways. Here, we make use of novel methane emissions-driven capability in the UK’s Earth System Model to explore the role of an interactive methane cycle, including wetland emissions, on the model’s equilibrium climate sensitivity and its transient climate response to changes in carbon dioxide concentration.

The climate response to external forcings is strongly influenced by climate feedbacks and with the inclusion of interactive methane in Earth System Models, it becomes important to understand the effects of changing carbon dioxide and meteorology on wetland emissions.  This work re-evaluates the CMIP6 assessment of the methane wetland emissions feedback in UKESM1 by taking account of wetland emissions’ sensitivity to both meteorology and carbon dioxide. 

This presentation demonstrates the need for including interactive methane in Earth System Models. By allowing changes in natural methane emissions to influence methane concentrations and climate, this novel capability enables scientists to determine the consequences of methane emission reduction policies or climate feedbacks on natural methane sources towards meeting global climate as well as global air quality targets.

How to cite: O'Connor, F., Folberth, G., Gedney, N., and Jones, C.: The role of an interactive methane cycle in climate sensitivity and climate feedbacks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8532, https://doi.org/10.5194/egusphere-egu23-8532, 2023.

EGU23-8610 | Orals | AS3.5

Beyond ozone hole impacts: Seamless composition-climate interactions explored with ICON-ART 

Peter Braesicke, Valentin Hanft, Katerina Kusakova, Roland Ruhnke, Khompat Satitkovitchai, Björn-Martin Sinnhuber, Stefan Versick, and Michael Weimer

The ICOsahedral Non-hydrostatic (ICON) modelling system was originally developed by DWD and MPI-M for a range of weather (forecast) and climate applications. An Aerosols and Reactive Tracers (ART) module was added by KIT to enable a comprehensive assessment of composition interactions within the atmospheric domain. Recognising that atmospheric processes happen on a multitude of temporal and spatial scales, flexible horizontal and vertical grid options are a key element of versatile model configurations in use. Here, we present a selection of results from different ICON-ART configurations that explore (stratospheric) ozone-climate interactions and stratosphere-troposphere coupling – e.g. regional climatic impacts of the ozone hole (and ozone losses in other regions) and global warming induced changes in jet-streams – in different types of integrations. In addition, we explore the potential to forecast “chemical weather” with ICON-ART, including environmental (UV) indices.

Starting with time-slice experiments, we provide a range of examples using the ICON-ART modelling system to investigate (idealised) climate change scenarios with respect to different threshold temperatures (reached under global warming) and the climatic impact of the ozone hole (and ozone losses in other regions). For the latter, halogen induced depletion of (stratospheric) ozone can be switched on and off in our modelling world. We illustrate how such integrations allow the unambiguous attribution of certain climate change effects, e.g. the contribution of the ozone hole (and other regional ozone losses) to regional surface warming in Antarctica and changes to regional and global “effective radiative forcing”, and the change of jet stream variability under global warming. Moving on, we explore the capability of ICON-ART to work with regionally nested grids to capture accurately smaller spatial scales and to provide “meaningful” forecasts of environmental (UV) indices, thus, demonstrating comprehensively the seamless philosophy regarding processes, scales and applications with the flexible ICON-ART modelling system.

How to cite: Braesicke, P., Hanft, V., Kusakova, K., Ruhnke, R., Satitkovitchai, K., Sinnhuber, B.-M., Versick, S., and Weimer, M.: Beyond ozone hole impacts: Seamless composition-climate interactions explored with ICON-ART, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8610, https://doi.org/10.5194/egusphere-egu23-8610, 2023.

Studies have demonstrated that black carbon (BC) tends to be underestimated by models in general, while NO2 and CO columns are also underestimated, although surface measurements are reasonable. These findings are at odds with increased regulations and incentives to improve air quality and address climate altering species.

Recent advances in analyzing large datasets allows new analytical methods to detect signals and quantify patterns among different in-situ species, which were not previously realized. This work adopts one such approach merging mass conservation, number conservation, first order thermodynamics and chemistry, single-particle MIE modeling, and remotely sensed measurements across the UV, VIS, and NIR in tandem. Using basic thermodynamical relationships of combustion under different energy use conditions to constrain the ratios between co-emitted species, first order in-situ chemistry, and advective and pressure-based transport, emissions and uncertainties of BC, CO, and NO2 are quantified. The total errors are explored in depth based on boundaries established from the first order physical laws and mathematical bootstrapping, with the overall error generally observed to be smaller than the day-to-day variability.

The significance of day-to-day, week-to-week, and grid-to-grid variation are quantified. This is especially true in the regions undergoing the most change. The impacts of dynamical transport, chemical-decay, thermodynamic initiation, and in-situ interactions with UV radiation are attributed using additional measurements not used to fit the mass-conserving model free approach used in this work. This work relies on AERONET, SONET, OMI, TROPOMI, GEMS, MOPITT, MISR, CEMS, and other ground-based platforms.

A few conclusions are discussed. First, regulations are working in urban centers and at large sources including powerplants, steel plants, and concrete plants, with overall emissions being reduced for at least one and in many cases two species. Second, there are large increases in suburban and rural areas, including in regions previously unidentified as being emission s free. Third, the effects of biomass burning are clearly identified and attributed, even in regions which were previously thought to be nearly completely controlled by urban sources, such as the megacities of Hong Kong, New Delhi, and Shanghai. Fourth, attribution has determined that emissions, UV radiation, and long-range transport are all significant. Fifth, there are biases in the observed TOA radiative forcing, in which a small but significant percentage of the total BC outcomes have a positive radiative forcing, and the median values are far less negative than current models can capture. Sixth, the concept of TOA and ABS radiative forcing per unit of AOD is found to not be reasonable, and a new framework is demonstrated that accounts for more than 90% of the possible cases computed.

How to cite: Cohen, J.: Top-Down Model-Free Computed Emissions, Size, Mixing State, and Radiative Forcing of BC, CO, and NOx: Increased Emissions and Less Negative Radiative Forcing in Rural Areas Coupled with Reduced Emissions and More Variable Radiative Forcing in Urban Areas, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8966, https://doi.org/10.5194/egusphere-egu23-8966, 2023.

EGU23-9839 | Orals | AS3.5

Lifetimes and timescales of tropospheric ozone  

Michael Prather and Xin Zhu

It is vital and informative to understand the lifetime and timescales of tropospheric O3 so that we can predict the impact of changing O3 sources on its abundance throughout the troposphere, and thence its climate and pollution damage.  As an example, current model intercomparison projects (MIPs) diagnose the impact of stratosphere-troposphere exchange (STE) flux of O3 into the troposphere by assuming that loss of this added O3 occurs through 3 specific reactions (O(1D)+H2O, HO2+O3, OH+O3) and is linear in O3, and that production through XO2+NO reactions is a constant.  A linearization of the full chemistry with respect to O3 clearly shows these assumptions are wrong (see ATom data, shown here).  Another example is the effort made to define odd-oxygen by a chemical family grouping (e.g., O3+O+NO2+…) to better understand the timescales for O3 loss, yet the true pattern of the odd-oxygen family should be apparent from the eigenvectors of the system. 

 

Here we define and test a new protocol for model experiments designed to understand how the coupling of O3 with the full chemistry can change the accumulation and the pattern of decay depending on the O3 source (stratosphere, surface pollution, aviation).  We take a full chemistry-transport model (UCI CTM) and generate a control run for the present day, then add direct O3 emissions (not in the control run) from (i) a large industrial region, (ii) aviation, and (iii) the mid-latitude tropopause where most STE occurs. These perturbation runs produce a seasonally varying additional O3 burden – which gives us the seasonally varying lifetime for such sources – and then we cut emissions and watch the decay pattern in terms of e-fold timescale and patterns of key species to derive the odd-oxygen family pattern.   Due to the large latitudinal and seasonal variation in reactivity rates (see ATom data: Guo et al. ACP, 23, 99–117, 2023), we expect lifetimes and timescale to vary with location and timing of O3 emissions.

 

How to cite: Prather, M. and Zhu, X.: Lifetimes and timescales of tropospheric ozone , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9839, https://doi.org/10.5194/egusphere-egu23-9839, 2023.

EGU23-10054 | ECS | Orals | AS3.5

Effect of aerosol changes on regional climate in East Asia 

Seungun Lee, Rokjin Park, Sang-Wook Yeh, and Yong-Cheol Jeong

This study investigates the effect of aerosol changes on regional climate in East Asia. Especially, we focus on the recent decreasing trend of aerosol concentrations in China from 2011 to 2018. We conduct climate sensitivity simulations using the Community Earth System Model (CESM) atmospheric general circulation model (AGCM) with observed monthly sea surface temperatures (SST) and sea ice concentrations (SIC) and coupled general circulation model (CGCM) with its own predicted SST and SIC from the coupled ocean and sea ice models. We prescribe the observed monthly aerosol optical depths from the Moderate Resolution Imaging Spectroradiometer (MODIS) onboard Terra and Aqua satellite for the base simulations and period-averaged monthly aerosol optical depths for the sensitivity simulations. Comparisons of 50 ensemble averages between the base and sensitivity simulations for the AGCM and CGCM models show that the decreasing aerosols in East Asia warm up the region due to increased net shortwave radiation. We also found that the CGCM simulations show much stronger and more extensive warming in East Asia due to decreasing aerosols than the AGCM simulations, implying the importance of the aerosol-ocean-atmosphere feedback.

How to cite: Lee, S., Park, R., Yeh, S.-W., and Jeong, Y.-C.: Effect of aerosol changes on regional climate in East Asia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10054, https://doi.org/10.5194/egusphere-egu23-10054, 2023.

EGU23-10731 | ECS | Posters on site | AS3.5

Oxidation precursors around the Arabian Peninsula – Evaluation of EMAC model results with ship-based measurements of HCHO, H2O2, ROOH and HOx 

Dirk Dienhart, Bettina Brendel, John N. Crowley, Philipp G. Eger, Hartwig Harder, Monica Martinez, Sergey Osipov, Andrea Pozzer, Roland Rohloff, Jan Schuladen, Sebastian Tauer, Jos Lelieveld, and Horst Fischer

Formaldehyde (HCHO), hydrogen peroxide (H2O2) and organic hydroperoxides (ROOH) play a key role in atmospheric oxidation processes. They act as sources and sinks for HOx radicals (OH + HO2), with OH as the primary oxidant that governs the atmospheric self-cleaning capacity. In this study, we use in situ observations in the marine boundary layer (MBL) to calculate trace gas budgets, determine dry deposition velocities and evaluate results of the general circulation model EMAC (ECHAM5/MESSy2 Atmospheric Chemistry).

The dataset was obtained during the AQABA (Air Quality and climate change in the Arabian BAsin) ship campaign around the Arabian Peninsula in summer 2017. This region is famous for high levels of anthropogenic air pollution related to the oil and gas industry, especially in the areas around the Suez Canal and the Arabian Gulf. High levels of air pollution with up to 12 ppbV HCHO, 2.3 ppbV ROOH but relatively low levels of H2O2 (≤ 0.5 ppbV) were detected over the Arabian Gulf.

We find that EMAC predicted mixing ratios of HCHO and ROOH mostly within a factor of 2, while the model overestimated ROOH in cleaner conditions and it failed to resolve the encountered high pollution events over the Arabian Gulf. Dry deposition velocities (Vdep) were determined for HCHO and H2O2 during night with 0.77 ± 0.29 cm s–1 for HCHO and 1.03 ± 0.52 cm s–1 for H2O2 over the Arabian Sea, which were matched by EMAC. Vdep was underestimated over the Mediterranean Sea by more than a factor of 2, which was mostly related to the models resolution and its wind speed dependency. Determination of the photochemical budget of H2O2 revealed overestimated HOx in EMAC, which resulted in an elevated net photochemical production over most regions. Results of the regional model WRF-Chem (Weather Research and Forecasting-Chem) increased the accuracy of H2O2 for most regions, while the model did not resolve the complex air pollution encountered over the Arabian Gulf, which may lead to missing anthropogenic emissions in the region.

How to cite: Dienhart, D., Brendel, B., Crowley, J. N., Eger, P. G., Harder, H., Martinez, M., Osipov, S., Pozzer, A., Rohloff, R., Schuladen, J., Tauer, S., Lelieveld, J., and Fischer, H.: Oxidation precursors around the Arabian Peninsula – Evaluation of EMAC model results with ship-based measurements of HCHO, H2O2, ROOH and HOx, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10731, https://doi.org/10.5194/egusphere-egu23-10731, 2023.

EGU23-12434 | Orals | AS3.5

Insect herbivory have significantly altered BVOC emissions, SOA concentration and radiative forcing over Fennoscandian birch forest 

Jing Tang, Hui Wang, Zhanzhang Cai, Alex Guenther, Riikka Rinnan, Per-Ola Olsson, Rikke Lauge Borchmann, Cleo Lisa Davie-Martin, Guy Schurgers, Zhengchao Ren, Jolanta Rieksta, and Tao Li

Over Fennoscandian mountain birch forest region, there are increased attacks of geometrid moth larvae. These herbivores can change forests from a carbon sink to a carbon source. When moths start to chew on leaves, large quantities of biogenic volatile organic compounds (BVOCs) are released. Herbivory-induced BVOC emissions have been observed and quantified at a few sites over Fennoscandian mountain birch forest, but we know very little of their potential regional implications for atmospheric processes.

In this work, we extracted birch defoliation information based on MODIS leaf area index (LAI) for an outbreak year 2012, and together with field-observed relationship between leaf defoliated level and changes in emissions, we modelled herbivory-induced BVOC emissions at regional scale using MEGAN. Taking a step further, we fed MEGAN-modelled BVOC emission data with or without considering herbivory impacts to a two-way coupled WRF-CMAQ system to dynamically assess the impacts of these emissions on the atmospheric chemistry and climate system .

During the whole growing season of 2012, the defoliation at some MODIS grids can be as high as 90%, and the large defoliation mainly occurs in June and July. For t-β-ocimene, Other Monoterpenes, Stress and Other compound groups, herbivory contributes to more than 30, 8, 5 and 16 times the increase in the seasonal sum for the defoliated regions. For terpenes, herbivory increased monthly emissions up to 3 times for June and July. The reduction of emissions caused by herbivory-caused decrease in LAI is much smaller than the herbivory-induced increase. We also found strong impacts of herbivory-induced BVOC emissions on downward shortwave radiation and cloud radiative forcing.

This is the first time we can link all these components, i.e., satellite monitoring of leaf defoliation, in-situ observation, ecosystem and atmospheric modelling together to answer the research questions related to the regional importance of insect herbivory on atmospheric composition and climate.

How to cite: Tang, J., Wang, H., Cai, Z., Guenther, A., Rinnan, R., Olsson, P.-O., Borchmann, R. L., Davie-Martin, C. L., Schurgers, G., Ren, Z., Rieksta, J., and Li, T.: Insect herbivory have significantly altered BVOC emissions, SOA concentration and radiative forcing over Fennoscandian birch forest, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12434, https://doi.org/10.5194/egusphere-egu23-12434, 2023.

EGU23-13213 | Orals | AS3.5

Aerosol-radiation interactions on global to local scales 

Øivind Hodnebrog, Camilla W. Stjern, and Gunnar Myhre

Black carbon (BC) aerosols absorb solar radiation and thus heat the atmosphere. This process occurs on a short time scale and can influence clouds, precipitation, and boundary layer meteorology. Global climate models (GCMs) strongly disagree in their representation of such rapid adjustments, adding to the uncertainty in the effective radiative forcing (ERF) due to BC. Disagreements are at least partly caused by differences in parametrization of the highly regional and potentially non-linear rapid adjustments, which are poorly resolved in coarse resolution GCMs. Knowledge of how the rapid adjustments depend on model resolution is therefore important.

Here we explore the dependence of rapid adjustments on model resolution by performing a set of idealized experiments using a GCM, the Community Earth System Model version 2 (CESM2) with fixed sea-surface temperatures, downscaled by a regional climate model, the Weather Research and Forecasting (WRF), for five years at 45 km horizontal resolution over East and South Asia and at 15 km resolution covering East China. To ensure a sufficient climate response in the models, we perturb BC emissions by a factor of ten, and compare the results to separate simulations with a fivefold increase in (scattering) sulfate emissions and a doubling of CO2 concentrations.

Preliminary results indicate similar BC-induced responses between CESM2 and 15 km WRF simulations in terms of tropospheric temperature and humidity, and mean precipitation, but strong dependence on model and/or resolution in the cloud response to BC. Potential differences in seasonal and extreme precipitation will be examined, and we plan to explore finer scales using the WRF model in Large Eddy Simulation (LES) mode down to 100 m horizontal resolution.

How to cite: Hodnebrog, Ø., Stjern, C. W., and Myhre, G.: Aerosol-radiation interactions on global to local scales, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13213, https://doi.org/10.5194/egusphere-egu23-13213, 2023.

EGU23-13947 | ECS | Posters on site | AS3.5

Global projection of potential effects of future air quality on bee visual navigation 

Yoori Cho, Sujong Jeong, and Dong Yeong Chang

Airborne aerosols can alter incoming solar radiation inducing different radiative responses, yet the potential ecological effects of changes in the degree of linear polarization (DoLP) by the light alteration remain largely unknown. Light polarization is an important navigational cue for honeybee for which a threshold intensity (i.e., the DoLP) for a reliable response is known as 15%. Here, we quantify the relationship between the mass concentration of airborne fine particulate matter (PM2.5) and the DoLP by ground-based observation to provide an estimate of how the quantity of PM2.5 changes the DoLP in general and how these changes will impair navigation of honeybee by limited-visibility at the global level. We find that the PM2.5 mass concentration exponentially decreases the DoLP, reducing the average and maximum DoLP, and the size of area containing perceivable polarization information by honeybee over the sky. Applying these results to global air quality prediction models, EMAC, MPI-ESM1.2-HAM, MIROC-ES2 under a BaU (for EMAC) and SSP370 (for MPI-ESM1.2-HAM, MIROC-ES2L) scenario, we find that projected areas and the number of days of limited-visibility that honeybee experience increases globally on average. Our estimates capture almost year-round risk hotspots of limited-visibility over sub-Saharan Africa, Eastern Mediterranean, Southeast Asian regions in 2050. In particular, India is projected to experience approximately a 10 folds increase in the number of days of limited visibility. Developing countries are more vulnerable to degrading air quality than developed countries in terms of limited-visibility for honey bees. Overall, our study demonstrates degrading air quality in 2050 as a result of business-as-usual emissions of air pollutants can affect bee navigation, threatening fundamental plant-pollinator interactions. Further, warming climate will exacerbate this impact.

This work was supported by the National Research Foundation of Korea (NRF) grant funded by the Korea government (MSIT) (No. RS-2022-00155875).

How to cite: Cho, Y., Jeong, S., and Chang, D. Y.: Global projection of potential effects of future air quality on bee visual navigation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13947, https://doi.org/10.5194/egusphere-egu23-13947, 2023.

EGU23-14506 | ECS | Orals | AS3.5

Stratospheric water vapor affecting atmospheric circulation 

Edward Charlesworth, Felix Plöger, Thomas Birner, Rasul Baikhadzhaev, Marta Abalos, Luke Abraham, Hideharu Akiyoshi, Slimane Bekki, Fraser Dennison, Patrick Jöckel, James Keeble, Doug Kinnison, Olaf Morgenstern, David Plummer, Eugene Rozanov, Sarah Strode, Guang Zeng, and Martin Riese

Water vapor plays an important role in many aspects of the climate system, by affecting radiation, cloud formation, atmospheric chemistry and dynamics. Even the low stratospheric water vapor content provides an important climate feedback, but current climate models show a substantial moist bias in the lowermost stratosphere. Here we report crucial sensitivity of the atmospheric circulation in the stratosphere and troposphere to the abundance of water vapor in the lowermost stratosphere. We show from a mechanistic climate model experiment and inter-model variability that lowermost stratospheric water vapor decreases local temperatures, and thereby causes an upward and poleward shift of subtropical jets, a strengthening of the stratospheric circulation, a poleward shift of the tropospheric eddy-driven jet and regional climate impacts. The mechanistic model experiment in combination with atmospheric observations further shows that the prevailing moist bias in current models is likely caused by the transport scheme, and can be alleviated by employing a less diffusive Lagrangian scheme. The related effects on atmospheric circulation are of similar magnitude as climate change effects. Hence, lowermost stratospheric water vapor exerts a first order effect on atmospheric circulation and improving its representation in models offers promising prospects for future research.

How to cite: Charlesworth, E., Plöger, F., Birner, T., Baikhadzhaev, R., Abalos, M., Abraham, L., Akiyoshi, H., Bekki, S., Dennison, F., Jöckel, P., Keeble, J., Kinnison, D., Morgenstern, O., Plummer, D., Rozanov, E., Strode, S., Zeng, G., and Riese, M.: Stratospheric water vapor affecting atmospheric circulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14506, https://doi.org/10.5194/egusphere-egu23-14506, 2023.

EGU23-14813 | Posters on site | AS3.5

A study on seasonal forecasting of air quality in East Asia using statistical-dynamical methods 

Jahyun Choi, Jee-Hoon Jeong, Sung-Ho Woo, Ji-Yoon Jeong, Sanghyuk Park, and JIn-Ho Yoon

In this study, we developed a statistical-dynamical model that predicts the concentration of particulate matter in Korea 2-3 months in advance using the correlation between meteorological and climate factors and presented its performance. Temperature and atmospheric circulation around the Arctic Ocean considering the predictive performance of the National Centers for Environmental Prediction (NCEP) climate forecast system version 2 (CFSv2), the concentration of particulate matter in winter in Korea, and the correlation between meteorological and climate factors, potential predictors such as sea surface temperature in the Bering Sea region and sea level pressure in the Atlantic region were discovered. Using this, a multiple linear regression model was constructed between the average concentration of particulate matter during the winter of that year and latent factors for the second half of October and the first half of November in NCEP CFSv2, respectively. Seasonal predictions were made for the concentration of particulate matter in winter for a total of 20 years from 2001 to 2020. The result of the winter predicted in the second half of October showed r=0.49. And the result predicted in the first half of November showed a predictive performance of r=0.45. Considering the linear trend of particulate matter reduction, which was strong during the study period, r=0.72 in the second half of October and r=0.71 in the first half of November. This is judged to be the result of maximizing climate prediction performance considering the relatively long time scale of seasonal forecasting. In addition, additional forecasting ability can be expected through improved predictability of climate prediction models such as multi-model ensemble technology. However, although the results of the dynamical model were reflected, there are still limitations of the statistical model, and additional research is needed, such as problems due to limitations in observational data.

How to cite: Choi, J., Jeong, J.-H., Woo, S.-H., Jeong, J.-Y., Park, S., and Yoon, J.-H.: A study on seasonal forecasting of air quality in East Asia using statistical-dynamical methods, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14813, https://doi.org/10.5194/egusphere-egu23-14813, 2023.

Dimethyl sulfide (DMS), which originates from phytoplankton, is the major natural source of sulfur compounds in the atmosphere. The oxidation products of DMS can form aerosols, which contribute to the formation of clouds, making them important for rain and the radiative balance of the planet. Additionally, due to DMS naturally occurring above oceans, an oxidation product of DMS, methanesulfonic acid (MSA), has been used to determine sea ice extent in ice cores up to 300 years in the past. However, due to gaps in the oxidation pathway of DMS, there are large uncertainties in the modelling of MSA formation. The aim of this work is to reduce the uncertainties in the DMS oxidation pathway, improving the modelling of the major products.

This project uses the KPP wrapper, BOXMOX, to compare box model outputs to chamber experiments from Albu et al. [1], Arsene et al. [2] and Ye et al. [3]. This comparison allows for an assessment of a near-explicit mechanism used in box models (the Master Chemical Mechanism) and a reduced mechanism useful for global models (CRI-Strat) regarding DMS oxidation in both low and high NOx environments. This work presents the outcomes from this assessment and recommendations for the mechanisms to improve their modelling of DMS oxidation.

[1] Albu, M.; Barnes, I.; Becker, K. H.; Patroescu-Klotz, I.; Benter, T.; Mocanu, R. In Simulation and Assessment of Chemical Processes in a Multiphase Environment, Barnes, I., Kharytonov, M. M., Eds.; Springer Science: Dortdrecht, 2008, pp 501–513.   

[2] Arsene, C.; Barnes, I.; Becker, K. H.; Mocanu, R. Atmos. Environ. 2001, 35, 3769–3780.

[3] Ye, Q.; Goss, M. B.; Krechmer, J. E.; Majluf, F.; Zaytsev, A.; Li, Y.; Roscioli, J. R.; Canagaratna, M.; Keutsch, F. N.; Heald, C. L.; Kroll, J. H. Atmos. Chem. Phys., 2022, 22, 16003–16015.

How to cite: Jacob, L., Giorio, C., and Archibald, A.: Assessment of dimethyl sulfide atmospheric oxidation mechanisms, used in both box models and global models, through the comparison with previous experiments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15130, https://doi.org/10.5194/egusphere-egu23-15130, 2023.

EGU23-15821 | ECS | Posters on site | AS3.5

Analysis of the GeoMIP G6sulfur experiment with SOCOLv4 

Elia Wunderlin, Gabriel Chiodo, Timofei Sukhodolov, Sandro Vattioni, Daniele Visioni, and Simone Tilmes

Climate change and its associated risks are becoming more and more prominent. Stratospheric solar geoengineering with sulfuric acid aerosols has been put forward as a way to temporarily mitigate some of the risks of climate change and is inspired by the cooling effect of large eruptions of tropical volcanoes. To learn more about the opportunities and dangers associated with stratospheric solar geoengineering, it is important to investigate the strategy beforehand, e.g., by means of climate modelling. To better understand the sources of model uncertainties, the Geoengineering Model Intercomparison Project (GeoMIP) introduced stratospheric solar geoengineering scenarios for an easier comparison of different models. Most models participating in GeoMIP either have no interactive chemistry or simplified aerosol micro-physics. In this study we perform the G6sulfur experiment with SOCOLv4, an atmosphere-ocean-aerosol-chemistry climate model. In the G6 sulfur experiment the aim is to bring the global average temperature of the SSP5-8.5 to the levels of the SSP2-4.5 sceanrio.

For the calibration we ran three different tests in order to analyse the sensitivity of the aerosol burden to the order in which the microphysical processes are simulated at each timestep - nucleation of new particles from H2SO4 vapours and condensation of H2SO4 on pre-existing particles. One experiment had nucleation first, one had condensation first and finally one had nucleation first but with an added subsubstep where coagulation is called again. For all these runs we used an injection of 5 TgS/year. In the run with nucleation first the global stratospheric aerosol burden is 25% bigger than in the run where condensation is called first and 10% bigger than in the run with 2 subsubsteps. This leads to a cooling effect over 2032-2047 which is 1.02 K for nucleation first, 0.95 K for the run with the additional substep and 0.65 K for condensation first. Based on the cooling efficiency of the 5 TgS/year injection, we then derive a time-dependent emission, to keep global mean surface temperatures close to the SSP2-4.5 scenario.

For the G6sulfur experiment we chose the setup of the run with 2 subsubsteps and performed three ensemble members to get a better understanding of the uncertainties within the model. We will discuss the effects on stratospheric aerosol burden, radiative forcing, temperature, ozone and precipitation changes and compare our results to other GeoMIP models. This will work provides useful insights concerning the radiative and climatic impacts of stratospheric aerosols on climate, elucidating the impact of uncertainties in the modelling of microphysical processes.

How to cite: Wunderlin, E., Chiodo, G., Sukhodolov, T., Vattioni, S., Visioni, D., and Tilmes, S.: Analysis of the GeoMIP G6sulfur experiment with SOCOLv4, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15821, https://doi.org/10.5194/egusphere-egu23-15821, 2023.

EGU23-941 | ECS | Posters on site | AS3.6

Can we predict the expected evolution of polar stratospheric clouds on climatic time scales ? 

Mathilde Leroux and Vincent Noel

During hemispheric winter a vortex forms on poles resulting in a very sharp drop in stratospheric temperatures. When the temperature drops below a particular threshold TNAT that allows nitric acid nucleation, polar stratospheric clouds (PSCs) can start to form. PSCs are responsible for the thinning of the ozone layer. According to climate models, the ozone layer is expected to return to 1960 levels around 2060. However this progress could be slowed down by enhanced PSC formation due to the cooler and wetter stratosphere that could be caused by climate change. 

The spaceborne lidar from CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) has helped us understand better the spatial and temporal occurrence of PSCs. The CALIPSO PSC product, derived from CALIPSO level 1B measurements, describes the spatial distribution, optical properties, and composition of PSCs along CALIPSO orbits. The product also includes reanalysis temperatures from MERRA2 and complementary information from the Microwave Limb Sounder (MLS), such as HNO3/H2O mixing ratios which are essential to PSCs formation and to TNAT calculation.

In this study we will present a statistical model based on the analysis of the CALIPSO PSC product from 2006 to 2020. It establishes a relationship between the PSC density observed by CALIOP and the density of stratospheric temperatures colder than TNAT. This model allows the prediction of PSC density by pressure level derived from stratospheric temperature. We will show that this model allows us to tell if there is a PSC or not in (2°x4°) boxes over monthly periods, even in places where the satellite CALIPSO doesn't overpass. We will discuss its application on temperatures predicted by Shared Socio-economic Pathways (SSP) scenarios to know the evolution of PSCs over this century. One of our eventual goals would be to investigate if observed PSC densities can constrain stratospheric temperatures predicted by GCMs. 

 

How to cite: Leroux, M. and Noel, V.: Can we predict the expected evolution of polar stratospheric clouds on climatic time scales ?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-941, https://doi.org/10.5194/egusphere-egu23-941, 2023.

The aim of this poster is to compare the discontinuity occurrence in the ozone data from the following reanalyses: ERA-5, MERRA-2 and JRA-55. We use the ozone concentration data from all layers between 500 hPa and 1 hPa in the period 1980-2020 in January. We also compute the total ozone content between these layers by vertical integration of ozone profile. We search for discontinuities also in this content.    This is important topic, because the presence of discontinuities influences the values of trends and their significance. Discontinuities arise from the changing in the assimilation procedure, introducing new observation to the reanalyse, and changing of data quality.  There are dates which the occurrence of discontinuities is expected in: 2004- transition from SBUV to EOS Aura data and 2015-  the 4.2 MLS data were started to use instead of version 2.2. We search for discontinuities in the following classes of extremity: 1st, 10th, 25th, 50th,75th,90th and 99th percentile as well as the mean. Ozone data with high occurrence of the discontinuities is not suitable for trend analyses.

How to cite: Krizan, P.: Comparison of discontinuity occurrence in ozone data in selected reanalyses, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1900, https://doi.org/10.5194/egusphere-egu23-1900, 2023.

Polar stratospheric clouds (PSCs) play a key role in the polar chemistry of the stratosphere. Nitric acid trihydrate (NAT) particles have been shown to lead to denitrification of the lower stratosphere. While the existence of large NAT particles (NAT "rocks") has been verified by many measurements, especially in the Northern Hemisphere (NH), most current chemistry-climate models use simplified parametrizations, often based on evaluations in the Southern Hemisphere where the polar vortex is stable enough that accounting for NAT rocks is not as important as in the NH. Here, we evaluate the probability density functions of various gaseous species in the polar vortex using one such model, the Whole Atmosphere Community Climate Model (WACCM), and compare these with measurements by the Michelson Interferometer for Passive Atmospheric Sounding onboard the Environmental Satellite (MIPAS/Envisat) and two ozonesonde stations for a range of years and in both hemispheres. Using the maximum difference between the distributions of MIPAS and WACCM as a measure of coherence, we find better agreement for HNO3 when reducing the NAT number density from the standard value of 1 x 10−2 cm-3 used in this model to 5 × 10−4 cm−3 for almost all spring seasons during the MIPAS period in both hemispheres. The distributions of ClONO2 and O3 are not greatly affected by the choice of NAT density. The average difference of WACCM to ozonesondes supports the need to reduce the NAT number density in the model. Therefore, this study suggests using a NAT number density of 5 × 10−4 cm−3 for future simulations with WACCM. 

How to cite: Kinnison, D., Weimer, M., Wilka, C., and Solomon, S.: Effects of denitrification on the distributions of trace gas abundances in the polar regions: Comparison of the Whole Atmosphere Community Climate Model with observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3650, https://doi.org/10.5194/egusphere-egu23-3650, 2023.

EGU23-3669 | Posters on site | AS3.6

Updated PSC climatology based on CALIOP measurements from 2006-2023 

Michael Pitts and Lamont Poole

After more than three decades of research, the roles of polar stratospheric clouds (PSCs) in stratospheric ozone depletion are well established. Heterogeneous reactions on PSCs convert the stable chlorine reservoirs HCl and ClONO2 to chlorine radicals that destroy ozone catalytically.  PSCs also prolong ozone depletion by delaying chlorine deactivation through the removal of gas-phase HNO3 and H2O by sedimentation of large nitric acid trihydrate (NAT) and ice particles. A substantial recovery of the ozone layer is expected by the middle of this century with reduced global production of ozone depleting substances in accordance with the Montreal Protocol and subsequent amendments.  But as climate changes, leading to a colder and perhaps wetter stratosphere and upper troposphere, reliable model predictions of recovery of the Antarctic ozone hole and of potentially more severe ozone depletion in the Arctic are challenging.  This is due both to a lack of detailed understanding of the underlying physics and the fact that many global models use simple parameterizations that do not accurately represent PSC processes.

A more complete picture of PSC processes on vortex-wide scales has emerged from the CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) instrument on the CALIPSO satellite that has been observing PSCs at latitudes up to 82 degrees in both hemispheres since June 2006.  The CALIOP Version 2.0 (v2) PSC algorithm was recently developed to address known deficiencies in previous algorithms and includes additional refinements to increase the robustness of the inferred PSC composition. In this paper, we present an updated PSC reference data record and comprehensive climatology constructed by applying the v2 algorithm to the more than 17-year CALIOP spaceborne lidar dataset.  In addition, we will examine the potential impact of aerosol and water vapor injections into the stratosphere from the January 2022 Hunga Tonga eruption on PSC occurrence in both the Arctic and Antarctic regions. 

How to cite: Pitts, M. and Poole, L.: Updated PSC climatology based on CALIOP measurements from 2006-2023, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3669, https://doi.org/10.5194/egusphere-egu23-3669, 2023.

EGU23-5658 | ECS | Posters virtual | AS3.6

Research on the stratospheric ozone depletion in the polar spring 

Qidi Li, Yuhan Luo, and Yuanyuan Qian

In recent years, the severe stratospheric ozone depletion events (ODEs) were reported in the polar spring. We retrieved the critical indicator ozone vertical column densities (VCDs) using zenith scattered light differential optical absorption spectroscopy (ZSL-DOAS) located in Chinese Great Wall Station, South Antarctic (62.22° S, 58.96° W) and Chinese Yellow River Station, Ny-Ålesund (78.92° N, 11.93° E). The ozone holes appeared above Antarctic in September and October each year (from 2017 to 2020), with ozone VCDs less than 220 DU. Furthermore, during March and April 2020, ozone VCDs over Ny-Ålesund, Arctic was only about 64.7% of that in normal years. The retrieved daily averages of ozone VCDs were compared with satellite observations from Global Ozone Monitoring Experiment 2 (GOME-2), Brewer spectrophotometer, and Système d’Analyze par Observation Zénithale (SAOZ) spectrometer; the resulting Pearson correlation coefficients were relatively high at 0.94, 0.86, and 0.91, with relative deviations of 2.3%, 3.1%, and 3.5%, respectively.

The polar vortex has strong influence on stratospheric ozone depletion. Potential vorticity (PV), which is used to characterize the polar vortex and determine the edge of polar vortex, is positively correlated with total ozone columns in Antarctic, and the trend of PV and total ozone columns is at the same pace. While during the 2020 Arctic spring ODE, the ozone VCDs and potential vorticity (PV) had a negative correlation with their fluctuations, which is opposite to Southern Hemisphere. The stratospheric ozone profiles and PV profiles show that the most severe ozone depletion caused by polar vortex appeared at the altitude of 19.5-20.5 km.

To better understand the cause of the ozone depletion, we considered the chemical components of ODE process in the Arctic winter of 2019/2020 with the specified dynamics version of the Whole Atmosphere Community Climate Model (SD-WACCM). The SD-WACCM model results indicated that both ClO and BrO concentrations peaked in late March, which was a critical factor during the ozone depletion observed in Ny-Ålesund. Chlorine activation was clearly apparent during the Arctic spring of 2020, whereas the partitioning of bromine species was different from that of chlorine. By combining observations with modeling, we provide a reliable basis for further research on global climate change due to polar ozone concentrations and the prediction of future polar ozone holes.

How to cite: Li, Q., Luo, Y., and Qian, Y.: Research on the stratospheric ozone depletion in the polar spring, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5658, https://doi.org/10.5194/egusphere-egu23-5658, 2023.

EGU23-6394 | ECS | Posters on site | AS3.6

Potential influence of volcanic aerosol on the colour index of ground-based spectroscopic measurements 

Bianca Lauster, Steffen Ziegler, Carl-Fredrik Enell, Udo Frieß, Myojeong Gu, Janis Pukite, Uwe Raffalski, and Thomas Wagner

Polar stratospheric clouds (PSCs) are an important component of the ozone stratospheric chemistry in polar regions. Ground-based spectroscopic measurements can be taken for detecting PSCs in various weather conditions using the so-called colour index (CI) and are a valuable complement to other PSC data sets such as satellite observations.

In this study, continuous long-term measurements from two DOAS (Differential Optical Absorption Spectroscopy) instruments at Kiruna, Sweden (68° N, 20° E), and at the German research station Neumayer, Antarctica (70° S, 8° W) are analysed. In 20 years of measurements, no significant trend is detected for either measurement station. However, the years with preceding large volcanic eruptions show unexpectedly high occurrences of PSC-like signatures during springtime which suggests the influence of volcanic aerosol. This is likewise indicated by enhanced aerosol extinction during these time periods as seen from OMPS (Ozone Mapping and Profiler Suite) data, but is not captured by other PSC climatologies. The observed springtime signal looks very similar to the CI of PSCs and can only be distinguished by other proxy data such as temperature. This ambiguity needs to be considered in the interpretation of colour index data. The potential importance of our results to stratospheric ozone chemistry is not yet clear.

How to cite: Lauster, B., Ziegler, S., Enell, C.-F., Frieß, U., Gu, M., Pukite, J., Raffalski, U., and Wagner, T.: Potential influence of volcanic aerosol on the colour index of ground-based spectroscopic measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6394, https://doi.org/10.5194/egusphere-egu23-6394, 2023.

EGU23-6721 | Posters on site | AS3.6

Redistribution of total reactive nitrogen in the lowermost Arctic stratosphere in winter 2015/2016: In-situ observations of nitrification, denitrification and particulate nitrate 

Helmut Ziereis, Peter Hoor, Jens-Uwe Grooß, Andreas Zahn, Greta Stratmann, Paul Stock, Michael Lichtenstern, Jens Krause, Vera Bense, Armin Afchine, Christian Rolf, Wolfgang Woiwode, Marleen Braun, Jörn Ungermann, Andreas Marsing, Christiane Voigt, Andreas Engel, Björn-Martin Sinnhuber, and Hermann Oelhaf

The Arctic winter 2015/2016 was characterized by extremely low temperatures in the stratosphere and by a very strong polar vortex, accompanied by extended fields of Polar Stratospheric Clouds.  During this winter, aircraft-based measurements were carried out with the research aircraft HALO (High Altitude and Long-Range Research Aircraft) from Kiruna/Sweden and Oberpfaffenhofen/Germany.

Total reactive nitrogen and its distribution between the gas and particle phases are key parameters for understanding processes controlling the ozone budget in the polar winter stratosphere. Tracer-tracer correlations were applied to study the vertical redistribution of gas-phase total reactive nitrogen.  The extended observation period from December to March provided the opportunity to study the changing distribution of reactive nitrogen in the lowermost Arctic stratosphere during the course of the winter. In early winter, during December, the lowermost Arctic stratosphere did not show any indications for disturbed conditions.

The situation changed during the observational period in January and February. Tracer-tracer correlations showed elevated levels of total reactive nitrogen of up to 6 nmol/mol. These observations could be interpreted by evaporation of polar stratospheric particles falling down from the stratosphere above and leading to a nitrification of the lowermost stratosphere. During some periods up to 60 % of the observed total reactive nitrogen can be attributed to evaporating particles. The observation of gas phase nitrification was accompanied by the occurrence of particulate nitrate in extended regions at altitudes between about 10 and 14 km. Usually, the occurrence of particulate nitrate is rare at such altitudes. The diameter of these particles was estimated to range between about 9 and 18 µm.

During the late-winter observation period, no indications for polar stratospheric cloud particles at flight altitude were found. However, extended regions with elevated gas-phase concentrations of total reactive nitrogen were still observed. In late winter, the subsidence of air masses from the polar vortex became increasingly important for the distribution of total reactive nitrogen in the lowermost stratosphere. Air masses with substantial denitrification of up to 5 nmol/mol were observed. In these cases, up to 50 % of the undisturbed total reactive nitrogen was missing. Concurrently lower ozone concentrations were observed, indicating destruction of ozone at higher altitudes.

Nitrification and denitrification of the lowermost stratosphere during the course of the winter are linked by heterogeneous processes in the above-lying stratosphere. Simulations with the CLaMS model confirm and complement the findings of the in-situ observations. They also suggest that the observations have been representative of the vortex-wide redistribution of total reactive nitrogen. The aircraft-based in-situ measurements provided a comprehensive picture of the temporal evolution of the distribution of total reactive nitrogen over the entire winter period 2015/2016.

How to cite: Ziereis, H., Hoor, P., Grooß, J.-U., Zahn, A., Stratmann, G., Stock, P., Lichtenstern, M., Krause, J., Bense, V., Afchine, A., Rolf, C., Woiwode, W., Braun, M., Ungermann, J., Marsing, A., Voigt, C., Engel, A., Sinnhuber, B.-M., and Oelhaf, H.: Redistribution of total reactive nitrogen in the lowermost Arctic stratosphere in winter 2015/2016: In-situ observations of nitrification, denitrification and particulate nitrate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6721, https://doi.org/10.5194/egusphere-egu23-6721, 2023.

EGU23-17448 | Posters on site | AS3.6

A study of T- matrix optical scattering modelling for mixed phase Polar Stratospheric Clouds 

Francesco Cairo, Terry Deshler, Luca Di Liberto, Andrea Scoccione, and Marcel Snels

Scattering codes are used to study the optical properties of Polar Stratospheric Clouds (PSC). Particle backscattering and depolarization coefficients can be computed with available scattering codes once the particle size distribution (PSD) is known and a suitable refractive index is assumed. However, PSCs often appear as external mixtures of Supercooled Ternary Solution (STS) droplets, solid Nitric Acid Trihydrate (NAT) and possibly ice particles, making questionable the assumption of a single refractive index and a single morphology to model the scatterers.
Here we consider a set of fifteen coincident measurements of PSCs above McMurdo Station, Antarctica, by ground-based lidar and balloon-borne Optical Particle Counter (OPC), and in situ observations taken by a laser backscattersonde and OPC during four balloon stratospheric flights from Kiruna, Sweden. This unique dataset of microphysical and optical observations allows to test the performances of optical scattering models when both spherical and aspherical scatterers of different composition and, possibly, shapes are present.
We consider particles as STS if their radius is below a certain threshold value Rth and NAT or possibly ice if above it. The refractive indices are assumed known from the literature. Mie scattering is used for the STS, assumed spherical, while scattering from NAT particles, considered as spheroids of different Aspect Ratio (AR), is treated with T-Matrix results where applicable, and of geometric-optics-integral-equation approach where the particle size parameter is too large to allow for a convergence of the T-matrix method.
The parameters Rth and AR of our model have been varied between 0.1 and 2 micrometers and between 0.3 and 3, respectively, and the calculated backscattering coefficient and depolarization were compared with the observed ones. The best agreement was found for Rth between 0.5 and 0.8 micrometers, and for AR less than 0.55 and greater than 1.5.
To further constrain the variability of AR within the identified intervals we have sought an agreement with the experimental data by varying AR on a case-by-case basis, and further optimizing the agreement by a proper choice of AR smaller than 0.55 and greater than 1.5, and Rth within the interval 0.5 and 0.8 micrometers. The ARs identified in this way cluster around the values 0.5 and 2.5.
The comparison of the calculations with the measurements is presented and discussed. The results of this work help to set limits to the variability of the dimensions and asphericity of PSC solid particles, within the limits of applicability of our model based on the T-matrix theory of scattering and on assumptions on a common particle shape in a PSD and a common threshold radius for all the PSDs. 

How to cite: Cairo, F., Deshler, T., Di Liberto, L., Scoccione, A., and Snels, M.: A study of T- matrix optical scattering modelling for mixed phase Polar Stratospheric Clouds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17448, https://doi.org/10.5194/egusphere-egu23-17448, 2023.

EGU23-606 | Orals | BG1.7

The African greenhouse gases budget: flux trends and uncertainties for the 2009-2019 period 

Yolandi Ernst and Sally Archibald and the RECCAP2 Africa team

Africa contributes significantly to the global greenhouse gases (GHG) budget through extensive land use change that is driven by rapid population growth and low human development status. As part of the REgional Carbon Cycle Assessment and Processes Phase 2 (RECCAP2) project, we developed a comprehensive GHG budget for the period 2009-2019 for Africa. We considered bottom-up process-based models, data-driven remotely sensed products, and national greenhouse gas inventories in comparison with top-down atmospheric inversions, accounting also for lateral fluxes. We incorporated emission estimates derived from novel methodologies for termites, herbivores, and fire, which are of particular importance in Africa. We further constrained global biomass change products with high-quality local observation data. During the RECCAP2 period, Africa remains a net sink for carbon. Emissions from land cover change represents the largest contribution to the African budget. However, land cover change emissions in the drier savanna regions were largely offset by increased vegetation growth in the wet tropics. Additionally, fire emissions decreased as suggested by strong reductions in burned area. Burning of fuelwood has however increased. As expected, an upward trend in anthropogenic fossil fuel emissions was evident, ascribed to an increasing demand for energy by a growing and developing population. For all the component fluxes, uncertainty and interannual variability is large, which highlights the need for increased efforts to address Africa-specific data gaps. However, for RECCAP2, we have improved our overall understanding of many of the important components of the African GHG budget that will help to inform climate policy and action.

How to cite: Ernst, Y. and Archibald, S. and the RECCAP2 Africa team: The African greenhouse gases budget: flux trends and uncertainties for the 2009-2019 period, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-606, https://doi.org/10.5194/egusphere-egu23-606, 2023.

EGU23-1333 | Orals | BG1.7

Synthesis, homogenisation and regionalisation of inland water greenhouse gas budget estimates for the RECCAP2 initiative 

Ronny Lauerwald, George H. Allen, Bridget R. Deemer, Shaoda Liu, Taylor Maavara, Pete Raymond, Lewis Alcott, David Bastviken, Adam Hastie, Meredith A. Holgerson, Matthew S. Johnson, Bernhard Lehner, Peirong Lin, Alessandra Marzadri, Lishan Ran, Hanqin Tian, Xiao Yang, Yuanzhi Yao, and Pierre Regnier

Inland waters are important sources of the greenhouse gasses (GHGs) carbon dioxide (CO2), methane (CH4) and nitrous oxide (N2O) to the atmosphere. While a growing number of global estimates of inland water GHG emissions exists, the integration of inland waters into regional GHG budgets is often hampered by the lack of adequate geo-spatial datasets. Moreover, existing estimates diverge substantially, in part due to persisting uncertainties related to the size and distribution of effective inland water surface areas.  In the framework of the 2nd phase of the REgional Carbon Cycle Assessment and Processes (RECCAP-2) initiative, we synthesize existing estimates of GHG emissions from streams, rivers, lakes and reservoirs, and homogenize them with regard to underlying global maps of inland water surface areas and the effects of seasonal ice cover. We then produce estimates of inland water GHG emissions for 10 extensive land regions that are used for the regional land budgets of RECCAP2. According to our synthesis, global inland waters emit 5.6 (3.5-9.1) Pg CO2 yr-1, 101 (83-135) Tg CH4 yr-1 and 326 (254-592) Gg N2O yr-1. South American rivers contribute about one third of global inland water CO2 emissions. North-American and Russian lakes contribute together one third of global inland water CH4 emissions. Finally, North America alone contributes one fourth of global inland water N2O emissions.

The global inland water emissions sum up to a global warming potential (GWP) of an equivalent emission of 13.6 (10.0-20.3) and 8.3 (5.8-12.7) Pg CO2 yr-1 at a 20- and 100-year horizon, respectively. At 100-year horizon, the contribution of CO2 dominates the GWP of global inland water GHG emissions, with rivers being the largest emitters. At the 20-year horizon, on the contrary, lakes and rivers are equally important emitters, and the contributions of CH4 to the GWP of inland water GHG emissions even exceed those of CO2. Contributions of N2O to the GWP appear to be less significant at both time horizons. Normalized to the area of the RECCAP-2 land regions, South America and South East Asia show the highest inland water emission rates in terms of GWP, dominated by riverine CO2 emissions.

How to cite: Lauerwald, R., Allen, G. H., Deemer, B. R., Liu, S., Maavara, T., Raymond, P., Alcott, L., Bastviken, D., Hastie, A., Holgerson, M. A., Johnson, M. S., Lehner, B., Lin, P., Marzadri, A., Ran, L., Tian, H., Yang, X., Yao, Y., and Regnier, P.: Synthesis, homogenisation and regionalisation of inland water greenhouse gas budget estimates for the RECCAP2 initiative, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1333, https://doi.org/10.5194/egusphere-egu23-1333, 2023.

EGU23-1609 | Posters on site | BG1.7

The Qinghai-Tibet Plateau may have already shifted to carbon source: Evidence from OCO-2 satellite XCO2 observations 

Wei He, Fei Jiang, Weimin Ju, Hengmao Wang, Ngoc Tu Nguyen, and Jing M. Chen

As one of the most sensitive regions to climate change on the Earth's surface, the Qinghai-Tibet Plateau is experiencing lasting warming, which has been evidenced to enhance surface carbon uptake but also could lead to carbon emission due to accelerated permafrost degradation and ecosystem respiration. Due to the difficulties of limited observations and imperfect modeling techniques, whether the Qinghai-Tibet Plateau is a carbon sink or source has been an ongoing debate. The recent satellite XCO2 Observations could provide some useful constraints on the carbon budget in this region.  Here, based on the recent OCO-2 XCO2 observations and the inversion results from the OCO-2 v10 MIP, we estimated the net biome carbon fluxes for the Qinghai-Tibet Plateau. Our results suggest that this region has become a carbon source (around -0.10 PgC/year) already, which is supported by an upscaling estimate with intensified eddy covariance flux measurements over China. Meanwhile, we found this carbon source signal is not detected by either in-situ CO2 inversions or terrestrial biosphere model simulations. Currently, although some studies based on flux measurements report this region is a carbon sink and even keeps increasing recently, many others hold opposite viewpoints about it. Our result provides an important piece of evidence supporting that the Qinghai-Tibet Plateau becomes a carbon source, albeit additional evidence is needed, especially from in-situ CO2 observations and aerial CO2 observations (e.g., by aircraft, unmanned aerial vehicle, and AirCore). In principle, atmospheric CO2 measurements could provide a more complete picture of the carbon budget in this region compared to discrete and limited eddy flux measurements. In the future, enhanced in-situ and aerial CO2 observations are expected to disentangle the puzzle of this carbon budget issue in this region.

How to cite: He, W., Jiang, F., Ju, W., Wang, H., Nguyen, N. T., and Chen, J. M.: The Qinghai-Tibet Plateau may have already shifted to carbon source: Evidence from OCO-2 satellite XCO2 observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1609, https://doi.org/10.5194/egusphere-egu23-1609, 2023.

EGU23-2813 | ECS | Orals | BG1.7

Is destabilisation risk increasing in land carbon sinks? 

Marcos Fernández-Martínez, Josep Peñuelas, Frederic Chevallier, Philippe Ciais, Michael Obersteiner, Christian Rödenbeck, Jordi Sardans, Sara Vicca, Hui Yang, Stephen Sitch, Pierre Friedlingstein, Vivek K. Arora, Daniel Goll, Atul K. Jain, Danica L. Lombardozzi, and Patrick C. McGuire

Global net biome production (NBP), or net land carbon uptake, has been repeatedly shown to increase during recent decades. However, whether the temporal variability and autocorrelation of NBP has changed during this period remains elusive. Answering this question is particularly relevant given that an increase in both could indicate destabilising C sinks and potentially lead to abrupt changes. We investigated the trends and controls of net land C uptake and its temporal variability and autocorrelation, from 1981 to 2018, using two atmospheric inversion models, the amplitude of the seasonal cycle of atmospheric CO2 derived from nine monitoring stations distributed across the Pacific Ocean, and 12 dynamic global vegetation models. Spatially, we found that plant biodiversity presented a convex parabolic relationship with NBP and its temporal variability at the global scale while nitrogen deposition generally increased annual NBP. We also found that annual NBP and its interdecadal temporal variability globally increased, but temporal autocorrelation decreased. Regions characterized by increasingly variable NBP were usually with warmer and with increasingly variable temperatures, and lower and weaker trends in NBP compared to those where NBP variability did not increase, where NBP became stronger. Annual temperature increase and its increasing temporal variability were the most important drivers of declining NBP and increasingly its variability. Our results show that increasing regional NBP variability can be mostly attributed to climate change.

How to cite: Fernández-Martínez, M., Peñuelas, J., Chevallier, F., Ciais, P., Obersteiner, M., Rödenbeck, C., Sardans, J., Vicca, S., Yang, H., Sitch, S., Friedlingstein, P., Arora, V. K., Goll, D., Jain, A. K., Lombardozzi, D. L., and McGuire, P. C.: Is destabilisation risk increasing in land carbon sinks?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2813, https://doi.org/10.5194/egusphere-egu23-2813, 2023.

EGU23-3228 | ECS | Orals | BG1.7 | Highlight

The contemporary Amazon Forest carbon budget 

Thais M. Rosan, Stephen Sitch, Michael O’Sullivan, Christopher Wilson, Luana S. Basso, Dominic Fawcett, Viola A. Heinrich, Jefferson G. Souza, Celso von Randow, Lina M. Mercado, Emanuel Gloor, Luciana Gatti, Pierre Friedlingstein, Andy Wiltshire, Julia Pongratz, Clemens Schwingshackl, and Luiz E.O.C. Aragão and the TRENDY-v11 Team

The Amazon is the largest continuous tropical forest in the world and plays a key role in the global carbon cycle. Human-induced disturbances (e.g., deforestation and wildfires) in combination with climate change have impacted its carbon cycling. However, uncertainties remain on the magnitude of carbon fluxes associated with human-induced disturbances and the old-growth forest sink, and thus the net land carbon balance of the Amazon. Here we synthesize state-of-the-art estimates of the land carbon flux components in the Amazon. To quantify the human-disturbance fluxes from deforestation, land use and land cover changes and degradation, we use a set of bookkeeping models. The annual intact sink was quantified using a set of 16 Dynamic Global Vegetation Models (DGVMs). We then combine the carbon flux estimates from disturbances with the intact sink estimates to provide a bottom-up estimate of the net land carbon flux and compare them alongside top-down estimates from atmospheric model inversions. Between 2010 and 2018, the net land carbon flux in the Brazilian Amazon estimated with the bottom-up approach was -59 (±160) Tg C yr-1 and +36 (±125) Tg C yr-1 with the top-down approach. Despite disagreeing on the sign of the flux, this analysis suggests that the Brazilian Amazon was on average near carbon neutral over the 2010-2018 period, given the large uncertainties underlying both methods. The net land carbon fluxes for the years 2019 and 2020 based on the bottom-up approach were larger than for 2010-2018. This is likely primarily due to direct emissions related to an increase in deforestation although it may possibly be partly caused by a weakening of the forest carbon sink, both in response to deforestation and a warming climate. Spatially, both methodologies agree that the south-eastern Amazon was a net carbon source over the whole study period. These results have important implications for the mitigation potential of Brazilian ecosystems within the goals of the Paris Agreement. 

 

How to cite: Rosan, T. M., Sitch, S., O’Sullivan, M., Wilson, C., Basso, L. S., Fawcett, D., Heinrich, V. A., Souza, J. G., von Randow, C., Mercado, L. M., Gloor, E., Gatti, L., Friedlingstein, P., Wiltshire, A., Pongratz, J., Schwingshackl, C., and Aragão, L. E. O. C. and the TRENDY-v11 Team: The contemporary Amazon Forest carbon budget, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3228, https://doi.org/10.5194/egusphere-egu23-3228, 2023.

EGU23-3303 | ECS | Orals | BG1.7

Near-real-time global gridded daily CO2 emissions 

Xinyu Dou, Zhu Liu, Philippe Ciais, Jinpyo Hong, Frédéric Chevallier, Yilong Wang, Feifan Yan, Steven J. Davis, Monica Crippa, Greet Janssens-Maenhout, Diego Guizzardi, Efisio Solazzo, Xuanren Song, Da Huo, Piyu Ke, Hengqi Wang, and Zhu Deng

Timely, fine-grained gridded carbon emission datasets are particularly important for global climate change research. Often, fine-grained datasets are challenging to visualize over the globe, and clear visualization tools are also needed. Therefore, we present a near-real-time global gridded daily CO2 emissions dataset (GRACED). GRACED provides gridded CO2 emissions at a 0.1° × 0.1° spatial resolution and 1-day temporal resolution from cement production and fossil fuel combustion over seven sectors, including power, industry, residential consumption, ground transportation, domestic aviation, international aviation, and international shipping. GRACED is prepared from the near-real-time daily national CO2 emissions estimates (Carbon Monitor), multi-source spatial activity data and satellite NO2 data for time variations of those spatial activity data. Here, we examined the spatial patterns of sectoral CO2 emission changes from January 1, 2019, to December 31, 2021. In 2021, most regions showed rapid rebounds in carbon emissions compared with 2020, reflecting the continuing challenges to accelerate climate mitigation in the post-COVID era. GRACED provides the most timely and more refined overview than any other previously published datasets, which enables more accurate and timely identification of when and where fossil CO2 emissions have rebounded and decreased as the world recovers from COVID-19 and witnesses contrasted efforts to decarbonize energy systems. Uncertainty analysis of GRACED gives a grid-level two-sigma uncertainty of value of ±19.9%, indicating the reliability of GRACED was not sacrificed for the sake of higher spatiotemporal resolution that GRACED provides. In addition, we also examined the distribution of emission in a grid-wise perspective for major emission datasets, and compared it with GRACED. The similarity in emission distribution was observed in GRACED and other datasets. One of the advantages of our dataset is that it provides worldwide near-real-time monitoring of CO2 emissions with different fine spatial scales at the sub-national level, such as cities, thus enhancing our comprehension of spatial and temporal changes in CO2 emissions and anthropogenic activities. With the continued extension of GRACED time series, we present crucial daily-level input to analyze CO2 emission changes in the post-COVID era, which will ultimately facilitate and aid in designing more localized and adaptive management policies for the purpose of climate change mitigation in the post-COVID era.

How to cite: Dou, X., Liu, Z., Ciais, P., Hong, J., Chevallier, F., Wang, Y., Yan, F., Davis, S. J., Crippa, M., Janssens-Maenhout, G., Guizzardi, D., Solazzo, E., Song, X., Huo, D., Ke, P., Wang, H., and Deng, Z.: Near-real-time global gridded daily CO2 emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3303, https://doi.org/10.5194/egusphere-egu23-3303, 2023.

Determining the temperature dependence of wetland CH4 and CO2 emissions is critical for predicting the impacts of climate change on greenhouse gas (GHGs) emissions in wetland ecosystems. However, the spatial variation for temperature dependence of wetland CH4 and CO2 emissions is poorly understood, especially at the global scale. Here, we investigate the temperature dependencies of wetland CH4 and CO2 emissions across large-scale climatic gradients using 56,271 daily paired observations of ecosystem-level CH4 and CO2 emissions in 45 widely distributed wetlands from the FLUXNET-CH4 database. The temperature dependencies of CH4 and CO2 emissions show contrasting spatial patterns across globally geographic climate gradients. Specifically, the temperature dependence of CH4 emissions  increased with increasing mean annual temperature (MAT), but the opposite was true for that of CO2 emissions. The ratio of CH4 to CO2 emissions was positively dependent on temperature when only MAT and mean annual precipitation were greater than 4.7 °C and 483 mm, respectively. Our results imply that the relative contribution of CH4 to total GHG emissions increases with ambient temperature increases in a warmer and wetter climate region and could act as a positive feedback mechanism in the future. 

How to cite: Chen, H. and Zhou, X.: Contrasting patterns in the temperature dependence of wetland CH4 and CO2 emissions across globally geographic climate gradients, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4684, https://doi.org/10.5194/egusphere-egu23-4684, 2023.

India is primarily concerned with comprehending regional carbon source-sink response in tandem with changes in atmospheric carbon dioxide (CO2) concentrations or human-caused anthropogenic emissions. Atmosphere CO2 is the most significant greenhouse gas contributing to climate change and global warming. To develop a countrywide mitigation policy, it is therefore critical to identify underlying source-sink locations and their mechanisms at various temporal scales and regional levels. To better understand the variability of CO2 and its relationship with the climate variables requires long-term observations. Recent advancements in high-resolution satellite measurements provide a viable opportunity to examine CO2 variability at a regional level. In this work, we presented the long-term variations and growth rates of the Greenhouse Gas Observing Satellite (GOSAT) and Orbiting Carbon Observatory-2 (OCO-2) satellite retrieved column-averaged dry-air mole fraction of CO2 (XCO2 ) and the relationship of XCO2 growth rate with ENSO and climate parameters (temperature, precipitation, soil moisture, and NDVI) over India for the period 2010 to 2021. Results revealed an increase of 2.54 (2.43) ppm/yr of XCO2 in GOSAT (OCO-2) retrievals during overlapping measurement period (2015-2021). In addition, a wavelet analysis shows an increase in XCO2 every year for GOSAT; however, OCO-2 decreases and increases in XCO2 every 5-6 months. This is attributable to high resolutions measurements of OCO-2 favouring better capture of source (high XCO2)-sink (low XCO2) signal than GOSAT. The Principal Component Analysis (PCA) analysis on XCO2 anomalies showed EOF-1 contributed mainly by the south and southeast of India. Further analysis demonstrated that the trend and seasonal cycle of XCO2 regulates the variability. The XCO2 growth rates strongly correlate with ENSO and NDVI (clear during major ENSO events), whereas precipitation and temperature show a weak correlation. Further, lag correlation analysis reveals that ENSO and climate parameters precede the GOSAT XCO2 growth rates, with soil moisture, NDVI, and ENSO having a good correlation with 8,4 and 3 months of leads, respectively.

How to cite: Das, C. and Kunchala, R. K.: Understanding long-term carbon dioxide (CO2) variability and its link with ENSO and climate parameters over India using satellite retrievals, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4738, https://doi.org/10.5194/egusphere-egu23-4738, 2023.

EGU23-5420 | ECS | Posters on site | BG1.7

A global tracer release experiment to help estimate OH tropospheric concentrations and benchmark chemistry-transport models 

Joel Thanwerdas, Dominik Brunner, and Stephan Henne

Despite the urgent need for reduction of greenhouse gas concentrations, their emissions remain at high levels worldwide. Atmospheric inverse modelling allows to quantify these emissions by leveraging observations of greenhouse gas mole fractions and chemistry-transport models. However, this technique largely relies on models with an imperfect representation of transport and chemical processes and the resulting errors propagate to emission estimates. Atmospheric scientists can improve their models by comparing simulated processes against available observational data.

One efficient, although challenging, way of acquiring such validation data is to perform a tracer release experiment. It consists of releasing one or multiple decaying tracers into the atmosphere at one or multiple locations in the world, and then observe their time-evolving mixing ratios to understand transport pathways, mixing and decay rates. To the best of our knowledge, tracer release experiments have only been performed at local or regional scales to study transport processes, but never at the global scale. A global tracer release experiment could generate invaluable data against which to compare model outputs. However, modelers must be able to disentangle transport and chemical processes from the data, which requires that the experiment be carefully designed. Subject to this requirement being met, it could help to better quantify and even reduce 1) transport errors by investigating inter- and intra-hemispheric transport and 2) chemistry errors by constraining OH tropospheric concentrations. These data could also help to create a benchmarking methodology to highlight the strengths and weaknesses of the regional and global models that are currently used to quantify greenhouse gas emissions.

Here, we present design considerations for such a global tracer release experiment based on simulations with the 3-D chemistry-transport model ICON-ART. Our first results indicate that releasing several hundred tons of two tracers with different lifetimes as pulses could be sufficient to obtain a good estimate of OH concentrations along the parcel trajectories. This method could be applied at different locations in order to sample a large part of the world and at different times, e.g., to account for seasonal variations in OH concentrations. However, we also show that many parameters influence the results and therefore we enumerate the benefits but also the limits of such an experiment.

How to cite: Thanwerdas, J., Brunner, D., and Henne, S.: A global tracer release experiment to help estimate OH tropospheric concentrations and benchmark chemistry-transport models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5420, https://doi.org/10.5194/egusphere-egu23-5420, 2023.

EGU23-6152 | ECS | Posters on site | BG1.7

The seasonal cycle of atmospheric CO2 in South America over the last ten years seen by GOSAT 

Lukas Artelt, Eva-Marie Metz, Sanam Vardag, Sourish Basu, and André Butz

The number of in-situ CO2 measurements in the Southern Hemisphere is very limited. This leads to large 
uncertainties in estimates of regional carbon fluxes by in-situ based inverse models. Satellite-based CO2 
measurements, on the other hand, are available in the Southern Hemisphere with a dense spatial 
coverage. By evaluating these, the regional carbon cycle can be studied in more detail and the results of 
carbon cycle models can be validated against the satellite data.

Here, we present a comparison of atmospheric CO2 data provided by the Greenhouse gases Observing 
SATellite (GOSAT) and in-situ based inverse models for South America from 2009 to 2019. The seasonal 
cycle of atmospheric CO2 concentrations measured by the GOSAT satellite shows differences in both,
amplitude and timing, compared to in-situ based atmospheric inversions. To determine the reason for
these discrepancies, we use the TM5-4DVar atmospheric inversion model assimilating GOSAT satellite 
data to obtain GOSAT based land-surface fluxes. This allows us to identify sub-regions responsible for the 
differences. In order to gain a deeper understanding of the underlying processes, we also analyse various 
climate parameters, fire emission data, and vegetation proxies (for example Solar Induced Fluorescence, 
SIF). By doing so, we aim at improving our understanding of the mechanisms that influence the seasonal 
carbon cycle in South America.

How to cite: Artelt, L., Metz, E.-M., Vardag, S., Basu, S., and Butz, A.: The seasonal cycle of atmospheric CO2 in South America over the last ten years seen by GOSAT, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6152, https://doi.org/10.5194/egusphere-egu23-6152, 2023.

EGU23-6173 | ECS | Orals | BG1.7

Carbon fluxes from different fire types in the Amazon and Cerrado biomes quantified using Earth-observation based modelling 

Dominic Fawcett, Leo Ng, Amos Tai, Xiaoyu Yan, Thais Rosan, Celso Silva Junior, Ana Bastos, Philippe Ciais, Clément Albergel, Luiz Aragão, and Stephen Sitch

Fires in the tropics are linked to both climate and land-use change. While in the Amazon, deforestation-related fires decreased following a substantial reduction in deforestation activities until 2012, there have been recent upturns in deforestation and forest fires. Furthermore, earth system models predict a further increase in the intensity of dry seasons in this region in the 21st century. Therefore, carbon emissions from drought-induced forest fires can counteract further pledged deforestation reductions in the following decades, yet they are only partially accounted for in national carbon emission estimates. Improved assessments of fire impacts, including the carbon fluxes arising from post-fire mortality and regrowth, are therefore highly important. 
Combining a range of available satellite products enables spatially specific fire emissions estimations. We developed a remote sensing based approach where biomass maps, observed forest loss, burned area and active fire data are combined to generate updated fuel load and emission estimates. In addition, space-for-time methods are employed to derive estimates of post-fire mortality as a function of pre-fire biomass. This high-resolution model guarantees an improved separation of fire types, and we can report emissions associated with deforestation, forest degradation and savanna fires for the entire Amazon basin and the Brazilian Cerrado at monthly intervals. 
Results show that over 2015-2020 fires cause annual gross emissions of ~300 Tg C over the Amazon and Cerrado. While instantaneous emissions from forest fires are small, the fire-induced mortality and subsequent decomposition cause legacy fluxes which are closer to deforestation fire emissions in magnitude, highlighting their importance. Recent upturns in deforestation fire emissions were observed, including in conservation areas established before 2004. There is overall good agreement with previous instantaneous fire emission estimates from other approaches (GFED4s, GFED 500 m) while remaining disagreements highlight areas of uncertainties, such as combustion completeness values, which could benefit from additional field measurements and spatial modelling supported by EO products.
Outputs from this work can further be used to improve regional greenhouse gas budgets and inform emission reduction and mitigation efforts.

How to cite: Fawcett, D., Ng, L., Tai, A., Yan, X., Rosan, T., Silva Junior, C., Bastos, A., Ciais, P., Albergel, C., Aragão, L., and Sitch, S.: Carbon fluxes from different fire types in the Amazon and Cerrado biomes quantified using Earth-observation based modelling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6173, https://doi.org/10.5194/egusphere-egu23-6173, 2023.

Increasing extreme events and drastic shifts in the variability, intensity and frequency of droughts, heavy precipitation and frost are predicted to accompany further climate change. It is most likely that an increasing occurrence of such events will be accompanied by soil feedback of GHG emissions, particularly of nitrous oxide (N2O) known to be an extremely sensitive GHG. The increase in extreme events can lead to an increased occurrence of short-term emission pulses, referred to as ‘hot moments’, which can contribute significantly to the total annual N2O emission balance.
To account for this potential feedback to the climate system, biogeochemical models driven by climate projections of multi-model ensembles (CPM) can be used to generate scenarios observing future trends in N2O emission behavior.
Most commonly, the CPM average is used as climate input in biogeochemical models. While averaging CPM’s may provide the best overall comparison with real mean climate change, it poses the risk of ‘averaging out’ expected extreme events, thereby biasing soil-atmosphere feedbacks and future N2O emission trends! 

We follow the hypothesis, that for nitrogen-saturated soils as common in industrialized countries, the annual N2O emissions simulated by the averaged CPM differ from the average annual N2O emissions simulated by the individual CPM’s, as hot moment inducing extreme climate events are averaged as well.

For our biogeochemical model simulations, we used weather data from ten selected individual climate-projections based on the multi-model ensemble of the EURO-CORDEX initiative. To focus on the effects of climate and to exclude possible biases, remaining input parameters were unified, i.e., homogeneous soil horizons and a single crop rotation were assumed. In addition, each simulation period was initialised with the same parameters to exclude possible changes in fluxes resulting from soil carbon and nitrogen cycling.

First results with CANDY and LDNDC seem to support our hypothesis, showing that annual N2O emissions simulated with the averaged CPM differ clearly from those resulting from the output mean of the individual CPM’s.

This emphasises to consider using the averaged output based on individual CPM’s rather than relying solely on averaged CPM’s for predicting future N2O emission trends.

How to cite: Hey, L., F. Jungkunst, H., and H. E. Meurer, K.: A potential bias using averaged climate projection multi model ensembles when forecasting nitrous oxide emissions from soils under climate change, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8208, https://doi.org/10.5194/egusphere-egu23-8208, 2023.

EGU23-8372 | Orals | BG1.7

Why atmospheric methane surged in 2020? 

Shushi Peng, Xin Lin, Rona Thompson, Yi Xi, Gang Liu, Xin Lan, Didier Hauglustaine, Benjamin Poulter, Michel Ramonet, Marielle Saumois, Yi Yin, Zhen Zhang, Bo Zheng, and Philippe Ciais

Methane (CH4) levels in the atmosphere increased by 15.1 ± 0.4 ppb in 2020, the highest annual increase from 1984 to 2020, despite a likely decrease in anthropogenic CH4 emissions during COVID-19 confinements. Here, we used bottom-up and top-down methods to quantify the changes in different sources of CH4, and in its atmospheric sink due to the hydroxyl radical (OH) in 2020 compared to 2019. Bottom-up methods showed that, globally, total anthropogenic emissions slightly decreased by ~1.2 Tg CH4 yr-1, fire emissions were lower than in 2019 by ~6.5 Tg CH4 yr-1, and wetland emissions increased by 6.0 ± 2.3 Tg CH4 yr-1. In addition to higher wetland emissions in 2020 than 2019 from bottom-up, we found a decrease of 1.6–1.8% in tropospheric OH concentration relative to 2019, mainly due to lower anthropogenic NOx emissions and associated lower free tropospheric ozone during the confinements. Based on atmospheric CH4 observations from the surface network, and considering the decrease in OH, using top-down inversions, we infer that global net emissions increased by 6.9 ± 2.1 Tg CH4 yr-1 in 2020 relative to 2019, while the global CH4 removal from reaction with OH in the atmosphere decreased in 2020 by 7.5 ± 0.8 Tg CH4 yr-1. Therefore, we attribute the positive growth rate anomaly of atmospheric CH4 in 2020 relative to 2019 to lower OH sink (53 ± 10%) and higher natural emissions (47 ± 16%), mostly from wetlands. Warmer and wetter climate conditions in the Northern Hemisphere promoted wetland emissions, but fires decreased in the Southern Hemisphere, compared to the previous year. Our study highlights that northern microbial emissions of CH4 are highly sensitive to a warmer and wetter climate and could act as a positive feedback in the future. Our study also hints that the global CH4 pledge must be implemented by taking into account NOx emissions trend, whose reduction lengthens the lifetime of atmospheric CH4.

How to cite: Peng, S., Lin, X., Thompson, R., Xi, Y., Liu, G., Lan, X., Hauglustaine, D., Poulter, B., Ramonet, M., Saumois, M., Yin, Y., Zhang, Z., Zheng, B., and Ciais, P.: Why atmospheric methane surged in 2020?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8372, https://doi.org/10.5194/egusphere-egu23-8372, 2023.

EGU23-9695 | ECS | Orals | BG1.7

Biomass recovery after fires dominates the carbon sink of boreal forests over the last three decades 

Yidi Xu, Philippe Ciais, Wei Li, Sassan Saatchi, Maurizio Santoro, Alessandro Cescatti, Dmitry Shchepashchenko, Guojin He, Ceccherini Guido, Jiaying He, Lei Fan, Martin Brandt, Rasmus Fensholt, Jean-Pierre Wigneron, Heather Kay, Stephen Sitch, Ana Bastos, Simon Bowing, François Ritter, and Ibrahim Fayad

Wildfires are an integral part of boreal forest dynamics. Understanding the carbon loss/recovery associated with fires is crucial to assess the stability of these slow-growing forests.  Yet, the carbon balance from fires and post-fire forest recovery remain uncertain at the biome scale due to the lack of spatial details about rates of forest regrowth. Here, we quantify carbon losses from fire emissions and gains from post-fire regrowth using high spatial-resolution satellite data and a bookkeeping model. We combined a 35-year long record of burned area from the Landsat satellites since 1985 with local biomass-age regrowth curves derived from high-resolution satellite-based above ground biomass (AGB) datasets. We found that forests in Eurasia tend to recover faster and reach higher biomass levels than those in North America. Young forests recovering from post-1985 wildfires produced a carbon sink of 652±200 TgC during the period 1985 to 2020. The additional recovery of older secondary forests that burned before 1985 further adds a cumulative sink of 1659±346 TgC. Comparatively, old-growth forests that did not burn accumulated 930±233 TgC during the period 1985-2020. This result shows 71% of the contemporary carbon sink in AGB is contributed by recovery from fires. After accounting for fire emissions each year and for the slow decay of coarse woody debris after burning, the net AGB carbon sink in boreal forests is 2108±234 TgC during 1985-2020. This study provides the first spatially explicit aboveground observation-based carbon budget of boreal forests and provides insights on the key factors that will control its future evolution.

How to cite: Xu, Y., Ciais, P., Li, W., Saatchi, S., Santoro, M., Cescatti, A., Shchepashchenko, D., He, G., Guido, C., He, J., Fan, L., Brandt, M., Fensholt, R., Wigneron, J.-P., Kay, H., Sitch, S., Bastos, A., Bowing, S., Ritter, F., and Fayad, I.: Biomass recovery after fires dominates the carbon sink of boreal forests over the last three decades, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9695, https://doi.org/10.5194/egusphere-egu23-9695, 2023.

EGU23-10462 | Posters virtual | BG1.7

An assessment of sea-air CO2 flux in the Arctic Ocean from 1985 to 2018 

Sayaka Yasunaka, Manfredi Manizza, Jens Terhaar, Are Olsen, Ryohei Yamaguchi, Peter Landschützer, Eiji Watanabe, Dustin Carroll, Hanani Adiwira, Jens Müller, and Judith Hauck

As a contribution to the Regional Carbon Cycle Assessment and Processes phase 2 (RECCAP2) project, we present synthesized estimates of the Arctic Ocean CO2 uptake and their uncertainties from state-of-the-art surface ocean pCO2-observation products, global and regional ocean biogeochemical models and atmospheric inversions. For the period of 1985−2018, the Arctic Ocean represents a net sink of CO2 of 103 ± 19 TgC yr−1 in the pCO2 products and 92 ± 30 TgC yr−1 in the ocean biogeochemical models. While the long-term mean CO2 uptake in the Arctic Ocean is primarily caused by steady-state fluxes of natural carbon, it is enhanced 28% by the atmospheric CO2 increase and 15% by climate change. Moreover, the climate effect in the Arctic Ocean has become more important in recent years. The CO2 uptake peaks in late summer and early autumn, and is low in winter because the sea ice cover inhibits sea-air fluxes. The annual mean of CO2 uptake increased due to the decreasing sea ice concentration both in the pCO2 products and the ocean biogeochemical models. Both, the mean CO2 uptake and the trend, is substantially weaker in the atmospheric inversions. Uncertainty across all estimates is large especially in the estimated surface ocean pCO2 values in the East Siberian Sea and the Laptev Sea, due to scarcity of observations and missing processes in models, such as land-sea fluxes and sediment dynamics.

How to cite: Yasunaka, S., Manizza, M., Terhaar, J., Olsen, A., Yamaguchi, R., Landschützer, P., Watanabe, E., Carroll, D., Adiwira, H., Müller, J., and Hauck, J.: An assessment of sea-air CO2 flux in the Arctic Ocean from 1985 to 2018, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10462, https://doi.org/10.5194/egusphere-egu23-10462, 2023.

An increasing trend is observed in the frequency of climate extremes. Drought is a widely observed extreme event that has a significant influence on the terrestrial ecosystem functioning and carbon balance. Interannual variability in the Indian summer monsoon (ISM) rainfall, an important meteorological phenomenon providing 90 percent of the country’s annual precipitation, also significantly influences the vegetation carbon processes and carbon balance. Identifying the changes in vegetation greenness and terrestrial carbon fluxes to droughts and variability in ISM is essential for planning mitigation strategies and policy making. The main objective of this study is to identify the impact of drought and ISM variability in terrestrial biosphere carbon processes and their impact on the national carbon budget. Here we attempt a comprehensive study using different meteorological datasets available and CO​2 flux data prescribed from inversion, process-based, and LUE-based models to quantify the impact of extreme events and monsoonal variability on the ecosystem behavior and, thereby, on the atmosphere-biosphere  CO​2 exchange fluxes over the Indian region while considering prominent vegetation classes. We also use the inference from the satellite-derived  Solar Induced Fluorescence (SIF) and eddy covariance flux observations over the region. Preliminary results will be presented and discussed. 

How to cite: Ravi P, A. and K Pillai, D.: Assessing the impact of climate extremes and Indian summer monsoon variability on terrestrial biosphere carbon fluxes over Indian region using satellite observations and modeling., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10881, https://doi.org/10.5194/egusphere-egu23-10881, 2023.

EGU23-10894 | Orals | BG1.7

Seasonal variabiltiy of the surface ocean carbon cycle: a global synthesis 

Keith Rodgers and the RECCAP2 coauthors: seasonal variabiltiy in surface ocean carbon cycle

Here we present a synthesis of surface ocean pCO2 and air-sea CO2 flux seasonality for a modern climatology and      their decadal trends between the 1980s and 2010s, as part of the REgional Carbon Cycle Assessment and Processes Phase 2 (RECCAP2) project. Working with both surface ocean pCO2-observation products (pCO2 products) and global ocean biogeochemistry models (GOBMs), our main findings are: (i) Over biome scales, both pCO2 products and GOBMs confirm increases in the seasonal amplitude of pCO2 and integrated CO2 fluxes between 1985-1989 and 2014-2018. (ii) For the 2014-2018 climatology, GOBMs exhibit a systematic bias with too-weak biologically-driven seasonal variability in surface dissolved inorganic carbon (DIC), such that the pCO2 seasonal cycle in subtropical biomes is spuriously large and both the amplitude and phase of seasonal pCO2 variations diverge from those in the pCO2 products in subpolar and circumpolar biomes. (iii) Decadal increases in pCO2 seasonal cycle amplitude in subtropical biomes are attributed to being largely driven by reducing CO2 buffering capacity and increasing sensitivity to temperature due to increasing anthropogenic carbon (Cant) content insurface waters for both the pCO2 products and GOBMs. In subpolar and circumpolar biomes, the seasonality change for GOBMs is dominated by Cant invasion, whereas for pCO2 products modulations of the climate state are equally important. (iv) Considered together, the subtropical biomes exhibit decadal increases in CO2 flux seasonality that are larger during winter than summer, consistent with the mechanism described by Fassbender et al. (2022) and potentially promoting a negative feedback in the climate system by increasing the CO2 uptake in winter, by virtue of surface winds being stronger in winter than summer. (v) Large ensemble simulations with ESMs were applied to confirm the validity of biomes as aggregation domains for identifying forced signals. Despite compromises to DIC seasonality impacting pCO2 seasonality, the chosen biome-scale is appropriate for representing the decadal rate of increase of pCO2 seasonality for both GOBMs  and pCO2 products.

How to cite: Rodgers, K. and the RECCAP2 coauthors: seasonal variabiltiy in surface ocean carbon cycle: Seasonal variabiltiy of the surface ocean carbon cycle: a global synthesis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10894, https://doi.org/10.5194/egusphere-egu23-10894, 2023.

EGU23-11163 | ECS | Posters on site | BG1.7

A new gap-filling method to avoid systematic bias in carbon balance estimates in northern ecosystems 

Henriikka Vekuri, Juha-Pekka Tuovinen, Liisa Kulmala, Dario Papale, Pasi Kolari, Mika Aurela, Jari Liski, Tuomas Laurila, and Annalea Lohila

Climate change mitigation requires – besides greenhouse gas emission reductions – actions to increase carbon sinks and storages in terrestrial ecosystems. However, quantification of sources and sinks of carbon depends on reliable estimates of the net ecosystem exchange of carbon dioxide (CO2). This also involves the eddy covariance technique (EC), a key method to directly measure the CO2 fluxes between ecosystems and the atmosphere. Various methods have been used to impute, or gap-fill, missing EC data and previous comparisons have shown that the accuracy of the best-performing methods, e.g. the widely-used marginal distribution sampling (MDS), is reaching the noise limit of measurements. However, knowledge on the performance of gap-filling methods is lacking from northern ecosystems.

By analyzing an extensive global data set, we show that MDS causes significant carbon balance errors for northern ecosystems. MDS systematically overestimates the carbon dioxide (CO2) emissions of carbon sources and underestimates the CO2 sequestration of carbon sinks. We discuss reasons for the errors and show how a machine learning method called extreme gradient boosting or a modified version of MDS can be used to minimize the northern site bias.

How to cite: Vekuri, H., Tuovinen, J.-P., Kulmala, L., Papale, D., Kolari, P., Aurela, M., Liski, J., Laurila, T., and Lohila, A.: A new gap-filling method to avoid systematic bias in carbon balance estimates in northern ecosystems, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11163, https://doi.org/10.5194/egusphere-egu23-11163, 2023.

EGU23-11303 | ECS | Posters on site | BG1.7

Recent methane trends derived from S5P/TROPOMI data 

Jonas Hachmeister, Oliver Schneising, Michael Buchwitz, John P. Burrows, Justus Notholt, and Matthias Buschmann

Methane (CH4) has a relatively long tropospheric lifetime and is consequently a well-mixed greenhouse gas. CH4, released by several
types of human activity and natural processes, is one important driver of climate change. The global mean concentration of CH4 has
increased by 156% between the beginning of the industrial revolution around 1750 and 2019, reaching roughly 1866 ppb in 2019 (IPCC).
The time dependence of this increase is not well understood. For example, it is not entirely clear why CH4 growth rates reached record 
high values in 2020 and 2021. Furthermore, the number of published growth rates (annual methane increases) is limited and includes data
from NOAA and the Copernicus Climate Change Service. Hence the rate of increase of CH4 calculated from independent data sources are
valuable for cross-verification and in furthering our understanding of the methane cycle.
The TROPOMI instrument onboard the Sentinel-5P satellite provides daily CH4 data with a spatial resolution of roughly 7x7 km²
and global coverage. We analyze the TROPOMI CH4 data with the goal of determining robust values of the annual methane increases (AMI)
for both global and zonally resolved data. For this we utilize a dynamic linear model approach to separate the underlying methane level,
the seasonal and short-term variations. The AMIs are defined as the difference in the underlying (i.e. fitted) methane level between
the first and last day of a year. In this contribution, we present first results for global and zonal TROPOMI AMIs for the years 2019-2022.
We compare the resulting global TROPOMI AMIs with data from NOAA and Copernicus and discuss the distribution of zonal AMIs for the given years.

How to cite: Hachmeister, J., Schneising, O., Buchwitz, M., Burrows, J. P., Notholt, J., and Buschmann, M.: Recent methane trends derived from S5P/TROPOMI data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11303, https://doi.org/10.5194/egusphere-egu23-11303, 2023.

EGU23-12203 | ECS | Posters on site | BG1.7

Fire emission estimates for Australian extreme fire season 2019/2020 using FLEXPART  

Ines Dillerup, Christopher Lüken-Winkels, Eva-Marie Metz, Sanam Vardag, Nicholas Deutscher, David Griffith, and André Butz

In Australia, increasing temperatures and prolonged drought periods lead to an intensification of wildfires. In particular, severe fires are expected to occur more frequently in Southeast Australia’s eucalyptus forests leading to strongly enhanced CO2 emissions and preventing the renewed uptake of the released CO2 by vegetation. However, current fire emission estimates presented by conventional fire emission databases show significant discrepancies in their emission estimates of extreme fire events like the Australian fire season 2019/2020.

Here, we investigate the fire emissions released during the Australian summer 2019/2020 based on total column measurements of CO2 and CO using the Lagrangian Particle Dispersion Model FLEXPART. We calculate footprints and backward trajectories of trace gases to inversely retrieve carbon emission estimates. In a first case study we focus on TCCON total column measurements of CO and CO2 taken in Wollongong located close to the hot-spot of eucalyptus fires. As the measurements show a significant enhancement of all mentioned tracers during the fire event, FLEXPART is used to calculate emission estimates for southeast Australia. Furthermore, we retrieve emission factors between the trace gases. Our results are compared to the conventional databases like GFED, GFAS and FINN and emission estimates published by other studies.

How to cite: Dillerup, I., Lüken-Winkels, C., Metz, E.-M., Vardag, S., Deutscher, N., Griffith, D., and Butz, A.: Fire emission estimates for Australian extreme fire season 2019/2020 using FLEXPART , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12203, https://doi.org/10.5194/egusphere-egu23-12203, 2023.

EGU23-12424 | ECS | Posters on site | BG1.7

Constraining land surface CO2 fluxes by ecosystem and atmospheric observations using atmospheric transport 

Samuel Upton, Wouter Peters, Markus Reichstein, Santiago Botia, Fabian Gans, Basil Kraft, and Ana Bastos

The growth rate of atmospheric CO2 mole fractions can be measured with high accuracy, but there are still large uncertainties in our ability to separate anthropogenic and natural sources and sinks. One major source of uncertainty is the net flux of carbon from the biosphere to the atmosphere, or Net Ecosystem Exchange (NEE). There are two major approaches to quantifying NEE; top-down approaches that typically use atmospheric inversions, and bottom-up estimates using process-based or data-driven terrestrial biosphere models, upscaled to the regional or global scale. Both approaches have known limitations. A system that harmonizes these approaches, providing a high-quality estimate of the spatial distribution of NEE, and an accurate integral of NEE at regional and global scales, would improve our ability to model the full carbon budget. With other component fluxes, a harmonized product could help improve our monitoring of regional and national greenhouse gas budgets, and thus verify the trajectory towards CO2 emission goals.

This study builds upon our previous work that connected the bottom-up eddy-covariance model to top-down estimates of regional NEE from atmospheric inversions using fixed regional linear oper-ators. That work demonstrated that top-down estimates of atmospheric CO2 provide an important additional constraint to a data-driven bottom up model. The use of top-down constraints improved the regional and global upscaling of NEE, leveraging the strengths of the two different approaches. However, the previous work had a simplified computational link between the top-down and bottom-up fluxes of NEE, and did not access the very large volume of atmospheric observations of atmospheric CO2. Here, we replace the regional atmospheric inversion estimates of NEE with direct observations of the atmospheric mole fractions of CO2. The fixed regional linear operators are replaced by estimating the near-field sources of an observation using an atmospheric transport model. For training, the bottom-up model is run for the source locations. We apply this technique to observations from to tropical, extra-tropical and boreal tall-tower sites over different meteorological conditions where we infer NEE from the observed atmospheric mole fraction, corrected for CO2 background and non-biogenic CO2 fluxes. This inference is combined in the objective function with tower-level inferences, and directly used to update the bottom-up model. The model can ‘see’ more varied inputs in the dynamic footprints, and the size of our pool of training data is increased. The new process improves our ability to accurately infer the regional and global distribution of NEE by directly learning across spatial scales, using diverse observations of CO2.

How to cite: Upton, S., Peters, W., Reichstein, M., Botia, S., Gans, F., Kraft, B., and Bastos, A.: Constraining land surface CO2 fluxes by ecosystem and atmospheric observations using atmospheric transport, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12424, https://doi.org/10.5194/egusphere-egu23-12424, 2023.

EGU23-12786 | Orals | BG1.7

Constraining regional and global ocean carbon fluxes in RECCAP2 

Judith Hauck, Nicolas Gruber, Masao Ishii, and Jens Daniel Müller and the RECCAP2 ocean chapter leads

Keeping global warming in line with the Paris Agreement requires rapid reductions in CO2 emissions. Tracking these reductions demands a thorough bookkeeping of natural and anthropogenic carbon fluxes. The second REgional Carbon Cycle Assessment and Processes (RECCAP2) activity of the Global Carbon Project aims to accurately assess land and ocean CO2 sources and sinks through the efforts of hundreds of scientists around the globe. 

For the ocean component, regional budgets are developed for the global ocean and five large regions for the period 1980-2018. In addition, four ‘special focus’ themes, namely the biological carbon pump, the seasonal cycle, the coastal ocean and model evaluation are addressed. We use state-of-the-art ocean models and observation-based datasets to provide robust estimates of regional CO2 budgets and constrain their uncertainties. Here, we will provide an overview of RECCAP2 activities, and showcase key results focusing on mean ocean carbon fluxes, and their trends and variability.

How to cite: Hauck, J., Gruber, N., Ishii, M., and Müller, J. D. and the RECCAP2 ocean chapter leads: Constraining regional and global ocean carbon fluxes in RECCAP2, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12786, https://doi.org/10.5194/egusphere-egu23-12786, 2023.

EGU23-12963 | ECS | Posters on site | BG1.7

High-resolution quantification of aboveground carbon change over the tropics 

Yu Feng, Philippe Ciais, Yidi Xu, Jean-Pierre Wigneron, Xiaojun Li, and Lei Fan

Tropical ecosystems play an important role in regulating the global carbon balance. Existing studies have extensively analyzed the carbon dynamics of tropical forests, the largest terrestrial component of the global carbon budget, showing a likely neutral contribution of tropical forests to the global carbon cycle. However, high-resolution dynamics of aboveground carbon (AGC) change of the whole tropical terrestrial ecosystem and its processes remain rarely investigated. In this study, we first used low-frequency L-band passive microwave observations to derive wall-to-wall maps of annual AGC stocks over the tropics at 25-km spatial resolution. Using high-resolution satellite observations of land-cover change and biomass maps and random forest models, we separated the AGC stock into various ecosystems, including forest, shrub, and short-vegetation (grass and crop), and attributed the change to different degradation processes such as fires and deforestation at 100-m resolution. Our preliminary results show that total AGC stocks in tropical ecosystems increased by  +2.25 [+1.19,+3.29] PgC (the range represents the minimum and maximums of the multiple estimates) from 2010 to 2020. The coast of Brazilian Mata Atlantica, Central African Republic, and east Tanzania are the hotspots of net increase, while the Arc of Deforestation in the Amazon basin and the Congo Basin show substantial net losses. Gross losses from non-fire deforestation and fire totaled -1.62 [-1.38,-1.86] PgC yr-1. We also observed strong recovery in African burned regions, possibly due to post-fire regrowth and additional recovery resulting from declining fires in the region. Our results highlight the importance of explicit temporal and spatial mapping of tropical carbon dynamics at high resolution, which can help us better understand the role of tropical terrestrial ecosystems in the global carbon cycle.

How to cite: Feng, Y., Ciais, P., Xu, Y., Wigneron, J.-P., Li, X., and Fan, L.: High-resolution quantification of aboveground carbon change over the tropics, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12963, https://doi.org/10.5194/egusphere-egu23-12963, 2023.

EGU23-13759 | Orals | BG1.7

An assessment of CO2 storage and sea-air fluxes for the Atlantic Ocean and Mediterranean Sea between 1985 and 2018  

Fiz F. Perez, Marion Gehlen, Jerry Tjiputra, Are Olsen, Meike Becker, Marta Lopez-Mozos, Jens D. Müller, Nadine Goris, and Judith Hauck

The dynamic and thermohaline characteristics of the Atlantic Ocean linked to the Atlantic Meridional Overturning Circulation (AMOC) give it a specific role in the accumulation of heat and CO2, either of natural or anthropogenic origin (Cant), from the surface layer to the deep waters, significantly mitigating the impacts of anthropogenic climate change. Here, we evaluate the annual mean, long-term trends, seasonal cycle and interannual variability of net sea-air CO2 fluxes (FCO2) between 1985 and 2018 based on observation products (pCO2-products) and global ocean biogeochemical models (GOBMs) for the Atlantic from 30ºS to the Nordic Seas (~79ºN) and the Mediterranean. The mean contemporary FCO(sum of anthropogenic and natural components) is estimated to be 0.362 ± 0.067 and 0.47 ± 0.15 Pg C yr-1 using pCO2-products and GOBMs, respectively. The GOBMs show consistent growth trends in CO2 uptake with rates similar to the atmospheric CO2 growth, however trends obtained from CO2-products show a sharp increase from the pre-2000 period to the post-2000 period. There is overall agreement between pCO2-products and GOBMs results for mean values, seasonal cycle and interannual variability in all biomes, except for the North Atlantic subpolar biome, where pCO2-products show lower mean values, larger trends, and a different seasonal cycle than GOBMs. The GOBMs and pCO2-products show very concordant values in equatorial and subtropical regions, where CO2 variability is strongly determined by temperature. For the period 1994-2007, GOBMs show concordant values in annual Cant storage rate with carbonate marine system observations (Gruber et al., 2019) with values of 0.506 ± 0.106 Pg C yr-1 vs 0.673 ± 0.066 Pg C yr-1, respectively. The Cant storage rate agreement between GOBMs and observations are also registered in the different biomes, although in both permanently stratified subtropical in North and South Atlantic biomes, the storage rates in GOBMs show a larger spread with their mean values 30 and 40% lower than those estimated from observations. In general, the Atlantic accumulates more Cant than that inferred from the cumulative FCO2 changes, partly due to a significant lateral Cant transport from the Southern Ocean (about 30%).

How to cite: Perez, F. F., Gehlen, M., Tjiputra, J., Olsen, A., Becker, M., Lopez-Mozos, M., Müller, J. D., Goris, N., and Hauck, J.: An assessment of CO2 storage and sea-air fluxes for the Atlantic Ocean and Mediterranean Sea between 1985 and 2018 , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13759, https://doi.org/10.5194/egusphere-egu23-13759, 2023.

EGU23-13792 | Orals | BG1.7

Impacts of land use and environmental change on the Eastern European land carbon sink 

Karina Winkler, Hui Yang, Raphael Ganzenmüller, Richard Fuchs, Guido Ceccherini, Grégory Duveiller, Giacomo Grassi, Julia Pongratz, Ana Bastos, Anatoly Shvidenko, Arnan Araza, Martin Herold, and Philippe Ciais

Land-based mitigation is essential in reducing carbon emissions. Yet, the attribution of land carbon fluxes to their sinks and sources remains highly uncertain, in particular for the forest-rich but data-poor region of Eastern Europe. Here we integrate various data sources (from top-down and bottom-up modelling, earth observation, inventories) to show that Eastern Europe accounted for an annual aboveground biomass (AGB) carbon sink of ~0.49 GtC in 2010‑2019, or about 75% of the entire European carbon uptake. However, we find that the land-based carbon sink is declining. This declining trend is mainly driven by changes in land use and land management, but also by increasing natural disturbances due to ongoing climate change. Despite the high overall importance of environmental factors such as soil moisture, nitrogen and CO2 for enhancing the land-based carbon sink, we find indicators of a saturation effect of the regrowth in abandoned former agricultural areas, combined with an increase in wood harvest, particularly in European Russia. Our results contribute to a better understanding of the regional carbon budget of Eastern Europe and its trend. This study sheds light on land use and management as drivers of the land-based carbon sink and their role for climate mitigation.

How to cite: Winkler, K., Yang, H., Ganzenmüller, R., Fuchs, R., Ceccherini, G., Duveiller, G., Grassi, G., Pongratz, J., Bastos, A., Shvidenko, A., Araza, A., Herold, M., and Ciais, P.: Impacts of land use and environmental change on the Eastern European land carbon sink, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13792, https://doi.org/10.5194/egusphere-egu23-13792, 2023.

EGU23-14171 | ECS | Posters on site | BG1.7

Numerical simulation of the atmospheric CH4 increase and the corresponding decrease of δ13C(CH4) after 2007 

Anna-Leah Nickl, Franziska Winterstein, and Patrick Jöckel

The global atmospheric CH4 growth rate stagnated between 2000 and 2007, and has continued to grow since 2007. This renewed CH4 rise has been analysed with respect to a 2007 onward decline in  δ13C(CH4), indicating changes in the relative contribution of CH4 sources. However, this is still subject to debate and a variety of hypotheses have been put forward. In our work, we present numerical sensitivity simulations that investigate the impact of different inventories of methane emission fluxes on the globally averaged δ13C(CH4) signature. We apply the state-of-the-art global chemistry-climate model EMAC and use a simplified approach to simulate methane loss. We include methane isotopologues and take the kinetic isotope effects in physical and chemical processes into account. We further consider regional differences in the isotopic signatures of individual emission source categories, such as, for example, the differences between signatures of tropical and boreal wetlands emissions. Based on recent emission inventories and isotopic source signatures from the literature, our chemistry climate model reproduces the actual atmospheric methane and δ13C(CH4) distribution adequately. We show that our setup is suitable to constrain the individual influence of different CH4 sources on the global average δ13C(CH4). We further present an approach to optimize the global methane level with respect to station measurements probing for a strategy to include the isotopic information into such an optimization process.

How to cite: Nickl, A.-L., Winterstein, F., and Jöckel, P.: Numerical simulation of the atmospheric CH4 increase and the corresponding decrease of δ13C(CH4) after 2007, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14171, https://doi.org/10.5194/egusphere-egu23-14171, 2023.

EGU23-15006 | ECS | Orals | BG1.7

A comprehensive synthesis of anthropogenic and natural sources and sinks of Australasia carbon budget (2010-2019) 

Yohanna Villalobos, Pep Canadell, Peter Briggs, Ian Harman, Elizabeth D. Keller, Beata Bukosa, Sara E. Mikaloff-Fletcher, Ben Smith, Miko UF. Kirschbaum, Donna Giltrap, Liyin Liang, Ronny Lauerwald, Judith Rosentreter, Taylor Maavara, Laure Resplandy, Peter J. Rayner, Eva Schöemann, and Sourish Basu

Accurate national carbon budget assessments allow nations to evaluate their progress in cutting carbon emissions and therefore be aligned with the Paris Climate Agreement goals. To support the initiative of The REgional Carbon Cycle Assessment and Processes (RECCAP-2), we built a synthesis of the Australasia (Australia and New Zealand) terrestrial carbon budget for 2010-2019 based on top-down and bottom-up approaches. Major carbon flux components in the bottom-up budget (e.g., net primary productivity and heterotrophic respiration) were simulated by CABLE model, Biome-BGC model and Cewn simulations. In addition, this budget include carbon flux components from the land-ocean aquatic continuum, such as inland waters, estuaries, blue carbon ecosystems, and continental shelves and carbon fluxes embodied in trade (export and import) of crops, woods, livestock and fossil fuel. We reconciled Australia and New Zealand bottom-up budgets separately with fluxes derived from regional and global OCO-2, GOSAT flux inversions, as well as fluxes obtained from in-situ measurement only (CarbonWatchNZ). We found that annual mean budgets for Australia agree relatively well (within the uncertainty range) with regional and global top-down GOSAT and OCO-2 flux estimates. New Zealand's annual bottom-up carbon budget also agrees relatively well with fluxes derived from CarbonWatchNZ inversion and GOSAT but disagrees with global flux estimates from OCO-2.

How to cite: Villalobos, Y., Canadell, P., Briggs, P., Harman, I., Keller, E. D., Bukosa, B., Mikaloff-Fletcher, S. E., Smith, B., Kirschbaum, M. UF., Giltrap, D., Liang, L., Lauerwald, R., Rosentreter, J., Maavara, T., Resplandy, L., Rayner, P. J., Schöemann, E., and Basu, S.: A comprehensive synthesis of anthropogenic and natural sources and sinks of Australasia carbon budget (2010-2019), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15006, https://doi.org/10.5194/egusphere-egu23-15006, 2023.

EGU23-15146 | ECS | Orals | BG1.7

A new approach for estimating anthropogenic carbon relying on an observational back-calculation method 

Marta López-Mozos, Fiz F. Pérez, Lidia I. Carracedo, Geoffrey Gebbie, and Antón Velo

Around 31% of carbon dioxide derived from human activities (Canth) has been absorbed by the ocean (DeVries, 2014; Gruber et al., 2019; Sabine et al., 2004). This accumulation helps to mitigate atmospheric carbon dioxide (CO2), but in turn leads to severe consequences on marine systems (IGBP, IOC, SCOR, 2013). Both components of CO2, i.e. anthropogenic and natural, present high variability and uncertainties difficult to observe and quantify. In particular, the Canth signal represents a small fraction of the total dissolved inorganic carbon pool (CT) and it is not directly distinguishable from the natural component, resulting in the emergence of back-calculation techniques (Brewer 1978; Chen and Millero, 1979) to derive it indirectly. Over the years, back-calculation techniques have undergone remarkable improvements (Gruber et al., 1996; Sabine et al., 2004; Touratier et al., 2004, 2007; Vázquez-Rodríguez et al., 2009a, 2009b, 2012), resulting in different methods for estimating Canth that, despite providing helpful and advanced results, show various biases and limitations. Here, we present a new approach for estimating Canth that relies on a back-calculation methodology, purely based on carbon data, and provides results that show good agreement with previous global Canth climatologies. Our approach mainly differs from previous methodologies by pioneering using the transport matrix output from a data‐assimilating ocean circulation inverse model (TMI: Total Matrix Intercomparison; Gebbie and Huybers, 2010) to obtain preformed properties, instead of the historical use of Optimum Multiparameter analysis (OMP). This improvement prevents from the need to use (sub)surface-property linear regressions to estimate preformed alkalinity or air-sea CO2 disequilibrium, and allows introducing different corrections for denitrification and, as a novelty, oxygen disequilibrium.

How to cite: López-Mozos, M., Pérez, F. F., Carracedo, L. I., Gebbie, G., and Velo, A.: A new approach for estimating anthropogenic carbon relying on an observational back-calculation method, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15146, https://doi.org/10.5194/egusphere-egu23-15146, 2023.

EGU23-15166 | ECS | Posters virtual | BG1.7

Significance of biological forcing on the spatio-temporal variability of carbon dioxide fluxes over the Northern Indian Ocean 

Lekshmi Krishna, Rishikesh Bharti, and Chandan Mahanta

The oceanic uptake and release of carbon dioxide (CO2) play a critical role in global carbon cycle since oceans can act both as sink and source of CO2 which vary spatially and temporally. The ocean primary productivity has significant effects on the CO2 flux, as it consumes the dissolved CO2 at the sea surface for the photosynthetic carbon production, reducing the surface carbon content, while higher production rates at surface layers cause higher respiration rates in the subsurface layers, thereby increasing the sea water CO2 partial pressures (pCO2) in these layers. Northern Indian Ocean is found to be a perennial source of CO2 and also one of the most productive regions of Indian Ocean, however, while the western sub basin acts as an annual source, the eastern counterpart is a seasonal sink, especially during the monsoon and winter seasons. The major factors contributing to its high productivity is the summer and winter blooms caused by the wind-driven upwelling and winter cooling as well as convective mixing. The present study attempts to understand the relation between the CO2 fluxes and primary productivity in the western and eastern sub basins of the northern Indian Ocean. The study divides the Sea in to North, West, East and Central parts based on the productivity and analyses the spatial and temporal variation of the CO2 exchange between the sea and atmosphere in connection with the primary production. Satellite as well as climatological data were used to derive the monthly CO2 fluxes and ocean primary productivity. Both sub basins exhibited high rates of productivity during the monsoon and winter seasons; high monsoon and winter CO2 outfluxes were observed over the western sub basin in the northern waters towards the coast, while the eastern basin was found to have strong influxes in both the seasons over the northern waters. Towards the open ocean part, both fluxes and productivity showed decreasing trends in the western basin, whereas, the eastern sub basin showed an increasing trend of CO2 outflux over the open ocean waters in the south. Surface stratification and limited nutrient availability have resulted in the low productivity rates during the pre- and post-monsoon seasons in both basins, while the absence of the surface mixing resulting from the stratification along with photosynthetic consumption lowered the fluxes. The primary production was observed to have a significant influence over the western basin fluxes while the fluxes over the eastern basin were primarily affected by the physical forcing i.e., the thermohaline stratification.

How to cite: Krishna, L., Bharti, R., and Mahanta, C.: Significance of biological forcing on the spatio-temporal variability of carbon dioxide fluxes over the Northern Indian Ocean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15166, https://doi.org/10.5194/egusphere-egu23-15166, 2023.

EGU23-16001 | Orals | BG1.7

The land-to-ocean loops of the global carbon cycle: How much do we know about long-term trends and drivers of changes in CO2 fluxes ? 

Pierre Regnier, Laure Resplandy, Judith Rosentreter, Raymond Najjar, and Philippe Ciais

This contribution presents a new view of the global carbon cycle which accounts for the land-to-ocean transport of carbon through inland waters, estuaries, tidal wetlands and continental shelf waters—the ‘land-to-ocean aquatic continuum’ (LOAC). We highlight how biogeochemical and ecological processes from land-to-ocean have been perturbed by human interventions, including atmospheric composition change, climate change and land-use change. The extend to which these anthropogenic perturbations have altered regional and global CO2 budgets and trends along the LOAC are also presented and the knowledge gaps that are key to reduce uncertainties in future assessments of LOAC fluxes are identified. Finally, broader implications regarding the quantification of the terrestrial and open ocean sinks of anthropogenic carbon are briefly discussed 

How to cite: Regnier, P., Resplandy, L., Rosentreter, J., Najjar, R., and Ciais, P.: The land-to-ocean loops of the global carbon cycle: How much do we know about long-term trends and drivers of changes in CO2 fluxes ?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16001, https://doi.org/10.5194/egusphere-egu23-16001, 2023.

EGU23-16482 | Posters on site | BG1.7

Measurement of the isotopic signature of boreal wetland methane emissions 

Rebecca Fisher, Ceres Woolley Maisch, David Lowry, James France, Thomas Rockmann, Carina van der Veen, C. Mary R. Fowler, and Euan G. Nisbet

The use of δ2H as well as δ13C methane isotope measurements will help improve regional and global source apportionment and understanding of reasons for methane’s continued and accelerating growth. However more data on regional variability in isotopic signatures of the main sources is required as well as regular measurements of both isotopes in methane in background air.

Field campaigns across Canada in June 2022 and to northern Finland and Norway in August 2022 were carried out to collect air samples for methane δ13C and δ2H isotopic characterisation from boreal wetlands.

In Finland and Norway a road campaign with continuous measurements of methane mole fraction was carried out from Södankyla, Finland to Aidejavri, Norway, with a generally decreasing gradient in methane from south to north and this has been compared with land cover maps. Air samples for isotopic analysis were collected at Södankyla, Kaamanen and Lompolojänkkä fens in Finland and Aidejavri and Suossjavri degrading palsa mires in Norway. In Canada δ2H and δ13C isotopic signatures were determined in methane emitted by wetlands in northern Ontario including at Fraserdale, and northern Saskatchewan (East Trout Lake).

Overall the mean signatures of emissions from the boreal samples collected were -67‰ for δ13C and -320‰ for δ2H, but there was significant local variability when sampling air close to ground level. Aircraft campaigns would be a better way of identifying the integrated isotopic signature of regional wetland emissions (as demonstrated previously for δ13C signatures across northern European wetlands). Weekly sampling for methane δ13C and δ2H was started at Pallas Sammaltunturi in northern Finland in August 2022. These data will be used to identify the regional source signature of emissions.

How to cite: Fisher, R., Woolley Maisch, C., Lowry, D., France, J., Rockmann, T., van der Veen, C., Fowler, C. M. R., and Nisbet, E. G.: Measurement of the isotopic signature of boreal wetland methane emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16482, https://doi.org/10.5194/egusphere-egu23-16482, 2023.

EGU23-16842 | Orals | BG1.7

Magnitude, trends, and variability of the global ocean carbon sink from 1985-2018 

Timothy DeVries, Kana Yamamoto, and Rik Wanninkhof and the RECCAP2 Global Ocean Team

The RECCAP2 global ocean project provides an assessment of the mean, trends, and variability of the global ocean carbon sink for the period 1985-2018. The analysis is based on a comprehensive assessment of models and observation-based products, including global ocean biogeochemical models (GOBMs), pCO2 observation-based air-sea CO2 flux products, ocean data assimilation models, and DIC-observation based products. We find that the mean ocean CO2 sink from 1985-2018 is -1.7±0.3 PgC yr-1 as diagnosed by pCO2-observation based air-sea CO2 flux products. The dominant component of the global air-sea CO2 flux is the oceanic uptake of anthropogenic CO2, which is estimated at between -2.0 to -2.6 PgC yr-1 using a range of GOBMs, assimilation models and DIC-based products. The second largest component of the global air-sea CO2 flux is the outgassing of terrestrially-derived CO2, which is estimated at 0.65±0.3 PgC yr-1 but is not yet fully resolved by RECCAP2 models. The trend in the global air-sea CO2 flux from 1985-2018 ranges from -0.26 PgC yr-1 decade-1 in the GOBMs to -0.39 PgC yr-1 decade-1 in the pCO2 products. Over the 2001-2018 period, when the pCO2-based estimates benefit from improved data coverage, they predict a strengthening trend in the ocean carbon sink of -0.63 PgC yr-1 decade-1. This is driven primarily by the trend in anthropogenic carbon uptake of -0.41 PgC yr-1 decade-1, and secondarily by a climate-forced trend of -0.28 PgC yr-1 decade-1. This climate-forced strengthening of the ocean carbon sink since 2001 is not diagnosed in the GOBMs, and the reasons for this trend remain unclear. We find that the interannual to decadal variability of the global carbon sink is mainly driven by climate variability, with the climate-driven variability exceeding the CO2-forced variability by 2-3 times. GOBMs suggest that the climate-driven variability is about 4-8% of the global mean carbon sink, while the climate-driven variability is about 9-14% of the global mean flux in the observation-based pCO2 products. In all, the RECCAP2 analysis provides a state-of-the-art summary of our current knowledge of the ocean carbon sink, and the mechanisms driving its magnitude, trends, and variability over time.

How to cite: DeVries, T., Yamamoto, K., and Wanninkhof, R. and the RECCAP2 Global Ocean Team: Magnitude, trends, and variability of the global ocean carbon sink from 1985-2018, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16842, https://doi.org/10.5194/egusphere-egu23-16842, 2023.

EGU23-16920 | Orals | BG1.7

Greenhouse gas budget for South Asia region 

Atul Jain, Jatin Anand, Naveen Chandra, and Prabir Patra

Understanding climate change and possible solutions to recent increases in concentrations of major GHG concentrations dependent upon quantifying the emission inventory of these gases. The objective of this study, which is part of the Regional Carbon Cycle Assessment and Processes-2 (RECCAP2) project, is to estimate the country-specific GHGs budget (sources and sinks) for the South Asia (SA) region for the 2010s. The region comprises seven countries: Afghanistan, Bangladesh, Bhutan, India, Nepal, Pakistan, and Sri Lanka. Each country in the region is experiencing rapid changes due to the continuous development of agriculture, deforestation, reforestation, afforestation, and the increased demand for land for people to live in. In this study, we synthesize top-down (TD) and bottom-up (BU) model results and ground-based and other data sets to estimate the GHG emissions for carbon dioxide (CO2), methane (CH4), and nitrous oxide (N2O) due to anthropogenic and natural biospheric activities. Major contributing factors include net biome productivity, fossil fuel emissions, inland waters, and wetland and wet/dry soils. Our study shows that the SA region was the net source of atmospheric CO2 for the 2010s. BU estimates for CO2, CH4, and N2O emissions were 1974, 1047, and 715 Tg CO2eq, and TD estimates were 2010, 1247, and 799 Tg CO2 eq. The total GHG emission for the region based on BP and TD were 3736 and 4056 Tg CO2 eq. Among SA countries, India was the most significant contributor to the total GHG emission.

How to cite: Jain, A., Anand, J., Chandra, N., and Patra, P.: Greenhouse gas budget for South Asia region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16920, https://doi.org/10.5194/egusphere-egu23-16920, 2023.

EGU23-17328 | Orals | BG1.7

RECCAP2 – Southern Ocean carbon fluxes and storage 

Lavinia Patara, Judith Hauck, and Luke Gregor and the RECCAP2 Southern Ocean team

Cool temperatures, vigorous overturning circulation, and high biological productivity make the Southern Ocean a key region for the air-sea CO2 exchanges. It is also the main gateway for anthropogenic CO2 into the ocean owing to the upwelling of old water masses with low anthropogenic CO2 concentration, and the transport of the newly equilibrated surface waters into the ocean interior. Here we present results from the Southern Ocean chapter of RECCAP2, which is the Global Carbon Project’s second systematic study on Regional Carbon Cycle Assessment and Processes. We analyse Southern Ocean contemporary carbon fluxes and anthropogenic carbon accumulation in 1985-2018 from a wide range of global ocean biogeochemical models (GOBMs), surface ocean pCO2-based data products (pCO2-products), and data-assimilated models, with the aim of identifying patterns of regional and temporal variability, model limitations and future challenges. Our results highlight agreement of GOBMs and pCO2-products on the mean Southern Ocean contemporary CO2 uptake (0.75 ± 0.28 PgC yr-1 and 0.74 ± 0.07 PgC yr-1 respectively). Compared with RECCAP1 (where the database of model- and observation-based estimates was significantly smaller), the new estimates suggest a weaker sink, possibly due to better representation of winter outgassing. Strong discrepancies exist between GOBMs and pCO2-products in seasonality and trend estimates between 1985-2018. The pCO2-products show the presence of a stagnation in uptake through the 1990’s followed by a rapid increase in uptake, while GOBMs show consistent uptake throughout the 1985-2018 period. On a regional level, the subtropical seasonally stratified (STSS) biome has the largest air-sea CO2 flux with uptake of CO2 peaking in winter, whereas the ice (ICE) biome is characterised by a generally small magnitude of fluxes into and out of the ocean and a pronounced seasonal cycle with the largest ocean uptake of CO2 in summer. Connecting these two, the subpolar seasonally stratified (SPSS) biome has intermediate flux magnitude, with GOBMs showing spread in the strength of winter outgassing and difficulties in simulating the strongest CO2 uptake in summer. The biases in GOBMs originate mainly from the non-thermal component of air-sea CO2 flux, and in particular from the difficulty in simulating the competing effects of circulation and biology on carbon draw-down in summer. Our analysis reveals a distinct zonal asymmetry (secondary to the latitudinal gradient) between the Atlantic, Pacific and Indian sectors. The zonal asymmetry is observed in the mean uptake and amplitude of the seasonal cycle rather than the phasing of the seasonal cycle. GOBMs show a 20% spread and an overall underestimate of their simulated anthropogenic carbon accumulation, pointing to insufficient water mass formation and interior ventilation. These first results confirm the global relevance of the Southern Ocean carbon sink and highlight the strong regional and interannual variability of the Southern Ocean carbon uptake in connection to physical and biogeochemical processes. 

How to cite: Patara, L., Hauck, J., and Gregor, L. and the RECCAP2 Southern Ocean team: RECCAP2 – Southern Ocean carbon fluxes and storage, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17328, https://doi.org/10.5194/egusphere-egu23-17328, 2023.

EGU23-223 | Posters on site | AS3.8

Microbial aerosol characteristics and health implications in the highly arid environment 

Kashif Rasool, Bilal Sajjad, Khadeeja Abdul Jabbar, Shaimaa Elmallah, and Azhar Siddique

Investigations into the suspected airborne transmission of pathogens in healthcare environments have posed a challenge to researchers for more than a century. If carried by a favorable air flow, bioaerosol material may be distributed over large distances with potentially fatal results. So the objective of this study is to perform the characterization of culturable and non-culturable bacteria, and fungi, and identify health-significant and antibiotic-resistant microbes. The ambient bioaerosols samples were collected in the greater Doha area, Qatar, during the autumn, winter, and summer seasons. Bacterial and fungal concentration, size distribution, and diversity were investigated by culture studies coupled with biochemical assays and next-generation sequencing. A total of over 70 samples were collected and processed with the Coriolis micro–microbial air sampler in each season from 7 stations. There was a significant increase in the concentration of bacteria and fungus during and after the rain. These concentrations were much lower than those in most cities worldwide may be due to the arid climate feature. The average concentration of bacteria was higher than the fungus throughout the winter season. Identification of culturable bacteria was done by biochemical assays using API 20E kit and fungus identification was done by microscopic analysis. Over 484 microbial species were detected using 16SrRNA gene-based next-generation sequencing.  Biodiversity analysis shows that bacterial and fungal diversity was the same at all the stations regardless of the location which shows that the local factors don’t have much impact on the bacterial and fungal biodiversity. However, there was a difference in microbial diversity in the winter season as compared to the summer, spring, and transition seasons. A scan of health significant pathogens has been performed on the identified microbes’ data. Several health-significant bacterial and fungal species were identified in Qatar ambient air including staphylococci, legionellae, tuberculous and nontuberculous, bacterial spore formers Clostridium difficile and Bacillus anthracis, and fungi Aspergillus, Penicillium, and Cladosporium spp and Stachybotrys chartarum which are strongly associated with allergic respiratory disease, especially asthma. Despite emerging significant public health concerns of antibiotic resistance genes (ARGs) and antibiotic-resistant bacteria (ARB) in urban air, it has not received significant attention. On the other hand, current air pollution health studies rely heavily on PM mass concentration, without considering biological parameters such as ARGs or ARB. An identification of the antibiotic-resistant strains was carried out according to the WHO priority classification and several microbes including Acinetobacter baumannii (WHO Priority 1: CRITICAL), Enterococcus faecium, Staphylococcus aureus, Campylobacter coli and Streptococcus pneumonia  (Priority 2: HIGH) were found in the ambient air. 

How to cite: Rasool, K., Sajjad, B., Abdul Jabbar, K., Elmallah, S., and Siddique, A.: Microbial aerosol characteristics and health implications in the highly arid environment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-223, https://doi.org/10.5194/egusphere-egu23-223, 2023.

EGU23-414 | ECS | Posters on site | AS3.8

35-years of aerosols-PBAPs research in Brazil: the need to think outside the Amazonian box 

Mauricio Mantoani, Jorge Martins, Leila Martins, Federico Carotenuto, Tina Šantl-Temkiv, Cindy Morris, Fábio Rodrigues, and Fábio Gonçalves

Whilst there is a consensus that aerosol particles and primary biological aerosol particles (PBAPs) play an important role in regulating the global climate, with aerosols-PBAPs research increasing lately in Brazil, information summarizing the available knowledge is limited. Here, we present a systematic review of research published during the last 35-years on aerosols-PBAPs in Brazil. A total of 212 studies encompassing 474 cases met the selection criteria. The Amazon rainforest was the most studied biome represented by 72% of cases, followed by the Atlantic Forest with 18%. Studies focusing on the Amazon rainforest mostly studied climate-related issues and aerosol physics, with less than 5% examining the biological identity of aerosols, whereas outside the Amazon rainforest this number reached 16%. In addition, more than half of the cases within Amazon (55%) were held at seven sampling sites only, but conclusions were mainly extrapolated to the entire biome. On the other hand, research beyond Amazon has mostly addressed temporal and biological characterization of PBAPs, and not only is it scattered, but also scarce. Regarding sampling effort, most cases (72%) have had less than 100 days of sampling, and 60% of them spanned less than half a year of study, confining research to one or two seasons at the most. Consequently, while research from different countries that conduce their studies within Brazil and scientific fields are focusing on the same area, inconsistences are slowing the progress of this research topic. We argue that scientists from different fields of research (e.g., biologists, physicists) and countries should work together to produce more detailed and complete assessments of aerosols-PBAPs in the country as a whole, particularly on regards to their biological identity, given their importance to global climate regulation.

How to cite: Mantoani, M., Martins, J., Martins, L., Carotenuto, F., Šantl-Temkiv, T., Morris, C., Rodrigues, F., and Gonçalves, F.: 35-years of aerosols-PBAPs research in Brazil: the need to think outside the Amazonian box, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-414, https://doi.org/10.5194/egusphere-egu23-414, 2023.

Pollen allergies affect a significant proportion of the global population, and this is expected to worsen in years to come. There is demand for the development of automated pollen monitoring systems to progress from conventional manual sampling techniques. Low-cost Optical Particle Counters (OPCs) are conventionally used for measuring particulate matter and have attractive advantages of real-time high time resolution data and affordable costs. Our study asks whether low-cost OPC sensors be used for meaningful monitoring airborne pollen and utilises data from the EUMETNET Autopollen ADOPT – COST Action Intercomparison Campaign (2021) in Munich, Germany.

We employ a variety of methods, including supervised machine learning techniques, to construct pollen proxies from hourly-average OPC data and evaluate their performance. The most successful methods are supervised machine learning Neural Network (NN) and Random Forest (RF) methods, trained from pollen concentrations collected from a Hirst-type sampler. These perform significantly better than using a simple particle size-filtered proxy or a Positive Matrix Factorisation (PMF) source apportionment pollen proxy. We developed a collection of models - varying by model type, input features (including particle size and meteorological data) and target variable (i.e. total pollen vs selected pollen taxa) - and evaluated their suitability for constructing a pollen proxy. The results show that such models can construct useful information on pollen from OPC particle size data with Spearman correlation coefficients up to 0.85 and coefficients of determination up to 0.67. Model-constructed proxies demonstrated an ability to distinguish high pollen events with promising results (F1 Scores up to 0.83) and to follow monthly and diurnal trends in pollen. We discuss the suitability of OPCs for monitoring pollen and offer advice for future progress. We demonstrate an attractive alternative for automated pollen monitoring that could provide valuable and timely information to the benefit of pollen allergy sufferers.

How to cite: Mills, S., MacKenzie, R., and Pope, F.: Constructing a pollen proxy from low-cost Optical Particle Counter (OPC) data processed with Neural Networks and Random Forests, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-433, https://doi.org/10.5194/egusphere-egu23-433, 2023.

EGU23-1123 | ECS | Posters on site | AS3.8

Toward a molecular level understanding of heterogeneous processes at atmospheric aerosol surfaces: ozonolysis of maleic acid droplets 

Rawan Abouhaidar, Denis Duflot, and Céline Toubin

Dicarboxylic acids are an essential component of tropospheric aerosols emitted directly or formed in chemical processes. The physiochemical properties and heterogeneous oxidation of aerosol particles containing maleic acid (MA) have been investigated using a mixed quantum and classical approach. The multiphase reactions of primary ozonide formation between the gas phase, the particle interface, and its bulk strongly influence the reaction mechanism and rate coefficients. Based on snapshots issued taken from molecular dynamics simulations, the mechanism of MA + O3 reaction is investigated in three different environments using ab initio method and density functional theory. The interfacial water molecules enhance the initial reaction step of MA + O3, with a larger rate constant at the air-water interface than in the gas phase. By assuming the Langmuir-Hinshelwood behavior and comparing it with the bulk, the ozonolysis of maleic acid mainly occurs in the bulk, and O3 diffusion in the bulk may be the limiting process.

How to cite: Abouhaidar, R., Duflot, D., and Toubin, C.: Toward a molecular level understanding of heterogeneous processes at atmospheric aerosol surfaces: ozonolysis of maleic acid droplets, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1123, https://doi.org/10.5194/egusphere-egu23-1123, 2023.

EGU23-1734 | Orals | AS3.8

Bacterial viability and air quality: experimental approach and results at the atmospheric simulation chamber ChAMBRe. 

Elena Gatta, Virginia Vernocchi, Marco Brunoldi, Dario Massabò, Franco Parodi, and Paolo Prati

Bio-aerosols consist of airborne particles such as pollens, fungi, bacteria, viruses and debris from biological matter, such as metabolites and toxins, that are present ubiquitously in the environment. In last decades, the interest in bioaerosols has increased rapidly to broaden the pool of knowledge on their identification, quantification, distribution, but also to understand how bioaerosols impact human health in both indoor and outdoor settings. Experiments conducted inside confined artificial environments, such as the Atmospheric Simulations Chambers (ASCs), where atmospheric conditions and composition are controlled, can provide valuable information on bio-aerosol viability, dispersion, and impact. At ChAMBRe (Chamber for Aerosol Modelling and Bio-aerosol Research), a 2.3 m3 stainless steel ASC, managed by INFN at the Physics Department of the University of Genoa, Italy, the research on bioaerosol is focused on the investigation of the airborne bacteria behavior in different atmospheric conditions (Massabò et al., AMT, 2018). Our experiments were performed with two types of bacteria, Bacillus Subtilis and Escherichia Coli evolutionarily divergent model organisms, Gram-negative and Gram-positive respectively, to compare cellular viability by varying of the atmospheric conditions in the simulation chambre. A great effort has been put in the assessment of an experimental protocol which includes bacteria cultivation, injection in the chamber of viable cells, exposure to peculiar environmental conditions and final verification of the loss/gain in viability. With first experiments, bacteria were exposed to high concentration of characterized soot particles (Black carbon ~ 600 μg m-3) and NOx exhausts, both produced by propane combustion (Vernocchi et al., 2021). The effects of NOx only were also separately investigated, in another set of experiments, in which different concentration of NOx were tested. Evidence of an impact of NOx concentration on the viability of the Gram-negative Bacillus Subtilis were observed and will be fully reported at the conference.

 

 

How to cite: Gatta, E., Vernocchi, V., Brunoldi, M., Massabò, D., Parodi, F., and Prati, P.: Bacterial viability and air quality: experimental approach and results at the atmospheric simulation chamber ChAMBRe., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1734, https://doi.org/10.5194/egusphere-egu23-1734, 2023.

EGU23-4481 | ECS | Posters on site | AS3.8

Theoretical study of the adsorption of Methyl Iodide on model sea-salt surfaces 

Céline Toubin, Maxime Infuso, Florent Louis, Sonia Taamalli, and Denis Duflot

Oceans, through algae and phytoplankton activities, are the main source of iodine, including monohalogenated organic compounds as CH3I [1].  There is missing knowledge about interactions between iodinated compounds and aerosols in the troposphere. In this context, this work investigates the adsorption of gaseous iodomethane (CH3I) on model sea-salt aerosols at various humidities. The water coverage tends to stabilize CH3I at the salt surface. The lifetime of CH3I in the atmosphere (in gas phase or adsorbed on aerosols) may be altered by its reaction with gas phase radicals. The reaction of CH3I with OH is thus investigated both in gas phase and in presence of water by means of quantum mechanical calculations.

 

References:

[1] Saiz-Lopez et al, Chem. Rev. 2012, 112, 1773–1804.

 

Acknowledgments:

I-SITE ULNE OVERSEE project (contract ANR-16-IDEX-004)

The CaPPA project (Chemical and Physical Properties of the Atmosphere) is funded by the French National Research Agency (ANR) through the PIA (Programme d’Investissement d’Avenir) under contract « ANR-11-LABX-0005-01 » and by the Regional Council « Hauts-de-France » and the « European Funds for Regional Economic Development » (FEDER)

How to cite: Toubin, C., Infuso, M., Louis, F., Taamalli, S., and Duflot, D.: Theoretical study of the adsorption of Methyl Iodide on model sea-salt surfaces, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4481, https://doi.org/10.5194/egusphere-egu23-4481, 2023.

Atmospheric loading of black carbon aerosols influences air quality and visibility, and their mixing state and aerosol chemistry were sensitive to both emission scenarios and regional transport. In this study, the aerodynamic size-resolved mixing state of refractory black carbon aerosols (rBC) and elemental composition were investigated using a novel tandem system consisting of an aerodynamic aerosol classifier (AAC), a single particle soot photometer (SP2), and single-particle-aerosol mass spectrometry (SPA-MS) during the XXIV Olympic Winter Games (OWG) at an urban site in Beijing. We found that rBC-containing particles with an aerodynamic diameter (Dae) of 300 nm were characterized by a rBC core with a count median diameter (CMD) of 108±4 nm that typically have regular morphology ( , higher relative coating thickness (RCT: mean ~1.8), and strong light absorption enhancement (Eabs: mean ~1.4). The rBC-containing particles with Dae = 200 nm normally had irregular shapes and weak Eabs. Classification based on air mass clustering and air pollution level revealed that the coating thickness of rBC particles only exhibited unimodal patterns under clean air conditions but bimodal distributions under heavy pollution conditions, implying multiple origins of rBC particles, even during OWG periods. Furthermore, the chemical compositions of the rBC coating quantitatively determined by SPA-MS were used to estimate the possible origins of rBC with Dae = 300 nm. Our results showed that rBC particles were primarily mixed with organics, nitrate, and sulfate during the XXIV OWG period. The organic components have a limited role in increasing rBC coatings under polluted conditions, while the alkali metal ions (K and Na) associated with traffic emissions and the secondary inorganic species favor the formation of thick coatings. Higher RH makes limited contributions to rBC mixed with sulfate and organics only (BCOC*_S) and pure BC. The relatively fresh BC could directly mix with organics and sulfate at low RH levels while evolving to mix with nitrate at high RH conditions. In addition to high concentrations of locally emitted precursors and high RH that tend to form thick coatings of nitrate-related rBC aerosols, secondary transport from the west and southwest also contributes to rBC aerosols mixed with nitrate with relatively thick coatings.

How to cite: Zhang, Y. and Pan, X.: Size–resolved mixing state of ambient refractory black carbon aerosols in Beijing during the XXIV Olympic Winter Games, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4752, https://doi.org/10.5194/egusphere-egu23-4752, 2023.

EGU23-5151 | Orals | AS3.8

Clouds boost microbial activity in the atmosphere 

Pierre Amato, Raphaëlle Péguilhan, Florent Rossi, Muriel Joly, Jean-Luc Baray, Laurent Deguillaume, and François Enault

The atmosphere transports biological material including living microorganisms. Whereas their survival is impaired during atmospheric transport due to desiccation and UV notably, certain organisms maintain metabolic activity and interact with physicochemical processes. This has especially been studied in clouds for its potential impacts on chemical processes such as the degradation of organic compounds and the oxidant capacity. However, it is still unknown whether the functioning of airborne microorganisms in clouds is specific and differs from the rest of the atmosphere; this question was investigated here. We developed a metagenomic/metratranscriptomic approach to investigate the in-situ functioning of airborne microbial communities and decipher its environmental drivers, notably the impacts of the presence of condensed water in clouds. Aerosol and clouds samples were collected from puy de Dôme mountain summit (1465 m asl, France) using series of high flow rate impingers, into a fixative agent to preserve nucleic acids (DNA and RNA), i.e. the identity and instantaneous functional signature of organisms. A bioinformatics pipeline was developed specifically to analyze these unprecedented and complex datasets. Comparative analyses revealed that clouds are genuine oases for living microorganisms in the atmosphere: although their microbial biodiversity is similar as that during clear atmospheric situations, droplets provide shelters especially against oxidative stress, which is found to characterize the metabolic functioning of airborne microbes in dry aerosols. The presence of condensed water boosts many biological functions, and functions related with starvation toward carbon and nitrogen notably indicate increased biological needs and evidence the existence of numerous interactions with chemical processes and atmospheric biogeochemical cycles. Regarding microbial ecology, the reactivation of metabolic functions in airborne microorganisms transiting through clouds could facilitate their settlement in their new environment.

How to cite: Amato, P., Péguilhan, R., Rossi, F., Joly, M., Baray, J.-L., Deguillaume, L., and Enault, F.: Clouds boost microbial activity in the atmosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5151, https://doi.org/10.5194/egusphere-egu23-5151, 2023.

EGU23-6193 | Posters on site | AS3.8

Collision-sticking rates of acid-base clusters in the gas phase determined from atomistic simulation and a novel analytical interacting hard-sphere model 

Bernhard Reischl, Huan Yang, Ivo Neefjes, Valtteri Tikkanen, Jakub Kubečka, Theo Kurtén, and Hanna Vehkamäki

Kinetics of collision-sticking processes between vapor molecules and clusters of low volatile compounds govern the initial steps of atmospheric new particle formation. Conventional non-interacting hard-sphere models underestimate the collision rate by neglecting long-range attractive forces, and the commonly adopted assumption that every collision leads to the formation of a stable cluster (unit mass accommodation coefficient) is questionable for small clusters, especially at elevated temperatures. Here, we present a generally applicable analytical interacting hard-sphere model for evaluating collision rates between molecules and clusters, accounting for long-range attractive forces. In the model, the collision cross section is calculated based on an effective molecule-cluster potential, derived using Hamaker’s approach. Applied to collisions of sulfuric acid or dimethylamine with neutral bisulphate-dimethylammonium clusters composed of 1-32 dimers, our new model predicts collision rates 2-3 times higher than the non-interacting model for small clusters, while decaying asymptotically to the non-interacting limit as cluster size increases, in excellent agreement with a collision rate theory-atomistic molecular dynamics simulation approach. Additionally, we calculated sticking rates and mass accommodation coefficients (MAC) using atomistic molecular dynamics collision simulations. For sulfuric acid, unit MAC is observed for collisions with all cluster sizes at temperatures between 200 K and 400 K. For dimethylamine, we find that MACs decrease with increasing temperature and decreasing cluster size. At low temperatures, the unit MAC assumption is generally valid, but at elevated temperatures MACs can drop below 0.2 for small clusters.

How to cite: Reischl, B., Yang, H., Neefjes, I., Tikkanen, V., Kubečka, J., Kurtén, T., and Vehkamäki, H.: Collision-sticking rates of acid-base clusters in the gas phase determined from atomistic simulation and a novel analytical interacting hard-sphere model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6193, https://doi.org/10.5194/egusphere-egu23-6193, 2023.

EGU23-6196 | Posters on site | AS3.8

Exploring metabolic acclimation of the cloud microflora to contrasting summer day and winter night conditions using metatranscriptomics and fluxomics approaches 

Muriel Joly, Domitille Jarrige, Jonathan Vyscocil, Florent Rossi, Céline Judon, Françoise Bringel, Emilie E.L. Muller, Stéphane Vuilleumier, Thierry Nadalig, Jean-Charles Portais, Lindsay Peyriga, Floriant Bellvert, Hanna Kulyk, Angelica Bianco, Laurent Deguillaume, Anne-Marie Delort, and Pierre Amato

Metabolically active microorganisms are increasingly acknowledged as actors of cloud chemical reactivity able to use organic compounds present in clouds (e.g. organic acids, aldhedydes) for their metabolism (Vaïtilingom et al., 2013). Uncharacterized biological activity may play a major role especially during the night, while during daytime the abiotic degradation of organic compounds would be driven and dominated by hydroxyl radical (•OH) chemistry (Vaïtilingom et al., 2011). To better understand and predict the impact of biological activity on atmospheric chemical reactivity, the metabolic pathways of the whole cloud microbiome and their modulations by environmental conditions (temperature, light, oxidants) must now be assessed.

The METACLOUD project addresses metabolic acclimatation of cloud microorganisms under two contrasted situations simulating a summer day (17°C, with solar light and presence of hydrogen peroxide) and a winter night (at 5°C, in the dark and without hydrogen peroxide). A focus is made on formaldehyde assimilations as this compound is a key intermediate both in cloud radical chemistry and in many C1 biological pathway, using fluxomics (LC-HRMS and IC-HRMS) on 13C-formaldehyde supplemented samples. Experiments were conducted in specially designed photobioreactors, either on (1) freshly sampled cloud water from the research station at the top of the puy de Dôme station (1465m asl, PUY, France) including naturally present microorganisms, or (2) an artificial consortium assembled from microbial strains isolated from cloud water sampled at PUY and resuspended in an artificial medium mimicking the composition of marine cloud water (major inorganic and organic compounds).

Metatranscriptomes and metabolomes indicate metabolic acclimations of the cloud microbiome to model summer/winter conditions, especially linked with fatty acid regulation and central metabolism (e.g. citrate cycle). First results with 13C-formaldehyde showed carbon incorporation from this molecule into several classes of metabolites (e.g. nucleotides, amino acids, central metabolites), illustrating the complex biological fate of this compound in the environment. The data will be used to implement biological activity on cloud chemistry models.

 

Vaïtilingom M. et al. (2011) Atmospheric chemistry of carboxylic acids: microbial implication versus photochemistry. Atmos. Chem. Phys. 11, 8721-8733. doi: 10.5194/acp-11-8721-2011.

Vaïtilingom M. et al. (2013) Potential impact of microbial activity on the oxidant capacity and organic carbon budget in clouds. Proc. Nat. Acad. Sci. USA 110, 559-564. doi: 10.1073/pnas.1205743110.

How to cite: Joly, M., Jarrige, D., Vyscocil, J., Rossi, F., Judon, C., Bringel, F., Muller, E. E. L., Vuilleumier, S., Nadalig, T., Portais, J.-C., Peyriga, L., Bellvert, F., Kulyk, H., Bianco, A., Deguillaume, L., Delort, A.-M., and Amato, P.: Exploring metabolic acclimation of the cloud microflora to contrasting summer day and winter night conditions using metatranscriptomics and fluxomics approaches, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6196, https://doi.org/10.5194/egusphere-egu23-6196, 2023.

EGU23-6582 | ECS | Posters on site | AS3.8

Biodegradation of formic and acetic acids is a significant atmospheric sink 

Leslie Nuñez Lopez, Pierre Amato, and Barbara Ervens

Bioaerosols include bacteria that comprise about <1% of the total aerosol number concentration in the atmosphere. In current atmospheric models, bacteria are considered as not being metabolically active during their atmospheric residence time. This assumption is contradicting laboratory studies that have revealed that small organic compounds, such as formic and acetic acids, can be efficiently biodegraded by bacteria found in the atmosphere.

Formic and acetic acids are ubiquitous in the atmosphere, constituting main organic acids in the gas and aqueous phases. Their sources are usually dominated by direct emissions from biomass burning, fossil fuel combustion, vegetation, and soil, besides secondary production from gas and aqueous phase photochemistry. Their sinks are usually considered to be limited to wet and dry deposition, and oxidation by radicals (OH, NO3).

To explore the potential role of biodegradation as an additional sink of formic and acetic acids, we implemented their biodegradation in cloud droplets in a detailed atmospheric multiphase chemistry model. As opposed to aqueous phase chemical reactions that occur in all droplets, biodegradation only occurs in a small fraction of droplets (~0.1%) taking into account the small number concentration of bacteria cells in the atmosphere.

We perform model sensitivity studies to identify atmospheric conditions (e.g., pH, cloud droplet size, processing time), under which biodegradation represents a significant sink of the two acids. Our model results show that the concentration of formic and acetic acids may be overestimated by up to 5% (~20 ppt) and 3% (~8 ppt), respectively if biodegradation is not included. The net formation or loss rates are predicted to be reduced by up to 20%. These contributions exceed by far the number concentration of bacteria-containing droplets, which implies that the acids evaporate from bacteria-free droplets and are efficiently taken up and biodegraded in the small portion of droplets. We show that the assumption of an average biodegradation rate in all droplets leads to an overestimate of the biodegradation rate, particularly at pH > 5. Generally, the highest importance of biodegradation is identified for large droplets and at pH ~5, which may be considered representative for remote locations. The results are highly sensitive to the pH value, as it not only increases the partitioning of the acids to the aqueous phase (effective Henry’s law constant) but also the rate constants of the OH reactions which compete with the biodegradation as acid sinks.

We conclude that current atmospheric chemistry models may be incomplete to assess the loss of organics in the atmospheric multiphase system as biodegradation might be a significant loss of formic and acetic acids and possibly of related organics.

How to cite: Nuñez Lopez, L., Amato, P., and Ervens, B.: Biodegradation of formic and acetic acids is a significant atmospheric sink, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6582, https://doi.org/10.5194/egusphere-egu23-6582, 2023.

EGU23-7108 | Posters on site | AS3.8

Computer simulation investigation of the adsorption of acetamide under atmospheric and interstellar conditions 

Pal Jedlovszky, Mirjam Balbisi, Reka Horvath, and Milan Szori

Acetamide is not only released into the atmosphere from natural sources, but its large-scale industrial use also results in its atmospheric emission. The main atmospheric sink of acetamide is its oxidation, however, other atmospheric fates are also plausible. In wet deposition, acetamide can be captured by ice grains through adsorption. Thus, we investigated the adsorption of acetamide at the surface of crystalline (Ih) and low density amorphous (LDA) ices by performing a set of grand canonical Monte Carlo simulations at the tropospheric temperature of 200 K. Besides calculating the adsorption isotherms, we also characterised the energetics of the adsorption and the orientational preferences of the first layer molecules. We demonstrated that at low enough surface concentrations, the adsorbed acetamide molecules prefer to lay parallel with the ice surface. With increasing surface coverage, acetamide molecules preferentially stay perpendicular to the surface, pointing by the CH3 group straight away from the ice phase, typically forming 2 H-bonds with each other and 2 with the surface waters. Finally, after the appearance of outer layer acetamide molecules, first layer molecules prefer to form 3 H-bonds with their acetamide neighbours and only 1 with the surface waters.

As acetamide has been detected in a relatively large amount in space as well, we extended our study by performing grand canonical Monte Carlo simulations at 50 and 100 K on LDA ice, which are more characteristic of typical domains of the interstellar medium. We found that the relative importance of the acetamide–acetamide H-bonds with respect to the acetamide–water ones increases with decreasing temperature. As a result of it, the saturated monolayer, which is stable in a broad range of chemical potentials at 200 K, shrinks with decreasing temperature, and, eventually, vanishes at 50 K, while multilayer adsorption becomes more and more pronounced at the lower temperatures. Furthermore, our results suggest that non-negligible acetamide adsorption might occur on LDA surfaces at low enough temperature (i.e., 50 K and below), thus, the interstellar formation of peptide chains through acetamide molecules might well be a plausible process in the cold domains of the interstellar medium; however, it is rather unlikely in the higher temperature domains.

How to cite: Jedlovszky, P., Balbisi, M., Horvath, R., and Szori, M.: Computer simulation investigation of the adsorption of acetamide under atmospheric and interstellar conditions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7108, https://doi.org/10.5194/egusphere-egu23-7108, 2023.

EGU23-7123 | Posters on site | AS3.8

Sugar like compounds in PM2.5 at three rural background sites in Central Europe 

Jaroslav Schwarz, Radek Lhotka, Petra Pokorná, Petr Vodička, Naděžda Zíková, Jakub Ondráček, Shubi Arora, Laurent Poulain, Hartmut Herrmann, and Vladimír Ždímal

Sugar like substances are usually small but important part of organic aerosol being often tracers for individual aerosol sources. Twelve hours samples (day and night) collected during winter and summer campaigns at three Central European rural background sites were utilized to characterize PM2.5 aerosol using complex set of analytical methods. Here we report concentrations of sugars, sugar like alcohols and sugar anhydrides.

PM2.5 samplings were performed during February–March and July–August 2021 at three sites, National Atmospheric Observatory Košetice – CZ (NAOK, N 49°35′, E 15°05′; 534 m a.s.l.), Frýdlant – CZ (N 50°94′, E 15°07′; 366 m a.s.l.) and Melpitz –DE (N 51°32', E 12°56'; 86 m a.s.l.). Each site was equipped with high volume Digitel sampler using sampling flow rate 500 l/min. Cut parts of the filter were extracted with ultrapure water and the extracts were analysed using HPAE-PAD analysis and Thermo Scientific 5000+ system for sugar-like substances using a method based on Iinuma et al. 2009.

The concentrations of sugar like substances were dominated by levoglucosan in winter at all sites, with 0.32±0.29 µg/m3 at Košetice, 0.21±0.13 µg/m3 at Frýdlant, and 0.15±0.13 µg/m3 at Melpitz. Mannosan/levoglucosan median ratio was the highest at Košetice (0.23) and lowest at Frýdlant (0.18).

The summer concentrations of sugar like substances were more evenly distributed in several major substances with concentrations one order lower in comparison to concentrations of levoglucosan in winter. The concentrations of individual sugars, sugar alcohols and sugar anhydrides were relatively evenly distributed, but some differences between the sites were found. The average sums of sugars were the highest of all categories at all sites, but while the sugar alcohols were the second highest in Melpitz, the content of sugar anhydrides was at the second place at Frýdlant and Košetice in summer.

 

Acknowledgements:

This work was supported within a German-Czech cooperation in the TRACE project funded by the GACR under grant 20-08304J and by DFG under grant 431895563, also by the MEYS of the Czech Republic under grants ACTRIS-CZ LM2018122 and ACTRIS-CZ RI (CZ.02.1 .01 / 0.0 / 0.0 / 16_013 / 0001315), and European Union's Horizon 2020 research and innovation program ACTRIS IMP (871115).

 

References:

  • Iinuma, G. Engling, H. Puxbaum, H. Herrmann, A highly resolved anion-exchange chromatographic method for determination of saccharidic tracers for biomass combustion and primary bio-particles in atmospheric aerosol, Atmos. Environ., 43 (2009), pp. 1367-1371, 10.1016/j.atmosenv.2008.11.020

How to cite: Schwarz, J., Lhotka, R., Pokorná, P., Vodička, P., Zíková, N., Ondráček, J., Arora, S., Poulain, L., Herrmann, H., and Ždímal, V.: Sugar like compounds in PM2.5 at three rural background sites in Central Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7123, https://doi.org/10.5194/egusphere-egu23-7123, 2023.

EGU23-7584 | ECS | Orals | AS3.8

Diurnal and seasonal patterns of fluorescent bioaerosol and meteorological parameters in Bucharest, Romania 

Rosianu Ana-Maria, Stefan Sabina, Marmureanu Luminita, and Iorga Gabriela

Pollen concentrations present in the atmosphere can raise serious human health problems, which is why they require studies with a higher precision and temporal resolution. The weather condition can produce direct changes in the growth and development of plants leading to changes in pollen concentrations or even changes in the pollen seasonal characteristics. This research was carried out on fluorescent bioaerosol concentrations obtained with the particle counter Rapid-E instrument that allows automatic collection. Fluorescent bioaerosol data were collected as hourly counts in the period 2018-2021 for the Bucharest-Magurele and were divided into three categories depending on the size of the particle diameter, namely small fluorescent particles (SF, particles less than 10 micrometers), large fluorescent particles (BF, greater than 10 micrometers) and, respectively, the total of fluorescent particles TF=SF+BF. In this research, diurnal variations of fluorescent bioaerosol concentrations as well as of temperature, relative humidity, wind speed and the height of the planetary boundary layer were studied. Hourly meteorological parameters were extracted from ECMWF global reanalysis ERA5 dataset from the Climate Change Service Copernicus platform. The multi-monthly averages and seasonal variations were also emphasized and local specificities were underlined. Statistical analyzes and graphical representations were performed using R software with the Openair package.

 

Key words: bioaerosol, pollen, allergens, meteorology, aerobiology, East Europe

How to cite: Ana-Maria, R., Sabina, S., Luminita, M., and Gabriela, I.: Diurnal and seasonal patterns of fluorescent bioaerosol and meteorological parameters in Bucharest, Romania, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7584, https://doi.org/10.5194/egusphere-egu23-7584, 2023.

EGU23-8213 | ECS | Posters on site | AS3.8

Surface propensity of atmospheric iodine oxides: AIMD and LJ-XPS investigation 

Antoine Roose, Lucia Iezzi, Anthony Boucly, Huanyu Yang, Matthias Krack, Markus Ammann, and Luca Artiglia

Iodine chemistry is implicated in atmospheric chemistry and can lead to the formation of several oxides such as HOI, I2, IO, OIO, and finally I2O5 or HIO3, which may nucleate as nanoparticles relevant for cloud formation in remote environments (Saiz-Lopez et al., 2012, Finkenzeller et al., 2022). These oxides can be formed through reaction with oxidants or other halogen compounds in the gas phase or the particle phase. Most of the iodide oxidation processes have been suggested to be enhanced at interfaces, similar to those involving other halogen species, either due to the surface propensity of intermediates (Artiglia et al., 2017) or the iodine species itself (Moreno and Beaza-Romero, 2019). However, no data are available about the surface concentration of iodine species other than iodide. After two decades of research into the surface propensity of iodide and bromide, the picture emerges that their surface propensity is not as extreme as initially thought (Jungwirth and Tobias, 2002; Ghosal et al., 2005; Olivieri et al., 2018).

Liquid jet X-ray photoelectron spectroscopy (XPS) experiments have been carried out at the SIM beamline at the Swiss Light Source. Acquisition of kinetic energy dependent (thus at different probing depth) I3d, I4d core level and valence level spectra has been done for iodide, iodate and iodic acid. This allows to retrieve the surface propensity of these iodine species at the aqueous solution – air interface. HIO3, HOI and iodide surface propensity has also been investigated by Ab Initio Molecular Dynamics computation at the revPBE-D3/DZVP-SR level using CP2K software (Khüne et al., 2020).

  • Artiglia et al., Nat. Commun., 8, 700 (2017).
  • Finkenzeller et al., Nat. Chem. (2022).
  • Ghosal et al., Science, 307, 563 (2005).
  • Jungwirth and D. Tobias, J. Phys. Chem. B, 106, 25, 6361 (2002).
  • D. Kühne et al., J. Chem. Phys., 152, 194103 (2020).
  • Moreno and M. T. Baeza-Romero, 21, 19835 (2019).
  • Olivieri et al., J. Phys, Chem. B, 122, 2, 910 (2018).
  • Saiz-Lopez et al., Chem. Rev., 112, 1773 (2012).

 

How to cite: Roose, A., Iezzi, L., Boucly, A., Yang, H., Krack, M., Ammann, M., and Artiglia, L.: Surface propensity of atmospheric iodine oxides: AIMD and LJ-XPS investigation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8213, https://doi.org/10.5194/egusphere-egu23-8213, 2023.

EGU23-9736 | ECS | Orals | AS3.8

Adsorption and Deposition Freezing on Silver Iodide Surface: A Computer Simulation Study 

Golnaz Roudsari, Mária Lbadaoui-Darvas, Athanasios Nenes, and Ari Laaksonen

Pure liquid water can remain liquid at temperatures as low as -38 oC in the atmosphere. However, ice nucleation can occur at temperatures even higher than -3 oC in the presence atmospheric particles. Cloud ice usually forms as a result of heterogeneous ice nucleation (HIN), where insoluble airborne particles catalyze the freezing process. The current models of HIN are based either on empirical fits to laboratory or field data, or on classical nucleation theory (CNT), which assumes that ice formation occurs in a single step. However, the results of these models can deviate significantly from experimental observations. Molecular simulations can provide an atomistic-level insight into the study of the mechanisms of HIN on different ice nucleating particles. 

In this study, a combination of molecular dynamics and grand canonical Monte Carlo simulations is used to study the deposition freezing on silver iodide surfaces at various saturation vapor pressures. Silver iodide (AgI) is known for excellent ice nucleating properties and has long been used in rain-seeding applications. The surfaces of ice nucleating particles first adsorb water molecules, forming liquid droplets that fluctuate stochastically until they freeze. 

Our results reveal atomistic level mechanisms of deposition freezing and further characterize the effects of ice nucleating particles on HIN phenomenon. Based on the simulation trajectories, we found that water molecules adsorb dropletwise on the AgI surfaces in hexagonal arrangements. We also observed simultaneous adsorption of the first and second layers of water molecules and a slightly delayed adsorption of the third layer. Afterward, the multilayer droplets merge into bigger droplets. In addition, our simulation results suggest that ice nucleation initiates after the adsorption of at least four layers of water.        

Acknowledgment:

This work was supported by the Academy of Finland Flagship ACCC (grant no. 337552) and
MEDICEN project (grant no. 345125).

How to cite: Roudsari, G., Lbadaoui-Darvas, M., Nenes, A., and Laaksonen, A.: Adsorption and Deposition Freezing on Silver Iodide Surface: A Computer Simulation Study, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9736, https://doi.org/10.5194/egusphere-egu23-9736, 2023.

EGU23-9950 | Orals | AS3.8

Long-range transport of airborne microorganisms by Asian dust events: Bioaerosols relating to human health 

Teruya Maki, Itaru Sano, Shigeru Shimamoto, Hiroki Miyata, Yua Fujiwara, Koichi Watanabe, Ysunori Kurosaki, Kazuma Aoki, Atsushi Matsuki, Jun Noda, Zhongwei Huang, Bin Chen, and Yasunobu Iwasaka

The bioaerosols relating to human health are possibly transported by the westerly wind traveling at high altitudes over East Asia. However, the long-range transport of bioaerosols has not been demonstrated by analyzing the microbial communities in aerosols such as desert mineral particles and anthropogenic pollutants transported by the westerly wind. Here, airborne microbial compositions were investigated in high-altitude aerosols collected during the Asian dust events in Japan island. This was further compared to the ground-level aerosols collected sequentially at more than seven sampling sites distributed from Asian dust source region to downwind areas in East Asia (Asian desert; Tsogt-Ovoo, Asian continental cities; Erenhot, Beijing, Yongin, Japanese island cities; Yonago, Suzu, Noto Peninsula). The cell concentrations and taxonomic diversities of airborne bacteria decreased from the Asian continental area to the Japan island area. Terrestrial bacterial populations belonging to Firmicutes and Actinobacteria showed higher relative abundance at downwind areas during Asian-dust events. Additionally, some pathogenic microorganisms such as NTM-PD bacteria (Mycobacterium species) increased in relative abundance in correspondence to the increase of black carbon concentrations. In contrast, the food fermenting bacteria, such as Natto bacteria (Bacillus subtilis), were detected and isolated from the high-altitude aerosols and actually made Natto. Presumably, Asian dusts carry potential pathogen and fermenting microorganisms, thereby impacting upon the human societies.

How to cite: Maki, T., Sano, I., Shimamoto, S., Miyata, H., Fujiwara, Y., Watanabe, K., Kurosaki, Y., Aoki, K., Matsuki, A., Noda, J., Huang, Z., Chen, B., and Iwasaka, Y.: Long-range transport of airborne microorganisms by Asian dust events: Bioaerosols relating to human health, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9950, https://doi.org/10.5194/egusphere-egu23-9950, 2023.

EGU23-10268 | Orals | AS3.8 | Highlight

Enhanced Light Absorption and Radiative Forcing by Black Carbon Agglomerates 

Georgios Kelesidis, David Neubauer, Liang-Shih Fan, Ulrike Lohmann, and Sotiris Pratsinis

The climate models of the Intergovernmental Panel on Climate Change list black carbon (BC) as an important contributor to global warming based on its radiative forcing (RF) impact. Examining closely these models, it becomes apparent that they might underpredict significantly the direct RF for BC, largely due to their assumed spherical BC morphology. Specifically, the light absorption and direct RF of BC agglomerates are enhanced by light scattering between their constituent primary particles as determined by the Rayleigh–Debye–Gans theory interfaced with discrete dipole approximation and recent relations for the refractive index and lensing effect. The light absorption of BC is enhanced by about 20 % by the multiple light scattering between BC primary particles regardless of the compactness of their agglomerates. The resulting light absorption agrees very well with the observed absorption aerosol optical depth of BC. ECHAM-HAM simulations accounting for the realistic BC morphology and its coatings reveal high direct RF = 3–5 W/m2 in East, South Asia, sub-Sahara, western Africa, and the Arabian peninsula. These results are in agreement with satellite and AERONET observations of RF and indicate a regional climate warming contribution by 0.75–1.25 °C, solely due to BC emissions.

How to cite: Kelesidis, G., Neubauer, D., Fan, L.-S., Lohmann, U., and Pratsinis, S.: Enhanced Light Absorption and Radiative Forcing by Black Carbon Agglomerates, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10268, https://doi.org/10.5194/egusphere-egu23-10268, 2023.

EGU23-11924 | Posters on site | AS3.8

Ice nucleation active site-independent stochasticity in heterogeneous ice nucleation 

Mária Lbadaoui-Darvas, Athanasios Nenes, and Ari Laaksonen

Clouds are central elements of the hydrological cycle and climate. They are responsible for precipitation and strongly impact global and regional temperature by reflecting incoming solar radiation, and absorbing heat emitted from Earth. The amount of ice contained in clouds determines much of their properties and their impact on climate. Cloud ice is mostly formed by heterogeneous nucleation (HIN), catalyzed by insoluble airborne particles (such as dust, biological particles and soot). Despite its importance, the description of HIN in climate models is vastly incomplete and remains one of the major challenges that impedes further progress in estimates of anthropogenic climate change.

 

One important open question is whether HIN should be modelled as a deterministic (time independent) or as a stochastic (time dependent) process. The typical sigmoidal shape of freezing curves - i.e., the fraction of frozen samples as a function of time - suggests the latter to be the correct approach. Current stochastic models cast the entire stochastic behavior on the differences between the IN activity of different ice nucleation active sites (INAS) in the sample. Recent studies however indicate that a large part of stochasticity may be independent from INAS variability.

 

The current work uses large scale molecular simulations freezing droplet ensembles on pure graphitic surfaces to explore the molecular scale origins of INAS independent stochasticity. We find that the interplay of three main factors: the size fluctuations of the pre-critical ice embryo, capillary wave fluctuations of the non-frozen droplet surface and the extent of stacking disorder - i.e.: cubic to hexagonal polymorph ratio - in the frozen droplet manifests as observable stochasticity even if the properties of the IN surface are identical. We conclude by quantifying the extent of INAS-independent stochasticity as a range of contact angles in the framework of the Adsorption Nucleation Theory. The resulting representation is then used to provide a stochastic adsorption-based parameterization of deposition freezing on soot particles. 

How to cite: Lbadaoui-Darvas, M., Nenes, A., and Laaksonen, A.: Ice nucleation active site-independent stochasticity in heterogeneous ice nucleation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11924, https://doi.org/10.5194/egusphere-egu23-11924, 2023.

EGU23-12521 | ECS | Posters on site | AS3.8

The cluster who came in from the cold: Nonisothermal nucleation in the gas phase is driven by cool subcritical clusters 

Valtteri Tikkanen, Bernhard Reischl, Hanna Vehkamäki, and Roope Halonen

Nucleation of clusters from the gas phase is a widely encountered phenomenon, e.g. regional air quality and global climate are both directly impacted by particle formation from atmospheric trace gases [1]. Still, the underlying out-of-equilibrium dynamics of this process are not well understood. The classical view of nucleation assumes isothermal conditions where the nucleating clusters are in thermal equilibrium with their surroundings. However, as in all first-order phase transitions, latent heat is released, potentially heating the clusters and suppressing the nucleation. The question of how the released energy affects cluster temperatures during nucleation as well as the growth rate remains controversial.

To investigate the nonisothermal dynamics and energetics of homogeneous nucleation, we have performed molecular dynamics (MD) simulations of a supersaturated Lennard-Jones (LJ) vapor in the presence of thermalizing carrier gas. In addition, a previous study of homogeneous nucleation of carbon dioxide in argon carrier gas [2] was revisited for temperature analysis of the growing CO2  clusters. The results obtained from these simulations are compared against kinetic modeling of isothermal nucleation and the classical nonisothermal theory by Feder et al. [3], which also predicts the existence of cool subcritical clusters, and has been quite controversial.

For the studied systems, we find that nucleation rates are suppressed by two orders of magnitude at most, despite substantial release of latent heat. Our analyses further reveal that while the temperatures of the entire cluster size populations are indeed elevated, the temperatures of the specific clusters driving the nucleation flux evolve from cold to hot when growing from subcritical to supercritical sizes. This resolves the apparent contradiction between elevated cluster temperatures and minor nonisothermal corrections to the nucleation rate, both often reported in literature, and is in excellent agreement with the theory of Feder et al. Our findings provide unprecedented insight into realistic nucleation events and allow us to directly assess earlier theoretical considerations of nonisothermal nucleation.

 

References

[1] M. Kulmala et al., Direct observations of atmospheric aerosol nucleation. Science 339, 943–946 (2013).

[2] R. Halonen et al., Homogeneous nucleation of carbon dioxide in supersonic nozzles II: Molecular dynamics simulations and properties of nucleating clusters. Phys. Chem. Chem. Phys. 23, 4517–4529 (2021).

[3] J. Feder, K. C. Russell, J. Lothe, G. M. Pound, Homogeneous nucleation and growth of droplets in vapours. Adv. Phys. 15, 111–178 (1966).

How to cite: Tikkanen, V., Reischl, B., Vehkamäki, H., and Halonen, R.: The cluster who came in from the cold: Nonisothermal nucleation in the gas phase is driven by cool subcritical clusters, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12521, https://doi.org/10.5194/egusphere-egu23-12521, 2023.

EGU23-12748 | Orals | AS3.8

Exploring the water structure on atmospheric particle surfaces 

Markus Ammann, Huanyu Yang, Anthony Boucly, Luca Artiglia, and Alexei Kiselev

Water is prevalent on all atmospheric particle surfaces, independent of material, phase state or water vapor saturation ratio. Under subsaturated relative humidity conditions, water occurs as reversibly adsorbed layers on solid surfaces or as concentrated aqueous solutions in aqueous particles, exhibiting different composition at the interface than in the bulk. The hydrogen bonding structure at these interfaces is affected by interactions with the substrate on solid surfaces and by ions and ionic or neutral surfactants on aqueous solutions. The water structure and its interplay with hydrated substrate features, hydrated free ions or neutral solutes or surfactant head groups are playing a key role in many chemical and physical processes at these interfaces. We have developed X-ray photoelectron spectroscopy (XPS) and electron yield near edge X-ray absorption fine structure (NEXAFS) spectroscopy to explore the interfacial water structure in situ. We will present examples of the structure of adsorbed water on different Feldspar surfaces, on silver iodide and titanium dioxide. We will also show cases related to the water structure on aqueous solutions containing salts or different surfactant species.

How to cite: Ammann, M., Yang, H., Boucly, A., Artiglia, L., and Kiselev, A.: Exploring the water structure on atmospheric particle surfaces, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12748, https://doi.org/10.5194/egusphere-egu23-12748, 2023.

EGU23-13943 | Orals | AS3.8 | Highlight

Assessing Exposure to Bioaerosols for Public Health Purposes: Turning the micro into the macro. 

Philippa Douglas and Emma Marczylo

Bioaerosols are ubiquitous in the environment and are comprised of a complex mix of different species and components of fungi, bacteria, pollen, and viruses. Exposure to some bioaerosols can be beneficial to health, and are an essential part of developing a normal, healthy immune system, whereas others can be detrimental and can cause or exacerbate a plethora of health conditions.

Understanding bioaerosol exposure is an essential part of understanding health effects and is often termed the ‘Achilles heel’ of environmental epidemiological studies. However, how do we assess exposure to such a complex mixture of biological matter, which changes spatially and temporally? How do we scale up what we discover at a handful of field sampling locations, or a cell model, to a larger national scale to help decision makers?

Here, I plan to present on current progress, gaps and challenges in assessing exposure to bioaerosols, using some past and ongoing work as key examples, and inviting opinions from the audience on how we can work together in the future to address gaps and challenges in this multidisciplinary field.

How to cite: Douglas, P. and Marczylo, E.: Assessing Exposure to Bioaerosols for Public Health Purposes: Turning the micro into the macro., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13943, https://doi.org/10.5194/egusphere-egu23-13943, 2023.

EGU23-14789 | Posters on site | AS3.8

Assessing exposure to fungal bioaerosols in transport environments: Analysing fungal composition of passive dust samples collected in UK railway stations 

Emma Marczylo, Sameirah Macchiarulo, James Isaac, Jodi Brookes, Brian Crook, Samuel Anees-Hill, Anna Hansell, and Philippa Douglas

Bioaerosols consist of a complex mixture of airborne microorganisms including fungi, bacteria, pollen, particulates and by-products of cells. While exposure to diverse microorganisms is essential for normal immune system development, bioaerosol inhalation has been associated with respiratory allergy and inflammation. Bioaerosol are ubiquitous, yet their composition within different environments is not well understood. Such information is essential for assessing exposure and associated health impacts. Here we focus on transport environments, namely railway stations (RSs), which pose a potential source of occupational and community exposure. 

Over 1200 passive dust samples were taken from 17 RSs across the UK from 03/2014-05/2015. GIS methods were used to provide information on population characteristics of the immediate surrounding area of the RSs. Together with information on RS layout and passenger numbers, this informed the selection of 250 samples, representing 9 RSs of varied geographical location, layout and footfall for further analysis. High throughput sequencing (HTS) with a metabarcoding approach targeting the ITS2 region was used to analyse the fungal composition of the sample subset. Such HTS techniques provide an opportunity to measure a wider range of microorganisms than traditional culture or microscopy techniques.

RS characteristics were varied and included indoor/enclosed and mostly outdoor layouts. Annual footfall varied from approximately 10-148 million.  The fungal composition of RS over time and relationships with different RS characteristics will be presented, identifying those driving any differences in composition.

How to cite: Marczylo, E., Macchiarulo, S., Isaac, J., Brookes, J., Crook, B., Anees-Hill, S., Hansell, A., and Douglas, P.: Assessing exposure to fungal bioaerosols in transport environments: Analysing fungal composition of passive dust samples collected in UK railway stations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14789, https://doi.org/10.5194/egusphere-egu23-14789, 2023.

EGU23-14945 | ECS | Orals | AS3.8

Modelling approaches for atmospheric ion-dipole collisions: all-atom trajectory simulations and central field methods 

Ivo Neefjes, Roope Halonen, Hanna Vehkamäki, and Bernhard Reischl

Collisions between ions and dipolar molecules can facilitate the formation of atmospheric aerosol particles and play an important role in their detection in chemical ionization mass spectrometers. Conventionally, analytical models or simple parametrizations have been used to calculate rate coefficients of ion-dipole collisions in the gas phase. Such models, however, neglect the atomistic structure and charge distribution of the collision partners.

         To determine the accuracy and applicability of these theoretical approaches, we calculated collision cross sections and rate coefficients from all-atom molecular dynamics collision trajectory simulations, sampling a relevant range of impact parameters and relative velocities, and from a central field model using an effective attractive interaction fitted to the long-range potential of mean force between the collision partners. We considered collisions between various atmospherically relevant molecular ions and dipoles, as well as charged and neutral dipolar clusters.

         We find excellent agreement between the collision cross sections and rate coefficients obtained from the molecular dynamics trajectory simulations and the central field model. Therefore, we conclude that the effective interactions between the collision partners are highly isotropic, and the central field model is able to capture the relevant physicochemical properties of the system.

         Comparing the molecular dynamics trajectory simulations with the often-used parametrization by Su and Chesnavich (1982), we find that the latter can predict the collision rate coefficient quite well for systems with a molecular dipole, but the agreement worsens for systems with a dipolar cluster.

         Based on our results, we propose the combination of potential of mean force calculation and central field model as a viable and elegant alternative to brute force sampling of individual collision trajectories over a large range of impact parameters and relative velocities.

         We are currently using the combination of potential of mean force calculation and central field model, as well as the atomistic trajectory simulations, to understand the relatively large increase in rate coefficient observed in chemical ionization mass spectrometers when sulfuric acid is charged with acetate, as compared to nitrate (Fomete, 2022).

 

Su, T. and Chesnavich, W. J.: J. Chem. Phys. 76, 5183–5185, 1982.

Fomete. S. et al.: J. Phys. Chem. A 126, 44, 8240–8248, 2022.

How to cite: Neefjes, I., Halonen, R., Vehkamäki, H., and Reischl, B.: Modelling approaches for atmospheric ion-dipole collisions: all-atom trajectory simulations and central field methods, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14945, https://doi.org/10.5194/egusphere-egu23-14945, 2023.

EGU23-15891 | Posters virtual | AS3.8

Rich microbial diversity in tropospheric samples above the planetary boundary layer confirms long-distance transport of potential human pathogens 

Xavier Rodó, Sofya Pozdniakova, Roger Curcoll, Alejandro Fontal, Atsushi Matsuki, Hiroshi Tanimoto, Maria Pilar Armengol, Irina Pey, Jordi Vila, Laura Muñoz, Lídia Cañas, Josep-Anton Morguí, and Sílvia Borràs

Existence of viable human pathogens in air above the planetary boundary layer (PBL) susceptible of reaching far-distance regions has never been demonstrated. Now ten aircraft monitoring surveys conducted over Japan in 2014 confirm the existence of a vast diversity of microbial species between 1000-3000 m a.s.l. being dispersed through wind currents for distances up to 2000 Km. Use of atmospheric particle dispersion models and LIDAR data has enabled us to confirm that under very predominant wintertime atmospheric conditions, aerosolised particles are uplifted by seasonal strong winds from areas in NE China, travel near 2000 Km away from their source well above the PBL and subside over Japan in less than 2 days. The area in NE China is covered with vast amounts of frozen decaying organic material originating from massive cereal croplands. Characterisation of microbial species attached to those particles shows dominance of known human pathogens typically originating from sewage, pesticides, fertilisers or agricultural debris from decaying organic matter. A majority of fungal taxa (over 90% concentration at times) and/or bacterial taxa (up to 67%) found therein are known for their potential adverse effects on human health. Noticeably, for bacteria less of a 30% of the taxa appearing could be identified to the species level and an additional 30% at most only at the family level. Similar numbers for fungi appear. Over 390 different fungal genera and over 340 bacterial genera showed up in flight samples comprised in the 10 aircraft transects, showing a great resemblance between flight and surface origin. Overall diversity is similar in high-altitudes and the surface when entrainment of air develops. In our study, microbial viability has also been observed as well as transport of antimicrobial resistance genes (ARG) in the cultured flight bacteria. The former constitutes one of the first evidences of very far distant transport of ARG and adds to the current known mechanisms for ARG propagation.

How to cite: Rodó, X., Pozdniakova, S., Curcoll, R., Fontal, A., Matsuki, A., Tanimoto, H., Armengol, M. P., Pey, I., Vila, J., Muñoz, L., Cañas, L., Morguí, J.-A., and Borràs, S.: Rich microbial diversity in tropospheric samples above the planetary boundary layer confirms long-distance transport of potential human pathogens, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15891, https://doi.org/10.5194/egusphere-egu23-15891, 2023.

EGU23-17161 | ECS | Posters on site | AS3.8

Monitoring airborne pathogens by nanopore sequencing 

Sofya Pozdniakova, Tim Reska, Lídia Cañas, Sílvia Borràs, Xavier Rodó, and Lara Urban

Next generation sequencing technologies have revolutionized the field of environmental science. Widely used short-read sequencing enables accurate microbial identification but is often slow, requires large centralised equipment, and does not allow to distinguish highly homologous genomic regions, making the taxonomic classification and genome assembly of closely-related species complicated. Those challenges may be resolved by the implementation of real-time long-read sequencing technologies such as Nanopore sequencing. Nanopore sequencing is a rapid technology that can be employed in situ through portable devices. The long sequencing reads can further improve precision of species identification in mixed microbial communities, and can provide more detailed characterisations of individual microorganisms. Despite its promising application to other environmental samples, nanopore sequencing has not yet been implemented to study bioaerosols and detect pathogens in air samples.

Here, we used nanopore sequencing to analyse the environmental DNA extracted from air samples collected in Barcelona, Spain, as an example of a highly urbanised area. As the total amount of DNA found in the air is significantly lower compared to other typical environmental material such as soil or water, we first optimised DNA extraction in combination with the newest nanopore rapid sequencing protocols to achieve a highly accurate genome assembly-based description of the air microbiome. We identified the presence of potentially pathogenic organisms, and annotated the genome assemblies with respect to phenotypic read-outs such as increased virulence and antimicrobial resistance.  We hereby compared the air microbiome assessed through a variety of air sampling methods, including high-volume air samplers, liquid impingers, and standard air filtering approaches. We further assessed if our optimized DNA extraction methods introduced a bias into the described microbiome composition by including positive controls. 

We were able to demonstrate that it is possible to identify airborne pathogens even when the amount of DNA is low, by leveraging cutting-edge nanopore sequencing technology without requiring cultivation or amplification. This method has the potential to enhance and speed up the surveillance of airborne diseases such as pneumonia, measles, and COVID-19. In upcoming research, we plan to utilise this framework to study the microorganisms present in the air in different settings in order to detect the potential emergence of antimicrobial resistance or highly virulent pathogens in real-time.

How to cite: Pozdniakova, S., Reska, T., Cañas, L., Borràs, S., Rodó, X., and Urban, L.: Monitoring airborne pathogens by nanopore sequencing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17161, https://doi.org/10.5194/egusphere-egu23-17161, 2023.

EGU23-589 | ECS | Orals | AS3.10

Airborne and marine microplastics in the Southern Ocean environment 

Alex Aves, Emelia Livingstone, Cliff Law, Laura Revell, and Sally Gaw

In recent years, microplastic transport through the atmosphere has gained interest. This pathway allows microplastics to reach remote regions of the world and draws attention to the impact which they may have on global climate processes and human health. Remote regions, particularly in the Southern Hemisphere, are currently under-researched and the understanding of airborne microplastics still in its infancy. Atmospheric deposition and seawater samples were collected on board a RV Tangaroa voyage, which sailed from Wellington, New Zealand to the Ross Sea, Antarctica in January 2021. Marine and atmospheric microplastics were collected and analysed spectroscopically to confirm polymer composition. The findings from this study will be discussed, highlighting the ubiquitous nature of microplastics throughout the Southern Ocean. This study contributes a unique data set from a remote region of the world, and further develops our understanding of marine-atmosphere fluxes of microplastics.

How to cite: Aves, A., Livingstone, E., Law, C., Revell, L., and Gaw, S.: Airborne and marine microplastics in the Southern Ocean environment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-589, https://doi.org/10.5194/egusphere-egu23-589, 2023.

EGU23-662 | ECS | Orals | AS3.10

Resuspension of microplastic particles from arid regions and global impacts on atmospheric concentrations and deposition 

Ioanna Evangelou, Daria Tatsii, Silvia Bucci, Christine Groot Zwaaftink, and Andreas Stohl

Microplastic particles (MP), i.e., plastic particles with a size between 1 µm and 1 mm, have been detected in all compartments of the Earth system. While we are beginning to develop a quantitative understanding of the primary emissions of MPs such as tire wear, secondary sources from polluted environmental compartments such as the oceans and arid land surfaces, are currently not understood at all.

In this study, we use reported MP concentrations in soils across the world combined with MP enrichment ratios (ER) in wind eroded sediments with respect to the soils (Bullard et al., 2021; Rezaei et al., 2019; Tian et al., 2022) and a population density map to estimate MP resuspension factors (RF) from arid regions.  We then use global, 3-hourly dust emissions at  0.5o x 0.5o resolution from FLEXDUST (Groot Zwaaftink et al., 2016, 2017), as a proxy for the spatial and temporal variation of MPs emitted by arid regions. Scaled with the resuspension factors, we estimate the global MP resuspensions. To calculate the uncertainty of our emission model, we conduct a one-thousand-member Monte Carlo simulation with 14 different RF scenarios for each population category, perturbing the MP concentration in soils, the ER and the spatial scale used for the population density.

We define, as a reference case, the emissions derived from the average ER, average soil concentrations and 50 km radius population categorization. These MP resuspension emissions are used as input to the Lagrangian atmospheric dispersion model FLEXPART (Pisso et al., 2019; Stohl et al., 2005) to simulate the global atmospheric cycle of resuspended MPs from arid regions. The simulations are driven by ERA5 meteorological fields at 0.5° horizontal resolution and 1-hour temporal resolution.  We simulate the global atmospheric concentration and the deposition of resuspended MPs for different size distributions as well as shapes (spheres, fibers) of MPs. Lastly, we quantify the impact and compare it with observations, to estimate the importance of resuspension from arid regions for global MP abundance.

How to cite: Evangelou, I., Tatsii, D., Bucci, S., Groot Zwaaftink, C., and Stohl, A.: Resuspension of microplastic particles from arid regions and global impacts on atmospheric concentrations and deposition, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-662, https://doi.org/10.5194/egusphere-egu23-662, 2023.

EGU23-1144 | Posters on site | AS3.10

Quantifying the uncertainty and errors between common analytical methods for measuring airborne microplastics 

Laura Revell, Alex Aves, Anna MacDonald, Deonie Allen, Steve Allen, Dusan Materic, Sally Gaw, Perry Davy, and Sebastian Naeher

In recent years airborne microplastics have emerged as a ubiquitous pollutant worldwide, with negative implications for ecosystems, climate and human health. The differing sampling and analysis techniques used amongst micro- and nanoplastic research groups limits our understanding of the global distribution of airborne microplastics and nanoplastics. We present plans and progress for an ongoing coordinated inter-laboratory experiment, designed to elucidate strengths and weaknesses of individual analysis methods. Daily active pumped air samples were collected in a controlled manner at a remote site in Canterbury, New Zealand, alongside weekly deposition samples. All samples were divided evenly, using specific contamination controls, into four sample sets for interlaboratory method comparisons, and distributed to participating research groups in New Zealand, Germany and the UK. Samples will be analysed using common microplastic analysis techniques: micro-Fourier transform infrared spectroscopy (µFTIR), micro-Raman spectroscopy (µRaman), fluorescence microscopy, pyrolysis – gas chromatography/mass spectrometry (Py-GC/MS), and thermal desorption – proton transfer reaction – mass spectrometry (TD-PTR-MS). The results will allow quantification of the relative uncertainties and biases associated with each individual method, and inform how future airborne microplastics studies performed with different analytical methods should be interpreted.

How to cite: Revell, L., Aves, A., MacDonald, A., Allen, D., Allen, S., Materic, D., Gaw, S., Davy, P., and Naeher, S.: Quantifying the uncertainty and errors between common analytical methods for measuring airborne microplastics, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1144, https://doi.org/10.5194/egusphere-egu23-1144, 2023.

EGU23-2736 | ECS | Posters on site | AS3.10

Qualitative and quantitative analysis of synthetic polymers in ambient aerosols by Curie Point Pyrolysis-Gas Chromatography/Mass Spectrometry 

Ankush Kaushik, Majda Mekic, Manuela van Pinxteren, and Hartmut Herrmann

Nano- and microplastics (NMP), including tire wear particles (TWP), are now a global concern in the terrestrial and marine environment and are subject of intense study. The existence of NMP and TWP in many different environments has been reported, including soil, sediment, dust, glaciers, lakes, rivers, seas, and oceans. However, only a few studies have examined the abundance and fate of synthetic polymers in ambient aerosol particles. The dispersion, atmospheric transport and deposition of NMP and TWP are important steps in the biogeochemical cycle of plastic. The inconsistencies in the methods of sampling, processing, analysis, and the Quality Assurance (QA)/ Quality Control (QC) procedures of NMP and TWP hinder our ability to examine these contaminants' spatial and temporal patterns in the atmosphere. Based on the previously reported research on the analysis of NMP and TWP in the air, it becomes necessary to develop a comprehensive standard methodology that should be established for detecting microplastics in the atmosphere at submicron level (PM10 and PM2.5). Since synthetic polymers are difficult to quantify at low concentrations, Pyrolysis-Gas Chromatography coupled with Mass Spectrometry provides an effective technique for detecting NMP and TWP. As part of the present study, we aim to develop and provide methods and measurement approaches that would facilitate the routine analysis of PM10 and PM2.5 samples for synthetic polymers in aerosol particles in terms of mass concentrations using Curie Point Pyrolysis-Gas Chromatography coupled with Mass Spectrometry (CPP-GC/MS). To follow this, reference standards were milled using a cryo-mill, and a calibration curve was obtained for the most common synthetic polymers present in the atmospheric environment, such as Polystyrene (PS), Polypropylene (PP), Polyethylene Terephthalate (PET), High-Density Polyethylene (HDPE), Low-Density Polyethylene (LDPE), Polyvinyl Chloride (PVC), Poly(methyl-methacrylate) (PMMA) and Styrene Butadiene Rubber (SBR). The present study determined the Limit of Quantification (LOQ) and Limit of Detection (LOD) of each standard by analysing it at different concentrations down to the lowest level with acceptable repeatability and accuracy. The current method of quantifying synthetic polymers was tested by spiking experiments on aerosol samples (PM10 and PM2.5) at different concentrations. This study examines open research questions in various main areas, including developing analytical methods, size-resolved sampling, and analysing NMP and TWP in ambient aerosol particles in urban, rural, and remote areas.

Keywords: Nano- and microplastics, tire wear particles, synthetic polymers, Curie Point Pyrolysis-Gas Chromatography/Mass Spectrometry.

How to cite: Kaushik, A., Mekic, M., van Pinxteren, M., and Herrmann, H.: Qualitative and quantitative analysis of synthetic polymers in ambient aerosols by Curie Point Pyrolysis-Gas Chromatography/Mass Spectrometry, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2736, https://doi.org/10.5194/egusphere-egu23-2736, 2023.

EGU23-3454 | ECS | Posters on site | AS3.10

Long-distance atmospheric transport of microplastic fibers depends on their shapes 

Qi Li, Shuolin Xiao, Yuanfeng Cui, Janice Brahney, and Natalie Mahowald

Recent studies have highlighted the importance of the atmosphere in the long-range transport of microplastic fibers (MPFs).  However, both dry deposition processes and sources of MPFs are poorly understood due to their complexity in size and shape, which can be 100s $\mu m$ long, possessing round or flat cross-sections with dimensions of $O(1)\,\mu m$ thickness, and $O(10)\,\mu m$ width. Here, we develop a theory-based settling velocity model for MPFs in the atmosphere, predicting a much smaller aerodynamic size than a volumetrically equivalent spherical particle. Incorrect identification of flat fibers as cylindrical ones due to uncertainty in the thickness of sampled MPFs overestimates their dry deposition rate. Accounting for fiber thickness in sampled MPFs leads to a mean residence-time enhancement above $450\%$ compared to spherical-shaped particles, suggesting a much more efficient long-range transport of flat fibers than previously thought and that the ocean might be a major source of atmospheric plastics.

How to cite: Li, Q., Xiao, S., Cui, Y., Brahney, J., and Mahowald, N.: Long-distance atmospheric transport of microplastic fibers depends on their shapes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3454, https://doi.org/10.5194/egusphere-egu23-3454, 2023.

EGU23-4226 | ECS | Orals | AS3.10 | Highlight

Detection and Quantification of Micro(nano)plastics Release from Photolysis of Surgical Masks 

Guyu Peng, Dusan Materic, and Thorsten Reemtsma

Since the Covid-19 pandemic, 129 billion masks have been consumed each month worldwide. Fate of masks not only include waste disposal sites and natural environments, but masks made from synthetic fibers may release micro(nano)plastics (MNPLs) that may reach respiratory tracts. However, degradation rate of MNPLs generated from masks have been unknown.

Here, we simulated the photolysis of surgical masks made from polypropylene equivalent to 900 days. Size-fractionated MNPL formation was quantified using vibrational spectroscopic imaging, and mask deformation and morphology were characterized with correlative microscopy. Three layers of masks did not exhibit signs of degradation from hydroxyl and carbonyl groups, however, the outer layer exhibited a linear increase in crystallinity calculated from the peak height of two characteristic bands, indicating that degradation started from amorphous regions. However, for microplastics > 10 μm, both groups were observed, and mass concentration was 10 mg/item calculated from FTIR imaging data. Fine microplastics <10 μm were imaged and fitted as ellipses, and the most abundant aspect ratio was 2. Nanoplastics (<1 μm) with an average size of 149 (59) nm were detected by SEM/STEM and Raman spectroscopy. Cluster analyses on spectra categorized three groups, suggesting different additives (e.g., dyes) were added. This study detected nanoplastics from degraded masks, which have major implications for their environmental fate and human health effects.

How to cite: Peng, G., Materic, D., and Reemtsma, T.: Detection and Quantification of Micro(nano)plastics Release from Photolysis of Surgical Masks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4226, https://doi.org/10.5194/egusphere-egu23-4226, 2023.

EGU23-5730 | ECS | Orals | AS3.10

Fine microplastics and nanoplastics in particulate matter samples from a high alpine environment 

Daniela Kau, Dušan Materić, Rupert Holzinger, and Anne Kasper-Giebl

The steady high demand for plastics and the degradation of discarded materials have led to microplastics and nanoplastics becoming important pollutants in various environmental compartments. While the situation, e.g. in the marine environment, is frequently described in the literature, a focused research on ambient air and especially different size classes of airborne particulate matter is scarce. Still, airborne particles are of special importance, as they have high mobility and can be transported and distributed rapidly.

We analysed particulate matter samples of two size classes, PM1 and PM10 (particles with aerodynamic diameters up to 1 or 10 µm, respectively), using thermal desorption-proton transfer reaction-mass spectrometry (TD-PTR-MS) and determined and quantified different polymer types from the spectra using a previously described method [1]. Particulate matter was collected at the remote high alpine Global Atmosphere Watch station Sonnblick Observatory, Austria, at more than 3100 m above sea level on quartz-fibre filters. Sampling time was one week. The samples covered a summer period (June 2021 to September 2021) and a winter period (December 2021 to April 2022). The periods were selected to include samples with and without mineral dust occurrence to allow a comparison. For the 23 samples of PM1 and PM10, analysis was done in triplicates. Field blanks were also available. Several lab and field tests were performed to check possible influences during the storage of samples (use of different containers including plastics and aluminium foil) and sample preparation (addition of hydrogen peroxide).

Our evaluations include the determination of six common types of plastics (PET, PE, PP/PPC, PS, PVC, tire wear) in both fractions and seasonal differences in their relative contributions. The most abundant plastic types were PET, PE and PP/PPC. Overall polymer concentrations reached up to 125 ng/m³. Field blanks showed comparably low presence of PET. We further compare the relative contributions of the summer and winter periods depending on the occurrence of mineral dust.

 

[1] Materić, D. et al., Micro- and Nanoplastics in Alpine Snow: A New Method for Chemical Identification and (Semi)Quantification in the Nanogram Range. Environmental science & technology 2020, 54(4), 2353-2359.

How to cite: Kau, D., Materić, D., Holzinger, R., and Kasper-Giebl, A.: Fine microplastics and nanoplastics in particulate matter samples from a high alpine environment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5730, https://doi.org/10.5194/egusphere-egu23-5730, 2023.

EGU23-6536 | Orals | AS3.10

High debit sampling of airborne micro and nanoplastics in remote sea 

Boris Eyheraguibel, Alexandra Ter Halle, Yann Ourmieres, Jean-Francois Ghiglione, and Pierre Amato

The occurrence of micro and nano plastics has been reported in every environmental compartment including marine and freshwaters, soils and sediments, air and atmospheric precipitations.  Recent evidence showing the presence of airborne microplastics in remote ecosystems highlights the extent of this pollution. The atmospheric transportation and the distribution of airborne microplastics still need to be better documented to understand the dynamic of microplastic transfer between ecosystems.

While most studies dedicated to the analysis of microplastics in the air use a passive sampling methodology through atmospheric deposition we developed an original stainless device to sample large volumes of air with high debit (2000 L/min) providing a fast sampling of aerosols within a small localized area. An optimized sampling protocol has been deployed in the North Western Mediterranean Sea from the Expedition 7th Continent (E7C) boat. 19 sampling sites have been studied during the E7C expedition in September-October 2019, including measurements in port and coastal areas as well as offshore environments. The analysis of micro/nano plastics was carried out using pyrolysis coupled with gas chromatography and tandem mass spectrometry (Py-GC-MS/MS). This approach allowed us to evaluate the concentrations of micro and nano plastics present in the samples for 5 types of plastics (polypropylene, polystyrene, polymethyl methacrylate, polyethylene terephthalate and polycarbonate) and for 2 size ranges (5-50μm and <5μm).

This study confirmed that plastic particles are present in the atmosphere even in remote areas such as the offshore environments. The results showed that airborne micro and nano plastics were detected at each sampling station, from the coast to the open sea, at various concentrations. Py-GC-MS/MS analysis allowed us to quantify the 5 types of polymer and revealed the predominance of PET and PP material. High-volume samplers and  Py-GC-MS/MS analysis have proven to be an efficient and powerful methodology to gather and quantify airborne plastic particles at micro and nanoscale level.

How to cite: Eyheraguibel, B., Ter Halle, A., Ourmieres, Y., Ghiglione, J.-F., and Amato, P.: High debit sampling of airborne micro and nanoplastics in remote sea, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6536, https://doi.org/10.5194/egusphere-egu23-6536, 2023.

EGU23-8026 | ECS | Orals | AS3.10

Freshly fallen snow with full of microplastics: A scientific research in Riga central and peripheral area, Latvia. 

Rupa Chand, Fan Liu, Asbjørn Haaning Nielsen, Ieva Putna -Nīmane, Elina Vecmane, and Jes Vollertsen

Abstract:

Atmospheric transportation can be an essential pathway for microplastics (MPs), yet the understanding of the abundance, composition and morphological characteristics of the air-transported MPs remain limited.

In this study, we sampled freshly fallen snow at six locations around Riga in Latvia, covering land uses of urban, rural, and remote regions (Figure 1): i) Central market (CM) at Riga Central Market, ii) Old town (OT) at Doma Church Square, iii) Parking lot (PL) at Spice Home Parking, iv) Suburb (SB) at Pavasara str. 4, v) City roof (CR) at about 50 m high on Latvian Academy of Science building and vi) Gauja National Park (NP). Samples were collected 8 – 9 December 2021. 20 L stainless steel buckets and a metal shovel were used to collect the samples. To minimize contamination, plastic tools were avoided except rubber boots and gloves. The collected snow was taken to the laboratory and kept at room temperature (22 – 23°C) until it melted. After measuring the volume of the melted snow, it was filtered through 10 µm mesh stainless steel filters. MPs were extracted from the collected particles through enzyme treatment, oxidation, and density separation (Chand et al., 2021; Simon et al., 2018). The extracted particles were analysed by FPA-µFTIR imaging, and the obtained hyperspectral images were analysed by siMPle for MP identification. Laboratory processes were conducted in a clean fume hood and only cotton lab coats were worn in the lab.

MPs were detected in all snow samples, covering 16 polymer types. The most common polymers were polyester, polypropylene (PP), polyvinyl chloride (PVC), polyethylene (PE), and polyamide (PA). The results showed a large variation in MP concentration between the sites (Figure 1), among which Central market had the highest MP accumulation with 2497±755 items L-1, followed by Parking (1278±394 items L-1) and Old town (1233±57 items L-1). The order was the same when quantifying MP mass. Though also located in the urban area, snow on the City roof had significantly fewer MPs (95±19 items L-1) than other urban snow samples. This indicates that the snow had collected much of its MP while falling the last few meters or while lying on the ground. The least contaminated snow was found in Gauja National Park, which is remote from the urban area.This concludes that the MP snow contamination closely depends upon the human activities as well as strongly affected by the local sources. 

Figure 1: MP particle concentration (above) and MP mass concentration (below) in the analysed samples from different sampling locations

 

References

Chand, R., Rasmussen, L.A., Tumlin, S., Vollertsen, J., 2021. The occurrence and fate of microplastics in a mesophilic anaerobic digester receiving sewage sludge, grease, and fatty slurries. https://doi.org/10.1016/j.scitotenv.2021.149287

Simon, M., van Alst, N., Vollertsen, J., 2018. Quantification of microplastic mass and removal rates at wastewater treatment plants applying Focal Plane Array (FPA)-based Fourier Transform Infrared (FT-IR) imaging. Water Res. 142, 1–9. https://doi.org/10.1016/j.watres.2018.05.019

 

How to cite: Chand, R., Liu, F., Haaning Nielsen, A., Putna -Nīmane, I., Vecmane, E., and Vollertsen, J.: Freshly fallen snow with full of microplastics: A scientific research in Riga central and peripheral area, Latvia., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8026, https://doi.org/10.5194/egusphere-egu23-8026, 2023.

EGU23-9154 | ECS | Orals | AS3.10

Global microplastic emission and deposition fluxes at the ocean-atmosphere interface 

Silvia Bucci, Camille Richon, Lucie Bakels, and Andreas Stohl

While microplastics (MP) have been recently identified and recognized as a pollutant for the atmospheric environment, little is known about their actual emissions and concentration in the atmosphere. In this work, we follow a bottom-up approach to estimate the fluxes of MP at the ocean-atmosphere interface.

Coupling a sea spray emission scheme (Grythe et al. 2014) with the MP concentrations over the ocean surface simulated by the NEMO-PISCES general circulation model (Nucleus for European Modelling of the Ocean, Pelagic Interaction Scheme for Carbon and Ecosystem Studies, Richon et al. 2022), we estimate the global sea spray MP emissions at 6-hourly resolution, over a one-year period.

The MP emission fluxes are then fed into the Lagrangian atmospheric dispersion model FLEXPART (Stohl et al., 2005; Pisso et al., 2019), driven with hourly ERA5 data at 0.5° horizontal resolution, to provide a global picture of the atmospheric cycle of the MP of marine origin.

We discuss the main emission areas and their marked seasonal variability, the resulting atmospheric concentration across the globe and the deposition fluxes on both land and ocean surfaces. Finally, we compare simulated fluxes and concentrations with existing observations of MP in the marine atmosphere.

How to cite: Bucci, S., Richon, C., Bakels, L., and Stohl, A.: Global microplastic emission and deposition fluxes at the ocean-atmosphere interface, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9154, https://doi.org/10.5194/egusphere-egu23-9154, 2023.

EGU23-10352 | Posters on site | AS3.10

In situ chemical characterization of airborne nanoplastic particles by aerosol mass spectrometry 

Arthur Chan, Michael Tawadrous, Xing Wang, and Alex Lee

Extensive use of plastic products has introduced a large amount of plastic pollutants in urban areas and even in remote environments. Nanoplastic particles, in particular, can remain airborne for weeks and transported across greater distances. Characterization of atmospheric nanoplastic particles has been limited. Sampling methods used for larger microplastic particles, such as deposition sampling, and characterization methods, such as spectroscopy, are not applicable to nanoplastic particles. Furthermore, offline sampling methods involve extensive sample preparation procedures which can alter physical and chemical properties of the particles.

In this work, we investigate the use of aerosol mass spectrometry (AMS) as an in situ technique to characterize nanoplastic particle size and composition. We generate plastic particles via three different techniques: thermal decomposition of PET plastic bottles, 3D printing (using PET, ABS, and PLA filaments) and mechanical abrasion. Particle size was characterized using a Scanning Mobility Particle Sizer (SMPS). Particles were also sampled into a high resolution time of flight aerosol mass spectrometer (HR-ToF-AMS) and onto quartz filters for offline characterization using pyrolysis gas chromatography mass spectrometry (Py-GC/MS).

We found that the AMS produced real-time particle mass spectra that were very similar to those measured by Py-GC/MS analysis of particles collected on filters. The consistency between the two techniques demonstrate that AMS can provide similar information about polymeric content as Py-GC/MS, which is a widely used technique for plastic materials, but at a substantially lower detection limit and higher time resolution. On the other hand, the use chromatographic separation in Py-GC/MS provides more comprehensive evaluation of polymeric composition. For example, we were able to detect changes in ratios between monomers and dimers of PET using Py-GC/MS. Py-GC/MS was also able to provide simultaneous measurement of rubber polymers and additives in tire wear particles, an important source of particles in the near road atmosphere.

Since AMS is a commonly used technique for non-refractory components in atmospheric aerosol, optimizing the AMS for nanoplastic particle detection will help understand the sources, dynamics, mixing state and fate of nanoplastic particles in the atmosphere.

How to cite: Chan, A., Tawadrous, M., Wang, X., and Lee, A.: In situ chemical characterization of airborne nanoplastic particles by aerosol mass spectrometry, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10352, https://doi.org/10.5194/egusphere-egu23-10352, 2023.

Nowadays, microplastics (MPs) are being found everywhere, ranging from water bottles to nearly pristine areas such as the Antarctic and Arctic regions. On the other hand, the physicochemical characteristics of airborne microplastics (AMPs) of inhalable size (<10 μm), which are particularly critical in respect of human health and climate change, are still poorly understood due to the lack of suitable analytical methods. An efficient and reliable analytical strategy is required for the investigation of inhalable AMPs, which constitute just a very small portion of ambient aerosol particles. In this study, a new analytical strategy that employs fluorescence microscopy, Raman microspectrometry (RMS), and scanning electron microscopy/energy dispersive X-ray spectrometry (SEM/EDX) in combination was demonstrated to be powerful for a reliable and detailed investigation of inhalable AMPs in ambient aerosols. Fluorescent staining and fluorescence microscopy can provide an efficient screening for high MP potential particles among ambient aerosols. The combined application of RMS and SEM/EDX to the same stained individual particles allows a detailed physicochemical characterization of stained particles. In this study, stained, high MP potential particles were observed with a probability of ~0.008(±0.005)%, corresponding to ~800 particles/m3, in a PM10 ambient aerosol sample. Among the stained particles of <10 μm, 27% were found to be plastics, including polystyrene, polyethylene, poly(ethylene terephthalate), and acrylonitrile butadiene styrene, and 73% were from tire/road wear. The number of inhalable AMPs was estimated to be 192(±127) particles/m3.

How to cite: Yoo, H., Lee, Y., and Ro, C.-U.: Single-particle investigation of airborne microplastics of inhalable size (<10 μm) using fluorescence microscopy, Raman microspectrometry, and scanning electron microscopy/energy dispersive X-ray spectrometry in combination, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11138, https://doi.org/10.5194/egusphere-egu23-11138, 2023.

EGU23-12251 | ECS | Posters on site | AS3.10

Is plastic dust different from mineral dust? Results from idealized wind tunnel experiments. 

Eike Esders, Sebastian Sittl, Inka Krammel, Wolfgang Babel, Georg Papastavrou, and Wolfgang Babel

Atmospheric transport has been shown to effectively disperse microplastic
particulate matter to virtually every environment on the planet. Despite this
efficient long-range transport, only few studies have examined the fundamental
mechanisms of the atmospheric transport of microplastics. Here, we present the
results of wind tunnel experiments, examining the detachment behavior of plastic
particles ranging from 38 to 125 µm in diameter from flat substrates.
Detachment was achieved solely by aerodynamic forces of the turbulent airflow.
The detachment behavior of spheric microplastic particles (Polyethylene) and
spheric glass microparticles (Borosilicate) of nominally the same diameter
(63-75 µm) are contrasted across substrates with hydrophilic to hydrophobic
surface coatings. We further examine the effect of particle-particle collisions on
the detachment behavior of both Polyethylene and glass spheres. The critical
friction velocity (u*,th), which is defined as the value at which 50% of all
microparticles detach, ranged from 0.1 to 0.3 ms −1. Particle-particle collisions
reduced the u*,th of glass, but not that for PE. Results were compared with
predictions of a Jonhson-Kendall-Roberts model. The relation of diameter to
u*,th compared well between results and prediction for Polyethylene spheres.
Glass spheres were predicted to detach at smaller u*,th than polyethylene
spheres, but detached at higher u*,th. Here, we argue that capillary forces
increased the adhesion, which is not covered by the model. The combination of
particle and substrate hydrophobicity influenced the relative humidity, at which
capillary forces increased u*,th.

How to cite: Esders, E., Sittl, S., Krammel, I., Babel, W., Papastavrou, G., and Babel, W.: Is plastic dust different from mineral dust? Results from idealized wind tunnel experiments., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12251, https://doi.org/10.5194/egusphere-egu23-12251, 2023.

EGU23-12323 | ECS | Posters on site | AS3.10

Atmospheric contribution of nanoplastics to rural and remote surface waters 

Dusan Materic, Mike Peacock, Joshua Dean, Martyn Futter, Trofim Maximov, Filip Moldan, Thomas Röckmann, and Rupert Holzinger

There is growing evidence for global environmental pollution caused by plastic particles <1 µm, here referred to as nanoplastics. Nanoplastic concentrations have been below the detection limits of many methods for quite some time, and thus they have passed undetected in complex environmental samples. However, recently using Thermal Desorption – Proton Transfer Reaction – Mass Spectrometry, many common nanosized polymers have been detected in seawater, ice and snow of rural and remote sites. In this work, we focused on the waterbodies of two contrasting sites: remote Siberian Arctic tundra and a forest landscape in southern Sweden. Nanoplastics of four polymer types (polyethylene, polyvinyl chloride, polypropylene, polyethylene terephthalate) were detected in all sampled Swedish lakes and streams (mean 563 µg/L, seven lakes, four streams). The amount of nanoplastic polymers showed a correlation with plastic demand in Europe (R2 = 0.91). In Siberia, two nanoplastic polymers (PVC and polystyrene) were detected in lakes, ponds and surface flooding, and concentrations were lower (mean 51 µg/L, three lakes, five ponds, overland flow from thawing permafrost and flooded tundra). Based on potential source analysis and HYSPLIT modelling of air mass trajectories and particle dispersion, we infer that nanoplastics predominantly arrive at both sites by atmospheric deposition from local and regional sources.

How to cite: Materic, D., Peacock, M., Dean, J., Futter, M., Maximov, T., Moldan, F., Röckmann, T., and Holzinger, R.: Atmospheric contribution of nanoplastics to rural and remote surface waters, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12323, https://doi.org/10.5194/egusphere-egu23-12323, 2023.

EGU23-12619 | Posters on site | AS3.10

Spatio-temporal inversion of atmospheric microplastics emmisions using block-coordinate descent method 

Ondřej Tichý, Václav Šmídl, and Nikolaos Evangeliou

We propose an inversion methodology that allows to estimate large-scale spatio-temporal emission profiles from deposition measurements of airborne microplastics from the Western USA. Traditionally, each spatio-temporal element is solved separately using linear inverse model, however, it is hard or even impossible to deduce which part of measurements is reconstructed by which spatio-temporal element. In this contribution, we treat the unknown spatio-temporal source term as a single unknown variable of a large scale optimization problem. To achieve a tractable algorithm, we propose to use the block coordinate descent (BCD) approach with each spatial element being a block of coordinates. The implied inversion method is an iterative procedure with selected linear inverse method in the inner loop. We have tested the standard linear inversion with Tikhonov regularization as well as self-tuning LS-APC (Least Squares with Adaptive Prior Covariance) Bayesian inversion as inner loop algorithms. The method converges within a small number of iterations. The results are compared with previous approaches for spatio-temporal emission estimation and the potential of the novel method is demonstrated.

How to cite: Tichý, O., Šmídl, V., and Evangeliou, N.: Spatio-temporal inversion of atmospheric microplastics emmisions using block-coordinate descent method, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12619, https://doi.org/10.5194/egusphere-egu23-12619, 2023.

EGU23-12884 | ECS | Orals | AS3.10

A novel online method for the detection, analysis, and classification of airborne microplastics 

Nicholas Beres, Julia Burkart, Elias Graf, Yanick Zeder, Erny Niederberger, Lea Ann Dailey, and Bernadett Weinzierl

The continued increase in global plastic production and poor waste management ensures that plastic pollution is a serious environmental concern for years to come. Because of their size, shape, and relatively low density, primary or secondary plastic particles in the environment between 1-1000 µm in size (known as microplastics, or MPs) may be entrained (and/or re-entrained) into the atmosphere through processes similar to other coarse-mode particles, such as mineral dust. MPs can thus be advected over great distances, reaching even the most pristine and remote areas of the Earth, and may have significant negative consequences for humans and the environment. The detection and analysis of MPs once airborne, however, remains a challenge because most observational methods are offline and resource-intensive, and, therefore, are not capable of providing continuous quantitative information.

In this study, we present results using an online, in situ airflow cytometer (SwisensPoleno Jupiter; Swisens AG; Horw, Switzerland) – coupled with machine learning – to detect, analyze, and classify airborne, single-particle MPs in near real time. The performance of the instrument to differentiate single-particle MPs of five common polymer types was investigated under laboratory conditions using combined information about their size and shape (determined using holographic imaging) and intrinsic fluorescence, known as autofluorescence, measured using three excitation wavelengths and five emission detection windows. The classification capability using these methods was determined alongside other coarse-mode aerosol with similar morphology or autofluorescence characteristics, such as a mineral dust and several pollen taxa.

The tested MPs exhibit a measurable autofluorescence signal that not only allows them to be distinguished from the other particles in this study demonstrating autofluorescence properties, such as pollen, but can also be differentiated from each other, with high (>90%) classification accuracy based on their multispectral autofluorescence signatures and morphology. The results using the presented novel methods are expected to provide a foundation towards significantly improving the understanding of properties and types of MPs present in the atmosphere.

How to cite: Beres, N., Burkart, J., Graf, E., Zeder, Y., Niederberger, E., Dailey, L. A., and Weinzierl, B.: A novel online method for the detection, analysis, and classification of airborne microplastics, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12884, https://doi.org/10.5194/egusphere-egu23-12884, 2023.

EGU23-13376 | ECS | Orals | AS3.10

Global Modeling of Microplastics in the Atmosphere 

Shanye Yang

Global Modeling of Microplastics in the Atmosphere
Shanye Yang, Guy Brasseur, Stacy Walters, Pablo Lichtig, Cathy Wing Yi Li, Xiaofei Wang

Global model simulations driven by bottom-up emissions show that more than 100 kilotons of microplastic particles are suspended in the atmosphere. The calculations are based on estimated emissions associated to traffic, agriculture, domestic activities and ocean exchanges. They make use of our laboratory measurements of microplastic exchanges at the water-air interface that is considerably less intensive than the emissions from land. Approximately 20 million tons are deposited each year on the Earth’s surface, and 3 million tons in the oceans. These model simulations show that the microplastic particle abundance is considerably higher over the continents, which is consistent with current observations. Exposure risks are highest in the most populated areas. Worldwide, adults inhale 2.4 × 107 - 1.5 × 109 microplastic particles per year. Remote areas including Antarctica and the Arctic are also important receptor regions for the particles with a diameter smaller than 1.5 μm.

How to cite: Yang, S.: Global Modeling of Microplastics in the Atmosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13376, https://doi.org/10.5194/egusphere-egu23-13376, 2023.

EGU23-17295 | Orals | AS3.10

Reactivity of selected model microplastics with ozone 

Liselotte Tinel, Eva Remoissenet, Mel Constant, Claire Allary, and Manolis Romanias

Microplastics (MPs) are nowadays observed in all environmental compartments. However, in the atmosphere, the presence of this new pollutant is not well documented and not well understood. So far, atmospheric microplastic particles have been observed in megacities,1 in remote mountain areas2 and even over the open ocean,3 albeit in low concentrations. Microplastics exposed to the atmosphere, undergo ageing under the influence of atmospheric oxidants and sunlight. As the MPs are altered over time, their physicochemical properties are modified. In particular, the polymer structure of MPs can become more porous increasing their exposed surface compared to their new counterparts. This in turn can lead to an increased reactivity between atmospheric oxidants / pollutants and polymers. Furthermore, their physicochemical changes can ultimately lead to fragmentation, giving rise to the formation of more and smaller particles. It therefore seems important to quantify the reactivity of these new pollutants with atmospheric oxidants, as this can affect the role of MPs in the atmosphere, and their environmental fate. The present study provides the first results of a laboratory study on the reactivity of model microplastics, PEEK, PTFE, LDPE, PET, with ozone in a in a DRIFT (Diffuse Reflectance Infrared Fourier Transform) optical cell for the in-situ monitoring of MPs surface aging, coupled with an ozone analyser and a soft ionization Mass spectrometer (SIFT-MS), for the real-time monitoring of the gas-phase. The in-situ monitoring of MPs properties with DRIFTs revealed important chemical changes on their surface due to their exposition to ozone. We suggest that carboxylic acids and/or esters are amongst the most prominent reaction products. We also determine the ozone uptake coefficient (γss) of the MPs, and the evolution of their specific surface area before and after exposure to ozone. The values of γss measured are in the range of 10-8 to 10-9, indicating that MPs are not an important sink of gaseous O3 in the atmosphere. Further analysis of the gas-phase with SIFT-MS, evidenced the formation of VOCs and particularly carboxylic acids amongst the most prominent reaction products of MPs reaction with ozone. The impact of the modification of chemical functionalities at the surface of these microplastic on their environmental behaviour (e.g. hygroscopicity) and the reactivity of microplastics on the composition of the atmosphere is further discussed.
Ref. : [1] Dris et al., 2015, Environ. Chem / [2] Allen et al., 2015, Nat. Geosci. / [3] Trainic et al., 2020, Commun. Earth Environ.

How to cite: Tinel, L., Remoissenet, E., Constant, M., Allary, C., and Romanias, M.: Reactivity of selected model microplastics with ozone, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17295, https://doi.org/10.5194/egusphere-egu23-17295, 2023.

EGU23-3091 | ECS | PICO | AS3.11

Modeling nitryl chloride and its source and effect on gaseous and aerosol chemistry 

Hyeonmmin Kim, Rokjin Park, Jean Jeong, Saewung Kim, Daun Jeong, Xiao Fu, and Seogju Cho

Nitryl chloride (ClNO2) has been reported as a critical species of chlorine chemistry. Its chemistry interrupts a nighttime sink of NOX and emits chlorine radical (Cl•) in the daytime, consequently altering gaseous and aerosol chemistry. Recent field studies have also measured considerable concentrations of ClNO2 in South Korea under the influences of natural and anthropogenic chlorine sources. However, the impacts of ClNO2 chemistry on air quality in South Korea have yet to be evaluated. We validate simulated ClNO2 and its chemistry in South Korea using observations and a 3-D chemical transport model (CTM) during the Korea-United States Air Quality field study. We implemented the latest Chinese and Korean anthropogenic chlorine emissions in the model. We found that the model reproduces the observed spatial and temporal variations of ClNO2, including its local and transboundary transport and precursors. We found that ClNOchemistry results in a more efficient conversion of NO to NO2 at night and daytime acceleration of the NOX-O3 cycle. It results in an increase of O3 (1.1%), NOX (3.1%), OH (2.0%), HO2 (0.8%), and Cl• (507.8%) and a decrease of TNO3(HNO3 + aerosol nitrate, 1.7%) on the campaign mean basis.

How to cite: Kim, H., Park, R., Jeong, J., Kim, S., Jeong, D., Fu, X., and Cho, S.: Modeling nitryl chloride and its source and effect on gaseous and aerosol chemistry, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3091, https://doi.org/10.5194/egusphere-egu23-3091, 2023.

EGU23-3524 | PICO | AS3.11

Impact of iodine injections from the suface and the small satellites using iodine propulsion system in the upper atmosphere on ozone depletion 

Wuhu Feng, John Plane, Martyn Chipperfield, Alfonso Saiz-Lopez, Jean-Paul Booth, Sarah McClory, and Doug Kinnison

Iodine has the potential to cause stratospheric ozone depletion.  However, there is still significant uncertainty concerning the magnitude of its effect, ranging from a few percent to 10% based on the literature studies. Moreover, these studies have only considered that up to  0.77±0.10 per trillion by volume (pptv) total inorganic iodine is entrained into the stratosphere from the surface emissions. Recently the first 12U CubeSat using the iodine electric propulsion was launched in November 2021 into an orbit at ~480 km. The system produces iodine ions after vaporizing solid iodine. Thus the launch of nanosatellites using iodine propulsion will inject gas-phase iodine species into the thermosphere, which upon re-entering the atmosphere could potentially cause depletion of the ozone layer and consequently impact climate. 

Here we use the 3-D Whole Atmospheric Community Climate Model (WACCM) to investigate stratospheric ozone depletion due to the launch of small satellites (e.g., CubeSats) with an iodine propulsion system and understand the potential risks caused to stratospheric ozone . We have separted the contribution to the stratospheric ozone depletion from the surface emissions of Iodine and its injection from the upper atmosphere. We have performed a number of model sensitivity runs with different additional scenarios of iodine injection at 120-140 km to explore the potential  stratospheric ozone depletion from small satellites powered in this way. For the base case scenario in the current condition (for example year 2014), a steady-state nanosatellite launch rate of 20,000/year (e.g., 8 tons of I+ injected), the perturbation to the total column ozone is negligible. However, a 10 or 100-fold increase in the mass of iodine launched into near-Earth orbit will cause significant ozone depletion. This study quantifies the extent to which the injection of iodine into the thermosphere can deplete stratospheric ozone, which will be a useful guide for limiting the population of satellites with iodine propulsions systems in low Earth orbit. The impact of iodine for the extreme large ozone depletion years (for example, 2020)  and future scenarios of the results will be also discussed.

How to cite: Feng, W., Plane, J., Chipperfield, M., Saiz-Lopez, A., Booth, J.-P., McClory, S., and Kinnison, D.: Impact of iodine injections from the suface and the small satellites using iodine propulsion system in the upper atmosphere on ozone depletion, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3524, https://doi.org/10.5194/egusphere-egu23-3524, 2023.

EGU23-6381 | PICO | AS3.11

Halocarbon dynamics from Las Palmas to Guayaquil in winter 2021/2022 – Results of SO287-CONNECT 

Birgit Quack, Dennis Booge, Helmke Hepach, Elliot Atlas, Josefine Karnatz, Alexandra Rosa, Claudio Cardoso, Stephen Ball, Philippe Potin, and Rüdiger Röttgers

Short-lived bromo-, chloro- and iodocarbons from marine and anthropogenic sources contribute to the atmospheric halogen budgets and to ozone depletion in the troposphere and stratosphere. Their spatial variations are poorly known, given the sparse observations of marine and atmospheric concentrations. The distribution and air-sea fluxes of halocarbons need to be quantified in order to clarify the oceanic contributions to future tropospheric and stratospheric ozone chemistry.

Here we present the first marine and atmospheric halocarbon dataset from the research cruise SO287-CONNECT (Pan-Atlantic connectivity of marine biogeochemical and ecological processes and the impact of anthropogenic pressures). The transit of RV SONNE from Las Palmas, Spain (departure: 11.12.2021) to Guayaquil, Ecuador (arrival: 11.01.2022) was conducted to decipher the coupling of biogeochemical and ecological processes and their influence on atmospheric chemistry along the transport pathway of water from the upwelling zones off Africa into the Sargasso Sea and further to the Caribbean and the equatorial Pacific. A comprehensive work program, which combined continuous underway and station work, marine and atmospheric measurements and sampling with incubation experiments was conducted.

The distribution of short-lived halocarbons, e.g. bromoform (CHBr3), dibromomethane (CH2Br2), methyl iodide (CH3I), and trichloromethane (CHCl3) was highly dynamic in both ocean and atmosphere. We calculate the air-sea exchange of the compounds and relate physical and biological parameters to our observations. Among these are transport processes (e.g. long-range transport, eddies) and we show the varying composition of air and water masses and the potential sources of the compounds. For the first time, we estimate the contribution of the floating macroalgae Sargassum to halocarbon cycling around the North Atlantic gyre and in the Caribbean. The evaluation of the comprehensive data set collected during SO287-CONNECT improves our knowledge on the general role of the great Atlantic Sargassum belt and anthropogenic pollution in elemental biogeochemical cycles, as well as on trace gas exchange across the ocean-atmosphere interface.

How to cite: Quack, B., Booge, D., Hepach, H., Atlas, E., Karnatz, J., Rosa, A., Cardoso, C., Ball, S., Potin, P., and Röttgers, R.: Halocarbon dynamics from Las Palmas to Guayaquil in winter 2021/2022 – Results of SO287-CONNECT, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6381, https://doi.org/10.5194/egusphere-egu23-6381, 2023.

EGU23-6677 | ECS | PICO | AS3.11

Detection of chlorine, bromine and bromine chloride (BrCl) in volcanic emissions: Studies at Mt. Etna (Italy), 2022 

Bastien Geil, Niklas Karbach, Nicole Bobrowski, and Thorsten Hoffmann

Halogens in volcanic plumes are important for both volcanic and environmental research. For example, changes in the composition of the volcanic plume can be an indication of changes in the activity of the volcano. Volcanic emissions consist mainly of emitted H2O, CO2 and SO2 and are rapidly mixed with surrounding background atmosphere. Additionally, HF, HCl and HBr are also significant constituents of volcanic emissions.

A particularly interesting element in this context is bromine because of its atmospheric relevance. Among others BrO forms in the volcanic plume and, like SO2, can be determined spectroscopically using remote sensing techniques, making it ideal for monitoring and surveillance of volcanoes. However, to interpret and use BrO concentrations, we need to fully understand the formation and evolution of BrO in volcanic plumes. Measuring all relevant halogen species can take us one step further in our understanding of the interaction between atmosphere and volcanic gas and particle emissions.

Currently, several methods are used to detect the various halogen compounds. Remote sensing methods exist for only a few (in general BrO, OClO, HCl, HF). We use in-situ sampling methods such as diffusion separators, filter packs or aqueous alkaline traps to collect reactive and total halogen species, respectively.

In this study, we will present results for Cl2, Br2 and BrCl in volcanic plumes using AV based in situ measurement with cis-Stilbene coated syringe filters for halogens and interhalogens (i.e., Cl2 ,Br2 and BrCl). The results are discussed considering the different degassing activities and halogen chemistry in volcanic plumes.

How to cite: Geil, B., Karbach, N., Bobrowski, N., and Hoffmann, T.: Detection of chlorine, bromine and bromine chloride (BrCl) in volcanic emissions: Studies at Mt. Etna (Italy), 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6677, https://doi.org/10.5194/egusphere-egu23-6677, 2023.

EGU23-8392 | PICO | AS3.11

Molecular Dynamics Studies of Halogen Bonding on the Freezing in Clouds 

Cooper J. Yerby, Gabriel G. Bertho, Chongqin Zhu, and Joseph S. Francisco

The retention coefficients for halogen gases upon freezing of water are currently not estimated. Estimating their retention coefficients is an important metric, enabling atmospheric chemists and modelers to better approximate the respective influences and lifetimes of trace gasses in the atmosphere. Using molecular dynamic simulations that simulate the freezing of cloud water droplets containing halogen gasses in the upper troposphere (220°K), we have revealed that Cl2, Br2, and I2 are entirely retained when water droplets are frozen during deep convection. The results of the simulations show that the presence of halogen gasses in cloud droplets retards their freezing rates by approximately 35% to 62%.  Enumeration of hydrogen and halogen bonds formed between gas species and water in cloud droplets shows that substantially more halogen bonding than hydrogen bonding occurs among halogen gasses. Additionally, data indicates the size of halogen species within cloud droplets may affect their freezing rates. Our results provide a theoretical framework to make the first estimates regarding halogen gas retention coefficients, helping to elucidate impacts halogens may have on the gas transportation dynamics and chemistries of the upper troposphere and lower stratosphere (UTLS). As halogen gas emissions continue to increase globally, this study calls upon the emergent need to assess the role of halogen gasses in UTLS chemistry, especially in the deep convective regions.

How to cite: Yerby, C. J., Bertho, G. G., Zhu, C., and Francisco, J. S.: Molecular Dynamics Studies of Halogen Bonding on the Freezing in Clouds, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8392, https://doi.org/10.5194/egusphere-egu23-8392, 2023.

EGU23-9539 | PICO | AS3.11

Halogens as tracers for magma evolution from the mantle source to the atmosphere – insights from simultaneous probing of tephra fallout and gas phase in the volcanic plume 

Nicole Bobrowski, Johanna Beikert, Roman Botcharnikov, Stephan Buhre, Andre Butz, Christopher Fuchs, Bastien Geil, Giovanni Bruno Giuffrida, Jaro Heimann, Christoph Helo, Thorsten Hoffmann, Marvin Knapp, Stepan Krasheninnikov, Jonas Kuhn, Marco Liuzzo, Thomas Ludwig, Alexander Nies, Axel Schmitt, and Anne Sturm

Besides H2O, CO2 and sulphur, halogens (F, Cl, Br, I) are important volatile components in magmas. The extremely high chemical activity of halogens in melts and liquids leads to a significant influence on (a) magmatic properties, (b) the degassing of magma, (c) the extraction, transport and deposition of metals, (d) the chemistry of volcanic emissions and (e) the composition of the atmosphere. Indeed, their geochemical behaviour can be used as a key indicator of the genetic conditions and evolution of magma.

In July 2021 a joint interdisciplinary campaign of petrologists, chemists and atmospheric physicists took place at Mt Etna volcano, Italy. Due to the favourable volcanic activity at Mt Etna (frequent paroxystic activity characterized by lava fountaining) we were able to collect  a unique dataset of simultaneously sampled fresh tephra fallout, in-situ gas samples (multiGAS, alkaline traps, 1,3,5-Trimethoxybenzene impregnated denuders) and spectral data with remote sensing techniques (DOAS, FTS, IFPICS) of the volcanic plume. The halogen and sulphur content was analysed in the volcanic plume as well as in the melt inclusion and glasses of the deposits. Results of the various applied techniques are presented. They allow us a direct comparison of degassing signatures (e.g., Cl/F, Br/Cl, and S/Cl) from the pre-eruptive melt to the volcanic plume.

How to cite: Bobrowski, N., Beikert, J., Botcharnikov, R., Buhre, S., Butz, A., Fuchs, C., Geil, B., Giuffrida, G. B., Heimann, J., Helo, C., Hoffmann, T., Knapp, M., Krasheninnikov, S., Kuhn, J., Liuzzo, M., Ludwig, T., Nies, A., Schmitt, A., and Sturm, A.: Halogens as tracers for magma evolution from the mantle source to the atmosphere – insights from simultaneous probing of tephra fallout and gas phase in the volcanic plume, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9539, https://doi.org/10.5194/egusphere-egu23-9539, 2023.

EGU23-10599 | PICO | AS3.11

Atmospheric observation and source analysis of CFCs, HCFCs and HFCs at the Medog background site on the southern slope of the Himalayas, China 

Jing Wu, Zehua Liu, Bo Yao, Minde An, Yueyuan Niu, Wanglin Zhao, Haibo Yu, Tong Wang, Bingqi Dong, and Lin Peng

The ozone-depleting substances chlorofluorocarbons (CFCs), hydrochlorofluorocarbons (HCFCs) and their major substitutes hydrofluorocarbons (HFCs) are all potent greenhouse gases, and their atmospheric concentrations and emission sources have received international attention. The relevant studies have been carried out at multiple background sites around the world, but there is no report on the southern slope of the Himalayas. For the first time, this study set up the Medog background observation site 30 km away from Medog County on the southern slope of the Himalayas (95.5262ºE, 29.5314ºN, 1298.8 m above sea level) in China. From August 10 to September 19 and November 3 to November 30 in 2021, 114 atmospheric samples were collected instantaneously using evacuated electro-polished stainless-steel canisters and manual pressurization equipment and 1-3 samples were collected per day. Nine substances (CFC-11, 12, 113; HCFC-22, 141b, 142b; HFC-23, 125, 134a) were analyzed using a high-precision measurement system of halogenated gases (ODS5-pro). For each substance, all the atmospheric samples were divided into two categories: background samples and polluted samples. The background samples are those whose concentrations were within the range of the background concentrations (measured at the Ragged Point site at the same latitude in 2021) ± 3σ (instrument precision), and the others were classified as polluted samples. Our results showed that the number of the polluted samples of each substance accounted for about 40%-90%. In addition, we found that the mixing ratios of CFC-113, HFC-23, and HCFC-22 in the polluted samples were 93, 44 and 311 pptv, respectively, with higher mixing ratios (31.6%, 24.5%, and 22.5%) above the background levels than other substances (4.3%~10.2%). Furthermore, CFC-113 and HFC-23 were significantly correlated (R = 0.429, P < 0.01), suggesting that they may have similar sources. Both Backward Trajectory and Potential Source Contribution Function of the polluted samples of CFC-113, HFC-23, and HCFC-22 found that the polluted air masses mainly came from the northeast of India and other regions southwest of the sampling site. In contrast, the background air masses mainly came from the local areas. The concentrations of CFC-113, HFC-23, and HCFC-22 in the polluted samples observed in this study, likely from the northeast of India, were about 20-30% higher than the results of aircraft samples conducted by Say et al. (2019) over Northern and Southern India in 2016. In the future, we will continue to carry out atmospheric observations at the Medog background site and try to use the suitable atmospheric transport model to inverse the emissions in the surrounding areas.

How to cite: Wu, J., Liu, Z., Yao, B., An, M., Niu, Y., Zhao, W., Yu, H., Wang, T., Dong, B., and Peng, L.: Atmospheric observation and source analysis of CFCs, HCFCs and HFCs at the Medog background site on the southern slope of the Himalayas, China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10599, https://doi.org/10.5194/egusphere-egu23-10599, 2023.

The chlorine (Cl·) and bromine atom (Br·) are known to destroy ozone, and Br· accelerates the deposition of toxic mercury (Hg). However, their abundances, sources and impacts in polluted regions are not well understood. In this talk, we give an overview of recent measurements of significant levels of Cl2 and Br2— a producer of Cl· and Br·, respectively —in the coastal atmosphere of Hong Kong. We present field and laboratory evidence to show photodissociation of particulate nitrate being a major production pathway for daytime Cl2 and Br2 and reactive uptake of N2O5 on aerosols as an important nighttime source. Model-calculated and Cl· and Br· from these di-halogens have significant impacts on VOC oxidation, OH radical, ozone production, and Hg oxidation. The findings suggest that reactive halogens may play a larger role in the atmospheric chemistry and air quality of polluted coastal regions than previously thought and call for more research on this issue.

How to cite: Wang, T. and the study team: Pollution-derived Cl2 and Br2 boost oxidation power of the coastal atmosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11587, https://doi.org/10.5194/egusphere-egu23-11587, 2023.

EGU23-11859 | ECS | PICO | AS3.11

Investigation of weather conditions and BrO during ozone depletion events between 2010 and 2021 in Ny-Ålesund 

Bianca Zilker, Andreas Richter, Anne-Marlene Blechschmidt, Ilias Bougoudis, Sora Seo, Peter von der Gathen, Tim Bösch, and John P. Burrows

Ozone Depletion Events (ODEs) have been observed since the late 1990s in the polar regions during spring, often in combination with Bromine Explosion Events (BEEs). In a heterogeneous, autocatalytic, chemical chain reaction cycle, inorganic bromine is released from the cryosphere into the troposphere and depletes ozone, sometimes to below detection limit. Besides low temperatures favoring the bromine explosion reactions, two different meteorological conditions are mainly observed during these events: on the one hand, low wind speeds and a stable boundary layer, where bromine can accumulate and deplete ozone, and on the other hand, high wind speeds above approximately 10 m/s with blowing snow and a higher, unstable boundary layer. The second condition often occurs in combination with polar cyclones, where bromine can be recycled aloft on snow and aerosol surfaces.

In this study, two long term ozone data sets, one from ozone sondes launched in Ny-Ålesund and the other from in-situ measurements on Zeppelin mountain – located close to Ny-Ålesund – have been evaluated from March until May between 2010 and 2021 to detect ODEs. To analyze the prevailing weather conditions during these events, ERA5 reanalysis data has been used and separated between weather conditions during ODEs and no-ODEs based on the respective ozone data set. The evaluation of the two data sets led to very consistent results: during ODEs, lower pressure is observed east of Svalbard and higher pressure over Greenland, leading to a transport of cold polar air from the north to Ny-Ålesund. Also higher wind speed and a higher boundary layer are noticed, supporting the assumption, that ODEs often occur in combination with polar cyclones.

Using the same approach, the long-term tropospheric BrO data set from Bougoudis et al., 2020 in combination with S5P TROPOMI retrievals of tropospheric BrO has been used to analyze BrO patterns. During ODEs in Ny-Ålesund, the satellite data show elevated values all over the Arctic, but especially north of Svalbard.

 

This work was supported by the DFG funded Transregio-project TR 172 “Arctic Amplification (AC)³“ in subproject C03.

How to cite: Zilker, B., Richter, A., Blechschmidt, A.-M., Bougoudis, I., Seo, S., von der Gathen, P., Bösch, T., and Burrows, J. P.: Investigation of weather conditions and BrO during ozone depletion events between 2010 and 2021 in Ny-Ålesund, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11859, https://doi.org/10.5194/egusphere-egu23-11859, 2023.

EGU23-11887 | ECS | PICO | AS3.11

Tropospheric BrO in Arctic Spring 2019 measured by S5-P/TROPOMI - A statistical analysis of the spatial expansion and shape of tropospheric BrO plumes 

Moritz Schöne, Holger Sihler, Simon Warnach, Christian Borger, Maximilian Herrmann, Eva Gutheil, Steffen Beirle, Ulrich Platt, and Thomas Wagner

Halogen radicals can drastically alter the atmospheric chemistry. In the polar regions, this is made evident by the ozone depletion in the stratosphere (ozone hole) but also by destruction of boundary layer ozone during polar springs. These recurrent episodes of catalytic ozone depletion, better known as “ozone depletion events” (ODEs) are driven by enhanced concentrations of reactive bromine compounds. The proposed mechanism by which these compounds are released into the troposphere is known as “bromine explosion” - reactive bromine is formed autocatalytically from the condensed phase.

In comparison to previous satellite missions, the TROPOspheric Monitoring Instrument (TROPOMI) onboard ESA’s S5-P satellite allows an improved localization and a more precise specification of these events due to its superior spatial resolution of up to 3.5 x 5.5 km2. Together with the better than daily coverage over the polar regions, this allows for investigations of the spatio-temporal variability of enhanced BrO levels and their relation to different possible bromine sources and release mechanisms.

We present tropospheric BrO column densities retrieved from TROPOMI measurements using Differential Optical Absorption Spectroscopy (DOAS). One advantage of our retrieval is its independence from any external input data, thereby avoiding systematic biases from external datasets. We used a modified k-means clustering and methods from statistical data analysis to separate tropospheric and stratospheric partial columns, relying only on NO2 and O3 columns measured by the same instrument. This ensures in particular that the derived tropospheric BrO data set keeps the same high spatial resolution as the TROPOMI instrument, because no model data with coarse resolution is used. In a second step, the retrieved tropospheric slant column densities (SCDs) are converted to vertical column densities (VCDs).

TROPOMI’s improved spatial resolution is then utilized to study the spatial extent and shape of BrO plumes detected in the Arctic region. For this, a combination of morphological filters and connected component labeling is used to provide a statistical overview of all enhanced BrO plumes detected above certain sensitivity thresholds in the Arctic spring of 2019. This provides a lower limit for the spatial extent of enhanced BrO events (and hence also for ODEs) of around 40-60 km. Additionally, seasonal trends in size and shape of the BrO plumes as well as correlations to relevant meteorological parameters are investigated.

How to cite: Schöne, M., Sihler, H., Warnach, S., Borger, C., Herrmann, M., Gutheil, E., Beirle, S., Platt, U., and Wagner, T.: Tropospheric BrO in Arctic Spring 2019 measured by S5-P/TROPOMI - A statistical analysis of the spatial expansion and shape of tropospheric BrO plumes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11887, https://doi.org/10.5194/egusphere-egu23-11887, 2023.

EGU23-12225 | ECS | PICO | AS3.11

Global and regional marine bromoform emissions in a fully coupled ocean-atmosphere-model 

Dennis Booge, Jerry Tjiputra, Dirk Olivié, Birgit Quack, Michael Schulz, and Kirstin Krüger

Bromoform (CHBr3) is one of the most important precursors of atmospheric reactive bromine with an atmospheric lifetime of ~20 days. Natural production, being the main source of oceanic CHBr3, is high at the coasts and in open ocean upwelling regions due to production by macroalgae and phytoplankton. Although highly relevant for the future halogen burden and ozone layer in the stratosphere, the global bromoform production in the ocean and their emissions are still poorly constrained in observations and are mostly neglected in Earth System Model (ESM) climate projections.

Here, we show first model results of fully coupled ocean-atmosphere bromoform interactions in the Norwegian ESM (NorESM) with the ocean model BLOM and the ocean biogeochemistry component iHAMOCC for the CMIP6 historical period from 1850 to 2014.

Our results are validated using oceanic and atmospheric measurements listed in the HalOcAt (Halocarbons in the Ocean and Atmosphere) data base and show an overall good agreement with those observations in open ocean regions. The NorESM open ocean emissions of CHBr3 are higher than previously published emission estimates from bottom-up approaches. Moreover, the emissions are mainly positive (sea-to-air fluxes) driven by the oceanic production, sea surface temperature and wind speed, dependent on season and location. However, during low-productive winter seasons, model results also show local negative fluxes (air-to-sea fluxes) in high latitudes, suggesting some oceanic regions to be a sink of atmospheric bromoform. Driving factors will be shown for different case studies, e.g. the tropical West Pacific, which is a hot spot for oceanic bromine delivery to the stratosphere.

How to cite: Booge, D., Tjiputra, J., Olivié, D., Quack, B., Schulz, M., and Krüger, K.: Global and regional marine bromoform emissions in a fully coupled ocean-atmosphere-model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12225, https://doi.org/10.5194/egusphere-egu23-12225, 2023.

EGU23-12850 | PICO | AS3.11

The effect of Natural Halogens on Tropospheric Ozone Chemistry in the Pre-Industrial vs Present-Day 

Javier A. Barrera, Douglas E. Kinnison, Rafael P. Fernandez, Jean-François Lamarque, Carlos A. Cuevas, Simone Tilmes, and Alfonso Saiz-Lopez

Halogens (I, Br and Cl) emitted from natural sources catalytically destroy a fraction of tropospheric ozone, a trace gas that plays a key role in atmospheric chemistry, both as a greenhouse gas and as a component of photochemical smog, affecting air quality and public health. Previous studies have explored the effect of halogens on ozone in present-day (PD) and future time, while the role of halogens in pre-industrial (PI) ambient conditions is quite uncertain. We use the Community Atmospheric Model with Chemistry (CAM˗Chem) to explore the effect of both natural sources and chemistry of halogens on tropospheric ozone in the PI and PD. The model results show that natural halogens have comparatively a larger impact on ozone under less polluted atmospheric conditions, with percentage changes in tropospheric ozone burden (TOB) of ˗14% for PI and ˗13% for PD. Individually, the role of iodine in ozone destruction is equivalent in both periods (ΔTOBI: ˗7%). Bromine plays a larger role in PI (ΔTOBBr: ˗5%) vs. PD (ΔTOBBr: ˗4%), while chlorine plays a larger role in PD (ΔTOBCl: ˗2.5% vs. ˗2%). The increase in anthropogenic ozone precursor emissions from PI to PD drives an enhancement in the inorganic halogen budget, as well as a change in the partitioning of inorganic halogens, shifting from reactive (X+XO, X= I, Br or Cl) to reservoirs (e.g. HOX and XONO2) species. Consequently, model results show that the halogen-mediated ozone depletion in the global lower troposphere is higher in PI than in PD. This study highlights the importance of including a complete chemical representation of natural halogens in chemistry-climate models to adequately assess their effects on tropospheric ozone in a changing climate

How to cite: Barrera, J. A., Kinnison, D. E., Fernandez, R. P., Lamarque, J.-F., Cuevas, C. A., Tilmes, S., and Saiz-Lopez, A.: The effect of Natural Halogens on Tropospheric Ozone Chemistry in the Pre-Industrial vs Present-Day, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12850, https://doi.org/10.5194/egusphere-egu23-12850, 2023.

EGU23-14999 | PICO | AS3.11

Interactions between natural short-lived halogens and atmospheric oxidation capacity 

Rafael Fernandez, Qinyi Li, Carlos Cuevas, Xiao Fu, Douglass Kinnison, Simone Tilmes, Anoop Mahajan, Juan Carlos Gomez-Martin, Fernando Iglesias-Suarez, Ryan Hossaini, John Plane, Gunnar Myhre, Jean-Francoise Lamarque, and Alfonso Saiz-Lopez

Observational evidence shows the ubiquitous presence of short-lived halogens in the global atmosphere. This includes the biogenic contribution of organic very short-lived halocarbons as well as the abiotic source of inorganic halogens throughout heterogeneous recycling. All of these species are naturally emitted from the oceans, polar ice, and the biosphere, presenting a pronounced spatio-temporal source strength that controls the regional, vertical and seasonal distribution in the troposphere. In addition, anthropogenic emissions of reactive halogens, both organic and inorganic, have been identified in the atmosphere. Most notably, short-lived halogen emissions influence the oxidative capacity of the troposphere and consequently the concentration of ozone and methane. In this communication, we use the halogen version of CAM-Chem to evaluate how these interactions evolve across pre-industrial, present-day, and future climates under different halogen emission scenarios.

How to cite: Fernandez, R., Li, Q., Cuevas, C., Fu, X., Kinnison, D., Tilmes, S., Mahajan, A., Gomez-Martin, J. C., Iglesias-Suarez, F., Hossaini, R., Plane, J., Myhre, G., Lamarque, J.-F., and Saiz-Lopez, A.: Interactions between natural short-lived halogens and atmospheric oxidation capacity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14999, https://doi.org/10.5194/egusphere-egu23-14999, 2023.

EGU23-15972 | PICO | AS3.11

Substantial contribution of iodine to Arctic ozone destruction 

Carlos A. Cuevas, Nuria Benavent, Anoop S. Mahajan, Qinyi Li, Julia Schmale, Hélène Angot , Tuija Jokinen, Lauriane L. J. Quéléver, Anne-Marlene Blechschmidt, Bianca Zilker, Andreas Richter, Jesus A. Serna, David Garcia-Nieto, Rafael P. Fernandez, Henrik Skov, Adela Dumitrascu, Patric Simões Pereira, Katarina Abrahamsson, Silvia Bucci, and Marina Duetsch  and the MOSAiC iodine Team

While the importance of bromine chemistry for the Arctic surface ozone budget is well documented, the effect of iodine chemistry has received less attention. Here we present observations performed as part of the ship-based Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition, where halogen oxides were measured during the sunlit period from March to October 2020. Ozone shows drastic loss during the boreal spring (March, April and May), when near-complete depletion is regularly observed, highlighting that ozone depletion in the central Arctic is widespread. The drastic ozone depletion coincides with ‘bromine explosion’ episodes, when bromine oxide (BrO) reaches values as high as 14.8±0.8pptv. In contrast, observations of IO show the presence of active iodine chemistry on most days during the whole sunlit period (including boreal spring, summer and autumn), presenting elevated levels of IO (usually between 0.2 and 1 pptv) that peak during spring (2.9±0.3 pptv). We find that chemical reactions between iodine and ozone are the second highest contributor to ozone loss over the study period, after ozone photolysis-initiated loss and ahead of bromine.

How to cite: Cuevas, C. A., Benavent, N., Mahajan, A. S., Li, Q., Schmale, J., Angot , H., Jokinen, T., Quéléver, L. L. J., Blechschmidt, A.-M., Zilker, B., Richter, A., Serna, J. A., Garcia-Nieto, D., Fernandez, R. P., Skov, H., Dumitrascu, A., Simões Pereira, P., Abrahamsson, K., Bucci, S., and Duetsch , M. and the MOSAiC iodine Team: Substantial contribution of iodine to Arctic ozone destruction, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15972, https://doi.org/10.5194/egusphere-egu23-15972, 2023.

EGU23-16987 | PICO | AS3.11

Study of ambient halocarbons in Hong Kong: temporal variability and implication on source origins 

Dasa Gu, Xiangyunong Cao, and Ka Fung Leung

Halocarbons have been recognized for their role as major ozone-depleting substances (ODSs) since the 1970s, and some also function as greenhouse gases (GHGs). International agreements, such as the Montreal Protocol, Kyoto Protocol, and Paris Agreement, were established for worldwide cooperation to gradually reduce the production and use of halocarbons. Initial success was achieved in phasing out global chlorofluorocarbon (CFC) production, but recent studies found an unexpected decrease in the rate of decline in the atmospheric concentration of trichlorofluoromethane (CFC-11) after 2012.

Historically, halocarbons have been emitted from various anthropogenic sources (e.g., the dry cleaning industry, electronic industry, and refrigeration) in Hong Kong. Emission sources in the Pearl River Delta (PRD) region, such as chemical manufacturing, also have remarkable impacts on the ambient halocarbons in Hong Kong. The ambient mixing ratios of major CFCs were declining in Hong Kong and the PRD region before 2010. However, no continuous measurements of ambient halocarbons were conducted in Hong Kong after 2010. Given that CFC emissions from the PRD region account for up to 25% of their total emissions in China, any unexpected CFC emissions in recent years will have significant impacts on the atmospheric abundance of halocarbons worldwide.

We have been continuously monitoring ambient halocarbons in Hong Kong since Fall 2020. The temporal variability of major halocarbons and their source origins have been extensively investigated using multiple approaches. Our results indicate lower enhancements beyond the background values for major regulated CFCs and CCl4 than later controlled HCFCs and HFCs, suggesting the greater progress of Montreal Protocol implementation for the former species. The notable high enhancement values of non-regulated halocarbons from the north direction indicate their widespread usage in China. This work provides insight into the progress made in implementing the Montreal Protocol in Hong Kong and the surrounding region and the importance of continuous emission control.

How to cite: Gu, D., Cao, X., and Leung, K. F.: Study of ambient halocarbons in Hong Kong: temporal variability and implication on source origins, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16987, https://doi.org/10.5194/egusphere-egu23-16987, 2023.

Abstract: Greenhouse gases and associated pollutants (CO, NOx, VOCs, aerosols) are measured from a small airplane, mobile laboratory, and towers.  Through mass balance calculations and comparison to numerical models such as CMAQ-GHG  we estimate the total flux from the cities of Baltimore, MD and Washington, DC.  Emissions inventories were found to underestimate methane emissions substantially and have been improved.  Major sources include leakage in the natural gas delivery system and biogenic processes including landfills.  Measurements with high spatial and temporal resolution reveal hot spots of high concentrations often associated with pollutants such as black carbon (BC) and NO2 that pose a health hazard in disadvantaged communities. 

How to cite: Dickerson, R., Ren, X., and Karion, A.: "Measurements and models of GHGs and short-lived pollutants in the Baltimore/Washington area: Emissions and environmental justice", EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-121, https://doi.org/10.5194/egusphere-egu23-121, 2023.

EGU23-508 | ECS | Posters on site | AS3.12

Sources of Methane Emissions in the Urban Atmosphere - Case Study: Cluj-Napoca City 

Mustafa Hmoudah, Calin Baciu, and Cristi Pop

Methane is considered to be the second largest contributor to the greenhouse effect after CO2, with a higher increase of its atmospheric concentration over the industrial era compared to other greenhouse gases, as CO2 or nitrous oxide. At least 50% of CH4 emissions come from anthropogenic activities in urban and rural areas, due to the combustion of fossil fuels, waste and wastewater treatment, leaks from the natural gas distribution system, etc.

Although, CH4 is more than 20 times more potent than CO2 in producing the greenhouse effect, it has a short residence time in the atmosphere, which makes the mitigation measures more effective in minimizing these emissions and bringing a short-term advantage to the climate.

Methane concentrations were determined at street-level in the city center, commercial area, residential area, and green area of Cluj-Napoca, Romania. A portable West Systems fluxmeter was used. The instrument is based on Tunable Diode Laser Absorption Spectroscopy, that allows high precision measurements and very low detection limit, of 0.1 ppm.  By eliminating wind effects at street-level, the residential area recorded the least values of these emissions, around the CH4 average atmospheric concentration. Similarly, the emissions in the commercial area were fluctuating around same atmospheric concentration average, but strongly depending on the traffic density. On the sidewalk, at about 1.3 m height, the recorded methane concentrations ranged between 1.9 and 6.0 ppm. The highest values occurred at the passage of heavy vehicles as trucks.

Concentrations of tens or even hundreds ppm CH4 were measured close to the drains that collect water run-off from the streets, and even higher at manhole covers of the sanitary sewerage system.

However, the outcomes of this study indicate the need for further investigation of CH4 emissions in the urban area and the importance of the isotopic characterization of these emissions in order to identify their sources for prioritizing the CH4 mitigation measures.

 

How to cite: Hmoudah, M., Baciu, C., and Pop, C.: Sources of Methane Emissions in the Urban Atmosphere - Case Study: Cluj-Napoca City, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-508, https://doi.org/10.5194/egusphere-egu23-508, 2023.

EGU23-1141 | ECS | Posters on site | AS3.12

Fugitive Methane Detection from UK Above Ground Gas Infrastructure 

Aliah Al-Shalan, Dave Lowry, Rebecca Fisher, James France, Julianne Fernandez, and Mathias Lanoiselle

Methane is a powerful greenhouse gas with a globally averaged atmospheric mole fraction of 1908±2 ppb in 2021, nearly three times the pre-industrial abundance. The annual increase of methane between 2020 and 2021 was the highest since continuous measurement began (WMO,2022).  More than 60% of global CH4 emissions are attributed to human activities. Reducing methane in the short term will help to achieve the Paris Agreement goal to keep warming to <1.5°C and help in reaching many Sustainable Development Goals due to multiple co-benefits of methane mitigation. The fossil fuel sector is one of the largest anthropogenic emitters of methane and a target for CH4 reductions, with the UN stating that an emissions reduction of 61% is possible, but there is now urgent need to implement this (Nisbet et al, 2019).

Sources of fugitive methane emissions in the UK have been identified and characterized by mobile measurement survey in vehicles (e.g. Lowry et al ,2020) and aircraft (e.g. France et al., 2021). Since 2017, vehicles surveys for UN and NERC-UK projects have identified emissions from production platforms, onshore terminals, compressor stations, offtake stations, gas governors and pipeline failures.

Vehicle surveys utilized different suites of instruments: Picarro G2301 and G2210-i Los Gatos Research Ultraportable Methane-Ethane (LGR UMEA), and LiCor 7810 GHG analyzers, all measuring methane. Air bags were filled in plumes during surveys to measure the carbon isotopic signature (δ13C) at different points in the gas distribution supply chain. The range of signatures identified is from -43.7 to -32.4 ‰ (n=182), showing an enrichment relative to atmospheric background (-48 to -47.5‰), with the southern North Sea production that feeds into the Bacton Terminal identified as the most enriched at -31.8 ±1.5‰ (n=13).

Ethane:methane ratio is a useful diagnostic for gas attribution. Since 2018 the LGR UMEA ethane data has been used to identify distribution leaks as this gas is not a component of waste, agricultural or coal sources. The ratio of C2H6:CH4 (C2:C1) during surveys of gas allows separation of pyrogenic and thermogenic (>0.03) from biogenic (<0.005) sources (Rella et al, 2015: Lowry et al, 2020), with UK gas distribution dominantly in the range 0.04 to 0.08, and it is consistent for fugitive plumes transected on multiple passes.

Most of the larger peaks have been located downwind of offtake stations on the high-pressure mains network. The 2021 surveys focused on identification of emitting facilities and their isotopic and C2:C1 characterization. Recent surveys in 2022 targeted emission plumes for multiple passes with 10Hz and 1Hz instruments to select suitable candidates for Gaussian plume emission modelling, with potential to upscale to a national emission for facilities of this category.

 

France et al., 2021, Atmos. Meas. Tech., 14, 71–88, 10.5194/amt-14-71-2021

Lowry et al., 2020, Science of the Total Environ., 708, 134600, 10.1016/j.scitotenv.2019.134600

Nisbet et al., 2019., Global Biogeochem. Cycles, 33, 25pp, 10.1029/2018GB006009 

Rella et al., 2015., Atmos. Meas. Tech., 8, 4539–4559, 10.5194/amt-8-4539-2015.

World Meteorological Organisation, 2022. (WMO) greenhouse gas bulletin. [Online]. Available at: https://public.wmo.int/en/resources/library/wmo-greenhouse-gas-bulletin. (Accessed 9 December 2022)

How to cite: Al-Shalan, A., Lowry, D., Fisher, R., France, J., Fernandez, J., and Lanoiselle, M.: Fugitive Methane Detection from UK Above Ground Gas Infrastructure, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1141, https://doi.org/10.5194/egusphere-egu23-1141, 2023.

EGU23-1261 | Orals | AS3.12

Variability of methane fluxes at the Ebro Delta due to rice field: comparison between inventories and Radon Tracer Method based results. 

Roger Curcoll, Josep-Anton Morguí, Alba Àgueda, Arturo Vargas, and Claudia Grossi

The Ebro River Delta, in the northwestern Mediterranean basin, has an extension of 320 km2 and is mainly covered by rice fields. Rice fields are known to be one of the main sources of anthropogenic methane emissions, and a better estimation of its temporal variability in relation to the different rice cultivation phases is important to help with the implementation of emission reduction strategies (Àgueda et al., 2017),

In the framework of the ClimaDat network, an atmospheric station was installed in the middle of the Ebro Delta in 2012. A Picarro G2301 for greenhouse gases (GHG) atmospheric concentrations and an ARMON (Atmospheric Radon Monitor) for atmospheric 222Rn concentrations were collocated among other instruments. Nocturnal hourly atmospheric observations of CH4 and 222Rn measured between 2013 and 2019 were used to apply the Radon Tracer Method (RTM) for retrieving CH4 fluxes over the footprint area.

The Ebro River Delta has a reduced dimension and a complex meteorological regime highly influenced by the Ebro channelled winds and the sea breezes, making it difficult to calculate GHG fluxes using global or regional inversion models. However, the use of high-resolution backtrajectories (model WRF-Flexpart) coupled with the traceRadon daily radon flux maps for Europe (Karsten et al., 2022), with a resolution of 0.05 degrees, has allowed the use of the RTM in this complex area.

Methane fluxes estimated by RTM were compared with fluxes directly measured with chambers in past studies (Martínez-Eixarch et al., 2018) and with data obtained by the EDGAR inventory (Crippa et al., 2022). Results show a promising agreement between methane fluxes obtained with different methods, and a variability clearly governed by the rice crop cycle which is not reflected in the methane emissions values reported in EDGAR inventories.

References

Àgueda, A., Grossi, C., Pastor, E., Rioja, E., Sánchez-García, L., Batet, Ò., Curcoll, R., Ealo, M., Nofuentes, M., Occhipinti, P., Rodó, X. and Morguí, J.-A.: Temporal and spatial variability of ground level atmospheric methane concentrations in the Ebro River Delta, Atmos. Pollut. Res., 8(4), 741–753, doi:10.1016/j.apr.2017.01.009, 2017.

Crippa, M., Guizzardi, D., Banja, M., Solazzo, E., Muntean, M., Schaaf, E., Pagani, F., Monforti-Ferrario, F., Olivier, J., Quadrelli, R., Risquez Martin, A., Taghavi-Moharamli, P., Grassi, G., Rossi, S., Jacome Felix Oom, D., Branco, A., San-Miguel-Ayanz, J. and Vignati, E., CO2 emissions of all world countries - 2022 Report, EUR 31182 EN, Publications Office of the European Union, Luxembourg, 2022, doi:10.2760/730164, JRC130363

Karstens, U., Levin, I. (2022). traceRadon monthly radon flux map for Europe 2006-2022 (based on ERA5-Land soil moisture), Miscellaneous, https://hdl.handle.net/11676/XPxf8v5gfDWmi6BZ597euAJ7

Martínez-Eixarch, M., Alcaraz, C., Viñas, M., Noguerol, J., Aranda, X., Prenafeta-Boldu, F. X., Saldaña-De la Vega, J. A., del Mar Catala, M. and Ibáñez, C.: Neglecting the fallow season can significantly underestimate annual methane emissions in Mediterranean rice fields, PLoS One, 13(5), doi:10.1371/journal.pone.0198081, 2018.

How to cite: Curcoll, R., Morguí, J.-A., Àgueda, A., Vargas, A., and Grossi, C.: Variability of methane fluxes at the Ebro Delta due to rice field: comparison between inventories and Radon Tracer Method based results., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1261, https://doi.org/10.5194/egusphere-egu23-1261, 2023.

EGU23-2237 | ECS | Posters on site | AS3.12

A view of 3D variability of atmospheric methane over India using  MIROC4-ACTM simulations 

Deep shikha, Sagnik Dey, and Prabir K. Patra

In this study, we examine a maximum of 13 years (2009-2021) of the observational datasets of columnar dry-air mole fractions of methane (XCH4), from the Greenhouse gases Observation SATellite (GOSAT) GOSAT-1 (2009-2021) on board the IBUKI satellite and vertical profiles of CH4 from the Atmospheric Infrared Sounder (AIRS) on board AQUA satellite. We also use the XCH4 and vertical distributions over the Indian subcontinent from the JAMSTEC’s MIROC4 atmospheric chemistry transport model (ACTM) from 2009-2021, after convolution with GOSAT-1 and AIRS a priori profiles and averaging kernels. 

A comparison of observed and modeled CH4 and XCH4 reveals that MIROC4-ACTM provides explicit insights into the spatio-temporal variability of atmospheric methane over the Indian region. Global CH4  emission inventory EDGARv7.0 reports a total of ~30 Mt of anthropogenic emissions in India in 2020 while GAINS emissions stand at ~33Mt for the same year. The ACTM simulations from this study are also examined to retrieve preliminary information on the quality of these constructed bottom-up fluxes of methane (EDGAR and GAINS).      

Our time series analysis of GOSAT-1 shows the annual mean XCH4 has increased by 100 ppb from 2009 to 2021 over the Indian subcontinent, compared to 85 ppb globally in the latitude band of 6.25 °N-41.25 °N. Observations from both AIRS and GOSAT-1 show distinct seasonality in the vertical profiles of CH4 and XCH4 over the entire region, respectively. Seasonality in the CH4  concentration over India in boundary layer heights (>850 hPa) is affected majorly by the local emission strengths while in the middle (400- 600 hPa) and upper (< 200 hPa) troposphere it is governed by the convective transport of surface emissions signals and redistribution in the monsoon winds in the upper troposphere. GOSAT-1 shows highest XCH4 of ~1900 ppb (2021) in northern India (North of 20° N) in winter season  (November) while AIRS shows highest CH4 ~1910 ppb in summer month of May at 200 hPa for the same year. Based on the findings from the vertical (AIRS) and total column (GOSAT-1) distribution of CH4, our analysis suggests that 3D variability of CH4 over the entire Indian region is governed by a diverse spread of surface emissions and global monsoon divergent wind circulations.  

Through this study, the reasons for these observed patterns of CH4 are explored in light of forward model results using an ACTM by combining and comparing the strengths of AIRS and GOSAT-1.

How to cite: shikha, D., Dey, S., and K. Patra, P.: A view of 3D variability of atmospheric methane over India using  MIROC4-ACTM simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2237, https://doi.org/10.5194/egusphere-egu23-2237, 2023.

EGU23-2304 | Orals | AS3.12

Insights on methane emissions using GHGSat’s constellation 

Mathias Strupler, Marianne Girard, Dylan Jervis, Jean-Phillipe MacLean, David Marshall, Jason McKeever, Antoine Ramier, and David Young

In May 2022, GHGSat added 3 satellites to its growing methane monitoring constellation, bringing the total to 5 commercial satellites now in operation. Each satellite has a detection threshold of about 100 kg/h and a 25 meters spatial resolution, enabling them to attribute industrial emissions to individual facilities. With its constellation, GHGSat can measure any site in the world with a repeatable methodology multiple times per year, giving a unique view of localized methane emissions on a global scale.

This presentation will focus on the insights that can be obtained from aggregate industrial methane emissions data measured by the GHGSat constellation. Example use cases ranging from local to global monitoring will be presented. In addition, we will discuss the constellation’s imaging capabilities and current methane measurement accuracy. Finally, an update on the next phase of the constellation will be given.

How to cite: Strupler, M., Girard, M., Jervis, D., MacLean, J.-P., Marshall, D., McKeever, J., Ramier, A., and Young, D.: Insights on methane emissions using GHGSat’s constellation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2304, https://doi.org/10.5194/egusphere-egu23-2304, 2023.

EGU23-4716 | ECS | Posters on site | AS3.12

Supporting Methane Mitigation Efforts by Improving Urban-scale Methane Emission Estimates in Melbourne, Australia. Part 1: Modelling 

Nasimeh Shahrokhi, Cathy M. Trudinger, Peter J. Rayner, Zoe M. Loh, Ann R. Stavert, Paul B. Krummel, Paul J. Fraser, David M. Etheridge, Bronwyn L. Dunse, Ashok Luhar, and Steven Thomas

This study establishes a regional inverse framework to refine methane (CH4) emission inventories for Melbourne, Australia. Methane is a long-lived greenhouse gas and the second most significant contributor to radiative forcing from greenhouse gases after carbon dioxide. Improved understanding of methane emissions from different sectors in Australia is necessary to focus and prioritise mitigation efforts and to track progress towards emissions reduction; however, methane emissions are uncertain, especially at fine resolution (urban and regional scales) needed for mitigation. Moreover, improving predictions of atmospheric methane mole fractions requires precise and accurate emission estimates; However, previous studies indicate a mismatch between current emission estimates and atmospheric observations.

Here, we use a combination of surface atmospheric measurements of methane and an inversion approach based on Bayes’ theorem to improve urban-scale methane emission estimates for Melbourne, Australia. Our inversion system is a Python-based four-dimensional variational (Py4DVar) data assimilation system. Due to lack of local methane inventories, prior emission estimates for Melbourne are compiled from globally-accessible datasets, including (1) anthropogenic emissions from the Emissions Database for Global Atmospheric Research (EDGAR), (2) fire emissions from the Global Fire Assimilation System (GFAS) dataset and (3) biogenic emissions from the Model of Emissions of Gases and Aerosols from Nature (MEGAN). Boundary condition adjustments are made using Kennaook/Cape Grim continuous in-situ CH4 mole fraction measurements and the Whole Atmosphere Community Climate Model (WACCM) dataset. The boundary condition adjustments are necessary to develop the efficiency of the regional inversion. The main goal of our inversion system is to provide more precise estimates of regional methane emissions. Independent satellite measurement comparisons are used to assess the system.

The comparison with assimilated data shows improvements in modelling methane mole fraction at the suburban Aspendale site with a bias reduction from ~70 ppb (prior) to ~3 ppb (posterior). Our detailed investigations indicate that although the prior results in a reasonable match of modelled mole fraction with observations, the EDGAR dataset does not provide a realistic spatial pattern for the main anthropogenic sources (enteric fermentation and landfills) around Melbourne. The possibility of improving the spatial distribution of the prior emissions has been tested using available local/global datasets, including national maps of livestock and landfills. Eventually, to obtain more comprehensive improved emission inventories in Melbourne, more CH4 mole fraction observational data are required in this area. The results of this study are being used to expand the methane monitoring network for Melbourne.

How to cite: Shahrokhi, N., Trudinger, C. M., Rayner, P. J., Loh, Z. M., Stavert, A. R., Krummel, P. B., Fraser, P. J., Etheridge, D. M., Dunse, B. L., Luhar, A., and Thomas, S.: Supporting Methane Mitigation Efforts by Improving Urban-scale Methane Emission Estimates in Melbourne, Australia. Part 1: Modelling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4716, https://doi.org/10.5194/egusphere-egu23-4716, 2023.

EGU23-5036 | ECS | Posters on site | AS3.12

Chinese Coal Mines Methane Emissions Constrained by High-Frequency Measurements 

Wei Hu, Kai Qin, Qin He, and Jason Blake Cohen

Methane’s high Global Warming Potential (GWP) and short atmospheric life relative to carbon dioxide have led to methane mitigation as a cost-effective and realistic near-term action that serves as a bridge to longer-term mitigation options. This paper calculated coal mine methane (CMM) emissions from 636 individual coal mines in Shanxi Province based on the Intergovernmental Panel on Climate Change (IPCC) Tier 2 approach. 5 sets of emission factors were used to compile this bottom-up inventory. Each coal mine is classified into 3 different coal mine gas ranks based on the method issued by the National Coal Mine Safety Administration and the National Energy Administration. Haft-hourly eddy-covariance measurements of methane flux from 1 mine (xhv) over a 5-month period were used to quantify and constrain the high-frequency variation in emissions. From the perspective of probability density, 15.5% of the total data is covered by the boxes overlapping the different bottom-up emissions estimates, while 53.5% of the total data falls in the single box below the floor of the bottom-up measurements. The in-situ measurements offer scaling factors (RATIO correction) for updating the preliminary bottom-up coal mine methane emissions datasets. A statistical approach is applied to individual coal mines by grouping them by coal mine gas rank. From the perspective of cumulative probability, the CMM flux shows a pattern that low gas rank < high gas rank < outburst rank. We have compared the CMM emissions with EDGAR-COAL and GFEI. In 2019, the EDGAR and GFEI inventory results show that methane emissions from coal mines in Shanxi Province are 7.27 Tg and 6.29 Tg, respectively. Our results range from 4.41-7.63 Tg. In Changzhi city, over the region in which this dataset has emissions that EDGAR-COAL and GFEI do not identify the emissions are [44.35,125.60,354.02] and [398.22,1125.81,3185.22] with the unit in ug (m-2 s-1), respectively. The values in brackets are results after RATIO correction, corresponding to cumulative percentages 30, 50 and 70 respectively. Over the region that EDGAR-COAL has misidentified coal mines, the emissions are 128.27 ug (m-2 s-1). Over the region that EDGAR and our inventory both have emissions, the EDGAR-COAL emissions are 357.65 ug (m-2 s-1), while our emissions are about 353.87 ug (m-2 s-1). Over the region where GFEI has misidentified coal mines, the emissions are 181.18 ug (m-2 s-1). Over the region that GFEI and our inventory both have emissions, the GFEI emissions are 164.04 ug (m-2 s-1). There are no regions where we have emissions while GFEI has no emissions in Changzhi city. These facility-level inventories can help identify mitigation opportunities at specific mines, and support the design of more effective policies.

How to cite: Hu, W., Qin, K., He, Q., and Cohen, J. B.: Chinese Coal Mines Methane Emissions Constrained by High-Frequency Measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5036, https://doi.org/10.5194/egusphere-egu23-5036, 2023.

EGU23-6606 | ECS | Posters on site | AS3.12

About the use of Satellite Hyperspectral Images for Methane Detection 

Fabrizio Masin, Tiziano Maestri, and Michele Martinazzo

As global warming continues to be one of the greatest threats to Earth environment, the detection and monitoring of natural and anthropogenic emissions of greenhouse gases holds a critical role as the first step of any danger reduction policy. New generation spaceborne hyperspectral instruments cover large portions of the Earth while maintaining a high enough spectral and spatial resolution to investigate the contribution of single molecular species and accurately localize their emission source. The Matched Filter method is used to search enhanced concentrations of methane in the atmospheric column. PRISMA, ASI’s newest hyperspectral sensor, data are analysed. Both strong and weak CH4 emissions, in multiple scenarios, are investigated. It is demonstrated that PRISMA data allow also the identification of methane non-punctual sources when the land gas emission is very high. An estimated flux in the order of 4000 kg/h is found for a case study considering a landfill in India.

How to cite: Masin, F., Maestri, T., and Martinazzo, M.: About the use of Satellite Hyperspectral Images for Methane Detection, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6606, https://doi.org/10.5194/egusphere-egu23-6606, 2023.

EGU23-6751 | Orals | AS3.12

Quantifying methane super-emitters from oil and gas production in Romania with the AVIRIS-NG imaging spectrometer 

Gerrit Kuhlmann, Dominik Brunner, Lukas Emmenegger, Stefan Schwietzke, Daniel Zavala-Araiza, Andrew Thorpe, Andreas Hueni, and Thomas Röckmann

Reported methane (CH4) emissions from Romania's onshore oil and gas (O&G) production contribute 16% to onshore O&G emissions in Europe (55 out of 346 kt, IEA estimate). In October 2019, CH4 emissions from the O&G infrastructure were measured during the ROMEO campaign with a wide range of in situ measurement techniques in southern Romania. The measurements confirmed a log-normal distribution of emissions with a small number "super-emitters" contributing strongly to the overall emissions.

However, overall emissions remain uncertain because some CH4 super-emitters are difficult to identify with ground-based campaigns due to the large number of potential sources and sometimes elevated emission plumes. In contrast, airborne imaging spectrometers are well suited for identifying super-emitters due to their good spatial coverage and sensitivity to vertical columns. To identify super-emitters, the airborne AVIRIS-NG imaging spectrometer was flown in July 2021 in southern Romania covering an area of about 3000 kmthat contains about 80% of known O&G infrastructure in the region.

CH4 enhancements in the AVIRIS-NG lines were retrieved using a quantitative matched-filter method. In total, 38 emission plumes were identified that were assigned to 26 individual sources. Emissions were estimated using the integrated mass enhancement approach and ranged from 13 to 515 kg/h, which suggests annual emissions of about 30 kt assuming continuous emission rates. The sites were visited by ground crews, who confirmed that at least 17 of the sources were also active in December 2022.

The observed 30 kt/a from only 26 sources already represent more than half of the reported emissions from the onshore O&G emissions in entire Romania. The campaign demonstrates the importance of airborne imaging spectrometers to identify and quantify CH4 super-emitters for monitoring CH4 emissions from O&G infrastructure.

How to cite: Kuhlmann, G., Brunner, D., Emmenegger, L., Schwietzke, S., Zavala-Araiza, D., Thorpe, A., Hueni, A., and Röckmann, T.: Quantifying methane super-emitters from oil and gas production in Romania with the AVIRIS-NG imaging spectrometer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6751, https://doi.org/10.5194/egusphere-egu23-6751, 2023.

EGU23-6837 | ECS | Posters on site | AS3.12

Methane cycling at buried abandoned wells in a peat-rich area in northern Germany – curse or blessing for atmospheric emissions and emission studies? 

Sebastian Jordan, Stefan Schlömer, Martin Krüger, and Martin Blumenberg

In the worldwide effort to reach the 1.5-degree target, governments try to mitigate anthropogenic methane emissions. One example is the oil & gas sector, which is responsible for the second most anthropogenic methane emission source after agriculture. Abandoned oil and gas wells are seen as a promising target, as they can in some cases emit up to several tons of methane per year. However, only the USA includes emissions from such wells into their yearly greenhouse gas emission inventory and only for a few other countries like Canada, the United Kingdom, Romania and the Netherlands measured data on methane emissions from abandoned gas wells are available. Most countries do not even have sufficient data regarding numbers, positions, and status of their abandoned wells let alone the related methane emissions. Germany has about 20,000 abandoned wells, which are generally filled and buried, however, it is unclear, whether they are emitting methane or not.

Here, we present our approach and first data to fill this knowledge gap for Germany regarding methane emissions from onshore-abandoned oil and gas wells. For our first measuring campaign we focused on five regions in Lower Saxony (Federal State in Northern Germany) measuring 29 wells, covering both backfilled exploration and abandoned production wells of oil and gas fields. We will present our preliminary results including rates of soil methanotrophy focusing on one region with both, shallow oil wells and industrial peat production. Our data demonstrate the necessity for detailed knowledge on background methane emissions and cycling particularly in such methane-laden settings.

How to cite: Jordan, S., Schlömer, S., Krüger, M., and Blumenberg, M.: Methane cycling at buried abandoned wells in a peat-rich area in northern Germany – curse or blessing for atmospheric emissions and emission studies?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6837, https://doi.org/10.5194/egusphere-egu23-6837, 2023.

EGU23-7158 | ECS | Orals | AS3.12

Nord Stream methane leaks case: ICON-ART model simulation versus observations at various ICOS stations 

Anusha Sunkisala, Buhalqem Mamtimin, Thomas Rösch, Franziska Roth, and Andrea Kaiser-Weiss

Methane is emitted during the production and transportation of fossil fuels. Methane emissions result also from intensive livestock farming and agricultural practices as well as by the decay of organic waste. The leakage throughout the extraction, processing and transportation of natural gas releases methane straight into the atmosphere. Due to the damage to the Nord Stream gas pipelines on 26 September 2022 leaks have appeared close to the Danish island of Bornholm in the Baltic Sea, which releases large amounts of methane in the pipeline into the atmosphere within just a few days. In our study, we simulated the transport of methane plume in Nord Stream case by using DWD’s regional Icosahedral Nonhydrostatic (ICON) model with its transport scheme ART (Aerosols and Reactive Trace gases) extension.

The model is run for Limited Area Mode (LAM) with a horizontal spatial resolution of 6.5 km and 60 model levels. As source strength of methane emissions were used the estimates which were calculated by the German Federal Environmental Agency (Umwelt Bundesamt). An assumption, that a constant 700 kg/s of gas had been leaking since September 26 was used for the hourly model run to simulate the methane plume between September 26 and October 1 2022.

The model results had been compared to the potential methane signals of Nord Stream leaks detected at Integrated Carbon Observation System (ICOS) stations. According to our simulations, we found a good fit with respect to ICOS observations for the stations Hyltemossa, Birkenes and Norunda. Further analysis has been conducted to look at vertical profiles at different heights and also into correlation coefficients between the model and observations.

In this Nord Stream case, our simulation demonstrates modelling capabilities of the ICON-ART model and its associated quantitative assessment of methane emissions.

This work has been funded by the German Federal Ministry for Digital and Transport programme for Development and Implementation of Copernicus services for public needs within the HoTC project.

How to cite: Sunkisala, A., Mamtimin, B., Rösch, T., Roth, F., and Kaiser-Weiss, A.: Nord Stream methane leaks case: ICON-ART model simulation versus observations at various ICOS stations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7158, https://doi.org/10.5194/egusphere-egu23-7158, 2023.

EGU23-7229 | Posters on site | AS3.12

UAV-based methane emission quantification at a UK landfill site 

Han Yong, Grant Allen, and Hugo Ricketts

A field campaign using UAV-based measurements to derive methane fluxes from a large landfill site in North Manchester was conducted in the summer of 2022. The system comprises the newly developed ABB lightweight (3kg) Hoverguard greenhouse gas analyser based on the off-Axis Integrated Cavity Output Spectroscopy (with a precision of 0.9 ppb for CH4 at 1 Hz), an on-board TriSonica™ Mini wind sensor and the DJI M600 pro hexacopter.  Fluxes and corresponding flux uncertainties were calculated using the mass-balance method from 6 flight surveys conducted downwind of the active landfill. Accurate and reliable wind measurements sampled from instrumentation onboard rotary-wing UAVs remains a challenge, which was found to dominate flux uncertainty in this study. This study presents a low-cost and repeatable methodology for hotspot methane emission quantification.

How to cite: Yong, H., Allen, G., and Ricketts, H.: UAV-based methane emission quantification at a UK landfill site, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7229, https://doi.org/10.5194/egusphere-egu23-7229, 2023.

EGU23-7282 | Orals | AS3.12

Methane emissions from abandoned hydrocarbon wells in Italy: inventory, measurement techniques and the role of mega-emitters 

Monia Procesi, Giuseppe Etiope, Giancarlo Ciotoli, and Monica Moroni

Abandoned hydrocarbon (oil and gas) wells (AOG) represent a poorly studied source of atmospheric methane, potentially contributing to total anthropogenic fossil methane emission and related climatic impact. Methane leakage from AOG was measured only in a few countries (U.S.A., Canada, the Netherlands, United Kingdom), and available inventories in other countries are incomplete or need quality checks. Methodologies for gas flux measurement are not standardized. New studies have recently started in Italy in order to inventory onshore AOG, design multiple and versatile techniques for methane flux measurement, which can be adaptable to different typologies of well-heads, and to execute first measurements. Preliminary data revealed the existence of several AOW releasing relevant amounts of methane (orders of 101 ton yr-1), which are up to two orders of magnitude above those typically observed in North America. Contextualization of such “mega-emitters” (their percentage with respect to total AOW, technical conditions, possible existence in other countries) is necessary to assess average emission factors and derive bottom-up methane emission estimates at national and global scale.

How to cite: Procesi, M., Etiope, G., Ciotoli, G., and Moroni, M.: Methane emissions from abandoned hydrocarbon wells in Italy: inventory, measurement techniques and the role of mega-emitters, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7282, https://doi.org/10.5194/egusphere-egu23-7282, 2023.

EGU23-7283 | Orals | AS3.12

First Quantitative Assessment of Anthropogenic Methane Sources Investigated by the CHARM-F Lidar during the CoMet 2.0 Arctic Airborne Campaign 

Christian Fruck, Mathieu Quatrevalet, Andreas Fix, Sebastian Wolff, Martin Wirth, and Gerhard Ehret

The CoMet 2.0 Arctic airborne greenhouse gas measurement campaign took place over Canada in Summer of 2022. For the campaign, the German research aircraft HALO has been equipped with various instruments for remote-sensing and in-situ measurements of CO2 and CH4 and flown over target areas with potential sources of greenhouse gases, either natural (wetlands, thawing permafrost, etc.) or anthropogenic (oil and gas drilling sites, oil-sand mining, open-pit coal mines, landfills as well as biomass-burning in forest fires). With the city of Edmonton, Alberta as campaign base, a variety of sources of methane released due to human activity and adding substantially to the Canadian anthropogenic CH4 budget were conveniently within reach for our measurements.

This presentation focuses on a selection of anthropogenic sources of CH4 in Canada as well as the Valdemingómez and Pinto landfill sites near Madrid, which were targeted during a test flight. We show first results of the evaluation of active remote-sensing measurements that were conducted with DLR's CHARM-F lidar system. By using the Integrated-Path Differential-Absorption (IPDA)-lidar technique, CHARM-F enables measurements of total column concentrations of methane and carbon dioxide along flight tracks. After further adding wind information from auxiliary measurements or models, emission fluxes from localized sources can be estimated. We will highlight the top emitters in terms of estimated emission rate of CH4 (in the 10kt/year range). Those are likely the most promising candidates for mitigation attempts.

How to cite: Fruck, C., Quatrevalet, M., Fix, A., Wolff, S., Wirth, M., and Ehret, G.: First Quantitative Assessment of Anthropogenic Methane Sources Investigated by the CHARM-F Lidar during the CoMet 2.0 Arctic Airborne Campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7283, https://doi.org/10.5194/egusphere-egu23-7283, 2023.

EGU23-7506 | ECS | Orals | AS3.12

Quantifying emission dynamics of coal mine ventilation shafts with a stationary hyperspectral camera 

Marvin Knapp, Leon Scheidweiler, Felix Külheim, Ralph Kleinschek, Jaroslaw Necki, Pawel Jagoda, and Andre Butz

The global warming potential of methane on a 20-year scale is 80 times larger than that of carbon dioxide. Therefore reducing anthropogenic methane emissions can mitigate greenhouse gas-induced atmospheric warming in the short term. Thus, source attribution and budgeting of methane emissions have received particular attention in recent years. Coal mining activities were found to be accountable for approximately one-tenth of anthropogenic methane emissions. Observations of point sources (like coal mine ventilation shafts) by plume imagery from aircraft of satellites are emerging as a powerful and reliable tool for emission estimates. Yet, while these measurements cover large areas in a short time, the instrument revisiting rates do not allow observation of temporal variability of sources.
We present the results of a case study on source dynamics of coal mine ventilation shafts conducted in the Upper Silesian Coal Basin (USCB), Poland, in June 2022. We deployed a HySpex SWIR-384 hyperspectral camera at 1 km distance to a coal mine ventilation shaft. The camera repeatedly observed blue-sky scattered sunlight above the shaft in the shortwave infrared spectral range, taking approximately 1 minute per image. We detect methane plumes reliably using an adapted matched filter algorithm in the 2.3 μm absorption band. Co-located wind-lidar measurements allow us to estimate source emissions rates by the integrated mass enhancement (IME) method. Thereby, we produce several hundred emission estimates per day based on plume imagery, with an average uncertainty below 300 kg/h for minutely estimates under favourable measurement conditions. Our case study covers four consecutive days and reveals substantial source dynamics on all observed time scales from minutes to days. A 10-minute running average of the emissions can be a factor of 2 smaller or larger than the daily mean and daily averaged emissions ranged from 1.39 tCH4/h to 4.44 tCH4/h.

How to cite: Knapp, M., Scheidweiler, L., Külheim, F., Kleinschek, R., Necki, J., Jagoda, P., and Butz, A.: Quantifying emission dynamics of coal mine ventilation shafts with a stationary hyperspectral camera, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7506, https://doi.org/10.5194/egusphere-egu23-7506, 2023.

EGU23-7706 | ECS | Posters on site | AS3.12

A statistical gap filling model for methane fluxes over an urban area in the Alps 

Michael Stichaner, Christian Lamprecht, Martin Graus, Ignacio Goded, Niels Jensen, and Thomas Karl

There is consensus that climate change is mostly driven by anthropogenic greenhouse gas emissions. In addition to CO2 emissions, which have been the subject of public debate for a long time, increased awareness of methane (CH4) emissions has developed in recent years. CH4 is considered the 2nd most important contributor to radiative forcing, making it the most important non-CO2 greenhouse gas.

Due to the relatively short lifetime of the gas in the  atmosphere compared to CO2, the reduction of methane emissions can lead to a climate benefit on relatively short time horizons. In order to effectively reduce emissions, the polluters must be better understood and recognized. Here, we combine methane eddy covariance observations in combination with a variety of other trace gases and meteorological parameters that have been recorded since August 2020 in an Alpine city (Innsbruck, Austria) to investigate urban methane emissions. For an accurate comparison with bottom-up emission inventories we test different gap-filling methods with the help of meteorological parameters as well as other tracer fluxes, such as NO, NO2, or CO2. In order to quantify methane emissions in urban areas as annual totals, a complete, gap-free flux dataset is desired. We have developed different statistical gap filling models which are able to predict CH4 fluxes at the study location. The method is based on a boosted regression tree model with a variety of meteorological and astronomical parameters, as well as other trace gas fluxes serving as input. Different combinations of these input parameters are tested for accuracy of their prediction. Contrasting other gap filling methods, used over uninhabited areas, adding gases like CO2 or NO can serve as important additional predictors, because sectors related to combustion processes are considered as important contributors to CH4 emissions.  In this presentation we discuss CH4 flux measurements performed during the last 2,5 years over an urban area, and highlight first results on the performance of the developed gap filling models. 

How to cite: Stichaner, M., Lamprecht, C., Graus, M., Goded, I., Jensen, N., and Karl, T.: A statistical gap filling model for methane fluxes over an urban area in the Alps, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7706, https://doi.org/10.5194/egusphere-egu23-7706, 2023.

EGU23-7910 | ECS | Orals | AS3.12

Current potential of CH4 emission estimates using TROPOMI in the Middle East 

Mengyao Liu, Ronald van der A, Michiel van Weele, Henk Eskes, Pepijn Veefkind, Xin Zhang, Hanqing Kang, and Jieying Ding

Methane (CH4) is the second most important greenhouse gas after CO2. The TROPOspheric Monitoring Instrument (TROPOMI) on board the Sentinel 5 Precursor (S5-P) satellite measures CH4 at a high horizontal resolution of 7 × 7 km2, showing the capability on identifying and quantifying the sources at a local to regional scale. The Middle East is one of the strong CH4-emitting regions in the world. However, it is difficult to estimate the emissions here because of the uncertainties caused by bright surfaces and high aerosol loadings. Furthermore, several sources are located near the coast or in places with complex topography, where satellite observations are often of reduced quality. We use the product from the University of Bremen, WMF-DOAS XCH4 v1.8 product, which has good spatial coverage over the ocean and mountains, to estimate the emissions in the Middle East. The Aerosol Optical Depth (AOD) data from the MODIS/Aqua satellite instrument, which has a similar overpass time as TROPOMI, was adopted to filter potential unreliable XCH4 in the product.

For the inversion, we use the divergence method of Liu et al., (2021), which has been proven to be a fast and efficient way to estimate CH4 emissions from satellite observations. We have improved our method by comparing the fluxes in different directions for better background corrections over areas with complicated topographies. The temporal filter was established to further filter false emissions caused by surface albedos. We derived CH4 emissions on a grid of 0.2° from 2018 to 2021 and compared them to the latest bottom-up inventory EDGAR v7.0 in the same years. We found significantly lower emissions than EDGAR for the locations that are mainly determined by observed gas-flaring from satellites. Apart from sources of oil/gas production, the emissions from livestock in Saudi Arabia's irrigation zones, which have been reported neither in EDGAR nor other previous studies, are identified and quantified by using our divergence method. Another unexpected finding is that emissions from landfills are fairly stable and strong in some cities like Tehran.

How to cite: Liu, M., van der A, R., van Weele, M., Eskes, H., Veefkind, P., Zhang, X., Kang, H., and Ding, J.: Current potential of CH4 emission estimates using TROPOMI in the Middle East, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7910, https://doi.org/10.5194/egusphere-egu23-7910, 2023.

EGU23-8659 | ECS | Orals | AS3.12

Oil and gas industry emissions in Saskatchewan, Canada: a case study in uncertain reduction trends 

Scott Seymour, Donglai Xie, Katlyn MacKay, and Hugh Li

The province of Saskatchewan, Canada, came under new oil and gas industry emission regulations in 2020 to meet Canada’s methane emission reduction target for 2025. Although the province reportedly met its reduction target only two years into a five-year commitment, this finding was based on a bottom-up inventory whose operator-reported data had not been public until very recently. With these data made public for the first time, we recreated the federal government inventory for Saskatchewan (2012-2022) to better understand where and how emissions have changed in response to new regulations. Not only will this shed light on the regulations themselves (an updated version of which will be under review for Canada’s longer-term targets), but this inventory will also permit more detailed comparisons with forthcoming top-down measurements.

Since new measurements are expected to be included in this inventory structure, we also used recently published aerial LiDAR measurements to update the inventory. Importantly, while the unmodified inventory confirms the significant emission reduction reported by the Saskatchewan Government (~45% reduction), the inclusion of aerial measurement data suggests that emissions may have actually increased over the same time period. We discuss how the manner in which new measurements are included can influence the emission reductions relative to an uncertain baseline year, and we discuss whether a trend can be calculated reliably. Careful consideration will therefore be needed when including new measurement data into existing inventories. 

How to cite: Seymour, S., Xie, D., MacKay, K., and Li, H.: Oil and gas industry emissions in Saskatchewan, Canada: a case study in uncertain reduction trends, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8659, https://doi.org/10.5194/egusphere-egu23-8659, 2023.

EGU23-8744 | Orals | AS3.12

Methane emissions from abandoned oil and gas wells: measurements and uncertainties 

Mary Kang, Jade Boutot, Lauren Bowman, and Khalil El Hachem

Measurements have shown that abandoned oil and gas wells emit methane to the atmosphere, but the estimates of methane emissions at the national scales remain highly uncertain. Here, we provide an overview of available measurement data and studies investigating factors linked to high methane-emitting abandoned wells. We then analyze abandoned oil and gas well data in Canada and the United States to estimate methane emissions for both countries and evaluate uncertainties in the national estimates. Available measurement data indicate that average methane emission rates used as emission factors vary by 3 orders of magnitude or more, even after accounting for plugging status. Plugging status has been shown to be an important predictor of high methane emitting wells; however, there may be other important factors such as age, depth, fluid type and geographical region. Such well attribute data are not consistently available for many abandoned and orphaned oil and gas wells in Canada and the United States. Overall, there is a need for additional measurements of methane emissions from abandoned oil and gas wells and compilation of well attributes to reduce uncertainties in national estimates.

How to cite: Kang, M., Boutot, J., Bowman, L., and El Hachem, K.: Methane emissions from abandoned oil and gas wells: measurements and uncertainties, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8744, https://doi.org/10.5194/egusphere-egu23-8744, 2023.

EGU23-9152 | Posters on site | AS3.12

Quantifying methane emissions from industrial activities: A novel helicopter-borne application for coal mine ventilation shafts in Poland and perspectives 

Heidi Huntrieser, Eric Förster, Michael Lichtenstern, Falk Pätzold, Lutz Bretschneider, Astrid Lampert, Jaroslaw Necki, Pawel Jagoda, Quentin Taupin, David Holl, and Anke Roiger

The Upper Silesian Coal Basin in southern Poland belongs to one of the strongest emitting regions of anthropogenic methane (CH4) in Europe. A major part of these CH4 emissions is related to the coal mining industry, which are in focus of the METHANE-To-Go-Poland project presented here. For the first time, a unique helicopter towed probe (HELiPOD) was used to capture CH4 plumes from selected coal mine ventilation shafts. The HELiPOD probe (weight 325 kg, length 5 m) was equipped with a 3D wind anemometer and trace gas in situ instrumentation (Picarro G2401-m and Licor-7700) to measure CH4 with a high precision (1 ppb) and temporal resolution (up to 40 Hz), which is necessary for a precise calculation of the CH4 mass flux. In June and October 2022, repeated upwind and downwind probing of the plumes from selected shafts (4 shafts, 16 flights) were performed at different horizontal distances from the source (~500 m - 5 km) and altitudes (~20 m – 2 km). This way, both the inflow amount of CH4 and the horizontal/vertical dispersion of the CH4 plumes from the shafts were captured. Depending on wind speed, wind direction and stability, suitable flight patterns were developed for every flight. In addition, two controlled CH4 releases were successfully carried out to prove the novel measurement concept. Mobile ground-based CH4 measurements complemented the airborne probing.

In this presentation, mass flux calculations based on measurements from the two airborne CH4 instruments (with different measurement techniques) will be compared and uncertainties determined. Furthermore, CH4 mass flux calculations resulting from coinciding satellite measurements (GHGSat: swath width <15 km, spatial resolution <27 m) over the same ventilation shafts combined with high-resolved GEOS-FP wind data are presented. Finally, the uncertainties of the two different top-down approaches (air- and satellite-borne) are compared, in addition to different flight strategies. Comparisons with production data from the Polish coal mine industry are foreseen in near future (bottom-up approach). Subsequently, the same kind of airborne concept is envisaged for the METHANE-To-Go-Oman field experiment in autumn 2023, which will focus on CH4 emissions from the on-shore oil and gas exploration and production in Oman. Our collected data, funded by the International Methane Emissions Observatory (IMEO), will help coal, oil and gas companies as well as governments, to prioritize their CH4 emission mitigation strategies, actions and policies.

How to cite: Huntrieser, H., Förster, E., Lichtenstern, M., Pätzold, F., Bretschneider, L., Lampert, A., Necki, J., Jagoda, P., Taupin, Q., Holl, D., and Roiger, A.: Quantifying methane emissions from industrial activities: A novel helicopter-borne application for coal mine ventilation shafts in Poland and perspectives, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9152, https://doi.org/10.5194/egusphere-egu23-9152, 2023.

EGU23-9174 | ECS | Posters on site | AS3.12

Detection of local atmospheric methane enhancements by analyzing Sentinel-5 Precursor satellite data 

Steffen Vanselow, Oliver Schneising-Weigel, Michael Buchwitz, Heinrich Bovensmann, and John P. Burrows

Methane CH4 is an important anthropogenic greenhouse gas and its rising concentration in the atmosphere contributes significantly to global warming. Satellite measurements of the column-averaged dry-air mole fraction of atmospheric methane, denoted as XCH4, can be used to provide information about the location of methane sources and on their emissions, which can help to improve emission inventories and review policies to mitigate climate change.   

The Sentinel-5 Precursor (S5P) satellite with the TROPOspheric Monitoring Instrument (TROPOMI) onboard was launched in October 2017 into a sun-synchronous orbit with an equator crossing time of 13:30. TROPOMI measures reflected solar radiation in different wavelength bands to generate various data products and combines daily global coverage with high spatial resolution. TROPOMI's observations in the shortwave infrared (SWIR) spectral range yield methane with a horizontal resolution of typically 5.5 x 7 km2

We used a monthly XCH4 data set (2018-2021) generated with the WFM-DOAS retrieval algorithm, developed at the University of Bremen, to detect regions with temporally persistent, locally enhanced XCH4. At first, we applied a spatial high-pass filter to the XCH4 data set to filter out the large-scale methane fluctuations. The resulting anomaly ΔXCH4 maps show the difference of the local XCH4 values compared to its surroundings. We then analyzed the monthly anomaly maps to identify potential source regions with persistent XCH4 enhancements by utilizing different filter criteria, such as the number of months in which the local methane anomalies ΔXCH4 must exceed certain threshold values. As a next step, we used a simple mass balance method to estimate the monthly emissions and the corresponding uncertainties of the detected potential source regions from the monthly averaged XCH4 maps. In the last step, we interpreted the emissions of the potential source regions in terms of the source type, by comparing the detected potential source regions with emission databases based on a spatial analysis. 

In this presentation, the algorithm and initial results concerning the detection of regions with temporally persistent, local XCH4 enhancements, originating from localized potential methane sources (e.g., wetlands, coal mining areas, oil and gas fields) are presented.     

How to cite: Vanselow, S., Schneising-Weigel, O., Buchwitz, M., Bovensmann, H., and Burrows, J. P.: Detection of local atmospheric methane enhancements by analyzing Sentinel-5 Precursor satellite data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9174, https://doi.org/10.5194/egusphere-egu23-9174, 2023.

EGU23-9429 | Orals | AS3.12

Mapping methane and carbon dioxide point sources from space with EMIT 

Andrew Thorpe, Robert Green, David Thompson, Philip Brodrick, John Chapman, Clayton Elder, Itziar Irakulis Loitxate, Daniel Cusworth, Alana Ayasse, Riley Duren, Luis Guanter, and Christian Frankenberg

Carbon dioxide and methane are the two primary anthropogenic climate-forcing agents and are the dominant source of uncertainty in the global carbon budget. We present the first observations of methane and carbon dioxide point source plumes from the oil&gas, waste management, and energy sectors using the Earth Surface Mineral Dust Source Investigation (EMIT) imaging spectrometer. An initial analysis of results from selected countries in the Middle East and Central Asia indicate that Turkmenistan has both the greatest number and largest methane emissions observed in this study. EMIT measures 285 distinct wavelengths between 381 and 2493 nm with a 7.4 nm spectral resolution and an 80 km image swath with a 60 m spatial resolution. EMIT’s daily coverage is equivalent to an area the size of South Africa and its revisit frequency will permit an assessment of emissions over time. By providing the locations of emission sources, these results offer the potential to improve our understanding of global greenhouse gas budgets and to inform mitigation strategies.

Figure 1: Example of 12 methane plumes observed by NASA’s Earth Surface Mineral Dust Source Investigation (EMIT) mission east of Hazar, Turkmenistan.

How to cite: Thorpe, A., Green, R., Thompson, D., Brodrick, P., Chapman, J., Elder, C., Irakulis Loitxate, I., Cusworth, D., Ayasse, A., Duren, R., Guanter, L., and Frankenberg, C.: Mapping methane and carbon dioxide point sources from space with EMIT, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9429, https://doi.org/10.5194/egusphere-egu23-9429, 2023.

EGU23-9548 | Orals | AS3.12

Methane Alert and response system (MARS): IMEO’s satellite-based system for detection and attribution of methane point sources around the world 

Luis Guanter, Itziar Irakulis-Loitxate, Joannes D Maasakkers, Ilse Aben, Christian Lelong, Cynthia A Randles, Daniel Zavala-Araiza, Steven P Hamburg, and Manfredi Caltagirone

The reduction of anthropogenic methane emissions, and especially those from the fossil fuel industry, is one of the most effective ways to slow down global warming in the next decade. Methane emissions from fossil fuel activities often happen as plumes emanating from strong point sources, such as flares, compressor stations, storage tanks, and mine vents.

The Sentinel-5P TROPOMI mission can detect the largest plumes from these sources daily and at a global scale thanks to its continuous spatial coverage and daily temporal resolution. Complementary to TROPOMI, several high spatial resolution satellite missions with sensitivity to methane are now being used to attribute plumes to point sources. These missions, so-called point-source imagers in the methane mapping context, sample the methane absorption features in the shortwave infrared with a spatial resolution of 20-60 m, enabling the detection and attribution of plumes from point sources >200-1000 kg/h. Point-source imagers can be hyperspectral (also known as imaging spectrometers), including the GHGSat, PRISMA, EnMAP, and EMIT missions, and multispectral instruments, such as Sentinel-2, Landsat, and WorldView-3. The observations by these point-source imagers often follow a previous identification of large methane hotspot areas by TROPOMI.

In connection with this increasing landscape of methane-observing satellites, the United Nations Environment Programme (UNEP) is implementing a Methane Alert and Response system (MARS) as part of its International Methane Emissions Observatory (IMEO). MARS was recently launched at COP27 in direct support to the Global Methane Pledge. It relies on the combined use of multiple methane-observing satellites for the systematic detection, attribution and monitoring of methane sources. In its initial phase, the focus is on point sources associated to the energy sector.  

In this contribution, we will describe the satellite component of MARS and will provide examples of how satellites are being used to detect and mitigate active methane point sources from the energy sector around the world.

 

How to cite: Guanter, L., Irakulis-Loitxate, I., Maasakkers, J. D., Aben, I., Lelong, C., Randles, C. A., Zavala-Araiza, D., Hamburg, S. P., and Caltagirone, M.: Methane Alert and response system (MARS): IMEO’s satellite-based system for detection and attribution of methane point sources around the world, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9548, https://doi.org/10.5194/egusphere-egu23-9548, 2023.

EGU23-9802 | ECS | Orals | AS3.12

Methane Emissions Across a Diverse Set of Large Landfills in the United States and Canada 

Daniel Cusworth, Riley Duren, Alana Ayasse, and Andrew Thorpe

Methane emissions from the waste sector may represent a significant fraction of the global anthropogenic methane budget. However, few comprehensive studies across the broad landscape of waste operations exist to validate existing bottom-up models that underpin reporting programs and national inventories. In this study, we flew two airborne imaging spectrometers to map emissions at large landfills across 18 states in the U.S. and three provinces in Canada between 2016-2022. This technology is particularly sensitive to point source methane emissions and can geolocate source locations to within several meters. We observed point sources at a high fraction (52%) of sites and observed high emission persistence (60%), or point source detection frequency, at sites we surveyed multiple times. Airborne derived emissions correlate poorly with EPA reported emission and are on average higher, which could point to some issues with models that underpin reporting protocols. We validated imaging spectrometer aerial emission rates against the Scientific Aviation mass balance technique at 15 landfills, and find good agreement between these two independent measurement systems. Sustained measurements across many landfills and waste sites are needed to validate inventories and provide actionable data for industry operators and enforcement agencies.

How to cite: Cusworth, D., Duren, R., Ayasse, A., and Thorpe, A.: Methane Emissions Across a Diverse Set of Large Landfills in the United States and Canada, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9802, https://doi.org/10.5194/egusphere-egu23-9802, 2023.

EGU23-10259 | Posters on site | AS3.12

Underestimation of reported methane emissions, and air pollutant loadings, from upstream oil and gas activities in Canada 

Martin Lavoie, David Risk, Katlyn MacKay, and Evelise Bourlon

Canada was an early adopter of methane regulation in the oil and gas sector, and recently announced a more ambitious goal to reduce 75% of methane emissions by 2030. New stricter methane regulations should also help reduce loading of air pollutants typically associated with methane emissions (H2S, VOCs, ozone). To examine regional emission trends and to derive an inventory estimate for Canada’s upstream oil and gas sector, we measured methane emissions at 6650 sites across six major oil and gas producing regions in Canada. Our research suggests that methane emissions from the oil and gas industry are underestimated in Canada by ~1.5. For Canada’s largest producing province, Alberta, we found a greater than 1000-fold variation in methane intensity per unit of fossil energy production within the cohort of oil and gas producers. Producer self-published methane emission intensities in ESG materials showed a low bias and tended to mirror regulatory submissions that require reporting only on specific source types. Our measurements suggest that methane-associated pollutants produced by oil and gas activities are also underestimated and communities near these activities may face higher loading of methane-accessory contaminants than might be predicted by Canada’s National Pollutant Release Inventory (NPRI). Using accepted pollutant emission factors, reported flaring and other combustion activity, the federal methane inventory, and our methane measurements, we generated air quality exposure maps reflecting air pollutant loads on Canadian communities. Stricter methane regulation has the potential to significantly decrease methane, but also pollutant loads in several heavy oil communities including the Lloydminster - Bonnyville area.

How to cite: Lavoie, M., Risk, D., MacKay, K., and Bourlon, E.: Underestimation of reported methane emissions, and air pollutant loadings, from upstream oil and gas activities in Canada, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10259, https://doi.org/10.5194/egusphere-egu23-10259, 2023.

EGU23-10442 | ECS | Orals | AS3.12

A comparison of methane source localization methods in landfills across Canada using truck-based measurement, Lagrangian stochastic back trajectory modeling, and Landsat thermal images 

Afshan Khaleghi, Evelise Bourlon, Jordan Stuart, Rebecca Martino, Judith Vogt, Lindelwa Coyle, Mackenzie LeVernois, Martin Lavoie, Gilles Perrine, Angus Kennedy, Meghan Boyd, Sarah Kennedy, Melanie Hammer, Sebastein Ars, Felix Vogel, Eric Gilbertson, Masoud Mahdianpari, and David Risk

Canada is a signatory to the Global Methane Pledge and is aiming to achieve a 75% cut in methane from 2030 levels from oil and gas production through regulatory updates and a 50% cut in waste sector emissions using new regulations. Despite numerous large-scale studies that have measured and identified emission sources from Canada's oil and gas sector, there are virtually no measurements of emissions from landfills in Canada. As such, inventory values for landfill emissions are based on a combination of industry-submitted data and emission factors. Canada could design better policies and regulations if policymakers had access to actual emission rates and source types. Therefore, we designed and carried out a large-scale measurement campaign targeting minimally 125 landfills across Canada, using aircraft mass balance measurements and truck-based measurements (i.e., downwind and onsite transects) coupled with Gaussian inversions to determine emission rate. This study focuses on methodologies used to determine source locations, or methane hotspots, on the landfill surface. In Particular, source attribution methods included a Lagrangian back trajectory footprint analysis of mobile surveys, onsite mixing ratios and winds measured with the truck, as well as Landsat thermal retrievals that have been shown in prior studies to correlate with methane hotspots. Measurements were carried out between June and December 2022 using one or more measurement methodologies for a total of 143 sites. We performed truck-based measurements of mixing ratios across navigable portions of 59 landfills. All indicators showed some correlation to mixing ratios collected onsite, although Lagrangian analysis products from downwind measurements were somewhat more reliable in flagging hotspots than the satellite thermal indices. The indicators often highlighted the active disposal face, leachate impoundment ponds, or compost areas, as the active source area. This study will help contribute much-needed source information for solid waste sector regulatory design in Canada and has the potential to help improve models of landfill methane generation.

How to cite: Khaleghi, A., Bourlon, E., Stuart, J., Martino, R., Vogt, J., Coyle, L., LeVernois, M., Lavoie, M., Perrine, G., Kennedy, A., Boyd, M., Kennedy, S., Hammer, M., Ars, S., Vogel, F., Gilbertson, E., Mahdianpari, M., and Risk, D.: A comparison of methane source localization methods in landfills across Canada using truck-based measurement, Lagrangian stochastic back trajectory modeling, and Landsat thermal images, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10442, https://doi.org/10.5194/egusphere-egu23-10442, 2023.

Canada is the third largest oil and gas producer, with over 500,000 active and inactive wells, mostly located in the Western Canada Sedimentary Basin (WCSB). A large, undetermined fraction of Canada’s GHG emissions emanate from oil and gas infrastructure. Governments and industry are all committed to immediately reducing methane leaks to the atmosphere from surface casing vent flows (SCVF) and ground migration (GM) of both new and old wells. Methane carbon isotopic composition offers insight into the source of unwanted gas emissions. A geospatial tool would help to attribute and reduce GHG emissions from contour maps of ẟ13C of methane and other hydrocarbons of production, SCVF, and GM gases across the WCSB. These “Isoscapes” of production gases vary systematically, reflecting the local geology. SCVF and GM isoscapes are offset from the production ones because the SCVF most often are shallower than the target formations, and the GM gas may be oxidized in soils. The difference between the production and SCVF isoscapes can be used to attribute methane emissions from tanks and production infrastructure, compared to leaks from the wells themselves. The isoscapes directly facilitate the plugging of problem wells.  The maps are based on over 3,000 locations where we used isotope fingerprinting (i.e., Rowe & Muehlenbachs, 1999) to identify the source depth of a leak.  Regulatory measurements mandate that the leaks are sealed at their source depth, greatly adding to the cost of plugging any well. The SCVF isoscapes suggest the likely source depth of an unsampled leaking well, thus greatly simplifying its remediation. Applying such information beyond a local case study may contribute to accounting for the GH contribution from regional oil and gas activities in Canada and elsewhere.

 

 

Reference

Rowe, D., & Muehlenbachs, A. (1999). Low-temperature thermal generation of hydrocarbon gases in shallow shales. Nature398(6722), 61­-63.

How to cite: Gonzalez Arismendi, G. and Muehlenbachs, K.: A proposal to use “Isoscapes” of fugitive gases from oil and gas wells to facilitate the reduction and attribution of methane emissions and plugging of faulty wells, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10636, https://doi.org/10.5194/egusphere-egu23-10636, 2023.

EGU23-10725 | ECS | Posters virtual | AS3.12

Supporting Methane Mitigation Efforts by Improving Urban-scale Methane Emission Estimates in Melbourne, Australia. Part 2: Developing the methane observation network for the Melbourne region 

Jhonathan Ramirez Gamboa, Zoe Loh, Ann Stavert, Paul Krummel, Nasimeh Shahrokhi, Cathy Trudinger, Christopher Caldow, Darren Spencer, and Christopher Roulston

Methane (CH4) is the second greatest contributor to climate forcing after carbon dioxide (CO2).  Methane has a considerably shorter atmospheric lifetime compared to CO2 (12 yr c.f. 300-1000 yr) but a higher warming potential in the atmosphere (GWP100yr 28, (IPCC, 2014)). Most anthropogenic emissions come from landfills, wastewater treatment plants, leaks in the fossil fuel supply chain and ruminant livestock.  The reduction of anthropogenic methane emissions is key to maintaining the feasibility of the Paris Agreement. The Global Methane Pledge launched at COP26 aims to reduce methane emissions by 30% relative to 2020 by 2030. Urban areas are an ideal target to reduce methane emissions given that they account for around 20% of the total emissions whilst they occupy only 3% of the land surface. Urban methane mitigations plans are proven to have a high impact reducing GHG emissions and bringing co-benefits in public health through improvements in air quality.

Australia is a signatory to both the Paris Agreement and the Global Methane Pledge and have an important potential emission reduction in urban areas. Melbourne is the second most populous city in Australia with over 5 million people (around 1/5 of Australia’s population) and it is projected to become the most populated by 2050. A recent study attempted to improve methane emission inventories for Melbourne using an inversion system, global emission data and atmospheric measurements (Shahrokhi , 2022).  Their results showed that current emission datasets do not accurately represent the spatial distribution and total estimates of methane emissions over Melbourne. Hence, an improved emission inventory is required for Melbourne. This will reduce the uncertainty and limitations of current methane emission estimates and support the formulation of effective emissions mitigation plans. Essential to this is the expansion of the Melbourne urban observational network, which is currently too sparse to accurately detect emissions. Here we present our preliminary progress on the development of a comprehensive methane observation network. This project aims to combine different measurement techniques to achieve a better representation of methane mole fraction variability in the Melbourne region, to inform inverse modelling estimates of emissions. We use a combination of mobile and stationary ground observations in key parts of the city to better capture and represent methane emissions. Future work includes the comparison of high precision analysers with low-cost sensors, improvement of source attribution by measurements of methane isotopes and other tracers, and the use of “AirCore” technology to obtain vertical methane profiles.

 

References

IPCC, 2014: Climate Change 2014: Synthesis Report. Contribution of Working Groups I, II and III to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change [Core Writing Team, R.K. Pachauri and L.A. Meyer (eds.)]. IPCC, Geneva, Switzerland, 151 pp.

Shahrokhi, N. 2022. Regional Methane Inversion for Melbourne, Australia, using in-situ measurements. Online poster [accessed 10 Jan 2022]. Available from: https://agu2022fallmeeting-agu.ipostersessions.com/default.aspx?s=2F-7B-00-39-98-DC-28-09-C3-90-81-25-D7-44-E2-D2#

How to cite: Ramirez Gamboa, J., Loh, Z., Stavert, A., Krummel, P., Shahrokhi, N., Trudinger, C., Caldow, C., Spencer, D., and Roulston, C.: Supporting Methane Mitigation Efforts by Improving Urban-scale Methane Emission Estimates in Melbourne, Australia. Part 2: Developing the methane observation network for the Melbourne region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10725, https://doi.org/10.5194/egusphere-egu23-10725, 2023.

EGU23-11170 | Posters on site | AS3.12

Quantification of methane emissions from urban sewer network 

Jaewon Joo, Sujong Jeong, Jaewon Shin, and Dong Yeong Chang

Sewer systems, which consist of wastewater treatment plants (WWTPs) and sewer networks, are important urban water infrastructure that helps to improve water quality and prevent flooding. While they are recognized as a major source of methane emissions with considerable potential, accurate quantification of methane emissions from sewage systems has not yet been achieved. Here, we measured atmospheric methane from the urban sewer network using a mobile laboratory, which consists of the electric vehicle and monitoring instruments for Greenhouse Gas (GHG) such as carbon dioxide (CO2), methane (CH4), and ethane (C2H6). The mobile measurements of sewer networks are conducted in Gwanak district of Seoul in South Korea from September 2022. More than 3,000 manholes and rain gutters in commercial and residential areas were measured for the methane emissions of the combined sewer network type in Gwanak district. The methane emissions from urban sewer network were found to be significant in the study area. However, these emissions are currently not included in the national GHG inventory. Further details of our findings will be introduced at the European Geosciences Union (EGU) General Assembly 23.   

This work was supported by Brain Pool Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Science and ICT (No.2019H1D3A1A01101988)

How to cite: Joo, J., Jeong, S., Shin, J., and Chang, D. Y.: Quantification of methane emissions from urban sewer network, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11170, https://doi.org/10.5194/egusphere-egu23-11170, 2023.

EGU23-11383 | ECS | Orals | AS3.12

Capabilities of CH4 source apportionment using atmospheric 14CH4 measurements: Switzerland as a case study 

Thomas Laemmel, Dylan Geissbühler, Stephan Henne, Dominik Brunner, Markus Leuenberger, and Sönke Szidat

Methane (CH4) is the second most important anthropogenic greenhouse gas after carbon dioxide (CO2). Main CH4 sources are linked to the human use of fossil fuels (oil, gas, coal) and human-related or natural biogenic processes such as agriculture, waste management or wetlands. While biogenic emissions of CH4 contain present-day atmospheric radiocarbon (14C) levels, CH4 derived from fossil sources is 14C-free so that 14CH4 measurements can be used as a source apportionment proxy to distinguish fossil from biogenic CH4 sources.

A dedicated setup to analyze 14CH4 was developed at the Laboratory for the Analysis of Radiocarbon with AMS, University of Bern. Typical samples are 60L of atmospheric air collected in bags, which, after extraction, result in about 60 µg carbon in CH4-derived CO2 form, enough for a 14C gas measurement on a MICADAS (Mini Carbon Dating System) accelerator mass spectrometer.

Since 2019, biweekly air samplings have been  conducted at three sites in Switzerland: the high altitude research station Jungfraujoch (3580 m asl) considered as a European continental background station, a tall tower in Beromünster and an urban site in Bern. A fourth site (with a tall tower) in Sottens has been visited since June 2021.

Beside these in situ measurements, an atmospheric 14CH4 transport model was developed to simulate 14CH4 values for each sampling. It is based on the Lagrangian transport and dispersion model FLEXPART, two CH4 emission inventories (Meteotest EKAT for Switzerland, TNO-CAMS v4.2 for the rest of Europe), a priori 14CH4 signatures for each emission type and the weather model COSMO. 14CH4 emissions from pressurized water reactors (PWR) of nuclear power plants in Switzerland and neighboring countries are also taken into consideration.

This contribution will show the in situ 14CH4 measurements as well as corresponding simulations and emphasize that the sporadic transport of 14CH4 emitted from PWRs is greatly influencing the overall signal measured over the Swiss Plateau making CH4 source apportionment for this region very challenging.

How to cite: Laemmel, T., Geissbühler, D., Henne, S., Brunner, D., Leuenberger, M., and Szidat, S.: Capabilities of CH4 source apportionment using atmospheric 14CH4 measurements: Switzerland as a case study, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11383, https://doi.org/10.5194/egusphere-egu23-11383, 2023.

EGU23-11773 | ECS | Posters on site | AS3.12

Application of the large-scale flux chamber for quantification of methane release rate at Transylvanian gas fields. 

Paweł Jagoda, Jarosław Nęcki, Jakub Bartyzel, Andrei Radovici, Alexandru Mereuta, Thomas Roeckmann, and Aleksandra Figura

The oil and gas (O&G) sector contributes significantly to the anthropogenic part of the methane cycle in the atmosphere while having the most effective opportunities for emission mitigation with technically feasible and cost-effective options. Romania is a key O&G producer within the EU Region of Transylvania with its active gas fields being in the focus of the second measurement campaign in the ROMEO project. Teams from European collaborations were deploying various techniques (GPM, OTM-33A, High Flow Sampler, Tracer release) for quantifications of the methane emission rates. In June of 2021, AGH deployed the large-scale flux chamber with help of scientists from  UBB, Romania,  and in cooperation with local O&G operator – Rom-Gas. Construction was designed and built to be used in the case of small gas installations like the single Christmas tree and was tested intensively during this campaign. A hemispheric structure with a diameter of 6 meters and volume of approximately 55 m3 was used to check the tightness of different gas wells in suitable conditions (size, terrain, meteorology). The methane concentration increase was measured by the OA-ICOS technique. We used an LGR MGGA-918 analyser while additional airflow and air mixing inside the chamber were provided with additional ventilators.

 

In this presentation, methane emission rates calculations based on deployments of large-scale flux chambers in Transylvania will be compared to other techniques. Verification of the chamber was developed using controlled release tests of methane and acetylene. Moreover, the estimated uncertainty of the measurement technique will be presented. Finally, the potential for use of a large-scale flux chamber as a direct ground based measurement technique and complementary to other direct and indirect techniques will be discussed.

 

The research results presented in this paper have been developed with the use of equipment financed from the funds of the "Excellence Initiative - Research University" program at AGH University of Science and Technology. The authors thank all the members of the ROMEO campaign, in particular, Thomas Roeckmann for providing an opportunity to be part of this measurement campaign.

How to cite: Jagoda, P., Nęcki, J., Bartyzel, J., Radovici, A., Mereuta, A., Roeckmann, T., and Figura, A.: Application of the large-scale flux chamber for quantification of methane release rate at Transylvanian gas fields., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11773, https://doi.org/10.5194/egusphere-egu23-11773, 2023.

EGU23-13484 | ECS | Orals | AS3.12

Anthropogenic and natural CH4 and CO2 emissions observed by a combination of passive, active, and in situ airborne measurements during the CoMet 2.0 Arctic mission in Canada 2022 

Sven Krautwurst, Jakob Borchardt, Oke Huhs, Konstantin Gerilowski, Christian Fruck, Michal Galkowski, John P. Burrows, Christoph Gerbig, Andreas Fix, Hartmut Bösch, and Heinrich Bovensmann

Anthropogenic greenhouse gas (GHG) emissions remain the main concern for global climate change. To reduce and mitigate those emissions both anthropogenic and natural sources must be identified and quantified. However, high northern latitude wetland regions may also overlap with, e.g., fossil fuel extraction sites. Consequently, commonly used passive satellite sensors are often challenged to observe and disentangle those emissions due to challenging illumination conditions and their large ground scene size, respectively.

To investigate anthropogenic and wetland GHG emissions, a team of scientists deployed a comprehensive suite of instruments aboard the German Research aircraft HALO (High Altitude and Long Range Research) during the CoMet 2.0 Arctic mission conducted in Canada in August and September 2022. During the campaign, passive airborne remote sensing measurements by MAMAP2D-Light (Methane airborne mapper 2D light) were combined with active airborne remote sensing measurements by CHARM-F (CH4 Airborne Remote Monitoring – Flugzeug) and in situ GHG concentration measurements, also including an extensive suite of meteorological parameters.

Those column and in-situ concentration observations of CH4 and CO2 will be used to identify and quantify emissions over a wide range of source types and scales in Canada (and Europe). This comprises single point source emissions (e.g., power plants), small areal sources such as landfills (e.g, the Valdemingomez and Pinto landfills in Madrid) and opencast coal mines, and extensive oil and gas exploration sites, including oil sand areas, which might be embedded in natural wetland regions or river deltas. The imaging capabilities of the MAMAP2D-Light instrument enable precise localisation of emissions and therefore mitigation strategies in the case of, e.g., leakages. This work will summarize and present first results and emission estimates from the CoMet 2.0 Arctic mission with a focus on localised emitters observed by the airborne imaging instrument MAMAP2D-Light.

How to cite: Krautwurst, S., Borchardt, J., Huhs, O., Gerilowski, K., Fruck, C., Galkowski, M., Burrows, J. P., Gerbig, C., Fix, A., Bösch, H., and Bovensmann, H.: Anthropogenic and natural CH4 and CO2 emissions observed by a combination of passive, active, and in situ airborne measurements during the CoMet 2.0 Arctic mission in Canada 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13484, https://doi.org/10.5194/egusphere-egu23-13484, 2023.

EGU23-13551 | Posters on site | AS3.12

Methane emissions from offshore oil and gas production activities in Gabon and Angola: First results from the airborne METHANE-To-Go campaign 2022 

Anke Roiger, Maximilian Eckl, Magdalena Puehl, Klaus-Dirk Gottschaldt, Tiziana Braeuer, Heinfried Aufmhoff, Lisa Eirenschmalz, Felicitas Sakellariou, Gregor Neumann, guilherme ventura, and Winne Cadete

Methane (CH4) is after carbon dioxide the second most important anthropogenic greenhouse gas. Due to its comparatively short lifetime of ~10 years, a significant reduction in anthropogenic CH4 emissions would help to reduce the atmospheric concentration within a decade with near term temperature benefits. However, the development of efficient mitigation strategies needs to be informed by identifying, locating and quantifying CH4 emissions from the different sectors. A large part of CH4 emissions from the global oil and gas sector is expected to arise from offshore production, which currently however is understudied. Off the coast of Gabon and Angola, oil and gas production is spread over more than 800 kilometres across a wide variety of offshore installations, covering both shallow waters and deep sea. Here we report on airborne measurements conducted using the DLR Falcon along the west coast of Central Africa in September 2022. The DLR Falcon was equipped with a suite of different in-situ instruments to measure CH4 and a series of other trace species, as well as meteorological variables. Measurements were taken during 15 science flights to quantify emissions related to offshore oil production. We will present and discuss our airborne results on regional and facility-scales, in dependency of e.g. infrastructure type and age, and compare them with available inventory estimates and industry reportings. Our collected data, co-funded by the International Methane Emissions Observatory (IMEO), will help coal, oil and gas companies and governments, to prioritize their methane emission mitigation .

How to cite: Roiger, A., Eckl, M., Puehl, M., Gottschaldt, K.-D., Braeuer, T., Aufmhoff, H., Eirenschmalz, L., Sakellariou, F., Neumann, G., ventura, G., and Cadete, W.: Methane emissions from offshore oil and gas production activities in Gabon and Angola: First results from the airborne METHANE-To-Go campaign 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13551, https://doi.org/10.5194/egusphere-egu23-13551, 2023.

EGU23-13865 | ECS | Posters on site | AS3.12

Methane source identification using Non-Methane Hydrocarbon (NMHC) source apportionment in the Eastern Mediterranean and Middle East region 

Emeric Germain-Piaulenne, Jean-Daniel Paris, Efstratios Bourtsoukidis, Pierre-Yves Quehe, Michael Michael Pikridas, Maximilien Desservettaz, Dominique Baisnee, Yunsong Liu, Valérie Gros, and Jean Sciare

Methane (CH4) is a potent greenhouse gas but its sources remain poorly quantified in the Eastern Mediterranean and Middle East (EMME) region where major oil and gas production takes place. Light alkanes, such as ethane (C2H6), are co-emitted with CH4 by oil and gas activities and are promising tracers for quantifying the methane emissions from this sector. Cyprus is an ideal location for studying the composition of regional air masses and for characterizing different emission source signatures at a regional scale. A Picarro G2401 greenhouse gas analyzer and two field-based Gas Chromatography Flame Ionization Detectors (GC-FID) for Non-Methane Hydrocarbons (NMHC) measurements were deployed during two campaigns, one in “urban” (Nicosia) and one in “regional background” (Cape Greko) environment respectively. The campaign at the regional background site consisted in continuous methane and NMHCs (C2-C12) observations using a mobile laboratory that was deployed at the south-eastern edge of the island between December 2021 and February 2022. This location was chosen to capture airmasses of remote south and eastern origin, uninfluenced by local sources. We use these observations to 1) evaluate the significance of long-range transported versus local sources in Cyprus, 2) identify and document regional anthropogenic methane sources, and 3) assess the accuracy of the EDGAR sectoral emission inventory over EMME. Positive Matrix Factorization (PMF) analysis of the NMHC dataset resulted in the identification of four distinct sources namely tropospheric background, urban, heavy oil combustion, and transported from Middle East. The latest occurred during three distinct episodes and on average, had the highest NMHC concentrations. Generally, the different urban and regional signatures/sources displayed good and variable correlations between CH4 and C2 to C6-NMHCs. By investigating the PMF results together with CH4 concentrations and an atmospheric dispersion model (FLEXPART), we provide a comprehensive characterization of the pollution sources at regional scale over the Eastern Mediterranean region.

How to cite: Germain-Piaulenne, E., Paris, J.-D., Bourtsoukidis, E., Quehe, P.-Y., Michael Pikridas, M., Desservettaz, M., Baisnee, D., Liu, Y., Gros, V., and Sciare, J.: Methane source identification using Non-Methane Hydrocarbon (NMHC) source apportionment in the Eastern Mediterranean and Middle East region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13865, https://doi.org/10.5194/egusphere-egu23-13865, 2023.

EGU23-14191 | ECS | Posters on site | AS3.12

Development and First Deployment of an Innovative Airborne δ13C(CH4) In Situ Measurement Setup 

Paul Waldmann, Michael Lichtenstern, Friedemann Reum, Helmut Ziereis, Alina Fiehn, Michał Gałkowski, Christoph Gerbig, Andreas Fix, and Anke Roiger

Recent atmospheric methane concentrations show an accelerated increase, but the contributions of the underlying emitters are poorly understood. Recording the stable carbon isotope ratio of methane (δ13C(CH4)) is a powerful tool for CH4 source attribution and the understanding of the global methane budget. The airborne measurement of δ13C(CH4) provides the advantages of reaching remote areas and covering large-scale regions, but is challenging regarding sufficient precision while maintaining high spatial measurement density. The state of the art technique is to collect airborne gas samples for subsequent laboratory analysis by isotope ratio mass spectrometry, with high δ13C(CH4) precision of 0.05 ‰. Here we present an innovative in situ airborne system for the measurement of δ13C(CH4), called MIRACLE. MIRACLE consists of a conventional Picarro cavity ring down greenhouse gas analyzer (G2210-i) for the measurement of CH4 and δ13C(CH4), and a sampler unit. The sampler enables the collection of six gas samples in 2 l stainless steel tanks, in a short time (20 s each) via a metal bellows pump, which allows for the specific sampling of small-scale features, such as point source emissions. The sampling is followed by an extended period of subsequent analysis (up to 10 min). Using this setup, we achieve sufficient δ13C(CH4) precision (1σ uncertainty of 0.34 ‰) and an average of five samples per flight hour, allowing for a large number of samples for long flights. Due to the resulting dense coverage with sufficient precision, this novel approach allows for airborne δ13C(CH4) characterization of small-scale methane emitters and large-scale gradients. We employed MIRACLE aboard the research aircraft HALO during the CoMet 2.0 Arctic campaign in summer 2022, which focused on characterizing natural and anthropogenic methane sources in Canada. In this presentation, a proof of concept for the instrument is elaborated, including the investigation of sample purity and measurement comparisons with other instruments. Additionally, we show δ13C(CH4) signatures revealed by the method of Keeling analysis of measurements obtained during CoMet 2.0 and compare them to previous studies. The airborne operation of the MIRACLE instrument combines the advantages of increased precision δ13C(CH4) measurements, typically only possible under stable laboratory conditions, with the in situ, near real time data analysis and the large-scale sampling of secluded areas. MIRACLE will be deployed during the DLR GHGMon campaign (June 2023) to investigate the δ13C(CH4) ratio of agricultural sources of methane in the Netherlands.

How to cite: Waldmann, P., Lichtenstern, M., Reum, F., Ziereis, H., Fiehn, A., Gałkowski, M., Gerbig, C., Fix, A., and Roiger, A.: Development and First Deployment of an Innovative Airborne δ13C(CH4) In Situ Measurement Setup, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14191, https://doi.org/10.5194/egusphere-egu23-14191, 2023.

EGU23-14408 | ECS | Orals | AS3.12

Methane emissions from the Baltic Sea nine days after the Nord Stream explosions 

Friedemann Reum, Julia Marshall, Lutz Bretschneider, Michael Glockzin, Heidi Huntrieser, Klaus-Dirk Gottschaldt, Astrid Lampert, Michael Lichtenstern, Scot M. Miller, Falk Pätzold, Magdalena Pühl, Gregor Rehder, and Anke Roiger

The sabotage of the Nord Stream pipelines on 26 September 2022 led to the largest event of methane venting to the atmosphere on record. The pipelines contained about 300 000 tonnes of methane, and an estimate based on Europe's ICOS network quantified the emissions to the atmosphere at 90 000-300 000 tonnes of methane in the first days of the event (Ramonet et al., 2022). The vast majority of methane that vented from the pipelines into the water likely escaped to the atmosphere near-instantly via bubble transport, which had largely ceased by 1 October 2022. However, a fraction dissolved into the water. To investigate the possibility of a "long tail" of release of this dissolved methane to the atmosphere, we conducted airborne surveys of the leak area on 5 October 2022. Methane data were recorded with a Picarro G2401m onboard the HELiPOD platform, a drag probe attached to a helicopter with a rope, down to 30 m above sea level. We observed methane enhancements of up to 300 ppb above atmospheric background, in an area about 30 km both up- and downwind of the leak locations. Using an inverse model of atmospheric transport, we show that the atmospheric data can be explained by an area source and estimate a source strength on the order of tens of tonnes of methane per hour on the day of observations. To better understand the spatial distribution of the emissions, especially emissions upwind of the leak locations, we further run a model of oceanic transport for tracers released at the leak locations and couple it to a Wanninkhof-model of diffusive emissions. The areal emission distribution we find with this model has some similarities to the emission pattern retrieved using the airborne measurements. We conclude that a significant amount of methane was dissolved in the Baltic Sea during the outgassing event following the Nord Stream explosions. Methane that was initially dissolved in the surface layer still escaped to the atmosphere days after the initial outgassing event.

How to cite: Reum, F., Marshall, J., Bretschneider, L., Glockzin, M., Huntrieser, H., Gottschaldt, K.-D., Lampert, A., Lichtenstern, M., Miller, S. M., Pätzold, F., Pühl, M., Rehder, G., and Roiger, A.: Methane emissions from the Baltic Sea nine days after the Nord Stream explosions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14408, https://doi.org/10.5194/egusphere-egu23-14408, 2023.

EGU23-15237 | ECS | Posters on site | AS3.12

O&GProfile : Automated attribution of GHGSat point source methane emissions detections to O&G infrastructures for site emissions profile analysis (Permian) 

Jade Eva Guisiano, Thomas Lauvaux, Claudio Cifarelli, Éric Moulines, and Jérémie Sublime

Methane emissions are the second leading cause of global warming. Because of the near-term warming potential of atmospheric methane, reducing its emissions will be essential to achieve the UNFCCC climate objectives. Reducing methane emissions from oil and gas operations is among the most cost-effective and efficient actions governments can take to meet global climate goals. In the "net zero emissions by 2050" scenario, methane emissions decline rapidly in the coming years, reaching this reduction potential by 2030. This is primarily a result of the rapid deployment of emission reduction measures and technologies, leading to the elimination of all technically avoidable methane emissions within this decade.
Current regulations are based on methane emissions figures from regional and national inventories. However, it has been shown repeatedly in the literature that these have a strong tendency to underestimate actual emission levels. In order to be able to move towards adapted and personalized regulations, it is necessary to aim at new methods -other than the current too generalized inventories- improving the current assessment of emission trends at the level of the whole O&G supply chain. Emission profiles should be estimated by operator, by type of O&G site, or by site infrastructures to design and to implement specific regulations.
In order to establish the most complete emission profiles possible - taking into account the current lack of continuous coverage - a maximum of measurements at various scales (satellite, UAVS, group) of methane emissions for a site or infrastructure should be collected by operator/site/infrastructure.
We therefore propose in this paper O&GProfile,an automatic method  to associate GHGSat methane plume detections to detections from other satellite and airbone campaign already tagged by oil and gas sites type (Gathering & boosting, processing, production) and their respective operators. O&GProfile is based on the use of unsupervised machine learning methods for classification purposes,with automated correction of the classification results. By association of GHGsat data to tagged CarbonMapper and Gao data (method mame), our method provides an informed GHGSat dataset necessary to study profile of emissions by site and operators. The study of these site emissions profiles over the period 2020-2021 in the Delaware and Midland basins in the Permian also allows us to connect GHGSat detections to the Gao and carbon mapper detections.

How to cite: Guisiano, J. E., Lauvaux, T., Cifarelli, C., Moulines, É., and Sublime, J.: O&GProfile : Automated attribution of GHGSat point source methane emissions detections to O&G infrastructures for site emissions profile analysis (Permian), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15237, https://doi.org/10.5194/egusphere-egu23-15237, 2023.

EGU23-15369 | Posters on site | AS3.12

MUCCnet visiting Vienna: refining inverse model prior information with tall-tower flux measurements 

Andreas Luther, Andreas Forstmaier, Haoyue Tang, Juan Bettinelli, Gamal Ghaith, Patrick Aigner, Moritz Makowski, Enrichetta Fasano, Kathiravan M. Meeran, Simon Leitner, Andrea Watzinger, Bradley Matthews, and Jia Chen

More than two thirds of global anthropogenic greenhouse gas (GHG) emissions originate from cities. Urban mitigation policies need a reliable emission data basis to effectively reduce emissions and given inventory uncertainties at the level of single cities, there is growing interest in measurement-based methods to support urban GHG emissions monitoring. Inverse modelling is a measurement-based approach that integrates atmospheric observations with emission inventories, whereby the inventories serve as prior estimates that are subsequently constrained against the observations. While such inverse systems rely on modelling frameworks that typically utilise in situ and/or remote measurements of atmospheric GHG mixing ratios, there is scope for city-scale inverse frameworks to utilise other types of GHG observations, such as flux measurements.

In this study, we investigate such an approach based on a two month field campaign between 15th of May and 20th of July in 2022 in Vienna, Austria. In particular, for the prior information, we use tall-tower eddy covariance observations to constrain the CH4 emissions within the tower's flux footprint and combine the measurements with 1km x 1km inventory data of the larger city area of Vienna. This refined and measurement-supported inventory serves as a-priori information for both, a Bayesian- and a Phillips-Tikhonov based inversion approach. The observational input for the inversion methods is delivered by MUCCnet (Munich Urban Carbon Column network) instruments consisting of four ground-based, sun-viewing FTIR spectrometers (EM27/SUN), with three of these instruments located on the outskirts of Vienna and one instrument located at the bottom of the tall-tower close to the city center. 

This study investigates the synergetic aspects of two different measurement systems: the eddy-covariance system is particularly sensitive to near field emissions with a range of hundreds of meters upwind of the tower, whereas the ground-based remote sensing instruments observe the differential total column concentration and are therefore sensitive to emissions originating several Kilometers upwind. Applying both measurement systems within a city inversion framework may indeed represent a viable option for further constraining city emissions and improving urban GHG emissions monitoring.

How to cite: Luther, A., Forstmaier, A., Tang, H., Bettinelli, J., Ghaith, G., Aigner, P., Makowski, M., Fasano, E., Meeran, K. M., Leitner, S., Watzinger, A., Matthews, B., and Chen, J.: MUCCnet visiting Vienna: refining inverse model prior information with tall-tower flux measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15369, https://doi.org/10.5194/egusphere-egu23-15369, 2023.

EGU23-15766 | Orals | AS3.12

Fugitive Methane Across the UK Gas Distribution Network from Terminals to Cities: Characterisation and Methodology Development 

David Lowry, James France, Julianne Fernandez, Aliah al-Shalan, Rebecca Fisher, Felix Vogel, and Euan Nisbet

Fugitive emissions from gas distribution are a top target for reduction of CH4 emissions to atmosphere with the UN considering that emissions from fossil fuel activities can be reduced by 61% (UN, 2021). Once the emissions are identified there are mitigation solutions to stop the leaks far more easily than emissions from waste and agricultural sectors. The RHUL group has identified fugitive methane from UK sources using a mobile survey vehicle since 2013, initially to identify plumes and characterise the emissions by source category using isotopic signatures (δ13C) and ethane to methane ratios (C2:C1). More recent measurements have focussed on CH4 emissions from buried city gas pipelines, primarily London, and development of methodology for interpreting data from a range of different high-precision instruments.

 

Much of the gas in the UK distribution system has very similar charactersistics once mixing downstream of terminals has taken place. This is typically characterised by δ13C signature of -39 ± 1 ‰ and C2:C1 of 0.055 ± 0.015, which make it distinct from agricultural, waste and combustion CH4 sources. The small proportion of gas coming from the Southern North Sea and Morecambe Bay fields (now <20%) is more enriched in 13C (-34 to -28 ‰) and terminals receiving gas from these locations have different emission signatures; that for the Bacton terminal can be traced downstream toward London.

 

City measurements by Picarro 2301 and LGR UMEA of London and Birmingham pipeline gas leaks in 2019 have been used to quantify emissions using methodology developed by Weller et al. (2019) and refined by Maazallahi et al. (2020). A total estimated emission for the Greater London area of 2.2 kT (Fernandez et al., in prep.), is much lower than the inventory suggests and lower than estimates and from aircraft or fixed site measurements. While fugitive gas emissions from rural areas (pipelines and above-ground infrastructure) are much larger than the inventory suggest, lowering expected urban emissions, and small peaks of <200 ppb cannot be definitively characterised as gas leaks, leading to underestimation, the methodology for leak emissions estimation needs further refinement for dense urban environments. A range of instruments measuring at 0.3 to 10Hz and different emissions methodologies are currently being assessed through repeat surveys of some London boroughs.

 

Maazallahi et al., 2020, Atmos. Chem. Phys., 20, 14717–14740, https://doi.org/10.5194/acp-20-14717-2020

United Nations Environment Programme, 2021, Emissions Gap Report 2021: The Heat Is On – A World of Climate Promises Not Yet Delivered, Nairobi

Weller et al., 2019, PLoS One 14, e0212287, https://doi.org/10.1371/journal.pone.0212287

How to cite: Lowry, D., France, J., Fernandez, J., al-Shalan, A., Fisher, R., Vogel, F., and Nisbet, E.: Fugitive Methane Across the UK Gas Distribution Network from Terminals to Cities: Characterisation and Methodology Development, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15766, https://doi.org/10.5194/egusphere-egu23-15766, 2023.

Acting on the significant contribution of methane to climate change, the global methane emission reduction pledge was launched at the 2021 United Nations Climate Change Conference (COP26) and has been signed by more than 100 countries. The majority of anthropogenic methane emissions have been spewed from the energy, waste and agriculture sectors which can be measured with source-specific choice of instruments, measurement platforms and evaluation methods to feed mitigation plans. Maaz Maps (www.maazmaps.com), with more than a decade of experience in methane emission studies, aims to support the global methane pledge with international collaborations by bridging between academia and industry to fill gaps and accelerate the global methane emission reduction efforts. Currently this startup is contracted by GERG (The European Gas Research Group) to scientifically evaluate methane emission reports from several technology providers: results of a measurement campaign performed at a compressor station will be shown. In this campaign, the technology providers applied bottom-up and top-down quantification methods using in-situ or remote sensing techniques. The instruments were either directly operated by walking individuals or installed on various platforms: helicopter, cars, tripods, drones, truck or poles. Various quantification methods including mass balance, tracer method and inverse modelling, correlation factors were applied to quantify sources. In this presentation, we are going to introduce the startup and reconciliation overview of the bottom-up and top-down quantification methods from the campaign. 

How to cite: Maazallahi, H.: Maaz Maps: a science-based startup to accelerate and support the global methane pledge, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16176, https://doi.org/10.5194/egusphere-egu23-16176, 2023.

EGU23-16557 | ECS | Posters on site | AS3.12

Automated detection and monitoring of methane super-emitters using satellite data 

Berend J. Schuit, Joannes D. Maasakkers, Pieter Bijl, Gourav Mahapatra, Anne-Wil Van den Berg, Mohamed Yaakoub, Sudhanshu Pandey, Alba Lorente, Tobias Borsdorff, Sander Houweling, Daniel J. Varon, Jason McKeever, Dylan Jervis, Marianne Girard, Itziar Irakulis-Loitxate, Javier Gorroño, Luis Guanter, Daniel H. Cusworth, and Ilse Aben

A reduction in anthropogenic methane emissions is vital to limit near-term global warming. A small number of so-called super-emitters is responsible for a disproportionally large fraction of total methane emissions. Since late 2017, the TROPOspheric Monitoring Instrument (TROPOMI) has been in orbit providing daily global coverage of methane mixing ratios at a resolution of up to 7x5.5 km2, enabling the detection of these super-emitters for the first time at global scale. However, TROPOMI produces millions of observations each day, which together with the complexity of the methane data, makes manual inspection infeasible. We have therefore designed a two-step machine learning approach using a Convolutional Neural Network to detect plume-like structures in the methane data and subsequently apply a Support Vector Classifier to distinguish emission plumes from retrieval artefacts. The models are trained on pre-2021 data, and subsequently applied to all 2021 observations. We detect 2974 plumes in 2021 with a mean estimated source rate of 44 t h-1 and 5-95th percentile range of 8-122 t h-1. These emissions originate from 94 persistent emission clusters and hundreds of transient sources. Based on bottom-up emission inventories, we find that most detected plumes are related to urban areas / landfills (35%), followed by plumes from gas infrastructure (24%), oil infrastructure (21%) and coal mines (20%). For twelve (clusters of) TROPOMI detections, we "tip-and-cue" targeted observations and analysis of high-resolution satellite instruments to identify the exact sources responsible for these plumes. Using the high-resolution observations from GHGSat, PRISMA and Sentinel-2, we detect and analyze both persistent and transient facility-level emissions underlying the TROPOMI detections. We will show observations of emissions from landfills and fossil fuel exploitation facilities, for the latter we find up to ten facilities contributing to one TROPOMI detection. In addition to our examination of 2021, we will show results from applying our automated machine learning pipeline continuously on TROPOMI data from as recently as three days ago. Our automated TROPOMI-based monitoring system in combination with high-resolution satellite data allows for the detection, precise identification and monitoring of these methane super-emitters, which is essential for mitigating their emissions and reaching the goals of the Global Methane Pledge of reducing global anthropogenic methane emissions with 30% by 2030.

How to cite: Schuit, B. J., Maasakkers, J. D., Bijl, P., Mahapatra, G., Van den Berg, A.-W., Yaakoub, M., Pandey, S., Lorente, A., Borsdorff, T., Houweling, S., Varon, D. J., McKeever, J., Jervis, D., Girard, M., Irakulis-Loitxate, I., Gorroño, J., Guanter, L., Cusworth, D. H., and Aben, I.: Automated detection and monitoring of methane super-emitters using satellite data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16557, https://doi.org/10.5194/egusphere-egu23-16557, 2023.

This presentation describes the design and implementation of stratospheric aerosol injection (SAI) events in an idealized configuration of the Department of Energy's (DOE) Energy Exascale Earth System Model (E3SMv2). These aerosols are implemented as "tracers" within the framework of the climate model, i.e. dimensionless mixing-ratio quantities which are advected with the winds by the model's transport scheme. The spatio-temporal description of the injected tracer species, as well as their chemical interaction and evolution, are encoded as sub-grid parameterizations via a set of simple ODEs. The form of the equations are designed to mimic materials characteristic of stratospheric volcanic eruptions, specifically those chemical species which are known to perturb the Earth system's energy balance, and thus climate (e.g. sulfate aerosols). Here we employ highly-simplified expressions of these processes by coupling the scalar tracer fields directly to the atmosphere's temperature-- an effect that is normally either mediated by complex chemistry, aerosol, and radiation packages, or prescribed without true tracer transport.  We impose this forcing in an idealized atmosphere that lacks almost all other diabatic forcings normally present in a coupled-climate model. In this way, the effect of specific atmospheric dynamics on the temperature response to the aerosols can be isolated. Output products from this model will be used as validation datasets for the climate source-impact attribution tools currently being developed by the United States Department of Energy's (DOE) CLDERA project.

How to cite: Hollowed, J. and Jablonowski, C.: A Simple Model of Volcanic Aerosol Forcing Against an Idealized Climatological Background in Support of the DOE CLDERA Project, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1720, https://doi.org/10.5194/egusphere-egu23-1720, 2023.

EGU23-1789 | ECS | Posters on site | AS3.13

Impacts of the mid-15th century eruption at Kuwae caldera, Vanuatu 

Sönke Stern, Shane Cronin, Stuart Bedford, Chris Ballard, Robert Henderson, and Salkon Yona

In the AD 1450s, one of the three largest climate-forcing eruptions of the largest 1000 years took place, with similar impacts as the AD 1815 event of Tambora, Indonesia, that caused the ‘year without a summer’ of AD 1816. The submarine caldera of Kuwae, Vanuatu, has long been suggested to be the source of the AD 1450s eruption, but this is still highly debated.

Today, the 12-by-6 km large Kuwae caldera lies between the islands of Epi and Tongoa. Here, an eruption occurred in the 15th century eruption and locally caused devastation, covering the islands surrounding it with vast amounts of pyroclastic material. We present the first full stratigraphy of the event, enabling us to reconstruct the eruptive sequence. First, a small ash plume produced fine ash deposits overlying faulted soil sequences, indicating a low-energy, precursory phase. Afterwards, the eruption built a Plinian eruption column, causing lapilli fall in excess of 3 m in proximal locations, and sending volcanic particles and gases high up into the atmosphere. This column then collapsed, producing the first pyroclastic flows that devastated the islands surrounding the caldera, incorporating many trees that became charcoalised and are still fully preserved in the deposits. Following further pyroclastic flow activity, a massive lithic lag breccia contains megaclasts (>10 m breccia), recording the collapse of a pre-existent edifice. Later pumice-rich pyroclastic flows occurred bring the total thickness of the sequence to between 30 and >80 m in proximal locations.

These results are combined with initial results from a recent bathymetric study, mapping the submarine caldera floor, addressing the question of whether the entire caldera was generated during the mid-15th century event, or whether earlier eruptions have played a part in its collapse. This is essential for estimating the total collapse volume of the mid-15th century event at Kuwae, representative of the total erupted volume.

We will use information on a) the eruptive sequence (based on field observations), b) eruptive volume (based on bathymetry), c) total emitted sulphur (based on eruptive volume and preliminary geochemistry data), and d) the eruptive date (based on radiocarbon analysis of collected charcoal samples) to characterise the mid-15th century eruption of the Kuwae caldera and test whether it was the source of the AD 1450s volcanic event that had a global climate impact.

How to cite: Stern, S., Cronin, S., Bedford, S., Ballard, C., Henderson, R., and Yona, S.: Impacts of the mid-15th century eruption at Kuwae caldera, Vanuatu, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1789, https://doi.org/10.5194/egusphere-egu23-1789, 2023.

EGU23-2604 | Posters on site | AS3.13

The Model Intercomparison Project on the Climatic Response to Volcanic Forcing (VolMIP): Status and Future Perspectives of the Initiative 

Davide Zanchettin, Claudia Timmreck, Myriam Khodri, Gabi Hegerl, Kirstin Krüger, Francesco S. R. Pausata, Alan Robock, Anja Schmidt, and Matthew Toohey

The Model Intercomparison Project on the climatic response to Volcanic forcing (VolMIP) is a protocol-driven international initiative under the umbrella of the sixth phase of the Coupled Model Intercomparison Project (CMIP6) aiming at coordinating the activities of different Research Institutes involved in numerical climate modelling focused on a multi-model assessment of climate models' performance under strong volcanic forcing conditions. The main objective of the initiative is to assess to what extent responses of the coupled ocean-atmosphere system to the same applied strong volcanic forcing are robustly simulated across state-of-the-art coupled climate models and identify the causes that limit robust simulated behavior, especially differences in their treatment of physical processes. To this purpose, four Tier-1 (mandatory) experiments branched into two main sets, named “volc-pinatubo” and “volc-long” were defined, together with eight more lower-priority experiments. Six years since the definition of the VolMIP protocol (Zanchettin et al., 2016), ensemble simulations of most of the mandatory VolMIP experiments have been completed and made publicly available through the Earth System Grid Federation open platform, with the first VolMIP results being currently published and several analyses in progress. The long turnover time between the experiment design, the integration of the simulations and the analysis of the output motivates an assessment of the overall effectiveness of the VolMIP strategy, particularly in the light of a possible second phase of the initiative.

In this contribution, we will illustrate the status of the initiative, highlight its major achievements and discuss its future perspective in the light of emergent scientific questions regarding volcanically forced climate variability.

Zanchettin, D., Khodri, M., Timmreck, C., Toohey, M., Schmidt, A., Gerber, E. P., Hegerl, G., Robock, A., Pausata, F. S. R., Ball, W. T., Bauer, S. E., Bekki, S., Dhomse, S. S., LeGrande, A. N., Mann, G. W., Marshall, L., Mills, M., Marchand, M., Niemeier, U., Poulain, V., Rozanov, E., Rubino, A., Stenke, A., Tsigaridis, K., and Tummon, F.: The Model Intercomparison Project on the climatic response to Volcanic forcing (VolMIP): experimental design and forcing input data for CMIP6, Geosci. Model Dev., 9, 2701–2719, https://doi.org/10.5194/gmd-9-2701-2016, 2016

How to cite: Zanchettin, D., Timmreck, C., Khodri, M., Hegerl, G., Krüger, K., Pausata, F. S. R., Robock, A., Schmidt, A., and Toohey, M.: The Model Intercomparison Project on the Climatic Response to Volcanic Forcing (VolMIP): Status and Future Perspectives of the Initiative, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2604, https://doi.org/10.5194/egusphere-egu23-2604, 2023.

EGU23-3331 | ECS | Orals | AS3.13

Insensitivity of global temperature response to the magnitude of volcanic eruptions 

Eirik Enger, Audun Theodorsen, Maria Rugenstein, and Rune Graversen

We investigate how the global mean temperature responds to single volcanic events of different magnitudes and to multiple events occurring close in time. We are using the Community Earth System Model version 2 (CESM2) to simulate the Earth system forced only with stratospheric aerosols from explosive volcanoes, with the rest of the climate system fixed at 1850 conditions. The model is run with a dynamical ocean component, and the Whole Atmosphere Community Climate Model version 6 (WACCM6) atmosphere component using middle atmosphere chemistry.

Previous efforts of estimating a response function assume a linear relationship between the forcing and the deterministic temperature response to the forcing [1], defined as Tdet(t)=L[F(t)]. Studies also show that the forcing is similar across forcing agents [2] (although this is not a settled debate [3]), in which case volcanoes could provide a valuable means of estimating global temperature response to radiative forcing due to their short-lived and large temperature responses.

We present simulations of single volcano events with ejected sulphate aerosol loadings differing in orders of magnitude and simulations where two volcanic eruptions are close enough in time that the second eruption occurs as the temperature is still recovering from the first event.

We show that the functional form of the temperature response is similar for volcanic events of different magnitudes and that non-linearities are not important as a second eruption occurs when the temperature is well below equilibrium in a perturbed state. The results further suggest the global mean temperature time series may be reduced to a simple superposition of individual pulses, and thus that it may be described by a convolution between a linear response function and some forcing, analogous to the model used by [1].

[1] K. Rypdal and M. Rypdal, ‘Comment on “Scaling regimes and linear/nonlinear responses of last millennium climate to volcanic and solar forcing” by S. Lovejoy and C. Varotsos (2016)’, Earth System Dynamics, 2016, vol. 7, no. 3, pp. 597–609.
[2] T. B. Richardson et al., ‘Efficacy of Climate Forcings in PDRMIP Models’, Journal of Geophysical Research: Atmospheres, 2019, vol. 124, no. 23, pp. 12824–12844.
[3] P. Salvi, P. Ceppi, and J. M. Gregory, ‘Interpreting differences in radiative feedbacks from aerosols versus greenhouse gases’, Geophysical Research Letters, 2022, vol. 49, no. 8, p. e2022GL097766.

How to cite: Enger, E., Theodorsen, A., Rugenstein, M., and Graversen, R.: Insensitivity of global temperature response to the magnitude of volcanic eruptions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3331, https://doi.org/10.5194/egusphere-egu23-3331, 2023.

EGU23-3638 | Posters on site | AS3.13

Revisiting the mechanisms of ENSO response to tropical volcanic eruptions 

Francesco S.R. Pausata, Yang Zhao, Davide Zanchettin, Rodrigo Caballero, and David Battisti

Large explosive volcanic eruptions can have major impacts on global climate, affecting both radiative balance and inducing interannual-to-decadal dynamical alterations of the atmospheric and ocean circulation. 

Despite some discrepancies across studies regarding the response of ENSO to volcanism based on paleoclimate data, the majority of ENSO reconstructions  display an El Niño–like warming in the year of eruption, while none display a significant La Niña–like response, Furthermore, there has been an emerging consensus from the numerous coupled General Circulation Model studies investigating the impact of tropical volcanism on ENSO, with the overwhelming majority displaying an El Niño–like warming occurring in the year following the eruption. However, the mechanisms that trigger a change in the ENSO state following volcanic eruptions are still debated. The center of the argument is understanding how volcanism can affect the trade winds along the equatorial Pacific.

Here, we shed light on the processes that govern the ENSO response to tropical volcanic eruptions through a series of sensitivity experiments with an Earth System Model where a uniform stratospheric volcanic aerosol loading is imposed over different parts of the tropics. Three tropical mechanisms are tested: the “ocean dynamical thermostat” (ODT); the cooling of the Maritime Continent; and the cooling of tropical northern Africa (NAFR). We find that the NAFR mechanism plays the largest role, while the ODT mechanism is absent in our simulations as La Niña-like rather than El-Niño-like conditions develop following a uniform radiative forcing over the equatorial Pacific.

How to cite: Pausata, F. S. R., Zhao, Y., Zanchettin, D., Caballero, R., and Battisti, D.: Revisiting the mechanisms of ENSO response to tropical volcanic eruptions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3638, https://doi.org/10.5194/egusphere-egu23-3638, 2023.

EGU23-3656 | Posters on site | AS3.13

Radiative forcing by stratospheric aerosol from volcanoes and major fires for the last 3 decades 

Christoph Brühl, Jennifer Schallock, Jos Lelieveld, and Landon Rieger

We present instantaneous forcing computed in a transient simulation with the chemistry climate model EMAC considering more than 600 explosive eruptions and plumes of major forest fires observed by limb scanning satellites in the period 1991 to 2021. If not available directly, perturbations of SO2 in the volcanic plumes, which we use as alternative to the "point source approach", were derived from observed extinctions. For the fires, black and organic carbon is injected at the top of the pyro-cumulonimbus and the resulting increase in extinction is compared with satellite data. Medium sized volcanic eruptions cause a total forcing of up to -0.35W/m2 at the top of the atmosphere while for the fires the forcing there can be positive (about 0.2W/m2).

How to cite: Brühl, C., Schallock, J., Lelieveld, J., and Rieger, L.: Radiative forcing by stratospheric aerosol from volcanoes and major fires for the last 3 decades, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3656, https://doi.org/10.5194/egusphere-egu23-3656, 2023.

EGU23-4474 | Orals | AS3.13

Initial meteorological conditions and eruption source parameters control on volcanic forcing 

Kirstin Krüger, Zhihong Zhuo, Herman Fuglestvedt, Mike Mills, and Matthew Toohey

Studying impacts of past volcanic eruptions on climate and society relies on volcanology, paleo proxies and archaeological records next to climate model simulations. Here we newly study the control of varying meteorological conditions and eruption source parameters on the volcanic forcing. Simulating explosive tropical and extratropical Northern Hemisphere (NH) volcanic eruptions are carried out by co-injecting sulfur and halogens into the stratosphere with the CESM2(WACCM) model including aerosol, chemistry, climate, and earth system processes. We consider different initial meteorological conditions (ENSO, QBO, and polar vortex states) and varying eruption source parameters injecting 17 Tg and 200 Tg of SO2 together with scaled halogens, at 24 km altitude and 15° N and 64° N latitude, during January and July pre industrial 1850 conditions. Varying initial meteorological conditions reveal a similar large impact on the volcanic forcing (SO2, SO4, aerosol optical depth, halogens) as varying source parameters for both tropical and NH extratropical eruptions. Our results are compared with available model experiments from MAECHAM5-HAM. Consequences and uncertainties of volcanic forcing and responses to past and future eruptions are discussed. 

How to cite: Krüger, K., Zhuo, Z., Fuglestvedt, H., Mills, M., and Toohey, M.: Initial meteorological conditions and eruption source parameters control on volcanic forcing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4474, https://doi.org/10.5194/egusphere-egu23-4474, 2023.

EGU23-4536 | Orals | AS3.13

Solar radiation management from Icelandic volcanoes during the Medieval Quiet Period 

Michael Sigl, Imogen Gabriel, Peter Abbott, Melanie Behrens, Andrea Burke, Nathan Chelman, Eliza Cook, Dominik Fleitmann, Herman Fuglestvedt, Maria Hörhold, William Hutchison, Kirstin Krüger, Joseph R. McConnell, Bergrún Arna Óladóttir, Gill Plunkett, Johannes Preiser-Kapeller, and Zhihong Zhuo

“Solar Radiation Management” aims to mitigate global warming by either seeding aerosols into clouds to change their radiative properties and occurrence frequency, or injecting sulfur into the atmosphere to shield the Earth’s surface from incoming solar radiation. These approaches are inspired, among other things, by the effect of volcanic eruptions on the climate system.

Here we provide a critical reassessment of a time period commonly referred to as the “Medieval Quiet Period”. For several centuries in early Medieval times (c. 750-1050 CE) the climate system was postulated to have been relatively unperturbed by natural climate forcing, resulting in a unique period of climate stability. We present evidence that just the opposite is true. In large parts of the Northern Hemisphere and in the Arctic, atmospheric aerosol loads were persistently high during this period as a result of increased volcanic activity, especially in Iceland.

Our new insight is supported by evidence taken from an array of synchronized ice cores from Greenland with high time-resolution records of a large suite of trace elements, including volcanic volatiles such as sulfur, chlorine, fluorine, and heavy metals. We use crypto-tephra in ice cores to provenance the sources of many volcanic eruptions and sulfur isotopes (33S, 34S) to delineate if volcanic gas emissions occurred above or below the ozone layer.

We define an “Iceland Active Period”, a time period of frequent and prolonged volcanic activity, producing persistently high levels in atmospheric aerosol burdens in the Northern Hemisphere Arctic’s preindustrial atmosphere lasting for decades to centuries. The frequency and cumulative amount of emissions of climate-impacting trace substances (e.g., sulfates, halogens, ash) is unprecedented in the late Holocene. It is exceeded at times only in the Anthropocene (since about 1900) and in the early-middle Holocene (e.g. during rapid deglaciation). We demonstrate that previous reconstructions of volcanic forcing used in PMIP3 and PMIP4 strongly underestimate volcanic aerosol emissions in the early Medieval and argue that this period should not be considered a reference climate state for the Common Era.

Finally, we investigate possible aerosol-climate interactions following these eruptions using climate proxies and state-of-the-art chemistry climate models with prognostic stratospheric aerosols and chemistry.

How to cite: Sigl, M., Gabriel, I., Abbott, P., Behrens, M., Burke, A., Chelman, N., Cook, E., Fleitmann, D., Fuglestvedt, H., Hörhold, M., Hutchison, W., Krüger, K., McConnell, J. R., Óladóttir, B. A., Plunkett, G., Preiser-Kapeller, J., and Zhuo, Z.: Solar radiation management from Icelandic volcanoes during the Medieval Quiet Period, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4536, https://doi.org/10.5194/egusphere-egu23-4536, 2023.

EGU23-4560 | Posters on site | AS3.13

Decline in the Mediterranean Etesian winds after large volcanic eruptions in the last millennium 

Stergios Misios, Ioannis Logothetis, Mads F. Knudsen, Christoffer Karoff, Vassilis Amiridis, and Kleareti Tourpali

The northerly Etesian winds are a stable summertime circulation system in the eastern Mediterranean, emerging from a steep pressure gradient between the central Europe and Balkans high-pressure and the Anatolian low pressure systems. Etesian winds are influenced by the variability in the Indian summer monsoon (ISM), but their sensitivity to external forcing on interannual and longer timescales is not well understood. Here we investigate the sensitivity of Etesian winds to large volcanic eruptions in a set of model simulations over the last millennium and reanalysis of the 20th century. We provide model evidence for significant volcanic signatures, manifested as a robust reduction in the wind speed and the total number of days with Etesian winds in July and August. These are robust responses to all strong eruptions in the last millennium, and in the extreme case of Samalas, the ensemble-mean response suggests a post-eruption summer without Etesians. The significant decline in the number of days with Etesian winds is attributed to the weakening of the ISM in the post-eruption summers, which is associated with a reduced large-scale subsidence and weakened surface pressure gradients in the eastern Mediterranean. Our analysis identifies a stronger sensitivity of Etesian winds to the Northern Hemisphere volcanic forcing, particularly for volcanoes before the 20th century, while for the latest large eruption of Pinatubo modelled and observed responses are insignificant. 

How to cite: Misios, S., Logothetis, I., Knudsen, M. F., Karoff, C., Amiridis, V., and Tourpali, K.: Decline in the Mediterranean Etesian winds after large volcanic eruptions in the last millennium, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4560, https://doi.org/10.5194/egusphere-egu23-4560, 2023.

Several studies have reported anomalous precipitation in the years that follow large volcanic eruptions. Here we assess precipitation anomalies in post-eruption years according to their rarity in non-volcanic periods. Using global simulations of climate over the last millennium, we reevaluate the response of precipitation to volcanic aerosols in terms of novel metrics. In this approach, the magnitude of the precipitation response is contextualized through comparisons to internal variability. We also examine the connections between global and regional-scale precipitation anomalies. Finally, we assess to what extent a unique ‘fingerprint’ of eruptions can be seen in the observational precipitation record in spite of concurrent internal variability.

How to cite: McGraw, Z. and Polvani, L.: Reassessing post-eruption precipitation anomalies in the context of natural variability, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4691, https://doi.org/10.5194/egusphere-egu23-4691, 2023.

EGU23-5428 | Posters on site | AS3.13

Linear precipitation response to increasingly strong volcanic eruptions and its emergence from internal variability 

Claudia Timmreck, Dirk Olonscheck, Andrew Ballinger, Roberta D'Agostino, Shih-Wei Fang, Gabriele Hegerl, and Andrew Schurer

Large explosive volcanic eruptions are a potential source of uncertainty in future climate projections as they cannot be predicted in advance, but eventually will occur, causing short-term climatic impacts on both local and global scale. Still, an open topic is the volcanic impact on tropical climate variability, in particular El Niño Southern Oscillation (ENSO) and tropical precipitation and the combined effect of both. Sufficient large ensembles simulations with the same model and radiative forcing scenario but varying initial conditions have become a great tool in recent years to disentangle forced and internal variability).  Here we use the EVA-ENS ensemble (Azoulay et al., 2021) which consists of 100-member ensembles of the MPI-ESM-LR for idealized equatorial Pinatubo-like eruptions of different eruption strength and an additional 100-member ensemble without forcing. We are in particular interested if there is a linear volcanic signal on tropical precipitation dependent on the eruption strength and when did it emerge from tropical internal variability.

Our results show that for Idealized tropical eruptions global and large hemispheric mean 2m temperature and precipitation anomalies seemed to be scalable with the sulfur emission strength above a certain threshold, except for tropical temperatures for an emission strength > 40 Tg  sulfur (S). 10 Tg S emission, the upper estimate of the 1991 Pinatubo eruption, seems to be a threshold where the signal is discernible from internal variability. We also find that seasonal and ensemble mean pattern correlation of 2m temperature and precipitation anomalies are highly correlated in particular for larger emission strengths in the tropics and strongly modulated by ENSO.  There is an increasing tendency for a warm ENSO increases with eruption strength. Emergence of the volcanic signal appears for smaller eruption strength when looking to ENSO composites.  Emergence of cooling appears on a hemispheric scale, while precipitation response is more localized and mainly confined to the tropics and subtropics.

 References:

Azoulay, A., Schmidt, H., and Timmreck, C.: The Arctic polar vortex response to volcanic forcing of different strengths, J. Geophys. Res., 126, e2020JD034450, doi.org/10.1029/2020JD034450, 2021.

How to cite: Timmreck, C., Olonscheck, D., Ballinger, A., D'Agostino, R., Fang, S.-W., Hegerl, G., and Schurer, A.: Linear precipitation response to increasingly strong volcanic eruptions and its emergence from internal variability, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5428, https://doi.org/10.5194/egusphere-egu23-5428, 2023.

EGU23-5788 | ECS | Orals | AS3.13

Stratospheric aerosol size decrease after volcanic eruptions 

Felix Wrana, Ulrike Niemeier, Sandra Wallis, and Christian von Savigny

The evolution of the size distribution of stratospheric aerosols after volcanic eruptions is still not understood very well, due to the temporal sparsity of in situ measurements, the low spatial coverage by ground based observations and the difficulties to derive aerosol size information from satellite measurements. To contribute to this ongoing research, we show data from our aerosol size retrieval using SAGE III/ISS solar occultation measurements. Using a three wavelength extinction approach the parameters of assumed to be monomodal lognormal particle size distributions are retrieved.

Surprisingly we find that some volcanic eruptions can lead to a decrease in average stratospheric aerosol size, in this case the eruptions of Ambae in 2018, Ulawun in 2019 and La Soufrière in 2021, while other eruptions have a more expected increasing effect on the average particle size, like the 2019 Raikoke eruption. We show how different parameters like the median radius, the absolute mode width and the number density evolve after the mentioned eruptions.

Additionally, as a part of our ongoing research to understand the underlying mechanisms controlling the observed aerosol size reduction, we show simulations of the aforementioned volcanic eruptions using the aerosol-climate model MAECHAM5-HAM. Although the initial conditions in the model simulations are different from observations due to missing smaller emissions in the time before the eruptions, a good agreement in the perturbations of the extinction coefficient was achieved.

How to cite: Wrana, F., Niemeier, U., Wallis, S., and von Savigny, C.: Stratospheric aerosol size decrease after volcanic eruptions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5788, https://doi.org/10.5194/egusphere-egu23-5788, 2023.

EGU23-5957 | Orals | AS3.13 | Highlight

Global perturbation of stratospheric water and aerosol burden by the Hunga Tonga eruption: a 1-year aftermath 

Sergey Khaykin, Aurelien Podglajen, Felix Ploeger, Jens-Uwe Grooß, Florent Tence, Konstantin Khlopenkov, Kristopher Bedka, Landon Rieger, Alexandre Baron, Valentin Duflot, Benjamin Clouser, Tetsu Sakai, Sophie Godin-Beekmann, Slimane Bekki, and Richard Querel

The eruption of the submarine Hunga Tonga Hunga Hapaii volcano on 15 January 2022 was associated with a powerful blast that injected sulfur and water to altitudes up to 58 km. In this study, we combine the data from various satellite instruments (MLS, OMPS-LP, CALIOP, SAGE III, Aeolus, COSMIC-2, ACE-FTS, GOES, Himawari), ground-based lidars at various locations, meteorological radiosoundings as well as model simulation using CLaMS chemistry-transport model to investigate the evolution of the stratospheric moisture and sulfate aerosol plume at a wide range of scales—from minutes and kilometres to monthly and planetary scale. We show that due to extreme altitude reach of the eruption, the volcanic plume has circumnavigated the Earth in only one week and dispersed nearly pole-to-pole in three months. The observations provide evidence for an unprecedented increase in the global stratospheric water mass by 13% as compared to climatological levels. As there are no efficient sinks of water vapour in the stratosphere, this perturbation is expected to persist several years. The eruption has also led to a 5-fold increase in the stratospheric aerosol load, the highest in the last three decades yet factor of 6 smaller than the previous major eruption of Mt Pinatubo in 1991.

The unique nature and magnitude of the global stratospheric perturbation by the Hunga eruption ranks it among the most remarkable climatic events in the modern observation era. Given the expected longevity of the stratospheric humidity perturbation, the Hunga eruption can be said to have initiated a new era in stratospheric gaseous chemistry and particle microphysics with a wide range of potential long-lasting repercussions for the global stratospheric composition and dynamics. The eruption has thus provided a unique natural testbed, lending itself to studies of climate sensitivity to strong change in both stratospheric gaseous and particulate composition.

Spanning more than one year, the satellite and ground-based observations available to-date enable the first accurate assessment of the annual-scale stratospheric aftermath of the Hunga Tonga eruption, uncovering its climate-altering capacity.

How to cite: Khaykin, S., Podglajen, A., Ploeger, F., Grooß, J.-U., Tence, F., Khlopenkov, K., Bedka, K., Rieger, L., Baron, A., Duflot, V., Clouser, B., Sakai, T., Godin-Beekmann, S., Bekki, S., and Querel, R.: Global perturbation of stratospheric water and aerosol burden by the Hunga Tonga eruption: a 1-year aftermath, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5957, https://doi.org/10.5194/egusphere-egu23-5957, 2023.

EGU23-6882 | Orals | AS3.13

Understanding the impact of Hunga-Tonga undersea eruption on the stratospheric aerosol population using Balloon measurements, Satellite data, and model simulations 

Hazel Vernier, Demilson Quintão, Bruno Biazon, Eduardo Landulfo, Giovanni Souza, Fabio J. S. Lopes, Neeraj Rastogi, Rohit Meena, Hongyu Liu, Suvarna Fadnavis, Johnny Mau, Amit K. Pandit, Gwenael Berthet, and Jean-Paul Vernier

The stratospheric aerosol layer has witnessed large perturbations in the last couple of years. From extreme wildfires in North America and Australia to medium-size volcanic eruptions like Ambae, in July 2018, Raikoke, in 2019, and finally the Hunga-Tonga Ha’apai in January 2022. Reported as the largest marine eruption ever recorded, researchers used Microwave Limb Sounder (MLS) satellite data to reveal that this volcano injected the equivalent of 10% of the total stratospheric water vapor content (100 Tg) into the stratosphere. As a consequence, increased OH radicals from water vapor were reported to further reduce the SO2 lifetime by 50%.

Here we outline the ionic composition, in parallel with microphysical, chemical, and optical properties of stratospheric aerosols using balloon measurements from Brazil 5-7 months after the eruption, in comparison with satellite data and model simulations. Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) and ground-based lidar measurements revealed the existence of a volcanic plume between 20 and 25 km. Particle size information derived from balloon-borne optical counters showed the presence of aerosols with a size radius >0.3µm and their subsequent sedimentation. In addition, ion chromatographic analysis of samples collected within the plume using a light-weight aerosol sampler revealed the presence of ammonia (0.3 ng/m3), sulfate (0.4 ng/m3), nitrate (1 ng/m3), and nitrite (1 ng/m3) in addition to Potassium (0.14 ng/m3), magnesium (0.12 ng/m3), and calcium (0.2 ng/m3). One of the striking findings of our measurements was the existence of traces of Dimethylamine (DMA) in our flights alongside the above-mentioned ionic components. DMA is known to enhance new particle formation upon reacting with H2SO4 and could have played an important role in the volcanic plume microphysical evolution. Although satellite data have revealed the presence of SO2 it is still uncertain if the SO2 only evolved from the Hunga-Tonga itself or as a consequence of a marine eruption that could have emitted Dimethylsulfuroxide (DMSO) into the stratosphere resulting in sulfate production.

 

 

How to cite: Vernier, H., Quintão, D., Biazon, B., Landulfo, E., Souza, G., J. S. Lopes, F., Rastogi, N., Meena, R., Liu, H., Fadnavis, S., Mau, J., K. Pandit, A., Berthet, G., and Vernier, J.-P.: Understanding the impact of Hunga-Tonga undersea eruption on the stratospheric aerosol population using Balloon measurements, Satellite data, and model simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6882, https://doi.org/10.5194/egusphere-egu23-6882, 2023.

EGU23-7109 | Orals | AS3.13

High-resolution sulfur isotopes from ice cores: improved estimates of the volcanic forcing of climate 

Andrea Burke, Helen Innes, Laura Crick, Kevin Anchukaitis, William Hutchison, Joseph McConnell, James Rae, Michael Sigl, and Robert Wilson

The record of the volcanic forcing of climate over the past 2500 years is reconstructed primarily from sulfate concentrations in ice cores. Of particular interest are stratospheric eruptions, as these afford sulfate aerosols the longest residence time and largest dispersion in the atmosphere, and thus the greatest impact on radiative forcing.  Sulfur isotopes can be used to distinguish between stratospheric and tropospheric volcanic sulfate in ice cores since stratospheric sulfur aerosols are exposed to UV radiation which imparts a mass independent fractionation (Savarino et al., 2003). Thus, sulfur isotopes in ice cores provide a means to identify stratospheric eruptions and calculate the proportion of sulfate deposited from a volcanic event that came the stratosphere, allowing us to refine the historic record of explosive volcanism and its forcing of climate.  Here we present high-resolution (sub-annual) sulfur isotope data from both Greenland and Antarctica across a suite of unidentified eruptions from the anomalously cold decades of the 530s CE, 1450s CE and 1600s CE, as well as the newly identified eruption of Okmok in 43 BC (McConnell et al., 2020), to investigate the stratospheric sulfur loading and climate forcing potential of these eruptions.

 

 

Savarino, J., Romero, A., Cole Dai, J., Bekki, S., & Thiemens, M. H. (2003). UV induced mass‐independent sulfur isotope fractionation in stratospheric volcanic sulfate. Geophysical Research Letters, 30(21). http://doi.org/10.1029/2003GL018134

McConnell, J. R., Sigl, M., Plunkett, G., Burke, A., Kim, W. M., Raible, C. C., et al. (2020). Extreme climate after massive eruption of Alaska’s Okmok volcano in 43 BCE and effects on the late Roman Republic and Ptolemaic Kingdom. Proc Natl Acad Sci USA, 117(27), 15443.

How to cite: Burke, A., Innes, H., Crick, L., Anchukaitis, K., Hutchison, W., McConnell, J., Rae, J., Sigl, M., and Wilson, R.: High-resolution sulfur isotopes from ice cores: improved estimates of the volcanic forcing of climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7109, https://doi.org/10.5194/egusphere-egu23-7109, 2023.

EGU23-7296 | ECS | Posters on site | AS3.13

Revisiting the volcanic forcing of high-latitude Northern Hemisphere eruptions 

Herman Fuglestvedt, Zhihong Zhuo, Matthew Toohey, and Kirstin Krüger

Large high-latitude explosive volcanic eruptions remain less well understood than their low-latitude counterparts, despite their potential for strong hemispheric climate impacts. Using the high-top coupled Earth system model CESM2-WACCM6 with prognostic stratospheric aerosols and chemistry, we simulate Pinatubo-magnitude Northern Hemisphere (NH) volcanic eruptions at 64° N. We show how the SO2 lifetime and growth of volcanic sulphate aerosols are strongly modulated by the initial state of the NH polar vortex for eruptions at this latitude. The resulting variability of the volcanic forcing is of comparable magnitude to its sensitivity to varying the plume composition, eruption season, and plume height. We compare the modelled volcanic sulphate deposition over the Greenland ice sheet to that assumed in current forcing reconstructions of past NH extratropical eruptions and provide a new model-based estimate of the magnitude and uncertainty of the transfer function used to reconstruct sulphur injections from such eruptions. Our results demonstrate the great potential for improvement in understanding and reconstructing the climatic impacts of NH high-latitude eruptions.

How to cite: Fuglestvedt, H., Zhuo, Z., Toohey, M., and Krüger, K.: Revisiting the volcanic forcing of high-latitude Northern Hemisphere eruptions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7296, https://doi.org/10.5194/egusphere-egu23-7296, 2023.

EGU23-9208 | Posters on site | AS3.13

Tomographic retrievals of Hunga Tonga-Hunga Ha’apai volcanic aerosol 

Adam Bourassa, Daniel Zawada, Landon Rieger, and Doug Degenstein

The 2022 eruption of the Hunga Tonga-Hunga Ha’apai volcano caused substantial impacts on the atmosphere, including a large increase of stratospheric aerosol at high altitudes and a massive injection of water vapor.  We show results from application of a two-dimensional tomographic retrieval of aerosol extinction profiles from limb scattered sunlight made by the NASA OMPS Limb Profiler instrument. The tomographic retrieval substantially improves the agreement in magnitude and vertical structure with coincident lidar and occultation observations compared to the standard retrieval. We also show a secondary effect of bias from uncertainty in assumed particle size distribution parameters that results in a systematic underestimation of the aerosol extinction in the altitude region of the peak of the volcanic aerosol layer.

How to cite: Bourassa, A., Zawada, D., Rieger, L., and Degenstein, D.: Tomographic retrievals of Hunga Tonga-Hunga Ha’apai volcanic aerosol, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9208, https://doi.org/10.5194/egusphere-egu23-9208, 2023.

EGU23-12631 | Orals | AS3.13

Inverse Modeling of the Initial Stage of the 1991 Pinatubo Volcanic Cloud Accounting for Radiative Feedback of Volcanic Ash 

Alexander Ukhov, Georgiy Stenchikov, Sergey Osipov, Nickolay Krotkov, Nick Gorkavyi, Can Li, Oleg Dubovik, and Anton Lopatin

The evolution of volcanic clouds is sensitive to the initial three-dimensional (3D) distributions of volcanic material, which are often unknown. Here, we conduct inverse modeling of the fresh Mt. Pinatubo cloud to estimate the time-dependent emissions profiles and initial 3D spatial distributions of volcanic ash and SO2. We account for aerosol radiative feedback and dynamic lofting of volcanic ash. It results in a lower (by 1 km for ash) injection height than that without ash radiative feedback. The solution captures the elevated ash layer between 14 and 24 km and the meridional height gradient during the first two days after an eruption. A significant fraction of the emissions (i.e., 6/16.6 Mt of  SO2 and 34/64.22 Mt of fine ash) did not reach the stratosphere. The results demonstrate that the Pinatubo eruption ejected ~78% of fine ash at 12 to 23 km, ~64% of  SO2 at 17 to 23 km, and most of the ash and  SO2 mass for the first two days after the eruption resides in the 15- to 22- km layer. 6 Mt of tropospheric  SO2 oxidized into sulfate aerosol within a week. This outcome might help to explain the discrepancies between the observations and model simulations recently discussed in the literature. The long-term evolution of the Pinatubo aerosol optical depth simulated using the obtained ash and  SO2 initial distributions converges with the available stratospheric aerosol and gas experiment (SAGE) observations a month after the eruption when the tropospheric aerosol cloud dissipated.

How to cite: Ukhov, A., Stenchikov, G., Osipov, S., Krotkov, N., Gorkavyi, N., Li, C., Dubovik, O., and Lopatin, A.: Inverse Modeling of the Initial Stage of the 1991 Pinatubo Volcanic Cloud Accounting for Radiative Feedback of Volcanic Ash, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12631, https://doi.org/10.5194/egusphere-egu23-12631, 2023.

The Raikoke volcano erupted on 21-22 June 2019 and emitted ~1.5 Tg volcanic ash into the atmosphere. Several previous studies have focused on the large-scale dispersion of volcanic aerosol plumes with space-borne observations and dispersion models. However, height-resolved ground-based observations are still necessary to trace and cross-check the 3-D evolution of aerosol plumes due to their complicated structures. Here, we present a rare ground-based lidar observation of Raikoke aerosol plumes in the mid-latitudes of the Northern Hemisphere (site: Wuhan; location: 30.5°N, 114.4°E) from 25 July to 30 September 2019. Two types of volcanic aerosol plumes were observed, including the main aerosol plume and a single impacted aerosol cloud (referred to as ‘CCC’, or coherent circular clouds). The main aerosol plume first arrived at Wuhan on 25 July and was intermittently observed during the following two months at altitudes of 15.0-20.5 km, with layer-integrated AODs (aerosol optical depths) of 0.001-0.017. From 22 August to 23 September, this aerosol plume underwent two quasi-elliptical transport pathways in East Asia driven by an Asian monsoon anticyclone. The CCC arrived at Wuhan twice at 20.2-21.7 km on 30 July and at 23.2-25.0 km on 24-26 August after self-lofting, corresponding to the former two circles of their transport around the Northern Hemisphere. Both arrivals of the CCC were closely followed by a thin and horizontally extended aerosol plume (named ‘trail’) with a duration of several days. The unique observation location provided us with an opportunity to study the evolution of the vertical distribution and optical properties of volcanic aerosols, which is anticipated to be a crucial supplement/reference for dispersion model simulation, data assimilation, and forecasting refinement.

How to cite: He, Y., Jing, D., and Yin, Z.: Evolution of aerosol plumes from 2019 Raikoke volcanic eruption observed with polarization lidar over central China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13549, https://doi.org/10.5194/egusphere-egu23-13549, 2023.

EGU23-13861 | Posters virtual | AS3.13

Stratospheric aerosol extinction profiles retrieved from twilight sky spectral measurements above Georgia, South Caucasus in 2021-2022. 

Nina Mateshvili, Iuri Mateshvili, Noel Baker, Antonin Berthelot, Christine Bingen, Emmanuel Dekemper, Philippe Demoulin, Ghislain Franssens, Didier Fussen, Erkki Kyrölä, Tamar Paatashvili, Didier Pieroux, and Filip Vanhellemont

Narrow field-of view spectral measurements of twilight sky brightness as a function of solar zenith angle in the 89°-95° range allow to retrieve lower stratospheric and tropospheric aerosol extinction profiles. The measurements were carried out over Tbilisi, Georgia, South Caucasus during 2021-2022 in the 700-800 nm wavelength range using a SBIG ST9 CCD camera and a SBIG SGS spectrograph. The Monte Carlo code Siro, developed in the Finnish Meteorological Institute was used to design a forward model. Aerosol extinction profiles at 780 nm were retrieved using the Levenberg–Marquardt algorithm.

Stratospheric aerosol loading was low in the considered period whereas the upper (about 9-10 km) and lower troposphere (about 4-5 km) were sometimes disturbed due to small volcanic eruptions and dust transport events. Particularly, ash clouds from Etna eruptions on 10 and 21 February were observed at about 9 km altitude.

How to cite: Mateshvili, N., Mateshvili, I., Baker, N., Berthelot, A., Bingen, C., Dekemper, E., Demoulin, P., Franssens, G., Fussen, D., Kyrölä, E., Paatashvili, T., Pieroux, D., and Vanhellemont, F.: Stratospheric aerosol extinction profiles retrieved from twilight sky spectral measurements above Georgia, South Caucasus in 2021-2022., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13861, https://doi.org/10.5194/egusphere-egu23-13861, 2023.

EGU23-14017 | ECS | Posters on site | AS3.13

How much does ice sheet sulfate deposition tell us about volcanic forcing? 

Lauren Marshall, Matthew Toohey, and Anja Schmidt

Current reconstructions of volcanic forcing over the last 2000 years rely on scaling volcanic sulfate measured in ice cores to estimates of stratospheric sulfate burdens and optical properties using relationships derived from the 1991 eruption of Mt. Pinatubo. However, there are large uncertainties associated with these conversions and consequently a large uncertainty in the reconstructions. Here, we explore the relationship between ice sheet sulfate deposition and volcanic forcing in model simulations of the last millennium conducted using the UK Earth System Model with an interactive stratospheric aerosol scheme. Treating the model sulfate deposition timeseries as a measured ice-core record and using established conversions, we explore how many of the large-magnitude volcanic events simulated in the model are missed by looking at deposition alone, and how the volcanic forcing may be overpredicted or underpredicted compared to the model itself. These results will enable us to further explore uncertainty in these relationships, and aid in improving methods to calculate forcing for past eruptions.

How to cite: Marshall, L., Toohey, M., and Schmidt, A.: How much does ice sheet sulfate deposition tell us about volcanic forcing?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14017, https://doi.org/10.5194/egusphere-egu23-14017, 2023.

EGU23-14591 | ECS | Posters on site | AS3.13

Evaluating the Uncertainties of the Global Atmospheric Sulphur Budget in a Multi-Model Framework 

Christina Brodowsky, Valentina Aquila, Slimane Bekki, Sandip Dhomse, Anton Laakso, Graham Mann, Ulrike Niemeier, Ilaria Quaglia, Eugene Rozanov, Takashi Sekiya, Simone Tilmes, Claudia Timmreck, Pengfei Yu, Yunqian Zhu, and Timofei Sukhodolov

Sulphate aerosol in the stratosphere recently became an interactive part of many global climate models and its uncertainties are not yet well constrained. Stratospheric sulphate aerosol is modulated by natural emissions of several sulphur-containing species, including volcanic eruptions, as well as anthropogenic emissions. If not directly injected into the stratosphere by large volcanic eruptions, sulphate aerosols and their precursors are transported into the stratosphere via the tropical tropopause. While there have been some model intercomparison activity for the large volcanic eruptions, the background conditions of sulphur species and in particular the stratospheric aerosol layer have thus far not been addressed at all. Evaluating the background conditions in global models allow to identify modelling issues that are usually masked by larger perturbations such as volcanic eruptions, yet may still be of importance after such a perturbation. Some key factors causing differences between models include different microphysical schemes, chemical schemes, as well as transport and cross-tropopause fluxes. In this work, we use 8 models and available observational data to quantify the full background atmospheric sulphur cycle (burdens, fluxes, and their variability) and investigate its uncertainties within the framework of the Interactive Stratospheric Aerosol Model Intercomparison Project (ISA-MIP). We focus on stratospheric aerosol and its transport with the Brewer-Dobson-Circulation, as well as the influence of the polar vortices. We find significant inter-model variations in the background burden of the major sulphur species. Seasonal cycles agree well in the southern hemisphere, whereas the northern hemisphere shows more inter-model differences due to the individual representations of the northern polar vortex.

How to cite: Brodowsky, C., Aquila, V., Bekki, S., Dhomse, S., Laakso, A., Mann, G., Niemeier, U., Quaglia, I., Rozanov, E., Sekiya, T., Tilmes, S., Timmreck, C., Yu, P., Zhu, Y., and Sukhodolov, T.: Evaluating the Uncertainties of the Global Atmospheric Sulphur Budget in a Multi-Model Framework, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14591, https://doi.org/10.5194/egusphere-egu23-14591, 2023.

EGU23-14847 | ECS | Posters on site | AS3.13

Utilizing a high vertical and horizontal resolution dataset of SO2 for modelling volcanic eruptions in WACCM 

Emma Axebrink, Johan Friberg, and Moa K. Sporre

The climate impact of volcanic SO2 is strongly correlated with the injection height into the stratosphere. We have used a dataset created with the dispersion model FLEXPART by combining vertical information from the CALIOP lidar with horizontal SO2 information from AIRS [1]. So far, the dataset represents the eruptions of Sarychev in June 2009 with a vertical resolution of 200 m. The original dataset for SO2 used in WACCM releases all SO2 in one latitude and longitude gridbox, spanning an altitude of 11 to 15 km. Our dataset is distributed over several latitude and longitude gridboxes and spans an altitude of 7.6 to 18.6 km [1].

 We have performed simulations in the Earth system model CESM2 WACCM with our dataset and WACCM’s original volcanic SO2 dataset. Aerosol distributions are compared with observations from the CALIOP lidar to investigate the impact of our dataset’s high vertical and horizontal resolution. We also compare outputs from simulations with the two datasets.

The first simulations with the two datasets show large differences in both horizontal and vertical SO2 distribution in the months following the eruption. This likely affects the duration of the radiative impact from sulfate particles formed from the SO2.

 We are presently investigating differences in aerosol formation and concentrations, time evolution of volcanic sulfate, and climate impact of simulations with the two datasets. Future work involves creation of SO2 datasets for all volcanic eruptions since 2006, with the goal of providing better representation of volcanism in Earth system models.

References

[1] Sandvik, O. S., Friberg, J., Sporre, M. K., and Martinsson, B. G.: Methodology to obtain highly resolved SO2 vertical profiles for representation of volcanic emissions in climate models, Atmos. Meas. Tech., 14, 7153–7165, https://doi.org/10.5194/amt-14-7153-2021, 2021.

How to cite: Axebrink, E., Friberg, J., and Sporre, M. K.: Utilizing a high vertical and horizontal resolution dataset of SO2 for modelling volcanic eruptions in WACCM, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14847, https://doi.org/10.5194/egusphere-egu23-14847, 2023.

EGU23-15879 | ECS | Posters on site | AS3.13

Analysing changes in stratospheric water vapour following Pinatubo-like volcanic eruption using UK Earth System Model 

Xin Zhou, Wuhu Feng, Sandip Dhomse, Graham Mann, and Martyn Chipperfield

Large tropical volcanic eruptions can significantly alter stratospheric water vapour either with direct injection or modifying entry pathways and the quantitative magnitude and time evolution of these changes remain uncertain. Using an ensemble volcanic forcing experiment carried out with version 1 of the UK Earth System Model (UKESM1), we explore the changes in the stratospheric water vapour (SWV) by a Pinatubo-like volcanic eruption via modification of the entry pathway. Our simulations show significant increases in SWV three months after the volcanic eruption for the ensemble mean. The increase peaks at 1 ppmv (~17% of the background levels) in the second post-eruption winter and then decays slowly, in accordance with the tropical cold point temperature anomalies. By decomposing the volcanic heating into diabatic aerosol heating and adiabatic dynamical heating, we show that the timing of tropopause heating after the eruption is determined by the seasonal variation of a general decelerated tropical upwelling imposed on the significant direct aerosol heating lasting two years.

How to cite: Zhou, X., Feng, W., Dhomse, S., Mann, G., and Chipperfield, M.: Analysing changes in stratospheric water vapour following Pinatubo-like volcanic eruption using UK Earth System Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15879, https://doi.org/10.5194/egusphere-egu23-15879, 2023.

EGU23-16560 | Posters on site | AS3.13

Interactive stratospheric aerosol simulations of the Hunga-Tonga aerosol cloud re: stronger than expected observed mid-visible stratospheric AOD 

Graham Mann, Sandip Dhomse, Sarah Shallcross, Nicholas Bellouin, Luke Abraham, Rosalyn Hatcher, Grenville Lister, Ghassan Taha, Alexandre Baron, Valentin Duflot, Fabio Lopes, and Eduardo Landulfo

In this presentation we present findings from a series of interactive stratospheric aerosol simulations of the Hunga-Tonga volcanic aerosol cloud with the UM-UKCA composition-climate model.   The model experiments apply the same version of the UM-UKCA model published for the Agung, El Chichon and Pinatubo aerosol clouds (Dhomse et al., 2020), those runs aligned with the Historical Eruption SO2 emissions Assessment experiment within ISA-MIP (Timmreck et al., 2018).

A consistent feature of interactive stratospheric aerosol simulations of Pinatubo (e.g. Dhomse et al., 2014; Sheng et al., 2015; Mills et al., 2016) is an over-prediction of stratospheric AOD, for a given emission of SO2, requiring a downward-adjustment of emitted SO2 (e.g. Timmreck et al., 2018). Dhomse et al. (2020) indicated models may be missing an important removal process such as heterogeneous uptake of SO2 onto fine ash particles, the process recently demonstrated to have removed ~43% more sulphate than SO2-only simulations for the Kelut aerosol cloud (Zhu et al., 2020).

For Hunga-Tonga, any volcanic ash was likely removed within the initial days (Sellitto et al., 2022) and the co-emission of ~100Tg of water vapour (e.g. Carn et al., 2022) has been shown by Zhu et al. (2022) to increase the scattering efficiency of the Hunga-Tonga cloud, both via hygroscopic growth and changes in coagulation, leading to a potential systematic underestimation of stratospheric AOD among interactive stratospheric aerosol models.

In a series of UM-UKCA model experiments, we explore the unexpectedly strong optical depth from Hunga-Tonga aerosol via SO2-only simulations, increasing by a factor 2 and 3 the observed 0.4-0.5Tg of SO2 (Carn et al., 2022), and aligning with the protocol from a multi-model Hunga-Tonga aerosol intercomparison co-ordinated by the University of Colorado (Clyne et al., 2021).  The Tonga-MIP protocol emits 0.5Tg of SO2 at 25-30km, within a 6-hour period, with models also enacting a meridional emission spread between 22S and 14S, matching approaches used to account for unresolved early-phase plume transport for Pinatubo (see e.g. Quaglia et al., 2022).

We evaluate the strength of the simulated Hunga-Tonga aerosol cloud in these SO2-only emission runs, comparing to the magnitude and timing of maximum strat-AOD observed from OMPS (Taha et al., 2022), and the altitude of the progressing aerosol cloud compared to ground-based lidar measurements from Reunion Island (Baron et al., 2022) and Sao Paulo (Landulfo et al., 2022).

How to cite: Mann, G., Dhomse, S., Shallcross, S., Bellouin, N., Abraham, L., Hatcher, R., Lister, G., Taha, G., Baron, A., Duflot, V., Lopes, F., and Landulfo, E.: Interactive stratospheric aerosol simulations of the Hunga-Tonga aerosol cloud re: stronger than expected observed mid-visible stratospheric AOD, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16560, https://doi.org/10.5194/egusphere-egu23-16560, 2023.

Soot particles emitted by aircraft in the troposphere can serve as ice nucleating particles (INPs) in the cirrus regime, which can compete with natural cirrus formation by homogeneous freezing of solution droplets and influence cirrus cloudiness and microphysics. Soot particles show varying ice nucleation (IN) abilities, depending on the particle properties that regulate the IN pathway and effectiveness. Pore condensation and freezing (PCF) is an important pathway for soot IN, which first forms supercooled water in soot mesopores (2-50 nm width) via capillary condensation and then freezes below homogeneous nucleation temperature. Soot PCF shows dependence on the particle mesopore abundance and soot-water contact angle (θ) according to the Kelvin equation. However, the relative importance of θ and mesopore abundance in soot PCF has not been disentangled.

In this study, the θ of organic-lean soot was changed after exposure to a high (20 ppmv) and a low (2 ppmv) O3 concentration condition to mimic a long- (~20 h) and short-term (~2 h) aging in the real atmosphere respectively, without changing the soot mesopore abundance. Secondary organic formation was avoided by establishing a volatile free experimental environment. The IN activities of both fresh and O3-aged soot particles, with aggregate size of 200 and 400 nm, were tested by the Horizontal Ice Nucleation Chamber (HINC) under cirrus cloud conditions for T≤233 K. The size and mass of soot particles for IN experiments were also monitored. The θ of bulk samples exposed to the same O3 concentration conditions (20, 2 or 0 ppmv) as used for IN experiments was directly measured by the Sessile-drop method. The O3-aging effects on soot chemical composition, soot-water interaction ability and porosity were also characterized by using thermogravimetric analysis (TGA), dynamic vapor sorption (DVS) and N2 Brunauer–Emmett–Teller (BET) techniques, respectively.

The adsorption of O3 onto soot particles was demonstrated by a particle mass increase after O3-exposure. The unchanged chemical functional group abundance and increased water-uptake ability at low relative humidity (RH) conditions after O3-aging implies that the soot-water interaction increase is likely due to direct O3-H2O binding rather than surface oxidation, which explains the θ decrease of O3-aged soot. Compared to unaged soot of the same size, a higher O3 exposure level leads to a larger decrease in soot-water θ and a more significant IN enhancement for O3-aged soot. However, O3-aged soot presents unchanged pore size distribution and particle size, irrespective of O3 exposure concentration. According to the Kelvin equation, the θ decrease induced by O3-aging can alone contribute to the IN enhancement of soot, given that the lower the θ is, the lower the RH condition required to trigger capillary condensation. In conclusion, this study highlights the single importance of θ in soot PCF in the cirrus regime, by modifying the soot-water θ through O3-aging while remaining the porosity.

How to cite: Gao, K. and Kanji, Z.: The importance of soot-water contact angle in soot ice nucleation ability in the cirrus regime, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-138, https://doi.org/10.5194/egusphere-egu23-138, 2023.

EGU23-1458 | Posters on site | AS3.14

Overview of ambient ice nucleation measurements from 1949 – 2000 

André Welti, Erik S. Thomson, Jann Schrod, Luisa Ickes, Robert O. David, Zeyao Dong, and Zamin A. Kanji

We report on the addition of 50 years of literature data to the Ice Nucleation DataBase (INDB) created for the EU FP7 BACCHUS project (https://www.bacchus-env.eu/in/). The database is intended to become a tool for the Ice Nucleation community to facilitate finding ice nucleating particle (INP) concentration data collected at specific locations and times. The INDB can be used for comparison reviews, to investigate temporal changes in INP concentrations, identify regions of interest, to inform the planning of future observations, and to facilitate data provision for modelling studies. Worldwide data from more than 170 publications between 1949 to 2000 were digitised and added to the INDB, and more than 130 additional publications have been identified and will be utilized to extend the compilation into 2020. Here we provide an overview of the digitised historical datasets, the times, locations, and experimental conditions under which INP were measured. Exemplary insights from the INDB are discussed by comparing ambient temperature spectra pre and post 1970 in different geographic regions.

How to cite: Welti, A., Thomson, E. S., Schrod, J., Ickes, L., David, R. O., Dong, Z., and Kanji, Z. A.: Overview of ambient ice nucleation measurements from 1949 – 2000, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1458, https://doi.org/10.5194/egusphere-egu23-1458, 2023.

EGU23-1834 | ECS | Posters on site | AS3.14

Singular versus Time-dependent Approach of Heterogeneous Ice Nucleation and Secondary Ice Production in Contrasting Clouds Simulated Numerically 

Deepak Waman, Sachin Patade, Arti Jadav, and Vaughan Phillips

Two approaches of heterogeneous ice nucleation have been proposed in previous studies. These are the singular approach (time-independent), and time-dependent approach. The present study numerically analyses the effect from the time-dependent approach of ice nucleation in deep convective, orographic, and supercooled stratiform clouds, sampled by aircraft. It is predicted that in all the simulated clouds, the singular approximation is a good representative of heterogeneous ice nucleation. At levels warmer than -36oC, the inclusion of time-dependence is predicted to form only about 10 % of the total ice, whereas secondary ice processes (the Hallett-Mossop process and fragmentation during ice-ice collisions, raindrop-freezing, and sublimation) form about 90 % of the total ice at these levels. The present study uses the ‘Aerosol-Cloud’ (AC) model. The AC represents microphysical species as rain, cloud-ice (‘crystal’), snow, and graupel/hail and treats cloud properties with a hybrid spectral bin, and two-moment bulk microphysics schemes. Also, radiative effects from ice nucleating particles on the simulated deep convective and orographic clouds will be discussed.

How to cite: Waman, D., Patade, S., Jadav, A., and Phillips, V.: Singular versus Time-dependent Approach of Heterogeneous Ice Nucleation and Secondary Ice Production in Contrasting Clouds Simulated Numerically, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1834, https://doi.org/10.5194/egusphere-egu23-1834, 2023.

EGU23-2067 | ECS | Posters on site | AS3.14

Scots pines (Pinus sylvestris) as sources of biological ice-nucleating macromolecules (INMs) 

Florian Reyzek, Teresa M. Seifreid, Paul Bieber, and Hinrich Grothe

Scots pine (Pinus sylvestris) is the most widespread pine species in the world. It is a major tree species found in the northern hemisphere and in large parts of the boreal forest. In recent studies, birch trees, another notable species in the boreal forest, have been identified as an important emission source of ice-nucleating macromolecules (INMs). The INMs were found in pollen1 and all over the tree’s tissue (e.g., branch wood, bark, petioles, and leaves)2,3. Similarly, Scots pine pollen were found to be ice nucleation active, but until now, no further investigation of INMs from other tissue types has been conducted.

In this laboratory and field study, we collected samples from six different Scots pine trees in urban parks in Vienna, Austria. We investigated the distribution of INMs among three different tissue types, namely bark, branch wood, and needles, by extracting them from the milled sample (as a bulk sample) and the surface of the intact tissue and measuring ice nucleation activity in immersion freezing mode. We aimed to quantify the overall INM content of this species and assume it is independent of the growing region, as previously reported for birch trees, allowing us to extrapolate our results to the vast locations where Scots pines are found. In addition, we investigated the ability of rain events to wash the INMs off trees in a field study. 

We found INMs in all samples with freezing onset temperatures ranging from -16°C to -29°C. The bulk samples showed INM concentrations ranging from 105 to 109 per mg dry weight active at -25°C and higher. In surface extracts from the intact tissue, we found concentrations from 105 to 108 INMs per cm2 of the extracted surface. Most importantly, we found all rain samples to contain INMs with similar freezing onset temperatures to the lab extracts.

On the basis of our results, we estimate that one square meter of Scots pine stand has the potential to release about 109 to 1012 INMs active at -25°C or higher. This estimation reveals pine trees as a massive reservoir of INMs. Boreal forests containing large numbers of birch and pine trees must be considered an essential source of atmospheric INMs. We propose Scots pine as an important emission source of INMs, nucleating ice in immersion freezing mode at moderate supercooled temperatures and thereby impacting the microphysics of mixed-phase clouds.

 

 

(1)          Pummer, B. G.; Bauer, H.; Bernardi, J.; Bleicher, S.; Grothe, H. Suspendable Macromolecules Are Responsible for Ice Nucleation Activity of Birch and Conifer Pollen. Atmospheric Chemistry and Physics 2012, 12 (5). https://doi.org/10.5194/acp-12-2541-2012.

(2)          Felgitsch, L.; Baloh, P.; Burkart, J.; Mayr, M.; Momken, M. E.; Seifried, T. M.; Winkler, P.; Schmale, D. G.; Grothe, H. Birch Leaves and Branches as a Source of Ice-Nucleating Macromolecules. Atmospheric Chemistry and Physics 2018, 18 (21). https://doi.org/10.5194/acp-18-16063-2018.

(3)          Seifried, T. M.; Bieber, P.; Felgitsch, L.; Vlasich, J.; Reyzek, F.; Schmale, D. G.; Grothe, H. Surfaces of Silver Birch (Betula Pendula) Are Sources of Biological Ice Nuclei: In Vivo and in Situ Investigations. Biogeosciences 2020, 17 (22). https://doi.org/10.5194/bg-17-5655-2020.

How to cite: Reyzek, F., Seifreid, T. M., Bieber, P., and Grothe, H.: Scots pines (Pinus sylvestris) as sources of biological ice-nucleating macromolecules (INMs), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2067, https://doi.org/10.5194/egusphere-egu23-2067, 2023.

This presentation will be an invitation to think differently about the possible oxidation pathways occurring in secondary organic aerosols.

Despite the importance of aerosols in atmospheric chemistry, climate and air pollution, our ability to assess their impact on atmospheric physics and chemistry is still limited due to insufficient understanding of many processes associated with the sources of particles, their chemical composition and morphology, and evolution of their composition and properties during their atmospheric lifetime. Indeed, atmospheric aerosols can be viewed as a complex conglomerate of thousands of chemical compounds forming a system that evolves in the atmosphere by chemical and dynamical processing including chemical interaction with oxidants and sunlight.

A significant body of literature on photo-induced charge or energy transfer in organic molecules from other fields of science (biochemistry and water waste treatment) exists. Such organic molecules are aromatics, substituted carbonyls and/or nitrogen containing compounds – all ubiquitous in tropospheric aerosols. Multiphase processes have also been shown to produce light absorbing compounds in the particle phase. The formation of such light absorbing species could induce new photochemical processes within the aerosol particles and/or at the gas/particle interface. Therefore, while bulk phase aquatic photochemistry has recognized several of these processes that accelerate degradation of dissolved organic matter, only little is known about such processes in/on atmospheric particles.

This presentation will discuss photosensitization in the troposphere as having a significant role in SOA formation and ageing as studied by means of laser transient absorption spectroscopy, flow tube and simulation chamber experiments, all coupled to advanced analytical techniques. We will provide kinetic and mechanistic information on how photosensitization may introduce new chemical pathways, so far unconsidered, which can impact both the chemical composition of the atmosphere and might thus contribute to close the current SOA underestimation.

How to cite: George, C.: Photosensitization is in the air and impacts the multiphase on oxidation capacity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2093, https://doi.org/10.5194/egusphere-egu23-2093, 2023.

Clouds between -42°C and 0°C may be in a phase of pure-liquid, pure-ice, or a mixture of both. The cloud’s phase affects its radiative effect. However, the cloud phase variability is poorly understood, resulting in a high uncertainty in the climate warming projected by models. Passive retrievals from space have the potential for resolving the temporal variability of cloud phase globally and could help to better understand the drivers of cloud glaciation. In our study, we show that daily passive retrievals of cloud phase are highly unreliable, but the monthly phase frequency for thick stratiform clouds offers a reliable constrain for cloud phase variability.

We find that for both the daily cloud phase and the monthly phase frequency, the agreement among different retrieval algorithms increase for thick stratiform clouds. Moreover, for these clouds, the hemispheric and seasonal contrast of cloud phase agrees better with previous estimations from active retrievals. Using thick stratiform clouds observed from space during 35 years, we offer for the first time an estimation of the seasonal cloud phase contrast resolved globally. This estimation will help increase our understanding of the yet poorly-known drivers of cloud glaciation. Moreover, we offer a previously missing benchmark for climate models to constrain the physical processes behind cloud glaciation in order to reduce the associated uncertainty in climate projections.

How to cite: Villanueva, D.: Retrieving global cloud top phase patterns: The reliability of spaceborne retrievals, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2441, https://doi.org/10.5194/egusphere-egu23-2441, 2023.

EGU23-3297 | Posters on site | AS3.14

Learning from the temperature sensitivity of biogenic and Arctic ice nucleating particles 

Heike Wex, Josephine Gundlach, Anna Theresa Backes, Janine Fröhlich-Nowoisky, Kevin Cheuk Hang Sze, Andi Massling, Henrik Skov, Russell Schnell, and Susan Hartmann

Ice nucleating particles (INPs) are a rare but important type of atmospheric aerosol particles, contributed mostly by mineral dust particles and by biogenic macromolecules expressed by a range of different microorganisms. INPs’ ability to nucleate ice in cloud droplets already far above their homogeneous freezing temperature (at ~ -38°C) influences for instance cloud radiative processes and precipitation formation.

Despite a recent surge of research on INPs, neither are all important sources of atmospheric INP sufficiently known, nor their atmospheric abundance which varies with location and season.

Here we examine the heat sensitivity of some types of INP of biogenic origin by exposing them to a range of different heating temperatures (60°C, 85°C, and 90°C) for one hour. The heating is expected to destroy proteinaceous ice active macromolecules. The ice activity of different samples was examined before and after heating.

Examined samples included birch pollen (Betula pendula), fungi (Mortierella alpina, Fusarium acuminatum), the bacteria Pseudomonas syringae (from a commercially available SNOMAX sample) and aspen leaves (from Populus tremuloides) which had been sampled and freeze-dried decades ago. We compare their heat sensitivity to that of INPs from airborne aerosol samples collected on filters in summer months at Villum Research Station (VRS) in North Greenland, which were exposed to the same heating procedure.

For samples from F. acuminatum and P. syringae, a continuing decrease in ice activity (expressed as INP per sample mass) was observed for each of the heating steps. The decrease was larger than one order of magnitude for each heating step across the examined temperature range (roughly -5°C to -25°C). For the B. pendula sample, highly ice active macromolecules inducing ice nucleation at > -10°C were already destroyed by heating to 60°C, while the signal below -15°C was changed much less by any of the heating steps. The M. alpina sample showed no change in ice activity after heating to 60°C, but a strong decrease across the examined temperature range after heating further to 85°C, and some additional decrease (roughly one order of magnitude) after heating to 90°C. The aspen leave samples showed no noticeable reaction to heating at freezing temperatures below -15°C, but behaved similar to the M. alpina sample at -10°C.

Interestingly, for freezing temperatures > -10°C, INP concentrations of VRS summer samples also showed no or only a small decrease in ice activity upon heating to 60°C, similar as the M. alpina and aspen leave samples. Also similar to these two, VRS samples showed a very pronounced decrease upon heating to 85°C and some further decrease upon heating to 90°C. This is interesting in the light that recent research suggested that M. alpina, together with the bacteria species Pantoea ananatis, are likely sources of the INPs present in a aspen leave sample of the same batch as the one examined here. Combining these findings, we speculate that M. alpina may be of considerable importance as terrestrially sourced atmospheric INPs for regions even including the summer Arctic.

How to cite: Wex, H., Gundlach, J., Backes, A. T., Fröhlich-Nowoisky, J., Sze, K. C. H., Massling, A., Skov, H., Schnell, R., and Hartmann, S.: Learning from the temperature sensitivity of biogenic and Arctic ice nucleating particles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3297, https://doi.org/10.5194/egusphere-egu23-3297, 2023.

EGU23-7153 | ECS | Posters on site | AS3.14

The relationship between surface tension and atmospheric ice-nucleating activity of agricultural soil 

Kathleen Thompson, Nicole Link, Benjamin Murray, and Nadine Borduas-Dedekind

Ice-nucleating particles (or INP) play an important role in controlling cloud radiative properties and lifetimes. Therefore, understanding the sources and mechanisms of ice formation in clouds is vital for understanding their impact on cloud radiative feedback. Agricultural dust contributes 25% of global dust emissions and has been shown to nucleate ice at temperatures up to -6°C. This high nucleating ability of agricultural soils suggests that they may be an essential source of INPs on regional or global scales. Many organic components, which have been shown to be important for ice nucleation in soils, have surface active properties that may enhance the ice-nucleating ability of the soil. In this work, lignin was used as a reference for investigating surfactant macromolecules as a potential component of ice nucleation. Lignin solutions showed high ice-nucleating activity in line with decreases in surface tension. We contrasted our observations of lignin with observations from soil extractions from samples taken in the field. Preliminary results suggest little correlation between surface tension measurements and the ice-nucleating activity of extracted soil samples. The presence of a correlation between ice-nucleating and surface activity in soil components such as lignin, but the absence of this correlation in complete soil samples suggests that surfactants can be important ice-nucleating macromolecules, but that highly active soil samples do not necessarily reduce the surface tension at the water-air interface.

How to cite: Thompson, K., Link, N., Murray, B., and Borduas-Dedekind, N.: The relationship between surface tension and atmospheric ice-nucleating activity of agricultural soil, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7153, https://doi.org/10.5194/egusphere-egu23-7153, 2023.

EGU23-8694 | Orals | AS3.14

The Puy de Dôme Ice Nucleation Intercomparison Campaign 

Larissa Lacher and Evelyn Freney and the PICNIC team

The formation and impact of ice crystals in clouds remain a challenge to understand and thus to be predicted in models. In recent years, measurements of ice-nucleating particles (INPs) in ambient air have become more frequent, using well-established and novel techniques such as mobile cloud chambers and filter-based freezing assays. To assure that these techniques are working as intended, validation and intercomparison measurements are required. This is especially relevant due to ongoing efforts for the establishment of INP monitoring networks at the European level (ACTRIS; Aerosol, Clouds and Trace Gases Research Infrastructure) and in the United States (ARM; Atmospheric Radiation Measurement).

Here we present results from PICNIC (The Puy de Dôme ICe Nucleation Intercomparison Campaign), conducted at a mountain site in Central France (1465 m a.s.l.) in October 2018. INP concentrations relevant in the mixed-phase cloud regime were determined using three online INP techniques (Colorado State University-Continuous Flow Diffusion Chamber, CSU-CFDC; Spectrometer for Ice Nuclei, SPIN; Portable Ice Nucleation Experiments, PINE) and seven filter-based offline freezing devices (FRankfurt Ice Nuclei Deposition FreezinG Experiment, FRIDGE; Ice Nucleation Droplet Array INDA; Ice Nucleation Spectrometer of the Karlsruhe Institute of Technology, INSEKT; CSU Ice Spectrometer, IS; Leipzig Ice Nucleation Array, LINA; LED based Ice Nucleation Detection Apparatus LINDA; Micro-Orifice Uniform Deposit Impactor–Droplet Freezing Technique, MOUDI-DFT). The campaign focused on INP concentration measurements performed at the same time and at comparable nucleation temperatures, which is why filter sampling for offline techniques was started and stopped simultaneously, and online INP measurements were conducted at similar thermodynamic conditions. While the ice chambers yielded reasonable agreements within factors of 2 to 5, with lower concentrations found by SPIN, a systematic deviation between filter samples collected directly outside on the station’s rooftop and those sampled downstream from a whole air inlet is observed. A potential loss of larger aerosol particles via the inlet and an impact of the disaggregation of larger aerosol particles in solution might cause these differences, which needs to be investigated in future studies.

How to cite: Lacher, L. and Freney, E. and the PICNIC team: The Puy de Dôme Ice Nucleation Intercomparison Campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8694, https://doi.org/10.5194/egusphere-egu23-8694, 2023.

Ice nucleation in the upper troposphere occurs either homogeneously or heterogeneously. For heterogeneous nucleation, mineral dust is known as an efficient ice nucleating particle (INP) or an aerosol that has the ability to nucleate ice. The global abundance of these mineral particles is poorly understood and thus it often limits accurate representation in model studies. The aim of this work is to simulate ice nucleation with deposition nucleation and compare the results to in-situ measurements.
The simulations are run with large-eddy model UCLALES-SALSA by applying multiple existing deposition nucleation parametrizations for mineral dust. These parametrizations are either based on laboratory measurements or classical nucleation theory. For the simulation setup, ECMWF reanalysis and campaign data from NASA MACPEX are used to create suitable conditions for in-situ cirrus formation. The simulations are based on the 16th of April 2011 science flight which was flown into a synoptic cirrus that formed over Northern Mexico to the Gulf of Mexico.
The simulated ice with all used parametrizations on average produced concentrations within two orders of magnitude of what was measured with onboard instruments. The main limiting factor for ice number concentration in the simulations is mineral dust concentration since every ice crystal formed only on mineral dust particles. The ice number concentration in measurements exceeded the mineral dust concentration which indicates that other INPs or freezing mechanisms might be involved in this scenario.
Further simulations are required to grasp a better understanding of the role of mineral dust in the cirrus cloud formation.

 

Acknowledgements

This work was supported by the Academy of Finland Flagship ACCC (grant no. 337552) and
MEDICEN project (grant no. 345125).

How to cite: Juurikkala, K., Laaksonen, A., and Welti, A.: Simulation of deposition nucleation using ice nucleation parametrizations and comparison of model results to measured cirrus cloud properties, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9420, https://doi.org/10.5194/egusphere-egu23-9420, 2023.

EGU23-10480 | ECS | Orals | AS3.14

Simulating the impacts of pollen on cloud formation by heterogeneous ice nucleation 

Yingxiao Zhang, Tamanna Subba, Brianna N. Hendrickson, Sarah D. Brooks, and Allison L. Steiner

Primary biological aerosol particles (PBAPs) are emitted from Earth’s biosphere, including pollen, fungal spores, virus, bacteria, and plant debris. PBAPs are linked to adverse health effects and have the potential to influence ice nucleation at warmer temperatures. Anemophilous (or wind-driven) pollen is one type of PBAP, and the emitted pollen grains can rupture under high humidity to form smaller sub-pollen particles (SPP). Both pollen and SPP can be lifted to the upper troposphere under convective conditions, readily take up water and serve as cloud condensation nuclei (CCN) and ice nucleating particles (INPs), and therefore impact cloud formation and reflectivity. Although these biological aerosol have proven to be effective INPs in previous studies, they are typically not included in emission inventories. Therefore, it is difficult to quantify their effects on cloud formation and local climate.

Here, we include the emission and rupture of pollen in WRF-Chem simulations and investigate the impacts of pollen and SPP on both warm and ice clouds in the United States South Great Plains (SGP) from April 11-20, 2013, a period with high pollen emission and convective events. We update the Morrison microphysics scheme inside WRF-Chem using aerosol-aware INP parameterizations, considering different freezing mechanisms including heterogeneous freezing (immersion, contact, and deposition freezing) and homogeneous freezing. We further incorporate heterogeneous ice nucleation from pollen and SPP in the model to evaluate pollen effects on ice cloud formation. The corresponding pollen and SPP INP parameterizations are obtained by laboratory experiments that indicate pollen grains are more efficient INPs than SPP and could contribute to ice cloud formation. The model simulation results are evaluated using observational data from Atmospheric Radiation Measurement (ARM) SGP sites.  We conducted a suite of sensitivity tests to examine the impacts of pollen and SPP on one convective event (April 17-18, 2013), and compare the newly developed pollen and SPP INP parameterizations with those developed in previous literature. Our results highlight that the addition of PBAPs such as pollen could shift the convective event onset timing and vertical structure.

 

How to cite: Zhang, Y., Subba, T., Hendrickson, B. N., Brooks, S. D., and Steiner, A. L.: Simulating the impacts of pollen on cloud formation by heterogeneous ice nucleation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10480, https://doi.org/10.5194/egusphere-egu23-10480, 2023.

EGU23-11479 | Orals | AS3.14

Enhancement of cloud glaciation and rain frequency by airborne pollen 

Jan Kretzschmar, Christian Wirth, Mira Pöhlker, Frank Stratmann, Heike Wex, and Johannes Quaas

Pollen belong to a subset of atmospheric aerosol particles that enable the glaciation of supercooled liquid water, which is present in clouds down to an ambient temperature of -38°C. While the ice nucleating properties of pollen are widely researched in laboratory studies, it is challenging to evaluate their effect on clouds in observations at a large scale. Using a combination of ground-based measurements of pollen concentration and satellite observations of cloud properties during springtime, we show that the ice nucleating properties of pollen promote the glaciation of supercooled liquid water. We further establish the link between the pollen-induced increase in cloud ice to a higher precipitation frequency. In light of anthropogenic climate change, the extended and strengthened pollen season and alterations in biodiversity can, therefore, introduce a localized climate forcing and a modification of the precipitation frequency and intensity, especially during springtime.

How to cite: Kretzschmar, J., Wirth, C., Pöhlker, M., Stratmann, F., Wex, H., and Quaas, J.: Enhancement of cloud glaciation and rain frequency by airborne pollen, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11479, https://doi.org/10.5194/egusphere-egu23-11479, 2023.

EGU23-11673 | ECS | Orals | AS3.14

Dynamics of biological ice nucleating particles during a phytoplanktonic bloom in the Arctic 

Corina Wieber, Lasse Z. Jensen, A. Sofia A. Ferreira, Leendert Vergeynst, Kai Finster, and Tina Šantl-Temkiv

With raising temperatures in the Arctic, the extent of sea ice is decreasing dramatically resulting in a larger fraction of the Arctic ocean surface being exposed to the atmosphere. Therefore, the ice-free ocean and in particular the sea surface microlayer (SML), which represents the upper 1 mm of the water column is becoming of increasing interest as a source of bioaerosols with ice nucleating properties. These biological ice nucleating particles (INPs) can be aerosolized by wave breaking and bubble bursting. In the atmosphere, they may trigger the freezing of cloud droplets and thus affect the lifetime of clouds as well as their radiative properties. Recent studies proposed a link between biological ice nucleating aerosols in the Arctic sea water and phytoplanktonic blooms.

Thus, we examined the concentration and characteristics of INPs in both, the sea bulk water, and the surface microlayer for two locations in southwest Greenland throughout a phytoplankton bloom. Further, we investigated possible links between INP concentrations in the sea water, the abundance and community composition of bacteria and algae, as well as the phytoplanktonic growth season derived from satellite data and in-situ chlorophyll concentrations. Preliminary results will be presented.

 

How to cite: Wieber, C., Jensen, L. Z., A. Ferreira, A. S., Vergeynst, L., Finster, K., and Šantl-Temkiv, T.: Dynamics of biological ice nucleating particles during a phytoplanktonic bloom in the Arctic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11673, https://doi.org/10.5194/egusphere-egu23-11673, 2023.

EGU23-11748 | ECS | Posters on site | AS3.14

Ice nucleating particle measurement at Helsinki 

Germán Perez Fogwill, André Welti, Henri Servomaa, Anttila Timo, Ana Piedehierro, Ari Leskinen, Mika Komppula, Antti Hyvärinen, and Eija Asmi

Ice nucleating particles (INPs) are particles in the atmosphere that are able to initiate the freezing of water droplets, a process known as ice nucleation. INPs are important to study because they play a crucial role in many atmospheric processes, including the formation of clouds, precipitation, and the radiative properties of clouds. For example, INPs can influence the concentration, size, and shape of ice crystals in clouds, which can in turn affect the reflectivity and lifetime of the clouds. This can have significant impacts on Earth's radiative balance and climate. The most relevant process of ice crystal formation in mixed-phase clouds (MPC) is by immersion freezing (Ansmann et al., 2009). Immersion freezing takes place when an INP is immersed in a water droplet and freezing is triggered on the particle's surface. In this research, we present a series of INP concentration measurements obtained using a novel assay under development at the Finnish Meteorological Institute in Helsinki. The focus of our research is to evaluate the consistency and replicability of these measurements.  To determine the contribution of different aerosols to the INP spectrum at different temperatures, we collect atmospheric particles onto membrane filters and analyze the concentration of INPs in a laboratory freezing experiment. In this experiment, we produce an aqueous solution with collected atmospheric particles and monitor identical aliquots of the aqueous solution while they are cooled until freezing. Finally, using the frozen fraction of aliquots at a given temperature, the volume of each aliquot, and the sample's air volume, the cumulative number of INPs in the given sample at each temperature is calculated following (Vali, 2019). Three automatic samplers were run in parallel to collect particles onto the membrane filters using different sampling schemes. For example, collecting daily samples with three different sampling flows. With these measurements, we will analyze the influence of the sampled air volume, air flow, and sampling duration on the INP concentration measurements.

 

References

Ansmann, A. et al. (2009) Evolution of the ice phase in tropical altocumulus: SAMUM lidar observations over Cape Verde Atmosphere, 9(9), 357

Vali, G., (2019). Revisiting the differential freezing nucleus spectra derived from drop-freezing experiments: Methods of calculation, applications, and confidence limits. Atmos. Meas. Tech., 12(2), 1219-1231. https://doi.org/10.5194/amt-12-1219-2019

How to cite: Perez Fogwill, G., Welti, A., Servomaa, H., Timo, A., Piedehierro, A., Leskinen, A., Komppula, M., Hyvärinen, A., and Asmi, E.: Ice nucleating particle measurement at Helsinki, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11748, https://doi.org/10.5194/egusphere-egu23-11748, 2023.

EGU23-12324 | Posters on site | AS3.14

Atmospheric Surface-Science Solar Simulator: An artificial solar irradiator for atmospheric photochemistry 

Ahmed Abdelmonem and Mohammed H. Fawey

Solar simulators are indispensable tools and are usually linked to industrial applications, e.g. for determining the precise characteristics of solar cells. In photochemistry, usually UV light is used to stimulate the photo-interactions without particular attention to the spectral distribution. However, the spectral distribution has a non-negligible effect on the photoreaction pathways. To address photochemistry under atmospheric conditions, it is necessary to use an irradiation source that emits light equivalent to the solar light. Solar simulator based on LED technology is the best candidate for irradiating natural photo-interactive substances at specific wavelength and intensity. We have devolved a homemade compact light source that is based on LED technology, and emits light with wavelength starts from 275 nm with tuneable intensity, selectable wavelength, homogenous illumination, compact size and light weight. In this presentation we present the design and characteristics of our homemade solar simulator and demonstrate potential application in atmospheric surface-chemistry.

How to cite: Abdelmonem, A. and Fawey, M. H.: Atmospheric Surface-Science Solar Simulator: An artificial solar irradiator for atmospheric photochemistry, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12324, https://doi.org/10.5194/egusphere-egu23-12324, 2023.

EGU23-12590 | ECS | Orals | AS3.14

Long-range transport effect on the ice nucleation properties of Saharan dust 

Ana A. Piedehierro, André Welti, Linnea Mustonen, Outi Meinander, Yrjö Viisanen, and Ari Laaksonen

Mineral dust is the main responsible ice nucleating particle (INP) type for mixed-phase clouds and has an influence over regions far from the dust source. Parameterizations of the dust ice nucleation (IN) ability used in models are normally obtained from experimental characterization of dust collected from the surface at origin (Ullrich et al., 2017). However, IN properties of long-range transported dust may differ from the dust at origin due to different mineralogy and physical or chemical transformations along the transport route. Here we present preliminary results of ice nucleation properties of Saharan dust transported to Spain and Finland in the temperature range relevant for mixed-phase cloud formation.

In this work, the IN ability in immersion mode is evaluated using an Mk-1 droplet-freezing cold stage (Sikora Scientific Instrumentation). The drop-freezing assays are performed by depositing a set of dust-containing droplets (1 μL) onto a hydrophobic glass that rests atop the cold stage, whose temperature can be varied at a specific cooling rate. A high-resolution camera captures images tracking the freezing events, while the temperature is decreased. Dilutions of the original suspensions are prepared to explore the colder temperature range. Heat treatments are applied to the samples to investigate the contribution of the sample’s biological-origin components to its ice nucleation ability. The BET surface area is measured for selected samples.

This work was supported by the Academy of Finland Flagship ACCC (grant no. 337552) and MEDICEN project (grant no. 345125).

Ullrich, R. et al. (2017). A New Ice Nucleation Active Site Parameterization for Desert Dust and Soot J. Atmos. Sci., 74, 699-717.

How to cite: Piedehierro, A. A., Welti, A., Mustonen, L., Meinander, O., Viisanen, Y., and Laaksonen, A.: Long-range transport effect on the ice nucleation properties of Saharan dust, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12590, https://doi.org/10.5194/egusphere-egu23-12590, 2023.

EGU23-13040 | Posters virtual | AS3.14

New Aerosol-sensitive Heterogeneous Ice Nucleation Parameterization in the EC-Earth3 Earth System Model: evaluation and climate response 

Montserrat Costa-Surós, Maria Gonçalves, Marios Chatziparaschos, Paraskevi Georgakaki, Luka Ilić, Gilbert Montane, Stelios Myriokefalitakis, Twan van Noije, Pilippe Le Sager, Maria Kanakidou, Athanasios Nenes, and Carlos Pérez García-Pando

Clouds are large contributors to uncertainty in climate projections, with aerosol-cloud interactions playing a key role. To better reproduce heterogeneous ice clouds and, ultimately, the Earth’s changing energy budget in EC-Earth3 (one of the CMIP6 Earth System Models), its heterogeneous ice nucleation scheme has been updated. Specifically, the temperature-based parameterization has been substituted by a combination of aerosol-and-temperature-sensitive ice nucleating parameterizations. In particular, the model now considers a dust-and-soot-sensitive deposition nucleation scheme for cirrus clouds and aerosol-sensitive immersion freezing schemes for mixed-phase clouds. The latter is sensitive to the mineralogical composition of dust, specifically to the content of K-feldspar and quartz, and to marine organic aerosols, which are explicitly traced in EC-Earth3. Moreover, a secondary ice production parameterization based on a random forest regressor enhances the ice formed by the primary processes.

We evaluate the model against an extended observational dataset of INP concentrations and analyze the effect of modelled aerosols upon heterogeneous ice nucleation in mixed-phase clouds and cirrus clouds produced with the new parameterizations. We also investigate the sensitivity of the simulated liquid and ice water content and the atmospheric radiative fluxes to the two different soil mineralogy atlases. Additionally, we use this updated model version to study in more detail a severe dust intrusion event that produced dust-infused clouds that affected Europe in March 2022.

The results with the new ice nucleation parameterizations show a clear association of the simulated ice crystal number concentrations with the aerosol sources and transported regions. We also show that replacing the temperature-dependent ice nucleation parameterization with an aerosol-sensitive parameterization in EC-Earth3 significantly impacts surface temperature at high latitudes.

How to cite: Costa-Surós, M., Gonçalves, M., Chatziparaschos, M., Georgakaki, P., Ilić, L., Montane, G., Myriokefalitakis, S., van Noije, T., Le Sager, P., Kanakidou, M., Nenes, A., and Pérez García-Pando, C.: New Aerosol-sensitive Heterogeneous Ice Nucleation Parameterization in the EC-Earth3 Earth System Model: evaluation and climate response, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13040, https://doi.org/10.5194/egusphere-egu23-13040, 2023.

EGU23-14850 | ECS | Orals | AS3.14

Ion specific Interactions and Surface Enrichment on Mixed Aerosol Surfaces 

Clara M. Saak, Sofie M. Mika, and Ellen H.G. Backus

Aerosols have a net cooling effect in our atmosphere, mainly due to their ability to act as cloud condensation nuclei (CCN) and to reflect incoming solar radiation [1]. In aerosols the surface is particularly important as it is the site for many processes which are central to cloud formation, in particular evaporation and condensation. Aerosol surfaces contain a wide variety of organic and inorganic chemical compounds. Understanding the resulting surface structure and composition is a necessary first step in gaining a better understanding of the role aerosols play in the atmosphere.

In particular, the surface composition affects the hygroscopicity of the particle and thereby its ability to act as a CCN [2]. While the surface propensity of individual compounds has been studied widely, much less is known about cooperative effects in more complex mixed systems [3]. Here we use sum-frequency-generation (SFG) spectroscopy in conjunction with surface tension data to study whether surface competition or cooperative enhancement can be observed in mixed solutions of halides and acids or alcohols of different chain length.

We find that in certain cases the presence of different ions can affect the surface structure in a unique way. However, these effects are not systematic and appear to depend on the specific nature of the interaction between the ions and the respective organic compound. This further highlights that the surface structure of mixed systems cannot be extrapolated from studies of simple solutions.

 

[1] IPCC. Climate Change 2013: The Physical Science Basis. [2] P. Zieger et al., Nat. Commun. 2017, 8, 15883. [3] M.T. Lee et al., Phys. Chem. Chem. Phys. 2019, 21, 8418

How to cite: Saak, C. M., Mika, S. M., and Backus, E. H. G.: Ion specific Interactions and Surface Enrichment on Mixed Aerosol Surfaces, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14850, https://doi.org/10.5194/egusphere-egu23-14850, 2023.

Effect of pH on pyruvic acid in bulk and at the air/liquid interface
Veronika Wank and Ellen H. G. Backus
University of Vienna, Faculty of Chemistry, Department of Physical Chemistry,Währinger Straße 42, 1090 Vienna, Austria
Abstract:
Pyruvic acid, known as a relevant carboxylic acid for plant metabolic processes is also a contributor to the formation of secondary organic aerosols (SOA) and thus of great importance for the atmospheric cycle, especially in aerosols. At the interface, the behavior of relevant atmospheric molecules in aerosols is a major topic, as the surface is one of the first areas where chemical processes take place and thus determines the main reactivity of the aerosol. For acidic molecules, the acid/base behavior, especially at the interface, is relevant for understanding the chemical interaction of organic matter in atmospheric aerosols, where reaction rates and product distributions change due to different pH conditions, e.g. chemical processing and molecule transport.
Since the pH of aqueous aerosols can vary widely, it is particularly important to understand changes in the surface structure due to the resulting (de)protonation reactions.
This encourages us to take a closer look at the interfacial region of pyruvic acid in aqueous solution by using a complex surface-specific spectroscopic technique, so called sum frequency generation spectroscopy (SFG). For comparison, infrared bulk measurements utilizing ATR spectroscopy were completed. By combining ATR and SFG, the protonation state of pyruvic acid for bulk and interface was determined by probing the vibrational signatures of the carboxylic acid groups.
Our results show that pyruvic acid at the water interface is more alkaline than in the bulk, which indicates that the carboxylic acid group deprotonates at a higher pH value at the surface than in the bulk. It is also evident from the SFG spectra that at lower pH the water molecules on the surface are displaced by PA molecules, whereas at higher pH the water molecules return to the surface and the PA molecules tend to go into the bulk.
This implies that the protonation state of carboxylic acids like PA can thus affect the molecular orientation, conformation and function of molecules on aqueous surfaces, which likely has a significant impact on the chemical processes taking place at the aerosol surface in the atmosphere.

How to cite: Wank, V.: Effect of pH on pyruvic acid in bulk and at the air/liquid interface, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15680, https://doi.org/10.5194/egusphere-egu23-15680, 2023.

EGU23-15693 | ECS | Posters on site | AS3.14

Observations of ice-nucleating particles during deep convective cloud development in New Mexico, USA 

Martin Daily, Joseph Robinson, Jim McQuaid, Declan Finney, Alan Blyth, and Ben Murray

Deep convective clouds produce severe weather and their reflective anvil tops play a role in climate feedbacks. As mixed-phase clouds, they can be greatly affected by the concentration and activity of ice-nucleating particles (INPs) (Hawker et al., 2021). INP are aerosol that initiate primary ice production in mixed-phase clouds and in-situ measurements of their concentrations are scarce. Here we present analysis of INP data from aerosol filter sampling done on the FAAM aircraft the DCMEX (Deep Convective Microphysics Experiment) field campaign in New Mexico, USA, during July-August 2022. The project aims to improve the representation in climate models of microphysical processes in deep convective clouds. This location was selected because clouds formed and developed almost daily in the same location over the Magdalena Mountains during the summer monsoon season, which allowed observation of the first primary ice particles and also repeated sampling of INP in the air that that flowed into the cloud bases.

Offline INP sampling consisted of filter sampling using the FAAM Bae-146 aircraft platform along circuits around the Magdalena Mountains (16 flights). Filters were analysed during the campaign for INP using microlitre droplet freezing assays and then combined with total air flow to determine INP concentrations. We found that airborne-derived INP concentrations were higher than the upper range of past observations from continental precipitation samples (Petters and Wright, 2015) but within those of primary ice-crystal concentrations observed in clouds (Cooper, 1986). Airborne sampling runs typically saw 1-10 L-1 at -15 °C with INP active above -10 °C and up to -5 °C frequently observed both below cloud base (>200 m above ground level) and also through a substantial portion of the free troposphere, typically to up to an altitude of 4,000-6,000 m (2,500-4,500m above ground level). INP concentrations decreased above this level by an order of magnitude. INP concentrations were normalised to aerosol surface area measurements derived from aircraft Passive Cavity Aerosol Spectrometer Probe data to derive spectra for number of active sites per aerosol surface area (ns(T)). This revealed that the ice-nucleating activity of the aerosol consistently was higher than that described by parameterisations for desert dust, inferring a biological origin for the INP population.

Further analysis including relating INP concentrations to aerosol composition and particle size distribution, comparison of INP number to cloud ice-crystal concentration are in progress to ultimately determine relationships between primary production via INP and ice concentrations in cloud. This will help us better understand the properties and development of and ultimately improve modelling of convective clouds.

References

Cooper, W. A.: Ice Initiation in Natural Clouds, in: Precipitation Enhancement—A Scientific Challenge,  American Meteorological Society, 29-32, 1986.

Hawker, R. E., Miltenberger, A. K., Wilkinson, J. M., Hill, A. A., Shipway, B. J., Cui, Z., Cotton, R. J., Carslaw, K. S., Field, P. R., and Murray, B. J.: The temperature dependence of ice-nucleating particle concentrations affects the radiative properties of tropical convective cloud systems, Atmos. Chem. Phys., 21, 5439-5461, 10.5194/acp-21-5439-2021, 2021.

Petters, M. D., and Wright, T. P.: Revisiting ice nucleation from precipitation samples, Geophysical Research Letters, 42, 8758-8766, 

How to cite: Daily, M., Robinson, J., McQuaid, J., Finney, D., Blyth, A., and Murray, B.: Observations of ice-nucleating particles during deep convective cloud development in New Mexico, USA, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15693, https://doi.org/10.5194/egusphere-egu23-15693, 2023.

EGU23-179 | ECS | Posters on site | AS3.15

Air Quality Monitoring for Sustainable Development in Cluj-Napoca 

Horia Camarasan, Andrei Radovici, Horatiu Stefanie, Alexandru Mereuta, Nicolae Ajtai, and Camelia Botezan

Apart from affecting citizens health and wellbeing across urban and rural areas, air pollution has significant economic implications which inhibit progress, especially for developing countries. The role of air quality monitoring to ensure population wellness is a key topic in the current pursuit for the sustainable development goals, promoting active response from decision-makers to address acute socio-environmental challenges and to promote a resilient and sustainable future. In this study, an integrated air quality monitoring system was proposed within the municipality of Cluj-Napoca, by adopting a novel methodology for sensor-placement throughout the city, composing an efficient network of stations with high spatial and temporal resolution. The purpose of this network is to assist the population and local authorities by providing a platform that offers real-time mapped data related to local air quality and potential health threats. This approach was based upon a thorough geospatial data analysis of land-use in the area, where possible correlations between air quality and anthropic activities that generate emissions were studied. Using these factors, an analysis of possible placement locations was carried out, in order to determine the most representative network shape that would reflect the air quality variations throughout different locations of the study area and will prove to be cost-efficient by using a limited number of sensors. A series of maps with various networks morphologies, were generated and compared. An innovative method of using a “natural pattern”-based approach for the network morphology, proved to be the most efficient in fulfilling all the proposed requirements of the network.

How to cite: Camarasan, H., Radovici, A., Stefanie, H., Mereuta, A., Ajtai, N., and Botezan, C.: Air Quality Monitoring for Sustainable Development in Cluj-Napoca, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-179, https://doi.org/10.5194/egusphere-egu23-179, 2023.

Particulate bound Polycyclic Aromatic Hydrocarbons (PAHs) are ubiquitous in the urban atmosphere, posing carcinogenic and mutagenic risk to urban population. The present study analysed the seasonal variation, identification of air pollution sources, and evaluation of carcinogenic risk for different geographical locations in the urban region structure. PM10 and PM2.5 concentrations were monitored at five different locations; Traffic, Commercial, Industrial, Residential, and Background during winter (January 2021) and summer season (April 2021) in the Vijayawada city, Andhra Pradesh, India. The average concentration of PM10 and PM2.5 at traffic (122±29 µg/m3, 70±14 µg/m3), commercial (106±20 µg/m3, 57±10 µg/m3), industrial (154±42 µg/m3, 82±21 µg/m3), residential (92±13 µg/m3, 54±12 µg/m3), and background (98±16 µg/m3, 61±10 µg/m3) during winter season respectively. All monitoring locations exceeds the National Ambient Air Quality Standards (NAAQS) (PM10~100 µg/m3, PM2.5~60 µg/m3). Similarly, in summer, the average concentration of PM10 and PM2.5 was evaluated at traffic (76±21 µg/m3, 38±09 µg/m3), commercial (59±17 µg/m3, 36±08 µg/m3), industrial (86±24 µg/m3, 52±15 µg/m3), residential (50±16 µg/m3, 26±05 µg/m3), and background (56±14 µg/m3, 26±05 µg/m3) respectively. The spatiotemporal variation illustrates the highest average ∑16PAHs concentration was at the industrial region (64.5-24.3 ng/m3), followed by commercial (47.9-15.5 ng/m3), traffic (44.1-33.2 ng/m3), background (43.4-19.6 ng/m3), and residential (35.5-17.0 ng/m3). High concentration in background region compared to residential is attributed with the local activities (coal and wood burning for cooking and heating purposes in slums), national highway, and international airport near the monitoring location. Winter to summer (W/S) ratio of average ∑16PAHs in PM10 ranges from 3.09 to 0.96 depicting high PAHs concentration even in summer especially at the traffic location where uniform vehicular emission can be observed. However, ∑16PAHs W/S ratio in PM2.5 ranges from 2.13 to 1.17.  Coefficient of Divergence (COD) revealed the similarity in PAHs sources in most of the cases for both size fractions. Source apportionment techniques like MDR and PCA-MLR indicated that the contribution from vehicular emission (i.e., gasoline and diesel combustion) was the highest in PAHs concentration, whereas stationary sources (coal combustion and biomass burning) also contributed to significant PAHs emissions in both sizes fractions. The results can be attributed to the heavy usage of coal, wood, briquettes, and other biomass products as fuel requirements in various industries operating inside the city boundaries. Total Benzo(A)Pyrene equivalent (BaPeq.) concentration for PM10 and PM2.5 ranges from (204.8-34.2 ng/m3) and (190.8-46.9 ng/m3) respectively. The Lifetime Lung Cancer Risk (3.01×10-3-1.01×10-4) and (1.39×10-3-1.40×10-4) in winter and summer, respectively, exceeds the acceptable limits i.e., (10-6) stated by the USEPA. High carcinogenic risk required the attention to reduce the toxic pollutants emissions from the vehicular emissions and biomass burning.

Keywords: PM10 and PM2.5, PAHs, Source Apportionment, Urban Air Quality, Lifetime Lung Cancer Risk

 

 

 

How to cite: Sharma, M. and Jain, S.: Atmospheric Particulate Bound Polycyclic Aromatic Hydrocarbons in Urban Region Structure: Spatiotemporal Variation, Source Apportionment, And Human Health Risk Analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-372, https://doi.org/10.5194/egusphere-egu23-372, 2023.

EGU23-397 | ECS | Posters on site | AS3.15

Air quality assement for Suceava County, Romania 

Liliana Gina Lazurca (Andrei), Dumitru Mihăilă, Petruț Ionel Bistricean, and Vasilică Dănuț Horodnic

According to the Air Quality Framework Directive, air pollutant concentration levels have to be assessed and reported annually by each European Union member state, taking into consideration European air quality standards. Plans and programmes should be implemented in zones and agglomerations where pollutant concentrations exceed the limit and target values. The main purpose of this research study is to analyse the concentrations of pollutants in the atmosphere, their spatial and temporal trends and to draw an overall picture of air quality in Suceava County. The study uses an hourly database for SO2, NO2, CO, PM10 and O3 pollutants, from 2009-2020, from 4 air quality monitoring stations in Suceava County. Pollutant levels were statistically and graphically / cartographically modeled for the entire 2009-2020 interval on the distributive-spatial and regime, temporal component. Inter-station differences and similarities were analyzed causally. The results showed that PM10 air pollution is the biggest challenge for the Suceava city, the highest multi-year average of 31.86 µg/m3 is recorded at the SV2 station in the Burdujeni district although it does not exceed the limit value for the protection of human health (40 µg/m3). Average daily PM10 levels place Suceava County in quality class III (good). SO2 pollution in Suceava County is limited, with average hourly concentrations well below the hourly limit for the protection of human health throughout the period analysed. Based on diurnal average levels, statistical calculations for SO2 and NO2 show that at all four stations in the county, air quality was excellent. The ozone is measured only at three stations: EM3, SV1, SV2. In Suceava county, the multi-year average ozone concentration was 49.61 μg/m3. According to the daily average level of O3, the study area falls into quality class II, very good.  The average CO levels indicate an excelent air quality.

How to cite: Lazurca (Andrei), L. G., Mihăilă, D., Bistricean, P. I., and Horodnic, V. D.: Air quality assement for Suceava County, Romania, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-397, https://doi.org/10.5194/egusphere-egu23-397, 2023.

EGU23-1234 | ECS | Orals | AS3.15

A Measurement Campaign in Thessaloniki, Greece, to Detect and Estimate Local Greenhouse Gas Emissions 

Lena Feld, Pablo Schmid, Frank Hase, Roland Ruhnke, Marios Mermigkas, Dimitrios Balis, and Peter Braesicke

The reduction of carbon emissions is required to limit global warming. Thus, measurement-based methods to monitor the progress in reducing emissions are essential. A significant part of the global emissions is produced in urban areas where also industry is located. Here, we investigate the urban area of Thessaloniki to better understand the distribution of local greenhouse gas sources during October 2021 and the summer of 2022.

We present results of a measurement campaign using a pair of Fourier-Transform Infrared (FTIR) Spectrometers of the type EM27/SUN developed by Bruker and KIT.
The measurement campaign took part in the framework of the Collaborative Carbon Column Observing Network (COCCON). During the campaign the spectrometers were used in an up- downwind setup. One spectrometer was located in a central position of the city while the second instrument was transported to various locations at the boundaries of the city, selected according to the prevailing wind direction. Additionally, measurements to characterize the advected background variability were performed. Here, the spectrometers were arranged orthogonal to the prevailing wind direction to estimate the variability of the background concentrations of carbon dioxide and methane.
In total, 30 days of measurements were collected, giving a comprehensive dataset to study the emissions of the city area. The measurements are interpreted using a box model to estimate the averaged emission area fluxes. We present results for both, carbon dioxide and methane, and discuss the temporal and spatial variability we encountered.

In a next step, we aim to confront these measurements with simulation results with idealized tracer emission patterns using the ICON-ART modeling framework, a numerical weather forecast model developed and used operationally by the German Weather Service (DWD). The results from the box model introduced above will be used as a starting point to combine measurements and simulations. First simulations produced for this purpose will be shown.

How to cite: Feld, L., Schmid, P., Hase, F., Ruhnke, R., Mermigkas, M., Balis, D., and Braesicke, P.: A Measurement Campaign in Thessaloniki, Greece, to Detect and Estimate Local Greenhouse Gas Emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1234, https://doi.org/10.5194/egusphere-egu23-1234, 2023.

EGU23-1379 | ECS | Orals | AS3.15

Summertime urban ammonia emissions may be substantially underestimated in Beijing, China 

Jiayu Xu, Lin Zhang, Mengran Lu, Yixin Guo, Youfan Chen, Zehui Liu, Mi Zhou, Weili Lin, Weiwei Pu, Zhiqiang Ma, Yu Song, Yuepeng Pan, Lei Liu, and Dongsheng Ji

Ammonia (NH3) emission control has been advocated for its potential to mitigate PM2.5 air pollution, yet emission quantifications at city levels are limited. Here we develop high-resolution (3 km) bottom-up emission inventories of agricultural NH3 in the Beijing-Tianjin-Hebei (BTH) region and traffic NH3 in Beijing for the year 2016. The resulting WRF-Chem simulated NH3 and PM2.5 are compared against ground-based and satellite observations. Our estimated annual BTH agricultural NH3 emissions (625 Gg) and Beijing’s traffic emissions (7.8 Gg) are within the ranges of published inventories. However, simulated NH3 concentrations are significantly lower than observations during August in urban Beijing, while wintertime underestimations are much more moderate. Further evaluation and sensitivity experiments show that such discrepancies cannot be attributed to biases in meteorology or regional transport. Using measurements as constraints, our inversed NH3 inventory indicates both agricultural and non-agricultural NH3 emissions in Beijing during August should increase by ~5 times to match NH3 and PM2.5 observations. Current underestimations may result from the missing power sector, urban green space emissions, the lack of representation of industrial hotspots, and uncertainties in traffic emissions. Our study highlights that denser and more frequent urban NH3 observations are urgently needed to constrain and validate bottom-up inventories.

How to cite: Xu, J., Zhang, L., Lu, M., Guo, Y., Chen, Y., Liu, Z., Zhou, M., Lin, W., Pu, W., Ma, Z., Song, Y., Pan, Y., Liu, L., and Ji, D.: Summertime urban ammonia emissions may be substantially underestimated in Beijing, China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1379, https://doi.org/10.5194/egusphere-egu23-1379, 2023.

EGU23-1535 | ECS | Orals | AS3.15 | Highlight

Neural network studies of air quality and socioeconomic predictors of mortality 

Michelle Wan and Alexander Archibald

After the Great Smog of London in 1952, the health impacts of air pollution exposure were launched into local public awareness. Today, these impacts have been established by epidemiological studies across the world. 

Machine learning (ML) techniques applied to this field of study in recent years have demonstrated potential advantages over traditional statistical approaches. These techniques are well-suited to large sets of input features, which can describe more holistically the numerous factors affecting human health. Additionally, the data-driven nature of these techniques eliminates the requirement for prior definition of the mathematical relationships between driving factors, confounders, and health outcomes. Previous examples of ML applications have included the identification of exposure profiles, and prediction of disease rates.

In this work, a simplified feature set was used to develop predictive ML models of daily mortality in Greater London, UK. The input features to the predictive models were: outdoor nitrogen dioxide concentrations recorded by the London Air Quality Network, outdoor temperature measurements recorded by the UK Met Office, and gross disposable household income per capita, as published by the UK Office for National Statistics. Preliminary work explored the trends and correlations observed in the dataset, which spanned the years 1997–2018. Predictive model performance was then compared between linear and neural network regressor models. Each of the three input features were also excluded in turn, to test the roles they played as predictors of mortality rates in London. 

Results found that, while both types of regressor architectures learnt to predict seasonal cycles in mortality rates, the neural network made test set predictions with a 73% reduction in mean squared error compared to the equivalent linear model. This illustrates the improved modelling power conferred by the nonlinear nature of neural networks, despite the network here being shallow in depth. 

Additionally, the ablation studies demonstrated that both types of models were dependent on the income input feature in order to accurately predict general trends in mortality rates over the two decades. Only this input feature provided information about changing trends through time, and its inclusion in this modelling approach was intended to represent the gradual improvement of societal and individual health factors.

In ongoing work, the exploration of factors affecting mortality is extended using long short-term memory neural network architectures. This type of neural network is additionally able to consider the temporal dimension by handling sequences of time series datapoints. Information is incorporated from the sequence of previous time steps into a memory vector, which then forms part of the input to the subsequent time step. Sequence length thus corresponds to the length of time-lagged associations learnt by the network. By varying sequence length, it is then possible to examine the significance of time-lag windows of different day lengths.

How to cite: Wan, M. and Archibald, A.: Neural network studies of air quality and socioeconomic predictors of mortality, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1535, https://doi.org/10.5194/egusphere-egu23-1535, 2023.

Since the Seoul Metropolitan Area, Republic of Korea, is highly populated, a large number of people are frequently exposed to high concentrations of particulate matter (PM) with mean aerodynamic diameters of <= 10 mm (PM10) in cold season. The concentration of PM10 in Seoul Metropolitan Area increases by transboundary transport, local direct emissions, and chemical reactions of aerosol precursors in the atmosphere. Here, the Seoul Metropolitan Area (Seoul, Gyeonggi-do, and Incheon) and surrounding region (Chungcheongnam-do, Daejeon, and Sejong) are regionally classified by clustering analysis based on the variability of PM10 concentrations. According to the inertia score by the number of clusters, the optimum cluster number of regional variability of PM10 is four. The region of cluster 1 is divided into southern Gyeonggi-do and eastern Chungcheongnam-do, the cluster 2 is mainly classified Incheon, western Gyeonggi-do, and Seoul. The cluster 3 region is western Chungcheongnam-do adjacent to Yellow Sea, and the cluster 4 is classified into eastern Gyeonggi-do. The variability of PM10 in each region is distinguished by the local chemical pollutants emission and weather conditions such as wind speed and direction in each region. This regional classification of PM10 variability is different from administrative districts. Considering most of policies for responding to high concentrations of PM10 are being prepared by administrative districts, this study suggests that a response on the basis of these regional PM10 distribution would be more effective way to improve air quality in the Seoul Metropolitan and Chungcheong Area.

How to cite: Choi, W.: Regional classification according to PM10 concentrations in the Seoul Metropolitan and Chungcheong Area, Republic of Korea, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1779, https://doi.org/10.5194/egusphere-egu23-1779, 2023.

EGU23-2239 | Orals | AS3.15

Ship-related ultrafine particles and SOA formation in a Mediterranean port city 

Matthias Karl, Martin O. P. Ramacher, Sonia Oppo, Ludovic Lanzi, Elisa Majamäki, Jukka-Pekka Jalkanen, Grazia Maria Lanzafame, Brice Temime-Roussel, and Barbara D'Anna

Ship emissions of air pollutants in and around ports adversely affect local air quality and human health, especially in harbour cities. In coastal Mediterranean cities, shipping activities are an important contributor to emissions of fine particulate matter (PM2.5) within the urban area. In addition to primary particles emitted in ship exhaust, secondary organic aerosols (SOA) may form in ship plumes through chemical oxidation of volatile organic compounds (VOC) and through condensation of intermediate volatile or semi-volatile organic gases. Shipping also emerges as a major source of ultrafine particles below 100 nm diameter in coastal cities. Ultrafine particles have been estimated to significantly affect human mortality in coastal areas. While a large number of studies investigated the effect of ship-related PM2.5 in coastal areas, currently only few studies deal with the effect of ship emissions on SOA concentrations and number concentrations of ultrafine particles in harbour cities.

In this study, we investigate the effect of ship emissions on SOA concentrations and number concentrations of UFP in the harbour city Marseille in southern France, which is an important hub of ferry and cruise ship traffic in the Mediterranean Sea. For city-scale simulations of Marseille, the urban chemistry transport model EPISODE-CityChem (https://doi.org/10.5281/zenodo.1116173) was applied in a coupled setup with the regional-scale Community Multiscale Air Quality Modelling System (CMAQ). EPISODE-CityChem combines a 3-D Eulerian grid model with sub-grid Gaussian plume models and solves the photochemistry of multiple reactive pollutants, including the chemistry of 12 different VOC. New developments in EPISODE-CityChem include the P8P+2 scheme for calculating particle number (PN) concentration and particle number size distribution (PNSD) and the SOA module of the aerosol model MAFOR v2.0 (https://github.com/mafor2/mafor). The STEAM-3 emission inventory for the local shipping in and around the port of Marseille consists of hourly emissions of major pollutants, VOC and particle numbers from ships on 250 m grid resolution. Hourly model output of EPISODE-CityChem for July 2020 was compared to measurements at monitoring stations in Marseille operated by AtmoSud and campaign data recorded at La Major, a site in proximity of the port.

Our results show that the potential impact from local shipping to the monthly mean concentration in the urban area of Marseille is only up to 3% for PM2.5, whereas it is up to 42% for total PN. The abundance of ship-related semi-volatile organic vapours is high in the areas of SOA formation, which indicates that volatile organics are mainly in the gas phase because available pre-existing particle surfaces and high ambient temperatures limit their condensation. Ship plumes at La Major were detected based on the difference of total PN concentration between the reference run and a model run excluding ship emissions. The maximum of the modelled and the observed PNSD notably corresponded to the typical size distribution maximum of ship exhaust particles. Total PN should be considered as a more suitable metric for monitoring ship emission impact than PM2.5 because it allows for a better discrimination of ship plumes from the background pollution.

How to cite: Karl, M., Ramacher, M. O. P., Oppo, S., Lanzi, L., Majamäki, E., Jalkanen, J.-P., Lanzafame, G. M., Temime-Roussel, B., and D'Anna, B.: Ship-related ultrafine particles and SOA formation in a Mediterranean port city, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2239, https://doi.org/10.5194/egusphere-egu23-2239, 2023.

Urban areas and cities play a crucial role in mitigating climate change. First, a large share of greenhouse gases (about 60%) is emitted in urban areas. Second, city networks have formed to implement climate change mitigation measures at the local level. Therefore, cities have great potential to significantly reduce greenhouse gas emissions.

Realizing this potential requires solid knowledge of local greenhouse gas sources, which can be obtained through robust measurements of greenhouse gases in an urban network. These measurements can then serve as a starting point for quantifying and thus verifying local emissions. In order to optimize the investment in a measurement network and maximize the knowledge gained from these measurements, several parameters need to be considered, such as the number and location of nodes, the uncertainty of the measurements, and the co-measured species.

These parameters can be evaluated and optimized in an Observing System Simulation Experiment (OSSE). In our study we perform a high-resolution OSSE using the atmospheric transport model GRAMM/GRAL. We first feed a high-resolution anthropogenic emission inventory into the model and simulate CO2 concentration in the urban atmosphere on 10 m resolution in a 12 km x 12 km domain. Next, we approximate CO2 fluxes on neighborhood scale using an inverse framework. We test different configurations of possible measurement networks to assess under which circumstances and how well we can estimate CO2 fluxes. We find that the accuracy of the estimated fluxes increases with node number and precision, reaching a mean error reduction of about 50 % for 16 nodes and a precision of 1.0 ppm in the best configurations. Sources emitted on ground level can be successfully estimated on hourly resolution, but the measurement stations are not sensitive enough to detect sources emitted from tall emission stacks in the vicinity of the measurement nodes. We further discuss the advantages of using CO as an additional tracer in the inversion with respect to measurement precision and sectoral source disaggregation. The framework developed allows for the planning of an optimal measurement network and can thereafter be used to derive fluxes and associated uncertainties in urban areas. This allows for verification of emissions and targeted monitoring of mitigation measures at the local scale.

How to cite: Maiwald, R. and Vardag, S. N.: Observing System Simulation Experiment for designing a monitoring network in urban areas using the GRAMM/GRAL model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2434, https://doi.org/10.5194/egusphere-egu23-2434, 2023.

EGU23-3614 | Posters virtual | AS3.15

Observation and source apportionment of atmospheric alkaline gases in urban Beijing, China 

Jun Zheng, Shengnan Zhu, Dongsen Yang, and Yan Ma

Atmospheric alkaline gases, including NH3 and amines, have been demonstrated to play crucial roles in atmospheric chemical processes, from enhancing atmospheric nucleation to promoting secondary particulate matter formation. It has been suggested that new particle formation can contribute significantly to haze formation in Beijing and other megacities in China. Although NH3 and amines have been ubiquitously detected in the atmosphere, little is known about the specific source profiles and the corresponding source contributions. It is well accepted that agriculture-related emissions dominate the global NH3 budget in the atmosphere. However, several recent field studies demonstrated that non-agricultural emissions are the primary NH3 sources in many urban areas in China. Therefore, atmospheric models based on emission inventories concentrated on agricultural emissions may not realistically simulate the atmospheric environment, particularly in the populated megacities of China. Recently, NH3, amines, amides, and imines emission characteristics of motor vehicles have been determined explicitly through in situ roadside measurements. However, the emission features from many other anthropogenic activities are still unknown. In this study, based on constrained SoFi-PMF analysis, we have investigated the specific impacts of motor vehicle emissions on NH3 and other alkaline gases in urban Beijing. It was found that motor vehicles can contribute a predominant portion of amines in the urban environment, particularly during daytime. Hence, reducing on-road vehicular emissions can decrease primary emissions of criteria air pollutants (such as NOx, SO2, and PM2.5) and suppress secondary aerosol formation. Although the PMF-based source apportionment analysis may be subjective to individual bias, it provides a valuable opportunity to explore other non-vehicular sources. The septic system in the urban area is recognized as a significant contributor to background NH3 and amines in urban Beijing. Motor vehicle emissions usually show less seasonal variability. Intense demands for central heating, power generation, and biofuel usage in suburban areas may play a significant role in wintertime haze formation. These emission activities, however, may highly depend on environmental conditions, such as temperature and humidity. Further investigations of the underlying releasing mechanisms and emission intensities are critically needed.

How to cite: Zheng, J., Zhu, S., Yang, D., and Ma, Y.: Observation and source apportionment of atmospheric alkaline gases in urban Beijing, China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3614, https://doi.org/10.5194/egusphere-egu23-3614, 2023.

EGU23-4163 | ECS | Posters on site | AS3.15

Analysis of wintertime ozone at two urban centres in western India. 

Shubham Dhaka and Amit Sharma

Western India is a region which is exposed to pollution contributed by both natural and anthropogenic sources that may be local, regional or remote sources as reported in limited observational studies that have been conducted in the region. In the present study, temporal variation of surface ozone is studied at two urban centres (Jodhpur and Ajmer) in western India during a winter season (December 2018 – February 2019) by using ground based observation data from Central Pollution Control Board (CPCB). Jodhpur is found to have the higher seasonal average ozone (~48 µg/m3) with the daily mean values reaching to as high as 87.5 µg/m3. Ajmer closely followed with seasonal average ozone as ~44 µg/m3 and the daily mean values reaching upto 80 µg/m3. Diurnal trend (seasonally averaged) for ozone at Ajmer reveals comparatively higher afternoon values (even exceeding 100 µg/m3) but lower night time levels (close to 20 µg/m3) thus suggesting a stronger ozone production rate (~9.2 µg/m3/hr) at Ajmer during daytime (0600 – 1500 hrs local time). The ozone production rate at Jodhpur is lower (5.4 µg/m3/hr) during the same time due to lower afternoon values (~80 µg/m3) and higher nighttime levels (> 30 µg/m3). Subsequently, a detailed analysis is performed for the monthly peak ozone days in each winter month for both urban centres using ground based observation data, a back trajectory model  and a widely used reanalysis dataset. The analysis reveals contribution of both regional as well as long range transport from different directions in different months to higher levels of surface ozone, in addition to enhanced photochemistry and/or weak ozone titration on some days.  The ozone levels even breached the Indian National Ambient Air Quality Standards (NAAQS) limit of 100 µg/m3 set by CPCB for daily maximum 8 hour ozone concentration on some of the monthly peak ozone days at both urban centres. The study highlights the importance of transported ozone in enhancing ozone levels over the western India region during winter which may have severe impacts on vegetation, human health and climate change.

How to cite: Dhaka, S. and Sharma, A.: Analysis of wintertime ozone at two urban centres in western India., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4163, https://doi.org/10.5194/egusphere-egu23-4163, 2023.

Transition metal components in PM2.5 induce inflammation of the respiratory system. The increase in aerosol acidity due to gaseous pollutants promotes metal dissolution and contributes to redox activation. In this study, the impact of renewable energy shifting, passenger car electrification and light-weighting on atmospheric concentration of PM2.5 total mass, Fe, Cu, Zn and aerosol acidity in Japan over 2050 was evaluated using a regional meteorology-chemistry model. The primary emissions of PM2.5, Fe, Cu, and Zn were reduced by 9%, 19%, 18% and 10%, and their surface wide-area concentrations decreased 6 – 8%, 10 – 12%, 16 – 18% and 2 – 4%, respectively. On a PM2.5 mass basis, battery electric vehicles (BEVs) have been considered to have no advantage in non-exhaust PM emissions because the increased tire and road wear and resuspension due to their heavy weight offset the benefit of brake wear reduction by regenerative brake. Indeed, passenger car electrification without light-weighting also did not significantly reduce total primary PM2.5 emissions in Japan in this study (-1.4%), but was highly effective in reducing metals, especially Fe and Cu (-6.7% and -11.4%, respectively). Furthermore, this study estimated that even tire and road wear and resuspension could be reduced if the drive battery and body frame were light-weighted, and the benefit would be larger. Therefore, vehicle electrification (mainly BEVs) and light-weighting could be one of the effective means of reducing the risks of respiratory inflammation. The renewable energy shifting reduced SOx and NOx emissions from thermal power plants and decreased aerosol acidity near power plants (approximately pH +0.2), while the passenger car electrification reduced NOx and NH3 emissions and slightly increased aerosol acidity in urban, as a result of acid-base balance (in July, approximately pH -0.1 – -0.2). However, anyway, the sensitivity of water-soluble metal concentrations was mostly dependent on changes in primary metal emissions and little affected by changes in aerosol acidity (0 – +2% for Fe, 0 – +0.5% for Cu and Zn). Therefore, it was suggested that primary emission control of metals is more important than gaseous pollutants in reducing water-soluble metal concentrations.

How to cite: Kayaba, S. and Kajino, M.: Impact of energy and vehicle transformation through 2050 on atmospheric PM2.5-metals concentration and aerosol acidity that induce respiratory inflammation in Japan;  focus on the changes in exhaust/non-exhaust and upstream emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4749, https://doi.org/10.5194/egusphere-egu23-4749, 2023.

EGU23-4794 | ECS | Posters on site | AS3.15

Machine learning based estimation of urban on-road CO2 concentration in Seoul 

Chaerin Park and Sujong Jeong

As it is predicted that the amount of urban on-road CO2 emissions will continue to increase, it is essential to manage urban on-road CO2 concentration for effective urban CO2 mitigation. However, limited observation of on-road CO2 concentration prevents the full understanding of the variation of urban on-road CO2 concentration. Therefore, in this study, a machine learning based model that predicts on-road CO2 concentration (CO2traffic) was developed for Seoul, South Korea. This model predicts hourly CO2traffic with high precision (R2 = 0.8 and RMSE = 22.9 ppm) by utilizing CO2 observation, traffic volume, traffic speed, and wind speed data as main factors. Analyzing the CO2traffic data predicted by the model, the high spatiotemporal inhomogeneity of CO2traffic over Seoul with 14.3 ppm by time and 345.1 ppm by road was found. The large spatiotemporal variability of CO2traffic is related to different road types (major arterial road, minor arterial road, and urban highway) and land-use types (residential, commercial, bare ground, and urban vegetation) where the road belongs. The cause of the increase in CO2traffic was different by its road type, and the diurnal variation of CO2traffic was different by its land-use type. Our results demonstrate that high spatiotemporal on-road CO2 monitoring is needed to manage the urban on-road CO2 concentration showing high inhomogeneity. In addition, it suggests that a model using machine learning techniques can be an alternative for monitoring CO2 concentrations on all roads without conducting the observation.

This work was supported by Korea Environment Industry &Technology Institute(KEITI) through "Climate Change R&D Project for New ClimateRegime.", funded by Korea Ministry of Environment(MOE) (2022003560006).

How to cite: Park, C. and Jeong, S.: Machine learning based estimation of urban on-road CO2 concentration in Seoul, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4794, https://doi.org/10.5194/egusphere-egu23-4794, 2023.

Fossil fuel combustion is one of the largest contributors to anthropogenic greenhouse gas (GHG) emissions, especially in megacities around the world. To characterize the vehicle emissions in Seoul, the megacity of South Korea, we collected air samples from the entry and exit points of three tunnels (Sang-Do, Bong-Cheon, and Gwan-Ak Tunnel) and Seoul National University Campus and measured dry molar mixing ratios of major greenhouse gases spices (CO2, CH4, and N2O). The N2O:CO2 emission molar ratio from vehicles is 4.3 ± 0.3 × 10-5, within a range of 1.8 – 18.7 × 10-5 previously reported in Germany, Switzerland, Sweden, and the USA. The CH4:CO2 emission molar ratio from the Sang-Do tunnel is 50.6 ± 18.0 × 10-5, which is significantly greater than those observed in Switzerland, the USA, and China (3.5 - 15 ± 4 ×10–5). In the Bong-Cheon and Gwan-Ak tunnels, however, there was little difference in entry and exit, or rather, the exit was smaller, and it might be related to the ventilation system and vehicle types. We also compared our estimation of the GHG emissions from vehicles with the National Greenhouse Gas Inventory Report of Korea (GIR, 2021) which is based on a bottom-up emission calculation method. With the CO2 emissions (8108.33 Gg CO2eq) from the GIR, the N2O and CH4 emissions in Seoul are estimated to be (108.08±24.60) Gg CO2eq and (62.75±18.92) Gg CO2 eq, respectively. The differences between our observations and inventory imply that the estimation of the non-CO2 gas (CH4, N2O) emission factors should be improved. To characterize the N2O from vehicles, we analyzed N2O stable isotopic compositions by an IRMS method. The δ15N and δ18O values of N2O emitted from the vehicles are estimated as -7.1 ± 1.5 ‰ and 41.2 ± 0.2 ‰, respectively. The δ15N values support the idea that the N2O is produced through catalytic convertors in vehicles which are attached to reduce the NOx emission at the tailpipe. The newly measured data from Seoul may help us better understand greenhouse gas emissions from vehicles in megacities.

How to cite: Kim, J., Ahn, J., and Ghosh, S.: Greenhouse gas emission from vehicles in Seoul megacity, South Korea: Molar ratios (N2O:CO2, CH4:CO2) and stable isotopic compositions of N2O (d15N, d18O), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4938, https://doi.org/10.5194/egusphere-egu23-4938, 2023.

EGU23-5216 | Orals | AS3.15 | Highlight

The Short-Term Impact of Air Pollution on Healthcare Expenditures 

Haofan Zhang, Dianyu Zhu, Pan He, Miaomiao Liu, and Jun Bi

Understanding the health impact of air pollution is critical for understanding the benefit of environmental regulations, especially under the synergies of carbon neutrality and air pollution control. We examine the effect of fine particulate matter (PM2.5) on individual healthcare expenditures in China from 2017 to 2019 using daily transaction data from 320 cities and evaluate the health co-benefits of carbon neutrality. Results show that each 10 μg/m3 increase in daily PM2.5 exposure is associated with a 0.31 percent increase in three-day healthcare consumption and a 0.53 percent increase in three-day individual healthcare expenses. Achieving carbon neutrality goals with the national air quality daily standard of 35 μg/m3 can save 1.5 billion yuan annually. Ambitious goals with World Health Organization Air Quality Guidelines of 15 μg/m3 can nearly double the saving. This study not only provides insight into the potential health benefits of carbon neutrality in China but also suggests that extensive benefits may result from more ambitious targets.

How to cite: Zhang, H., Zhu, D., He, P., Liu, M., and Bi, J.: The Short-Term Impact of Air Pollution on Healthcare Expenditures, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5216, https://doi.org/10.5194/egusphere-egu23-5216, 2023.

EGU23-6009 | ECS | Orals | AS3.15

MAX-DOAS measurements characterise severe ozone pollution in Central London during summer 2022 heatwaves 

Eleanor Gershenson-Smith, Robert G. Ryan, Eloise A. Marais, Robbie Ramsay, Jan-Peter Muller, Jan-Lukas Tirpitz, and Udo Friess

In the UK, the public health threat of heatwaves is exacerbated by the co-occurrence of ozone pollution episodes. Here we present retrieved vertical profiles of nitrogen dioxide (NO2) and formaldehyde (HCHO) over Central London from a newly installed long-term Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) instrument on a 60-m altitude rooftop site during two of three heatwaves in the hottest summer on record. We evaluate routine space-based sensor observations of air pollutant precursors over London and enhance the permanent air quality monitor network. Daily mean tropospheric column densities of NO2 and HCHO from the TROPOspheric Monitoring Instrument (TROPOMI) are consistent with those from the MAX-DOAS (both R = 0.71) after accounting for different vertical sensitivities. As expected, TROPOMI NO2 is 27-31% less than MAX-DOAS NO2, due to horizontal dilution of local sources of road-traffic NO2. TROPOMI HCHO is 20% more than MAX-DOAS HCHO; a larger difference than in past validation studies, but within the range of systematic retrieval errors. MAX-DOAS lowest layer (0-110 m) retrievals have analogous day-to-day variability to surface site NO2 (R ≥ 0.7). Surface site measurements of isoprene, which rapidly oxidises to HCHO with a high yield, also have similar diurnal variations to MAX-DOAS HCHO (R > 0.6). Generally, daytime ozone production, which is diagnosed with MAX-DOAS HCHO:NO2 tropospheric column ratios, is limited by the availability of volatile organic compounds. During heatwaves, ozone production shifts from NOx-saturated to NOx-limited as biogenic emissions of isoprene increase exponentially with temperature, leading to non-compliance with ozone regulatory standards. In ongoing work, we are assessing the ability to retrieve the NOx (NO + NO2) reservoir compound nitrous acid (HONO) to address uncertainties in HONO chemistry. This will aid understanding of the oxidation capacity of the atmosphere and ozone budget in centres of megacities such as London.

How to cite: Gershenson-Smith, E., Ryan, R. G., Marais, E. A., Ramsay, R., Muller, J.-P., Tirpitz, J.-L., and Friess, U.: MAX-DOAS measurements characterise severe ozone pollution in Central London during summer 2022 heatwaves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6009, https://doi.org/10.5194/egusphere-egu23-6009, 2023.

EGU23-6240 | Posters on site | AS3.15

Low-cost NO2 measurements at an urban high traffic site 

Christoph Beck, Verena Fricke, Andreas Philipp, Carlos Pusch, Florian Reich, and Jonathan Simon

A network of low-cost air quality sensors for monitoring NO2- and O3-concentrations has been installed at an urban high traffic site in the city of Munich (Bavaria, South Germany). NO2-measurements conducted over a period of several seasons are used to analyse the effectiveness of novel air filtering systems that have been installed alongside the street section.

Estimates of hourly mean NO2-concentrations at the network sites are determined by applying several calibration methods (linear and non-linear models) that were fitted, validated and compared based on data gathered during two periods where all sensors were co-located at an on site official reference station.

Resulting NO2-estimates at the low-cost network sites are further analysed with respect to spatiotemporal variations in NO2-concentrations. Thereby the effects of local scale variations in the urban environment, varying traffic loads, changing synoptic weather types and different operating conditions of the air filtering systems are considered.

The contribution presents and discusses different approaches for the calibration of the low-cost NO2 measurements and shows preliminary results of the analyses of spatiotemporal NO2 variations in a high traffic urban environment under special consideration of the effectiveness of novel air filtering systems.

How to cite: Beck, C., Fricke, V., Philipp, A., Pusch, C., Reich, F., and Simon, J.: Low-cost NO2 measurements at an urban high traffic site, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6240, https://doi.org/10.5194/egusphere-egu23-6240, 2023.

EGU23-6314 | Orals | AS3.15

Black carbon, organic carbon, and nitrogen oxide emission factors for traffic and domestic heating in an urban environment 

Balint Alfoldy, Asta Gregorič, Matič Ivančič, Irena Ježek-Brecelj, and Martin Rigler

Urban air quality deterioration has different reasons in warm and cold seasons. During summer, the photochemical production of secondary air pollution causes problems (ozone, secondary particles), while domestic heating significantly increases the primary emission during winter. In addition, the elevated emission is concentrated in a shallow mixing layer that leads to high air pollution levels. The source profile of domestic heating depends on the heating method. In European cities gas heating and wood combustion are the most common heating methods. Although distant heating is also commonly used, its emissions appear at the industrial source and are negligible for local air quality (similarly for less spread electric heating). In this work, we determined the emission ratios (ER) and emission factors (EF) of black carbon (BC), organic carbon (OC), and nitrogen oxide (NOX) in an urban environment, during the heating season. BC and OC concentrations were measured by the Carbonaceous Aerosol Specification System (CASS, Aerosol d.o.o, Slovenia), while NOX data was recorded by a nCLD-AL2 NOX analyzer (Eco Physics AG., Switzerland). The monitoring system was complemented by a Carbocap GMP-343 CO2 sensor (Vaisala, Finland) in order to measure the CO2 concentration for the EF calculation. The measurement took place in the atmospheric monitoring station of the Aerosol d.o.o in Ljubljana, Slovenia, which can be characterized as an urban background location. The source apportionment was implemented by using the Aethalometer model – multilinear regression combination (AM-MLR) assuming two major sources of urban air pollution: traffic and domestic heating. Fossil fuel-derived BC (BCFF) concentration was assumed as the tracer of traffic emission, while biomass burning-related BC (BCBB) was considered as the tracer of domestic heating. The Aethalometer model provides the source-specific (FF- or BB-derived) BC component. During the AM-MLR method, we supposed that the source-specific pollution component is correlated with the corresponding BC component (BCFF or BCBB). The slope of the regression line provides the ER, while the ratio of CO2 to the other pollutants can be converted to EF (g(kg fuel)-1) using the carbon balance approach. We applied the AM-MLR method to the dataset for the winter of 2021-2022 and determined the ER and EF values. The obtained EFs for traffic-related BC, OC, and NOX are 0.39, 0.33, and 0.03 g(kg fuel)-1 respectively, while the heating-related EFs are 0.13, 0.48, and0.01 g(kg fuel)-1 respectively. This work provided real-world emission factor data of a city that can help to estimate the total BC, OC, and NOX emissions in a city based on the sold fuel or consumed wood and gas.

How to cite: Alfoldy, B., Gregorič, A., Ivančič, M., Ježek-Brecelj, I., and Rigler, M.: Black carbon, organic carbon, and nitrogen oxide emission factors for traffic and domestic heating in an urban environment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6314, https://doi.org/10.5194/egusphere-egu23-6314, 2023.

EGU23-7014 | ECS | Orals | AS3.15

Black Carbon source apportionment using time-dependent Absorption Angstrom Exponent (AAE) 

Marjan Savadkoohi, Marco Pandolfi, Andrés Alastuey, Xavier Querol, and Olivier Favez

Among the aerosol particles optical properties, the Absorption Angstrom Exponent (AAE) is a crucial parameter describing the spectral dependence of light absorption by aerosols. It is intensively employed for black carbon (BC) source apportionment and aerosol characterization (e.g., BC, Brown Carbon “BrC,” and dust). AAE has been widely investigated using data from filter-based absorption photometers such as the AE33 that measure light absorption at seven wavelengths (370-950 nm). BC source contribution is commonly obtained by applying the most frequent source apportionment method, the Aethalometer model. This model requires a-priori knowledge of the AAE of the fossil and non-fossil (e.g. biomass burning) BC sources and values of around 1 (AAEff; fossil) and 2 (AAEwb; non-fossil) are commonly used. In this work, in order to improve the results of the aethalometer model for BC source apportionment, we investigate the model performances resulting from using site-dependent AAEff and AAEwb determined from the experimental data. These latter were obtained by studying the frequency distributions of experimental AAE calculated from AE33 data collected at urban sites in the frame of the RI-URBANS project. However, AAE can also vary with time depending on changing burning fuels and burning conditions, and single constant AAEff and AAEwb values cannot be representative of the whole measurement period considered. For this reason, we also evaluated the use in the Aethalometer model of experimental time-dependent rolling AAEff and AAEwb. This improved AAE-frequency-distribution-based Aethalometer model could be applied in near-real time to obtain the BC source apportionment. Thus, it could help to improve our understanding of AAE values considering uncertainties to provide a better and more accurate quantity to differentiate between BC sources.

How to cite: Savadkoohi, M., Pandolfi, M., Alastuey, A., Querol, X., and Favez, O.: Black Carbon source apportionment using time-dependent Absorption Angstrom Exponent (AAE), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7014, https://doi.org/10.5194/egusphere-egu23-7014, 2023.

EGU23-7172 | ECS | Orals | AS3.15

Design, deployment, and exploitation of a high-density CO2 sensor network in Zürich City 

Stuart Grange, Pascal Rubli, Christoph Hueglin, Andrea Fischer, Simone Baffelli, Dominik Brunner, and Lukas Emmenegger

Since July 2022, a high-density CO2 monitoring network has been operating in and around Zürich City, Switzerland as part of the ICOS Cities project. The network is formed of 80 sites that have been equipped with CO2 monitors with varying performance and cost points. Three high-precision CO2 gas analysers, 20 mid-cost sensors (installed with reference gas cylinders), and 114 low-cost sensors are in use with some sites having multiple sensors installed. Combined with several modelling approaches, the observations from the sensor network will allow for the characterisation of the city's emissions and to validate the city's CO2 emission inventory. The different types of CO2 monitors are combined with different data processing strategies to ensure their observations are adjusted for sensor drift and changes in responses so they can be used for robust analysis in near-real time. Between July 2022 and early January 2023, the CO2 network's mean concentration was 446 ppm and the difference between the network's background and urban-traffic sites was 31 ppm suggesting a significant urban enhancement during this period. Distinct daily and seasonal patterns were observed for different types of sensor locations, reflecting diverse emission regimes across the urban area. Despite careful efforts during the site selection process, local contamination has been observed for many rooftop sensors due to their proximity to heating stacks. However, the installation of wind sensors allows for the observations to be flagged for such situations, which will be important for downstream data users. Details on the sensor adjustment strategies, the technologies in use for the data processing pipeline, the results from several months of CO2 monitoring, and future plans with the other two ICOS Cities sensor network collaborators (Munich and Paris) will be discussed. 

How to cite: Grange, S., Rubli, P., Hueglin, C., Fischer, A., Baffelli, S., Brunner, D., and Emmenegger, L.: Design, deployment, and exploitation of a high-density CO2 sensor network in Zürich City, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7172, https://doi.org/10.5194/egusphere-egu23-7172, 2023.

EGU23-7484 | Orals | AS3.15

Effects of the closure of Berlin-Tegel Airport on ultrafine particle concentration on the airport site 

Sabine Fritz, Sebastian Aust, and Tobias Sauter

Airports contribute significantly to the concentration of ultrafine particles (UFP) at the local level. UFP from combustion processes are produced when aircraft take off and land, during aircraft movements on the tarmac, when turbines are started, but also by vehicles transporting goods and people on the airfield. UFP are considered particularly harmful to human health due to their large surface area. They can also penetrate far into the human body due to their small size.

This study examines the extent to which particle number concentration (PNC) responds to the cessation of air traffic due to the relocation of an airport. PNC and wind data were measured at one station on the airfield downwind of the runways for the prevailing wind direction for about three weeks each before and after the closure of the airport.

We observed a 30 - 40 % drop in PNC after the closure of the airport regardless of the wind direction. 70 % higher PNC on average, 2.5 times higher maximum values as well as a three times higher dispersion of PNC occured with wind from the direction of the airport before the closure of the airport than afterwards. These differences are only evident during the day when air traffic is active and not during the nighttime flight restrictions. More frequent and higher concentration peaks occur in conjunction with wind from the airport before flight operations ceased.

The special circumstances resulting from the relocation of the airport allow clear conclusions to be drawn about the importance of airport operations for PNC in the area of the airfield. As the study took place under Covid-19 pandemic conditions, it shows the impact of aircraft movements on PNC, but does not allow conclusions about air pollution during normal air traffic. Further studies or modelling on the spatial dispersion of airport-related air pollutants and thus on the exposure of the population living and working nearby can close the gap on health effects of air traffic.

The study has been published as Fritz S., Aust S. and Sauter T. (2022): Impact of the closure of Berlin-Tegel Airport on ultrafine particle number concentrations on the airfield. Front. Environ. Sci. 10:1061584, doi: 10.3389/fenvs.2022.1061584. The study was supported by the German Federal Ministry of Education and Research (BMBF) under grant FKZ 01LP 1912B (Urban Climate under Change, Phase II, Module 3DO + M).

How to cite: Fritz, S., Aust, S., and Sauter, T.: Effects of the closure of Berlin-Tegel Airport on ultrafine particle concentration on the airport site, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7484, https://doi.org/10.5194/egusphere-egu23-7484, 2023.

EGU23-7542 | ECS | Orals | AS3.15

Application of the ICON-ART model for CO2 fluxes estimation in the city of Zurich 

Nikolai Ponomarev, Michael Steiner, Erik Koene, Lionel Constantin, Pascal Rubli, Lukas Emmenegger, and Dominik Brunner

Switzerland like many other countries has set ambitious goals to reach net zero CO2 emissions by 2050. The city of Zurich has committed to an even more ambitious goal of becoming climate neutral by 2040. Recent developments in atmospheric observations and inverse modelling, including the results of the European infrastructure project ICOS, have already laid down the foundations for estimating emissions on national and continental scales. At urban scales, however, only few emission estimation studies have been conducted so far, and it is still an open question, which observational and modeling approaches are best suited and to what level of accuracy they are able to quantify the emissions of a city. The project ICOS-Cities/PAUL aims to answer these questions by evaluating different monitoring approaches in three European pilot cities. One of these cities is Zurich, where a street-level network of about 93 low-cost sensors at 60 locations is combined with a network of 21 mid-cost sensors, located mainly on roof-tops, and high-precision instruments at 3 background sites.

Our goal is to estimate the CO2 emissions of Zurich by combining the observations from the mid-cost and high-precision instruments with the state-of-the-art atmospheric transport model ICON-ART. To this end, numerical experiments were conducted for two offline-nested domains, a European domain at ~6.6 km resolution and a second domain centered over the city of Zurich with a much higher resolution of ~0.6 km to represent the main topographic features of the urban area. Anthropogenic emission inputs were produced by merging three different inventories: the TNOGHGco inventory for areas outside Switzerland, a Swiss national inventory at 100 m resolution, and a detailed inventory of point, line and area sources produced by the city of Zurich. The biogenic fluxes of CO2 were computed online using the Vegetation Photosynthesis and Respiration Model (VPRM) integrated into ICON-ART.

Here we present a first analysis of comparisons between model simulations and CO2 observations inside and surrounding the city. This allows us to better understand the capabilities and weaknesses of the model at urban scales as well as to design optimal strategies for setting up an inversion framework.  A particular focus is placed on biospheric CO2 and on how much it contributes to variability within the city in comparison with anthropogenic CO2. The next steps will include the use of the CTDAS (The CarbonTracker Data Assimilation Shell) assimilation system in order to obtain information on CO2 fluxes in the urban and suburban areas of Zurich and to apply the model system also to the city of Paris. During this work, we strive to develop approaches which can then be shared and applied by researchers to other cities around the world.

How to cite: Ponomarev, N., Steiner, M., Koene, E., Constantin, L., Rubli, P., Emmenegger, L., and Brunner, D.: Application of the ICON-ART model for CO2 fluxes estimation in the city of Zurich, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7542, https://doi.org/10.5194/egusphere-egu23-7542, 2023.

EGU23-7589 | ECS | Posters on site | AS3.15

Eddy covariance measurements of black carbon emissions in central London 

Zixuan Cheng, James Allan, Dawei Hu, Eiko Nemitz, Ben Langford, Carole Helfter, Will Drysdale, James Lee, James Cash, Sam Cliff, Dantong Liu, and Joshi Rutambhara

Black carbon (BC) is a significant environmental health and climate forcing concern. Direct measurement of black carbon fluxes using eddy covariance can quantify emissions and identify sources. Previous studies have quantified urban black carbon emissions in highly polluted countries such as China and India, but to date no research has been done in the UK and Europe. This study uses an eddy covariance system using a Single Particle Soot Photometer (SP2) deployed on the BT Tower in London to directly measure BC fluxes in central London. This is as part of the UK Integrated Research Observation System for Clean Air (OSCA). We have produced some primary results including time series of black carbon concentrations and fluxes in central London in winter and summer and diurnal profiles. Comparisons with NOx and organic matter fluxes are also underway to identify the main sources of black carbon in central London and suggest that due to recent emissions controls, cooking may now be the most significant local source rather than transport or space heating.

How to cite: Cheng, Z., Allan, J., Hu, D., Nemitz, E., Langford, B., Helfter, C., Drysdale, W., Lee, J., Cash, J., Cliff, S., Liu, D., and Rutambhara, J.: Eddy covariance measurements of black carbon emissions in central London, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7589, https://doi.org/10.5194/egusphere-egu23-7589, 2023.

EGU23-7665 | ECS | Posters on site | AS3.15

Monitoring and quantifying CO2 emissions of isolated power plants from space 

Xiaojuan Lin, Ronald van der A, Jos de Laat, Henk Eskes, and Zhu Liu

CO2 emissions of power plants are often self-reported and calculated based on fuel consumption. The authenticity of CO2 emission data from power plants are preferable to be verified by independent measurements. Satellite observations can provide these CO2 emission observations from isolated power plants. However, there are two difficulties in the current top-down anthropogenic CO2 emission inversions, that is, (1) the anthropogenic CO2 emission signal is difficult to distinguish from the background of other emitted CO2, and (2) the temporal and spatial resolution of CO2 satellite observation data are currently limited. In this study, we focus on how to improve the accuracy of CO2 emissions using different methods and wind data estimates. We assess these emission estimates by comparison with USA EPA emission data, and identify and explore suitable cases elsewhere in the world. We have selected only isolated power plants for this study, to avoid complications because of multiple sources in close proximity. We first compare the Gaussian plume model and cross-sectional flux methods for estimating CO2 emissions of power plants. Then we examine the sensitivity of the emission estimates to possible choices for the wind field. For verification we have used power plant emissions that are reported on an hourly basis by the Environmental Protection Agency (EPA) in the United States. By using the OCO-2 and OCO-3 observations over the past four years we identified emission signals of isolated power plants and arrived at a total of 50 collocated cases involving 22 power plants. We found the wind field halfway the height of planetary boundary layer (PBL) yielded the best results. We found that the instantaneous satellite estimated emissions of these 50 cases and reported emissions display a weak correlation (R2=0.12). The correlation improves with averaging over multiple observations of the 22 power plants (R2=0.40). The method was subsequently applied to 106 power plants cases worldwide. We demonstrate that accurate estimation of power plant emissions can be achieved by monitoring from future satellite missions with more frequent observations.

How to cite: Lin, X., van der A, R., de Laat, J., Eskes, H., and Liu, Z.: Monitoring and quantifying CO2 emissions of isolated power plants from space, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7665, https://doi.org/10.5194/egusphere-egu23-7665, 2023.

EGU23-7712 | Orals | AS3.15

Development, intercomparison and analysis of city emission inventories in support of independent verification of city greenhouse gas budgets 

Hugo Denier van der Gon, Rianne Dröge, Ingrid Super, Arjan Droste, Dominik Brunner, Ivo Suter, Lionel Constantin, Olivier Perrussel, Olivier Sanchez, Jia Chen, Patrick Aigner, and Daniel Kühbacher

The ICOS-cities PAUL project aims to support the European Green Deal by solving specific scientific and technological problems related to the observation and verification of greenhouse gas (GHG) emissions from densely populated urban landscapes. To this end, comprehensive city observatories, applying various in situ and ground-based remote sensing GHG measurement technologies, will be developed and evaluated in a relatively large (Paris), medium (Munich) and small (Zürich) city. A critical input for the optimal design of such observatories are complete, spatially explicit, state-of-the-art city emission inventories for greenhouse gases and co-emitted species. Currently the emission data available for European cities vary considerably in source sector completeness, spatial resolution, base year and temporal disaggregation. Our target resolution in the ICOS-cities PAUL project is 100 x 100 meter, hourly resolution for a recent year like 2018 or 2019 to avoid impact of the Covid-19 pandemic. Such data would allow evaluation of the city budget and more detailed district level budgets, which can support tailored climate action plans. For Paris (3 x 3 km) and Zurich (100 x 100 m), emission inventories are developed by respectively, AIRPARIF and EMPA in collaboration with the municipality of Zurich. The emission inventory for Munich is based on the downscaling of the 1 x 1 km TNO-GHGco inventory where key source sectors are stepwise replaced by bottom-up estimates by TUM and TNO. Here we harmonize source sectors and evaluate and intercompare the emission inventories of the three cities. We identify dominant source sectors and potentially missing sources, and determine ratios between GHG and co-emitted species necessary for source sector attribution. Furthermore, we compare the results against downscaled national reported emission data in line with the official reporting to UNFCCC, and draw conclusions on consistency between national scale and city scale inventories. Lessons learned will lead to the development of a more general methodology to provide city emission data to other European cities and, as part of the overall ICOS-cities objective, robust observation-based methods for quantifying city GHG emissions and sinks to assess the impact of city climate actions.

How to cite: Denier van der Gon, H., Dröge, R., Super, I., Droste, A., Brunner, D., Suter, I., Constantin, L., Perrussel, O., Sanchez, O., Chen, J., Aigner, P., and Kühbacher, D.: Development, intercomparison and analysis of city emission inventories in support of independent verification of city greenhouse gas budgets, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7712, https://doi.org/10.5194/egusphere-egu23-7712, 2023.

EGU23-7768 | Orals | AS3.15

CO2 net ecosystem flux in Krakow, Poland 

Alina Jasek-Kaminska, Miroslaw Zimnoch, Lukasz Chmura, and Jakub Bartyzel

Urban areas, with dynamically changing, varied sources and sinks in highly heterogeneous terrain, are one of the most complicated ecosystems to explore. Being also a significant CO2 net source, they contribute largely to uncertainty in local and global carbon balance calculations. Experimental data are required to verify existing CO2 emission inventories and to become a reliable input to climate models.

Since 2021 an eddy covariance site has operated in Krakow, southern Poland. Site neighborhood includes various anthropogenic sources and sinks such as traffic, household heating, mainly with natural gas, and people themselves. On the other hand, a significant part of the source area is covered in green, with a municipal park and a number of home gardens.

We are presenting a data record from the beginning of the measurements in February 2021 up to the present. As expected, the area is a net CO2 source, emitting on average around 7 kg of CO2 per square meter yearly. Clear diurnal and seasonal patterns of CO2 net flux were observed: morning and evening traffic peaks and negative values during the day due to active photosynthesis; also higher diurnal amplitude during the warm season but on average higher net CO2 emission in winter. Directional flux analysis reveals that 1) the highest emissions come from the area where individual households as well as busy traffic lanes are located; and 2) urban green areas have a potential to become a net CO2 sink during the day in all seasons except winter, however, mean diurnal emission on average remains positive.

This project has been partially supported by the European Union’s Horizon 2020 research and innovation program CoCO2 under grant agreement No. 958927, "Excellence Initiative - Research University" program at AGH University of Science and Technology, and the subsidy of the Ministry of Education and Science.

How to cite: Jasek-Kaminska, A., Zimnoch, M., Chmura, L., and Bartyzel, J.: CO2 net ecosystem flux in Krakow, Poland, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7768, https://doi.org/10.5194/egusphere-egu23-7768, 2023.

EGU23-8003 | ECS | Posters on site | AS3.15

Development and deployment of a “Mid Cost” sensor network for urban Greenhouse Gases and Air Quality monitoring with a focus on CO2. 

Mali Chariot, Olivier Laurent, Damien Delanoe, Guillaume Nief, Hervé Utard, and Luc Lienhardt

As part of the European research project ICOS-Cities, the Laboratoire des Sciences du Climat et de l'Environnement (LSCE) and Origins.earth are seeking to extend the Greenhouse Gases (GHG) measurement network in Paris and its immediate suburbs by installing new sensors on the roofs of tall buildings. Each sensor will measure CO2 concentration in real time, which will then be used in an inversion model to determine CO2 emissions at the scale of a district. Several sensors will be upgraded in a second phase with the addition of an Air Quality (AQ) measurement cell.

We present a new stand-alone sensor box design (called AtmoBox) that allows to connect GHG and AQ sensors in a single box, as well as the implementation of these Atmoboxes in a ground-based atmospheric monitoring network. In addition to 9 long-term stations equipped with high precision CRDS spectrometers, about 30 Mid Cost instruments are deployed within Paris and its near suburb, measuring CO2 through NDIR sensors. We will detail the steps from the search for suitable sites for the urban measurements, the characterisation of the sensors in relation to the environmental parameters in the laboratory, the related calibration and quality control strategy to meet the performance objective and the performance assessment of the sensors.

How to cite: Chariot, M., Laurent, O., Delanoe, D., Nief, G., Utard, H., and Lienhardt, L.: Development and deployment of a “Mid Cost” sensor network for urban Greenhouse Gases and Air Quality monitoring with a focus on CO2., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8003, https://doi.org/10.5194/egusphere-egu23-8003, 2023.

EGU23-8403 | ECS | Orals | AS3.15

Winter 2022 thermal anomaly and energy crisis impact on air quality in urban and rural areas assessed with dense sensor networks 

Tommaso Giordano, Lorenzo Brilli, Federico Carotenuto, Alice Cavaliere, Giovanni Gualtieri, Beniamino Gioli, Carolina Vagnoli, and Alessandro Zaldei

The current socio-economic and political scenario is posing serious challenges to energy usage, mobility, residential and industrial activities, which may impact local emission patterns, fossil fuel vs alternative fuels usage and air quality in unknown ways. On top of this, winter 2022-23 is being exceptionally warm across the European continent.

The investigation of the interactions between air quality, meteorological factors and emissions sources at high spatio-temporal resolution plays a crucial role to detect areas and periods characterized by critical conditions, especially in complex urban environments. Data at such fine resolution can today be obtained through dense low-cost sensor networks integrating sparse official air quality stations. This research aims to assess meteorological forcing, emission proxies (i.e., population density, CO2 local enhancement, land-use) and particulate matter concentrations (PMs) for the last three winter seasons (2020-2023) characterized by contrasting conditions. The study was focused on the Lucca plain (central Italy), an area characterized by heterogeneous emission sources and classified among the most polluted in the region. Sixteen low-cost stations (“AirQino”), equipped with high-frequency sensors to detect PM10, PM2.5, air-temperature, relative humidity (RH), and CO2 concentration were installed on an area spanning approximately 10 x 20 km. Local land use surrounding the measurement stations was obtained from the Corine Land Cover. Mixing Layer Height (Hmix) and wind data were obtained from a WRF-CALMET coupled model. Population density was computed with demographic data from the Global Human Settlement database. For CO2 data, the nocturnal enhancement normalized by wind speed with respect the minimum midday values was used as an emission proxy (ΔCO2). Population density and land use including fractions of residential, industrial, and agricultural areas were computed in a 1-km radius surrounding each station.

Preliminary comparisons between winter 2021/2022 and 2022/23 were performed to assess the effects of energy crisis and climatic conditions on air-quality. Different multivariate regression models were developed to investigate the inference between Hmix, air-temperature, RH, ΔCO2, population density, land use and PMs concentrations.

Most recent analysis shows a consistent and robust positive air temperature anomaly in November-December 2022 vs 2021 (+ 1.25 °C). CO2 enhancements were on average 20% lower (-19.0 to +3.7 ppm in 2022 vs 2021 respectively) suggesting a relevant emission reduction occurring at the landscape scale. However, these reductions did not always translate into PM10 and PM2.5 reductions and air quality improvements. Among the 16 stations, 11 exhibited a decrease in PM2.5 concentration (-21.60 % on average) and only 9 in PM10 (-21.55 % on average). The locations where air quality did not improve or was even worse this year are characterized by the lowest population density and lowest presence of residential neighborhoods, being mostly in rural or rural/industrial contexts. This suggests that alternative fuels such as wood biomass are likely replacing natural gas in peri-urban areas for domestic heating, generating a negative impact on air quality that could be much worst when usual lower temperature conditions will be met. A complete multivariate analysis to confirm these patterns will be presented.

How to cite: Giordano, T., Brilli, L., Carotenuto, F., Cavaliere, A., Gualtieri, G., Gioli, B., Vagnoli, C., and Zaldei, A.: Winter 2022 thermal anomaly and energy crisis impact on air quality in urban and rural areas assessed with dense sensor networks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8403, https://doi.org/10.5194/egusphere-egu23-8403, 2023.

EGU23-8718 | Posters on site | AS3.15

Characterization of PM10 fraction before pandemic and during pandemic COVID-19 at the traffic station in Krakow, Poland 

Lucyna Samek, Anna Ryś, Zdzisław Stęgowski, and Katarzyna Styszko

Samples of PM10 were collected at the traffic station in Krakow, Poland during two periods: 2nd February- 30th May 2018 and 2nd February 17th June 2020. PM10 concentrations were determined gravimetrically. PM10 concentrations dropped by 50% from 74±29 µg/m3 to 37±13 µg/m3 in 2018 and 2020, respectively. Elemental concentrations were determined by energy dispersive X-ray fluorescence method (EDXRF) and ion concentrations by ion chromatography (IC). 18 elements and 8 ions were measured. Ratios of concentrations in 2018 to 2020 were above 1.7 for the following elements: S, Cl, K, Zn, Br and ions SO42-, Na+, NH4+. The above-mentioned ratio was equal to 1.4 for Cu, Fe and Co. Similar concentrations in 2018 and 2020 were observed for the following chemical species: Ca, Ti, Mn, Ni, Rb, Sr, K+, Mg2+, Ca2+, PO43-. Cr concentration was higher in 2020 compared to 2018. Four factors were obtained from PMF (Positive Matrix Factorization) modelling. The following sources were attributed: solid fuel combustion, secondary inorganic aerosols, traffic/industry/construction work and soil. The contribution of traffic/industry/construction work to PM10 mass was the highest. It was equal to 24.6 µg/m3 and 23.4 µg/m3 in 2018 and 2020, respectively. The contribution of solid fuel combustion and secondary inorganic aerosols was five times lower in 2020 than in 2018. Contribution of solid fuel combustion was 14.5 µg/m3 and 2.6 µg/m3 in 2018 compared to 2020. SIA was lowering from 15.7 µg/m3 in 2018 to 2.5 µg/m3 in 2020. Traffic/industry/construction work and soil contribution was on the similar level in both years. Two factors affected characteristic of PM10: one was a ban of using coal and wood for heating purpose introduced in Krakow in September 2019 and second one was pandemic of COVID-19 started in March 2020. Our study will be helpful for the local authority in preparing future plans for reducing air pollution within the city.

Acknowledgments: This research project was supported/partly supported by the program “Excellence initiative—research university” for the University of Science and Technology. The bilateral cooperation  project nr BPN/BPT/2021/1/00001 between Poland and Republic of Portugal partially financed this work together with the subsidy of the Ministry of Science and Higher Education, grant number 16.16.220.842.

How to cite: Samek, L., Ryś, A., Stęgowski, Z., and Styszko, K.: Characterization of PM10 fraction before pandemic and during pandemic COVID-19 at the traffic station in Krakow, Poland, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8718, https://doi.org/10.5194/egusphere-egu23-8718, 2023.

EGU23-9195 | Orals | AS3.15

A low-cost airbox network to assist air quality policy-making and citizen involvement: Eindhoven city, Southeast Brabant, the Netherlands 

Jun Zhang, Ruben Goudriaan, Janot Tokaya, Arjan Hensen, Daniëlle van Dinther, Sjaak Kaandorp, Marcus Blom, and Arjan Plomp

Air pollution may threaten both human health and ecosystem vitality in Eindhoven city, the Netherlands. Although air quality changes are monitored hourly with high-end equipment at multiple national stations, it remains difficult for individual cities or citizens to trace local air quality based on national-scale information. A monitoring network of 44 low-cost airbox sensors was established around Eindhoven city to measure atmospheric concentrations of particulate matter (PM10, PM2.5, PM1) and nitrogen dioxide (NO2) at 10-min intervals from January 2021 onwards, with ultra-fine particle (UFP) sensors added at 3 dedicated sites around the airport. To address local government and citizen’s health concerns, the monitoring network was spread among three major areas: urban area (23), Eindhoven airport (3), and rural area outside of the city (18). The urban area was further divided into clean-background area, downtown, industrial zone, traffic intensified ring-roads and highways. Based on a one-year seasonal and diurnal analysis, we concluded that at least 70% of the average PM concentration was determined by the regional background contribution whilst 60% - 72% of total PM10 was contributed by fine particles with a diameter below 2.5 µm. On average, the PM values of the urban background area were still 10 - 15% higher than those for the rural area despite the assistance of city-greening facilities (such as tree-lined streets and parks). However, higher PM10 values were also frequently observed downwind of the livestock farms within the rural area across seasons. On the other hand, NO2 concentrations were mainly driven by local sources’ behavior, notably traffic emissions during morning and evening rush-hours. The three UFP sensors located around the airport showed more frequent peaks and higher values related to flight activities and airport traffic, also outside the airport terrain. The combined results underline the importance of taking spatial variability of urban air pollution sources into explicit account. Moreover, a good-quality airbox real-time monitoring network will allow local policy-makers to take proper actions to mitigate air pollution, inform local citizens and reduce health impacts at the appropriate scale.

How to cite: Zhang, J., Goudriaan, R., Tokaya, J., Hensen, A., van Dinther, D., Kaandorp, S., Blom, M., and Plomp, A.: A low-cost airbox network to assist air quality policy-making and citizen involvement: Eindhoven city, Southeast Brabant, the Netherlands, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9195, https://doi.org/10.5194/egusphere-egu23-9195, 2023.

EGU23-9755 | ECS | Orals | AS3.15 | Highlight

In-vehicle exposure to NO2 and PM2.5: influences of environmental, vehicle and driving factors 

Vasileios Matthaios, Roy Harrison, Petros Koutrakis, and William Bloss

In many developed cities, commuters spend more than 1.5-h inside vehicles daily, which may result in elevated exposures to traffic-related NO2 and PM2.5, which are known to have harmful health effects. In addition, time spend inside vehicles is likely to be greater for professional drivers, whereas the impacts of these exposures may be greater for vulnerable groups such as the elderly or obese. Therefore, reducing in-vehicle exposure and the associated risk for adverse health effects is very important.

This study measured in-vehicle NO2 and PM2.5 during repeated transects of the same route on city streets for 10 vehicles under real-world conditions, and as a function of ventilation settings and cabin filters. The results were used to assess personal exposure for driver/passengers, and to develop stepwise general additive models in order to identify important controllable factors that can reduce in-vehicle exposure.

The overall variability of in-vehicle exposure explained by these models was R2 = 0.58 and 0.52, for NO2 and PM2.5 respectively. From the model’s explained variability, the most significant predictor for both pollutants was on-road NO2 and PM2.5 levels accounting for 25.4 and 35.6% respectively. Vehicle-based predictors included car type, odometer, use of activated carbon filter, air exchange rate and use of air conditioning/air recirculation ventilation settings that, in combination, explained 48.9% and 61.1%, of NO2 and PM2.5, variability, respectively. Driving-based predictors included road traffic conditions, presence of traffic lights roundabouts and high emitters, explained 25.7% and 3.3% of NO2 and PM2.5 in-vehicle concentration variability, respectively. By carefully regulating vehicle-based factors under driver or passenger control, such as ventilation and filtration options, vehicle occupants can significantly reduce their exposure to NO2 and PM2.5.

How to cite: Matthaios, V., Harrison, R., Koutrakis, P., and Bloss, W.: In-vehicle exposure to NO2 and PM2.5: influences of environmental, vehicle and driving factors, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9755, https://doi.org/10.5194/egusphere-egu23-9755, 2023.

EGU23-10675 | Posters on site | AS3.15

Temporal variations of black carbon and nitro polycyclic aromatic hydrocarbons in Morelos, México 

Violeta Mugica, Jesús Figueroa, Brenda Valle, Tamara Alvarez, Mirella Gutiérrez, and Miguel Torres

Carbonaceous species such as nitro-polycyclic aromatic hydrocarbons (NPAHs) are toxic ubiquitous pollutants contained in the organic fraction of airborne particles, since several of them have mutagenic and carcinogenic properties. Black carbon has been recognized as a short live climatic pollutant which must be controlled in order to mitigate climatic change. Morelos is a little state of Mexico located at the South of the Metropolitan Area of Mexico City which has grown in the last years, but only few studies related with atmospheric pollution have been performed, then, with the aim to have better information related with carbonaceous compounds contained in the PM2.5 of the two main cities of Morelos, a monitoring campaign was carried out in Cuernavaca City, from 2016 to 2018, whereas in the Cuautla city the campaign was performed from 2017 to 2018. PM2.5 were collected with HighVol Tish equipment every six days. Elemental and organic carbon were analyzed with a Sunset Lab and toxic NPAHs were extracted with dichloromethane and sonication and further analyzed by gas chromatography–mass spectrometry (GC-MS). Median annual PM2.5 concentrations were 22.5 ± 7.2 mg m-3 and 19.6 ± 6.1 mg m-3, for Cuautla and Cuernavaca, respectively. Black carbon concentrations were higher in Cuautla than in Cuernavaca with 1.9 ± 0.5 mg m-3, and 1.3 ± 0.4 mg m-3 respectively, since Cuautla is a rural zone with frequent biomass burning The highest NHAPs concentrations were found in Cuautla with medians of 280.74 pg m-3, 90.67 pg/m-3 and 156.61 pg m-3, for the warm dry season (March-June), the rainy season (July-October) and the cold dry season (November-February) respectively. In Cuernavaca, the NHAPs presented lower concentrations in the three seasons with 116.41 pg m-3, 63.82 pg/m-3 and 128.99 pg m-3, respectively. 1-nitronaphtalene, 2-nitrophenentrene and 2-nitroanthracene were the most abundant compounds in both sites. Although PM2.5 Mexican Standard was not exceeded, the high concentrations of black carbon and NPAHs are of concern since black carbon is a climatic pollutant and some of the NHAPs compounds are carcinogenic.

How to cite: Mugica, V., Figueroa, J., Valle, B., Alvarez, T., Gutiérrez, M., and Torres, M.: Temporal variations of black carbon and nitro polycyclic aromatic hydrocarbons in Morelos, México, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10675, https://doi.org/10.5194/egusphere-egu23-10675, 2023.

Air pollution is recognized as the biggest environmental health risk in urban cities, as air pollution is pervasive and hard to escape. As one of the notorious atmospheric pollutants, nitrogen oxides (NOx, NO + NO2) not only promotes the formation of ozone and secondary aerosols but also have direct adverse health effects on human beings. As a typical densely populated modern metropolis, Hong Kong can serve as a reference for world cities in terms of air pollution control. Even though air quality in Hong Kong Environment Protection Department (HKEPD) has improved over recent decades, the roadside NO2 level in Hong Kong still exceeds the Hong Kong Air Quality Objectives (HKAQO), European Union Air Quality Directives (EUEQD) and the most stringent World Health Organization Air Quality Guidelines (WHOAQG). Nanomaterial-based photocatalysis that only relies upon solar energy excitation provides a sustainable solution for air pollution redemption. Generally, photocatalysts developed in the laboratory are in powder form which is not appropriate for real-world applications. However, these limitations can be overcome by coating photocatalysts on the surfaces of various substrates to immobilize those powders as films. More importantly, photocatalytic coatings are available to be supported on different substrates without changing or affecting existing settings. In this study, enhancement of NOx photocatalytic degradation ability and solar light utilization were implemented in a reformative Titanium Dioxide (TiO2) film. Hydrogen peroxide solution was utilized to peptize the crystallized nanoparticles around 5-6 nm at room temperature instead of the traditional calcination process at high temperatures, which limited the commercialization due to the expensiveness of heating. Moreover, the nanosized TiO2 film was expected to provide more active sites for reactions, which contributes to a promising photocatalytic degradation ability. Based on ISO 22197-1 evaluation standards, the as-developed photocatalytic coating possesses a NOx degradation rate of 4.402 mg*m-2h-1 when applied on the concrete surface, which was higher than Degussa (Evonik) P25 and other commercial coating products at the same conditions. An artificial weather resistance test investigation implies the photocatalytic coating will provide a strong bonding interaction with substrate materials which is beneficial to the lifetime of the coating. Further investigating from a 180-day field trial in a roadside environment in Hong Kong, the as-developed coating concrete specimen presented about 5% of attenuation in the first 30 days and sustained 13.9%-18.5% photocatalytic activity after the entire 180-day outdoor exposure. The application of photocatalytic coatings is supposed to convert the roadside NOx compounds to NO2- and NO3- which are harmless in small quantities and would be washed away by water droplets. In response to practical demands, functional nanomaterials-based photocatalytic technology has been gradually promoted as a green strategy for improvements in the air quality of megacities all over the world.

How to cite: Li, X. and Lee, S.: Development and Application of Nanomaterials-based Photocatalytic Technology for Improvement of Urban Air Quality, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10906, https://doi.org/10.5194/egusphere-egu23-10906, 2023.

EGU23-10970 | ECS | Posters virtual | AS3.15

The effect of meteorological parameters on PM2.5 pollutant by CCM method in Tehran megacity, Iran 

Soroosh Roozitalab, Khosro Ashrafi, and Kiana Yahyazadeh Shourabi

Tehran, the capital and most populous city of Iran, is always listed as one of the most air-polluted cities in the world. Nevertheless, it has not received much attention until recent years. Tehran’s PM2.5 (i.e., particulate matters with diameter smaller than 2.5 µm) annual mean concentration in 2022 was 40 µg/m3 and it experienced less than 10 days with clean air. While high emissions are the main reason of air pollution in Tehran, some studies have suggested that meteorology is also another major driver of its air pollution. Here, we investigate the correlation between PM2.5 and different meteorological parameters such as temperature, wind speed, visibility, relative, humidity, and dew point temperature. In particular, we use Multiple Linear Regression and CCM (Convergent Cross Mapping) statistical methods to analyze the ground measurements data for one year. Our primary results show that, several meteorological parameters have a significant impact on PM2.5 concentrations. The findings of this study helps characterizing the source of air pollution in Tehran.

How to cite: Roozitalab, S., Ashrafi, K., and Yahyazadeh Shourabi, K.: The effect of meteorological parameters on PM2.5 pollutant by CCM method in Tehran megacity, Iran, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10970, https://doi.org/10.5194/egusphere-egu23-10970, 2023.

EGU23-11085 | ECS | Orals | AS3.15 | Highlight

Personal air pollution exposure assessment using wearable sensors 

Sheng Ye, Melanie Ziemann, and Mark Wenig

Air quality have become a global issue with increasing attention. There is a growing concern in the public about both in- and outdoor air quality. In order to monitor individual air pollutants exposure in real-time, we developed several wearable air quality monitoring devices to study personal exposure to different pollutants in different environments. The devices are equipped with different type of sensors to measure NO2, aerosols, CO2, etc, in addition to environmental parameters sensor to measure temperature, relative humidity and pressure. In order to optimize the accuracy, we compared different retrieval approaches such as multiple linear regression, generalized linear model, neural network, etc. This allows us to perform the personal exposure study with a high temporal resolution in the order of seconds. We classified daily activities into different categories: different ways of commuting such as bus, tram, subway, bicycle, on foot; indoor activities like cooking, lighting candles, etc.; outdoor exercises next to busy street, in a park, etc. In this presentation, we will present our first result of this personal exposure study.

How to cite: Ye, S., Ziemann, M., and Wenig, M.: Personal air pollution exposure assessment using wearable sensors, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11085, https://doi.org/10.5194/egusphere-egu23-11085, 2023.

EGU23-11110 | ECS | Orals | AS3.15

Using air quality sensor networks to compare variations of PM2.5 in a small town and a city in Ireland. 

Rósín Byrne, John C Wenger, and Stig Hellebust

High density air quality sensor (AQS) networks offer a unique opportunity to better understand the local variations and temporal patterns of air pollutant levels in a city. With the coordination of reference instrumentation and meteorological data, they are even more useful. This work compares two sensor networks that are the first or their kind in Ireland. The first is in Cork City (population ~ 220,000) in the south of Ireland, which currently has five regulatory monitoring stations, three of which monitor PM2.5. The second location is Edenderry which is a rural town (population ~ 8,000) in the Irish midlands served by one regulatory monitoring site. The Cork City AQS network is comprised solely of PurpleAir devices, while the Edenderry network combines both PurpleAir and Clarity Movement Co. devices. The networks provide increased spatial and temporal data in relation to PM2.5.

Both locations experience seasonally elevated levels of PM2.5 due to higher instances of domestic solid fuel burning during the winter months. However, Edenderry generally experiences significantly higher levels, despite its much smaller size. During the winter heating period of 2020-2021 (01/10/20 - 31/0321), there were 23 instances where the PM2.5 24-hour mean at a regulatory monitoring site in Cork exceeded the WHO Global Air Quality Guidelines of 15 µg m-3, while there were 83 instances in Edenderry over the same period.

A correction model was applied to the AQS data collected in both networks to align the values with respective local reference data. Multiple linear regression (MLR) models were used to calibrate the networks using data from periods of colocation of the reference instrument with air quality sensors. By combining these robustly calibrated and co-ordinated networks with local meteorological information, the data was used to investigate the local spatial and temporal variations in PM2.5 for the period 01/02/2022 to 29/07/2022. The typical daily cycle of PM pollution in Ireland was observed in both locations, with a dominant afternoon/evening peak during the colder months due to solid fuel burning for home heating. Significant PM2.5 variations between sensor locations in each network were found. The results showed that a small town in Ireland can experience PM2.5 pollution levels that are as substantially higher than more populated urban areas.

This work was supported by the EU LIFE Programme through the project LIFE Emerald - LIFE19 GIE/IE/001101 and the Cork City AQS network is supported by Cork City Council.

How to cite: Byrne, R., Wenger, J. C., and Hellebust, S.: Using air quality sensor networks to compare variations of PM2.5 in a small town and a city in Ireland., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11110, https://doi.org/10.5194/egusphere-egu23-11110, 2023.

EGU23-11161 | ECS | Posters on site | AS3.15

Spatio-Temporal Prediction of PM1.0 Concentration in South Korea Using a Machine Learning Algorithm 

Hyemin Hwang, Jong Sung Park, Joon Young Ahn, Kwang Yul Lee, Jong Bum Kim, and Jae Young Lee

Since smaller particles can get through deeper into the human body, a model that predicts PM1.0 concentration temporally and spatially is important. Despite their importance, there are significantly fewer PM1.0 measurement stations than PM2.5 and PM10 in South Korea. Therefore, in this study, PM1.0 prediction models were constructed using a machine learning algorithm to predict the spatiotemporal concentration of PM1.0 in a place where the PM1.0 measurement was not available.

From January to December 2021, hourly data for the concentration of particulate matters(PM10 and PM2.5), the composition of PM2.5, the concentration of gaseous pollutants(SO2, O3, CO, NO, NOy, NH3), and weather conditions(wind direction, wind speed, temperature, relative humidity, press, precipitation, cloud) measured at three different Air Quality Measurement Systems were collected. PM1.0 concentrations were collected at two of these sites which are Seoul and Ansan(Gyeonggi-do), and no PM1.0 concentration was measured at the other site which is Seosan(Chungcheongnam-do). Since the three measurement stations were located close to each other and had similar sources and characteristics, the concentration of PM1.0 in Seosan was predicted by using a model trained based on Seoul and Ansan data.

Based on collected data, the importance of variables in the model was identified and variables that are important in predicting PM1.0 concentration were selected. Ensemble models (Random Forest, gradient boosting) and sequence models (RNN, LSTM, GRU) were compared to find a better model. Each model was evaluated by calculating the coefficient of determination and the proportion of impossible concentrations. Finally, based on the model with the best prediction result, the PM1.0 concentration was predicted at the target location (Ansan) where the PM1.0 concentration was unknown.

Our results showed that PM1.0 concentration can be predicted with high accuracy considering both the spatial distribution and temporal variability of the concentration. The results of this study can be used as data for selecting models in air quality prediction studies using machine learning. In addition, economical and efficient choices can be made in the construction of new monitoring stations in the future.

 

Acknowledgments

This study was supported by the National Research Foundation of Korea (grant number NRF-2021R1C1C1013350) and by a grant from the National Institute of Environmental Research (NIER), funded by the Ministry of Environment (ME) of the Republic of Korea (NIER-2022-04-02-087).

How to cite: Hwang, H., Park, J. S., Ahn, J. Y., Lee, K. Y., Kim, J. B., and Lee, J. Y.: Spatio-Temporal Prediction of PM1.0 Concentration in South Korea Using a Machine Learning Algorithm, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11161, https://doi.org/10.5194/egusphere-egu23-11161, 2023.

EGU23-11286 | Posters on site | AS3.15

Relationship between air pollution and synoptic scale weather in South Korea 

Jin-Ho Yoon, Dasom Lee, Hyun Cheol Kim, Jee-Hoon Jeong, Baek-Min Kim, and Shih-Yu (Simon) Wang

East Asia, including South Korea, has become a regional hot spot for the deteriorating air quality in recent years. During winter and spring, Particulate Matter (PM) is a dominant air pollutant. On the other hand, ozone becomes a major issue during summer season. In this talk, we’d like to show how synoptic scale weather pattern affects both PM and ozone in South Korea. Particularly, spatial synoptic classification (SSC) data are used to analyze characteristics of PM and ozone concentration according to synoptic weather patterns. During winter, dry moderate (DM) types occur frequently alongside high PM cases. The composite weather map showed a weak northwesterly wind field as a potential cause. On the contrary, it is interesting to note that dry polar (DP) types can be associated with low PM cases as well as high PM depending on near-surface wind speed. On the other hand, we found that DM, DT, and MT are commonly associated with high ozone; dry tropical (DT) produces ozone with the greatest efficiency, especially high levels of concentration. This finding implies a strong connection between surface ozone and climate change, because the occurrence of DT weather has increased by more three times over the past fifty years in South Korea.

How to cite: Yoon, J.-H., Lee, D., Kim, H. C., Jeong, J.-H., Kim, B.-M., and Wang, S.-Y. (.: Relationship between air pollution and synoptic scale weather in South Korea, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11286, https://doi.org/10.5194/egusphere-egu23-11286, 2023.

EGU23-11503 | ECS | Orals | AS3.15

Characterization and Evaluation of Long-term Air Quality Across Urban Hong Kong 

Shuwen Han, Yan Tan, and Shun-cheng Lee

Air pollution is a serious environmental issue and has attracted much attention owing to the rapid urbanization and industrialization worldwide. Hong Kong, one of the well-developed cities located in the southeast of the Pearl River Delta (PRD) region, struggling with frequent air pollution episodes because of the intensive land use, dense daily anthropogenic activities, and enormous vehicle emissions. Therefore, a 10-year evaluation of air pollutants across roadside, urban and background sites was conducted to analyze the variations of air quality and contamination in Hong Kong. The continuous decrease of annual averaged concentrations of traffic-related NO2, SO2, CO, PM2.5 and PM10 and numbers of days with severe pollution conditions validated the efficiency of the series of air pollution control schemes implemented by the Hong Kong government. However, the concentration of O3 at roadside and urban stations increased by 135% ± 25% and 37% ± 18% from 2011 to 2020, respectively, meanwhile the highest 8-hour averaged O3 concentration was observed as 294 μg/m3 at background station in 2020, which pointed out the worsening ozone pollution in Hong Kong. To further investigate typical precursors of ozone and secondary organic aerosols, the intensive measurements of VOCs and OVOCs were conducted at both urban roadside station with heavy traffic and coastal station in suburban area to study the chemical compositions and emission patterns of ambient VOCs and OVOCs thoroughly. Results from those two campaigns showed significant differences across Hong Kong. Acetone, formaldehyde, and acetaldehyde were the most abundant species at roadside environment, while formaldehyde, methanol and acetone were the major species in suburban atmosphere. The major contributors to ozone formation were formaldehyde (89.64 μg/m3) at roadside and isoprene (13.46 μg/m3) at suburban among the measured VOCs in Hong Kong. In addition, the source apportionment results from positive matrix factorization (PMF) analysis showed that the sampling site at the southeastern tip of Hong Kong was strongly influenced by urban plumes from the PRD region and by oceanic emissions as well.

How to cite: Han, S., Tan, Y., and Lee, S.: Characterization and Evaluation of Long-term Air Quality Across Urban Hong Kong, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11503, https://doi.org/10.5194/egusphere-egu23-11503, 2023.

EGU23-11781 | Orals | AS3.15

Comparison of emission factors of particles from shipping using different equipment 

Daniëlle van Dinther, Andreas Weigelt, Jörg Beecken, Johan Mellqvist, Vladimir Conde Jacobo, Marcus Blom, and Jan Duyzer

Air quality in urban cities with ports can significantly be impacted by shipping. For example Visschedijk and Denier van der Gon (2022) showed that, within Rotterdam area (the Netherlands), sea shipping is the main source of ultra-fine particles (UFP) with a contribution of 56% to total UFP emissions. Within EU-project SCIPPER (Shipping Contributions to Inland Pollution Push for the Enforcement of Regulations) a measurement campaign of six weeks was undertaken at the river Elbe near Hamburg (Germany). Sea going vessels pass by on the way to or from the port of Hamburg, which is located about 10 km upstream of the measurement site. Three different groups measured side-by side different gaseous compounds and aerosols on-shore. The aerosol measurements consisted of different equipment measuring different sizes ranging from 6 to 10 000 nm, also black carbon was measured by two groups. The emission factors (EF) of the different ships were calculated in #/kg fuel as well as mg/kg fuel from these measurements. This provides a unique dataset to better understand the emission characteristics of different ships as well as the comparability of different devices. This comparability is important if in the future legislation to decrease aerosol emissions of shipping is applied and needs to be verified. Results showed the relatively large contribution of mainly ultrafine particles, with 90% of the total amount of particles being smaller 80 nm and 75% of the total particle mass comes from particles smaller 200 nm. The comparison showed very promising results when the same equipment was tested side-by-side (R2 above 0.85 for all size ranges). The comparability of EFs of same sources that were measured by different devices was somewhat lower, but especially for smaller size ranges still promising (R2 of 0.69 for particle number ranging from 90 to 300 nm). For black carbon the experimental set-up proved to be too different (drying vs non-drying and different inlet cut-offs) to give comparable emission factors. Concluding the data showed promising results to be able to use on-shore monitoring in the future to monitor aerosol ship emissions, also when using different equipment.

References:

Visschedijk, A., Denier van der Gon, H. (2022). UFP emissie in de Rijnmond regio in 2019 (in Dutch). Utrecht: TNO-report R10616.

How to cite: van Dinther, D., Weigelt, A., Beecken, J., Mellqvist, J., Conde Jacobo, V., Blom, M., and Duyzer, J.: Comparison of emission factors of particles from shipping using different equipment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11781, https://doi.org/10.5194/egusphere-egu23-11781, 2023.

EGU23-11897 | ECS | Posters on site | AS3.15

Atmospheric concentrations of carbon dioxide and its isotopic composition in Krakow (Southern Poland) based on one-year CoCO2 measurement campaign 

Alicja Skiba, Mirosław Zimnoch, Zbigniew Gorczyca, Mikita Maslouski, and Michał Marzec

Regular, monthly based, diurnal measurements of atmospheric carbon dioxide concentration and its carbon isotope composition (13C/12C and 14C/12C ratios) were performed between 9 February 2021 and 1st February 2022 in Krakow, the second biggest city of Poland, populated by around 780,000 inhabitants. Spot air samples were collected in 3 l glass flasks every 4 hours from the roof of the building (50°04’ N 19°55’ E 220 AMSL, ∼ 20 m above the surface) during each measurement campaign. A total of 72 air samples were collected during 12 measurement campaigns. The samples were analyzed with Picarro G2101i (Picarro Inc., Santa Clara, California, USA) to determine the carbon dioxide. After that, the samples were analyzed with Isotope-Ratio Mass Spectrometry (IRMS) and Accelerator Mass Spectrometry (AMS) in order to determine δ13C and Δ14C composition. The carbon dioxide concentration during the campaign ranged from 404 ppm (7 September 2021) to 617 ppm (1 February 2022) with the one-year average of 463 ppm. δ13C ranged from -14.79 ‰ (1st February 2022) to -8.5 ‰ (7th September 2021). The one-year average results of Δ14C were -35 ‰.

Furthermore, measurement of gas concentration and its isotopic composition, along with the use of the isotope-mass balance, allowed determination of fossil fuel-related and biogenic contributions to the total measured CO2 load during campaign days, allowing to characterise the diurnal and seasonal variability of those components in the urban environment. Based on the obtained results, a dataset dedicated for the validation of WRF-CHEM high-resolution simulations of the city atmosphere has been prepared.

 

ACKNOWLEDGEMENTS

The presented work was funded by the CoC02 project, which has received funding from the European Union's Horizon 2020 research and innovation programme under Grant Agreement No. 958927 and the "Excellence Initiative - Research University" program at AGH University of Science and Technology.

How to cite: Skiba, A., Zimnoch, M., Gorczyca, Z., Maslouski, M., and Marzec, M.: Atmospheric concentrations of carbon dioxide and its isotopic composition in Krakow (Southern Poland) based on one-year CoCO2 measurement campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11897, https://doi.org/10.5194/egusphere-egu23-11897, 2023.

EGU23-11991 | ECS | Posters on site | AS3.15 | Highlight

Evaluation of air quality sensors for environmental epidemiology 

Miriam Chacón-Mateos, Ulrich Vogt, Bernd Laquai, Héctor García-Salamero, Christian Witt, Uta Liebers, and Frank Heimann

The increase in evidence on the adverse health effects of air pollution has been possible thanks to the advances in technology for air pollution monitoring and personal exposure. In this context, air quality sensors present a huge potential for enhancing long-term personal exposure prediction. In order to prove the potential of air sensors for health research, a pilot study with patients suffering from chronic obstructive pulmonary diseases or Asthma was carried out in Stuttgart (Germany) in cooperation with the University Hospital Charité in Berlin, and an outpatient pulmonary practice in Stuttgart.

Prior to the pilot study, we first tested several sensor models for PM and NO2 in the laboratory as well as in the field. The sensors with the best performance were selected to build two different sensor boxes for indoor and outdoor measurements. Temperature and relative humidity sensors were also included in the boxes. To avoid the overestimation of the PM readings due to hygroscopic growth, a low-cost dryer was designed and evaluated for the PM sensor of the outdoor boxes (Chacón-Mateos et al. 2022).

The measurements inside and outside the houses were carried out over 30 days. Passive sampling of NO2 was done additionally for quality assurance of the NO2 measurements. Participants completed spirometry, a questionnaire assessing respiratory symptoms, and a protocol of activities on a daily basis. The calibration and validation of the sensors were conducted two weeks before the start of the measurements. To perform the quality assurance, the sensor boxes for indoors were collocated in the laboratory, and the sensor boxes for outdoors in the field, together with reference-grade instruments. The PM2.5 concentrations were corrected using univariate linear regression whereas multilinear regression and machine learning algorithms were tested and applied to correct the raw data of the NO2 sensors.

The sensor validations have shown that measuring low concentrations of PM2.5 and NO2 has higher expanded uncertainty, but high concentrations can be measured with expanded uncertainties that fulfill the Data Quality Objectives (DQO) set by the Air Quality Directives for indicative measurements. However, we also found a high unit-to-unit variability which means that model coefficients cannot be transferred from one sensor to another. We also recommend collocating NO2 passive samples close to the sensor boxes to determine whether or not the sensor is measuring within the expected range as the signal of some NO2 sensors drifted unexpectedly during the measurements in the houses of the patients.

In conclusion, air sensors are not yet to be recommended to quantify the effects of low-level air pollution but they are a promising tool to increase the ubiquity of epidemiological studies for low- and middle-income countries where high air pollution is expected. Moreover, it is important to consider that in order to get actionable data with air sensors, a significant amount of time in sensor calibration should be invested.

References:

Chacón-Mateos, M., Laquai, B., Vogt, U., and Stubenrauch, C.: Evaluation of a low-cost dryer for a low-cost optical particle counter, Atmos. Meas. Tech., 15, 7395–7410, https://doi.org/10.5194/amt-15-7395-2022, 2022

How to cite: Chacón-Mateos, M., Vogt, U., Laquai, B., García-Salamero, H., Witt, C., Liebers, U., and Heimann, F.: Evaluation of air quality sensors for environmental epidemiology, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11991, https://doi.org/10.5194/egusphere-egu23-11991, 2023.

EGU23-12300 | Posters on site | AS3.15

Air Pollution knowledge Assessments (APnA) City Program in Asia and Africa 

Sarath Guttikunda, Puja Jawahar, and Sai Krishna Dammalapati

Representative emissions and pollution data is a critical requirement for supporting clean air action plans for cities. The data can be used for both long-term policy assessments and short-term pollution alert systems via modeling at various scales. In a data sparse environment, several assumptions are made, and several data resources are accessed to construct a reliable emissions and pollution modeling framework to support public and policy dialogue. These assumptions include interpolation of observations from one zone to another, extrapolation of operational conditions from one country to another, and utilization all available source and emissions data, complemented with open satellite retrievals and global databases with information on population, topography, land use, urbanization level, road network, locations of commercial and other points of interest, to compile a city’s spatially and temporally representative dynamic emissions map. The urban airshed inventory is maintained at a spatial resolution of 0.01 degrees (~1km) and with monthly and hourly temporal modulation suitable for chemical transport modeling. Here, we will present examples from the Air Pollution knowledge Assessments (APnA) program implemented for 60 Indian cities and expansion of the program to Balkan, Central Asian, and African cities, while addressing data gaps using emerging technology and big data feeds, combined with traditional meteorological and chemical transport modeling (WRF-CAMx) systems. Where available validation of the model results against available monitoring data from reference-grade and sensor networks is also included in the study. All the methodologies and data resources are accessible @ https://www.urbanemissions.info

How to cite: Guttikunda, S., Jawahar, P., and Dammalapati, S. K.: Air Pollution knowledge Assessments (APnA) City Program in Asia and Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12300, https://doi.org/10.5194/egusphere-egu23-12300, 2023.

EGU23-12404 | ECS | Posters on site | AS3.15

Variations in particulate matter chemical composition in the urban coastal city of India 

Shruti Tripathi, Abhishek Chakraborty, and Debayan Mandal

Particulate matter (PM) is collected in the urban coastal city of Mumbai. The PM2.5 concentrations averaged from 200 μg m−3 to 90 μg m−3 throughout the year during sampling. These values were substantially higher than national ambient air quality standards (60 μg m−3). The Organic carbon (OC) concentration in PM ranged from 6 μg m−3 to 17 μg m−3 from summer to winter, whereas elemental carbon (EC) has varied from 1.2 μg m−3 to 4.8 μg m−3. The OC/EC ratio was lower in winter than summer because of high EC emissions during winter and low photochemical activities. The summer samples have a high percentage of low volatile OC fraction (53%) than the winter samples. The calculated secondary organic carbon (SOC) also varies seasonally. The fraction of SOC in overall OC was highest in summer (65.7%), whereas the concentration of SOC was higher in winter, i.e., 9 μg m−3. High temperatures and strong solar radiation favor SOC formation during the summer, resulting in a high percentage of low volatile OC in total OC. The overall chemical composition of PM2.5 reveals that almost 68% of the total mass was elemental composition (SO42−, NO3, NH4+, Na+, Ca2+and K+) in winter and 16% in summer. Seasalt contribution to PM2.5 was 32% and 5% in winter and summer, respectively. Chlorine to sodium molar ratios was below the seawater ratio line in both seasons (0.69 winters and 0.30 summers), but the drop in the summer season might indicate more loss of chlorine. In summer, aerosols are slightly less acidic than in winter and pH value ranged from 3.2 to 7.1. Therefore, we can say that Mumbai suffers from air pollution problems during the winter, despite being a coastal city. These high concentrations of PM have an adverse effect on the health of the urban population.

How to cite: Tripathi, S., Chakraborty, A., and Mandal, D.: Variations in particulate matter chemical composition in the urban coastal city of India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12404, https://doi.org/10.5194/egusphere-egu23-12404, 2023.

This work used a Mass-Conserving inversion estimate framework based on daily TROPOMI NO2 and CO columns and observed stack fluxes of large industrial and commercial combustion sources from the continuous emissions monitoring systems (CEMS) to quantify three years of daily-scale, grid-by-grid emissions of NOx and CO at 0.05°×0.05° over Shanxi Province. This region was selected due to its complex topography, rapid development, and the fact that it currently contributes to more than 25% of China’s total coal production and consumption. For these reasons, the region is also highly representative in terms of rapid changes in the spatial-temporal distribution of emissions found in many different regions of the Global South. The calculated emissions, their ratio, and the day-to-day emissions variability are calculated and explained over four different land-use types: rural, natural, urban, and industrial. It is observed that relatively high NOx emissions, high NOx/CO and high NOx/NO2 ratios are consistent with known industrial areas; relatively lower NOx emissions, high NOx/CO and low NOx/NO2 ratio are consistent with known urban aeras. While the time series of both NOx and CO emissions are found to decrease from 2019-2021 overall, there are some complicated inter- and intra-year variations in the emissions, and such trends are not statistically significant over specific sub-regions. The observed variations include both known and unknown special events, as results of intentional policy changes, properties of the climate, and long-range transport atmospheric events. Combined with the Empirical Orthogonal Functions Principal Components Analysis (EOF), the joint composition of PM2.5, NO2, and CO emission in the largest city in Shanxi show further insights. Special festivals and economic events including Chinese New Year are clearly observed. There is also a significant decrease in the NOx to CO emissions ratio observed in urban and rural areas during the COVID-19 induced lockdowns in 2020, but an obvious increase after first-order lockdown. Specifically, it is observed that while there was a drop from 2019 to 2020 due to the COVID lockdowns, that the lowest emissions levels observed actually were found in 2021. On top of this, there was an observed see-saw effect with further reduction of pollution from large enterprises and poorer control of small sources and residential combustion sources. Finally, a switch in the NOx to CO emissions ratio is observed to rapidly change for strict control measures were introduced during the 2022 Winter Olympics. Diagnosis of pollution events using emissions of NOx and CO integrated with detailed PM2.5 chemical components is successfully attempted for the first time.

How to cite: Li, X., Cohen, J. B., Qin, K., and Geng, H.: Diagnosis of pollution events by NOx and CO Emissions calculated by Mass-Conserving Inversion method and composition of PM2.5 in Big City of Energy Rich Northern China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12644, https://doi.org/10.5194/egusphere-egu23-12644, 2023.

EGU23-12661 | ECS | Orals | AS3.15

Comparison between Eulerian and Lagrangian models for simulating atmospheric conditions in urban environments 

David Jean du Preez, Christoph Knote, and Maximilian May

Populations in urban areas have continued increasing in developing and developed countries worldwide. The ability to accurately simulate the dynamical and chemical atmospheric conditions in urban areas is essential when investigating the health impacts related to environmental conditions in urban areas. To simulate atmospheric conditions in urban areas one must consider how the airflow is affected by urban structures, vegetation, and mesoscale meteorology as well as local emitters and non-linear chemical reactions. 

There are a variety of different models available to simulate atmospheric conditions in urban areas. These models differ in many ways such as numerical methods, spatial and temporal resolution, and initial and lateral boundary conditions. Here we compare an Eulerian (PALM) and a Lagrangian (GRAL) model to determine which model can best simulate atmospheric conditions in an urban environment. These numerical differences affect the computational resources required and therefore influence how each model can be used to study the urban environment. The initial and lateral boundary conditions used in the simulations are derived from the Weather Research and Forecasting (WRF) model coupled with Chemistry (WRF-Chem) and a library of horizontal wind fields for PALM and GRAL, respectively. The results from both models will be compared for a domain over Heidelberg, Germany over a two-week period against hourly surface observations of wind and air quality parameters. 

How to cite: du Preez, D. J., Knote, C., and May, M.: Comparison between Eulerian and Lagrangian models for simulating atmospheric conditions in urban environments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12661, https://doi.org/10.5194/egusphere-egu23-12661, 2023.

EGU23-12910 | ECS | Posters virtual | AS3.15

Suitability of Particulate matter low-cost sensor data for land-use-based modeling 

Janani Venkatraman Jagatha, Tobias Sauter, and Christoph Schneider

Urban climate research is primarily based on point or location-based measurements of climate and air quality data. Advances in microsensor technologies and low cost due to production facilities, sensors for measuring air quality have spread to a large scale in the last decade. In contrast to reference devices, sensors are simple in design, lightweight, and easier to deploy in larger scales.

United Nations environment programme regards Air pollution to be a major global health concern that causes one in nine deaths worldwide. Although a number of sources and factors have been identified as a cause of air pollution it is difficult to pinpoint a particular source and manage it due to the variability of the pollutants in space, time, and the socio-economic factors involved.

This study aims to answer two questions: the possibility to use mobile measurement systems to identify the major sources that contribute to higher aerosol concentration in time and space and if low-cost particulate matter sensors are suitable for land-use-based modeling using conventional regression analysis and machine learning methods such as random forest and neural networks.

The data used was collected using the OPC-N2 sensor from Alphasense Ltd., as a part of the measurement campaign of the project Urban Climate under Change, Phase 1 and 2 [2016-2023].

How to cite: Venkatraman Jagatha, J., Sauter, T., and Schneider, C.: Suitability of Particulate matter low-cost sensor data for land-use-based modeling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12910, https://doi.org/10.5194/egusphere-egu23-12910, 2023.

EGU23-13016 | Orals | AS3.15

Evaluating climate mitigation and air quality synergies and trade-offs throughout the Covenant of Mayors initiative 

Fabio Monforti-Ferrario, Luana Valentini, Enrico Pisoni, and Marta Giulia Baldi

Tackling Climate Change is a priority for the European Union, who has set targets for reducing greenhouse gas emissions progressively up to 2050. In 2008, acknowledging the role of local authorities, the European Commission (EC) launched the Covenant of Mayors (CoM) initiative to endorse their efforts in the implementation of sustainable energy and climate policies. The JRC plays a central role in the CoM ecosystem, providing the methodological guidelines that enable cities to process their own GHG emission data. Furthermore, the JRC provides scientific supervision and makes comprehensive GHG datasets available to the whole CoM community (Baldi et al., 2022).

Since 2018, in the frame of its support to the EU Covenant of Mayor (CoM) initiative, the JRC is bringing to the attention of the city administrators the importance of tuning climate change mitigation and air quality. For this goal, in cooperation with the CoM stakeholders we have developed a specific tool aimed at allowing the CoM signatories to evaluate the consequences of their mitigation policies on the air pollutants emissions taking place in their territory.

 

The tool was developed in two steps: (1) in the first part of the research project, a pilot version of the tool has been developed based on the methodology reported in two previous studies, Monforti-Ferrario et al. (2018) and Peduzzi et al. (2020); (2) after setting up the tool, the pilot tool has been made available to a group of of CoM signatories. Their comments and feedbacks  have been through a questionnaire and showed how the tool i especially useful for small and middle-sized signatories.

As reported in Peduzzi et al. (2020) the tool is based on the comparison between the Baseline Emission Inventory (BEI) and the successive Monitoring Emission Inventories (MEI) the signatories need to submit to comply with CoM requirements.The changes in energy consumption (by sector and carrier) between BEI and MEI were translated into the corresponding changes in air pollutant emissions by means of estimated emission factors.

 

Updated data on the actual use of the tool and feedback from users and practitioners will be provided and discussed. We will complete the presentation with reflections and suggestions for local authorities to practically improve the co-designing of climate and air pollution policies based on the experience collected throughout the CoM initiative.

 

 

References

Baldi et al., (2022): GCoM - MyCovenant, 2021, Second release. European Commission, Joint Research Centre (JRC) [Dataset] PID: http://data.europa.eu/89h/9cefa6ca-1391-4bcb-a9c8-46e029cf99bb

Monforti-Ferrario et al, 2018, The impact on air quality of energy saving measures in the major cities signatories of the Covenant of Mayors initiative. Environmental International, 118, 222-234

Peduzzi  et al, 2020, Impacts of a climate change initiative on air pollutant emissions: Insights from the Covenant of Mayors, Environment International, Volume 145,  106029

How to cite: Monforti-Ferrario, F., Valentini, L., Pisoni, E., and Baldi, M. G.: Evaluating climate mitigation and air quality synergies and trade-offs throughout the Covenant of Mayors initiative, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13016, https://doi.org/10.5194/egusphere-egu23-13016, 2023.

EGU23-13131 | Orals | AS3.15

Using Mobile Monitoring to Understand Vehicle Emissions in Urban Areas 

Shona Wilde, Naomi Farren, Rebecca Wagner, James Lee, Samuel Wilson, Lauren Padilla, Greg Slater, Daniel Peters, Ramon Alvarez, and David Carslaw

Tailpipe emissions from road transport have fallen dramatically over the last 30 years due to the combined
effect of increasingly stringent regulations and technological improvements. However, the air pollution
burden due to road vehicle emissions remains the dominant source of many air pollutants in urban
areas. Policies such as Low Emission Zones (LEZs) have become increasingly popular as a method of reducing
on-road emissions by restricting access to the oldest and most polluting vehicles. Most modern vehicles
are fitted with sophisticated exhaust aftertreatment systems, which should lead to significantly reduced
emissions of pollutants such as nitrogen oxides (NOx = NO + NO2). However, the performance of such
systems is non-uniform across all driving conditions. Urban driving conditions are among the most challenging,
where vehicle speeds are often low and congestion results in a considerable amount of stop-start
driving with repeated accelerations and decelerations. Under such conditions some aftertreatment systems
cannot reach the high temperatures required to operate efficiently, which may limit the effectiveness of
policies that target vehicle type alone. Therefore, to develop effective air quality management strategies it
is necessary to understand the relative importance of factors that influence vehicle emissions, such as fleet
composition, traffic state, driver behaviour and ambient temperature.
In this work we present results from a mobile monitoring campaign in London, UK. Measurements were
made in two unique locations (central and outer London) in order to provide a quantitative understanding
of the main drivers for concentrations in terms of traffic conditions. We show that there is a significant low
speed penalty for NOx concentrations in central London, where there is a high proportion of diesel vehicles,
which are predominately taxis and buses. This effect arises due to the near constant congestion and
slow average moving speed of only 12 km h-1, resulting in the non-optimal performance of aftertreatment
technologies fitted to diesel vehicles. Moreover, despite the heavy restrictions imposed by the Ultra Low
Emissions Zone, which requires all diesel vehicles in the zone to be Euro 6/VI (light/heavy vehicles) compliant,
we find that the mean emissions intensity (ΔNOx/ΔCO2) in central London was 0.0039 ppb ppb-1, a
factor of 2 higher than outer London (0.0021 ppb ppb-1). For context we compared the measured emissions
intensity to an “urban average" value (0.0018 ppb ppb-1) derived from 135,000 remote sensing measurements
made directly at the tailpipe. Whilst good agreement was found for outer London, central London
was twice as high, suggesting there is a highly unfavourable mix of technology and conditions, which may
hinder the improvements due to current policies. This work aims to quantify the unique effect of congestion
on different vehicle types and to provide policy makers with the information needed to better understand
the benefits of congestion control, given that restrictions on technology alone may not always be enough to
reduce emissions.

How to cite: Wilde, S., Farren, N., Wagner, R., Lee, J., Wilson, S., Padilla, L., Slater, G., Peters, D., Alvarez, R., and Carslaw, D.: Using Mobile Monitoring to Understand Vehicle Emissions in Urban Areas, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13131, https://doi.org/10.5194/egusphere-egu23-13131, 2023.

EGU23-13203 | ECS | Orals | AS3.15

A portable, ground-based FTS for reflected sunlight: Performance evaluation for mapping CO2 and CH4 above Los Angeles 

Benedikt Hemmer, Vincent Enders, Frank Hase, Ralph Kleinschek, Julian Kostinek, Thomas Pongetti, Stanley Sander, Zhao-Cheng Zeng, and André Butz

Precise knowledge of sources and sinks in the carbon cycle is desired to understand its sensitivity to climate change and to account and verify man-made emissions. In this context, extended sources like urban areas play an important role. While in-situ measurements of carbon dioxide (CO2) and methane (CH4) are highly accurate but localized, satellites measure column-integrated concentrations over an extended footprint. The CLARS-FTS [1, 2] stationed at the Mt. Wilson observatory looking downward into the Los Angeles basin has pioneered an innovative measurement technique that fills the sensitivity gap between in-situ and satellite measurements. The technique enables mapping the urban greenhouse gas concentration fields by collecting spectra of ground scattered sunlight and scanning through the region.

We develop a similar but portable instrument using a CLARS-FTS-like measurement geometry. It is based on the EM27/SUN FTS with a modified pointing system, increased throughput and a more sensitive detector than the standard type. The compact setup enables campaign-based observations in various source regions of interest, utilizing the increased sensitivity to boundary layer concentration by the horizontal light path component.

Here, we present the portable instrument setup and its performance. Throughout April 2022, we observed the Los Angeles basin with both the portable setup and the CLARS-FTS simultaneously. The retrieval algorithm is based on the RemoTeC software, previously employed for solar backscatter satellite measurements. From this, we evaluate the XCO2 and XCH4 precision of our setup under field conditions, and compare our instrument to the concurrent CLARS-FTS measurements.

 

References:
[1] Fu, D. et al., 2014: Near-infrared remote sensing of Los Angeles trace gas distributions from a mountaintop site, Atmos. Meas. Tech., 7, 713–729, https://doi.org/10.5194/amt-7-713-2014
[2] Wong, K. W. et al., 2015: Mapping CH4 : CO2 ratios in Los Angeles with CLARS-FTS from Mount Wilson, California, Atmos. Chem. Phys., 15, 241–252, https://doi.org/10.5194/acp-15-241-2015

How to cite: Hemmer, B., Enders, V., Hase, F., Kleinschek, R., Kostinek, J., Pongetti, T., Sander, S., Zeng, Z.-C., and Butz, A.: A portable, ground-based FTS for reflected sunlight: Performance evaluation for mapping CO2 and CH4 above Los Angeles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13203, https://doi.org/10.5194/egusphere-egu23-13203, 2023.

EGU23-13255 | ECS | Orals | AS3.15

Tall tower measurements with laser isotope spectrometry to investigate urban CO2 emissions in Vienna 

Kathiravan Meeran, Bradley Matthews, Simon Leitner, Hans Sanden, Jia Chen, and Andrea Watzinger

Cities contribute significantly to global carbon dioxide (CO2) emissions, and it is important to understand and accurately measure these emissions in order to effectively mitigate climate change. Current methods for estimating emissions, such as emission inventories, can be very uncertain at the scale of individual cities. Measurement methods that involve analyzing local atmospheric CO2 levels and the respective stable carbon isotopic composition of CO2 can provide additional, independent information on local emissions, particularly in terms of source contributions from combustion of different fossil fuels and natural respiration. As part of the Vienna Urban Carbon Laboratory (VUCL), a cavity-ring-down laser isotope spectrometer (G2201-i, Picarro Inc., USA) has been operating on a radio tower in Vienna’s city centre since May 2022 to measure atmospheric mixing ratios of CO2 and stable carbon isotopic composition of CO213C) 144 m above the surface.

The overall objective here is to establish an analysis framework to best utilize these measurements in combination with tall-tower eddy covariance measurements for the identification and quantification of local CO2 emission emitters in Vienna. Initial analysis of the half-hourly CO2 concentrations and fluxes between May and Dec 2022 show that a night-time increase of measured CO2 concentrations are followed by an early morning peak, due to a nocturnal build-up of surface-level CO2 that is followed by an upward flush of CO2 in the morning. The δ13C of CO2 (based on keeling plot analysis) suggests that fluxes from natural respiration are dominant over the night. In the afternoon, the δ13C of CO2 sources decreases, which may be due to an increased contribution from sources with isotopically depleted CO2, such as traffic emissions and small-scale stationary methane combustion. We also observed higher concentrations CO2 that are isotopically depleted, during the summer when winds came from the area southeast of the tower, which has more industrial and refinery activity. In addition to these initial results from keeling plot analysis, our presentation will also include results from the ongoing winter measurements, where we expect to see indications of enhanced methane combustion for space heating. Furthermore, results from ongoing tests of other analysis methods for identifying emitting sources (e.g., application of the miller trans model method, analysis of the data at higher temporal resolutions) will be presented.

How to cite: Meeran, K., Matthews, B., Leitner, S., Sanden, H., Chen, J., and Watzinger, A.: Tall tower measurements with laser isotope spectrometry to investigate urban CO2 emissions in Vienna, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13255, https://doi.org/10.5194/egusphere-egu23-13255, 2023.

EGU23-13290 | Posters on site | AS3.15

Air pollution in Rotterdam: urban vs. port contributions and the role of neighborhood design 

Juliane Fry, Pascale Ooms, Roel Vermeulen, and Jules Kerckhoffs

The Ruisdael Rotterdam campaign in August - September, 2021 featured a comprehensive suite of air pollutant, greenhouse gas, and meteorological data collection across the city and port of Rotterdam, Netherlands. We will present data from the Utrecht University Air Quality car mobile platform, which was deployed for >80 hours of sampling across the region, measuring particulate matter (PM1, PM2.5 and PM10), ultrafine particulate matter count (UFP), black carbon (BC), carbon dioxide (CO2), and nitrogen dioxide (NO2). We analyze this data with particular focus on the relative contribution of urban and port emissions to air pollution levels across the city, and on the role of neighborhood design in determining street-level concentrations of pollutants.

How to cite: Fry, J., Ooms, P., Vermeulen, R., and Kerckhoffs, J.: Air pollution in Rotterdam: urban vs. port contributions and the role of neighborhood design, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13290, https://doi.org/10.5194/egusphere-egu23-13290, 2023.

EGU23-14015 | Orals | AS3.15 | Highlight

A single instrument for simultaneous monitoring of greenhouse gases and air pollutants 

Marco Brunner, Morten Hundt, and Oleg Aseev

Urban air pollution and greenhouse gas emissions are two closely linked problems. They can be attributed to a variety of sources, such as transportation and buildings, waste management and agricultural production, natural events such as forest fires and many others. Monitoring air pollutants and GHG simultaneously with high selectivity and sensitivity enables to detect and evaluate their sources and sinks and to discover the links between them. Precise measurements at various spatial and temporal scales are required for modelling and validation of emission inventories or satellite observations. 

Solutions to monitor air pollutants or GHG with high precision and temporal resolution were commonly offered as “one-species-one-instrument”, leading to large, immobile measurement setups with high energy consumption. We provide a new compact laser absorption spectrometer that combines several mid-IR lasers. Our solution allows simultaneous high-precision measurements of the greenhouse gases CO2, N2O, H2O and CH4, and the pollutants CO, NO, NO2, O3, SO2 and NH3 within a single instrument and is therefore well suited to detect the relations of the co-emitted pollutants and GHGs.

In our contribution, we will demonstrate examples of our instruments’ applications for mobile monitoring of 10 GHGs and air pollutants in urban areas and airborne measurements with airships. Furthermore, we will present the results of parallel monitoring with our instrument and standard conventional gas analysers used for GHG and air pollutant measurements. It demonstrates the ability of our instrument to serve as an all-in-one solution and to replace up to 7 standard gas analysers opening a wide range of new mobile multi-compound gas monitoring applications, for example, in (small) airplanes or cars.

How to cite: Brunner, M., Hundt, M., and Aseev, O.: A single instrument for simultaneous monitoring of greenhouse gases and air pollutants, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14015, https://doi.org/10.5194/egusphere-egu23-14015, 2023.

EGU23-14039 | Posters on site | AS3.15

High-resolution simulation of CO2 dispersion in urban atmosphere of Krakow, Southern Poland 

Miroslaw Zimnoch, Michał Gałkowski, Piotr Sekula, and Lukasz Chmura

Effective mitigation efforts in the face of observed climate change require independent tools based on atmospheric observations to estimate greenhouse gas emissions at different spatial and temporal scales. Atmospheric transport models constitute a key element of anthropogenic emissions monitoring and verification systems. It represents atmospheric transport in such systems, which allows the use of inverse methodology to estimate emissions from observed concentrations. Reliable numerical simulations of atmospheric transport over complex urban areas require model configurations that provide adequate resolution reflecting the complex topography and land cover, as well as parameterization of physical processes optimised for the specifics of urban areas. This study presents an attempt to apply the WRF-CHEM model for the simulation of CO2 transport in the urban area of Krakow, the second largest city located in the southern part of Poland. The simulation has been performed for a 3 day period in October 2021 and was validated by a CO2 molar fraction vertical measurements performed on board of a tethered balloon operating as a commercial touristic attraction in the city centre. The modelling results have been compared with the observations to determine model performance in terms of: (i) capture the temporal dynamics of the nocturnal boundary layer formation and (ii) identifying detected CO2 plume originating from a point source to confirm the expected source position and estimate the CO2 emission from that source.

The presented work was funded by the CoCO2 project, which has received funding from the European Union's Horizon 2020 research and innovation program under Grant Agreement No. 958927 and the "Excellence Initiative - Research University" program at AGH University of Science and Technology.

How to cite: Zimnoch, M., Gałkowski, M., Sekula, P., and Chmura, L.: High-resolution simulation of CO2 dispersion in urban atmosphere of Krakow, Southern Poland, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14039, https://doi.org/10.5194/egusphere-egu23-14039, 2023.

EGU23-14432 | ECS | Posters on site | AS3.15

Air quality simulations of PM10 and NO2 for Zagreb using ADMS-Urban dispersion modeling system 

Darijo Brzoja, Velimir Milić, Vesna Gugec, Valentina Jagić, and Stipica Šarčević

This study aims to improve the knowledge of air quality in Zagreb, the capital of Croatia. It gives insight into the spatial distribution of concentrations of the main city pollutants (fraction of particulate matter < 10 µm and nitrogen dioxide) within the process of developing an air quality modeling system in high resolution. The work is a part of an ongoing AIRQ project (AIRQ - Expansion and Modernisation of the National Network for Continuous Air Quality Monitoring) funded by the European Regional Development Fund and Environmental Protection and Energy Efficiency Fund (FZOEU).

Air pollution is perceived as the second biggest environmental concern for Europeans, next to climate change, as quoted by European Commission in 2017., and it is the most important environmental risk to human health. Over the last three decades, policies to reduce air pollution have led to improved air quality, nevertheless, in some European cities, air pollution still poses risks to health. Zagreb is, unfortunately, one of them. Based on the levels of fine particulate matter measured in the air in 2019. and 2020., among 323 European cities, Zagreb is ranked 256th, and air quality in the city is categorized as „poor“ (EEA, 2022.).

In cities, pollutant concentrations have strong gradients, in particular those related to traffic. Since continuous air quality measurements are usually representative of several square kilometers for urban background locations or representative of a specific street, authorities are encouraged to use dispersion models to complement the observations for a city.

In this study, the ADMS-Urban model was set up for the Zagreb agglomeration. Within the model, measurement data from the Desinic site were used as background data representing the contribution of long-range transport to the city. Gridded emissions (500 m by 500 m resolution) were obtained from the Croatian National Emission Inventory (source: Ministry of Economy and Sustainable Development). Since emission sectors with low emission heights, such as traffic and household emissions, generally make larger contributions to surface concentrations and health impacts in urban areas than emissions from high stacks, special attention was given to road emissions, their spatial distribution, and time profiles taking into consideration the limitation of available data.  Thus, road emissions and two large point sources were modeled explicitly. The meteorology data used within the model were from the Maksimir measurement site and are representative of the whole modeling domain.

                The focus of the analysis was the main pollutants usually found to exceed EU limit values within the city and the surrounding area PM10 and NO2. The model's performance is assessed against measurements from 14 urban, urban-background, and near-traffic sites using a range of metrics concerning annual averages, high hourly average concentrations, and diurnal cycles. The model shows good performance compared to measurements for PM10, although it underestimates concentration values during high-pollution winter episodes. First NO2 results show characteristic high concentrations at the traffic hot spots and next to the main roads.

How to cite: Brzoja, D., Milić, V., Gugec, V., Jagić, V., and Šarčević, S.: Air quality simulations of PM10 and NO2 for Zagreb using ADMS-Urban dispersion modeling system, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14432, https://doi.org/10.5194/egusphere-egu23-14432, 2023.

EGU23-14901 | ECS | Orals | AS3.15 | Highlight

Transport and emissions of gaseous air pollutants in a high-traffic urban street canyon 

Leyla Sungur, Wolfgang Babel, Sophie Arzberger, Sophia Ramer, Johann Schneider, Frederik R. Bachmann, Ines Bamberger, Anke Nölscher, and Christoph Thomas

Urban air quality directly determines urban quality of life. To improve it, we need to know about local emissions, chemical transformations, and transport processes of the energy-containing vortices in the air. The combination of high-resolution ultrasonic anemometers and state-of-the-art vortex-resolving Large Eddy Simulation (LES) technique is a powerful key tool enabling this understanding. Here, we investigated the dynamics and transport of air with particular focus on nitrogen dioxide (NO2) in a highest-traffic street canyon with eight driving lanes in the urban setting of the city of Munich, Germany. Using spatially distributed observations and results from flow-resolving simulations, temporally and spatially resolved patterns and trends of airflow and pollutant concentrations are presented. The airflow conditions in the wide (approx. 80m) urban street canyon are largely decoupled from the synoptic flow over the city. The street is mostly characterized by a channeled, northerly current and weak wind speeds and turbulence kinetic energy (TKE) during the day, independent of prevailing synoptic forcing conditions. At night, the channeled current shifts to southern flow and reverses back to northerly winds in the early morning transition. One exception to this rule are infrequent synoptic easterly flows perpendicular to the street canyon orientation, which lead to a deflection of the flow by the building fronts and a flow reversal to westerly flows at the street level. In this case, TKE is strongly enhanced, and pollutant concentrations are low due to enhanced mixing and inflow of less polluted above-city air. Emission coefficients from the Handbook for Emission Factors for Road Transport (HBEFA) have been used in combination with traffic demand data from loop detectors to compute the respective NO2 emissions. These emissions show daily peaks in the morning and afternoon hours, and a significant differentiation between weekday, Saturday, and Sundays with less traffic. The individual lanes also differentiate in amount of emission. Linking the results from the point turbulence and NO2 measurements with the LES approach helps to understand the turbulent air transport and NO2 in parts of the street canyon where no observations exist. The first results from an LES run in a twofold nested domain with a spatial resolution of Δx,y,z = 1m for the street canyon and buildings show promising similarities in airflow patterns and dynamics compared to the observations and are currently undergoing further validation. This study is financed by the Bavarian Ministry of the Environment and Consumer Protection.

How to cite: Sungur, L., Babel, W., Arzberger, S., Ramer, S., Schneider, J., Bachmann, F. R., Bamberger, I., Nölscher, A., and Thomas, C.: Transport and emissions of gaseous air pollutants in a high-traffic urban street canyon, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14901, https://doi.org/10.5194/egusphere-egu23-14901, 2023.

EGU23-15106 | ECS | Orals | AS3.15 | Highlight

Low-cost air quality sensors: The good, the bad, and the ugly. Preliminary findings from the QUANT study 

Stuart E Lacy, Sebastian Diez, Thomas J Bannan, Michael Flynn, Nathan Watson, Nicholas Marsden, Max Priestman, and Pete M Edwards

Low-cost air pollution sensors (LCS) have a potentially vital role to play in tackling air pollution. Their affordability facilitates the creation of dense networks, which coupled with their intrinsic high time resolution offers a vast spatio-temporal coverage unlike that possible with conventional instrumentation, offering a paradigm shift in the way we measure key pollutants, evaluate health impacts of air pollution exposure and assess clean air policies. However, despite the availability of numerous commercial LCS products, there is limited current understanding as to their suitability for these tasks.

 

The QUANT project aims to address this deficit in order to enable the use of LCS to support UK clean air ambitions. Over a period of three years, 52 commercial LCS instruments from 14 companies have been measuring real world air quality data in a range of UK urban environments, collocated with reference grade instruments. With the data collection period having ended in November 2022, there now exists a comprehensive dataset of measurements from multiple pollutants across a variety of LCS systems, differing in both the underlying sensor technology as well as the software layer that converts the noisy raw signals into meaningful concentrations. 

 

This talk summarises the initial conclusions emerging from this study, highlighting the various factors that should be taken into account when considering LCS for a specific task, for example: the robustness of the calibration algorithm, variability between devices from the same company, how well the measurements transfer between sites, and differing response to meteorological conditions. To help make this knowledge accessible to a wider audience, a web-app is presented that can allow researchers and decision makers to interactively explore the dataset to assess the applicability of devices to their particular requirements.

How to cite: Lacy, S. E., Diez, S., Bannan, T. J., Flynn, M., Watson, N., Marsden, N., Priestman, M., and Edwards, P. M.: Low-cost air quality sensors: The good, the bad, and the ugly. Preliminary findings from the QUANT study, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15106, https://doi.org/10.5194/egusphere-egu23-15106, 2023.

EGU23-15178 | ECS | Orals | AS3.15

Remote sensing of columnar trace gases during the Ruisdael Rotterdam campaign in 2022 

Katharina Heimerl, Sander Houweling, Frank Hase, Mahesh Kumar Sha, Filip Desmet, Nicolas Kumps, Bavo Langerock, Thorsten Warneke, Nils Hase, Jonas Hachmeister, and Andre Butz

Urban areas are home to many people on the globe, and centres of industry. Emissions from cities contribute to atmospheric concentrations of greenhouse gases like CO2 and CH4, which influence the Earth’s energy budget. The Ruisdael Observatory is a Dutch research infrastructure to investigate the atmosphere over the Netherlands by bringing together measurements and high resolution modelling. One part of it is a semi-mobile trailer to be flexibly deployed as measurement station for targeted field measurements. Mounted on the roof of this trailer are a Bruker EM27/SUN (EM27) for columnar trace gas measurements and a Cimel for columnar aerosol measurements. A targeted field campaign was conducted in August and September 2022 to study Rotterdam, one of the biggest city in the Netherlands and the biggest harbour in Europe. Three EM27s were set up around Rotterdam in an upwind-downwind configuration. To ensure the comparability of the data, the instruments measured in parallel for three days before and after the measurement period, which showed good agreement between the instruments. Four different configurations of instrument locations were used during the three week campaign to account for changes in wind direction and investigate specific targets as well as separate between the influence of the harbour area and the city itself. Enhancements in the CO2 column were around 1-3 ppm across the harbour and about 1 ppm across the city. CH4 columnar concentrations were not significantly enhanced across the city, but increased by several ppb across the harbour area. The CO columnar concentrations increased across the harbour by up to 10 ppb and 5 ppb across the city area.

How to cite: Heimerl, K., Houweling, S., Hase, F., Sha, M. K., Desmet, F., Kumps, N., Langerock, B., Warneke, T., Hase, N., Hachmeister, J., and Butz, A.: Remote sensing of columnar trace gases during the Ruisdael Rotterdam campaign in 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15178, https://doi.org/10.5194/egusphere-egu23-15178, 2023.

EGU23-15411 | Orals | AS3.15

Impact of transport sector on air quality in Warsaw – a multi-tool study 

Joanna Struzewska, Marcin Kawka, Anahita Sattari, Aleksandra Starzomska, Aleksander Norowski, Grzegorz Jeleniewicz, Lech Gawuć, and Karol Szymankiewicz

Urban air quality is one of the challenges due to high exposure resulting from high population density and high pollutant concentrations. Developing effective strategies to improve air quality requires determining the contribution of different emission sources within the city compared to the influence of the inflow from surrounding areas.

In Polish cities, the residential sector is a dominant source of particulate matter. However, transportation is also a significant source of pollution, especially concerning NO2.

The main goal of the project was to assess the impact of the transportation sector on air quality in Warsaw. We have applied a muti-tool approach. The analysis of a 5-year series of air quality observations at urban background stations and the traffic station let to identify systemic differences attributed to road transport. Based on the GEM-AQ model results, the contribution of the transport setor in selected districts was assessed. The SHERPA bottom-up tool for Poland was applied to estimate the impact of line sources on PM10, PM2.5 and NO2 concentrations in Warsaw metropolitan area. Also, two local models were used – the IEP-NRI gaussian model combined with the machine learning techniques, and the ATMOSYS model developed by VITO. The intercomparison brought a valuable outcomes on the completeness and accuracy of the emission data applied.

We will present and discuss the percentage contribution of road transport-related pollutant concentrations in Warsaw based on the different model results.

How to cite: Struzewska, J., Kawka, M., Sattari, A., Starzomska, A., Norowski, A., Jeleniewicz, G., Gawuć, L., and Szymankiewicz, K.: Impact of transport sector on air quality in Warsaw – a multi-tool study, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15411, https://doi.org/10.5194/egusphere-egu23-15411, 2023.

EGU23-15484 | Posters on site | AS3.15 | Highlight

A modular data management approach for environmental observation campaigns in multiple cities 

Matthias Zeeman, Kit Benjamins, Ferdinand Briegel, Marc-Antoine Drouin, Gregor Feigel, Daniel Fenner, Simone Kotthaus, Rainer Hilland, Fred Meier, William Morrison, Marvin Plein, Swen Metzger, Karthik Reddy, Nektarios Chrysoulakis, Sue Grimmond, and Andreas Christen

Field observation networks are becoming denser, more diverse, and more mobile, while being required to provide real-time results. The ERC urbisphere program is coordinating multiple field campaigns simultaneously to collect datasets on urban atmospheric and environmental conditions and processes in cities of different sizes. The datasets are used for improving climate and weather models and services, including assessing the impact of cities on the atmosphere (e.g. aerosols, greenhouse gases) as well as the exposure of urban populations in the context of atmospheric extreme events (heat waves, heavy precipitation, air pollution). For model development and evaluation, we are using meshed networks of in-situ observations with ground-based and airborne (remote-)sensing platforms. This contribution describes the urbisphere data management infrastructure and processes required to handle a variety of data streams from primarily novel modular observation systems deployed in complex urban environments.

The modular observation systems consist of short-term deployed instrumentation and are separated into three thematic modules. Module A aims at characterizing urban form and function affecting urban climates. Module B quantifies the impact of urban emissions (heat, pollutants, greenhouse gases, etc.) on the urban boundary layer over and downwind of cities. Module C provides data on human exposure at street and indoor-level. The three modules are served with consistent data management, documentation and calibration. Systems deployed in Modules A, B and C include customized automatic weather stations, (Doppler) lidars and ceilometers, scintillometers, balloon radio sounding and spectral camera imaging. Systems are street-light-mounted, located on building roof-tops or indoors as well as on mobile platforms (vehicles, drones). Data ingestion processes are automated, delivering moderate data volumes in real-time to central data infrastructure through mobile phone and IOT connectivity. A meta data system helps keep track of the location and configuration of all deployed components and forms the backbone for conversion of instrument records into location-aware, conventions-aligned and quality-assured F.A.I.R. data products. Furthermore, the data management infrastructure provides services (APIs, Apps, IDEs, etc.) for data inspection and computations by scientists and students involved in the campaigns. Select datasets are integrated in near real-time into other global or local data systems such as, e.g., AERONET, the Phenocam Network, ICOS, or PANAME, for multiple uses.

Besides technical aspects and design considerations, we discuss how cooperation and attribution are safeguarded when data are being accessed for immediate academic and citizen data science.

 

How to cite: Zeeman, M., Benjamins, K., Briegel, F., Drouin, M.-A., Feigel, G., Fenner, D., Kotthaus, S., Hilland, R., Meier, F., Morrison, W., Plein, M., Metzger, S., Reddy, K., Chrysoulakis, N., Grimmond, S., and Christen, A.: A modular data management approach for environmental observation campaigns in multiple cities, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15484, https://doi.org/10.5194/egusphere-egu23-15484, 2023.

EGU23-17283 | Posters on site | AS3.15

How VOC Emissions by Asphalt Pavements under Service Conditions Impact Air Quality in Cities? 

Manolis N. Romanias, Jerome Lasne, Anais Lostier, Sabine Vassaux, Didier Lesueur, Vincent Gaudion, Marina Jamar, Richard Derwent, Sebastian Dusanter, and Therese Salameh

Outdoor air pollution is the fourth cause of death worldwide, linked to around 4.2 million deaths per year. Air pollution is more severe in urban environments of cities/megacities, due to the high population density and intense anthropogenic activities. More than 50% of global population lives currently in urban areas,1 and a projected 70% is anticipated by 2050,2 even reaching 84% of the population in the EU.3

Around 40% of urban areas are covered by asphalt pavements, a fraction that keeps increasing with urbanization.4,5 Asphalt is a petroleum byproduct composed of a large number of organic species 6-8 capable of emitting a wide variety of organic compounds. Although emission of pollutants by asphalt mixtures have been investigated at deposition temperatures (120-160°C), data at service temperatures (i.e., atmospheric relevant conditions) are lacking.

Among atmospheric pollutants, Volatile Organic Compounds (VOCs) play a key role in urban atmospheres, as efficient ozone (O3) and Secondary Organic Aerosol (SOA) precursors. In the present work, we characterize and quantify VOC emissions by fresh and aged asphalt surfaces as a function of temperature. Experiments were performed inside a Teflon atmospheric simulation chamber coupled with PTR-ToF-MS, and GC-MS/FID for VOC speciation and quantification. We observe that at atmospheric relevant temperatures, asphalt surfaces significantly contribute to urban pollution, and therefore urgently need to be included in emission inventories, and in air quality models. Emissions are shown to be key in terms of ozone and SOA formation potential in urban areas to account for observations of urban air pollution.

 

References

(1)          Ritchie, H.; Roser, M. Urbanization. Our World in Data 2018.

(2)          United Nations “World Urbanization Prospects: The 2018 revision ”, 2018.

(3)          EuropeanCommission; Eurostat. Urban Europe : statistics on cities, towns and suburbs : 2016 edition; Publications Office, 2016.

(4)          Akbari, H.; Shea Rose, L.; Taha, H. Analyzing the land cover of an urban environment using high-resolution orthophotos. Landsc. Urban Plan. 2003, 63 (1), 1.

(5)          Pacheco-Torgal, F.; Labrincha, J.; Cabeza, L. Eco-efficient Materials for Mitigating Building Cooling Needs; 1st Edition ed., 2015.

(6)          Lesueur, D. The colloidal structure of bitumen: Consequences on the rheology and on the mechanisms of bitumen modification. Advances in Colloid and Interface Science 2009, 145 (1), 42.

(7)          Hung, A. M.; Goodwin, A.; Fini, E. H. Effects of water exposure on bitumen surface microstructure. Construction and Building Materials 2017, 135, 682.

(8)          Mirwald, J.; Nura, D.; Eberhardsteiner, L.; Hofko, B. Impact of UV–Vis light on the oxidation of bitumen in correlation to solar spectral irradiance data. Construction and Building Materials 2022, 316, 125816.

How to cite: Romanias, M. N., Lasne, J., Lostier, A., Vassaux, S., Lesueur, D., Gaudion, V., Jamar, M., Derwent, R., Dusanter, S., and Salameh, T.: How VOC Emissions by Asphalt Pavements under Service Conditions Impact Air Quality in Cities?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17283, https://doi.org/10.5194/egusphere-egu23-17283, 2023.

EGU23-17285 | Orals | AS3.15 | Highlight

Identifying strategies to reduce diesel particulate matter levels in cities 

Linda George, Andrew Rogers, Kirsten Sarle, and Lyndsey DeMarco

Diesel emissions are ubiquitous around the world and adversely impacts human and environmental health. One of the primary pollutants of concern from diesel combustion are the solid particles formed as a byproduct of the combustion diesel fuel, known as diesel particulate matter. In regions where there is significant transport of goods, such as port cities, emissions from trucks, ships and trains can raise ambient levels of diesel particulate matter above health standards. We studied diesel emissions in Portland, Oregon USA, a mid-sized port city through a combination of source testing/evaluation, ambient monitoring and modeling (CALPUF) to produce a validated model of ambient diesel particulate matter. Similar work is starting in Rotterdam, Netherlands. Through our model we were able to identify policies that can be used to reduce emissions and ambient concentrations of diesel particulate matter. We collaborated with a state regulators and community groups identify mitigation strategies to model. For example, we modeled the potential effect of electrification of trucks and the use of cleaner diesel construction equipment. In addition, we were able, through modelling, to explore the impact of shipping distribution centers, an emerging and growing source of diesel emissions within cities in an era of on-line shopping. Validated modeling can improve understanding of the drivers of elevated levels of diesel particulate level as well as identify potential mitigation strategies.

Keywords: Air pollution, diesel emissions, diesel particulate matter, air pollution monitoring, air pollution modeling

How to cite: George, L., Rogers, A., Sarle, K., and DeMarco, L.: Identifying strategies to reduce diesel particulate matter levels in cities, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17285, https://doi.org/10.5194/egusphere-egu23-17285, 2023.

EGU23-17536 | Orals | AS3.15 | Highlight

Novel Sensor Networks and Methods for Urban Greenhouse Gas Monitoring 

Jia Chen, Adrian Wenzel, Andreas Luther, Andreas Forstmaier, Patrick Aigner, Vigneshkumar Balamurugan, Florian Dietrich, Daniel Kühbacher, Moritz Makowski, Haoyue Tang, Xinxu Zhao, Friedrich Klappenbach, Hossein Maazallahi, Thomas Roeckmann, Hugo Denier van der Gon, Taylor Jones, and Bradley Matthews

As more than 70% of fossil fuel-based carbon dioxide (CO2) is emitted in urban areas, urban greenhouse gas (GHG) monitoring plays a crucial role in achieving emission reduction goals. Nowadays, most cities rely on downscaled national data to calculate their total emissions, or on bottom-up methods, where emission factors are multiplied with activity data, such as energy consumption, economic activity, and traffic density. However, at the scale of individual cities, errors of 50-100% in fossil fuel CO2 emission estimates have been reported. Furthermore, in terms of methane (CH4), urban emissions are suspected to be substantially underestimated by inventory methods.

Measurements of atmospheric GHG concentrations offer opportunities to identify unknown emission sources and to address biases in urban emission inventories. Urban areas however pose significant challenges to measurement-based emissions quantification, due to the heterogeneous geometry of the cities and the complex atmospheric circulation in this environment. Therefore, representative measurements combined with sophisticated atmospheric models are vital to arrive at robust estimates of urban GHG emissions.

In Munich, Germany, we created an integrated measurement and modeling framework to better understand urban GHG emissions. MUCCnet (Munich Urban Carbon Column network) is a permanent urban GHG sensor network, consisting of five automated ground-based remote sensing systems. It is based on the differential column method (DCM), which features high precision and is relatively insensitive to vertical redistribution of tracer mass and surface fluxes upwind of the city, thus providing favorable input for urban flux inversions. MUCCnet serves to validate satellite measurements, to independently monitor local GHG emissions over the long term, and to detect unknown emission sources.

Using the Munich Oktoberfest as an example, large festivals have been identified as a potentially significant source of fossil fuel CH4, despite likely being poorly represented in CH4 emission inventories. In a recent measurement campaign in Hamburg, where DCM was deployed, we have found several significant anthropogenic sources, such as refineries and a farm as well as large area sources such as the River Elbe, whose CH4 emissions are not yet included in the standard inventories or are highly underestimated.

To assess emissions from the measured concentrations, inverse modeling is an essential tool. We developed a novel Bayesian inversion framework to inversely model emissions using column measurements. We further use mobile in-situ measurements, isotopic measurements, and eddy covariance measurements to enhance the prior knowledge of the emission map.

Within the ICOS Cities project (PAUL), we have been improving the GHG emission assessments in Munich by refining the prior emission localization and timing and by adding additional monitoring capacities, including 100 street-level low-cost CO2 sensors as well as 20 roof-level mid-cost CO2 sensors based on the NDIR measurement principle. In addition, we are establishing an autonomous NOx, PM, CO and O3 network in Munich with 50 stand-alone sensor nodes. This network is used to study the spatial distribution of urban air pollutants and to assess co-emitted species of CO2 emitters.

How to cite: Chen, J., Wenzel, A., Luther, A., Forstmaier, A., Aigner, P., Balamurugan, V., Dietrich, F., Kühbacher, D., Makowski, M., Tang, H., Zhao, X., Klappenbach, F., Maazallahi, H., Roeckmann, T., Denier van der Gon, H., Jones, T., and Matthews, B.: Novel Sensor Networks and Methods for Urban Greenhouse Gas Monitoring, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17536, https://doi.org/10.5194/egusphere-egu23-17536, 2023.

EGU23-170 | ECS | Posters on site | AS3.16

Understanding Climate Impact and Indoor Emission Nexus: Size Resolved Exfiltration Factor 

Navinya Chimurkar and Harish C. Phuleria

One-third of the Indian population relies on biomass for cooking and heating which makes the residential sector a major source of particulate matter (PM)emissions. The climate impact of indoor PM depends on the fraction of particles advecting out of the house, which is either not considered in climate impacts or some thumb rule is used. The removal mechanism can have a distinct impact on different size ranges, thus size-based characterization of exfiltration factor (fraction of particles that are advected outdoors) is very important to underpin accurate climate impact. This study examines the size-dependent ExF of PM and the influence of different parameters such as room size, type of circulation, and ventilation status on exfiltration factor (ExF). CO is used as a reference gas to understand decay associated with the air exchange, while PM removal is considered to be dependent on deposition and air exchange. An Optical Particle Sizer and an Indoor Air Quality Monitor are used for PM and CO real-time measurements. We find a significant difference in PM2.5 ExF during natural (25±7 %) and forced (34±12 %) circulation. PM2.5 ExF was lowest  (i.e. 22%)  when both door and window were closed. Opening the window or both window and door increased the exfiltration slightly (26 and 27 %,  respectively). However, the exposure time to significantly elevated indoor PM levels can vary from 10 mins to 360 mins depending on ventilation, thus health impacts can differ significantly due to ventilation despite having an insignificant change in climate impacts. Size-based ExF for PM0.9, PM2.5, and PM10 ExF were 43±28, 30±9 and 29±9 % respectively.The integration of ExF, total PM emissions, and kitchen-type information would bring more certainty to the climate impact assessment. An extended analysis is underway to understand the importance of room size and shape.

 

Figure 1. The decay of gas and aerosol concentration from the room under different removal mechanisms. (Here, EF stands for emission factor)

How to cite: Chimurkar, N. and Phuleria, H. C.: Understanding Climate Impact and Indoor Emission Nexus: Size Resolved Exfiltration Factor, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-170, https://doi.org/10.5194/egusphere-egu23-170, 2023.

EGU23-672 | ECS | Orals | AS3.16

Simulation of trace gases over the Indian domain: evaluation of the SILAM model 

Priyanka Sinha, Chinmay Jena, Anikender Kumar, Vijay Kumar Soni, and Tanu Jindal

The global-to-meso-scale dispersion model System for Integrated modeling for atmospheric composition (SILAM) has been implemented over the Indian region for operational air quality forecast. The regional SILAM model generates 96 hours forecasts over a domain at 3kmx3km horizontal resolution. The meteorological forcing is provided from the operational 3 km WRF model. The initial condition is derived from the forecast of the previous cycle of the regional SILAM model and the boundary condition is supplied from the global version of the model. Predicted mixing ratios of trace gases in the atmosphere are compared with the available ground-based observations over the North-Western Indian domain for two consecutive years (2021 and 2022). The paper presents a comprehensive evaluation of SILAM model performance against the observed surface data for trace gases (Surface O3, NO2, and CO). The spatial and temporal variability of trace gases over the domain is well simulated by the model.  The model was also able to catch well the seasonality of trace gases (Surface Ozone, NO2, and CO) over the selected Indian domain. The forecast is found to be very skillful for trace gases and has been helping the air pollution control authorities in India to make informed decisions.

How to cite: Sinha, P., Jena, C., Kumar, A., Soni, V. K., and Jindal, T.: Simulation of trace gases over the Indian domain: evaluation of the SILAM model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-672, https://doi.org/10.5194/egusphere-egu23-672, 2023.

EGU23-1453 | Orals | AS3.16

Response of the ozone chemistry to changes in emissions over the Catalonia region 

Alba Badia, Veronica Vidal, Sergi Ventura, Roger Curcoll, Ricard Segura, and Gara Villalba

Tropospheric ozone (O3) is an important surface pollutant in urban areas with complex formation mechanisms that depend on the atmospheric chemistry composition and meteorological factors. The severe reduction in anthropogenic emissions during the COVID-19 pandemic can serve to further our understanding of the photochemical mechanisms that lead to O3 formation to provide guidance for policy aiming to reduce air pollution. In this study we use the air quality model WRF-Chem coupled with the urban canopy model BEP-BEM to investigate changes in the ozone chemistry over the Metropolitan Area of Barcelona (AMB) and its atmospheric plume northward, which is responsible for the highest number of hourly O3 exceedances in Spain. The aim is to investigate the response of the ozone chemistry to changes in precursor emissions. Results show that with the reduction in emissions: 1) the ozone chemistry formation tends to go to the NOx-limited or transition regimes, however urban areas over highly polluted areas are still in the VOC-limited regime, 2) the reduced O3 production is overwhelmed by the less nitric oxide (NO) titration resulting in a net increase of O3 concentration (up to 20 %) in the afternoon, 3) the increase in maximum O3 (up to 6%) during the lockdown could be attributed to an enhancement in the atmospheric oxidation capacity, 4) ozone and odd oxygen (Ox) maximum levels generally decrease (up to 4 %) in the relaxation period with a reduced atmospheric oxidation capacity (AOC), indicating an improvement of the air quality, and, 5) changes in ozone concentrations in the AMB contribute to the pollution plume along the S–N valley to the Pyrenees. Our results indicates that a protocol with strict measures to control NOx emissions, without cutting significantly anthropogenic sources of VOCs (e.g. for power plants and heavy industry) is essential for O3 abatement plans. In addition, our results show that the design of a mitigation strategy to reduce O3 cannot be related only on emissions reductions because ozone chemistry depends on several other factors (AOC, ozone regimes, local meteorology, transport).

How to cite: Badia, A., Vidal, V., Ventura, S., Curcoll, R., Segura, R., and Villalba, G.: Response of the ozone chemistry to changes in emissions over the Catalonia region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1453, https://doi.org/10.5194/egusphere-egu23-1453, 2023.

EGU23-1575 | Posters on site | AS3.16

A study of CO emission adjustment and its implication in Taiwan using WRF-CMAQ model 

Chieh-Sen Tsai and Hui-Ming Hung

The concentrations of air pollutants are mainly controlled by local emissions, physical processes, and chemical reactions. Emissions provide the primary pollutants or the precursors, while physical processes affect the concentration through transport or deposition, and chemical processes cause the production and loss of pollutants. Evaluation of emission inventories plays a crucial role in understanding the local pollutant concentration variation. In this study, we focus on carbon monoxide (CO), which is a low-reactivity species with a lifetime of 2 months. It can act as a pollutant tracer for a regional condition. Our earlier simulation of Taiwan CO based on Taiwan Emission Data System 9.0 (TEDS 9.0), shows that CO is underestimated compared with observation roughly by a factor of 3, whereas nitrogen oxide (NOX) and ozone (O3) have slight differences. Thus, we apply Community Multiscale Air Quality (CMAQ) model with Weather Research and Forecasting (WRF) model to re-evaluate the required emission adjustment and investigate the possible influence on other chemical species. With the minimum root mean square error (RMSE) between simulation and observation, the optimal emission correction factors are estimated as 2, 4, and 3.6 for northern, central, and southern Taiwan, respectively. The simulation result of applying emission factor adjustment shows significant improvement of simulated CO concentration, both on values and patterns. The underestimation of current emission inventories might indicate possible uncertainties in emission sources. The considerable adjustment in CO might modify the impact on climate (completing OH radicals with CH4 and forming CO2) and could further influence NOX, O3, and particle-phase nitrate, which will be discussed in this presentation.

How to cite: Tsai, C.-S. and Hung, H.-M.: A study of CO emission adjustment and its implication in Taiwan using WRF-CMAQ model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1575, https://doi.org/10.5194/egusphere-egu23-1575, 2023.

EGU23-1713 | Orals | AS3.16

Modeling global fire emissions of organics and their impact on reactivity 

Colette Heald and Therese Carter

Fires are a large source of non-methane organic gas (NMOG) emissions to the global atmosphere. These emissions can contribute to the formation of secondary pollutants such as ozone and particulate matter. However, the abundance and impacts of these emissions are uncertain and historically not well constrained. In this presentation, I will describe recent efforts to expand the representation of NMOGs from fires in a global model (GEOS-Chem) as well as the evaluation of the resulting simulation against airborne observations from the FIREX-AQ and ARCTAS campaigns. We use this expanded model to make the first estimate of the fire contribution to OH reactivity (OHR). We find that fires make an important contribution to global mean surface OHR (15%), and can be a dominant source of reactivity (up to 75%) over fire source regions. This work highlights the importance of representing the emissions and chemical oxidation of the suite of NMOGs emitted from fires in models.

How to cite: Heald, C. and Carter, T.: Modeling global fire emissions of organics and their impact on reactivity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1713, https://doi.org/10.5194/egusphere-egu23-1713, 2023.

EGU23-1748 | Posters on site | AS3.16 | Highlight

Modelling past and future O3 and PM2.5 surface levels over Europe under various emission scenarios 

Ulas Im, Zhuyun Ye, Jesper H. Christensen, Camilla Geels, Risto Hanninnen, Mikhail Sofiev, Øivind Hodneborg, and Marit Sandstad

We have used the Danish Eulerian Hemispheric Model (DEHM), offline-coupled with the Weather Research and Forecast model (WRF) to model the ozone (O3) and fine particulate matter (PM2.5) surface levels over Europe in the period 1981-2050. Several future emission projections adopted from the Coupled Model Intercomparison Project Phase 6 (CMIP6) have been used to simulate the O3 and PM2.5 levels in the 2015-2050 period. Results showed that under the high emission mitigation scenario (SSP1-2.6), surface O3 and PM2.5 levels will decrease by up to 20% and 80%, respectively, compared to the 2015 levels, while middle-of-the-road scenario (SSP2-4.5) will lead to a 3% and 60% decrease in O3 and PM2.5 levels, repectively. The low mitigation scenario (SSP3-7.0) will lead to an increae of 3% in Euoprean O3 levels, while a 40% reduction is calculated for the Eueropean PM2.5 levels in 2050. Results also showed that O3 levels are expected to increase mainly over the southern Europe in all scenarios, while PM2.5 levels are expected to decrease in particular over central Europe.

 

How to cite: Im, U., Ye, Z., Christensen, J. H., Geels, C., Hanninnen, R., Sofiev, M., Hodneborg, Ø., and Sandstad, M.: Modelling past and future O3 and PM2.5 surface levels over Europe under various emission scenarios, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1748, https://doi.org/10.5194/egusphere-egu23-1748, 2023.

EGU23-2132 | ECS | Posters on site | AS3.16

Improved assessment of OVOC sources and sinks over Reunion Island through WRF-Chem model evaluation against PTR-MS data and satellite retrievals 

Catalina Poraicu, Jean-François Müller, Trissevgeni Stavrakou, Crist Amelynck, Niels Schoon, Bert Verreyken, Camille Mouchel-Vallon, Pierre Tulet, and Jérôme Brioude

Oxygenated volatile organic compounds (OVOC) have a significant impact on atmospheric oxidation capacity and climate. OVOCs are directly emitted from biogenic sources and are produced from the oxidation of hydrocarbons in the atmosphere. However, their budget remains poorly understood, due to incomplete representation of photochemical OVOC production and uncertainties in terrestrial emissions and ocean/atmosphere exchanges. In addition, OVOC atmospheric measurements are scarce in remote areas, in particular in tropical regions. In this work, we exploit a 2-year high-temporal resolution dataset of mass spectrometry (PTR-MS) measurements of OVOC compounds at a remote high-altitude tropical site, the Maïdo Observatory (2155m asl) on Reunion Island. More precisely, the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) is used to provide an updated evaluation of the budget of OVOCs over Reunion Island, based on the PTR-MS dataset complemented with meteorological measurements and satellite (TROPOMI) retrievals of relevant compounds. The model is configured to allow three nested domains centred on Reunion Island, with spatial resolution from 12.5, 2.5 and 0.5 km. The finest resolution is needed due to the complex orography of the island and the spatially heterogeneous distribution of reactive species. For computational reasons, the focus is on two one-month simulations in January and July 2019, allowing analysis of seasonal differences and their impacts on model performance and chemical budget.

The WRF-simulated meteorology is first evaluated against meteorological measurements at a remote site (Maïdo) and two urban sites (Saint Denis and Saint Pierre). The impact of physical parameterizations (i.e. planetary boundary layer parameterizations, surface scheme, etc.) is tested through sensitivity simulations. A high-resolution (1km2) anthropogenic emission inventory for Reunion is implemented, complemented with information from global inventories. Biogenic VOC emissions (primarily isoprene) are calculated on-line using the MEGAN algorithm and high-resolution distributions of standard emission factors and plant functional types (PFTs). The MOZART chemical mechanism is adopted. The chemical simulations are evaluated against (1) NO2 and HCHO vertical columns from TROPOMI, (2) the PTR-MS OVOC dataset at Maïdo, and (3) network air quality measurements at several sites. Those comparisons will provide new constraints on the emissions of NOx and VOCs, and will result in recommendations for further refinements. This work will lead to a better appraisal of OVOC sources and sinks over the island. The main unknowns and potential issues will be discussed.

How to cite: Poraicu, C., Müller, J.-F., Stavrakou, T., Amelynck, C., Schoon, N., Verreyken, B., Mouchel-Vallon, C., Tulet, P., and Brioude, J.: Improved assessment of OVOC sources and sinks over Reunion Island through WRF-Chem model evaluation against PTR-MS data and satellite retrievals, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2132, https://doi.org/10.5194/egusphere-egu23-2132, 2023.

Aerosol particles, one major air pollution, are getting serious attention not only for health concerns, but also affecting global radiation budgets. They can be directly emitted into the atmosphere (primary aerosol), including black carbon, sea salt, dust, and some organic substances, and produced by chemical reactions in the atmosphere (secondary aerosol), such as sulfate (SO­42-), nitrate (NO3-), and ammonium (NH4+). Secondary inorganic composition accounts for a significant proportion in particulate matter (PM) and controls the pH value of PM, which can further affect the secondary organic matter formation. In this study, we focus on the secondary inorganic species, SO­42-, NO3- and NH4+ due to the complex interaction of NH3 and HNO3 partitioning on the aerosols containing SO­42- using the Community Multiscale Air Quality (CMAQ) model with Weather Research and Forecasting (WRF) model for the meteorological conditions for December 2018. With either the decrease of SO2 or having the SO42- formation pathway off, NH4+ has a similar trend as SO42- while NO3- has a minor variation. The model analysis indicates an ammonia-saturated condition for most of Western Taiwan. With such an ammonia-saturated condition, the emission adjustment results show that the reduction of either NOX or NH3 emission can reduce both NO3- and NH4+ and lead to a more significant effect on PM2.5 than changing SO2. The simulated ammonia is significantly higher over Western Taiwan than the observation data of the ground stations, and that promotes the dissolution of available nitric acid. Furthermore, sensitivity tests suggest that the accuracy of ammonia emission plays an important role in ruling the PM concentration via the interaction with nitric acid, which will be further discussed to reveal the feasible PM reduction via emission reduction.

How to cite: Huang, P.-C. and Hung, H.-M.: A study of the interaction of sulfate, ammonium and nitrate on the particulate matter (PM) concentration in Taiwan using WRF-CMAQ, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2200, https://doi.org/10.5194/egusphere-egu23-2200, 2023.

EGU23-2480 | ECS | Posters on site | AS3.16

Hybrid ANN and physically-based models for regional PM2.5 forecasts 

Pu-Yun Kow, Jia-Yi Liou, Li-Chiu Chang, and Fi-John Chang

Air pollution has affected people's health and lowered our living quality. Among all pollutants, PM2.5, which is smaller than 2.5 microns, can easily penetrate human lungs and seriously affect human health. Therefore, PM2.5 control is a very crucial action. Air pollution modelling can roughly categorize into two types, stochastic model (Artificial neural network (ANN) model) and deterministic model (physically-based model). Since the variation of PM2.5 concentrations is dynamic, the physically-based model struggles to handle the uncertainty from its complex interaction. With the aid of the nonlinearity of ANNs, we can overcome these uncertainties. We proposed a hybrid convolutional (CNN)-based ANN to extract features from the dataset to provide three days ahead PM2.5 forecast. The physically-based model first generates the simulated dataset. Over 40 thousand historical and simulated hourly datasets are collected to construct the deep learning model. This hybrid model that learns historical information and future trends performs better in terms of R2 (0.58-0.72) than the baseline model (0.40-0.44). Besides that, its forecast time horizon is relatively long (<72 hours) if we compare it with the pure ANN model (<12 hours). As a result, the proposed hybrid model can provide accurate regional air pollution forecasts by inheriting the characteristics of physically-based model and ANN.

Keywords: Artificial Neural Network; Deep learning; Convolutional neural network (CNN); Regional air quality forecast

How to cite: Kow, P.-Y., Liou, J.-Y., Chang, L.-C., and Chang, F.-J.: Hybrid ANN and physically-based models for regional PM2.5 forecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2480, https://doi.org/10.5194/egusphere-egu23-2480, 2023.

EGU23-2850 | Posters on site | AS3.16

Observationally constrained analysis of sulfur species in the marine troposphere 

Huisheng Bian, Mian Chin, Peter Colarco, Mingxu Liu, Marianne Tronstad Lund, Hitoshi Matshi, Joyce Penner, Hailong Wang, Kai Zhang, and Jialei Zhu

The NASA Earth Venture Suborbital (EVS-2) Atmospheric Tomography Mission (ATom) provided rich gas and aerosol measurements over the global oceans. In this study, we investigate the sulfur species of dimethyl sulfide (DMS), sulfur dioxide (SO2), methane sulfonic acid (MSA), and sulfate (SO4) that were measured during the ATom aircraft campaigns and simulated by five AeroCom models. This study focuses on remote regions over the Pacific, Atlantic, and Southern Oceans from near the surface to ~12 km altitude and covers all four seasons. We examine the vertical and seasonal variations of these sulfur species over tropical, mid-, and high latitude regions in both hemispheres. We identify their origins from land versus ocean and from anthropogenic versus natural sources with sensitivity studies by applying tagged tracers linking to emission types and regions. Using the GEOS model, we also investigate impact of cloud simulation (i.e., one-moment bulk cloud module, 1MOM vs two-moment cloud microphysics module, 2MOM) on the sulfur cycle and identify critical mechanisms of cloud impact by performing process-level budget analyses. Generally, SO4 has a better model-observation agreement than DMS, SO2 and MSA, and there are much larger DMS simulated concentrations close to the sea surface than measured, indicating all model DMS emissions may be too high. Anthropogenic emissions are the dominant source (44-60% of the total amount) for atmospheric SO4 simulated along ATom flight tracks in almost every altitude, followed by volcanic eruptions (18-33%) and oceanic sources (16-28%). GEOS SO4 simulations differ significantly between the 1MOM and 2MOM cloud schemes, with the sulfate chemical production via aqueous phase reactions seeming to be the critical process.

How to cite: Bian, H., Chin, M., Colarco, P., Liu, M., Tronstad Lund, M., Matshi, H., Penner, J., Wang, H., Zhang, K., and Zhu, J.: Observationally constrained analysis of sulfur species in the marine troposphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2850, https://doi.org/10.5194/egusphere-egu23-2850, 2023.

Dry deposition is a major sink of ozone in the planetary boundary layer (PBL). In this study, we investigate how different PBL parameterizations influence the simulations of surface ozone and its dry deposition fluxes over eastern China using the Weather Research and Forecasting Model coupled to Chemistry (WRF-Chem), and quantify the contributions of dry deposition to ozone change rates in the PBL with an integrated process rates (IPR) analysis method. As the exacerbated ozone pollution in urban areas of China has aroused extensive concern, we limit our discussion to the model results for three main city agglomerations: Beijing-Tianjin-Hebei (BTH) region, Yangtze River Delta (YRD) and Pearl River Delta (PRD). Firstly, three PBL schemes applying distinct turbulence closures are employed to examine the model sensitivities, including nonlocal closed Yonsei University (YSU), local closed Mellor–Yamada–Janjić (MYJ) and hybrid local-nonlocal scheme Asymmetric Convective Model v2 (ACM2), each coupling with one or two specific surface layer schemes. The results show that using different PBL schemes leads to the uncertainty of 6.5~18.5% for surface ozone concentration simulations, and of 3.6~15.3% for accumulated ozone dry deposition fluxes, while scarcely impacts the simulated surface ozone diurnal cycles. Among all schemes, MYJ generally calculates the lowest surface ozone concentration and dry deposition flux, especially during nighttime. According to the multiple linear regression analysis, the differences in dry deposition fluxes are dominated by the differences in surface ozone levels, and the contributions of differences in dry deposition velocities are more substantial at nighttime than at daytime. Secondly, by switching ozone dry deposition on-off based on simulation with YSU scheme, we find the absence of ozone dry deposition enhances surface ozone levels by 24~30% during daytime and by 61~82% during nighttime over the three regions. The IPR analyses indicate that when adding dry deposition process, the positive contributions of vertical mixing are elevated by 1~4 μg m-3 hr-1, partially compensating the accessorial negative contributions from dry deposition itself (by up to -8 μg m-3 hr-1) to the change rates of ozone within the PBL. Furthermore, IPR analysis is also conducted for the model results in July 20 to 23 over BTH, during which period YSU_MM5 simulates contrary ozone trend against MYJ_Eta scheme. In this episode, the choice of PBL schemes influences significantly on dry deposition, gas chemistry and advective transport processes, and the absolute contribution by simulation deviations of dry deposition process account 13% for the difference in gross ozone trend. Our study quantifies the influence of different PBL parameterization schemes on ozone simulations, emphasizing the importance of dry deposition process on governing the ozone change near surface and in the PBL.

How to cite: Li, D., Zhang, L., Liu, Z., Zhou, M., and Zhao, Y.: The influences of dry deposition process on surface ozone simulations under different planetary boundary layer parameterization schemes over eastern China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3001, https://doi.org/10.5194/egusphere-egu23-3001, 2023.

EGU23-3044 | Posters on site | AS3.16

Analysis of the Factor Affecting in the recent Air Quality changes in South Korea and China in winter 

Yesol Cha, Chang-Keun Song, Kwon-ho Jeon, Jae-Hyun Lim, and Cheol-Soo Lim

 The factors affecting the change in air quality must be objectively analyzed, and this study used chemical transport model and observational data to investigate the contributions of each factor. The data analysis focuses on air quality changes in China and South Korea from 2016 to 2020, and existing emission data were adjusted based on observational data to reflect the trend of emission reduction into chemical transport model. The observational data revealed that in China and South Korea, respectively, the PM2.5 concentration in winter in 2020 reduced by -23.7% (-11.58 µg/m3) and -19.2% (-4.97 µg/m3) compared to 2016. Meteorological condition, emission control policy, and unexpected events are major factors which may affect the change in air quality, and each of these factors has a different effect on the concentration of PM2.5. The impact of meteorological conditions in China and South Korea in 2020, resulted in increases in PM2.5 concentration of +7.6% and +9.7%, respectively, compared to 2016. However, due to the long-term emission control polices implemented in both countries, PM2.5 concentration decreased in China (-26%) and South Korea (-5%). In addition, the newly imposed policy during the study period (winter) and the unexpected coronavirus outbreak had an impact on the PM2.5 concentration in 2020. It was discovered to have decreased by -5% and -19.5%, respectively, in China and South Korea, which was not a negligible amount. Considering the impact of each quantified factors can provide a reliable scientific foundation for upcoming policymaking or air quality assessments.

This work was supported by Korea Environment Industry &Technology Institute(KEITI) through "Climate Change R&D Project for New Climate Regime." , funded by Korea Ministry of Environment(MOE) [Grant Number : 1485018907].

How to cite: Cha, Y., Song, C.-K., Jeon, K., Lim, J.-H., and Lim, C.-S.: Analysis of the Factor Affecting in the recent Air Quality changes in South Korea and China in winter, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3044, https://doi.org/10.5194/egusphere-egu23-3044, 2023.

EGU23-3050 | Posters on site | AS3.16

Comparison of PM2.5 Concentration Changes in Northeast Asia by pcSOA option in CMAQv5.2 

Jaeho Choi, Chang-Keun Song, Hyeon-Kook Kim, Kyung-Mi Lee, and Kwon-ho Jeon

The atmospheric chemical transport model, CMAQ, has been used to study the behavioral characteristics of air pollutants in Northeast Asia. To improve the performance of the simulated particulate matter, we used the CMAQ version 5.2 which newly considers pcSOA (Potential Secondary Organic Aerosol from Combustion Emissions) of fossil fuel combustion origin based on studies in North America. This study examines whether pcSOA is also effective in CMAQ modeling in Northeast Asia. Model experiments were simulated in January (Winter), April (Spring), July (Summer), and October (Autumn), representing the season in 2019, and China, South Korea, BTH (Beijing-Tianjin-Hebei), and SMA (Seoul Metropolitan Area) were selected as the target areas. To increase the reliability of the model experiment, a modeling emission inventory (e.g., UNIMIXv2) reflecting the latest air pollution emission information was used for anthropogenic emission sources in China and South Korea. According to the results of the CMAQ model experiment in January 2019, the difference between the pcSOA applied-unapplied model based on PM2.5 (particulate matter less than 2.5μm in size) concentration was about 17.23μg/m3 (-23.6%) and about 5μg/m3 (-16.5%) in China and South Korea, respectively. As a result of analyzing the chemical composition of PM2.5 simulated by the CMAQ model, ‘OC’ and ‘Unspec1’ were identified as the most affected variables by the change in the pcSOA option, and characteristics were found in the diurnal variation graph for these two substances. Therefore, when operating the CMAQv5.2 model in Northeast Asia, it is expected to help improve the model's performance in the future and understand the behavioral characteristics of air pollutants through regional and seasonal interrelated mechanisms understanding of substances caused by differences in the pcSOA option.

 

This work was supported by Korea Environment Industry &Technology Institute(KEITI) through "Climate Change R&D Project for New Climate Regime." , funded by Korea Ministry of Environment(MOE) (1485018907)

How to cite: Choi, J., Song, C.-K., Kim, H.-K., Lee, K.-M., and Jeon, K.: Comparison of PM2.5 Concentration Changes in Northeast Asia by pcSOA option in CMAQv5.2, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3050, https://doi.org/10.5194/egusphere-egu23-3050, 2023.

EGU23-3785 | ECS | Posters on site | AS3.16

Biogenic emissions-related ozone enhancement in two major city clusters during a typical typhoon process 

Jiawei Xu, Derong Zhou, Xin Huang, Steve Arnold, and Aijun Ding

Typhoons could influence air quality via multiple chemical and physical process and has attracted much scientific attention. A typical typhoon, In-Fa, passed through Yangtze River Delta (YRD) and Jing-Jin-Ji (JJJ) after it made a landfall in China. Under such influences, two city clusters both experienced high ozone (O3) concentrations, with JJJ about 5 days earlier than YRD. Data from several environmental monitoring sites indicated that cross-regional transport and biogenic emissions both played an important role in O3 formation. During the typhoon process, O3 precursors were first transported from YRD and its surrounding areas to JJJ due to the summer monsoon. After that, air masses from northern China returned to YRD due to the peripheral winds of typhoon. High O3 was concentrated in downwind regions, causing fast secondary formation. The peripheral winds and downdrafts of typhoon led to high temperature and stagnant weather, favorable for biogenic emissions. The modeling results showed the contribution of BVOCs to O3 could reach 10 ppb in JJJ when the typhoon made its landfall in YRD. When the typhoon moved to JJJ, the cross-transport of air masses from northern China to YRD contributed half of biogenic-emission-related O3. Our research extends the knowledge into the importance of biogenic emissions to O3 and cross-regional transport during a typhoon process.

How to cite: Xu, J., Zhou, D., Huang, X., Arnold, S., and Ding, A.: Biogenic emissions-related ozone enhancement in two major city clusters during a typical typhoon process, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3785, https://doi.org/10.5194/egusphere-egu23-3785, 2023.

EGU23-3818 | ECS | Orals | AS3.16

Towards more realistic modelling of tropospheric NO2 with WRF-Chem using fine-tuned temporal emission profiles 

Leon Kuhn, Steffen Beirle, Vinod Kumar, Sergey Osipov, Andrea Pozzer, Tim Bösch, Rajesh Kumar, and Thomas Wagner

NO2 is an important air pollutant and has been recognized for its hazardous impact on human health. Although routine in-situ measurements of NO2 are available in many regions of the earth, models for regional chemistry and transport (RCT) are often used to predict trace gas concentrations where no direct measurements are available. An important aspect of realistic NO2 modelling is to use accurate NOx emissions with high temporal resolution. The standard practice is to use a monthly or yearly resolved emission inventory in combination with sector-specific hourly emission weights (“temporal profiles”) in order to simulate diurnal, weekly, and seasonal emission patterns. Temporal profiles are typically derived from empirical data, e.g. car counts on highways, and have been known to improve RCT simulations significantly. Nonetheless, in comparison against in-situ measurements, simulated NO2 concentrations are usually too low at daytime and too high at nighttime, with relative deviations of up to 50 %. This hints towards faulty temporal emission profiles.

We present a novel method to determine improved temporal emission profiles for NOx emissions in a WRF-Chem simulation for May 2019 in central Europe. The temporal profiles are determined in an iterative procedure that consists of running the simulation, comparing the simulated NOx concentrations to in-situ reference measurements, and adjusting the hourly temporal profiles to compensate deviations between simulation and reference values. In a subsequent intercomparison of model results with observational datasets (surface concentrations from in-situ measurements, tropospheric vertical column densities from the TROPOMI satellite instrument, and concentration profiles from MAX-DOAS retrievals), we validate our simulation results. In particular, the typical NO2 underestimation at noontime is resolved and the monthly average of simulated vertical column densities deviates less than 7% from the TROPOMI reference data.

How to cite: Kuhn, L., Beirle, S., Kumar, V., Osipov, S., Pozzer, A., Bösch, T., Kumar, R., and Wagner, T.: Towards more realistic modelling of tropospheric NO2 with WRF-Chem using fine-tuned temporal emission profiles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3818, https://doi.org/10.5194/egusphere-egu23-3818, 2023.

EGU23-3973 | ECS | Posters on site | AS3.16

Identifying and optimizing the key parameterization processes and parameters associated with land-atmosphere interactions in WRF-Chem model to better predict O3 pollution 

Tian Han, Jing Zhang, Philipp Franke, Yunfei Che, Lihua Zhou, and Xiaoqing Deng

The Weather Research and Forecasting  with Chemistry model (WRF-Chem) is one of the state-of-art models for studying air quality. Its meteorological module and chemical module are fully coupled, making it an ideal model for exploring the interaction between meteorological and chemical processes. However, it still needs great improvement in simulating near-surface ozone in a heavy pollution event. Except for the emissions, the model parameterization processes and parameters are one of the most critical factors, meanwhile, existing great uncertainties. It is of great significance to find out the most important parameterization processes and parameters that affect the simulation results for accurate simulation. The model simulation performance is usually estimated by comparing the simulation variable with observations of some indicators, such as relative humidity, wind speed, temperature, short-wave radiation flux and boundary layer height, which have important effects on ozone concentration. By calculating the sensitivity of ozone concentration and these factors to the parameters through some parameter sensitivity experiments, the key parameters and physico-chemical processes for ozone simulation can be found out. At present, it is known that the land-atmosphere coupling process has a great influence on ozone simulation, but it is not clear which mechanism and parameter are the key factors. For this purpose, a series of parameter sensitivity experiments were designed. This study considered the land surface process, planetary boundary process, cloud microphysics process, near-surface layer process and cumulus cloud process. Six microphysics schemes, three groups of near-surface schemes, six boundary layer schemes and three cloud microphysics schemes with the best performance in WRF-Chem were selected, and a total of 120 simulations were performed. The Morris one-at-a-time (MOAT) method was used to screen out the physical and chemical processes and parameters that have important effects on ozone pollution and adaptive surrogate modeling-based optimization (ASMO) method was used to optimize these key parameters, which can explore the role of different physical processes in regulating land-atmosphere interaction, quantify the uncertainty of model physical processes, and provide evidence to improve the model physical parameterization, so as to improve the near-surface ozone simulation.

How to cite: Han, T., Zhang, J., Franke, P., Che, Y., Zhou, L., and Deng, X.: Identifying and optimizing the key parameterization processes and parameters associated with land-atmosphere interactions in WRF-Chem model to better predict O3 pollution, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3973, https://doi.org/10.5194/egusphere-egu23-3973, 2023.

EGU23-4764 | Posters on site | AS3.16

Intercomparison of air quality simulations in 2019 using three chemical transport models 

EunRyoung Kim, Hyeon-Kook Kim, Yujin J. Oak, Rokjin J. Park, Ganghan Kim, Myong-In Lee, and Chang-Keun Song

Strong air pollution control policies have been implemented to reduce health damage from heavy air pollution, but the PM2.5 concentration level is still high in Southeast Asia. This study aims to identify the causes of air pollution in East Asia using chemical transport models (CTMs). Using three CTMs (CMAQ, WRF-Chem, and GEOS-Chem), air quality was simulated by season in 2019 in Northeast Asia including China and Korea. The prediction performance of PM2.5 and its major components was evaluated, and the causes affecting the difference between CTMs were analyzed, and ways to improve the prediction performance were considered. The 2019 emission inventory updated to reflect recent changes in air pollution emissions was used in common for all three models.

As a result of analyzing the total mass concentration of simulated PM2.5 and major chemical components, the performance of each model was different for each season. CMAQ in January, WRF-Chem in July, and GEOS-Chem in October tended to overestimate the PM2.5 concentrations. For CMAQ, secondary organic aerosol (SOA) was produced by semivolatile/intermediate-volatility organic compounds (S/IVOC), and PM2.5 concentrations was high in winter. This is because CMAQ includes a new pathway for potential combustion secondary organic aerosol (pcSOA). Also, WRF-Chem simulated a particularly high concentration of sulfate because it affected the scavening function according to the aqueous phase chemistry.

These multi-model intercomparison of air quality simulations will be helpful in future research to increase understanding of the differences between CTMs in Northeast Asia and to identify the causes of air pollution.

How to cite: Kim, E., Kim, H.-K., Oak, Y. J., Park, R. J., Kim, G., Lee, M.-I., and Song, C.-K.: Intercomparison of air quality simulations in 2019 using three chemical transport models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4764, https://doi.org/10.5194/egusphere-egu23-4764, 2023.

EGU23-4777 | Posters on site | AS3.16

Investigating biases and uncertainties of air quality model used in GMAP 2021 field campaign 

Jongjae Lee, Chang-Keun Song, Rokjin Park, Chul-Han Song, Soontae Kim, Myong-In Lee, Jung Hun Woo, Hyeonmin Kim, Jinhyeok Yu, Minah Bae, Seung-Hee Lee, and Jinseok Kim

The GEMS MAP of Air Pollution (GMAP) 2021 field campaign for South Korea was conducted in October-November 2021 to understand the changes in air quality after the KORUS-AQ field study and to support efficient pollution management for ozone and aerosol. Extensive aircraft and ground network observations from the campaign offer an opportunity to reduce model-observation disagreements. This study examines these issues using model evaluation against the GMAP 2021 observations and intercomparisons between models. Four regional and one global chemistry transport model using identical anthropogenic emissions participated in the model intercomparison study. Based on the KORUSv5.0 emission inventory that supported the KORUS-AQ campaign, GMAP/SIJAQv2.0 emission inventory was developed to reflect the latest emission trends of major countries affecting South Korea’s air quality.

From the results of the model using Global Forecast System (GFS) and final (FNL) Operational Global Analysis data during and after the campaign, the accuracy of the modeling results using FNL was higher than that of GFS, which is a result of informing that the accurate meteorological input data is important for the prediction of aerosol and ozone. In comparisons of simulated versus observed (AirKorea network) CO, O3, NO2, SO2, and PM2.5 concentrations in surface air averaged for the campaign period, the models successfully reproduced observed pollutants in surface air but similar to the results in KORUS-AQ showed low biases for carbon monoxide (CO), implying that there were possible missing CO sources in the inventory in East Asia. Observations show the highest values in the Seoul Metropolitan Area (SMA) and industrial regions except for O3, which is strongly titrated by high NOx levels from traffic emissions. Relative contributions to air quality in South Korea by local and long-range transport pollution influences were classified using the Brute Force Method (BFM) for the campaign period. Observed aerosol chemical composition at the Olympic Park ground site showed that inorganic components (nitrate, sulfate, ammonium) contributed to PM2.5 by 83% during the transboundary dominant case. On the other hand, in the case of local dominant, the contribution of organic carbonaceous aerosol was 42% to PM2.5, indicating a clear difference between the two cases. In model simulations, there is a difference in the ratio between organic and inorganic aerosol, but the difference between the two cases was well simulated. And models showed a tendency to simulate Elemental Carbon (EC) at a concentration more than twice as high as observed due to the effect of emissions. From the model evaluation, we find that ensemble results of multiple models show the most consistent results with observations during the campaign period. In addition to improving the accuracy of individual models and emission inventory, evaluation of model accuracy according to ensemble techniques is necessary to improve forecast results.

 

This research was supported by the FRIEND(Fine Particle Research Initiative in East Asia Considering National Differences) Project through the National Research Foundation of Korea (NRF) funded by the Ministry of Science and ICT (Grant No.: 2020M3G1A1114615)

How to cite: Lee, J., Song, C.-K., Park, R., Song, C.-H., Kim, S., Lee, M.-I., Woo, J. H., Kim, H., Yu, J., Bae, M., Lee, S.-H., and Kim, J.: Investigating biases and uncertainties of air quality model used in GMAP 2021 field campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4777, https://doi.org/10.5194/egusphere-egu23-4777, 2023.

EGU23-4795 | Posters on site | AS3.16

A Numerical Study on Estimation of the Trees’ Effects on the Distributions of Fine Particles (PM2.5) in an Urban area 

Sang Cheol Han, Alejandra González-Pérez, Jung-Eun Kang, Geon Kang, and Jae-Jin Kim

In this study, we investigated the effects of trees planted in an urban area on PM2.5 reduction using a computational fluid dynamics (CFD) model. For realistic numerical simulations, the Local Data Assimilation and Prediction System (LDAPS) operated by the Korea Meteorological Administration was used to provide the initial and boundary conditions to the CFD model. The CFD model was validated against the PM2.5 concentrations measured by the sensor networks in the area. We conducted the numerical simulations for three configurations of the trees: 1) no tree (NT) case, 2) a case considering only trees’ drag effect (TD), and 3) a case considering trees’ drag and dry deposition effects (DD). Comparison of the average concentrations showed that the trees in the area reduced the PM2.5 concentrations during the simulation period. The results showed that trees’ dry deposition can offset the concentration increase caused by trees’ drag effect and, resultantly reduce the PM2.5 concentrations in the tree-plated area.

How to cite: Han, S. C., González-Pérez, A., Kang, J.-E., Kang, G., and Kim, J.-J.: A Numerical Study on Estimation of the Trees’ Effects on the Distributions of Fine Particles (PM2.5) in an Urban area, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4795, https://doi.org/10.5194/egusphere-egu23-4795, 2023.

With semiconductor technology gradually approaching its physical and thermal limits, Graphics processing units (GPUs) are becoming an attractive solution in many scientific applications due to their high performance. This paper presents an application of GPU accelerators in air quality model. We endeavor to demonstrate an approach that runs a PPM solver of horizontal advection (HADVPPM) for air quality model CAMx on GPU clusters. Specifically, we first convert the HADVPPM from its original Fortran form to a new Compute Unified Device Architecture C (CUDA C) code to make it computable on the GPU (GPU-HADVPPM). Then, a series of optimization measures are taken, including reducing the CPU-GPU communication frequency, increasing the size of data computation on GPU, and optimizing the GPU memory access order to improve the overall computing performance of CAMx. Finally, a heterogeneous, hybrid programming paradigm (MPI+CUDA) is presented and utilized with the GPU-HADVPPM on GPU clusters. When the consistency of its results is verified, offline experiment results show that running GPU-HADVPPM on one K40 and V100 GPU can achieve up to 845.4x and 1113.6x acceleration. By implementing a series of optimization schemes, the CAMx model coupled with GPU-HADVPPM resulted in a 12.7x and 94.8x improvement in computational efficiency using a GPU accelerator card on a K40 and V100 cluster, respectively. The multi-GPU acceleration algorithm enables 3.9x speedup with 8 CPU cores and 8 GPU accelerators on V100 cluster.

 

Figure 1. The calling and computation process of the HADVPPM function on the CPU-GPU.

Figure 2. (a) The offline performance of the HADVPPM scheme on CPU and GPU. The unit of the wall times for the offline performance experiments is millisecond(ms); (b) The total elapsed time of CAMx-CUDA V1.3 on multiple GPUs. The unit of elapsed time for experiments is seconds (s). The orange bar indicates the elapsed time of CAMx on the CPU, the blue bar shows the elapsed time on the CPU-GPU heterogeneous platform, and the red line indicates its speedup ratio on the heterogeneous platform.

How to cite: Cao, K. and Wu, Q.: GPU-HADVPPM: high-efficient parallel GPU design of the Piecewise Parabolic Method (PPM) for horizontal advection in air quality model (CAMx), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4859, https://doi.org/10.5194/egusphere-egu23-4859, 2023.

As the Beijing-Tianjin-Hebei (BTH) region of China is one of the key areas with PM2.5 air pollution and various control policies, to project the future air quality in this region under different climate scenarios and emission scenarios is of great significance. Under the comprehensive considering meteorology and anthropogenic emission, the target accessibility of 35 µg/m3 annual mean PM2.5 concentration (the Interim Target-1 by World Health Organization) in 2030, similar to the command of the carbon emissions peak and carbon neutrality, will be analyzed based on the sensitivity experiments. This study explored and quantified the influence of climate change and anthropogenic emission on the future air quality in BTH region under the future climate scenario RCP8.5, RCP4.5, and RCP2.6 with the baseline and reduced emission inventory (Base and EIT1 scenarios). The future air quality research modeling system including global climate model BNU-ESM, regional meteorological model WRF, emission process model SMOKE and air quality model CMAQ is utilized. The BNU-ESM provided the global meteorological field, and the more specific meteorological data simulated by WRF using dynamical downscaling method were adopted to drive the SMOKE model to calculate emission inventory and CMAQ model to generate air pollutant results. The results show that the future PM2.5 concentrations over BTH still present the seasonal variation, higher in winter and lower in summer. Moreover, the annual PM2.5 concentrations under various climate scenarios and under Base emission scenario are almost consistent, about 40µg/m3. However, the annual PM2.5 concentrations over BTH under the identical RCP4.5 climate scenario and under diverse emission scenario shows huge differences. The annual PM2.5 concentrations under EIT1 emission scenario is 37.5% less than the value under Base emission scenario and could achieve the annual target of 35µg/m3. Besides, the shape of high PM2.5 concentrations follows the area with high emission inventory. In a word, the future PM2.5 concentrations over BTH region is highly related to anthropogenic emission by human activities, while the climate change in 2030 has little impact on the future air quality over BTH region. That indicates emission reduction is significantly required to achieve the new Chinese PM2.5 target in 2030.

How to cite: Li, D. and Wu, Q.: The Influence of Climate Change and Human Activities on the Future Air Quality in the Beijing-Tianjin-Hebei Region of China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5090, https://doi.org/10.5194/egusphere-egu23-5090, 2023.

We will show some preliminary results of our NOAA Joint Technology Transfer Initiative (JTTI) 2-year project with the goal of applying a machine learning (ML) post-processing to improve the Community Multi-scale Air Quality (CMAQ) model operational air quality forecasts issued over the US by National Air Quality Forecasting Capability (NAQFC) at NOAA/NCEP. Specifically, we have tested an extension of the analog ensemble (AnEn) model currently implemented at the NAQFC from point-based to 2D gridded predictions.

The AnEn utilizes a training dataset comprising predictions from CMAQ and corresponding observations of the quantity to be predicted (i.e., O3 or PM2.5) to generate future ensemble predictions based on past observations. The ensemble is constructed for a given deterministic CMAQ forecast by collecting past observations corresponding to the best matching past CMAQ forecasts (called analogs) to the current CMAQ prediction.

We have conducted a preliminary application of the AnEn to reduce the errors of CMAQ PM2.5 and ozone surface gridded concentrations using a combination of past gridded chemical reanalysis from the Copernicus Atmosphere Monitoring Service (CAMS) Near-Real-Time model with measurements from AirNow stations. The analog method requires a continuous training dataset of hourly values of observed chemical concentrations obtained by merging the CAMS surface PM2.5 and ozone fields with the respective observations from the AirNow network using the Satellite-Enhanced Data Interpolation technique (SEDI) (Dinku et al. 2015). SEDI removes the bias from CAMS analysis and short-term forecast fields while preserving the AirNow-measured values at the station locations.

We will first show validation of the SEDI bias-corrected CAMS concentrations against AirNow PM2.5 and ozone-measured concentrations from stations not used in the SEDI correction process. Then, we will verify the performance of the whole forecasting system in some regions of the contiguous United States in the 0-72 hours lead time range.

 

How to cite: Alessandrini, S.: Post-Processing of CMAQ forecast for Improving Air Quality Predictions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5238, https://doi.org/10.5194/egusphere-egu23-5238, 2023.

Reliable results for the fine particulate matter (PM2.5) predictions are very useful for air policy establishment to reduce air pollution and adverse health effects caused by PM2.5. To this end, it is necessary to establish reliable emission input data for air quality models based on air pollutants' emission inventory data. In this study, we examine the characteristics of major air pollutants emitted from various emission sources in the southeast region in Korea, one of the four regions being recognized as the air pollution is serious, using a gathered information on recent 10-year's air emissions. In addition, we search the points to be carefully considered for the development of the detailed modeling emission inventory necessary for the reliable predictions of PM2.5 in the Southeast region.

 

Acknowledgements

This research was supported by the FRIEND (Fine Particle Research Initiative in East Asia Considering National Differences) Project through the National Research Foundation of Korea (NRF) funded by the Ministry of Science and ICT (Grant No.: 2020M3G1A1114615).

Correspondence to: Chang-Keun Song (cksong@unist.ac.kr)

How to cite: Kim, H.-K., Kang, Y., and Song, C.-K.: Investigation of air emissions’ characteristics in the southeast part of Korea to create modeling emission inventories for PM2.5 predictions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5408, https://doi.org/10.5194/egusphere-egu23-5408, 2023.

EGU23-5758 | ECS | Orals | AS3.16

Analyzing ozone formation conditions for aged ship plumes in a local scale chemistry transport modeling study 

Ronny Badeke, Karl Schneider, and Volker Matthias

Freshly emitted ship exhaust gas contributes to the local reduction of boundary layer ozone levels through the reaction of the emitted nitric oxide with ozone and the formation of NO2. However, after a certain time of plume aging and depending on meteorological conditions as well as the availability of other oxidizing species, new ozone will be formed from NO2. This implies that ship emissions will act as an ozone source in some distance from the ship. Considering the new and stricter recommendations for ozone limit values from the World Health Organization, it becomes important to analyze and quantify conditions for ozone formation through ship emissions in coastal areas. This study investigates impacts of various parameters like the season, diurnal cycle, cloud coverage and emitted substances on the rate of ozone destruction and formation in ship exhaust gas plumes with the local scale chemistry transport model EPISODE-CityChem. First results show the highest potential of ozone formation under clear-sky daytime conditions during the summer season. A total solar radiation >300 Wm-2 is necessary for ozone formation in Central European latitudes. A maximum ozone formation rate was found for a plume aging time of ~4 hours. A lower NO/NO2 emission ratio as well as lower CO emissions show tendencies of stronger O3 formation in the aged plume. The highest ozone formation goes together with a maximum loss rate of carbon monoxide (CO) and the hydroperoxyl radical (HO2) as well as the maximum formation of the hydroxyl radical (OH). This indicates that the effects of ship emissions on coastal air quality is highly variable and depends, beneath meteorological influences, on the distance of the ship to the coast and the mixture of pollutants in the plume. 

How to cite: Badeke, R., Schneider, K., and Matthias, V.: Analyzing ozone formation conditions for aged ship plumes in a local scale chemistry transport modeling study, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5758, https://doi.org/10.5194/egusphere-egu23-5758, 2023.

EGU23-5882 | ECS | Orals | AS3.16

Comparison of street-level atmospheric pollutant concentrations simulated with a subgrid-scale against a street-network model 

Alexis Squarcioni, Myrto Valari, Yelva Roustan, Fabrice Dugay, Youngseob Kim, Lya Lugon, Karine Sartelet, and Jérémy Vigneron

A large fraction of the European population is exposed to atmospheric pollutant concentration levels above health-related thresholds, leading to excess mortality and morbidity. Densely populated urban areas are generally more concerned than rural regions due to higher emission of atmospheric pollutants especially from the road network. Atmospheric modelling is a necessary tool to assess urban scale air-quality for both research and operational purposes. It provides a spatially and temporally resolved information for several gaseous and particulate species. It is also used for forecast and scenario evaluation for policy making. 

Modelling atmospheric composition at street level is challenging because pollutant concentration within street-canyons depends largely on local emissions but also on the transport of polluted air masses from remote areas. Therefore, regional scale modelling and local applications must be combined to provide accurate simulations of the atmospheric composition at urban scale. In our study we compare two such strategies. In both cases the regional scale chemistry-transport model CHIMERE, fed by WRF meteorological fields, provides urban background concentrations. To simulate the local component of pollutant concentrations over roads we use i) the statistical sub grid-scale approach embedded in the chemistry-transport model and ii) the street-network model MUNICH. Simulation results over the city of Paris from both modelling approaches are compared to in-situ measurements of the local air-quality network for all available traffic monitors.

The major challenge of this inter comparison exercise is to find a consistent configuration setup for both models allowing a one-to-one comparison of the simulations. To do so we had to implement the same chemical and dynamical mechanisms for gases and suspended particles in both models. We also tested several vertical discretizations to obtain a consistent first-layer depth. Different turbulence parametrizations, including or not the urban canopy model (UCM) within WRF, were compared to obtain stable results for concentrations. We show these latter are particularly sensitive to the parametrization of the anthropogenic heat flux. To obtain realistic heat fluxes and satisfactory results for both modelling strategies we have to include in the simulations all three of the following aspects i) a highly resolved land-cover database (CORINE) ; ii) a three urban class distinction in the UCM and iii) the sub-grid scale urban fraction.

Results of two-month wintertime simulations for NOx, NO2, PM2.5 are discussed. The street-network approach provides better results for both gases and particles especially at high-traffic highways. The conclusion is less straightforward at low-traffic roads. Our results highlight the need to develop a consistent coupling of the street-network model MUNICH with the regional scale chemistry transport model CHIMERE to accurately simulate gases and particulate matter concentrations over the street network.

How to cite: Squarcioni, A., Valari, M., Roustan, Y., Dugay, F., Kim, Y., Lugon, L., Sartelet, K., and Vigneron, J.: Comparison of street-level atmospheric pollutant concentrations simulated with a subgrid-scale against a street-network model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5882, https://doi.org/10.5194/egusphere-egu23-5882, 2023.

EGU23-7452 | ECS | Posters on site | AS3.16 | Highlight

Enhancing Ireland’s Dispersion Modelling Capabilities for Human, Animal & Plant Health 

Padraig Flattery, Klara Finkele, David O'Connor, Guy McGrath, and Robert Ryan

This poster will present details of a novel research project which aims to assist the Irish government to mitigate the impact of various incidents on Ireland such as infectious diseases for animals, contamination of animal feedstuffs, nuclear accidents/incidents/events abroad, radioactive contamination, environmental pollution, fire, and volcanic eruptions impacting Ireland.

Atmospheric dispersion modelling is the mathematical simulation of how air pollutants disperse in the atmosphere. It is performed using computer simulations which use algorithms to solve mathematical equations that govern the dispersion of airborne particles. Dispersion models estimate the downwind ambient concentration of air pollutants emitted from 1) man-made sources (e.g. industrial plants, vehicular traffic, accidental chemical/nuclear releases), and 2) natural sources (e.g. small insects, pollen, dust or volcanic ash). Dispersion models can also be used to predict future concentrations of particles under specific scenarios (e.g. pollen forecasting based on weather data, the spread of Bluetongue virus, and the spread of Foot & Mouth disease).

Currently, Ireland’s national meteorological service (Met Éireann) provides numerical weather prediction data to Ireland’s Environmental Protection Agency (EPA), to simulate the dispersion of nuclear material into the atmosphere. Met Éireann supports the EPA’s modelling capability by producing a daily automated simulated nuclear release. Met Éireann performs operational Bluetongue Virus forecasting, which is sent to relevant agricultural stakeholders, and supports University College Dublin (UCD) in their modelling of Foot and Mouth disease.

As climate change continues, a range of pests previously unknown in Ireland are likely to find favourable conditions here, which could potentially harm native species of plants and animals. Investigation of potential sources of these pests, and assessment of their ability to travel over large distances on prevailing winds, could help prevent losses of livestock, crops and biodiversity.

To improve Ireland’s national dispersion modelling capabilities, Met Éireann propose to commence a 4-year research project in 2023 using dispersion models and high-resolution meteorological data to build forecast capacity for a range of airborne particles that can affect human, animal and plant health. Such airborne particles include bioaerosols (vector-borne diseases, pollen and fungal spores), forest fire smoke, volcanic ash plumes and Saharan dust. High-resolution meteorological data and ensemble prediction systems will be employed to identify the locations in Ireland that are likely to be affected by various aerosols under different weather conditions. Met Éireann seeks to be an authoritative source for dispersion forecasts in Ireland, which could be of significant benefit to the agriculture industry and the significant number of Irish people who suffer from asthma, hay-fever and other respiratory illnesses. 

How to cite: Flattery, P., Finkele, K., O'Connor, D., McGrath, G., and Ryan, R.: Enhancing Ireland’s Dispersion Modelling Capabilities for Human, Animal & Plant Health, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7452, https://doi.org/10.5194/egusphere-egu23-7452, 2023.

Inorganic heterogeneous chemistry (the reactions taking place between inorganic components of the gas-particle system) is one of the most complex and computationally demanding parts of atmospheric chemistry models. Accurate and highly computationally efficient algorithms for carrying out these calculations are essential for these models. Here we present a revised and updated approach for carrying out these calculations, called HETV2.

HETV2 updates the original HETV metastable state subroutines (Makar et al., 2003) expanding the aerosol system to include base cations (Mg2+, K+, Ca2+, Na+), and partitioning between chlorine, ammonium, and nitrate ions and HCl, NH3 and HNO3 gases. HETV2 is based on the algorithms of ISORROPIA II (Fountoukis and Nenes, 2007), with several key improvements for accuracy and computational efficiency of the calculations. First, the accuracy and stability of polynomial roots have been improved by using a Taylor series expansion of the quadratic formula, for times when the coefficients differ by orders of magnitude. Second, the new algorithms in HETV2 enforce mass conservation for cases where all species are present and the ratio of total base cations to sulfate is between 1.0 and 2.0. Third, the code has been optimized using a “vectorization by gridpoint” approach, allowing a single call to each subroutine for n sets of input conditions, reducing the subroutine call factor overhead. Fourth, the code has been optimized to remove unnecessary calculations, and the programming language has been updated from Fortran 77 to Fortran 90. Fifth, all subroutines that require bisection to obtain an equilibrium solution (i.e., the ‘major systems’) have had their root-finding method updated to the ‘Interpolate, Truncate and Project (ITP)’ method (Oliveria et al., 2021); the ITP method can obtain superlinear convergence, and therefore may significantly reduce the number of iterations, and hence the computational time, required to obtain the same result as ISORROPIA II. The new algorithms significantly improve both the computational speed and accuracy for inorganic heterogeneous chemistry calculations relative to ISORROPIA II. In this talk, we will describe the inorganic heterogeneous chemistry systems that are solved, the improvements to the algorithms, and compare the computational speed of ISORROPIA II to the new HETV2 code (depending on the chemical subspace examined, the new code is up to 2x faster than ISORROPIA II).

References                                                                                                

Fountoukis, C., & Nenes, A., 2007. ISORROPIA II: A computationally efficient thermodynamic equilibrium model for Aerosols. Atmospheric Chemistry and Physics, 7(17), 4639–4659.

Makar, P. A., Bouchet, V. S., & Nenes, A., 2003. Inorganic Chemistry calculations using HETV—a vectorized solver for the SO42−–NO3–NH4+ system based on the ISORROPIA algorithms. Atmospheric Environment, 37(16), 2279–2294.

Oliveira, I. F., & Takahashi, R. H., 2021. An enhancement of the bisection method average performance preserving Minmax optimality. ACM Transactions on Mathematical Software, 47(1), 1–24.

How to cite: Miller, S., Makar, P., and Lee, C.: HETV2: An update the vectorized inorganic chemistry solver HETV to include Na+-Cl--Ca2+-K+-Mg2+ in the metastable state option based on ISORROPIA II algorithms, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7812, https://doi.org/10.5194/egusphere-egu23-7812, 2023.

EGU23-7984 | ECS | Orals | AS3.16

A New Plume Rise Algorithm – Incorporating the Thermodynamic Effects of Water for Plume Rise Prediction in Air Quality Models 

Sepehr Fathi, Paul Makar, Wanmin Gong, Mark Gordon, Junhua Zhang, and Katherine Hayden

Plume rise is commonly parameterized based on ambient atmospheric conditions and emission source metrics (e.g. stack effluent temperature and exit momentum), with empirical formulae (e.g., Briggs, 1984) employed in large-scale air-quality models (e.g. Environment and Climate Change Canada’s GEM-MACH model). Past evaluations against observed plume heights emitted from industrial sources (e.g., Canadian Oil Sands) have attributed the discrepancies between observed and predicted plume heights to various causes, such as spatial variability of meteorological fields between observation and stack locations and/or inaccuracies in model meteorological predictions. It has been shown that stack-location-specific meteorology and layered (vertical) calculation of plume buoyancy can improve predicted plume heights (Akingunola et al. 2018).  However, more recent observations have shown that predicted plume heights remain biased low relative to aircraft observations of well-characterized SO2 plumes, particularly under colder winter conditions, and demonstrate the need for further improvements to plume rise predictions. 
We introduce a new algorithm for plume rise calculation, which incorporates thermodynamic effects of the emitted water vapour from industrial stack combustion sources on the resulting calculation of plume height. The high temperature effluent from these stacks usually contain significant amounts of combustion-generated water. As the plume rises and cools, this water vapour condenses, increasing plume temperature and buoyancy through the release of latent heat, which can result in additional plume rise. We have developed a revised plume rise algorithm for implementation within the regional models, through combining the Briggs’ empirical parameterization with concepts of cloud parcel thermodynamic effects for the release or uptake of latent heat associated with the phase change of water. Our results show significant improvement in model plume rise prediction, through evaluation against SO2 plumes observed during a 2018 aircraft campaign over the Canadian Oil Sands. We also discuss results from long-term (15-month duration) model simulations with the new versus the original algorithm, along with evaluations against aircraft-based and surface monitoring network observed concentrations. The potential impact of the condensed in-plume liquid water on aqueous phase chemistry will also be discussed. This work is the first plume rise algorithm to incorporate the effects of latent heat release of both combustion-emitted and in-plume ambient-entrained water, for implementation in air quality models. 


References

  • Akingunola, A., Makar, P. A., Zhang, J., Darlington, A., Li, S.-M., Gordon, M., Moran, M. D., and Zheng, Q.: A chemical transport model study of plume-rise and particle size distribution for the Athabasca oil sands, Atmos. Chem. Phys., 18, 8667–8688, https://doi.org/10.5194/acp-18-8667-2018, 2018.
  • Briggs, G. A.: Plume rise and buoyancy effects, atmospheric sciences and power production, in: DOE/TIC-27601 (DE84005177), edited by: Randerson, D., TN, Technical Information Center, US Dept. of Energy, Oak Ridge, USA, 327–366, 1984.

How to cite: Fathi, S., Makar, P., Gong, W., Gordon, M., Zhang, J., and Hayden, K.: A New Plume Rise Algorithm – Incorporating the Thermodynamic Effects of Water for Plume Rise Prediction in Air Quality Models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7984, https://doi.org/10.5194/egusphere-egu23-7984, 2023.

EGU23-8498 | Orals | AS3.16

Representation of Precipitation Phases and a New Parameterization for Below-Cloud Scavenging in Regional Air Quality modelling 

Roya Ghahreman, Wanmin Gong, Paul Makar, Alexandru Lupu, Amanda Cole, Kulbir Banwait, Colin Lee, and Ayodeji Akingunola

Below-cloud scavenging is the process of aerosol removal from the atmosphere between cloud-base and the ground by precipitation (e.g. rain or snow), and affects aerosol number/mass concentrations, lifetime and distributions. An accurate representation of precipitation phases is important in treating below-cloud scavenging as the efficiency of aerosol scavenging differs significantly between liquid and solid precipitation. To study cloud processes and precipitation chemistry, we examined representation of below-cloud aerosol scavenging of in the current GEM-MACH model, including a revised approach in precipitation phase partitioning and implementing a new aerosol below-cloud scavenging scheme (from Wang et al., 2014) and comparing with the GEM-MACH’s existing scavenging scheme, based on Slinn (1984). 

Overall, the multi-phase partitioning and Wang et al. (2014) scavenging scheme improve GEM-MACH performance as compared with observations. Including multi-phase approach leads to a decrease on SO42- scavenging and impacts the below-cloud scavenging of SO2 into the aqueous phase. The impact of the new scheme on wet deposition of NO3- and NH4+ varies, with both increases and decreases in wet scavenging, and is more important at specific cloud locations. The two aerosol scavenging rates differ during liquid precipitation in the 0.1-1 µm size range mostly at high precipitation intensity. The two aerosol scavenging schemes diverge for aerosols smaller than 1 µm for solid precipitation at lower intensity (R=0.01 mm/h), while at higher precipitation intensities (R=10 mm/h), the two schemes show larger differences for aerosols larger than 1 µm. The changes on the speciated particles (sulphate, nitrate and ammonium) are consistent with the changes in the wet scavenging, leading to higher modelled concentrations of particulate sulphate in the atmosphere.

How to cite: Ghahreman, R., Gong, W., Makar, P., Lupu, A., Cole, A., Banwait, K., Lee, C., and Akingunola, A.: Representation of Precipitation Phases and a New Parameterization for Below-Cloud Scavenging in Regional Air Quality modelling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8498, https://doi.org/10.5194/egusphere-egu23-8498, 2023.

EGU23-8605 | ECS | Orals | AS3.16

Impact of aircraft NOx and aerosol emissions on atmospheric composition : a model intercomparison 

Yann Cohen, Didier Hauglustaine, Nicolas Bellouin, Sebastian Eastham, Marianne Tronstadt Lund, Sigrun Matthes, Agnieszka Skowron, and Robin Thor

Aircraft emissions consist of carbon dioxide (CO2), nitrogen oxides (NOx), sulfur dioxide (SO2) and particulate matter (black carbon, sulfate) and water vapour. The non-CO2 effects have been recently evaluated as twice the CO2 effects regarding their radiative forcing of climate in 2018 [1]. Among the non-CO2 effects, nitrogen oxides emissions impact several greenhouse gases concentrations. Increased tropospheric ozone production results in a positive radiative forcing (climate impact), but the subsequent increased OH concentrations enhance methane chemical destruction, thus decreasing stratospheric water vapour and the methane-linked background ozone levels in the troposphere. The net radiative forcing caused by the aircraft NOx emissions is evaluated as a net positive forcing but still shows important uncertainties.

In order to investigate representation of key mechanisms involved for climate forcing, in the framework of the ACACIA (Advancing the Science for Aviation and Climate) EU project, six global chemistry-climate models have been used to reevaluate the climate effects of NOx and aerosol aircraft emissions on atmospheric composition following a common protocol. As a first step, the standard runs have been assessed regarding ozone, carbon monoxide (CO), water vapour and reactive nitrogen (NOy) against the IAGOS airborne measurements during 1994-2018, separately in the upper troposphere and in the lower stratosphere.

As a second step, the models have been used to assess the impact of NOx and aerosol emissions on atmospheric composition. The subsonic aircraft perturbations are calculated based on the CEDS aircraft emission inventories [2] for the present-day conditions and based on different socioeconomic scenarios [3] for future (2050) conditions. Several sensitivity simulations will be presented in order to investigate the sensitivity of the results to background atmospheric conditions (present, future) and to lightning emissions. The changes in atmospheric composition will be presented and compared for the different models and scenarios.

 

Acknowledgement:

This study was supported by the European Union’s Horizon 2020 research and innovation programme under grant agreement No 875036 within the Aeronautics project ACACIA.

 

References:

[1] D.S. Lee, D.W. Fahey, A. Skowron, M.R. Allen, U. Burkhardt, Q. Chen, S.J. Doherty, S. Freeman, P.M. Forster, J. Fuglestvedt, A. Gettelman, R.R. De León, L.L. Lim, M. T. Lund, R.J. Millar, B. Owen, J.E. Penner, G. Pitari, M.J. Prather, R. Sausen, and L. J. Wilcox, Atmospheric Environment 244, 117834 (2021)

[2] R. M. Hoesly, S. J. Smith, L. Feng, Z. Klimont, G. Janssens-Maenhout, T. Pitkanen, J. J. Seibert, L. Vu, R. J. Andres, R. M. Bolt, T. C. Bond, L. Dawidowski, N. Kholod, J. Kurokawa, M. Li, L. Liu, Z. Lu, M. C. P. Moura, P. R. O’Rourke, and Q. Zhang, Geosci. Model Develop. 11, 369-408 (2018)

[3] M. J. Gidden, K. Riahi, S. J. Smith, S. Fujimori, G. Luderer, E. Kriegler, D. P. van Vuuren, M. van den Berg, L. Feng, D. Klein, K. Calvin, J. C. Doelman, S. Frank, O.Fricko, M. Harmsen, T. Hasegawa, P. Havlik, J. Hilaire, R. Hoesly, J. Horing, A. Popp, E. Stehfest, and K. Takahashi, Geosci. Model Develop. 12, 1443-1475 (2019)

How to cite: Cohen, Y., Hauglustaine, D., Bellouin, N., Eastham, S., Lund, M. T., Matthes, S., Skowron, A., and Thor, R.: Impact of aircraft NOx and aerosol emissions on atmospheric composition : a model intercomparison, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8605, https://doi.org/10.5194/egusphere-egu23-8605, 2023.

EGU23-8873 | ECS | Posters on site | AS3.16

Atmospheric oxidation of imine derivative of piperazine by OH radical 

Thomas Golin Almeida and Theo Kurtén

Amines are emitted to the Earth's atmosphere by several biogenic and anthropogenic sources. One such source, expected to increase in importance in the coming decades, is Carbon-Capture (CC), which often employs amine solvents as CO2 filters. Given that atmospheric oxidation of amines have the potential to produce nitrosamines (R1R2NNO) and nitramines (R1R2NNO2), known carcinogenic compounds, several chemical kinetics studies have investigated these reactions aiming to assess the impact on air quality from CC emissions. Piperazine is a widely employed CC amine solvent whose reaction with OH radical, the main atmospheric oxidant, has been the target of previous works, revealing a low yield of hazardous products. However, almost nothing is known about the fate of the major oxidation product, the cyclic imine 1,2,3,6-tetrahydropyrazine (THP). In fact, only a few studies focused on the atmospheric chemistry of imines in general, despite consistently appearing as major products of amine oxidation. In this work, we employed quantum chemistry and theoretical kinetics methods to investigate the mechanism and kinetics of reaction between THP and OH radical. Our findings predict that this reaction has a low, but not negligible potential to produce nitrosamines and nitramines, with a maximum yield of ~18% under high NOx conditions. The major reaction channels involve the formation of a second imine functional group, leading to the diimines 2,3-dihydropyrazine and 2,5-dihydropyrazine. Our calculations also revealed two new oxidation pathways, both involving fast C-C bond scissions. One of these pathways produce an isocyanate (RN=C=O), which is also potentially toxic. While this channel is minor for THP + OH radical (maximum yield of 14%), we argue that it could be more important during the OH radical-initiated oxidation of other imines relevant to the atmosphere.

How to cite: Golin Almeida, T. and Kurtén, T.: Atmospheric oxidation of imine derivative of piperazine by OH radical, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8873, https://doi.org/10.5194/egusphere-egu23-8873, 2023.

EGU23-9274 | ECS | Orals | AS3.16

The Atmosphere’s Oxidizing Capacity in China: Role and Influence of different photochemical processes 

Jianing Dai, Guy Brasseur, Mihalis Vrekoussis, Yijuan Zhang, and Hongliang Zhang

With the drastic actions initiated by the Chinese authorities to improve air quality, the level of several secondary pollutants including near-surface ozone still has been increasing significantly between years 2013 and 2020, most notably in the Northern China Plain. Alleviating ozone pollution requires a quantitative understanding of the different processes that contribute to the photochemical formation and destruction of secondary species. It also requires that the budget of fast-reacting radicals that are directly involved in photochemical oxidation processes be investigated in detail. Here, we used a modified regional chemical transport model (the WRF-Chem) to analyze the influence of different photochemical processes on the entire geographical area covered by China. This analysis provides a quantitative estimate of the different factors that affect the oxidation capacity of the atmosphere in different regions of the country. Besides that, our model simulations will assess the relative importance of different photochemical processes that contribute to the budget of near-surface ozone in different chemical environments and provide some theoretical considerations on which our analysis is based. This study should support to reduction of ozone and other secondary pollutants in China.

How to cite: Dai, J., Brasseur, G., Vrekoussis, M., Zhang, Y., and Zhang, H.: The Atmosphere’s Oxidizing Capacity in China: Role and Influence of different photochemical processes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9274, https://doi.org/10.5194/egusphere-egu23-9274, 2023.

EGU23-9306 | Orals | AS3.16

Key Processes in Canadian Oil Sands Gas and Aerosol Chemistry Identified through Model Evaluation Against Monitoring Network and Aircraft-Based Data 

Paul Makar, Colin Lee, Ayodeji Akingunola, Wanmin Gong, Craig Stroud, Junhua Zhang, Mahtab Majdzadeh, Roya Ghahreman, Stefan Miller, Sepehr Fathi, Alexandru Lupu, Ali Katal, John Liggio, Katherine Hayden, Ralf Staebler, Kevin Strawbridge, Eric Edgerton, Matthew Landis, Emily White, and Samar Moussa and the remainder of the Oil Sands Modelling and Measurement Team

Multiple simulations were conducted using Environment and Climate Change Canada’s Global Environmental Multiscale-Modelling Air-quality and CHemistry (GEM-MACH) in order to evaluate the model’s predictive capabilities for concentrations, height of plume emissions, and deposition for regions within and downwind of the Canadian Oil Sands.  The innermost domain of the nested setup was 1350x1345 km in extent, centered on the Canadian provinces of Alberta and Saskatchewan, with a grid-cell size of 2.5 km.  Successive model science updates were carried out in a series of 15-month simulations covering the period August 1, 2017 through October 31, 2018.  The simulations were compared to local (Wood Buffalo Environmental Association, Lakeland Industry and Community Association, Peace River Area Monitoring Program), provincial (Alberta Precipitation Quality Monitoring Program (APQMP)), and national (National Air Pollution Surveillance (NAPS) and Canadian Air and Precipitation Monitoring Network (CAPMoN)) monitoring network data for the entire period, as well as to aircraft and ground-based measurement intensive data from August 2017, April 2018 and June to July 2018. 

The series of simulations included successive updates to the model’s gas-phase chemistry, secondary organic aerosol formation, photolysis rate calculations, particle speciation, plume rise, inorganic heterogeneous chemistry, cloud processing of gases and aerosols, gas reactions on particle surfaces, the addition of a tracer for the emissions, transport and deposition of total organic carbon gas, the addition of H2S as a transported species, and numerous updates to the model’s input emissions making use of inventory and observation-based emissions.  While the model evaluation is still underway, the evaluation thus far has identified key chemical and physical processes relevant to the Oil Sands area, which will be highlighted in this presentation, including:

(1) Concentrations of particulate base cations are dominated by fugitive dust, , and exhibit strong seasonality (higher in summer than winter).  This seasonality can be reasonably well simulated by the model if coarse mode emissions of fugitive dust are shut off at temperatures slightly below the freezing point of water;

(2) Low biased model surface ozone predictions from January through April are potentially due to insufficient simulated Troposphere / Stratosphere exchange, in turn identifying the process as a driver for springtime ozone in the area;

(3) The concentrations of NO2, particulate matter and nitric acid are all linked via a combination of surface reactions transforming NO2 to HONO and HNO3, and inorganic heterogeneous chemistry, with the former reaction probabilities being highly uncertain;

(4) Aircraft-based estimates of total organic carbon gas emissions and deposition used as a tracer within the model suggest high molecular mass hydrocarbons are emitted as gases from OS facilities and are being deposited in the surrounding area.  Conventional gas-phase deposition algorithms may not explain observed deposition rates; absorptive partitioning to landscape surfaces is presented as a possible alternative pathway for deposition.

How to cite: Makar, P., Lee, C., Akingunola, A., Gong, W., Stroud, C., Zhang, J., Majdzadeh, M., Ghahreman, R., Miller, S., Fathi, S., Lupu, A., Katal, A., Liggio, J., Hayden, K., Staebler, R., Strawbridge, K., Edgerton, E., Landis, M., White, E., and Moussa, S. and the remainder of the Oil Sands Modelling and Measurement Team: Key Processes in Canadian Oil Sands Gas and Aerosol Chemistry Identified through Model Evaluation Against Monitoring Network and Aircraft-Based Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9306, https://doi.org/10.5194/egusphere-egu23-9306, 2023.

EGU23-9830 | ECS | Orals | AS3.16

An assessment of the performance of bias correction techniques for surface ozone burdens simulated by global chemistry-climate models 

Christoph Stähle, Harald E. Rieder, Arlene M. Fiore, and Ramiro Checa-Garcia

Despite continuous improvement during recent decades, state of the art global chemistry-climate models (CCMs) are still showing biases compared to observational data, illustrating remaining difficulties and challenges in the simulation of atmospheric processes governing ozone production and decay. Therefore, CCM output is frequently bias-corrected in studies seeking to explore changing air quality burdens and associated impacts on human health (e.g., Rieder et al., 2018). Here we assess the strengths and limitations of different bias correction techniques for CCM simulations with focus on maximum daily 8-hour average surface ozone. Ozone fields are chosen as ozone is known as regional pollutant and thus shows smaller spatial heterogeneity in its burden than e.g. particulate matter. Within our comparison a set of different innovative, as well as, common bias correction techniques are applied to output of selected global coupled CCMs contributing hindcast simulations to the Coupled Model Intercomparison Project Phase 6 (CMIP6). For bias correction and evaluation, we utilize gridded observational data for the European and US domains according to Schnell et al. [2014]. The statistical bias-correction techniques applied and compared are quantile mapping, delta-function, relative and mean bias correction. As surface ozone pollution is commonly associated with a strong seasonal cycle, the adjustment techniques are applied to model data on monthly basis, and skill scores for individual bias correction techniques are compared across individual CMIP6 models for both seasonal and annual timescales over the period 1995-2014. Our results highlight large differences among individual bias correction techniques and advocate for the use of more complex correction strategies involving corrections across the spatio-temporal distribution of the ozone field.

References:

Rieder, H.E., Fiore A.M., Clifton, O.E., Correa, G., Horowitz, L.W., Naik, V.: Combining model projections with site-level observations to estimate changes in distributions and seasonality of ozone in surface air over the U.S.A., Atmos. Env., 193, 302-315, https://doi.org/10.1016/j.atmosenv.2018.07.042, 2018.

Schnell, J. L., Holmes, C. D., Jangam, A., and Prather, M. J.: Skill in forecasting extreme ozone pollution episodes with a global atmospheric chemistry model, Atmos. Chem. Phys., 14, 7721–7739, https://doi.org/10.5194/acp-14-7721-2014, 2014.

How to cite: Stähle, C., Rieder, H. E., Fiore, A. M., and Checa-Garcia, R.: An assessment of the performance of bias correction techniques for surface ozone burdens simulated by global chemistry-climate models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9830, https://doi.org/10.5194/egusphere-egu23-9830, 2023.

The Korean Air Chemistry Modeling System (K_ACheMS) has been developed to enhance the predictability of PM2.5 in South Korea. In the current version (v2.0) of K_ACheMS, two meteorological models are used to produce meteorological fields. The first model is version 4.1.5 of the Weather Research and Forecasting (WRF) model. The WRF v4.1.5 model is initialized using four cycles (00Z, 06Z, 12Z, and 18Z) of real-time Global Forecasting System (GFS) data from the National Oceanic and Atmospheric Administration (NOAA). The other model is the Regional Data Assimilation and Prediction System (RDAPS), which is the regional operational model of the Korean Meteorological Administration (KMA) based on the Unified Model (UM) developed by the Met Office of the United Kingdom.

For air quality model simulations, the Community Multi-scale Air Quality version GIST (CMAQ-GIST) model has been developed based on the CMAQ v5.2.1 model. The CMAQ-GIST model mainly uses a modified version of the Statewide Air Pollution Research Center 07 (SAPRC07TC) chemical mechanism with several important updates, including the following: (i) daytime HONO photo-chemistries; (ii) heterogeneous HO2 reactions; (iii) gas- and aqueous-phase halogen chemistries; and (iv) new yield data for SOA formation acquired from multiple smog chamber experiments conducted under typical conditions of northeast Asia. In order to update chemical initial conditions for the CMAQ-GIST model simulations, a three-dimensional variational (3D-VAR) method is applied to the operational mode of K_ACheMS.

Here, we introduce the development of the K_ACheMS v2.0 and present the current performances of the operational mode of K_ACheMS v2.0 by comparing the ground-based observations in South Korea.

How to cite: Yu, J., Song, C. H., and Kim, M. C.: Development of the Korean Air Chemistry Modeling System version 2.0 (K_ACheMS v2.0) and its performance of operational mode, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10089, https://doi.org/10.5194/egusphere-egu23-10089, 2023.

EGU23-10220 | ECS | Orals | AS3.16

Towards an integrated anthropogenic emission inventory for China 

Yijuan Zhang, Guy Brasseur, Claire Granier, Nikos Daskalakis, Alexandros Panagiotis Poulidis, Kun Qu, Jianing Dai, and Mihalis Vrekoussis

The implementation of the Air Pollution Prevention and Action Plan (2013–2017) in China has led to a significant decrease in anthropogenic emissions. However, at the same time, ozone (O­3), a secondary pollutant formed from nitrogen oxides (NOx) and volatile organic compounds (VOCs) in the presence of sunlight, has increased in the large urban agglomerations of China. To better understand the reasons behind this increase, high-quality anthropogenic emission inventories are needed. In this study, we compared ozone precursor emissions in China from various anthropogenic emission inventories (EIs), including the national EI, Multi-resolution Emission Inventory for China (MEIC), and three global EIs from the Copernicus Atmosphere Monitoring Service (CAMs), Community Emission Data System (CEDS), and Hemispheric Transport of Air Pollution project (HTAP). Differences in emission magnitudes, trends, and spatial distributions were investigated. Global-scale and regional EIs were homogenized by sector and specie to obtain ‘harmonized’ EIs. These harmonized inventories were then used to drive WRF-Chem simulations for the winter and summer of 2017, and the results for each EI were evaluated against observations from the air quality monitoring network developed by the Ministry of Environmental Protection of China. The outcome of this study denotes that using harmonized regional and global EIs can significantly improve the performance of the numerical models when simulating the atmospheric composition of large agglomerations in China. 

How to cite: Zhang, Y., Brasseur, G., Granier, C., Daskalakis, N., Poulidis, A. P., Qu, K., Dai, J., and Vrekoussis, M.: Towards an integrated anthropogenic emission inventory for China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10220, https://doi.org/10.5194/egusphere-egu23-10220, 2023.

With our growing understanding of the risks of air pollution to human health, air quality forecasting has become a very important tool to enable decision makers to take preventive and corrective measures for current and future policies. In addition, accurate predictions of air quality can help predict the impacts of wildfires on human health, which have an increased risk due to anthropogenic climate change, and mitigate their impacts.  However, errors in air quality forecasts limit their value in long-term decision-making processes. Thus, increasing the accuracy of forecasts is of significant importance.

In this study, we have utilized the Community Multiscale Air Quality (CMAQ) modeling system with a 12 km horizontal grid resolution to generate air quality forecasts for the CONUS domain for June 1st through September 29th. Our study spans the seven years from 2015 to 2021, and covers the months when there is a high risk of wildfires. CMAQ is an open-source Cartesian modeling system that simulates the concentrations of atmospheric pollutants at regional scales using emission data and meteorological inputs. We generate these meteorological inputs using the Unified Forecast System (UFS) numerical weather prediction model. We create daily 48-hr forecasts of fine particulate matter (PM2.5), ozone, and related species. We have also included a Carbon Monoxide-FIRE (CO-FIRE) tracer in CMAQ, which tracks CO emitted by wildfires.

Our study consists of three parts. First, we analyze the performance of the CMAQ air quality and UFS meteorological forecasts over seven years of simulation for every EPA defined region using the Air Quality System (AQS) ambient air pollution data from over a thousand monitoring sites across the CONUS. We have found that on average, the CMAQ model performs the best in the east of the CONUS with the lowest RMSE (2 µg/m3) while in the west, where there is a high risk of wildfires, the model has the highest RMSE of up to 8 µg/m3. Temporally, the model under/over-estimates the PM2.5 concentrations during the day/night time, respectively. Next, we quantify the uncertainties in the model’s prediction, and we explore the reasons behind the model biases. Finally, we employ the state-of-the-art Analog Ensemble (AnEn) method to improve the accuracy of the forecasts and quantify the forecast improvements by AnEn. To achieve this, AnEn relies on the current deterministic forecasts, here generated from the CMAQ model, and the past archive of analogous predictions with relative prior observations. By considering the history of predictions along with the current forecast, AnEn has previously shown a significant increase in the accuracy of probabilistic forecasts by requiring significantly less computation resources compared to model-based ensembles. Despite the challenges of using AnEn for wildfires, we hypothesize that it will significantly improve the CMAQ model forecast in the proposed scenarios.

How to cite: Golbazi, M., Kumar, R., and Alessandrini, S.: Enhancing air quality forecasts across the contiguous United States (CONUS) during wildfires using an Analog-based post-processing methods, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10607, https://doi.org/10.5194/egusphere-egu23-10607, 2023.

Vegetation is an important component for modulating urban air quality. It can affect scalar transport, which is one of the most concerning processes in urban environment, by organizing the airflow around. In previous urban environment studies, the morphological characteristics of vegetation were usually parameterized as porosity or leaf area index (LAI), performing a spatially uniform aerodynamic behaviour. Whereas, a vegetation element has complex multi-scale structures. Predicting the scalar transport around the vegetation accurately is challenging due to the simplified parameterization. The transport processes around multi-scale vegetation should be further studied.

In this study, a fractal tree model is built to preserve the length scales of sub-branches. The large-eddy simulation (LES) is employed to investigate the scalar transport around the multi-scale tree. The spatial distribution of aerodynamic behaviour and scalar transport after and over the tree is determined. The scalar transport characteristics are compared with previous studies, demonstrating the importance of preserving sub-scales in urban air quality research.

How to cite: Liu, S. and Liu, C.-H.: Airflow and scalar transport around a single fractal tree based on large-eddy simulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10633, https://doi.org/10.5194/egusphere-egu23-10633, 2023.

EGU23-10647 | ECS | Posters virtual | AS3.16

Data-driven Versus Expertise-based AI Prediction of Industrial Air Pollutants 

Seunghui Choi, Jonghun Kam, and Kwanghun Lee

With the development of industrialization, air pollution problems are rapidly accelerated. Industrial air pollutants can deteriorate human lives while accelerating global warming. Thus it is important to figure out the variables that affect air pollutants in an industry. With the growth of artificial intelligence, many researches on the prediction of industrial air pollutants have been conducted to prove high performance. Yet the prediction of the air pollutants with the data-driven selected input was not evaluated compared to the expertise-based input. Herein, we predicted emissions of nitrogen oxides (NOx), sulfur oxides (SOx), and total suspended particles (TSP) at once in a heat recovery steam generator system by constructing four different multivariate AI models; a random forest regressor, a shallow long-short term memory (LSTM), a shallow bidirectional LSTM (BiLSTM), and a BiLSTM based autoencoder (BiLSTM-AE). The input of a prediction model was selected by combining the results of three univariate random forest regressors where one model predicts each air pollutant and a multivariate random forest regressor. Through average one-minute predictions to averaged 30-minute predictions, we compared the performances of the AI models. Among all of them, the random forest regressor showed the best performance for predicting NOx and SOx, and the BiLSTM-AE for predicting TSP with respect to the mean absolute error. We also compared the sensitivity by differentiating input variables of the BiLSTM-AE, the data-driven and the expertise-based selection. We constructed a multivariate random forest to examine the importance of each variable in the prediction of three air pollutants. Both the data-driven input and the expertise-based input include the gas turbine variables and some thermal variables as important variables. As a result, the expertise-based input may be good standards, but the data-driven input can be complementary to the expertise-based input for generalization and ease of selection. This study enables self-diagnosis and proactive action for each industry to regulate its air pollutants in advance of the law regulation.

How to cite: Choi, S., Kam, J., and Lee, K.: Data-driven Versus Expertise-based AI Prediction of Industrial Air Pollutants, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10647, https://doi.org/10.5194/egusphere-egu23-10647, 2023.

EGU23-10734 | ECS | Posters on site | AS3.16

Direct radiative effects of black carbon and brown carbon from Southeast Asia biomass burning with the WRF-CMAQ two-way coupled model 

Yeqi Huang, Xingcheng Lu, Zhenning Li, Jimmy Fung, and David Wong

Black carbon (BC) and brown carbon (BrC) have been considered light-absorbing components of particulate matter and affect weather and climate. Biomass burning (BB) emission from Southeast Asia (SEA) is a key source of BC and BrC on the planet. In this study, the Weather Research and Forecasting-Community Multiscale Air Quality (WRF-CMAQ) two-way coupled model was used with the Global Fire Emissions Database Version 4, to investigate the direct radiative effect (DRE) of BC and BrC in March 2015 over SEA. The Rapid Radiative Transfer Model for the Global Circulation Model was employed in the WRF-CAMQ to calculate the aerosol optical properties in 14 shortwave spectral bands. Parameterization of the light absorption property of BrC described by Saleh et al. (2014) is coded and embedded into the WRF-CMAQ. The light absorption property of BrC is determined by the BB BC to organic carbon ratio in each grid and each time step, which is more in line with the smog chamber experiments compared to the originally fixed coefficient in the model. Experiments with and without BC/BrC DRE were conducted. Preliminary results show that the monthly mean DRE from BB BC can reach 18.3 W/m2 in the Indochina region and 3.0 W/m2 in southern China, decreasing the surface temperature by up to 0.2 and 0.1 °C, respectively. The monthly DRE from BB BrC can reach 1.3 W/m2 in the Indochina region but only around 0.1 W/m2 in southern China. Meanwhile, the maximum instant DRE of BrC can reach 10.0 W/m2, which is expected to exert a local synoptic scale influence.

How to cite: Huang, Y., Lu, X., Li, Z., Fung, J., and Wong, D.: Direct radiative effects of black carbon and brown carbon from Southeast Asia biomass burning with the WRF-CMAQ two-way coupled model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10734, https://doi.org/10.5194/egusphere-egu23-10734, 2023.

Fine particulate matter (PM2.5) pollution and its long-term exposure is one of the most critical environmental and public health risks in India, and has caused an enormous disease burden. However, the particle load is being shared from various sectoral contributions and a significant proportion found at any specific state would have originated from distant sources that are often outside the immediate jurisdiction and control of local authorities. This poses an injustice to some of the states which are emitting less emission but suffering from excess health burden. This study quantifies the burden apportionment under three model scenarios (baseline, advanced technology, and sustainable development) for the years 2015 and 2030, which forecast the future PM2.5 exposure based on current emission, and partial or full implementations of cost-effective interventions, as part of the Global Burden of Diseases, injuries, and Risk factor study. In 2030, the total excess mortality burden is projected to be 0.79-0.8 million (0.57-1.1) and DALYs burden of 24.1-24.3 million (16.6-30.4) from regional and sectoral emissions, respectively. Low SDI states would have a higher share in India. The state itself, outside, and neighbouring state emissions would be the leading contributors under the regional emission scenario; however, emissions from the secondary, power plant, high stack, transport and waste sectors would lead to higher burden apportionments in 2030. IHD, COPD, and type-2 diabetes would be the leading causes of health burden, especially in adults. The results add evidence for prioritizing sectors and efficacy for revising relevant environment standards and health policies. Immediate adaptation to the best available cost-effective modern technologies (SDS scenario) in households and commercial emission sectors is extremely necessary to reduce the substantial avoidable deaths and disease burden from this major environmental risk factor, improving the medical infrastructure and awareness in low and middle SDI states that are commensurate with the magnitude of air pollution.

How to cite: Sarkar, D. and Dey, S.: Burden Apportionment of India: Prioritizing the Regional and Sectoral Emissions to Maximize the Health Benefit at Near Future, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10754, https://doi.org/10.5194/egusphere-egu23-10754, 2023.

EGU23-10884 | ECS | Orals | AS3.16

Dynamic ozone evaluation using a model intercomparison study for Germany. 

Markus Thürkow, Tim Butler, Florian Pfäfflin, Bernd Heinold, and Martijn Schaap

Air quality remains a key topic for human wellbeing worldwide. Ozone (O3) is still one of the most toxic and ecologically detrimental air pollutants in Europe and supplies a crucial impact factor for the air quality planning as millions of people are exposed to O3 levels above the WHO guidelines. The chemical reaction processes leading to the formation of ozone are well documented in literature for long: O3 is not emitted but rather formed through complex chemical reactions from precursor emissions such as nitrogen oxides or biogenic volatile organic compounds. Processes influencing ozone variability are highly sensitive to several meteorological parameters such as temperature, moisture or solar radiation. These processes can impact the emission rate of ozone precursors, the chemical production and destruction as well as the rate of ozone loss through dry deposition. The ambient air pollution for ozone is often assessed and forecasted using chemical transport models (CTMs). These CTMs aim to reproduce observed ozone variability as good as possible by comprehensively accounting the abovementioned processes.

To evaluate CTMs and identify directions for improvement multi-model intercomparison studies have proven very useful on the past. Often the ensemble mean or median shows a better model skill than the ensemble members. The quality of model (ensemble) results is normally assessed by calculating a number of statistical indicators in a paired comparison to measured timeseries. In addition, to assess the model quality and uncertainty one can use a dynamic evaluation. The dynamic evaluation relates the model error to input data such as the meteorology. The degree to which changes in ozone levels caused by varying meteorological conditions are then evaluated. This allows to assess whether numerical models can capture the chemical response to temperature, humidity or another meteorological parameter.

In this study we also make use of such an ensemble assessment to evaluate the multi-model performance and the skill for each ensemble member. We conducted air pollution simulations for four models (LOTOS-EUROS, REM-CALGRID, COSMO-MUSCAT and WRF-CHEM) across Germany for January 1st to December 31st, 2019. The models show a very consistent picture in the ranking of the model skill. Main differences between the four ensemble members we found for ozone episodes, the timing of daytime maxima or even the representation of the nighttime concentration. We further enhanced the understanding of the modelled ozone response to temperature and humidity and provided an in-depth understanding for differences occurring in the ozone production rates for all participating models separated by season and region. First results indicate main differences in the ozone productivity especially for warm and humid conditions during the ozone season. The COSMO-MUSCAT and REM-CALGRID models show largest variability for ozone production rates with respect to temperature and humidity. The overall best performance can be seen for LOTOS-EUROS and WRF-CHEM.

How to cite: Thürkow, M., Butler, T., Pfäfflin, F., Heinold, B., and Schaap, M.: Dynamic ozone evaluation using a model intercomparison study for Germany., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10884, https://doi.org/10.5194/egusphere-egu23-10884, 2023.

EGU23-11268 | Posters on site | AS3.16

Modelling of PM formation in cooling tower plumes 

Ralf Wolke, Kathrin Gatzsche, and Andreas Tilgner

The PM fraction in ambient air due to the formation of secondary inorganic sulphate and nitrate from the emissions of large lignite-fired power plants in Germany is investigated. The power plants are equipped with natural draft cooling towers. The flue gases are fed directly into the cooling towers, giving them an additional lift. The exhausted gas-steam mixture contains the gases CO, CO2, NO, NO2 and SO2, the directly emitted primary particles and additionally an excess of "free" sulphate ions in water solution, which are not neutralized by cations after the desulfurization stages.  The precursor gases NO2 and SO2 are capable of forming nitric and sulfuric acids by various routes. The acids can be neutralized by ammonia and produce secondary particulate matter by heterogeneous condensation on pre-existing particles.

The investigations are carried out with the regional chemical transport model COSMO-MUSCAT as well as with the air parcel model SPACCIM, with which multiphase chemical processes can be described in great detail. Possible formation pathways and dependencies, especially on pH and the meteorological situation, will be identified. The aim is also to estimate the maximum PM load in "worst case" scenarios. The metal ions released from the ash and the emitted fraction of "free" sulphate ions remaining in excess after the desulfurization steps play an important role.

How to cite: Wolke, R., Gatzsche, K., and Tilgner, A.: Modelling of PM formation in cooling tower plumes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11268, https://doi.org/10.5194/egusphere-egu23-11268, 2023.

EGU23-11352 | ECS | Orals | AS3.16

Impacts of meteorological biases on forecasting surface PM2.5 concentration over the Beijing-Tianjing-Hebei region 

Qiuyan Du, Chun Zhao, Jiawang Feng, Zining Yang, Jiamin Xu, Jun Gu, Mingshuai Zhang, Mingyue Xu, and Shengfu Lin

Forecast biases in the meteorological fields have long been recognized as the main limitation on accuracy and predictability of air quality forecast. However, the quantitative studies on the impacts of meteorological forecast biases on air quality forecast are insufficient, and its mechanisms in different seasons are still unclear. In this study, series of forecasts from 2-Day (24 ~ 48-hour) to 7-Day (144 ~168-hour) for January, April, July, and October of 2018 are conducted over the Beijing-Tianjing-Hebei (BTH) region and the impacts of meteorological forecast bias on surface PM2.5 concentration forecast at each leading-time are analyzed. The results show that the forecast biases of surface PM2.5 concentration caused by meteorological forecast biases keep increasing with the increasing leading-time in all seasons. The impacts of meteorological forecast biases are strongest in spring, with the forecast bias of PM2.5 concentrations up to 187% in the 7-Day forecast, followed by autumn (123%), summer (112%) and winter (80%). By the contribution analysis of relevant processes and their changes with the increase of leading-time, it is found that the dry deposition, transport and PBL mixing are the main processes contributing to the growth of forecast bias of surface PM2.5 concentrations. In addition, the correspondence between the contributions of relevant processes and the meteorological factor are examined. It is found that the changes of contributions of processes are closely related to the difference in the forecasted meteorological factors such as surface winds, wind fields at 850hPa, PBL height, shortwave radiation and precipitations at each leading-time. This study highlights the importance of meteorological forecast bias in surface PM2.5 concentration forecasting, and provides useful information for the improvement of air quality forecast accuracy and supports the policies of air pollution controlling.

How to cite: Du, Q., Zhao, C., Feng, J., Yang, Z., Xu, J., Gu, J., Zhang, M., Xu, M., and Lin, S.: Impacts of meteorological biases on forecasting surface PM2.5 concentration over the Beijing-Tianjing-Hebei region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11352, https://doi.org/10.5194/egusphere-egu23-11352, 2023.

The Ensemble Kalman Filter (EnKF) has been employed for updating the initial condition, and promising results have been reported. Unlike the variational assimilation method, the advantages of EnKF are flow-dependent background error covariance which is important in a fast-developing air quality system. However, assimilation of air quality observations often suffers from insufficient model background error due to a small ensemble spread when applying EnKF methods. This study suggests methods for effectively increasing model background error covariance (BEC) by perturbing prognostic variables and employing multiple physics parameterizations in the atmospheric chemical transport model.

This study developed an aerosol data assimilation system with the WRF-Chem model and EnKF approach. In spite of considering flow-dependent BEC, the baseline run analysis exhibits poor performance, primarily due to the small ensemble spread. This study conducted new two effective methods for increasing ensemble spread: one considering the uncertainty of model physics and the other considering the uncertainty in the prognostic variables. Both methods improved the quality of surface PM analysis substantially, compared with the baseline run. And the DA_all experiment which incorporates both uncertainty in model physics and prognostic variables, demonstrates the best performance. Physical perturbation and multiplicative perturbation have a non-linear relationship. The forecast skill is also improved. With the substantial increase of BEC, the revised EnKF system has significantly improved the PM2.5 forecast skills.

How to cite: Lee, S. and Lee, M.-I.: Effective Methods for Increasing Model Background Error in the Ensemble Kalman Filtering in Aerosol Data Assimilation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11371, https://doi.org/10.5194/egusphere-egu23-11371, 2023.

The influence of sub-grid particle formation (SGPF) in point source plumes on aerosol particles over eastern China was firstly illustrated by implementing a SGPF scheme into a global-regional nested chemical transport model with aerosol microphysics module. The key parameter in the scheme was optimized based on the observations in eastern China. With the parameterization of SGPF, the spatial heterogeneity and diurnal variation of particle formation processes in sub-grid scale were well resolved. The SGPF scheme can significantly improve the model performance in simulating aerosol components and new particle formation processes at typical sites influenced by point sources. The comparison with observations at Beijing, Wuhan, and Nanjing showed that the normal mean bias (NMB) of sulfate and ammonium could be reduced by 23%-27% and 12%-14%, respectively. When wind fields were well reproduced, the correlation of sulfate between simulation and observation can be increased by 0.13 in Nanjing. Considering the diurnal cycle of new particle formation, the SGPF scheme can greatly reduce the overestimation of particle number concentration in nucleation and Aitken mode at night caused by fixed-fraction parameterization of SGPF. In the regional scale, downwind areas of point source got an increase of sulfate concentration by 25%-50%. The results of this study indicate the significant effects of SGPF on aerosol particles over areas with the point source and necessity of reasonable representation of SGPF processes in chemical transport models.

How to cite: Wei, Y. and Chen, X.: Investigating the importance of sub-grid particle formation in point source plumes over China using chemical transport model with a sub-grid parameterization, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11675, https://doi.org/10.5194/egusphere-egu23-11675, 2023.

EGU23-11932 | ECS | Posters on site | AS3.16

Parametrization of temporal emission variability for greenhouse gases and air pollutants 

Ilona Jaekel, Sabine Banzhaf, Edward Chan, Richard Kranenburg, Stijn Dellaert, and Martijn Schaap

The basis for modelling greenhouse gases and air pollutants is an explicit spatially and temporally resolved specification of the anthropogenic emissions. Although a lot effort has been put in to improve the spatial allocation for emission inventories, the temporal variability for many sectors is not aligned with real-world conditions and often prescribed using static or constant time profiles. We have been developing a modelling system to predict the spatial-temporal behaviour of anthropogenic emissions of air pollutants and greenhouse gases in which we aim to also include the influence of e.g. meteorological conditions on activities and emission factors. As such, we are replacing the static emission profiles with parametrizations one by one. Here, we present the approaches we are taking for 3 sectors. First, for large power plants the point source metadata of the CAMS-REG inventory have been matched to those from the ENTSO-E database to link the hourly production statistics to the emission inventory. Next, we tried to group the production time series of the different kinds of power plants, but this turned out not to be possible as they show very specific profiles. It was affordable to include for each power plant its individual emission time profile into the emission model. Second, for small stationary combustion the temporal variability is calculated for two building types, i.e. office and residential buildings, using the heating degree day method for oil and gas. For residential wood and coal combustion additional constraints with respect to heating behaviour have been applied. Third, for methane emissions from landfills we based our parametrization on investigations showing a significant pressure dependency of the emission flux. The original (constant) emission profile is exchanged with a profile which is spatially and temporally dependent on the change of atmospheric pressure, which leads to a variability of a factor 4 around the annual mean flux. Given the impact of synoptic variability the behaviour shows comparable patterns across large regions. At the meeting we will also show our planned approach to detail the emission variability of methane and PM from the agricultural sector (enteric fermentation, livestock housing and land management).

How to cite: Jaekel, I., Banzhaf, S., Chan, E., Kranenburg, R., Dellaert, S., and Schaap, M.: Parametrization of temporal emission variability for greenhouse gases and air pollutants, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11932, https://doi.org/10.5194/egusphere-egu23-11932, 2023.

EGU23-12152 | ECS | Orals | AS3.16

Large-eddy simulation of air quality in Hong Kong 

Yuting Wang, Yong-Feng Ma, Guy Brasseur, and Tao Wang

To perform realistic high-resolution air quality modeling in a polluted urban area, the WRF (Weather Research and Forecasting) model was used with an embedded large-eddy simulation (LES) module and with online chemistry. As an illustration, the numerical experiment was conducted in the polluted megacity of Hong Kong, which is characterized by multi-type pollution sources as well as complex topography. The multi-resolution simulations from mesoscale to LES scales were evaluated by comparing the calculated fields with ozone sounding profiles and with the observations at surface monitoring stations. The comparison shows that both mesoscale and LES simulations reproduced well the mean concentrations of the chemical species and their diurnal variations at the background sites; however, the mesoscale simulations largely underestimated the NOXconcentrations and overestimated O3 near roadside stations due to the coarse representation of the traffic emissions. The LES simulations improved the agreements with the measurements near the road traffic, and the LES with highest spatial resolution (33 m) provided the best results. The LES simulations showed more detailed structures of the spatial distributions of chemical species than the mesoscale simulations, indicating the capability of LES of resolving high-resolution photochemical transformations in urban areas like Hong Kong. The LES simulations showed similar trends with the mesoscale model in the evolution of the profiles of the chemical species with the development of the boundary layer over a diurnal cycle. The vertical fluxes of the chemical species are stronger in the 33 m LES than the 100 m LES, because the high-resolution LES can better resolve the turbulent eddies.

How to cite: Wang, Y., Ma, Y.-F., Brasseur, G., and Wang, T.: Large-eddy simulation of air quality in Hong Kong, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12152, https://doi.org/10.5194/egusphere-egu23-12152, 2023.

EGU23-12276 | Posters on site | AS3.16

Intercomparison of black carbon emissions from biomass burning using FLEXPART-WRF and ground-based observation in Alaska 

Masayuki Takigawa, Fumikazu Taketani, Yugo Kanaya, Hideki Kobayashi, Takeshi Kinase, Chunmao Zhu, and Yongwon Kim

Black carbon aerosols (BC) are emitted into the atmosphere by incomplete combustion processes of fossil fuels and biomass. Especially in the Arctic region, anthropogenic emissions from mid-latitudes (e.g., China) are transported by large-scale atmospheric circulation, and local emissions such as forest fires in boreal forests and gas flares are also considered to contribute significantly. In this study, we report on the result of intercomparison for Poker Flat, Alaska, especially focusing on the biomass burning emission inventories, which still show large differences among the inventories.

Since April 2016, observations of BC and CO have been conducted at the Poker Flat Research Range (PFRR; 65.12°N, 147.49°W) in cooperation with the University of Alaska Fairbanks. The pathways of air parcels that were observed at PFRR were estimated using the Lagrangian particle diffusion model FLEXPART-WRF version 3.3. Backward calculations were performed for 20 days using 40,000 particles every 6 hours from April 2016 to December 2020. The meteorological field was calculated by a regional meteorological model (WRF) covering the Northern Hemisphere. The concentration and source attribution has been estimated using the residence time estimated by FLEXPART-WRF and emissions at each grid. ECLIPSEv6 and 6 different inventories (FINNv1,5 FINNv2.5(MODIS, MODIS+VIIRS), GFEDv4.1a, GFASv1.2, QFEDv2.5r1, FEERv1.0-G1.2) are used as the anthropogenic and biomass burning emissions, respectively.

The concentration in the wintertime was generally well reproduced by the model, and it was estimated that anthropogenic emissions in Alaska (especially domestic and transport sectors in ECLIPSEv6) were dominant in that period. It was also found that there were very large differences in the contribution of biomass burning among inventories, especially in summer when the forest fires are active. Among them, GFEDv4.1 generally succeeded in capturing large fire events, especially in 2017 and 2019 (r=0.93). FINN inventories (version 1.5, version 2.5 with MODIS, and MODIS+VIIRS) tended to underestimate such eventual increases. In contrast, QFED sometimes overestimated concentrations at large events. If we assume the ‘event period’ as observed BC concentration exceeds the 95 percentiles for the whole period, the contribution of biomass burning was estimated to be higher at the event period (47%) than that during the non-event period (22%) in the simulation with GFEDv4.1.

How to cite: Takigawa, M., Taketani, F., Kanaya, Y., Kobayashi, H., Kinase, T., Zhu, C., and Kim, Y.: Intercomparison of black carbon emissions from biomass burning using FLEXPART-WRF and ground-based observation in Alaska, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12276, https://doi.org/10.5194/egusphere-egu23-12276, 2023.

EGU23-12311 | Orals | AS3.16

Applying space-time activity data and socio-economic profiles to assess the variation of personal air pollution exposures 

Oliver Schmitz, Kees de Hoogh, Nicole Probst-Hensch, Ayoung Jeong, Benjamin Flückiger, Danielle Vienneau, Gerard Hoek, Kalliopi Kyriakou, Roel C. H. Vermeulen, and Derek Karssenberg

Long-term personal air pollution exposures estimates from nationwide cohorts are useful in studies of the relationship between air pollution exposure and chronic diseases such as diabetes or cardiovascular disease. Ignoring space-time activity patterns and neglecting mobility in exposure assessment may lead to incorrect exposure distributions and bias in downstream exposure health relations. In our study we estimate personal air pollution exposures nationwide and across socio-economic and age profiles to identify the relevance of location or profiles on exposure analysis.

We developed a set of characteristic diurnal activity profiles that we use to calculate exposures for each home address in Switzerland. The profiles are specified by different characteristics such as age group, social economic status, or commute type (e.g. by car, bicycle, on foot). Potential working locations are retrieved from origin-destination matrices for a particular profile, derived from the annual Structural Survey data from the Swiss Population Census (https://www.bfs.admin.ch/bfs/en/home/statistics/population/surveys/se.html), at the level of municipalities. Commute trips between residential and work location are then calculated using the shortest route on OpenStreetMap data. For each profile and each residential address, we run an agent-based model in Monte Carlo mode, generating a database of personal long-term exposures to NO2 and PM2.5 for further epidemiological analysis.

Our activity-based mobility simulation provides a representative description of space-time activities of individuals. We present the model results at all unique 1.8 million residential address locations in Switzerland. We compare the exposure assigned from residential address alone to the exposures derived from 20 different activity profiles and present the differences between profiles. We also demonstrate the spatial variability of exposures per profile and the associated uncertainty.

The generated exposure database can be used for epidemiological analysis of large-scale cohorts, and enables follow-up studies to evaluate whether including commuting and other activities and therefore more detailed estimates of individual exposure results in more accurate risk estimates in health studies.

How to cite: Schmitz, O., de Hoogh, K., Probst-Hensch, N., Jeong, A., Flückiger, B., Vienneau, D., Hoek, G., Kyriakou, K., Vermeulen, R. C. H., and Karssenberg, D.: Applying space-time activity data and socio-economic profiles to assess the variation of personal air pollution exposures, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12311, https://doi.org/10.5194/egusphere-egu23-12311, 2023.

EGU23-12861 | Orals | AS3.16

Ozone source apportionment with a tagging approach in the LOTOS-EUROS model 

Martijn Schaap, Richard Kranenburg, Markus Thuerkow, Aura Lupascu, and Tim Butler

As the majority of the population is exposed to air pollutant levels above the WHO guidelines, poor air quality remains one of the key challenges to increase human wellbeing in Europe. To further improve the ambient air quality it is important to know the extent to which the different anthropogenic activities contribute to the population exposures of particulate matter, nitrogen oxides and ozone. Source attribution is a process of tracing pollution levels back to its origin. Within the LOTOS-EUROS chemistry transport model a labelling technique has been developed and applied extensively for particulate matter and nitrogen oxides. So far, ozone source apportionment was not available.

The existing labelling approach was extended for ozone inspired by the implementation of the TOAST module in WRF-CHEM (Lupascu and Butler, 2019). We implemented an additional labelling family for the Ox family. For all reactions in which NO is oxidized to NO2 by a peroxide (RO2 or HO2) the NO2 produced in the Ox family receives the origin of the NO from the NOy family. By capitalizing on the existing labelling modules of LOTOS-EUROS we benefit from the more efficient implementation than simply increasing the number of tracers in the chemical mechanism.     

The new implementation was applied for the year 2019 by adopting zooming approach with a European domain and a higher resolution nest across northwestern Europe. Evaluation against measurements shows that the model is well capable to reproduce the observed variability across the country. During winter time in northwestern Europe the regional background ozone levels are largely determined by influx from the hemispheric background. Regional production from road transport and other combustion sources are important from July to September, whereas increased levels during spring show considerable contributions from ozone formed in southern Europe. To investigate in how far two modelling systems agree or deviate from each other in terms of source apportionment, simulations with LOTOS-EUROS and WRF-CHEM with a consistent model setup and labelling strategy were performed. The results of this analysis will also be shown at the meeting.

 

Lupaşcu, A. and Butler, T.: Source attribution of European surface O3 using a tagged O3 mechanism, Atmos. Chem. Phys., 19, 14535–14558, https://doi.org/10.5194/acp-19-14535-2019, 2019

How to cite: Schaap, M., Kranenburg, R., Thuerkow, M., Lupascu, A., and Butler, T.: Ozone source apportionment with a tagging approach in the LOTOS-EUROS model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12861, https://doi.org/10.5194/egusphere-egu23-12861, 2023.

EGU23-12878 | ECS | Orals | AS3.16

European modeling of atmospheric copper, iron and manganese as key players for aerosol toxicity 

Nicolas Dubois, Gilles Foret, Matthias Beekmann, Guillaume Siour, Matthieu Vida, Jean-Marc Andre, Sophie Moukhtar, Gaelle Uzu, Jean-Luc Jaffrezo, Sébastien Conil, Lise Le Berre, Nicolas Marchand, Benjamin Chazeau, Grégory Gille, Andres Alastuey, Xavier Querol, Cristina Reche, Stéphane Socquet, Clément Bret, and Mario Duval

Exposure to air pollution, especially aerosols, can lead to adverse health effects. Particle toxicity has been generally linked to its mass concentration. However, toxicity is determined by the chemical composition of the aerosol, which varies greatly depending on pollution sources. Reactive oxygen species (ROS) can be formed in the lung when particles are inhaled and can trigger inflammatory processes. Transition metals strongly contribute to ROS, among which copper, iron and manganese. However, these metals are generally not included in current emission inventories and chemistry-transport models. Thus, to ultimately model aerosol toxicity, it would be necessary to add these three metals into a chemistry-transport model, and use it to provide inputs to a lung chemistry model (Lelieveld et al, 2021).

Country-wise copper emissions are available from the EMEP database (https://www.ceip.at/) for the majority of European Union countries. Methods for evaluating emissions differ from country to country, and it is necessary to homogenize them to standardize emissions, at least for the main emitting countries around France which is the main target of the study. For iron and manganese, European scale inventories do not exist yet. Data from the French Citepa and ADEME, from EMEP reports, SPECIEUROPE and a bibliography of 16 references were used to build these two bottom-up inventories. Many sources have been studied: abrasion of tires, brakes and road for the road transport sector, wear of catenaries, brakes and rails for the rail sector, combustion of coal, biomass and of petroleum, the burning of motor oils, and the incineration of waste.

Also, long term measurements from several dozens of rural, urban and traffic sites were collected to build a large database. These data come from EBAS website (https://ebas-data.nilu.no/), UKAIR website (https://uk-air.defra.gov.uk/data/), CARA program (Favez et al., 2021), the Spanish IDAEA and the French Atmo Auvergne-Rhône-Alpes and Marseille-Longchamp. Fe/Cu and Mn/Cu ratios were calculated for both the bottom-up emission inventories and measurements data. As these ratios turned out to be significantly lower in emission inventories, observed ratios were used to adjust Fe and Mn emissions from Cu ones.

Using these two inventories, emission ratios with coarse particles for each country and sector were created and applied to the spatialized particles emission data. We then implemented the obtained spatialized Cu, Fe and Mg emission inventories into the CHIMERE chemistry-transport model, to simulate ambient copper, iron and manganese mass concentrations in Europe for the year 2014.

How to cite: Dubois, N., Foret, G., Beekmann, M., Siour, G., Vida, M., Andre, J.-M., Moukhtar, S., Uzu, G., Jaffrezo, J.-L., Conil, S., Le Berre, L., Marchand, N., Chazeau, B., Gille, G., Alastuey, A., Querol, X., Reche, C., Socquet, S., Bret, C., and Duval, M.: European modeling of atmospheric copper, iron and manganese as key players for aerosol toxicity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12878, https://doi.org/10.5194/egusphere-egu23-12878, 2023.

EGU23-12970 | ECS | Orals | AS3.16

Validation of a WRF-Chem setup aiming aerosol-radiation-cloud interactions studies over the Iberian Peninsula 

Rui Silva, Ana Cristina Carvalho, David Carvalho, and Alfredo Rocha

In an ever-growing demand for solar energy production and technologies, atmospheric aerosols pose a great challenge for solar power suppliers due to their high spatio-temporal variability, their direct influence on the scattering and absorption of the incoming solar radiation, and their role as cloud condensation nuclei, indirectly affecting cloud formation and precipitation. Hence, atmospheric aerosols are a preponderant element of an accurate weather and solar forecasting system. Located in Southwestern Europe, the Iberian Peninsula (IP) represents one of the regions with the highest solar power potential in Europe, but it is frequently affected by forest fires and high-concentration dust episodes with their origin in the major African deserts during the warmer months. In this study, a model setup using the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) is evaluated during an extreme dust episode that affected the IP in August 2010, aiming to perform aerosol-radiation-cloud interactions studies over the region. Model results, such as particle concentration and aerosol optical properties, are compared against different in-situ observations and remote sensing data from regional air quality stations and from the Aerosol Robotic Network (AERONET) to assess the model performance under these kinds of events.

How to cite: Silva, R., Carvalho, A. C., Carvalho, D., and Rocha, A.: Validation of a WRF-Chem setup aiming aerosol-radiation-cloud interactions studies over the Iberian Peninsula, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12970, https://doi.org/10.5194/egusphere-egu23-12970, 2023.

EGU23-13814 | ECS | Orals | AS3.16

Hourly LUR modeling of hyperlocal NO2 using mobile monitoring data 

Zhendong Yuan, Jules Kerckhoffs, Youchen Shen, Gerard Hoek, and Roel Vermeulen

BACKGROUND:

Distinguished from the real-time forecast task, the hourly mapping in this work stands for spatiotemporal interpolations of long-term (e.g., annual) average concentrations of air quality in hourly intervals. These long-term-averaged hourly maps facilitate environmental epidemiology studies by enabling dynamic environmental exposures assessment based on human time activities. Over the past decade, several mobile campaigns have been conducted where high-frequency sensors were mounted on vehicles roaming around the entire studied region. Since not all locations can be measured repeatedly for every hour, there are rarely previous studies using opportunistic mobile measurements to reconstruct long-term NO2 hourly maps. In this work, we evaluated the merit of land-use regression (LUR) models that use mobile measurements paired with land-use and traffic predictors to interpolate hourly air pollution concentrations at fine spatial resolutions.

METHOD:

We monitored 1-second NO2 concentrations in Amsterdam with two Google StreetView cars, from 8:00 to 20:00 on weekdays from May 2019 to March 2020 (5.7 Million measurements). These measured GPS points were aggregated into 50m road segments and divided into one-hour intervals. Using this hourly mobile data as the response, we explored two spatiotemporal LUR models, namely ST-Kriging (the spatiotemporal version of kriging methods) and GTWR (Geographical and Temporal Weighted Regression), and two spatial LUR models implemented separately in each hour, namely RF_LUR (a LUR model based on the random forest) and LSR (Stepwise Linear Regression). Model performance was assessed by averaging measurements over the same period collected from independent routine monitoring stations in Amsterdam (RIVM, n=9).

RESULT:

The hourly averaged mobile measurements of NO2 across the city varied from 40 (rush hours) to 28 ug/m3 (non-rush hours). Routine measurements (RIVM) showed significantly different patterns in road types (major vs residential roads) and seasons (winter vs summer). Therefore, the spatiotemporal models were trained separately for these four scenarios and then merged their predictions into the final maps. GTWR captured more accurate spatiotemporal correlations than Kriging methods under the limitation of opportunistic mobile data and temporally static covariates (ST-Kriging: R2 = 0.35, MAE, RMSE = 9.46, 12.14 ug/m3, GTWR: R2 = 0.50, MAE, RMSE = 6.07, 7.64 ug/m3). Better overall accuracy and more smoothing distributions in both space and time were captured by the spatiotemporal models as compared to spatial models separated in each hour (LSR: R2 = 0.47, MAE, RMSE = 6.48, 8.04 ug/m3; RF_LUR: R2 = 0.33, MAE, RMSE = 10.33, 14.74 ug/m3). The spatiotemporal distribution of NO2 predictions was found to strongly follow the intra-urban commuting pattern.

 CONCLUSION:

The spatiotemporal LUR model is able to capture spatiotemporal correlations hidden in opportunistic mobile measurements. The reconstructed spatiotemporal maps can be broadly applied to estimate human exposure to NO2 considering time-activity patterns.

How to cite: Yuan, Z., Kerckhoffs, J., Shen, Y., Hoek, G., and Vermeulen, R.: Hourly LUR modeling of hyperlocal NO2 using mobile monitoring data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13814, https://doi.org/10.5194/egusphere-egu23-13814, 2023.

EGU23-14483 | ECS | Posters on site | AS3.16

Prediction of H2S Concentration Around Geothermal Power Plants Using Multiple Regression Analysis 

Merve Aydin and Burcak Kaynak

Investments in geothermal resources are growing worldwide with a view of being clean and sustainable, however it may also have negative impacts on air quality, ecosystem and health. Geothermal resources are used in different areas such as power generation and direct use including heating, thermal use, greenhouse and drying activities. The electricity production from geothermal power plants (GPPs) is closely associated with hydrogen sulfide (H2S) emissions negatively affecting ecosystems at certain concentrations and exposure. H2S is oxidized to SO2 after released to the atmosphere at a rate depending on temperature, sunlight and radicals.

Turkey has been ranked 4th worldwide in terms of electricity generation from GPPs with a total capacity of 1676 MW in 2021. With recent legal restrictions about GPPs, additional H2S measurements were started recently along with criteria air pollutants at selected air quality monitoring stations (AQMSs) in regions with GPPs in Turkey. Our preliminary result showed a significant correlation via exploratory data analysis between H2S and SO2 measurements in 2021 from one of these AQMSs. The wind speed and direction analysis showed these air pollutants were transported from the same directions coinciding with GPP locations. This study aims to analyze the relationship between H2S and SO2 in GPP regions in southwestern Turkey. The study area focuses on four regions specified according to GPP locations and H2S measuring AQMS locations along with SO2 measurements. Time period includes 2021-22 with ground-based H2S, ground and satellite-based SO2, ground-based meteorology measurements as well as other related parameters such as topography, GPP locations and capacities. There are peaks observed in H2S concentrations around noon at all seasons for three regions, at similar times SO2 concentrations usually peak as well. The Pearson correlations (R) between daily H2S and SO2 measurements are 0.76, 0.60, 0.46 and 0.42 for four regions. Correlations between H2S and SO2 measurements at lag times using 1-hr and 6-hr moving averages showed higher correlations with 6-hr moving averages indicating H2S to SO2 conversion. SO2 satellite retrievals are also investigated around these regions on these days when H2S was the highest. These findings strengthen our hypothesis of SO2 in the region being from the oxidation of H2S released from GPPs.

A linear model based on multiple regression analysis is developed using H2S as a dependent variable and other parameters as independent variables for understanding the levels of H2S in the region. Principal component analysis (PCA) approach is used to understand the importance and contribution of the selected parameters. This model will be used to predict H2S concentrations, because H2S measurements are not continuous and mandatory in the whole region. Moreover, the spatial distribution of H2S will be investigated for the region to understand the negative impacts on human health, ecosystems, and agriculture.

Keywords: Geothermal Power Plants, H2S, MRA

How to cite: Aydin, M. and Kaynak, B.: Prediction of H2S Concentration Around Geothermal Power Plants Using Multiple Regression Analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14483, https://doi.org/10.5194/egusphere-egu23-14483, 2023.

EGU23-14559 | ECS | Orals | AS3.16 | Highlight

Extreme Compound Events of Air Pollution and Effects on European Mediterranean Cities 

Francisco Sánchez-Jiménez, Eloisa Raluy-López, Leandro Segado-Moreno, Ester García-Fernández, Juan Pedro Montávez, and Pedro Jiménez-Guerrero

Air pollution is a significant concern for society due to its negative impact on human health. The ability to forecast pollutant concentrations and predict extreme pollution events is essential for mitigating their harmful effects. These events are commonly presented as compound and can have serious consequences (Zscheischler et al., 2020) for public health, making it important to identify and understand the variables that contribute to them.

In this study, we used state-of-the-art techniques based on artificial intelligence and machine learning methodologies to analyze data from a selection of European Mediterranean cities in order to identify the meteorlogical and preceding pollution variables that best explain extreme pollution events involving PM10, O3and NO2. Furtheremore, the role of the combined effect of these variables and recent climatic conditions is also examined on excess mortality rates using the likelihood multiplication factor parameter (Ridder et al., 2020) as well as the importance given by Random Forest Regression  Models.

Our results show that these events show a clear compound nature, understanding the non-linearity changes in the intensity of compound events. The main driver factors depend on the pollutant specie as well as the season of the year.

 

References
Ridder N. N., Pitman A. J., Westra S., Ukkola A., Do H. X., Bador M., Hirsch A. L., Evans J. P., Di Luca A., Zscheischler J. (2020). Global hotspots for the occurrence of compound events. Nature communications 11(1), 1–10.
Zscheischler J., Martius O., Westra S., Bevacqua E., Raymond C., Horton R. M., van den Hurk B., AghaKouchak A., Jézéquel A., Mahecha M. D., et al. (2020). A typology of compound weather and climate events. Nature reviews earth & environment 1(7), 333–347.

How to cite: Sánchez-Jiménez, F., Raluy-López, E., Segado-Moreno, L., García-Fernández, E., Montávez, J. P., and Jiménez-Guerrero, P.: Extreme Compound Events of Air Pollution and Effects on European Mediterranean Cities, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14559, https://doi.org/10.5194/egusphere-egu23-14559, 2023.

EGU23-14689 | ECS | Orals | AS3.16

GHOST: A globally harmonised dataset of surface atmospheric composition measurements 

Dene Bowdalo, Sara Basart, Marc Guevara, Oriol Jorba, and Carlos Pérez García-Pando

A critical measure for our understanding of the complex non-linear processes which determine atmospheric composition is through the use of Chemical Transport Models and Earth System Models. In order to evaluate the veracity of these models, observations are required, however the availability and quality of these observations serves as a major impediment to this process. The most temporally consistent measurements have been made at the surface by established measurement networks, typically for the purpose of monitoring local exceedances of air quality limits. There are multiple networks which report this data, in disparate formats, requiring harmonisation to allow for synthesis.

On the occasion that evaluation efforts use data from multiple networks, there is typically little to no detail given about the methodology used for the data synthesis across the different networks, or regarding the quality assurance (QA) or station classifications employed to subset the data. Therefore, evaluation efforts across different research groups are often incomparable.

As a response to this common challenge, we established GHOST (Globally Harmonised Observational Surface Treatment). GHOST can be succinctly stated as an effort to standardise the data / metadata from the major public reporting networks which provide in situ atmospheric measurements at the surface. In total the dataset comprises of ~20 billion processed measurements, for ~200 components, across 32 networks, from 1970 to 2022. This represents the biggest collection of harmonised atmospheric composition surface measurements ever composed. 

Substantial efforts have been made towards standardising almost every facet of provided data / metadata from across the networks. On top of this, additional metadata was added by processing various commonly utilised globally gridded datasets (e.g. land use), as well as adding temporal classifications per measurement (e.g. weekday / weekend). As the dataset spans many decades, metadata is handled dynamically and allowed to vary through the record, important for instances when there are changes in measurement instrumentation or the measurement position.

Major efforts were made for the standardisation of the numerous metadata fields detailing measurement procedures, with all measurements linked to a dictionary of standard measurement methods and standard instruments. Great effort was also spent in the standardisation of station classifications, providing large flexibility for the subsetting of stations. Rather than dropping any measurements which are labelled as potentially erroneous by the measurement provider, standardised data flags are associated with each individual measurement. On top of this, GHOST own QA flags are also associated per measurement.

All data is now freely available to the community.

How to cite: Bowdalo, D., Basart, S., Guevara, M., Jorba, O., and Pérez García-Pando, C.: GHOST: A globally harmonised dataset of surface atmospheric composition measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14689, https://doi.org/10.5194/egusphere-egu23-14689, 2023.

EGU23-14890 | ECS | Orals | AS3.16

Estimation of exhaust emissions of inland shipping - a case study on German waterways 

Daniel Weber, Hauke Stachel, Michael Schröder, and Christian Noss

Traffic is a significant contributor to anthropogenic air pollution. Although inland shipping constitutes only a small part of the total traffic and transports cargo very energy-efficient, inland vessels emit not negligible amounts of pollutants like nitrogen oxides and particulate matter. In order to quantify the contribution of inland transportation to the air pollution as well as to develop necessary strategies to mitigate current emissions, exact knowledge about vessel-born emission rates along waterways are required.

A mechanistic model has been developed to simulate fuel demand and emission rates of inland vessels with high temporal and spatial resolution. It links ship positions reported in the signals of the Automatic Identification System (AIS) with representative emission factors of inland vessel engines. The resistance, propulsion and brake power are calculated for each point of a vessel’s trajectory. Emission rates for quasi steady-state estimations of the brake power will be obtained via power-related emission factors. The integral of a large number of these point values ​​provides a quantification of inland shipping emissions along a waterway, e.g., in section-related emission rates.

This new model was applied on relevant German inland waterways. We present current exhaust emission rates and an example for a simulation to evaluate the mitigation potential of a modernized fleet.

How to cite: Weber, D., Stachel, H., Schröder, M., and Noss, C.: Estimation of exhaust emissions of inland shipping - a case study on German waterways, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14890, https://doi.org/10.5194/egusphere-egu23-14890, 2023.

EGU23-14938 | ECS | Orals | AS3.16 | Highlight

Modeling aviation’s air quality impacts over time in the context of the changing atmospheric composition 

Irene Dedoussi and Flávio Quadros

Aviation’s growth has historically outpaced technological and operational improvements to mitigate emissions. Despite the short-term slowdown due to COVID-19, the sector’s growth is forecast to resume in the coming years. Being a unique sector in terms of the altitude that the majority of the emissions are deposited in, aviation contributes to air pollution near and far from airports, in the form of PM2.5, ozone, and NO2, through a series of chemical and physical pathways. Aviation’s growth is heterogeneous globally, with emissions in some regions (e.g., Asia) growing faster than elsewhere (e.g., Europe and North America).

Using recent aviation emissions inventories and future forecasts, and the GEOS-Chem global atmospheric chemistry-transport model, we quantify aviation’s global air quality and associated human health impacts in recent years and under different future atmospheric pathways. Both emissions during landing and take-off operations and emissions during cruise are assessed in different regions globally. We isolate the air quality changes attributable purely to the growth of aviation emissions, and those associated with the evolving (background) atmospheric composition which affects the nonlinear pathways between aviation emission and air pollution formation. Given the long timelines associated with the aviation sector, our results highlight the need for the integrated assessment of present-day and future aviation impacts together with those of other evolving sources.

How to cite: Dedoussi, I. and Quadros, F.: Modeling aviation’s air quality impacts over time in the context of the changing atmospheric composition, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14938, https://doi.org/10.5194/egusphere-egu23-14938, 2023.

EGU23-15438 | ECS | Posters virtual | AS3.16

Modelling and prediction of daily, pan-European estimates of PM2.5 and PM10 based on Quantile Machine Learning applied to different mode Aerosol Optical Depth and reanalysis data 

Zhaoyue Chen, Raul Méndez, Hervé Petetin, Aleksander Lacima, Carlos Pérez García-Pando, and Joan Ballester

Among the different air pollutants, Particulate Matter (PM) poses a prominent threat to human health. In 2020, the exposure to PM2.5 (i.e. particles smaller than 2.5 micrometres in diameter) caused over 238,000 premature deaths in Europe, almost five times higher than the contribution from nitrogen dioxide, and ten times larger than ozone. Epidemiological studies for Europe generally rely on ground-level daily measurements to assess ambient PM exposures. However, the uneven distribution and discontinuous daily measurements of ground-level sites is a major constraint to develop large-scale, continental-wide epidemiological studies, biassing the results towards urban regions and areas with more ground-level sites.

In recent years, Aerosol Optical Depth (AOD) has increasingly become a useful alternative source of proxy data to estimate ground-level PM concentrations, because (i) AOD depicts the total column of aerosol in atmosphere, while PM depicts the surface aerosol, and (ii) its global spatiotemporal distribution can be easily obtained from satellites at high resolution. Despite the evident advantages, (i) the relationship between satellite AOD and PM is spatially heterogeneous, (ii) the number of missing data of satellite AOD is relatively high (up to 85% globally) due to cloudiness, and (iii)  the quality of measurements depends upon geographical factors like surface reflectivity. Europe is the one of the continents with lowest correlation between satellite AOD and PM concentration, so estimating PMs with satellite AOD in Europe becomes a great challenge. Furthermore, the components of AOD (fine and coarse-mode AOD, fAOD and cAOD respectively) are generally not available from satellite data. Thus, fewer studies used fAOD in the estimation of PM2.5, even when some studies found that fAOD is more highly associated with PM2.5.

Reanalysis data is another source to obtain available PM estimates,  (e.g., the PMs from Copernicus Atmosphere Monitoring Service Global Reanalysis (CAMSRA) and NASA’s Modern-Era Retrospective Analysis for Research and Applications v2 (MERRA-2)). However, they generally have lower resolution (on the order of 50-100 km) and have relatively large biases when it comes to the representation of surface pollution.

Here we downscaled and calibrated existing aerosol reanalysis, with the help of the AOD componental products (AOD and fAOD) generated in a previous study. To avoid the model  overfits in areas with dense monitoring sites (e.g., large cities), we used distance weighted loss functions (higher penalty weight on those places with fewer sites) to train the Quantile Machine Learning (QML) model. Then we predicted 18-year daily estimates and 95% predictive intervals for PM2.5 and PM10 at 10km resolution. In the model, we included atmosphere, land and ocean variables (e.g., boundary layer height, downward UV radiation, temperature, air pressure, humidity, cloud cover, local climate zone, leaf area index, surface reflectivity and road information). The results show that the out-of-sample r-squared (R2) of our PM2.5 and PM10 models is equal to 0.69 and 0.63, respectively, and largely outperform PM2.5 and PM10 estimates from CAMSRA (R2 = 0.25-0.35) and MERRA-2 (R2 = 0.22-0.33). Our approach provides more accurate PM estimates in Europe for the last 18 years, and opens new avenues for large-scale, high-resolution epidemiology studies.

How to cite: Chen, Z., Méndez, R., Petetin, H., Lacima, A., Pérez García-Pando, C., and Ballester, J.: Modelling and prediction of daily, pan-European estimates of PM2.5 and PM10 based on Quantile Machine Learning applied to different mode Aerosol Optical Depth and reanalysis data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15438, https://doi.org/10.5194/egusphere-egu23-15438, 2023.

Seasonal Variation of Simulated Carbonaceous Fine Particulate Matter over
the Indian Region by using WRF-Chem with two emission Inventories:

EDGAR-HTAP and SAFAR-2018

Praveen Kumar1

, Gufran Beig1,4, Vikas Singh2

, B.S. Murthy1

, B.R. Bamniya3

1
Indian Institute of Tropical Meteorology, Pune- 411008
2 National Atmospheric Research Laboratory, Gadanki, AP-517112
3Mohan LalSukhadiya University, Udaipur, 313001

4National Institutes of Advanced Studies (NIAS), Indian Institute of Science (IISc) Campus,

BANGALORE-560012

Abstract:

This study better evaluates Black Carbon (BC) using Weather Research and Forecasting model
coupled with chemistry (WRF-Chem) v3.9.1.1, with newly developed emission inventory
SAFAR-2018 and global one EDGAR-HTAP for the year 2018. The simulation provides a view
of the seasonal and regional pattern BC concentrations, confirmed by comparing surface
meteorological parameters and BC concentrations to the MERRA reanalysis for the Indian
region. It found that the model simulated surface C-PM concentration with SAFAR-2018
emission inventory is slightly overestimated, but simulation with EDGAR emission inventory is
under-estimated than MERRA. It also found that the model-simulated meteorological parameters
( e.g., wind speed at 2 m, the surface temperature at 2 m, and Planetary Boundary Layer height
showed better agreement with observation. Compared to the simulation with EDGAR emission
inventory, simulated geographic patterns of seasonal mean BC with SAFAR-2018 emission
inventory exhibit good agreement with MERRA. In the IGP region, the concentration of BC
showed the highest peak during the winter, followed by the post-monsoon season compared to
other subcontinents of India. The correlation coefficients of annual hourly time series of surface
BC_sf (SAFAR-2018 emission) concentrations with MERRA over India were higher (0.92) with
RMSE 0.45. These correlations were higher than those (EDGAR emission) observed for the
surface BC_ed (R = 0.91 & RMSE = 0.48) concentrations. It appears that model simulation with
SAFAR-2018 emission inventory well-captured pattern and magnitude over the Indian region,
increasing magnitude of BC concentrations may help to quantify better the effect on climate and
atmospheric condition over the Indian region.

How to cite: Kumar, P.: Seasonal Variation of Simulated Carbonaceous Fine Particulate Matter overthe Indian Region by using WRF-Chem with two emission Inventories:EDGAR-HTAP and SAFAR-2018, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15761, https://doi.org/10.5194/egusphere-egu23-15761, 2023.

EGU23-15843 | Orals | AS3.16

Aviation-induced changes of atmospheric composition in the UTLS in the multi-scale Earth system model MECO(1) 

Sigrun Matthes, Anna-Leah Nickl, Patrick Peter, Mariano Mertens, Patrick Jöckel, Helmut Ziereis, Theresa Harlaß, and Andreas Zahn

Aviation is concerned by its climate effects which results from CO2 and non-CO2 effects, comprising NOx-induced changes of atmospheric ozone and methane. Here climate-chemistry models are required to advance our understanding on induced changes of reactive species and the associated radiative forcing associated to aviation emissions. Evaluation of such comprehensive models is key in order to be able to investigate associated uncertainties can use observational datasets from research infrastructures like IAGOS and DLR aircraft measurement campaign data.

We use the MECO(n) system which is a “MESSy-fied ECHAM and COSMO nested n-times”, relying on the Modular Earth Submodel System (MESSy) framework. For this purpose, both models have been equipped with the MESSy infrastructure, implying that the same process formulations (MESSy submodels) are available for both models. Modelled atmospheric distributions from the multi-scale model system MECO(n) are systematically compared to observational data from aircraft measurements in the upper troposphere and lower stratosphere. Nudging of meteorology to reanalysis data, and special diagnostics available within the modular MESSy infrastructure are implemented in the numerical simulations. Online sampling along aircraft trajectories allows to extract model data with a high temporal resolution (MESSy submodel S4D), in order to evaluate model representation and key processes. Beyond systematic evaluation with IAGOS scheduled aircraft measurements, particular focus on those episodes where dedicated measurements from aircraft campaigns are available. We present an analysis of reactive species, NOy and ozone, which also identifies those weather pattern and synoptic situations where aviation contributes strong signals. We evaluate model representation of the NOx-induces effect on radiatively active species ozone and hydroxyl radical in both model instances, ECHAM5 and COSMO. This is key for advancing the scientific understanding of NOx-induced effects from aviation non-CO2 effects required in order to quantify potential compensation and trade-offs and eventually in order to identify robust mitigation options for sustainable aviation.

This project has received funding from the European Union’s Horizon 2020 research and innovation programme under grant agreement No 875036 (ACACIA, Advancing the Science for Aviation and Climate) and has been supported by the DLR-Projekt Eco2Fly. This work uses measurement data from the European Research Infrastructure CARIBIC/IAGOS. High-Performance Super Computing simulations have been performed by the Deutsches Klima-Rechenzentrum (DKRZ, Hamburg) and the Leibniz-Rechenzentrum (LRZ, München).

How to cite: Matthes, S., Nickl, A.-L., Peter, P., Mertens, M., Jöckel, P., Ziereis, H., Harlaß, T., and Zahn, A.: Aviation-induced changes of atmospheric composition in the UTLS in the multi-scale Earth system model MECO(1), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15843, https://doi.org/10.5194/egusphere-egu23-15843, 2023.

EGU23-15883 | Orals | AS3.16 | Highlight

Eco2Fly - An aviation climate impact assessment 

Katrin Dahlmann, Volker Grewe, Sigrun Matthes, Johannes Hendricks, Mattia Righi, Christian Weder, Mariano Mertens, and Sabine Brinkop

Air traffic facilitates our society’s requirements for mobility. However, air traffic also contributes to climate change. Especially in view of the 2°C-climate target, it is important to make aviation eco-efficient. Here, the project Eco2Fly aimed at revising the estimate of the climate impact of aviation, by means of numerical simulations as well as in-situ and remote sensing measurements. Eco2Fly was a DLR funded project, which focuses on the climate impact of aviation, how atmospheric processes can be better understood and how we can reduce the climate impact of aviation. In this poster we focus on the aviation climate impact assessment.

Lee et al. (2021) published already a comprehensive climate impact assessment two years ago, which gives an excellent overview of the different climate species and their contribution to nowadays climate impact. Here, we like to add some new methods and processes to a climate impact assessment. One point is the difference between perturbation und tagging approach. While the perturbation approach provides the impact of changed emissions in the chemistry-climate system, the tagging approach gives the contribution of one sector to the total climate impact. Additionally, new insights from numerical simulations for the direct and indirect aerosol impact were obtained.

It is important for such a climate impact assessment, to use model results which are based on a realistic spatial distribution of emissions as different emission inventories can cause significantly different climate impact estimates, despite unchanged total emissions. In cooperation with the DLR project TraK (Transport and Climate) emission calculation and climate modelling approaches are applied to assess the climate impacts of the 2019 aviation emissions.

How to cite: Dahlmann, K., Grewe, V., Matthes, S., Hendricks, J., Righi, M., Weder, C., Mertens, M., and Brinkop, S.: Eco2Fly - An aviation climate impact assessment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15883, https://doi.org/10.5194/egusphere-egu23-15883, 2023.

EGU23-15917 | ECS | Orals | AS3.16 | Highlight

Assessing WHO2021 air quality guideline levels in Europe: Population exposure and PM2.5 reduction potential 

Philipp Franke, Anne Caroline Lange, and Astrid Kiendler-Scharr

Although anthropogenic emissions have decreased during the last two decades, air pollution is still problematic in many regions in Europe. In 2021, the World Health Organisation has released updated air quality guideline levels that base on newest medical research and have drastically decreased in comparison to the previous levels, except for SO2. These levels reflect the minimum concentration for which evidence of adverse health effects have been found. This study analyses the air quality in Europe using simulations by EURAD-IM for the year 2016 with optimized emissions to evaluate guideline exceedances for PM2.5, NO2, and O3. All air pollutant concentrations in Europe exceed the WHO2021 annual guideline levels by a large amount. High PM2.5 and O3 concentrations are homogeneously distributed across Europe with 99 % and 100 % of the EU38 population (European Union and eleven other European states) exposed to concentrations above the guideline levels. High NO2 concentrations are linked to densely populated areas. However, 61% of the EU38 population is exposed to concentrations above the guideline level. For PM2.5, the effect of different aerosol classes on the bulk mass and different PM reduction scenarios are analysed. NO3- shows the largest contribution to total PM2.5 while primary anthropogenic aerosols are mainly responsible for extremely high PM2.5 concentrations of up to 30 μg m−3. In the extreme case of completely removing different aerosol classes from the bulk mass, jointly removing NO3- and primary anthropogenic aerosols as well as removing all secondary inorganic aerosols decrease PM2.5 annual concentrations to below 5 μg m−3, which is the WHO2021 annual guideline level, in most parts of Europe. However, a more realistic scenario, in which the decrease of aerosol concentrations linearly follows the targeted anthropogenic emission reductions by the European Union, still shows an exceedance of the annual WHO2021 guideline levels by a factor of 2 - 3 throughout Europe. Thus, besides implementing strong emission reduction plans, other ways of removing air pollutants from the atmosphere need to be designed and implemented.

How to cite: Franke, P., Lange, A. C., and Kiendler-Scharr, A.: Assessing WHO2021 air quality guideline levels in Europe: Population exposure and PM2.5 reduction potential, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15917, https://doi.org/10.5194/egusphere-egu23-15917, 2023.

EGU23-16003 | ECS | Posters on site | AS3.16

Estimation of NOx Emission in China by Use of Data Assimilation and Machine Learning Methods 

Yiang Chen, Jimmy C.H. Fung, and Xingcheng Lu

Nitrogen oxides (NOx, mainly comprising NO and NO2) is the essential precursor of secondary air pollutants, such as ozone and particulate nitrate. To better understand NOx emission levels and acquire reasonable simulation results for further analysis, a reasonable emission inventory is needed. In this study, a new method, combining the three-dimensional chemical transport model simulation, surface NO2 observations, the three-dimensional variational assimilation method, and an ensemble back propagation neural network, was proposed and applied to correct NOx emissions over China for the summers of 2015 and 2020. Compared with the simulation using prior NOx emissions, the root-mean-square error and normalized mean bias decreased by approximately 40% and 60% in the NO2 simulation using posterior NOx emissions. Compared with the emissions for 2015, the NOx emission generally reduced by an average of 5% in the simulation domain for 2020, especially in Henan and Anhui provinces, where the percentage reductions reached 24% and 19%, respectively. The proposed framework is sufficiently flexible to correct emissions in other periods and regions. It can provide policymakers and academic researchers with the latest emission information for better emission control and air pollution research.

How to cite: Chen, Y., Fung, J. C. H., and Lu, X.: Estimation of NOx Emission in China by Use of Data Assimilation and Machine Learning Methods, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16003, https://doi.org/10.5194/egusphere-egu23-16003, 2023.

EGU23-193 | ECS | PICO | AS3.17

Climatology and trends derived from columnar aerosol measurements in Cluj-Napoca, Romania. 

Andrei Radovici, Horatiu Stefanie, Alexandru Mereuta, Horia Camarasan, Camelia Botezan, Dan Costin, and Nicolae Ajtai

It is well known that in the climate and air quality studies, the monitoring process of aerosols and their temporal evolution is very important as they generate a significant impact on meteorology, air quality, climate, and human and ecosystem health. In this study, we present an overview of aerosol optical and microphysical properties over Cluj-Napoca, Romania- based on more than 12 years of observations from a Cimel sun-photometer operating in the framework of AErosol RObotic NETwork (AERONET) and part of the Aerosol, Clouds and Trace Gases Research Infrastructure (ACTRIS). This site is located in the north-western part of Romania and contributes to AERONET with sun photometer observation since 2010. As the atmosphere in the region is characterized by a mixture of aerosols from multiple sources: urban/industrial (dominant) biomass burning, Saharan dust, etc., this study aims to present the aerosol trends and the temporal variation of their properties based on long-term observations. The analysis highlighted that the aerosol load over the area is characterized by high inter-annual and seasonal variation of AOD due to variation of local sources and long-range transport. The same variability was observed for the Ångström Exponent, suggesting the presence of aerosols of different sizes. The methods used in this study can be extended to other stations for identifying the long-term variability of aerosols.

How to cite: Radovici, A., Stefanie, H., Mereuta, A., Camarasan, H., Botezan, C., Costin, D., and Ajtai, N.: Climatology and trends derived from columnar aerosol measurements in Cluj-Napoca, Romania., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-193, https://doi.org/10.5194/egusphere-egu23-193, 2023.

Seasonal, annual and long-term changes of carbon monoxide (CO) are investigated in the tropical (30° N ̶ 30° S) middle atmosphere (20 ̶ 80 km) for the period 2005 ̶ 2021. CO shows a semi-annual oscillation in the higher heights of both stratosphere and mesosphere. The CO response to the solar cycle increases with altitude (>2 ppmv/100 SFU) in the mesosphere. CO response to Quasi Biennial Oscillation (QBO) and El Niño and Southern Oscillation (ENSO) is negligible in stratosphere, however, that to ENSO is significantly negative in mesosphere. In the altitude range 60 ̶ 70 km, we find a positive trend (0.03 ppmv/dec) at 64 km. Furthermore, the CO trend is positive in mesosphere (70 ̶ 80 km), with a peak at 75 km (0.19 ppmv/dec). The observed changes in middle atmospheric CO in the tropics are well reproduced by the Whole Atmospheric Chemical Climate Model (WACCM). Therefore, this study provides new insights into the long-term changes in the tropical middle atmospheric CO and its connection to dynamics of the region.

How to cite: Nath, O.: Seasonal, inter-annual and long-term changes in the middle atmospheric Carbon Monoxide over the tropics, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-250, https://doi.org/10.5194/egusphere-egu23-250, 2023.

In recent times, Surface Ozone has become a widely studied constituent due to its emergence as a short-lived secondary pollutant and its damaging impacts on human health and crop production. Recent studies show increased surface ozone across different parts of the world including the Indian region. The modern reanalysis dataset provides meteorological parameters as well as atmospheric chemical compositions such as tropospheric ozone etc. In this study, we validated the spatial-temporal ozone variability using ground-based observation and reanalysis datasets such as over the North-west Indo Gangetic region. Reanalysis datasets are the Copernicus Atmospheric Monitoring Service reanalysis (CAMSRA) and NASA Modern-Era Retrospective analysis for Research and Application version 2 (MERRA2) which tells the spatial-temporal variability of surface ozone over the Northwest region of India. The result shows a lesser correlation over the study region. Through a validation process, it was determined that the CAMSRA compares fairly to ground-based observations with correlations (> 0.5)  over the Northwest region of India. This agreement has also been quantified in terms of range, Mean Absolute Error (MAE), and Root Mean Square Error (RMSE). The CAMSRA captures seasonal variations regardless of location, according to a time series analysis. Spatial distribution of surface ozone shows higher concentration during pre-monsoon followed by post-monsoon. Over the northwest region, a notable rise is noticed during May over the Indo-Gangetic Plains in particular (IGP) of the Indian region. These seasonal differences are associated with solar radiation (SR), temperature, low-level circulation, and boundary layer height (BLH).In order to further examine the spatial and temporal variability of surface ozone, we have performed the Principal Component Analysis (PCA). PCA explains the relationship between dominant modes of spatial variability and their temporal evolution. Overall, the findings show that variations in the precursors or in the meteorological conditions have a considerable impact on the surface ozone concentrations across the northwest region of India.

 

How to cite: Saroj, P., Ghosh, C., and Singh, S.: Evaluation of surface ozone variability using ground-based observation and reanalysis dataset over the North-West Indo-Gangetic Plain of Indian region., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-660, https://doi.org/10.5194/egusphere-egu23-660, 2023.

EGU23-940 | PICO | AS3.17

Aerosol composition at EMEP remote sites in France : mass balance and de-weathered trends of PM2.5 and its main components 

Anna Font, Aude Bourin, Corentin Gouillou, Cécile Debevec, Nicolas Bonnaire, Stéphane Sauvage, Joel F. de Brito, and Véronique Riffault

Atmospheric particulate matter with an aerodynamic diameter < 2.5 µm (PM2.5) is associated with adverse effects on the climate system, the human health, vegetation and the ecosystems. The World Health Organization (WHO) lowered the guideline limit for PM2.5 in autumn 2021 and this is exceeded in many regions including rural and remote areas in mainland Europe. Measurements of the chemical composition of PM2.5 is essential to assess the sources which contribute to PM2.5 mass concentrations and to further design meaningful policies to tackle sources at their origin.

Here we report 6 years (2014- 2020) of PM2.5 mass and chemical speciation at five remote sites across France belonging to the EMEP network (European Monitoring and Evaluation Programme). The seasonal and spatial variability of aerosol composition and source contributions based on the proximity of sources and long-range transport are discussed. Trends in PM2.5 and the main components at the five locations were evaluated by means of random-forest modelling coupled with a de-weathering algorithm. This approach is advantageous as resulting trends are driven by changes in emission or atmospheric processes and not by changes in weather conditions and/or long-range transport patterns. Random-forest regression modelling was built using meteorological data, backtrajectory information and temporal variables at each site and quantified the most important factors that explain PM2.5 concentrations at remote rural areas in France.

All sites observed statistically significant downward trends in PM2.5 at a rate of -4 to -9% year-1 for the period 2014 – 2020. The decrease in PM2.5 concentrations was mostly explained by changes in the secondary inorganic species (sulphate, nitrate and ammonium) and not by changes in primary PM2.5 emissions. The variability in trends in PM2.5 and components observed across the sites is discussed with their implications for policy makers.

How to cite: Font, A., Bourin, A., Gouillou, C., Debevec, C., Bonnaire, N., Sauvage, S., F. de Brito, J., and Riffault, V.: Aerosol composition at EMEP remote sites in France : mass balance and de-weathered trends of PM2.5 and its main components, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-940, https://doi.org/10.5194/egusphere-egu23-940, 2023.

EGU23-1154 | PICO | AS3.17

Air quality and air pollution sources in a national park. A case study 

Ana Maria Rodriguez Cervantes

National parks or biosphere reserves are usually places far away from urban or industrial sites, which facilitates their protection from anthropogenic air pollution. Even though, transport of persistent air pollutants from distant sources may lead to evident effects on the natural protected area.  On the other hand, there are also several examples of national parks located near cities or industrial facilities with significant emissions to the atmosphere, meaning a direct risk to the preservation of ecosystems. In such situations, not only synoptic but also regional effects must be considered to assess the air quality of the site.

This work shows that biosphere reserves and national parks require in situ tools to monitor and detect local and remote air pollution sources which may constitute a threat to flora, fauna, water, and soil. The rising of new industries in surrounding areas, traffic, and remote transport, can change with time and meteorology and so each national park should have a historical database of the air quality in the site. This study reports the research of air pollutants in ‘Las Tablas de Daimiel’ a wetland Mediterranean national park bordered by different cities and new industries in the field of the revalorization of agricultural wastes. Simultaneous data from San Pablo de los Montes, a background station in a rural area isolated from air pollution, are considered as reference.

The work was extended from March 2020 to July 2021, involving the continuous measurement of meteorological data, of surface O3, NO, NO2, CO, SO2 and PM2.5 inside the park. Twelve campaigns, one week duration, were also performed to sample air in sorbent tubes and analyse volatile organic compounds from anthropogenic sources. The results are discussed considering meteorology, especially wind and speed direction together with the assessment of back-trajectories of remote air masses. The results show that air quality in the park was affected slightly by local and remote air pollution, excepting for the observed high levels of ozone, with a mean value of 71mg.m-3. Measured mass loadings for the rest of pollutants were low and not in exceedance of the air quality standards. NOx and SO2 average concentrations (3.2 and 0.4 mg m-3, respectively) were below the recommended critical levels for vegetation. The results confirmed the presence of 26 VOCs, potentially coming from anthropogenic sources, mainly aromatics, including BTXs in average concent ration levels below 0.5 mg m-3. Although a clear diurnal behavior couldn´t  be established, slightly higher concentrations were observed during working days. From the study of local winds and diurnal profiles of VOCs, we could not identify local sources of these pollutants. This indicates that potential nearby sources did not emit significant quantities of these compounds or emissions were sufficiently diluted by dispersion before reaching the park.

Saharan dust events were frequent and contributed to PM2.5 levels in the site. AOT-40 values above the established threshold for the protection of vegetation were obtained, 25,500 and 19,900 mg m-3 for 2020 and 2021, respectively. 

How to cite: Rodriguez Cervantes, A. M.: Air quality and air pollution sources in a national park. A case study, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1154, https://doi.org/10.5194/egusphere-egu23-1154, 2023.

EGU23-1940 | PICO | AS3.17

Online measurement of ambient toxic volatile organic compounds using thermal desorption gas chromatography-mass spectrometry (TD-GC/MS) 

Jia-Lin Wang, Chieh-Heng Wang, Hsin-Cheng Hsieh, Chen-Hsuan Chu, Mei-Hui Tseng, Kuan-Chun Lee, and Po-Sheng Tseng

Toxic volatile organic compounds (VOCs) or air toxics are part of the hazardous air pollutants (HAPS) to affect public health. In this work, the thermal desorption (TD) technique was coupled with gas chromatography mass spectrometry (GC/MS) to form an online technique to provide hourly data of 86 air toxics. Due to the perennial high humidity of the sub-tropical weather, water removal prior to TD-GC/MS analysis is necessary to prevent icing during cryo-trapping but still kept limited water vapor to maintain the required recoveries for the target species. Adding internal standards drastically offset the instrumental drift in detection and greatly secured the accuracy of the analytes. A month-long field measurement of TD-GC/MS was conducted near an industrial park with two other techniques of proton transfer mass spectrometry (PTR-MS) and flask sampling for validation. Time series data of TD-GC/MS showed distinct spikes in the hourly measurements induced by the pollution plumes, which were divided into two categories of non-chlorinated vs chlorinated compounds. The non-chlorinated species showed consistency in the occurrence of spikes between the online GC and PTR-MS. The canister data, however, missed most of the spikes of the measured species, but captured the single most prominent spikes of carbon tetrachloride and styrene by pure coincidence, showcasing the superiority of the online vs. the offline method. The strength of plume detection by online TD-GC/MS was further illustrated by back trajectories of the pronounced spikes of benzene and carbon tetrachloride, which were only several hours apart but pointed to entirely different directions of the upwind sources due to the rapid change in wind directions in this brief period.

How to cite: Wang, J.-L., Wang, C.-H., Hsieh, H.-C., Chu, C.-H., Tseng, M.-H., Lee, K.-C., and Tseng, P.-S.: Online measurement of ambient toxic volatile organic compounds using thermal desorption gas chromatography-mass spectrometry (TD-GC/MS), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1940, https://doi.org/10.5194/egusphere-egu23-1940, 2023.

Multiwavelength aerosol optical depth (AOD) has been defined as an essential climate variable for the Global Climate Observing System (GCOS) and the Global Atmosphere Watch (GAW) Program of the World Meteorological Organization. It is the most important parameter related to aerosol radiative forcing studies. PMOD/WRC have developed the Precision Filter Radiometer (PFR) that has been used for long term AOD measurements under a GAW-PFR Network of sun-photometers started in 1995 at Davos Switzerland and from 1999 at other locations, worldwide.

Here we present an overview of the stations measurements till 2021 including station statistics and AOD trends.

An overview of the results of the long term GAW-PFR AOD series for four high altitude stations (Izana/Spain, Mauna Loa/USA, Mt. Walliguan/China and Jungfraujoch/Switzerland). Mean AODs at 500nm were from 0.01 up to 0.1 with small negative changes per year for all stations.

Also we present an overview of the homogenization activities performed by the world aerosol optical depth research and calinration center (WORCC) towards a harmonization of AOD measurements worldwide and some examples on uncertainties and effects on global trend analysis and satellite AOD validation initiatives.

How to cite: Kazadzis, S., Kouremeti, N., and Groebner, J.: Aerosol Optical Depth Measurements and trends from the  Global Atmospheric Watch - PFR Network and aerosol homogenization initiatives, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2340, https://doi.org/10.5194/egusphere-egu23-2340, 2023.

EGU23-2755 | ECS | PICO | AS3.17

Air Pollution from Agriculture: Using Satellite Observations to Study Ammonia Emissions 

Adriana Iorga, Jeremy Harrison, and David Moore

Ammonia (NH3) is one of the most common nitrogen gas species and pollutants present in the lower troposphere. Ammonia enters the atmosphere through volatilisation from soils through the usage of nitrogen-based fertilisers in agriculture [1]. Because of its short lifetime (up to a few hours) [2], ammonia is highly reactive and can react chemically with acids in the atmosphere to form fine particulate matter (PM2.5), playing an important role in secondary aerosol formation [3]. Wet and dry deposition of ammonia on soils and water bodies has shown to be detrimental to ecosystem biodiversity as it leads to acidification of the environment [3]. Therefore, observations of ammonia are essential for establishing air quality and environmental regulations for agricultural practices.

By using combined satellite measurements from the Infrared Atmospheric Sounding Interferometer (IASI) and the Cross-track Infrared Sounder (CrIS) instruments, we aim to study trends and the diurnal cycle of ammonia on regional scales, particularly in areas subjected to intensive agricultural activity, such as the Indo-Gangetic Plain (northern India). This research makes use of an optimal estimation-based method of monitoring ammonia with satellites called the University of Leicester IASI retrieval Scheme (ULIRS).

References:

[1] Van Damme M. et al (2021), Environ. Res. Lett., 16 055017

[2] Dammers E. et al (2019), Atmos. Chem. Phys., 12261–12293

[3] Erisman, J. W. et al (2007), Environ. Pollut., 150, 140– 149

How to cite: Iorga, A., Harrison, J., and Moore, D.: Air Pollution from Agriculture: Using Satellite Observations to Study Ammonia Emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2755, https://doi.org/10.5194/egusphere-egu23-2755, 2023.

EGU23-3209 | ECS | PICO | AS3.17

A comprehensive study on atmospheric pollution over Ploiesti, Romania 

Bianca Mihalache, Marilena Colt, Sabina Stefan, and Gabriela Iorga

The accumulation of both particulate matter (PM10, PM2.5) and gaseous species (NO2, CO, SO2, O3) in the atmosphere in urban agglomerations can cause a significant degradation of air quality. The additional impact on human health, visibility, cultural heritage and urban climate has been recognized in studies worldwide. This study represents an air quality assessment in the urban agglomeration of Ploiesti, which is located north of Bucharest (the highest polluted city of Romania), in the central-northern part of Romanian Plain. In Ploiesti operates some of the most important refineries of the country. The city also represents an important link between Bucharest and south of Romania and the northern and western parts of the country.

The study is focused on major air pollutants, particulate matter (PM10, PM2.5), and also gaseous species (NO2, CO, SO2, O3) at six monitoring sites (traffic, industrial and background). To highlight temporal and spatial variations, a synthetic database covering a four-year period (2018-2021) consisting of time series of hourly and daily values of major air pollutants mass concentrations were statistically investigated. To analyze the influence of meteorological conditions on the air quality in Ploiesti area meteorological observations was constructed.

Present research shows that although Ploiesti is significantly smaller than Bucharest, the anthropogenic activity in Ploiesti strongly affects atmospheric pollution levels on daily timescales (multiannual mean ratio PM2.5/PM10 = 0.71) at almost same level that in Bucharest area. Additionally, we found the central area impact on surroundings is major, as significant differences were not identified.

We identified both local and regional pollution episodes, but also episodes strongly influenced by the long-range transport of dust pollution.

PM10 pollution roses showed the dominance of local pollution sources in most of the time. On shorter timescale, the long-range transport of fine particulate matter coming from desert dust (Saharan or from Middle East deserts) contributed supplementary to increased pollution as we identified in 13 episodes (during 2018-2021). It has been shown that the atmospheric stability has an important role in the accumulation of PM10 at the scale of Ploiesti urban agglomeration. Trend analysis of annual pollutant mass concentrations for all air quality stations was performed using a larger dataset, since 2008 (first monitoring year) to present (end of 2021), using Mann-Kendal and Sen’slope analysis. Diurnal profile of particulate matter PM10 and the influence of the lockdown restrictions in spring 2020 on PM10 levels were also quantified.

Acknowledgment

The research leading to these results has received funding from the NO Grants 2014-2021, under Project contract no. 31/2020, EEA-RO-NO-2019-0423 project. Data regarding ground-level air pollution and local meteorology by site was extracted from the public available Romanian National Air Quality Database, www.calitateaer.ro, last accessed in December 2022. Meteorological data were extracted from Copernicus Climate Change Service (C3S) Climate Data Store (CDS) ERA5 hourly data on single levels and pressure levels from 1959 to present https://cds.climate.copernicus.eu (last accessed in December 2022).

How to cite: Mihalache, B., Colt, M., Stefan, S., and Iorga, G.: A comprehensive study on atmospheric pollution over Ploiesti, Romania, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3209, https://doi.org/10.5194/egusphere-egu23-3209, 2023.

EGU23-3232 | ECS | PICO | AS3.17

Global and regional anthropogenic emissions inventories for air quality atlases 

Antonin Soulie, Thierno doumbia, Sekou Keita, Claire Granier, Hugo Denier Vand der Gon, Jeroen Kuenen, Santiago Arellano, Sabine Darras, Michael Gauss, Marc Guevara, Jukka-Pekka Jalkanen, Cathy Liousse, David Simpson, and Katerina Sindelarova

We present two inventories of anthropogenic emissions as well as an air quality atlas linked to Copernicus, the European earth observation system. CAMS-GLOB-ANTv5.3, a global anthropogenic emissions inventory, has been developed and provides emission data for the major atmospheric pollutants and greenhouse gases, as well as 25 speciated Volatile Organic Compounds (VOCs), for the period 2000-2023. This inventory is used as input for the Copernicus Atmosphere Monitoring System (CAMS) atmospheric reanalysis and forecasts.

A mosaic inventory of anthropogenic emissions was also developed as part of the Copernicus CO2 project (CoCO2) focusing on greenhouse gases emissions. This mosaic uses the CAMS-GLOB-ANTv5.3 inventory as a global basis, and the DACCIWA2 (Dynamics-Aerosol-Chemistry-Cloud interactions in West Africa) inventory, a regional African emissions inventory. DACCIWA2 provides 0.1x0.1 degree resolution emissions of greenhouse gases and atmospheric pollutants for the period 2010-2018.

The CAMS reanalysis is being used to develop an atlas of air quality called AQWA (Air Quality Worldwide Atlas). The AQWA atlas gives precious information about historical, climatological and current atmospheric composition, as well as air quality indexes. These statistics are available for all countries around the world, as well as states/provinces for the United States and China.

This presentation describes the methodology used to develop and evaluate the two inventories and shows a few visualization examples from the atlas, which is still in development.

How to cite: Soulie, A., doumbia, T., Keita, S., Granier, C., Denier Vand der Gon, H., Kuenen, J., Arellano, S., Darras, S., Gauss, M., Guevara, M., Jalkanen, J.-P., Liousse, C., Simpson, D., and Sindelarova, K.: Global and regional anthropogenic emissions inventories for air quality atlases, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3232, https://doi.org/10.5194/egusphere-egu23-3232, 2023.

EGU23-3498 | ECS | PICO | AS3.17

The response of the North Pacific jet and stratosphere-to-troposphere transport of ozone over western North America to RCP8.5 climate forcing 

Dillon Elsbury, Amy H. Butler, John R. Albers, Melissa L. Breeden, and Andrew O'Neil Langford

Stratosphere-to-troposphere transport (STT) is an important source of ozone for the troposphere, particularly over western North America. STT in this region is predominantly controlled by a combination of the variability and location of the Pacific jet stream and the amount of ozone in the lower stratosphere, two factors which are likely to change if greenhouse gas concentrations continue to increase. Here we use Whole Atmosphere Community Climate Model experiments with a tracer of stratospheric ozone (O3S) to study how end-of-the-century Representative Concentration Pathway (RCP) 8.5 sea surface temperatures (SSTs) and greenhouses gases (GHGs), in isolation and in combination, influence STT of ozone over western North America relative to a preindustrial control background state.

            We find that O3S increases up to 39% at 700 hPa over western North America in response to RCP8.5 forcing with the largest increases occurring during late winter and tapering off during spring and summer. The GHGs are primarily responsible for these tropospheric O3S changes. Both the future SSTs and the future GHGs accelerate the Brewer Dobson circulation, which increases extratropical lower stratospheric ozone mixing ratios. While the GHGs promote a more zonally symmetric lower stratospheric ozone change due to enhanced ozone production and some transport, the SSTs increase lower stratospheric ozone predominantly over the North Pacific via transport associated with a stationary planetary-scale wave. Ozone accumulates in the trough of this anomalous wave and is reduced over the wave’s ridges, illustrating that the composition of the lower stratospheric ozone reservoir in the future is dependent on the stationary planetary-scale wave response to future SSTs. In addition, the future SSTs are found to prompt most changes to the large-scale circulation in the troposphere and stratosphere compared to the effect of the GHGs. These changes include modifying the position and speed of the future North Pacific jet, lifting the tropopause, accelerating both the Brewer-Dobson Circulation’s shallow and deep branches, and enhancing two-way isentropic mixing in the stratosphere.

How to cite: Elsbury, D., Butler, A. H., Albers, J. R., Breeden, M. L., and Langford, A. O.: The response of the North Pacific jet and stratosphere-to-troposphere transport of ozone over western North America to RCP8.5 climate forcing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3498, https://doi.org/10.5194/egusphere-egu23-3498, 2023.

Monitoring the atmospheric concentrations of the reactive species in the stratosphere, including greenhouse gases (GHGs), is crucial in order to improve our understanding of their climate impact. Although progress has been made towards construction of long-term ozone profile data sets, limited long-term profile data are available for other species. Here, we merge TOMCAT chemical transport model (CTM) output and profile measurements from two solar occultation instruments, the HALogen Occultation Experiment (HALOE) and the Atmospheric Chemistry Experiment - Fourier Transform Spectrometer (ACE-FTS), to construct a long-term (1991-2021), gap-free stratospheric profile data set (hereafter TCOM). The Extreme Gradient Boosting (XGBoost) regression model is used to estimate the corrections needed to apply to the CTM profiles to bring them into line with the observations.

We have already released data sets for two important greenhouse gases: methane and nitrous oxide. For methane (TCOM-CH4), we use both HALOE and ACE satellite profile measurements (1992-2018) to train the XGBoost model and profiles from three later years (2019-2021) are used as an independent evaluation data set. As there are no nitrous oxide profile measurements for the earlier years, XGBoost-derived correction terms for TCOM-N2O profiles are derived using only ACE-FTS profiles for 2004-2018 time period with profiles from 2019-2021 again being used for the evaluation.

Overall, both TCOM-CH4 and TCOM-N2O profiles show excellent agreement with the available satellite measurement-based data sets. Biases in TCOM-CH4 and TCOM-N2O are less than 10% and 50% throughout the stratosphere, respectively. Daily zonal mean TCOM-CH4 and TCOM-N2O profile data sets on altitude (15--60~km) and pressure (300--0.1~hPa) are publicly available via https://doi.org/10.5281/zenodo.7293740 and https://doi.org/10.5281/zenodo.7293740, respectively.

Our presentation will discuss the construction, performance and availability of the TCOM data sets. We aim to release data sets for ozone (TCOM-O3), hydrogen chloride (TCOM-HCl), hydrogen fluoride (TCOM-HF), water vapour (TCOM-H2O), nitric acid (TCOM-HNO3), nitric oxide (TCOM-NO) and nitrogen dioxide (TCOM-NO2) shortly.

How to cite: Dhomse, S. and Chipperfield, M.: Using machine-learning to construct long-term, gap-free stratospheric species profile data sets based on satellite occultation measurements and TOMCAT 3-D model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4542, https://doi.org/10.5194/egusphere-egu23-4542, 2023.

EGU23-4629 | ECS | PICO | AS3.17

Does surface warming over Western Europe affect the occurrence frequency of contrail forming regions? 

Yun Li, Susanne Rohs, Martina Krämer, and Andreas Petzold

The decade, 2012 to 2021, was the warmest on record, with the global mean near-surface air temperature in the most recent seven years, 2015 to 2021, keeping hitting record high. Europe, with an increase of 1.94 to 2.01 °C in the mean annual temperature since pre-industry level, is warming much faster than the global average (1.11 to 1.14 °C) (https://www.eea.europa.eu/ims/global-and-european-temperatures). Surface warming disrupts upper-air temperature, which will affect the humidity fields in the upper troposphere. Both ambient temperature and relative humidity with respect to ice (RHice) are key factors determining the formation and persistence of contrail cirrus clouds, which exert a net warming radiative forcing among aviation emissions (Lee et al., 2009; Lee et al., 2021).

Previous studies have provided insights into the long-term trend and seasonal variability of upper-air temperature and relative humidity using airborne, radiosonde and reanalysis datasets (Petzold et al., 2020; Chen et al., 2015; Philandras et al., 2017; Essa et al., 2022). The variation of RHice in relation to the changing upper tropospheric temperature because of surface warming has, however, rarely been investigated.

In this work, we use the temperature and RHice measurements over Western Europe from the European research infrastructure IAGOS (In-Service Aircraft for a Global Observing System; www.iagos.org) to study how the upper-air temperature and RHice distributions in the warmest seven years have changed seasonally and regionally compared to the IAGOS-MOZAIC period, 1995 to 2010, when the surface warming was not so drastic. We will focus on whether the occurrence frequency of contrail forming regions, i.e., slightly ice subsaturated to supersaturated regions in the upper troposphere, would be affected by the increasing warming climate, which could promote our understanding of contrail mitigation.

[Note: This work is carried out under the frame of EU H2020 Research and Innovation Action “Advancing the Science for Aviation and Climate (ACACIA)”, Grant Agreement No. 875036.]

How to cite: Li, Y., Rohs, S., Krämer, M., and Petzold, A.: Does surface warming over Western Europe affect the occurrence frequency of contrail forming regions?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4629, https://doi.org/10.5194/egusphere-egu23-4629, 2023.

Abstract

It has been proven that air pollution is closely related to the level of socio-economic development of a country. Various levels of development generate different level of by-products, including air pollution, deteriorating therefore the air quality at regional levels in peculiar ways. Romania is the largest country in southeastern Europe with a very complex economic development level and air pollution disparities among cities.

This paper aims to study main socio-economic indicators (as measures of the effect of human activities on air pollution and climate) for over 30 cities in Romania with diferent levels of economic development, to determine the relationship between these variables and air pollution condition. We focused on the spatial relationship between main gaseous air pollutants and the following indicators GDP, GDP/capita, resident population, number of private vehicles and life expectancy.

In this research we created two data sets as follow: first one consists of daily values of air pollutant (CO, NO2, O­­3, SO2) mass concentrations extracted from the Romanian National Air Quality Network and the second set consists of socio-economic indicators (GDP, GDP/capita, resident population, number of private vehicles and life expectancy) obtained from Romanian National Institute of Statistics. The study was conducted over five years, from 01.01.2016 to 31.12.2020 using yearly means of air pollutants from the first dataset in all selected urban areas in the Romanian territory and corelate them with the socio-economic indicators from the second data set using univariate LISA and bivariate LISA statistical analysis methods.

The analysis demonstrated the correlation of socio-economic indicators with the increase of the air pollution in the study area. Other highlights of the study: (a) Range of major air pollutant levels in 30 urban agglomerations across Romania from 2016 to 2020 was assessed (b) Maps of interpolated mass concentrations reveal regional significant differences with pollutant-specific hot- and cold-spots in Romania. Regional significant differences can be observed; (c) Results show pollution decreases for most pollutants in most cities in 2020 due to pandemic restrictions.

The results of present study can be beneficial to local authorities in order to help them in their decisions for abatement pollution strategies at the country scale combined with regional measures.

 

Acknowledgment

The research leading to these results has received funding from the NO Grants 2014-2021, under Project contract no. 31/2020, EEA-RO-NO-2019-0423 project. Data regarding ground-based air pollutants were extracted from the Romanian National Air Quality Database, www.calitateaer.ro. Economy indicators were provided by National Institute of Statistics http://statistici.insse.ro:8077/tempo-online/. Databases were last accessed in December 2022.

How to cite: Chiritescu, R. V. and Iorga, G.: Air pollution over Romania: spatial relationship betweensocio-economic indicators and air pollutants using univariate and bivariate local indicators, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4913, https://doi.org/10.5194/egusphere-egu23-4913, 2023.

EGU23-5347 | ECS | PICO | AS3.17

The characteristics of atmospheric SF6 in the Korean Peninsula during 2017-2020 

Soojeong Lee, Haeyoung Lee, and Shanlan Li

Sulfur hexafluoride (SF6) is a most potent anthropogenic greenhouse gas with a global warming potential of 23,900 over a 100-year time horizon. There are no natural sink sources in the troposphere and they are destructed by photolysis and electron attachment in the mesosphere.  SF6 is mainly used for electrical insulation, circuit breaker, and plasma etching processes in the semiconductor industry. For monitoring changes in atmospheric SF6 in Korean Peninsula, 3 surface in-situ greenhouse gas monitoring stations, Anmyeondo (AMY), Jeju Gosan (JGS), and Ulleungdo (ULD), have been operating. AMY started its operation in 2007 and JGS and ULD followed in 2017. Due to the advantage of their locations surrounding the Korean Peninsula at the Western, Southern, and Eastern ends, they can provide information on the inflow and outflow of the SF6 in the Korean Peninsula. According to the data from 2017 to 2020, the increasing trend of background mole fraction of SF6 from the stations was in good agreement with that of the global monitoring stations, Mauna Loa and Cape Grim. Each station shows the characteristic enhancement tendency by wind direction and speed, which implies the possible influence of the regional emission source and long-range transport. In addition, based on the analysis with HYSPLIT model the central area of the Korean Peninsula is identified as an emission source region, as well as central part of China and Japan.

How to cite: Lee, S., Lee, H., and Li, S.: The characteristics of atmospheric SF6 in the Korean Peninsula during 2017-2020, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5347, https://doi.org/10.5194/egusphere-egu23-5347, 2023.

EGU23-5673 | ECS | PICO | AS3.17

Modelling the near future air-quality over Central Europe 

Alvaro Patricio Prieto Perez, Peter Huszar, and Jan Karlicky

Air quality is not only dependent on emissions, but on climate and meteorology as well. This makes the study of the evolution of air pollution varying some of its drivers crucial. In this study, the present day and near future air quality in Central Europe is studied following RCP4.5 and RCP8.5 scenarios for the 2026-2035 and 2046-2055 decades, while considering present-day climate conditions. We assume that the climate changes a little while the main driver for air-quality changes in near future are the modified emissions. The emission input for the 2010-2019 decade were compiled using the Flexible Universal Processor for Modeling Emissions (www.fume-ep.org), and the two future decades are being prepared by scaling the present day emissions based on the mentioned RCPs. We are performing simulations using the Weather Research and Forecast with online chemistry version 4.0.3 (WRF-Chem) model and the Comprehensive Air-quality Model (CAMx). Several pollutants and meteorological variables will be studied and compared with observational data.

How to cite: Prieto Perez, A. P., Huszar, P., and Karlicky, J.: Modelling the near future air-quality over Central Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5673, https://doi.org/10.5194/egusphere-egu23-5673, 2023.

EGU23-6135 | PICO | AS3.17

Prognostic Ozone For ICON: Enabling UV Forecasts 

Valentin Hanft, Roland Ruhnke, Axel Seifert, and Peter Braesicke

Stratospheric ozone (O3) absorbs biologically harmful solar ultraviolet radiation, mainly in the UV_B and UV_C spectral range. When reaching the surface, such UV radiation poses a well documented hazard to human health. In order to quantify this amount of UV radiation and to make it generally understandable, the World Health Organization has defined an UV Index[1]. It is calculated by weighting the incoming solar irradiance at surface level between 250 and 400 nanometers with their ”harmfulness” to the skin and scaling the results to values that normally range between 1 and 10, surpassing 10 for excessive UV exposure.

Implementing UV Index forecasts in numerical weather prediction (NWP) models allows to alert the public in time if special care for sun protection needs
to be taken. The German Weather Service (DWD) uses its NWP model ICON (ICOsahedral Nonhydrostatic Model)[2] to offer such a forecast for Germany[3]
using external data such as ozone forecasts by the Royal Dutch Weather Service (KNMI) and radiation lookup tables[4].


In our project we extend the capability of ICON to provide a configuration of self-consistent UV Index forecasts that do not require external data. For this, we use ICON-ART[5],[6] with a linearized ozone scheme (LINOZ)[7] and couple the prognostic ozone to the atmospheric radiation scheme Solar-J[8].
Here we present the current state of our UV Index forecast system and compare our results to available reference data.

References:

[1] World Health Organization, World Meteorological Organization, United Nations Environment Programme, and International Commission on Non-
Ionizing Radiation Protection. Global solar uv index : a practical guide,2002.

[2] Günther Zängl et al.. The icon (icosahedral non-hydrostatic) modelling framework of dwd and mpi-m:
Description of the non-hydrostatic dynamical core. Quarterly Journal of the Royal Meteorological Society, 2015.

[3] https://kunden.dwd.de/uvi/index.jsp.

[4] Henning Staiger and Peter Koepke. Uv index forecasting on a global scale. Meteorologische Zeitschrift, 2005.

[5] D. Rieger et al.. Icon–art 1.0 – a new online-coupled model system from the global to regional scale. Geoscientific Model Development, 2015.

[6] J. Schröter et al.. Icon-art 2.1: a flexible tracer framework and its application for composition studies in numerical weather forecasting and climate simulations. Geoscientific Model Development, 2018.

[7] C. A. McLinden et al. Stratospheric ozone in 3-d models: A simple chemistry and the cross-tropopause flux. Journal of Geophysical Research: Atmospheres, 2000

[8] J. Hsu, M. J. Prather et al.. A radiative transfer module for calculating photolysis rates and solar heating in climate models: Solar-j v7.5. Geoscientific Model Development, 2017.

How to cite: Hanft, V., Ruhnke, R., Seifert, A., and Braesicke, P.: Prognostic Ozone For ICON: Enabling UV Forecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6135, https://doi.org/10.5194/egusphere-egu23-6135, 2023.

EGU23-7671 | ECS | PICO | AS3.17

Investigating zonal asymmetry in stratospheric ozone trends at northern high latitudes using satellite limb observations and CTM simulations 

Carlo Arosio, Martyn P. Chipperfield, Alexei Rozanov, Mark Weber, Sandip Dhomse, Wuhu Feng, and John P. Burrows

Observations in limb geometry from satellite platforms are very valuable for monitoring the stratospheric ozone layer on a global scale, as they provide information with high spatial and temporal coverage and good vertical resolution. At the University of Bremen, ozone profiles were retrieved from observations from two limb sounders, SCIAMACHY (2002-2012) and OMPS-LP (2012-present), using similar retrieval algorithm setups. These two data sets were merged to obtain a consistent time series of longitudinally resolved global ozone distribution, referred to below as SCIA+OMPS. Recently, the OMPS-LP data set has been re-processed by using improved L1 data produced by the NASA team, with the main aim to mitigate the long-term drift affecting the OMPS-LP time series. The results of this re-processing will be presented; the use of the updated data set gives more confidence in the trend studies from the SCIA+OMPS time series.

The overarching aim of this study is the investigation of vertically consistent patterns in the longitude-resolved trends, particularly at northern mid- and high-latitudes above 30 km altitude, detected in the SCIA+OMPS data set. Large positive trends are found over the Atlantic sector, whereas close-to-zero changes are detected over the Siberian/Pacific sector. To investigate the origin of this behaviour, we performed full chemistry simulations of the TOMCAT global 3-D chemistry transport model (CTM), forced by ERA5 reanalysis, for the 2003-2020 period. We then applied a multi-linear regression model including dynamical proxies to both the satellite observations and TOMCAT simulations. First, we compare the trend resulting from the merged data set with those from the model simulations to check the consistency of the detected zonal and longitudinally resolved patterns. Then, seasonally and monthly resolved trends are studied as they provide valuable insight into the observed zonal asymmetry of the trends. We find the largest variability with longitude occurring in winter- and springtime, and a good consistency between observations and the CTM.

By comparing ozone changes, with trends in temperature and meridional wind fields from ERA5, we investigated potential mechanisms driving the observed asymmetry. Dedicated TOMCAT simulations showed the negligible role of photochemical processes for the observed pattern. We therefore consider the behaviour to be mainly dynamically driven. A composite analysis supports the hypothesis that the long-term change in the position of the polar vortex has influenced the winter- and springtime ozone concentrations and has led to the zonal asymmetry identified in the data and model.

How to cite: Arosio, C., Chipperfield, M. P., Rozanov, A., Weber, M., Dhomse, S., Feng, W., and Burrows, J. P.: Investigating zonal asymmetry in stratospheric ozone trends at northern high latitudes using satellite limb observations and CTM simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7671, https://doi.org/10.5194/egusphere-egu23-7671, 2023.

EGU23-7891 | PICO | AS3.17

Development of a merged HCHO climate data record from the EUMETSAT AC SAF GOME-2 Level-2 products 

Isabelle De Smedt, Gaia Pinardi, Pieter Valks, Klaus-Peter Heue, Steven Compernolle, Jeroen Van Gent, Jonas Vlietinck, Huan Yu, Diego Loyola, Nicolas Theys, and Michel Van Roozendael

Within the framework of the EUMETSAT AC SAF project, the production of climate data records (CDRs) of short lived O3 precursors (HCHO and NO2) is under development, based on the three GOME-2 instruments and the future S5 and S4 Copernicus platforms.

This work presents the development of the formaldehyde CDR, combining the current GOME-2 A, B and C operational AC SAF Level-2 orbital products to create one single L3 averaged product using advanced gridding tools. To this aim, the consistency between the three GOME-2 instrument needs to be improved by means of suitable correction schemes accounting for inter-sensor biases due to inconsistent auxiliary data or instrumental issues. The use of the CAMS model reanalysis as a source of prior HCHO profiles is explored with the aim to produce one consistent dataset from 2007 to now. Estimation of the random and systematic uncertainty is included for each grid cell. Furthermore, we plan to include meteorological re-analysis data (surface temperature and winds) in the output files to further support the interpretation of the data and of their observed variations.

Validation results of this new monthly averaged CDR dataset will be presented, with a special focus on bias, precision and stability in time. To this aim, long-term ground-based HCHO measurements are collected and assessed.

How to cite: De Smedt, I., Pinardi, G., Valks, P., Heue, K.-P., Compernolle, S., Van Gent, J., Vlietinck, J., Yu, H., Loyola, D., Theys, N., and Van Roozendael, M.: Development of a merged HCHO climate data record from the EUMETSAT AC SAF GOME-2 Level-2 products, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7891, https://doi.org/10.5194/egusphere-egu23-7891, 2023.

EGU23-8845 | PICO | AS3.17

Complex geographical causes of different levels of air pollution changes caused by COVID-19 sanctions in Europe 

György Varga, Adrienn Csávics, and Fruzsina Gresina

Our globalised world, with its many acute natural and social problems, has now created all the conditions for pandemics. The COVID-19 pandemic is the first real manifestation of this in our modern history, affecting every geographical region, every social class and almost every single economic sector. The spread of the epidemic, which was accompanied by extremely severe social and economic devastation and damage, was sanctioned by reducing people's social activity and high mobility. The measures have also been accompanied, obviously, by a reduction in some of the environmental stresses resulting from anthropogenic activity.

Our research investigates the relationship between satellite remote sensing air pollution data and sanctions related to the coronavirus epidemic, taking into account complex physical- and socio-geographical factors. Spatially and temporally differentiated COVID-19 sanctions and lockdowns (home office orders, curfews, service closures, shutdowns) have different atmospheric environmental impacts in different physical geographic regions (topography and circulation, vegetation cover, natural aerosol loads, etc.) and in areas with different socio-economic characteristics. Our aim was to identify the individual effects of the complex processes underlying the changes in atmospheric environment indicators that have not been observed before.

In this paper, NO2 and atmospheric aerosol are presented in detail, with a clear distinction between atmospheric substances of purely anthropogenic origin and those typically interpreted as natural pollutants (e.g. Saharan dust). A comparative analysis of these, using data from 2019, 2020 and 2021, highlights the spatiotemporal characteristics of the period before, during and after COVID-19 sanctions. For this purpose, Sentinel-5p and MODIS Aerosol Optical Depth data were used. The different changes in the air environment in Western and Eastern European countries, and in particular in some industrial regions, are clearly visible in the series of maps presented.

The research was supported by the project POST-COVID2021-29 of the Hungarian Academy of Sciences.

How to cite: Varga, G., Csávics, A., and Gresina, F.: Complex geographical causes of different levels of air pollution changes caused by COVID-19 sanctions in Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8845, https://doi.org/10.5194/egusphere-egu23-8845, 2023.

EGU23-9271 | ECS | PICO | AS3.17

Long-term trends and radiative impact in vertically resolved stratospheric water vapour from ESA WV_cci data records 

Hao Ye, Michaela Hegglin, Daan Hubert, Jean-Christopher Lambert, Kaley Walker, Chris Sioris, Luis Millan, Gloria Manney, Lucien Froidevaux, Brian Kerridge, Richard Siddans, Ray Wang, David Plummer, Martina Krämer, Christian Rolf, and Keith Shine

Water vapour in the upper troposphere and stratosphere has a significant impact both on the radiative and chemical properties of the atmosphere.  Reliable water vapour climate data records (CDRs) are essential for use in climate research, to assess vertically resolved trends and associated radiative impacts. Within the ESA Water Vapour Climate Change Initiative (WV_cci), new vertically resolved water vapour CDRs in the stratosphere and UTLS were merged from a range of satellite observations. In this contribution, we provide an overview of these CDRs, highlighting innovations in the merging methodologies and results from a detailed quality assessment. In particular, the long-term trends derived from the new water vapour CDRs are compared to other merged datasets, reanalyses, and simulations from chemistry-climate models, with the ESA WV_cci CDRs deemed to be valuable new datasets for climate studies.  We conclude that, mostly driven by dynamical variability, the derived water vapour trends vary significantly depending on the dataset used, chosen time period and location in the atmosphere. Using an off-line radiative transfer model, we estimate the consequence of these differences on the radiative forcing from water vapour changes in the upper troposphere and stratosphere over the past 30+ years.

How to cite: Ye, H., Hegglin, M., Hubert, D., Lambert, J.-C., Walker, K., Sioris, C., Millan, L., Manney, G., Froidevaux, L., Kerridge, B., Siddans, R., Wang, R., Plummer, D., Krämer, M., Rolf, C., and Shine, K.: Long-term trends and radiative impact in vertically resolved stratospheric water vapour from ESA WV_cci data records, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9271, https://doi.org/10.5194/egusphere-egu23-9271, 2023.

EGU23-9414 | PICO | AS3.17

ACE-FTS water vapour trends in the stratosphere-mesosphere 

Patrick Sheese, Kaley Walker, Paul Jeffery, and Chris Boone

The Atmospheric Chemistry Experiment – Fourier Transform Spectrometer (ACE-FTS) is a high spectral resolution (0.02 cm-1) spectrometer on the SciSat satellite that has been taking solar occultation measurements of the Earth’s limb since February 2004. ACE-FTS measures vertical profiles of temperature/pressure and concentrations of over 60 trace gases, including ozone and water vapour, with a vertical resolution of ~2-6 km. From the beginning of the mission, ACE-FTS water vapour data exhibits a significant positive trend on the order of a few percent per decade throughout the stratosphere and mesosphere, in agreement with similar measurements from the Microwave Limb Sounder (MLS) and the Sounding of the Atmosphere using Broadband Emission Radiometry (SABER) instruments. This study will investigate the link between ACE-FTS water vapour trends and decadal variations in other atmospheric parameters, including local and tropopause temperatures, ozone and methane concentrations, and solar flux, and will discuss how ACE-FTS measurements of HDO can be used to continue measuring background water vapour trends post-eruption of the Hunga Tonga-Hunga Ha’apai volcano, which injected ~160 Tg of water vapour (more than 10% of the stratospheric water vapour budget) into the stratosphere.

How to cite: Sheese, P., Walker, K., Jeffery, P., and Boone, C.: ACE-FTS water vapour trends in the stratosphere-mesosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9414, https://doi.org/10.5194/egusphere-egu23-9414, 2023.

EGU23-9518 | ECS | PICO | AS3.17

Optimization of simulated CO2 & NO2 concentrations for a detailed infrastructure map in the Middle East 

Ioannis Cheliotis, Thomas Lauvaux, Jinghui Lian, Theodoros Christoudias, George Georgiou, Frédéric Chevallier, Ruixue Lei, and Philippe Ciais

Atmospheric chemistry models play a major role for relating greenhouse gases and pollutants concentrations to emissions at high temporal resolutions over large areas. On that account, it is fundamental to use up-to-date anthropogenic emissions maps as model inputs. Despite efforts by researchers to create global emission datasets with high temporal resolutions, for countries with no national data, generic activity maps and emission factors are used, thus the accurate representation of the anthropogenic emissions in a local scale still remains challenging. This study presents an improved spatially explicit dataset for anthropogenic emissions of CO2 and NOx over the Middle-East, a region characterized by extensive gas power plants and heavy industries operations. Our dataset was developed by combining a detailed infrastructure map for point sources in the area and it is used to simulate the distribution of CO2 and NO2 using the WRF-Chem mesoscale atmospheric transport chemistry model. Furthermore, the chemistry scheme of the WRF-Chem model in the simulation of CO2 and NO2 plumes is examined, in comparison with satellite observations.
   
In the framework of the Eastern Mediterranean and Middle East – Climate and Atmosphere Research (EMME-CARE) project, our new detailed infrastructure map for power plants and gas flaring has been implemented in WRF-Chem simulations for the Middle-East region to complete the Emission Database for Global Atmospheric Research (EDGAR) as input. The EDGAR data consists of emissions by various sectors such as power plants, industry, residential, transportation and agriculture. Furthermore, hourly scaling factors have been applied to the anthropogenic emissions according to the electricity consumption of the particular urban areas, taking into account the weekly as well as the monthly variations. The periods under study are January 2021 and June 2021. By comparing the WRF-Chem outputs to TROPOMI satellite observations for NO2, the results show that the addition of point sources was crucial for the detection of some NO2 plumes. Moreover, the WRF-Chem model systematically overestimated the NO2 concentrations in the area with the current EDGAR dataset, therefore we introduced a new relationship between monthly and annual emissions for the Middle-East region. By carrying out WRF-Chem simulations with NO2 acting as a passive tracer it was also possible to examine the impact of the model chemistry in NO2 plumes development. Finally, CO2 was also simulated by the WRF-Chem model as a passive tracer and the results showed a good agrement with XCO2 data observed by the OCO-2 and OCO-3 instruments.

How to cite: Cheliotis, I., Lauvaux, T., Lian, J., Christoudias, T., Georgiou, G., Chevallier, F., Lei, R., and Ciais, P.: Optimization of simulated CO2 & NO2 concentrations for a detailed infrastructure map in the Middle East, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9518, https://doi.org/10.5194/egusphere-egu23-9518, 2023.

EGU23-10637 | ECS | PICO | AS3.17

Source characterization of VOCs at a coastal site in Hong Kong 

Qi Yuan, Meng Wang, Tao Wang, and Shuncheng Lee

Volatile organic compounds (VOCs) are important gaseous constituents in the troposphere, impacting local and regional air quality, human health, and climate both directly and indirectly (IPCC, 2013). With the participation of nitrogen oxides (NOx), oxidation of VOCs leads to tropospheric ozone (O3) formation, causing regional photochemical smog (Atkinson, 2000). In recent years, with the decline of ambient concentrations of other pollutants (e.g., fine particulate matter), the concentrations of O3 in many locations increased. Therefore, accurately apportioning the emission sources of ambient VOCs and then controlling them more effectively will play an important role in reducing O3 and secondary organic aerosol pollution in the atmosphere and improving public health.

  In this study, field measurements were conducted at a coastal site (Hok Tsui; HT) in Hong Kong from October to November 2020 with proton-transfer-reaction time-of-flight mass spectrometry (PTR-TOF-MS). VOC data coupled with air mass back trajectory cluster analysis and receptor modelling were applied to discuss the pollution pattern, regional transport, and emission sources of ambient VOCs at Hok Tsui in autumn 2020. Seven sources were identified from positive matrix factorization (PMF) analysis, namely vehicular + industrial, solvent usage, primary oxygenated VOCs (OVOCs), secondary OVOCs 1, secondary OVOCs 2 (aged), biogenic emissions, and background + biomass burning, contributing on average to 20.8%, 10.5%, 13.1%, 33.6%, 6.7%, 4.3%, and 10.9% of total VOC mixing ratios, respectively. Secondary OVOCs and vehicular + industrial emissions are the vital sources of ambient VOCs at Hok Tsui supersite. Integrated with backward trajectory analysis, long-range transport of air masses from inland and coastal regions of Southeast China brought more hydrocarbons from vehicular and industrial sources, and consequently more OVOCs in aged air masses. The results of this study highlighted the regional transport of anthropogenic VOCs should be considered in control strategies of VOCs and secondary air pollutants.

How to cite: Yuan, Q., Wang, M., Wang, T., and Lee, S.: Source characterization of VOCs at a coastal site in Hong Kong, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10637, https://doi.org/10.5194/egusphere-egu23-10637, 2023.

Current approaches to estimate NOx emissions fail to account for new and small sources, sources with large spatial and temporal variability, and sources which have significantly changed. Furthermore, the current generation of NOx emissions estimates don’t provide a sufficiently robust uncertainty analysis. They tend to use a fixed combination of localized models (in space and time), and do not adequately consider the variability in observed chemistry, dynamics, and thermodynamics. This work introduces a new, model-free analytical approach that assimilates daily-scale remotely sensed tropospheric columns of NO2 from TROPOMI in a mass-conserving manner, to invert daily NOx emissions. This approach is flexibly applied over a rapidly developing and energy-consuming region of Northwest China which is chosen due to substantial economic and population changes, new environmental policies, large use of coal, and access to independent emissions measurements for validation [EGT]. It is also applied over two densely urbanized regions, as well as their surrounding rural and rapidly developing outer suburban regions, including the Pearl River Delta and the Yangtze River Delta, both of which are chosen due to the amount and variability of sources, rapid economic development, and strong changes in environmental emissions policy and regulation. Over the EGT area, this technique computes a net NOx emissions gain of 70% distributed in a see-saw manner: emissions are more than doubled in cleaner regions, at chemical plants, and in regions thought to be emissions-free, while at the same time, emissions are more than halved in city centers and at other well-regulated and large commercial locations such as steel smelters and powerplants. There is a considerable amount of NOx emissions observed in suburban areas and rapidly developing rural areas, while a priori datasets do not account for these sources. A few interesting scientific points are explained in detail. First, the error over land surfaces which are not changing is smaller than the day-to-day variability, supporting the idea that daily variability is essential. The errors over areas undergoing land-use change and water are similar to or larger than the day-to-day variability. Second, source attribution is quantified with respect to the local thermodynamics of the combustion temperature, with measured atmospheric transport, and with in-situ chemical processing. Third, there are a significant number of sources identified which do not exist in the a priori datasets, but which are consistent with surface observations. Fourth, sensitivity runs are performed which account for the wide-range of uncertainty estimates of TROPOMI and the self-consistency of the estimated emissions is analyzed on a grid-by-grid and day-by-day basis, showing that the physically realistic constrains on the first order differential equation terms and bootstrapping approach are robust. It is hoped that these findings will drive a new approach to emissions estimation, one in which emissions are based consistently on remotely sensed measurements and associated uncertainties. Such approaches are essential in rapidly developing regions and in the Global South, where local measurements do not otherwise exist.

How to cite: Lu, L., Qin, K., and Cohen, J. B.: Computing Daily NOx Inversion over Energy Consuming and Urbanized Regions Using TROPOMI Data – A Novel Model Free Approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10999, https://doi.org/10.5194/egusphere-egu23-10999, 2023.

EGU23-11229 | ECS | PICO | AS3.17

Characterizing CO2 enhancements at major hotspots in South Korea using OCO-3 XCO2 retrievals 

Sung-Bin Park, Yeri Kang, Young-suk Oh, Chang-Keun Song, and Sang Seo Park

Consistent and long-term monitoring and understanding spatiotemporal distributions of carbon dioxide (CO2) in the atmosphere and local emission sources are essential to achieve the carbon neutrality by 2050. Quantifying accurate spatiotemporal CO2 enhancements is uneasy task because of its relatively long lifetimes in the atmosphere compared with methane and nitrogen dioxide. If the observatory is situated close to the area affected by transboundary air pollutants and local emission sources (e.g., cities, power plant, industrial areas etc.), estimating CO2 enhancements are even more challenging. Satellite CO2 observations are powerful to examine local to regional CO2 enhancements from the emission hotspot regions with wider spatial coverage compared with ground-based observatory. Especially, NASA's Orbiting Carbon Observatory-3 (OCO-3) has demonstrated its feasibility to quantify local CO2 emissions from the emission hotspots. To better understand source-sink characteristics of CO2 in South Korea, we examined spatiotemporal distributions in local CO2 enhancements of the several hotspots from the OCO-3 Level 2 bias-corrected column-averaged dry-air mole fractions of CO2 (XCO2) v10.4r. We determined CO2 enhancements utilizing monthly climatology statistics from the Fourier Transform Spectrometer (FTS) XCO2, Anmyeon-do (36.5382N, 126.3311E) in South Korea, subtracted from OCO-3 XCO2 at each pixel. We used FTS-XCO2 measurements from the update Total Carbon Column Observing Network (TCCON) GGG2020 retrieval algorithm. Our preliminary results suggest that CO2 enhancements over the major hotspots in South Korea showed wide ranges from -5 ~ 12 ppm measured from Snapshot Area Maps (SAMs) measurement modes. This large variability may be associated with the definition of enhancement determination, geographical location, and seasonal wind characteristics. We will discuss these potential error sources of uncertainties and how we can enhancement estimates to better quantify CO2 emissions. We anticipate our study provide insights for the robust and reliable quantifications of CO2 enhancements, establish an advanced level of the greenhouse gases and air quality monitoring strategy in South Korea.

How to cite: Park, S.-B., Kang, Y., Oh, Y., Song, C.-K., and Park, S. S.: Characterizing CO2 enhancements at major hotspots in South Korea using OCO-3 XCO2 retrievals, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11229, https://doi.org/10.5194/egusphere-egu23-11229, 2023.

EGU23-11273 | PICO | AS3.17

Is there an Ozone hole in the Tropics? 

Jayanarayanan Kuttippurath and Gopalakrishna Pillai Gopikrishnan

Amount of ozone in the stratosphere is very small as compared to other trace gases in the atmosphere. Yet, significant changes in its concentrations have great consequences in the environment and ecosystems. However, such drastic changes in ozone happens only in the high and middle latitudes, particularly in the polar spring, where chemical ozone loss occurs due to halogen-catalysed chemistry on polar stratospheric clouds. In the tropics, the amount of column ozone is very small and the ozone loss is also very small over the years, as compared to high and mid-latitudes. The ozone analyses in the tropical latitudes show a consistent picture of ozone evolution in the past four decades, as there is no significant loss or increase, although small negative trends are found. Recent studies have demonstrated that these negative trends in the tropical upwelling region are due to the increase in the speed of Brewer-Dobson Circulation, which brings tropospheric ozone to the lower stratosphere. This is clearly pictured in the time series of tropical ozone in recent years. The long-term trend in tropical total column ozone also shows no noticeable difference in recent years from the past decades. No measurements and no analyses show any signature of ozone hole in the tropics and all claims so far made are scientifically not sound and unconvincing. It is very unlikely that we would get an ozone hole outside the polar region.

How to cite: Kuttippurath, J. and Gopikrishnan, G. P.: Is there an Ozone hole in the Tropics?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11273, https://doi.org/10.5194/egusphere-egu23-11273, 2023.

EGU23-11281 | PICO | AS3.17

Greenhouse Gases Validation and Monitoring over the East Asia by Satellite-based Observation 

Byung-il Lee, Eunha Sohn, Junhyung Heo, Youngsuk Oh, Sangwon Joo, Junyeob Choi, Hyein Park, Myunghee Lee, and Yoonjae Kim

According to the 6th IPCC report, the concentration of greenhouse gases has increased about 20% since pre-industrial revolution, and 17% of them have increased over the last 10 years. The Korea Metoeorological Administration has analyzed satellite-based greenhouse gases to monitor climate change and support government’s achievement of net zero. The KMA has validated satellite-based greenhouse gases using CO2  observed in situ and retrieved TCCON in Anmyeon, the South Korea which is a GAW site. Both ground- and satellite-based CO2 showed a good agreement in their increasing trends with seasonal variations. However, satellite-based CO2 observed total column appear smaller than in situ observations affected by local sources due to observe near the surface, but agree well with TCCON observed the total column. The RMSD of GOSAT, and OCO2 with in situ and TCCON is estimated about 14.85, 16.93 and 2.81, 2.01 ppmv for a 1.0 degree × 1.0 degree spatial resolution on a daily time scale from January 2014 to December 2018. The results show that satellite-based products could be used greenhouse gases monitoring, but it needs to be verified more validation data.  We will present the detailed methods and results in the conference.

This work was funded by the Korea Meteorological Administration’s Research and Development Program “Technical Development on Weather Forecast Support and Convergence Service using Meteorological Satellites” under Grant (KMA2020-00120).

How to cite: Lee, B., Sohn, E., Heo, J., Oh, Y., Joo, S., Choi, J., Park, H., Lee, M., and Kim, Y.: Greenhouse Gases Validation and Monitoring over the East Asia by Satellite-based Observation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11281, https://doi.org/10.5194/egusphere-egu23-11281, 2023.

EGU23-11532 | PICO | AS3.17

Comprehensive measurements of speciated reactive nitrogen NOy and non-methane volatile organic compounds in Tokyo 

Satoshi Inomata, Hiroshi Tanimoto, Jun Matsumoto, Yasuhiro Sadanaga, and Shungo Kato

In Japan, concentrations of precursors of photochemical oxidants such as nitrogen oxides (NOx) and non-methane hydrocarbons (NMHCs) are decreasing year by year, but an improvement regarding photochemical oxidants is recently stagnant. To elucidate the reason, we have planned seasonal intensive observations in Tokyo, in which comprehensive measurements of speciated reactive nitrogen NOy and non-methane volatile organic compounds are performed. In summer of 2022, the observation was carried out at a campus of Tokyo Metropolitan University, a suburban area of Tokyo. In the intensive observation, NO, NO2, ΣPANs, ΣONs, HONO, HNO3, H2O2, SO2, O3, NH3, 28 NMHCs, and 10 oxygenated volatile organic compounds (OVOCs) were measured simultaneously. The ΣPANs and ΣONs were measured by thermal dissociation-cavity attenuated phase shift (CAPS) spectroscopy. The HONO, HNO3, and H2O2 were measured by negative ion chemical ionization mass spectrometry using I·(H2O)n as the reagent ion. The NMHCs, OVOCs and NH3 were measured by selected ion flow tube mass spectrometry and the data of NMHCs were compared and corrected with the data from gas chromatography/flame ionization detector (GC/FID). The ozone formation in Tokyo will be discussed.

How to cite: Inomata, S., Tanimoto, H., Matsumoto, J., Sadanaga, Y., and Kato, S.: Comprehensive measurements of speciated reactive nitrogen NOy and non-methane volatile organic compounds in Tokyo, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11532, https://doi.org/10.5194/egusphere-egu23-11532, 2023.

EGU23-11726 | ECS | PICO | AS3.17

A Comparison of Aircraft SO2 Measurements in Remote and Polluted Marine Environments 

Loren Temple, Stuart Young, Thomas Bannan, Stephanie Batten, Stéphane Bauguitte, Hugh Coe, James Lee, Emily Matthews, Dominika Pasternak, Andrew Rollins, Jake Vallow, and Pete Edwards

Sulfur dioxide (SO2) plays a pivotal role in the chemistry of the troposphere, ultimately affecting the Earth’s radiation balance and climate. Within the atmosphere, SO2 is oxidised by gas- and aqueous-phase chemistry to sulfate and is therefore a major precursor to atmospheric aerosols, particularly in the remote marine atmosphere. Both the direct radiative forcing from aerosols and the indirect forcing from aerosol-cloud interactions are poorly understood and produce large uncertainties in climate models. Therefore, it is of interest to precisely quantify the concentration of atmospheric SO2 if we are to predict the effects of changing emission rates on both climate and air quality.

Anthropogenic SO2 emissions have fallen dramatically in recent decades, resulting in significant reductions in atmospheric concentrations. Current commercial SO2 detection techniques, for example pulsed fluorescence, are no longer sensitive enough to detect trace levels of SO2 such as those found in remote marine environments. We report the development of a laser-induced fluorescence instrument for in situ SO2 measurements using a custom-built, tunable fiber-amplified laser system. Based on the system initially developed by Rollins et al. (2016), the University of York LIF-SO2 system has a detection limit of 50 ppt for 30 seconds and its relatively small size, weight and power requirements makes this instrument suitable for a variety of field campaigns.

Here we present aircraft measurements of SO2 made by the York LIF-SO2 instrument on board the UK FAAM research aircraft in both the remote and polluted marine boundary layer. These are then compared to simultaneous SO2 measurements made by the University of Manchester I- chemical ionisation mass spectrometer (I- CIMS) instrument and the FAAM pulsed fluorescence commercial SO2 detector.

How to cite: Temple, L., Young, S., Bannan, T., Batten, S., Bauguitte, S., Coe, H., Lee, J., Matthews, E., Pasternak, D., Rollins, A., Vallow, J., and Edwards, P.: A Comparison of Aircraft SO2 Measurements in Remote and Polluted Marine Environments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11726, https://doi.org/10.5194/egusphere-egu23-11726, 2023.

EGU23-12077 | ECS | PICO | AS3.17

Insights into the impact of COVID-19 lockdowns on USEPA PMF-5 derived PM2.5 source contributions at Bhopal, India 

Delwin Pullokaran, Ramya Sunder Raman, Ankur Bhardwaj, Deeksha Shukla, and Diksha Haswani

Fine particulate matter (PM2.5) is one of the major atmospheric components that is responsible for poor air quality and adverse health and climate effects. An identification of both primary emission sources as well as secondary formation mechanisms of PM2.5 is important to develop effective and efficient strategies to control and mitigate these adverse effects.

The COVID-19 pandemic had a significant impact on air quality across the globe through reduction in source emissions. This study examines the impact of the lockdown measures on PM2.5 and its chemical composition in Bhopal, India by comparisons with pre-lockdown period. Positive Matrix Factorization (PMF) (Paatero and Tapper, 1994) is the most widely used approach for factor analysis-based source apportionment studies. In this study the EPA PMF program version 5.0, was used to solve the PMF model. A comprehensive suite of instruments was used to measure the 24-hour integrated PM2.5 mass and its chemical composition collected onto various filter substrates every other day for two years (2019-2020) at Bhopal. This period coincides with the pre-lockdown, lockdown, and post-lockdown phases in India. The mass concentrations during the study period ranged between 54.7 µg m-3 during pre-lockdown and 45.1 µg m-3 in lockdown phase. PMF5 was applied to a dataset of organic and elemental carbon fractions (OC1, OC2, OC3, OC4, OP, EC1, EC2, EC3), nine major water-soluble inorganic components namely F-,Cl-, NO3- ,SO4-2,Na+, NH4+,Mg+2, K+, Ca+2, and elements (Al, Mg, Ca, Si, P, K, V, Ti, Co, Ni, Cu, As, Cr, Cd, Fe, Ni, Zn, Se, Sb, Ba, Pb) were used in the analysis.

Overall, the combined datasets (2019-2020) approach helped in better model resolution as several zeroes were present in both the loading and score matrices compared to a model run with 2019 data alone. An 8-factor solution was resolved with factors identified as coal and gasoline combustion, biomass burning, secondary sulfate, secondary nitrate, re-suspended crustal dust, diesel emissions, brick kiln emissions and mixed industrial emissions. Further, assessment of the pre-COVID and lockdown scenarios revealed a decreased in the mass contribution of diesel emissions (21.3%), mixed industrial emissions (13.7%), secondary sulfate (10.6%) and secondary nitrate (4.7%) during the lockdown phase compared to the pre-lockdown period at the study site. However, there was no decrease in the biomass burning source contribution due to no curbs on agricultural activities during the lockdown period in India. Overall, this study provides key insight into the source composition and contribution variations due to the reduction of specific anthropogenic source emissions due to COVID-19 lockdowns. Further, it is an added impetus for policymakers to implement targeted strategies and regulations, to reduce local and regional air pollution.

How to cite: Pullokaran, D., Sunder Raman, R., Bhardwaj, A., Shukla, D., and Haswani, D.: Insights into the impact of COVID-19 lockdowns on USEPA PMF-5 derived PM2.5 source contributions at Bhopal, India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12077, https://doi.org/10.5194/egusphere-egu23-12077, 2023.

EGU23-12745 | ECS | PICO | AS3.17

Unreported VOC emissions from road transport including from electric vehicles 

Samuel Cliff, Ally Lewis, Marvin Shaw, James Lee, Michael Flynn, Stephen Andrews, Jim Hopkins, Ruth Purvis, and Amber Yeoman

There are widespread policy assumptions that the phase-out of gasoline and diesel internal combustion engines will over time lead to much reduced emissions of Volatile Organic Compounds (VOCs) from road transport and related fuels. However, the use of real-world emissions measurements from a new mobile air quality monitoring station demonstrated a large underestimation of alcohol-based species in road transport emissions inventories. Scaling of industry sales statistics enabled the discrepancy to be attributed to the use of ancillary solvent products such as screenwash and deicer which are not included in internationally applied vehicle emission methodologies. A fleet average non-fuel non-exhaust VOC emission factor of 58 ± 39 mg veh−1 km−1 was calculated for the missing source, which is greater than the total of all VOCs emitted from vehicle exhausts and their associated evaporative fuel losses. These emissions are independent of the vehicle energy/propulsion system and therefore applicable to all road vehicle types including those with battery-electric powertrains. In contrast to predictions, vehicle VOC emissions may actually increase given a predicted growth in total vehicle kilometers driven in a future electrified fleet and will undergo a complete VOC respeciation due to the source change.

How to cite: Cliff, S., Lewis, A., Shaw, M., Lee, J., Flynn, M., Andrews, S., Hopkins, J., Purvis, R., and Yeoman, A.: Unreported VOC emissions from road transport including from electric vehicles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12745, https://doi.org/10.5194/egusphere-egu23-12745, 2023.

EGU23-12788 | ECS | PICO | AS3.17

Stratospheric ozone trends and attribution over 1984-2020 based on satellite data and model simulations with a regularised regression method 

Yajuan Li, Sandip Dhomse, Martyn Chipperfield, Wuhu Feng, Yuan Xia, Dong Guo, and Jianchun Bian

Accurate quantification of long-term trends in stratospheric ozone can be challenging due to their sensitivity to natural variability, the quality of the observational datasets, non-linear changes in forcing processes as well as the statistical methodologies. Multivariate linear regression (MLR) is the most commonly used tool for ozone trend analysis. However, the complex coupling in most atmospheric processes makes it prone to the over-fitting or multi-collinearity-related issue when using the conventional Ordinary Least Squares (OLS) setting. To overcome the multi-collinearity, we adopt a regularised (Ridge) regression method to quantify ozone trends and the influence of individual processes. Our MLR model setup is similar to the one used in Dhomse et al., (2022). Here, we use the Stratospheric Water and OzOne Satellite Homogenized (SWOOSH, Davis et al., 2016) merged data set (v2.7) to derive stratospheric ozone profile trends for the period 1984-2020. Beside SWOOSH, we also analyse a machine-learning-based satellite-corrected gap-free global stratospheric ozone profile dataset from a chemical transport model (ML-TOMCAT) (Dhomse et al., 2021), and output from two chemical transport model (TOMCAT) simulations forced with ECMWF reanalyses ERA-Interim and ERA5 (Li et al., 2022).

With Ridge regression, the stratospheric ozone profile trends from SWOOSH data show smaller declines during 1984-1997 compared to OLS with the largest differences in the lowermost stratosphere (>4 % per decade at 100 hPa). Upper stratospheric ozone has increased since 1998 with maximum (~2 % per decade near 2 hPa) in local winter for mid-latitudes. Negative trends with large uncertainties are observed in the lower stratosphere and are most pronounced in the tropics. The largest difference in post-1998 trend estimates between OLS and Ridge regression methods also appears in the tropical lower stratosphere (about ~7 % per decade difference at 100 hPa). Ozone variations associated with natural processes such as solar variability, ENSO, AO and AAO also indicate that Ridge regression coefficients are somewhat smaller and less variable compared to the OLS-based estimates. The ML-TOMCAT data set shows similar results to those using SWOOSH data while model simulations show larger inconsistencies especially in the lower stratosphere. The considerable differences between the satellite data and model simulations indicate that there are still large uncertainties in ozone trend estimates especially in the lower stratosphere where dynamical processes dominate, and caution is needed when discussing results if explanatory variables used are correlated.

References:

 Davis, S. M., et al., The Stratospheric Water and Ozone Satellite Homogenized (SWOOSH) database: a long-term database for climate studies, Earth Syst. Sci. Data, 8, 461–490, https://doi.org/10.5194/essd-8-461-2016, 2016.

Dhomse, S. S., et al., ML-TOMCAT: machine-learning-based satellite-corrected global stratospheric ozone profile data set from a chemical transport model, Earth Syst. Sci. Data, 13, 5711–5729, https://doi.org/10.5194/essd-13-5711-2021, 2021.

Dhomse, S. S., et al., A single-peak-structured solar cycle signal in stratospheric ozone based on Microwave Limb Sounder observations and model simulations, Atmos. Chem. Phys., 22, 903–916, https://doi.org/10.5194/acp-22-903-2022, 2022.

Li, Y., et al., Effects of reanalysis forcing fields on ozone trends and age of air from a chemical transport model, Atmos. Chem. Phys., 22, 10635–10656, https://doi.org/10.5194/acp-22-10635-2022,2022.

How to cite: Li, Y., Dhomse, S., Chipperfield, M., Feng, W., Xia, Y., Guo, D., and Bian, J.: Stratospheric ozone trends and attribution over 1984-2020 based on satellite data and model simulations with a regularised regression method, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12788, https://doi.org/10.5194/egusphere-egu23-12788, 2023.

EGU23-13119 | PICO | AS3.17

Are trends in total ozone consistent with stratospheric ozone trends from satellite observations? Are trends in total ozone consistent with stratospheric ozone trends from satellite observations? 

Mark Weber, Carlo Arosio, Alexei Rozanov, John P. Burrows, Viktoria Sofieva, Melanie Coldewey-Egbers, Diego Loyola, Vitali Fioletov, Stacey M. Frith, and Jeannette D. Wild

Total ozone is a measure of the protection of the biosphere from UV radiation. Extratropical total ozone recovery trends of about +0.5%/decade are consistent with the continuous decline in stratospheric halogen loading since the middle 1990s as a consequence of the Montreal Protocol and its Amendments on phasing out ODS. Nevertheless, the recovery (or chemistry-related) trends in the northern hemisphere (NH) are compensated by changes in atmospheric dynamics leading to stable ozone levels since about 2000 (apart from year-to-year variability). The near-global (60°S-60°N) average total ozone level is currently about 2-3% below the 1964-1980 mean.

Lower stratospheric ozone, the dominating contributor to the total ozone column and derived from limb satellite observations, shows globally (below 60° latitude) a slightly negative (but mostly statistically insignificant) trend of about -1.5%/decade since 2000, which is not consistent with the stable total ozone levels in the NH.  Some studies suggested that increases in tropospheric ozone compensate for negative lower stratospheric trends leading to stable column levels. The trend regression models applied to ozone profiles and total ozone also differ. For instance, proxies representing changes in atmospheric dynamics and transport have been included for total ozone, but not for ozone profiles, which may also lead to inconsistencies between total and stratospheric column trends.

This presentation will report updated total ozone trends from five merged total ozone datasets up to 2022. The same regression model, including proxies representing atmospheric dynamics and transport, will be then applied to ozone profiles from the merged limb dataset (SAGE II-SCIAMACHY-OMPS) to evaluate the consistency between column and profile trends.

How to cite: Weber, M., Arosio, C., Rozanov, A., Burrows, J. P., Sofieva, V., Coldewey-Egbers, M., Loyola, D., Fioletov, V., Frith, S. M., and Wild, J. D.: Are trends in total ozone consistent with stratospheric ozone trends from satellite observations? Are trends in total ozone consistent with stratospheric ozone trends from satellite observations?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13119, https://doi.org/10.5194/egusphere-egu23-13119, 2023.

EGU23-13122 | ECS | PICO | AS3.17

Trace gas retrievals from infrared emission spectrometry in the Arctic 

Lukas Heizmann, Mathias Palm, Justus Notholt, and Matthias Buschmann

Trace gas measurements are routinely performed using ground-based solar absorption spectroscopy in measurement networks such as NDACC (Network for Detection of Atmospheric Composition Change) and TCCON (Total Carbon Column Observing Network). For water vapour there exist radiosonde measurements providing high vertical resolution but limited temporal resolution. Retrievals from infrared emission spectrometry bridge a temporal gap in the measurement of trace gases during polar night. Measurements are possible dayround under cloud free conditions. At the AWIPEV site in Ny-Ålesund, Svalbard, we deploy a Bruker Vertex 80 FTIR emission spectrometer with a maximum resolution of 0.08 cm⁻¹ which is able to resolve individual spectral lines. We present optimal estimation retrievals of water vapour and methane. The results are compared to daily radiosonde measurements and TCCON retrievals. First results of applying our retrieval to emission spectra with a reduced resolution are also shown. This will in the future allow to include the retrieval on E-AERI-type instruments with their lower resolution deployed e.g. during the MOSAiC campaign.

How to cite: Heizmann, L., Palm, M., Notholt, J., and Buschmann, M.: Trace gas retrievals from infrared emission spectrometry in the Arctic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13122, https://doi.org/10.5194/egusphere-egu23-13122, 2023.

EGU23-13141 | ECS | PICO | AS3.17

Radiative impact of long-lived halocarbons and their atmospheric trends, derived from 15 years of IASI/Metop measurements 

Hélène De Longueville, Lieven Clarisse, Simon Whitburn, Cathy Clerbaux, and Pierre Coheur

In addition to being harmful to the ozone layer (for chlorinated and brominated compounds), halocarbons are also potent greenhouse gases. Their monitoring is therefore essential. Here we exploit measurements from the infrared satellite sounder IASI which offers the potential to robustly assess trends in the atmospheric abundances of trace gases owing to the stability and the consistency of the measurements made by three successive instruments over a period of more than 15 years. Despite their weak spectral signatures, we have recently reported the detection of eight long-lived halocarbons in IASI spectra: CFC-11, CFC-12, HCFC-22, HCFC-142b, HFC-134a, CF4, SF6 and CCl4.

In this work we exploit the available record of continuous IASI measurements to (1) determine the temporal evolution in atmospheric abundance of these species (2) quantify their radiative impact for the first time. We calculate their global radiative forcing based on integration over specific bands of IASI spectrally resolved fluxes (Whitburn et al., 2020[1]). Our results are validated with ground-based measurement networks and other remote sensors data. We conclude by assessing the usefulness of IASI and follow-on missions to contribute to the global monitoring of CFCs and their substitutes.


[1] Whitburn, S. et al. Spectrally resolved fluxes from IASI data: retrieval algorithm for clear-sky measurements. J. Clim. 33, 6971—6988 (2020).

How to cite: De Longueville, H., Clarisse, L., Whitburn, S., Clerbaux, C., and Coheur, P.: Radiative impact of long-lived halocarbons and their atmospheric trends, derived from 15 years of IASI/Metop measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13141, https://doi.org/10.5194/egusphere-egu23-13141, 2023.

Merging data records from different instruments into a consistent long-term data record is challenging process, especially when the parent datasets have a very short overlap or do not overlap at all. In addition, parent datasets can have different vertical resolutions and temporal and spatial samplings. In these cases, there is a need for a transfer standard - an independent data record that overlaps with parent datasets, allowing to characterize differences between the parent datasets and to derive absolute adjustments. In this study we discuss requirements for the transfer standard including long-term stability, spatial and temporal sampling. We estimate how various properties of the transfer standard affect stability of the merged record and derived long-term trends. We assess the impact of the transfer function on the trends of merged datasets from satellite observations, on the examples of merging ozone records from SAGE II / MIPAS / OMPS NASA and temperature records from HALOE / MIPAS, using EMAC, CMAM and WACCM model fields as transfer standards.

How to cite: Laeng, A.: Creating long-term climate data records using transfer functions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13965, https://doi.org/10.5194/egusphere-egu23-13965, 2023.

Measurements of BrO obtained in situ from the NASA ER-2 aircraft and balloons (HALOZ balloon-borne ClO/BrO instrument) between 1987 and 2000 are used to estimate the trend in total inorganic bromine (Bry). Despite the significance of ozone destruction by BrO, due to the analytical difficulty in quantifying very low abundances of bromine radicals present in the stratosphere these were the only direct observations of the dominant species of inorganic bromine that were made often enough over this period to allow for this analysis. In particular, this work focuses on observations in the perturbed polar vortices when BrO chemistry is dominated by reaction with ClO, and thus is less sensitive to systematic errors due to uncertainties in reactions with compounds such as HOx and NOx that dominate at lower latitudes. We use a detailed one-dimensional photochemical model with recommended rate parameters for key chemical processes, initialized with simultaneous observations of ClO and O3, to determine the atmospheric bromine partitioning under the specific photochemical conditions of each observation. We find that total inorganic bromine increased by ~43% over this time and reaches a value in 2000 that agrees well with the other observations that have since shown a leveling off, and small decrease, of inorganic bromine in the stratosphere since 2000. Within the accuracies of the BrO measurements and modeled partitioning, our results are consistent with a relatively constant value of 4 ppt find for very short-lived bromine substances (VSLSs) over the period of these observations. These results extend the Bry record deduced in recent WMO ozone assessments by 13 years and add further confidence to our understanding of ozone depletion due to bromine compounds over this critical period when inorganic bromine was increasing rapidly due to emissions of anthropogenic compounds, such as Halons and methyl bromide used in fire extinguishers and for fumigating crops.

How to cite: Toso, L. and Toohey, D. W.: The trend in stratospheric bromine from 1987 to 2000 deduced from in situ measurements of BrO in the Winter Polar Vortices, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14464, https://doi.org/10.5194/egusphere-egu23-14464, 2023.

Water vapour is the most important greenhouse gas in the Earth’s atmosphere, both, due to radiative forcing and the formation of clouds. The upper troposphere and lowermost stratosphere (UTLS) region is an especially sensitive region for climate radiative forcing. In the UTLS the air is cold with a large spatial and temporal variability of water vapour.  With the MOZAIC (Measurement of Ozone and Water Vapor by Airbus In-Service Aircraft) data it was recently shown that in the extratropical UT close to the tropopause the air is nearly saturated with respect to ice and contains a significant fraction of ice-supersaturated regions (ISSRs) (Petzold et al., ACP, 2020, doi.org/10.5194/acp-20-8157-2020).

In the present study we investigate the long-term changes of water vapour in the tropopause region using the combined time series of MOZAIC and IAGOS (In-Service Aircraft for a Global Observing System; www.iagos.org). Their observation systems are deployed on a fleet of commercial aircraft and aim at the provision of long-term, regular, and spatially resolved in situ observations of the atmospheric composition on a global scale. The combined water vapour and relative humidity time series spans now more than 27 years and is comprised of nearly 65000 flights. This makes the data set well-suited for long-term characterization of the water vapour distribution in the extratropical UTLS, namely at mid-latitudes with highest flight densities.

 We will present analyses of the time series from 1996 to 2020 for long-term changes of absolute humidity, temperature, relative humidity with respect to ice (RHice) and occurrence of ISSRs. Our focus lies on different altitude levels in the UTLS at northern mid-latitudes over the regions Eastern North America, North Atlantic and Europe.

How to cite: Rohs, S., Smit, H., Blomel, T., Li, Y., Bundke, U., and Petzold, A.: Evaluation of long-term changes of upper tropospheric and lower stratospheric water vapour and ice supersaturated regions in different altitudes and geographical regions derived from MOZAIC and IAGOS routine in-situ observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14733, https://doi.org/10.5194/egusphere-egu23-14733, 2023.

EGU23-14974 | ECS | PICO | AS3.17

Sensitivities of atmospheric ozone to supersonic emissions above the transatlantic flight corridor 

Jurriaan van 't Hoff, Volker Grewe, and Irene Dedoussi

The rapid growth of the global aviation market has spurred commercial interest in the redevelopment of a civil supersonic aviation market. The emissions of these aircraft are expected to have an adverse impact on climate, as well as changing the composition of the ozone layer [1,2,3,4]. There is however still considerable uncertainty about the scale of future civil supersonic adoption, as well as future emissions, due to the rapid development of the technology and potential changes in regulations.

Evaluating the impacts of the wide range of future adoption scenarios is computationally demanding, but atmospheric sensitivities might be used to assist the evaluation. Here, we use the GEOS-Chem global chemistry transport model to evaluate the impact of supersonic fuel burn perturbations above the transatlantic flight corridor on global ozone in a modern atmosphere over a period of 10 years. Variations of this scenario are evaluated to assess global ozone sensitivities to the emission of NOx, SOx, H2O, CO, and hydrocarbons across multiple altitudes between 17.2 and 21.4 km, as well as the cross-sensitivities between the emissions of NOx, SOx, and H2O.

From the sensitivities it is found that changes in global ozone columns are primarily driven by NOx emissions in this emission region, followed by SOx and H2O, with marginal contributions from CO and hydrocarbon emissions. The impact of these emissions is found to depend strongly on altitude, with higher emission altitudes increasing ozone depletion from NOx, SOx, and H2O, emissions. For kerosene-based emissions above the transatlantic flight corridor, the effect of cross-sensitivities between the emitted species is estimated to be up to two orders of magnitude smaller than direct responses to emission species. This difference implies that the effect of cross-sensitivities on ozone may be neglected in predictive models at a small cost in accuracy, simplifying future development efforts. Considering this application, future work will first need to apply this method to global emission networks where the effect of cross-sensitivities might differ from the region presented here.

 

References:

[1] Matthes, S., Lee, D. S., …, Terrenoire, E., Review: The Effects of Supersonic Aviation on Ozone and Climate, Aerospace, 9(1), 41, (2022).

[2] Eastham, S. D., Fritz, T.,  …, Barrett, S. R. H., Impacts of a near-future supersonic aircraft fleet on atmospheric composition and climate. Environmental Science: Atmospheres. doi:10.1039/d1ea00081k, (2022).

[3] Zhang, J., Wuebbles, D., Kinnison, D., & Baughcum, S. L., Stratospheric Ozone and Climate Forcing Sensitivity to Cruise Altitudes for Fleets of Potential Supersonic Transport Aircraft. Journal of Geophysical Research: Atmospheres, 126(16), (2021).

[4] Grewe, V., Stenke, A., ..., Pascuillo, E., Climate impact of supersonic air traffic: an approach to optimize a potential future supersonic fleet – results from the EU-project SCENIC. Atmospheric Chemistry and Physics, 7(19), 5129-5145, (2007).

How to cite: van 't Hoff, J., Grewe, V., and Dedoussi, I.: Sensitivities of atmospheric ozone to supersonic emissions above the transatlantic flight corridor, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14974, https://doi.org/10.5194/egusphere-egu23-14974, 2023.

EGU23-15201 | PICO | AS3.17

The state of greenhouse gases in the atmosphere using global observations through 2021 

Oksana Tarasova, Alex Vermeulen, Yousuke Sawa, Sander Houweling, and Ed Dlugokencky

This paper highlights the main findings of the eighteenth annual Greenhouse Gas Bulletin (https://library.wmo.int/index.php?lvl=notice_display&id=22149) of the World Meteorological Organization (WMO). The results are based on research and observations performed by laboratories contributing to the WMO Global Atmosphere Watch (GAW) Programme (https://community.wmo.int/activity-areas/gaw).

The Bulletin presents global analyses of observational data collected according to GAW recommended practices and submitted to the World Data Center for Greenhouse Gases (WDCGG). Bulletins are prepared by the WMO/GAW Scientific Advisory Group on Greenhouse Gases in collaboration with WDCGG.

Observations used for the global analysis are from more than 100 marine and terrestrial sites worldwide for CO2 and CH4 and at a smaller number of sites for other greenhouse gases. The globally averaged surface mole fractions calculated from this in situ network reached new highs in 2021, with CO2 at 415.7 ± 0.2 ppm, CH4 at 1908 ± 2 ppb and N2O at 334.0 ± 0.1 ppb. These values constitute, respectively, 149%, 262% and 124% of pre-industrial (before 1750) levels. The increase in CO2 from 2020 to 2021 was equal to that observed from 2019 to 2020 and larger than the average annual growth rate over the last decade. For CH4, the increase from 2020 to 2021 was higher than that observed from 2019 to 2020 and considerably higher than the average annual growth rate over the last decade. For N2O, the increase from 2020 to 2021 was slightly higher than that observed from 2019 to 2020 and also higher than the average annual growth rate over the last decade.

The Bulletin highlights the exceptional growth of CH4 in 2020 and 2021. The causes of these exceptional increases are still being investigated though analyses of measurements of atmospheric CH4 abundance and its stable carbon isotope ratio 13C/12C indicate that the increase in CH4 since 2007 is associated mostly with biogenic processes, but the relative contributions of anthropogenic and natural sources to this increase are unclear.

The Bulletin further highlights that the accuracy of emissions estimates from atmospheric measurements depends on the geometry of the surface network, pointing to the large observational gaps in tropical regions and the interior of the Asian continent. The tropics accommodate not only highly uncertain emissions from natural wetlands, but also the atmospheric hydroxyl radical sink of CH4, which is largest there. Surface measurements provide limited information to distinguish between increasing surface emissions and decreasing atmospheric sinks, which could both explain the increasing atmospheric CH4 abundance.

WMO is working with the broader greenhouse gas community to develop a framework for sustained, internationally coordinated global greenhouse gas monitoring. These efforts are envisaged to result in an internationally coordinated approach to observing network design and acquisition, international exchange and use of the observations. It is foreseen that this will result in the expansion of the in-situ network, especially in currently undersampled regions and lead to reduced uncertainties in the quantification of the net atmospheric balance of CH4 and other greenhouse gases.

How to cite: Tarasova, O., Vermeulen, A., Sawa, Y., Houweling, S., and Dlugokencky, E.: The state of greenhouse gases in the atmosphere using global observations through 2021, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15201, https://doi.org/10.5194/egusphere-egu23-15201, 2023.

EGU23-16386 | PICO | AS3.17

Measuring Atmospheric Hydrogen Ahead of the Anticipated Hydrogen Economy 

Blagoj Mitrevski, Elise-Andree Guerette, Ray Langenfelds, Matthew Woodhouse, Darren Spenser, Paul Krummel, and Paul Steele

The continuous population and economy growth demands more energy, currently provided predominantly by burning of fossil fuels. However, the depletion of fossil fuel resources and the detrimental environmental impacts of burning fossil fuels are driving the public opinion and governments towards renewable energy (RE) sources. Solar and wind power are the most promising, but its reliability is shadowed by their weather dependence. Hydrogen is considered as a very promising energy carrier which can overcome the limitations of the existing RE sources. Producing hydrogen at the solar panel fields or incorporating water electrolysers within wind turbines will smooth the energy supply, and even reduce the energy transport. If the hydrogen economy takes effect as anticipated, then the hydrogen impact on the climate needs to be re-assessed. In order to simulate future hydrogen concentrations, it is necessary to build a model which can simulate present day hydrogen emissions and sinks, and resultant atmospheric concentrations, which are currently infrequently measured. Building a history of hydrogen measurements opens up possibilities in the future to determine background and pre-existing hydrogen sources, and gives a baseline before the switch to a hydrogen economy.

Historically, Reduction Gas Analysers (RGA) were the workhorse in the laboratory and field, where reductive gasses like hydrogen or carbon monoxide release mercury gas by passing along a heated solid mercuric oxide bed, which in turn is analysed by ultraviolet (UV) absorption. The method is well established but lacks linear response and stability. CSIRO is working on novel methods for more accurate and precise hydrogen measurement. The Pulsed Discharge Helium Ionization Detector, or simply PDD, is an alternative to the RGA. CSIRO has been operating a PDD for hydrogen at Cape Grim (along with the classic RGA) for 7.5 years using shared calibration tanks. The mean difference between them (50,000+ matched data points, when pollution events are removed) is just 0.02 ppb, proving PDD’s incredible compatibility with the established RGA technique. The PDD also has a demonstrated superior precision and linearity compared to the RGA. Another two PDD systems are operational at Aspendale measuring urban hydrogen since 2019 and 2021. The later one is to be deployed at the CSIRO Clayton site, where Aspendale will relocate to in 2025. Another PDD system is in a development stage, able to measure not just hydrogen, but many other atmospheric gases (CH4, CO2, N2O, Kr, Xe). The inability of optical instruments to measure hydrogen (homonuclear diatomic molecule) will mean that there will be an increased demand for RGA or PDD measurements of hydrogen in the future.

How to cite: Mitrevski, B., Guerette, E.-A., Langenfelds, R., Woodhouse, M., Spenser, D., Krummel, P., and Steele, P.: Measuring Atmospheric Hydrogen Ahead of the Anticipated Hydrogen Economy, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16386, https://doi.org/10.5194/egusphere-egu23-16386, 2023.

EGU23-17382 | PICO | AS3.17

The MAESTRO Spectrophotometer on Canada’s SCISAT satellite: Advances in data processing and improved data products 

C. Thomas McElroy, Kaley A. Walker, James R. Drummond, Jiansheng Zou, and Paul S. Jeffery

The ACE-FTS and MAESTRO instruments have now been operating on the Canadian Space Agency’s SCISAT satellite as the Atmospheric Chemistry Experiment (ACE) for nearly 20 years.  The ACE satellite is approximately 1 m in diameter and 1 m deep and has a mass of 150 kg.  The Measurement of Aerosol in the Stratosphere and Troposphere Retrieved by Occultation (MAESTRO) spectrophotometer continues to measure ozone, water vapour and aerosol in the stratosphere and upper troposphere.  Like the ACE‑FTS, MAESTRO delivers results from nearly 30 occultation measurements per day, but with a higher vertical resolution of just over 1 km over a range as large as 5 to 40 km as meteorological conditions allow.  It measures from 500 nm to 1000 nm with a resolution of 1 to 2 nm.  The instrument design and performance will be briefly discussed and the algorithms developed to process the data and deal with peculiarities in the performance of the satellite will be described. 

Significant progress has been made recently in improving the retrievals that has resulted in improved accuracy and a larger number of successful retrievals at lower altitudes.  A new dataset with these improvements will be available for other researchers.  Some examples which illustrate the improvements will be presented.

The ACE satellite was funded by the Canadian Space Agency (CSA) and launched by NASA. The CSA funds the MAESTRO data processing.  Environment Canada (EC) partly funded the construction of the MAESTRO instrument. 

How to cite: McElroy, C. T., Walker, K. A., Drummond, J. R., Zou, J., and Jeffery, P. S.: The MAESTRO Spectrophotometer on Canada’s SCISAT satellite: Advances in data processing and improved data products, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17382, https://doi.org/10.5194/egusphere-egu23-17382, 2023.

EGU23-905 | ECS | PICO | AS3.18

Ozone production and chemical regime analysis in the upper tropical troposphere 

Clara M. Nussbaumer, Andrea Pozzer, Jos Lelieveld, and Horst Fischer

Ozone is a greenhouse gas and, after water, the second most relevant contributor to global warming in the upper troposphere. Therefore, understanding and monitoring the processes contributing to ozone production is an important tool in observing the progression of climate change. The two main tropospheric precursors to ozone formation are nitrogen oxides (NOx = NO + NO2) and volatile organic compounds (VOC). Depending on their availability, ozone production can be limited by either of its precursors. In our study, we focus on processes contributing to ozone formation and loss in the upper tropical troposphere, where changes in ozone have one of the largest impacts on the radiative forcing. Based on modeled trace gas concentrations and meteorological parameters by the EMAC atmospheric chemistry - general circulation model, we analyze a variety of metrics including net ozone production rates (NOPR), the formaldehyde (HCHO) to NO2 ratio and the share of methyl peroxyradicals (CH3O2) forming HCHO (αCH3O2) in their ability to indicate the dominating ozone regime in the upper troposphere between 30°N and 30°S latitude.

How to cite: Nussbaumer, C. M., Pozzer, A., Lelieveld, J., and Fischer, H.: Ozone production and chemical regime analysis in the upper tropical troposphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-905, https://doi.org/10.5194/egusphere-egu23-905, 2023.

Many studies have been conducted to address the surface ozone pollution issue over China, but few model works focus on the background ozone, a metric to represent the best surface ozone levels that can be achieved through emission controls. Here we apply a state-of-art global chemical transport model GEOS-Chem High Performance (GCHP) to understand the sources contributing to Chinese background (CNB) daily maximum 8 h average (MDA8) ozone, and to identify the driving factor of its interannual variability from 2015 to 2019.

The five-year-mean CNB ozone is estimated as 37.8 ppbv, showing a general west-to-east downward gradient. The national-mean CNB ozone levels are the largest in summer (42.5 ppbv), but distinct seasonality can be seen at different regions. Using the tagged ozone technique, we show that the high background levels in western China are due to abundant transport from the free troposphere and adjacent foreign regions, while in eastern China, domestic ozone formation near surface from natural precursors is also important and exhibits intensive seasonal variation. CNB ozone enhancements from lightning NOx, soil NOx, and biogenic volatile organic compound (BVOC) emissions are estimated as 8.1, 6.4 and 3.9 ppbv, respectively, in summertime. We found the greater importance of BVOC over soil NOx to ozone as reported in previous studies is reversed when domestic anthropogenic emissions are turned off, reflecting a more NOx-sensitive ozone chemical regime in a “clean” atmosphere.

The interannual variability (IAV) of CNB ozone shows the peak in summer, with standard deviation values during five years of ~5 ppbv over Qinghai-Tibet Plateau (QTP) and >3.5 ppbv over vast eastern China. CNB levels in QTP are found to be well correlated with horizontal circulation anomalies at 500 hPa, while in the east, year-to-year changes in soil NOx emissions dominate the IAV of CNB ozone. We further explore the role of El Nino-Southern Oscillation (ENSO) in modulating the IAV of CNB ozone over southern China in spring. Compared to the La Nina event, the enhanced precipitation and decreased temperature during El Nino inhibit CNB ozone formation in southeast China. However, heat and drought events, as well as enhanced biomass burning emissions during El Nino in Mainland Southeast Asia can largely worsen ozone there, and further rise CNB levels in southwest China under the southerly wind.

How to cite: Ye, X. and Zhang, L.: The Exploration of 2015-2019 Surface Background Ozone over China: A Model Study by GEOS-Chem High Performance (GCHP), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1272, https://doi.org/10.5194/egusphere-egu23-1272, 2023.

Ozone is a highly oxidative gas affecting human health, especially the impacts on the cardiovascular and respiratory systems. Ozone is usually formed through photochemical reactions outdoors and transported to the indoor environment. Occupants indoors might face an accumulated irritant issue due to high ozone reacting with human skin to produce several volatile organic compounds (VOCs), such as geranyl acetone (Ga), 6-methyl-5-hepten-2-one (6-MHO) and 4-oxopentanal (4-OPA), which might irritate skin and respiratory tract. In this study, the indoor air quality in a university classroom was monitored using air quality boxes (AQBs) comprising low-cost sensors for various gas species, including ozone, CO2, NOx, etc. The interaction processes between outdoor and indoor air, and human interference were investigated via a box model simulation of CO2 and ozone temporal profiles. Both indoor CO2 and ozone were significantly affected by the ventilation and number of occupants. CO2 is primarily produced via human respiration and diluted via ventilation in the classroom, so the simulation of CO2 profiles retrieves the ventilation efficiency and occupancy variation. With the derived parameters, ozone, mainly transported from the outdoors and consumed by room and human surface, is estimated to have deposition velocities of 0.028±0.0053 cm s-1 and 0.45±0.15 cm s-1 for room and human surface, respectively, consistent with the literature. The generation of Ga, 6-MHO, and 4-OPA depends on ozone consumption on human surfaces, and those VOCs might accumulate indoors for several ppb in a crowned room with poor ventilation. The integration of observation using low-cost sensors with the model simulation quantifies the physical and chemical processes controlling indoor ozone and organic ozonolysis. Furthermore, it might provide proper ventilation strategies to maintain good indoor air quality with energy efficiency based on the occupants.

How to cite: Chen, F., Huang, W.-C., Hwang, W.-C., and Hung, H.-M.: The Interaction and Health Impacts between Ozone and Occupants Indoor: Observation and Model Simulation in a University Classroom, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1564, https://doi.org/10.5194/egusphere-egu23-1564, 2023.

EGU23-1594 | ECS | PICO | AS3.18

The Footprint of Growing Stratospheric Transport Contribution in Tropospheric Ozone 

Xiaodan Ma, Jianping Huang, Michael Sprenger, Michaela Imelda Hegglin, Patrick Jöckel, and Tianliang Zhao

The long-term ozone changes in the middle to upper troposphere, of importance to climate radiative forcing and setting the baseline for tropospheric ozone pollution, are not well quantified from observations in East Asia. In this study, three decades of observations from ozone soundings are examined with meteorological reanalysis data and climate model simulations to characterize regional features in tropospheric ozone and investigate their driving factors along the northwestern Pacific coastal region. A rapid increase in ozone is observed in the middle to upper troposphere over Naha (26 oN), Tsukuba (36 oN), and Sapporo (43 oN) in the warm season during 1990‒2020. Coincidentally, tongue-shaped hotspots with high tropospheric ozone extending from the stratosphere occur during the warm season. The timing for these ozone hotspots shows a time lag from late spring to summer with the increasing latitude of the observation sites. Intensified stratospheric intrusion (i.e., tropopause folding) events and enhanced buildup of ozone abundance in the lowermost stratosphere (likely driven by climate change) are the key factors causing the large increase over this region. With the aid of the chemistry climate model EMAC, the enhanced downward transport of stratospheric ozone into the troposphere is revealed by a surge in the stratospheric ozone tracer in the troposphere.

How to cite: Ma, X., Huang, J., Sprenger, M., Hegglin, M. I., Jöckel, P., and Zhao, T.: The Footprint of Growing Stratospheric Transport Contribution in Tropospheric Ozone, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1594, https://doi.org/10.5194/egusphere-egu23-1594, 2023.

EGU23-1848 | PICO | AS3.18

The TOAR data infrastructure: A generalised database infrastructure for environmental time series 

Sabine Schröder, Niklas Selke, and Martin G. Schultz

In all areas of research, robust, versatile and high-performance data infrastructures are needed.

TOAR is a global research project to analyze the spatial distribution and temporal evolution of ozone in the troposphere and to provide data of surface ozone measurements and its precursors for assessing the impact of ozone on human health, vegetation and climate.

These observational data are collected from various environmental agencies and programs, universities and individual researchers under different requirements for data formats, metadata standards and quality control, and are harmonized and quality-controlled into the TOAR database using our infrastructure. All data in the database are easily accessible through open, freely available and well-documented web services. The TOAR data centre team is committed to the FAIR principles and aims to achieve the highest standards with respect to data curation, archival, and re-use. We established a common approach for data ingestion to ensure that data from different sources is handled in a defined and equal way and that all modifications are recorded in a provenance log. Clear rules are defined how the submitted metadata is mapped into the metadata schema used by the TOAR database. To harmonize the data quality, we employ automated tests of different granularity using statistical methods and heuristics, which assign a score for each data point. Those scores are then translated into categorical data quality flags.

The TOAR data infrastructure has proven that it can handle large amounts of data operationally in a performant way. It not only provides standardized REST-API access to the underlying database but also allows for the integration and linking of additional services. For example, the results of the quality control tool mentioned above can be accessed as interactive charts with tables of aggregated figures. Furthermore, we offer analysis services that implement a variety of statistical evaluations and metrics to allow users to get aggregated, ready-to-use data in a consistent, reproducible, and interoperable manner and also allow for bulk raw data downloads. It is also possible to invoke a service to calculate air pollution trends with quantile regression.

During development, we emphasized the reusability of the database infrastructure code. Therefore, we believe that the database layout, the related workflows for data ingestion and processing, and the service architecture can be transferred to other types of environmental data and perhaps even to data from other disciplines.

With the TOAR database infrastructure, the TOAR community receives a cutting-edge repository and system of web services that allows for easy-to-use, fast, flexible, and reproducible analyses of air pollution and associated data.

How to cite: Schröder, S., Selke, N., and Schultz, M. G.: The TOAR data infrastructure: A generalised database infrastructure for environmental time series, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1848, https://doi.org/10.5194/egusphere-egu23-1848, 2023.

Statistical downscaling models are used to estimate historical and future ozone concentrations in Europe for the summer months from April to September. The basis is formed by over 700 measuring stations from the hourly Air Quality eReporting ozone pollution data from the European Environment Agency. Daily maximum 8-hr running means (MDA8) as well as daily maximum 1-hr values (MDA1) of ozone are the target variables. Meteorological (ERA5) as well as ozone (CAMS) reanalysis data serve as predictors in the perfect prognosis (PP) approaches. A station-specific, individualized predictor screening guarantees site-specific optimums. The predictor selection is performed using regularization with varying shrinkage. Multiple Linear Regression (MLR) is used to model the relationship between all selected predictors and MDA8/ MDA1. An ensemble of seven CMIP6 Earth system models is used to estimate future ozone concentrations. Projections are calculated for the years 2041-2060 and 2081-2100 under two different future scenarios (SSP2-4.5 and SSP3-7.0). The CMIP6 data is bias corrected with a univariate quantile delta mapping method, before being used in the statistical models.

With respect to predictor selection, a sensitivity study is conducted, testing different sets of predictors to examine their influence on future ozone concentrations. Predictor sets with and without ozone, with only thermal and radiative predictors, and additionally thermo-dynamical or circulation-dynamical information are analyzed, in addition to the site-specific optimums described above.

The projection results of the different predictor settings highlight the importance of ozone as predictor. In all predictor sets with included ozone, the results of the two scenarios SSP2-4.5 and SSP3-7.0 differ in their sign depending on the scenario used. The SSP2 scenario, called "Middle of the Road", leads to decreasing ozone concentrations in Europe, while the more pessimistic SSP3 scenario results in partly strong increases of harmful ground-level ozone concentrations. In contrast, all predictor sets that do not take ozone into account show consistently positive change signals.

On the one hand, our results point to the need to include information on emission changes in statistical assessments in order to obtain a realistic picture of future ozone development. Furthermore, our research underscores the need to further reduce air pollution in Europe to better protect human health from direct emissions such as NOx and indirect pollutants such as ozone.

How to cite: Kaspar-Ott, I., Jahn, S., and Hertig, E.: Future ground-level summer ozone concentrations in Europe: the importance of ozone as predictor in a statistical downscaling approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2204, https://doi.org/10.5194/egusphere-egu23-2204, 2023.

EGU23-2687 | ECS | PICO | AS3.18

An investigation of the contributions of VOCs to urban ozone production in the U.K. 

Rayne Holland, M. Anwar H. Khan, and Dudley Shallcross

Ambient concentrations of 23 volatile organic compounds (VOCs) measured at London Marylebone Road (LMR), an urban traffic site in the UK were analysed over a period of 22 years (1998-2019) to assess the impact of pollution control strategies. A significant decrease in ambient concentration is seen for the majority of VOCs analysed with total VOC burden decreasing by 76% across the period studied, likely as a result of legislative controls. This analysis was extended to consider the contribution of VOCs to ozone formation at this site utilising POCP values. Similarly, the overall reactivity of the VOC burden at LMR has resulted in a significant decrease of just under 12% per year in ozone formation potential over 1998-2019 at this site. The declines in ozone formation potential for VOCs associated with road traffic emissions are all in good agreement at 11-13% decrease per year. VOCs related to non-traffic sources, namely ethane and propane from natural gas leakage, did not see a significant decline over the study period. The variation and composition of the overall VOC burden was compared across three decadal time periods (1998-2000, 2001-2010, 2011-2019) and saw an increase in significance of these pollutants (with ethane and propane moving from the fifth and eleventh largest contributors in 1998-2000 to the first and second largest contributors in 2011-2019, respectively) suggesting they are not sufficiently controlled under current legislation. The increase in significance of ethane and propane was mirrored in their contribution to ozone generation potential but ethene continues to substantially dominate in contribution to ozone formation potential by a factor of 4 and 5 compared with ethane and propane, respectively. Alkanes are typically considered to be less important in the context of ozone formation potential due to their low reactivity in comparison to other VOCs. Analysis presented herein demonstrates the negative impact of ignoring such emissions as their influence begins to grow such that alkanes now represent 3 of the 5 highest contributors to tropospheric ozone formation at this site (in order of contribution: ethene > propene > n-butane > ethane > propane). The importance of high-quality gas-phase kinetic studies to determine the impact of VOCs in ozone production is clear and the usefulness of metrics such as POCPs is demonstrated.

How to cite: Holland, R., Khan, M. A. H., and Shallcross, D.: An investigation of the contributions of VOCs to urban ozone production in the U.K., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2687, https://doi.org/10.5194/egusphere-egu23-2687, 2023.

Carbon monoxide (CO) plays an important role in both air quality and climate. Photochemical oxidation of CO produces ozone (O3) and carbon dioxide (CO2) while also affecting the lifetime of methane (CH4) through reactions with the hydroxyl radical (OH). Because CO2, CH4 and O3 are greenhouse gases, emissions of CO have an indirect radiative forcing, estimated at 0.22 W/m2. Ground-level O3 and CO are also air pollutants that affect human and ecosystem health. Quantifying trends in carbon monoxide is essential for understanding trends in tropospheric ozone, especially in background regions. Using the 22-year data record from MOPITT (Measurements of Pollution In The Troposphere), we show global and regional trends from satellite observations of atmospheric CO. We also examine trends in CO emissions based on model inversions for CO emitted by biomass burning (BB) and fossil fuels (FF) and from chemical production from emissions of biogenic (BG) VOCs (volatile organic compounds). We find that CO concentrations and CO emissions from BB and FF have been mostly decreasing globally, with some notable regional exceptions.

How to cite: Worden, H. and Buchholz, R.: Global and regional trends of atmospheric carbon monoxide – a background ozone precursor, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2952, https://doi.org/10.5194/egusphere-egu23-2952, 2023.

EGU23-2959 | PICO | AS3.18 | Highlight

Global-scale reductions in free tropospheric ozone in 2020-2022 associated with decreased pollution due to COVID-19 and impact on trends 

Jerry Ziemke, Natalya Kramarova, Stacey Frith, and Liang-Kang Huang

NASA satellite measurements show that ozone reductions throughout the Northern Hemisphere (NH) free troposphere reported for spring-summer 2020 during the COronaVIrus Disease 2019 (COVID-19) pandemic have occurred again in spring-summer 2021.  The satellite measurements show that tropospheric column ozone (TCO) (mostly representative of the free troposphere) for 20oN-60oN during spring-summer for both 2020 and 2021 averaged ~3 Dobson Units (DU) (or ~7-8%) below normal.  These ozone reductions in 2020 and 2021 were the lowest over the 2005-2021 record.  We also include satellite measurements of tropospheric NO2 that exhibit reductions of ~10-20% in the NH in early spring-to-summer 2020 and 2021, suggesting that reduced pollution was the main cause for the low anomalies in NH TCO in 2020 and 2021.  Reductions of TCO ~2 DU (7 %) are also measured in the Southern Hemisphere in austral summer but are not associated with reduced NO2.  We also extend our analyses to show that year 2022 spring-summer anomalies in NH tropospheric NO2 and free tropospheric ozone from the satellite measurements still remained below pre-COVID levels.

 

How to cite: Ziemke, J., Kramarova, N., Frith, S., and Huang, L.-K.: Global-scale reductions in free tropospheric ozone in 2020-2022 associated with decreased pollution due to COVID-19 and impact on trends, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2959, https://doi.org/10.5194/egusphere-egu23-2959, 2023.

EGU23-3552 | PICO | AS3.18

Tropospheric Ozone Trends in the Arctic 

Katharine Law, Jens Liengaard Hjorth, Jakob Pernov, Cyndi Whaley, Henrik Skov, Martine Collaud Coen, Joakim Langner, and Stephen Arnold and the Arctic tropospheric ozone team

Tropospheric ozone, an important air pollutant and short-lived climate forcer, is changing globally with reported increases over emission regions that can influence ozone downwind. Here, ozone trends are examined in the Arctic troposphere, where surface warming is around four times faster than the global mean. Trends at the surface and in the free troposphere are estimated for 1993-2019 using available surface and ozonesonde data. Observed trends are also compared to modelled trends from the Arctic Monitoring Assessment Project (AMAP) multi-model evaluation, where models were run with the same anthropogenic emissions from 1990 to 2015 (Whaley et al., 2022, ACP). Findings include observed increases in annual mean surface ozone at Arctic coastal sites notably driven by increases during winter that are concurrent with decreasing surface carbon monoxide trends. Positive trends are also diagnosed at most high-Arctic ozonesonde sites in the wintertime free troposphere (up to 400 hPa). These ozone increases, which tend to be overestimated by the multi-model median (MMM) trends, are likely to be due to reductions in anthropogenic emission of nitrogen oxides at mid-latitudes leading to less ozone titration and influencing northern hemispheric ozone. Springtime increases are also found at the surface in northern coastal Alaska/Greenland but not in the MMMs. Causes are unknown but may be related to changing Arctic sea-ice or weather patterns affecting ozone sources or sinks. In contrast, surface ozone trends in northern Scandinavia are negative during spring, likely a response to decreasing ozone precursor emissions in Europe. MMM trends are also negative but generally overestimated. Springtime trends in the free troposphere also tend to be negative while summer trends are positive. Changes in ozone precursor emissions, the downward stratospheric ozone flux or general circulation may be contributing to these seasonal variations in the trends. The implications of these reported trends and model behaviour are discussed.

How to cite: Law, K., Liengaard Hjorth, J., Pernov, J., Whaley, C., Skov, H., Collaud Coen, M., Langner, J., and Arnold, S. and the Arctic tropospheric ozone team: Tropospheric Ozone Trends in the Arctic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3552, https://doi.org/10.5194/egusphere-egu23-3552, 2023.

EGU23-3737 | PICO | AS3.18

The global distribution and trends of ozone health-based metrics:  New results from the TOAR-II Database 

Owen Cooper, Kai-Lan Chang, Sabine Schröder, Niklas Selke, J. Jason West, and Marc Serre

The first phase of the Tropospheric Ozone Assessment Report (TOAR-I), an activity of the International Global Atmospheric Chemistry Project (IGAC), provided the first comprehensive view of surface ozone’s global distribution and trends, based on all available surface ozone observations.  TOAR-I focused on a present-day period of 2010-2014, and calculated trends for a range of periods, but primarily focused on the most recent years of 2000-2014, plus long-term trends from the 1970s/1980s through 2014.  Subsequent studies of ozone trends using data after the TOAR-I cut-off of 2014, have shown a wide range of trends, both positive and negative, at monitoring sites around the world.  To keep up with the rapid changes of ozone at urban, rural and remote locations this study provides current world-wide ozone trends using observations through 2021, archived in the newly updated TOAR-II Database of Surface Observations.  Focus is placed on two ozone metrics relevant to human health impacts:  1) the annual peak of the 6-month running mean of maximum daily 8-hour average ozone; this metric is used by Global Burden of Disease (GBD) to estimate mortality due to long-term ozone exposure; 2) the number of days per year that exceed 70 ppbv, based on the maximum daily 8-hour average ozone value; this value corresponds to the primary U.S. National Ambient Air Quality Standards for ozone and is relevant to short-term ozone exposure.  Global maps will indicate the regions of the world where the potential for ozone impacts on human health are greatest (and least), and will show regions where ozone air quality is either improving or degrading.  Despite our effort to use all available surface ozone observations, large data gaps exist across many regions of the world, especially in developing nations, and GBD maps generated by data fusion will be used to identify, and to estimate ozone levels in the data-poor regions. 

How to cite: Cooper, O., Chang, K.-L., Schröder, S., Selke, N., West, J. J., and Serre, M.: The global distribution and trends of ozone health-based metrics:  New results from the TOAR-II Database, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3737, https://doi.org/10.5194/egusphere-egu23-3737, 2023.

EGU23-5103 | ECS | PICO | AS3.18

Drivers of Increasing Ozone during the Two Phases of Clean Air Actions in China 

Yuxi Liu, Guannan Geng, Jing Cheng, Yang Liu, Qingyang Xiao, Liangke Liu, Qinren Shi, and Qiang Zhang

In response to the severe air pollution issue, the Chinese government implemented two phases (Phase I: 2013-2017, Phase II: 2018-2020) of clean air actions since 2013, resulting in a significant decline in fine particles (PM2.5) during 2013-2020, while the maximum daily 8 h average ozone (MDA8 O3) increased by 2.6 μg m-3 yr-1 during the same period. Here, we derived the drivers behind the rising O3 concentrations during the two phases of clean air actions by using a bottom-up emission inventory, a regional chemical transport model, and a multiple linear regression model. We found that both meteorological variations (3.6 μg m-3) and anthropogenic emissions (6.7 μg m-3) contributed to the growth of MDA8 O3 from 2013 to 2020, with the changes in anthropogenic emissions playing a more important role. The anthropogenic contributions to the O3 rise during 2017-2020 (1.2 μg m-3) were much lower than that in 2013-2017 (5.2 μg m-3). The lack of volatile organic compound (VOC) control and the decline in nitrogen oxides (NOX) emissions were responsible for the O3 increase in 2013-2017 due to VOC-limited regimes in most urban areas, while the synergistic control of VOC and NOX in Phase II initially worked to mitigate O3 pollution during 2018-2020, although its effectiveness was offset by the penalty of PM2.5 decline. Future mitigation efforts should pay more attention to the simultaneous control of VOC and NOX to improve O3 air quality.

How to cite: Liu, Y., Geng, G., Cheng, J., Liu, Y., Xiao, Q., Liu, L., Shi, Q., and Zhang, Q.: Drivers of Increasing Ozone during the Two Phases of Clean Air Actions in China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5103, https://doi.org/10.5194/egusphere-egu23-5103, 2023.

EGU23-5293 | PICO | AS3.18

Present-day distribution of tropospheric ozone and precursors in the tropics 

Bastien Sauvage, Audrey Gaudel, Suvarna Fadnavis, Maria Tsivlidou, Pallavi Saxena, Brice Barret, Meng Li, Bhupendra Bahadur Singh, Renu Masiwal, Saurabh Sonwani, Ulas Im, Yann Cohen, Saumya Singh, Daan Hubert, Arno Keppens, Jean-Christopher Lambert, Catherine Wespes, Irina Petropavlovskikh, Giacomo Gerosa, and Helen Worden and the List of co-authors

As part of the Ozone and Precursors in the Tropics (OPT) working group of the Tropospheric Ozone Assessment Report Phase 2 (TOAR-II), we present the first results on the distribution of tropospheric ozone (O3) and its precursors (carbon monoxide, CO; formaldehyde, HCHO; nitrogen dioxide, NO2) in the tropics over the past 20-25 years. The goal is to give an overview of the seasonal, geographical and vertical variabilities of tropical tropospheric O3 and its precursors. To do so, we use in situ measurements of O3 and its precursors from surface sites, sounding balloons (SHADOZ) and instrumented aircraft (IAGOS and ATOM), as well as ground-based (FTIR) and spatial (IASI, OMI, GOME-2) remote-sensed observations. The observations are averaged monthly over the longest available time-period as well as over the first five years of the time period. The results for these two time periods give the context to interpret distributions and variabilities of O3 and its precursors over the most recent five years as we call it “Present-day”.  Special emphasis is given to the differences of O3 and its precursors’ distributions between remote and polluted regions and to the relationships between the gaseous species. Model output will be included to fill gaps in space and time when necessary to help the interpretation of the analysis based on observations.

From IAGOS measurements, the highest O3 and CO maxima occur in the lower troposphere of Northern Hemisphere Africa, which remains the most influenced by biomass burning. CO maxima are attributed using SOFT-IO model to anthropogenic emissions by 60%. Second maxima are observed in the lower troposphere of Asia, mostly due to anthropogenic emissions. The highest amount of transported CO in the tropics originates from Africa.

How to cite: Sauvage, B., Gaudel, A., Fadnavis, S., Tsivlidou, M., Saxena, P., Barret, B., Li, M., Singh, B. B., Masiwal, R., Sonwani, S., Im, U., Cohen, Y., Singh, S., Hubert, D., Keppens, A., Lambert, J.-C., Wespes, C., Petropavlovskikh, I., Gerosa, G., and Worden, H. and the List of co-authors: Present-day distribution of tropospheric ozone and precursors in the tropics, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5293, https://doi.org/10.5194/egusphere-egu23-5293, 2023.

EGU23-5600 | ECS | PICO | AS3.18 | Highlight

Long-term Ozone Trends in Different Urban Developments 

Beth Nelson, James Lee, and Keding Lu

High emissions of NOx and anthropogenic VOCs from urban areas are a major source of tropospheric ozone production. Tropospheric ozone is a secondary air pollutant that is harmful to human health as well as crop and ecosystem productivity, and an important greenhouse gas. It is formed from the chemical processing of NOx and VOCs in a non-linear cycle, making ozone reduction strategies challenging. Urban centres across the world are developing at different rates and emitting different combinations and concentrations of chemical species, resulting in location specific drivers of urban ozone concentrations. Alongside this, different countries and cities have implemented a wide range of location specific air quality and climate change measures to reduce air pollution and greenhouse gas emissions. The diversity of these policies over the past few decades has further led to different outcomes for secondary pollutant formation across the globe.

As part of TOAR-II, the Urban Ozone Working Group explores the long-term trends in urban ozone concentrations over the past 20 years on a global scale. Using ground based data from global Air Quality networks, trends in ozone concentrations of > 12 cities across different continents are presented, and temporal changes in ozone trends are identified. This study utilises the TOAR database, accessed via the TOAR Data Portal, which collects hourly data of long-term surface air quality measurements from over 10,000 stations globally. Where sufficient long-term NOx and VOC data are available, ozone concentration trends are compared to trends in its precursor species. 

Trends in ozone concentrations are then related to the state of development of the city using factors such as GDP and the UN City Development Index, and an assessment of how cities in different phases of development are contributing to tropospheric ozone across the world is discussed. Trends in ozone will also be compared to country and city specific changes in air quality and net zero policy interventions.

How to cite: Nelson, B., Lee, J., and Lu, K.: Long-term Ozone Trends in Different Urban Developments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5600, https://doi.org/10.5194/egusphere-egu23-5600, 2023.

EGU23-6682 | ECS | PICO | AS3.18 | Highlight

Fingerprints of the COVID-19 economic downturn and recovery on ozone anomalies at remote high-altitude sites in North America and Western Europe 

Davide Putero, Owen R. Cooper, Gregory Beachley, Kai-Lan Chang, Cédric Couret, Peter Effertz, Dan Jaffe, Jason Lynch, Irina Petropavlovskikh, Melissa Puchalski, Timothy Sharac, Barkley C. Sive, Martin Steinbacher, Carlos Torres, and Paolo Cristofanelli

With a few exceptions, most of the studies on tropospheric ozone (O3) variability following the restriction measures related to the spread of COVID-19 focused on emissions-prone or urban environments. In this work, we investigated the impact of the pandemic restriction measures on surface O3 at several high-altitude remote and rural sites across North America and Western Europe. O3 monthly anomalies, computed with respect to the baseline period 2000–2019, were calculated for 2020 and 2021, to explore the impact of the economic downturn in 2020 and the economic recovery in 2021. A total of 41 high-altitude sites were analyzed: 5 remote stations in western Europe, 19 rural sites in the western US, 4 sites in the western US downwind of highly polluted areas, 4 sites in the eastern US, plus 9 remote sites across the globe to provide a "global" picture for comparison. In 2020, most of European high-altitude sites showed persistent negative anomalies for spring (March-May, i.e., MAM; average of -1.8 ppb) and summer (June-August, i.e., JJA; -2.7 ppb), except for April (1.8 ppb). The pattern was similar in 2021 (-1.8 ppb for both MAM and JJA), except for June (1.8 ppb). The sites in the western US showed similar behavior, with negative anomalies in 2020 (-2.1 ppb for MAM and -0.5 ppb for JJA), and 2021 (-0.5 ppb for MAM). However, the JJA seasonal average was influenced by strong positive anomalies in July, due to the large spread of wildfires in the western US. The polluted rural sites in the western US showed a negative O3 anomaly for MAM 2020, and a slight recovery in 2021, resulting in a positive anomaly for MAM and alternating positive and negative anomalies in JJA. The eastern US sites were characterized by below baseline numbers for both MAM and JJA 2020, while in 2021 the negative values generated a "dipole" structure, with the western sites influenced by the presence of wildfires. Concerning the rest of the world, a global picture could not be drawn, as the sites, spanning a range of different environments, did not show consistent anomalies across the globe. A few sites did not experience any relevant variations (e.g., the Antarctic sites), while others showed signals of influence from the surrounding environment, or behaviors like those observed for European and US remote sites. We also attempted anomaly attribution by analyzing the behavior of several O3 precursors (e.g., surface and columnar CO, NO, and NO2) from the CAMS reanalysis, and the patterns of emissions reductions for 2019, 2020, and 2021.

How to cite: Putero, D., Cooper, O. R., Beachley, G., Chang, K.-L., Couret, C., Effertz, P., Jaffe, D., Lynch, J., Petropavlovskikh, I., Puchalski, M., Sharac, T., Sive, B. C., Steinbacher, M., Torres, C., and Cristofanelli, P.: Fingerprints of the COVID-19 economic downturn and recovery on ozone anomalies at remote high-altitude sites in North America and Western Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6682, https://doi.org/10.5194/egusphere-egu23-6682, 2023.

EGU23-7127 | ECS | PICO | AS3.18

Emerging of surface ozone pollution beyond summer season over the North China Plain 

Ke Li, Danyuting Zhang, and Jie Hou

Surface ozone pollution is of great concern in current air quality management in China. The North China Plain (NCP), which is home to 300 million people, has the highest ozone level and increasing trend.  While earlier studies of ozone pollution focused on summer season, here we show that ozone pollution out of summer season over the North China Plain is also very emerging.  Firstly, ozone has been very low during winter haze (particulate) pollution episodes. However, the abrupt decrease of NOx emissions following the COVID-19 lockdown in January 2020 reveals a switch to fast ozone production during winter haze episodes with MDA8 ozone of 60 to 70 ppb. This remarkable switch to an ozone-producing regime in January–February following the lockdown illustrates a more general tendency since 2013 of increasing winter–spring ozone in the North China Plain and increasing association of high ozone with winter haze events, as pollution control efforts have targeted NOx emissions while VOC emissions have limited regulations. Secondly, we find that ozone episodes comparable with those in summer season can also occur in early-autumn over NCP, resulting in the emerging of two-peak ozone pollution (June and September) for some years. The statistical analysis show that this interannual variation is driven by the anomalies in the large-scale sea surface temperature (SST) patterns. These results highlight the urgency of ozone pollution controls out of summer season in China.

How to cite: Li, K., Zhang, D., and Hou, J.: Emerging of surface ozone pollution beyond summer season over the North China Plain, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7127, https://doi.org/10.5194/egusphere-egu23-7127, 2023.

EGU23-7163 | PICO | AS3.18

Decreasing trends in extreme ozone events across the United States 

Kai-Lan Chang and Owen Cooper
This work presents a comprehensive regional trend analysis of surface ozone observations across the contiguous United States, using 25 years of data from 62 rural monitoring sites, and based on quantile regression and change point analysis. We highlight that the ozone exceedance events (based on the daily maximum 8-hour average and a threshold of 70 ppb) in recent years (2017-2021) are largely diminished compared to two decades ago (1995-2003) in the eastern US and across much of the western US. Ozone exceedance events in recent years are mainly observed in California during the fire season. Results based on thresholds of 60, 50 and 35 ppb will also be discussed.
 

How to cite: Chang, K.-L. and Cooper, O.: Decreasing trends in extreme ozone events across the United States, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7163, https://doi.org/10.5194/egusphere-egu23-7163, 2023.

EGU23-7946 | PICO | AS3.18

Assessment of crop yield losses for Triticum aestivum in Punjab and Haryana using in-situ measurements, relay seeding experiments and the DO3SE model 

Baerbel Sinha, Sneha Saha, Aakanksha Meena, Sukhwinder Singh, Pankaj Kharra, Adarsh Adarsh, Ashish Ashish, Sanjay Anand, and Yadav Ram Kishore

Measurements of leaf-level stomatal conductance (gsto) are central to the ozone (O3) risk assessment as the allow to recorded environmental response functions that describe how a wheat cultivar responds to different environmental stressors. The calculation of Triticum aestivum yield loss based on the absorbed O3 phytotoxic dose over a threshold of y (PODy) has been introduced as a new way to conduct ozone  risk assessment. 

In this study we present environmental response functions of two triticum aestivum cultivars grown as irrigated winter wheat in the state of Punjab, in the North West Indo Gangetic Plain based on measurements conducted during winter 2016-17, 2017-18, and 2018-19. The cultivars PBW550 and HD2967 were directly obtained from breeders and were sown on November 15th in 2016-17 and 2017-18, and in a relay seeding experiment on November 1st, 15th and December 1st in 2018-19.

We use meteorological observations and ozone measurements obtained at the Central Atmospheric Chemistry facility of IISER Mohali in Punjab, India between November 2016 and April 2019 to derive environmental response function for these two cultivars and estimate triticum aestivum relative yield losses and crop production losses due to ozone. We demonstrate that environmental response functions are not only useful to assess the impact of ozone on plant growth but that they can also be used to assess the impact of heat stress and climate change on yields. We show that modifying the phenology function used in the DO3SE assessment such that it incorporates the impact of heat stress experienced between anthesis to maturity permits a more accurate assessment of the impact of ozone on the wheat yield. We also demonstrate that a thermal time calculation method that is consistent with the temperature response function used in the DO3SE improves the quality of the assessment.

We evaluate the impact of both heat stress and ozone exposure during different growth stages on several yield parameters including the number of active tillers, 1000-grain weight, flower sterility, number of shrivelled grains.

Late sowing typically not only results into high thermal stress during sensitive growth stages, but also in higher ozone exposure. We find that PBW550 is more sensitive to stress during the grain filling stage than HD2967. However, for both cultivars moderate heat and ozone stress can be associated with superior rather than reduced yields in the real world. We explain this yield-loss yield paradox with the help of meteorological observations.

How to cite: Sinha, B., Saha, S., Meena, A., Singh, S., Kharra, P., Adarsh, A., Ashish, A., Anand, S., and Ram Kishore, Y.: Assessment of crop yield losses for Triticum aestivum in Punjab and Haryana using in-situ measurements, relay seeding experiments and the DO3SE model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7946, https://doi.org/10.5194/egusphere-egu23-7946, 2023.

EGU23-9365 | PICO | AS3.18

Trends of tropical tropospheric ozone and its precursors 

Audrey Gaudel and Bastien Sauvage and the TOAR-OPT Paper 2 "Trends" Team

As part of the Tropospheric Ozone Assessment Report Phase 2 (TOAR-II), the Ozone and Precursors in Tropics (OPT) working group counts three deliverables dedicated to quantifying 1) the distribution, 2) the trends of tropospheric ozone (O3) and its precursors (carbon monoxide, CO; formaldehyde, HCHO; nitrogen dioxide, NO2) in the tropics over the past 20-25 years, and 3) their impacts on a global scale. This presentation will focus on the trends estimate. We answer the following scientific questions: How have tropical tropospheric ozone and its precursors changed with time? What sources (e.g. anthropogenic emissions, biomass burning, lightning) drive these trends and to what extent?

To accomplish this, we use both observations and model output.  The observations include in situ measurements of O3 and its precursors from surface sites, sounding balloons (SHADOZ) and instrumented aircraft (IAGOS), as well as ground-based (FTIR) and spatial (IASI, OMI, GOME-2) remote-sensed observations. Global model output come from ECHAM6-HAMMOZ, LMDZ-OR-INCA, MIROC-CHASER, CAM4-Chem, GISS-E2 and the CESM2-WACCM6 ensemble.

The trends estimates are based on monthly anomalies and are calculated after considering climate variabilities such as El Niño- Southern oscillation (ENSO) and quasi-biennial oscillation (QBO).

From IAGOS and SHADOZ ozone profiles, we estimate positive ozone trends between 1994 and 2019 throughout the troposphere above the Americas, Africa, India, Southeast Asia and Malaysia/Indonesia. Trends may reach up to 6 ± 1.6 ppb/decade in the free troposphere and up to 12.5 ± 2 ppb/decade in the boundary layer. There is also considerable regional variability. For example, trends are +0 to 4 ppb/decade in the free troposphere above the remote Pacific and Atlantic SHADOZ stations (1998-2019). According to OMI satellite retrievals, tropospheric ozone burden increases between 2004 and 2021 across the tropical latitude band (20˚N-20˚S) and the trends range between 0.09 Tg/yr (OMI CCD retrieval in the southern hemisphere) and 0.3 Tg/year (OMI/MLS retrieval in the northern hemisphere).

The presentation will also include trends estimates of observed ozone’s precursors such as CO, NO2 and formaldehyde as well as trends estimate of ozone and its precursors from model output.

How to cite: Gaudel, A. and Sauvage, B. and the TOAR-OPT Paper 2 "Trends" Team: Trends of tropical tropospheric ozone and its precursors, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9365, https://doi.org/10.5194/egusphere-egu23-9365, 2023.

EGU23-9772 | PICO | AS3.18 | Highlight

Surface ozone trends and precursor attribution in South America 

Rodrigo Seguel, Lucas Castillo, Charlie Opazo, Néstor Rojas, Thiago Nogueira, María Cazorla, Mario Gavidia, Laura Gallardo, Yasin Elshorbany, and Camilo Menares

Several Working Groups have been established within the frame of the second phase of the Tropospheric Ozone Assessment Report (TOAR-II). The Tropospheric Ozone Precursors focus Working Group (TOP WG) aims to examine the current regional and global distribution, variability and trends of ozone precursors. Part of our strategy has been to analyze in greater detail different regions of the globe. In particular, this work addresses South America, a region characterized by densely populated urban areas with high air pollution levels.

We use data from air quality monitoring networks that measure surface-level ozone, nitrogen oxides, carbon monoxide and meteorological variables. To date, we have validated and incorporated monitoring stations from Brazil (51), Chile (18), Colombia (13) and Ecuador (6) into our central database. To evaluate short- and long-term ozone exposure, we use the maximum daily 8-hour average (MDA8) and the peak season guideline proposed by the World Health Organization (WHO) set at 51 and 31 ppbv, respectively. We applied the Quantile Regression (QR) method to analyze ozone and precursor network trends. We also identified points in time series that mark changes in trends through a piecewise function.

The highest MDA8 ozone for 2015-2021 was found in São Paulo (52 ppbv) and Santiago (51 ppbv). In São Paulo, the short-term ozone exposure decreased by 7% compared to the average of the years prior to 2015 (period analyzed in TOAR phase I), while in Santiago, it increased by 10%. In Bogota and Quito, the MDA8 complied with the WHO guidelines (33 and 32 ppbv, respectively). Similarly, the long-term ozone exposure guideline was exceeded in São Paulo (39 ppbv) and Santiago (40 ppbv), while Bogota (25 ppbv) and Quito (26 ppbv) complied. The trend analysis showed that Quito was the only city with a negative ozone trend of -0.10 ppb/year (50th percentile) for the analyzed period. In turn, the São Paulo trend increased after 2008 (0.43 ppbv/year), while Santiago and Bogota have increased since 2017 (0.93 ppbv/year and 1.3 ppbv/year, respectively). We highlight that the positive trend in Santiago is driven mainly by the high percentiles (>70th). Underlying processes that explain trends involve more efficient photochemical ozone formation (e.g., NO2/NOx trend) and meteorological factors.

This ongoing work aims to include more South American cities and background stations already available in the new TOAR database. Finally, we will project ozone trends for the next decade using machine learning techniques (random forest) under precursor emission scenarios and temperature projections.

How to cite: Seguel, R., Castillo, L., Opazo, C., Rojas, N., Nogueira, T., Cazorla, M., Gavidia, M., Gallardo, L., Elshorbany, Y., and Menares, C.: Surface ozone trends and precursor attribution in South America, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9772, https://doi.org/10.5194/egusphere-egu23-9772, 2023.

EGU23-10700 | ECS | PICO | AS3.18

The influences of ozone precursor changes in tropical regions on tropospheric ozone burden 

Yuqiang Zhang, Lin Li, Tao Tang, Audrey Gaudel, Bastien Sauvage, and J. Jason West and the Yuqiang Zhang

Tropospheric ozone is an important greenhouse gas, is detrimental to human health and crop and ecosystem productivity, and controls the oxidizing capacity of the troposphere. Previous studies, using models, aircraft and remote observation datasets, have shown that the tropospheric ozone has increased significantly in the tropical regions. Sensitivities studies have also showed that the ozone precursor emissions in these tropical regions have been increasing for the past three decades. For this paper, we will work with worldwide scientists to investigate how the emission evolves in the tropical regions from 1995 to 2019, and how these changes have contributed to the global and other receptor regions tropospheric ozone burden increases, by using ensemble state-of-the-art global and regional chemical transport models.

How to cite: Zhang, Y., Li, L., Tang, T., Gaudel, A., Sauvage, B., and West, J. J. and the Yuqiang Zhang: The influences of ozone precursor changes in tropical regions on tropospheric ozone burden, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10700, https://doi.org/10.5194/egusphere-egu23-10700, 2023.

EGU23-10969 | PICO | AS3.18

Volatile Organic Compound Measurements and Oxidant Modeling at a Remote Mountain Site in the western North Pacific 

Stephen M. Griffith, Wen-Tzu Liu, Fang-I Chen, Elmia Hidayati, Chih-Chung Chang, Jia-Lin Wang, and Neng-Huei Lin

Anthropogenic pollution, including primary compounds such as nitrogen oxides (NOx) and organics, but also secondary pollutants such as ozone, are a threat to sensitive mountain ecosystems, which are already under continued threat of diminished area, due to climate change. This study analyzes two days of volatile organic compound (VOC) concentrations, including a limited set of carbonyls, at the Lulin Atmospheric Background Station (LABS; 2,862 meters asl), which is a well-known remote sub-tropical site that receives long-range transported air masses from various clean and polluted origins. VOCs were sampled in a canister and analyzed by GC-MS/FID, while carbonyls were trapped on Supelco DNPH-coated cartridges and quantified by HPLC-UV. Routine LABS measurements of ozone, CO, and PM2.5 were also utilized; Copernicus Atmospheric Monitoring Service (CAMS) reanalysis NOx and HNO3 concentrations were further incorporated into an oxidant modeling analysis. In comparing the two sampling days, the first day was characterized by hazier conditions (~3 times higher PM2.5 concentrations) and 2-3 times higher VOC and CO concentrations and calculated OH reactivity values. Based on a HYSPLIT back-trajectory analysis, the first day was influenced by air that had a longer residence time at lower altitudes over South China, while the second day was characterized by higher level transport. Also influential at the site are subsidence events that bring drier air that can contain high ozone and NOy species. The measurement and reanalysis data were incorporated into a 0-dimensional modeling analysis (F0AM) of the gas-phase oxidation chemistry in order to further characterize the different air masses that influence this sensitive mountain area. While the first day also was simulated to have higher level of ozone production, the second day captured an afternoon spike in pollutants and ozone production that was likely driven by upslope mountain valley air sourced for lower altitudes in Taiwan. Thus, the oxidation potential in this environment is characterized by large swings driven by local upslope pollution, subsidence events, and long-range transported pollution from the Asian continent, which ultimately dictate the pollutant exposure for this sensitive ecosystem.

How to cite: Griffith, S. M., Liu, W.-T., Chen, F.-I., Hidayati, E., Chang, C.-C., Wang, J.-L., and Lin, N.-H.: Volatile Organic Compound Measurements and Oxidant Modeling at a Remote Mountain Site in the western North Pacific, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10969, https://doi.org/10.5194/egusphere-egu23-10969, 2023.

The variability of ozone (O3) concentration in China has received wide attention since the emission reduction policies were implemented in 2013. At present, it is still a great challenge to clarify the causes of O3 change in the Yangtze River Delta (YRD) region. In this work, we applied the Community Multiscale Air Quality (CMAQ) model to investigate the impacts of precursor emissions (such as non-methane volatile organic compounds (NMVOCs) and nitrogen oxides (NOX)) and meteorological conditions on the summertime maximum daily 8-h average (MDA8) O3 variation in Nanjing, a megacity in YRD between 2015 and 2020. The meteorological contribution was quantified by the difference between the sensitive scenario fixing the anthropogenic emission at 2015 level while remaining the meteorology unchanged in 2020 and baseline scenario in 2015. The impact of anthropogenic emissions was then estimated by the difference between the total change of observed MDA8 O3 and the meteorological contribution. Compared with 2015, the observed MDA8 O3 in Nanjing decreased by 19.1 μg/m3 during August in 2020, with the meteorological conditions and anthropogenic emissions contributing 8.4 μg/m3 (44%) and 10.7 μg/m3 (56%), respectively. The anthropogenic emissions of VOCs and NOX in Nanjing in August 2020 decreased by 7.8% and 11.7%. Temperature, relative humidity (RH) and wind filed are key meteorological parameters affecting the O3 formation. The lower temperature (30.3 ℃ in 2020 compared with 32.4 ℃ in 2015) and higher RH (76.9% in 2020 and 56.9% in 2015) in early August (especially in 4-5) as well as the clean air mass brought by the stronger wind (5.1 m/s in 2020 and 2.5 m/s in 2015) during August 13-14 in 2020 mainly resulted in a drop of O3. The longer hydroxyl radical (OH) chain length and higher ozone production efficiency (OPE) indicate that the reduction of anthropogenic emissions accelerated the NOX cycle and makes O3 more sensitive to NOX. Using the EKMA diagram, we estimated that O3 formation has shifted from VOCs-limited in 2015 to a transition regime jointly controlled by VOCs and NOX in 2020. Our study is consistent with previous ones that in reducing the urban ozone pollution, both the precursor emissions and meteorological conditions should be considered that with the benefit of meteorological conditions, reasonable emission reduction measures could have a positive effect on the reduction of O3 concentration in Nanjing during August in 2015 and 2020.

How to cite: Li, L., Li, J., Qin, M., Xie, X., and Hu, J.: Impacts of anthropogenic and non-anthropogenic factors on summertime ozone variation from 2015 to 2020 in the Yangtze River Delta, China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11130, https://doi.org/10.5194/egusphere-egu23-11130, 2023.

We present an update on the status of the tropospheric ozone data products retrieved from satellite observations. Specifically, we will highlight data from the TRopospheric Ozone and its Precursors from Earth System Sounding (TROPESS) project which is a NASA effort that provides retrievals of atmospheric ozone utilizing radiances from a variety of different satellite instruments. The TROPESS project provides ozone data that provides additional data that can used with record established by the Tropospheric Emission Spectrometer (TES) which flew on NASA’s Aura satellite. The new multispectral retrievals of ozone utilize the (Multi-Spectra, Multi-Species, Multi-Sensors Retrievals of Trace Gases (MUSES) retrieval framework to produce consistent estimations of ozone from different satellite radiances. TROPESS ozone data products include those using data from the Atmospheric Infrared Sounder (AIRS), the Ozone Monitoring Instrument (OMI) and the Cross-track Infrared Sounder (CrIS) instruments. The TROPESS joint-satellite data products provide ozone retrievals with vertical sensitivity similar to that seen in TES observations and allow a continuation of the TES ozone data record. Utilizing satellite instruments that observe with wide swaths will provide much broader spatial sampling than TES was able to provide.

The TROPESS team is currently processing ozone data records using radiances from CrIS, AIRS, OMI, TROPOMI and retrievals using combinations of the different satellites. All of the TROPESS products are being validated through comparisons to ozonesondes as well as comparisons to chemical reanalysis products. We will provide an update on the results from these comparisons as well highlighting the differences in vertical sensitivity and spatial sampling of the different products. We will highlight the differences in the sensitivity of the retrievals to ozone in the troposphere and validation of the satellite retrievals at those pressure levels. We will show statistical analysis for the errors in the satellite retrievals and their comparisons to the ozonesondes.

Lastly, we will present results showing the time record of the different ozone products, including showing how the comparisons to models and ozonesondes change with time. Utilizing the AIRS and OMI instrument data will allow us to examine the tropospheric ozone data record going back to 2005 and we will share results of how the TROPESS products can contribute to determining trends in tropospheric ozone.

How to cite: Osterman, G. and Bowman, K.: Update on the TROPESS ozone data products: Evaluation, validation and a preliminary examination of their utility in tropospheric ozone trend analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11258, https://doi.org/10.5194/egusphere-egu23-11258, 2023.

EGU23-11274 | ECS | PICO | AS3.18

Trends in health and agriculture-relevant ozone metrics over the United States from WRF-CMAQ reanalysis simulations 

Forrest Lacey, Rajesh Kumar, Cenlin He, Jennifer Boenhert, Cassandra O'Lenick, Olga Wilhelmi, Matthew Casali, and Kevin Sampson

Ozone concentrations have resulted in significant impacts on both human health and crop production throughout the beginning of the 21st century. Results presented here are from a NASA funded WRF-CMAQ model run at a 12km x 12km gridded horizontal resolution using data assimilation of MODIS AOD and MOPITT CO for a fourteen-year (2005-2018) period to show shifts in atmospheric composition over the continental United States (CONUS). This publicly available data has been aggregated to the maximum daily 8-hour ozone (MDA8) and seasonal ozone (OSDMA8) metrics for each of the EPA regions to show the regional drivers to human health as well as calculation of the accumulated ozone exposure (AOT40 and W126) metrics varying temporally and geographically based on crop data for CONUS available from the United States Department of Agriculture. These aggregation techniques have allowed us to identify both trends and some of the meteorological and atmospheric composition drivers in ozone-related risk for specific outcomes and how they vary geographically. The work presented here will also outline the GIS-based information dissemination platform that can be used by researchers and stakeholders to both access data and assess more detailed collaborative and convergent research questions.

How to cite: Lacey, F., Kumar, R., He, C., Boenhert, J., O'Lenick, C., Wilhelmi, O., Casali, M., and Sampson, K.: Trends in health and agriculture-relevant ozone metrics over the United States from WRF-CMAQ reanalysis simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11274, https://doi.org/10.5194/egusphere-egu23-11274, 2023.

EGU23-11324 | PICO | AS3.18

The GOME-type Tropical Tropospheric Ozone Essential Climate Variable (GTTO-ECV) satellite data record and an updated S5P-BASCOE dataset 

Klaus-Peter Heue, Diego Loyola, Melanie Coldewey-Egbers, Martin Dameris, Christophe Lerot, Michel van Roozendael, Daan Hubert, Quentin Errera, and Simon Chabrillat

A tropospheric ozone time series from 1995 until end 2022 has been generated within ESA’s Climate Change Initiative+ programme. The GOME-type Tropical Tropospheric Ozone Essential Climate Variable (GTTO-ECV) satellite data record combines data from GOME, SCIAMACHY, OMI and the three GOME-2 missions. The retrieval is based on the Convective Cloud Differential technique, which limits the coverage to the tropical belt (20°S to 20°N). We generated two monthly mean data sets at 1° x 1° resolution: one corresponds to a tropospheric column up to 200 hPa as in the previous CCI data release (Heue et al., 2016), while the other is limited to 270 hPa and includes the operational Sentinel-5P data as an additional sensor. An internal reprocessing of S5P CCD using 200 hPa is planned but might not be ready in time. Besides a consistent reprocessing of the CCD data for individual sensors, we also updated the harmonising scheme. The mean bias as well as the mean annual cycle relative to the reference instrument (OMI) are used to correct for the differences between the sensors.

Heue et al (2016) claimed a mean tropospheric ozone trend of +0.7 DU/decade (1995-2015). How did the trend change with the extended data set? The GTTO-ECV data record will be used to investigate the tropical mean trend as well as temporal and local changes in the trends. Also, a comparison with modelled tropospheric ozone data and the respective trends might be given.

As a second data product we provide the global S5P-BASCOE tropospheric ozone data. The complete time series of the S5P total ozone columns has been reprocessed recently. The reprocessing includes an update of the Level1 data as well as reprocessed cloud and O3 total columns. We use the reprocessed OFFL ozone data set in combination with BASCOE assimilation constrained stratospheric ozone profiles to calculate the tropospheric ozone columns. Relative to ground-based observations the total OFFL columns show a small positive bias. Before the retrieval of the tropospheric ozone column this bias is subtracted. The updated tropospheric ozone columns might also be compared to modelled tropospheric ozone columns.

How to cite: Heue, K.-P., Loyola, D., Coldewey-Egbers, M., Dameris, M., Lerot, C., van Roozendael, M., Hubert, D., Errera, Q., and Chabrillat, S.: The GOME-type Tropical Tropospheric Ozone Essential Climate Variable (GTTO-ECV) satellite data record and an updated S5P-BASCOE dataset, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11324, https://doi.org/10.5194/egusphere-egu23-11324, 2023.

EGU23-11944 | PICO | AS3.18

Tropospheric ozone and precursors (HCHO and CO) from the NDACC FTIR ground-based network 

Corinne Vigouroux and the FTIR data providers

Ground-based FTIR (Fourier transform infrared) stations contributing to the Network for Detection of Atmospheric Composition Change (NDACC), deliver time-series of ozone and some of its precursors at more than 20 sites, starting from the 90’s for the oldest stations. In the context of the Tropospheric Ozone Assessment Report (TOAR-II), we will present the status of the ground-based FTIR tropospheric ozone, formaldehyde (HCHO), and carbon monoxide (CO) measurements.

From high-resolution solar absorption spectra, O3, HCHO and CO total columns are obtained with a precision of about 2%, 8%, and 1%, respectively. In addition, the pressure dependence of fully resolved absorption lines allows retrieving low vertical resolution profiles and thus deriving few independent partial columns. For O3, the degrees of freedom for signal (DOFS) are about 4.5, allowing O3 amounts to be retrieved in four independent altitude layers: one in the troposphere and three in the stratosphere up to about 45 km, with a precision of 5–6 % for each partial column. For HCHO, the DOFS are only of order 1.0-1.5, with a sensitivity mainly located in the troposphere where most of the HCHO lies. For CO, about 2 DOFS can be obtained, with one of them located in the troposphere.

We will show the variability and trends (when long time-series are available) of O3, HCHO, and CO tropospheric partial columns at many FTIR stations, covering a wide range of latitudes and pollution conditions. To derive the trends, we use a multiple linear regression model including seasonal cycles and dynamical proxies explaining the species’ variability such as, e.g., the tropopause height, the El Niño-Southern Oscillation (ENSO), or the Quasi-Biennial Oscillation (QBO).

How to cite: Vigouroux, C. and the FTIR data providers: Tropospheric ozone and precursors (HCHO and CO) from the NDACC FTIR ground-based network, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11944, https://doi.org/10.5194/egusphere-egu23-11944, 2023.

EGU23-13047 | ECS | PICO | AS3.18

Long-term trend of ozone pollution in China during 2014-2020: distinct seasonal and spatial characteristics and ozone sensitivity 

Wenjie Wang, Hang Su, Yafang Cheng, David D. Parrish, Siwen Wang, Fengxia Bao, Ruijing Ni, and Xin Li

In the past decade, ozone (O3) pollution has become a severe environmental problem in major cities in China. Here, based on available observational records, we investigated the long-term trend of ozone pollution in China during 2014–2020. Ozone concentrations were slightly higher in urban areas than in non-urban areas. During these seven years, the highest ozone concentrations primarily occurred in summer in northern China, and in autumn or spring in southern China. Although ozone precursors, including nitrogen oxides (NOX) and carbon monoxide (CO), continuously decreased, ozone concentrations generally increased throughout the seven years with a slower increasing rate after 2017. The long-term trend of ozone concentrations differed across seasons; especially from 2019 to 2020 when ozone concentrations decreased in summer and increased in winter. To analyze the causes of this observed trend, a photochemical box model was used to investigate the change in ozone sensitivity regime in two representative cities – Beijing and Shanghai. Our model simulations suggest that the summertime ozone sensitivity regime in urban areas of China has changed from a VOC-limited regime to a transition regime during 2014–2020; by 2020, the urban photochemistry is in a transition regime in summer but in a VOC-limited regime in winter. This study helps to understand the distinct trends of ozone in China and provides insights into efficient future ozone control strategies in different regions and seasons.

How to cite: Wang, W., Su, H., Cheng, Y., Parrish, D. D., Wang, S., Bao, F., Ni, R., and Li, X.: Long-term trend of ozone pollution in China during 2014-2020: distinct seasonal and spatial characteristics and ozone sensitivity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13047, https://doi.org/10.5194/egusphere-egu23-13047, 2023.

Tropospheric ozone (O3) is an important greenhouse gas relevant for global warming projections as well as secondary pollutant affecting air quality on the regional scale. In this Communication, we use halogen version of the CAM-Chem model to investigate the evolution of the O3 budget during the 21st century following two different climate scenarios (RCP6.0 and RCP8.5) and halogen emissions. Our results indicate that the global ozone net chemical change (NCC) will decrease by ~50%, notwithstanding increasing or decreasing trends in ozone production and loss. However, a wide range of surface NCC variations (from −60% to 150%) are projected over polluted regions depending on the evolution of anthropogenic O3 precursor emissions. Most notably, water vapor and iodine are found to be key drivers of future tropospheric O3 destruction, while the largest changes in O3 production are determined by the future evolution of peroxy radicals. Overall, future surface ozone destruction due to halogens will become more important moving into the future for both scenarios, reaching a net reduction from −30 to −35 Tg (−11 to −15%) on the global O3 burden.

How to cite: Saiz-Lopez, A.: Influence of Natural Halogens on Global Tropospheric Ozone During the 21st Century, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13226, https://doi.org/10.5194/egusphere-egu23-13226, 2023.

EGU23-13237 | ECS | PICO | AS3.18

Evaluating the effects of climate warming and precursor emission changes on surface ozone air quality over coming decades: a case study for Austria 

Christian Schmidt, Monika Mayer, Christoph Stähle, Jessica Kult-Herdin, Peter Huszár, Jan Karlický, Hanns Moshammer, and Harald Rieder

Ozone production and loss in surface air is determined by ambient temperature,  chemical conditions and precursor emissions. Despite efforts to abate surface ozone air pollution, the daily maximum 8-hour average ozone target value for the protection of human health  is regularly exceeded at several monitoring sites in Austria especially during the warm seasons. 

Here we investigate projected changes in the surface ozone burden and effects of climate warming and changes in precursor emissions over the next decades in a series of tailored chemistry-transport model (CTM) experiments, performed with WRF-Chem and CAMx. Specifically we contrast changes in ozone air quality in decadal time slices for 2026-2035 and 2046-2055 with the recent past (2007-2016). Our CTM ensemble comprises simulations following the Representative Concentration Pathways (RCPs) 2.6, 4.5 and 8.5. Our results show a persistent large variability in ozone abundances driven by the large intra- and interannual  variability in meteorological conditions. Overall we find general improvements in the surface ozone burden for low emission scenarios (RCP2.6 and RCP4.5) driven by ambitious NOx controls. In contrast under RCP8.5 we find, on the one hand an increase in the frequency of non-attainment days and on the other a shift in the prime ozone season from summer towards spring. These increases are driven by both a climate penalty and changes in the chemical production regime (NOx vs. VOC limitation) and increasing methane and ozone backgrounds. Furthermore, we investigate impacts of projected ozone changes on human health at the municipal level in Austria.

How to cite: Schmidt, C., Mayer, M., Stähle, C., Kult-Herdin, J., Huszár, P., Karlický, J., Moshammer, H., and Rieder, H.: Evaluating the effects of climate warming and precursor emission changes on surface ozone air quality over coming decades: a case study for Austria, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13237, https://doi.org/10.5194/egusphere-egu23-13237, 2023.

The air pollutant emissions play a decisive role in the control of air quality. In recent years, the anthropogenic emission reduction measures have effectively reduced the PM2.5 levels over China improving air quality in China. However, due to the complex physical and chemical processes in atmospheric environment, O3 pollution events still occur frequently. To assess the impact of recent-year emission reduction of emissions on variations of summertime O3 pollution in the North China Plain, this study conducted the simulations with the air quality model WRF-Chem by using China's Multiresolution Emission Inventory (MEIC) with 0.1° resolution in 2012 and 2019, and we understand the characteristics of summer O3 pollution in the NCP under the scenario of anthropogenic emission reduction. The results show that the anthropogenic emissions of PM2.5, PM10, SO2, CO, black carbon (BC), and organic carbon (OC) in the NCP region decreased significantly from 2012 to 2019, while the emissions of NMVOCs (non-methane volatile organic compounds) increased distinctly in urban areas, and NOx emissions decreased in urban and increased in rural, reflecting the uneven emission reduction of anthropogenic air pollutants in North China. The control of anthropogenic pollutant emissions induced an elevated concentrations of atmospheric oxidants (O3 and multiple free radicals) in the NCP region, enhancing the atmospheric oxidation capacity, and then strengthening the chemical conversions of SO2 and NOx to generate sulfate, nitrate, and other secondary particles. As a result, the proportion of secondary PM2.5 in urban and rural areas markedly raised , especially during the O3 pollution period, offsetting the reduction of primary PM2.5 emissions. In addition, these emission reduction measures promote the transformation of O3 generation mechanism in the NCP from VOC-control to NOx-control. This study reveals the complex effects of anthropogenic emission reduction altering the atmospheric physical and chemical processes on atmospheric environmental change.

How to cite: Luo, Y. and Zhao, T.: Atmospheric environment change in a summertime O3 pollution event over the North China Plain under the influence of recent-year anthropogenic emission reduction, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14125, https://doi.org/10.5194/egusphere-egu23-14125, 2023.

EGU23-14161 | PICO | AS3.18

Harmonisation of Free Tropospheric Ozone Satellite Data Records in Support of TOAR Phase II 

Daan Hubert, Arno Keppens, Tijl Verhoelst, Steven Compernolle, and Jean-Christopher Lambert

The first TOAR assessment encountered several observational challenges that limited the confidence in estimates of the burden, short-term variability and long-term changes of ozone in the free troposphere. One of these challenges is the difficulty to interpret tropospheric observations from space, especially when combining data records from multiple satellites with differences in vertical sensitivity, prior information, resolution and spatial domain. Additional confounding factors are time-varying biases and the lack of harmonisation of geophysical quantities, units and definition of the tropospheric top level. All together, these increased the uncertainty on the distribution and trends of tropospheric ozone, impeding firm assessments relevant for policy and science. These challenges motivated the Committee on Earth Observation Satellites (CEOS) to initiate a coordinated activity on improving assessments of tropospheric ozone measured from space. Here, we report on work that contributes to this CEOS activity and to various Working Groups (SOWG, OPT, HEGIFTOM, TOP, ROSTEES, ...) of the ongoing second TOAR assessment.

Our primary objective is to harmonise the vertical perspective of different satellite data records. A first class of tropospheric ozone products is obtained through an inversion of spectral measurements by nadir-viewing sounders into a vertical profile. We describe two complementary approaches (Prior Replacement and Complete Data Fusion) to harmonise the differing profile retrieval set-up for GOME-2, IASI and other UV-visible and infrared nadir sensors, using information conveyed in the prior and the averaging kernels. A second class of products is obtained through subtraction of the stratospheric component from total column retrievals. The stratospheric column is derived with various methods, resulting in differing spatial coverage, tropospheric top level, sampling frequency, etc…  We present how all tropospheric ozone products, from both classes, are harmonised to a common tropospheric top level. We then intercompare all harmonised satellite records, and report on the differences and how these reduce upon harmonisation. Finally, we reflect on the importance of the vertical harmonisation process to improve constraints of the spatial distribution and trends in tropospheric ozone.

Acknowledgements : We are grateful to the sustained effort and committment of the teams, institutes and agencies that collect and provide satellite and ozonesonde data records of high quality.

How to cite: Hubert, D., Keppens, A., Verhoelst, T., Compernolle, S., and Lambert, J.-C.: Harmonisation of Free Tropospheric Ozone Satellite Data Records in Support of TOAR Phase II, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14161, https://doi.org/10.5194/egusphere-egu23-14161, 2023.

EGU23-14693 | ECS | PICO | AS3.18

Intercomparison of long-term ground-based tropospheric ozone measurements 

Robin Björklund, Corinne Vigouroux, Bavo Langerock, Dan Smale, Irina Petropavlovskikh, Peter Effertz, James Hannigan, Richard Querel, Ivan Ortega, Miyagawa Koji, John Robinson, Penny Smale, Michael Kotkamp, Gerald Nedoluha, Deniz Poyraz, and Roeland Van Malderen

Ground-based observations are indispensable for the long-term monitoring of atmospheric constituents. In this work, we take advantage of multiple collocated instruments to analyze potential biases and drifts in ground-based ozone observations, within the context of the HEGIFTOM (Harmonization and Evaluation of Ground-based Instruments for Free Tropospheric Ozone Measurements) working group in the Tropospheric Ozone Assessment Report, Phase II (TOAR-II). This work is performed at Lauder (New Zealand), Boulder (Colorado), and Mauna Loa (Hawaii) where comparisons are made between Fourier Transform Infrared (FTIR) spectroscopy, Dobson Umkehr, and ozonesonde observations. The validation is performed with respect to FTIR as arbitrary reference, while considering the differences between the a priori profile information for the techniques that employ these as well as accounting for the different vertical resolution of each measurement technique. Such intercomparison is done for a handful discrete altitude partial columns, defined to have independent pieces of information also in the case of the low vertical resolution techniques (FTIR and Umkehr). This leads to 4 independent vertical layers to be compared, including one in the troposphere where ozone plays an important role as a greenhouse gas and as a risk to human health. In this tropospheric layer we compare the FTIR, Dobson Umkehr and ozonesonde techniques and derive a consistent bias from the FTIR data of about 5%, which we attribute in part to the assumed spectroscopy. Fitting the time series of the relative measurement differences using multiple linear regression, we obtain a linear trend, which quantifies the drift between pairs of techniques. Within the uncertainties, we find no significant drift between FTIR and Umkehr or ozone sonde data in the troposphere.

How to cite: Björklund, R., Vigouroux, C., Langerock, B., Smale, D., Petropavlovskikh, I., Effertz, P., Hannigan, J., Querel, R., Ortega, I., Koji, M., Robinson, J., Smale, P., Kotkamp, M., Nedoluha, G., Poyraz, D., and Van Malderen, R.: Intercomparison of long-term ground-based tropospheric ozone measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14693, https://doi.org/10.5194/egusphere-egu23-14693, 2023.

Tropospheric ozone is a greenhouse gas and a secondary pollutant that has negative impact on human health, crop yield and the environment. Therefore information on the long-term trends in surface ozone, particularly in the regional representative site is crucial for assessing the impact on climate and environment. While there are extensive observations of surface ozone in Europe, North America and East Asia, there are very limited observations in South Asia, particularly in the Himalayan regions. In this reference, surface ozone observations were initiated at a mountain site in Nainital (29.40° N, 79.50° E, 1948 m amsl) situated in central Himalaya in October 2006. Here, we present the observed long-term trends in surface ozone over the central Himalayas and underlying factors influencing its diurnal and seasonal variabilities. In general, ozone diurnal variations indicates least daytime photochemical ozone buildup at this remote site, except during episodes of biomass burning in the plain regions of northern India during spring. Instead, ozone levels at this site are primarily influenced by transported air masses, mountain-valley breezes and stratospheric intrusions. The long-term trend found not to be very prominent, but it showed a very slight negative (about 1 ppbv/yr) for 2007-2014 period, while a positive trend (about 0.7 ppbv/yr) for 2014-2022 period. The negative trend during 2007-14 was more prominent in spring while positive trend was prominent in winter. Trend analysis in AIRS ozone data at different pressure levels is being studied and residence time analysis of air-masses, obtained from the back air-trajectories simulations is in progress, which will be presented during the conference. These observations will be very useful for the ongoing efforts by TOAR

How to cite: Tomar, V. and Naja, M.: Long term trends and characteristics of surface ozone at high altitude site in the central Himalayas, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15405, https://doi.org/10.5194/egusphere-egu23-15405, 2023.

Tropospheric ozone (trop-O3) is a regional air pollutant and an important greenhouse gas. Major sources of trop-O3 are: transport from the stratosphere; and photochemical production within the troposphere involving reactions of ozone precursors: oxides of nitrogen (NO and NO2, collectively NOx) and volatile organic compounds (VOC), including methane.

Trop-O3 has an atmospheric lifetime of about a few weeks making it transportable over inter-continental distances. This makes ozone precursor emissions from one “source” region affect the ozone concentration at local and remote “receptor” regions, making it important for us to understand source-receptor relationships. These source-receptor relationships can be modelled using the source-attribution technique (also known as Tagging) where ozone molecules are tagged/labelled with their source identities allowing a direct attribution of sources in receptor regions, thereby, the relative contribution of various sources can be obtained.

Simulations using CESM 1.2.2- CAM4-Chem are performed for a global study of trop-O3 source attribution for the 2000-2018 period. Here, we modify the default chemical mechanism to output the ozone and its tags attributed to the source region/sector of its emitted precursors. For example, an NO molecule originating from biogenic source would be called NO_BIO, and all the other chemical species emanating from NO_BIO (NO2, NO3, O3 etc.) will hold the tag “BIO”.

Separate simulations are performed for tagging trop-O3 with its NOx and VOC precursor emission sources. We specify separate tag identities for emissions from anthropogenic, biogenic, biomass burning, and aircraft sources. Additional tags are specified for lightning NOx in the NOx-tagged simulation, and for methane in the VOC-tagged simulation. Here, all surface-based anthropogenic emissions hold tags representing the geographical location at which the emissions occur. Further, the ship-NOx emissions hold tags representing the ocean basin from which they are emitted.

The design of these simulations and several prominent results will be presented.

How to cite: Nalam, A., Lupascu, A., and Butler, T.: Attribution of Tropospheric Ozone to Sources of NOx and VOC Precursor Emissions in a Global Chemistry-Climate Model (CESM1.2.2-CAM4-Chem) for the 2000-2018 Period, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15618, https://doi.org/10.5194/egusphere-egu23-15618, 2023.

EGU23-1963 | Orals | AS3.20

High-sensitivity detection of HO2 radical by cavity ring-down spectroscopy: prospects for future applications of narrow linewidth lasers 

Weixiong Zhao, Chunhui Wang, Bo Fang, Nana Yang, Feihu Cheng, Xiao Hu, Yang Chen, Weijun Zhang, Christa Fittschen, and Weidong Chen

The hydroperoxyl radical (HO2) plays a key role in atmospheric chemistry. It reacts with NO to generate hydroxyl radical (OH) and nitrogen dioxide (NO2), resulting in the HOx (= OH + HO2) cycle that governs the atmospheric oxidation capacity and the formation of air pollution, and a net production of ozone that determines the troposphere ozone budget. Quantitative measurement of its absolute concentration is very important. However, due to its short lifetime and low concentration (typically about 108 to 109 molecule/cm3 under atmospheric condition), most of the currently used methods are indirect methods that require chemical conversion; direct measurement remains very challenging.

The cavity ring-down spectroscopy (CRDS) technique uses high reflectivity mirrors to increase the effective absorption pathlength to tens of kilometers, enabling very high detection sensitivity; the absolute concentration of the target absorbers can be quantitatively determined by the Beer-Lambert law, providing a powerful tool for direct measurement of free radicals. In this work, we report the development of a portable cavity ring-down spectrometer for direct and absolute measurement of HO2 radical concentration using a distributed feedback (DFB) diode laser operating at 1506 nm. At a pressure of 100 mbar, a detection limit of ~ 7.3×107 molecule/cm3 (1σ, 10s) was achieved with a ring-down time (τ0) of 136 μs. The corresponding detection sensitivity was 1.5×10-11 cm-1, which was close to the state-of-the-art performance.

In cavity ring down spectroscopy, the coupling efficiency of the laser beam into the cavity depends on the laser frequency tuning speed and the ratio of the laser linewidth to the cavity mode width. For the DFB laser system, the laser linewidth (~ 2 MHz) was about thousands of times larger than that of the cavity mode (~ 1.2 kHz), which results in the conversion of laser phase noise into amplitude fluctuation, making the cavity injection noisy and limiting the improvement of detection sensitivity. Here, by replacing the DFB diode laser with a narrow linewidth erbium-doped fiber (EDF) laser, the amplitude fluctuation caused by the laser phase noise was reduced and the cavity mode injection efficiency was improved. The sensitivity was improved to 3.9×10-12 cm-1 with a short data-acquisition time of 0.2 s. The one order of magnitude improvement makes further ambient applications look promising.

How to cite: Zhao, W., Wang, C., Fang, B., Yang, N., Cheng, F., Hu, X., Chen, Y., Zhang, W., Fittschen, C., and Chen, W.: High-sensitivity detection of HO2 radical by cavity ring-down spectroscopy: prospects for future applications of narrow linewidth lasers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1963, https://doi.org/10.5194/egusphere-egu23-1963, 2023.

EGU23-3245 | ECS | Posters on site | AS3.20

Comparison of Fence Line Monitoring by mobile monitoring vehicle and Chimney Measuring Devices in Large Industrial Complexes 

Juhyeon Sim, Dukhyeon Kim, Juseon Shin, Yuseon Lee, Sohee Joo, Jaewon Kim, Gahyeon Park, and Youngmin Noh

In the case of large industrial complexes, there are state management equipment to monitor pollutants emitted from chimneys, but there are undetected sources of pollution, such as leaks during processes, leaks from pipes, and leaks from unsealed warehouses, except for chimneys. In this study, mobile observation was conducted using SOF, Sky DOAS, in-situ MeDOAS, and MeFTIR equipment. The observation method used in this study is fence line monitoring, which surrounds a large factory area and observes both the upwind and downwind sides. method of observation. The observation site was conducted in July and August 2021 at the Yeosu Industrial Complex located in Yeosu, Jeollanam-do, South Korea, one of the three largest industrial complexes in South Korea. In order to find out whether and the extent of leakage, four areas where Telemonitoring System(TMS), a chimney measuring device managed by the Korea Environment Corporation, exist were designated as observation sites. The results observed for the same period of time were compared for SO2 and NO2, which are substances with overlapping measurement items of mobile monitoring vehicle(MMV) and TMS. Although a direct comparison was not possible because the MMV expresses the emission per hour and the TMS expresses the emission concentration, it was confirmed that leaks that were not captured by the TMS on a specific date appeared as a result of the MMV measurement. This study confirmed that even in industrial complexes where TMS is installed for management purposes, air pollution and economic losses due to leaks can be reduced if fan line monitoring is conducted to detect unexpected leaks.

 

acknowledgment

This work was supported by the National Research Foundation of Korea(NRF) grant funded by the Korea government(MSIT) (No. 2018R1D1A3B07048047)

 

How to cite: Sim, J., Kim, D., Shin, J., Lee, Y., Joo, S., Kim, J., Park, G., and Noh, Y.: Comparison of Fence Line Monitoring by mobile monitoring vehicle and Chimney Measuring Devices in Large Industrial Complexes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3245, https://doi.org/10.5194/egusphere-egu23-3245, 2023.

EGU23-3470 | ECS | Posters on site | AS3.20

Artifact-Free Measurements of Isotopic Composition for Atmospheric and Planetary Gas Analysis 

D. Michelle Bailey, Abneesh Srivastava, Joseph Hodges, and Adam Fleisher

The isotopic composition of gaseous species can provide critical information regarding the age and chemical or physical origin of sample material. However, the challenge of maintaining isotope abundance scales – generated by comparing sample measurements to those of a reference material having finite quantity and stability – may limit inter-laboratory agreement and consequently the uncertainty evaluation of new measurement methods. Here we will present progress towards realization of artifact-free isotope scales and rapid measurements of isotopic composition enabled by absolute SI-traceable measurement schemes.

We will discuss how cavity ring-down spectroscopy techniques, capable of highly precise and accurate measurements of transition-resolved peak areas, can be leveraged in combination with quantum chemical calculations of transition moments to enable measurement of molecular isotopologue ratios [1]. We will also introduce direct frequency comb spectroscopy methods for rapid and precise measurement of isotopic abundance [2]. This discussion will include demonstrations in the near- and mid- infrared spectral regions employing cross-dispersed spectrometers. Implications for carbon, nitrogen, and oxygen isotopic analysis will be presented.

Applications of these SI-traceable measurement approaches include accurate source apportionment and greenhouse gas inventories, radiocarbon dating, isotope forensics, with the potential for high-impact contributions to emerging advances in exoplanetary studies and astrophysics.

[1] A. J. Fleisher, H. Yi, A. Srivastava, et al., Nat. Phys. 2021, 17, 889-893

[2] D. M. Bailey, G. Zhao, and A. J. Fleisher, Anal. Chem. 2020, 92 (20), 13759–13766

How to cite: Bailey, D. M., Srivastava, A., Hodges, J., and Fleisher, A.: Artifact-Free Measurements of Isotopic Composition for Atmospheric and Planetary Gas Analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3470, https://doi.org/10.5194/egusphere-egu23-3470, 2023.

EGU23-3685 | Orals | AS3.20

Two-Channel, Fast Time-Response CAPS-Based NOx Monitor 

Andrew Freedman, Joseph Roscioli, Benjamin Moul, and Timothy Onasch

We have developed a turnkey, fast response two-channel NOx monitor (NO=NO + NO2) which provides  simultaneous measurements of both NOx and NO2 and thus NO by subtraction.  The NOx channel employs a carefully controlled concentration of photolytically-produced ozone (O3) to convert NO into NO2.  The monitor can measure NO2 and NOx with an accuracy of better than 5% and precision of < 0.2 ppb (1s, 1s) with <1 second physical time constant in each measurement channel.  The monitor is based on Aerodyne Research’s patented CAPS (Cavity Attenuated Phase Shift) technology previously employed to measure NO2concentrations, aerosol optical extinction and aerosol single scattering albedo. 

A CAPS-based NO2 monitor utilizes a light-emitting diode (LED) as a light source (450 nm for the NO2 channel and 405 nm for the total NOx channel) and a sample cell incorporating two high reflectivity mirrors; a vacuum photodiode is used to detect the light emitted from the cell. The square wave modulated light from the LED passes through the absorption cell and is detected as a distorted waveform which is characterized by a phase shift with respect to the initial modulation.   The amount of that phase shift is a function of fixed instrument properties - cell length, mirror reflectivity, and modulation frequency– and of the presence of variable concentrations of nitrogen dioxide.  The mixing ratio is calculated from the value of the cotangent of the phase shift, the speed of light, LED modulation frequency and the absorption coefficient of NO2.  The use of 405 nm detection in the total NOx channel greatly reduces the possible interference caused by the presence of several ppm of O3 in the sample flow.

We present data from an intercomparison of the NOx monitor with Aerodyne TILDAS monitors measuring both NO and NO2.  The TILDAS monitors utilize infrared diode lasers to probe individual ro-vibrational absorption lines and are considered the “gold standard” for measuring concentrations of small molecules.  The monitors were deployed on the Aerodyne Mobile Laboratory during the MOOSE (Michigan Ontario Ozone Source Experiment) campaign in late 2021.  The figure presented below compares the measurement of both NO2 and the sum of NO+NO2 measured by the TILDAS monitors compared with that obtained by the CAPS NO monitor at 1 second resolution.  Note the excellent agreement with respect to both magnitude and time resolution.  Long term comparisons indicate that correlation coefficients at 1 second  resolution approach 1. 

How to cite: Freedman, A., Roscioli, J., Moul, B., and Onasch, T.: Two-Channel, Fast Time-Response CAPS-Based NOx Monitor, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3685, https://doi.org/10.5194/egusphere-egu23-3685, 2023.

EGU23-4403 | ECS | Orals | AS3.20

Long open-path measurements of CO2 and CH4 with an 125HR FTS in an urban environment. 

Tobias Schmitt, Jonas Kuhn, Lukas Pilz, Robert Maiwald, Maximilian May, Ralph Kleinschek, Paul Edinger, Stefan Schmitt, Frank Hase, David W. T. Griffith, and André Butz

Quantifying sources and sinks, as well as chemical activity of trace gases in the lower troposphere, requires accurate measurements of the concentrations of the species of interest. While there exist in-situ measurement techniques, which are highly accurate, point-like measurements are only sufficiently representative in the spatial domain for a small area. This holds true in particular in high-gradient environments, e.g., urban settings. Hence, measuring those concentrations averaged on the length scale of a few kilometers is desirable. Furthermore, quantifying emissions requires combining concentration measurements with regional transport models, which cover a comparable spatial resolution.

We present a long open-path setup that measures average concentrations on the kilometer-scale in the urban boundary layer. Our setup, which is operational since March 2022, is based on a Bruker IFS 125 HR Fourier transform spectrometer, a commercially available spectrometer, which offers high resolution and throughput. The instrument choice provides flexible and explorative experimental setups such as variable and high spectral resolution and the extension of spectral coverage from the shortwave-infrared to the near ultra-violet spectral range. Here, we present the results on CO2 and CH4 from our 2022 measurement campaign as well as analysis of the diurnal variability in comparison to the prediction of local and regional transport models.

How to cite: Schmitt, T., Kuhn, J., Pilz, L., Maiwald, R., May, M., Kleinschek, R., Edinger, P., Schmitt, S., Hase, F., Griffith, D. W. T., and Butz, A.: Long open-path measurements of CO2 and CH4 with an 125HR FTS in an urban environment., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4403, https://doi.org/10.5194/egusphere-egu23-4403, 2023.

EGU23-5232 | Orals | AS3.20

A portable, high-precision optical analyzer based on hybrid laser absorption cell for simultaneous measurements of N2O, CH4, and CO2 fluxes from soils 

Longfei Yu, Ying Wang, Zetong Niu, Zhelin Su, Lintao Zheng, and Ting-Jung Lin

Laser spectrometers have shown good capability in measuring mixing ratios for atmospheric greenhouse gases (GHGs). Given the fact that spectral bands of CO2, CH4, and N2O covering from near to mid-infrared (NIR to MIR) wavelengths, and the limitations in the wavelength coverage of the laser and photodetector, it is very challenging to analyze CO2, CH4, and N2O simultaneously for most cavity-enhanced analyzers using NIR lasers. Alternative solutions, such as combining multiple quantum cascade laser (QCL) beams and analyzing all GHGs in the MIR wavelengths, would significantly increase the instrumental cost.

Here, we present a recently developed analyzer utilizing the advantages of detecting CO2/H2O in the NIR spectral region and N2O/CH4 in the MIR region, respectively. Through a unique optical design, two independent optical paths are formed in a single Herriott gas cell so that low temperature-related drift and mechanical robustness are achieved. The mixing ratios of CO2 and H2O are analyzed by a NIR laser and a photodetector at ~4995cm-1, while CH4 and N2O are analyzed by a QCL and an MCT photodetector at ~1275cm-1. The analyzer facilitates high-sensitivity, field-deployable measurements of CO2, CH4, N2O and H2O altogether in a compact, portable instrumental design. In addition, this analyzer can be completely powered by rechargeable battery, facilitating all-day in situ measurements without grid power supply.

In the laboratory, side-to-side comparisons were performed between our newly developed analyzer and another commercial gas analyzer based on cavity ring down spectroscopy (CRDS). The results showed high consistency in GHG mixing-ratio measurements with the two spectrometers. Attached to soil chambers, we also found comparable performance of two analyzers in determining GHG fluxes. In particular, we found that the presented analyzer could precisely capture transient changes in gas mixing ratios from the soil chamber. Recently, field deployment in different soil conditions, including upland forest soils and riparian soils, was carried out for simultaneous N2O, CH4, CO2 soil flux measurements. The overall results suggest that our analyzer is suitable for continuous GHG flux monitoring under variable field conditions, and shows potentials in simultaneous measurements of multiple GHG fluxes from natural ecosystems.

How to cite: Yu, L., Wang, Y., Niu, Z., Su, Z., Zheng, L., and Lin, T.-J.: A portable, high-precision optical analyzer based on hybrid laser absorption cell for simultaneous measurements of N2O, CH4, and CO2 fluxes from soils, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5232, https://doi.org/10.5194/egusphere-egu23-5232, 2023.

EGU23-5538 | Posters on site | AS3.20

Detection of the regional concentrations of various trace gases using LP-DOAS at Hefei Xinqiao International Airport 

Jun Duan, Min Qin, Wu Fang, Zhitang Liao, Huaqiao Gui, Pinhua Xie, and Wenqing Liu

Correspondence: Min Qin(mqin@aiofm.ac.cn)

Abstract: A measurement campaign using long-path differential optical absorption spectroscopy (LP-DOAS) instrument at Hefei Xinqiao International Airport to investigate the regional concentrations of various trace gases in the airport’s northern area and the variation characteristics of the gas concentrations during an aircraft’s taxiing and take-off phases. The total light path of the LP-DOAS system was about 964 meters and the time resolution of the LP-DOAS instrument was approximately 10 seconds. The measured light path of the LP-DOAS passed through an aircraft taxiway and take-off runway concurrently without affecting aircraft operations. The results of NO2 and SO2 pollution peaks were clearly visible, and their timing was well matched to the time the aircraft crossed the light path. While the aircraft take-offs increased the regional average NO2 concentrations by 10-20 ppbV and flight take-offs increased the regional average SO2 concentrations by 1-5 ppbV, the overall pollution levels in the airport area were low due to the airport's openness and rapid dispersion of pollutants, and the maximum hourly average NO2 and SO2 concentrations during the observation period were better than the Class 1 ambient air quality standards in China. Additionally, we discovered that the NO2 and SO2 emissions from the Boeing 737-800 aircraft used in this experiment were positively related to the age of the aircraft.

Acknowledgements: This work was supported by the Plan for Anhui Major Provincial Science & Technology Project (Grant No. 202203a07020003), the Anhui Provincial Key R&D Program (No.202104i07020010) and the HFIPS Director’s Fund (Grant No. YZJJQY202205).

How to cite: Duan, J., Qin, M., Fang, W., Liao, Z., Gui, H., Xie, P., and Liu, W.: Detection of the regional concentrations of various trace gases using LP-DOAS at Hefei Xinqiao International Airport, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5538, https://doi.org/10.5194/egusphere-egu23-5538, 2023.

EGU23-5828 | ECS | Posters virtual | AS3.20

Development of a high-finesse broadband optical cavity using prism based on total internal reflection for applied spectroscopy 

Ruyue Cui, Gaoxuan Wang, Azer Yalin, Lingshuo Meng, Cécile Coeur, Lei Dong, and Weidong Chen

The use of high reflectivity dielectric mirrors to form a high finesse optical cavity allows one to achieve long optical path lengths of up to several kilometres for high-sensitivity spectroscopy applications [1,2]. The high reflectivity of a dielectric mirror is achieved via constructive interference of the Fresnel reflection at the interfaces produced by multilayer coatings of alternate high and low refractive index materials [3]. This wavelength-dependent coating limits the bandwidth of the mirror's high reflectivity to only a few percent of the designed central wavelength.

We report on the recent development of a novel optical cavity based on prisms as cavity reflectors [4-6], which offers a high-finesse optical cavity operating in a broadband spectral region from 400 to more than 1600 nm [7] and provides a very suitable high-sensitivity spectroscopic technique for frequency-comb application.

 

Acknowledgments : This work is supported by the French national research agency (ANR) under the MABCaM (ANR-16-CE04-0009), the CaPPA (ANR-10-LABX-005), the ICAR-HO2 (ANR-20-CE04-0003) contracts, and the regional ECRIN program.

 

References

[1] S. S. Brown, Chem. Rev. 103 (2003) 5219-5238.

[2] M. Mazurenka, A. J. Orr-Ewing, R. Peverallb and G. A. D. Ritchie, Annu. Rep. Prog. Chem. Sect. C101 (2005) 100-142.

[3] G.R. Fowles, Introduction to Modern Optics, 2nd ed. (Rinehart and Winston, 1975), p. 328.

[4] H. Moosmuller, App. Opt. 37 (1998) 8140-8141.

[5] P. S. Johnston and K. K. Lehmann, Opt. Express 16 (2008) 15013-15023.

[6] B. Lee, K. Lehmann, J. Taylor and A. Yalin, Opt. Express 22 (2014) 11583-11591.

[7] G. Wang, A. Yalin, C. Coeur, S. Crumeyrolle, R. Akiki, E. Fertein, W. Chen, 6th International Workshop on Infrared Technologies, October 29-30, 2019, Princeton, New Jersey, USA.

How to cite: Cui, R., Wang, G., Yalin, A., Meng, L., Coeur, C., Dong, L., and Chen, W.: Development of a high-finesse broadband optical cavity using prism based on total internal reflection for applied spectroscopy, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5828, https://doi.org/10.5194/egusphere-egu23-5828, 2023.

EGU23-6065 | ECS | Posters on site | AS3.20

Development of a spectroscopic sensor for accurate, real-time monitoring of personal exposure to nitrogen dioxide 

Eibhlín F. Halpin and Dean S. Venables

Nitrogen dioxide (NO2) is a major air pollutant that can lead to increased risks of lung cancer, cardiovascular mortality, and a 50% increased likelihood of children developing asthma. Expanding the scope and range of NO2 measurements is therefore desirable to quantify NO2 levels and emissions in different settings. Current research and regulatory instruments are too expensive and bulky for widespread deployment and personal exposure measurements, while low-cost sensors do not have the required sensitivity, accuracy, and response time for many applications.

Here we describe a spectroscopic, optical cavity approach to sensitively quantify NO2 based on the differential absorption at two nearby wavelengths. The system uses a modulated blue LED, an optical cavity for high absorption sensitivity, and lock-in amplification to measure the light transmitted through the cavity. Careful spectral filtering is needed to remove unwanted wavelengths. We report the system performance and Allan deviation of the system, and compare the system response against a standard IBBCEAS set-up for in situ measurements of NO2. Strategies to improve the instrument performance and reduce sensor size and cost are discussed.

How to cite: Halpin, E. F. and Venables, D. S.: Development of a spectroscopic sensor for accurate, real-time monitoring of personal exposure to nitrogen dioxide, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6065, https://doi.org/10.5194/egusphere-egu23-6065, 2023.

EGU23-8892 | ECS | Posters on site | AS3.20

Magnetic characterization of PM10 using non-linear Preisach maps. Toward domain state identification of magnetic anthropogenic particles 

Adriana Dumitru, Cristian Necula, Marius Dumitru, and Gabriela Iorga

According to World Health Organization, nowadays almost the entire global population (99%) breathes air that threatens its health (WHO, 2022), The greatest concern is related to air pollution by particles and nitrogen dioxide, people living in cities facing every day’s unhealthy levels of these pollutants. Due to their multitude of sources, natural (mineral dust, sea salt, volcanoes, etc.) and anthropogenic (traffic, industry, constructions, agricultural activities, etc.), atmospheric particulate matter (PM) levels and physical properties vary greatly in time and space. Here we investigate the magnetic properties of PM10 (PM less than 10 µm) sampled in three different locations from Romania chosen so as to reflect as much as possible different origin of atmospheric particles. We use non-linear Preisach maps in tandem with Scanning Electron Microscopy (SEM) coupled with Energy-Dispersive X-ray spectroscopy (EDS), SEM/EDS, to specify more precisely domain states and characteristic magnetic signature of magnetic grains in PM10 fraction. PM10 aerosol samples were collected at three different sites in southern Romania: Bucharest site as urban, heavy impacted by traffic in the very center of the city, Magurele as suburban, under the influence of Bucharest and of the agricultural activities in the surrounding areas and Matasari, a rural site located in south-western Romania that was heavily impacted by the industrial activities at the open-pit coal mines located in the proximity. Our study highlighted three main types of magnetic mineral pollutants in the PM10 samples from Romanian industrial, urban traffic and suburban environments. 

Acknowledgment
AD and GI gratefully acknowledge the funding from the NO Grants 2014-2021, under Project contract no. 31/2020, EEA-RO-NO-2019-0423 project. This work was also supported by a grant of Ministry of Research, Innovation and Digitization, CCCDI - UEFISCDI, project number PN-III-P2-2.1-PED-2021-3678, within PNCDI III

How to cite: Dumitru, A., Necula, C., Dumitru, M., and Iorga, G.: Magnetic characterization of PM10 using non-linear Preisach maps. Toward domain state identification of magnetic anthropogenic particles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8892, https://doi.org/10.5194/egusphere-egu23-8892, 2023.

EGU23-9167 | Posters on site | AS3.20

The Four-Wavelength Photoacoustic Aerosol Absorption Spectrometer PAAS-4λ 

Martin Schnaiter, Claudia Linke, Eija Asmi, Henri Servomaa, Antti-Pekka Hyvärinen, Sho Ohata, Yutaka Kondo, and Emma Järvinen

Light absorbing particulate emissions, known as black carbon (BC) or brown carbon (BrC), are major contributors to the atmospheric aerosol and have a significant impact on climate forcing. The spectral light absorption coefficient of these particles, which is essential for understanding their impact on the climate, can vary greatly depending on the combustion process and atmospheric aging, particularly in the Arctic where concentrations of BC and BrC are low but the climate is sensitive to changes in the atmospheric aerosol. Traditional filter-based methods for characterizing light absorbing aerosol can be prone to errors in environments where the relationship between particle light scattering and absorption is high due to cross-sensitivity to co-deposited light scattering particles. The photoacoustic absorption spectroscopy (PAS) method is less sensitive to particle light scattering and has a high measurement precision and accuracy, but is not widely used for long-term monitoring due to ist assumed lack of sensitivity and robustness.

The Photoacoustic Aerosol Absorption Spectrometer PAAS-4λ has been developed for use in unattended air quality monitoring stations and utilizes four wavelengths coupled to a single acoustic resonator in a compact and robust design. It has a low detection limit of below 0.1 Mm-1 and has been calibrated in the laboratory using NO2/air mixtures and Nigrosin aerosol. The PAAS-4λ has been validated at an air quality monitoring station in the European Arctic and its performance during 12 months of deployment is presented. Comparisons with filter-based photometers demonstrate the capabilities and value of the PAAS-4λ for both long-term monitoring and the validation of filter-based instruments.

How to cite: Schnaiter, M., Linke, C., Asmi, E., Servomaa, H., Hyvärinen, A.-P., Ohata, S., Kondo, Y., and Järvinen, E.: The Four-Wavelength Photoacoustic Aerosol Absorption Spectrometer PAAS-4λ, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9167, https://doi.org/10.5194/egusphere-egu23-9167, 2023.

EGU23-10765 | ECS | Orals | AS3.20

A three-channel thermal dissociation cavity ring-down spectrometer for the continuous measurement of ambient NO2, total peroxy nitrates and total alkyl nitrates 

Chuan Lin, Renzhi Hu, Pinhua Xie, Guoxian Zhang, Jinzhao Tong, and Wenqing Liu

A newly constructed thermal dissociation cavity ring-down spectrometer (TD-CRDS) for simultaneous measuring NO2, total peroxy nitrates (ΣPNs) and total alkyl nitrates (ΣANs) was presented. NO2 is detected directly at around 405.46 nm, ΣPNs and ΣANs are detected as NO2 after thermal decomposition at 180℃ and 360℃. The influences of the recombination reaction of RO2 radicals in two different types of heated inlets were discussed and compared, and the thermal decomposition efficiency of PNs was found to be higher with the value of 96% at the heated inlet filled with glass beads than the other (72%). Possible interferences, mainly O3 (including reactions of O3 via NO and O3 via NO2) and NOx (such as the recombination reactions of NOx and peroxy radicals at different thermal temperatures), were quantitatively characterised. The effects were found to be much weaker in the heated inlet filled with glass beads. Thus, a calibration method for measuring ΣPNs and ΣANs was established, especially to solve the accurate measurement of ΣPNs and ΣANs under high amounts of ambient NOx and O3 in China. At the time resolution of 20 s, the detection limits of the TD-CRDS instrument for NO2, ΣPNs and ΣANs are 6 pptv (1σ), 15 pptv (1σ) and 15 pptv (1σ), respectively. Finally, we applied the instrument to the Hefei field campaign, obtaining the concentration distribution and variation characteristics of ΣPNs and ΣANs.

 

 

How to cite: Lin, C., Hu, R., Xie, P., Zhang, G., Tong, J., and Liu, W.: A three-channel thermal dissociation cavity ring-down spectrometer for the continuous measurement of ambient NO2, total peroxy nitrates and total alkyl nitrates, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10765, https://doi.org/10.5194/egusphere-egu23-10765, 2023.

EGU23-12051 | Posters on site | AS3.20

A Broadband Cavity-Enhanced Absorption Spectrometer for Simultaneous measurements of NO2 and particulate matter 

Weidong Chen, Gaoxuan Wang, Lingshuo Meng, Qian Gou, Benjamin Hanoune, Suzanne Crumeyrolle, Thomas Fagniez, Cécile Coeur, and Rony Akiki

A novel instrument based on broadband cavity enhanced absorption spectroscopy has been developed using a supercontinuum broadband light source, which showcases its ability in simultaneous measurements of the concentration of NO2 and the extinction of particulate matter (PM). Side-by-side intercomparison was carried out with the reference NOx analyzer for NO2 and OPC-N2 particle counter for particulate matter, which shows a good linear correlation with r2 > 0.90. Measurement limits (1σ) of the developed instrument were experimentally determined to be 230 pptv in 40 s for NO2 and 1.24 Mm-1 for the PM extinction in 15 s, respectively.

This work provides a promising method in simultaneously monitoring atmospheric gaseous compounds and particulate matter, which would further advance our understanding on gas-particle heterogeneous interactions in the context of climate change and air quality.

Experimental details and the preliminary results will be discussed and presented.

 Acknowledgments

The authors thank the financial supports from the French national research agency (ANR) under the MABCaM (ANR-16-CE04-0009), the CaPPA (ANR-10-LABX-005) contracts, the CPER ECRIN program, and the EU H2020-ATMOS project.

How to cite: Chen, W., Wang, G., Meng, L., Gou, Q., Hanoune, B., Crumeyrolle, S., Fagniez, T., Coeur, C., and Akiki, R.: A Broadband Cavity-Enhanced Absorption Spectrometer for Simultaneous measurements of NO2 and particulate matter, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12051, https://doi.org/10.5194/egusphere-egu23-12051, 2023.

Methane (CH4) is the second strongest anthropogenic greenhouse gas in terms of radiative forcing after carbon dioxide (CO2). It has a relatively short atmospheric lifetime for a greenhouse gas (~9 years)and so is an attractive target for near-term climate mitigation strategies. While the total amount fraction of atmospheric CH4 is currently measured by atmospheric monitoring stations to calculate global and regional budgets, it is not currently possible to distinguish the total amount of CH4 emitted by individual sectors. Different sources emit CH4 with unique isotope ratios, and so continuous isotope ratio measurements have the potential to provide the data needed to disaggregate emissions sources.  

We have developed Boreas, an automated field deployable CH4 preconcentrator coupled to a laser spectrometer able to provide continuous, high frequency measurements of both δ 13C (CH4) and δ 2H (CH4) and the total CH4 amount fraction in ambient air. Boreas was deployed to a UK atmospheric monitoring site located in Heathfield, East Sussex, in May 2021.  

We compare atmospheric measurements of δ13C(CH4) and δ2H(CH4) made from Spring 2021 to Spring 2023 with equivalent model output and analyse similarities and differences in the context of currently known isotopic source signatures in Europe. We also consider potential future CH4 emission scenarios and show how these measurements could be used under future emission reduction strategies. 

How to cite: Safi, E., Rennick, C., Chung, E., and Arnold, T.: A novel Laser-based technique for in-situ automated measurements of atmospheric CH4 isotopologues and implications for current and future emission scenarios , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12554, https://doi.org/10.5194/egusphere-egu23-12554, 2023.

EGU23-12978 | Orals | AS3.20

SPECIES: a balloon-borne and airborne instrument coupling infrared lasers with Optical Feedback Cavity Enhanced Absorption Spectroscopy technique for atmospheric in-situ trace-gas measurements 

Valery Catoire, Patrick Jacquet, Michel Chartier, Daniele Romanini, Gisèle Krysztofiak, Irène Ventrillard, and Claude Robert

The balloon-borne and airborne instrument SPECIES (SPECtromètre Infrarouge à lasErs in Situ) recently built in our laboratory will be described. This is a mid-infrared absorption spectrometer, including four channels by coupling Interband or Quantum Cascade Lasers (ICLs or QCLs) to Optical-Feedback Cavity-Enhanced Absorption Spectroscopy (OF-CEAS). Using cavities of 50 cm length, this leads to very high resolution (< 0.005 cm-1) spectra and very long optical paths (> 5 km) and thus, low detection limits for the trace gases to be measured. It can contribute to the detailed description and understanding of the functioning of the free troposphere and stratosphere in terms of composition, chemical reactivity and circulation of air masses by carrying out fast (< 2 s) in-situ measurements of reactive trace gases and greenhouse gases among CO, NOx, CH2O, 12CO2, 13CO2, CH4 and N2O, at very high spatial resolution, i.e. a few meters vertically or hundred meters horizontally. Mini-SPECIES is the lightened version of SPECIES, comprising two lasers coupled to two cavities and reduced electrical power, which allows its integration in aircraft or its operation for long-duration stratospheric balloon flights (> 4 days). High accuracies are obtained when calibration in flight, or at ground before and after the flight, is performed against standards. In addition to providing reference measurements for calibration/validation of space missions, these performances can lead to in-depth characterization of particular atmospheric processes.

How to cite: Catoire, V., Jacquet, P., Chartier, M., Romanini, D., Krysztofiak, G., Ventrillard, I., and Robert, C.: SPECIES: a balloon-borne and airborne instrument coupling infrared lasers with Optical Feedback Cavity Enhanced Absorption Spectroscopy technique for atmospheric in-situ trace-gas measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12978, https://doi.org/10.5194/egusphere-egu23-12978, 2023.

EGU23-13161 | Posters on site | AS3.20

SI-traceable balloon-borne measurements of water vapor in the upper atmosphere 

Béla Tuzson, Simone Brunamonti, Manuel Graf, Tobias Bühlmann, and Lukas Emmenegger

Water vapor (H2O) in the upper troposphere-lower stratosphere (UTLS) is of great importance to the Earth's radiative balance. Yet, accurate measurements of H2O in this region are notoriously difficult, and significant discrepancies were found in the past between different techniques (both in-situ and remote sensing). Currently, cryogenic frostpoint hygrometry is considered as the reference method for balloon-borne measurements of UTLS H2O [1]. However, these devices must be fundamentally reconceived due their use of fluoroform (HFC-23) as cooling agent, which has to be phased out due to its high global warming potential. There is thus an urgent need for alternative, reliable technologies to monitor UTLS H2O, e.g. in long-term global observing networks, such as the GCOS Reference Upper Air Network (GRUAN).

Here we present a new mid-IR quantum-cascade laser absorption spectrometer for balloon-borne measurements of UTLS H2O (ALBATROSS). The spectrometer incorporates a specifically designed segmented circular multipass cell (SC-MPC) that allows for an optical path length of 6 m [2], and it fulfills stringent requirements in terms of mass (< 3.5 kg), size, and temperature resilience. Two successful test flights demonstrated the instrument's outstanding capabilities under real atmospheric conditions up to 28 km altitude [3].

During flights, the instrument experiences a harsh environment with up to 80 K temperature variations and two orders of magnitude change in pressure and H2O amount fraction. To achieve reliable and SI-traceable, we determined the spectral performance and the accuracy of the retrieved amount fractions of ALBATROSS at UTLS-relevant conditions using a dynamic-gravimetric permeation method [4]. SI-traceable reference mixtures were generated with H2O amount fractions as low as 2.5 µmol/mol (or parts per million, ppm) in synthetic air. The results show that ALBATROSS achieves an accuracy better than ±1.5 % at all investigated pressures (30–250 mbar) and H2O amount fractions (2.5–35 ppm). The 1 s relative precision is better than 0.3 %, while 5 nmol/mol (i.e., parts per billion, ppb) is reached by averaging for 100 s. Furthermore, ALBATROSS reaches a linear response within ±2 ppm up to 180 ppm H2O.

To achieve this level of performance, the Voigt profile was found to be inadequate. Therefore, we empirically determined all parameters needed to implement the quadratic speed-dependent Voigt profile (qSDVP), which accounts for speed-dependent collision broadening. The qSDVP more accurately captures the H2O line shape at all pressure conditions, and thus significantly improves the accuracy of the retrieved water vapor amount fraction.

Overall, ALBATROSS achieves an unprecedented level of accuracy and precision for a balloon-borne hygrometer, and it demonstrates the exceptional potential of mid-IR laser absorption spectroscopy for in-situ measurements of UTLS H2O. Further in-flight validation campaigns from Lindenberg (Germany) and Payerne (Switzerland) are currently in preparation.

 

[1] Brunamonti et al., J. Geophys. Res. Atmos., 2019, 124, 13, 7053-7068.

[2] Graf et al., Atmos. Meas. Tech., 2021, 14, 1365-1378.

[3] Graf, Emmenegger and Tuzson, Opt. Lett., 2018, 43, 2434-2437.

How to cite: Tuzson, B., Brunamonti, S., Graf, M., Bühlmann, T., and Emmenegger, L.: SI-traceable balloon-borne measurements of water vapor in the upper atmosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13161, https://doi.org/10.5194/egusphere-egu23-13161, 2023.

EGU23-14492 | ECS | Posters virtual | AS3.20

Highly sensitive laser heterodyne radiometer based on a balanced photodetector for carbon dioxide measurement in the atmospheric column 

Tingting Wei, Jingjing Wang, Fengjiao Shen, Tu Tan, Zhensong Cao, Xiaoming Gao, Pascal Jeseck, Yao-Veng Te, Stéphane Plus, Lei Dong, Houston Miller, and Weidong Chen

An all-fiber coupled laser heterodyne radiometer (LHR), using a wideband tunable external cavity diode laser (1500–1640 nm) as local oscillator laser, was developed for ground-based remote sensing of carbon dioxide. Optimal absorption lines and transmission spectra of carbon dioxide in this wavelength range were determined. High sensitivity of the LHR was achieved by using a balanced photodetector to suppress the relative intensity noise of the local oscillator laser. The noise model of the highly sensitive LHR was analyzed and compared with the traditional LHR using single photodetector [1-2]. Finally, field campaigns were performed on the roof of the platform of IRENE building in Dunkerque (51.05°N/2.34°E). The measured LHR spectra in the atmospheric column are compared, in good agreement, with referenced Fourier-transform infrared spectra from the TCCON observation network and with the simulation spectra resulting from an atmospheric transmission modeling. Experimental details including noise analysis and LHR spectra will be discussed and presented.

 

Acknowledgments

The authors thank the financial supports from the LABEX CaPPA project (ANR-10-LABX005), the CPER ECRIN program, the EU H2020-ATMOS project as well as the funding from China Scholarship Council (CSC).

 

References

[1] T. G. Blaney. "Signal-to-noise ratio and other characteristics of heterodyne radiation receivers", Space Science Reviews 17 (1975) 691-702.

[2] F. Shen, G. Wang, J. Wang, T. Tan, G. Wang, P. Jeseck, Y.-V. Te, X. Gao, W. Chen. "A transportable mid-infrared laser heterodyne radiometer operating in the shot-noise dominated regime", Opt. Lett.46 (2021) 3171-3174.

How to cite: Wei, T., Wang, J., Shen, F., Tan, T., Cao, Z., Gao, X., Jeseck, P., Te, Y.-V., Plus, S., Dong, L., Miller, H., and Chen, W.: Highly sensitive laser heterodyne radiometer based on a balanced photodetector for carbon dioxide measurement in the atmospheric column, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14492, https://doi.org/10.5194/egusphere-egu23-14492, 2023.

EGU23-15362 | Orals | AS3.20

Advances and results of two novel sensors for Surveying the Atmospheric Carbon Cycle 

Marta Ruiz-Llata, Pedro Martín-Mateos, Oscar Bonilla-Marique, Aldo Moreno-Oyervides, Yuliy Moreno-Sanoyan, and Omaira García

We will present the preliminary results of the CarbonSurvey project (Towards the Next Generation of Sensors for Surveying the Atmospheric Carbon Cycle). As outlined by the European Commission green report in the framework of the Operational Anthropogenic CO2 Emissions Monitoring and Verification Support (MVS) capacity, the existing ground-based networks currently do not meet all the operational requirements for the Copernicus CO2 MVS capacity due to the lack of in situ measurement data from urban areas and other emission hot spots. The main expected contribution of this project is to address this weakness through the development of a new generation of instruments to enable unprecedented CO2 monitoring capabilities, the biggest GHG contributor to human-caused global warming. The necessary scientific and technical contributions required to reach the main goal of the project involve two complementary developments: (i) firstly, a gas analyzer capable of obtaining the vertical profile (with resolution in altitude) of CO2 concentration. The system, which is based on the Laser Heterodyne Radiometry (LHR) technique, will operate from the Earth's surface analyzing the effect in the spectrum of the received sunlight of the atmospheric components to accurately find the distribution of the concentration of CO2 in the atmospheric column. Thus, this instrument will provide a characterization of the CO2 in the atmospheric volume located above the measurement site. Secondly, (ii) the project aims to develop Photacoustic Spectroscopy (PAS) cost-competitive photonic solution for in situ urban GHG measurements. As a main difference with today’s commercially available instrumentation, the system proposed, based on a compact photoacoustic sensing cell, will combine small-size, high sensitivity, and a straightforward field deployment capacity. This directly enables the possibility of providing an accurate, and potentially gap-free, map of the concentration of gases at ground level. These two sets of instruments provide indeed complementary information for a full reconstruction of the map of CO2 around the areas of interest. It is important to remark that both instrument designs will be equipped as well with an important additional feature: the ability to determine the isotopic fingerprint of CO2 in order to discern between natural and anthropogenic CO2 sources, such as fossil fuel combustion or biogenic respiration.

The CarbonSurvey project is funded by the Spanish State Research Agency, it started December 2022 and last until November 2024. We will present the sensors design and the preliminary laboratory results. By the end of the project, we will have both sensor prototypes fully operational and calibrated at the Izaña Atmospheric center. Moreover, the sensing systems will be specifically designed for a straightforward in situ deployment in different areas of interest, providing full coverage of the most important blind spots existing today. This new generation of sensors could establish the necessary basis to guide decision-making policies in the green transition process ahead.

How to cite: Ruiz-Llata, M., Martín-Mateos, P., Bonilla-Marique, O., Moreno-Oyervides, A., Moreno-Sanoyan, Y., and García, O.: Advances and results of two novel sensors for Surveying the Atmospheric Carbon Cycle, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15362, https://doi.org/10.5194/egusphere-egu23-15362, 2023.

EGU23-16250 | Orals | AS3.20

Low-temperature mid-IR absorption spectroscopy for isotopomer-specific measurements 

Lukas Emmenegger, Akshay Nataraj, Michele Gianella, Jérôme Faist, and Béla Tuzson

The measurement of singly substituted, stable isotopologues, such as 13CO2, by mid-IR spectroscopy is well established. In addition, there is a great interest to exploit the information carried by more exotic isotopologues, i.e. of low abundance, multiply substituted (clumped) isotopic species or site-specific isotopomers. This information on isotopic composition can be used as proxy to constrain formation pathways, source attribution, temperature histories or dating (radioactive isotopes) of the respective molecules. The established method to perform such isotopic analysis is isotope ratio mass spectrometry (IRMS). This approach, however, in particular for rare isotopologues, typically requires very demanding instruments, several hours of analysis time and extensive sample preparation to separate isobaric interferences.

Here, we demonstrate an alternative analytical method based on optical interrogation of the molecules by directly probing their ro-vibrational frequencies. This makes the method inherently suitable to distinguish between isotopomers (structural isomers). Furthermore, we propose a low temperature approach that substantially reduces the spectral interferences due to hot-band transitions of more abundant isotopologues. The effectiveness and versatility of this strategy are highlighted by three different applications: i) high-precision mid-IR measurements of clumped 12C18O2, ii) the detection of 14CO2 in enriched CO2 samples, and iii) a new scheme for determination of the intramolecular distribution (terminal and central positions) of 13C in propane.

We developed a quantum cascade laser (QCL) spectrometer using a Stirling-cooled circular multipass absorption cell. The distributed feedback (DFB) QCL is driven in intermittent continuous wave (iCW) mode [1] with a repetition rate of 6.5 kHz. Its beam passes through a compact segmented circular multipass cell (SC-MPC) [2] with an optical path length of 6 m. The SC-MPC is placed in a vacuum chamber that is maintained at 5ּ 10-5 mbar and cooled down to 150 K.

The precision in the ratios [12C18O2]/[12C16O2] and [12C16O18O]/[12C16O2] is 0.05 %₀ with 25 s integration time. Its accuracy is confirmed by agreement with literature values of the equilibrium constant, K, of the exchange reaction for CO2 samples equilibrated at 300 K and 1273 K [3].

As proof of concept, we adapted the system to allow the detection of the radiocarbon 14C in enriched CO2 samples. Due to its ultra-low abundance (10-12), the absorption signatures of this isotopic species is completely hidden by the spectral contributions of the other, more abundant, CO2 isotopologues. Therefore, it is the perfect candidate for low-temperature spectroscopy. We present first results on 14CO2 with a precision of 50 ppt.

And finally, we demonstrate the first high-resolution spectra of propane and its site-specific isotopomers (1-13C and 2-13C). We distinguish their individual contributions to the overall absorption spectrum and show a precision better than 0.1 ‰ for both isotopomer ratios (2-13C)/12C and (1-13C)/12C.

 

 

[1] M. Fischer et al., Opt. Express, 22(6), 7014–7027 (2014), doi: 10.1364/OE.22.007014.

[2] M. Graf, L. Emmenegger, and B. Tuzson, Opt. Lett., 43(11), 2434-2437, (2018), doi: 10.1364/OL.43.002434.

[3] A. Nataraj et al. Opt. Express 30, 4631-4641 (2022): doi.org/10.1364/OE.447172.

 

How to cite: Emmenegger, L., Nataraj, A., Gianella, M., Faist, J., and Tuzson, B.: Low-temperature mid-IR absorption spectroscopy for isotopomer-specific measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16250, https://doi.org/10.5194/egusphere-egu23-16250, 2023.

EGU23-16612 | ECS | Orals | AS3.20

An Analysis of Spectral Simulation Methods for Laser Heterodyne Radiometry for the Vertical Profiling of Greenhouse Gas (GHG) Mixing Ratios 

J. Houston Miller, Monica Flores, David Bomse, and Anthony Gomez

George Washington University and Mesa Photonics are developing and deploying a Laser Heterodyne Radiometer (LHR) that simultaneously measures CO2, CH4, H2O, and O2 mixing ratios throughout the troposphere and lower stratosphere. Spectral fits are constrained by fitting the oxygen spectral line shape – which depends only on pressure and temperature – to improve GHG retrieval precision and provide dry-air corrections. This constraint is achieved by fitting pressure and temperature profiles obtained from the meteorology data measured by radiosondes (vertical resolution ranging from 5-500 m) as part of NOAA’s Integrated Global Radiosonde Archive (IGRA).

Atmospheric spectra are simulated for the column using a spectral simulation package (“LahetraSim”) that uses parameters from the HITRAN spectral database to model spectra through the HITRAN Application Programming Interface (HAPI). Integrated path absorption spectra are calculated using the initial sun angle and estimated radiosonde pressure and temperature profiles. Concentration profiles for CO2, CH4, and H2O can then be iterated on their vertical distributions and refining the pressure and temperature profiles to best fit the oxygen spectrum.

Here we present a comparison of our spectral simulation software to that of an alternative method that has been presented for LHR data processing which makes use of the Planetary Spectrum Generator (PSG) API. Spectral simulations are generated using several atmospheric databases, templates, and transfer models. This tool allows for the extraction of Modern Era Retrospective Analysis, Version 2 (MERRA-2) vertical profiles of pressure and temperature and species abundances from HITRAN. Two limitations of the MERRA-2 database are the latency of approximately 2 months for the latest data availability and the coarse vertical resolution (~1 km) of the available data.  Another benefit of our approach is that approximation of both Planetary Boundary Layer (PBL) and Tropopause Heights can be extracted from the temperature and pressure profiles and these heights can be iterated to refine atmospheric layers; thus increasing their relevance of LHR to GHG modeling.

How to cite: Miller, J. H., Flores, M., Bomse, D., and Gomez, A.: An Analysis of Spectral Simulation Methods for Laser Heterodyne Radiometry for the Vertical Profiling of Greenhouse Gas (GHG) Mixing Ratios, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16612, https://doi.org/10.5194/egusphere-egu23-16612, 2023.

Measuring atmospheric water vapor is an essential but challenging task. The naturally occurring concentrations varies over four orders of magnitude and adsorption and desorption processes on sensors and in sampling systems can distort and attenuate the signal. During airborne measurements H2O concentration gradients that exceed 1400 ppm/s are common and pose an additional challenge [1]. Despite the highly dynamic conditions, especially on research aircrafts like HALO, instrument calibration under static conditions is the norm. This leads to unknown sensor behavior in dynamic conditions and makes it difficult to reliably correct or even identify the influences of dynamic concentration changes on the data. With dynH2O we present an approach to characterize the dynamic response behavior of hygrometers in a metrological and traceable way [2]. dynH2O consists of A) a preparative unit to generate fast and repeatable steps in the water vapor concentration. To generate the concentration steps fast pneumatic valves are used to switch between the flow of two humidity generators which is than mixed into a base flow of dry air. This approach allows the lower and upper bound of the concentration step to be selected independently over a flow range from 13 to 120 standard liters per minute (= sl/min). The generated gas mixture is than passed into B) a flow channel optimized to create a flat concentration front which is monitored by C) an open-path, calibration-free direct Tunable Diode Laser Absorption Spectroscopy (dTDLAS) hygrometer. The dTDLAS reference instrument is operated as a traceable optical gas standard with a temporal resolution of up to 1000 Hz and no sampling delays due to the use of a rotational symmetric multipath cell which is embedded into the walls of the flow channel of the setup. A device under test (DUT) is placed directly behind the optical measurement plane. To characterize the DUT the ideal sensor response is simulated based on the data from the optical reference instrument. The simulated ideal DUT response is used to separate the dynamic response from the setup from the response of the DUT, making the results independent from the setup and easier to transfer to the field. A first order lowpass is used to model the corrected response behavior of the DUT. The characterization of a polymer-based hygrometer will be presented and possibilities to apply the characterization to correct or mitigate the nonlinear distortions of the time axis caused by dynamic H2O concentration changes, by means of different deconvolution methods, will be discussed.
[1] Buchholz, B.; Afchine, A.; Klein, A.; Schiller, C.; Krämer, M.; Ebert, V. HAI, a new airborne, absolute, twin dual-channel, multi-phase TDLAS-hygrometer: background, design, setup, and first flight data. Atmos. Meas. Tech. 2017, 10, 35–57, doi:10.5194/amt-10-35-2017.
[2] Witt, F.; Bubser, F.; Ebert, V.; Bergmann, D. C9.1 Temporal Hygrometer Characterization: Design and First Test of a New, Metrological Dynamic Testing Infrastructure. In System of Units and Metreological Infrastructure. SMSI 2021, digital, 5/3/2021 - 5/6/2021; AMA Service GmbH: Wunstorf, Germany, 2021 - 2021; pp 308–309.

How to cite: Witt, F. and Ebert, V.: dynH2O: A Metrological Approach to Manage the Effects of Dynamic H2O Concentration Changes on Hygrometers in the Field, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17526, https://doi.org/10.5194/egusphere-egu23-17526, 2023.

EGU23-147 | ECS | Posters on site | AS3.21

Oil smoke plumes as seen through MODIS and CALIPSO 

Alexandru Mereuta, Nicolae Ajtai, Andrei Radovici, Camelia Botezan, Horatiu Stefanie, Horia Camarasan, Dan Costin, and Alexandru Ozunu

The main focus of this study is in the analysis and identification of a large number of petrochemical smoke plumes from data records spanning over a decade. The events presented in this study where focused on aerosol resulting from major industrial accidents involving offshore oil rigs, oil tank depots and onshore oil wells. The method is based on a synergistic approach of retrieving aerosol optical and microphysical properties using satellite remote sensing and sun photometer data. Data and instruments used in this study include the Moderate Resolution Imaging Spectroradiometer (MODIS), the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) and Aerosol Robotic Network (AERONET) aerosol retrievals. The study also highlighted the inherit limitation of each individual algorithm, thus depicting the importance of further work on aerosol optical depth (AOD) retrievals from major oil smoke plumes. Results show a wide range of values in part due to the varying magnitude of each event in particular. Based on these results we believe that the AOD from the MODIS instruments show lower than expected values. The CALIPSO retrievals where heavily dependent on the type of lidar solutions showing a large degree of discrepancy between constrained and unconstrained retrievals. Unconstrained solutions were attributed to oil smoke plumes identified as part of a larger local aerosol layer. Conversely, lofted smoke was treated as opaque aerosol layers and the measured lidar solutions showed large values and uncertainty. The MODIS retrieval algorithms over land could not successfully retrieve aerosol properties for petrochemical smoke plumes, thus only the ocean algorithm was used for data analysis. When comparing to other studies that utilized ground-based retrievals, the Ångström exponent (AE) and effective radius (Reff) values seem to be in good agreeance. The measured lidar ratios (LR) and particulate depolarization ratios (PDR) seem to indicate higher values similar to values in the upper ranges of biomass burning smoke. We conclude that further work, utilizing remote sensing ground based systems, is needed to properly assess aerosols properties stemming from oil smoke plumes. These results also show how important a synergic approach is for a complete understanding of such phenomena.

How to cite: Mereuta, A., Ajtai, N., Radovici, A., Botezan, C., Stefanie, H., Camarasan, H., Costin, D., and Ozunu, A.: Oil smoke plumes as seen through MODIS and CALIPSO, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-147, https://doi.org/10.5194/egusphere-egu23-147, 2023.

EGU23-278 | ECS | Posters on site | AS3.21

A 9-YearThee-Dimensional Dust Climatology of the Eastern Mediterranean Basin via CALIPSO-Derived Product 

S. Yeşer Aslanoğlu, Emmanouil Proestakis, Antonis Gkikas, Gülen Güllü, and Vassilis Amiridis

The Eastern Mediterranean Basin is an intricate transition region between Eurasia and the Middle East along with Alpine-Himalayan orogenic belt. It is almost amidst the dusty belt and a unique hot spot of climate change in the grand picture. As it involves desert source areas, dust-carrying winds to remote downstream locations enable the entire basin to expose particulate matter throughout the year. As well as global oscillation systems, increasing surface temperatures promote uplifted and remotely transported dust particles. In order to clarify this phenomenon, the main aim is to determine the aerosol and, particularly, dust climatology of the Eastern Mediterranean Basin via CALIPSO onboard Lidar CALIOP. This prominent instrument enables us to better understand aerosols, clouds, and their interactions associated with climatic processes. Using the 9-year CALIPSO-derived aerosol-dust dataset, horizontal and vertical distributions, transport heights and case incidences were analyzed. Multi-year climatology results indicated that the dust extinction coefficient, dust mass in the total aerosol bulk, and uplifted heights increased as the location shifted from west to east. Moreover, for dust transport, spring months are more dominant in the western part, while summer and autumn are in the central and eastern parts. Mountain range systems in the Alpine-Himalayan Orogenic belt obstruct the lofted and buoyant particles from reaching higher latitudes in the north. Besides, dust particles prone to accumulate on the southern slopes of the high ridges pose air quality degradation of the distant cities from the dust source areas. In addition to remote cities having ~0.2 peak AOD values, source regions exceed 1.0 aerosol and 0.8 dust optical depth values. The whole basin's ambient air has an average of 40% dust mass in the total aerosol load. From the eastern shores of the Mediterranean Sea, desert areas and particulate matter are more prone to intrude into inner lands with a continental connection. So, south-eastern Anatolia in Turkey reflects the desert levels with approximately a dust load of 70%.

How to cite: Aslanoğlu, S. Y., Proestakis, E., Gkikas, A., Güllü, G., and Amiridis, V.: A 9-YearThee-Dimensional Dust Climatology of the Eastern Mediterranean Basin via CALIPSO-Derived Product, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-278, https://doi.org/10.5194/egusphere-egu23-278, 2023.

EGU23-728 | ECS | Posters virtual | AS3.21

Assessment of Impact of air pollution using deep learning-based Air Quality data Model 

Remya Ravikumar, Nagesh Subbana, Alka Singh, and Raian Vargas Maretto

Air pollution poses a major concern to people’s lives. Over two million Indians are said to lose their life to causes attributed to air pollution (Balakrishnan et al., 2019). Most of this pollution comes from industries closely followed by vehicular pollution, unrestrained emission sources, periodic agricultural pollutants, and household pollution. The air quality data obtained from orbital sensors like Sentinel 5 and 5P, MODIS and Landsat and ground sensors (Central pollution control board sensors, CPCB) provide a large amount of information about the particle pollutants present in the atmosphere. This study explored the fusion of data obtained from ground (CPCB) and orbital sensors to better estimate the air quality parameters like PM2.5, NO2, CO and SO2. The combination of these improved parameters will subsequently enhance the air quality index (AQI) approximation. The region of study is the Indo-Gangetic plain, North India because this region hosts eight out of the top ten most polluted cities worldwide.

In this study, we propose a deep neural network-based air quality model by combining fine-grained properties of in-situ (CPCB) data with coarse-grained satellite images. Deep Neural Networks like Convolutional Neural Network (CNN) and Long short-term memory (LSTM) have shown major advantage in solving nonlinear spatio-temporal problems. They can extract valuable contextual features to combine temporal attributes, and model temporal and spatial dependencies accurately. Therefore, we propose the combination of CNN and LSTM models for precise air quality prediction in the Indo Gangetic Plain for the upcoming twenty-four hours based on data acquired on the preceding twenty-four hours.

How to cite: Ravikumar, R., Subbana, N., Singh, A., and Vargas Maretto, R.: Assessment of Impact of air pollution using deep learning-based Air Quality data Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-728, https://doi.org/10.5194/egusphere-egu23-728, 2023.

EGU23-1606 | Orals | AS3.21

High-resolution mapping of nitrogen oxides emissions in US large cities from TROPOMI retrievals of tropospheric nitrogen dioxide columns 

Fei Liu, Steffen Beirle, Joanna Joiner, Sungyeon Choi, Zhining Tao, K. Emma Knowland, Steven Smith, Daniel Q. Tong, and Thomas Wagner

We map high-resolution nitrogen oxides (NOx) emissions in US cities from the retrieved TROPOspheric Monitoring Instrument (TROPOMI) tropospheric nitrogen dioxide (NO2) columns. A new database of gridded emissions at a horizontal spatial resolution of 0.05°×0.05° has been developed using our newly-developed CTM-Independent SATellite-derived Emission estimation Algorithm for Mixed-sources (MISATEAM). We validate the accuracy of MISATEAM using synthetic NO2 observations derived from the NASA-Unified Weather Research and Forecasting (NU-WRF) model at a horizontal spatial resolution of 4 km × 4 km. The validation results demonstrate the excellent agreement between the inferred emissions magnitudes and the NU-WRF given ones with a correlation coefficient (R) of 0.99 and a normalized mean bias (NMB) of -0.08. They also show a consistent spatial pattern with R of 0.88 ± 0.06 for all investigated cities when comparing inferred and given emissions at grid level. The TROPOMI-based database derived in this study includes annual emission maps for 39 US large cities from 2018 to 2021. While there is a good agreement with national emission inventory (NEI) in general, there are noticeable differences in spatial pattern in some cases. The satellite-derived spatiotemporal patterns of NOx emissions complement information difficult to capture in the conventional emission inventories compiled with “bottom-up” methods by suggesting the misallocation of emissions and/or missing sources. We expect to extend the database globally and also include estimates based on NO2 observations from OMI to provide a longer time record. The method could also be applied to data from future geostationary satellites, such as Geostationary Environment Monitoring Spectrometer (GEMS) or the Tropospheric Emissions: Monitoring Pollution (TEMPO) instrument, to provide diurnal variations in NOx emissions.

How to cite: Liu, F., Beirle, S., Joiner, J., Choi, S., Tao, Z., Knowland, K. E., Smith, S., Tong, D. Q., and Wagner, T.: High-resolution mapping of nitrogen oxides emissions in US large cities from TROPOMI retrievals of tropospheric nitrogen dioxide columns, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1606, https://doi.org/10.5194/egusphere-egu23-1606, 2023.

EGU23-1806 | ECS | Posters virtual | AS3.21

Sulfur dioxide (SO2) trends over the urban regions of China during 2007–2020 using MERRA-2 and CAMSRA 

Abdallah Shaheen, Robabeh Yousefi, Fang Wang, Quansheng Ge, and Renguang Wu

Sulfur dioxide (SO2) plays a key role in the formation of atmospheric sulfate that can adversely affect urban environment, human health, air quality, and the Earth’s climate system. In this talk, we present results of SO2 trends over the 4 urban regions (YRD, BTH, PRD, and SCB) of China during 2007-2020, using the SO2 massconcentrations of the Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2), and the SO2 total column of Copernicus Atmosphere Monitoring Service Reanalysis (CAMSRA). The SO2 concentration decreased significantly during 2007-2020 over the 4 regions: YRD, BTH, PRD, and SCB, with the rate of -0.04 µg.m-3 per year, -0.05 µg.m-3 per year, -0.01 µg.m-3per year, and -0.03 µg.m-3 per year, receptively. Using CAMSRA data, total column of SO2 also experienced significant decreasing trends during 2007-2020 over YRD, PRD, and SCB, with the rate of -0.15 mg.m-2 per year, -0.05 mg.m-2 per year, and -0.06 mg.m-2 per year, receptively. The decreasing SO2 levels after 2007 were mainly attributed to Chinese air pollution control policies. This work contributes to a better understanding of the impact of Chinese policies on the SO2 level over the urban regions of China.

How to cite: Shaheen, A., Yousefi, R., Wang, F., Ge, Q., and Wu, R.: Sulfur dioxide (SO2) trends over the urban regions of China during 2007–2020 using MERRA-2 and CAMSRA, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1806, https://doi.org/10.5194/egusphere-egu23-1806, 2023.

EGU23-1826 | Orals | AS3.21

Operational Algorithm of Aerosol Effective Height from the Geostationary Environment Monitoring Spectrometer (GEMS) 

Sang Seo Park, Jhoon Kim, Yeseul Cho, and Junsung Park

The Geostationary Environment Monitoring Satellite (GEMS) retrieves several species of trace gases and aerosol properties. For the aerosol property, retrieval results from the GEMS can be used for the surface air quality analysis and aerosol effect for the airmass factor (AMF) calculation. To provide accurate information on aerosol, in addition, aerosol vertical information is also retrieved from the GEMS defined by the aerosol effective height (AEH). The AEH can help to estimate the AMF for tropospheric trace gases and surface concentration of particulate matter (PM). 

The aerosol vertical distribution is relatively difficult to retrieve compared to those of clouds, because the optical property of aerosol is various due to the various aerosol types in the atmosphere. For the UV-visible hyperspectral observation, the aerosol vertical distribution can estimate from the absorption bands based on the Oxygen molecules, such as O2-A, O2-B, and O2-O2 absorption. Because of the limitation for the spectral coverage from 300~500 nm, however, GEMS is only available to use O2-O2 absorption bands. For the possibility of the AEH retrieval algorithm from GEMS, Park et al. (2016) investigated the theoretical sensitivity test of the AEH retrieval by solely using the O2-O2 absorption band with considering the aerosol and surface properties. Based on the previous studies, we introduce the operational retrieval algorithm for AEH with the theoretical basement. Also, we showed the performance of the operational AEH algorithm from GEMS based on case studies and the validation study using Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP).

How to cite: Park, S. S., Kim, J., Cho, Y., and Park, J.: Operational Algorithm of Aerosol Effective Height from the Geostationary Environment Monitoring Spectrometer (GEMS), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1826, https://doi.org/10.5194/egusphere-egu23-1826, 2023.

EGU23-1935 | Posters on site | AS3.21

Comparative assessment of ozone profile retrievals from OMI, GEMS, and TROPOMI measurements using daily ozonesonde soundings during the ACCLIP summer campaign in 2022 

Juseon Bak, Cheol-Hee Kim, Hyo-Jung Lee, Ja-Ho Koo, Jae-Hwan Kim, Joowan Kim, Kanghyun Baek, SangSeo Park, Wonbae Jeon, and Xiong Liu

Ozone in the troposphere is an important air pollutant and greenhouse gas, and also acts as a principal oxidant in the lower atmosphere. This ozone is not emitted directly from anthropogenic sources, but formed though the photochemical reaction of nitrogen oxides with hydrocarbons in the presence of heat and sunlight. Ozone and its precursor can be transported across continents and to the oceans. As well, the downward transport from the stratosphere plays an important role in controlling the tropospheric ozone abundance. The spatial distribution and trends of tropospheric ozone should be regularly monitored and described to improve our understanding of the chemical and physical processes controlling tropospheric ozone and hence supplement the emission control suppressing the ozone pollution and climate change. In support of monitoring air quality, climate change, and ozone layer from space, hyperspectral UV measurements have been regularly accumulated from polar orbiting satellites since the late 1990s as well as geostationary service was recently started in 2019, but retrieving ozone profiles are still uncertain, especially over the troposphere. In this study, we present an optimal estimation-based ozone profile algorithm which is matured for processing OMI measurements with the state of art soft calibration. The capability of this research algorithm is also evaluated for retrieving ozone profiles from TROPOMI and GEMS. Each research ozone profile retrieval is inter-compared with the corresponding operational product. As a reference, we use daily ozonesonde soundings launched at Anmyeondo Island in South Korea during August 2022. It is collected as a part of the ACCLIP (Asian Summer Monsoon Chemical & Climate Impact Project) airborne field campaign in July-August, 2022 to investigate the upper troposphere and lower stratosphere composition under the influence of the Asian summer monsoon. In this study, quantitative differences between ozonesonde measurements and satellite data are assessed with the qualitative evaluation of how satellite measurements represent the ozone variability influenced by the atmospheric circulation.

How to cite: Bak, J., Kim, C.-H., Lee, H.-J., Koo, J.-H., Kim, J.-H., Kim, J., Baek, K., Park, S., Jeon, W., and Liu, X.: Comparative assessment of ozone profile retrievals from OMI, GEMS, and TROPOMI measurements using daily ozonesonde soundings during the ACCLIP summer campaign in 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1935, https://doi.org/10.5194/egusphere-egu23-1935, 2023.

EGU23-2036 | ECS | Posters on site | AS3.21

Modelling the impact of Biogenic Volatile Organic Compound emissions on Formic Acid concentrations above Central Europe 

Marina Liaskoni, Cathy Clerbaux, and Peter Huszar

Formic acid (HCOOH) is among the most abundant carboxylic acids in the atmosphere however, its sources are poorly understood. Photochemical production is thought to be the dominant source of atmospheric HCOOH globally, contributing 60–80% of its total budget. Particularly, he OH‐initiated  oxidation of isoprene produces HCOOH via several known pathways. Here we present a study of how BVOC emissions estimated by the MEGAN model contribute to HCOOH concentrations above central Europe for the 2021 year while the CAMx chemistry transport model was used to calculate the species concentrations. The CAMx produced HCOOH column densities are compared with IASI/AERIS columns while the modelled near surface isoprene concentrations are compared with AirBase data. Although, spatially there is a good agreement between the modeled and the observed values, their magnitude is underestimated in most cases indicating some missing source or underestimated production of formic acid.

How to cite: Liaskoni, M., Clerbaux, C., and Huszar, P.: Modelling the impact of Biogenic Volatile Organic Compound emissions on Formic Acid concentrations above Central Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2036, https://doi.org/10.5194/egusphere-egu23-2036, 2023.

EGU23-2471 | Posters on site | AS3.21

Diurnal variation of columnar and surface in-situ HCHO over Seoul in SIJAQ 2021 

Lim-Seok chang, Donghee Kim, Min-Suk Bae, and Rokjin Park

The GEMS capability to monitor daily changes in key air pollutants was examined with ground-based remote sensing in the SIJAQ 2021 campaign (October 16 - November 11, 2021). In particular, HCHO, a type of GEMS primary product, plays an important role in urban photochemistry as a unique radical source. Diurnal cycles of both columnar and in situ HCHOs were measured in Seoul during SIJAQ 2021. Surface in situ HCHO was higher than toluene known to be abundant in Seoul during the KORUS-AQ period. We analyzed the sensitivities for the main factors controlling HCHO behavior using the land surface-meteorology-chemistry coupled 0-D box-model. Primary emissions, along with background HCHO, contributed significantly to the diurnal variation of HCHO in Seoul. Assuming that HCHO is well mixed within PBL, the vertical integration of modeled HCHO was well matched with  the columnar HCHO.

How to cite: chang, L.-S., Kim, D., Bae, M.-S., and Park, R.: Diurnal variation of columnar and surface in-situ HCHO over Seoul in SIJAQ 2021, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2471, https://doi.org/10.5194/egusphere-egu23-2471, 2023.

Satellite remote sensing techniques can provide detailed information on the spatial and temporal distribution of nitrogen dioxide (NO2) in the troposphere, which enables us to monitor changes in NO2 levels over time and assess the effectiveness of emissions reduction measures. The TROPOspheric Monitoring Instrument (TROPOMI/Sentinel-5P) is particularly useful for identifying pollution sources within individual urban areas, as it has a higher spatial resolution with daily global coverage. In this study, we first compared the S5P-PAL reprocessing data with offline products (processor versions are earlier than v2.3.1) and used ground-based Multi-AXis Differential Optical Absorption Spectroscopy (MAX-DOAS) observations in Xuzhou (a city in eastern China) to evaluate the performance. It was found that the size of the footprint can impact the validation results, and the smaller pixels (<29 km2) have a higher correlation with MAX-DOAS (R=0.91). Then we explored its serendipitous capability with the advantages of orbital characteristics and the high spatial resolution of the sensor. Using the overlapping orbits of TROPOMI at high latitudes, we applied a model-free inversion approach to derive diurnal NOx emissions. The orbits of Sentinel-5P allow for a greater than 20% probability of being observed twice within a 100-minute interval on the same day within a range from 35° to high latitudes.  Besides that, we proposed a downscaling method to generate high-resolution (0.05°) NO2 columns from the Ozone Monitoring Instrument (OMI/Aura) retrievals, which has provided continuous measurements since 2004 while having the limitation of relatively low spatial resolution. This model used data from the common observation period of TROPOMI and OMI after 2018 to derive the relationship between high- and low-resolution NO2 concentrations and applied to the historical dataset. Overall, this study demonstrates the utility of overlapping NO2 columns for investigating diurnal variability and highlights the importance of the spatial scale when analyzing and interpreting NO2 data.

How to cite: He, Q., Qin, K., and Cohen, J. B.: Exploring the utility of global high-resolution NO2 columns from TROPOMI for investigating the diurnal variability and downscaling historical measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2616, https://doi.org/10.5194/egusphere-egu23-2616, 2023.

EGU23-2717 | ECS | Posters on site | AS3.21

Data assimilation of NOAA surface and MIPAS satellite observations for improvements towards the global budget of carbonyl sulfide 

Jin Ma, Norbert Glatthor, Marc von Hobe, Steve A. Montzka, and Maarten Krol

Carbonyl sulfide (COS) is a long-lived trace gas with an average tropospheric mixing ratio of approximately 485 pmol mol-1 and a lifetime of about 2 years. In the absence of a significant atmospheric trend, its budget is considered balanced, but significant uncertainties remain on individual sources and sinks. Although challenging, accurate quantification of the COS budget is important because COS uptake by terrestrial biosphere has the potential to be used for improved assessment of Gross Primary Productivity (GPP). Here, we will report inversion progress of optimizing COS global budgets by using TM5-4DVAR. To this end, we assimilate data from the MIPAS limb sounder onboard the ENVISAT satellite that measured atmospheric emission profiles down to the upper troposphere from 2002 – 2012. Tropospheric COS retrievals are assimilated together with NOAA COS surface observations, and a bias correction scheme is employed to correct for potential calibration differences. We will show that: 1) inversion experiments close the budgets and are in favor of reduced biosphere uptake; 2) co-assimilation and bias correction scheme improve fitting ground and satellite retrievals and validation against HIAPER Pole-to-Pole Observations (HIPPO); 3) the prior flux errors are also important for achieving more realistic inversions.

How to cite: Ma, J., Glatthor, N., von Hobe, M., Montzka, S. A., and Krol, M.: Data assimilation of NOAA surface and MIPAS satellite observations for improvements towards the global budget of carbonyl sulfide, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2717, https://doi.org/10.5194/egusphere-egu23-2717, 2023.

EGU23-2937 | ECS | Posters on site | AS3.21

Quantifying nitrogen oxide emissions in the Eastern Mediterranean - Middle East region using TROPOMI observations 

Anthony Rey-Pommier, Frédéric Chevallier, Philippe Ciais, Jonilda Kushta, Theodoros Christoudias, and Jean Sciare
Urban areas and industrial facilities are major sources of air pollutants, as they concentrate a large part of human activity and industrial production. For most of these pollutants, emission inventories are highly uncertain, especially in developing countries. In this context, satellite observations can be used to observe column densities of chemical species to reduce uncertainties in inventories.
 
Here, we use three years of TROPOMI daily nitrogen dioxide (NO2) retrievals to map nitrogen oxide (NOx) emissions at high resolution in Egypt, Qatar and Cyprus. We use a flux-divergence scheme, which expresses NOx emissions as the sum of a wind transport term and a chemical sink term representing the reaction between NO2 and hydroxyl radical (OH).
 
The model allows to identify major NOx hotspots. Among these, heavy industrial facilities, such as cement plants and fossil-fuel fired power plants, are characterized by a predominance of the transport term over the sink term. Heavily populated urban centers can also be identified, with a predominance of the sink term. In Egypt, our model is able to detect a weekly cycle in NOx emissions, reflecting Egyptian social norms, and to quantify the drop of emissions in 2020 due to the Covid-19 pandemic. In Qatar, it is able to infer the emission factor of isolated power plants, which is consistent with reported values. In Cyprus, it is able to quantify the emissions from different power plants, with higher emissions on the north side of the island due to the use of different technologies and fuels. These results demonstrate a high potential for satellite-based emission mapping at the scale of large urbanised areas well observed by TROPOMI.

How to cite: Rey-Pommier, A., Chevallier, F., Ciais, P., Kushta, J., Christoudias, T., and Sciare, J.: Quantifying nitrogen oxide emissions in the Eastern Mediterranean - Middle East region using TROPOMI observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2937, https://doi.org/10.5194/egusphere-egu23-2937, 2023.

EGU23-2972 | Orals | AS3.21

Introduction to GEMS version two air pollutants retrieval algorithm 

Hyunkee Hong, Junsung Park, Hanlim Lee, Wonjin Lee, deokrae Kim, Jhoon Kim, and Dongwon Lee

Geostationary Environment Monitoring Spectrometer (GEMS), the world's first geostationary environmental senor onboard Geo-Kompsat 2B, was launched in February, 2020 to monitor atmospheric pollutants (such as -> e.g. Aerosol properties, Nitrogen dioxide, Sulphur dioxide, Formaldehyde and Ozone) with high temporal and spatial resolution over ASIA. Environmental Satellite Center (ESC) of National Institute of Environmental Research has distributed these data since March, 2021 after in-orbit test was completed. 
We performed the accuracy validation of GEMS atmospheric pollutants retrieval algorithm using other environmental satellite (such as TROPOMI, OMPS, etc.) and ground-based measurements (such as Pandora, Max-DOAS, etc.) data through GEMS Map of Air Pollution (GMAP) and Satellite Integrated Joint monitoring of Air Quality (SIJAQ) campaign. 
We validated the accuracy of GEMS atmospheric-pollutants-retrieval algorithm using the data from other environmental satellites (e.g. TROPOMI, OMPS, etc.) and ground-based measurements data (e.g. Pandora, Max-DOAS, etc.).
After that, we improved the accuracy of retrieval algorithm and released GEMS version two data in November last year. In this version two data, we found improvements needed in a priori data, cloud data, and surface reflectance data. In this present study, we introduce the difference and improvements GEMS version two and one data.

How to cite: Hong, H., Park, J., Lee, H., Lee, W., Kim, D., Kim, J., and Lee, D.: Introduction to GEMS version two air pollutants retrieval algorithm, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2972, https://doi.org/10.5194/egusphere-egu23-2972, 2023.

EGU23-3543 | Orals | AS3.21

Estimation of anthropogenic and volcanic SO2 emissions from satellite data in the presence of snow/ice on the ground 

Vitali Fioletov, Chris McLinden, Debora Griffin, Nickolay Krotkov, Can Li, Joanna Joiner, Nicolas Theys, and Simon Carn

Early versions of satellite nadir-viewing UV SO2 data products assumed snow-free surface conditions. Snow covered terrain, with its high reflectance in the UV, typically enhances satellite sensitivity to boundary layer pollution. However, a significant fraction of high-quality cloud-free measurements over snow is currently excluded from analyses.  This leads to increasing the uncertainties of the satellite emissions estimates and introducing potential seasonal biases due to the lack of data in winter months for some high-latitudinal sources. In this study, we investigated how OMI and TROPOMI satellite SO2 measurements over snow-covered surfaces could be used to improve the annual emissions reported in our SO2 emissions catalogue (version 2, Fioletov et al., 2023). Although only 100 out of 759 sources listed in the catalogue have 10% or more of the observations over snow, for 40 high-latitude sources more than 30% of measurements suitable for emission calculations were made over snow-covered surfaces. For example, in the case of Norilsk, the world’s largest SO2 emissions point source, annual emissions estimates in the SO2 catalogue were based only on 3-4 summer months, while addition of data for snow conditions extends that period to 7 months.

 

Emissions in the SO2 catalogue were based on satellite measurements of SO2 slant column densities (SCDs) that were converted to vertical column densities (VCDs) using site-specific clear-sky air mass factors (AMFs), calculated for snow-free conditions. The same approach was applied to measurements with snow on the ground whereby a new set of constant, site-specific, clear-sky with snow AMFs was created, and these were applied to the measured SCDs. Annual emissions were then estimated for each source considering (i) only snow-free days, (ii) only clear-sky with snow days and (iii) a merged dataset (snow and no snow conditions). For individual sources, the difference between emissions estimated for snow and snow-free conditions is within ±20% for three quarters of smelters and oil and gas sources, and with practically no systematic bias. This is excellent consistency given that there is typically a 3-5 times difference between AMFs for snow and snow-free conditions. For coal-fired power plants, however, emissions estimated for snow conditions are on average 25% higher than for no snow conditions; this difference is likely real and due to larger production (consumption of coal) and emissions in wintertime.

 

Reference:

Fioletov, V. E., McLinden, C. A., Griffin, D., Abboud, I., Krotkov, N., Leonard, P. J. T., Li, C., Joiner, J., Theys, N., and Carn, S.: Version 2 of the global catalogue of large anthropogenic and volcanic SO2 sources and emissions derived from satellite measurements, Earth Syst. Sci. Data, 15, 75–93, https://doi.org/10.5194/essd-15-75-2023, 2023.

How to cite: Fioletov, V., McLinden, C., Griffin, D., Krotkov, N., Li, C., Joiner, J., Theys, N., and Carn, S.: Estimation of anthropogenic and volcanic SO2 emissions from satellite data in the presence of snow/ice on the ground, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3543, https://doi.org/10.5194/egusphere-egu23-3543, 2023.

TROPOMI Monitoring of NO2 Sources and Spread during the Beirut 2020 Seaport  Ammonium Nitrate Explosion

 

Nayla El-Kork1,2, Ashraf Farahat3

1Space and Planetary Science Center, Khalifa University,P.O. Box 127788, Abu Dhabi, United Arab Emirates;

nayla.elkork@ku.ac.ae 

2Department of Physics, Khalifa University, P.O. Box 127788, Abu Dhabi, United Arab Emirates;

3Department of Physics, College of Engineering and Physics, King Fahd University of Petroleum, & Minerals, Dhahran 31261, Saudi Arabia.; ashraf.farahat@kfupm.edu.sa 

Ammonium nitrate (NH₄NO₃) is a white crystalline solid chemical compound consisting of ions of ammonium and is commonly used as a high-nitrogen garden and farm fertilizer. Ammonium nitrate can trigger explosions if exposed to a temperature above 190 °C. More than thirty ammonium nitrate accidents have occurred since the beginning of the 19th century, including explosions in the United Kingdom (1916), Germany (1921), the United States (1942, 1947, and 2013), France (2001), and China (2015).  The most recent massive explosion occurred on August 4, 2020, in Beirut, Lebanon. The explosion killed over 200 people, injured about 7,000, damaged significant properties in Beirut, and loaded large amounts of particulate matter, dust, and toxic gases into the atmosphere. 

In this work, we use NO2 measurements from the Level 2 NO2 TROPOspheric Monitoring Instrument (TROPOMI), onboard S5P (100 – 700 nm) to investigate the generation of the toxic NO2 gas during the Beirut explosion. Interestingly a high NO2 emission over Beirut was observed from 28 July – 3 August 2020, a few days before the Beirut blast, with the highest emission on 28 July. This high NO2 background is attributed to many reasons: vehicle and ship emissions and the armed conflict in Syria. To confirm the possible effects of vehicles and ships in increasing NO2 loading in the atmosphere, the NO2 emission from Cairo, Egypt (known for its high population and high traffic volume); Nicosia, Cyprus (known for its low population and low traffic volume); and Suez Canal, Egypt (known for its high ship traffic and high traffic volume) are compared to Beirut NO2 emissions. Meanwhile, to understand the spatiotemporal distribution of NO2 (before, during, and after the explosion), the emission is examined in seven locations with four coastal (Beirut, Jounieh, Batron, and Tripoli) and three inland cities (Ehden, Baalbek, and Ain El Bnaiyyeh) in Lebanon. Results indicate that although NO2 was emitted during the Beirut blast, its amount was not significantly high, and it only affected some of the coastal locations within 20 – 25 km of Beirut, while it did not seem to affect the inland regions. The reported NO2 emission from the explosion could be overestimated, as there is an already high NO2 background in Beirut from vehicles, ships, and the armed conflict in Syria.  

 

How to cite: El-Kork, N. and Farahat, A.: TROPOMI Monitoring of NO2 Sources and Spread during the Beirut 2020 Seaport Ammonium Nitrate Explosion, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4187, https://doi.org/10.5194/egusphere-egu23-4187, 2023.

EGU23-4729 | ECS | Posters on site | AS3.21

Toward diurnal observations of tropospheric NO2 from Chinese polar-orbiting satellite series 

Chengxin Zhang and Cheng Liu

Nitrogen oxides (NOx=NO2+NO) play an important role in atmospheric chemistry and human health. Satellite measurements of atmospheric NO2 have been made available by satellite ultraviolet‒visible spectrometers such as GOME, SCIAMACHY, OMI, and TROPOMI. To enhance the stereoscopic monitoring of air quality, China has launched the series of Environmental trace gases Monitoring Instruments (EMI) onboard multiple satellites including GaoFen-5 (2018 May–2020 April), GaoFen-5A (since 2022 December), GaoFen-5B (since 2021 September), and DQ-1 (since 2022 April), as well as more satellites to be planned. The EMI-series instruments can measure NO2 at two local overpass times, i.e., 10:30 in the morning (DQ-1) and 13:30 in the afternoon (others), with a nadir spatial resolution of 12×13 km2. In this study, we optimized a consistent retrieval algorithm for tropospheric NO2 from the EMI series by fitting spectra with an earthshine reference over the remote ocean, masking cloudy pixels by the cloud fraction, and calculating the air mass factor by using high-resolution a priori profiles from a global chemical model and surface Lambertian-equivalent reflectivity. We have compared the EMI NO2 retrievals with ground-based remote sensing measurements from NDACC, TCCON and other MAX-DOAS networks, as well as other satellites such as OMI, TROPOMI and GEMS. In general, both ground and satellite validations show good correlations and high precision of EMI NO2 datasets. Finally, we explored the potential of detecting the diurnal variability of atmospheric NO2 in different global cities by using EMI NO2 observations. Such diurnal patterns can be helpful for the understanding of atmospheric chemistry and the design of geostationary satellite instruments in different global regions.

How to cite: Zhang, C. and Liu, C.: Toward diurnal observations of tropospheric NO2 from Chinese polar-orbiting satellite series, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4729, https://doi.org/10.5194/egusphere-egu23-4729, 2023.

EGU23-4767 | Orals | AS3.21

Remote sensing of trace gases with Chinese satellite instruments 

Cheng Liu, Chengxin Zhang, Wenjing Su, Qihou Hu, Fei Zhao, Ziwei Li, Chengzhi Xing, Haoran Liu, and Wei Tan

Remote sensing from hyperspectral satellite instruments, such as OMI, TROPOMI and OMPS, can simultaneously obtain the spatio-temporal distribution of several species of trace gases, which has been widely used to study the emissions, regional transport and physical and chemical evolution of trace gases. Nevertheless, there were very few relevant studies using Chinese satellite instruments, because the poor spectral quality makes it extremely difficult to retrieve data from the spectra of the Environmental Trace Gases Monitoring Instrument (EMI), the first Chinese satellite-based ultraviolet–visible spectrometer monitoring air pollutants. In this study, we performed on-orbit wavelength calibration to calculate daily instrumental spectral response functions (ISRFs) and wavelength shifts to diminish the fitting residuals. For the retrieval under the low signal-to-noise ratio (SNR) of EMI, an adaptive iterative retrieval algorithm is set up to select the retrieval setting best with minimum uncertainty. Besides, we used simulated irradiance instead of measured irradiance to obtain the requisite daily solar spectrum for the following retrieval algorithm, because EMI only provides the solar spectrum once every six months. Through these algorithm updates, several trace gases, such as Ozone (O3), nitrogen dioxide (NO2), sulfur dioxide (SO2) and formaldehyde (HCHO), were retrieved from EMI with comparable accuracy of OMI and TROPOMI. The retrieval results from EMI were used to locate emission sources, evaluate regional transport and trace the change of air quality due to important events, such as COVID-19 pandemic, China International Import Expo and Beijing Winter Olympic Games.

How to cite: Liu, C., Zhang, C., Su, W., Hu, Q., Zhao, F., Li, Z., Xing, C., Liu, H., and Tan, W.: Remote sensing of trace gases with Chinese satellite instruments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4767, https://doi.org/10.5194/egusphere-egu23-4767, 2023.

EGU23-5029 | Orals | AS3.21 | Highlight

Improved catalog of NOx point source emissions (version 2) 

Steffen Beirle, Christian Borger, Adrian Jost, and Thomas Wagner

We present an updated (v2) catalog of NOx emissions from point sources 
as derived from TROPOMI measurements of NO2 (PAL product) combined with wind fields from ERA5.
Several improvements have been introduced to the algorithm. 
Most importantly, several corrections are applied, 
accounting for the effects of plume height on satellite sensitivity, 3D topographic effects, 
and the chemical loss of NOx
resulting in considerably higher and more accurate NOx emissions. 
In addition, error estimates are provided for each point source.
        
The catalog v2 is based on a fully automated iterative detection algorithm of point sources worldwide.
It lists 1139 locations that have been found to be significant NOx sources.
The majority of these locations match to power plants listed in the global power plant database.
Other NOx point sources correspond to cement plants, metal smelters, industrial areas, or medium-sized cities.
        
The emissions listed in v2 of the catalog show good agreement (within 20% on average) 
to emissions reported by German Environment Agency (Umweltbundesamt, UBA) 
as well as the United States Environmental Protection Agency (EPA). 

How to cite: Beirle, S., Borger, C., Jost, A., and Wagner, T.: Improved catalog of NOx point source emissions (version 2), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5029, https://doi.org/10.5194/egusphere-egu23-5029, 2023.

EGU23-5209 | Orals | AS3.21

NH3 spatio-temporal variability over Paris, Mexico and Toronto and its link to PM2.5 during pollution events 

Camille Viatte, Rimal Abeed, Shoma Yamanouchi, William Porter, Sarah Safieddine, Martin Van Damme, Lieven Clarisse, Beatriz Herrera, Michel Grutter, Pierre-Francois Coheur, Kimberly Strong, and Cathy Clerbaux

Large cities can experience high levels of fine particulate matter (PM2.5) pollution linked to ammonia (NH3) mainly emitted from agricultural activities. Using a combination of PM2.5 and NH3 measurements from in situ instruments, satellite infrared spectrometers, and atmospheric model simulations, we demonstrate the role of atmospheric NH3 and meteorological conditions in pollution events occurring in Paris, Toronto, and Mexico City.

Ten years of measurements from the Infrared Atmospheric Sounding Interferometer (IASI) are used to assess the spatio-temporal NH3 variability over and around the three cities. The three regions are subject to long range transport of NH3, as shown using HYSPLIT cluster back-trajectories. The results show that the NH3 variability is mainly driven by meteorology, and interestingly, we can detect the fertilizers application period by looking at the NH3 – temperature relationship. To check how well chemistry transport models perform during pollution events, we evaluate simulations made using the GEOS-Chem model for March 2011. In these simulations we find that NH3 concentrations are overall underestimated, though day-to-day variability is well represented. PM2.5 is generally underestimated over Paris and Mexico, but overestimated over Toronto.

We use complementary information derived from IASI, and ground-based open-path measurements over Paris. We, therefore, assess the NH3 temporal variabilities at different timescales (diurnal, seasonal, and interannual), to unravel NH3 sources (agriculture and traffic) in Paris.

How to cite: Viatte, C., Abeed, R., Yamanouchi, S., Porter, W., Safieddine, S., Van Damme, M., Clarisse, L., Herrera, B., Grutter, M., Coheur, P.-F., Strong, K., and Clerbaux, C.: NH3 spatio-temporal variability over Paris, Mexico and Toronto and its link to PM2.5 during pollution events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5209, https://doi.org/10.5194/egusphere-egu23-5209, 2023.

EGU23-5261 | ECS | Posters on site | AS3.21

IASI Carbon Monoxide Global and Regional Trends over the period [2008 - 2022] 

Selviga Sinnathamby, Sarah Safieddine, Camille Viatte, Juliette Hadji-Lazaro, Maya George, and Cathy Clerbaux

Carbon monoxide (CO) is a key atmospheric pollutant that is closely monitored for its role in
tropospheric chemistry as a modulator of the oxidizing capacity of the atmosphere. It is mainly
emitted into the atmosphere during combustion processes linked to anthropogenic activities
(heating, industry, transport) and during biomass combustion (natural fires or burning of agricultural
waste).

Since 2007, three IASI (Infrared Atmospheric Sounding interferometer) instruments have been
successively embarked on board of the polar-orbiting meteorological satellites Metop-A, -B and -C.
They provide a global and daily coverage of CO concentrations in the atmosphere, with two daily
overpasses (at 9:30 am and 9:30 pm local time). In February 2022, EUMETSAT reprocessed the whole
IASI CO dataset , providing a homogeneous record of CO, since the beginning of the mission.

In this study, and for the first time, we use this 15-years of continuous and homogenized dataset to
analyze the evolution of daytime CO concentrations from January 2008 to December 2022. The
Theil-Sen method is applied on the deseasonalized dataset in order to compute the slope of the
trend. The p-value of Sen’s Slope is determined by using the Mann-Kendall test.

Here, we analyze the evolution of CO concentrations on a global and regional scale, and show the
evolution of CO concentrations in each hemisphere and in specific regions of the world that are
sensitive to biomass fires (Central Africa, South America) and anthropogenic emissions (South and
East Asia, Europe and North America). The results are compared with the documented trends in
emission inventories.

How to cite: Sinnathamby, S., Safieddine, S., Viatte, C., Hadji-Lazaro, J., George, M., and Clerbaux, C.: IASI Carbon Monoxide Global and Regional Trends over the period [2008 - 2022], EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5261, https://doi.org/10.5194/egusphere-egu23-5261, 2023.

EGU23-5353 | ECS | Orals | AS3.21

Improving the detection of global NOx emissions from shipping in S5P/TROPOMI data 

Miriam Latsch, Andreas Richter, and John P. Burrows

Ships are important emission sources of nitrogen oxides (NOx), which are relevant pollutants in the atmosphere affecting the environment and human health. Global shipping plays a big role in transporting goods around the world. For decades, some of the busiest shipping lanes have been tracked by satellites from space. With TROPOMI aboard the Sentinel 5-Precursor (S5P), the potential for detecting shipping emissions has increased due to its low noise and high spatial resolution of 5.5 x 3.5 km2. Previous studies have shown that even individual ship plumes can be identified from TROPOMI data.

In this study, we use different filtering methods to identify on a global scale as many shipping emission signals as possible from the TROPOMI data. One important aspect is to focus on finding real shipping signals and avoiding inadvertently interpreting a priori information. The aim of this study is to contribute to the progress of satellite remote sensing of shipping emissions and to better understand air pollution caused by the shipping sector and their effect on the environment.

How to cite: Latsch, M., Richter, A., and Burrows, J. P.: Improving the detection of global NOx emissions from shipping in S5P/TROPOMI data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5353, https://doi.org/10.5194/egusphere-egu23-5353, 2023.

Observations of the vertical distribution of nitrogen oxides (NOx ≡ NO + NO2) in the troposphere are severely limited, despite its influence on ozone formation. Here, we derive vertical profiles of the NOx component NO2 by applying cloud-slicing to partial columns of NO2 from the space-based TROPOMI instrument. This yields seasonal means of NO2 volume mixing ratios at ~100 km resolution for multiple years (March 2018 to February 2022) on a global scale in the upper troposphere (180-320 hPa and 320-450 hPa), the middle troposphere (450-600 hPa and 600-800 hPa) and the boundary layer (800 hPa to the Earth’s surface). We evaluate our product against in situ NO2 measurements from NASA DC-8 aircraft campaigns over Canada (ARCTAS, ATom, INTEX-A), the Eastern US (ATom, SEAC4RS, INTEX-A), the North and South Atlantic (ATom), and the Central and South Pacific (ATom) and use our validated dataset to assess state-of-knowledge of global tropospheric NOx as simulated by GEOS-Chem.  In the middle troposphere, cloud-sliced NO2 has a mean value of 20-40 pptv and deviates by < 5 pptv where NO2 from aircraft observations exceeds the instrument detection limit. The consistency between cloud-slicing results and aircraft observations here is due to high sampling frequency and ideal conditions for cloud-slicing. Differences with aircraft observations are larger (up to 120 pptv) in the upper troposphere between 320-180 hPa where aircraft observations may be susceptible to biases and where cloud-sliced NO2 data are relatively sparse. In the boundary layer, retrievals consistent with the aircraft observations are only possible over marine environments where NO2 concentrations differ by < 35 pptv compared to > 450 pptv over terrestrial regions. This is because large land-based NOx sources cause steep vertical NO2 gradients that are problematic for cloud-slicing which assumes NO2 is well mixed throughout the troposphere. We find that NO2 concentrations above the Eastern US differ by < 20 pptv when comparing cloud-sliced tropospheric vertical profiles to simulated vertical profiles from the GEOS-Chem chemical transport model. However, GEOS-Chem consistently underestimates concentrations of NO2 in the remote troposphere, simulating concentrations that are 50% less than the mean cloud-sliced NO2 observations. This is a result of the limited number of current NO2 observations used to validate models like GEOS-Chem which are limited in both time and space. By deriving tropospheric vertical profiles from cloud-slicing satellite observations there is an opportunity to obtain routine NO2 observations which can then be compared to aircraft measurements and simulations from the GEOS-Chem model. From this, we can determine the environmental factors that impact tropospheric NOx on a global scale and address long-standing uncertainties in our understanding of NOx in the troposphere.

How to cite: Horner, R., Marais, E., and Wei, N.: Retrieval and validation of global tropospheric nitrogen dioxide (NO2) vertical profiles obtained via cloud-slicing TROPOMI partial columns, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5358, https://doi.org/10.5194/egusphere-egu23-5358, 2023.

EGU23-5653 | Orals | AS3.21

TROPOMI tropospheric ozone data: Quality assessment and application 

Arno Keppens, Daan Hubert, Jean-Christopher Lambert, Serena Di Pede, Pepijn Veefkind, Klaus-Peter Heue, Diego Loyola, and Angelika Dehn and the S5P MPC VAL team, CHEOPS-5p validation team, and the SHADOZ ozonesonde station PIs and staff

Contributing to the European Union’s Copernicus Earth Observation programme since October 2017, the Sentinel-5 Precursor (S5P) satellite mission is dedicated to global atmospheric composition measurements for the monitoring and study of air quality and climate. On board of the S5P early afternoon polar satellite, the imaging spectrometer TROPOMI (TROPOspheric Monitoring Instrument) performs nadir measurements of the Earth’s radiance from the UV-visible to the short-wave-infrared spectral ranges at a much finer spatial resolution than its predecessors do, and from which the global distribution of several atmospheric trace gases is retrieved daily, including ozone.

Ozone in the troposphere is the third most important anthropogenic contributor to greenhouse radiative forcing. The distribution of tropospheric ozone is highly variable over a wide range of spatial and temporal scales due to a complex interplay between dynamical, chemical, and radiative processes. Global measurement systems are faced with the challenge of accurately capturing this variability at the scale of interest. In this contribution, we therefore present a comprehensive quality assessment of the recently reprocessed and hence homogenous TROPOMI tropospheric ozone data records, and demonstrate their application. A distinction is made between the tropospheric column and profile products.

The Convective Cloud Differential technique (CCD) is applied to derive three-day running mean ozone columns between surface and 270 hPa over the tropical belt, covering nearly five years of TROPOMI data. These data are characterized primarily by analysing comparisons to SHADOZ ozonesonde and other, currently operating GOME-type sounders (EOS-Aura OMI, Metop-B GOME-2). We will show that the TROPOMI bias varies somewhat with reference instrument, but generally remains below about four Dobson Units. We find signs of a weak latitudinal pattern and a moderate seasonal pattern in the mean differences, again, depending on the reference instrument.

TROPOMI’s operational ozone profile retrieval algorithm is based on the optimal estimation method and was implemented in November 2021, now covering over one year of data. Validation results are collected from both the ESA/Copernicus Atmospheric Mission Performance Cluster/Validation Data Analysis Facility (ATM-MPC/VDAF) and from the S5P Validation Team (S5PVT) AO project CHEOPS-5p. The quality assessment relies on the analysis of retrieval diagnostics in terms of data and information content studies, and on the comparison of TROPOMI data with ground-based measurements. The latter are acquired by ozonesondes and lidars taking part in WMO's Global Atmosphere Watch and its contributing networks NDACC and SHADOZ, and are collected in a harmonized formatting from the ESA Atmospheric Validation Data Centre (EVDC). With a mean comparison bias below 10 % throughout the entire profile and a dispersion of the order of 20 % in the troposphere, the mission requirements are mostly met.

Finally, our verification of the presence of known geophysical structures and cycles confirms that TROPOMI tropospheric ozone data meet the needs of the atmospheric research community. Ultimately, this work paves the way for a more comprehensive evaluation of tropospheric ozone data records contributing to the ongoing tropospheric ozone assessment report (TOAR).

How to cite: Keppens, A., Hubert, D., Lambert, J.-C., Di Pede, S., Veefkind, P., Heue, K.-P., Loyola, D., and Dehn, A. and the S5P MPC VAL team, CHEOPS-5p validation team, and the SHADOZ ozonesonde station PIs and staff: TROPOMI tropospheric ozone data: Quality assessment and application, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5653, https://doi.org/10.5194/egusphere-egu23-5653, 2023.

EGU23-6227 | ECS | Posters on site | AS3.21

Processing of the future IRS-MTG NH3 and temperature products 

Nadir Guendouz, Camille Viatte, Anne Boynard, Sarah Safieddine, Solène Turquety, Martin Van Damme, Lieven Clarisse, Pierre Coheur, Raymond Armante, Pascal Prunet, and Cathy Clerbaux

Ammonia (NH3) is an atmospheric pollutant mainly emitted by the agricultural sector. It is a precursor of fine particles (PM2.5) and therefore has a major effect on public health, and climate change. The volatilization process of NH3 and its lifetime in the atmosphere, as well as its transformation into particles, are poorly constrained and strongly depend on meteorological parameters, in particular temperature.

Although current satellite measurements have evaluated NH3 spatio-temporal variabilities at various scales (global, regional, and local), observations of NH3 diurnal variability and their diurnal variability and dependence to temperature are poorly constrained. This strongly influences our ability to correctly simulate NH3 emissions and associated particulate pollution events in atmospheric models.

The IRS (InfraRed Sounder) instrument which will be launched on the MTG (Meteosat Third Generation) satellite into geostationary orbit in late 2024, will offer the ability to deepen this analysis with more frequent measurements (every 30-45 minutes over Europe and Africa) and better spatially resolved observations (4 km x 4 km at the Equator).

In this presentation, we show the potential of the new geostationary IRS-MTG mission to assess spatio-temporal variabilities of ammonia and temperature focusing on a case study over the high NH3 emitted region of Brittany (France). Using atmospheric states simulated using the CHIMERE chemistry-transport model at the effective spatial resolution of IRS over Brittany, synthetic spectra are computed using the 4A/OP radiative transfer model. NH3 measurement-sensitivity of the future IRS-MTG mission is discussed with regards to the presently available IASI observations.

How to cite: Guendouz, N., Viatte, C., Boynard, A., Safieddine, S., Turquety, S., Van Damme, M., Clarisse, L., Coheur, P., Armante, R., Prunet, P., and Clerbaux, C.: Processing of the future IRS-MTG NH3 and temperature products, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6227, https://doi.org/10.5194/egusphere-egu23-6227, 2023.

EGU23-6310 | Orals | AS3.21

Potential of space-based TROPOMI observations for understanding the spatial  and temporal variability of surface NO2 and its dependencies upon land use over south-western Europe 

Hervé Petetin, Marc Guevara, Steven Compernolle, Dene Bowdalo, Pierre-Antoine Bretonnière, Santiago Enciso, Oriol Jorba, Franco Lopez, Albert Soret, and Carlos Pérez García-Pando

This study presents a comprehensive analysis of the spatio-temporal variability of TROPOMI NO2 tropospheric columns (TrC-NO2) over the Iberian Peninsula over the period 2018-2021 (using the recently released PAL product to ensure consistency).

A first exploration of the impact of cloud cover on the availability of TROPOMI TrC-NO2 observations indicates that data gaps range between 20-30% in summer to 55-70% in April and November, with substantial spatial differences between northern and southern and/or arid areas. The spatial distribution of TrC-NO2 highlights strong hotspots over urban areas (especially Madrid and Barcelona), with additional enhancements along international maritime routes and major highways. A reasonable correlation with surface NO2 mixing ratios is found, around 0.7-0.8 depending on the averaging time.

The weekly and monthly variability of TrC-NO2 over the peninsula is then analyzed at the light of the urban cover fraction (taken from the Copernicus Land Monitoring Service). From least to most urbanized areas, the weekend reduction is found to range from -10 to -40%. A detailed analysis at the intra-agglomeration scale highlights that strongest weekend effects do not always peak in the center but sometimes in surrounding cities, which suggests a larger contribution of commuting to total NOx anthropogenic emissions. Similarly, the monthly profiles strongly change depending on the level of urbanization, from -40%/+26% in summer/winter in most urbanized areas, to -10%/+20% in least urbanized ones. Interestingly, the same analysis applied to cropland fraction highlight an enhancement in June-July that could be due to natural soil NO emissions that are known to peak during the warm season. Beyond some specific discrepancies, a generally good consistency is found between the variability of NO2 seen from space with TROPOMI and the one observed at the surface.

Our study thus illustrates the potential of TROPOMI TrC-NO2 to provide a valuable complement to surface monitoring network, especially in agricultural and maritime areas where surface NO2 observations are missing but yet crucial for better understanding the impact of local NOx emissions, especially for the production of tropospheric ozone.

 

Petetin, H., Guevara, M., Compernolle, S., Bowdalo, D., Bretonnière, P.-A., Enciso, S., Jorba, O., Lopez, F., Soret, A., and Pérez García-Pando, C.: Potential of TROPOMI for understanding spatio-temporal variations in surface NO2 and their dependencies upon land use over the Iberian Peninsula, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2022-1056, 2022.

How to cite: Petetin, H., Guevara, M., Compernolle, S., Bowdalo, D., Bretonnière, P.-A., Enciso, S., Jorba, O., Lopez, F., Soret, A., and Pérez García-Pando, C.: Potential of space-based TROPOMI observations for understanding the spatial  and temporal variability of surface NO2 and its dependencies upon land use over south-western Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6310, https://doi.org/10.5194/egusphere-egu23-6310, 2023.

EGU23-6388 | ECS | Posters on site | AS3.21

Validation of TROPOMI orbital observations on the total column of carbon monoxide by the ground-based measurements at the OIAP stations in Moscow and Zvenigorod. 

Vadim Rakitin, Natalia Kirillova, Andrey Skorokhod, Eugenia Fedorova, and Alexander Safronov

Carbon monoxide (CO) total column (TC) measurements of the TROPOMI high-resolution orbital spectrometer have been validated by ground-based spectroscopic measurements at sites of the A.M. Obukhov Institute of Atmospheric Physics RAS (OIAP RAS) in Moscow and Zvenigorod for the period from 06.28.2018 to 12.31.2021. Correlation coefficients (R) between TROPOMI orbital data and ground-based stationary data have been determined and analyzed. For different resolution of satellite data dependence of correlation parameters on the viewing orbital angles, underlying surface albedo and the height of atmospheric boundary layer (ABL) has been investigated. The high values of the correlation coefficient (R ~ 0.81 – 0.97) were obtained depending on the observation point, spatial averaging and applied filtration. The average systematic difference between TROPOMI and ground-based CO TC measurements was -1.1±7.5% (ZSS) and 1.3±5.7% (Moscow) for orbital data resolution 0.1°×0.1°. The correlation coefficients depend on the viewing azimuthal angles and the height of the atmospheric boundary layer. Correlation increase was obtained during observations at viewing azimuthal angles of less than 40º (up to R~0.97), as well as under increase of ABL height (up to R~0.90). For both sites no influence of surface albedo on the correlation parameters of orbital and ground-based measurements has been found. Also, no significant dependence of correlation on the viewing zenith angle has been detected. 
The study was supported by Russian Science Foundation under grant №21-17-00210.

How to cite: Rakitin, V., Kirillova, N., Skorokhod, A., Fedorova, E., and Safronov, A.: Validation of TROPOMI orbital observations on the total column of carbon monoxide by the ground-based measurements at the OIAP stations in Moscow and Zvenigorod., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6388, https://doi.org/10.5194/egusphere-egu23-6388, 2023.

EGU23-6463 | ECS | Orals | AS3.21

Bayesian estimation of CO2 flux divergence maps using joint (CO2M-like) NO2 and CO2 images 

Erik Koene, Gerrit Kuhlmann, Lukas Emmenegger, and Dominik Brunner

To support the ambition of national and EU legislators to substantially lower greenhouse gas (GHG) emissions as ratified in the Paris Agreement on Climate Change, an observation-based "top-down" GHG monitoring system is needed to complement and support the legally binding "bottom-up" reporting in national inventories. For this purpose, the European Commission is establishing an operational anthropogenic GHG emissions Monitoring and Verification Support (MVS) capacity as part of its Copernicus Earth observation programme. A constellation of up to three CO2, NO2, and CH4 monitoring satellites (CO2M) will be at the core of this MVS system. The satellites, to be launched from 2026, will provide images of CO2, NO2, and CH4 at a resolution of about 2 km  2 km along a 250-km wide swath. This will not only allow observing the large-scale distribution of the two most important GHGs (CO2 and CH4), but also capturing the plumes of individual large point sources and cities.

The divergence method can be used to estimate point source emissions from satellite images, using fewer assumptions than other light-weight plume quantification methods (e.g., no a-priori source locations have to be known). However, the method only uses a few pixels near a point source, while pixels downstream of the source are implicitly excluded. Combined with the high noise of, in particular, CO2 satellite images, the divergence computed from a single overpass image is usually too noisy for CO2 emission quantification. In order to improve the information content in divergence maps, it is therefore common to average the map over many images (e.g., computing monthly or yearly averages) to get better emission estimates. As a result, the temporal resolution of the divergence method is limited.

In this work, we present a novel approach to improve the information content in CO2 divergence maps, by exploiting the joint information content present in the simultaneously acquired CO2 and NO2 images. The purpose of this approach is to allow us to compute accurate divergence maps based on fewer images than typically required for the divergence method, and thus to obtain a finer temporal resolution of emission estimates. The method assumes that the signal-to-noise ratio of NO2 images is better than that of CO2 images, while both images contain a similar set of plumes related to emission point sources. Based on the signal-to-noise ratio in the CO2 and NO2 images and their covariances, we can estimate the optimal CO2 image and optimal CO2 divergence map in the minimum mean square error (MMSE) sense using a linear MMSE estimator. We demonstrate the effectiveness of this estimator on examples from the SMARTCARB dataset (Kuhlmann et al., 2020), and show that an about +20 dB boost in the peak signal-to-noise ratio (PSNR) can be achieved for individual overpass CO2 divergence maps, which is roughly equivalent to the PSNR improvement otherwise obtained by averaging 10 images. Our approach therefore allows us to estimate CO2 emissions over shorter observation periods and increases the emission estimation accuracy of weaker sources.

How to cite: Koene, E., Kuhlmann, G., Emmenegger, L., and Brunner, D.: Bayesian estimation of CO2 flux divergence maps using joint (CO2M-like) NO2 and CO2 images, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6463, https://doi.org/10.5194/egusphere-egu23-6463, 2023.

The Geostationary Interferometric Infrared Sounder (GIIRS) onboard FengYun-4 series satellites is the world’s first geostationary hyperspectral infrared sounder. With hyperspectral measurement covering the carbon monoxide (CO) and ammonia (NH3) absorption windows around 2150 cm-1 and 9150 cm-1, respectively, GIIRS provides a unique opportunity for monitoring the diurnal variabilities of atmospheric CO and NH3 over East Asia. In this study, we develop the FengYun Geostationary satellite Atmospheric Infrared Retrieval (FY-GeoAIR) algorithm to retrieve the CO and NH3 profiles from FY-4B/GIIRS data and provide CO and NH3 maps at a spatial resolution of 12 km and a temporal resolution of 2 hours. The performance of the algorithm is first evaluated by conducting retrieval experiments using simulated synthetic spectra. The result shows that the GIIRS data provide significant information for constraining CO and NH3 profiles. The degree of freedom for signal (DOFS) and retrieval error are both significantly correlated with thermal contrast (TC), the temperature difference between the surface and the lower atmosphere. Retrieval results from one month of GIIRS spectra in July 2022 show that the DOFS for the majority is between 0.6 and 1.2 for the CO total column and between 0 and 1.0 for the NH3 total column. Consistent with retrievals from low-earth-orbit (LEO) infrared sounders, the largest observation sensitivity, as quantified by the averaging kernel (AK), is in the free troposphere for CO and in the lower troposphere for NH3. The diurnal changes in DOFS and vertical sensitivity of observation are primarily driven by the diurnal TC variabilities. This study demonstrates the capability of GIIRS in observing the diurnal CO and NH3 changes in East Asia, which will have great potential in improving local and global air quality and climate research.

How to cite: Zeng, Z.-C., Lee, L., and Qi, C.: Observing Tropospheric Carbon Monoxide and Ammonia from the Geostationary Interferometric Infrared Sounder (GIIRS) onboard FengYun-4B, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6705, https://doi.org/10.5194/egusphere-egu23-6705, 2023.

Tropomi (Tropospheric Monitoring Instrument) is the payload on board of the European Copernicus Sentinel 5 Precursor satellite, dedicated to atmospheric composition monitoring. Tropomi is an imaging spectrometer developed by The Netherlands in cooperation with ESA, measuring in the UV, visible, near infrared and shortwave infrared, with a spectral resolution in the range of 0.25 to 0.5 nm. The spatial sampling of Tropomi is approximately 3.5 x 5.5 km2 for most of the bands and 3.5 x 7.0 km2 in the shortwave infrared. The high spatial resolution in combination with the daily global coverage, are key features for the uptake of the Tropomi data for air quality and climate research, as well as for operational applications. The nominal lifetime of the Tropomi mission is 7 years, however there are currently no technical limitations to extent the lifetime many years longer.

Tropomi was launched in 2017 and the operational data recors starts in April 2018. All operational data products have recently been reprocessed to provide a 5-year consistent data record. The operational data products include short lived pollutants (NO2, SO2, CO, tropospheric O3 and HCHO), O3 total column and profiles, greenhouse gases (CH4 and tropospheric O3), and cloud and aerosol parameters. Furthermore, there are several research products for additional trace gases (CHOCHO, HONO and OClO), aerosol optical thickness, surface parameters (reflectance and vegetation fluorescence) and ocean color.

Tropomi already observed many important events, for example the monitoring of the reduced emissions due to global COVID-19 lockdowns, the discovery of several methane leaks of the oil and gas industry and landfills, the monitoring of the ash cloud of the Hunga Tonga volcanic eruption and the observation of large wildfire plumes from Australia, North and South America, Africa and Siberia.

In this contribution we present the current status, achievements and outlook of the Tropomi mission.

How to cite: Veefkind, J. P. and Team, T. T.: Tropomi on Sentinel 5 Precursor: 5 Years Data Record of the Atmospheric Composition for Air Quality, Climate and Ozone Layer Monitoring, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6815, https://doi.org/10.5194/egusphere-egu23-6815, 2023.

EGU23-7191 | ECS | Orals | AS3.21

Total Column Water Vapour Retrieval from GEMS 

Christian Borger, Steffen Beirle, and Thomas Wagner

Atmospheric water vapour plays a key role for the Earth's energy budget and temperature distribution via radiative effects and latent heat transport. Moreover, the distribution and transport of water vapour is closely linked to atmospheric dynamics on all spatiotemporal scales. In this context, monitoring of the water vapour distribution is essential for numerical weather prediction as well as for climate modelling.

The Geostationary Environment Monitoring Spectrometer (GEMS) instrument on board the GEO-KOMPSAT-2B satellite offers new opportunities for observing and investigating the regional water vapour distribution over East Asia, especially phenomena such as typhoons or atmospheric rivers, and could thus represent another valuable data source, e.g. for nowcasting systems of natural hazards.

In this study, we show the first total column water vapour (TCWV) results retrieved from GEMS UV/vis spectra based on the algorithm of Borger et al. (2020). In addition, we also present an update of the existing algorithm, which, for example, replaces the previous simplified determination of the a priori water vapour profile with a deep neural network. We also compare our results to different reference data sets from ground-based in situ and remote sensing observations, reanalysis models, and satellite measurements.

How to cite: Borger, C., Beirle, S., and Wagner, T.: Total Column Water Vapour Retrieval from GEMS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7191, https://doi.org/10.5194/egusphere-egu23-7191, 2023.

EGU23-7614 | ECS | Posters on site | AS3.21

Testing the CO2M NO2 Retrieval Algorithm using TROPOMI Spatial Zoom Data 

Benjamin Leune, Pepijn Veefkind, Victor Trees, Jos van Geffen, and Ruediger Lang

The future Copernicus Anthropogenic CO2 Monitoring Mission (CO2M) will provide CO2 data at a high resolution of 2x2 km2 with unprecedented accuracy and precision. In addition to bands in the near-infrared and shortwave infrared, the CO2I spectrometer on board of CO2M also contains a visible band for the retrieval of NO2 tropospheric columns. NO2 observations will be performed to aid the detection and identification of CO2 emission plumes, as NO2 is co-emitted during combustion processes and acts as a tracer of CO2. Due to its relatively low tropospheric background value and biospheric influence, local enhancements of tropospheric NO2 are better detectable than those of CO2 and allow for more accurate CO2 emission estimates. Furthermore, this NO2 product will be very valuable for air quality applications, especially emission source quantification.

To fully exploit the high resolution of the NO2 measurements, five times higher than the operational resolution of the TROPOMI instrument onboard Sentinel 5P, improvements on multiple aspects of the air-mass correction in the tropospheric NO2 retrieval algorithm are considered: (1) anisotropic surface treatment at high spatial resolution using MODIS-like products, (2) effective cloud/aerosol parameter retrieval as a scattering layer using co-registered cloud information provided by the on-board cloud imager instrument (CLIM) and the measured O2-O2 and O2-A absorption bands and (3) high resolution NO2 a-priori profiles from the CAMS global/regional model forecasts.

The TROPOMI instrument produced a limited data set during the commissioning phase, where measurements were performed with increased spatial sampling of 2.4x1.8 km2. This data set captures typical scenes showing NO2 emission plumes at a similar spatial resolution as the planned CO2M measurements, allowing for the CO2M NO2 retrieval algorithm to be tested on real data. These TROPOMI zoom data are processed with the new prototype algorithm for CO2M and impacts of the improvements are quantified.

How to cite: Leune, B., Veefkind, P., Trees, V., van Geffen, J., and Lang, R.: Testing the CO2M NO2 Retrieval Algorithm using TROPOMI Spatial Zoom Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7614, https://doi.org/10.5194/egusphere-egu23-7614, 2023.

EGU23-7796 | ECS | Orals | AS3.21

Evaluation of TROPOMI observations for estimating surface NO2 concentrations over Europe using XGBoost Model 

Shobitha Shetty, Philipp Schneider, Kerstin Stebel, Arve Kylling, Terje Koren Berntsen, and Paul Hamer

Nitrogen dioxide (NO2) is among the major air pollutants in Europe posing severe hazard to environmental and human health. The concentrations of surface NO2 are measured by ground monitoring stations which are fairly limited in representation and distribution. While NO2 estimates from chemical transport models are realistic, their complexity makes them computationally intensive. Satellite observations from instruments such as TROPOMI provide high spatiotemporal distribution of NO2. However, these instruments capture NO2 density only along the tropospheric column and not on the surface. Exploiting the availability of ground station measurements and spatially continuous information from TROPOMI, this study estimates surface NO2 concentrations over Europe at 1km spatial resolution for 2019-2021 using XGBoost machine learning model. While ground measurements are used as target reference features, satellite observations such as tropospheric column density of NO2 (from TROPOMI), night light radiance (from VIIRS), NDVI (from MODIS) and modelled meteorological parameters such as planetary boundary layer height, wind velocity, temperature are used as input features to the model. We find an overall mean absolute error of 7.87µg/m3, mean bias of -3.13µg/m3 and spearman correlation of 0.61 during model validation. We found that the performance of the model is influenced by NO2 concentration levels and is most reliable for predictions at concentration levels <40µg/m3 with a relative bias of <40%. The spatial error analysis also indicates the spatial robustness of the model across the study area. The importance of input features is evaluated using SHapley Additive exPlanations (SHAP), which shows TROPOMI NO2 being the most important source for the modelled NO2 predictions. Furthermore, SHAP values also highlight the role of VIIRS night light radiance in deriving finer detailed spatial patterns of surface NO2 estimates. Despite the complex non-linear relationship of the input features, the trained XGBoost model requires an average of 570 seconds to predict single day surface NO2 concentrations for the large study area of continental scale. Thus, this work evaluates the importance of TROPOMI data and reliability of machine learning models for estimating surface NO2 concentrations on a larger spatial scale.

How to cite: Shetty, S., Schneider, P., Stebel, K., Kylling, A., Koren Berntsen, T., and Hamer, P.: Evaluation of TROPOMI observations for estimating surface NO2 concentrations over Europe using XGBoost Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7796, https://doi.org/10.5194/egusphere-egu23-7796, 2023.

EGU23-7951 | ECS | Posters on site | AS3.21

Estimation of anthropogenic NO2 emissions over polluted regions using the LMDZ-INCA model and satellite observations from TROPOMI and OMI 

Santanu Halder, Pramod Kumar, Philippe Ciais, Didier Hauglustaine, Gregoire Broquet, Audrey Fortems, Frederic Chevallier, Anne Cozic, and Bo Zheng

Nitrogen dioxide (NO2), one of the major pollutants, impacts air quality (especially in industrial and urban regions), climate change, etc. We utilize tropospheric vertical column NO2 for 2019 and 2020 from a high-resolution nadir viewing spectrometer TROPOspheric Monitoring Instrument (TROPOMI) which is on board the Sentinel-5 Precurser (S5P) satellite and also from polar orbiting Ozone Monitoring Instrument (OMI) which is on-board the NASA Aura satellite. The high quality observations for TROPOMI are selected using qa_value >= 0.75 and for OMI using cloud radiation fraction < 0.5, zenith angle < 70°, etc. First, we present the simulations of atmospheric NO2 tropospheric vertical columns from a global couple chemistry transport model LMDZ-INCA (Laboratoire de Météorologie Dynamique - INteraction with Chemistry and Aerosol) with a spatial resolution of 1.26×2.5×79 (lat×lon×hybrid σ-level) and temporal resolution of one hour. Further, we utilize monthly global anthropogenic emission inventories from open-source Community Emissions Data System (CDES) and evaluate the model abilities in simulating the observation. In the northern hemisphere, we observe high atmospheric NO2 concentration during the winter season as compared to the summer season from TROPOMI and model due to a longer lifetime and increase in anthropogenic emission. The tropospheric vertical column NO2 in the model is overestimated during winter and underestimated during summer seasons over East US, East Europe, and West Europe. The 50 percentile values between the model and observations are comparable over East US, East Europe, West Europe, and China. However, the model shows high concentration during winter over East and West Europe.

Furthermore, TROPOMI L2 retrievals of tropospheric vertical column NO2 are employed to estimate the surface anthropogenic fluxes of NOx (=NO+NO2). A specific inversion system has been utilized for the estimation of global anthropogenic NO2 emissions based on LMDZ-INCA and TROPOMI NO2 tropospheric vertical columns for 2020 and 2021. It follows a scheme adapted from Zheng et al. (2020). The posterior fluxes are derived by calculating two components. First, we calculated the gridded local sensitivity of concentrations due to changes in the emission. Second, relative observation changes due to the meteorology of a year of interest (e.g. for 2020 or 2021) are calculated using the fluxes of 2019. The reduction of posterior tropospheric total column NO2 as compared to prior during the COVID lockdown period of 2020 is noticed over all the regions. The posterior NOx is decreased by ~30% over China during February-April 2020 compared to the same period of 2019. A relative reduction of anthropogenic NOx fluxes in 2020 as compared to 2019 is observed over other regions (East US, East Europe, West Europe, India, etc.) as well. Our result shows a relative increase in anthropogenic NOx fluxes for 2021 and 2022 as compared to 2019 and 2020 over our study regions.

How to cite: Halder, S., Kumar, P., Ciais, P., Hauglustaine, D., Broquet, G., Fortems, A., Chevallier, F., Cozic, A., and Zheng, B.: Estimation of anthropogenic NO2 emissions over polluted regions using the LMDZ-INCA model and satellite observations from TROPOMI and OMI, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7951, https://doi.org/10.5194/egusphere-egu23-7951, 2023.

EGU23-7964 | Orals | AS3.21

A new generation UV-VIS TROPOMI Aerosol Algorithm 

Omar Torres, Changwoo Ahn, Hiren Jethva, Vinay Kayetha, and Diego Loyola

The NASA S5P-TROPOMI (Sentinel 5 Precursor-Tropospheric Monitoring Instrument) aerosol algorithm (N-TropOMAER) extends the continuous 17-year record of near UV aerosol properties started by the Aura Ozone Monitoring Instrument (OMI) in 2005.  Aerosol optical depth (AOD) and single scattering albedo (SSA) for clear sky conditions and above-cloud aerosol optical depth (ACAOD) are retrieved.  In this presentation we will describe a second-generation UV-VIS algorithm that includes retrieval capability in the visible, and derivation of aerosol layer height (ALH) using TROPOMI O2B band observations. We will also discuss recent theoretical advances that allow extending retrieved aerosol absorption information in the ultraviolet to the visible. Initial results and comparison to other satellite and ground-based observations will be presented.

How to cite: Torres, O., Ahn, C., Jethva, H., Kayetha, V., and Loyola, D.: A new generation UV-VIS TROPOMI Aerosol Algorithm, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7964, https://doi.org/10.5194/egusphere-egu23-7964, 2023.

EGU23-8160 | ECS | Orals | AS3.21

Bromine monoxide composition in volcanic plumes measured by S-5P/TROPOMI – Global survey of magmatic composition 

Simon Warnach, Christian Borger, Nicole Bobrowski, Holger Sihler, Moritz Schöne, Steffen Beirle, Ulrich Platt, and Thomas Wagner

Bromine monoxide (BrO) is a halogen radical influencing atmospheric chemical processes, in particular the abundance of ozone, e. g. in the polar boundary layer and above salt lakes, in the stratosphere as well as in volcanic plumes. Furthermore, the molar bromine to sulphur ratio in volcanic gas emissions is a proxy for the magmatic composition of a volcano and potentially an eruption forecast parameter.

The high spatial resolution combined with the better signal-to-noise ratio of the S-5P/TROPOMI instrument (up to 3.5x5.5km2) and its daily global coverage offer the potential to detect BrO and its corresponding ratio with sulphur dioxide (BrO/SO2) even during minor eruptions and for continuous passive degassing volcanoes.

Here, we present a global overview of BrO/SO2 molar ratios in volcanic dispersion gas plumes derived from a systematic long-term investigation covering four years (January 2018 to December 2021) of TROPOMI data.

We retrieved column densities of BrO and SO2 using Differential Optical Absorption Spectroscopy (DOAS) and calculated mean BrO/SO2 molar ratios for various volcanoes. The calculated BrO/SO2 molar ratios differ strongly ranging from several 10-5 up to several 10-4 both between different volcanoes, but also between measurements at one volcano at different points in time. In our four-year study of S-5P/TROPOMI data we successfully recorded 4232 volcanic plumes, 3063 of which can be clearly assigned to 43 volcanoes. Subsequently, the mean BrO/SO2 ratio is calculated for these plumes - increasing the global data-base of reported BrO/SO2 ratios from 28 to 60 volcanoes. For the first time, BrO/SO2 ratios were successfully determined for six hot spot volcanoes - all of which yield low BrO/SO2 ratios between 2-5x10-5, in contrast to 2-16x10-5 for subduction zone volcanoes, suggesting a depletion of bromine in the Earth’s mantle.

In addition, time-series of the BrO/SO2 ratio were derived for 19 volcanoes, with more than 200 daily measurements of the BrO/SO2 ratio at the five volcanoes Mt. Etna, Italy, Dukono, Indonesia, Popocatepetl, Mexico, Nevado del Ruiz, Colombia, and Sangay, Ecuador.

How to cite: Warnach, S., Borger, C., Bobrowski, N., Sihler, H., Schöne, M., Beirle, S., Platt, U., and Wagner, T.: Bromine monoxide composition in volcanic plumes measured by S-5P/TROPOMI – Global survey of magmatic composition, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8160, https://doi.org/10.5194/egusphere-egu23-8160, 2023.

EGU23-8200 | Posters on site | AS3.21

Assessing the quality of the Sentinel-5p TROPOMI cloud products and their reprocessing using ground-based Cloudnet data 

Steven Compernolle, Athina Argyrouli, Ronny Lutz, Maarten Sneep, Jean-Christopher Lambert, Ann Mari Fjaeraa, José Granville, Daan Hubert, Arno Keppens, Diego Loyola, Ewan O'Connor, Gaia Pinardi, Olivier Rasson, Fabian Romahn, Piet Stammes, Tijl Verhoelst, and Ping Wang

The retrieval of atmospheric composition from space-based measurements, by e.g., Sentinel-5p TROPOMI, is strongly affected by radiative interferences with clouds. Dedicated cloud data products, typically retrieved from measurements by the same sounder, are therefore essential. Cloud information is used to filter data and as input to the modelling of atmospheric radiative transfer and the conversion of slant column densities into vertical column densities.

The three main TROPOMI cloud retrieval algorithms are: (i) L2_CLOUD OCRA/ROCINN CAL (Optical Cloud Recognition Algorithm/Retrieval of Cloud Information using Neural Networks; Clouds-As-Layers), (ii) L2_CLOUD OCRA/ROCINN CRB (Clouds-as Reflecting Boundaries), and (iii) the S5P support product FRESCO-S (Fast Retrieval Scheme for Clouds from Oxygen absorption bands for Sentinel). The cloud variables provided by these products (radiometric cloud fraction, cloud (top) height, and cloud albedo/cloud optical thickness) are subsequently used in the retrieval of the TROPOMI trace gas products. The quality of cloud products and trace gas products is routinely assessed by the ESA/Copernicus Atmospheric Mission Performance Cluster (ATM-MPC) validation service, with ad hoc support from Sentinel-5p Validation Team (S5PVT) AO projects.

Version upgrades have had a significant impact on the characteristics of S5P cloud data. The change of the wavelength window in the FRESCO product since version 1.4 (‘FRESCO-wide’) leads to a clear increase in the height of low clouds with a large impact on the tropospheric NO2 retrieval (van Geffen, 2022), and improving the validation results regarding the tropospheric and total NO2 column. The first upgrades of the ROCINN products (from v1 to v2.1-v2.3) led to an increase in correlation with CLOUDNET cloud height, but to a more negative bias for the low clouds, with ROCINN CRB cloud height even dropping below the CLOUDNET cloud base height on average. However, this effect seems alleviated with the latest upgrade to v2.4. The impact on the HCHO validation results is investigated but is less clear compared to the NO2 case.

To resolve the discontinuities due to the processor version jumps, a full mission reprocessing is currently ongoing and largely carried out for the L2_CLOUD and FRESCO-S products. The reprocessed ROCINN data have a lower dispersion and higher correlation with respect to the CLOUDNET cloud heights. The bias of the L2_CLOUD OCRA/ROCINN CAL CTH becomes more negative, but that of L2_CLOUD OCRA/ROCINN CRB CH bias improves. Finally, we also discuss the impact of the FRESCO-S reprocessing on the validation results.

How to cite: Compernolle, S., Argyrouli, A., Lutz, R., Sneep, M., Lambert, J.-C., Fjaeraa, A. M., Granville, J., Hubert, D., Keppens, A., Loyola, D., O'Connor, E., Pinardi, G., Rasson, O., Romahn, F., Stammes, P., Verhoelst, T., and Wang, P.: Assessing the quality of the Sentinel-5p TROPOMI cloud products and their reprocessing using ground-based Cloudnet data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8200, https://doi.org/10.5194/egusphere-egu23-8200, 2023.

EGU23-8272 | Orals | AS3.21

Evaluation of satellite-derived NOx emissions over Europe 

Ronald van der A, Jieying Ding, Bas Mijling, Henk Eskes, and Marc Guevara

Nitrogen oxides (NOx) emissions play an important role in air quality, the nitrogen cycle, and as precursor for climate gasses. The most important sources of NOx emissions are fossil fuel burning (industry and traffic) and the release from soil.

With the inversion algorithm DECSO (Daily Emissions Constrained by Satellite Observations) we derive quantitative NOx emissions on a 5 to 20 km resolution from TROPOMI (on Sentinel 5p) observations of NO2, taking advantage of the fine spatial resolution (5 x 3.5 km) of the TROPOMI instrument. DECSO is a full inversion algorithm based on data assimilation of satellite observation and the Chemical-transport model CHIMERE. For the data assimilation a Kalman Filter technique is used. For the inversion no apriori information of the NOx emissions is needed and for this reason new sources can be detected. In the postprocessing we use the seasonal cycle to distinct between soil emissions (having strong seasonal cycle with summer peak) and anthropogenic emissions (having low variability over the year).

To assess the quality of satellite-derived NOx emissions on various scales, i.e. national, regional, city and points-sources, they are compared to various bottom-up inventories. For bottom-up emissions we selected NEC (National Emission Ceilings Directive inventory), LRTAP (LRTAP convention data), the CAMS (Copernicus Atmosphere Monitoring Service) regional anthropogenic emission database and the high-resolution emission inventory HERMES (High-Elective Resolution Modelling Emission System) for Catalonia. Detailed results will be shown, including the spatial and temporal variation per emission category.

How to cite: van der A, R., Ding, J., Mijling, B., Eskes, H., and Guevara, M.: Evaluation of satellite-derived NOx emissions over Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8272, https://doi.org/10.5194/egusphere-egu23-8272, 2023.

EGU23-8481 | ECS | Posters on site | AS3.21

Enhancing global SO2 emission inventories using Sentinel-5P TROPOMI satellite data 

Adrian Jost, Steffen Beirle, Christian Borger, Nicolas Theys, Steffen Ziegler, and Thomas Wagner

We report a newly developed global anthropogenic SO2 emission inventory. Within this study, SO2 measurements from the Tropospheric Monitoring Instrument (TROPOMI) onboard the Sentinel-5P satellite have been used to detect and quantify SO2 emissions from point sources for the time range 2018-2022. Our algorithm derives the advection of SO2 by combining TROPOMI SO2 column densities and wind fields from ERA5, i.e. taking the product of vertical column densities and the horizontally projected wind speed. In addition, several corrections, e.g., for satellite sensitivity and topography are applied. The results will be compared to existing emission datasets.

The study is part of the World Emission project funded by ESA and the complete SO2 emission inventory will be available via the World Emission Portal at https://app.world-emission.com.

How to cite: Jost, A., Beirle, S., Borger, C., Theys, N., Ziegler, S., and Wagner, T.: Enhancing global SO2 emission inventories using Sentinel-5P TROPOMI satellite data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8481, https://doi.org/10.5194/egusphere-egu23-8481, 2023.

EGU23-8715 | ECS | Orals | AS3.21

Modelling of near-surface NO2 and O3 concentration over Germany using machine learning 

Vigneshkumar Balamurugan, Jia Chen, Adrian Wenzel, and Frank N. Keutsch

Chemical transport models (CTMs) are commonly used to model air pollutant concentrations. CTMs, on the other hand, require a lot of computing power and sometimes yield biased findings that result from emission inventories and chemical mechanisms employed. Machine learning algorithms are used in a wide range of fields, including Earth system science. Its popularity stems from its ability to learn complex non-linear relationships. As a follow-up of our previous study [1], we attempted to deduce the capability of Machine Learning (ML) in modelling air pollutant concentrations.

In this study, we employed the Gradient Boosted Tree (GBT) algorithm to model near-surface NO2 and O3 over Germany at 0.1 degree resolution and daily intervals. The GBT model is trained using TROPOMI satellite column NO2, O3, HCHO data, as well as meteorology and road density as an information for NOX emission sources. Government air quality (NO2 and O3) observations from urban, suburban, and background stations are used as target variables; 321 stations are considered for NO2 ML model training and 256 stations are considered for O3 ML model training. The GBT model trained for near-surface NO2 explains 68-88% of observed concentrations, whereas, for near-surface O3, the GBT model explains 74-92% of observed concentrations. 

Road density and TROPOMI NO2 data are the most important features in the fitted model for near-surface NO2. This is due to the fact that road density (a proxy for traffic) is the main source of near-surface NOX emission, and the TROPOMI tropospheric NO2 column is a good representation of near-surface NO2 concentration. The downward UV radiation (DUV) at the surface and temperature are the most important features in the fitted model for near-surface O3. Since O3 is formed from the photolysis of NO2, DUV plays an important role in the fitted model for O3. Temperature is the driver of biogenic Volatile Organic Compounds (VOCs), which are an important precursor to O3

In all cases, the GBT model outperforms feed-forward neural networks. Furthermore, the developed GBT model for near-surface O3 is reliably transferable to other locations and countries (R2=0.87-0.94), whereas the developed model for near-surface NO2 is moderately transferable (R2=0.32-0.68). The reason could be that the road density is not the best representative of traffic NOX emissions and can be improved in a future study. Overall, we developed a new machine learning model to cost-effectively model the near-surface NO2 and O3 concentrations, which could help us to better understand the air pollution distribution at a moderate resolution.

References:

Balamurugan, V., Balamurugan, V. and Chen, J., 2022. Importance of ozone precursors information in modelling urban surface ozone variability using machine learning algorithm. Scientific reports12(1), pp.1-8.

How to cite: Balamurugan, V., Chen, J., Wenzel, A., and Keutsch, F. N.: Modelling of near-surface NO2 and O3 concentration over Germany using machine learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8715, https://doi.org/10.5194/egusphere-egu23-8715, 2023.

EGU23-8772 | Orals | AS3.21

Investigation of 3D-effects for UV/vis satellite observations of volcanic plumes 

Thomas Wagner, Simon Warnach, Steffen Beirle, Nicole Bobrowski, Janis Puķīte, Tjarda Roberts, Luke Surl, and Nicolas Theys

Usually, horizontally homogenous atmospheric properties are assumed for the analysis of satellite observations of atmospheric trace gases. While for most atmospheric quations, this simplification causes only small to moderate errors, for the observation of volcanic plumes this neglecting 3D effects can lead to very large errors. These errors (3D effects) can become especially important for satellite observations with high spatial resolution like TROPOMI on Sentinel-5 Precursor.

Different 3D effects were recently investigated for volcanic plumes by Wagner et al. (2022). It was found that especially the so-called light mixing effect can lead to a strong underestimation of the true trace gas amount of volcanic plumes if 1D atmospheric properties were assumed in the retrieval. For strong absorbers like SO2, the underestimation can further be increased by the saturation effect. In that study, different 3D effects were separately studied for idealised plumes.

Here we investigate the combined 3D effects for realistic volcanic plumes using radiative transfer simulations. We focus on two scenarios: first on observations of the ascending part of the plume above a volcano and second on the horizontally advected plume at a distance from the volcanic vent. In addition to the 3D effect of the volcanic plume (trace gases and aerosols), also the influence of the surface elevation is investigated.

 

Wagner, T., Warnach, S., Beirle, S., Bobrowski, N., Jost, A., Puķīte, J., and Theys, N.: Investigation of 3D-effects for UV/vis satellite and ground based observations of volcanic plumes, Atmos. Meas. Tech. Discuss. [preprint], https://doi.org/10.5194/amt-2022-253, in review, 2022.

How to cite: Wagner, T., Warnach, S., Beirle, S., Bobrowski, N., Puķīte, J., Roberts, T., Surl, L., and Theys, N.: Investigation of 3D-effects for UV/vis satellite observations of volcanic plumes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8772, https://doi.org/10.5194/egusphere-egu23-8772, 2023.

EGU23-8804 | Posters on site | AS3.21

An improved tropospheric NO2 product for the GEMS instrument 

Andreas Richter, Kezia Lange, Tim Boesch, Bianca Zilker, Miriam Latsch, Lisa Behrens, John P. Burrows, Si-Wan Kim, Hyunkee Hong, Hanlim Lee, and Junsung Park

Nitrogen oxides are among the most important pollutants in the troposphere. They are emitted in many anthropogenic activities such as fossil fuel use for energy production and transportation or agricultural burning. At high concentrations, nitrogen oxides are a health hazard. They also are involved in the formation of tropospheric ozone and acid rain.

There are many different ways to measure nitrogen oxides in the atmosphere. Satellite observations of NO2 are one of the most powerful as they provide excellent coverage. However, the spatial resolution is limited and in the case of measurements from low-earth satellites, there is only one measurement per day. The latter problem can be overcome by using geostationary satellites, and the Korean GEMS instrument is the first to provide hourly NO2 observations over Asia.

In this study, a full year of tropospheric NO2 columns are retrieved from GEMS observations. Different retrieval settings are applied and the results compared with a particular emphasis on the analysis of the diurnal variation of NO2. Sensitivity tests include correction for the polarisation sensitivity of the GEMS instrument, different stratospheric correction schemes, different surface reflectances and different a priori profiles. While all of these parameters affect the retrieved NO2 columns, the pattern of the diurnal variation of the retrieved tropospheric columns appears to be robust, at least over regions with large pollution signals.

How to cite: Richter, A., Lange, K., Boesch, T., Zilker, B., Latsch, M., Behrens, L., Burrows, J. P., Kim, S.-W., Hong, H., Lee, H., and Park, J.: An improved tropospheric NO2 product for the GEMS instrument, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8804, https://doi.org/10.5194/egusphere-egu23-8804, 2023.

EGU23-9232 | ECS | Posters on site | AS3.21

Improved CCD tropospheric ozone from S5P/TROPOMI satellite data using local cloud fields 

Swathi Maratt Satheesan, Kai-Uwe Eichmann, Mark Weber, and John Burrows

Tropospheric ozone is an important pollutant and greenhouse gas in the Earth’s atmosphere. Due to its short lifespan and dependence on sunlight and precursor emissions from natural and anthropogenic sources, tropospheric ozone exhibits a high spatio-temporal variability on seasonal, inter-annual and decadal time scales, which, in turn, poses a clear challenge to the satellite observing system. The Convective Cloud Differential (CCD) and Cloud Slicing Algorithms (CSA) are two standard tropospheric ozone retrieval methods limited to the tropical band (20◦S-20◦N). In particular, the CCD approach has been successfully applied to currently operating satellite sensors such as Aura OMI, MetOp GOME-2 and Sentinel-5 Precursor TROPOMI to derive tropical tropospheric column ozone (TTCO). In this study, we present the CHORA-CCD (Cloud Height Ozone Reference Algorithm-CCD) for retrieving TTCOs from TROPOMI. It uses a local cloud reference sector (CLC, CHORA-CCD Local Cloud) rather than the more common CCD approach using the Pacific region (CPC, CHORA-CCD Pacific Cloud) to determine the TTCO by subtracting the stratospheric (above cloud) column from the total column in clear-sky scenes in the same zonal band. An important assumption for this method is the zonal invariance of stratospheric ozone, which is only valid in the tropics. The local cloud approach is the first step to avoid this constraint and to extend the CCD method to middle latitudes, where stratospheric ozone variations are larger. An iterative approach has been developed for the automatic selection of an optimal local cloud reference sector around each retrieval grid box varying longitudinally from ±5◦ to a maximum of ±50◦. The CLC algorithm is further adapted and optimised in the CLCT algorithm by introducing a homogeneity criterion for total ozone to overcome the inhomogeneities in stratospheric ozone. An alternative method to directly estimate the above cloud column down to a reference altitude (270 hPa) is also introduced based on the Theil-Sen regression. The latter allows combining the CCD method with the CSA. Monthly averaged TTCOs using the Pacific cloud reference sector (CPC) and local cloud reference sector (CLC, CLCT) have been determined over the tropics and subtropics (26◦S-21◦N) from TROPOMI for the time period from 2018 to 2021. The accuracy of the various methods was investigated by comparisons with collocated NASA/GSFC SHADOZ ozonesonde retrievals. At eight out of twelve stations, TTCOs using CLC and CLCT yields better agreement with ozonesondes than CPC. In the tropics, the overall mean CLCT bias and dispersion of -6±8% is lower than the 11±12% of CPC. Similarly, in the subtropics, the CLCT algorithm significantly improves overall bias and scatter (-15±9%) compared to CPC (-25±19%). The overall statistical dispersion is effectively reduced to 2DU using CLCT from 5DU using CPC. In this presentation, a detailed validation of the new local CCD retrievals will be given. Our results demonstrate the advantage of using the local cloud reference sector in the subtropics, thereby providing an important basis for subsequent systematic applications in current and future missions of geostationary satellites, like ESA Sentinel 4, NASA Tempo, and GEMS covering only middle latitudes.

How to cite: Maratt Satheesan, S., Eichmann, K.-U., Weber, M., and Burrows, J.: Improved CCD tropospheric ozone from S5P/TROPOMI satellite data using local cloud fields, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9232, https://doi.org/10.5194/egusphere-egu23-9232, 2023.

EGU23-9309 | ECS | Posters on site | AS3.21

Developing Deep Learning Methods for Surface NO2 Estimation from GEMS Satellite Data 

Janek Gödeke, Hyunkee Hong, Andreas Richter, Peter Maaß, Kezia Lange, Hanlim Lee, and Junsung Park

Recent works on using Machine Learning methods for deriving estimates of the NO2 concentration at the Earth's surface from satellite observations exploit measurements taken from low Earth orbits, e.g. from the TROPOMI instrument on the Copernicus Sentinel-5P satellite. However, given geographic location, the time resolution is quite low, with a single measurement per day, which leads to rather small data sets. In order to increase the performance of Machine Learning methods, large data sets would be desirable.

Launched in 2019, the Korean Geostationary Environmental Monitoring Spectrometer (GEMS) mission has been the first geostationary satellite mission for observing trace gas concentrations in the Earth's atmosphere over Asia. Geostationary orbits allows for hourly measurements, which leads to a much higher temporal resolution compared to measurements taken from low Earth orbits. Within the next years, two further geostationary missions will follow: NASA‘s TEMPO and ESA‘s Sentinel-4 mission, providing additional data with high temporal resolution over North America and Europe.

One of the GEMS level-2 data products is the NO2 tropospheric vertical column density (VCD). In our research project we discuss and develop Deep Learning methods that use not only these NO2 VCDs, but also additional data such as meteorological and geographical data, to derive estimates of the NO2 surface concentration in high spatial as well as high temporal resolution, enabled by the geostationary GEMS measurements mentioned above. The validation of the network‘s prediction is realized by the consideration of in-situ NO2 observations from the air quality network of South Korea.

How to cite: Gödeke, J., Hong, H., Richter, A., Maaß, P., Lange, K., Lee, H., and Park, J.: Developing Deep Learning Methods for Surface NO2 Estimation from GEMS Satellite Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9309, https://doi.org/10.5194/egusphere-egu23-9309, 2023.

EGU23-9634 | Orals | AS3.21

The diurnal variation of pollutant distributions over Asia using observations from the Geostationary Environment Monitoring Spectrometer (GEMS) 

David Edwards, Sara Martinez-Alonso, Duseong Jo, Ivan Ortega, Louisa Emmons, Helen Worden, and Jhoon Kim

Over the last 20 years, low-Earth orbit (LEO) atmospheric composition observations have provided amazing satellite measurements of atmospheric pollutants, mainly at continental-to-global, weekly-to-seasonal scales. The new-generation geostationary (GEO) satellite perspective, with high spatial resolution and hourly measurements, represents a major step forward in capability for understanding how air quality processes change diurnally at the local scale. South Korea's Geostationary Environment Monitoring Spectrometer (GEMS) was launched in February 2020 over Asia and is the first member of the GEO constellation that will eventually include the Tropospheric Emissions: Monitoring Pollution (TEMPO) mission over North America, and Sentinal-4 over Europe. The measurement hourly time resolution is truly the new perspective that the GEO platform provides, and in this presentation, we use a combination of satellite observations from GEMS and chemical transport model simulations to investigate the diurnal variation of pollution over several Asian regions. When considering the GEMS whole-Asia field-of-regard, the most striking impression of the NO2 diurnal variation is of how large it is in magnitude as well as how much the spatial distribution changes hour-by-hour. This questions our understanding of the distributions of reactive species based on the representativeness of once-a-day LEO observations. To help understand daily differences in diurnal patterns at regional and local scales, we use the Multi-Scale Infrastructure for Chemistry and Aerosols (MUSICA-V0). This uses a global modeling framework with regional grid refinement to resolve chemistry at emission and exposure relevant scales. The model shows reasonable agreement with the GEMS data and captures the different diurnal patterns at the different spatial scales and the degree of day-to day variability. The model also allows the drivers of variability due to emissions, meteorology, and photochemistry to be considered separately. The results of this analysis are further compared with the NO2 diurnal variability observed by PANDORA sun spectrometer measurements at polluted and less-polluted Korean and other Asian sites. We investigate spatial scale, including the city-scale within Seoul, at which GEMS captures the differences in diurnal variability between the PANDORAs.

How to cite: Edwards, D., Martinez-Alonso, S., Jo, D., Ortega, I., Emmons, L., Worden, H., and Kim, J.: The diurnal variation of pollutant distributions over Asia using observations from the Geostationary Environment Monitoring Spectrometer (GEMS), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9634, https://doi.org/10.5194/egusphere-egu23-9634, 2023.

EGU23-9659 | Orals | AS3.21

Emissions from Mining-related Activities in Africa using TROPOMI Satellite Observations 

Sara Martínez-Alonso, Pepijn Veefkind, Barbara Dix, Benjamin Gaubert, Claire Granier, Antonin Soulié, Sabine Darras, Nicolas Theys, Louisa Emmons, Henk Eskes, Wenfu Tang, Helen Worden, Joost deGouw, and Pieternel Levelt

We have analyzed TROPOMI NO2 data over the Copperbelt, a mining region which straddles the Democratic Republic of Congo and Zambia. While the ore mined there is primarily copper, this region is currently of great strategic interest because it is the world’s biggest producer of cobalt. Demand for cobalt, key to clean energy technologies (e.g., electric car batteries), is increasing worldwide and cobalt control is becoming a matter of national and global energy security. The impact of increasing mining-related activities on local air quality (high NOx is harmful to respiratory systems and crops) is unknown.

TROPOMI, onboard ESA’s Sentinel-5 Precursor, is an imaging spectrometer in a sun-synchronous orbit at 824 km of altitude which measures concentrations of relevant atmospheric species (trace gases, aerosols, cloud) with quasi-global daily coverage and at high spatial resolution (~ 3.5 x 5.5 km2 in the case of NO2).

We show that mining-related activities (such as extraction, smelting, and refining) can be remotely detected based on their TROPOMI NO2 signature, even in the presence of high background NO2 from biomass burning. Annual TROPOMI NO2 means for 2019, 2020, and 2021 show local enrichments consistent with point sources spatially collocated with both mines and large cities where mining-related activities take place. We have identified temporal trends in NO2 from these point sources and, when possible, we have compared those to production figures from the mining companies involved. We have quantified top-down annual NOx (NO+NO2) emissions for each of the point sources identified by applying the divergence method to the TROPOMI retrievals, using ancillary ERA5 meteorological data. Because in situ NOx measurements are not available, we contrast our emission results with emissions from the CAMS-GLOB-ANT v5.1 inventory.

Our results show that NOx emissions from mining-related activities can be quantified remotely, which is important in the absence of local air quality monitoring. They also demonstrate that NO2 trend analysis can be a good indicator of mine production. This is particularly relevant for non-publicly traded mining companies, which are not required to publish their production figures. Lack of TROPOMI SO2 enhancements colocated with our NO2 point sources is consistent with SO2 capture and transformation into H2SO4, which is then used in mining-related processes or commercialized.

How to cite: Martínez-Alonso, S., Veefkind, P., Dix, B., Gaubert, B., Granier, C., Soulié, A., Darras, S., Theys, N., Emmons, L., Eskes, H., Tang, W., Worden, H., deGouw, J., and Levelt, P.: Emissions from Mining-related Activities in Africa using TROPOMI Satellite Observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9659, https://doi.org/10.5194/egusphere-egu23-9659, 2023.

EGU23-9674 | ECS | Posters on site | AS3.21

Inferring near-surface NO2 concentrations for Belgium using multiple machine learning models and TROPOMI data 

Wenfu Sun, Frederik Tack, Lieven Clarisse, Rochelle Schneider, and Michel Van Roozendael

Near-surface nitrogen dioxide (NO2) is of great concern due to its impact on air quality and human health. Inferring the high-resolution spatiotemporal distribution of surface NO2 is necessary to assess the NO2 effects on human society and the ecosystem. Machine learning (ML) is an efficient approach to establishing a data-driven nonlinear mapping between targets and predictors. Various ML models have been used in past studies to estimate ground NO2 distributions from satellite observations (e.g., TROPOMI and OMI) and ancillary predictors (e.g., meteorology, land cover, and anthropogenic emissions) with good resolution, efficiency, and accuracy. In spite of these successes, the application of ML to infer near-surface NO2 remains challenging due to model stability issues and missing uncertainty estimations. In this research, we compare different ML models with respect to their predictive accuracy and spatiotemporal patterns. Moreover, we analyze the impact of the satellite remote sensing dataset and different predictors on model predictions using ML interpretation techniques. Based on these, we further investigate the possibility of assembling various ML models to provide a reliable ground NO2 estimation with uncertainty assessments. Overall, this study explores how ML models can be used to produce surface NO2 products, offering a perspective on practical applications for ML methods in atmospheric science.

How to cite: Sun, W., Tack, F., Clarisse, L., Schneider, R., and Van Roozendael, M.: Inferring near-surface NO2 concentrations for Belgium using multiple machine learning models and TROPOMI data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9674, https://doi.org/10.5194/egusphere-egu23-9674, 2023.

EGU23-9720 | Posters on site | AS3.21

An Overview of TROPESS Data Products and Services at the NASA GES DISC 

James Johnson, Lena Iredell, Irina Gerasimov, Kristan Morgan, and Jennifer Wei

The TRopospheric Ozone and Precursors from Earth System Sounding (TROPESS) project generates Earth System Data Records (ESDRs) of ozone, and other atmospheric constituents (CH4, CO, H2O, HDO, NH3, PAN and temperature) by processing data from multiple satellites through a common retrieval algorithm and ground data system. Satellite Level-1B input data used in generating the TROPESS L2 data products include CrIS NOAA-20 (JPSS-1), CrIS SNPP, AIRS Aqua, OMI Aura, and TROPOMI S5P. The common retrieval framework is known as the MUlti-SpEctra, MUlti-SpEcies, Multi-SEnsors (MUSES) science data processing system (MUSES-SDPS). Several of the TROPESS data products are now available from the NASA Godddard Earth Sciences Data and Information Service Center (GES DISC) for users to download.

In this presentation we provide an overview of the various TROPESS data products. These data products can be divided into the following Forward Stream types: Standard Products, Summary Products, and Full-Archival Products.  Standard Products are for users that are doing full analysis with avenging kernel and covariance corresponding to retrieved vertical profiles. Summary products have a smaller file size and are more convenient for first-look and rapid analysis, include total and partial columns, as well as column averaging kernels. The Full-Archival Products will contain all information used in creating the data. TROPESS also creates Special Products, provided on an as-needed and as-available basis to support NASA field missions and individual-investigator requests over specific regions. Eventually, TROPESS will also produce and deliver a set of Reanalysis Stream products.

Data at the GES DISC are being transitioned into the "Cloud". This will allow users with "Cloud" access to perform data analysis directly on the data without downloading the data to their system. Services, such as subsetting and data visualization, will also be provided for TROPESS data products at the GES DISC.

How to cite: Johnson, J., Iredell, L., Gerasimov, I., Morgan, K., and Wei, J.: An Overview of TROPESS Data Products and Services at the NASA GES DISC, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9720, https://doi.org/10.5194/egusphere-egu23-9720, 2023.

EGU23-9967 | Posters on site | AS3.21

Aerosol effective height retrieval using O4 absorption property based on GEMS measurements 

Wonei Choi, Hanlim Lee, Seung Hee Kim, and Menas Kafatos

In this study, we developed an aerosol effective height (AEH) retrieval algorithm based on O4 absorption properties at 477 nm from the hyperspectral measurements of the Geostationary Environment Monitoring Spectrometer (GEMS). The GEMS, successfully launched in February 2020 onboard Geostationary Korea Multi-Purpose SATellite (GeoKOMPSAT-2B), is currently monitoring the air quality (O3, NO2, SO2, HCHO, and aerosol) over Asia. In the AEH retrieval algorithm, an O4 slant column density (SCD) is retrieved using the differential optical absorption spectroscopy (DOAS) technique, then the O4 air mass factor (AMF) is derived by dividing O4 SCD by O4 vertical column density (VCD) to account for the variation of O4 VCD associated with changes in atmospheric temperature and pressure. A spatiotemporal variation of O4 VCD and its effect on AEH retrieval accuracy was investigated. In addition, a temperature-dependent cross-section for O4 (TDCS) was applied to the O4 AMF calculation. The AEHs were retrieved from hyperspectral radiance from the GEMS measurements for the Asian dust period in 2021. Additionally, we tried to compare the retrieved GEMS AEH with lidar measurement data to validate the performance of our retrieval.

How to cite: Choi, W., Lee, H., Kim, S. H., and Kafatos, M.: Aerosol effective height retrieval using O4 absorption property based on GEMS measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9967, https://doi.org/10.5194/egusphere-egu23-9967, 2023.

EGU23-10309 | Posters on site | AS3.21

Neighborhood-scale NO2 variations and enhanced capability of human exposure assessment 

Hyung Joo Lee, Yang Liu, and Robert Chatfield

This study estimated ambient long-term average NO2 concentrations using TROPOspheric Monitoring Instrument (TROPOMI) tropospheric column NO2 data and land use parameters in California, U.S. for the years 2018–2019. Exploiting unprecedentedly high spatial resolution of TROPOMI NO2 (3.5×7 km prior to August 6, 2019 and 3.5×5.5 km thereafter) and the point statistics function implemented in ArcGIS (Environmental Systems Research Institute, ESRI), the NO2 concentration estimates were downscaled to 500 m, which enabled the neighborhood-scale exposure assessment of ambient NO2. Our satellite-land use hybrid regression model demonstrated cross-validation R2= 0.76, mean absolute error (MAE)= 1.95 ppb, and root mean squared error (RMSE)= 2.51 ppb in a comparison between site-specific average measured and estimated NO2 concentrations. These high-resolution NO2 concentration estimates enhanced the capability of human exposure assessment, enabling (1) the evaluation of ground NO2 monitors to represent population exposures and (2) the attribution of micro-level NO2 exposures. When measured NO2 concentrations were compared to population-weighted NO2 concentrations, calculated by using the satellite-based NO2 estimates, in each county, the differences in NO2 concentrations (i.e., population-weighted average NO2 – arithmetic average NO2 measurements) ranged from -38.6% (San Bernardino) to 82.2% (Humboldt). Though both negative and positive differences represented exposure errors without considering the spatial co-variations of NO2 and populations, monitor-based NO2 higher than the population-weighted NO2 demonstrated the overestimation of population NO2 exposures and was at least protective with current NO2 monitoring locations in the counties. However, the opposite was detrimental, while underestimating population NO2 exposures and likely not motivating NO2 mitigation efforts. In addition, the high-resolution NO2 estimates were further overlaid with parcel-level property data in Los Angeles County to attribute the spatial variation of NO2 exposures to that of the property types. The micro-level NO2 hotspots were identified at high-density residential complexes such as (high-rise) apartments. When the traffic impacts on NO2 were adjusted, the NO2 hotspots at the residential complexes still remained. This finding may suggest residential complexes as an emerging source type of NO2 due to emissions from boilers (space heating and hot water) and other indoor-to-outdoor ventilation systems.

How to cite: Lee, H. J., Liu, Y., and Chatfield, R.: Neighborhood-scale NO2 variations and enhanced capability of human exposure assessment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10309, https://doi.org/10.5194/egusphere-egu23-10309, 2023.

EGU23-10465 | Orals | AS3.21

Investigating Freeze/Thaw soil emissions of nitric oxide using in situ and Tropomi observations 

Jonathan Hickman, Enrico Dammers, Sally Pusede, Madeline Miles, Andy Suyker, Tala Awada, Jude Maul, and Peter Groffman

Agricultural emissions of nitric oxide (NO) from soils can cause formation of tropospheric ozone and particulate matter pollution, and in the presence of ozone NO is rapidly transformed nitrogen dioxide (NO2), itself an air pollutant. Emissions of NO from soils can be highly episodic, with a large proportion of annual emissions occurring in pulses following fertilization or wetting of dry soils. Freeze-thaw events may also be an important source of NO pulses, but the magnitude of these emissions is poorly understood, as are the mechanisms underlying freeze-thaw NO pulses and their influence on atmospheric composition and air quality.  Here we use daily observations of NO2 and air temperature for 2018-2021 from atmospheric monitoring stations in the Corn Belt of the midwestern United States to evaluate the potential influence of freeze/thaw events on atmospheric NOx.  We supplement these data with retrievals of NO2 from the Tropospheric Pollution Monitoring Instrument (TROPOMI) screened to include acceptable retrievals over snow, retrievals of soil freeze/thaw status from the Soil Moisture Active Passive project (SMAP), and observed and reanalyzed soil temperature.  We find evidence for elevated NO2 concentrations during winter months, including instances of elevated concentrations at the onset of spring thaw.  Freezing degree days—the accumulation of average daily temperature for days with soil temperature maxima of 0°C or less—fail to act as a clear predictor of the magnitude of post-thaw concentrations.  These results will be integrated with complementary high temporal-resolution eddy covariance flux measurements at a long-term agricultural research station in Nebraska, along with soil core incubations involving biogeochemical and molecular analyses, to provide insights into the magnitude of freeze/thaw fluxes and their underlying mechanisms.

How to cite: Hickman, J., Dammers, E., Pusede, S., Miles, M., Suyker, A., Awada, T., Maul, J., and Groffman, P.: Investigating Freeze/Thaw soil emissions of nitric oxide using in situ and Tropomi observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10465, https://doi.org/10.5194/egusphere-egu23-10465, 2023.

EGU23-10841 | Orals | AS3.21 | Highlight

The hourly volcanic SO2 column density and physical characteristics using Geostationary Environment Monitoring Spectrometer (GEMS) measurements 

Jeonghyeon Park, Hanlim Lee, Jiwon Yang, Hyunkee Hong, Jhoon Kim, Michel Van Roozendael, Nicolas Theys, Can Li, Myong-Hwan Ahn, Dong-won Lee, Junsung Park, Wonei Choi, Rokjin Park, and Daewon Kim

The Geostationary Environment Monitoring Spectrometer (GEMS) onboard the Geostationary Korea Multi-Purpose Satellite-2B (GEO-KOMPSAT-2B) satellite observes the hourly volcanic SO2 over Asia. In this study, the various physical characteristics of volcanic plumes have been investigated based on hourly volcanic SO2 measurements. The transport direction, path and speed, and altitude of volcanic SO2 plume emitted from Nishinoshima in Japan, Etna in Italy, and Dukono located in Halmahera, Indonesia were calculated. The SO2 plume from Nishinoshima, Japan, moved westward at a maximum speed of 57 km/h on August 4, 2020. The SO2 plume generated from Etna was observed to move over China using both GEMS and TROPOMI, and moved at an altitude of 11–14 km and a speed of 162–190 km/h. In the case of the SO2 plume from the Dukono volcano flowed into an average of 3.6 Mg of SO2 per hour to the cities of nearby islands. GEMS can be utilized for an improvement in the prediction accuracy of SO2 plume transport using a chemical transport model due to the availability of hourly volcanic SO2 height information. In addition, hourly observations of SO2 concentrations are expected to protect SO2 exposure through rapid forecasting for people in cities around the volcano.

How to cite: Park, J., Lee, H., Yang, J., Hong, H., Kim, J., Roozendael, M. V., Theys, N., Li, C., Ahn, M.-H., Lee, D., Park, J., Choi, W., Park, R., and Kim, D.: The hourly volcanic SO2 column density and physical characteristics using Geostationary Environment Monitoring Spectrometer (GEMS) measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10841, https://doi.org/10.5194/egusphere-egu23-10841, 2023.

The past two decades have been the golden age of tropospheric composition sounding with instruments like the Tropospheric Emission Spectrometer (TES), the Infrared Atmospheric Sounding Interferometer (IASI), SCanning Imaging Absorption spectroMeter for Atmospheric CHartographY (SCIAMACHY),  the Ozone Mapping Interferometer (OMI) harnessing spectral radiation from the thermal infrared to the ultraviolet to pioneer new products such as tropospheric ozone, ammonia, methane, nitrogen dioxide, and water vapor deuterium.  As a new generation of sounders that include both geostationary and low earth orbiting satellites become the anchor of a global air quality monitoring system, there is an urgent need to shift away from an instrument focus, which is a confined to a  band of frequencies,  to a measurement focus, which incorporates the best available information.  The TROPESS project is a new measurement focused approach that uses a common retrieval algorithm applied to a suite of instruments either singularly or in combination.  Building on the heritage of TES, we show how the MUlti-SpEctra, MUlti-SpEcies, Multi-SEnsors (MUSES) algorithm has been applied to produce ozone from TES, AIRS, and OMI as well as its potential to combine CrIS and TROPOMI radiances.  Employing proven optimal estimation techniques, we further show how data produced from MUSES can be ingested into chemical data assimilation providing a comprehensive understanding of global atmospheric chemistry and its evolution.  The suite of products and their scientific impact on atmospheric composition are surveyed.  TROPESS points to a new paradigm that can effectively harness a constellation of data to quantify the rapid changes in the landscape of emissions and their impact on air quality and climate. 

How to cite: Bowman, K.: Towards the next generation of tropospheric composition sounding: the NASA TRopospheric Ozone and its Precursors from Earth System Sounding (TROPESS), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10973, https://doi.org/10.5194/egusphere-egu23-10973, 2023.

EGU23-11298 | Posters on site | AS3.21

Development of a long-term SO2 column data record from satellite nadir UV sensors 

Nicolas Theys, Can Li, Isabelle De Smedt, Christophe Lerot, Huan Yu, Jonas Vlietinck, Pascal Hedelt, Nickolay Krotkov, and Michel Van Roozendael

As part of its Climate Change Initiative extension program (CCI+), the European Space Agency started a new activity aiming to develop space-based long-term climate data records for precursors gases involved in the formation of aerosols and ozone (https://climate.esa.int/en/projects/precursors-for-aerosols-and-ozone/about/). The targeted trace gases are NO2, SO2, HCHO, CHOCHO, CO and NH3.

For SO2 in particular the project relies on recent developments for Sentinel-5 Precursor/TROPOMI based the Covariance-Based Retrieval Algorithm (COBRA). This algorithm will be used to build consistent column retrievals from a series of four satellite sensors (GOME, SCIAMACHY, OMI and TROPOMI), covering nearly three decades of observations.

Here, we give an overview of the SO2 development activities in the Precursors CCI+ project. To achieve the project objectives, an extensive comparison of results is performed in the form of a round Robin exercise. This includes comparison of different algorithms, but also testing of various processing options for ancillary data such as cloud and surface reflectance parameters. First results from the round Robin exercise are presented with a focus on OMI, in particular the comparison between COBRA and Principal Component Analysis (PCA) column retrievals. Preliminary results using COBRA for the historical sensors GOME and SCIAMACHY are also shown.

 

How to cite: Theys, N., Li, C., De Smedt, I., Lerot, C., Yu, H., Vlietinck, J., Hedelt, P., Krotkov, N., and Van Roozendael, M.: Development of a long-term SO2 column data record from satellite nadir UV sensors, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11298, https://doi.org/10.5194/egusphere-egu23-11298, 2023.

EGU23-11408 | Posters on site | AS3.21

First results from the ESA Precursors for aerosols and ozone ECVs project: user requirements and intercomparison of tropospheric retrievals of NO2, HCHO, SO2, CO, NH3, and glyoxal 

K. Folkert Boersma, Michel Van Roozendael, and Andreas Richter and the the ESA Precursors for aerosols and ozone ECVs project team

Satellite-based observations of tropospheric trace gas concentrations are used extensively to test models, infer emissions and their trends. These observations are also needed to develop emission-based scenarios for radiative forcing by tropospheric ozone and secondary aerosols, both from anthropogenic and natural sources. Although the detection of trace gases from space is feasible and operational data streams are in place for most relevant sensors, limited effort has been devoted to the generation and quality assessment of consistent multi-decadal climate data records. The ESA Climate Change Initiative (CCI) program was established for the systematic generation of Essential Climate Variables (ECVs). It builds on long-term global satellite observational datasets. Regarding atmospheric composition, the ECVs covered have recently been extended with trace gases that lead to the formation of ozone and aerosols.

Here we present first results from the ‘Precursors for aerosols and ozone ECVs’ project, funded by ESA, and the first steps in developing long-term climate data records on the precursor gases nitrogen dioxide (NO2), formaldehyde (HCHO), carbon monoxide (CO), sulfur dioxide (SO2), ammonia (NH3), and glyoxal (CHOCHO). The project’s main goal is to build consistent and harmonized long-term data records from satellite instruments including GOME, SCIAMACHY, GOME-2, OMI, TROPOMI, IASI and MOPITT. A second goal is to demonstrate the fitness-for-purpose of the data records for various users including the European Copernicus Atmosphere Monitoring Service, currently operated by ECMWF. In this presentation, we report on what users need from such data records, and on round robin activities to test and evaluate the different retrieval approaches used in the scientific community. One key motivation will be to reconcile retrieval approaches so far independently developed in the EU QA4ECV and EUMETSAT AC-SAF projects, with the aim to harmonize products from all sensors.

How to cite: Boersma, K. F., Van Roozendael, M., and Richter, A. and the the ESA Precursors for aerosols and ozone ECVs project team: First results from the ESA Precursors for aerosols and ozone ECVs project: user requirements and intercomparison of tropospheric retrievals of NO2, HCHO, SO2, CO, NH3, and glyoxal, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11408, https://doi.org/10.5194/egusphere-egu23-11408, 2023.

EGU23-11428 | Posters on site | AS3.21

A high spatial and temporal coverage global gridded tropospheric NO2 dataset (2007-2021) based on OMI and GOME-2 

kai qin, Xuanchen Liu, Qin He, and Jason Cohen

NOx interacts with both air pollution and short lived climate forcers, including ozone, nitrate aerosol, CO, and VOCs, which in turn cause damage to the atmosphere, degrade the environment and threaten human health. Based on the DOAS algorithm, satellite measurements can provide decadal and long-term and grid-by-grid coverage over the entire globe for NO2 and a few other trace gasses. This work merges two different satellites using NO2 retrieved by DOAS. The overpass times, wavebands used for the retrieval, and the uncertainties of the sensors are different. We take advantage of this variability to produce a merged product which relies on the local strengths of each sensor. Applying machine learning and the DINEOF method, this work generates a 15-year dataset with more overall data, fewer cloud-covered pixels, and data which is of higher quality and lower error. The spatial coverage of the reconstructed dataset is improved by 60% compared with the original datasets. A few specific and scientifically important results of this are explained in detail including: first, higher data coverage and quality over mountain basin regions which are even more clear than using the TROPOMI product, and second higher precision as compared with surface based remotely sensed profiles in highly polluted regions.

 

 

How to cite: qin, K., Liu, X., He, Q., and Cohen, J.: A high spatial and temporal coverage global gridded tropospheric NO2 dataset (2007-2021) based on OMI and GOME-2, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11428, https://doi.org/10.5194/egusphere-egu23-11428, 2023.

EGU23-12034 | Posters on site | AS3.21

Improving SO2 emissions over the Middle East. 

Alexander Ukhov and Georgiy Stenchikov

The Middle East is one of the most polluted regions on Earth. Besides strong natural air pollution caused by frequent dust storms, anthropogenic emissions of SO2 from power and desalination plants significantly deteriorate air quality and, as a consequence, reduce life expectancy. Additionally, sulfate aerosol formed through the chemical oxidation of SO2 has an effect on climate and cloud formation. Therefore, accurate modeling of SO2 emissions is crucial, especially in such harsh conditions as the Middle East.

In this work, we attempt to improve existing SO2 emissions using inversion modeling, a high-resolution regional WRF-Chem model, and satellite observations of SO2 columns available from OMI and TOMS instruments. Obtained SO2 emission dataset is planned to be open to the community.

How to cite: Ukhov, A. and Stenchikov, G.: Improving SO2 emissions over the Middle East., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12034, https://doi.org/10.5194/egusphere-egu23-12034, 2023.

EGU23-12135 | Orals | AS3.21

Monitoring Belgian air quality with LEO and GEO atmospheric composition data 

Tijl Verhoelst, Steven Compernolle, Jean-Christopher Lambert, Frans Fierens, and Charlotte Vanpoucke

Air Quality (AQ) monitoring in Belgium has hitherto been relying mostly on in-situ measurements of surface concentration, with geographical gaps between observations filled in with numerical modelling ingesting (proxies for) bottom-up emission estimates.   However, a new generation of satellite sounders on sun-synchronous Low Earth Orbits (LEO) – like the Copernicus Sentinel-5(p) series – performs now daily global mapping of atmospheric composition down to the 3-km scale. Soon this daily global mapping will be complemented with geostationary instruments (GEO, e.g. Sentinel-4) observing the diurnal cycle in trace gas concentrations, although over the limited geographical area accessible from a geostationary viewpoint. This new constellation of satellite sounders is built to support detailed monitoring of AQ on the different relevant scales: from point-like emissions to intercontinental transport, and from city-level to international regulations established by public authorities to manage AQ in their area of responsibility. Nevertheless, uptake of these new satellite AQ data by the various Belgian stakeholders is not guaranteed.  Indeed, to realize the full complementary impact of this constellation of LEO and GEO satellites, i.e. to make their observations fit-for-purpose for air quality applications at the different scales, several challenges need to be addressed. These include (1) the need to enhance to sub-city scales the resolution of satellite data to make them better suited for the monitoring of e.g. the impact of the Low Emission Zones enforced in several European cities, (2) to characterize the non-trivial relation between the column amount of the pollutant measured by a satellite and the near-surface concentrations measured by in-situ networks, and (3) to determine how the different LEO and GEO vantage points lead to a different perception of atmospheric and surface details and how we can benefit from - or correct for - these differences.

Work on these challenges is taking place in the dedicated Belgian federal research project LEGO-BEL-AQ (2020-2023, https://lego-bel-aq.aeronomie.be/index.php) funded by BELSPO, with a particular focus on AQ in Belgium.  In this contribution, we demonstrate that a combination of temporal aggregation, careful data selection, and horizontal oversampling can produce a meaningful increase in horizontal resolution in S5P tropospheric NO2 column maps, revealing policy-relevant features in the NO2 distribution over Belgium’s major cities. Comparisons between our high-resolution S5P NO2 maps and the near-surface in-situ observations as procured by the Belgian authorities, reveal high correlation when considering longer time scales (seasonal and annual), allowing a pragmatic conversion from tropospheric columns to near-surface concentrations over the complete Belgian domain, and consequently also a confrontation to WHO annual thresholds at the level of individual Belgian municipalities.

Acknowledgements

This work has been supported by the BELSPO BRAIN-be 2.0 project LEGO-BEL-AQ (https://lego-bel-aq.aeronomie.be)

How to cite: Verhoelst, T., Compernolle, S., Lambert, J.-C., Fierens, F., and Vanpoucke, C.: Monitoring Belgian air quality with LEO and GEO atmospheric composition data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12135, https://doi.org/10.5194/egusphere-egu23-12135, 2023.

EGU23-12195 | Orals | AS3.21

SO2 emission estimates using satellite observations from TROPOMI and OMI and the global chemistry transport model LMDz-INCA 

Pramod Kumar, Philippe Ciais, Santanu Halder, Gregoire Broquet, Didier Hauglustaine, and Nicolas Theys

Sulfur dioxide (SO2) is released into the Earth’s atmosphere through natural and anthropogenic processes and the latter category amounts to the majority of the global SO2 emissions. Satellite SO2 observations have been used to monitor SO2 emissions at different regional and global scales and to detect large-point sources of SO2 emissions of diverse origins. In this study, we conducted atmospheric inversions at the global scale to estimate daily SO2 emissions at 1.26o×2.5o (latitude×longitude) spatial resolution over polluted regions for two years 2020 and 2021 using satellite SO2 total vertical column densities (TVCDs) obtained by the Sentinel 5p TROPOspheric Monitoring Instrument (TROPOMI) and AURA Ozone Monitoring Instrument (OMI). We used the global chemistry coupled transport model LMDz-INCA with 1.26o×2.5o (latitude×longitude) horizontal resolution and 79 hybrid σ-p vertical levels extending to the stratosphere to simulate the model SO2 TVCDs. The model uses a priori monthly global anthropogenic emission inventories from the open-source Community Emissions Data System (CDES). As the TROPOMI operational offline L2 SO2 data product has high noise levels, we used the TROPOMI COBRA SO2 data product in this study which has comparatively smaller noise. First, we evaluated the SO2 TVCDs from the LMDz-INCA model simulations for a reference year 2019 with the observed SO2 TVCDs from TROPOMI and OMI. The daily average (10-day running average) of the model simulated SO2 TVCDs over the major polluted regions like India, China, and the Middle East, and over less polluted regions like South Africa, and South America mostly follow the trend of the observed SO2 TVCDs from both TROPOMI and OMI. The model overestimates SO2 TVCDs over India and the Middle East and underestimates them over China, South Africa, and South America. For Europe and North America, the noise levels in the daily averaged TVCDs from both TROPOMI and OMI are too high for a meaningful comparison. In order to estimate anthropogenic SO2 emissions, we used a recently developed inversion approach (Zheng et al., 2020), which was previously used to estimate anthropogenic NOx emissions over China. We performed the model simulation for 2019 with 40% reduced anthropogenic SO2 emission to calculate the gridded local sensitivities of the TVCDs to the change in the anthropogenic SO2 emissions. The inversion approach combines these gridded local sensitivities and the relative change of the observed satellites and the modelled TVCDs to derive the relative change of anthropogenic SO2 emissions from the reference year 2019 to the inversion years 2020 and 2021. The estimated total SO2 emissions from TROPOMI and OMI observations for 2020 and 2021 are mostly higher compared to the reference year total emissions over the world and over the selected regions. The total SO2 emissions from TROPOMI and OMI observations at the common model grids for both inversion years are consistent with each other.

How to cite: Kumar, P., Ciais, P., Halder, S., Broquet, G., Hauglustaine, D., and Theys, N.: SO2 emission estimates using satellite observations from TROPOMI and OMI and the global chemistry transport model LMDz-INCA, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12195, https://doi.org/10.5194/egusphere-egu23-12195, 2023.

EGU23-12287 | Posters on site | AS3.21

Decreasing trends of NH3 over Europe seen from space 

Nikolaos Evangeliou, Ondrej Tichy, Sabine Eckhardt, Yves Balkanski, and Didier Hauglustaine

Ammonia (NH3), the only basic gas in the atmosphere, constitutes one of the most reactive nitrogen species. It mainly originates from agricultural-related activities, with emissions contributing over 80% globally, while locally they can reach as high as 94%. Once it is emitted, it is transported and deposited to water bodies, soil or vegetation and can then lead to eutrophication of water bodies, modulate soil pH and burn vegetation. It also reacts in the atmosphere with the abundant sulfuric and nitric acids forming fine particulate matter (PM2.5), which affect Earth’s radiative balance, causes visibility problems, but also affects human health, as it penetrates the human respiratory system. However, despite its significance, ammonia source emissions are poorly constrained due to lack of ground-based measurement. Today, several satellite products have become available mainly from satellite sounders.

In the present study, we use direct comparisons between the CrIS (Cross-track Infrared Sounder ) observations and model retrievals using the Least Squares with Adaptive Prior Covariance (LS-APC) algorithm, which reduces the number of tuning parameters in the method significantly using variational Bayes approximation technique. We constrain ammonia emissions over Europe over 2013–2020 and validate the results against ground-based observations from the EMEP (European Monitoring and Evaluation Programme). We find that emissions of ammonia decreased from 5431 Gg in 2013 to 3994 Gg in 2020 (-26%). Regionally, emissions declined by 38% in Central and Eastern Europe, 37% in Western Europe, 8% in Southern Europe and -17% in Northern Europe.

How to cite: Evangeliou, N., Tichy, O., Eckhardt, S., Balkanski, Y., and Hauglustaine, D.: Decreasing trends of NH3 over Europe seen from space, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12287, https://doi.org/10.5194/egusphere-egu23-12287, 2023.

EGU23-12469 | Orals | AS3.21

15 years of pyrogenic HONO plumes observed with IASI 

Bruno Franco, Lieven Clarisse, Nicolas Theys, Juliette Hadji-Lazaro, Cathy Clerbaux, and Pierre Coheur

Nitrous acid (HONO) plays a key role in atmospheric chemistry as a major source – through rapid photolysis – of the hydroxyl radical (OH), the primary oxidant in the Earth's atmosphere. However, significant uncertainties remain on the spatial and temporal variability of HONO, on its formation pathways in the atmosphere, and on the contribution of its primary emissions over its secondary formation. Recently, spaceborne measurements in the UV-Vis spectral domain, taken in the early afternoon with the S5P/TROPOMI instrument, have provided a first global picture of HONO in fresh biomass burning plumes, demonstrating the importance of satellite data for improving our representation of atmospheric HONO. With daily overpass times in the early morning and early evening, the polar-orbiting IASI/Metop instruments and their global measurements of the Earth's radiance in the thermal infrared, have the potential to contribute to tackling remaining uncertainties on HONO and to complement the TROPOMI measurements.

So far detected by infrared satellite sounders in the exceptional 2009 and 2019/2020 Australian bushfires only, we use a sensitive detection method to demonstrate that unambiguous HONO enhancements can also be identified in IASI spectra recorded in concentrated fire plumes worldwide. With this method, we analyse the long, unique observational timeseries (2007-2022) of IASI and we report a 15-year record of fire events in which HONO has been detected. This dataset reveals first that HONO is primarily captured by IASI at the Northern Hemisphere mid and high latitudes, and secondly that the IASI evening measurements allow a significantly higher number of HONO detections than during daytime despite the overall weaker thermal contrast and lower measurement sensitivity affecting such night-time observations. We discuss different factors that can explain these features, such as the sharp intra-day variability of HONO, the links with the diurnal variations and intensity of fires, and the vertical sensitivity of the IASI measurements. We apply a retrieval approach based on an artificial neural network to quantify the vertical abundance of HONO in IASI measurements. For selected fires, we analyse the temporal evolution of the HONO total columns along with TROPOMI data. 

How to cite: Franco, B., Clarisse, L., Theys, N., Hadji-Lazaro, J., Clerbaux, C., and Coheur, P.: 15 years of pyrogenic HONO plumes observed with IASI, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12469, https://doi.org/10.5194/egusphere-egu23-12469, 2023.

EGU23-12496 | Orals | AS3.21

Enhanced situational awareness in Finland using atmospheric (and other) space-based observations 

Iolanda Ialongo, Henrik Virta, Janne Hakkarainen, Monika Szelag, Anu-Maija Sundström, and Johanna Tamminen

New remote sensing satellites for Earth Observation provide information to enhance situational awareness during exceptional socio-economic and natural events. Specifically, satellite-based observations of air pollutants, when combined with auxiliary (spaceborne and not) data, can provide new insights on societal and economic changes taking place around the world. Here we present a few applications of space-based atmospheric observations to support Finnish authorities. A recent history of such episodes includes: monitoring air quality changes in Helsinki during the COVID-19 pandemic; assessing methane emissions from the NordStream pipeline leakage over the Baltic Sea; assessing the environmental and social effects of the war in Ukraine as part of Finnish international cooperation projects. We integrate multiple data sources acquired by different spaceborne sensors including, e.g., the nitrogen dioxide (NO2) retrievals from the Copernicus Sentinel-5 Precursor/TROPOMI (TROPOspheric Monitoring Instrument), Sentinel-2 false color imagery, NASA VIIRS fire products as well as models and other environmental data.

How to cite: Ialongo, I., Virta, H., Hakkarainen, J., Szelag, M., Sundström, A.-M., and Tamminen, J.: Enhanced situational awareness in Finland using atmospheric (and other) space-based observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12496, https://doi.org/10.5194/egusphere-egu23-12496, 2023.

EGU23-12993 | ECS | Posters on site | AS3.21

Aerosol Optical Depth Retrieval by Machine Learning Methods from Geostationary Environmental Monitoring Spectrometer 

Audrieauna Beatty, Hyunyoung Choi, Miae Kim, and Jungho Im

Globally, aerosols, emissions, and greenhouse gases have an impact on the environment. With the help of satellite data and field instruments we can understand and continue to study the atmosphere. Specifically, in terms of understanding air quality and aerosol optical depth (AOD), the radiative transfer model is traditionally used but can have unpredictability and is time consuming. With use of machine learning, one can improve accuracy and can be more time efficient. In this paper, we present machine learning methods to estimate AOD from the Geostationary Environmental Monitoring Spectrometer (GEMS). GEMS has a hyperspectral scanning spectrometer that monitors air pollutants over Asia by different observation nodes. Random Forest (RF), and Light Gradient Boosting Machine (LGBM) with auxiliary. meteorological, and ground-based observation data were used to estimate hourly AOD. Inclusion of meteorological data can support the model in performance and reflecting dynamic conditions in the atmosphere. The two machine learning models were evaluated by random, spatial, and temporal 10-fold cross validation to test the transferability and robustness. The results showed that random forest model performed lower than the light-gradient boosting model. LGBM produced R2 of 0.286 – 0.680 and RSME of 0.025-0.057. Random forest produced R2 of 0.283 – 0.643 and RSME of 0.028-0.057. Overall, the model was able to show that AOD can be retrieved from machine learning methods from the Geostationary Environmental Monitoring Spectrometer (GEMS).

How to cite: Beatty, A., Choi, H., Kim, M., and Im, J.: Aerosol Optical Depth Retrieval by Machine Learning Methods from Geostationary Environmental Monitoring Spectrometer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12993, https://doi.org/10.5194/egusphere-egu23-12993, 2023.

EGU23-13487 | ECS | Orals | AS3.21 | Highlight

NH3 emissions derived from CRIS observations over Europe 

Jieying Ding, Ronald van der A, Henk Eskes, Enrico Dammers, and Mark Shephard

Over the past century ammonia (NH3) emissions have increased with human population growth and fertilizer usage. The abundant NH3 emissions lead to climate change, reduction in biodiversity and affect the human health. Up-to-date information of NH3emissions are essential to better understand the impact of NH3. In this study we adapted the existing DECSO (Daily Emissions Constrained by Satellite Observations) algorithm for use of NH3 observations from the Cross-track Infrared Sounder (CrIS) to estimate NH3 emissions. By considering the interaction between NH3 and NOx, we implemented DECSO to estimate NOx and NH3 emissions simultaneously on 20 km resolution over European domain. NH3 and NOx emissions over Europe are derived for 2020 on a daily basis from CrIS and TROPOMI (on Sentinel 5p). Due to the sparseness of daily satellite observations of NH3, monthly emissions of NH3 are constructed and analysed.  The comparison of these emissions with other existing emission inventories will be presented.

How to cite: Ding, J., van der A, R., Eskes, H., Dammers, E., and Shephard, M.: NH3 emissions derived from CRIS observations over Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13487, https://doi.org/10.5194/egusphere-egu23-13487, 2023.

EGU23-13654 | ECS | Orals | AS3.21

Aircraft validation reveals a 20% low bias in TROPOMI NO2 over sea caused by TM5 a priori profiles 

T. Christoph V.W. Rieß, Jasper van Vliet, Ward Van Roy, Jos de Laat, Enrico Dammers, and Folkert Boersma

Scattering of light in the atmosphere and low sea surface albedo decrease the sensitivity of satellites to air pollution close to the sea surface. To reliably retrieve tropospheric nitrogen dioxide (NO2) columns using the TROPOspheric Monitoring Instrument (TROPOMI), it is therefore necessary to have good a priori knowledge of the vertical distribution of NO2. In this study, we used an aircraft of the Royal Belgian Institute of Natural Sciences, part of the Belgian coastguard structure, which was already equipped with a sniffer sensor system, measuring CO2, NOx and SO2. This instrumentation enables us (1) to capture pollution plumes originating from ships sailing within an Emission Control Area, and (2) to validate TROPOMI tropospheric NO2 columns over the polluted North Sea in summer 2021 and (3) to evaluate vertical profile shapes from several chemical models. We observe multiple clear signatures of ship plumes from seconds after emission to multiple kilometers downwind. Besides that, our results show that the chemical transport model TM5, which is used in the retrieval of the operational TROPOMI data, tends to underestimate surface level pollution while overestimating NO2 at higher levels over the polluted North Sea. The higher horizontal resolutions in the regional CAMS ensemble mean and LOTOS EUROS improve the surface level pollution estimates, but the models still systematically overestimate NO2 levels at higher altitudes, indicating exaggerated vertical mixing in the models. When replacing the TM5 a priori NO2 profiles with the aircraft-measured NO2 profiles in the air mass factor (AMFs) calculation, we find that recalculated AMFs reduce, and the retrieved NO2 columns increase by 20%. This indicates a significant low bias in TROPOMI tropospheric NO2 measurements over the North Sea. This low bias has important implications for estimating emissions over the sea. While TROPOMI NO2 low biases caused by the TM5 a priori profiles have previously also been reported over land, the reduced vertical mixing and smaller surface albedo over sea makes this issue especially relevant over sea and coastal regions. 

How to cite: Rieß, T. C. V. W., van Vliet, J., Van Roy, W., de Laat, J., Dammers, E., and Boersma, F.: Aircraft validation reveals a 20% low bias in TROPOMI NO2 over sea caused by TM5 a priori profiles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13654, https://doi.org/10.5194/egusphere-egu23-13654, 2023.

EGU23-13791 | ECS | Posters on site | AS3.21

Spatial and temporal variations of thermal contrast in the planetary boundary layer 

Tommaso Di Gioacchino, Lieven Clarisse, Martin Van Damme, and Pierre Coheur

Short-lived atmospheric pollutants mainly reside in the planetary boundary layer (PBL). In recent years, the sensitivity of high-resolution infrared sounders to the PBL has been amply demonstrated, most notably through observations of local emission sources of sulphur dioxide (SO2), carbon monoxide (CO) and ammonia (NH3). However, sensitivity of infrared sounders to the PBL varies strongly as a function of thermal contrast (TC), the temperature difference between the Earth’s skin temperature and the temperature of the atmosphere. Enhanced contrast, typically seen during daytime when the surface is typically (much) warmer than the air, provides favourable measurement conditions. At night, TC is smaller, and can even become negative, providing again favourable measurement conditions. More generally speaking, TC is highly variable in both time (inter and intraday) and space. Up to now, no study has provided insight in the global statistical behaviour of the TC or answered the question when and where thermal infrared sounders experience optimal measurement conditions.

Here we combine the Copernicus Global Land Services land surface temperature (LST) dataset, derived from geostationary satellite measurements, with air temperatures from the ERA5 reanalysis dataset to obtain a global TC dataset at high temporal (1 hour) and high spatial (31 km) resolution. TC is analysed at two different altitudes, the standard meteorological height of 2 meters, and at half the boundary layer height. In addition to the ERA5-based dataset, we also present an additional TC dataset obtained with data from a global constellation of meteorological stations.

We analyse and present statistics on the dependence of TC as function of time of the day, time of the year and land cover.  These provide constraints on the time windows and boundary conditions (e.g., land cover type) for which the sensitivity of the TIR instruments is best. It also allows optimal planning of overpass times for future infrared satellite sounders or the organization of aerial measurement campaigns for near-surface pollutants. Finally, this unique dataset can be used to statistically assess the measurement sensitivity of infrared sounders.

How to cite: Di Gioacchino, T., Clarisse, L., Van Damme, M., and Coheur, P.: Spatial and temporal variations of thermal contrast in the planetary boundary layer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13791, https://doi.org/10.5194/egusphere-egu23-13791, 2023.

EGU23-13983 | ECS | Posters on site | AS3.21

Investigation of Spatio-temporal Variation of Ammonia Concentrations in the Dominican Republic 

Seda Tokgoz, Carlos A. Sanlley, and Burcak Kaynak

Ammonia (NH3) whose main source is agriculture is a reactive and alkaline gas pollutant. Apart from eutrophication and acidification, it contributes to the production of secondary inorganic aerosol. Therefore, it has a significant impact on the ecosystem, air quality. Agriculture, especially activities such as livestock management and fertilizer applications, accounts for 70% of global NH3 emissions, and it is one of the main industries in the Dominican Republic. Ground-based NH3 measurements are not regularly available in the Dominican Republic and globally. No study determined NH3 concentrations using ground-based measurements and satellite retrievals in the Dominican Republic. The aim of this study is to investigate the seasonal and spatial changes of NH3 via all available measurements to understand the source regions.

In this study, MetOp (A,B and C) Infrared Atmospheric Sounding Interferometer (IASI) Level 2 NH3 retrievals are used to investigate the NH3 levels in the Dominican Republic. Spatially processed average NH3 retrievals are calculated for the interval between January 2020 and June 2022. Seasonal spatial distributions indicated highest NH3 levels in the fall season, and larger regions with high NH3 levels in the spring season. High average NH3 levels were observed in the northern Cibao region for all seasons. Monte Cristi, Santiago, Espaillat, La Vega, Monseñor Nouel were the main cities with high NH3 levels.

In addition to satellite retrievals, limited ground-level biweekly averaged NH3 measurements along with other air pollutants are available via published reports at seven different locations between August 2020 and June 2022. The highest average NH3 concentrations (≥ 56 ppb) are in the two locations at the capital city, Santo Domingo with high urbanization. The third highest location is in Santiago, where high values ​​are also observed in IASI NH3 retrievals. A location in Barahona (southwestern part) has the lowest average NH3 concentration. The spatio-temporal changes over sampling locations via both measurements are examined. Comparison of satellite retrievals with ground-based measurement is performed and correlations are estimated for seven different locations. In addition, average NH3 levels according to land cover will also be examined for three classes: urban, agricultural and forested areas. The results will provide information for future ground-based measurement studies and incorporate remote sensing measurements in assessment where only limited ground-level measurements are available. The findings of this study can also help to understand the role of NH3 for secondary inorganic aerosol formation.

Keywords: Ammonia, remote sensing, the Dominican Republic

How to cite: Tokgoz, S., Sanlley, C. A., and Kaynak, B.: Investigation of Spatio-temporal Variation of Ammonia Concentrations in the Dominican Republic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13983, https://doi.org/10.5194/egusphere-egu23-13983, 2023.

EGU23-14116 | ECS | Posters on site | AS3.21

Using a regional model as intermediate between in situ airborne measurements and Sentinel 5P δD column retrievals 

Iris Thurnherr, Harald Sodemann, Tim Trent, Martin Werner, and Hartmut Bösch

The isotopic composition of water vapour is a natural tracer of moisture cycling and moist processes such as rain-out efficiency in the atmosphere. The abundancy of deuterium (denoted as δD) in atmospheric water vapour can be studied using a variety of observational platforms that have a wide range of spatial and temporal resolutions. Recently, high-resolution and high-frequency δD total column retrievals from the Sentinel 5P satellite have become available, and need validation from in situ measurements. While satellite-retrieved products of δD in water vapour allow to study δD variability on spatial scales of several 1000km every 12-24h, the few available in-situ water vapour measurements of δD are at a much higher temporal resolution (seconds) and cover a more limited spatial extent (10s of km). In this study, we present a methodology for comparing datasets with different scales to each other. Thereby, it is important to take the principal time and length scales of water vapour δD features into account. To this end, we use model simulations with the isotope-enabled weather prediction model COSMOiso as an intermediate to bridge the scales between the newly developed retrieval of water isotopologues for the Sentinel 5P satellite, based on the University of Leicester Full Physics retrieval algorithm, and in-situ vertical profiles of δD from ultralight aircraft acquired during the L-WAIVE campaign in June 2019. We illustrate that the assessment of spatial and temporal δD correlated patterns in COSMOiso can serve as a proxy for spatial representativeness, and as such guides towards an unbiased comparison of datasets. Overall, we demonstrate that the combination of in-situ measurements and COSMOiso simulations with satellite-retrieved δD can help to better constrain vertical δD gradients and to understand the temporal evolution of large scale δD patterns and associated moist processes. From our findings, we also derive more general recommendations for future comparison studies of in-situ measurement, satellite products, and model-simulated δD.  

How to cite: Thurnherr, I., Sodemann, H., Trent, T., Werner, M., and Bösch, H.: Using a regional model as intermediate between in situ airborne measurements and Sentinel 5P δD column retrievals, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14116, https://doi.org/10.5194/egusphere-egu23-14116, 2023.

EGU23-15585 | Orals | AS3.21

Monitoring of atmospheric ammonia (NH3) in Auvergne-Rhône-Alpes region (France): comparison between satellite, ground-based observations, and simulations from a chemistry-transport model 

Benoît Tournadre, Harry Dupont, Sabrina Pontet, Marie-Pierre Vagnot, Julie Cozic, Claire Chappaz, and Stéphane Socquet-Juglard

Atmospheric ammonia (NH3) is a gaseous precursor of secondary inorganic aerosols, which represent a significant part of concentrations of fine particulate matter PM2.5 measured in the French region Auvergne-Rhône-Alpes (AuRA). Although French State gives an objective for reducing territorial NH3 emissions, ammonia concentrations in ambient air are not regulated. Very few continuous measurement stations exist in France and cover a time range of a few years at most. Ammonia can also be monitored by satellite remote sensing, which offers a better spatial coverage over more than a decade. 

Atmo Auvergne-Rhône-Alpes (Atmo AuRA) is a regional observatory of air quality approved by the French State. Atmo AuRA extends its activities to the use of satellite remote sensing data as an external source of information to test the consistency of its emission cadastres, air quality forecasts and hindcasts and potentially improve them. 

Since 2015, Amo AuRA maintains a station in Lyon with an analyzer measuring continuously NH3 mixing ratios. The association also builds regional emission inventories of air pollutants, including NH3, and runs routinely CHIMERE chemistry-transport model to evaluate and forecast regional air quality. The chemistry-transport modeling can be used to simulate NH3 atmospheric content for given emissions from inventories and be compared with actual measurements. 

In this study, we compare different datasets describing NH3 atmospheric content in AuRA region. Morning in situ measurements in Lyon are compared with NH3 level 2 data of total columns retrieved from the Infrared Atmospheric Sounding Interferometer (IASI), to evaluate their covariations on the period 2016-2021. The temporal consistency between ground measurements and simulations from CHIMERE is also investigated over the same period. Finally, a comparative analysis on CHIMERE and IASI data is done both in terms of spatial distribution and temporal evolution. 

How to cite: Tournadre, B., Dupont, H., Pontet, S., Vagnot, M.-P., Cozic, J., Chappaz, C., and Socquet-Juglard, S.: Monitoring of atmospheric ammonia (NH3) in Auvergne-Rhône-Alpes region (France): comparison between satellite, ground-based observations, and simulations from a chemistry-transport model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15585, https://doi.org/10.5194/egusphere-egu23-15585, 2023.

Despite a relatively simple chemistry, nitrogen dioxide (NO2) remains challenging to reproduce accurately in current air quality models, notably due to persistent uncertainties affecting the representation of its anthropogenic and natural emission sources. Another reason for these uncertainties lies is the lack of surface in-situ observations in many rural areas where nitrogen oxides (NOX) are yet playing a strong role in ozone formation.

In this study, we take benefit from the TROPOMI NO2 tropospheric columns (TrC-NO2) observations complemented by surface NO2 observations to comprehensively evaluate the MONARCH chemical weather model. We focus our analysis over the Iberian Peninsula during the year 2019. MONARCH reproduces relatively well the spatial variability of TrC-NO2 observed by TROPOMI, although with a negative bias. A lack of NOx emission in rural areas over the Iberian Peninsula is strongly suggested by the results. In order to investigate more deeply the corresponding underestimation of rural NOx, different sensitivity analyses are performed, notably on anthropogenic NOX and natural soil nitric oxide (NO) emissions. The sensitivity analysis showed a spatially and seasonally dependent response of the emissions used as inputs in MONARCH on the modeled TrC-NO2. The combined evaluation on surface and TrC NO2 provide some interesting insights on the vertical distribution and its representation in MONARCH.

This study thus illustrates the strong interest of such satellite-based observations to complement surface monitoring stations, especially in areas such as croplands where almost no surface observations are available.

How to cite: Lopez, F., Petetin, H., and Jorba, O.: Evaluation of the MONARCH-simulated NO2 tropospheric columns against Sentinel-5P TROPOMI observations over the Iberian Peninsula, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15833, https://doi.org/10.5194/egusphere-egu23-15833, 2023.

EGU23-15936 | Orals | AS3.21

Sentinel-5P TROPOMI NO2 reprocessing v2.4.0: Impact of the surface albedo 

Henk Eskes, Jos van Geffen, K. Folkert Boersma, Gijs Tilstra, Maarten Sneep, and Pepijn Veefkind

The Sentinel-5P TROPOMI instrument provides unique observations of atmospheric composition at a high spatial resolution of about 5 km with near-daily global coverage. A new mission reprocessing of all official data products for the full operational phase (30 April 2018 until the present) is currently being generated, co-ordinated by ESA, and is expected to become available in March/April 2023. 

For NO2 this reprocessing will result in a uniform dataseries for the full mission based on processor version 2.4.0 and on version 2 level-1B input data. The reprocessing is replacing the currently available data record for NO2, based on processor versions 1.2 x, 1.3.x, 1.4.0, 2.2.0 and 2.3.1. The upgrades to v1.4 and v2.2 involved major upgrades. Validation activities indicated that the older versions 1.2 and 1.3 had a low bias, a problem which was (at least partly) resolved by introducing v1.4 and v2.y. However, this also implies that trend studies are severely hampered by the jumps in the data series resulting from this sequence of updates. In order to support COVID-19 lockdown air pollution studies an intermediate "PAL" reprocessing of NO2 was made available in December 2021 based on the v2.3.1 NO2 processor and v1 L-1B data (https://data-portal.s5p-pal.com/products/no2.html).  The new official reprocessing with v2.4.0 and v2 L-1B will replace this PAL dataset. The new official reprocessing is expected to be of great use for studying the inter-annual variability in NO2 in recent years.  

The major change in v2.4.0 compared to v2.3.1 is the replacement of the surface albedo datasets with a directional (viewing-angle dependent) Lambertian equivalent reflectivity (DLER) database derived from TROPOMI observations. Before the TROPOMI NO2 processor made use of the OMI (for the NO2 fitting window) and GOME-2 (for the O-2A band spectral region used for the cloud retrieval) LER. The use of the TROPOMI DLER is especially important for the cloud fraction and cloud pressure retrievals, because the clear-sky reflectivity in the NIR is very sensitive to the (viewing) geometry. 

In our contribution we will present the new reprocessed TROPOMI NO2 v2.4 dataset and quantify the impact of the use of the TROPOMI DLER on the cloud properties, air-mass factor and tropospheric NO2 column. 

How to cite: Eskes, H., van Geffen, J., Boersma, K. F., Tilstra, G., Sneep, M., and Veefkind, P.: Sentinel-5P TROPOMI NO2 reprocessing v2.4.0: Impact of the surface albedo, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15936, https://doi.org/10.5194/egusphere-egu23-15936, 2023.

EGU23-16516 | ECS | Posters on site | AS3.21

Estimating surface-level nitrogen dioxide concentrations from Sentinel-5P/TROPOMI observations in Finland 

Henrik Virta, Iolanda Ialongo, and Monika Szeląg

In recent decades, satellite instruments have been providing observations of air pollutants such as nitrogen dioxide (NO2) with global coverage. Since late 2018, the TROPOspheric Monitoring Instrument (TROPOMI) on-board the Copernicus Sentinel-5 Precursor satellite has produced NO2 vertical column densities (VCDs) with the best spatial resolution (currently 5.5x3.5 km at nadir). In order to compare satellite-based observations to traditional NO2 surface concentration measurements available from air quality (AQ) stations, methods based on chemical-transport model (CTM) simulations can be applied to convert satellite-based VCDs to surface concentrations. Such methods have been mostly developed and applied in regions with high NO2 concentrations at middle-low latitudes.

In this paper, we test and adapt two methods to estimate surface-level NO2 concentrations from TROPOMI observations in Finland, which is characterised by low NO2 concentrations at a high latitude location. Satellite-based estimates show good correlation with co-located surface NO2 measurements from the Finnish AQ network, although the method lacking a correction for the level of NO2 mixing within the boundary layer is more prone to underestimation. New cut-off values accounting for the level of mixing were calculated to adapt the column-to-surface conversion to specific conditions in Finland. We also present an alternate approach to reduce the underestimation based on the linear relation between in situ measurements and surface-level estimates.

We utilise chemical transport model simulations to correct our surface-level NO2 estimates to derive full annual mean concentration estimates compatible with annual limit values defined in AQ legislation. This correction is based on the temporal sampling differences between in situ station measurements and TROPOMI observations. The annual estimates tend to overestimate concentrations compared to ground-based measurements, but can be considered as an upper estimate of surface concentrations. They can therefore complement existing AQ station measurements, especially in regions where the surface networks are sparse. Despite the uncertainties, we find that the two Finnish AQ monitoring regions currently lacking surface stations have estimated mean annual concentrations well below existing limit values, suggesting no need for new ground-based monitoring stations.

Overall, the results provide new information to complement traditional surface-based AQ measurements and to support national environmental authorities in air quality assessment and reporting.

How to cite: Virta, H., Ialongo, I., and Szeląg, M.: Estimating surface-level nitrogen dioxide concentrations from Sentinel-5P/TROPOMI observations in Finland, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16516, https://doi.org/10.5194/egusphere-egu23-16516, 2023.

EGU23-16698 | ECS | Posters on site | AS3.21

French NOx emissions as estimated from TROPOMI-PAL NO2 observations 

Robin Plauchu, Audrey Fortems-Cheiney, Grégoire Broquet, Isabelle Pison, Antoine Berchet, Elise Potier, Adriana Coman, Dilek Savas, and Gaëlle Dufour

Since 2018, TROPOMI onboard Sentinel-5P has brought images of NO2 tropospheric columns at an unprecedented high spatial resolution. We attempt to exploit the potential of this high-resolution information to estimate NOx emissions at the national scale based on atmospheric inversion approaches, with a 10-km spatial resolution. This study focuses on France and assesses the Covid-19 pandemic effects.

Our analysis is based on the variational mode of the recently developed Community Inversion Framework (CIF), coupled with France's configuration of the CHIMERE regional chemistry transport model and its adjoint code. Both CHIMERE and its adjoint code include the MELCHIOR-2 chemical scheme with more than 100 reactions (24 for inorganic chemistry). This variational framework allows to solve high-dimensional inversion problems and thus investigate fine-scale patterns in the concentration and emission fields. It also allows to properly account for the non-linearities associated with the chemistry. CHIMERE is driven by the European Centre for Medium-Range Weather Forecasts (ECMWF) operational meteorological forecast. The inversion corrects anthropogenic emissions from the French National Spatialized Inventory (INS, Inventaire National Spatialisé), mapping NOx emissions at a 1 x 1 km2 horizontal resolution. It also corrects biogenic emissions from the MEGAN model. We use the last TROPOMI reprocessed data: the PAL product. 

We present different tests that have been conducted to improve the implementation of the observation and control vector in order to strengthen the robustness of the inversion. Then, we evaluate the potential of the TROPOMI-PAL observations to quantify emissions at the national to local scale and at the annual to monthly scale based on the analysis of the reference inversions for the years 2019 and 2020. Finally, we focus on the differences found between the emission estimates for spring 2020 and 2019 to assess the impact of the Covid-19 pandemic.

How to cite: Plauchu, R., Fortems-Cheiney, A., Broquet, G., Pison, I., Berchet, A., Potier, E., Coman, A., Savas, D., and Dufour, G.: French NOx emissions as estimated from TROPOMI-PAL NO2 observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16698, https://doi.org/10.5194/egusphere-egu23-16698, 2023.

EGU23-301 | ECS | Orals | AS3.22

From political pledges to the quantitative mapping of climate mitigation plans: comparison of two European cities 

Ivonne Albarus, Giorgia Fleischmann, Patrick Aigner, Philippe Ciais, Hugo Denier van der Gon, Rianne Droge, Jinghui Lian, Miguel Andrey Narvaez Rincon, Hervé Utard, and Thomas Lauvaux

Urban agglomerations play a crucial role in reaching global climate objectives. Many cities have committed to reducing their greenhouse gas emissions, but current emission trends remain unverifiable. The quantification of mitigation policies is often incomplete or unavailable, raising serious concerns about how and if climate mitigation targets will be achieved. To support the effective traceability of urban emissions trajectories, atmospheric monitoring of greenhouse gases (GHG) has been deployed over several metropolitan areas. This approach offers an independent and transparent solution to measuring urban emissions. However, careful design of the monitoring network is crucial to be able to monitor the most important sectors as well as to adjust to rapidly changing urban landscapes.

We present here a joint study of Paris and Munich emissions trajectories to demonstrate how climate action plans, carbon emission inventories, and urban development plans can be combined to construct high-resolution projected emissions maps and to help design optimal atmospheric monitoring networks. We show that these two European cities will encounter widely different GHG emission trajectories in space and time, reflecting different emission reduction strategies and different constraints due to administrative boundaries. The projected CO2 emissions for the milestone years 2030 and 2050 are based on the 2019 spatially distributed 1km x 1km TNO inventory. Future emissions scenarios are based on the analysis of their respective Climate Action Plan. Individual mitigation measures are quantified, sectorized and the resulting saving potentials are applied to the 2019 TNO inventory, used as baseline. The projected CO2 emissions rely on future actions, hence uncertain, but we demonstrate how emission reductions vary significantly at the sub-city level. 

We show here how climate actions, population growth, and urbanization plans produce mixed spatial patterns across both cities. We conclude that quantified individual cities’ climate actions are essential for strengthening climate policies and their effectiveness at the city scale. Harmonization and compatibility of climate plans from various cities are necessary to make intercity comparisons of climate targets possible. In terms of atmospheric monitoring, our results demonstrate the need for additional measurement stations located inside the densest areas of the two cities but also in the cities’ outskirts to track local positive and negative emission trends over the coming decades. 

How to cite: Albarus, I., Fleischmann, G., Aigner, P., Ciais, P., Denier van der Gon, H., Droge, R., Lian, J., Narvaez Rincon, M. A., Utard, H., and Lauvaux, T.: From political pledges to the quantitative mapping of climate mitigation plans: comparison of two European cities, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-301, https://doi.org/10.5194/egusphere-egu23-301, 2023.

EGU23-770 | ECS | Orals | AS3.22

Atmospheric CO2 monitoring over a large tropical metropolitan area: fossil fuel and biogenic CO2 fluxes over the Sao Paulo Metropolitan Area 

Rafaela Cruz Alves Alberti, Ricard Segura Barrero, Gara Villalba Mendez, Maria Fátima Andrade, Thomas Lauvaux, Humberto Ribeiro da Rocha, Osvaldo Machado Rodrigues Cabral, and Rita Ynoue

Sao Paulo Metropolitan Area, with 39 municipalities and a population of about 22 million inhabitants, aims to reach carbon neutrality by 2050. More than half of its population resides in Sao Paulo city, which, in 2018, was responsible for emitting nearly 18 million tons of CO2 equivalent. Two high-accuracy CO2 sensors have been deployed (Picarro CRDS analyzers)  from the first conventional in situ measurement network installed in South America for GHG monitoring.  The Weather Research and Forecasting model coupled with Chemistry (WRF-Chem V4.0) with a modified version of the greenhouse gas chemistry module (WRF-GHG) was used to simulate the transport of the mole fraction of carbon dioxide (CO2) at a horizontal resolution of 3 km in the São Paulo Metropolitan Area during August 2020. Biogenic CO2 fluxes were simulated using an improved version of the “Vegetation Photosynthesis and Respiration Model” (VPRM) (Mahadevan et al., 2008) included offline in WRF-GHG. The VPRM parameters were optimized using flux tower data (Net Ecosystem Exchange) for the three main vegetation types in the area (Atlantic Forest, Sugarcane, and Cerrado). Anthropogenic CO2 emissions were simulated with the vehicle emission model VEIN (Ibarra et al., 2018) combined with industrial emissions from EDGAR (Crippa et al., 2020) and ODIAC (Oda et al., 2018). The initial and lateral boundary conditions (IC-BCs) were imported from CAMS and from CARBON-TRACKER global reanalysis for greenhouse gases.

The simulated CO2 concentrations from the WRF-GHG model captured both day-to-day and diurnal variations compared to in situ observations in suburban and urban areas (Pico do Jaraguá and IAG). We examined the magnitude of the fossil fuel contribution compared to biogenic signals across the domain, and the anthropogenic signals are heavily influenced by local and nearby sources and sinks. Additionally, the signal includes respiration from vegetation that is carried by winds from vegetation regions.

 We conducted a long-term analysis of CO2 concentration measurements at the two stations (2019-2022) to determine the seasonality and its relationship with both flux variability and local circulation. Finally, we estimated CO2 concentration gradients from three additional measurement stations around the Sao Paulo metropolitan area to assess the potential of our future urban atmospheric inversion system. 

How to cite: Cruz Alves Alberti, R., Segura Barrero, R., Villalba Mendez, G., Fátima Andrade, M., Lauvaux, T., Ribeiro da Rocha, H., Machado Rodrigues Cabral, O., and Ynoue, R.: Atmospheric CO2 monitoring over a large tropical metropolitan area: fossil fuel and biogenic CO2 fluxes over the Sao Paulo Metropolitan Area, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-770, https://doi.org/10.5194/egusphere-egu23-770, 2023.

EGU23-1647 | ECS | Orals | AS3.22

Development of a new global CO2 emission database with highly-resolved source category and sub-country information: methodology and 1970-2021 emissions 

Ruochong Xu, Qiang Zhang, Dan Tong, Qingyang Xiao, Xinying Qin, Cuihong Chen, Liu Yan, Jing Cheng, Can Cui, Hanwen Hu, Wenyu Liu, Xizhe Yan, Huaxuan Wang, Xiaodong Liu, Guannan Geng, Dabo Guan, and Kebin He

CO2 emission database lays the foundation of climate research and climate governance. Most current global CO2 emission inventories were developed with energy statistics from International Energy Agency (IEA) and were available at country level with limited source categories. Here, as the first step toward a high-resolution and dynamic updated global CO2 emission database, we developed a data-driven approach to construct seamless and highly-resolved energy consumption data cubes for 208 countries/territories, 797 sub-country administrative divisions in 29 countries, 42 fuel types, and 52 sectors, with the fusion of energy consumption from 24 international statistics and 66 regional/local statistics. Global CO2 emissions from fossil fuel combustion and cement production in 1970-2021 were then estimated with highly-resolved source category (1484 of total) and sub-country information (797 of total). Specifically, 73% of global CO2 emissions in 2021 were calculated based on sub-country information, providing considerably improved spatial resolution for global CO2 accounting. With the support of detailed information, the dynamics of global CO2 emissions across sectors and fuels were presented, representing the evolution of global economy and progress of climate governance. Remarkable differences of sectoral contribution were found across sub-country administrative divisions within a given country, revealing the uneven distribution of energy and economic structure among different regions. Our estimates were generally consistent with existing databases at aggregated level for global total or large emitters, while large discrepancies were observed for middle and small emitters. Our database, named Multi-resolution Emission Inventory model for Climate and air pollution research (MEIC) is publicly available through http://meicmodel.org.cn with highly-resolved information and timely update, which provides an independent carbon emission accounting data source for climate research.

How to cite: Xu, R., Zhang, Q., Tong, D., Xiao, Q., Qin, X., Chen, C., Yan, L., Cheng, J., Cui, C., Hu, H., Liu, W., Yan, X., Wang, H., Liu, X., Geng, G., Guan, D., and He, K.: Development of a new global CO2 emission database with highly-resolved source category and sub-country information: methodology and 1970-2021 emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1647, https://doi.org/10.5194/egusphere-egu23-1647, 2023.

EGU23-2527 | Posters on site | AS3.22

Simulation setup for atmospheric CH4 concentrations in the ICON-ART Limited Area Mode 

Buhalqem Mamtimin, Thomas Rösch, Franziska Roth, Anusha Sunkisala, and Andrea Kaiser-Weiss

An experimental setup within ICON (ICOsahedral Non-hydrostatic)-ART (Aerosols and Reactive Trace gases) has been  carried out to simulate the atmospheric CH4 concentration over Europe during the investigation period from 01 May 2018 to 30 June 2018.

Modelling CH4 in the Limited Area Mode (Europe, 6.5 x 6.5 km), the model requires as accurate as possible initial and boundary atmospheric conditions as well as spatially highly resolved emissions. Temporal resolved emissions are to be included in the next step. While the intial data denote here the state of the atmosphere (meteorological and CH4 concentration fields) at the start of the model run, the boundary conditions shall denote the data in the lateral boundary zone where the model is forced by the meteorological and CH4 concentration data outside the domain. We have used DWD's operational numerical weather prediction output as meteorological boundary conditions. The Copernicus Atmosphere Monitoring Service (CAMS) provides the necessary initial and boundary CH4 data, which are made applicable  for the ICON-ART before the model run in Limited Area Mode. The regional CH4 emissions for Europe have been  provided by TNO and are processed with the ART module.  

Since CAMS uses a vertical coordinate of a hybrid sigma-pressure system, the data had been horizontally and vertically interpolated to the height based SLEVE coordinate system of ICON. The sectorial CH4 emissions for Europe and for Germany were mapped separately to the target ICON grid by preprocessing the corresponding reported methane emissions of various sectors (resulting in 36 distinct methane variables in the model). The 50 largest point emissions from each sector are treated separately, smaller point emissions are treated together with the area emissions.

To run a hourly experimental setup for two month the Basic Cycling environment (BACY) tool was used. The fields for meteorological parameters were initialized daily by using the DWD's operational data, while the atmospheric CH4 concentrations are taken from the previous ICON-ART CH4 simulation results (e.g., the 24 h CH4 forecast from the previous day). Then, the merged concentration fields for meterological conditions and atmospheric methane are used as “DWD first guess”, which served for a daily start of the simulation process in the ICON-ART Limited Area Mode. In order to compare the model results and measurements from the Integrated Carbon Observation System (ICOS) stations, the model equivalents have been extracted at the locations of the  ICOS montoring stations  using the “Model Equivalent Calculator”.

In this work, the ICON-ART CH4 simulation setup for Limited Area Mode (Europe) was forced by ICON meteorology and CAMS CH4 boundary data and had been started daily by the merged “DWD first guess”. These are shown to be a useful method to simulate the CH4 atmospheric concentrations at the regional scale.

How to cite: Mamtimin, B., Rösch, T., Roth, F., Sunkisala, A., and Kaiser-Weiss, A.: Simulation setup for atmospheric CH4 concentrations in the ICON-ART Limited Area Mode, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2527, https://doi.org/10.5194/egusphere-egu23-2527, 2023.

NASA’s Carbon Monitoring System (CMS) has a 12-year record of production of prototype data products from across Carbon Cycle Science that have potential usefulness for stakeholders outside the standard science community.   CMS originated from US Congressional direction through the budget process back in 2010 and remains currently.  CMS activities all include significant use of remote sensing data, as that is NASA’s strong suit.  We have been emphasizing increased engagement with stakeholders as CMS has progressed.  Prototype products exist currently related to GHG fluxes, terrestrial biomass, and ocean/coastal carbon.  Satellite sensors currently employed in CMS prototype products include OCO-2, OCO-3, S5P, GOSAT, GEDI, MODIS, and LandSat.  These various product development teams are coordinated through related working groups to help learn from the other projects, exchange ideas to improve outreach to stakeholders, and set potential direction for future CMS solicitations.  Many of the CMS products, that have existed for years and further developing, especially those related to GHG fluxes, have participants from numerous US agencies and have direct relationship to the coordination activities being discussed by many nations. 

How to cite: Jucks, K.: NASA’s Carbon Monitoring System; lessons learned from 12 years of producing society-relevant, science-based, prototype Carbon-related products., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3626, https://doi.org/10.5194/egusphere-egu23-3626, 2023.

EGU23-3759 | Posters on site | AS3.22 | Highlight

PARIS - Process Attribution of Regional emISsions 

Sylvia Walter, Anita Ganesan, Thomas Röckmann, and Aoife Grant and the PARIS team

PARIS is a 4-year Horizon Europe research project that aims to significantly increase our knowledge about the emissions of climate forcers from 8 European countries. PARIS focuses on the interface between bottom-up and top-down approaches and aims to strengthen the collaboration between scientists and national inventory teams for the evaluation and development of national inventories.

Seventeen European partners will work together to quantify emissions of carbon dioxide, methane, nitrous oxide, fluorinated gases (F-gases), and black carbon.  To engage inventory teams early in the project, we focus early on emission estimates for fluorinated gases (F-gases), which have relatively simple source distributions, but poorly understood magnitudes. For greenhouse gases with a more complex mixture of sources, methane and carbon dioxide, research in PARIS focuses on the attribution of fluxes to particular sources and sinks. We will advance isotopologue measurements and multi-tracer analysis methods for source characterization, providing inventory teams with new information to target areas of uncertainty. For nitrous oxide, a greenhouse gas for which most European inventories rely on highly simplified and uncertain bottom-up methods, two process-level models will be advanced to produce time- and space-resolved estimates that will be evaluated against isotopic data. For the important, but complex, climate forcers, organic matter aerosol and black carbon, we will take the next steps required towards robust top-down emissions inference by developing source apportionment methods. To generate maximum impact, we will synthesise our efforts in the form of draft annual Annexes to National Inventory Reports (NIRs) for eight European PARIS focus countries.

The overall objectives of PARIS are:

1) Quantify top-down emissions from a selection of European countries of all the major GHGs reported under the UNFCCC (CO2, CH4, N2O and F-gases), and black carbon aerosol (BC) reported under CLRTAP.

2) Quantify the contribution of major source sectors of GHG and BC emissions and organic matter aerosol (OM) abundance through the implementation of innovative measurement and analysis technologies.

3) Derive time- and space-resolved flux estimates for GHGs with complex or uncertain source distributions (N2O, F-gases)

4) Produce draft Annexes to the annual National Inventory Reports (NIRs) for a selection of ‘focus’ countries.

This presentation will give a general overview of the PARIS project, its objectives and implementation. It aims to introduce the project to the scientific community, and to set up a network for future collaborations with related projects, e.g.EYE-CLIMA (https://cordis.europa.eu/project/id/101081395) or AVENGERS (https://cordis.europa.eu/project/id/101081322).

How to cite: Walter, S., Ganesan, A., Röckmann, T., and Grant, A. and the PARIS team: PARIS - Process Attribution of Regional emISsions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3759, https://doi.org/10.5194/egusphere-egu23-3759, 2023.

EGU23-4138 | ECS | Orals | AS3.22

Building Integral Gridded Carbon Emission Disaggregating Model (BIGCarbonEDM): Near real-time community-level CO2 emission evaluations for twelve cities in Egypt, South Africa, and Turkey 

Chuanlong Zhou, Mathieu de Castelbajac, Biqing Zhu, Da Huo, Zhu Liu, Antoine Benoit, Chandan Deuskar, Craig Mesner, Julian Akani-Guéry, Margaux Boucher, and Philippe Ciais

Cities generate the majority of CO2 emissions, the largest climate change contributor. Near real-time CO2 emission monitoring and modeling at relatively high resolutions are beneficial to fill the knowledge gaps for the spatial and temporal emission patterns in different regions, and to provide the public and the policymakers with accurate and timely information on major emission sources and emission amounts for better public awareness and decision making. On the other hand, there are even larger knowledge and information shortage in Global South counties for the city-/community- level CO2 emissions due to the lack of well-monitored official data with high latency and low transparency.

Data-driven models with big data embedded can be one of the most robust and efficient approaches for addressing those challenges in regions without well-documented data. Therefore, we developed the Building Integral Gridded Carbon Emission Disaggregating Model (BIGCarbonEDM) that disaggregates Scope 1&2 CO2 emissions to community-level (with a resolution at 500 meters) using machine learning models trained with building- to regional-level features. Multiple open datasets were used as model inputs, 1) building-level datasets: Microsoft Building Footprints, OpenStreetMap, and OpenStreetMap Building, 2) regional-level datasets: Global Human Settlement, World Settlement Footprint, VIIRS Nightlights, Local Climate Zone, Copernicus Digital Elevation, and land surface temperature, 3) economical and census datasets were collected from the national statistical report and world bank surveys, and 4)city-level near real-time CO2 emission: Carbon Monitor City (https://cities.carbonmonitor.org/), one of our previous projects.

BIGCarbonEDM for the first time proposed the approach for capturing the emission patterns for the community level based on building-level and regional-level features and provides the near real-time CO2 emission for twelve major cities in Egypt, South Africa, and Turkey. The cities are Adana, Trabzon, Ordu, and Manisa for Turkey; Cairo, Alexandria, Luxor, and Sheikh Zayed for Egypt; and Johannesburg, Tshwane, Ekurhuleni, and eThekwini for South Africa. BIGCarbonEDM was designed as a modular platform including modules for data collection, data fusion, spatial and temporal emission feature learning, emission estimation model, and data visualization. BIGCarbonEDM modules can be updated and modified separately, which simplifies the improvements and extensions of the final delivered dataset, also all the individual modules can be used by the research community for other relevant research.

How to cite: Zhou, C., de Castelbajac, M., Zhu, B., Huo, D., Liu, Z., Benoit, A., Deuskar, C., Mesner, C., Akani-Guéry, J., Boucher, M., and Ciais, P.: Building Integral Gridded Carbon Emission Disaggregating Model (BIGCarbonEDM): Near real-time community-level CO2 emission evaluations for twelve cities in Egypt, South Africa, and Turkey, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4138, https://doi.org/10.5194/egusphere-egu23-4138, 2023.

EGU23-4302 | ECS | Posters on site | AS3.22 | Highlight

Emission trend and drivers of CO2 emission in Chinese cities from 2012 to 2018 

Qinren Shi, Bo Zheng, Qiang Zhang, and Kebin He

China has pledged to peak CO2 emissions before 2030 and achieve carbon neutrality before 2060, and climate actions are urgently needed. Cites are basic administrative units and leaders in implementing emission reduction policies in China, and a comprehensive analysis of characteristics and historical emission trends in Chinese cities is of great importance. This study developed a city-level CO2 emission inventory in China during 2012-2018 by merging multiple databases. The results reveal spatial heterogeneity and inequality in Chinese cities’ CO2 emissions. In general, eastern cities emit more CO2 than western cities. According to the emission-Lorenz curve, the top 10% of 336 cities contribute over 30% of total CO2 emissions in 2018. From the perspective of emission trends, more than 60% of cities in China failed to achieve the decoupling of GDP growth and carbon emissions. The overall positive correlation between per capita GDP and per capita carbon emission in Chinese cities indicates that even cities with a relatively high level of development still need to further promote carbon emission reduction. As for sectoral drivers, industrial boilers and cement sectors were the major drivers for CO2 emission reduction in most cities, while the increase in carbon emissions from thermal power and industrial boiler sectors led to the rebound of carbon emissions in most cities.

How to cite: Shi, Q., Zheng, B., Zhang, Q., and He, K.: Emission trend and drivers of CO2 emission in Chinese cities from 2012 to 2018, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4302, https://doi.org/10.5194/egusphere-egu23-4302, 2023.

EGU23-4558 | ECS | Orals | AS3.22 | Highlight

Carbon Monitor Europe, a near-real-time and country-level monitoring of daily CO2 emissions for European Union and the United Kingdom 

Piyu Ke, Zhu Deng, Biqing Zhu, Bo Zheng, Yilong Wang, Olivier Boucher, Simon Ben Arous, Chuanlong Zhou, Xinyu Dou, Taochun Sun, Zhao Li, Feifan Yan, Duo Cui, Yifan Hu, Da Huo, Jean Pierre, Richard Engelen, Steven J. Davis, Philippe Ciais, and Zhu Liu

With the urgent need to implement the EU countries pledges and to monitor the effectiveness of Green Deal plan to reduce greenhouse gases emissions, Monitoring Reporting and Verification tools are needed to track how emissions are changing for all the sectors. Current official inventories only provide annual estimates of national CO2 emissions with a lag of 1+ year which do not capture the variations of emissions due to recent shocks including COVID lockdowns and economic rebounds, supply chains tensions and rising prices of energy and commodities, war in Ukraine. Here we present a near-real-time dataset of daily fossil fuel and cement emissions to monitor country-level emissions from January 2019 through December 2021 for 27 European Union countries and the United Kingdom. This dataset is called Carbon Monitor Europe. The data are calculated separately for six sectors: power, industry (incl. cement production), ground transportation, domestic aviation, international aviation, residential emissions which includes the built environment. Daily CO2 emissions are estimated from a large set of activity data compiled from different sources, including hourly to daily electrical power generation data, monthly production data and production indices of industry, daily mobility data and indices for the ground transportation. Individual flight location data and monthly data were for aviation sector estimates. Monthly fuel consumption data downscaled in time with daily air temperature are used to estimate daily emissions from commercial and residential buildings. The goal of this dataset is to improve the timeliness and temporal resolution of emissions for European countries, to inform the public and decision makers about current emissions changes in Europe.

How to cite: Ke, P., Deng, Z., Zhu, B., Zheng, B., Wang, Y., Boucher, O., Ben Arous, S., Zhou, C., Dou, X., Sun, T., Li, Z., Yan, F., Cui, D., Hu, Y., Huo, D., Pierre, J., Engelen, R., J. Davis, S., Ciais, P., and Liu, Z.: Carbon Monitor Europe, a near-real-time and country-level monitoring of daily CO2 emissions for European Union and the United Kingdom, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4558, https://doi.org/10.5194/egusphere-egu23-4558, 2023.

Atmospheric carbon dioxide (CO2) in the atmosphere has increased mainly due to anthropogenic fossil fuel emissions, resulting in accelerating global warming and increasing climate variability. Atmospheric chemical transport models are powerful tools for understanding mechanisms between emission/sink and the spatiotemporal distribution of atmospheric CO2.

We aim to provide information on GEOS-Chem CO2 simulation to assess the mitigation strategies over East Asia under future emission scenarios. To achieve this, we first need to evaluate the model performance of the global simulation. We investigated trends and characteristics of atmospheric CO2 from the model with ground-based in-situ observations from the World Data Centre for Greenhouse Gases; (WDCGG), Total Carbon Column Observing Network (TCCON), and satellite observations (e.g., the Greenhouse Gases Observing Satellite; GOSAT, the Orbiting Carbon Observatory 2; OCO-2).

Overall, modeled CO2 concentrations showed reasonable seasonal, annual amplitudes, and spatiotemporal distributions. They also agreed well with ground-based observations and satellite observations. Our global simulation was highly correlated with in-situ observations (Index of agreement (IOA) ≈ 0.9), and also showed excellent performance (Correlation coefficient (R) > 0.9) compared with satellite observations. Our study provides broad information on global simulation to identify features of monitoring measurements and modeling. We anticipate that our model configuration is capable of studying future emission scenarios in East Asia.

How to cite: Kang, Y. and Song, C.-K.: An evaluation of global atmospheric CO2 simulation by the GEOS-Chem using multiple observations in the period 2010-2020, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4763, https://doi.org/10.5194/egusphere-egu23-4763, 2023.

EGU23-4955 | ECS | Posters on site | AS3.22

Modeling fuel- and vehicle- type specific CO2 emissions from global on-road vehicles during 1970-2020 

Liu Yan, Qiang Zhang, and Kebin He

Vehicles are one of the most important contributors to global anthropogenic CO2 emissions. However, lack of fuel- and vehicle- type specific information about global on-road CO2 emissions from existing datasets, which are only available at sector level, makes it insufficient to support establishment of emission mitigation strategies. Thus, a fleet model is developed in this study and CO2 emissions from global on-road vehicles during 1970-2020 are estimated at vehicle level. Here we access the fuel- and vehicle- type specific characteristics of both vehicular CO2 emissions and vehicle ownership, and highlight the trend in the intensity of CO2 emissions and ownership of on-road vehicles in hotspot regions. We find that, heavy-duty trucks and buses which account for less than 10% of global vehicle ownership but represent over 30% of on-road CO2 emissions. Contribution of diesel vehicles to global on-road CO2 emissions has doubled during 1970-2020, driven by the shift in fuel-type distribution of vehicle ownership. As the top four vehicle markets, vehicles per thousand people in the United States, European Union, China and India all increased significantly from 1970 to 2020 while vehicle intensity China and India was still lower than global average level, which indicates that developing countries have to face great challenges in vehicular decarbonization in the future. CO2 emissions per vehicle in these regions generally decreased for the last 50 years, but vehicular CO2 emission intensity in the United States and European Union were relatively higher, meaning that there're still large potentials for developed countries in vehicular CO2 emission mitigation. These findings provide better understanding of trends of historical CO2 emissions from on-road vehicles, as well as insights into the effective governance of CO2 emissions in the future.

How to cite: Yan, L., Zhang, Q., and He, K.: Modeling fuel- and vehicle- type specific CO2 emissions from global on-road vehicles during 1970-2020, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4955, https://doi.org/10.5194/egusphere-egu23-4955, 2023.

EGU23-6154 | ECS | Orals | AS3.22 | Highlight

Following the temporal and spatial variability of atmospheric 14CO2 across Switzerland to estimate source contributions to the national CO2 emissions. 

Dylan Geissbühler, Thomas Laemmel, Philip Gautschi, Lukas Wacker, and Sönke Szidat

Perturbations to the natural carbon cycle due to anthropogenic and induced natural emissions of carbon dioxide (CO2) into the atmosphere are strongly linked with the current trend of global climate change. Efforts aiming at measuring amounts of CO2 emitted by different ecosystems and industrial activities have been increasing in the past years, in order to gather information about necessary mitigations efforts towards reduced future emissions.

Radiocarbon (14C) measurements of atmospheric CO2 are unique in their capabilities to provide information on carbon sources and transport. The radiocarbon method allows an apportionment between "modern" sources, with 14CO2 signatures close to the global atmospheric average and fossil-fuel derived sources which are 14C-depleted. The capability to determine the fraction of fossil CO2 in atmospheric samples provides insight on the contribution of different emissions to the current rise in atmospheric CO2 concentration. When associated with meteorological data and atmospheric dispersion models, radiocarbon data can be used to identify fossil-fuel emissions patterns from a local to a regional scale, across time.

The Radiocarbon Inventories of Switzerland (RICH) project aims to build the first database and model of the distribution and cycling of 14C at a national scale and across the atmosphere, soils, rivers and lakes of the country. The project presented here (RICH-Air) will serve to construct complementary monitoring and snapshots approaches of atmospheric 14CO2 measurement in this larger scope. For the monitoring aspect, air masses passing over Switzerland are collected and measured every two weeks at three tall tower sites situated over the populated Swiss plateau and one background site (Jungfraujoch). As for the snapshots, we focus on three industrial point sources (two cement plants, and a combined refinery-cement site) and use an Upwind-Downwind approach to have emissions and background samples at each site. As a complementary method, tree leaf samples will also be collected close to sites of interest, to have more temporally-integrated data.

First results show that the seasonality has a huge influence on the monitoring of the 14CO2 signature, with a decrease in the winter months, due to limited atmospheric mixing, and accumulation of ground emissions. For the industrial hotspots, plume catching was shown to be challenging, even though an increased signal of a few ppm was generally visible.

How to cite: Geissbühler, D., Laemmel, T., Gautschi, P., Wacker, L., and Szidat, S.: Following the temporal and spatial variability of atmospheric 14CO2 across Switzerland to estimate source contributions to the national CO2 emissions., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6154, https://doi.org/10.5194/egusphere-egu23-6154, 2023.

EGU23-6344 | Posters on site | AS3.22

The DLR project ELK: Mapping the global, regional and national emissions of transport 

Mattia Righi, Angelika Schulz, Johannes Hendricks, Simone Ehrenberger, Rainer Schmid, Daniel Krajzewicz, André Twele, Volker Matthias, and Markus Quante and the ELK Consortium

Transport and the related economic sectors contribute significantly to climate change. Emissions from these sectors are continuously growing, challenging the achievement of the Paris agreement. These sectors also have detrimental impacts on air quality and noise pollution. None of the currently available emission inventories can consistently account for the emissions (gas, particles and noise) of all transport modes (land transport, aviation, and shipping), while also considering the emissions from transport-related energy production, industrial processes and infrastructures. Moreover, most of the available inventories do not include information at subsector level, for example, they neither distinguish among different vehicle types nor consider key transport-related quantities other than emissions. However, emission inventories at such a level of detail are essential for a reliable quantification of the impact of transport at global, regional and national scales. In addition, consistent emission inventories are required for the development of future emission scenarios to assess the effectiveness of climate policies and other measures to improve air quality and to reduce noise pollution. To master this challenging task, the new strategic impulse project ELK – EmissionsLandKarte (en.: emission map) combines the interdisciplinary expertise of the German Aerospace Center (DLR) through a collaboration of 24 institutes and the Helmholtz-Zentrum Hereon. ELK aims to establish a primary source of information for different stakeholders and working groups, such as national policy makers, the scientific community dealing with climate, air quality and noise modelling, and the Intergovernmental Panel for Climate Change (IPCC). A collaborative and interdisciplinary approach is necessary in order to cover the wide spectrum of topics inherent to the compilation of emission inventories. This includes, for instance, transport demand, emission indices, and the development of models, together with dedicated methods for data visualization and management. The diversity of data sources and the heterogeneity of data formats from different sectors and data providers require the combination of different modelling tools and approaches, along with the use of measurements and satellite data. Available DLR data and data from external providers will be processed and used as input to quantify spatially and temporally resolved transport volumes and emission distributions. Based on already available inventories, precise criteria for the design of the ELK emission inventories will be defined and their quality and usability in real-world applications will be assessed. Finally, a database structure and user interface will be established to guarantee an easy and reliable access to the final products for both internal and external users. The ELK project links the aeronautics, space, transport and energy research programs of the DLR.

How to cite: Righi, M., Schulz, A., Hendricks, J., Ehrenberger, S., Schmid, R., Krajzewicz, D., Twele, A., Matthias, V., and Quante, M. and the ELK Consortium: The DLR project ELK: Mapping the global, regional and national emissions of transport, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6344, https://doi.org/10.5194/egusphere-egu23-6344, 2023.

EGU23-6978 | ECS | Posters on site | AS3.22

Using aircraft observations of atmospheric CO2 to evaluate vertical transport within the CarboScope Regional inverse model. 

Danilo Custódio, Saqr Munassar, Frank-Thomas Koch, Christian Rödenbeck, and Christoph Gerbig

This work was developed on the scope of the national initiative of the Integrated Greenhouse Gas Monitoring System for Germany – ITMS, which focus on reducing and characterizing uncertainties/errors introduced in the full retrieval chain of models, making use of observational data. 

Determining the magnitude, cause, and agents of carbon fluxes is important to advance our current understanding of the carbon budget and cycle, permitting more accurate predictions of its future behaviour. Sources and sinks of CO2at the Earth's surface can, in principle, be estimated from atmospheric concentrations by inverting atmospheric transport in the atmospheric tracer inversions.

Solving for CO2 fluxes in the inversions is highly desirable to better understand the carbon cycle but also to support policies aimed at reducing CO2 emissions. The Jena CarboScope inversion developed based on Bayesian inverse methods is used to obtain data-driven estimates of trace gas exchange, quantifying the large-scale sources and sinks of CO2.

To make Jena CarboScope estimates more reliable in understanding sources, sinks and transport of atmospheric CO2from the surface into the troposphere, the reliability of this data product should be evaluated based on independent observations. Quantifying the quality of the inversion estimation by decomposing the inherent uncertainty components is a challenging and key component in product reliability and its use. The overall objective in validating and evaluating uncertainties of the Bayesian data product provided by Jena CarboScope, is to explicitly answer the question: How good is the inversion estimation?

The assessment of these products is of special importance for further development and possibly allows for judging the trustworthiness of the inversion outcome.

This study explores the potential of CarboScope to reproduce CO2 concentrations recorded during regular flights and aircraft campaigns during the past two decades. The inversion estimations are accomplished by forward runs performed with the inversion having the measurement locations as receptors.

This study examines biases and uncertainties in the CarboScope estimations evaluated against flights’ data. It has been found that the CO2 simulated by CarboScope in the forward run (using the transport model TM3 for background concentration and STILT for regional signal) agree reasonably well, into the 10/90th percentile for 3-sigma of the distribution. On the other hand, the inversion exhibit some systematic biases at the edges of the distribution under and overestimating at high and lower mixing ratios, respectively. 

The CarboScope strength and concerns were enhanced by understanding the differences among observations and the inversion estimation. In comprehensive statistics comparing measurement data from hundreds of flights, we assess the compliance CarboScope`s CO2 estimation. Furthermore, we discuss the estimation and observation mismatches, exploiting the model constraints to reproduce atmospheric transport from the boundary layer to the upper troposphere. Understanding such constraints has the potential to reduce uncertainties of the atmospheric inversion estimates.

 

How to cite: Custódio, D., Munassar, S., Koch, F.-T., Rödenbeck, C., and Gerbig, C.: Using aircraft observations of atmospheric CO2 to evaluate vertical transport within the CarboScope Regional inverse model., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6978, https://doi.org/10.5194/egusphere-egu23-6978, 2023.

EGU23-7010 | ECS | Orals | AS3.22 | Highlight

Emissions of SF6 in China inferred from atmospheric observations 

Minde An, Ronald Prinn, Luke Western, Bo Yao, Jianxin Hu, and Matthew Rigby

Sulfur hexafluoride (SF6) is the most potent non-CO2 Greenhouse Gas currently incorporated in the Paris Agreement, with a global warming potential of around 25,000 over a 100-year time horizon and lifetime of around 1,000 years. Global mole fractions and emissions of SF6 have increased substantially since the 2000s. The increasing SF6 emissions worldwide are thought to originate from its growing emissions in Kyoto Protocol non-Annex-I countries, where China is a major contributor. 

Top-down emission estimates provide evaluation of national bottom-up inventories, based on information from atmospheric observations. Previous top-down emissions of SF6 in China were determined by observations made outside of China (e.g., in Korea and Japan), which lack sensitivity to emissions in regions far from the measurement sites (like the western or southern parts of China). In this study, emissions of SF6 in China over 2011-2020 were derived using observations of SF6 from 9 sites within China, coupled with a Lagrangian transport model and a hierarchical Bayesian inference algorithm. Analysis of the sensitivity maps (footprints) of these measurement sites suggest broad sensitivity to the major emission areas in China. The emissions in China show a substantial increase throughout the study period and contribute substantially to the rise in global emissions. The spatial distribution of SF6 emissions in different regions or provinces in China and their changes are further analyzed. Finally, the potential industrial drivers behind the changes in emissions in China, and the necessity of continuous atmospheric observations in some key regions like in the northwest of China are discussed.

How to cite: An, M., Prinn, R., Western, L., Yao, B., Hu, J., and Rigby, M.: Emissions of SF6 in China inferred from atmospheric observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7010, https://doi.org/10.5194/egusphere-egu23-7010, 2023.

EGU23-7658 | ECS | Orals | AS3.22

Cross-verification of local inventory CO2 emissions and tall tower eddy covariance fluxes measurements in Vienna 

Enrichetta Fasano, Bradley Matthews, Francesco Vuolo, and Helmut Schume

Curbing carbon dioxide (CO2) emissions from cities is critical for climate change mitigation given the substantial urban contribution to global anthropogenic greenhouse gas (GHG) emissions. Despite relatively robust inventory estimates of total urban CO2 emissions at regional and global scales, emission inventories at the level of individual cities can be very uncertain due to unavailability of input data and/or uncertainties in downscaling aggregated statistics or emissions. A growing field of research is thus investigating the application of atmospheric measurement and modelling to support CO2 emissions monitoring in cities. Here we present ongoing research comparing local emission inventories of the city of Vienna, Austria with tall tower eddy covariance measurements of CO2 fluxes. In contrast to inverse modelling methods, eddy covariance allows net surface emissions to be directly inferred from the  measured vertical turbulent fluxes in the surface layer above cities. For this analysis local emission inventories were processed with external data (e.g., measurements of local traffic counts and air temperature, proxies from literature) to produce temporally-resolved emissions maps (hour-hectare resolution) from the annual, aggregate inventory estimates for the years 2018 to 2020. For the comparison with the flux measurements, these emission maps were cropped after overlapping these layers with an average flux footprint calculated from flux measurements made during northwesterly flows, when the most densely inhabited districts of the city were sampled. On an annual scale, the flux measurements and inventory estimates of total CO2 emissions agree well with one another. Furthermore, encouraging results were obtained when comparing annual space-heating and traffic emissions from the inventories with respective estimates derived from regression analyses of the eddy fluxes against local air temperature and traffic counts. At sub-annual scales, seasonal and hourly divergences between the inventories and the eddy covariance measurements were indicative of boundary layer dynamics (decoupling between turbulent exchange and fluxes at the surface) as well as a seasonal influence of urban vegetation on net CO2 fluxes.

How to cite: Fasano, E., Matthews, B., Vuolo, F., and Schume, H.: Cross-verification of local inventory CO2 emissions and tall tower eddy covariance fluxes measurements in Vienna, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7658, https://doi.org/10.5194/egusphere-egu23-7658, 2023.

EGU23-7711 | ECS | Posters on site | AS3.22

User-oriented development of global emission inventories: Bottom-up modeling of emissions from land transport, aviation and shipping in the DLR project ELK 

Jens Hellekes, Simone Ehrenberger, Nina Thomsen, Sabine Brinkop, Johannes Hendricks, Christian Weder, Paweł Banyś, Isheeka Dasgupta, Mario Feinauer, Manuel Löber, Tobias Schripp, Mattia Righi, and Angelika Schulz

The transport sector accounts for about one quarter of worldwide anthropogenic carbon dioxide emissions. Since a robust growth in transport activity is expected over the coming decades, reducing associated emissions to mitigate human-caused climate change is a particular challenge. In order to achieve high-quality comparative monitoring, to develop scenarios for future emissions, and to enable a robust assessment of climate protection measures, the allocation of emissions to the subsector level is a necessary prerequisite. The DLR project ELK – EmissionsLandKarte (en.: emission map) contributes here in several respects: (1) requirements are specified in an application-based manner, i.e. compatibility with existing inventories, such as the ones generated for IPCC, is ensured and insufficiencies in spatial resolution and methodological detail are addressed, (2) an input database congruent with both statistical data and SSP scenarios is provided, and (3) bottom-up calculations are performed that allow attribution of climate impacts to specific transport services, as well as prospective analyses where, for example, activity levels change or alternative fuels affect regional emission factors. The resulting prototype global gas and particle emission inventories for land transport, aviation and shipping reflect the status quo as of 2019.

For land transport, fine-grained activity and vehicle fleet data as well as technology-specific emission factors are applied. This allows emissions from passenger and freight transport to be disaggregated by mode and vehicle type. New approaches for spatial disaggregation of emissions will increase transparency of the methodology. For aviation, calculations are based on fleet composition and transport performance for both passenger and cargo traffic at the airport pair level, while real flight tracks serve as the foundation for spatial allocation. For both transport sectors, complementary analyses are performed to characterize particulate emissions in order to fill gaps in data availability. For shipping, transport performance on inland waterways and maritime routes are considered, including technical data describing propulsion and bunkering. Finally, all mode-specific results are subjected to an innovative uncertainty assessment aligned with the needs of other emission inventory creators through a detailed evaluation per uncertainty factor, as well as aggregated values for climate modelers and practitioners. The consistent assessment of uncertainty factors along the entire calculation chain, such as activity levels, emission factors, and proxy data used for spatial or temporal disaggregation, promotes comparability across all transport sectors. In this paper, we outline the new methodological approaches for mapping transport emissions and present first results.

How to cite: Hellekes, J., Ehrenberger, S., Thomsen, N., Brinkop, S., Hendricks, J., Weder, C., Banyś, P., Dasgupta, I., Feinauer, M., Löber, M., Schripp, T., Righi, M., and Schulz, A.: User-oriented development of global emission inventories: Bottom-up modeling of emissions from land transport, aviation and shipping in the DLR project ELK, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7711, https://doi.org/10.5194/egusphere-egu23-7711, 2023.

EGU23-7757 | Orals | AS3.22

Inclusion of additional data streams within atmospheric inverse modelling systems: first results from ITMS 

Christoph Gerbig, Frank-Thomas Koch, Saqr Munassar, Danilo Custodio, Michal Galkowski, and Christian Rödenbeck

Within the Integrated Greenhouse Gas Monitoring System for Germany (ITMS), a national initiative targeted at the provision of estimates of GHG fluxes for Germany, the CarboScope-Regional (CSR) inversion system operated at the MPI-BGC is envisioned as a back-bone and reference system for future developments using the ICON-ART modelling system at the German Weather Service (DWD). It utilizes ICOS atmospheric observations

Additional focus of the research involving CSR is the evaluation and improvement of vertical transport in atmospheric models, as well as the inclusion of additional data streams (e.g. vertical profile information) to improve both, GHG flux estimates and their uncertainty characterization. In this context, the assessment of mixing heights as represented within CSR against independent information derived from radiosondes over a timespan of more than a decade has revealed problems vertical mixing during wintertime that have the potential to cause biased flux retrievals. First results related to this and other experiments will be presented.

How to cite: Gerbig, C., Koch, F.-T., Munassar, S., Custodio, D., Galkowski, M., and Rödenbeck, C.: Inclusion of additional data streams within atmospheric inverse modelling systems: first results from ITMS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7757, https://doi.org/10.5194/egusphere-egu23-7757, 2023.

EGU23-8067 | Posters on site | AS3.22

Fossil fuel CO2 emission signatures over India captured by OCO-2 satellite measurements 

Jia Chen and Vigneshkumar Balamurugan

Recent developments in space-based measurements provide new possibilities for monitoring greenhouse gas (GHG) emissions at all scales, from global to local. We traced CO2 emission sources such as power plants over India using OCO-2 satellite measurements from 2014 to 2021. India is the third-largest CO2 emitter in the world, with coal accounting for nearly 60% of total fossil fuel combustion.

The Gaussian plume model was used to assess the power plant emissions. Cross-sectional (c/s) CO2 emission flux is estimated to validate the results. In 13 out of 26 cases, the estimated power plant CO2 emissions agreed within ± 25% of the emissions reported in the Carbon Brief (CB) database, and in 21 cases, the estimated emissions are within ± 50%. There is one case where the CB database significantly overestimated the CO2 emission for power plants. Further, in two cases, in which the Gaussian plume model gives much higher estimated CO2 emissions, there are emission sources other than the power plants in the vicinity. The c/s emission flux and emission inventories can be used to confirm such cases. 

In addition, the c/s emission flux method was employed to assess the emissions reported in the EDGAR and ODIAC CO2 emission inventories. Our study demonstrated the capability of OCO-2 to uncover missing or underestimated CO2 emission sources in emission inventories. Our approach could be a vital tool to conduct an initial estimate of missing or underestimated sources in the databases and emission inventories at various scales, as c/s emission flux estimation and Gaussian plume model require less computation than other modeling approaches. More sophisticated methods, such as Bayesian inversion combined with extensive transport modeling, can then be used to derive emissions with less uncertainty. Future satellites with high spatio-temporal resolution and coverage (e.g., Microcarb, Tansat2, CO2M) will enhance the possibilities of continuous monitoring of point sources as well as detecting missing or underestimated emission sources. 

How to cite: Chen, J. and Balamurugan, V.: Fossil fuel CO2 emission signatures over India captured by OCO-2 satellite measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8067, https://doi.org/10.5194/egusphere-egu23-8067, 2023.

EGU23-9456 | ECS | Orals | AS3.22

Carbon Monitor AutoForecast-Asia: a real-time emission estimates of the residential sector for Asian major emitters with an automatic machine learning framework  

Taochun Sun, Yuanhao Geng, Rohith Teja Mittakola, Jinpyo Hong, Zhongyan Li, Xuanren Song, Da Huo, Zhu Deng, Lixing Wang, Chenxi Lu, and Zhu Liu

Carbon monitoring is crucial for mitigating urban climate change and expediting urban responses to emission changes. This requires monitoring and reporting emissions on a timely basis. However, existing inventories mainly consider scope-1 (in boundary emissions) with a time lag of more than 2 years. The Carbon Monitor (carbonmonitor.org) and the following Carbon Monitor Cities (cities.carbonmonitor.org) project thus developed the near-real-time (NRT) inventories for the global high emitters worldwide at the country level and city level, pushing forwards the efforts of global NRT monitoring in an around time lag of 3 months to ensure the unprecedented timeliness of carbon data. However, the immediate monitoring of emissions in more rapid governmental responses and short-term future policy design is still urgently needed in the future, especially for getting real-time estimates of major emitters by developing the “nowcasting” and even forecasting framework. We choose the residential sector as the initial exploration of this kind given the sectoral characteristics of Asian big emitters, including China, Japan, and India.

By developing an automatic machine learning ensemble framework (Carbon Monitor AutoForecast-Asia), we essentially achieve the nowcasting from the perspective of city-level emission dynamics. Specifically, this framework utilizes data from multiple sources, including the Carbon Monitor datasets, Carbon Monitor Cities datasets, and the ERA5 reanalysis datasets. Time-series and tree-based models are incorporated into the entire framework with automatic finetuning pipelines, as well as designed algorithms for capturing the seasonalities of daily emissions, and the holiday impacts as demonstrated in our previous studies. We use the Carbon Monitor and the Carbon Monitor Cities datasets up to the end of 2021 to train and test the entire framework by parallelizing the framework of more than 400 cities for acceleration. After running correction models to reduce the induced uncertainties from the Carbon Monitor to the Carbon Monitor Cities, we get the R squared metrics of 0.95, 0.94, 0.97 for China, India, and Japan respectively at the country level. Note that, we use the Carbon Monitor data from 2022.1.1 to the latest for comparisons in this procedure, and the framework could nowcast the residential emissions in the time lag of 1 week.

Subsequently, deep learning-based models (i.e., LSTM) are used as the baselines with the same configurations (i.e., train and test splits) and we find that the ensemble results could outperform the baseline models in terms of common metrics, including MAE, MSE, RMSE, MAPE. This suggests that the real-time estimates of emissions may depend on more complicated ensemble methods rather than the deep learning models due to the trade-off between the small volume of near-real-time data and the complex patterns of daily emissions.

In the future, we may include more high emitters globally by extending the developed framework to at least satisfy the needs of real-time and even future estimates of the residential sector.

 

 

How to cite: Sun, T., Geng, Y., Teja Mittakola, R., Hong, J., Li, Z., Song, X., Huo, D., Deng, Z., Wang, L., Lu, C., and Liu, Z.: Carbon Monitor AutoForecast-Asia: a real-time emission estimates of the residential sector for Asian major emitters with an automatic machine learning framework , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9456, https://doi.org/10.5194/egusphere-egu23-9456, 2023.

EGU23-9934 | Posters on site | AS3.22

Deep learning based XCO2 global map generation using satellite observations 

Yeji Choi and Eunbin Kim

Greenhouse (GHG) gases are the primary driver of climate change. There are two approaches to measuring GHG emissions: bottom-up and top-down. Bottom-up measurement involves collecting data based on local emissions and modeling individual sources and sinks of carbon. This is useful for understanding the specific drivers of GHG emissions; however, there is a time lag for collecting data from each source, and good national statistics are required. Meanwhile, top-down measurement involves estimating GHG emissions based on atmospheric measurements and modeling. In general, the bottom-up approach is considered to be more accurate than the top-down approach, but the top-down approach is helpful for providing broad-scale estimates of GHG emissions, and it allows for spatial mapping on a global scale.

In this study, we use OCO-2 satellite products to generate a XCO2 global map using a deep-learning-based technique. Although OCO-2 measurement provides the CO2 concentrations with the highest spatial resolution on a global scale, there are limitations to the FOV coverage and the low temporal resolution of the low-earth orbit satellite. To solve this problem, we use additional satellite products, which can be a precursor to CO2, and we applied TabNet which is firstly introduced at the International Conference on Machine Learning (ICML) 2020. TabNet is an attention-based network that uses a self-attention mechanism. The preliminary results showed that the XCO2 global map for every half of the month could be provided using integrated satellite observations. The validation results will be discussed in the presentation.

How to cite: Choi, Y. and Kim, E.: Deep learning based XCO2 global map generation using satellite observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9934, https://doi.org/10.5194/egusphere-egu23-9934, 2023.

Seabeds are a geological source for methane via natural release at seeps, dispersive methanogenic degradation of sedimentary organic matter as well as anthropogenic well leakage. Global estimates of methane seepage fluxes vary around severals tens of Tg/y. The associated release to the atmosphere is lowered by attenuation in the water column. Large uncertainties are associated with these figures as emphasized by the researchers that performed these investigations. 
Our goal is to investigate which quantitative data is available on both natural seepage and anthropogenic well leakage and which unknowns emerge from this for upscaling to regional basin scale and beyond. We focused on the Gulf of Mexico (GoM) and the North Sea basin (NSB) as these are relatively well studied marine areas.
For the two areas together, the number of quantitative studies on natural seepage is about 30 for seabed fluxes and 6 for sea/air emissions. One unknown that emerges is what flux data should be used for further upscaling: that from the studied region or from a global data-set as done before? The population statistics are different for the two. Another unknown for GoM is the fate of methane released at deep seeps (> 500 m below sea surface) that dissolves in seawater and does not reach the sea surface (as bubbles): does it get oxidised, does it interfer with biological methane, does it stay dissolved at large depth? Several quantitative studies focus on the bubble fluxes and neglect mass transport of dissolved methane. How justified is this when we recall that methane from rising bubbles dissolves into surrounding seawater and incidental storms mix seawater at shallow depth enabling transfer to air.
Globally, most (quantitative) studies on natural seepage happened at the Northern hemisphere. Natural seeps are commonly found in oil and gas producing basins and oil and gas exploration in several basins at the Southern hemisphere has been performed only recently. This means that natural seepage at such basins is probable as well but has been neglected so far. This puts another unknown forward.
The emission related to exploitation and transport of fossil fuels is a major, global anthropogenic source. For onshore wells, the contribution of subsurface leakage has obtained large attention in the past years with considerable numbers of local to national investigations. However, the contribution is far from clear for offshore wells whereas offshore wells may show more frequent well integrity issues as well as barrier integrity issues. Two blowouts have been studied in detail: the Deep Water Horizon blowout in GoM that was capped after 84 days and the UK22/4b blowout in NSB that is continuously leaking since 1990. Additionally, methane fluxes at three leaking, abandoned Norwegian wells were quantified. The data gap for GoM and NSB as well as globally will be illustrated taking into account data on well integrity issues and blowouts.
In conclusion, several major unknowns exist on methane fluxes associated with natural seeps and anthopogenic well leakage. These should be addressed to further constrain their contribution to the global methane budget.

How to cite: Griffioen, J., Geel, K., and Koning, M.: Identifying known unknowns in estimating regional methane fluxes from natural seeps and anthropogenic well leakage in the marine environment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9953, https://doi.org/10.5194/egusphere-egu23-9953, 2023.

EGU23-10282 | ECS | Posters on site | AS3.22

CO2 gradients and variability in Mexico City from in situ measurements and simulations 

Sandra Porras, Eugenia González del Castillo, Omar López, Thania Arredondo, José Agustín García-Reynoso, Olivier Laurent, Michel Ramonet, Marc Delmotte, and Michel Gutter

Emission inventories are the primary source of information regarding the spatial and temporal distribution of CO2 sources and sinks in urban environments. In most cities around the world, the impact of mitigation strategies is evaluated conventionally through an inventory methodology which -by nature- is subject to high uncertainties.  In this work, we report on the utility of deploying a small network of medium-cost, non-dispersive infrared (NDIR) CO2 microsensors in Mexico City, to directly quantify the gradients and variability of the molar fraction of atmospheric CO2. The measurements obtained were compared with simulations of a high-resolution 3D transport model (WRF-Chem), prescribed with city-scale, inventory-based CO2 emission maps. The focus of this presentation is on the description of the sensors construction, the characterization of each individual sensor’s performance evaluated against a reference instrument, and the ability of the network to represent the spatial and temporal variability of CO2 in a complex urban environment. Preliminary results of a multivariate calibration of the medium-cost microsensors using a Picarro G2401 as reference instrument, along with air temperature, relative humidity and pressure, results in RMSE ranging from 1 to 5 ppm of CO2. We discuss the potential that this network of sensors offer to evaluate whether the distribution of sources and sinks declared in an inventory can result in the variability of concentrations of CO2 measured in the atmosphere, and the possibility of being used as a tool to incorporate the contribution of out-of-city emissions or mobile sources emissions, currently not accounted for in the inventory.

How to cite: Porras, S., González del Castillo, E., López, O., Arredondo, T., García-Reynoso, J. A., Laurent, O., Ramonet, M., Delmotte, M., and Gutter, M.: CO2 gradients and variability in Mexico City from in situ measurements and simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10282, https://doi.org/10.5194/egusphere-egu23-10282, 2023.

EGU23-10367 | Orals | AS3.22 | Highlight

Trend and seasonal cycle of US methane emissions 

Lei Hu, Arlyn Andrews, Stephen Montzka, Ed Dlugokencky, Scot Miller, Sergio Ibarra-Espinosa, Colm Sweeney, Lori Bruwhiler, Natasha Miles, and Kenneth Davis

Methane is a major greenhouse gas (GHG) that has contributed to one third of the warming induced by all GHGs since the preindustrial era (IPCC, 2021).  Reliable quantification of methane emissions is critical for tracking progress towards methane mitigation, especially for the countries that join the Global Methane Pledge and that have firm plans for reducing methane emissions over the next decades, such as the US.  In this study, we quantified US methane emissions using inverse modeling of ground- and airborne- methane measurements made from the NOAA Greenhouse Gas Reference Network for 2007 – 2021. We conducted 12 inversion runs using two high-resolution transport models (HYSPLIT-NAMs and WRF-STILT), three background estimates, and two prior emission fields.  Multiple estimates of wetland emissions were considered and subtracted from our inversion-derived total emission estimates.  Our derived anthropogenic emissions show a consistent increasing trend after 2015 across our inversion ensemble members and a seasonal cycle in emission magnitude that repeats every year during our study period.  Both the trend and seasonal variation seem to correlate with US natural gas consumption.  A similar seasonal variability has been reported previously, but only on an urban scale; this is the first time it has been derived on a national scale.  Furthermore, we also compared our estimates with US EPA’s national GHG inventory reporting and investigated the impact of the COVID-19 pandemic on emissions in 2020 relative to 2019 and 2021.    

How to cite: Hu, L., Andrews, A., Montzka, S., Dlugokencky, E., Miller, S., Ibarra-Espinosa, S., Sweeney, C., Bruwhiler, L., Miles, N., and Davis, K.: Trend and seasonal cycle of US methane emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10367, https://doi.org/10.5194/egusphere-egu23-10367, 2023.

EGU23-10545 | ECS | Posters virtual | AS3.22

Quantification and Evaluation of OCO-2 measured XCO2 against COCCON 

Saswati Das, Matthäus Kiel, Joshua Laughner, Vivienne Payne, and Gregory Osterman

Carbon dioxide (CO2) is the primary greenhouse gas emitted from anthropogenic activities. Although it is naturally present as a part of Earth’s carbon-cycle, human activities influence the ability of natural sinks to reduce CO2 from the atmosphere, thus altering the carbon-cycle and necessitating the long-term monitoring of atmospheric CO2. Precise, accurate and continuous measurements of CO2 are important to this end.

The Orbiting Carbon Observatory-2 (OCO-2) was launched in 2014. It is NASA’s first Earth-orbiting satellite dedicated to making observations of CO2 in the atmosphere and measuring its column-averaged dry-air mole fraction (XCO2). The primary goal of the OCO-2 mission is to provide XCO2 measurements with sufficient precision and accuracy alongside quantifying its seasonal and interannual variability. In this study, we use the new and improved OCO-2 B11 data set.

In the past, the space-based XCO2 measurements from OCO-2 data have been validated against independent data sets such as the Total Carbon Column Observing Network (TCCON). In this study, we use independent measurements from the COllaborative Carbon Column Observing Network (COCCON) to identify potential biases and errors in the B11 data version and establish its robustness for use by the science community. COCCON uses portable Fourier-Transform InfraRed (FTIR) spectrometers (EM27/SUN) to measure greenhouse gases at several global sites.  

Comparison of OCO-2 measurements against COCCON sites indicate similar temporal trends in XCO2 variability, with OCO-2 typically reporting higher values. Further, we evaluate the differences between the B11 OCO-2 and COCCON data sets. Finally, we analyze how OCO-2’s B11 version compares to selected COCCON and TCCON sites’ measurements in terms of capturing the seasonal cycle and growth rate of XCO2.

How to cite: Das, S., Kiel, M., Laughner, J., Payne, V., and Osterman, G.: Quantification and Evaluation of OCO-2 measured XCO2 against COCCON, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10545, https://doi.org/10.5194/egusphere-egu23-10545, 2023.

EGU23-10615 | Posters on site | AS3.22

Evaluation of the OCO-2 and OCO-3 ACOS data products against TCCON 

Matthäus Kiel, Saswati Das, Gregory Osterman, Joshua Laughner, Vivienne Payne, and Abhishek Chatterjee

The Orbiting Carbon Observatory-2 (OCO-2), launched in 2014, is NASA’s first satellite dedicated to measure sources and sinks of carbon dioxide (CO2) in Earth’s atmosphere on regional scales. Since 2019, measurements from the Orbiting Carbon Observatory-3 (OCO-3) have complemented OCO-2’s data record. In addition, OCO-3’s Snapshot Area Mapping (SAM) mode observations over emission hotspots like cities, power plants, and volcanoes provide a novel data set for carbon cycle studies on local scales. Data from both instruments are analyzed with the Atmospheric Carbon Observations from Space (ACOS) retrieval algorithm to estimate column-average dry-air mole fractions of carbon dioxide (XCO2) in Earth’s atmosphere. Evaluating these space-based estimates of XCO2 against independent validation data sets provides information about the quality, potential biases, and errors in the OCO-2/3 data record. Here, we present comparisons of the ACOS V10 XCO2 from OCO-3 and the new and improved ACOS V11 XCO2 from OCO-2 against ground-based measurements from the Total Carbon Column Observing Network (TCCON).

For both instruments, the root-mean-square error (RMSE) is below 1 ppm for all observational modes when compared to collocated TCCON observations. The OCO-3 V10.4 data version, an improvement over the initial vEarly data version, reduces an XCO2 time-dependent bias that was present in the previous OCO-3 data record. Consequently, data from both instruments does not indicate any significant time-dependent bias over the span of several years. Further, we evaluate differences between OCO-3 and TCCON related to different local overpass times. On average, OCO-3’s equator crossing time occurs about 20 minutes earlier every day. Comparisons against TCCON indicate no significant local time of day bias in the OCO-3 XCO2 data, however, comparisons over individual TCCON sites indicate a dependence which provides insight into potential airmass and viewing geometry related biases. The improved OCO-2 V11 data version reduces the mean bias against TCCON to ~0.15ppm from previously ~0.4ppm in V10. We find the largest reduction in RMSE over ocean due to an improved ocean glint surface treatment in V11. Both OCO data products are of comparable quality and are an improvement over earlier OCO data versions. Finally, we analyze how well OCO-2 captures the mean seasonal cycle amplitudes and growth rates over selected TCCON sites.

How to cite: Kiel, M., Das, S., Osterman, G., Laughner, J., Payne, V., and Chatterjee, A.: Evaluation of the OCO-2 and OCO-3 ACOS data products against TCCON, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10615, https://doi.org/10.5194/egusphere-egu23-10615, 2023.

EGU23-10659 | Orals | AS3.22 | Highlight

Observed changes in China’s methane emissions linked to policy drivers 

Yuzhong Zhang, Shuangxi Fang, Jianmeng Chen, Yi Lin, Yuanyuan Chen, Ruosi Liang, Ke Jiang, Robert J. Parker, Hartmut Boesch, Martin Steinbacher, Jian-Xiong Sheng, Xiao Lu, Shaojie Song, and Shushi Peng

China is set to actively reduce its methane emissions in the coming decade. A comprehensive evaluation of the current situation can provide a reference point for tracking the country’s future progress. Here, using satellite and surface observations, we quantify China’s methane emissions during 2010–2017. Including newly available data from a surface network across China greatly improves our ability to constrain emissions at subnational and sectoral levels. Our results show that recent changes in China’s methane emissions are linked to energy, agricultural, and environmental policies. We find contrasting methane emission trends in different regions attributed to coal mining, reflecting region-dependent responses to China’s energy policy of closing small coal mines (decreases in Southwest) and consolidating large coal mines (increases in North). Coordinated production of coalbed methane and coal in southern Shanxi effectively decreases methane emissions, despite increased coal production there. We also detect unexpected increases from rice cultivation over East and Central China, which is contributed by enhanced rates of crop-residue application, a factor not accounted for in current inventories. Our work identifies policy drivers of recent changes in China’s methane emissions, providing input to formulating methane policy toward its climate goal.

How to cite: Zhang, Y., Fang, S., Chen, J., Lin, Y., Chen, Y., Liang, R., Jiang, K., Parker, R. J., Boesch, H., Steinbacher, M., Sheng, J.-X., Lu, X., Song, S., and Peng, S.: Observed changes in China’s methane emissions linked to policy drivers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10659, https://doi.org/10.5194/egusphere-egu23-10659, 2023.

EGU23-10714 | Orals | AS3.22 | Highlight

Making best use of atmosphere- and inventory-based approaches for quantifying and understanding emissions of greenhouse gases and ozone-depleting substances on a range of spatial scales. 

Stephen Montzka, Lei Hu, Phil DeCola, Dave Godwin, Isaac Vimont, Bart Croes, Toshi Kuwayama, Geoff Dutton, David Nance, Brad Hall, Colm Sweeney, and Arlyn Andrews

The likelihood for successful emission control and mitigation efforts of trace gases having adverse environmental effects can be enhanced by using a multi-faceted framework for quantifying and understanding emissions. While bottom-up activity-based inventories provide a quantification of various source sectors, appropriately designed atmosphere-based (top-down) approaches are able to independently evaluate the inventory and further refine temporal changes and spatial distributions.  Differences between bottom-up and top-down estimates are oftentimes observed and represent prime opportunities for increasing understanding and refining estimates of emissions.  Here we will present results derived from atmospheric observations made in the remote global atmosphere as well as from our North American measurement network.  The remote global observations enabled the identification of an apparent violation of the Montreal Protocol.  After our atmospheric measurements identified this unexpected issue, fairly quick resolution appears to have been achieved, in part due to the additional understanding of likely underlying causes provided by industry experts. Our North American measurement network also allows for trace-gas emission estimates on national and state scales.  Results from these efforts will be discussed, with an emphasis on describing how the interaction between inventory-derived and atmosphere-based information has led to an improved understanding of emission magnitudes along with identifying areas needing additional study.

How to cite: Montzka, S., Hu, L., DeCola, P., Godwin, D., Vimont, I., Croes, B., Kuwayama, T., Dutton, G., Nance, D., Hall, B., Sweeney, C., and Andrews, A.: Making best use of atmosphere- and inventory-based approaches for quantifying and understanding emissions of greenhouse gases and ozone-depleting substances on a range of spatial scales., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10714, https://doi.org/10.5194/egusphere-egu23-10714, 2023.

EGU23-10805 | Orals | AS3.22 | Highlight

A WMO-coordinated Global Greenhouse Gas Monitoring Infrastructure 

Lars-Peter Riishojgaard

Beyond water vapor, the three most important greenhouse gases (GHGs) in terms of their radiative forcing are carbon dioxide (CO2), methane (CH4), and nitrous oxide (N2O). Increasing concentrations of these gases driven by human activities are the primary cause of the observed climate change according to the Intergovernmental Panel on Climate Change (ref AR6 WG1). The Paris Agreement, adopted by 196 countries at the UNFCCC Conference of the Parties in 2015, sets specific targets for maximum rise in global mean temperature and identifies reduction in net greenhouse emissions as the primary means to achieve this target.
However, even very accurate estimates of anthropogenic emissions alone will not be enough to design meaningful mitigation efforts or to monitor their effectiveness. Greenhouse gas concentrations are influenced by both natural and anthropogenic processes, and some of the natural carbon sources and sinks in particular are associated with very large uncertainties, both as they currently operate and as they may change in the future in response to climate change. 
Sustained, routine monitoring of greenhouse gas concentrations, using monitoring of weather and climate as a paradigm and role model, will provide a wealth of quantitative data to help constrain the modelling of all parts of the carbon cycle. This will be extremely valuable for the work of the World Climate Research Programme (WCRP) and IPCC, it will complement and supplement existing methodologies used to estimate anthropogenic emissions, and it will help put mitigation steps taken by Parties to the Paris Agreement on a solid scientific footing. 
This presentation introduces a WMO-coordinated effort to establish an operational Global Greenhouse Monitoring Infrastructure to directly observe and model greenhouse gas concentrations in the atmosphere, and thereby support/enable estimates of net greenhouse gas fluxes between atmosphere, land, and oceans. The atmospheric component of this infrastructure builds on the research infrastructure for greenhouse gas observations and modelling supported by WMO since 1975, and promotes its operationalization and further advancement by utilizing the existing infrastructure and methodologies employed for more than 50 years for operational weather forecasting. 

How to cite: Riishojgaard, L.-P.: A WMO-coordinated Global Greenhouse Gas Monitoring Infrastructure, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10805, https://doi.org/10.5194/egusphere-egu23-10805, 2023.

EGU23-10862 | Posters on site | AS3.22 | Highlight

US National Academy report on Greenhouse Gas Information for Decision Making 

kevin gurney, Don Wuebbles, Kamal Bawa, gabrielle Dreyfus, Annmarie Eldering, fiji george, heather graven, angel Hsu, Tomohiro Oda, Irene Xueref-Remy, Rachel Silvern, Amanda Stoudt, Bridget McGovern, and Patricia Razafindrambinina

The National Academy of Sciences convened a committee to generate a report titled “Development of a Framework for Evaluating Global Greenhouse Gas Emissions Information for Decision Making”. The report:

 

  • Described approaches used to develop global anthropogenic greenhouse gas emissions inventories, including the use of surveys
  • Discussed the potential uses and limitations of these approaches
  • Provided a framework to evaluate emissions information and inventories
  • Presented several case studies to demonstrate how the framework could be applied to evaluate emissions information and inventory approaches and identify strengths and opportunities for improvement for each case study.
  • Identified ways to improve methodological transparency, sustainability and continuity of relevant observations, and product confidence in global anthropogenic greenhouse gas emissions inventories

 

To accomplish this the committee identified a series of “pillars” that were deemed ideal characteristics of GHG inventories for decisionmaking. Three dominant GHG inventory development approaches were identified from the existing work and ranked within the series of pillars. The committee made a series of recommendations for continued development of inventories to enhance their quality and utility to decisionmakers.

In this presentation I will describe the major content of the report, describing the evaluation matrix and a summary of the committee’s recommendations.

How to cite: gurney, K., Wuebbles, D., Bawa, K., Dreyfus, G., Eldering, A., george, F., graven, H., Hsu, A., Oda, T., Xueref-Remy, I., Silvern, R., Stoudt, A., McGovern, B., and Razafindrambinina, P.: US National Academy report on Greenhouse Gas Information for Decision Making, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10862, https://doi.org/10.5194/egusphere-egu23-10862, 2023.

EGU23-10863 | Orals | AS3.22 | Highlight

The role(s) of remote sensing in reducing methane emissions 

Riley Duren, Daniel Cusworth, Frances Reuland, Andrew Thorpe, Alana Ayasse, and Deborah Gordon

Success in achieving the methane emission reduction targets of industry, national and subnational governments, the Paris agreement, and Global Methane Pledge will critically depend on access to emissions data that is actionable, complete and trustworthy. Despite recent improvements, current methane monitoring systems are still limited in their ability to offer timely delivery of precise, quantitative, and reproduceable emissions data to facility operators, regulators, front-line communities and other stakeholders. There are multiple use-cases for accelerating data-enabled methane mitigation including but not limited to leak detection and repair programs, diagnostics to guide process emission reductions and infrastructure model improvements, emissions trending, and supply-chain methane intensity certification. Each use-case translates to specific requirements on methane data products and the observational and analytic frameworks that deliver them. Meanwhile, a nascent global system of systems for operational methane emissions monitoring is emerging that offers the potential to synergistically combine observations from multiple sensor types, vantage points, and quantification methods.  Additionally, new programs offering improved data access, transparency, independent validation, 3rd party reporting, and user capacity-building are also gaining traction.

Remote sensing offers unique contributions to the expanding methane tiered observing system. Satellites in particular can complement continuous data from surface sensors at selected facilities and periodic regional airborne surveys by providing dense and sustained sampling of diverse jurisdictions globally without being constrained by access restrictions. We discuss use-cases for regional- to facility-scale monitoring and challenges in scaling up methane remote sensing systems for sustained operational decision support. We also present pilot studies involving collaborative data sharing between researchers, regulators and facility operators that resulted in measurable and verifiable emission reductions.

How to cite: Duren, R., Cusworth, D., Reuland, F., Thorpe, A., Ayasse, A., and Gordon, D.: The role(s) of remote sensing in reducing methane emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10863, https://doi.org/10.5194/egusphere-egu23-10863, 2023.

India needs a high-resolution estimation of carbon sources and sinks to implement the country’s climate change action plans and mitigation strategy effectively. Current carbon estimates over the Indian region based on the “Bottom-up” approach suffer from significant uncertainty, which calls for more process-based models and atmospheric inverse modelling to obtain a more accurate budget. Inverse models constrain the carbon fluxes based on atmospheric observation of CO2 mole fractions. The unavailability of amble observations over the Indian domain critically impacts estimation accuracy. Fortunately, there are increasing efforts to improve the availability of CO2 observation over the domain. Along with the observations, the availability of a suitable transport model to simulate the CO2 distribution is essential to the accurate inverse estimation of carbon fluxes. The inability of coarse-resolution global models to simulate the fine-scale variability in CO2 distribution warrants developing a regional high-resolution modelling system. Here we evaluate the performance of a regional high-resolution modelling system which utilises meteorological fields from the Weather Research and Forecasting (WRF) model to simulate the CO2 transport over the Indian domain using a lagrangian particle dispersion model, Stochastic Time-Inverted Lagrangian Transport Model (STILT). Using lagrangian models enables us to study the CO2 distribution at very high resolution (even at sub-grid scale) with reduced cost. We use the vegetation photosynthesis and Respiration Model (VPRM), coupled with the modelling system, to simulate the biospheric fluxes. The anthropogenic and biomass burning fluxes are obtained from different available inventories. We use CO2 in-situ observations from different parts of the Indian domain, which utilises flask measurements and PICARRO CRDS instruments, to evaluate the modelling system. Our high-resolution modelling framework shows good skill in simulating the CO2 variability over the region. The results of the evaluation will be discussed in detail during the presentation.

How to cite: Thilakan, V., Pillai, D., and S Kumar, J.: Evaluation of the performance of regional transport models in simulating CO2 variability over India employing WRF-STILT modelling framework, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10975, https://doi.org/10.5194/egusphere-egu23-10975, 2023.

EGU23-11169 | Orals | AS3.22

Building and road segment scale fossil fuel CO2 emissions estimation across multiple US cities spanning the 2010-2021 time period 

Kevin Gurney, Pawlok Dass, Anna Kato, Bhaskar Mitra, and Geoffrey Roest

The Hestia Project estimates fossil fuel carbon dioxide (FFCO2) emissions to the scale of buildings, factories, and road segments for whole cities every hour. Recent updates to the Vulcan Project (version 4) are now realized in 3 large urban domains in the US: the LA Megacity, the NE corridor (Washington DC to Baltimore and beyond) and the city of Indianapolis. Here, we present the latest developments in the estimation from these 3 urban areas and apply a series of hypothetical mitigation efforts, demonstrating the enabling features of high space/time resolution urban FFCO2 emissions estimation. Furthermore, we analyze the spatial patterns of emissions and place them in the context of indicators of social and environmental justice.

How to cite: Gurney, K., Dass, P., Kato, A., Mitra, B., and Roest, G.: Building and road segment scale fossil fuel CO2 emissions estimation across multiple US cities spanning the 2010-2021 time period, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11169, https://doi.org/10.5194/egusphere-egu23-11169, 2023.

EGU23-11511 | ECS | Posters on site | AS3.22

A method for estimating localized CO2 emissions from co-located satellite XCO2 and NO2 images 

Blanca Fuentes Andrade, Maximilian Reuter, Michael Buchwitz, Heinrich Bovensmann, and John P. Burrows

CO2 emissions need to be rapidly reduced in order to peak greenhouse gas emissions and limit global warming to well below 2ºC. Most of these anthropogenic CO2 emissions result from the combustion of fossil fuels from localized sources. Therefore, it is essential to monitor these emissions to corroborate the compliance with the objectives of the Paris Agreement. Under this agreement, the parties report their national greenhouse gas inventories, usually computed using bottom-up methods based on statistical activity data and emission factors. Top-down approaches, based on atmospheric observations, can complement and verify these inventories. Satellite-based observations have the advantage of potential global coverage and the feasibility of providing independent emission estimates from localized sources, like cities and power plants.

In this study we present a top-down method to quantify the CO2 emissions from localized sources by using XCO2 (the column-averaged dry-air mole fraction of CO2) retrievals from the Orbiting Carbon Observatory 3 (OCO-3) in its snapshot area mode. It is a cross-sectional flux method, so that our estimate of the source rate is obtained from the flux through a number of cross-sections downwind of the source.

The detection of CO2 emission plumes is challenging due to the small enhancements resulting from anthropogenic emissions from individual source points compared to the background concentrations and the satellite’s instrument noise. NO2 is co-emitted with CO2 in the combustion of fossil fuels and its vertical column densities can exceed background values and sensor noise by orders of magnitude in emission plumes, what makes it a suitable tracer for recently emitted CO2. Therefore, our plume detection method uses TROPOMI NO2 data which is co-located with the XCO2 snapshot.

We expose the CO2 emissions estimates for 7 overpasses over the Bełchatów power plant, in Poland, together with bottom-up emission estimates for comparison, showing that we can repeatedly monitor power plant CO2 emissions.

How to cite: Fuentes Andrade, B., Reuter, M., Buchwitz, M., Bovensmann, H., and Burrows, J. P.: A method for estimating localized CO2 emissions from co-located satellite XCO2 and NO2 images, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11511, https://doi.org/10.5194/egusphere-egu23-11511, 2023.

EGU23-11521 | Posters on site | AS3.22 | Highlight

EYE-CLIMA: developing inverse modelling approaches for monitoring national GHG inventories 

Wilfried Winiwarter, Glen Peters, and Rona Thompson and the EYE-CLIMA consortium

Emissions of greenhouse gases (GHG) reported by countries in their GHG inventories represent the central information used in international policies based on the Paris agreement and in the Global Stocktake process to help curb global GHG emissions. To maximize trust in these national emission inventories reported to the UNFCCC, procedures for quality control, quality assurance, and verification have been described in the IPCC 2006 national GHG inventory guidelines and extended further in its 2019 refinement. Quantifying emission fluxes via atmospheric measurements and inverse modelling provides an independent assessment of the inventories and can help determine the quality of national inventories and make improvements. While tested in scientific studies, routine applications of inverse modelling in national inventory reports are rare. As a new Horizon Europe project, EYE-CLIMA will perform inverse modelling of a range of important radiative forcers (methane, nitrous oxide, selected fluorinated gases, black carbon) as a monitoring tool on a national scale for selected European countries, together with national inventory agencies, to help develop complementary methods to ensure the robustness and lead to improvements in inventories. The presentation will lay out the overall project concept, including stakeholder involvement, and provide an overview on past experiences with inverse modelling approaches and strategies to implement them in a way useful for national inventory agencies.

How to cite: Winiwarter, W., Peters, G., and Thompson, R. and the EYE-CLIMA consortium: EYE-CLIMA: developing inverse modelling approaches for monitoring national GHG inventories, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11521, https://doi.org/10.5194/egusphere-egu23-11521, 2023.

EGU23-11603 | ECS | Posters on site | AS3.22 | Highlight

Seoul carbon emissions estimated with Bayesian inverse modeling of measurements from ground and space 

Sojung Sim and Sujong Jeong

The bottom-up method of estimating carbon emissions from fossil fuel use based on socio-economic databases has significant uncertainty. In particular, this uncertainty increases when the spatial and temporal scales are fine, such as in cities. Therefore, an independent and complementary top-down method has been used to verify carbon emissions estimated by the bottom-up method. This method uses the atmospheric CO2 measurement, transport model, and the inverse model. In this study, carbon emissions provided by ODIAC were improved using ground and satellite CO2 observation data measured in 2019 for Seoul. We used atmospheric CO2 concentration from four observation sites located in Seoul and the column-averaged dry air mole fractions of CO2 from OCO-2. In order to quantify the footprint, which is the flux sensitivities on observation sites, STILT and X-STILT model was used for the ground observation and satellite observation, respectively. The result showed that prior carbon emissions in specific areas including power plants and airport were underestimated. The carbon emission uncertainty decreased through Bayesian inverse model, and it was found that the calculated observation and emission error covariance were appropriate through the reduced chi-square calculation. We assessed Bayesian inverse modelling of Seoul carbon emission from fossil fuel use using measurement from ground and space, which will enable effective carbon neutrality policy decisions for Seoul.

This work was supported by Korea Environment Industry &Technology Institute (KEITI) through "Climate Change R&D Project for New Climate Regime", funded by Korea Ministry of Environment (MOE) (2022003560006)

How to cite: Sim, S. and Jeong, S.: Seoul carbon emissions estimated with Bayesian inverse modeling of measurements from ground and space, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11603, https://doi.org/10.5194/egusphere-egu23-11603, 2023.

EGU23-12043 | ECS | Posters on site | AS3.22

Validation of Boreas: an instrument for simultaneous measurement of amount fraction and stable isotope ratios in methane 

Cameron Yeo, Chris Rennick, Emmal Safi, and Tim Arnold

Methane (CH4) is the second most important anthropogenic greenhouse gas in terms of its impact on climate to date and its current rates of emissions. It has a wide variety of emission sources including agriculture, landfills and fossil fuel combustion alongside a short atmospheric lifetime, making it a justifiable short-term target of emissions mitigation strategies. To aid the global drive on reducing emissions, it is integral to quantify emissions estimates for the validation of CH4 inventories. Each source of CH4 is identified by distinct isotopic ratios which proves a useful appliance in the sectoral division of amount fraction measurements.

We have developed Boreas, an automated preconcentrator sample preparation system coupled to an infrared laser spectrometer, capable of making hourly measurements of δ13C(CH4) and δ2H(CH4) of ambient air samples. Deployed at National Physical Laboratory’s atmospheric monitoring site in May 2021, Boreas makes continuous, high-frequency hourly measurements capable of capturing pollution events.

As concentration calibration and linearity has been verified using synthetic mixtures, we present a method of validation of Boreas measurements, comparing them to simultaneous one-minute-average measurements made by cavity-ring down spectroscopy. We use Keeling and Miller-Tans analysis to examine the source signature δ13C(CH4) and δ2H(CH4) of local pollution events, distinguishing agricultural sources from northern hemisphere background. We will show that the calibrated concentration reported by Boreas agrees with that of a Picarro G2401 making simultaneous measurements over a wide range of ambient background and polluted air. Moreover, we will show that the preconcentration step has no concentration dependence e.g., breakthrough or carry over.

How to cite: Yeo, C., Rennick, C., Safi, E., and Arnold, T.: Validation of Boreas: an instrument for simultaneous measurement of amount fraction and stable isotope ratios in methane, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12043, https://doi.org/10.5194/egusphere-egu23-12043, 2023.

EGU23-12172 | Orals | AS3.22

Observations of radiatively active halogenated species at MonteCImone WMO-GAW station and their use in inverse modelling techniques to derive emission estimates at the regional scale. 

Jgor Arduini, Saurabh Annadate, Rita Cesari, Paolo Cristofanelli, Serena Falasca, Umberto Giostra, and Michela Maione

Long term measurement activities carried out at the WMO GAW global station of Monte Cimone (CMN) provide a useful insight into the characterization of the composition of the Southern European atmosphere. Since 2003, ozone depleting substances (ODSs) and halogenated Greenhouse Gases (GHGs) have been measured at CMN in the frame of the AGAGE (Advanced Global Atmospheric Gases Experiment) programme, with the aim of tracking progress towards the implementation of the international treaties on stratospheric ozone depletion and climate, and getting a better understanding of emissions both in terms of magnitude and localisation at the regional (EU) scale. CMN is often influenced by the advection of polluted air masses from the Po basin, one of the most polluted areas in Europe, as well as by the transport from other highly anthropised regions in Central EU. However, during the cold months and at night-time in the warm season, the site is representative of the free troposphere.

By providing high quality, high frequency, continuous -almost uninterrupted- observations of ODSs (chlorofluorocarbons and hydrochlorofluorocarbons) and their radiatively active substitutes (hydrofluorocarbons) to modellers, the monitoring activities at CMN  are crucial for improving the overall sensitivity of the inverse modelling techniques used to derive emissions through the so called “top-down” approach. Such approach represents an important quasi-independent cross-check of national GHG emission inventories submitted annually by the parties to the United Nations Framework Convention on Climate Change (UNFCCC). Here we will present results of the Bayesian inverse modelling technique used to derive emissions at the EU national scale based on the observations described above.

How to cite: Arduini, J., Annadate, S., Cesari, R., Cristofanelli, P., Falasca, S., Giostra, U., and Maione, M.: Observations of radiatively active halogenated species at MonteCImone WMO-GAW station and their use in inverse modelling techniques to derive emission estimates at the regional scale., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12172, https://doi.org/10.5194/egusphere-egu23-12172, 2023.

EGU23-12722 | Orals | AS3.22 | Highlight

The International Methane Emissions Observatory (IMEO): Bringing together policy-relevant methane emissions data 

Daniel Zavala-Araiza, Stefan Schwietzke, Andreea Calcan, Itziar Irakulis Loitxate, Cynthia Randles, Meghan Demeter, Luis Guanter, Manfredi Caltagirone, and Steven P. Hamburg

To fill gaps in knowledge and refine global understanding of the location and magnitude of methane emissions across sectors, integration and use of data from a range of sources is needed. As countries and industry establish ambitious mitigation targets, accurate and measurement-based emission estimates are critical to accelerate emission reductions and assess progress by tracking changes in emissions over time.

The International Methane Emissions Observatory (IMEO) was launched in 2021 at the G20 summit and is hosted by the United Nations Environment Program (UNEP). IMEO is providing reliable, public, policy-relevant data to facilitate actions to reduce methane emissions.

IMEO is collecting and integrating diverse methane emissions data streams, including satellite remote sensing data, science studies, inventories, and measurement-based industry reporting to establish a global, centralized public record of empirically verified methane emissions.

In this work, we will summarize (i) IMEO’s current efforts to integrate spatio-temporally dynamic methane emissions data (ii) details of the Methane Alert and Response System (MARS) -a recently-launched system for satellite-based detection, attribution, and monitoring of methane sources to notify emitters and assist mitigation efforts, (iii) insights from measurement campaigns across the world, and (iv) activities for the direct engagement with relevant stakeholders to accelerate mitigation of methane emissions.

How to cite: Zavala-Araiza, D., Schwietzke, S., Calcan, A., Irakulis Loitxate, I., Randles, C., Demeter, M., Guanter, L., Caltagirone, M., and Hamburg, S. P.: The International Methane Emissions Observatory (IMEO): Bringing together policy-relevant methane emissions data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12722, https://doi.org/10.5194/egusphere-egu23-12722, 2023.

EGU23-12997 | ECS | Posters on site | AS3.22

Bottom-up estimation of traffic emissions in Munich based on macroscopic traffic simulation and counting data 

Daniel Kühbacher, Patrick Aigner, Ingrid Super, Arjan Droste, Hugo Denier van der Gon, Mario Ilic, and Jia Chen

Cities are home to more than half of the world’s population, a share that will continue to grow in the future and account for more than 70% of the global fossil fuel CO2 emissions. To avoid dangerous climate change, cities will be required to reduce their energy consumption and cut carbon emissions significantly. Emission inventories are the basis for any carbon mitigation efforts. They determine the current status, allocate emissions to various sectors and indicate their reduction potential. The ICOS-Cities project fosters this development and aims to set up integrated city observatories in three pilot cities (Paris, Zurich and Munich). Reliable prior data is essential for modeling efforts in this project and road transport is a key emission sector in urban areas.

We present a newly developed, highly spatially and temporally resolved bottom-up traffic emission inventory for the area of Munich (311 km2), covering outer circle motorways as well as inner city roads. The inventory accounts for greenhouse gases (CO2, CH4) and co-emitted species/ air pollutants (CO, NO2, O3 and PM). It has a temporal resolution of one hour and is compiled for the years 2019 to 2022. The emissions are represented as line sources along the road network, which allows for emission sampling ranging from several tens of meters in densely interconnected inner-city environments to a kilometer-scale on highways.

The inventory is based on the city’s official macroscopic traffic model (VISUM), which we validate using traffic counts from more than hundred permanent traffic monitoring stations in Munich since this data is not implemented in the traffic model. Additionally, we extrapolate the traffic model to unobserved days (e.g., weekends, holidays) by means of traffic counts, and distinguish between vehicle classes (private car, heavy duty vehicle, light duty vehicle, coach and motorbike) based on categorized traffic counts. HBEFA emission factors (Handbook for Road Transport Emission Factors) are applied to estimate the emissions.

A comparison with the official emission numbers of the City of Munich and other spatially explicit inventories available in the same region, such as TNO GHGco database, is conducted. We will present the main discrepancies and provide insights for other cities aiming to develop similar inventories.

How to cite: Kühbacher, D., Aigner, P., Super, I., Droste, A., Denier van der Gon, H., Ilic, M., and Chen, J.: Bottom-up estimation of traffic emissions in Munich based on macroscopic traffic simulation and counting data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12997, https://doi.org/10.5194/egusphere-egu23-12997, 2023.

EGU23-13186 | ECS | Posters on site | AS3.22

Comparing imaging processing techniques with physical based inverse radiative transfer models for methane and carbon dioxide point emissions 

Ida Jandl, Leon Scheidweiler, Jochen Landgraf, Joannes D. Maasakkers, and André Butz

Satellite remote sensing techniques offer the possibility of an independent global monitoring of carbon dioxide (CO2) and methane (CH4) emissions. Recently, point sources such as oil and gas facilities and power plants, which emit a high concentration of greenhouse gases (GHG) locally, have received particular attention. Therefore, present and upcoming satellite missions focus on collecting GHG concentration images with a high spatial resolution. The PRISMA (PRecursore IperSpettrale della Missione Applicativais) spaceborne imaging spectrometer is an Italian satellite which has been launched on March 22, 2019. It is the first satellite which provides open access hyperspectral images of backscattered sunlight with a spatial resolution of 30x30 meter and a spectral resolution of around 11nm. The measured absorption spectra in the shortwave infrared range cover strong CO2 and CH4absorption bands. Various methods can be used to retrieve 2-dimensional CO2 and CH4fields above localized GHG sources.

Here, we compare data-driven and physics-based retrieval methods in application to PRISMA measurements above localized GHG sources such as oil and gas production facilities in Turkmenistan for CH4 and coal-fired power plants for CO2. The data-driven methods are variants of the matched filter technique while the physics-based methods built on spectroscopic radiative transfer modeling. While matched filter techniques use the spatial covariance of the observed scene, traditional physics-based retrievals operate on individual spectra without considering the two-dimensional scene. For a few cases, we examine the differences between both methods and conclude on strengths and weaknesses.

How to cite: Jandl, I., Scheidweiler, L., Landgraf, J., Maasakkers, J. D., and Butz, A.: Comparing imaging processing techniques with physical based inverse radiative transfer models for methane and carbon dioxide point emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13186, https://doi.org/10.5194/egusphere-egu23-13186, 2023.

EGU23-13336 | Orals | AS3.22

CO2 and CH4 observation-based budgets in support to future Copernicus CO2 emissions Monitoring and Verification Support (CO2MVS) capacity user communities 

Ana Maria Roxana Petrescu, Glen P. Peters, Robbie M. Andrew, Matthew J. McGrath, Philippe Peylin, Frederic Chevallier, and Richard Engelen and the VERIFY and CoCO2 project participants

Knowledge of the spatial distribution of the fluxes of greenhouse gases and their temporal variability as well as flux attribution to natural and anthropogenic processes is essential to monitoring the progress in mitigating anthropogenic emissions under the Paris Agreement and to inform its Global Stocktake.

This study identifies, quantifies and explains possible divergences between global inventories, atmospheric inversions, process-based models, and national inventories submitted to the UNFCCC. The focus is on the EU27, the world’s largest emitters, or other smaller regions that can be used to draw generic results or lessons. The analysis builds on the methodological approach developed previously in the EU-funded VERIFY project’s GHG syntheses (Petrescu et al., 2020, 2021a, 2021b, 2022 and McGrath et al., 2022). Most of the data products are from the VERIFY project, with a gradual inclusion of EU-funded CoCO2 project’s specific products as the project evolves. Reported inventory-based emissions and removals are generally estimated using bottom-up statistical inventory estimates. Top-down, observation-based estimates are required by multiple stakeholders and at multiple scales to verify bottom-up emission estimates. These estimates are performed at different scales for a variety of applications: the global and continental scale for science purposes, country scale for reporting to the UNFCCC, sub-country scale for urban planning, and point sources like large power plants for verification (Pinty et al., 2019). Several examples will be provided for different sectors of CO2/CH4 budgets to illustrate (e.g., EU27) the aforementioned divergences as well as the current level of convergence between methods.

A key conclusion across all components analysed is the difficulty of harmonising datasets into a comparable format. The tradition of comparing datasets as published is easy, but problematic and potentially misleading. To reconcile differences between alternative datasets requires a much deeper understanding of each dataset, such as the system boundaries, methods, and input data sources. Often the necessary data is not available or time consuming to access. A systematic reconciliation and comparison often requires a close dialogue between analysts, data providers, and modelers.

Building on our experiences, we discuss a Decision Support Blueprint, outlining potential mechanisms and tools to provide diverse, but targeted, information to the relevant users wanting to reconcile these different datasets. The blueprint is informed by several user consultation meetings and workshops. The blueprint will help tailor a Decision Support System (DSS), as a component of the Copernicus CO2MVS, to help inventory agencies, governments and their initiatives (e.g. Covenant of Mayors, C40, ICLEI), industry, NGOs, and other interested actors to utilize the expanding observation datasets to support monitoring and verification activities.

How to cite: Petrescu, A. M. R., Peters, G. P., Andrew, R. M., McGrath, M. J., Peylin, P., Chevallier, F., and Engelen, R. and the VERIFY and CoCO2 project participants: CO2 and CH4 observation-based budgets in support to future Copernicus CO2 emissions Monitoring and Verification Support (CO2MVS) capacity user communities, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13336, https://doi.org/10.5194/egusphere-egu23-13336, 2023.

EGU23-13451 | ECS | Orals | AS3.22

CO2 bottom-up emission inventory based on municipal power generation and heating data in Munich 

Patrick Aigner, Michael Suhendra, Beyza Yirtar, Daniel Kühbacher, Ingrid Super, Arjan Droste, Hugo Denier van der Gon, Dominik Brunner, Helmut Kohlmeier, Thomas Althammer, and Jia Chen

Cities’ climate action efforts towards carbon neutrality will be challenged in the next decades by more and more people moving into cities and the correspondingly growing demand for services and infrastructure. By 2050, over 70% of the world's population is projected to be living in densely populated urban areas. This will add another level of difficulty to fulfilling the demand for clean energy and heating considering the available technology and infrastructure. It will be important for city stakeholders to understand current and future demands in detail to make informed decisions, implement effective carbon mitigation measures, and achieve a good return on investment. To kick this off, the ICOS-cities project chose three pilot cities (Paris, Munich, and Zurich) to generate high-resolution spatial and temporal bottom-up inventories for CO2 and co-emitted species. 

Existing municipal emission inventories for Munich report annual emissions estimates without spatial information. We present a temporal (1h) and spatial (100m x 100m) explicit high-resolution bottom-up inventory for public power production consisting of electricity and district heating (GNFR A) and other stationary combustion (GNFR-C) in Munich. Both sectors are derived from power and heating plant data of the year 2019 provided by the Stadtwerke München (SWM) and the latest municipal geospatial datasets provided by the City of Munich. Furthermore, we compare state-of-the-art but more generic TNO activity and temporal profiles with temporal profiles derived from data from local CHP plants data and a heat demand function validated with Munich’s reported yearly heat demand.  Additionally, we present emission factors calculated from the fuel composition (2019) of inflowing gas and burned waste alongside available state-of-the-art emissions factors from IPCC (2019), EPA (2022), and UBA (2022). 

How to cite: Aigner, P., Suhendra, M., Yirtar, B., Kühbacher, D., Super, I., Droste, A., Denier van der Gon, H., Brunner, D., Kohlmeier, H., Althammer, T., and Chen, J.: CO2 bottom-up emission inventory based on municipal power generation and heating data in Munich, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13451, https://doi.org/10.5194/egusphere-egu23-13451, 2023.

EGU23-13875 | Posters on site | AS3.22 | Highlight

Global emissions of five controlled CFCs have increased since 2010 

Luke Western, Martin Vollmer, Paul Krummel, Karina Adcock, Paul Fraser, Christina Harth, Ray Langenfelds, Stephen Montzka, Jens Mühle, Simon O'Doherty, David Oram, Stefan Reimann, Matt Rigby, Isaac Vimont, Ray Weiss, Dickon Young, and Johannes Laube

Production and consumption of ozone-depleting chlorofluorocarbons (CFCs) are controlled under the Montreal Protocol. CFC production for most applications was banned globally in 2010, albeit with exemptions for uses assumed to cause negligible emissions to the atmosphere, such as in the production of other chemicals. A few years ago, emissions of CFC-11 were reported to be increasing after their phase-out, most likely due to unreported production and non-compliance, which sparked widespread, renewed attention to this topic. Here we show that emissions of five other CFCs have increased since 2010, namely CFC-13, CFC-112a, CFC-113a, CFC-114a and CFC-115. Three of these CFCs are likely increasing due to their involvement in the production of non-ozone-depleting HFCs, which have largely replaced CFCs and HCFCs in many applications. The drivers behind the increase in the other two CFCs is unclear. While the impact of these CFCs on ozone layer recovery will likely be small, these long-lived CFCs are potent greenhouse gases and their CO2-equivalent emissions in 2020 were comparable to those of a mid-sized European country.

How to cite: Western, L., Vollmer, M., Krummel, P., Adcock, K., Fraser, P., Harth, C., Langenfelds, R., Montzka, S., Mühle, J., O'Doherty, S., Oram, D., Reimann, S., Rigby, M., Vimont, I., Weiss, R., Young, D., and Laube, J.: Global emissions of five controlled CFCs have increased since 2010, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13875, https://doi.org/10.5194/egusphere-egu23-13875, 2023.

EGU23-14275 | ECS | Posters on site | AS3.22

Identifying needs for urban greenhouse gas monitoring in Seoul using ground-based EM27/SUN measurements 

Hayoung Park and Sujong Jeong

Anthropogenic emissions of greenhouse gases from fossil fuel combustion have a significant impact on the global climate. Cities, which are home to more than half of the global population, account for over 70% of anthropogenic greenhouse gas emissions and are the major sources of air pollution that we face today. However, as much as they are big emitters, cities also have great potential to be drivers of global greenhouse gas reductions. To better manage atmospheric greenhouse gases, it is necessary to accurately monitor and quantify emissions at all spatial scales from national to urban levels. In addition to using satellites which provide global coverage with high space and time resolutions for greenhouse gas monitoring, several studies have used portable ground-based remote sensing Fourier transform infrared (FTIR) spectrometers, EM27/SUNs, to measure the column-averaged concentrations of greenhouse gases. This study analyzes the column-averaged dry air mole fractions of CO2, CH4, and CO (XCO2, XCH4, XCO) in the atmosphere over Seoul using two EM27/SUNs which is the first to be done in South Korea. Moreover, we compare our measurements with satellite measurements of the Orbiting Carbon Observatory-2 (OCO-2), Orbiting Carbon Observatory-3 (OCO-3), and Sentinel-5 Precursor TROPOspheric Monitoring Instrument (TROPOMI). Together, this study aims to analyze the three-dimensional structure of greenhouse gases in Seoul which has been difficult to do due to the absence of domestic greenhouse gas observation satellites. Furthermore, this study identifies the need for more ground-based column measurements of greenhouse gases in cities and plume areas, as well as locally adaptable methods of greenhouse gas emissions monitoring in urban areas.

How to cite: Park, H. and Jeong, S.: Identifying needs for urban greenhouse gas monitoring in Seoul using ground-based EM27/SUN measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14275, https://doi.org/10.5194/egusphere-egu23-14275, 2023.

EGU23-15380 | Posters on site | AS3.22

Impacts of prescribed fossil fuel CO2 emissions on subnational level inverse flux estimates 

Tomohiro Oda, Liang Feng, Paul Palmer, and Lesley Ott

Atmospheric-based approaches have been recognized as promising tools for QA/QC and verification of greenhouse gas (GHG) emission inventories reported by countries. Atmospheric-based approaches also help provide GHG estimates for countries and regions with less robust inventory building capacities, and direct estimates for key subnational levels, which are not often covered by national inventories. Conventional CO2 flux inversion approaches, unlike urban inversion applications, often prescribe fossil fuel CO2 emissions (FFCO2) and mostly optimized natural fluxes. Thus, errors in prescribed FFCO2 impact the final flux estimates.

We implemented two sets of inversions with two different emission inventories in order to examine the impact of the prescribed FFCO2 on the inverse flux estimates. The emission inventory difference was used to approximate potential errors in the prescribed FFCO2. Our inversion result demonstrated how the FFCO2 errors, particularly due to sub-annual seasonal emission pattern differences, can have an impact on posterior emission estimates via flux optimization. Our result also demonstrated that FFCO2 errors from large emitting countries could significantly bias sub-national flux estimates by mis-attributing their flux corrections to natural fluxes to compensate for the FFCO2 errors. The magnitude of the potential errors might be small compared to that of large-scale fluxes. However, the errors could be significant in relation to small sub-national scale fluxes or emissions from lesser emitting countries. We also examined the impact of two observation systems, such as global in-situ network and a satellite, to FFCO2 errors.

We discuss the existing challenges that need to be addressed to further enhance the use of atmospheric inversions with country level inventories. In addition to improvements in inversions, improving inventories (prescribed FFCO2) should have a direct benefit to improved accuracy of inverse flux estimates. For example, extended data collection at sub-national scales should greatly mitigate potential errors in the prescribed FFCO2. This study highlights the importance of developing GHG emission information in a hybrid fashion to support science and the emission reporting and monitoring.

How to cite: Oda, T., Feng, L., Palmer, P., and Ott, L.: Impacts of prescribed fossil fuel CO2 emissions on subnational level inverse flux estimates, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15380, https://doi.org/10.5194/egusphere-egu23-15380, 2023.

EGU23-15854 | ECS | Posters on site | AS3.22

Using Satellite Column Observations with a Bayesian Inversion System for constraining the GHG budget over India 

Rakesh Subramanian, Rona Thompson, Martin Vojta, and Andreas Stohl

The source-sink estimation of greenhouse gases and the accurate quantification of their flux distributions are a major scientific challenge of our times. Although statistically developed inventory-based carbon emissions improve understanding of emissions, they are uncertain and occasionally, they do not reflect actual emissions, especially at finer scales. By using GHG observations in conjunction with numerical atmospheric models, GHG budgets can be constrained. However, the sparseness in the in-situ observation networks of GHGs, makes this a challenging problem, especially in certain regions like India. However, satellite remote sensing can fill this data gap. This study applies the Bayesian inversion system, FLEXINVERT (Thompson and Stohl 2014), coupled with a Lagrangian Particle Dispersion Model, FLEXPART (Stohl et al 1998), to assimilate TROPOMI satellite observations of CH4 and constrains the CH4 fluxes over India domain. This inverse modeling system uses the Source-Receptor Relationship derived from Flexpart as the Transport operator while minimizing the cost function for optimization.  The system will use various prior fluxes and initial concentration fields to test the set-up over Indian domain, which have strong fluxes of CH4 and are not well constrained by the existing ground-based measurement networks. The results will be compared with the limited in-situ observations available for the region.

How to cite: Subramanian, R., Thompson, R., Vojta, M., and Stohl, A.: Using Satellite Column Observations with a Bayesian Inversion System for constraining the GHG budget over India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15854, https://doi.org/10.5194/egusphere-egu23-15854, 2023.

EGU23-15895 | Posters on site | AS3.22

Characterizing major anthropogenic point sources in the South African Highveld region using OCO-3 carbon dioxide Snapshot Area Maps and Sentinel-5P/TROPOMI nitrogen dioxide columns 

Janne Hakkarainen, Iolanda Ialongo, Tomohiro Oda, Monika Szeląg, Christopher W. O'Dell, Annmarie Eldering, and David Crisp

We characterize major anthropogenic point sources in the South African Highveld region using Orbiting Carbon Observatory-3 (OCO-3) Snapshot Area Map (SAM) carbon dioxide (CO2) and Sentinel-5 Precursor (S5P) TROPOspheric Monitoring Instrument (TROPOMI) nitrogen dioxide (NO2) observations. Altogether we analyze six OCO-3 SAMs. We estimate the emissions of six power stations (Kendal, Kriel, Matla, Majuba, Tutuka and Grootvlei) and the largest single emitter of greenhouse gas in the world, Secunda CTL synthetic fuel plant. We apply the cross-sectional flux method for the emission estimation, and we extend the method to fit several plumes at the same time. Overall, the satellite-based emission estimates are in good agreement (within the uncertainties) as compared to emission inventories, even for the cases where several plumes are mixed. We also discuss the advantages and challenges of the current measurement systems for greenhouse gas emission monitoring and reporting, and the applicability of different emission estimation approaches to future satellite missions such as the Copernicus CO2 Monitoring Mission (CO2M) and the Global Observing SATellite for Greenhouse gases and Water cycle (GOSAT-GW), including the joint analysis of CO2 and NOobservations.

How to cite: Hakkarainen, J., Ialongo, I., Oda, T., Szeląg, M., O'Dell, C. W., Eldering, A., and Crisp, D.: Characterizing major anthropogenic point sources in the South African Highveld region using OCO-3 carbon dioxide Snapshot Area Maps and Sentinel-5P/TROPOMI nitrogen dioxide columns, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15895, https://doi.org/10.5194/egusphere-egu23-15895, 2023.

EGU23-16064 | Orals | AS3.22

Quantifying localized carbon dioxide emissions from space: the CO2Image mission 

Dietrich G. Feist, Anke Roiger, Julia Marshall, Klaus-Dirk Gottschaldt, Friedemann Reum, Günter Lichtenberg, Andreas Baumgartner, Philipp Hochstaffl, Claas Köhler, Franz Schreier, David Krutz, Carsten Paproth, Andreas Pohl, Ilse Sebastian, Ingo Walter, and André Butz

Space-based observations of carbon dioxide (CO2) are the backbone of the global and national-scale carbon monitoring systems that are currently being developed to support and verify greenhouse gas emission reduction measures. Current and planned public satellite missions, such as GOSAT 1+2, OCO 1-3 and the European Union's Anthropogenic Carbon Dioxide Monitoring mission CO2M, aim at constraining national and regional-scale emissions down to scales of urban agglomerations and large point sources with emissions in excess of ~10 MtCO2/year.

We report on the DLR demonstrator mission CO2Image, which is planned for launch in 2026. The mission will complement the suite of planned CO2 sensors by zooming in on facility-scale emissions, detecting and quantifying emissions from point sources as small as 1 MtCO2/year. A fleet of CO2Image sensors would be able to monitor roughly 90% of the CO2 emissions from coal-fired power plants worldwide. The key feature of the mission is a target region approach, measuring approximately 75 tiles of size ~50 x 50 km2 per day at a resolution of 50 x 50 m2. Thus, CO2Image will be able to resolve plumes from individual localized sources, essentially providing super-resolution nests for survey missions such as CO2M. In addition, the choice of the spectral window will allow the detection of point sources of methane as small as 100 kg CH4/hr will also be possible.

We present the instrument concept, a spaceborne push-broom imaging grating spectrometer developed and built by DLR. It will measure spectra of reflected solar radiation in the short wave infrared spectral band around 2000 nm. It relies on a comparatively compact design with a single spectral window and a spectral resolution of approximately ~1 nm. This spectral resolution has been optimized for greenhouse gas retrieval and should provide improved precision and accuracy compared to hyperspectral sensors with comparable spatial resolution. We will further discuss the overall mission concept in terms of the sampling strategy, outlining how target scenes will be selected. As a publicly-funded mission, CO2Image will provide public, transparent information about anthropogenic greenhouse gas emissions from space.

How to cite: Feist, D. G., Roiger, A., Marshall, J., Gottschaldt, K.-D., Reum, F., Lichtenberg, G., Baumgartner, A., Hochstaffl, P., Köhler, C., Schreier, F., Krutz, D., Paproth, C., Pohl, A., Sebastian, I., Walter, I., and Butz, A.: Quantifying localized carbon dioxide emissions from space: the CO2Image mission, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16064, https://doi.org/10.5194/egusphere-egu23-16064, 2023.

EGU23-16636 | Orals | AS3.22

CO2 emissions estimate from Mexico City using ground- and space-based remote sensing 

Ke Che, thomas Lauvaux, noemie Taquet, Yang Xu, Morgan Lopez, Wolfgang Stremme, Agustín García-Reynoso, Phillipe Ciais, Yi Liu, Michel Ramonet, and Michel Grutter

The Mexico City Metropolitan Area (MCMA) has become the most populous urban region in North America and in the top five megacities worldwide (around 22 million inhabitants). To quantify the urban CO2 emissions of MCMA, a dense network of  Fourier Transform Infrared (FTIR) spectrometers with 6 portable EM27/SUN and 1 IFS 125HR were deployed within and around the MCMA  tracking gradients in atmospheric column CO2 concentrations (XCO2) from October 2020 to May 2021 (part of the French-Mexican MERCI-CO2 project). During these 7 months, twenty  XCO2 images (Snapshot Area Mode)  were collected by the NASA Orbiting Carbon Observatory (OCO-3) mission over the MCMA. By comparing  ground- and space-based observations, we found a positive XCO2 difference with a mean (± one standard uncertainty) of 1.16 (± 1.14) ppm between OCO-3 and FTIR column measurements, most probably caused by their respective calibration procedures. XCO2 gradients observed between the urban plume and its surroundings  show a good agreement between OCO-3 and the FTIR stations with a correlation coefficient (R) of 0.92,  decreasing significantly when comparing intra-city gradients (R=0.24). 

In a second phase, we assimilated these two types of dense column-integrated observations (FTIR network and OCO-3 SAM observations) separately to optimize the anthropogenic emissions from the MCMA and the biogenic CO2 fluxes in and around the city limits, in addition to the CO2 background concentrations. The X-Stochastic Time-Inverted Lagrangian Transport (X-STILT) model driven by the Weather Research and Forecasting (WRF) at 1-km resolution was used here to relate our atmospheric observations to surface fluxes and background conditions. An analytical Bayesian inversion technique was used here to robustly update the prior estimates at 1-km and 1-hour resolution. High-resolution prior biogenic CO2 emissions were computed with the light-use efficiency model CASA and our prior backgrounds from the global CAMS CO2 atmospheric inversion (version: v21r2). Prior anthropogenic CO2 emissions at 1 km are coming from a Mexico-specific inventory UNAM and from the global inventory ODIAC. These two inventories contain large discrepancies over MCMA (~40 %), while UNAM provides more detailed  information of point sources across our inversion domain. We performed sensitivity control experiments to quantify the effects from different prior fluxes and different covariance parameters. Furthermore, we combine OCO-3 and FTIR together in the same inversion process, a promising step toward providing a verification to  combine multiple data streams over a specific city. 

How to cite: Che, K., Lauvaux, T., Taquet, N., Xu, Y., Lopez, M., Stremme, W., García-Reynoso, A., Ciais, P., Liu, Y., Ramonet, M., and Grutter, M.: CO2 emissions estimate from Mexico City using ground- and space-based remote sensing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16636, https://doi.org/10.5194/egusphere-egu23-16636, 2023.

EGU23-16832 | ECS | Orals | AS3.22

National CO2 budgets (2015–2020) inferred from atmospheric CO2observations in support of the Global Stocktake 

Brendan Byrne and Kevin Bowman and the other authors

Accurate accounting of emissions and removals of CO2 is critical for the planning and verification of emission reduction targets in support of the Paris Agreement. Here, we present a pilot dataset of country-specific net carbon exchange (NCE; fossil plus terrestrial ecosystem fluxes) and terrestrial carbon stock changes aimed at informing countries’ carbon budgets. These estimates are based on “top-down” NCE outputs from the v10 Orbiting Carbon Observatory (OCO-2) modeling inter-comparison project (MIP), wherein an ensemble of inverse modeling groups conducted standardized experiments assimilating OCO-2 column-averaged dry-air mole fraction (XCO2) retrievals (ACOS v10), in situ CO2 measurements, or combinations of these data. The v10 OCO-2 MIP NCE estimates are combined with “bottom-up” estimates of fossil fuel emissions and lateral carbon fluxes to estimate changes in terrestrial carbon stocks, which are impacted by anthropogenic and natural drivers. These flux and stock change estimates are reported annually (2015–2020) as both a global 1° × 1° gridded dataset and as a country-level dataset. Across the v10 OCO-2 MIP experiments, we obtain increases in the ensemble median terrestrial carbon stocks of 3.29–4.58 PgCO2 yr−1 (0.90–1.25 PgC yr−1). This is a result of broad increases in terrestrial carbon stocks across the northern extratropics, while the tropics generally have stock losses but with considerable regional variability and differences between v10 OCO-2 MIP experiments. We discuss the state of the science for tracking emissions and removals using top-down methods, including current limitations and future developments towards top-down monitoring and verification systems.

How to cite: Byrne, B. and Bowman, K. and the other authors: National CO2 budgets (2015–2020) inferred from atmospheric CO2observations in support of the Global Stocktake, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16832, https://doi.org/10.5194/egusphere-egu23-16832, 2023.

EGU23-16996 | Posters on site | AS3.22

Investigating national methane sources with satellite retrievals: a case of South Korea 

changsub shim, jungi moon, and Jihyun han
Methane is the second largest greenhouse gas after carbon dioxide in its impact on climate change. Atmospheric methane has stagnated from 2000 to 2006, and then began to increase again in 2007, showing the largest increase since observation in 2021(19.94 ppb/yr).
As part of UNFCCC’s goals for carbon neutrality, it is necessary to verify each country's GHG’s emissions sources and the verifications using satellite observations and atmospheric models are one of the important approaches.
Currently, satellite data have been useful for methane monitoring, particularly the retrievals measured by TROPOMI with a high resolution(~7km) and good spatial coverage.
Here we investigated the spatio-temporal characteristics of national methane distribution and the spatial correlation between satellite concentrations and the national emission sources over South Korea to identify the characteristics of high-level methane distributions from August 2018 to July 2019 .
During the period, the average concentration of XCH4 in Korea was ~1858 ppb and the monthly mean concentrations of methane in Korea were higher from June to October, which in fact reflected the characteristics of rice paddy and wetlands in monsoon season.
The spatial correlation analysis (SDM) found that there are some areas showing specific contributing emissions sources with higher methane levels. There are areas with high correlations with livestock production, fossil fuel uses(gas & oils), wastes(& landfill), and rice paddies, while there are areas with high correlations with complex effects of the four fields or with no clear correlations.
Based on our analysis, the spatial correlation analysis with various emission sources and satellite data can provide the information to evaluate the CH4 emissions inventory and give some ideas to manage regional greenhouse gases reduction policies

How to cite: shim, C., moon, J., and han, J.: Investigating national methane sources with satellite retrievals: a case of South Korea, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16996, https://doi.org/10.5194/egusphere-egu23-16996, 2023.

EGU23-17172 | Orals | AS3.22

A Bayesian Framework for Verifying Methane Inventories and Trends With Atmospheric Methane Data 

John Worden, Sudhanshu Pandey, Yuzhong Zhang, Daniel Cusworth, Qu Zhen, Anthony Bloom, Shuang Ma, Bram Maasakkers, Brendan Byrne, Riley Duren, David Crisp, Debbie Gordon, and Daniel Jacob

The 2015 Paris Climate Agreement and Global Methane Pledge formalized agreement for countries to report and reduce methane emissions to mitigate near-term climate change. Emission inventories generated through surface activity measurements are reported annually or bi-annually and evaluated periodically through a “Global Stocktake”.  Emissions inverted from atmospheric data support evaluation of reported inventories, but their systematic use is stifled by spatially variable biases from prior errors combined with limited sensitivity of observations to emissions (smoothing error), as-well-as poorly characterized information content. Here, we demonstrate a Bayesian, optimal estimation (OE) algorithm for evaluating a state-of-the-art inventory (EDGAR v6.0) using satellite-based emissions from 2009 to 2018. The OE algorithm quantifies the information content (uncertainty reduction, sectoral attribution, spatial resolution) of the satellite-based emissions and disentangles the effect of smoothing error when comparing to an inventory. We find robust differences between satellite and EDGAR for total livestock, rice, and coal emissions: 14 ± 9, 12 ± 8, -11 ± 6 Tg CH4/yr respectively. EDGAR and satellite agree that livestock emissions are increasing (0.25 to 1.3 Tg CH4/ yr / yr), primarily in the Indo-Pakistan region, sub-tropical Africa, and the Brazilian arc of deforestation; East Asia rice emissions are also increasing, highlighting the importance of agriculture on the atmospheric methane growth rate. In contrast, low information content for the waste and fossil emission trends confounds comparison between EDGAR and satellite;  increased sampling and spatial resolution of satellite observations are therefore needed to evaluate reported changes to emissions in these sectors.

How to cite: Worden, J., Pandey, S., Zhang, Y., Cusworth, D., Zhen, Q., Bloom, A., Ma, S., Maasakkers, B., Byrne, B., Duren, R., Crisp, D., Gordon, D., and Jacob, D.: A Bayesian Framework for Verifying Methane Inventories and Trends With Atmospheric Methane Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17172, https://doi.org/10.5194/egusphere-egu23-17172, 2023.

EGU23-17282 | ECS | Orals | AS3.22

Dairy sector greenhouse gas and ammonia emissions estimates based on seasonal measurements from 200 farms in California 

Nathan Li, Daniel Moore, Hongming Yi, Lei Tao, James McSpiritt, Lars Wendt, Vladislav Sevostianov, Nidia Rojas Robles, Francesca Hopkins, and Mark Zondlo

We report facility-scale emissions measurements of carbon dioxide (CO2), methane (CH4), nitrous oxide (N2O), and ammonia (NH3) from over 200 farms in California, representing 2.4% of the total dairy cow population of the United States. The dairy industry—and its 270 million cattle—are responsible for a significant proportion of global greenhouse gas and reactive nitrogen emissions. Open-path laser spectrometers mounted on top of an electric vehicle were used to conduct measurements downwind of facilities. Emission rates and associated uncertainties for each facility were quantified using in-plume observations and an inverse Gaussian plume atmospheric dispersion model with Bayesian inference. A subset of 53 farms were revisited quarterly to investigate seasonal variability and changes in management practices. 24 farms were sampled multiple times a week on different days for select seasons in order to capture inter-day variability. We partnered with 6 farms for intensive 24-hour measurements to study diurnal variability in emissions. 

Measurements of emissions were compared with national and state emissions inventories, and they were also evaluated against bottom-up estimates using activity data from the Vista-CA database. The median of the top-down CH4 emissions agreed with the median of facility-level bottom-up emissions to within 8%. Measured N2O emissions were 2.5 times higher than current inventories. N2O was responsible for about 15% of total greenhouse gas emissions in terms of CO2-equivalents (CO2e). NH3 was 40% lower than the values indicated by the 2017 US EPA national emissions inventory (NEI). 

For N2O, we found that emissions were dominated by large emission events (≈30 kg N2O hr-1) with high spatial and temporal variability. These events are potentially not captured by shorter measurement campaigns that focus only on a few farms. The top 10% largest N2O emission events were responsible for 58% of total N2O emissions. Focused studies on such events may elucidate potential opportunities for reduction of N2O emissions. 

For CH4, 14 out of the 207 dairies that we sampled had verified anaerobic digestion systems installed for manure management. The effectiveness of these systems for reducing methane emissions will be evaluated by comparing emissions from farms with digesters to emissions from farms without digesters.

How to cite: Li, N., Moore, D., Yi, H., Tao, L., McSpiritt, J., Wendt, L., Sevostianov, V., Robles, N. R., Hopkins, F., and Zondlo, M.: Dairy sector greenhouse gas and ammonia emissions estimates based on seasonal measurements from 200 farms in California, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17282, https://doi.org/10.5194/egusphere-egu23-17282, 2023.

AS4 – Interdisciplinary Processes

EGU23-1981 | ECS | Posters on site | GI3.3

Total stratospheric bromine inferred from balloon-borne solar occultation bromine oxide (BrO) measurements using the new TotalBrO instrument 

Karolin Voss, Philip Holzbeck, Ralph Kleinschek, Michael Höpfner, Gerald Wetzel, Björn-Martin Sinnhuber, Klaus Pfeilsticker, and André Butz

Halogenated organic and inorganic compounds, in particular those containing chlorine, bromine and iodine are known to contribute to the global ozone depletion as well as directly and indirectly to climate forcing. As a result of the Montreal Protocol (1987), the chlorine and bromine loadings of the stratosphere are closely monitored, while the role of iodinated compounds to the stratospheric ozone photochemistry is still uncertain.

To address the questions concerning bromine and iodine compounds, a compact solar occultation instrument (TotalBrO) has been specifically designed to measure BrO, IO (iodine oxide) and other UV/Vis absorbing gases by means of Differential Optical Absorption Spectroscopy (DOAS) from aboard a stratospheric balloon. The instrument (power consumption < 100 W) comprises of an active camera-based solar tracker (LxWxH ~ 0.40 m x 0.40 m x 0.50 m, weight ~ 12 kg) and a spectrometer unit (LxWxH ~ 0.45 m x 0.40 m x 0.40 m, weight ~ 25 kg). The spectrometer unit houses two grating spectrometers which operate in vacuum and under temperature stabilization by an ice-water bath.

We discuss the performance of the TotalBrO instrument during the first two deployments on stratospheric balloons launched from Kiruna in August, 2021 and from Timmins in August, 2022 within the HEMERA program. Once the balloon gondola was azimuthally stabilized the solar tracker was able to follow the sun with a 1σ precision lower than 0.02° up to solar zenith angles (SZAs) of 95°. The spectral retrieval (of 46 spectra acquired at SZA between 84° and 90°) allowed us to infer the BrO mixing ratio above 32 km altitude. The total bromine in the middle stratosphere is inferred by accounting for the BrO/Bry partitioning derived from a photochemical model.

How to cite: Voss, K., Holzbeck, P., Kleinschek, R., Höpfner, M., Wetzel, G., Sinnhuber, B.-M., Pfeilsticker, K., and Butz, A.: Total stratospheric bromine inferred from balloon-borne solar occultation bromine oxide (BrO) measurements using the new TotalBrO instrument, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1981, https://doi.org/10.5194/egusphere-egu23-1981, 2023.

EGU23-2923 | ECS | Posters on site | GI3.3

Total organic carbon measurements reveal large discrepancies in reported petrochemical emissions 

Megan He, Jenna Ditto, Lexie Gardner, Jo Machesky, Tori Hass-Mitchell, Christina Chen, Peeyush Khare, Bugra Sahin, John Fortner, Katherine Hayden, Jeremy Wentzell, Richard Mittermeier, Amy Leithead, Patrick Lee, Andrea Darlington, Junhua Zhang, Samar Moussa, Shao-Meng Li, John Liggio, and Drew Gentner

Oil sands are a prominent unconventional source of petroleum. Total organic carbon measurements via an aircraft campaign (Spring-Summer 2018) revealed emissions above Canadian oil sands exceeding reported values by 1900-6300%. The “missing” compounds were predominantly intermediate- and semi-volatile organic compounds, which are prolific precursors to secondary organic aerosol formation. 

Here we use a novel combination of aircraft-based measurements (including total carbon emissions measurements) and offline analytical instrumentation to characterize the mixtures of organic carbon and their volatility distributions above oil sands facilities. These airborne, real-time observations are supplemented by laboratory experiments identifying substantial, unintended emissions from waste management practices, emphasizing the importance of accurate facility-wide emissions monitoring and total carbon measurements to detect potentially vast missing emissions across sources.

Detailed chemical speciation confirms these observations near both surface mining and in-situ facilities were oil sands-derived, with facility-wide emissions around 1% of extracted petroleum—a comparable loss rate to natural gas extraction. Total emissions, spanning extraction through waste processing, were equivalent to total Canadian anthropogenic emissions from all sources. These results demonstrate that the full air quality and environmental impacts of oil sands operations cannot be captured without complete coverage of a wider volatility range of emissions.

How to cite: He, M., Ditto, J., Gardner, L., Machesky, J., Hass-Mitchell, T., Chen, C., Khare, P., Sahin, B., Fortner, J., Hayden, K., Wentzell, J., Mittermeier, R., Leithead, A., Lee, P., Darlington, A., Zhang, J., Moussa, S., Li, S.-M., Liggio, J., and Gentner, D.: Total organic carbon measurements reveal large discrepancies in reported petrochemical emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2923, https://doi.org/10.5194/egusphere-egu23-2923, 2023.

EGU23-3473 | Posters on site | GI3.3 | Highlight

The FAAM large atmospheric research aircraft: a brief history and future upgrades 

James Lee

The UK’s large atmospheric research aircraft is a converted BAe 146 operated by the Facility for Airborne Atmospheric Measurements (FAAM). With a range of 2000 nautical miles, the FAAM aircraft is capable of operating all over the world and it has taken part in science campaigns in over 30 different countries since 2004. The aircraft can fly as low as 50 feet over the sea and sustain flight at 100 feet high. The service ceiling is nearly 11 km high. Typically, flights will last anywhere between one and six hours, and we will carry up to 18 scientists onboard, who guide the mission and support the operation of up to 4 tonnes of scientific equipment. Currently, the aircraft is undergoing a £49 million mid-life upgrade (MLU) program, which will extend its lifetime to at least 2040. The three overarching objectives of the MLU are to:

Safeguard the UK’s research capability – allowing the facility to meet the needs of the research community, enhance the range of services available, and respond to environmental emergencies.

Provide frontier science capability – meeting new and existing research needs and supporting ground-breaking science discoveries, with a flexible and world-class airborne laboratory.

Reduce environmental impact – maintaining and improving the performance of the facility, and minimising emissions and resource use from aircraft operation.

Presented here will be a brief history of the aircraft operations, including example science outcomes from all flights all over the world. In addition, detail of the ongoing upgrades, in particular the new and cutting-edge measurement capability for gases, aerosols, clouds, radiation and meteorology. Also presented will be the expected reductions in environmental impact of the aircraft and how these will be monitored.

How to cite: Lee, J.: The FAAM large atmospheric research aircraft: a brief history and future upgrades, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3473, https://doi.org/10.5194/egusphere-egu23-3473, 2023.

EGU23-6620 | ECS | Posters on site | GI3.3

Airborne observations over the North Atlantic Ocean reveal the first gas-phase measurements of urea in the atmosphere 

Emily Matthews, Thomas Bannan, M. Anwar Khan, Dudley Shallcross, Harald Stark, Eleanor Browne, Alexander Archibald, Stéphane Bauguitte, Chris Reed, Navaneeth Thamban, Huihui Wu, James Lee, Lucy Carpenter, Ming-xi Yang, Thomas Bell, Grant Allen, Carl Percival, Gordon McFiggans, Martin Gallagher, and Hugh Coe

Despite the reduced nitrogen (N) cycle being central to global biogeochemistry, there are large uncertainties surrounding its sources and rate of cycling. Here, we present the first observations of gas-phase urea (CO(NH₂)₂) in the atmosphere from airborne high-resolution mass spectrometer measurements over the North Atlantic Ocean. We show that urea is ubiquitous in the marine lower troposphere during the Summer, Autumn and Winter flights but was found to be below the limit of detection during the Spring flights. The observations suggest the ocean is the primary emission source but further studies are required to understand the processes responsible for the air-sea exchange of urea. Urea is also frequently observed aloft due to long-range transport of biomass-burning plumes. These observations alongside global model simulations point to urea being an important, and as yet unaccounted for, component of reduced-N to the remote marine environment.  Since we show it readily partitions between gas and particle phases, airborne transfer of urea between nutrient rich and poor parts of the ocean can occur readily and could impact ecosystems and oceanic uptake of CO2, with potentially important atmospheric implications.  

How to cite: Matthews, E., Bannan, T., Khan, M. A., Shallcross, D., Stark, H., Browne, E., Archibald, A., Bauguitte, S., Reed, C., Thamban, N., Wu, H., Lee, J., Carpenter, L., Yang, M., Bell, T., Allen, G., Percival, C., McFiggans, G., Gallagher, M., and Coe, H.: Airborne observations over the North Atlantic Ocean reveal the first gas-phase measurements of urea in the atmosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6620, https://doi.org/10.5194/egusphere-egu23-6620, 2023.

EGU23-7804 | Posters virtual | GI3.3

In-situ trace-gas measurements from the ground to the stratosphere by an OF-CEAS balloon-borne instrument 

Valery Catoire, Chaoyang Xue, Gisèle Krysztofiak, Patrick Jacquet, Michel Chartier, and Claude Robert

Monitoring climate change and stratospheric ozone budget requires accurate knowledge of the abundances of greenhouse gases and ozone depleting substances from the lower troposphere to the stratosphere. An infrared laser absorption spectrometer called SPECIES (acronym for SPECtromètre Infrarouge à lasErs in Situ) has been developed for balloon-borne trace gases measurements.

The complete instrument has been validated on the occasion of a flight in August 2021 in the polar region (Kiruna, Sweden) within the frame of the “KLIMAT 2021” campaign managed by CNES for the “MAGIC” project using concomitant balloon and aircraft flights. Results of this flight concerning CH4 and CO2 will be presented.

How to cite: Catoire, V., Xue, C., Krysztofiak, G., Jacquet, P., Chartier, M., and Robert, C.: In-situ trace-gas measurements from the ground to the stratosphere by an OF-CEAS balloon-borne instrument, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7804, https://doi.org/10.5194/egusphere-egu23-7804, 2023.

EGU23-7986 | ECS | Posters on site | GI3.3

Ship emissions and apparent sulphur fuel content measured of board of a large research aircraft in international waters and Sulphur Emission Control Area 

Dominika Pasternak, James Lee, Beth Nelson, Magdalini Alexiadou, Loren Temple, Stéphane Bauguitte, Steph Batten, James Hopkins, Stephen Andrews, Emily Mathews, Thomas Bannan, Huihui Wu, Navaneeth Thamban, Nicholas Marsden, Ming-Xi Yang, Thomas Bell, Hugh Coe, and Keith Bower

Since 1st January 2020 the legal sulphur content of shipping fuel was decreased – from 3.5% to 0.5% by mass outside of the Sulphur Emission Control Areas (SECAs) to improve coastal air quality. A possible downside of this change was acceleration of climate change since sulphur is believed to be a negative climate forcer and sipping is one of its main sources. Further question was the level of compliance to the new rules, especially in the open waters. Another climate related aspect of shipping is recent growth in the liquified natural gas (LNG) tanker fleets. LNG is considered the greenest of the fossil fuels, however there are few empirical studies of methane emissions from marine LNG transport.

The Atmospheric Composition and Radiative forcing changes due to UN International Ship Emissions regulations (ACRUISE) project aims to address the above considerations. During three field campaigns the FAAM Airborne Laboratories’ large research aircraft was deployed to target ships in coastal shipping lanes and open waters. First measurements were performed in July 2019 (before regulation change) in shipping lanes along the Portuguese coast, the English Channel SECA and the Celtic Sea. Further two campaigns were delayed by the COVID-19 pandemic until September 2021 and April 2022, targeting ships in the Bay of Biscay, the English Channel SECA and the Celtic Sea. Throughout the project, nearly 300 ships were measured during 30 research flights, varying from plume aging and cloud interaction studies, through collecting bulk statistics in busy shipping lanes to comparing emissions in and out of SECA. This work focuses on the gaseous species measurements (SO2, CO2, CH4 and VOCs from whole air samples). They are used to study changes in apparent sulphur fuel content of the ships observed throughout ACRUISE, plume composition and methane emissions from LNG tankers.

How to cite: Pasternak, D., Lee, J., Nelson, B., Alexiadou, M., Temple, L., Bauguitte, S., Batten, S., Hopkins, J., Andrews, S., Mathews, E., Bannan, T., Wu, H., Thamban, N., Marsden, N., Yang, M.-X., Bell, T., Coe, H., and Bower, K.: Ship emissions and apparent sulphur fuel content measured of board of a large research aircraft in international waters and Sulphur Emission Control Area, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7986, https://doi.org/10.5194/egusphere-egu23-7986, 2023.

EGU23-8329 | ECS | Posters on site | GI3.3 | Highlight

Airborne remote sensing research infrastructure for strengthening science, international collaboration and capacity building in the Arctic 

Shridhar Jawak, Agnar Sivertsen, William D. Harcourt, Rudolf Denkmann, Ilkka Matero, Øystein Godøy, and Heikki Lihavainen

Svalbard Integrated Arctic Earth Observing System (SIOS) is an international collaboration of 28 scientific institutions from 10 countries to build a collaborative research infrastructure that will enable better estimates of future environmental and climate changes in the Arctic. SIOS' mission is to develop an efficient observing system in Svalbard, share technology and data using FAIR principles, fill knowledge gaps in Earth system science and reduce the environmental footprint of science in the Arctic. This study presents SIOS' efforts to strengthen science, international collaboration and capacity building in the high Arctic archipelago of Svalbard through its airborne research infrastructure. SIOS supports the coordinated usage of its airborne remote sensing resources such as the Dornier aircraft and uncrewed aerial vehicles (UAVs) for improved research activities in Svalbard, complementing in situ and space-borne measurements and reducing the environmental footprint of research in Svalbard. Since 2019, SIOS in collaboration with its member institution Norwegian Research Centre (NORCE) installed, tested, and operationalised optical imaging sensors in the Lufttransport Dornier (DO228) passenger aircraft stationed in Longyearbyen under the SIOS-InfraNor project making it compatible with research use in Svalbard. Two optical sensors are installed onboard the Dornier aircraft; (1) the PhaseOne IXU-150 RGB camera and (2) the HySpex VNIR-1800 hyperspectral sensor. The aircraft with these cameras is configured to acquire aerial RGB imagery and hyperspectral remote sensing data in addition to its regular logistics and transport operation in Svalbard. Since 2020, SIOS has supported and coordinated around 50 flight hours to acquire airborne data using the Dornier aircraft and UAVs in Svalbard supporting around 20 scientific projects. The use of airborne imaging sensors in these projects enabled a variety of applications within glaciology, biology, hydrology, and other fields of Earth system science: Mapping glacier crevasses, generating DEMs for glaciological applications, mapping and characterising earth (e.g., minerals, vegetation), ice (e.g., sea ice, icebergs, glaciers and snow cover) and ocean surface features (e.g., colour, chlorophyll). The use of passenger aircraft warrants the following benefits: (1) regular logistics and research activities are optimally coordinated to reduce flight hours in carrying scientific observations, (2) project proposals for the usage of aircraft-based measurements facilitate international collaboration, (3) measurements conducted during 2020-21 are useful in filling the gaps in field based observations occurred due to the Covid-19 pandemic, (4) airborne data are used to train polar scientists as a part of the annual SIOS training course and upcoming data usability contest, (5) data is also useful for Arctic field safety as it can be used to make products such as high-resolution maps of crevassed areas on glaciers. In short, SIOS airborne remote sensing activities represent optimized use of infrastructure, promote capacity building, Arctic safety and facilitate international cooperation.

How to cite: Jawak, S., Sivertsen, A., Harcourt, W. D., Denkmann, R., Matero, I., Godøy, Ø., and Lihavainen, H.: Airborne remote sensing research infrastructure for strengthening science, international collaboration and capacity building in the Arctic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8329, https://doi.org/10.5194/egusphere-egu23-8329, 2023.

EGU23-11813 | Posters on site | GI3.3

First evaluation of a 6-months Meteodrone campaign 

Maxime Hervo, Julie Pasquier, Lukas Hammerschmidt, Tanja Weusthoff, Martin Fengler, and Alexander Haefele

 From December 2021 to May 2022, MeteoSwiss conducted a proof of concept with Meteomatics to demonstrate the capability of drones to provide data of sufficient quality and reliability on a routine operational basis. Meteodrones MM-670 were operated automatically 8 times per night at Payerne, Switzerland. 864 meteorological profiles were measured and compared to co-localized measurements including radiosoundings and remote-sensing instruments. To our knowledge, it is the first time that Meteodrone measurements are evaluated in such an intensive campaign.

The availability of the Meteodrone measurements over the whole campaign was 75.7% with 82.2% of the flights reaching the nominal altitude of 2000m above sea level. Using the radiosondes as a reference, the quality of the Meteodrone measurements can be quantified according to WMO requirements (WMO OSCAR , 2022). Applying this method, the temperature measured by the Meteodrone can be considered as a “breakthrough”, meaning that they are a significant improvement if they are used for high resolution Numerical Weather Prediction. The Meteodrone’s humidity and wind profiles are classified as “useful” for high-resolution numerical weather predictions, suggesting they can be used for assimilation in numerical models. The quality is similar compared to the temperature measured by a microwave radiometer and the humidity measured by a Raman Lidar. However, the wind measured by a Doppler Lidar was more accurate than the estimation of the Meteodrone.

This campaign opens the door for operational usage of automatic drones for meteorological applications.

How to cite: Hervo, M., Pasquier, J., Hammerschmidt, L., Weusthoff, T., Fengler, M., and Haefele, A.: First evaluation of a 6-months Meteodrone campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11813, https://doi.org/10.5194/egusphere-egu23-11813, 2023.

EGU23-13766 | ECS | Posters on site | GI3.3

How inlet tubing material affects the response time of water vapor concentration measurements 

Markus Miltner, Tim Stoltmann, and Erik Kerstel

Measurements involving water in the vapor phase have to deal with the stickiness of the H2O molecule: The associated adsorption and desorption processes can increase the response time of these measurements significantly. To achieve short response times in scientific instrument design, hydrophobic surface materials are used to reduce surface interactions in the tubing that guides the sample towards the analyzer. The study presented here focuses on the effects of the tubing material choice, length, humidity level, gas flow rate, and temperature on the observed response time. We use an Optical Feedback Cavity Enhanced Absorption Spectrometer (OFCEAS) designed for stable water isotope measurements at low water concentration (< 1000 ppm), which we connect to two bottles containing humidified synthetic air of different water concentration using 6.6-m tubing of different materials and surface treatments. Other parameters that are varied are the flow rate and the temperature of the tubing. With proper selection of tubing material and surface treatment, the contribution from the tubing to the overall response time for low water concentration isotopic measurements can be sufficiently suppressed for it to be neglected.

How to cite: Miltner, M., Stoltmann, T., and Kerstel, E.: How inlet tubing material affects the response time of water vapor concentration measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13766, https://doi.org/10.5194/egusphere-egu23-13766, 2023.

EGU23-14164 | ECS | Posters virtual | GI3.3

Multi-angular airborne thermal observations: A new hyperspectral setup for simulating thermal radiation and emissivity directionality at the satellite scale 

Mary Langsdale, Callum Middleton, Martin Wooster, Mark Grosvenor, and Dirk Schuettemeyer

Land Surface Temperature (LST) is a key parameter to the understanding and modelling of many Earth system processes. Viewing and illumination geometry are known to have significant impacts on remotely sensed retrieval of LST, particularly for heterogeneous regions with mixed components. However, it is difficult to accurately quantify these impacts, in part due to the challenges of retrieving high-quality data for the different components in a scene at a variety of different viewing and illumination geometries over a time period where the real surface temperature and sun-sensor geometries are invariant. Previous field studies have attempted this through observations with aircraft-mounted single-band thermal cameras to further understanding of real-world conditions, but these sensors have limited accuracies and cannot be used to consider the angular variability of emissivity or to simulate multi-band satellite observations.

To redress this, the National Centre for Earth Observation’s Airborne Earth Observatory (NAEO) have developed and manufactured a modified mount for their state-of-the-art commercial pushbroom longwave hyperspectral airborne sensor, the Specim AisaOWL (102 narrowband channels across the 7.6 – 12.6 µm region). When mounted in standard mode, the field-of-view of the OWL sensor is 24° (± 12°), however the modified mount enables off-nadir measurements up to 48°. This has the potential to evaluate both thermal radiation and spectral emissivity directionality up to and beyond the view angles of most thermal satellite sensors. With LST now classified as an Essential Climate Variable, this work is particularly relevant as it will help to improve the accuracy of retrievals from current and future satellites (e.g. LSTM, SBG, TRISHNA).

In this presentation, we first present an overview of the design modifications that enable these high-angle observations and preliminary results from test flights before detailing how this setup will be used in an upcoming joint ESA-NASA campaign dedicated to quantifying and simulating thermal radiation directionality over agricultural regions at the satellite scale.

How to cite: Langsdale, M., Middleton, C., Wooster, M., Grosvenor, M., and Schuettemeyer, D.: Multi-angular airborne thermal observations: A new hyperspectral setup for simulating thermal radiation and emissivity directionality at the satellite scale, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14164, https://doi.org/10.5194/egusphere-egu23-14164, 2023.

EGU23-14187 | ECS | Posters on site | GI3.3

Aircraft observations of NH3 from agricultural sources 

Lara Noppen, Lieven Clarisse, Frederik Tack, Thomas Ruhtz, Alexis Merlaud, Martin Van Damme, Michel Van Roozendael, Dirk Schuettemeyer, and Pierre Coheur

Ammonia (NH3) is mainly emitted in the atmosphere by anthropogenic activities, especially by agriculture. Excess emissions greatly disturb ecosystems, biodiversity, and air quality. Despite our awareness of these deleterious consequences, NH3 concentrations are increasing in most industrialized countries. This underlines the need for more stringent regulations and good knowledge of the species gained through effective monitoring.

Since a decade, NH3 is monitored from space, daily and globally, with thermal infrared sounders. However, their coarse spatial resolution (above 10 km) renders accurate quantification of NH3 sources particularly challenging. Indeed, only the largest and most isolated NH3 point sources have been identified and quantified from current observations and often only by exploiting long-term averages. To address the urgent need for better constraining NH3 emissions, a new satellite, called Nitrosat, has been proposed in response to the 11th ESA’s Earth Explorer call. The mission aims at mapping simultaneously NO2 and NH3 at a spatial resolution of 500 m at a global scale. With the support of ESA, almost 30 aircraft demonstration flights took place in Europe between 2020 and 2022. These flights mapped gapless areas of at least 10 by 20 km containing various sources of NO2 and NH3 using two instruments: the SWING instrument targeting NO2 in the UV-VIS and Hyper-Cam LW measuring infrared spectra to observe NH3.

Here we present NH3 observations from campaigns performed in Italy in spring 2022. The Po Valley was the main target, as it is the largest (agricultural) hotspot of NH3 in Europe.  Despite the presence of large background concentrations in the Po Valley, we show that the infrared measurements are able to expose a multitude of local agricultural hotspots such as cattle farms. A particularly successful campaign covering the region from Vetto to Colorno demonstrates measurement sensitivity to the gradual increase of NH3 background concentrations outside and inside the Po Valley. We also discuss flights carried out further south in Italy targeting other emissions of NH3, such as those from a soda ash plant, and the emissions from a fertilizer release experiment that was organized in collaboration with a farmer. We present the measurements both at their native horizontal resolution of 4 m and downsampled at the 500 m resolution of Nitrosat.

How to cite: Noppen, L., Clarisse, L., Tack, F., Ruhtz, T., Merlaud, A., Van Damme, M., Van Roozendael, M., Schuettemeyer, D., and Coheur, P.: Aircraft observations of NH3 from agricultural sources, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14187, https://doi.org/10.5194/egusphere-egu23-14187, 2023.

EGU23-15334 | ECS | Posters on site | GI3.3

Global measurements of cloud properties using commercial aircraft 

Gary Lloyd and Martin Gallagher

In-Service Aircraft for a Global Observing System (IAGOS) is a European research infrastructure that uses the infrastructure of commercial aviation to make in-situ measurements of the atmosphere. We present data from the cloud sensing instrument installed on these aircraft between 2011 and 2021. This includes 1000s of flights across the globe that detect the concentration of cloud particles over the range 5-75 um and this provides information about seasonal variation in cloud frequency across different parts of the globe. From these measurements we are able to estimate properties such as Liquid/Ice Water Content (LWC/IWC), The Effective Diameter (ED) and Mean Volume Diameter (MVD).

How to cite: Lloyd, G. and Gallagher, M.: Global measurements of cloud properties using commercial aircraft, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15334, https://doi.org/10.5194/egusphere-egu23-15334, 2023.

EGU23-17533 | ECS | Posters on site | GI3.3

Synergy of active and passive airborne observations for the evaluation of the radiative impacts of aerosols. Application to the AEROCLO-SA field campaign in Namibia 

Mégane Ventura, Fabien Waquet, Gerard Brobgniez, Frederic Parol, Marc Mallet, Nicolas Ferlay, Oleg Dubovic, Philippe Goloub, Cyrille Flamant, and Paola Formenti

Aerosols have important effects on both local and global climate, as well as on clouds and precipitations. We present here some original results of the AErosol RadiatiOn and CLOud in Southern Africa (AEROCLO-sA) field campaign led in Namibia in August and September 2017. This region shows a strong response to climate change and is associated with large uncertainties in climate models. Large amounts of biomass burning aerosols emitted by vegetation fires in Central Africa are transported far over the Namibian deserts and are also detected over the stratocumulus clouds covering the South Atlantic Ocean along the coast of Namibia. Absorbing aerosols above clouds are associated with strong positive direct radiative forcing (warming) that are still underestimated in climate models (De Graaf etal.,2021). The absorption of solar radiation by absorbing above clouds may also cause a warming where the aerosol layer is located. This warming would alter the thermodynamic properties of the atmosphere, which would impact the vertical development of low-level clouds impacting the cloud top height and its brightness.

The airborne field campaign consisted in ten flights performed with the French F-20 Falcon aircraft in this region of interest. Several instruments were involved: the OSIRIS polarimeter, prototype of the next 3MI spaceborne instrument of ESA (Chauvigné etal.,2021), the LNG lidar, an airborne photometer called PLASMA, as well as fluxmeters and dropsondes used to measure thermodynamical quantities, supplemented with in situ aerosol measurements of particles size distribution.

In order to quantify the aerosols radiative impact on the Namibian regional radiative budget, we use an original approach that combines polarimeter and lidar data to derive heating rate of the aerosols. This approach is evaluated during massive transports of biomass burning particles. To calculate this parameter, we use a radiative transfer code and additional meteorological parameters, provided by the dropsondes. We will introduce, the flight of September 8, 2017, aerosol pollution was very important. Emissions and dust were carried along the Namibian coast, and an aerosol plume was observed above a stratocumulus. We will present vertical profiles of heating rates computed in the solar and thermal parts of the spectrum with this technique. Our results indicated particularly strong heating rate values retrieved above clouds due to aerosols, in the order of 8K per day, which is likely to perturbate the dynamic of the below cloud layers.

In order to validate and to quantify this new methodology, we used the flux measurements acquired during loop descents performed during dedicated parts of the flights, which provides unique measurements of flux distribution (upwelling and downwelling) and heating rates in function of the altitude.

Finally, we will discuss the possibility to apply this method to available spaceborne passive and active observations in order to provide the first estimates of heating rate profiles above clouds at global scale.

How to cite: Ventura, M., Waquet, F., Brobgniez, G., Parol, F., Mallet, M., Ferlay, N., Dubovic, O., Goloub, P., Flamant, C., and Formenti, P.: Synergy of active and passive airborne observations for the evaluation of the radiative impacts of aerosols. Application to the AEROCLO-SA field campaign in Namibia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17533, https://doi.org/10.5194/egusphere-egu23-17533, 2023.

EGU23-144 | ECS | Posters on site | BG2.2

Calibration of an optical methane clumped isotope thermometer 

Ivan Prokhorov, Béla Tuzson, Nico Kueter, Malavika Sivan, Maria Elena Popa, Thomas Röckmann, Lukas Emmenegger, Stefano M. Bernasconi, and Joachim Mohn

Methane clumped isotope thermometry relies on accurate measurements of relative abundances of the doubly-substituted isotopologues 12CH2D2 and 13CH3D. Calibration of the thermometer requires, regardless of the applied technique, i.e., laser absorption spectroscopy or high-resolution mass spectrometry, routine preparation of thermally re-equilibrated samples spanning the temperature and bulk isotopic composition (δ13C-, δD-CH4) range of the target applications.

Here we present a practical method for methane isotopologue re-equilibration over activated γ-Al2O3. We demonstrate complete and reproducible re-equilibration of clumped isotope signatures with minimal alteration of the bulk isotope composition, almost complete sample recovery, and no detectable formation of decomposition products. Samples spanning a range in δD-CH4 of 100 ‰ were equilibrated between 100 °C and 500 °C and used to calibrate a high-resolution quantum cascade laser absorption spectrometer. In addition, we report on a comparison between the spectroscopic measurements carried out at Empa and an independently calibrated high-resolution mass spectrometric technique using a Thermo MAT253 Ultra at IMAU, Utrecht University.

This study is supported by the European Commission under the Horizon 2020 – Research and Innovation Framework Programme, H2020-INFRAIA-2020-1 (grant no. 101008004) and the Swiss National Science Foundation project no. 200021_200977.

How to cite: Prokhorov, I., Tuzson, B., Kueter, N., Sivan, M., Popa, M. E., Röckmann, T., Emmenegger, L., Bernasconi, S. M., and Mohn, J.: Calibration of an optical methane clumped isotope thermometer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-144, https://doi.org/10.5194/egusphere-egu23-144, 2023.

EGU23-1424 | Posters on site | BG2.2

Satellite-based dry-wet seasonal changes of OCS surface budgets over the Amazon rainforests 

Lin Tan, King-Fai Li, Xun Jiang, Le Kuai, and Danie Liang

Carbonyl sulfide (OCS) is the most dominant sulfur-containing species in the atmosphere and is an important tracer of the terrestrial gross primary productivity as it is involved only in photosynthesis. Biomass burning and terrestrial uptakes by plants and soil is the primary terrestrial source and sink of OCS, respectively.  The Amazon basin alone accounts for 10% of the global biomass burning emission and 33% of the global plant/soil uptake. However, both terms are sensitive to water stress, heat stress, and the associated wildfires in the dry seasons. Here, we estimate the dry-wet seasonal difference of the terrestrial OCS budget over the Amazon region by constraining the NCAR MOZART4 chemistry-transport model with the mid-tropospheric OCS abundances retrieved from NASA’s Thermal Emission Spectrometer (TES) measurements during 2004 and 2012.  Our perturbative calculations show that biomass-burning emissions that are predominant in the south rim of the Amazon have more influence on the mid-tropospheric OCS over the southeast subtropical Amazon. In comparison, the plant/soil uptakes that are predominant in the tropical Amazon have more influence over the northwest tropical Amazon.  This dipole spatial pattern helps distinguish the mid-tropospheric OCS seasonal variability due to biomass-burning emissions and plant/soil uptakes.

How to cite: Tan, L., Li, K.-F., Jiang, X., Kuai, L., and Liang, D.: Satellite-based dry-wet seasonal changes of OCS surface budgets over the Amazon rainforests, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1424, https://doi.org/10.5194/egusphere-egu23-1424, 2023.

Combining measurements, modeling and machine learning to improve N2O accounting for sustainable agricultural development in sub-Saharan Africa

 

  • Ouma1,2, E. Harris1, M. Barthel2, J. Six2, A. Otinga3, R. Njoroge3, F. Perez-Cruz1, S. Leitner4

 

1 Swiss Data Science Centre, ETH Zurich, 8092 Zurich, Switzerland

2 Department of Environmental Systems Science, ETH Zurich, Switzerland

3 Department of Soil Science, University of Eldoret, Eldoret, Kenya

4 International Institute of Livestock Research (ILRI), Nairobi, Kenya

 

Sub-Saharan Africa continues to grapple with food insecurity due to low crop yields. While an increase in synthetic fertilisers could potentially increase agricultural productivity in the region, it would lead to an increase in emissions of nitrous oxide (N2O). Moreover, in this region, the lack of quantification of parameters and documentation of the processes relevant to N2O emissions have hampered the adoption of climate-smart agricultural practices and advancement of N2O inventories. This study aims to conduct the first online measurements of N2O fluxes and isotopic composition from agricultural soils in Uasin Gishu County, Kenya, using the TREX-QCLAS system: quantum cascade laser absorption spectrometer (QCLAS) coupled to a preconcentration unit-TRace gas EXtractor (TREX). The isotopic measurements obtained will be useful in the inference of N2O production and consumption rates for different pathways and will improve understanding of the key drivers of variability in tropical cropland N2O fluxes. Further, a collation and analysis of available N2O flux and isotope data along with campaign measurements and data science approaches will enhance the potential to predict future emissions and promote the development of targeted mitigation strategies.

 

A pilot phase of initial flux measurements set at the plant research station in Eschikon, Switzerland in early 2023 using the TREX-QCLAS system coupled with automated dynamic chambers optimised for continuous unattended N2O flux measurements will be conducted before deployment in Kenya. Using clover and grass plots, we aim to understand N2O fluxes and drivers in a simple system. N2O measurements will be based on a three-stage calibration protocol (preconcentrated ambient air, preconcentrated compressed air, and calibration of the instrumental concentration dependence using progressive dilution of the anchor standard) followed by measurement of chamber air. Preliminary results of automated quality control and data analysis procedures will be key to ensure success of the instrumental deployment in Kenya in late 2023.

 

References:

  • Harris, E., Diaz-Pines, E., Stoll, E., Schloter, M., Schulz, S., Duffner, C., Li, K., Moore, K. L., Ingrisch, J., Reinthaler, D., Zechmeister-Boltenstern, S., Glatzel, S., Brüggemann, N., & Bahn, M. (2021). Denitrifying pathways dominate nitrous oxide emissions from managed grassland during drought and rewetting. Science advances, 7(6), eabb7118. https://doi.org/10.1126/sciadv.abb7118

 

  • Ibraim, E., Denk, T., Wolf, B., Barthel, M., Gasche, R., Wanek, W., … Mohn, J. (2020). Denitrification is the main nitrous oxide source process in grassland soils according to quasi‐continuous isotopocule analysis and biogeochemical modeling. Global Biogeochemical Cycles, 34(6), e2019GB006505 (19 pp.). https://doi.org/10.1029/2019GB006505

 

How to cite: Ouma, T.: Combining measurements, modeling and machine learning to improve N2O accounting for sustainable agricultural development in sub-Saharan Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1731, https://doi.org/10.5194/egusphere-egu23-1731, 2023.

EGU23-1754 | ECS | Orals | BG2.2

Stratospheric observations of carbonyl sulfide using AirCore and LISA 

Alessandro Zanchetta, Steven van Heuven, Michel Ramonet, Thomas Laemmel, Jin Ma, Maarten Krol, and Huilin Chen

Carbonyl sulfide (COS) is a long-lived sulfur compound present in the atmosphere with an average mole fraction of around 450-500 ppt, and has been suggested as a potential tracer to partition gross primary production (GPP) and net ecosystem exchange (NEE) in plants’ photosynthesis, possibly by satellite observations. However, its sources and sinks have not been fully understood, and remote sensing observations of COS still require validation and to be linked with a reference measurement scale, e.g., NOAA’s. In this work, we have made vertical profiles of COS mole fractions using AirCore at Trainou, France (47°58' N, 2°6' E), in June 2019, and at Kiruna, Sweden (67°53' N, 21°04' E) in August 2021, using both AirCore and a new version of lightweight stratospheric air (LISA) sampler. Besides COS, simultaneous measurements of CO2, CO, CH4 and N2O have also been made. These results will be compared with COS simulations from the TM5-4DVAR modeling system to get a better understanding of the behavior of this species in the stratosphere, i.e., the sources and the sinks COS, as well as vertical structures due to atmospheric transport. These will be helpful to improve our understanding of the budget and the variabilities of COS in the stratosphere, and advance the use of remote sensing observations of COS from satellite and ground-based spectrometers to study the carbon cycle.  

How to cite: Zanchetta, A., van Heuven, S., Ramonet, M., Laemmel, T., Ma, J., Krol, M., and Chen, H.: Stratospheric observations of carbonyl sulfide using AirCore and LISA, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1754, https://doi.org/10.5194/egusphere-egu23-1754, 2023.

Isotopocules of the greenhouse gas nitrous oxide (N2O), i.e. δ18O, average δ15N (δ15Nbulk), and 15N site preference (SP) values were used to distinguish between N2O production pathways in soil. However, as many N2O production pathways coexist and N2O can be reduced to N2, it is not possible to distinguish pathways based only on the natural abundance of N2O. This applies especially to nitrification and fungal denitrification, where the specific high SP values overlap. Combining 15N tracer approaches and natural abundance approaches (especially using SP values) could serve to disentangle such pathways, but with the disadvantage that both approaches have to be carried out as parallel experiments.

With this contribution, we present an experimental concept based on the theory, that low level labelling with 15N of N2O precursors may allow both, a clear distinction of nitrate or ammonium (NO3- or NH4+, respectively) derived N2O fluxes by 15N tracing, and the use of SP values of N2O as additional constraint. This could potentially expand possibilities to evaluate and validate current natural abundance isotopocule mapping approaches.

We will present first results of three experiments to investigate the impact of low labelled precursors on SP values of N2O produced. Each experiment included treatments with unlabeled and low labelled 15N precursors to test if low labelling with 15N affects N2O isotopocules. In one incubation experiment (i) various levels of 15N labelling of NO3- (between 0.6 and 5 at% 15N) were used for incubations with Pseudomonas aureofaciens. In another experiment (ii) two pure bacterial (P. aureofaciens and Paracoccus denitrificans) and one pure fungal culture (Fusarium oxysporum) known to be capable of reducing NO3- or NO2-, respectively, were used. In all experiments, isotopocules of N2O were unaffected by N2O reduction as this reduction step could be excluded with selected species. To further investigate isotopocules of N2O affected by co-occuring processes as well as N2O reduction a third incubation experiment with two repacked soils was conducted. For this approach, nitrification and/or denitrification was induced by applying NH4SO4 and KNO3 as N2O precursors, either unlabeled in one treatment or with 15N labelled KNO3 (max. 1.1 at% 15N) in another treatment, both under dry (40% water filled pore space (WFPS)) or wet (80% WFPS) soil conditions.

Based on the results presented, we will be able to give an outlook whether this method can be used to distinguish between nitrification and fungal denitrification.

How to cite: Rohe, L. and Well, R.: Combining low level labelling with 15N and 15N site preference to distinguish N2O production by nitrification and fungal denitrification, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4990, https://doi.org/10.5194/egusphere-egu23-4990, 2023.

EGU23-5286 | ECS | Orals | BG2.2

Carbon and water fluxes of the boreal evergreen needleleaf forest biome constrained by assimilating ecosystem carbonyl sulfide flux observations 

Camille Abadie, Fabienne Maignan, Marine Remaud, Kukka-Maaria Kohonen, Wu Sun, Linda Kooijmans, Timo Vesala, Ulli Seibt, Nina Raoult, Vladislav Bastrikov, Sauveur Belviso, and Philippe Peylin

Boreal forests absorb a significant amount of atmospheric CO2 through gross primary production (GPP), representing about 20% of the global GPP. However, direct observations of GPP over the whole boreal region are not available as plant photosynthetic rate cannot be measured at scales larger than the leaf scale. At large scales, Land Surface Models (LSMs) can simulate GPP but the lack of direct GPP measurements makes it challenging to evaluate and improve the GPP representation in LSMs. In addition, boreal forests are highly sensitive to environmental changes, impacting gas exchanges and leading to high uncertainties in GPP estimates simulated by LSMs or obtained from data driven methods. Carbonyl sulfide (COS) has emerged as a promising proxy to infer GPP estimates or to better constrain GPP representation in LSMs. Because COS is absorbed by vegetation following the same diffusion pathway as CO2 during photosynthesis and not emitted back to the atmosphere, implementing a mechanistic representation of vegetation COS uptake in LSMs allows using COS data to constrain GPP representation. In this study, we performed ecosystem COS flux and GPP assimilations to constrain the COS and GPP related parameters in the ORCHIDEE LSM. We focused on Hyytiälä forest, where the longest time-series of ecosystem COS flux measurements was reported. We found that assimilating ecosystem COS fluxes increases the estimated net ecosystem COS uptake by 14%. However, a persistent underestimation of the ecosystem COS flux seasonal amplitude after data assimilation points towards structural errors in the COS model, possibly related to COS internal conductance representation. In comparison with an assimilation of GPP only, adding ecosystem COS flux assimilation leads to a stronger reduction in the stomatal conductance, highlighting the potential of COS to inform stomatal diffusion. Consequently, including COS data in the assimilations also impacts the resulting latent heat flux and water use efficiency. Finally, we scaled up this assimilation framework to the boreal region and found that the joint assimilation of COS and GPP fluxes increased the modeled vegetation COS uptake up to 18%, but not the GPP budget. This contrasts with previous inversion studies that simultaneously increase vegetation COS uptake and GPP budgets based on a linear relationship relating the two. 

How to cite: Abadie, C., Maignan, F., Remaud, M., Kohonen, K.-M., Sun, W., Kooijmans, L., Vesala, T., Seibt, U., Raoult, N., Bastrikov, V., Belviso, S., and Peylin, P.: Carbon and water fluxes of the boreal evergreen needleleaf forest biome constrained by assimilating ecosystem carbonyl sulfide flux observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5286, https://doi.org/10.5194/egusphere-egu23-5286, 2023.

EGU23-5713 | ECS | Orals | BG2.2

Sources of oceanic carbonyl sulfide revealed by sulfur isotopes measurements 

Chen Davidson, Yasmin Avidani, Alon Angert, Sinikka Lennartz, and Alon Amrani

Carbonyl sulfide (COS) is the major long-lived sulfur gas in the troposphere, and an important precursor for stratospheric sulfate aerosols, which increases earth’s albedo. The main sink of COS is the uptake by terrestrial plants, in a similar pathway to CO2. Therefore, COS is used as a promising proxy for CO2 removal by terrestrial plants (gross primary production, GPP), which regulates the earth’s climate. Currently, COS budget estimates have large uncertainties associated with the magnitude of COS sources and sinks. The COS ocean-atmosphere flux is the largest natural source of tropospheric COS, however, its magnitude is at the heart of a scientific debate with estimates ranging between  200 to 800 Ggr S Yr-1 [1-2].

Sulfur isotopes measurements (34S/32S; δ34S) are recently used in an isotopic mass-balance to constrain the COS budget, assuming each end-member has a unique isotopic signature [3]. However, in our previous work [3], we estimated the isotopic signature of the ocean-atmosphere COS flux, based on limited samples from the Mediterranean and Red Seas, which may not be representative of the oceans. In the current work, we present measurements of photochemistry experiments and natural samples from the Atlantic Ocean, sampled during dawn, afternoon, and sunset. Atlantic Ocean samples that were taken during dawn (min COS concentrations) show δ34S value of 14±2‰ (n=8, one outlier with δ34S value of 19.2‰ was excluded). However, samples taken during the afternoon (max concentration) show heavier δ34S values of 18±1‰ (n=6).  This significant difference in δ34S values between dawn and afternoon (P-value 0.0003) indicates that COS “dark production” is associated with an isotopic fractionation that produces isotopically lighter COS, supporting the hypothesis that COS “dark production” is related to biotic processes. While COS photoproduction is associated with heavier isotopic values, which we assume are closer to the δ34S value of its biogenic source. This assumption is also supported by our photochemistry experiments, which indicate a small isotopic fractionation of COS photoproduction from cysteine (≤1‰). The isotopic signatures we present here will be used to better understand the main processes controlling oceanic COS production, and better constrain the ocean-atmosphere COS flux.   

 

[1] Lennartz, Sinikka T., et al. "Marine carbonyl sulfide (OCS) and carbon disulfide (CS2): a compilation of measurements in seawater and the marine boundary layer." Earth system science data 12.1 (2020): 591-609.

[2] Berry, Joe, et al. "A coupled model of the global cycles of carbonyl sulfide and CO2: A possible new window on the carbon cycle." Journal of Geophysical Research: Biogeosciences 118.2 (2013): 842-852.

[3] Davidson, Chen, Alon Amrani, and Alon Angert. "Tropospheric carbonyl sulfide mass balance based on direct measurements of sulfur isotopes." Proceedings of the National Academy of Sciences 118.6 (2021): e2020060118.

How to cite: Davidson, C., Avidani, Y., Angert, A., Lennartz, S., and Amrani, A.: Sources of oceanic carbonyl sulfide revealed by sulfur isotopes measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5713, https://doi.org/10.5194/egusphere-egu23-5713, 2023.

EGU23-6222 | ECS | Posters on site | BG2.2

The formation and transport of nitrogen-containing species in aerosols over central mountain area of Taiwan using isotope analysis 

Ming-Hao Huang, Ting-Yu Chen, Haojia Ren, and Hui-Ming Hung

Particulate matter (PM) is one major air pollutant that affects human health and the radiation balance of the earth. Thus, it is essential to identify the sources of air pollutants to provide feasible control strategies. In this study, we investigated the size-dependent 15N and 18O isotope ratio of N-containing species in aerosols to specify their sources, transport, and formation processes. Aerosol samples of different size ranges were collected using a micro-orifice uniform deposit impactor (MOUDI) on a half-day basis over Xitou Experimental Forest of National Taiwan University (23.40°N, 120.47°E, 1178 m a.s.l.) site at the valley southwest to the central Metropolitan of Taiwan in April 2021. Due to its location and topography, Xitou is downstream of the local circulation, which is dominated by the land-sea breeze and mountain-valley wind and brings the pollutants from the coastal industrial and agricultural activities to the forest during the daytime. Therefore, the samples collected at Xitou are a mixture of complex information. Chemical functional groups measurement was performed using Fourier-transform infrared spectroscopy with attenuated total reflection (FTIR-ATR) technique beforehand to provide a grasp of the concentration-size distribution for both nitrate and ammonium as a reference to ensure sufficient nitrogen requirement for further isotope analysis at gas chromatography–isotope ratio mass spectrometer (GC-IRMS). The daily average concentration is 3.78±1.82 and 2.47±2.47 ug/m3 for ammonium (NH4+) and nitrate (NO3), respectively. The concentration during daytime is higher than at nighttime by a factor of 1.3-1.8. The result suggests that pollutants brought by the sea breeze windward contribute to nitrogen-containing aerosols. During a persistent 24-hour weak wind fog event, a significant concentration decreases for both substances (NH4+: 5.34 to 2.12 ug/m3 and NO3: 4.62 to 0.56 ug/m3) in PM10, likely due to sedimentation. The observed δ15N in NO3 increasing with diameter suggests NO3 at larger particles formed at the upper stream and NO3 at finer particles formed locally. On the other hand, δ18O in nitrate shows a similar trend which might be the contribution of RO2 as the oxidant locally. As NH4+ in aerosols is contributed by ammonia partitioning, δ15N-NH4+ only reflects the fractionation process during phase change and initial emission. The size-dependent trend of δ15N-NH4+ shows similar behavior to our previous study in December 2018 and reflects the time points of partitioning. Furthermore, the quantitative analysis of the transport and formation processes based on the size-dependent isotope will be deconvoluted to understand the partitioning of N-containing species in aerosols, which would be necessary for the pollution control strategy and their impact evaluation.

How to cite: Huang, M.-H., Chen, T.-Y., Ren, H., and Hung, H.-M.: The formation and transport of nitrogen-containing species in aerosols over central mountain area of Taiwan using isotope analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6222, https://doi.org/10.5194/egusphere-egu23-6222, 2023.

EGU23-6260 | Posters on site | BG2.2

Tracking Biogenic Carbon in Liquid Fuel Blends using Conventional Mass Spectrometry and Infrared Spectroscopy 

Scott Herndon, David Nelson, Sophie Lehmann, Alejandro Heredia-Langner, James Moran, and J. Timothy Bays

This work demonstrates the analytical basis for an IR (isotope ratio) laser measurement system with the potential to perform routine quantification of biogenic carbon content in liquid fuel products at working refineries. We will present the performance potential for routine quantification for mixtures of C3 and C4 biogenic carbon sources mixed with fossil feedstock.  We will show the progress toward an operational on-line portable monitor. Initial work employed a predilution stage that required challenging transfer techniques to suppress fractionation.  More recent work has explored the potential for the IR based apparatus to directly quantify stable isotopologues that are isobaric in IRMS (isotope ratio mass spectrometry) instruments. The IR system results for 13CO2/12CO2 compare favorably with gold-standard IRMS. 

How to cite: Herndon, S., Nelson, D., Lehmann, S., Heredia-Langner, A., Moran, J., and Bays, J. T.: Tracking Biogenic Carbon in Liquid Fuel Blends using Conventional Mass Spectrometry and Infrared Spectroscopy, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6260, https://doi.org/10.5194/egusphere-egu23-6260, 2023.

EGU23-6847 | ECS | Posters on site | BG2.2

Isotopic fractionation of sulfur during COS hydrolysis 

Yasmin Avidani, Chen Davidson, Alon Angert, and Alon Amrani

Carbonyl Sulfide (COS) is the most abundant sulfur-containing gas in the atmosphere, and it is used as a proxy for terrestrial gross primary productivity (GPP). There are uncertainties in the COS fluxes estimations that limit this approach. Oceans are the major source of COS to the atmosphere. In the oceans, the COS is produced by photochemical reactions and "dark production", whose mechanism is not well understood. Hydrolysis is the major process that removes COS from the ocean's surface. Identifying the sulfur isotope values (δ34S) and the isotopic fractionation (e) associated with these major sources and sinks could decrease the uncertainties in the fluxes, based on an improved COS global model with an isotopic mass balance [1]. In the current study, we aim to determine the e  during the hydrolysis process of COS (eh).  We use a purge and trap system coupled to a GC/MC-ICPMS to measure δ34S values during hydrolysis under different pH, salinity (S), and temperature, representing various oceanic conditions. We calculate from our δ34S and COS concentration measurements a eh of −2.6 ± 0.3‰ in natural seawater from the Gulf of Aqaba (pH 8.2, 22 , S=41‰). Using an artificial solution at similar pH and temperature conditions (pH 8.0, 22 , S=0.2‰) we found eh of −2.3 ± 0.2‰, hence, salinity has no significant effect on the fractionation. Using the same artificial solution at 4   we found eh  of −3.9 ± 0.2‰, thus fractionation increases with decreasing temperatures, as can be expected from theory. We will also report the effect of acidity on eh from experiments in pH of 4 and 9 (at 22 ). This information on the eh will help us to understand the contribution of COS hydrolysis to the oceanic source and in the future to establish an isotope mass balance model to decrease the uncertainty of this major source.

[1] Davidson, Chen, Alon Amrani, and Alon Angert. "Tropospheric carbonyl sulfide mass balance based on direct measurements of sulfur isotopes." Proceedings of the National Academy of Sciences 118.6 (2021): e2020060118. 

How to cite: Avidani, Y., Davidson, C., Angert, A., and Amrani, A.: Isotopic fractionation of sulfur during COS hydrolysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6847, https://doi.org/10.5194/egusphere-egu23-6847, 2023.

EGU23-6955 | ECS | Posters on site | BG2.2

Quantifying the COS fluxes from plane, willow, beach and oak litter 

Florian Kitz, Herbert Wachter, and Georg Wohlfahrt

Flux partitioning, the quantification of photosynthesis and respiration, is a major uncertainty in modelling the carbon cycle and in times when robust models are needed to assess future global changes a persistent problem. A promising new approach is to derive gross primary production (GPP) from measurements of the carbonyl sulfide (COS) flux, the most abundant sulfur-containing trace gas in the atmosphere, with a mean concentration of about 500 pptv in the troposphere. The method is based on the observation that COS and CO2 enter the leaf via a similar pathway and are processed by the same enzyme (carbonic anhydrase), in case of COS a unidirectional process, allowing researchers to use COS uptake as a proxy for the gross CO2 uptake by plants. A prerequisite for using COS as a proxy for photosynthesis is a robust estimation of all non-living-leaf sources and sinks in an ecosystem. One major uncertainty in this regard is the contribution of soils and their respective litter layers to the overall ecosystem COS flux.

COS and CO2 fluxes from litter were measured in real-time using a quantum cascade laser (QCL). The plant litter from four different broadleaf tree species (plane, willow, beech and oak), collected a maximum of one hour before measurements started in the lab (to retain in situ moisture and the microbial biome), was measured under alternating dark and light (UV-A) conditions.

COS litter fluxes varied between the tree species, with plane primarily emitting COS, beech consuming COS and oak and willow being on average neutral (willow with a huge variance). COS litter fluxes within a species seem to correlate with litter moisture. The COS flux was ranging between -4 and 4 pmol kg DW-1 s-1, which is relevant in magnitude compared to the overall ecosystem COS flux and shouldn’t be neglected in future assessments of the global COS budget. 

How to cite: Kitz, F., Wachter, H., and Wohlfahrt, G.: Quantifying the COS fluxes from plane, willow, beach and oak litter, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6955, https://doi.org/10.5194/egusphere-egu23-6955, 2023.

EGU23-7308 | ECS | Posters on site | BG2.2

First principles model of isotopic fractionation in formaldehyde photolysis: wavelength and pressure dependence 

Luisa Pennacchio, Andreas E. Hillers-Bendtsen, Kurt V. Mikkelsen, and Matthew S. Johnson

Experimental studies show large isotope-dependent effects in the photolysis rates of formaldehyde isotopologues, that are both wavelength and pressure dependent. These effects are on the order of 10-20% for 13C and 18O (L. Feilberg et. al, J. Phys. Chem. A, 109, 8314-8319, 2004), and 60% for CHDO (E. J. K Nilsson et. al, ACP, 14, 551–558, 2014). We have made a model of the elementary processes involved in the photodissociation including unimolecular dissociation, collisional quenching and crossing between excited state surfaces. Computational chemistry is used to characterize some of these processes. The model is validated by comparison to all existing experimental data and is then used to make predictions about the isotopic fractionation in additional isotopicules (and for conditions not yet addressed by experiment) including fractionation in clumped molecules. The following isotopologues of formaldehyde have been investigated; HCHO, DCHO, DCDO, D13CHO, H13CHO, HCH17O, HCH18O, H13CH17O and H13CH18O. Rice–Ramsperger–Kassel–Marcus (RRKM) theory was used to calculate the rates for decomposition of the S0, S1 and T1 states with CCSD(T)/aug-cc-pVTZ, ωB97X-D/aug-cc-pVTZ and CASPT2/aug-cc-pVTZ levels of theory. Furthermore, the rates and likelihood of intersystem crossing were investigated by including the spin-orbit coupling between the excited states. The model was able to replicate the experimental pressure trends accurately, however, the kinetic isotope effect was one order of magnitude too small for the non-deuterated isotopologues. We predict a large clumped isotope anomaly in 13C18O produced by formaldehyde photolysis.

How to cite: Pennacchio, L., E. Hillers-Bendtsen, A., V. Mikkelsen, K., and S. Johnson, M.: First principles model of isotopic fractionation in formaldehyde photolysis: wavelength and pressure dependence, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7308, https://doi.org/10.5194/egusphere-egu23-7308, 2023.

EGU23-9030 | Orals | BG2.2 | Highlight

ISAMO (Iron Salt Atmospheric Methane Oxidation) 

Matthew S. Johnson, Maarten M. J. W. van Herpen, Berend v/d Kraats, Qinyi Li, Alfonso Saiz-Lopez, Jesper B. Liisberg, Luisa Pennacchio, and Thomas Röckmann

Methane is a well-mixed greenhouse gas responsible for >1/3 of global warming since pre-industrial times whose atmospheric burden continues to increase with a new record set in 2022. Active chlorine in the atmosphere is poorly constrained and so is its role in the oxidation of methane. This uncertainty propagates into methane source budgets through isotope-constrained top-down models, in which the observed abundance of 13C in tropospheric methane (commonly expressed as δ13C-CH4) is used to constrain the sources of methane using their characteristic δ13C-CH4 values. These models need to account for the change in the observed δ13C-CH4 by the Cl and OH sinks, which shift the observed isotope towards higher δ13C-CH4 values of fossil fuel sources, and away from 13C depleted biological sources. The ISAMO project focuses on the hypothesis that Cl atoms are produced naturally by the action of sunlight on particles containing iron and chloride and these chlorine atoms oxidize atmospheric methane. To study this, we use the sensitive and selective indirect quantification of the concentration of atomic Cl through the strong carbon kinetic isotope effect (KIE) in the CH4 + Cl reaction, which leaves the remaining CH4 enriched in 13C, and producing extremely 13C-depleted CO. We will present field and laboratory observations and global modelling, including CO isotope measurement from flasks samples across the North Atlantic. We show how this mechanism affects 13C depletion in atmospheric CO and how the corresponding 13C enrichment in CH4 affects global methane emission estimates.

How to cite: Johnson, M. S., van Herpen, M. M. J. W., v/d Kraats, B., Li, Q., Saiz-Lopez, A., Liisberg, J. B., Pennacchio, L., and Röckmann, T.: ISAMO (Iron Salt Atmospheric Methane Oxidation), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9030, https://doi.org/10.5194/egusphere-egu23-9030, 2023.

EGU23-10234 | ECS | Posters on site | BG2.2

Interannual variability and seasonality of carbonyl sulfide fluxes of an Austrian Scots pine forest 

Felix M. Spielmann, Albin Hammerle, Katharina Scholz, and Georg Wohlfahrt

The gross primary productivity (GPP), that is the gross uptake of carbon dioxide (CO2) by plants, cannot be measured on ecosystem level but must be inferred by either applying models or measuring proxies. One of those proxies is the trace gas carbonyl sulfide (COS), which is of particular interest, because it shares a very similar pathway into plant leaves as CO2 and is, contrary to the latter, generally not re-emitted.

Due to the need of expensive and sensitive instrumentation, e.g., quantum cascade lasers, only a limited amount of ecosystem measurements and even fewer long-term studies at this scale have been conducted. Consequently, more data focusing on the seasonality and the interannual variability of COS ecosystem fluxes are needed to understand the relationship of the COS to CO2 uptake, i.e., the leaf relative uptake (LRU), for reliable GPP calculations.

To investigate the impact of environmental changes on the LRU we conducted COS, CO2 and H2O eddy covariance flux (EC) measurements at our newly established forest field site in Mieming (Austria) for the last two years. The field site's dominating tree species is Scots pine (Pinus sylvestris) with Juniper trees (Juniper communis) in the understory.
In addition to the EC measurements, we conducted branch chamber measurements within the crown of the Scots pine, two at the treetop and one within the canopy.

Our EC measurements indicate a strong interannual variability of the COS fluxes. While we observed the highest COS uptake in 2021 during May, the COS uptake in 2022 was higher in the period from June to August. We also observed this pattern for the net CO2 fluxes. The fluxes of COS and CO2 concurrently decreased during the winter month and the forest turned into a net source for CO2, while COS was taken up continuously.

The mean LRU across all branch chamber measurements was 1.67 (-) with the chambers within the canopy generally having lower LRUs (1.39 (-)).

How to cite: Spielmann, F. M., Hammerle, A., Scholz, K., and Wohlfahrt, G.: Interannual variability and seasonality of carbonyl sulfide fluxes of an Austrian Scots pine forest, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10234, https://doi.org/10.5194/egusphere-egu23-10234, 2023.

EGU23-10454 | ECS | Posters virtual | BG2.2

Sulfate aerosol formation mechanisms constrained by oxygen and sulfur isotopes at coastal Hong Kong 

Qianjie Chen, Allison Moon, Andrew Schauer, Tao Wang, and Becky Alexander

Sulfate plays a key role in the formation and growth of aerosol particles and cloud droplets in the troposphere and is thus important for air quality and climate. The formation mechanisms of sulfate vary with oxidant levels and environmental conditions and can be partially revealed by its isotopic signatures. Here we measure oxygen (16O, 17O, 18O) and sulfur isotopes (32S, 34S) of the sulfate aerosol samples collected at coastal Hong Kong, downwind of the highly urbanized Pearl River Delta region. Based on ion measurements, most (95%) of the sulfate collected is non-sea-salt sulfate. The δ34S of sulfate is on average 4.0±2.0 ‰ (range 0.7 – 8.0 ‰), at an average sulfur oxidation ratio of 79±9%. The average oxygen-17 excess (Δ17O) is -0.1±0.3 ‰, suggesting an important role of OH / transition metals / reactive halogens. The δ18O of sulfate is on average 4.9±2.1 ‰. The Markov-Chain Monte Carlo model will be used to further constrain sulfate formation mechanisms.

How to cite: Chen, Q., Moon, A., Schauer, A., Wang, T., and Alexander, B.: Sulfate aerosol formation mechanisms constrained by oxygen and sulfur isotopes at coastal Hong Kong, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10454, https://doi.org/10.5194/egusphere-egu23-10454, 2023.

EGU23-11890 | Posters on site | BG2.2

Tracing N2O production pathways in aqueous ecosystems by quasi-simultaneous online analysis of 15N in reactive nitrogen species and gaseous emissions 

Joachim Mohn, Kun Huang, Wolfram Eschenbach, Jing Wei, Damian Hausherr, Claudia Frey, André Kupferschmid, Jens Dyckmans, Adriano Joss, and Moritz F. Lehmann

Natural and engineered nitrogen (N) removal processes in aqueous systems represent important sources of nitrogenous gas emissions, including the potent greenhouse gas nitrous dioxide (N2O). The relevance of microbial and abiotic formation pathways can be assessed using 15N tracing techniques. While 15N-N2O analysis using optical analyzers is straightforward, quantification of 15N fractions in inorganic N compounds, ammonium (NH4+), nitrite (NO2-), and nitrate (NO3-), is typically time-consuming and labor-intensive.

In this study, we developed an automated sample-preparation unit coupled to a membrane-inlet quadrupole mass spectrometer (3n-ASSP-MIMS) for the online quasi-simultaneous analysis of 15N fractions in NH4+, NO2-, and NO3-. The technique was designed and validated for applications at moderate (100 - 200 μmol L-1) to high (2 – 3 mmol L-1) N, as found in sewer systems, wastewater in treatment plants, or eutrophic surface waters, and 15N spiking (f15) between 1 and 33%.

The potential of 3n-ASSP-MIMS was demonstrated in a feasibility study, where the technique, in conjunction with 15N-N2O analyses by FTIR spectroscopy, was applied to pinpoint nitrifier denitrification as the primary N2O formation pathway during partial NH4+ oxidation to NO2- in a lab-scale sequencing batch reactor.

How to cite: Mohn, J., Huang, K., Eschenbach, W., Wei, J., Hausherr, D., Frey, C., Kupferschmid, A., Dyckmans, J., Joss, A., and Lehmann, M. F.: Tracing N2O production pathways in aqueous ecosystems by quasi-simultaneous online analysis of 15N in reactive nitrogen species and gaseous emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11890, https://doi.org/10.5194/egusphere-egu23-11890, 2023.

N2O isotopic composition, i.e., δ15N-N2O, δ18O-N2O and especially site preference (SP; difference of substitution frequencies at terminal or central position in N-N-O molecule) has been shown to provide information on N2O source processes, and allows for source partitioning of N2O emissions to nitrification and denitrification. The advent of laser spectrometers more than a decade ago has spawned first datasets of N2O isotopic composition in daily resolution, but they have remained scarce. This is because until recently, the precision of commercially available spectrometers did not allow direct determination of N2O isotopic composition without technically challenging liquid nitrogen free cryogenic preconcentration of N2O. The specifications of the latest commercially available spectrometers promised preconcentration free in-situ determination of N2O isotopic composition, but a recent instrument intercomparison showed that for most of the analyzers, specific correction functions are still necessary. While some available instruments were thoroughly characterized with regard to short term precision, repeatability, drift, amount effects, matrix effects and spectral interferences, instrument performance during field deployment and on the time scale of long measurement campaigns has not been analysed so far.

Here we present a setup and results of an automated chamber system in conjunction with a laser spectrometer that was installed in the field and in use for a period of approx. two years. Initially, amount dependence was in the range of 4 to 2 ‰ ppm N2O-1 for the various isotopic species, but instrument optimizations reduced this dependence to less than 1 ‰ ppm N2O-1. CH4 dependence was constant through the whole period and in the range of 1 to 2 ‰ ppm CH4-1, with affecting only δ15Nα and δ18O. In contrast, CO2 dependence was variable and in the same range as N2O amount dependence. The uncertainty budget was dominated by instrument noise, calibration and N2O amount dependence, indicating that improvements of instrument precision and availability of more suitable reference materials have a high potential to further decrease uncertainty of measurements. Analysis of the effect of uncertainty on the error of determined soil air N2O isotopic composition based on Keeling plots resulted in an error of 2 ‰ and 1 ‰ at N2O concentration increases of 70 and 140 ppb, respectively. Consequently, source partitioning based on SP will be associated with an error of 17 and less than 12% at the moment. Compared to growing-season emissions, SP and δ18O-N2O during freeze-thaw cycles were distinctly different. SP was ~0, indicating that N2O reduction to N2 was negligible during freeze-thaw events.

How to cite: Wolf, B., Xia, L., Smerald, A., Mohn, J., and Kiese, R.: Intramolecular N2O isotopic composition using laser spectrometers: Correction functions, uncertainty budget, freeze-thaw events and source process identification, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12962, https://doi.org/10.5194/egusphere-egu23-12962, 2023.

EGU23-13488 | ECS | Orals | BG2.2

What drives the variability in isotopic fractionation of O2 during enzymatic reactions? 

Carolina F. M. de Carvalho, Moritz F. Lehmann, and Sarah G. Pati

Molecular oxygen (O2) is one of the most important electron acceptors for a large variety of biotic and abiotic processes in the environment. A wide range of oxygen isotopic fractionation associated with biological O2 consumption (e.g., respiration) has been reported in field and laboratory studies (18ɛO2 from -29 to -1 ‰). The observed variability in 18ɛO2 values has mainly been attributed to the different types of respiring organisms. But, to better understand what ultimately causes the variation in isotopic fractionation of O2, it is necessary to start investigating at the lowest level of biological complexity. All biological O2 consumption, including respiration, detoxification, and biosynthesis, occurs at the enzyme-level. A few 18ɛO2 values have been reported for isolated enzymatic O2 reduction reactions. However, these laboratory-scale studies also displayed a wide range of O-isotope effects (18ɛO2 from -33 to -10 ‰), without any systematic correlation between 18ɛO2 values and the type of enzyme, substrate, or O2-reduction mechanism. In this study, we aimed at applying O2 stable isotope analysis to a systematic selection of O2 consuming enzymes, to improve our molecular understanding of isotopic fractionation of O2 at the enzyme-level. In a first series of experiments, we have determined kinetic parameters, as well as 18ɛO2 (and 17ɛO2) values of O2 reduction for a series of copper- and flavin-dependent oxidase enzymes. O2 reduction by these oxidase enzymes occurs separately from substrate oxidation, i.e., O2 is reduced to water (four-electron reduction) or to hydrogen peroxide (two-electron reduction), independently from the type of substrate. Thus, the variability in observed O isotopic fractionation should only depend on the active-site structure and/or the O2 reduction mechanism. Our experimental 18ɛO2 values covered the same range as those previously reported for laboratory-scale studies with other enzymes. Most of the studied flavin- and copper-dependent oxidases displayed no deviation from mass-dependent fractionation (17ɛO2/18ɛO2 ≈ 0.52). We demonstrate that 18ɛO2 values systematically correlate with a given enzyme’s affinity for O2 in flavin-dependent oxidases. Furthermore, our data suggest that the range of 18ɛO2 and 17ɛO2 values differs significantly between flavin- and metal-dependent O2 consuming enzymes. These results represent an important first step towards an improved understanding and generalization of the isotopic fractionation of O2 at the enzyme- and, ultimately, at the organism-level.

How to cite: F. M. de Carvalho, C., Lehmann, M. F., and Pati, S. G.: What drives the variability in isotopic fractionation of O2 during enzymatic reactions?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13488, https://doi.org/10.5194/egusphere-egu23-13488, 2023.

EGU23-14266 | ECS | Orals | BG2.2

Sulfur and carbon isotope measurements of carbonyl sulfide (COS) from small air samples; an overview and recent findings 

Sophie Baartman, Maarten Krol, Thomas Röckmann, and Maria Elena Popa

Carbonyl sulfide (COS) is the most abundant sulfur-containing trace gas in the atmosphere, with an average mixing ratio of 500 parts per trillion (ppt). It has a relatively long lifetime of about 2 years, which permits it to travel into the stratosphere. There, it likely plays an important role in the formation of stratospheric sulfur aerosols (SSA), which have a cooling effect on the Earth’s climate. Furthermore, during photosynthetic uptake by plants, COS follows essentially the same pathway as CO2, and therefore COS could be used to estimate gross primary production (GPP). Unfortunately, significant uncertainties still exist in the sources, sinks and global cycling of COS, which need to be overcome. Isotopic measurements of COS could be a promising tool for constraining the COS budget, as well as for investigating its role in the formation of stratospheric sulfur aerosols.

Within the framework of the COS-OCS project, we developed a GC-IRMS based measurement system at Utrecht University that can measure δ33S, δ34S and δ13C from S+ and CO+ fragment ions of COS from small air samples of 2 to 5 L. With this system, we have measured various types of air samples, including outside air, firn air from Greenland, and air from the upper troposphere – lower stratosphere region. We conducted photosynthesis experiments using a plant gas exchange chamber and we are also planning to measure firn air from Antarctica. Here, we will present an overview of the COS isotope measurements conducted within the COS-OCS project, and we will highlight the most interesting findings.

How to cite: Baartman, S., Krol, M., Röckmann, T., and Popa, M. E.: Sulfur and carbon isotope measurements of carbonyl sulfide (COS) from small air samples; an overview and recent findings, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14266, https://doi.org/10.5194/egusphere-egu23-14266, 2023.

EGU23-14497 | ECS | Posters virtual | BG2.2

Isotopic and chemical characterization of saline lake and playa salts: Implication for climate on Earth and Mars 

Yuxin Hao, Yuhe Qiu, Lanxiadi Chen, Jun Li, Wanyu Liu, Mingjin Tang, Xiying Zhang, Zhenchuan Niu, Jan Pettersson, Sen Wang, and Xiangrui Kong

Evaporite salts from saline lakes and playas play active roles in the atmospheric cycles and the climate system, especially in the context of changing climate. Similar processes also occurred on Mars, where large water bodies dried up and formed saline lakes and then salt evaporites and deposits. In this study, various salt samples (brines, lakebed salts, crust salts, playa surface salts, and a series of salts collected at different depths) were collected from two Martian analogue sites (Mang’ai and Dalangtan, MA and DLT) in Qaidam Basin. The salt samples were measured for their ionic compositions and pH as the fundamental characterization, and the effects of sample types and sampling sites are discussed. The hygroscopic properties of solid salts, including crystalized brines, were experimentally determined. The results show strong connections between the ionic composition and hygroscopic properties though discrepancy exists, indicating that the hygroscopicity is sensitive to the molecular forms and the hydrate degrees of salts. Sulfur and chlorine isotopes were measured, and the results are presented as δ34S and δ37Cl. The δ34S values of samples from MA and DLT show great difference. The δ34S values of MA samples are comparable to previously reported fresh water, brines and local precipitation, indicating that the MA samples are strongly influenced by materials exchanged from local environments. The DLT samples have higher δ34S values, which suggest that the material exchanges with surrounding environments are limited. The δ37Cl values are confined within a relatively narrow window compared to literature values. A trend is that the δ37Cl values vary with sample types, i.e., crust > lakebed > brine. This is likely caused by the isotopic fractionation during evaporite precipitation, where the heavier 37Cl isotope is preferably precipitated. The study of salt samples from MA and DLT areas improves the understanding of the active role of evaporite salts in the material cycle and climate system of both Earth and Mars.

Keywords: δ34S, δ37Cl, hygroscopicity, climate, Mars, Qaidam Basin

How to cite: Hao, Y., Qiu, Y., Chen, L., Li, J., Liu, W., Tang, M., Zhang, X., Niu, Z., Pettersson, J., Wang, S., and Kong, X.: Isotopic and chemical characterization of saline lake and playa salts: Implication for climate on Earth and Mars, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14497, https://doi.org/10.5194/egusphere-egu23-14497, 2023.

EGU23-14514 | ECS | Orals | BG2.2

Measurements of the clumped isotopic composition of atmospheric methane 

Malavika Sivan, Thomas Röckmann, Carina van der Veen, Caroline P. Slomp, and Maria Elena Popa

Atmospheric methane (CH4) is the second most important anthropogenic greenhouse gas after CO­2. Global scale measurements of CH4 mole fraction show an increasing trend since pre-industrial times. Various studies have attempted to attribute the temporal change to variations in the balance between different CH4 sources and atmospheric sink reactions. Measurements of bulk isotopic composition (δ13C and δD) are used for this purpose, but due to the overlap of source signatures, it is difficult to distinguish between biogenic, thermogenic, and pyrogenic CH4. With the advancement of high-resolution mass spectrometry, it is now possible to measure the two most abundant clumped isotopologues of CH4: 13CDH3 and CD2H2. The clumping anomalies denoted as Δ13CD and ΔDD can be used as an additional tool to constrain CH4 sources.

Most of the clumped isotope studies so far, have focused on high-concentration samples, which can easily deliver the large quantity of pure CH4 (several mL) needed to measure the clumped isotopologues. But these measurements could be particularly interesting for atmospheric CH4, for which the explanations of the recent variations are still under debate. As shown by a recent modeling study (1), clumping anomalies, especially ΔDD, have the potential to help distinguish between the main drivers of change in the atmospheric CH4 burden.

In our laboratory, we use the 253-Ultra mass spectrometer to measure the clumped isotopologues of CH4. These measurements require 4-5 mL of pure CH4 to achieve a precision of 0.3 ± 0.1 ‰ for Δ13CD and 2.4 ± 0.8 ‰ for ΔDD. For atmospheric air at 2 ppm, this translates to extracting CH4 from at least 2000 L of air.

We have recently developed a method for extracting and purifying CH4 from this large quantity of air, without modifying its isotopic composition. We will present the current capabilities of this extraction system, and the first results of the clumped isotopic composition of the ambient air.

Reference:

1. Chung, E & Arnold, T 2021, 'Potential of Clumped Isotopes in Constraining the Global Atmospheric Methane Budget', Global Biogeochemical Cycles, vol. 35, no. 10, https://doi.org/10.1029/2020GB006883

How to cite: Sivan, M., Röckmann, T., van der Veen, C., Slomp, C. P., and Popa, M. E.: Measurements of the clumped isotopic composition of atmospheric methane, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14514, https://doi.org/10.5194/egusphere-egu23-14514, 2023.

I will present a newly developed method for analyzing major air components and their isotopic composition, using the high resolution Thermo Ultra mass spectrometer. The main characteristics of this instrument that are interesting in this context are the high resolution, stability and sensitivity.  The high resolution results in fewer isobaric interferences; low abundance compounds (e.g. multiply substituted molecules) can be observed due to the high resolution and high sensitivity; and the instrument stability allows long measurements, as needed for obtaining high precision for the low abundance compounds.

The species that can be analyzed so far with useful precision are:

- O2/N2 and Ar/N2 (precision in permeg range)

- O2 isotopologues, including clumped: 16O2, 16O17O, 16O18O, 17O18O, 18O2

- N2 isotopologues, including clumped: 14N2, 14N15N, 15N2

- Ar isotopes: 36Ar, 38Ar, 40Ar

The whole suite of measurements uses about 10 ml of dry air, and takes up to two days for one sample.

The first application of this method is planned for stratospheric and icecore samples.

How to cite: Popa, M. E.: Direct air measurements using the high resolution Thermo Ultra mass spectrometer: O2/N2 and Ar/N2 ratios, and O2, N2 and Ar isotopic composition, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15560, https://doi.org/10.5194/egusphere-egu23-15560, 2023.

EGU23-15737 | ECS | Posters on site | BG2.2

Evaluation of nine years of continuous δ13CO2 measurements in Heidelberg, Germany 

William Cranton, Henrik Eckhardt, Antje Hoheisel, and Martina Schmidt

Measurements of atmospheric CO2 mole fraction in combination with δ13CO2 contain additional information on the CO2 source mixture at a measurement station. Instrumental developments, such as cavity ring-down spectroscopy (CRDS), have facilitated the conduction of continuous in-situ measurements of CO2 mole fraction and δ13CO2 with a high temporal resolution. This has enabled a robust and detailed local time series to be established at an urban station in Heidelberg in south-western Germany, where a CRDS G2201-i analyser has been used to measure the CO2 mole fraction and 13C/12C ratio from 2014 to 2023. This nine year time series is analysed for seasonal variations and trends in regional and local CO2 sources. We applied different approaches based on the Keeling/Miller-Tans method to identify δ13CO2 source signatures within the Heidelberg catchment area. Doing this gave δ13CO2 source values that were less depleted in the summer and more depleted in the winter, indicating a stronger biogenic effect in summer and stronger fossil fuel contributions in winter.

How to cite: Cranton, W., Eckhardt, H., Hoheisel, A., and Schmidt, M.: Evaluation of nine years of continuous δ13CO2 measurements in Heidelberg, Germany, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15737, https://doi.org/10.5194/egusphere-egu23-15737, 2023.

EGU23-16104 | Orals | BG2.2

Sedimentary and dark production sources of COS and CS2 identified by their sulfur isotopic values 

Alon Amrani, Chen Davidson, Sinikka T. Lennartz, and Alon Angert

Carbonyl sulfide (COS) is a long-lived trace gas, and an important precursor for stratospheric sulfate aerosols, which reduce solar radiation reaching earth surface and may regulates earth's climate. The main sink of COS is the uptake by terrestrial plants similar to CO2. Thus, COS is used as a proxy for CO2 removal by terrestrial plants (gross primary production, GPP). Oceans are the major source of COS to the atmosphere , either directly or indirectly by emitting other volatile sulfur compounds such as CS2 and DMS that partially oxidize to COS in the atmosphere.  In the surface ocean, COS is produced by photochemical reactions and by "dark production" deeper in the water column and from sediments. In the present study we aim to determine and quantifying the COS and CS2 “dark production” by using sulfur isotopes measurements (34S/32S; δ34S) of surface, deep water and sediment samples. In addition, laboratory experiments were conducted to follow the productions of COS and CS2 by direct reactions with CO and HS-/SX2- and by incubations experiments of seawater. Our preliminary results from the Atlantic Ocean, the Mediterranean, North, Wadden, and Red Seas show surface δ34S values in the range of -4 to 20‰ for COS, and -10 to 22‰ for CS2 while DMS was 18-21‰. The δ34S values of DMS are in line with previous measurements of the surface ocean and reflect its biological source with small isotopic fractionation relative to marine sulfate (21‰). This was also expected for COS and CS2 that also produced from biological sources. However, their δ34S values extended over large ranges up to 30‰, while their heaviest δ34S value are closed to DMS. There are clear mixing lines for COS and CS2 between the surface ocean sources (heavy) and the sedimentary sources (light) in shallow water. The isotopic values of sedimentary-production are calculated as -4‰ for COS and -10‰ for CS2, based on the samples from the sediment rich waters of the Wadden Sea. These values suggest abiotic sulfurization of light organic compounds by 34S depleted HS-/SX2- from the microbial sulfate reduction (MSR) in the sediment. Indeed, the intertidal sands of the Wadden Sea are known to host intense MSR activity and produce large amounts of H2S and polysulfides. The specific organic precursors are still unknown and will be the subject of our upcoming experiments. Also, the “dark production” isotopic signals of the surface water is not yet well resolved, but seems also to be isotopically lighter then DMS and marine sulfate. These new findings show that the COS/CS2 sources in the ocean are complex combining contributions from several biotic and abiotic processes which seem to have unique isotopic signatures.   

How to cite: Amrani, A., Davidson, C., T. Lennartz, S., and Angert, A.: Sedimentary and dark production sources of COS and CS2 identified by their sulfur isotopic values, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16104, https://doi.org/10.5194/egusphere-egu23-16104, 2023.

EGU23-16611 | Orals | BG2.2

Seasonal and spatial variation in 13C signature of emitted methane and pore water methane in northern mires 

Janne Rinne, Xuefei Li, Patryk Łakomiec, Patrik Vestin, Per Weslien, Julia Kelly, Lukas Kohl, Lena Ström, Timo Vesala, and Leif Klemedtsson

Methane emission from northern mires shows typically strong spatial and seasonal variations. These variations have been assigned to e.g. differences in methane production due to variation in substrate input, transport pathways, methane oxidation in aerobic peat layers, and temperature variations. Stable isotope signatures of the emitted methane and methane in pore water can help us to constrain our hypotheses of these variations.

We have measured δ13C of methane emission in Mycklemossen mire in Sweden by automated chamber system for two years. We also have measured δ13C of methane in pore water in three depths in Siikaneva mire in Finland by an automated diffusion tube system for one seasonal cycle. At both sites ecosystem scale δ13C of emitted methane was measured using nocturnal boundary layer accumulation (NBLA) approach.

We observed systematic spatial variation in δ13C of emitted methane at Mycklemossen site, which mostly indicated the importance of substrate availability in explaining the spatial variability. At Siikaneva we observe systematic differences in the depth distribution of δ13C of pore water methane. Interestingly, this distribution is different in summer and winter.  The ecosystem scale δ13C of emitted methane derived by chambers and NBLA approach very close to each other. We will discuss the observations, their implications, and future integration of the data and new measurement.

 

How to cite: Rinne, J., Li, X., Łakomiec, P., Vestin, P., Weslien, P., Kelly, J., Kohl, L., Ström, L., Vesala, T., and Klemedtsson, L.: Seasonal and spatial variation in 13C signature of emitted methane and pore water methane in northern mires, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16611, https://doi.org/10.5194/egusphere-egu23-16611, 2023.

EGU23-132 | ECS | Orals | NP6.1

Airborne observations of shoaling and breaking internal waves 

Teodor Vrecica, Nick Pizzo, and Luc Lenain

Internal waves are crucial contributors to the transport of sediment, heat, and nutrients in coastal areas. While internal waves have been extensively studied using point measurements, their spatial variability is less well understood. Here, we present a unique set of high-resolution infrared imagery collected from a helicopter, hovering over very energetic shoaling and breaking internal waves. We compute surface velocities by tracking the evolution of thermal structures at the ocean surface and find horizontal velocity gradients with magnitudes that are more than 100 times the Coriolis frequency. Under the assumption of no vertical shear we determine vertical velocities from the obtained horizontal divergence estimates and identify areas of the wave undergoing breaking. The spatial variability of the internal wave occurs on scales from a few to a few hundred meters. These results highlight the need to collect spatio-temporal observations of the evolution of internal waves in coastal areas.

How to cite: Vrecica, T., Pizzo, N., and Lenain, L.: Airborne observations of shoaling and breaking internal waves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-132, https://doi.org/10.5194/egusphere-egu23-132, 2023.

This work addresses the effects of time-dependent, mesoscale turbulence on the wind-driven ocean circulation in a closed basin with variable topography. The main results concern the so-called Neptune effect, which involves the generation of persistent flows correlated with topography, but in this case, such currents are formed in the presence of a continuous, stochastic forcing. Numerical simulations of a single-layer fluid with sloping bottom topography near the boundaries are performed. The forcing is a suitable combination of a steady, basin-scale wind that generates the classical western-intensified anticyclonic gyre, plus a shorter, time-dependent forcing that injects energy at a narrow range of scales. Two contrasting situations are considered. First, in the absence of large-scale forcing, the turbulence generates a cyclonic flow that follows the geostrophic contours around the basin. This configuration corresponds to the most probable state equivalent to that expected in statistical equilibrium. Second, the resulting mean circulation is studied when the large and small-scale forcing terms are considered together. The main consequence is the alteration of the anticyclonic gyre due to the turbulent-induced cyclonic circulation. This result implies that large-scale, semi-steady circulations might be altered according to the turbulence characteristics.

How to cite: Zavala Sanson, L.: Effects of mesoscale turbulence on the wind-driven circulation in a closed basin with topography, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-623, https://doi.org/10.5194/egusphere-egu23-623, 2023.

EGU23-1200 | Orals | NP6.1

Light-limited dynamics of sinking phytoplankton in a convective flow model with ice-covered waters 

Stefano Berti, Vinicius Beltram Tergolina, Enrico Calzavarini, and Gilmar Mompean

Plankton dynamics are controlled by an often subtle interplay between biological and physical processes. Among the latter, fluid transport is known to play a prominent role. Field studies have, e.g., provided evidence of the effects of turbulent-convection upwelling and downwelling motions on phytoplankton survival. Recent numerical investigations have emphasized, in addition, that relatively large-scale coherent flow features on the vertical can considerably hinder survival and thus negatively impact plankton blooms.

In nutrient-rich polar marine environments phytoplankton growth is critically limited by light availability, especially in waters that are partially covered by ice. In these conditions, the heterogeneity of the light intensity distribution, in association with a large-scale coherent fluid flow, can give rise to complex biological dynamics. In the Arctic ocean, several studies reported under-ice phytoplankton blooms that were initiated by the onset of ice melt. Nevertheless, it is still only partially known how such blooms are controlled by the interaction between different factors, such as the increase of light transmittance, leads (openings in the ice), convective mixing, and biological processes. Under-ice blooms are expected to become more common in the future, due to increasingly thinner and dynamic ice coverage, and thus more frequent lead formation. This could significantly alter primary production, and have important consequences on local marine food webs.

In this work we consider an advection-reaction-diffusion model of phytoplankton light-limited vertical dynamics in the presence of convective transport, intended as an idealized representation of nonuniformly ice-covered polar waters. Specifically, we assume that the incident light intensity at the surface is horizontally modulated by the presence of opaque obstacles, giving rise to regions of the water column that are characterized by different production regimes. We focus on the impact of advection, and more generally of the different transport processes occurring in the fluid, on the average biomass. By means of numerical simulations we show that convective motions may be harmful to under-ice blooms, in agreement with previous findings. In the present setup, such effect depends on the positions of the surface obstacles with respect to the upwelling and downwelling flow regions. We further find, however, that the sinking speed, due to the density difference between phytoplankton organisms and water, also plays an important role, which depends on how it adds to the flow. While small, the sinking speed has a measurable impact on the growth dynamics of the population and can even be critical for its survival, which may have ecological relevance, as different phytoplankton species have different densities and, hence, different settling velocities.

How to cite: Berti, S., Tergolina, V. B., Calzavarini, E., and Mompean, G.: Light-limited dynamics of sinking phytoplankton in a convective flow model with ice-covered waters, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1200, https://doi.org/10.5194/egusphere-egu23-1200, 2023.

In late winter many lakes are iced over, and hence remain cut off from the mechanical forcing due to wind.  At the same time, strong radiative forcing modifies the inverse stratification associated with wintertime conditions.  The inverse stratification occurs due to the fact that freshwater has a temperature of maximum density (around 4 degrees Centigrade) and the equation state of freshwater is thus nonlinear.  In this talk I will demonstrate that this nonlinearity has a profound influence on the characteristics of nonlinear internal solitary-like waves in the cold water regime.  In particular, predcitions of waves made using a piecewise linear density profile yield waves with the opposite polarity to those calculated using temperature profiles and the full nonlinear equation of state.  I will present results based on the Dubreil-Jacotin Long theory, but similar conclusions can be made based on weakly nonlinear (KdV) theory.  Time permitting I will discuss implications of these results for shoaling.

How to cite: Stastna, M.: Nonlinearity of the equation of state effects dynamics of nonlinear internal waves in late winter lakes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1470, https://doi.org/10.5194/egusphere-egu23-1470, 2023.

EGU23-1554 | Posters on site | NP6.1

Interaction of Fully-Nonlinear Internal Solitary Waves with Cores 

Kevin Lamb

Under appropriate background conditions internal solitary waves may have surface or subsurface cores. Both types of waves have been observed in the ocean. Solutions of the Dubreil-Jacotin-Long equation predict cores with closed isopycnals and, in a reference frame moving with the wave, closed streamlines. In numerical simulations of a time-evolving field these cores are unsteady and leaky: fluid is continually being entrained into the core and leaking out of the rear of the core. In this talk I will present results of the interaction of two internal solitary waves, one with a core over-taking a smaller wave without a core. In general, during the interaction the large ISW decrease in amplitude while transferring energy to the smaller ISW. During this process the large ISW loses its core and the fluid inside the core is left behind. The smaller wave grows in amplitude and forms a new core. In many cases the final small ISW is considerably smaller than the initial small ISW while the larger ISW may be larger than the iniitial ISW. ISW energy is also transferred to small amplitude internal waves. 

How to cite: Lamb, K.: Interaction of Fully-Nonlinear Internal Solitary Waves with Cores, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1554, https://doi.org/10.5194/egusphere-egu23-1554, 2023.

EGU23-1766 | Posters on site | NP6.1

Numerical analysis of breather interactions 

Keisuke Nakayama and Kevin Lamb

While the existence of breathers in the ocean is not clearly revealed, Rouvinskaya et al. (2015) suggested the possibility that breathers occurred in the Baltic Sea. In three-layer symmetric stratifications with the same density difference across each interface, the modified KdV equation (the Gardner equation with the quadratic nonlinear coefficient equal to zero) predicts that breathers exist. Therefore, the soliton-like characteristics of fully nonlinear breathers must be better understood. Thus, this study used fully nonlinear numerical simulations to investigate breather interactions by analysing overtaking collisions of two breathers in a three-layer fluid. As a result, an overtaking collision of two breathers is almost elastic when the ratio of the breather amplitude to the upper and lower layer thickness is smaller. Furthermore, the collision is found to remove the mode-2 structure, resulting in a significant role in forming breathers.

How to cite: Nakayama, K. and Lamb, K.: Numerical analysis of breather interactions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1766, https://doi.org/10.5194/egusphere-egu23-1766, 2023.

EGU23-2594 | ECS | Orals | NP6.1

Laminar transport and turbulent cascades in downslope rotating gravity currents. 

Sévan Rétif, Maria-Eletta Negretti, Achim Wirth, and Axel Tassigny

We present experimental results from large-scale laboratory experiments of rotating downslope gravity currents intruding into a two-layer stratified ambient performed in the Coriolis Rotating Platform in Grenoble. By means of PIV velocity and conductivity data for the density measurement, we show that mixing occurs mostly on the slope area during the descent rather than once the current has penetrated the stratified ambient, where the Richardson number remains above the stability threshold of 1/4. Looking at the time evolution of the vertical density profile in the stratified receiving ambient, two distinct mixing regimes can be identified, the first issued by laminar transport through Ekman dynamics, the second by turbulent transport due to intermittent cascading events. Vertical density gradients reveal a linear piece-wise dependence on the density anomaly, highlighting an advection-diffusion process as proposed by the theoretical model of Munk & Wunsch (1998). If the gravity current flow is laminar on the slope, the structure shows a linear variation of the density with depth ; For the turbulent transport regime characterized by intermittent cascades, an exponential shape is rather observed. The shape of the density structure allows to estimate bulk mixing coefficients and entrainment velocities at the top and the bottom of the intruding gravity current, which can be further compared to oceanographic observational data.

How to cite: Rétif, S., Negretti, M.-E., Wirth, A., and Tassigny, A.: Laminar transport and turbulent cascades in downslope rotating gravity currents., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2594, https://doi.org/10.5194/egusphere-egu23-2594, 2023.

EGU23-3642 | ECS | Orals | NP6.1

The sensitivity of internal solitary waves to localized patches of mixing 

Nicolas Castro-Folker and Marek Stastna

While most theoretical work on internal waves idealizes the stratification, geophysical stratifications are typically much more complicated.  We build on recent work on nearly linear stratifications by adopting perturbations that take the form of a localized patch of mixing. We present a data-centric framework that seeks to identify which locations and widths of a mixing patch yield the largest effect on the structure of exact waves (computed via the Dubreil-Jacotin-Long equation), linear waves (computed via the longwave Taylor-Goldstein equation), and evolving nonlinear waves (via time-dependent simulations using the incompressible Navier-Stokes equations). We find that the vertical structure functions of linear waves are most sensitive to perturbations below (above) the pycnocline when the pycnocline is above (below) mid-depth; furthermore, as the pycnocline approaches mid-depth, the depth of the perturbation layer with the greatest impact approaches the depth of the pycnocline. In contrast, the centre streamwise velocity profile of a DJL wave is perturbed most by layers above (below) the pycnocline when the pycnocline is above (below) mid-depth. Finally, we present the results of simulations of evolving nonlinear waves, where we compare pairs of cases with and without a perturbation layer. Despite the presence of an initial patch of unstable fluid, the perturbation layer is sustained during the simulation; nevertheless, slight Rayleigh-Taylor instabilities are observed within and about the perturbation layer. Modulations in the horizontal velocity field about the leading solitary wave are compared with the results of the linear and DJL analyses.

How to cite: Castro-Folker, N. and Stastna, M.: The sensitivity of internal solitary waves to localized patches of mixing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3642, https://doi.org/10.5194/egusphere-egu23-3642, 2023.

EGU23-4236 | Orals | NP6.1

New method of directional spectrum estimation accounting for ambient shearing currents 

Yaron Toledo, Rotem Soffer, and Eliezer Kit

Realistic currents in seas and oceans are almost always changing in depth thus indicating on the presence of shear in the mean ambient flow. However, analysis methodologies interpreting directional wave data gathered by in-situ measurement devices such as: buoys, pressure gauges and Acoustic Doppler Current Profilers (ADCPs) utilize potential irrotational flow theory which cannot account for the rotational shearing currents. The effects of shearing currents on the wave direction estimations were studied on synthetic ADCP data of waves propagating in a predetermined spread. The synthetic data was generated employing the Rayleigh Boundary Value Problem (BVP) and a selected ambient current profile. The potential data processing led to significant errors in wave directional spread estimation for common shearing currents (~10°  in mean wave direction for the presented example). This finding is of great importance, as it addresses the influence of an ambient current profile on wave propagation direction. The obtained results suggest that there is an uncertainty with the confidence of any wave directional spread ever presented by in-situ wave measurement devices.

A new methodology was developed for estimating directional wave spectra based on rotational flow physics by acquiring new terms emanate from wave-shearing current interaction governing equations. This included a derivation of new numerical transfer functions for the fluid’s physical properties based on the Rayleigh BVP. Then, by applying classical cross- and auto-spectral analysis on time-series data sets, the directional spread function was numerically reconstructed. The newly derived data processing methodology was applied to the same synthetic ADCP data sets. It was found to be capable of reconstructing the spread with great accuracy (0.4° in mean wave direction for the presented example). In addition, to modeling and synthetic data, field measurement data from several campaigns were also analyzed showing the importance of accounting for the vertical shear. This makes it a prominent methodology for estimating directional wave spectra in realistic oceanic conditions.

How to cite: Toledo, Y., Soffer, R., and Kit, E.: New method of directional spectrum estimation accounting for ambient shearing currents, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4236, https://doi.org/10.5194/egusphere-egu23-4236, 2023.

EGU23-5170 | ECS | Posters virtual | NP6.1

Scaling analysis of wave profiles 

Yang Gao, Francois Schmitt, Jianyu Hu, and Yongxiang Huang

In the field of wind-wave interaction, scaling features for both wind and waves are often found experimentally. Several theoretical explanations of the scaling law for wind speed and sea surface wave height have been advocated, while a theoretical consideration for the significant wave height (Hs) is still lacking. In this work, we considered a long-term (more than 20 years) and high sampling frequency (about 0.78 Hz) wave profile data collected by buoys provided by Coastal Data Information Program (CDIP). The scaling features for Hs and for the absolute value of the wave profile are evident in the sense of the Fourier power spectrum. The same scaling features were obtained for frequencies below 10-4 Hz, with a scaling exponent close to 3. While the spectrum for wave profile shows a plain-like distribution under the frequency around 0.02 Hz due to the band pass filter. Furthermore, measured Hs is well overlapped with the absolute value of the wave profiles, which indicates that the amplitude modulation is still preserved after band pass filtering, and that might be the reason for the existence for the scaling features for Hs.

How to cite: Gao, Y., Schmitt, F., Hu, J., and Huang, Y.: Scaling analysis of wave profiles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5170, https://doi.org/10.5194/egusphere-egu23-5170, 2023.

EGU23-5470 | ECS | Posters on site | NP6.1

Bassin study of vetically sheared currents from the dispersion of surface gravity wave 

Alexandra Cuevas, Vincent Rey, Julien Touboul, and Fabrice Ardhuin

Wave conditions from the open sea to the coast, provide necessary information, the good understanding and modeling of coastal dynamics, the design of coastal engineering structures coastal engineering structures, for navigation or the flooding risks evaluation. It is also a potential way to access information present below the surface. Refraction, diffraction and reflection of waves are not only forced by variations in bathymetry but also by the presence of currents. However, the effects of current in propagation models have long been limited to the consideration of homogeneous current in the water column. Nevertheless, currents are usually observed to be sheared vertically by wind, tides or waves. When wave propagate in the presence of currents their celerity is modified. It is also affected by the vertical structure of the current.

This work proposes and discusses methods for reconstructing current fields from wave data based on synchronous analysis of wave spectra at different points in space. We consider here the 2D case of progressive or partially stationary waves in the presence of homogeneous currents or with a vertical sheared profile. The study is based on data from experiments carried out at the Bassin de Génie Océanique FIRST(BGO), for progressive or partially stationary waves in the framework of the ANR project MORHOC'H 2. These test campaigns allowed us to test the sensitivity of the wave’s phase evolution during its propagation in order to estimate the feasibility of reconstructing either constant or sheared currents in the water column. Under the assumption of a progressive wave, the study of the phase evolution shows a significant influence of the current, allowing to reach the intensity of a uniform current. The calculated phase evolution in the presence of sheared current is consistent with the theory, but for small values of shear, the phase velocity changes are much smaller, making the method more sensitive to "noise". Furthermore, for a partially stationary wave, a significant impact of its phase evolution is observed in the propagation direction of the incident wave even for weak reflections, making it necessary to include this parameter in the reconstruction of currents from synchronous wave measurement data.

Acknowledgements:

The DGA is thanked for funding the AID thesis grant of Alexandra CUEVAS, as well as for the ANR grant: ANR-21-ASM1-003.

How to cite: Cuevas, A., Rey, V., Touboul, J., and Ardhuin, F.: Bassin study of vetically sheared currents from the dispersion of surface gravity wave, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5470, https://doi.org/10.5194/egusphere-egu23-5470, 2023.

EGU23-5790 | Orals | NP6.1

Droplet dynamics in homogeneous and isotropic turbulence 

Sergio Chibbaro, Marco Crialesi-Esposito, and Luca Brandt

Emulsions are a major class of multiphase flows, crucial in industrial process (e.g. food and drug production) and ubiquitous in environmental flows (e.g. oil spilling in maritime environment). Already at volume fractions of few precents, the dispersed phase interacts with pre-existing turbulence created at large scale, yet the interaction between phases and the turbulent energy transport across scales is not yet fully understood.

In this work, we use Direct Numerical Simulation to study emulsions in homogeneous and isotropic turbulence, where the Volume of Fluid (VoF) method is used to represent the complex features of the liquid-liquid interface.

We consider a mixture of two matching-density phases, where we vary volume fraction, viscosity ratio and large-scale Weber number aiming at understanding the turbulence modulation and the observed droplet size distributions.  The analysis, based on the spectral scale-by-scale analysis, reveals that energy is consistently transported from large to small scales by the interface, and no inverse cascade is observed. We find that the total surface is directly proportional to the amount of energy transported, and that the energy transfer in the inertial range provides information about the droplet dynamics. We observe the -10/3 and -3/2 scaling on droplet size distributions, suggesting that the dimensional arguments which led to their derivation are verified in HIT conditions and denser conditions. Finally, we discuss the highly intermittent behaviour of the multiphase flow, which can be directly related to the polydisperse nature of the flow.

The study provides some significant observations towards a more comprehensive understanding of multiphase turbulence, opening new questions for future studies. 

How to cite: Chibbaro, S., Crialesi-Esposito, M., and Brandt, L.: Droplet dynamics in homogeneous and isotropic turbulence, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5790, https://doi.org/10.5194/egusphere-egu23-5790, 2023.

EGU23-6336 | ECS | Orals | NP6.1

Use of HDG oceanic models to study eddy formation in coastal upwelling areas 

Inés Hernández García, Albert Oliver Serra, and Francisco Machín Jiménez

The Canary Islands region is located in the North-East Atlantic Ocean, next to the African coast. It is situated within the equatorward travelling Canary Current.

This area has a high mesoscale activity. Some important features of this area are the African Upwelling System, the filaments originated by the upwelling, and long-lived cyclonic and anticyclonic mesoscale eddies. The generation of these mesoscale eddies, by the perturbation of the Canary Current caused by the islands, has been largely studied.

The aim of this work is to use a novel Hybridisable Discontinuous Galerkin (HDG) oceanic model, based on Finite Elements, in addition to real in situ and satellite data, in order to study different generation mechanisms and the evolution of the mesoscale eddies south of the Canary Islands.

How to cite: Hernández García, I., Oliver Serra, A., and Machín Jiménez, F.: Use of HDG oceanic models to study eddy formation in coastal upwelling areas, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6336, https://doi.org/10.5194/egusphere-egu23-6336, 2023.

EGU23-6774 | ECS | Orals | NP6.1

Prolate microswimmer in surface gravity waves 

Francesco Michele Ventrella, Filippo De Lillo, Guido Boffetta, Massimo Cencini, Jean-Luc Thiffeault, and Nimish Pujara

Planktonic microorganisms immersed in a fluid interact with the ambient flow, altering their trajectories. In surface gravity waves, a common goal for microswimmers is vertical migration. By modeling phytoplankton as spheroidal bodies with a certain swimming velocity, we investigate how the combination of swimmer's dynamical characteristics and fluid velocity gradients affect the motion. We investigate the case of prolate, negative buoyant swimmers. We consider also the case of gyrotactic swimmers. We find that it is possible for microswimmers to be trapped at a finite depth below the sea level. This phenomenon is due to the coupling between swimming, gyrotaxis and flow-induced reorientations. The trajectories obtained by numerical simulations, indicate that the dynamics consist of fast oscillations at the surface wavelength superposed with a slower trend at a longer timescale. This suggests using a multiple time-scale expansion to remove the fast oscillations. The presence of stable fixed points for the slow dynamics allows the trapping behaviour.

How to cite: Ventrella, F. M., De Lillo, F., Boffetta, G., Cencini, M., Thiffeault, J.-L., and Pujara, N.: Prolate microswimmer in surface gravity waves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6774, https://doi.org/10.5194/egusphere-egu23-6774, 2023.

EGU23-8518 | Posters virtual | NP6.1

Dynamics of small-scale turbulence in the upper ocean under the action of currents and internal waves 

Lev Ostrovsky, Daria Gladskikh, Irina Soustova, and Yuliya Troitskaya

We study the evolution of a turbulent layer in a stratified ocean layer using the theory of unsteady turbulent flows in a stratified fluid developed in [1] and subsequent works. The theory starts from a kinetic equation for turbulence parameters and results in the set of equations involving the mutual transformation of the kinetic and potential energies of turbulence that is shown to significantly affect the overall dynamics of energy exchange between small-scale turbulence and mesoscopic motions and the formation of the upper mixed layer. Besides, this approach allows an account for some important but usually neglected effects such as the dependence of vertical anisotropy of turbulence on stratification. Notably, the transformation between kinetic and potential energies eliminates the restriction on the existence of turbulence at large Richardson numbers.  The results are applied to the analysis of in situ data for turbulence evolution under the action of shear flows and internal waves, obtained in different regions that are significant for climate research, including the upper equatorial ocean. The fundamental role of potential energy in the formation of a turbulent flow is demonstrated.

The work was supported by RSF project No. 23-27-00002.

[1] Ostrovsky L.A., Troitskaya Yu.I. (1987) A model of turbulent transfer and dynamics of turbulence in a stratified shear flow. Izvestiya, Atm. and Oceanic Phys., 23(10), 767-773 (1987).

How to cite: Ostrovsky, L., Gladskikh, D., Soustova, I., and Troitskaya, Y.: Dynamics of small-scale turbulence in the upper ocean under the action of currents and internal waves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8518, https://doi.org/10.5194/egusphere-egu23-8518, 2023.

EGU23-9604 | Posters on site | NP6.1

Transformation of internal solitary waves under ice cover edge 

Kateryna Terletska, Vladimir Maderich, and Elena Tobisch

Internal wave-driven mixing is an important factor in the balance of heat and salt fluxes in the Polar Regions. The interaction between internal waves and ice cover in these areas of the ocean is complex and depends on both the characteristics of the ice and the characteristics of internal waves. Harsh environment in Arctic Ocean obstructs direct field observations of internal solitary waves thus, numerical modellings are an essential tool to overcome this shortcoming. The numerical three dimensional, free-surface, non-hydrostatic model for stratified flows using the Navier-Stokes equations in the Boussinesq approximation so called NH-POM was used for simulations of transformation of internal solitary waves under ice cover edge. As the result of the research it was shown, that propagation of internal solitary waves under edge of the ice cover may lead to their destabilization through overturning and breaking events. Such parameters as ice cover depth and internal waves amplitudes were responsible for the evolution and disintegration of an ISW beneath the ice cover while the boundary friction beneath the ice cover had little effect. During the interaction, maximum energy loss could reach about 60% near the ice edge. Interaction of ISWs with the ice edge significantly enhanced the turbulent dissipation and consequentially could potentially accelerated melting of the ice. It was suggested that the blocking parameter B, that is ratio of incident amplitude to the depth of the upper layer beneath the ice, controls the transfer of energy across the ice edge, that is, more energy is reflected if the ratio increases. When the ice depth decreased, the ice-ISW interaction and resultant dissipation weakened.

How to cite: Terletska, K., Maderich, V., and Tobisch, E.: Transformation of internal solitary waves under ice cover edge, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9604, https://doi.org/10.5194/egusphere-egu23-9604, 2023.

EGU23-9614 | Orals | NP6.1

Diapycnal Mixing in the Bransfield Strait 

Ángel Rodríguez-Santana, Borja Aguiar-González, Ángeles Marrero-Díaz, Luis Pablo Valencia, and Francisco Machín

During the austral midsummer near the South Shetland Islands, an interdisciplinary cruise (COUPLING) was carried out in January 2010 (Sangrà et al, 2014). For this study we selected one transect of 12 stations across the Central Bransfield Strait with vertical profiles of Conductivity, Temperature and Depth (CTD) and Acoustic Doppler Current Profiler (ADCP). Vertical profiles of microstructure turbulence were measured at stations of the transect located in specific dynamic features (two fronts: Bransfield Front and Peninsula Front; and an anticyclonic eddy) from a free-fall turbulence profiler. Using CTD and ADCP data, we computed the Thorpe scales, gradient Richardson numbers and density ratios that were compared with microstructure data.

We found that the most active turbulent layer was observed within the upper mixed layer (UML) of the anticyclonic eddy between stations 3 and 6 of the transect. However, intense inversions below the UML were found at the axis of the Peninsula Front (station 9). In the region of the Bransfield Front, it is noteworthy that there were obtained relative high values of kinetic energy dissipation rate (ε) with mixing processes due to vertical shear instabilities and double diffusion.  With this work, we have a deeper understanding of the mixing processes in the Bransfield Strait, which will allow a better estimation of the vertical fluxes of heat, salt and nutrients for this region.

Key words:

Bransfield Strait, Diapycnal Mixing, Microstructure Turbulence.

References:

Sangrà, P., C. García-Muñoz, C.M. García, A. Marrero-Díaz, C. Sobrino, B. Mouriño-Carballido, B. Aguiar-González, C. Henríquez-Pastene, A. Rodríguez-Santana, L. M. Lubián, M. Hernández-Arencibia, S. Hernández-León, E. Vázquez, S.N. Estrada-Allis (2014). Coupling between upper ocean layer variability and size-fractionated phytoplankton in a non-nutrient-limited environment. Marine Ecology Progress Series, 499, 35-46.

How to cite: Rodríguez-Santana, Á., Aguiar-González, B., Marrero-Díaz, Á., Valencia, L. P., and Machín, F.: Diapycnal Mixing in the Bransfield Strait, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9614, https://doi.org/10.5194/egusphere-egu23-9614, 2023.

EGU23-10079 | ECS | Posters on site | NP6.1

The role of turbulence and double-diffusion in the exchange of central waters at the Cape Verde Frontal Zone 

Luis P. Valencia, Ángel Rodríguez-Santana, Antonio Martínez-Marrero, Nadia Burgoa, Carmen Gordo, Diana Grisolía, and Ángeles Marrero-Díaz

The Cape Verde Frontal Zone (CVFZ) separates North and South Atlantic Central Waters (NCAW and SACW, respectively) in the eastern North Atlantic Subtropical Gyre. This front is described as a strong meandering thermohaline front near Cape Blanc at latitudes close to 20ºN. It shows sharp gradients in temperature and salinity in the upper 600 m with the presence of large lateral intrusions. One important aspect of the CVFZ is the compensating character of the temperature and salinity fields, which cause horizontal density gradients to be relatively small across the front. This frontal feature is an important factor in reducing vertical shear of horizontal velocity in some parts of the frontal region, allowing double diffusion processes to be one of the main causes of the observed diapycnal mixing. However, the presence of large lateral intrusions could favor diapycnal mixing induced by vertical shear instabilities which could overcome double diffusion effects. Despite its importance, studies in the CVFZ with direct turbulence measurements focused on diapycnal mixing and its relation with lateral thermohaline intrusions are scarce. In this study, we use microstructure measurements from a vertical free-falling profiler together with CTD-O and SADCP records of two high spatial resolution (each oceanographic stations ~9 km apart) oceanographic transects along and across the CVFZ (~300 and 100 km, respectively) during November of 2017. An assessment of the turbulent and double-diffusive mixing related to the lateral intrusions was made, identifying the latter through the diapycnal spiciness curvature method. Lateral intrusions ranging from ~20-100 km at subsurface and central levels of the water column showed relative increments in dissipation and diapycnal diffusivity. Therefore, at their boundaries occur the exchange of properties between the NACW and SACW.

How to cite: Valencia, L. P., Rodríguez-Santana, Á., Martínez-Marrero, A., Burgoa, N., Gordo, C., Grisolía, D., and Marrero-Díaz, Á.: The role of turbulence and double-diffusion in the exchange of central waters at the Cape Verde Frontal Zone, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10079, https://doi.org/10.5194/egusphere-egu23-10079, 2023.

EGU23-10130 | Orals | NP6.1

The stability of an asymmetric slice of the Gulf Stream 

Francis Poulin

The Gulf Stream plays an important role in the meridional overturning circulation in the North Atlantic, one of the primary mechanism by which the warm, salty water can move from low to high latitudes. It also provides closure to the North Atlantic subtropical gyre circulation as a western boundary current and makes Western European countries much warmer by transporting warm water across the ocean.

Observational data of the Gulf Stream (along the Oleander line, between New Jersey and Bermuda) has found that its stream-wise velocity skews to the right with increasing depth. This has motivated our development of an idealized model of a laterally skewed Gulf Stream jet that is surface trapped overlying a flat bottom. The nonlinear evolution of this unstable asymmetric jet is investigated using the Oceananigans.jl library for multiple values of a skewness parameter. The results show that the maximum growth rate has a nonlinear dependency on the skewness parameter, though weak and strong skew tend to be stabilizing and destabilizing, respectively. 

How to cite: Poulin, F.: The stability of an asymmetric slice of the Gulf Stream, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10130, https://doi.org/10.5194/egusphere-egu23-10130, 2023.

EGU23-10892 | ECS | Posters on site | NP6.1

Triadic resonance of internal wave modes with background shear 

Ramana Patibandla, Anubhab Roy, and Manikandan Mathur

In this work we study resonant triad interactions among discrete internal wave modes in a finite-depth, two dimensional uniformly stratified shear flow. The primary wave-field is considered to be a linear superposition of various internal wave modes. The weakly-nonlinear solution of the primary wave-field consists of a superharmonic (2ω) part and a mean-flow part (ω=0).  For a given modal interaction, we study the location in the frequency (ω) -Richardson number (Ri) parameter space where the amplitude of the superharmonic part attains a maximum i.e, where two primary internal wave modes of modenumbers 'm' and 'n' resonantly excite a secondary wave mode of modenumber 'q'. Using asymptotic theory we show that, unlike the case of no-shear, the presence of weak-shear, doesn't require the vertical wavenumber condition to be satisfied for resonance. This entails an activation of several new resonances in the presence of arbitrarily weak shear, where only the frequency and the horizontal wavenumber conditions are satisfied. This also leads to the possibility of self-interaction and resonances close to ω = 0. A similar asymptotic theory can be extended to other inhomogeneities (eg: non-uniform stratification) as well. For an exponential background shear flow, we track the location of these resonances in the (ω, Ri) parameter space and present their behaviour.

How to cite: Patibandla, R., Roy, A., and Mathur, M.: Triadic resonance of internal wave modes with background shear, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10892, https://doi.org/10.5194/egusphere-egu23-10892, 2023.

EGU23-12895 | Posters on site | NP6.1

Growth and chain formations of diatoms (Pseudo-nitzschia) under different turbulent conditions: a laboratory analysis 

Vasileios Bampouris, Emilie Houliez, Francois G. Schmitt, Muriel Crouvoiser, Kostas Kormas, and Urania Christaki
Diatoms have high productivity and are highly influenced by turbulent conditions. We consider here diatoms of the species Pseudo-nitzschia,  which are chain forming. The objective of this work was to show how the turbulent environment affects the growth and the chain forming of these species. For this, cultures of the species Pseudo-nitzschia multiseries and Pseudo-nitzschia fraudulenta were performed in the laboratory and submitted to stationary turbulent conditions, using the Agiturb system developed in the LOG at Wimereux (Le Quiniou et al. 2022). 
In the Agiturb system, the turbulent flow is produced using four contra-rotating agitators that are placed under a cubic tank, generating a statistically stationary, spatially inhomogeneous flow with compression and stretching. The injection of the energy in the flow is produced by 4 stirring bars activated by 4 magnetic stirrers situated at symmetric positions. The cubic tank is almost half-full with 15 liters of sea water. For each experiment, the magnitude of the rotation rate of each agitator was identical, with two agitators rotating clockwise and two anti-clockwise, the same directions being along the diagonal. Different values of the rotation rate were chosen to reach different turbulence levels, characterized by the microscale Reynolds number Rλ going from 130 to 360. These Reynolds numbers correspond to typical values found in the ocean, from the epicontinental zone, to coastal, surf zones and even storm conditions. 
In the experiments, all the other parameters that affect the diatoms’ proliferation were kept the same. Formation and growth of the chains were assessed through microscopy.  P. fraudulenta displayed higher growth than P. multiseries in all turbulence levels except from the control condition (Rλ=0) where the growth was approximately the same. The level of turbulence that was more beneficial for the growth of P. multiseries was the agitated (Rλ= 240) whereas for P. fraudulenta it was for a smaller Reynolds number (Rλ = 160). The chain length were also considered in relation with turbulence level, by considering the probability density of single chains, small chains (2 or 3 cells) and long chains (more than 4 cells). The result was that the predominant form of the cells for both species was the single cells. However, P. multiseries presented higher variations in chain forming throughout the whole experiment than P. fraudulenta. Within this approach, the optimal turbulence level, for growth as well as chain formation, can be assessed for each phytoplankton species.

How to cite: Bampouris, V., Houliez, E., Schmitt, F. G., Crouvoiser, M., Kormas, K., and Christaki, U.: Growth and chain formations of diatoms (Pseudo-nitzschia) under different turbulent conditions: a laboratory analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12895, https://doi.org/10.5194/egusphere-egu23-12895, 2023.

EGU23-12946 | ECS | Orals | NP6.1

A Semi-Lagrangian solver for the free surface Euler system with application to rotational wave flows 

Andreas Alexandris-Galanopoulos and Kostas Belibassakis

Even though the majority of the classical water wave theory is restricted to potential flows, vortical flows are abundant in nature. This necessitates the need for the development of accurate and efficient methods for the simulation of rotational phenomena, such as the propagation of waves over bathymetry in the presence of a sheared current [1, 2].

In the present work, a numerical method for the free surface Euler system with constant density and general bathymetry is developed within the framework
of classical Computational Fluid Dynamics (CFD). Specifically, using the well known σ coordinate system, a layer-wise integration followed by an operator
splitting is performed. The resulting horizontal advection component is, treated as a multilayered Shallow Water Equations (mSWE) system (see, e.g. [3]) 
and it is solved with a conventional Finite Volume solver. The vertical counterpart (that works similar to remeshing operator) regulates if the system is treated with a Lagrangian or an Eulerian approach. Finally, the dynamic pressure component coupled with the incompressibility constraint is treated using the well-known projection of Chorin [4].

The method’s main advantages stem from its highly modular character that makes it both robust and easy to implement. The method’s performance is tested in the case of waves propagating on top of a sheared current. Results concerning the dispersion and propagation characteristics for general current profiles are presented and compared with other models [1,2,5].

References
[1] Julien Touboul and Kostas Belibassakis. A novel method for water waves propagating in the presence of vortical mean flows over variable bathymetry. Journal of Ocean Engineering and Marine Energy, 5(4):333–350, 2019
[2] Kostas Belibassakis and Julien Touboul. A nonlinear coupled-mode model for waves propagating in vertically sheared currents in variable
bathymetry—collinear waves and currents. Fluids, 4(2):61, 2019.
[3] Fracois Bouchut and Vladimir Zeitlin. A robust well-balanced scheme for multi-layer shallow water equations. Discrete and Continuous Dynamical
Systems-Series B, 13(4):739–758, 2010.
[4] Zhe Liu, Lei Lin, Lian Xie, and Huiwang Gao. Partially implicit finite difference scheme for calculating dynamic pressure in a terrain-following coordinate
non-hydrostatic ocean model. Ocean Modelling, 106:44–57, 2016. [5] Ellingsen SA, Li Y (2017) Approximate dispersion relations for waves on arbitrary shear flows. J Geophys Res Oceans 122(12):9889–9905
[5] Ellingsen SA, Li Y (2017) Approximate dispersion relations for waves on arbitrary shear flows. J Geophys Res Oceans 122(12):9889–9905

How to cite: Alexandris-Galanopoulos, A. and Belibassakis, K.: A Semi-Lagrangian solver for the free surface Euler system with application to rotational wave flows, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12946, https://doi.org/10.5194/egusphere-egu23-12946, 2023.

EGU23-13078 | ECS | Orals | NP6.1

In situ observation of mode 1 nonlinear internal waves of opposite polarity in a changing environment 

Adèle Moncuquet, Nicole Jones, Lucie Bordois, Andrew Zulberti, François Dufois, Florent Grasso, and Pascal Lazure

The Bay of Biscay (Bob) is a hot spot for the generation of internal tides and nonlinear internal waves (NLIW). However, no studies have focused on internal waves on the continental shelf of the Bob. Here, we present 22 days of collocated temperature, velocity and backscatter profiles within a water depth H of 65 m. The background stratification evolved from two pycnoclines, with the strongest one near the sea bed, to a continuous profile due to wind-driven upwelling.

Under the double pycnocline situation, we observed trains of elevation emerging from each internal tidal front with amplitude reaching up to H/4 and propagating at speeds between 0.1 and 0.35 m/s. Sporadically depression waves were measured within the train and can propagate substantially faster (between 0.36 and 0.54 m/s). With the continuous stratification, the trains of NLIWs of elevation and containing opposite polarities were no longer observed.

These observations suggest that depression waves can cross the train of elevation waves. Resulting interactions could have significant impacts on sediment dynamics over the shelf. The double pycnocline regime and the impact of the stratification modification due to wind will be investigated numerically in future work.

How to cite: Moncuquet, A., Jones, N., Bordois, L., Zulberti, A., Dufois, F., Grasso, F., and Lazure, P.: In situ observation of mode 1 nonlinear internal waves of opposite polarity in a changing environment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13078, https://doi.org/10.5194/egusphere-egu23-13078, 2023.

EGU23-13754 | ECS | Posters on site | NP6.1

Multi-scale analysis of atmospheric and oceanic pCO2 time series and of their difference 

Kévin Robache, François G. Schmitt, and Yongxiang Huang
The oceans play an important role in the carbon cycle by exchanging CO2 with the atmosphere. These exchanges correspond to the biological pump, where the ocean can be sink or source of atmospheric CO2. Our hypothesis is that CO2 concentration, either atmospheric or oceanic, are chemical tracers being strongly influence by turbulence: we thus study separately their dynamics, and also their difference which is giving indication of the direction of the air-sea CO2 flux.
For this we use a publicly available data set of pCO2 simultaneous measurements at high frequency (typically 3 hours time step) at 40 difference places around the globe, from surface buoys (Sutton et al. 2019). We consider here the scaling properties of these quantities in order to characterize their multi-scale fluctuations, which are considered in the framework of passive or active scalars in turbulence.  For each site, this is done by analyzing temperature, salinity, oceanic (pCO2sw), atmospheric (pCO2air) pCO2 and their difference $\delta = pCO2sw - pCO2air$. Power spectral density are estimated in Fourier space and using Hilbert spectral analysis, with adapted methodologies to take into account the missing data problem. Spectral slopes are recorded and are interpreted in relation with the local climatology, depth and other factors.

How to cite: Robache, K., Schmitt, F. G., and Huang, Y.: Multi-scale analysis of atmospheric and oceanic pCO2 time series and of their difference, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13754, https://doi.org/10.5194/egusphere-egu23-13754, 2023.

We report on results from laboratory experiments performed in a quasi-two-layer system of cold and warm water in a rectangular laboratory tank. Warm front propagation is initiated by removing a vertical barrier from between the two prepared sections of the tank containing cold and warm water filled up to the same level. The warm front propagation in the vicinity of the free water surface is monitored using a high precision infrared camera from above, and with dye visualisation from the side simultaneously. After the warm front reaches the sidewall of the tank, its "head" is reflected, and hence an internal bore emerges along the interface separating the two layers. Following further reflections the bore splits to a train of internal solitary waves, resembling the solutions of the KdV equation. We find that, interestingly, although the waves propagate along the internal interface, certain surface signatures of the bore and wave dynamics can be detected from the water surface temperature fields due to secondary convective flows. This result may have certain applicability for the detection of internal waves using infrared sea-surface temperature data from satellites.

How to cite: Vincze, M. and Kiss, Z. Á.: Laboratory experiments on internal solitary wave reflections and their detectability via water surface infrared thermography, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14424, https://doi.org/10.5194/egusphere-egu23-14424, 2023.

EGU23-14457 | Orals | NP6.1

Weakly nonlinear wave energy flux and radiation stress 

Paolo Pezzutto

It is known that the wave action propagated in spectral wave models is a small steepness approximation of the observable wave action. For relevant steepness, we need higher order corrections to get a proper representation of the sea states [Janssen, 2009]. For the same reasons, other diagnostic variables should be corrected. Based on the fifth order Stokes solution obtained by Fenton [1985], Jonsson and Arneborg [1995] showed the importance of higher order corrections for determining the energy properties of long crested waves.

Proceeding from Longuet-Higgins and Stewart [1960], assuming a mean stream velocity, we see that how, using Krasitskii [1994] canonical transformations, we can derive general 2D weakly non linear corrections to the rate of transfer of energy across a surface fixed in space. For a monochromatic wave, the resulting equations are compared with truncated expressions given by Jonsson and Arneborg [1995], confirming that second order contributions (in terms of wave energy) can be relevant, depending on steepness and relative water depth.
After applying a proper statistical closure, the derived equations can be used to correct the wave energy properties of wave models spectra, for example to refine the informations transferred to a coupled circulation model.

John D. Fenton. A Fifth-Order Stokes Theory for Steady Waves. Journal of Waterway, Port, Coastal, and Ocean Engineering, 111(2):216–234, 1985. ISSN 0733-950X.
Peter a. E. M. Janssen. On some consequences of the canonical transformation in the Hamiltonian theory of water waves. J. Fluid Mech., 637(November):1–44, 2009. ISSN 1469-7645.
Ivar G. Jonsson and Lars Arneborg. Energy properties and shoaling of higher-order stokes waves on a current. Ocean Engineering, 22(8):819–857, 1995. ISSN 00298018.
Vladimir P. Krasitskii. On reduced equations in the Hamiltonian theory of weakly nonlinear surface waves. J. Fluid Mech., 272(-1):1–20, 1994. ISSN 0022-1120.
M. S. Longuet-Higgins and R W Stewart. Changes in the form of short gravity waves on long waves and tidal currents. Journal of Fluid Mechanics, 8(04): 565–583, 1960.

 

How to cite: Pezzutto, P.: Weakly nonlinear wave energy flux and radiation stress, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14457, https://doi.org/10.5194/egusphere-egu23-14457, 2023.

EGU23-15036 | Orals | NP6.1

Resonant water-waves in a circular channel: forced KdV solutions 

Uwe Harlander, Franz-Theo Schön, Ion D. Borcia, Sebastian Richter, Rodica Borcia, and Michael Bestehorn

Tidal bores are natural phenomena observed in at least 450 river estuaries all around the world from Europe to America and Asia. Tidal bores manifest as a series of waves propagating over long distances upstream in the estuarine zone of a river. Bores can be studied experimentally using sloshing water tanks where sloshing itself is a process with many applications, not only relevant for environmental flows. In a remarkable paper, Cox and Mortell (1986) showed that for an oscillating water tank, the evolution of small-amplitude, long-wavelength, resonantly forced waves follow a forced Korteweg-de Vries (fKdV) equation. The solutions of this model agree well with experimental results by Chester and Bones (1968). At first glance this is surprising since their experimental setup is in conflict with a number of assumptions made for deriving the fKdV equation. It is hence worth to repeat the experiment by Chester and Bones but using a long narrow channel setup.

We use a long circular channel and repeat the experiments by Chester and Bones. We compare the results with solutions from the fKdV equation but also with the one from a full nonlinear model solving the Navier-Stokes equations. Under resonance conditions, depending on the parameters, we find a range of nonlinear localized wave types from single and multiple solitons to undular bores. As shown by Cox and Mortell, when the fluid is considered to be inviscid a kind of Fermi-Pasta-Ulam recurrence is observed for the fKdV model. Stationarity is reached by including a weak damping to the fKdV equation. 

References
A.A. Cox, M.P. Mortell 1986. J. Fluid Mech. 162, pp. 99-116.
W. Chester and J.A. Bones 1968. Proc. Roy. Soc. A, 306, 23 (Part II).

How to cite: Harlander, U., Schön, F.-T., Borcia, I. D., Richter, S., Borcia, R., and Bestehorn, M.: Resonant water-waves in a circular channel: forced KdV solutions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15036, https://doi.org/10.5194/egusphere-egu23-15036, 2023.

EGU23-15066 | Orals | NP6.1

Breaking threshold and energy dissipation in solitary waves in a depth transition 

Wouter Mostert, Hunter Boswell, and Guirong Yan

Energy dissipation due to the breaking of surface waves remains an important open topic in both the open ocean and in coastal waters. Here we will discuss similarities between the deep- and shallow-water regimes. To do this, we first present data from direct numerical simulations of shoaling and breaking solitary waves in bathymetric depth transition. In an abrupt depth transition, we investigate the influence of the severity of the depth transition on whether the incident wave will break, finding good agreement with experimental data of Losada et al. (1988). We next investigate the energy dissipation rate in a gradual, linear depth transition. The resulting dataset is compared with an array of existing physics-based scaling arguments, and finds especially good agreement with an inertial model of Mostert & Deike (2020). We then discuss possible scaling approaches for understanding breaker dissipation in shallow water and draw comparisons with deep-water data and models. We will conclude with some insights towards a potential universal breaking parametrisation.

How to cite: Mostert, W., Boswell, H., and Yan, G.: Breaking threshold and energy dissipation in solitary waves in a depth transition, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15066, https://doi.org/10.5194/egusphere-egu23-15066, 2023.

EGU23-16032 | ECS | Orals | NP6.1

Imprint of ocean currents on signicant wave height 

Han Wang, Bia Villas Bôas, Jacques Vanneste, and William Young

Ocean currents have been observed to impact the spatial distribution of significant wave height (hereafter "Hs") of surface gravity waves profoundly, with implications for air-sea fluxes, extreme waves, and error budget in satellite observations. In this work, we derive analytic formulas that relate Hs to current velocities under the weak-current approximation, cross-validate the results with WAVEWATCH III, and find implications potentially useful for observational and modelling studies. 

First, we show that when swell-like surface waves interact with a localized current, caustics, where rays cross in real space, do not lead to singularities in Hs if the wave energy spectra have a realistic directional spread in wavenumber space. This has implications for understanding the origin of freak waves, where caustics have been postulated as a possible source. Then, we consider another regime where weak turbulent flows are considered. Analytic formulas are found that deterministically link the patterns of Hs to currents. The formulas' statistical counterparts are applied to study how the spectral slopes, amplitudes and directionality of Hs are related to currents. Our results demonstrate that the variations of Hs are controlled by the rotational component of the currents, suggesting the potential of using information from surface wave to infer current properties in real observations, or vice versa.

How to cite: Wang, H., Villas Bôas, B., Vanneste, J., and Young, W.: Imprint of ocean currents on signicant wave height, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16032, https://doi.org/10.5194/egusphere-egu23-16032, 2023.

EGU23-16131 | ECS | Posters on site | NP6.1

Lagrangian flow networks for passive dispersal: tracers versus finite-size particles 

Deoclécio Valente, Ksenia Guseva, and Ulrike Feudel

Passive dispersal of different materials in ocean flows has gotten considerable attention over the last decade to increase our knowledge about the distribution of seeds plants among islands and coastal areas, the transport of larvae of different organisms between habitats and the transport of litter. Most studies have treated these objects as tracers to investigate distribution patterns and connectivity between different areas. We compare this approach with a study that considers the objects' size and density and discusses the deviation from the tracer approach. To this end, we introduce a two-dimensional kinematic velocity field which allows us to study the connectivity between an arbitrary number of islands located at arbitrary but prescribed positions in an open flow of a given direction. First, the mixing induced by the islands, which act as obstacles in the flow, was accounted for with the inclusion of a von K\'arm\'an vortex street in the wake of each island. Furthermore, we accounted for the size and density of particles approximated as spheres. Finally, we treated the particles as inertial particles experiencing various forces in the flow and computed their trajectories in a given flow field by solving the Maxey-Riley equations. In this way, we have constructed a Lagrangian flow network reflecting the connectivity between islands depending on the properties of the finite-size particles and comparing them with the motion of tracers. We show that the density differences, the flow properties, and the islands' position geometry substantially change the connectivity between islands. That change leads to segregating inertial particles according to their size and density. Nevertheless, the most striking observation is how the tracer transport (independently of geometry) overestimates the probabilities for specific pathways. In fact, the connectivity for inertial particles is much sparser than for tracers, such that certain pathways have extremely low probabilities; they practically do not exist. These results suggest that the transport probabilities can be highly under or overestimated by tracers' often-used approximation of inertial particles.

How to cite: Valente, D., Guseva, K., and Feudel, U.: Lagrangian flow networks for passive dispersal: tracers versus finite-size particles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16131, https://doi.org/10.5194/egusphere-egu23-16131, 2023.

EGU23-16217 | Posters on site | NP6.1

A cumulant analysis of ocean waves fluctuations over the global ocean, using CFOSAT data 

Amine Benbelkacem, François Schmitt, and Yongxiang Huang

The China France Oceanography Satellite (CFOSAT) was launched in October, 2018 and records over the oceans the wind field as well as the ocean waves. We consider here the ocean wave data, which are given through the significant wave height (Hs). We analyse along-track fluctuations of $Hs$ by considering its fluctuations of the form $y_r = \Delta_r Hs = Hs(x+r)-Hs(x) $, with values of the spatial scale $r$ between 12.5 km and a global and large scale of 2000 km. For this we consider a cumulant approach: we estimate the cumulant generating function (of $\log y_r$) $\Psi(q) = \log <y_r^q>$. This function is considered in a log-stable framework, where its development is non-analytical of the form $\Psi(q)= C_1 q + C_{\alpha} q^{\alpha}$, where $C_1$ is the first cumulant ($C_1 = < \log y_r>$), $0< \alpha \leq 2$ is the non-analycity parameter and $C_{\alpha}$ a parameter. The analysis is done by partionning the global ocean into several oceans: Indian ocean, South and North Pacific, South and North Atlantic. The statistics of the three parameters are considered over the scale $r$ and for each ocean. This provides a global view of the significant wave height multi-scale fluctuations and is complementary to a previous analysis done using Fourier spectral analysis (Gao et al 2021).

How to cite: Benbelkacem, A., Schmitt, F., and Huang, Y.: A cumulant analysis of ocean waves fluctuations over the global ocean, using CFOSAT data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16217, https://doi.org/10.5194/egusphere-egu23-16217, 2023.

EGU23-16425 | ECS | Posters on site | NP6.1

Comparison of wavelet- and FFT-based bathymetry retrieval methods and its application to nearshore X-band radar image sequenses 

Pavel Chernyshov, Michael Stresser, Ruben Carrasco, and Jochen Horstmann

Wavelet- and Fast Fourier Transform (FFT)-based methods for bathymetry retrieval from X-band radar image sequences are compared and analyzed. Both methods utilize the similar idea of the waves' phase shift estimation using cross-spectral analysis. Within the FFT-based approach the corresponding technique is used to determine wave vector's components from the image sequence frequency decomposition. The last means that the time FFT is applied to the original image sequence. Then for each frequency slice the corresponding wavenumber is derived applying the cross-spectrum analysis of the one pixel shifted images in the corresponding spatial direction. In such a way a set of wavevector-frequency (k, ω) pairs are formed and filtered according to a confidence criterion that reflects the stability of the local phase pattern. In the case of a wavelet-based method the corresponding cross-spectral analysis is applied to the 2D Continuous Wavelet Transform (CWT) directional complex spectra for pairs of successive images, resulting in a set of wavevector-celerity (k, c) pairs. Further, the corresponding set of pairs are fitted to the unknown depth using nonlinear least-square method and finite water depth linear dispersion relationship as a model. Weights proportional to the spectral power density and confidence values are used in the fitting process for the wavelet- and FFT-based methods correspondingly. Furthermore, both methods are verified by applying it to stochastic simulations of corresponding shoaling sea elevation image sequences and real X-band radar image sequences collected near the Hofn tidal inlet (Iceland). For the wave simulations, a linear solution of a mild slope equation is utilized. In order to accout for the effects ofthe ambient currents, a ray-tracing technique is applied. As a testing case, the shoaling of an incident JONSWAP spectrum-based wavefields are evaluated both on the following and opposing currents. A radar image model including tilt and shadowing modulations together with speckle noise is further applied to the modeled surface elevations. Both methods are able to reconstruct the original bathymetry for intermediate to shallow water depths (kph<1.2) with plausible accuracy both for all the synthetic cases (with varied probing geometries, bottom topography, ambient current, and sea state conditions) and real radar data case. In the last case, the accuracy of the FFT-based method is on the level 0.7-0.9 m in terms of the mean absolute error value with fairly small bias the standard deviation of the error is also less than 1 m in the whole area studied except the tidal channel, where the depth gradients are significantly larger. The wavelet-based method showes a higher bias with comparable mean absolute error and standard deviation.

How to cite: Chernyshov, P., Stresser, M., Carrasco, R., and Horstmann, J.: Comparison of wavelet- and FFT-based bathymetry retrieval methods and its application to nearshore X-band radar image sequenses, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16425, https://doi.org/10.5194/egusphere-egu23-16425, 2023.

EGU23-16723 | Orals | NP6.1

Three-dimensionnal Wave-Current Interactions can significantly affect a Strong Tidal Current in a Complex Environment: Application to Alderney Race 

Anne-Claire Bennis, Lucille Furgerot, Pascal Bailly du Bois, Emmanuel Poizot, Yann Méar, and Franck Dumas

Due to the climate change, it is necessary to modify the energy modes of production. The mix energetic, based on renewable energies as tidal currents, is one of the solutions to decrease the energy production carbon footprint. This study focuses on hydrodynamic interactions in Alderney Race (France), which is the most energetic tidal site in Western Europe. The impact of a winter storm occurring during spring tide is assessed thanks to numerical modeling with a 3D fully-coupled wave-current model and in-situ data. Firstly, an analysis of the impacts of the storm on the wave field and the current effects on waves is performed. Then, the modifications of the current and tidal stream energy caused by waves are discussed. After a successful validation step with excellent PBIAS and R2 scores, the main finding are : i) although the current intensity is strong (around 3-4m/s), wave effectssignificantly change the vertical profile of the current, with a reduction of the PBIAS by a factor of 1.78 between simulations with and without wave effects, ii) ocean waves affect the tidal assymmetry, with a flood current whose intensity is 13% higher than for the ebb current, inducing a decrease of 30% in the tidal stream energy, iii) the flow is very sensitive to the angle between the directions of propagation of waves and current, with an acceleration or a reduction of the velocity, as observed in the presence of a 3D turbulent structure, iv) current effects on waves cause a wavenumber shift, changes in significant wave height (modulated by tide), wave direction due to refraction and an increase of the energy transfer from waves to ocean ascribed to the wave breaking. By a feedback mechanism, the modifications of the wave field by current and water level significantly alter the flow with a decrease of its velocity when waves propagate against current. This study shows that the 3D wave-current interactions need to be considered during a storm even during a spring tide event where currents are the strongest.

How to cite: Bennis, A.-C., Furgerot, L., Bailly du Bois, P., Poizot, E., Méar, Y., and Dumas, F.: Three-dimensionnal Wave-Current Interactions can significantly affect a Strong Tidal Current in a Complex Environment: Application to Alderney Race, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16723, https://doi.org/10.5194/egusphere-egu23-16723, 2023.

EGU23-16817 | ECS | Posters virtual | NP6.1

Comparison of CPU and GPU parallelization approaches between two programming languages in copepod model simulations 

Varshani Brabaharan, Sachithma Edirisinghe, and Kanchana Bandara

This study presents a comparative assessment to evaluate between two high performance computing languages, Java and FORTRAN for the computation vs. communication trade-off observed during a strategy-oriented copepod model simulation. Here we compared the computational time of (i) sequential processing, (ii) latency (CPU) and (iii) throughput (GPU) oriented designs. CPU based parallelization was accomplished on a 4-core Intel i7 processor with a clock speed of 1.99 GHz. On this CPU, we implemented a (i) fork/join framework design based on work-stealing algorithm in Java and (ii) Open Multi- Processing (OpenMP), a directive-based application programming interface (API) with shared memory architecture on FORTRAN 95. The GPU processing power was leveraged using the CUDA framework in Java and OpenACC API on FORTRAN on a NVIDIA GeForce MX230 with 256 unified pipelines. The simulation time for sequential CPU execution was ca. 41% lower in FORTRAN compared to Java (18 s vs. 25 s). Furthermore, the FORTRAN simulation was ca. 43% lower in execution time in latency-oriented CPU design compared to Java (10s vs. 13s). In the simulation regarding GPU-approach with unified memory space accessibility, Java computation consumed ca. 38% less time than FORTRAN (5s vs. 8s). Unlike FORTRAN, Java is purely an object-oriented language and therefore, object handling is not optimized in GNU compliers of FORTRAN. Nevertheless, memory consumption of FORTRAN can be fine-tuned thereby, decreasing latency unlike in Java. OpenMP API is based on self-consistency, shared memory architecture and its temporary view memory allows threads to cache variables and thereby reduce latency by avoid accessing the memory for each reference of variables unlike the fork/join framework in Java. Furthermore, OpenMP has a thread private memory, which allows efficient synchronization within the code. OpenACC is designed as a high-level platform, which is an independent abstract programming accelerator that offers a pragmatic alternative for accessing GPU programming without much programming effort. Nevertheless, some uses of unified memory space accessibility on NVIDIA GPU’s are better represented in CUDA despite OpenACC having a cache directive. Therefore, its best to investigate the performances of different accelerator models and different programming languages depending on the simulation needs and efficiency targets desired by the model.

Keywords: FORTRAN, Java, OpenMP, OpenACC, high-performance computing, copepods, modelling

How to cite: Brabaharan, V., Edirisinghe, S., and Bandara, K.: Comparison of CPU and GPU parallelization approaches between two programming languages in copepod model simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16817, https://doi.org/10.5194/egusphere-egu23-16817, 2023.

Phytoplankton populations have been in a steep decline in the elbe estuary since several decades. Previous studies using concentration based biochemical models helped to further the understanding of the ecosystem in general but fail to pinpoint specific reasons due to their high complexity.

We approach this problem with a novel langrangian model. By explicitly simulating phytoplankton trajectories, we are able to examine bathymetry-related effects. These effects can play a big role in the Elbe estuary due the high average depth in the navigational channel of Hamburg’s harbor.  In detail, or model represent processes like turbulent dispersion, vertical migration and stranding mechanics to study this problem. To our knowledge this is the first time that this problem is tackled with such a method that includes biological processes in an estuarine context.

We will present results from experiments looking at Phytoplankton retention mechanics to avoid outwashing and depth related mortality in the navigational channel.

How to cite: Steidle, L.: Phytoplankton trajectories in the Elbe estuaries - examinig retention and die-off in the Hamburg harbor, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16913, https://doi.org/10.5194/egusphere-egu23-16913, 2023.

EGU23-17262 | ECS | Posters on site | NP6.1

Internal tides off the Amazon shelf: importance to structure ocean's temperature during two contrasted seasons 

Fernand Assene, Ariane Koch-Larrouy, Isabelle Dadou, Michel Tchilibou, Guillaume Morvan, Jérôme Chanut, Vincent Vantrepotte, Damien Allain, and Trung-Kien Tran

Tides and internal tides (IT) in the ocean can significantly affect local to regional ocean temperature and even sea surface temperature (SST), via processes such as vertical mixing, vertical advection and transport of water masses. Offshore of the Amazon River, IT have already been detected and studied; however, their impact on temperature, SST and associated processes are not known in this region. In this work, we use high resolution (1/36°) numerical simulations with and without the tides from an ocean circulation model (NEMO) which explicitly resolves the internal tides (IT), to assess how they can affect ocean temperature in the studied area. We distinguish the analysis for two contrasted seasons, from April to June (AMJ) and from August to October (ASO), since the seasonal stratification off the Amazon River modulates the IT’s response and their influence in temperature.  

The IT are well reproduced by the model, and are in good agreement with observations, for both their generation and their propagation. The simulation with tides is in better agreement with satellite SST data compared to the simulation without tides. During ASO season, stronger meso-scale currents, deeper and weaker pycnocline are observed in contrast to the AMJ season. Results show that the observed coastal upwelling during ASO season is well reproduced by the model including tides, whereas the no-tide simulation is too warm by +0.3 °C at sea surface. In the subsurface above the thermocline, the tide simulation is cooler by -1.2 °C, and warmer below the thermocline by +1.2 °C compared to the simulation without the tides. The study further highlights that the IT induce vertical mixing on their generation site along the shelf break and on their propagation pathways towards the open ocean. This process explains the cooler temperature at the ocean surface and in the subsurface water above the thermocline and a warming in the deeper layers (below the thermocline). The surface cooling induced in turn an increase of the net heat flux from the atmosphere to the ocean surface, which could induce significant changes in the local and even for the regional tropical Atlantic atmospheric circulation and precipitation. We therefore demonstrate that IT, mainly via vertical diffusivity along their propagation pathways of approximately 700 km offshore, and tides over the continental shelf, play a key role on the temperature structure off the Amazon River mouth, particularly in the coastal cooling enhanced by IT.  

How to cite: Assene, F., Koch-Larrouy, A., Dadou, I., Tchilibou, M., Morvan, G., Chanut, J., Vantrepotte, V., Allain, D., and Tran, T.-K.: Internal tides off the Amazon shelf: importance to structure ocean's temperature during two contrasted seasons, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17262, https://doi.org/10.5194/egusphere-egu23-17262, 2023.

EGU23-17324 | Orals | NP6.1

Inertial torque on a squirmer 

Bernhard Mehlig, Fabien Candelier, Jingran Qiu, Lihao Zhao, and Greg Voth

A small spheroid settling in a quiescent fluid experiences an inertial torque that aligns it so that it settles with its broad side first. Here we show that an active particle experiences such a torque too, as it settles in a fluid at rest. For a spherical squirmer, the torque is T = -9/8  mf (vs(0)  x vg(0)), where vs(0)  is the swimming velocity, vg(0) the settling velocity in the Stokes approximation, and mf the equivalent fluid mass. This torque aligns the swimming direction against gravity: swimming up is stable, swimming down is unstable. This talk is based on Candelier, F., Qiu, J., Zhao, L., Voth, G., & Mehlig, B. (2022). Inertial torque on a squirmer. Journal of Fluid Mechanics, 953, R1.

How to cite: Mehlig, B., Candelier, F., Qiu, J., Zhao, L., and Voth, G.: Inertial torque on a squirmer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17324, https://doi.org/10.5194/egusphere-egu23-17324, 2023.

Dispersion and deposition of mineral dust from natural or anthropogenic sources can have both positive and negative effects on the environment depending on the geochemical and mineralogical composition of the dust. In Greenland, proglacial river systems draining the Greenland Ice Sheet occupy extensive areas of dust prone deposits, which are commonly mobilized and transported by winds of both katabatic and cyclonic origin and subsequently deposited as high latitude dust. The geochemical fingerprint of natural dust emitted along the latitudinal transect reflects the mineralogical and elemental composition of the bedrock underlying the Ice Sheet in the different geological provinces of Greenland. As dust emissions respond to changes in climate-sensitive drivers such as soil moisture, winds speed and precipitation, marked variations in natural dust emissions are present along the climatic gradient in Greenland, ranging from high latitude arctic deserts in North Greenland to low latitude shrub tundra in the South.

With a changing climate, interest has increased to access and exploit the rich mineral resources located in the Arctic. In Greenland, development of large-scale mines range from rare earth element mines in the sub-arctic South to zinc-lead mines in the high-arctic North. While the mining sector provides society with essential raw materials for a wide range of industrial processes as well as forming the basis for the transition into a global green economy, it also has significant environmental pitfalls, which should be avoided or mitigated. Mobilization, transport, and deposition of mineral dust from mine sites is often significant in regions susceptible to wind erosion because of the dry climate and lack of vegetation. Once dispersed into the environment, this mineral dust may impair important ecosystem functions due to its potential content of heavy metals and other trace elements, as well as cause concerns for public health.

To support the sustainable development of environmentally safe mining in sensitive Arctic land areas and reduce airborne environmental pollution, an improved understanding of processes leading to the dispersion of mineral dust in a changing Arctic is needed. This involves improved methods for monitoring dust emissions and dust deposition in a cold environment as well as analytical tools and methods to source trace and differentiate between natural and mining related dust. Accurate identification of individual dust sources subsequently makes it possible to mitigate emissions and target the regulation of mining activities towards these sources.

In the following, we present a new high latitude dust sampling location in Kangerlussuaq, West Greenland, where dust is collected using a wide array of passive and active dust samplers, including a continuously operated high volume dust sampler, which will offer filter samples of large air volumes (13.000 m3) at a weekly sampling frequency over multiple years. In addition, we would like to present data from a study (1) in which we developed a fast and cost-effective surface screening methodology that is easily applicable for dust source characterization in remote Arctic areas such as Greenland, where dry conditions and high winds create a high natural dust generation potential.

(1) Søndergaard, J. & Jørgensen, C.J. (2021) DOI: 10.1007/s11270-021-05095-2

How to cite: Jørgensen, C. J., Søndergaard, J., and Mosbech, A.: Geochemical fingerprinting of high latitude dust – potential environmental impacts of natural and mining related dust in Greenland in a changing climate., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2609, https://doi.org/10.5194/egusphere-egu23-2609, 2023.

EGU23-3776 | Posters on site | ITS2.6/AS4 .5

The lifecycle of snow in the Sierra Nevada USA: from snowfall to snowmelt and effects on endangered bighorn sheep 

Yun Qian, Huilin Huang, Cenlin He, Ned Bair, and Karl Rittger

Snow is a valuable resource in California. Snow from the Sierra Nevada sustains a diverse ecosystem and provides 3/4 of California’s Agricultural water supply. Because of its importance in water supply and global climate, snow accumulation, melt, and sublimation were ranked as the most important objectives in the 2017 Decadal Survey. This study employs a fully coupled meteorology‐chemistry‐snow model to investigate the impacts of both global warming and light‐absorbing particles (LAPs) on snow in the Sierra Nevada. Using self-organizing map (SOM) analysis with dust deposition and flux data from model and observations, we identify four typical dust transport patterns across the Sierra Nevada, associated with the mesoscale winds, Sierra barrier jet, North Pacific High, and long-range cross-Pacific westerlies, respectively. The satellite retrievals and model results show that LAPs in snow reduce snow albedo by 0.013 (0–0.045) in the Sierra Nevada during the ablation season (April-July), producing a midday mean radiative forcing of 4.5 W m−2 which increases to 15–22 W m−2 in July. LAPs in snow accelerate snow aging processes and reduce snow cover fraction, which doubles the albedo change and radiative forcing caused by LAPs. The impurity-induced snow darkening effects decrease snow water equivalent and snow depth by 20 and 70 mm in June in the Sierra Nevada bighorn sheep habitat. The earlier snowmelt reduces root-zone soil water content by 20%, deteriorating the forage productivity and playing a negative role in the survival of bighorn sheep. We also conduct the simulations using our coupled regional model to compare the impact of global warming vs. LAPs on snow melting by adopting the pseudo-global warming (PGW) approach to generate projections of future meteorological forcing. These results will be used to examine snow effects on endangered Sierra Nevada bighorn sheep and how a future climate might modify habitat and behavior.

How to cite: Qian, Y., Huang, H., He, C., Bair, N., and Rittger, K.: The lifecycle of snow in the Sierra Nevada USA: from snowfall to snowmelt and effects on endangered bighorn sheep, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3776, https://doi.org/10.5194/egusphere-egu23-3776, 2023.

The amplified climate effect of black carbon (BC) in the Arctic is widely acknowledged. Despite this, information on its deposition patterns and particularly sources are still scarce from the area. Arctic-wide atmospheric BC monitoring show decreasing BC concentrations since the 1990s. However, increasing amounts of BC deposition records from the area show more spatial variability in long-term trends, and some records suggest deviating trends between atmospheric BC concentrations and deposition. Particularly in the European Arctic (northern Fennoscandia and northwestern Russia) BC deposition trends seem to have increased in recent decades rather than decreased as suggested by models and observed for atmospheric concentrations. Such dissimilarities between atmospheric BC concentrations and deposition trends suggest different meteorological processes and sources driving these, which need to be further studied to understand the effects of different BC emissions on the Arctic climate. Although we have quantified different BC fractions from lake sediments and ice cores in the European Arctic indicating variable deposition trends during the last 300 years, the records suggest surprisingly similar sources of the deposited BC particles. Our future endeavors lie in further illuminating the sources of deposited BC in the Arctic and particularly studying the potential significance of Russian gas flaring and increasing peatland fires.

How to cite: Korhola, A. and Ruppel, M.: Past black carbon deposition and sources in the European Arctic depicted from lake sediments and ice cores, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5032, https://doi.org/10.5194/egusphere-egu23-5032, 2023.

EGU23-5749 | Posters virtual | ITS2.6/AS4 .5

15-yr long records of aerosol and surface snow chemical composition at Dome C (High Antarctic Plateau) 

Rita Traversi, Silvia Becagli, Laura Caiazzo, Paolo Cristofanelli, Raffaello Nardin, Davide Putero, and Mirko Severi

The study of aerosol chemical composition in the Antarctic plateau can provide basic information on the main natural (and also anthropogenic) inputs, atmospheric reactivity, and long-range transport processes of the aerosol components. Moreover, chemical and physical processes occurring at the atmosphere-snow interface are yet not fully understood and work is needed to assess the impact of atmospheric chemistry on snow composition and to better interpret ice core records retrieved at those sites.

At this purpose, simultaneous aerosol and surface snow samplings were set up and run at Dome C station (75° 06’ S; 123° 20’ E, 3233 m a.s.l) all year-round since 2004/05 and are still ongoing through various PNRA Projects, particularly LTCPAA (2016-2020) and STEAR (2020-2023).

Aerosol and snow samples were analysed for main and trace ion markers, aiming to better constrain extent and timing of the main natural sources (sea salt, marine biogenic, mineral dust) and to detect the possible contribution of anthropic inputs (biomass burning, wildfires, local contamination). In addition, such a study might help in improving our knowledge of transport processes (free troposphere, stratosphere-troposphere exchange) and atmospheric reaction processes (such as neutralization, chemical fractionation).

A comparison with ozone measurements, carried out continuously over the same period, is also attempted, to better address the atmospheric processes involving the atmosphere-snow exchanges of N-cycle species and atmosphere oxidative properties.

How to cite: Traversi, R., Becagli, S., Caiazzo, L., Cristofanelli, P., Nardin, R., Putero, D., and Severi, M.: 15-yr long records of aerosol and surface snow chemical composition at Dome C (High Antarctic Plateau), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5749, https://doi.org/10.5194/egusphere-egu23-5749, 2023.

EGU23-6458 | ECS | Posters on site | ITS2.6/AS4 .5

An overview of recent High Latitude Dust (HLD) and aerosol measurements in Iceland, Antarctica, Svalbard, and Greenland, including HLD impacts on climate 

Pavla Dagsson Waldhauserova, Outi Meinander, Olafur Arnalds, and IceDust members

Two billion tons of dust are annually transported in our atmosphere all around the world. High latitudes include active desert regions with at least 5 % production of the global atmospheric dust. Active High Latitude Dust (HLD) sources cover > 1,600,000 km2 and are located in both the Northern (Iceland, Alaska, Canada, Greenland, Svalbard, North Eurasia, and Scandinavia) and Southern (Antarctica, Patagonia, New Zealand) Hemispheres. Recent studies have shown that HLD travels several thousands of km inside the Arctic and > 3,500 km towards Europe. In Polar Regions, HLD was recognized as an important climate driver in the IPCC Special Report on the Ocean and Cryosphere in a Changing Climate in 2019. In situ HLD measurements are sparse, but there is increasing number of research groups investigating HLD and its impacts on climate in terms of effects on cryosphere, cloud properties and marine environment.

Long-term dust in situ measurements conducted in Arctic deserts of Iceland and Antarctic deserts of Eastern Antarctic Peninsula in 2018-2023 revealed some of the most severe dust storms in terms of particulate matter (PM) concentrations. While one-minute PM10 concentrations is Iceland exceeded 50,000 ugm-3, ten-min PM10 means in James Ross Island, Antarctica exceeded 120 ugm-3. The largest HLD field campaign was organized in Iceland in 2021 where 11 international institutions with > 70 instruments and 12 m tower conducted dust measurements (Barcelona Supercomputing Centre, Darmstadt, Berlin and Karlsruhe Universities, NASA, Czech University of Life sciences, Agricultural University of Iceland etc.). Additionally, examples of aerosol measurements from Svalbard and Greenland will be shown. There are newly two online models (DREAM, SILAM) providing daily operational dust forecasts of HLD. DREAM is first operational dust forecast for Icelandic dust available at the World Meteorological Organization Sand/Dust Storm Warning Advisory and Assessment System (WMO SDS-WAS). SILAM from the Finnish Meteorological Institute provides HLD forecast for both circumpolar regions. 

Icelandic dust has impacts on atmosphere, cryosphere, marine and terrestrial environments. It decreases albedo of both glacial ice/snow similarly as Black Carbon,  as well as albedo of mixed phase clouds via reduction in supercooled water content. There is also an evidence that volcanic dust particles scavenge efficiently SO2 and NO2 to form sulphites/sulfates and nitrous acid. High concentrations of volcanic dust and Eyjafjallajokull ash were associated with up to 20% decline in ozone concentrations in 2010. In marine environment, Icelandic dust with high total Fe content (10-13 wt%) and the initial Fe solubility of 0.08-0.6%, can impact primary productivity and nitrogen fixation in the N Atlantic Ocean, leading to additional carbon uptake.

Sand and dust storms, including HLD, were identified as a hazard that affects 11 of the 17 Sustainable Development Goals. HLD research community is growing and Icelandic Aerosol and Dust Association (IceDust) has > 100 members from 55 institutions in 21 countries (https://icedustblog.wordpress.com, including references to this abstract). IceDust became new member aerosol association of the European Aerosol Assembly in 2022. 

 

How to cite: Dagsson Waldhauserova, P., Meinander, O., Arnalds, O., and members, I.: An overview of recent High Latitude Dust (HLD) and aerosol measurements in Iceland, Antarctica, Svalbard, and Greenland, including HLD impacts on climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6458, https://doi.org/10.5194/egusphere-egu23-6458, 2023.

EGU23-6600 | ECS | Posters on site | ITS2.6/AS4 .5

Topographic controls on the distribution of dark ice on the surface of the Greenland Ice Sheet 

Shunan Feng, Joseph Mitchell Cook, Alexandre Magno Anesio, Liane G. Benning, and Martyn Tranter

The Greenland Ice Sheet (GrIS) is the largest single cyospheric contributor to global sea level rise. The surface ice albedo modulates the absorption of solar radiation and the current darkening of the GrIS enhances the surface meltwater production. However, the dark ice is unevenly distributed on the GrIS. Remote sensing observations found that dark ice is limited to the margin in the southeast region, while the spatial extent of dark ice stretches further inland in the southwest GrIS. This band of dark ice, with an albedo that is significantly lower than the surrounding ice in the melt season, is known as the Dark Zone. One hypothesis is that the spatial distribution of dark ice is influenced by topography, and surface slope in particular. This study attempts to verify this hypothesis and presents the first medium resolution (30 m) analysis of the topographic controls on the distribution of dark ice on the surface of the GrIS. The association between albedo and topographic factors, such as elevation, slope and aspect, and the distance from the ice margin, and the duration of bare ice exposure, are investigated using the ArcticDEM and a satellite albedo product derived from a harmonized Landsat and Sentinel 2 dataset. The results may allow certain controls on glacier ice algal growth, a key contributor to the progressive darkening of the ice surface, to be surmised.

How to cite: Feng, S., Cook, J. M., Anesio, A. M., Benning, L. G., and Tranter, M.: Topographic controls on the distribution of dark ice on the surface of the Greenland Ice Sheet, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6600, https://doi.org/10.5194/egusphere-egu23-6600, 2023.

EGU23-7762 | ECS | Posters on site | ITS2.6/AS4 .5

Regional Impact of Snow-Darkening During a Severe Saharan Dust Deposition Event in 2018 Across Eurasia 

Anika Rohde, Heike Vogel, Gholam Ali Hoshyaripour, Christoph Kottmeier, and Bernhard Vogel

Aerosols such as mineral dust particles reduce the surface albedo when deposited on snow. This leads to increased absorption of solar radiation. Especially in spring, this phenomenon can lead to increased snowmelt, which triggers further feedbacks at the land surface and in the atmosphere. Quantifying the magnitude of dust-induced variations is difficult because of the high variability in the spatial distribution of mineral dust and snow. We present an extension of a fully coupled atmospheric and land surface model system to investigate the effects of mineral dust on snow albedo across Eurasia. In a comprehensive ensemble simulation study, we investigated the short-term effects of an extreme Saharan dust deposition event in 2018. We found region-dependent feedbacks. Mountainous regions and areas near the snowline showed a strong impact from mineral dust deposition. The former showed a particularly strong decrease in snow depth. For instance, in the Caucasus Mountains we found a mean significant decrease in snow depth of -1.4 cm after one week. The latter showed a stronger feedback effect on surface temperature. In the flat region around the snow line, we found a mean significant surface warming of 0.9 K after one week. This study shows that the effects of mineral dust deposition depend on several factors. Primarily, these are elevation, slope, snow depth, and fraction of snow cover. Therefore, especially in complex terrain, it is necessary to use fully coupled models to study the effects of mineral dust on the snowpack and the atmosphere.

How to cite: Rohde, A., Vogel, H., Hoshyaripour, G. A., Kottmeier, C., and Vogel, B.: Regional Impact of Snow-Darkening During a Severe Saharan Dust Deposition Event in 2018 Across Eurasia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7762, https://doi.org/10.5194/egusphere-egu23-7762, 2023.

EGU23-8920 | Posters on site | ITS2.6/AS4 .5

Meridional Saharan dust transport towards higher latitudes 

György Varga, Ágnes Rostási, Adrienn Csávics, Pavla Dagsson-Waldhauserova, Outi Meinander, and Fruzsina Gresina

Over the past decades, an increasing number of Saharan dust storm events have been identified across Europe, using satellite measurements and imagery, numerical simulation data, meteorological analyses, air mass dispersion trajectories and surface observations, thus excluding subjective forcing factors. Both the frequency and intensity of dust storm events have been increasing over the last decade.
Saharan dust reached the Carpathian Basin at least 250 times between 1979 and 2022. The episodes of intense dust deposition in Hungary clearly showed the effect of the downwelling of high-latitude jet streams, leading to (1) extreme weather events and intense dust storms in the Atlas region and (2) increased atmospheric meridionality, which transported the large amounts of dust northwards.
To identify such events, we started our research in the North Atlantic region, where we identified 15 Saharan dust storm events in Iceland between 2008 and 2020, two of which were also surface sampled. The scope of these studies has now been extended to 1980 to 2022 to identify further events. Laboratory analyses of the sampled dust material have found abundant quartz particles larger than 100 µm, indicating that large dust particles can sometimes travel thousands of kilometres.
Similar studies have been initiated in the region of Finland, where 59 Saharan dust storm events were identified between 1980 and 2022. Note that we also found 22 dust storm events from the Aral-Caspian region and 5 episodes with Middle Eastern sources.
The research was supported by the NRDI projects FK138692 and RRF-2.3.1-21-2021.

How to cite: Varga, G., Rostási, Á., Csávics, A., Dagsson-Waldhauserova, P., Meinander, O., and Gresina, F.: Meridional Saharan dust transport towards higher latitudes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8920, https://doi.org/10.5194/egusphere-egu23-8920, 2023.

EGU23-9330 | ECS | Posters on site | ITS2.6/AS4 .5

Glacier darkening quantified from airborne imaging spectroscopy, Place Glacier, British Columbia, Canada 

Christopher Donahue, Brian Menounos, Nick Viner, Steven Beffort, Santiago Gonzalez Arriola, Rob White, and Derek Heathfield

Seasonal to long-term changes in albedo, or glacier darkening, is a critical parameter for energy and mass balance models. Yet many of these models employ simple parameterization schemes that darken snow and ice surfaces non-linearly through time. This simplification is not representative of the complex controls on albedo that vary spatially and temporally, driven by atmospheric processes, surface-atmosphere interaction, topography, and timing of glacier ice exposure. Albedo also spectrally varies, controlled by concentrations of light absorbing constituents (LACs) in the visible wavelengths and grain size in the near infrared wavelengths. Radiative forcing by LACs can enhance grain growth, leading to more rapid glacier darkening over the full solar spectrum. This process can accelerate as snow and ice melts because LACs tend to accumulate at the surface which can lead to increased radiative forcing over time for some glaciers. As temperatures warm, and aerosols increase due to land use change, drought, fire, and urbanization, it is likely that glacier darkening will intensify. To better quantify seasonal rates of darkening, and understand controls on intra- and interannual variability, we collected and analyzed a rich dataset obtained from imaging spectroscopy and lidar collected over Place Glacier in the Coast Mountains of British Columbia, Canada. Over the years 2021-2022, we acquired monthly data during the period of snow and glacier melt (March to October for 2021 and July to October 2022) using an aircraft with dedicated lidar (Riegl-780) and hyperspectral (Specim-Fenix; 451 bands) sensors. We processed these monthly acquisitions into 1-m, analysis-ready products. We describe our workflow for these products including development of snow and ice surface property retrievals in complex mountainous terrain. Our workflow yields retrievals that include broadband albedo, radiative forcing by LACs, and grain size. Radiative forcing from LACs can originate from abiotic and biotic sources, and we use the Modern-Era Retrospective Analysis for Research and Applications, Version 2 (MERRA-2) to interpret our retrievals with respect to contributions from dust and black carbon. We also highlight how these data can be used to understand seasonal glacier darkening events that occurred during a heat dome, snow algae blooms, and a late start to accumulation season. All these events are expected to increase in frequency or intensity due to climate change and hence, a better understanding of these physical processes will lead to improved physical models for future glacier evolution.

How to cite: Donahue, C., Menounos, B., Viner, N., Beffort, S., Gonzalez Arriola, S., White, R., and Heathfield, D.: Glacier darkening quantified from airborne imaging spectroscopy, Place Glacier, British Columbia, Canada, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9330, https://doi.org/10.5194/egusphere-egu23-9330, 2023.

EGU23-16143 | ECS | Posters on site | ITS2.6/AS4 .5

Multi-scale remote sensing and modeling for estimating liquid water content and LAPs on snow in the European Alps 

Claudia Ravasio, Roberto Garzonio, Biagio Di Mauro, and Roberto Colombo

The spectral reflectance of snow and ice varies widely depending on several quantities related (1) to the local environmental variables, such as the solar zenith angle and the surface slope, (2) to the physical properties of the snow, such as the grain size and the snow liquid content, and (3) to the presence of light-absorbing particles (LAPs).  Different absorption features are displayed in snow spectra. In particular, the absorption at 1030 nm has been exploited for estimating the grain effective radius of snow both from remote and proximal sensing data (Dozier et al., 2009, Garzonio et al., 2018). This absorption feature has been also used for the retrieval of the liquid water content (LWC) of surface snow since it is characterized by a shift toward shorter wavelengths when LWC increases (Green et al., 2006). Taking benefit of this spectral shift of the absorption feature, we applied a continuum removal approach to obtain both the grain equivalent radius and the LWC value. Furthermore, the accumulation of LAPs, such as dust, black carbon, volcanic ash, and pigmented snow algae on the snowpack albedo increases the absorption of solar radiation and induces a positive surface radiative forcing, enhancing the surface melting.

In this contribution, we show a retrieval algorithm to estimate the variables of snow (i.e., snow grain size, snow water equivalent, LAPs concentration) by using the openly available radiative transfer model BioSnicar (Bio-optical Snow, Ice, and Aerosol Radiative model) to simulate the spectral albedo of snow and the absorption of solar light in the snowpack. We present data from two experimental sites located in the Eastern Alps (Stelvio Pass and Brenta Dolomites) collected using a Spectral Evolution spectroradiometer. Measured variables of snow with a Snow Sensor device were compared with those estimated from BioSnicar simulations. Moreover, the impurities content in snow samples collected will be analyzed in a laboratory to better constrain modeling results. Remote sensing is a fundamental tool for characterizing snow cover properties, from the accumulation of LAPs to the wet/dry state of the snow, and the use of satellite sensors (e.g. PRISMA) opens the possibility for monitoring their spatial and temporal variability. This may have an important impact on snow hydrology studies, mainly for monitoring snow melting and improving the management of freshwater resources in the Alpine environment.

How to cite: Ravasio, C., Garzonio, R., Di Mauro, B., and Colombo, R.: Multi-scale remote sensing and modeling for estimating liquid water content and LAPs on snow in the European Alps, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16143, https://doi.org/10.5194/egusphere-egu23-16143, 2023.

EGU23-17351 | ECS | Posters on site | ITS2.6/AS4 .5

Stable Pb isotope signals in the Arctic: does the general background exist? 

Blanca Astray, Vladislav Chrastný, and Adela Šípková

The crucial historical milestone, phasing out leaded gasoline, has rapidly affected atmospheric Pb's concentration and isotope composition. Distant Arctic localities, often without significant industrial contamination sources, can be influenced by foreign transport. For instance, Greenland is affected by Eurasian and Canadian sources in spring and summer, and North American sources in autumn and winter.

Using snow samples, we chose three Arctic/Subarctic localities of Svalbard, Greenland, and Iceland to study the Pb stable isotope signals from the atmosphere. To learn more about possible sources of Pb pollution, we also processed local rock and fuel samples.

We filtrated the melted snow to analyze the solid snow particles and the dissolved Pb pool in the snow. The Pb isotope composition in the solid particles was more related to the rock samples in Iceland and Greenland. Signals from rock samples in Greenland are less radiogenic than those we found in Icelandic rocks. In Svalbard, the solid particles are enriched with coal content which is still mined at this locality. In filtrates, the signals from fuel (gasoline/diesel) Pb are present, which indicates that the local sources of car and snowmobile traffic are a significant source of Pb in this area. In Greenland, we also found extremely radiogenic signals in filtrate snow samples. The origin of this source would be more likely related to distant sources by transboundary pollution transfer.  

From our data, we conclude that several local and distant sources of Pb exist in pristine Arctic and Subarctic localities. Fuel seems to be the predominant source in Nuuk, while other sources, such as coal, are significant in Iceland and Svalbard, even in areas of higher local traffic.

How to cite: Astray, B., Chrastný, V., and Šípková, A.: Stable Pb isotope signals in the Arctic: does the general background exist?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17351, https://doi.org/10.5194/egusphere-egu23-17351, 2023.

EGU23-17546 | ECS | Posters on site | ITS2.6/AS4 .5

Local dust plume analysis and classification using ground-based remote sensing and microphysical measurement acquired at Lhù’ààn Mân’ (Kluane Lake), Yukon 

Seyedali Sayedain, Norman T. O’Neill, James King, Patrick L. Hayes, Daniel Bellamy, Richard Washington, Sebastian Engelstaedter, Andy Vicente-Luis, Jill Bachelder, and Malo Bernhard

The sub-Arctic Lhù’ààn Mân’ (Kluane Lake) region in the Canadian Yukon is subject to regular drainage wind-induced dust plumes emanating from the Slims River basin. This dust emissions site is just one of many current and potential future proglacial dust sources in the Canadian North. We employed ground-based passive and active remote sensing (RS) techniques to analyze the complementarity and redundancy of such RS retrievals relative to springtime (May 2019) Kluane Lake microphysical measurements. This included correlation analyses between ground-based coarse mode (CM) aerosol optical depth (AOD) retrievals from AERONET AOD spectra, CM AODs derived from co-located Doppler lidar profiles and OPS (Optical Particle Sizer) surface measurements of CM particle-volume concentration ( ). An automated dust classification scheme tied to intercorrelations between lidar-derived CM AOD, AERONET-derived CM AODs and  variations was developed to objectively identify local dust events. Lidar ratios derived from a priori refractive indices and OPS-derived effective radius statistics were also validated using AERONET-derived CM AODs. Bi-modal CM PSDs from AERONET inversions showed CM peaks at ~ 1.3 µm and 5 – 6.6 µm radius: we argued that this was associated with springtime Asian dust and Lhù’ààn Mân’ dust, respectively. Correlations between the CIMEL-derived fine-mode (FM) AOD and FM OPS-derived particle-volume concentration suggest that remote sensing techniques can be employed to monitor FM dust (which is arguably a better indicator of the long-distance transport of HLD).

How to cite: Sayedain, S., O’Neill, N. T., King, J., Hayes, P. L., Bellamy, D., Washington, R., Engelstaedter, S., Vicente-Luis, A., Bachelder, J., and Bernhard, M.: Local dust plume analysis and classification using ground-based remote sensing and microphysical measurement acquired at Lhù’ààn Mân’ (Kluane Lake), Yukon, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17546, https://doi.org/10.5194/egusphere-egu23-17546, 2023.

EGU23-3472 | Posters on site | AS4 .6 | Highlight

Evidence for Large Increases in Clear-Air Turbulence over the Past Four Decades 

Paul D. Williams, Mark C. Prosser, Graeme J. Marlton, and R. Giles Harrison

Clear-air turbulence (CAT) is hazardous to aircraft and is projected to intensify in response to future climate change. However, our understanding of past CAT trends is currently limited, being derived largely from outdated reanalysis data. Here we analyse CAT trends globally during 1979–2020 in a modern reanalysis dataset using 21 diagnostics. We find clear evidence of large increases around the globe at aircraft cruising altitudes. For example, at an average point over the North Atlantic, the total annual duration of light-or-greater CAT increased by 17% from 466.5 hours in 1979 to 546.8 hours in 2020, with even larger relative changes for moderate-or greater CAT (increasing by 37% from 70.0 hours to 96.1 hours) and severe-or-greater CAT (increasing by 55% from 17.7 hours to 27.4 hours). Our study represents the best evidence yet that CAT has increased over the past four decades.

How to cite: Williams, P. D., Prosser, M. C., Marlton, G. J., and Harrison, R. G.: Evidence for Large Increases in Clear-Air Turbulence over the Past Four Decades, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3472, https://doi.org/10.5194/egusphere-egu23-3472, 2023.

Recent studies showed that the modified YSU scheme, which added a fog top-down diffusion mechanism (ysu_topdown_pblmix), facilitated the bottom lifting of valley fog and sea fog by taking into account the “top-down” turbulent mixing and entrainment enhancement due to radiative cooling at the fog top, thus eliminating false fog areas. The applicability of this scheme to fog processes over the North China Plain is of interest. In this paper, we compared and analyzed the simulated effects of the modified YSU scheme on three fog events over the North China Plain with conventional ground-based data, 15-layer gradient and 5-layer eddy-related observations from atmospheric boundary tower. It was found that, unlike the results of existing studies, considering the fog-top turbulent diffusion mechanism resulted in lower TS scores for the fog area in the North China Plain, especially for the deep fog processes. A specific analysis of the simulated performance of a frontal fog on 17-20 December, 2016 showed that although the modified YSU scheme improved the simulation of nighttime near-surface temperature, humidity and vertical development of the fog layer, the simulated fog-top turbulence was too strong compared with the actual observations, resulting in a shorter fog duration and a significantly reduced fog area. By adjusting the parameter to reduce the intensity of the fog top turbulence entrainment, this operation can effectively reduce the under-reporting of the fog area and improve the simulation of fog over the North China Plain.

How to cite: Tian, M. and Wu, B.: The Evaluation of Modified YSU Scheme and Parameter Adjustment on the Simulation of Fog over the North China Plain, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4263, https://doi.org/10.5194/egusphere-egu23-4263, 2023.

EGU23-8632 | Posters on site | AS4 .6

Improving Nowcasts and Forecasts via Operational Use of Meteomatics Meteodrones 

Brad Guay, Martin Fengler, and Lukas Hammerschmidt

The Meteomatics Meteodrone is a small Unmanned Aircraft System (UAS) designed to collect high-resolution vertical profiles of atmospheric parameters such as temperature, humidity, wind speed and direction, and barometric pressure. Since its founding in 2012, Meteomatics has undertaken an iterative development of the Meteodrone technology, with regular releases of incremental enhancements. The newest model, the MM-670, features major improvements to measurement accuracy, flight capabilities and reliability, and safety and regulatory compliance, making it suitable for routine operational and research use.

In 2023, Meteomatics is continuing to install a network of 15 Meteodrones around Switzerland and has initiated a pilot weather forecasting project at one site in North Dakota, USA in collaboration with its partners Grand Sky and TruWeather Solutions. In both cases, Meteodrones are launched remotely from semi-automated Meteobase drone-in-a-box systems and routinely flown to collect profiles to a maximum of approximately 6,000 metres AMSL.

The data collected by the Meteodrones can fill gaps in the existing weather observation network, especially in the boundary layer regions where extreme weather events occur. This data is used for nowcasting purposes and to improve the accuracy of Meteomatics-developed 1 km-resolution Weather and Research Forecasting (WRF) models. In this presentation, we will share learnings from our research that has enabled the transition to operational use of Meteodrones, including how the technology has evolved and specific issues have been investigated and addressed.  In addition, future applications of this new technology, including improvements to nowcasts and forecasts, will be be discussed and evaluated.

How to cite: Guay, B., Fengler, M., and Hammerschmidt, L.: Improving Nowcasts and Forecasts via Operational Use of Meteomatics Meteodrones, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8632, https://doi.org/10.5194/egusphere-egu23-8632, 2023.

EGU23-9169 | ECS | Posters on site | AS4 .6

Weather patterns characterizing eco-efficient aircraft trajectories 

Federica Castino, Feijia Yin, Volker Grewe, Hiroshi Yamashita, and Sigrun Matthes

Aviation emissions perturb the atmosphere through CO2 and non-CO2 effects, which include, for instance, the radiative effects of contrail cirrus, H2O emissions, and NOx induced changes on atmospheric ozone and methane concentrations. The life-time of these non-CO2 perturbations is in the order of hours to days or weeks, and thus the resulting climate impact is highly dependent on the background atmospheric conditions, which vary with time, location, and altitude of emission. Mitigation strategies to reduce aviation climate impact could exploit this dependency on weather conditions, e.g., optimizing aircraft trajectories to minimize their climate impact. In particular, previous research shows the potential of “eco-efficient” trajectories, which lead to significant climate impact reductions at limited cost increases [1]. However, a strategy to identify days with a high mitigation potential is currently missing. For this purpose, we investigate in our study the correlation between days characterized by the identification of anomalously high numbers of eco-efficient trajectories, and the atmospheric conditions simulated on those days, e.g., considering the strength and location of the jet stream.

We use the ECHAM/MESSy Atmospheric Chemistry (EMAC) model, a numerical chemistry and climate simulation system that includes sub-models describing tropospheric and middle atmosphere processes and their interaction with oceans, land and human influences [2]. Our simulations include the submodels ACCF [3], using prototype algorithmic Climate Change Functions (aCCFs) to estimate the climate effects of aviation emissions, and AIRTRAF [4], optimizing aircraft trajectories under the atmospheric conditions simulated by EMAC. The total Average Temperature Response in 20 years (ATR20) of NOx, contrails, CO2, and H2O from each flight is computed using the aCCFs [5]. We conduct 1-year simulations optimizing 100 European flights per day. Our results show that 20% of the flights are responsible for about 70% of the total climate impact reduction, and that these flights are not homogeneously distributed over the simulated days: a strong daily variability is found, due to the aCCFs gradients variability under different atmospheric conditions.

Acknowledgment: FlyATM4E has received funding from the SESAR Joint Undertaking under grant agreements No. 891317 under European Union's Horizon 2020 research and innovation program. ClimOp has received funding from European Union’s Horizon 2020 Research and Innovation Programme under Grant Agreement No. 875503.

[1] Matthes, S., et al.: Climate-optimized trajectories and robust mitigation potential: Flying atm4e, Aerospace, 7, 1–15, https://doi.org/10.3390/aerospace7110156, 2020.

[2] Jöckel, P., et al.: Development cycle 2 of the Modular Earth Submodel System (MESSy2), Geoscientific Model Development, 3, 717–752, https://doi.org/10.5194/gmd-3-717-2010, 2010.

[3] Yin, F., et al.: Predicting the climate impact of aviation for en-route emissions: The algorithmic climate change function submodel ACCF 1.0 of EMAC 2.53, Geosci. Model Dev. Discuss. [preprint], https://doi.org/10.5194/gmd-2022-220, in review, 2022.

[4] Yamashita, H., et al.: Newly developed aircraft routing options for air traffic simulation in the chemistry–climate model EMAC 2.53: AirTraf 2.0, Geoscientific Model Development, 13, 4869–4890, https://doi.org/10.5194/gmd-13-4869-2020, 2020.

[5] Dietmüller, S., et al.: A python library for computing individual and merged non-CO2 algorithmic climate change functions: CLIMaCCF V1.0, Geosci. Model Dev. Discuss. [preprint], https://doi.org/10.5194/gmd-2022-203, in review, 2022.

How to cite: Castino, F., Yin, F., Grewe, V., Yamashita, H., and Matthes, S.: Weather patterns characterizing eco-efficient aircraft trajectories, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9169, https://doi.org/10.5194/egusphere-egu23-9169, 2023.

EGU23-10484 | Posters virtual | AS4 .6

Profiling of Shallow Marine Fog using a UAV and Remote Sensing Observations over the Sable Island during FATIMA 

Ismail Gultepe, Joe H. Fernando, Eric Pardyjak, Qing Wang, Sebastian Hoch, Alexei Perelet, Ruiz-Plancarte Jesus, and Clive Dorman

The objective of this study is to investigate the vertical profiles of shallow fog events that occurred during the FATIMA (Fog and turbulence in the marine atmosphere) field campaign. The project took place over Sable Island and the surrounding ocean during July 2022. The profiles of meteorological and physical parameters were collected by instruments on 1) an Aeryon UAV (Unmanned Aerial Vehicle), 2) a TBS (Tethered Balloon System), 3) a MWR (microwave radiometer), 4) meteorological towers, and 5) radiosonde balloons released approximately every 3 hrs. Atmospheric profiles of temperature (T), relative humidity with respect to water (RHw), horizontal wind speed (Uh), as well as particle counts from the OPC-N3 (23 bins from 0.3 μm to 40 μm) when RHw~100%, and the fog vertical microphysics structure using in-situ observations are evaluated. Various parameters such as liquid water content (LWC), droplet number concentration (Nd), mean volume diameter (MVD), and aerosol number concentration (Na) are analyzed to elicit issues related to measurements. Based on the profiles of visibility (Vis), droplet size spectra, and meteorological parameters such as RHw, T, and Uh from the UAV and turbulence towers, we will be able to investigate the vertical variability for several shallow marine fog events.

In this presentation, issues related to atmospheric boundary layer profiling and vertical mixing processes will be investigated using in-situ observations from the profiling platforms, as well as a well instrumented UAV. Results will be discussed by emphasizing the future sensor developments and investigating the microphysical parameterizations.

This work was funded by the Grant N00014-21-1-2296 (Fatima Multidisciplinary University Research Initiative) of the Office of Naval Research, administered by the Marine Meteorology and Space Program.

How to cite: Gultepe, I., Fernando, J. H., Pardyjak, E., Wang, Q., Hoch, S., Perelet, A., Jesus, R.-P., and Dorman, C.: Profiling of Shallow Marine Fog using a UAV and Remote Sensing Observations over the Sable Island during FATIMA, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10484, https://doi.org/10.5194/egusphere-egu23-10484, 2023.

EGU23-11108 | ECS | Posters virtual | AS4 .6

Droplet Growth and Its Impact on Visibility During Freezing Fog Events from CFACT 

Onur Durmus, Ismail Gultepe, Zhaoxia Pu, Sebastian Hoch, Eric Pardyjak, Anna Gannet Hallar, and Alexi Perelet

Freezing fog is a type of cold fog that forms when the air temperature (Ta) is below 0℃. Although Ta is below 0℃, the water droplets can remain in a liquid state rather than freezing. Freezing-fog conditions can pose a significant hazard to aviation and marine operations because it can reduce visibility severely, and ice accumulates rapidly on the surfaces such as aircraft, ship, and roads. Observations collected during the CFACT (Cold Fog Amongst Complex Terrain) Project from 7 January – 24 February, representing cold-fog events over Heber Valley of Utah, are used in the analysis. The objectives of this study are to characterize freezing fog microstructure in detail with respect to droplet size distribution, critical diameter related to activation, and visibility. In the analysis, freezing fog (FZFG) and droplet size spectra will be examined theoretically and experimentally. The droplet activation and critical diameter forming in frozen-fog droplets will be revealed using the Köhler curve. The effect of the droplet-growth process on visibility changes for two cold-fog cases is examined and results are discussed. Preliminary analysis suggests that freezing-fog droplet growth strongly depends on environmental conditions, including Ta, relative humidity (RH), and liquid water content (LWC) as well as droplet number concentration (Nd). It is concluded that microphysical parameterizations should investigate freezing-fog droplet formation and growth in more detail because presently it is lacking in NWP predictions. 

How to cite: Durmus, O., Gultepe, I., Pu, Z., Hoch, S., Pardyjak, E., Hallar, A. G., and Perelet, A.: Droplet Growth and Its Impact on Visibility During Freezing Fog Events from CFACT, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11108, https://doi.org/10.5194/egusphere-egu23-11108, 2023.

Based on mesoscale automatic weather stations, NCEP FNL reanalysis data and satellite retrivaled fog from 2015 to 2020, the distinction of the land fog and sea fog over the Bohai coastal zone were analyzed. It shows although Bohai coastal fog often occur, they frequently divided into land fog or sea fog by western coastline. In order to explore the causing of this phenomenon, the Bohai coastal fog were selected as the research object in this work. Four types of fog events were taken into account according the following situations, (1) only land fog, (2) Land fog drifting to over marine areas, (3) only Sea fog, (4) Sea fog drifting to over inlands.

According to the statistics of the above four fog types, the characteristics and diurnal variation difference of fog show that, although the sea fog and land fog have the same inter-monthly distribution trend and all the most in winter, the difference was still significant. Land fog was more than sea fog in the autumn and winter, while on the contrary in the spring and summer. The event of sea fog and land fog clearly separated by the western coastline mostly occurs in the spring and winter night and lasted less than 12 h.

In order to further understand the reason that the coastal fog do or not cross the coastline, Firstly, we compared the two land fog events. One land fog occurred while not crossing the coastline, the other spread to the sea. The results show that, under the condition of a weaker weather systematic low-level circulation, the sea-land breeze thermal circulation humidify the inland air, which is favorable to land fog formation. The eastward inland fog moving into the marine area and dissipate due to the higher sea temperature. The stronger offshore wind is favorable for land fog drifting to the sea, and the fog over the sea can develop with the lower sea temperature. The sensitivity simulation experiment using WRF further made sure, when the SST increased by 5%, as the sea-land breeze strengthened, the fog area that is slightly offshore in the control experiment would retreat to the west of the coastline, and the land fog also showed more dense; while when the SST decreased by 5%, the sea-land wind is suppressed, resulting in the fog cases that originally stopped at the west coastline will spread and cover the Bohai area and maintain for a long time.

Secondly, by comparing the two marine fog events, which did or not diffuse westerly across the coastline, the results explore that, under the condition of obvious weather systematic low-level circulation, sea wind is favorable for sea fog diffusing to inland. Without systematic low-level circulation transportation, intensity of thermal differences between sea and land and suitable land temperature will determine whether sea fog can cross the western coastline. In conclusion, the thermal differences and its intensity between sea and land jointly to the favorable systematic low-level atmospheric circulation determine the finely location of fog in the coastal zone area.

How to cite: Wu, B.: Effect of both sea-land thermal difference and low-level circulation on finely location of Bohai coastal fog, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14627, https://doi.org/10.5194/egusphere-egu23-14627, 2023.

EGU23-15969 | Posters on site | AS4 .6 | Highlight

How much Desert Dust do Aircraft Engines Ingest at Major Airports? 

Claire Ryder, Clement Bezier, Helen Dacre, Rory Clarkson, Eleni Marinou, Manolis Proestakis, Vassilis Amiridis, Mark Vaughan, Zak Kipling, Angela Benedetti, and Mark Parrington

Mineral dust is the most abundant aerosol in the atmosphere and in particular regions exists in high concentrations. Ingestion of dust by aircraft engines can result in erosion, corrosion or a build-up of deposits damaging internal components. A move towards more efficient engines over recent years restricts capacity to tolerate detrimental impacts in engines. Air traffic in arid areas such as the Middle East has also increased dust exposure. However, it is not currently known how much dust is ingested by aircraft during take-off and landing. In order to quantify this, the vertical profile of dust is required. Here we present a climatology of vertical profiles of dust from the ECMWF Copernicus Atmospheric Monitoring System (CAMS) reanalysis at 10 major global airports, as well as their seasonal and diurnal variability, between 2003-2020. We evaluate the CAMS dust profiles against spaceborne lidar retrievals of dust from the Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) instrument aboard the CALIPSO satellite using both the standard NASA Level 3 product and the LIdar climatology of Vertical Aerosol Structure (LIVAS) product. Finally, using expected aircraft ascent and descent rates and associated mass flow into an engine, dust dose is calculated for take-off, climb, descent, hold, approach, land and taxi phases, as well as for the entire ascent/descent at different airports, using both CAMS and CALIOP datasets.

We show that vertical distribution of dust varies significantly between airports and across seasons, which has a large impact on the total engine dust ingestion. Diurnal dust variations at some airports such as Dubai are extremely large, with night time surface concentrations reduced by over 20%.  Vertical profiles from CAMS show considerable differences to the standard CALIOP L3 retrievals, though agreement with LIVAS profiles is much better. Aircraft engine dose is found to be highest for Delhi (where dose exceeds 7g for a single descent in summer), Niamey and Dubai. During ascent, ingestion is largest during the take-off phase of flight, such that airports with large concentrations of lower altitude dust incur higher doses. During descent, dose is strongly dependent of the altitude of holding pattern relative to the altitude of maximum dust concentration, such that Delhi and Dubai incur the largest dust dose. Therefore, it is recommended that measures to reduce dust ingestion are airport-specific, and could include practices such as night time take-off and adjustment of holding pattern altitude.

How to cite: Ryder, C., Bezier, C., Dacre, H., Clarkson, R., Marinou, E., Proestakis, M., Amiridis, V., Vaughan, M., Kipling, Z., Benedetti, A., and Parrington, M.: How much Desert Dust do Aircraft Engines Ingest at Major Airports?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15969, https://doi.org/10.5194/egusphere-egu23-15969, 2023.

EGU23-16062 | ECS | Posters on site | AS4 .6

Investigation of mid-latitude contrail formation regions in EMAC in comparison to in-situ observations from aircrafts 

Patrick Peter, Sigrun Matthes, Christine Frömming, and Volker Grewe

Aviation has long been associated with environmental problems such as pollution, noise and climate change. While CO2 emissions are at the forefront of public debate, non-CO2 emissions from aviation can have similar impacts on climate as carbon dioxide from aviation, such as contrails, nitrogen oxides, or cloud cover caused by aviation. Previous studies investigated the influence of different weather situations on the climate impact of aviation, identified climate-sensitive regions, and created data products such as 4-dimensional climate change functions (CCFs) that enable air traffic management (ATM) to plan for climate optimized trajectories. However, the applicability and potential implementation of climate change functions for climate-optimized flight planning is only possible if the CCFs and the corresponding mitigation potential are validated [1,2].

The research presented here is part of the European Horizon 2020 project ClimOP and focuses on a further validation of the modular global chemistry climate model EMAC to analyze whether the model is able to represent real-world situations. For the comparison, we focus on contrail parameter as contrails have the largest uncertainties among all CCFs [2,3]. To investigate which vertical resolution in EMAC is suitable to study key atmospheric parameters for contrail formation, we compared different model setups. Furthermore, results from nudged simulation are compared with measurement data from the DLR ML-CIRRUS campaign.

The study shows a systematic cold and dry/wet bias between EMAC and aircraft measurements that differs with a nudging approach. These variations have implications for relative humidity, ice supersaturated regions, and potential contrail coverage in the model and must also be considered when using CCFs. Thus, this study represents a first step toward the applicability and potential implementation of climate change functions for climate-optimized flight planning.

The project leading to this study has received funding from the European Union’s Horizon 2020 research and innovation programme under grant agreement No 875503 (ClimOP). High performance supercomputing resources were used from the German CARA Cluster in Dresden.

References:
[1] Matthes S. et al., Aerospace 7, 156 (2020).
[2] Frömming C. et al. Atmos. Chem. Phys., 21, 9151–9172 (2021).
[3] Peter P. et al. (2021) EASN Conference Sep 2021 (2021).

How to cite: Peter, P., Matthes, S., Frömming, C., and Grewe, V.: Investigation of mid-latitude contrail formation regions in EMAC in comparison to in-situ observations from aircrafts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16062, https://doi.org/10.5194/egusphere-egu23-16062, 2023.

EGU23-17054 | Posters on site | AS4 .6

Fog formation, causes and types over the Abu Dhabi International Airport, United Arab Emirates 

Alreem Almaskari, Yasmeen Alrashdi, Salama Alshehhi, and Seyda Tilev

Fog is a meteorological event which has a significant impact on many human activities such as transportation, civil aviation, and military operations. UAE experiences many dense fog episodes over the course of a year which effect the visibility conditions strongly, especially during the winter months. In this research, we studied the fog events over Abu Dhabi International Airport, which is located at the northeastern coast of UAE, using METAR (2012 to 2022) and ERA5 data. The number of fog days per year, the seasonal cycle, the diurnal cycle, and the duration of fog events were analyzed. Fog events are most frequent between September to March with a peak during December and January.  Statistics of the fog events and the related atmospheric variables such as temperature, relative humidity, wind speed and direction during the fog episodes will be presented. Additional case studies that were conducted to understand and explain the reasons and types of the fog events over the region will also be displayed.

How to cite: Almaskari, A., Alrashdi, Y., Alshehhi, S., and Tilev, S.: Fog formation, causes and types over the Abu Dhabi International Airport, United Arab Emirates, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17054, https://doi.org/10.5194/egusphere-egu23-17054, 2023.

EGU23-17403 | Posters virtual | AS4 .6

Fog and low-level stratus characteristics at the airport of Lviv from surface observations 

Inna Khomenko and Oleksii Hustenko

Fog and low-level stratus have been recognised as a hazardous weather phenomenon leading to several losses in time, money and even human life above all in aviation but also in other forms of transportation, such as navigation and land transportation. The forecast of low-level stratus and fog is one of the most difficult issues of aviation meteorology due to spatial and temporal variability of their characteristics and high dependence on local conditions. So, weather observations can be used for statistical dependencies of fog/low-level stratus characteristics on numerical model outputs.

To study fog and low-level stratus characteristics occurring at the airport of Lviv, Ukraine, three-hourly meteorological observations in the period of 2010-2020 are used. Applying a statistical approach annual, seasonal and diurnal distribution of fog and low stratus and their frequency distribution associated with various meteorological parameters are obtained.

It was shown that at the airport of Lviv low-level stratus more frequently (60% of all cases) forms in the November-December-January-February period, whereas in July and August it is least frequently observed (less than 5% of all cases). Distribution of the fog observations with respect to months also is inhomogeneous. Fog mainly forms from October to January (56% of all cases) with the maximum (19%) in November. From March to September fog happen rarely with minimum in June (3% of all cases). No distinct diurnal cycle of the low-level stratus occurrence can be revealed from the data, however low-level stratus more frequently occurs during the nighttime and in morning. As opposed to low-level stratus for fog the highest frequency is observed in the hours before sunrise, while when the day sets in, frequencies are declining and increasing at night.

Low-level stratus is the most commonly associated with surface temperatures of 0.0 to +8.0°С and relative humidity of 80 to 95% (32% of all cases), by comparison with 35% of all fog cases observed at temperatures of 0.0 to +6.0°С and relative humidity of 96 to 100%.

In all seasons of the year, the highest frequency of low-level stratus (from 35 to 40% of all cases) is in interval of 3...4 m/s, whereas fog is the most frequently observed in calm weather (from 37 to 77% of all cases). In autumn and winter, both under low-level stratus and fog, surface wind is characterized by high occurrence frequency of west, north-west (around 25% of low-level stratus cases and 10% of fog cases) and south, south-east (around 30% of all cases) directions. In spring and summer, north, north-west and west directions are most frequently reported in low-level stratus cases (47% of low-level stratus cases in spring and 69% in summer). For fog in spring and summer the same wind directions are typical (18% of fog cases in spring and 10% in summer). However, it should be noticed that in spring the east direction is often observed for both fog and low-level stratus.

 

How to cite: Khomenko, I. and Hustenko, O.: Fog and low-level stratus characteristics at the airport of Lviv from surface observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17403, https://doi.org/10.5194/egusphere-egu23-17403, 2023.

EGU23-17422 | Posters virtual | AS4 .6

Effectively Communicating Aviation Hazards through Modernized Web Products 

Austin Cross, Stephanie Avay, Robert Hepper, Dan Vietor, and Nicole Stevens

Effectively communicating hazardous weather conditions to the general aviation (GA) community is a
continuously evolving effort of US National Weather Service (NWS) Aviation Weather Center (AWC)
operations. AWC has started to transition text heavy products in favor of easily interpreted dynamic
graphics that provide additional information that was never fully realized through text alone.
AWC provides domestic and international aviation weather forecasts and warnings, disseminated
through traditional product dissemination as well as directly to end users through AviationWeather.gov.
The web site is currently undergoing a complete rewrite, in order to both modernize and improve
consistency. Customer feedback has been gathered over multiple years and the rewrite is intended to
address a number of issues in a comprehensive manner.
Many products that were previously available in multiple formats are now presented through a more
integrated framework, allowing for the user to combine different datasets as desired. The Graphical
Forecasts for Aviation (GFA), first developed as a replacement for the traditional text Area Forecast,
now spans a wide variety of weather information in a one stop Geographic Information Systems (GIS)
interactive web framework. The site is designed to adjust to available screen real estate, making the
same data and interface available on a variety of platforms from desktop computers to tablets and
phones.
The new site has been in an experimental status since spring of 2022, while AWC collects feedback on
the new design and performed a social science user assessment in partnership with the US Federal
Aviation Administration’s (FAA) Aviation Weather Demonstration and Evaluation service group. This
presentation will discuss the design and features of the new site, as well as lessons learned from the
aviation weather user community during the development and evaluation.

How to cite: Cross, A., Avay, S., Hepper, R., Vietor, D., and Stevens, N.: Effectively Communicating Aviation Hazards through Modernized Web Products, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17422, https://doi.org/10.5194/egusphere-egu23-17422, 2023.

EGU23-412 | ECS | Orals | BG1.2

Assessing changes in post-fire vegetation resilience in Mediterranean basin over the past 22 years 

Tiago Ermitão, Célia Gouveia, Ana Bastos, and Ana Russo

Fire is an integral component of ecological dynamics, playing an important role in biome distribution and biomass variability. Nonetheless, fires can also pose a  threat to both ecosystems and humans, by imposing severe economic and social consequences, and potentially contributing to biodiversity loss, carbon loss and soil erosion, whose effects can last from months to years.

The Mediterranean basin is a fire-prone region where vegetation is in general well adapted to fire, with several species showing resistance to fire itself or being able to recover quickly following fire events. However, as a consequence of climate change, more intense and frequent summer hot and dry conditions are expected to occur, which can promote more frequent and severe wildfires, with return periods potentially outpacing recovery times. Understanding recovery dynamics is therefore crucial to assess the impact of changing fire regimes in ecological dynamics and stability of ecosystems. 

In our study, we use the “Enhanced Vegetation Index” (EVI), remotely-sensed by MODIS sensor with a temporal span of 22 years, to evaluate vegetation dynamics before, during and following large fire seasons. We use a mono-parametric recovery model to assess recovery times in different burn scars across the Mediterranean basin, covering different fire regimes and land cover types. We find a tendency for slower recovery in areas that burned more often, which may indicate a decrease in ecosystems’ resilience in the past 22 years.

This study was performed under the frameworks of the 2021 FirEUrisk project (funded by European Union’s Horizon 2020 research and innovation programme under the Grant Agreement no. 101003890) and of the PhD MIT Portugal MPP2030-FCT programme (Grant no.22405886350).

How to cite: Ermitão, T., Gouveia, C., Bastos, A., and Russo, A.: Assessing changes in post-fire vegetation resilience in Mediterranean basin over the past 22 years, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-412, https://doi.org/10.5194/egusphere-egu23-412, 2023.

EGU23-1406 | ECS | Orals | BG1.2 | Highlight

Large-scale fire events substantially impact plant-soil water relations across ecosystem types 

Martin J. Baur, Andrew D. Friend, and Adam F. A. Pellegrini

Wildfire is a global scale ecosystem phenomenon with substantial impact on the carbon cycle, climate warming, and ecosystem resilience. Fire and the hydrological cycle are strongly interlinked, with water availability determining the amount and combustibility of fuel, and fire influencing infiltration, runoff rates and evapotranspiration. Consequently, understanding soil moisture (SM) and vegetation water content (VWC) dynamics pre- and post-fire is fundamental for predicting fire occurrence, fire severity, and ecosystem recovery. Fire can modulate SM and VWC dynamics by influencing interception of rainfall, soil porosity, plant water uptake, and runoff; however, much evidence for fire effects on the hydrological cycle is obtained at the field- to watershed-scale. Therefore, we ask the following research question: What are the effects of large-scale fire events on SM and VWC dynamics across biomes globally?

Here we use over six years of global SM, VWC and vapor pressure deficit (VPD) derived from different remote sensing datasets to investigate the effects of large-scale fires on SM and VWC dynamics. We apply a dry down framework, only analyzing consecutive observations of decreasing soil moisture, to describe post-fire response rates for SM, VWC and VPD relative to a pre-fire reference state.

We find large scale evidence that the post-fire rate of change of SM over time is more negative, indicating faster water loss. Vegetation recovery, indicated by a positive change in VWC over time, exceeds the pre-fire reference state, which suggests that post-fire recovery is predominantly faster than undisturbed seasonal vegetation growth, likely due to succession of fast-growing plant species. Furthermore, fire affects ecosystem hydrology on shorter timescales as well, reducing diurnal VWC variation over a wide range of SM and VWC conditions. Our findings confirm several trends previously only observed at smaller scales and suggest global remote sensing of SM and VWC can substantially contribute to understanding the dynamics of post-fire plant and soil water status.

How to cite: Baur, M. J., Friend, A. D., and Pellegrini, A. F. A.: Large-scale fire events substantially impact plant-soil water relations across ecosystem types, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1406, https://doi.org/10.5194/egusphere-egu23-1406, 2023.

EGU23-1412 | Posters on site | BG1.2

PyroCbs from Australia Fires and its Impact Study Using Satellite Observations from CrIS and TROPOMI and Reanalysis Data 

Xiaozhen Xiong, Xu Liu, Wan Wu, Liqiao Lei, Qiguang Yang, Daniel Zhou, and Allen Laura

Australia’s unprecedented fire disasters at the end of 2019 to early 2020 emitted huge amounts of carbon monoxide (CO) and fire aerosol particles to the atmosphere, particularly during the Pyrocumulonimbus (pyroCb) outbreak that occurred in southeast Australia between 29 December 2019 and 4 January 2020. It was estimated that at least 18 pyroCbs were generated during this episode, and some of them injected ice, smoke, and biomass burning gases above the local tropopause.  An unprecedented abundance of H2O and CO in the stratosphere, and the displacement of background ozone (O3) and N2O from rapid ascent of air from the troposphere and lower stratosphere were found from satellite observations. Some other studies also found that the fire emissions and their long-range transport resulted in stratospheric aerosol, temperature, and O3 anomalies after the 2020 Australian bushfires and altered the Antarctic ozone and vortex, posing great impact to local air qality and climate change.

            This study will focus on the thermodynamic state of atmosphere associated with these pyroCbs, and its impact on the change of the cloud properties and trace gases during this unprecedented Australia fires, mainly based on a new single Field of View (SFOV) Sounder Atmospheric Products (SiFSAP) and TROPOMI. SiFSAP was developed by NASA using the Cross-track Infrared Sounder (CrIS) and Advanced Technology Microwave Sounder (ATMS) onboard SNPP and JPSS-1, and will soon be available to the public at NASA DAAC. Since this product has a spatial resolution of 15 km at nadir, which is better than most global weather and climate models and other current operational sounding products, a process-oriented analysis of the dynamic transport of CO and fire plumes during this unprecedented fire disasters will be made in this study.  Based on a Principal Component Radiative Transfer Model (PCRTM) and an optimized estimation retrieval algorithm, a simultaneously retrieval is made using the whole spectral information measured by CrIS,  and the derived SiFSAP include temperature, water vapor, trace gases (such as O3, CO2, CO, CH4 and N2O), cloud properties and surface properties. Use of ATMS together with CrIS allows SiFSAP to get accurate retrieval products under thick pyroCb conditions. An algorithm to detect pyroCb based on the hyperspectral infrared sounder spectrum from CrIS will be developed and verified. In addition to SiFSAP sounding products,  CO, O3, NO2 from TROPOMI and O3 from OMPS will be used. The wind fields from the NASA’s Modern-Era Retrospective Analysis for Research and Applications Version-2 (MERRA-2) and ERA5 will be used to characterize the transport, and the SiFSAP temperature and water vapor profiles within and around pyroCbs will be compared with MERRA-2 and ERA5 products.     

How to cite: Xiong, X., Liu, X., Wu, W., Lei, L., Yang, Q., Zhou, D., and Laura, A.: PyroCbs from Australia Fires and its Impact Study Using Satellite Observations from CrIS and TROPOMI and Reanalysis Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1412, https://doi.org/10.5194/egusphere-egu23-1412, 2023.

EGU23-1975 | ECS | Orals | BG1.2

Drivers of spatial and temporal variability in savanna fire emission factors 

Roland Vernooij, Tom Eames, Jeremy Russel-Smith, Cameron Yates, Robin Beatty, Jay Evans, Andrew Edwards, Natasha Ribeiro, Martin wooster, Tercia Strydom, Marcos Giongo, Marco Borges, Carol Barradas, Maximo Menezes, Dave van Wees, and Guido van der Werf

Roughly half of global fire emissions originate from savannas, and emission factors (EF) are used to quantify the amount of trace gases and aerosols emitted per unit dry matter burned. It is well known that these EFs vary substantially even within a single biome but so far quantifying their dynamics has been hampered by a lack of EF measurements. Therefore, global emission inventories currently use a static averaged EF for the entire savanna biome. To increase the spatiotemporal coverage of EF measurements, we collected over 4500 EF bag measurements of CO2, CO, CH4 and N2O using an unmanned aerial system (UAS) and measured fuel parameters and fire severity proxies during 129 individual landscape fires. These measurements spanned various widespread savanna ecosystems in Africa, South America and Australia, with early and late dry season campaigns. We trained random forest (RF) regressors to estimate daily dynamic EFs for CO2, CO, CH4 and N2O at 500×500-meter resolution based on satellite and reanalysis data. The RF models reduced the difference between measured and modelled EFs by 60-85% compared to static biome averages. The introduction of EF dynamics resulted in a spatial redistribution of CO, CH4 and N2O emissions compared to the Global Fire Emissions Database version 4 (GFED4s) with higher emissions in higher rainfall savanna regions. While the impact from using dynamic EFs on the global annual emission estimates from savannas was relatively modest (+2% CO, -5% CH4 and -18% N2O), the impact on local EFs may exceed 60% under dry seasonal conditions.

How to cite: Vernooij, R., Eames, T., Russel-Smith, J., Yates, C., Beatty, R., Evans, J., Edwards, A., Ribeiro, N., wooster, M., Strydom, T., Giongo, M., Borges, M., Barradas, C., Menezes, M., van Wees, D., and van der Werf, G.: Drivers of spatial and temporal variability in savanna fire emission factors, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1975, https://doi.org/10.5194/egusphere-egu23-1975, 2023.

EGU23-2097 | Orals | BG1.2

Linked fire activity and climate whiplash in California during the early Holocene 

Jessica Oster, Julia Homann, Cameron de Wet, Sebastian Breitenbach, and Thorsten Hoffmann

Recent wildfire activity in semi-arid regions like western North America exceeds the range of historical records. High-resolution paleoclimate archives such as stalagmites could illuminate the link between hydroclimate, vegetation change, and fire activity in pre-anthropogenic climate states beyond the timescale of existing tree-ring records. Here we present an analysis of levoglucosan, a combustion-sensitive anhydrosugar, and lignin oxidation products (LOPs) in a stalagmite from White Moon Cave in the California Coast Range in order to reconstruct fire activity and vegetation composition across the 8.2 kyr event. Elevated levoglucosan concentrations suggest increased fire activity while altered LOP compositions indicate a shift toward more woody vegetation during the event, with the shift in vegetation preceding the increase in fire activity. These changes are concurrent with increased hydroclimate volatility as shown by carbon and calcium isotope proxies. Together, these records suggest that climate whiplash (oscillations between extreme wetness and aridity) and fire activity in California, both projected to increase with anthropogenic climate change, were tightly coupled during the early Holocene.

How to cite: Oster, J., Homann, J., de Wet, C., Breitenbach, S., and Hoffmann, T.: Linked fire activity and climate whiplash in California during the early Holocene, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2097, https://doi.org/10.5194/egusphere-egu23-2097, 2023.

EGU23-2233 | ECS | Orals | BG1.2

Fire impacts on soil carbon in a non-fire adapted alpine forest 

Melissa Torres, Caroline Poyntner, Sampriti Chaudhuri, Marc Pignitter, Hannes Schmidt, Thilo Hofmann, and Gabriel Sigmund

An increase in fire-prone conditions in non-fire adapted regions is rooted in climatic and anthropogenic changes. Such pyrogeographical shifts are observable, for example, in alpine regions. In 2021, Austria, experienced a fire larger than 100 ha for the first time in a century in the Schneeberg-Rax mountain region. In depth understanding of post-fire effects on carbon cycling at such non-fire adapted sites is still scarce. To help close this knowledge gap, post-fire changes were investigated at the abovementioned site, including soil organic matter composition and soil chemical conditions. 

Samples were taken immediately after the fire, 3 months, 6 months and 12 months thereafter from four sampling sites. Selected sites consisted of 1. a pine forest affected by a crown fire, 2. a pine and beech mixed forest affected by a surface fire, and two non-fire affected controls with similar site conditions (vegetation, slope, altitude, and exposition). Samples were analyzed for pH, carbon content, elemental composition, leachable dissolved organic carbon and trace elements, organic matter composition, and environmentally persistent free radical concentrations. 

pH increased after the fire at both sites investigated. This increase was the strongest (up to 1.5 units) immediately after the fire but was still substantial 1 year after the fire. Carbon contents decreased approximately 2fold in the crown fire affected soil compared to the control soil, but remained similar between surface fire affected soil and the respective control. However, aromaticity of bulk carbon and the leachable fraction increased in both fire-affected soils, which can be related to the formation of pyrogenic carbon during the fire. Pyrogenic carbon is a highly aromatic and recalcitrant carbon pool produced during incomplete combustion of biomass. Pyrogenic carbon can also contain substantial amounts of environmentally persistent free radicals (EPFR), which can form reactive oxygen species, which can induce oxidative stress on microbiota. Our EPFR measurements showed an increase by at least 1.5 orders of magnitude of EPFR in fire affected soils. This study suggests that changes in soil carbon cycling can be expected following fires in non-adapted alpine forests. 

How to cite: Torres, M., Poyntner, C., Chaudhuri, S., Pignitter, M., Schmidt, H., Hofmann, T., and Sigmund, G.: Fire impacts on soil carbon in a non-fire adapted alpine forest, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2233, https://doi.org/10.5194/egusphere-egu23-2233, 2023.

EGU23-2932 | Posters on site | BG1.2

Hydrological conceptual model for reconstructing fire history from cave stalagmites 

Pauline Treble, Campbell Micheline, Andy Baker, McDonough Liza, and Kosarac Nevena

Cave stalagmites (speleothems) are highly-valued archives of environmental information owing to their preservation of climate sensitive proxies and well-defined chronologies.  Yet the reconstruction of fire history from stalagmites is a relatively unexplored approach, with some advantages over traditional fire proxy archives.  For example, stalagmites may contain annual laminae (visible or chemical) which can be exploited for seasonal to annual proxy information with precise chronologies.  Thus stalagmites have the potential to yield annually-resolved records of fire and climate that could be used to (1) better understand the fire-climate relationship, (2) fire recurrence interval information, (3) understand ecosystem resilience and (4) inform land management policy.

The development of fire proxies from stalagmites is still in its infancy. Robust interpretations of any proxy information relies on an understanding of the environmental processes that lead to the preservation of proxies in the archive.  Cave stalagmites may record fire history via dripwater, or via the cave entrance as aerosols.  The focus here is on the transportable constituents in dripwater such as solutes, colloids and suspended matter.  A fire event produces ash (a source of leachates) and can alter soil properties (hydrophobicity, pH, organic matter etc) producing temporary enrichments (or depletions) in transported constituents via dripwater.  The resulting signal may be detected in stalagmites using high-resolution methods such as laser ablation mass spectrometry, fluorescence and infrared microscopy techniques.  Cave depth is an important factor in the preservation process with the detection of a fire signal more likely to be observed in dripwater from shallow caves (e.g. 5-10 m) owing to the potential for attenuation and mixing that may occur in deeper caves (Campbell et al., 2022).  However, owing to the karstification of carbonate rocks which host caves, there commonly exists different flow types: diffuse/slow flow through the matrix, preferential/fast flow through fractures and conduits.  Fracture (or conduit) influenced flowpaths have higher permeability and enhance rapid and deep percolation of water from the surface towards the cave.  Several studies have shown that stalagmites fed by dripwater with a fracture-flow component contain higher concentrations of soil-derived trace metals and organics indicating a stronger hydrological connection with the surface.  It logically follows that fracture-influenced flowpaths are more likely to transmit proxies for fire.  Furthermore, flowpaths may be a more important factor than cave depth in some settings, e.g., Campbell et al. (2022) presented a case study of a historical fire event recorded in a stalagmite that was located ~40 m below the surface.  

Understanding the hydrological setting of a cave system including rainfall recharge and flowpaths is valuable in the interpretation of speleothem records in general.  This contribution presents a conceptual model illustrating how these factors influence the preservation of fire proxies in stalagmites and makes recommendations for ideal sample selection for fire proxy records based on cave characteristics as well as stalagmite attributes such as morphology and colour.

Campbell. M. et al., Speleothems as Archives for Palaeofire Proxies. ESS Open Archive. July 24, 2022. DOI:10.1002/essoar.10511989.1

How to cite: Treble, P., Micheline, C., Baker, A., Liza, M., and Nevena, K.: Hydrological conceptual model for reconstructing fire history from cave stalagmites, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2932, https://doi.org/10.5194/egusphere-egu23-2932, 2023.

EGU23-3238 | ECS | Orals | BG1.2

Feeding the flames: how colonialism led to unprecedented wildfires across SE Australia 

Michela Mariani, Simon Connor, Michael-Shawn Fletcher, Simon Haberle, Janelle Stevenson, Peter Kershaw, Annika Herbert, Martin Theuerkauf, and David Bowman

The Black Summer bushfires (2019-2020) cost the Australian economy over 100 billion dollars and burnt a total of 18 million hectares. In just one season, around 20% of Australia's Eucalyptus forests burnt down and billions of animals perished. Recent catastrophic fires in Australia and North America have made scientists and policymakers question how the disruption of First Nations' burning practices has impacted fuel loads. For instance, we have learnt from modern Australian Indigenous communities, historical literature, and art works that Indigenous peoples have used cultural burning to rejuvenate patches of land and preserve open vegetation for hunting and cultural purposes. The advent of British invasion brought a change in the type of fire regimes and landscape management across much of the continent, which may have led to an increase in flammable fuels in forest settings. However, the actual degree of land-cover modification by early settlers has only been often debated in the academic literature and within management stakeholders.

The quantification of past land cover is needed to address such debates. Pollen is the key proxy to track past vegetation changes, but pollen spectra suffer from some important biases e.g. taphonomy, pollen productivity, dispersal capability. Estimating past vegetation cover from sedimentary pollen composition requires to correct for productivity and dispersal biases using empirical-based models of the pollen-vegetation relationship. Such models for quantitative vegetation reconstruction (e.g. REVEALS) have yet been mostly applied in the Northern Hemisphere in the last 15 years - here we present recent applications of this methodology from Australia. We show the quantification of land cover changes through pre- and post- British invasion on multiple records (n=51) across the southeastern Australian region. This represents the first regional application of REVEALS within the Australian continent.

We provide the first empirical evidence that the regional landscape before British invasion was a cultural landscape with limited tree cover as it was maintained by Indigenous Australians through cultural burning. Our findings suggest that the removal of Indigenous vegetation management has altered woodland fuel structure and that much of the region was predominantly open before colonial invasion. The post-colonial land modification has resonance in wildfire occurrence and management under the pressing challenges posed by climate change.

How to cite: Mariani, M., Connor, S., Fletcher, M.-S., Haberle, S., Stevenson, J., Kershaw, P., Herbert, A., Theuerkauf, M., and Bowman, D.: Feeding the flames: how colonialism led to unprecedented wildfires across SE Australia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3238, https://doi.org/10.5194/egusphere-egu23-3238, 2023.

EGU23-3310 | ECS | Orals | BG1.2

PEAT-FWI: Improving the Fire Weather Index for peatlands with Hydrological Modeling and L-band Microwave Observations 

Jonas Mortelmans, Anne Felsberg, Gabriëlle De Lannoy, Sander Veraverbeke, Robert Field, Niels Andela, and Michel Bechtold

The Fire Weather Index (FWI) is used worldwide to estimate the danger of wildfires. The FWI system integrates meteorological parameters and empirically combines them into several moisture codes, each representing a different fuel type. These moisture codes are then used in combination with wind speed to estimate a fire danger. Originally, the FWI system was developed for a standard jack pine forest, however, it is widely used by fire managers to assess the fire danger in different environments as well. Furthermore, it is often also used to assess the vulnerability of organic soils, such as peatlands, to ignition and depth of burn. The utility of which is often questioned.

 

This research aims at improving the original FWI for northern peatlands by replacing parts of the original, purely weather-based FWI system with satellite-informed model estimates of peat moisture and water level. These come from a data assimilation output combining the NASA catchment model, including the peat modules PEATCLSM, and Soil Moisture and Ocean Salinity (SMOS) L-band brightness temperature observations. The predictive power of the new, peat-specific FWI (PEAT-FWI) is evaluated against the original FWI against fire data of the global fire atlas from 2010 through 2018 over the major northern peatlands areas. For the evaluation, the fires are split up in early and late season fires, as it is hypothesized that late fires are more hydrological driven, and the predictive power of the PEAT-FWI will thus differ between the two types of fires. Our results indeed indicate that the PEAT-FWI improves the predictive capability of estimating fire risk over northern peatlands in particular for late fires. By using a receiver operating characteristics (ROC) curve to evaluate the predictive power of the FWI against a random estimate, the area under the curve increases by up to 10% for the PEAT-FWI compared to the original FWI. The recent version 7 release of the operational Soil Moisture Active Passive (SMAP) Level-4 Soil Moisture Data Assimilation Product now includes PEATCLSM, thus, the proposed PEAT-FWI is straightforward to include in operational FWI products.

How to cite: Mortelmans, J., Felsberg, A., De Lannoy, G., Veraverbeke, S., Field, R., Andela, N., and Bechtold, M.: PEAT-FWI: Improving the Fire Weather Index for peatlands with Hydrological Modeling and L-band Microwave Observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3310, https://doi.org/10.5194/egusphere-egu23-3310, 2023.

EGU23-3332 | ECS | Orals | BG1.2

How changes in ignition sources influence fire probability in the Amazon and Cerrado biomes: a perspective based on frontier age 

Andreia F. S. Ribeiro, Lucas Santos, Maria R. Uribe, Rafaella A. Silvestrini, Ludmila Rattis, Marcia N. Macedo, Douglas C. Morton, James T. Randerson, Sonia I. Seneviratne, Jakob Zscheischler, and Paulo M. Brando

Agricultural expansion and ongoing climate change are rapidly altering the fire regime of natural ecosystems along the Cerrado-Amazon biome boundary. While agricultural intensification has driven a decrease in fire ignitions in some regions, agricultural expansion has increased fire usage in other landscapes for deforestation and managing pasturelands. These contrasting patterns of fire activity across different land-use frontiers limits our ability to accurately predict where and when fires may occur, particularly under the context of climate change.

To predict fire activity with land-use transitions, we modelled fire probability as a function of the age of different land-use transitions across the Amazon and Cerrado. We investigated annual land-use and associated burned areas based on the MapBiomas Collection 6.0 and MapBiomas Fire Collection 1.0 data, respectively, from 1986 to 2020. This allowed us to quantify how the time-since conversion of native vegetation (forest, savanna, and grassland) to pasture and farming influence fire occurrence. Additionally, we explored the joint impact of land-use change and climate extremes in fire activity in terms of estimated vapor pressure deficit (VPD) and maximum cumulative water deficit (MCWD), two common measures of flammability and drought impact. 

Our results confirm that transition age is a strong predictor of fire probability. They also suggest that fire probability increases (decreases) at different rates before (after) clearing in Amazon and Cerrado. The role of climate extremes in modulating burning activity associated with land-use transitions varied by biome, post-fire land use, and the size of the burned area associated with the conversion. These findings provide insight into incorporating the effect of land-use transition age on ignition probability for fire modelling in combination with climate drivers. From an operational point of view, our results aim to contribute to environmental policies capable of sustaining ecosystem integrity at the ecotone between the Amazon and Cerrado biomes.

How to cite: Ribeiro, A. F. S., Santos, L., Uribe, M. R., Silvestrini, R. A., Rattis, L., Macedo, M. N., Morton, D. C., Randerson, J. T., Seneviratne, S. I., Zscheischler, J., and Brando, P. M.: How changes in ignition sources influence fire probability in the Amazon and Cerrado biomes: a perspective based on frontier age, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3332, https://doi.org/10.5194/egusphere-egu23-3332, 2023.

EGU23-3632 | ECS | Posters virtual | BG1.2

BPCA-derived PyC may reflect fire signals over regional scales from the western Amazon Basin fire record 

Jing Lyu, Andrew Zimmerman, Mark Bush, and Crystal McMichael

Fire alters the biogeochemical cycling of important elements, plays a role in climate change, and shapes the composition of global biological communities. Detection of past fires has long been used to reconstruct human settlement and climate records. Charcoal and phytolith abundance has been the most commonly used paleofire proxies but may only represent evidence of local fires. Chemical analyses of pyrogenic carbon (PyC) have been more recently used, but are also not without controversy. Thus far, very few intercomparisons of these proxies have been conducted. Here, the fire records contained in soil and lake sediments of Western Amazon (at lakes Ayauchi, Parker, Gentry, and surrounding regions) were determined by charcoal microscopy, chemical thermal oxidation (CTO), and benzene polycarboxylic acids (BPCA) molecular biomarkers. Charcoal represented a smaller portion of PyC and, with its patchy distribution, likely indicated local or larger regional fire events. With a median value of about 15% of organic carbon, PyC via CTO oxidation was of the highest concentrations, which suggests a larger PyC detection window and lower sensitivity of reflecting regional fire. With a median value of about 3% of organic carbon, the BPCA-derived PyC distributions bore the closest resemblance to both spatial and temporal regional fire variations, established via archeological, pollen and phytolith records, thus may be a more sensitive indicator of fire over larger regional scales. Molecular ratios of BPCA molecules in Lake Ayauchi soils indicated higher temperature fires (> 600°C) and suggested a history of more human occupation and human-caused fire in the Lake Ayauchi region compared with the Lake Gentry & Parker region. However, our findings suggest that the use of a combination of fire proxy methods provides a fuller picture of the fire history of a region than any single approach. Establishing a better understanding the differences in the information provided by various paleofire proxies will allow a more complete understanding of the drivers, history and ecological and biogeochemical effects of fire, both regionally and globally.

How to cite: Lyu, J., Zimmerman, A., Bush, M., and McMichael, C.: BPCA-derived PyC may reflect fire signals over regional scales from the western Amazon Basin fire record, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3632, https://doi.org/10.5194/egusphere-egu23-3632, 2023.

EGU23-3695 | ECS | Orals | BG1.2

Wildfires alter nitrifier communities and increase soil emissions of NOx but not N2O in California chaparral 

Elizah Stephens, Aral Greene, Alexander Krichels, and Peter Homyak

Background:

Fires burn roughly 3% of Earth’s land surface each year and are predicted to become more frequent and severe as human-caused climate change progresses. Fires can drive ecosystem N loss by volatilizing N bound in plant biomass to the atmosphere and by leaving behind ash rich in ammonium (NH4+) and organic N that can run off when it rains. While N volatilization and runoff account for a large fraction of N loss after fires, budget imbalances suggest soil emissions of nitric oxide (NO) and nitrous oxide (N2O) may also be significant N loss pathways after fire. Identifying sources of NO and N2O is important because NO is a precursor for tropospheric O3 which causes high rates of asthma hospitalizations,and N2O is a powerful greenhouse gas with 300× the warming potential of CO2. Soil emissions of NO and N2O are largely governed by the microbial processes of nitrification and denitrification. Under aerobic conditions typical of dry soils, nitrifying organisms such as ammonia-oxidizing bacteria (AOB) and ammonia-oxidizing archaea (AOA) oxidize NH4+ to nitrate (NO3-) and release NO and N2O as byproducts. AOA and AOB process N with different efficiencies, suggesting shifts in AOA:AOB ratios may change N emissions. Specifically, AOB are dominant in soils with high NH4+and pH and produce higher NO and N2O emissions. Since such soil conditions are frequently observed after fires, we hypothesize NO and N2O emissions will increase as AOB communities become dominant. To test this, we collected soil cores from 5 plots in the Sequoia National Park, CA over a time series starting two weeks after a high severity chaparral fire. We selectively inhibited AOA and AOB communities to measure their contributions to NO and N2O emissions. We also measured the isotopic composition of N2O emissions from these soils using an LGR isotopic N2O analyzer to better understand the processes responsible for post-fire N2O production.

Results/Conclusions

One month after the fire, soil bulk emissions of NO over 72hrs were 1.5 times higher in the burned plots (101.4 ± 22.4 µg N-NO/g soil burned; 67.1 ± 19.3 µg N-NO/g soil unburned; ±SE). Bulk soil emissions of N2O over 72hrs were 7.5 times lower in burned plots compared to before the fire (0.0616 ± 0.04 ng N-N2O/g soil burned; 0.463 ± 0.19 ng N-N2O/g soil unburned; ±SE). Although the effects of fire on nitrifier communities were not significant at one month post-fire (Control: p=0.14, AOA: p=0.09, AOB: p=0.162), both AOA and AOB contributions to NO emissions increased in response to fire. Results for nitrifier contributions to N2O emissions were highly variable and non-significant with no clear trends as all N2O emissions were near zero. Further analysis over the time series may yield clearer results as microbial communities have more time to recover. Pairing these data with isotopic information (in progress) may yield one of the most in-depth understandings of post-fire NO and N2O emissions to date.

How to cite: Stephens, E., Greene, A., Krichels, A., and Homyak, P.: Wildfires alter nitrifier communities and increase soil emissions of NOx but not N2O in California chaparral, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3695, https://doi.org/10.5194/egusphere-egu23-3695, 2023.

EGU23-4520 | ECS | Orals | BG1.2

Examining the response of different wildfire properties to changes in climate and CO2 levels at the Last Glacial Maximum 

Olivia Haas, Iain Colin Prentice, and Sandy P. Harrison

Climate change and atmospheric CO2 levels can influence wildfire properties through separate and potentially contrasting impacts on vegetation and climate. One way to examine the sensitivity of global wildfire properties to changes in climate and CO2 levels is using an out-of-sample experiment, such as the Last Glacial Maximum (LGM; 21 ka BP). Charcoal records show reduced burning at the LGM, when CO2 levels were ~ 185 ppm and the climate was cooler and drier. In this analysis, we isolated out the potential effects of LGM CO2 levels and LGM climate on the spatial patterns of global wildfire properties.

Using three statistical models, we conducted simulations of the spatial distribution of global burnt area, fire size and fire intensity under four scenarios: modern climate/modern CO2 levels, LGM climate/LGM CO2 levels, modern climate/LGM CO2 levels and LGM/ modern CO2 levels. We used outputs from three coupled ocean–atmosphere models representative of the range of simulated LGM climates. The ecophysiological effect of CO2 levels was explicitly accounted for through vegetation inputs. Gross primary productivity (GPP) and land cover were derived for the LGM and modern climate keeping either CO2 levels at 395 ppm (modern), or setting them to 185 ppm, using the P Model, a first-principles model of GPP which allows continuous acclimation of photosynthetic parameters to environmental variations, and the BIOME4 equilibrium global vegetation model.

Our results show a reduction in burnt area under LGM CO2 levels, both with modern and LGM climate inputs. In the case of the warmest of the LGM climate scenarios, this reduction was of the same magnitude as the combined LGM climate/LGM CO2 levels scenario. However, the driest and coldest LGM climate scenario produced a reduction in burnt area even with modern CO2 levels, and the largest reduction in burnt area with LGM CO2.  The reduction was primarily driven by changes in vapour pressure deficit (VPD). Fire size increased under LGM climates, due to changes in wind and VPD. The lower CO2 values at the LGM had no impact on fire size. Fire intensity increased under LGM climates and LGM CO2 levels, with both effects of similar amplitude and changes driven primarily by VPD, GPP and diurnal temperature range. 

We compared our outputs with sedimentary charcoal records from the Reading Palaeofire Database (RPD). Overall, the burnt area LGM CO2 levels/LGM climate scenario showed the greatest agreement, though depending on how cold and dry the LGM climate was, this agreement was either equal to LGM CO2 levels or LGM climate alone. These results suggest that whilst there was reduced global burning at the LGM, there may have been larger and more intense fires. They also highlight the importance of the ecophysiological effect of CO2 levels on fuels, a major control of burnt area and fire intensity regardless of climate. They point to the importance of including this effect in process-based fire models, as well as the importance of accurately estimating the amplitude of projected change for different climate variables in order to increase the reliability of future projections.

How to cite: Haas, O., Prentice, I. C., and Harrison, S. P.: Examining the response of different wildfire properties to changes in climate and CO2 levels at the Last Glacial Maximum, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4520, https://doi.org/10.5194/egusphere-egu23-4520, 2023.

EGU23-5113 | ECS | Orals | BG1.2

Speleothem organic biomarkers trace last millennium fire history at near-annual resolution in northwestern Australia 

Elena Argiriadis, Rhawn F. Denniston, Stefania Ondei, and David Bowman

Recent developments in speleothem science are showing their potential for paleofire reconstruction through a variety of inorganic and organic proxies including trace metals (1) and the pyrogenic organic compound levoglucosan (2). Previous work by Argiriadis et al. (2019) presented a method for the analysis of trace polycyclic aromatic hydrocarbons (PAHs) and n-alkanes in stalagmites (3). These compounds reflect biogeochemical processes occurring at the land surface, in the soil, and in the cave. PAHs are primarily related to combustion of biomass while n-alkanes, with their potential for vegetation reconstruction (4), provide information on fuel availability and composition, as well as fire activity. These organic molecules are carried downward by infiltrating water and incorporated into speleothems (5), thereby creating the potential to serve as novel paleofire archives.

Using this approach, we developed a high-resolution stalagmite record of paleofire activity from cave KNI-51 in tropical northwestern Australia. This site is well suited for high resolution paleofire reconstruction as bushfire activity in this tropical savanna is some of the highest on the continent, the cave is shallow and overlain by extremely thin soils, and the stalagmites are fast-growing (1-2 mm yr-1) and precisely dated. We analyzed three stalagmites which grew continuously in different time intervals through the last millennium - KNI-51-F (CE ~1100-1620), KNI-51-G (CE ~1320-1640), and KNI-51-11 (CE ~1750-2009). Samples were drilled continuously at 1-3 mm resolution from stalagmite slabs, processed in a stainless-steel cleanroom to prevent contamination.

Despite a difference in resolution between stalagmites KNI-51-F and -G, peaks in the target compounds show good replication in the overlapping time interval of the two stalagmites, and PAH abundances in a portion of stalagmite KNI-51-11 that grew from CE 2000-2009 are well correlated with satellite-mapped fires occurring proximally to the cave.

Our results suggest an increase in the frequency of low intensity fire in the 20th century relative to much of the previous millennium. The timing of this shift is broadly coincident with the arrival of European pastoralists in the late 19th century and the subsequent displacement of Aboriginal peoples from the land. Aboriginal peoples had previously utilized “fire stick farming”, a method of prescribed, low intensity burning, that was an important influence of ecology, biomass, and fire.  Prior to the late 1800s, the period with the most frequent low intensity fire activity was the 13th century, the wettest interval of the entire record. Peak high intensity fire activity occurred during the 12th century.

Controlled burn and irrigation experiments capable of examining the transmission of pyrogenic compounds from the land surface to cave dripwater represent the next step in this analysis. Given that karst is present in many fire-prone environments, and that stalagmites can be precisely dated and grow continuously for millennia, the potential utility of a stalagmite-based paleofire proxy is high.

 

 

(1) L.K. McDonough et al., Geochim. Cosmochim. Acta. 325, 258–277 (2022).

(2) J. Homann et al., Nat. Commun., 13:7175 (2022).

(3) E. Argiriadis et al., Anal. Chem. 91, 7007–7011 (2019).

(4) R.T. Bush, F. A. McInerney, Geochim. Cosmochim. Acta. 117, 161–179 (2013).

(5) Y. Sun et al., Chemosphere. 230, 616–627 (2019).

How to cite: Argiriadis, E., Denniston, R. F., Ondei, S., and Bowman, D.: Speleothem organic biomarkers trace last millennium fire history at near-annual resolution in northwestern Australia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5113, https://doi.org/10.5194/egusphere-egu23-5113, 2023.

EGU23-5429 | ECS | Posters on site | BG1.2

Smoke self-lofting towards the lower stratosphere: an alternative process to pyroCb-lofting 

Kevin Ohneiser, Albert Ansmann, Jonas Witthuhn, Hartwig Deneke, Alexandra Chudnovsky, Gregor Walter, and Fabian Senf

Wildfire smoke is known as a highly absorptive aerosol type in the shortwave wavelength range. The absorption of Sun light by optically thick smoke layers results in heating of the ambient air. This heating is translated into self-lofting of the smoke up to more than 1 km in altitude per day. The main goal is to demonstrate that radiative heating of intense smoke plumes is capable of lofting them from the lower and middle free troposphere (injection heights) up to the tropopause without the need of pyrocumulonimbus (pyroCb) convection. The further subsequent ascent within the lower stratosphere (caused by self-lofting) is already well documented in the literature. Simulations of heating rates which are then converted into lofting rates are conducted by using the ECRAD (European Centre for Medium-Range Weather Forecasts Radiation) scheme. As input parameters thermodynamic profiles from CAMS (Copernicus Atmosphere Monitoring Service) reanalysis data, aerosol profiles from ground-based lidar observations, radiosonde potential temperature profiles, CALIOP (Cloud Aerosol Lidar with Orthogonal Polarization) aerosol measurements, and MODIS (Moderate Resolution Imaging Spectroradiometer) aerosol optical depth retrievals were used. 


The sensitivity analysis revealed that the lofting rate strongly depends on aerosol optical thickness (AOT), layer thickness, layer height, and black carbon (BC) fraction. We also looked at the influence of different meteorological parameters such as cloudiness, relative humidity, and potential temperature gradient. Lofting processes in the stratosphere observed with CALIOP after major pyroCb events (Canadian fires, 2017, Australian fires 2019-2020) are compared with simulations to demonstrate the applicability of our self-lofting model. We analyzed long-term CALIOP observations of Siberian smoke layers and plumes evolving in the troposphere and UTLS (upper troposphere and lower stratosphere) region over Siberia and the adjacent Arctic during the summer season of 2019 and found several indications (fingerprints) that self-lofting contributed to the vertical transport of smoke. We hypothesize that the formation of a near-tropopause aerosol layer, observed with CALIOP over several months, was the result of self-lofting processes because this is in line with the self-lofting simulations. 


We will show a detailed analysis of tropospheric and stratospheric smoke lofting rates based on simulations and observations.

How to cite: Ohneiser, K., Ansmann, A., Witthuhn, J., Deneke, H., Chudnovsky, A., Walter, G., and Senf, F.: Smoke self-lofting towards the lower stratosphere: an alternative process to pyroCb-lofting, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5429, https://doi.org/10.5194/egusphere-egu23-5429, 2023.

EGU23-5803 | ECS | Orals | BG1.2 | Highlight

Which is the role of post-fire SOC erosion in the C cycle? 

Antonio Girona-García, Cristina Santín, Diana Vieira, and Stefan Doerr

Wildfires burn on average 448 million hectares globally every year, releasing around 2.2 Pg of carbon (C) into the atmosphere [1, 2]. The net effect of wildfires in the C cycle goes, however, beyond emissions and involves many other interacting processes. Among those, there is a significant knowledge gap on the role of post-fire soil organic carbon (SOC) erosion as a carbon sink mechanism.

Post-fire erosive response is greatly enhanced by the direct and indirect effects of wildfires on soil and vegetation, such as the loss of protective cover and soil structure or the development of a water-repellent layer [3]. In addition, biomass and soil organic matter undergo quantitative and qualitative changes during wildfires, such as the formation of pyrogenic carbon, highly resistant to degradation. The resulting PyC and non-PyC carbon fractions, with contrasting physical properties and chemical stability, will be differently redistributed and mineralized during the erosion process [4]. Ultimately, post-fire SOC erosion will act as a carbon sink when the post-fire burial and stabilization of eroded carbon, together with the recovery of net primary production and soil organic carbon content, exceed the SOC losses during its post-fire transport [5]. All these processes have been scarcely investigated and poorly quantified to the date. In this presentation, we will provide new insights into this potential C sink mechanism, critically reviewing the state of the art and highlighting key research gaps.

References

[1] Boschetti et al., 2021. Global Wildfire Information System (GWIS). https://gwis.jrc.ec.europa.eu/apps/country.profile/downloads

[2] Randerson et al., 2012. J Geophys Res. https://doi.org/10.1029/2012JG002128

[3] Shakesby & Doerr, 2006. Earth-Sci Revs. https://doi.org/10.1016/j.earscirev.2005.10.006

[4] Doetterl et al., 2016. Earth-Sci Revs. https://doi.org/10.1016/j.earscirev.2015.12.005

[5] Santín et al., 2015. Glob Change Biol. https://doi.org/10.1111/gcb.12800

How to cite: Girona-García, A., Santín, C., Vieira, D., and Doerr, S.: Which is the role of post-fire SOC erosion in the C cycle?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5803, https://doi.org/10.5194/egusphere-egu23-5803, 2023.

EGU23-6083 | ECS | Posters on site | BG1.2

Representing Northern High Latitude Peat Fires in the JULES-INFERNO Fire Model 

Katie Blackford, Apostolos Voulgarakis, Colin Prentice, Chantelle Burton, and Matthew Kasoar

Anthropogenic activities and climate change are increasing the vulnerability of carbon rich peatlands to wildfires. Peat fires, which are dominated by smouldering combustion, are some of the largest and most persistent wildfires on Earth. Across the northern high latitudes, peat fires have the potential to release vast amounts of long term stored carbon and other greenhouse gases and aerosols. Consequently, peat fires can have huge implications on the carbon cycle and result in a positive feedback effect on the climate system. Peat fires also impact air quality and can lead to haze events, with major impacts on human health. Despite the importance of peat fires they are currently not represented in most fire models, leading to large underestimations of burnt area and carbon emissions in the high latitudes. Here, I present a representation of peat fires in the JULES-INFERNO fire model (INFERNO-peat). INFERNO-peat improves the representation of burnt area across the high latitudes, with notable areas of improvement in Canada and Siberia. INFERNO-peat also highlights a large amount of interannual variability in carbon emissions from peat fires. The inclusion of peat fires into JULES-INFERNO demonstrates the importance of representing peat fires in models, and not doing so may heavily restrict our ability to model present and future fires and their impacts across the northern high latitudes.

How to cite: Blackford, K., Voulgarakis, A., Prentice, C., Burton, C., and Kasoar, M.: Representing Northern High Latitude Peat Fires in the JULES-INFERNO Fire Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6083, https://doi.org/10.5194/egusphere-egu23-6083, 2023.

EGU23-6184 | ECS | Orals | BG1.2 | Highlight

A global model for estimating fuel consumption and fire carbon emissions at 500-m spatial resolution 

Dave van Wees, Guido R. van der Werf, James T. Randerson, Brendan M. Rogers, Yang Chen, Sander Veraverbeke, Louis Giglio, and Douglas C. Morton

Fires constitute a key source of emissions of greenhouse gasses and aerosols. Fire emissions can be quantified using models, and these estimates are influenced by the spatial resolution of the model and its input data. Here we present a novel global model based on the Global Fire Emissions Database (GFED) modelling framework for the estimation of fuel consumption and fire carbon emissions at a spatial resolution of 500 m. The model was primarily based on observation-derived data products from MODIS, reanalysis data for meteorology, and an updated field measurement synthesis database for constraining fuel load and fuel consumption. Compared to coarser models, typically with a resolution of 0.25°, the 500-m spatial resolution allowed for increased spatially resolved emissions and a better representation of local-scale variability in fire types. The model includes a separate module for the calculation of emissions from fire-related forest loss, using 30-m Landsat-based forest loss data. We estimated annual carbon emissions of 2.1 Pg C yr-1, of which around 24% was from fire-related forest loss. Fuel consumption was on average a factor 10 higher in case of fire-related forest loss compared to fires without forest loss. Up to now, emission estimates from our new model are based on MODIS burned area with a 500-m resolution, leading to global emissions similar to GFED4s. However, novel high-resolution burned area datasets based on the Landsat and Sentinel-2 missions reveal substantially more global burned area. Our 500-m global fire model provides a suitable framework for converting these burned area products to emissions, with the prospect of substantially higher global emissions.

How to cite: van Wees, D., van der Werf, G. R., Randerson, J. T., Rogers, B. M., Chen, Y., Veraverbeke, S., Giglio, L., and Morton, D. C.: A global model for estimating fuel consumption and fire carbon emissions at 500-m spatial resolution, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6184, https://doi.org/10.5194/egusphere-egu23-6184, 2023.

EGU23-6286 | ECS | Posters on site | BG1.2

Hysteresis of fire-prone weather to CO2 forcing 

Jin-Soo Kim, Hyo-Jeong Kim, and Soon-Il An

CO2 emission from biomass burning (BB) is one of the essential elements of the global carbon budget, with its annual mean of about 2.0 PgC/year equivalent to 15 % of 2020 fossil fuel emissions. However, while a global increase in fire-prone weather is projected alongside climate change, a quantitative understanding of how much carbon will further be released due to increased fires is highly limited, which could result in large uncertainty in meeting the net zero target. Thus, in this study, we evaluate future changes in fire-prone weather based on the fire weather index (FWI) and estimate the potential fire-induced emissions on a global scale that could be induced by climate change. To this end, 28 ensembles of idealized CO2 reduction simulations with the CESM climate model were analyzed. The results show that when CO2 in the atmosphere is doubled (2xCO2) from 367 ppm by 1 % per year, the additional emission due to increased fire weather could reach about 1.7 PgC/year, which corresponds to 82% of the current BB emission. Moreover, even if the atmospheric CO2 concentration further peaks and is reduced back to 2xCO2, the lagged response of the climate system can cause fire-prone weather and its resulting C emissions to remain higher than its previous state in many countries. These results highlight that more focus is required on the climate-fire-carbon feedback not only for more accurate future predictions but also for achieving net zero emissions in each country through a proper wildfire management strategy.

How to cite: Kim, J.-S., Kim, H.-J., and An, S.-I.: Hysteresis of fire-prone weather to CO2 forcing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6286, https://doi.org/10.5194/egusphere-egu23-6286, 2023.

EGU23-6777 | ECS | Posters on site | BG1.2

Characterisation of large-scale urban fire emissions by inverse modelling 

Emilie Launay, Virginie Hergault, Marc Bocquet, Joffrey Dumont Le Brazidec, and Yelva Roustan

Large-scale fires such as warehouse fires that have occurred in recent years or dramatic accidents like the Paris Notre-Dame Cathedral fire in 2019 have stressed the need to develop means of assessing the toxicity risks to the population and the environment of smoke plumes. A key challenge is to quickly provide the authorities with information on the areas impacted by the plume and the pollutant concentration levels to which the population is likely to be or to have been exposed. The Laboratoire Central de la Préfecture de Police (LCPP) aims to deploy a number of devices for measuring pollutants and tracers of smoke combustion during a fire. Subsequently, the application of an atmospheric dispersion model within the framework of a data assimilation approach should provide a source characterisation and a finer estimate of the concentration levels at points of interest.

To characterise the source, noticeably the released mass of pollutants and the emission height linked to a plume rise, an inverse problem method has been implemented. It is based on a Bayesian Markov Chain Monte Carlo (MCMC) technique meant to quantify the uncertainties associated with the emission estimation. Since the emission height strongly influences the atmospheric dispersion in the vicinity of the source, two approaches are used to estimate it. The first one consists in finding the emission time rate for each considered height and the second one consists in focussing on a single emission height and its associated emission time rate using a discrete distribution to describe the vertical profile. We use the Lagrangian Parallel Micro Swift Spray (PMSS) model developed by AriaTechnologies fed with meteorological fields provided by Météo-France to represent the atmospheric dispersion of smoke.

Our inverse method is applied to a large warehouse fire that occurred in Aubervilliers near Paris in 2021 using real observations. Abnormal concentrations of particulate matter were recorded, with a peak at 160 µg.m-3, located in the centre of Paris about 6 km from the source. They were collected by the LCPP and AirParif, the local air quality agency, and are used to retrieve the emission with a quantification of uncertainties and a sensitivity analysis of model error. The resulting emission height of the source, mainly between 200 and 300 m, coincides with the terrain observation for an emission rate of less than 1000 kg/h throughout the duration of the fire. A sensitivity analysis to the initial approximation of the source (the prior) shows its importance. It suggests to improve our method by incorporating the statistical parameters of the observation error into the MCMC method.

How to cite: Launay, E., Hergault, V., Bocquet, M., Dumont Le Brazidec, J., and Roustan, Y.: Characterisation of large-scale urban fire emissions by inverse modelling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6777, https://doi.org/10.5194/egusphere-egu23-6777, 2023.

EGU23-6797 | ECS | Posters on site | BG1.2

Variability of CO and aerosols plumes from wildfires in the Northern Hemisphere in 2008-2022 using satellite observations. 

Antoine Ehret, Solène Turquety, Maya George, and Cathy Clerbaux

Wildfires are responsible for significant emissions of greenhouse gases, pollutants and aerosols. In addition to being a large source of carbon monoxide (CO) and carbon dioxide (CO2), they alone account for more than half of black carbon emissions and the majority of primary organic aerosol emissions.

Despite proactive fire suppression policies in the Northern Hemisphere (NH), allowing a decrease in fires, especially in Europe, an increase in the number of extreme fires can be noted in recent years. In the NH, this increase is mainly in Western America and boreal regions. The pollution plumes produced during extreme fires can be transported over thousands of kilometers, impacting background pollutant levels on a hemispheric scale. Thus, variability in fire intensity may explain a large part of the spatial and temporal variability of many atmospheric pollutants. For longer lived pollutants, wildfires may significantly increase background levels.

In this study, the link between extreme fire weather (high temperature), large fires and background pollution in the Northern Hemisphere is analyzed based on satellite observations. The impact of large wildfires on background levels of CO and aerosols above Europe is studied more specifically. We present the variability of fire frequency in the NH, their intensity and the related emissions using 20 years (2003-2022) of MODIS fire observations analyzed with the APIFLAME model. The link between large events and fire weather is studied using the ERA5 reanalyses and the Canadian Fire Weather Index (FWI). The related impact on the variability of total CO and AOD in the NH is analyzed using 15 years (2008-2022) of satellite observations from IASI/Metop and MODIS/Terra and Aqua, respectively. Finally, plume retro trajectories are computed in order to assess the contribution of the different geographical areas of the NH on the CO and AOD variability.

How to cite: Ehret, A., Turquety, S., George, M., and Clerbaux, C.: Variability of CO and aerosols plumes from wildfires in the Northern Hemisphere in 2008-2022 using satellite observations., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6797, https://doi.org/10.5194/egusphere-egu23-6797, 2023.

EGU23-7379 | Orals | BG1.2 | Highlight

Changes in global fire regimes under idealized overshoot scenarios 

Lars Nieradzik, Hanna Lee, Paul Miller, Jörg Schwinger, and David Wårlind

Within the framework of the project IMPOSE (Emit now, mitigate later? IMPlications of temperature OverShoots for the Earth system) six idealized emission-overshoot simulations have been performed with the Earth System Model NorESM2-LM2 and used as forcing for the 2nd generation dynamic global vegetation model LPJ-GUESS with its fire-model SIMFIRE-BLAZE to investigate the impact of different CO2 overshoots on global wildfire regimes.

The simulations describe a set of scenarios with high, medium, and low accumulative CO2 emissions and each of which has a short (immediate) and a long (100 years) peak of accumulative CO2 emissions before declining towards a baseline simulation of 1500 PgC accumulatively emitted within the first 100 years.

The results show that the height of the overshoot has an impact on global fire regimes while its duration does not seem to play a significant role 200 years after peak CO2. Overall, we can see that changes in vegetation composition following the temperature anomaly are the main driver for changes in global wildfire frequency. While in the low overshoot scenarios burnt area has almost converged towards the baseline simulation, the extremest scenarios show the lowest burnt area at the end of the simulation period, indicating that vegetation changes, especially in low latitudes, have been most significant and/or are still ongoing.

How to cite: Nieradzik, L., Lee, H., Miller, P., Schwinger, J., and Wårlind, D.: Changes in global fire regimes under idealized overshoot scenarios, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7379, https://doi.org/10.5194/egusphere-egu23-7379, 2023.

EGU23-7449 | ECS | Orals | BG1.2

The role of vegetation in UK upland wildfires: Risk, Resilience, and Remote Sensing 

Kirsten Lees and Tim Lenton

Wildfires are becoming a growing concern in the UK, as climate change increases the occurrence and persistence of periods of hot, dry weather. Vegetation type and management play an important but contested role in UK fire risk and resilience, and questions remain over the best ways to prevent large fires developing. Remote sensing can provide vital data on fire size, severity, and recovery times, but method effectiveness is dependent on understanding specific ecosystems. This research uses ground validation of four wildfires in the UK Peak District National Park to deliver insights which improve interpretation of satellite data in wildfire monitoring. These insights are then applied to a three-year remote sensing database of large wildfires in England and Wales, to give novel results on the links between vegetation type and management, and fire size and severity. Ecosystem resilience and recovery is further explored through analysing the vegetation growth post-fire at three of the four Peak District study sites. This project therefore develops and validates remote sensing methodology in wildfire research by combining field data with satellite imagery to yield new understandings of the relationships between vegetation and fire. 

How to cite: Lees, K. and Lenton, T.: The role of vegetation in UK upland wildfires: Risk, Resilience, and Remote Sensing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7449, https://doi.org/10.5194/egusphere-egu23-7449, 2023.

EGU23-7853 | Posters on site | BG1.2

Current Operational Implementation of the Canadian Forest Fire Weather Index System in the Republic of Ireland 

Klara Finkele, Padraig Flattery, Ciaran Nugent, and Paul Downes

Since 2006 the Canadian Forest Fire Weather Index System (FWI) has been employed operationally at Met Éireann to predict the risk of forest fires in Ireland (Walsh, S, 2006). Around 11% or 770,000 ha of the total land area of Ireland is afforested, but there are also large areas of open mountain and peatlands covered in grasses, dwarf-shrub and larger woody shrub type vegetation which can provide fuel for spring wildfires under suitable conditions. Following winter, vegetation can be dead or have a very low live moisture content, and the flammability of this vegetation can be readily influenced by prevailing weather, especially following prolonged dry periods.

The Department of Agriculture, Food and Marine is the Forest Protection authority in Ireland responsible for issuing Fire Danger Notices. These notices improve preparedness for fire responses and are based on information provided by Met Éireann who calculate the FWI and FWI components using observation data at synoptic stations, and the predicted FWI for the next five days ahead based on numerical weather prediction data.

The FWI is determined based on the types of forest fuel and how quickly they dry out/get rewetted, and components of fire behaviour. The FWI represents the fire intensity as the rate of energy per unit length of fire front (kW/m). The components which provide the most accurate indication of risk under Irish conditions are the Fine Fuel Moisture Code and Initial Spread Index, based on the fuels involved and ignition patterns observed to date. Since 2022 Met Eireann provide the FWI as well as the individual components Fine Fuel Moisture Content and Initial Spread Index via the public website for synoptic stations. These indices are based on observations and a seven-day forecast into the future using ECMWF predictions. This allows all county councils responsible for wildfire preparedness to access this information swiftly and directly.

Met Éireann also use the ANYWHERE multi-hazard warning tool which allows for visualisation of multiple fire-related risk factors and warning indices to be viewed simultaneously. The ANYWHERE system, in combination with our station-based forecast and antecedent conditions, provide fire managers and response teams with excellent information with which to make decisions. 

How to cite: Finkele, K., Flattery, P., Nugent, C., and Downes, P.: Current Operational Implementation of the Canadian Forest Fire Weather Index System in the Republic of Ireland, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7853, https://doi.org/10.5194/egusphere-egu23-7853, 2023.

EGU23-7913 | ECS | Posters on site | BG1.2

Fate of Fire altered Organic Carbon in the arctic river-to-ocean continuum: Resolving Mackenzie River Black Carbon in the Beaufort Sea 

Linn G. Speidel, Lisa Bröder, Julie Lattaud, Negar Haghipour, Timothy I. Eglinton, and Alysha I. Coppola

Keywords: Black carbon, Dissolved organic carbon, BPCAs, Mackenzie River, Beaufort Sea, Climate change

Climate change is amplified in the arctic and boreal regions. This causes higher average temperatures and less precipitation in the summer months and is resulting in longer wildfire seasons, severity, frequency and extent. This increases the relies of carbon into the atmosphere as greenhouse gases and aerosols, amplifying climate change even further. Black carbon (BC) is a fraction of organic carbon, resulting from the incomplete combustion of biomass and fossil fuels. BC may be inaccessible for biodegradation, because of its highly condensed aromatic molecular structure and therefore stores carbon on long timescales on land and in the ocean. BC is produced on land, but is transported as dissolved BC (DBC) by the rivers to the oceans, where it cycles on millennial timescales, sequestering BC. Thus, it is important to understand the significance of BC in the context of increased fires in this vulnerable region in the face of climate change.

The Mackenzie River is a major source of terrestrial dissolved organic carbon (DOC) and the largest source of sediments to the Arctic Ocean. Here, we resolve the cycling of riverine DBC from the Mackenzie River to its fate in the Beaufort Sea, and the influence of mixing with Pacific water masses entering from the Chukchi Sea. We present DBC concentration data in ocean water, which was collected on two cruises in the Beaufort Sea in 2021 and 2022 covering the outflow of the Mackenzie River.

For DBC concentrations, we digested solid phase extracts of DOC with nitric acid to oxidize BC molecules into benzenepolycarboxylic acids (BPCAs), which were then quantified on High Performance Liquid Chromatography (HPLC). We compare the concentrations of the DBC and DOC to trace the mixing of DBC river outflow with the ocean water. Since DBC originates on land and is relatively stable to biodegradation we can resolve the pathways of DBC from the Mackenzie River to the Arctic Ocean.

 

 

How to cite: Speidel, L. G., Bröder, L., Lattaud, J., Haghipour, N., Eglinton, T. I., and Coppola, A. I.: Fate of Fire altered Organic Carbon in the arctic river-to-ocean continuum: Resolving Mackenzie River Black Carbon in the Beaufort Sea, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7913, https://doi.org/10.5194/egusphere-egu23-7913, 2023.

EGU23-7937 | ECS | Orals | BG1.2

A New Method for Nowcasting Wildfire Risk 

Theodore Keeping, Sandy Harrison, and Iain Prentice

Wildfire risk prediction relies on the often-heuristic assessment of diverse fire potential indices, fuel maps, fire weather indices and prior fire activity data. Here we present a model nowcasting daily wildfire genesis probability and expected wildfire sizes in the contiguous US.

Predictors were selected and developed to account for climate, vegetation, topographic and human effects on wildfire genesis. Climate factors are represented by multiple fuel wetting and drying processes at daily to seasonal-scale antecedences, snowpack, and wind. We use GPP to predict fuel mass and recent growth, and dominant vegetation type. Human factors include population, landscape accessibility and ignition sources such as powerlines.

The first stage of the model predicts wildfire genesis probability as a zero-inflated process with an explicit probability of fire preclusion, whilst the second stage models fire sizes according to a generalised extreme value distribution. Nonlinear effects are accounted for via global optimisation for the domain for which each variable drives changes in fire genesis behaviour and the appropriate variable transform.

The model has good predictive and explanatory power, as shown by various performance metrics and the meaningful nonlinear relationships identified in the optimisation process. We show that this method can resolve seasonal wildfire risk dynamics well over smaller ecoregions than the observational record permits, allowing us to quantify the extent to which fire risk is determined by seasonal-scale versus daily-scale effects.

How to cite: Keeping, T., Harrison, S., and Prentice, I.: A New Method for Nowcasting Wildfire Risk, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7937, https://doi.org/10.5194/egusphere-egu23-7937, 2023.

EGU23-8075 | Posters on site | BG1.2

Impact of socio-economic factors in burnt area for future climate scenarios 

João Teixeira, Chantelle Burton, Douglas I. Kelley, Gerd Folberth, Fiona M. O'Connor, Richard Betts, and Apostolos Voulgarakis

Fire processes are a complex component of the Earth System processes and their full representation has proven to be difficult to represent Earth System Models (ESM). Because of this, these processes are often simplified in fire enabled ESMs, for instance ignitions are usually modelled to increase at low population densities up to a threshold, and reduce thereafter, as suppression effects become dominant with the increase of population density. However, socio-economic, and cultural factors can play a significant role in shaping the behaviour of fire ignitions. This study aims to address this by implementing a socio-economic factor in the fire ignition and suppression parametrisation in the INteractive Fire and Emission algoRithm for Natural envirOnments (INFERNO) based on the Human Development Index (HDI). The inclusion of this factor reduced a large long-standing positive bias found in regions of Temperate North America, Central America, Europe, and Southern Hemisphere South America. This change also leads to improvements in the model representation of fire weather and anthropogenic drivers in tropical regions, by reducing the influence of population density changes. Therefore, this framework can be used to improve understanding of the anthropogenic impacts of fire in future scenarios based on different Shared Socioeconomic Pathways.

How to cite: Teixeira, J., Burton, C., Kelley, D. I., Folberth, G., O'Connor, F. M., Betts, R., and Voulgarakis, A.: Impact of socio-economic factors in burnt area for future climate scenarios, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8075, https://doi.org/10.5194/egusphere-egu23-8075, 2023.

EGU23-9361 | ECS | Posters on site | BG1.2

Investigating Emergency Room Visits for Cardiorespiratory Diseases in Alberta and Ontario, Canada in Relation to Wildfires 

Victoria Flood, Kimberly Strong, Rebecca Buchholz, Sheryl Magzamen, and Grace Kuiper

Carbon monoxide (CO) is released during biomass burning events, resulting in decreased air quality and leading to the formation of climate forcing pollutants. An increase in wildfires has resulted in a change to the CO seasonal cycle of the North American Pacific Northwest, when comparing 2012-2018 to 2002-2011. This trend was reported using data from the Measurements of Pollution in the Troposphere (MOPITT) instrument on NASA’s Terra satellite. Similarly, an increase in summertime CO values was identified with the Fourier Transform Infrared (FTIR) spectrometer at the University of Toronto Atmospheric Observatory (TAO), over the same time period. Studies have shown correlations between wildfire smoke exposure and healthcare utilization for cardiovascular and respiratory conditions. Monthly counts of Emergency Department admissions for cardiovascular and respiratory diseases for Alberta and Ontario are investigated in relation to wildfire events in Canada and the USA. MOPITT and TAO FTIR CO columns, the Moderate Resolution Imaging Spectroradiometer (MODIS) burned area product, and provincial burned areas from Natural Resources Canada are assessed to estimate wildfire smoke exposure in the study region. This work aims to evaluate if CO can be used as a complementary tracer for health impacts from wildfire smoke exposure. 

 

How to cite: Flood, V., Strong, K., Buchholz, R., Magzamen, S., and Kuiper, G.: Investigating Emergency Room Visits for Cardiorespiratory Diseases in Alberta and Ontario, Canada in Relation to Wildfires, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9361, https://doi.org/10.5194/egusphere-egu23-9361, 2023.

EGU23-9575 | Orals | BG1.2

FRYv2.0 : a global fire patch morphology database from FireCCI51 and MCD64A1 

Florent Mouillot, Wentao Chen, Manuel Campagnolo, and Philippe Ciais

The assessment of global burned area from remote sensing is an essential climate variable driving land surface GHG emissions and energy/water budget. Gridded 0.25° or 0.5° monthly burned area have been largely used for biosphere/atmosphere interactions modelling, while recent fire/weather analysis or model developments increasingly request fire events, defined as a fire patch with intrinsic fire spread properties. Pixel level information, the finest resolution from global burned area, defined by their burn date, can be aggregated within a spatio-temporal threshold and delineate these fire events. Uncertainties in burn date, the coarse resolution of pixel resolution, multiple ignition points, or the specified values in spatio-temporal thresholds can however lead to various final fire event delineation. Currently, three major global fire event database exist (FRY, Fire Atlas, GlobFire), mostly derived from MCD64A1 pixel level 500m-resolution burned area. We propose here a new version of FRY, based on MCD64A1 and FireCCI51 at 250m, with an updated pixel aggregation method allowing for single ignition fire patches. Fire patch morphology indicators as elongation, direction, complexity have been conserved from v1.0, with additional information as ignition points from minimum burn date from burned area and more timely-accurate hotspots (VIIRS and MCD14ML), rate of spread, fire Radiative power and burn severity, as well as fraction of land cover affected, based on user requirements. The dataset is delivered as a yearly shapefile, with an attribute table referencing all information on ignition, spread and final shape. Global comparison of major information from FRYv2.0 (fire size distribution, fire number, ROS) will illustrate the effects of increasing spatial resolution and better timing from hotspots provided in this new version, freely available for the scientific community for the period 2001-2020.

How to cite: Mouillot, F., Chen, W., Campagnolo, M., and Ciais, P.: FRYv2.0 : a global fire patch morphology database from FireCCI51 and MCD64A1, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9575, https://doi.org/10.5194/egusphere-egu23-9575, 2023.

EGU23-9791 | Orals | BG1.2 | Highlight

Lightning in a changing climate and its impacts on fire area burned 

Cynthia Whaley, Courtney Schumacher, Montana Etten-Bohm, Vivek Arora, David Plummer, Jason Cole, Michael Lazare, and Ayodeji Akingunola

Lightning is an important atmospheric process for igniting forest fires – often in remote locations where they are not easily suppressed – which results in potentially large emissions of many pollutants and short-lived climate forcers. Lightning also generates reactive nitrogen, resulting in the production of tropospheric ozone, the third most important greenhouse gas. Furthermore, the changing climate is expected to change the frequency and location of lightning. As such, lightning is an important component of climate models. The Canadian Atmospheric Model, CanAM, is one such climate model that did not contain an 'online' lightning parameterization. Fire ignition in CanAM was done via an unchanging climatological lightning input. In this study, we have added a new logistical regression lightning model (Etten-Bohm et al, 2021) into CanAM, creating the capacity for future lightning predictions with CanAM under different climate scenarios. The modelled lightning and fire area burned were evaluated against measurements in a historical period with good results. Then we simulate lightning and fire area burned in a future climate scenario in order to provide an estimate on how lightning and its impacts will change in the future. This study also presents the first time that CanAM’s land fire model was used online with its atmosphere to fully simulate fires in the global earth system.

Reference:

Etten-Bohm, M., J. Yang, C. Schumacher, and M. Jun : Evaluating the relationship between lightning and the large-scale environment and its use for lightning prediction in global climate models, JGR-atmospheres, 126, e2020JD033990, 2021.

How to cite: Whaley, C., Schumacher, C., Etten-Bohm, M., Arora, V., Plummer, D., Cole, J., Lazare, M., and Akingunola, A.: Lightning in a changing climate and its impacts on fire area burned, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9791, https://doi.org/10.5194/egusphere-egu23-9791, 2023.

EGU23-10336 | Posters on site | BG1.2

A hybrid deep learning framework for predicting point-level Alaskan fires 

Hocheol Seo and Yeonjoo Kim

Fires in high latitudes are becoming more critical in terrestrial ecosystem modeling. With climate warming and dry weather condition, the fires have spread more, and widespread burning has severely damaged the ecosystem. As the fire dynamics cannot be described with the mass or energy balance equations, the fire models have been developed with different input variables, linked with different vegetation models, and widely coupled with the earth system models (ESMs) or land surface models (LSMs) with different complexities of parameterization. Here, we designed a new approach using hybrid deep learning [Long Short-Term Memory (LSTM) - Artificial Neural Network (ANN)] for predicting Alaskan natural fires and aimed to understand the impacts of fires with from the NCAR community land model 5 – biogeochemistry (CLM5-BGC). This study was conducted based on fire information provided by Alaska Interagency Coordination Center (AICC), which provides the data for each fire point, start date, end date, and total burned area from 2016-2020. As the fire duration was identified as the most important in predicting the burned area, we first trained the LSTM for predicting fire duration (i.e., fire ignition and fire persistence period) with ERA5 atmospheric forcings. Also, we trained ANN to predict the burned area with both ERA5 atmospheric forcings and fire duration. Then, we combined two models (LSTM and ANN) to simultaneously predict the fire days and burned area with climate and vegetation datasets. This hybrid model has the strength to capture large fires (>10000ha), comparing the burned area from CLM5-BGC (Correlation: 0.79). When this hybrid model is coupled with CLM5-BGC, we found that the carbon fluxes changed over Alaska. In particular, total net ecosystem exchange (NEE) increased by more than two times that of only CLM5-BGC, which could primarily affect terrestrial carbon exchanges.

Acknowledgement

This work was supported by the Korea Polar Research Institute (KOPRI, PE22900) funded by the Ministry of Oceans and Fisheries and the Basic Science Research Program through the National Research Foundation of Korea, which was funded by the Ministry of Science, ICT & Future Planning (grant no. 2020R1A2C2007670) and by the Ministry of Education (2022R1A6A3A13073233).

How to cite: Seo, H. and Kim, Y.: A hybrid deep learning framework for predicting point-level Alaskan fires, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10336, https://doi.org/10.5194/egusphere-egu23-10336, 2023.

EGU23-10389 | Orals | BG1.2

Towards mechanistic representation of wildfire effects on soil – downscaling to quantify subsurface heat fluxes 

Dani Or, Hamid Vahdat-Aboueshagh, Eden Furtak-Cole, and Sean A. McKenna

Advances in wildfire modeling have focused on refining atmospheric interactions for obvious links between local airflows, combustion dynamics, fire line advance and smoke plume transport. Yet, lasting impacts of wildfires on landscapes are linked primarily with changes in soil characteristics and alteration of ecological and hydrologic processes. Quantitative assessment of wildfire impacts requires metrics for fire-surface thermal interactions beyond qualitative surrogates such as burn severity used for ecological assessment. The highly transient and localized nature of wildfire intensity and its coarse spatial and temporal representation hinder quantitative translation of wildfire dynamics to soil heat fluxes even with the most advanced wildfire models (e.g., QuicFire, WRF-Fire, WFDS). Inspired by the pioneering works of Byram, Rothermel and Albini, we seek to derive high resolution information on fire line intensities from highly resolved fuel maps informed by fire line dynamics derived from numerical wildfire model representation. This hybrid downscaling approach (limited by the quality and resolution of fuel maps) offers a means for constraining soil surface heat fluxes at resolutions relevant to quantifying critical temperatures and duration at depth to estimate pyrolysis of soil organic carbon and the degree of soil structure alteration. Examples will be presented and discussed. 

How to cite: Or, D., Vahdat-Aboueshagh, H., Furtak-Cole, E., and A. McKenna, S.: Towards mechanistic representation of wildfire effects on soil – downscaling to quantify subsurface heat fluxes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10389, https://doi.org/10.5194/egusphere-egu23-10389, 2023.

EGU23-10651 | ECS | Posters on site | BG1.2

An annually resolved stalagmite record of fire frequency for the last 250 years in south west Australia 

Liza McDonough, Pauline Treble, Andy Baker, Andrea Borsato, Silvia Frisia, Micheline Campbell, Gurinder Nagra, Katie Coleborn, Michael Gagan, Jian-xin Zhao, and David Paterson

Stalagmites provide records of past changes in climate, vegetation, and surface events, which can be identified through variability in their chemical composition over time. This variability is the result of changes in surface environmental properties, which are reflected in the physical and chemical properties of the water that percolates into the cave, ultimately affecting the composition of the speleothem calcite. Wildfires have the potential to alter soil properties and soluble element concentrations. Consequently, stalagmite compositions have been shown to respond to increases in soil nutrients, trace metal concentrations, and changes in soil/karst bedrock hydraulic conductivity. It is, therefore, likely that stalagmites, and particularly those grown in shallow caves for which transmission of the surface signal is rapid, capture the environmental effects of wildfires in their chemical and physical properties.

We analysed a stalagmite from a shallow cave in a region known to be affected by wildfires in south-west Western Australia. Fire proxies were assessed using a multi-proxy approach. This includes water isotopes via stable-isotope ratio mass spectrometry and trace element analyses via synchrotron X-ray fluorescence microscopy and laser ablation inductively coupled plasma mass spectrometry. This approach shows that the timing of known fire events coincided with a multi-proxy response in stalagmite chemistry, including increased concentrations of phosphorus, copper, aluminium, lead, and zinc, which are interpreted to be derived from leaching of ash from burned vegetation above the cave. We also identified lower and less variable peaks in phosphorus concentrations during the pre-colonisation period, suggesting that Indigenous land management resulted in more frequent but low intensity burning. This contrasted with less frequent but more intense fires associated with post-colonisation land-management. A particularly large paleo-fire identified in 1897 appears to coincide with a peak in 𝛿18O, interpreted to have resulted from evaporation of sub-surface water during the heat of the fire. This large fire was preceded by a multi-decadal dry period identified by trace element proxies. The intensity of the 1897 fire was then exacerbated by the combination of a multi-decadal drought and a transition away from cultural burning practices by Indigenous Australians, which resulted in build-up of vegetation and dry combustible material on the forest floor.

This research is a world-first demonstration of fire events recorded in stalagmites and shows their potential to provide accurate records of both fire frequency intervals and changes in climate. Further records of past fire events from stalagmites will help to understand how past fire regimes have varied with climate, land-use change and colonisation, and will help to better guide land management practices in the future.

How to cite: McDonough, L., Treble, P., Baker, A., Borsato, A., Frisia, S., Campbell, M., Nagra, G., Coleborn, K., Gagan, M., Zhao, J., and Paterson, D.: An annually resolved stalagmite record of fire frequency for the last 250 years in south west Australia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10651, https://doi.org/10.5194/egusphere-egu23-10651, 2023.

EGU23-11016 | ECS | Posters on site | BG1.2

Speleothems as archives for palaeofire proxies 

Micheline Campbell, Liza McDonough, Pauline Treble, Andy Baker, Nevena Kosarac, Katie Coleborn, Peter Wynn, and Axel Schmitt

Environmental proxy archives such as tree rings, sediment cores, and ice cores are commonly used to investigate past fire regimes. Speleothems, naturally forming cave decorations mainly comprising of stalagmites, stalactites, and flowstones, have been extensively used as palaeoenvironmental archives as their physical attributes and chemical composition change with changed environment. Research has shown that cave drip water chemistry responds to fire events, and more recently, that speleothems can record past fire events due to physical and chemical processes which alter speleothem composition. These processes include changes to water stores due to evaporation, fracturing of the host rock, changed soil hydrophobicity, production of highly soluble lime, changes in soil CO2 production, destruction of vegetation and deposition of ash above the cave. These changes can result in shifts in δ18O and δ13C, altered concentrations of vegetation, soil and bedrock-derived elements, and incorporation of soluble ash derived elements (including phosphorus, aluminium, copper, zinc, and lead) in speleothems (McDonough et al., 2022; Campbell et al., 2022).

Changes in speleothem chemistry are typically determined using micro-analytical techniques (such as Synchrotron X-ray Fluorescence Microscopy and laser ablation inductively coupled plasma mass spectrometry) and isotope ratio mass spectrometry. These changes can be precisely and absolutely dated via uranium-series and carbon dating, and can often be resolved at high resolution via manual counting of seasonal fluctuations in organic matter and trace element concentration. This makes speleothems, particularly those grown in shallow caves in highly seasonal climates, ideal for identifying both short-lived events such as wildfires, and longer-term changes such as shifts in climate. This novel application of speleothems as archives for coupled climate and palaeofire proxies is still in its infancy but holds great potential.

Here, we present a review of this new sub-discipline. We cover its origins in cave dripwater monitoring, discuss site and sample selection, and describe the current analytical and statistical approaches used to extract fire information from speleothems. Such records will enable land managers to develop improved methods for managing fire regimes.

McDonough, L.K., Treble, P.C., Baker, A., Borsato, A., Frisia, S., Nagra, G., Coleborn, K., Gagan, M.K., Zhao, J., Paterson, D., 2022. Past fires and post-fire impacts reconstructed from a southwest Australian stalagmite. Geochimica et Cosmochimica Acta. https://doi.org/10.1016/j.gca.2022.03.020
 
Campbell, M., McDonough, L., Treble, P., Baker, A., Kosarac, N., Coleborn, K., Wynn, P.M., Schmitt, A., 2022. Speleothems as Archives for Palaeofire Proxies [preprint], https://www.authorea.com/doi/full/10.1002/essoar.10511989.1
 

How to cite: Campbell, M., McDonough, L., Treble, P., Baker, A., Kosarac, N., Coleborn, K., Wynn, P., and Schmitt, A.: Speleothems as archives for palaeofire proxies, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11016, https://doi.org/10.5194/egusphere-egu23-11016, 2023.

EGU23-11297 | Orals | BG1.2

Effects of land use, fuel loads and fuel moisture on fire intensity and fire emissions in South America derived by reconciling bottom-up and top-down satellite observations 

Matthias Forkel, Niels Andela, Vincent Huijnen, Christine Wessollek, Alfred Awotwi, Daniel Kinalczyk, Christopher Marrs, and Jos de Laat

Emissions from vegetation fires in tropical forests have the potential to turn the global land carbon sink into a source, affect atmospheric chemistry, and hence air quality. While natural forest fires are a rare phenomenon in tropical forests of South America and are usually of rather low intensity, deforestation fires and small land clearings in systems with high fuel loads can cause intense fires and high emissions. However, the high moisture content in tropical forests causes incomplete combustion and higher emissions of carbon monoxide (CO) than of carbon dioxide. The interacting effects of land use change, fuel load and moisture on fire intensity and emissions is, however, difficult to quantify at large scales because not all of those components are readily available from Earth observations in a consistent way. 

Here, we make use of several satellite products on vegetation, fire activity and atmospheric composition to quantify the effects of land use, fuel loads, fuel moisture on fuel consumption, emission factors and hence on emissions and atmospheric trace gas concentration. First, we use observations of active fires and fire radiative power from the VIIRS and Sentinel-3 SLSTR sensors to map different fire types (forest fires, deforestation fires, small land clearing and agricultural fires, savannah fires). Second, we integrate satellite products of canopy height, above-ground biomass, leaf area index, land cover and soil moisture in a novel data-model fusion framework to estimate fuel loads and moisture in vegetation, surface litter and woody debris. We then combine in a bottom-up approach the fire types with fuel loads and moisture to estimate fuel consumption and fire emissions using default emission factors. Third, we use observations from Sentinel-5p TROPOMI and the Integrated Forecast Systems (IFS) of the Copernicus Atmosphere Monitoring Service to compare the bottom-up estimates with distributions of CO and NOx in the atmosphere, which allows optimising emissions and associated emission factors.

Our reconciled estimates of fire emissions outperform previous CO estimates e.g. from the Global Fire Assimilation System, which demonstrates an improved estimation of fire carbon emissions. The results show that the high fire intensity and emissions in tropical deforestation fires originate from the burning of high loads of woody biomass and coarse woody debris. The high fuel moisture content causes higher emission factors of CO in tropical forests than in savannah fires and hence higher absolute emissions of CO. Our new model approaches and satellite products allow to provide an integrated assessments on the effects of fuel and fire behaviour on fire emissions.

How to cite: Forkel, M., Andela, N., Huijnen, V., Wessollek, C., Awotwi, A., Kinalczyk, D., Marrs, C., and de Laat, J.: Effects of land use, fuel loads and fuel moisture on fire intensity and fire emissions in South America derived by reconciling bottom-up and top-down satellite observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11297, https://doi.org/10.5194/egusphere-egu23-11297, 2023.

EGU23-11559 | ECS | Orals | BG1.2

Identifying the limits to fire growth in Eastern Siberia 

Thomas Janssen and Sander Veraverbeke

Boreal forests store about one third of the world’s forest carbon and may store even more carbon in the future because of the positive effects of rising atmospheric CO2 concentrations on photosynthesis and plant growth. However, fire frequency and severity have also been increasing in boreal forests in the last decades, which might offset their carbon sink potential. In Eastern Siberia, the dry and hot summers of 2020 and 2021 showed exceptionally high fire activity. However, even large fires that can spread for several months, eventually come to an end. This can be because of a change in the weather or because fires run out of fuels. Here, we aim to quantify the controls of fire growth in Eastern Siberia using high resolution landscape variables and hourly ERA-5 meteorological variables. We harmonized the burned area product from the Fire Climate Change Initiative and active fire product from the Visible Infrared Imaging Radiometer Suite, and derived fire perimeters from them for the period between 2012 and 2021. Along these fire perimeters, we then identified spatial changes in landscape variables (i.e. a decline in tree cover or increase in surface water) and temporal changes in hourly vapor pressure deficit and wind. By doing so, we could attribute causes of why fires stopped spreading.

How to cite: Janssen, T. and Veraverbeke, S.: Identifying the limits to fire growth in Eastern Siberia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11559, https://doi.org/10.5194/egusphere-egu23-11559, 2023.

EGU23-11992 | Orals | BG1.2

Assessing the feasibility of prescribed burning as a fire risk reduction tool for The Netherlands 

Niels van Manen, Albert Buxó, Linde Egberts, Laura Houwaard, Lennard Jacobsen, Jip Keesom, Martijn Reijners, David van Slooten, Anneloes Teunisse, and Anoek van Tilburg

Climate change is expected to cause prolonged and more severe droughts in Europe, increasing landscape fire occurrence. Since The Netherlands has a high population density in areas typified as ‘Wildland-Urban Interface’, a genuine risk for Dutch society arises. Landscape management, such as prescribed burning, can reduce fire risk. Prescribed burning is executed by intentionally burning the low and understory vegetation, limiting fuel for a landscape fire, under controlled conditions. In this interdisciplinary research, conducted by a team of (early career) researchers from climate science, cultural studies, hydrology, mathematics and spatial economics, we aim to assess whether prescribed burning can be used in The Netherlands as a fire risk reduction tool in natural areas with a high fire risk.

 

The Netherlands has a well-developed flood management system. However, it lacks such holistic approaches to landscape fire management. Landscape managers and researchers can learn from Dutch flood management by applying the secondary objective, improvement of spatial quality, to prescribed burning. In this research we assess the potential for improving spatial quality through prescribed burning, by adapting the spatial quality framework of the Dutch Room for the River project. Our framework looks at the three pillars burning effectiveness, ecological robustness, and cultural meaning at the potential prescribed burning sites. Burning effectiveness is highest in natural areas (Natura 2000 sites), with high fire risk and the presence of low vegetation. Ecological robustness measures the disturbance prescribed burning could cause in a landscape. Disturbance depends on the burning frequency and intensity, as well as on the type of vegetation that is burned and the usage of the area. In groundwater protection areas, seepage of harmful elements could cause more disturbance. These areas are therefore excluded from the analysis. From the perspective of cultural meaning, social perceptions influence the measure’s performance. Cultural significance and landscape identification provide various perspectives on fires and prescribed burning. Categorizing the different levels of engagement, based on an engagement pyramid, can deliver a basis for implementing prescribed burning.

 

Preliminary analyses result in a selection of 15 Natura 2000 sites in The Netherlands where prescribed burning could be feasible, varying from the Voornes Duin (14 km2) to the Veluwe (885 km2). These areas are mostly vegetated with coniferous and mixed forests. Prescribed burning potentially causes more disturbance in grasslands. However, since none of the 15 areas contain more than 24% grassland, prescribed burning could still be feasible at all locations. In the area of the Veluwe, qualitative interviews with the local population indicate support for fire management, such as prescribed burning, as they are aware of the risks imposed by landscape fires.

 

The final research results can contribute to the improvement of fire management in both The Netherlands and other North-Western European countries with similar vegetation and climate change effects.

How to cite: van Manen, N., Buxó, A., Egberts, L., Houwaard, L., Jacobsen, L., Keesom, J., Reijners, M., van Slooten, D., Teunisse, A., and van Tilburg, A.: Assessing the feasibility of prescribed burning as a fire risk reduction tool for The Netherlands, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11992, https://doi.org/10.5194/egusphere-egu23-11992, 2023.

EGU23-12559 | ECS | Posters on site | BG1.2

High-latitude wildfires, atmospheric composition, and climate 

Eirini Boleti, Katie Blackford, Stelios Myriokefalitakis, and Apostolos Voulgarakis

In high-latitude regions, larger and more frequent fires have been occurring over recent years, a tendency that is expected to continue in the coming decades due to warmer temperatures and regionally decreased precipitation imposed by climate change (IPCC,2019). Boreal wildfires in general are a significant source of CO2 emissions, as well as other greenhouse gases and aerosols (Akagi et al. 2011; Van Der Werf et al. 2010), e.g. emissions from boreal forests between 1997 and 2016 accounted for 7.4% of the global emissions (van der Werf et al. 2017). The effects of boreal fires on future climate have not been investigated and are potentially of great importance since climate change is occurring more rapidly in those high-latitude areas. More flammable forests in addition to the large carbon-rich peatlands, will potentially lead to devastating consequences.

The overall goal of our project is to quantify the effects of high-latitude wildfire emissions on atmospheric composition as well as climate. For this purpose, simulations with the EC Earth Earth System Model (ESM) are being employed to characterize the past, present and future variability and changes of wildfires especially in high latitudes. In the results presented here, we demonstrate how the EC Earth model performs when forced with prescribed fire emissions (GFED4) and with a more detailed peat fire module developed by our team. The mean state, seasonality, and interannual variability of fire emissions and key atmospheric constituent abundances (black carbon, organic carbon, NOx, CO, ozone, amongst others) are validated in the model, using a range of observational datasets. This validation exercise is a key step before employing the EC-Earth model for quantifying future impacts of high-latitude fires on atmospheric composition and climate.

 

IPCC,2019: Jia, G., E. Shevliakova, P. Artaxo, N. De Noblet-Ducoudré, R. Houghton, J. House, K. Kitajima, C. Lennard, A. Popp, A. Sirin, R. Sukumar, L. Verchot, 2019: Land–climate interactions. In: Climate Change and Land: an IPCC special report on climate change, desertification, land degradation, sustainable land management, food security, and greenhouse gas fluxes in terrestrial ecosystems [P.R. Shukla, J. Skea, E. Calvo Buendia, V. Masson-Delmotte, H.-O. Pörtner, D.C. Roberts, P. Zhai, R. Slade, S. Connors, R. van Diemen, M. Ferrat, E. Haughey, S. Luz, S. Neogi, M. Pathak, J. Petzold, J. Portugal Pereira, P. Vyas, E. Huntley, K. Kissick, M, Belkacemi, J. Malley, (eds.)]. In press.

Akagi, S.K. et al., 2011: Emission factors for open and domestic biomass burning for use in atmospheric models. Atmos. Chem. Phys., 11, 4039–4072, doi:10.5194/acp-11-4039-2011.

Van Der Werf, G.R. et al., 2010: Global fire emissions and the contribution of deforestation, savanna, forest, agricultural, and peat fires (1997–2009). Atmos. Chem. Phys., 10, 11707–11735, doi:10.5194/acp-10-11707-2010.

Van Der Werf, G.R. et al., 2010: Global fire emissions and the contribution of deforestation, savanna, forest, agricultural, and peat fires (1997–2009). Atmos. Chem. Phys., 10, 11707–11735, doi:10.5194/acp-10-11707-2010.

How to cite: Boleti, E., Blackford, K., Myriokefalitakis, S., and Voulgarakis, A.: High-latitude wildfires, atmospheric composition, and climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12559, https://doi.org/10.5194/egusphere-egu23-12559, 2023.

EGU23-12604 | Orals | BG1.2

Causes of uncertainty in simulated burnt area by fire-enabled DGVMs 

Matthew Forrest, Chantelle Burton, Markus Drüke, Stijn Hantson, Fang Li, Joe Melton, Lars Nieradzik, Sam Rabin, Stephen Sitch, Chao Yue, and Thomas Hickler

Fire-enabled dynamic global vegetation models (DGVMs) can be used to study how fire activity responds to its main drivers, including climate/weather, vegetation and human activities, at coarse spatial scales. Such models can also be used to examine the effects of fire on vegetation, and, when embedded in Earth system models, investigate the feedback of fire on the climate system. Thus they are valuable tools for studying wildfires. Accordingly, the Fire Model Intercomparison Project (FireMIP) was established to evaluate and utilise these models using consistent protocols.

Here we present the second round of FireMIP simulations to focus historic wildfire drivers (1901 to present). A six-member ensemble of simulations from fire-enabled DGVMs was compared to remotely-sensed burnt area observations and to the previous round of historical FireMIP simulations. We found that the model skill when simulating spatial patterns of burnt area shows modest improvements compared to the previous FireMIP round, and that the simulations mostly reproduce the decreasing trend in global burnt area found over the last two decades. However, whilst the broad global patterns are reasonable, there are considerable discrepancies with regards to regional agreement and timing of burnt area. Furthermore, the models show diverging trends in the pre-satellite era.

To investigate further and inform future model development, we explored the residuals between simulated burnt area from the FireMIP models and remotely-sensed burnt area as a function of climate, vegetation, anthropogenic and topographic variables using generalised additive models (GAMs). We found some common responses across the models, with many over-predicting fire activity in arid/low productivity areas and all models under-predicting at low road density. However, with respect to other variables, such as wind speed and cropland fraction, the models residuals showed divergent responses. It is anticipated that these results should aid further development of global fire models in terms of driving variables, process representations and model structure.

How to cite: Forrest, M., Burton, C., Drüke, M., Hantson, S., Li, F., Melton, J., Nieradzik, L., Rabin, S., Sitch, S., Yue, C., and Hickler, T.: Causes of uncertainty in simulated burnt area by fire-enabled DGVMs, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12604, https://doi.org/10.5194/egusphere-egu23-12604, 2023.

EGU23-12731 | ECS | Posters on site | BG1.2

Quantifying the direct influence of climate change on the rate of spread of wildfires in the Iberian Peninsula 

Martín Senande-Rivera, Damián Insua-Costa, and Gonzalo Míguez-Macho

Due to its strong connection with meteorological conditions and vegetation structure, fire activity is affected by anthropogenic climate change. As a direct effect, climate regulates fuel moisture, so warmer and drier conditions are linked to higher fuel flammability, increasing fire risk. We use data from ERA5 and different CMIP6 models to build a database of fuel moisture (for both live and dead fuels) under real conditions (factual) and modified conditions without the influence of global warming (counterfactual). We then calculate the rate of spread of some observed wildfires in the Iberian Peninsula from 2001 to 2021, from both factual and counterfactual data. We find that climate change influence is already noticeable and significant. We also identify the areas most vulnerable to the impacts of climate change and the time of the year when these impacts are strongest. 

How to cite: Senande-Rivera, M., Insua-Costa, D., and Míguez-Macho, G.: Quantifying the direct influence of climate change on the rate of spread of wildfires in the Iberian Peninsula, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12731, https://doi.org/10.5194/egusphere-egu23-12731, 2023.

Tropospheric ozone (O3) is a key greenhouse gas and pollutant that is receiving increasing attention globally.  While there are many sources of tropospheric O3, precursors from human activity (Anthro) and open biomass burning (BB) are the only ones that can be controlled. As such, it is crucial for policymakers to understand the relative contributions of the two. However, determining the contribution of O3 can be challenging as it cannot be directly observed. It must be calculated by chemical transportation model (CTM) simulation which could be biased for unreal emission inventory, or estimated by real observations that assumes too simple chemical and transportation processes.

In this paper, we propose a solution by developing a deep learning (DL) model that combines both CTM simulations and observations. The DL model is able to learn a generalized relationship between unobservable O3 contribution from Anthro or BB sectors and observable mixing ratio of tracers simulated by CTM with full chemistry and transportation processes. The DL model then, when applied to observed tracers, could avoid the bias from model to provide an accurate estimation of the contributions in reality.

Our results indicate the contribution from BB to tropospheric remote ozone mixing ratio is no larger than that from Anthro emission from a global perspective, even when uncertainties are deliberately tuned to bias BB. Therefore, the reduction of anthropogenic emissions should be the top priority for controlling global background O3 levels, at least for the time period of 2016-2018 studied.

How to cite: Ma, C., Cheng, Y., and Su, H.: Biomass Burning Contributes Less to Remote Tropospheric Ozone than Human Activity, Indicated by a Deep Learning Approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13307, https://doi.org/10.5194/egusphere-egu23-13307, 2023.

EGU23-13544 | ECS | Posters on site | BG1.2

Seasonal skew of tropical savanna fires 

Tom Eames, Jeremy Russell-smith, Cameron Yates, Roland Vernooij, and Guido van der Werf

Tropical savannas and grasslands are the most frequently burned biome in the world, and fire constitutes an important part of the ecosystem. In this ecosystem it can have both rejuvenating and destructive effects, depending on several factors including fuel conditions, weather conditions, and time of year. For centuries humanity has used fire in these landscapes for hunting, land clearance, agriculture, and most recently carbon offsetting. Land managers in locations with a monsoonal climate and frequent fire regimes such as tropical savannas use prescribed burning as a management tool in the ‘early dry season’ (EDS) shortly after the last rains of the year. Fires at this time tend to be cooler, restricted to surface level and less severe, meaning they can be controlled more easily and tend to go out at night without external input. Commonly a specific, fixed date is used to indicate when this window of safe burning has expired, set based on experience of the local or regional authority. In this work, we have defined a method of determining when this window expires on the basis of active fire hotspot data from the twin MODIS instruments from 2001 through to 2021. By using the relationship between day and night-time active fire detections, we set a flexible date for the transition between the early and late dry seasons in fire-prone savannas globally in the five major tropical savanna regions - Northern & Southern hemisphere South America (NHSA & SHSA), Northern & Southern hemisphere Africa (NHAF & SHAF), and Australia (AUST). The variability across each region was high (lowest mean standard deviation annually was 24 days in NHAF and highest was 56 in AUST). The fraction of area burned in the late dry season ranged from 15% (SHSA) to as high as 85% (AUST) on average, with many parts of Africa and Australia especially showing a significant skew towards the late dry season. This suggests potential for implementation of prescribed burning programmes to increase the amount of desirable fire in the global savanna ecosystems.

How to cite: Eames, T., Russell-smith, J., Yates, C., Vernooij, R., and van der Werf, G.: Seasonal skew of tropical savanna fires, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13544, https://doi.org/10.5194/egusphere-egu23-13544, 2023.

EGU23-13603 | ECS | Orals | BG1.2

Simulating wildfire impacts on boreal forest structure over the past 20,000 years since the Last Glacial Maximum in Central Yakutia, Siberia 

Ramesh Glückler, Josias Gloy, Elisabeth Dietze, Ulrike Herzschuh, and Stefan Kruse

Even though wildfires are an important ecological component of larch-dominated boreal forests in eastern Siberia, intensifying fire regimes may induce large-scale shifts in forest structure and composition. Recent paleoecological research suggests that such a state change, apart from threatening human livelihoods, may result in a positive feedback on intensifying wildfires and increased permafrost degradation [1]. Common fire-vegetation models mostly do not explicitly include detailed individual-based tree population dynamics. However, setting a focus on patterns of forest structure emerging from interactions among individual trees in the unique forest system of eastern Siberia may provide beneficial perspectives on the impacts of changing fire regimes. LAVESI (Larix Vegetation Simulator) has been previously introduced as an individual-based, spatially explicit vegetation model for simulating fine-scale tree population dynamics [2]. It has since been expanded with wind-driven pollen dispersal, landscape topography, and the inclusion of multiple tree species. However, until now, it could not be used to simulate effects of changing fire regimes on those detailed tree population dynamics.

We present simulations of annually computed tree populations during the past c. 20,000 years in LAVESI, while applying a newly implemented fire module. Wildfire ignitions can stochastically occur depending on the monthly fire weather. Within the affected area, fire intensity is mediated by surface moisture. Fire severity depends on the intensity, with scaled impacts on trees, seeds and the litter layer. Each tree has a chance to survive wildfires based on a resistivity estimated from its height and species-specific traits of bark thickness, crown height, and their ability to resprout. The modelled annual fire probability compares well with a local reconstruction of charcoal influx in lake sediments. Simulation results at a study site in Central Yakutia, Siberia, indicate that the inclusion of wildfires leads to a higher number of tree individuals and increased population size variability compared to simulations without fires. In the Late Pleistocene forests establish earlier when wildfires can occur. The new fire component enables LAVESI to serve as a tool to analyze effects of varying fire return intervals and fire intensities on long-term tree population dynamics, improving our understanding of potential state transitions in the Siberian boreal forest.

References:

[1] Glückler R. et al.: Holocene wildfire and vegetation dynamics in Central Yakutia, Siberia, reconstructed from lake-sediment proxies, Frontiers in Ecology and Evolution 10, 2022.

[2] Kruse S. et al.: Treeline dynamics in Siberia under changing climates as inferred from an individual-based model for Larix, Ecological Modelling 338, 101–121, 2016.

How to cite: Glückler, R., Gloy, J., Dietze, E., Herzschuh, U., and Kruse, S.: Simulating wildfire impacts on boreal forest structure over the past 20,000 years since the Last Glacial Maximum in Central Yakutia, Siberia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13603, https://doi.org/10.5194/egusphere-egu23-13603, 2023.

EGU23-13941 | Orals | BG1.2 | Highlight

Wildfires, chromium and freshwater quality at tropical ultramafic catchments : A prospective study on laboratory-heated soils from New Caledonia 

Farid Juillot, Gael Thery, Cecile Quantin, Quentin Bollaert, Michael Meyer, Thomas Quiniou, Philippe Jourand, Marc Ducousso, Emmanuel Fritsch, and Guillaume Morin

During the last decade, the world faced record-breaking giant fires as observed in Australia and California, a trend that is expected to increase in the forthcoming years due to climate change (Palinkas, 2020; Sharples et al., 2016; van Oldenborgh et al., 2021). In addition to their large ecological impacts, wildfires are more and more regarded for their potential threat to human health through air pollution (Xu et al., 2020). However, water pollution resulting from wildfires represents an underestimated pathway for wildfires-induced health risk (Abraham et al., 2017). This latter impact is related to the heat generated by wildfires that can propagate towards several centimeters in the soil and transform/destroy soil components. In addition to weakening soil physical stability, such transformation/destruction can change the speciation of potentially toxic elements (PTEs) that are associated with these soil components, leading to enhanced mobility towards waterways (Abraham et al., 2017; Terzano et al., 2021). One notable PTE is chromium, which is naturally present in soils mostly as trivalent Cr(III), but can represent an environmental and health issue when occurring as hexavalent Cr(VI). Recent studies reported Cr(III) oxidation to Cr(VI) upon laboratory-heating of Cr(III)-doped Fe-oxyhydroxides (Burton et al., 2019a; 2019b). Besides, Cr(III) oxidation to Cr(VI) upon controlled heating was also demonstrated for different types of soils (Burton et al., 2019b; Rascio et al., 2022; Thery et al., 2023). All these considerations suggest a significant effect of wildfires on Cr(III) oxidation to Cr(VI) in soils, with a possible influence on Cr mobility that could further impact freshwater quality. This risk of freshwater Cr(VI) pollution is expected to particularly concern ultramafic catchments because of the related occurrence of Cr-rich soils.

We have tried to address this question by performing laboratory-heating of several soils types (Ferralsols, Cambisols and Vertisols) developed on various geological settings (ultramafic, mafic and volcano-sedimentary) in New Caledonia, a French overseas territory which is a good representative of wildfires-threatened tropical ultramafic catchments (Toussaint, 2020). The results obtained revealed a significant influence of soil heating on Cr(III) oxidation to Cr(VI), followed by an enhanced Cr(VI) mobility, in all soil types. However, the magnitude of Cr(III) to Cr(VI) oxidation and Cr mobility depended on the actual nature of the soil, Ferralsols showing the highest Cr(VI) release compared to Cambisols and Vertisols. These differences were further interpreted on the basis of the changes in Cr speciation (including redox) induced by laboratory-heating of the investigated soils, as revealed by synchrotron-based X-ray absorption spectroscopy analyses. Finally, a simple risk assessment relying on the hypothesized concentration of suspended particulate matter (SPM) issued from burned soils in the related waterways allowed to emphasize a risk of wildfires-induced freshwater Cr(VI) pollution for ultramafic catchments composed of Ferralsols (Thery et al., 2023). Beyond the single case of New Caledonia, the results of this study point to the need to foster collaborative studies in order to further evaluate this risk of wildfires-induced freshwater Cr(VI) pollution at tropical ultramafic catchments on a global scale.

How to cite: Juillot, F., Thery, G., Quantin, C., Bollaert, Q., Meyer, M., Quiniou, T., Jourand, P., Ducousso, M., Fritsch, E., and Morin, G.: Wildfires, chromium and freshwater quality at tropical ultramafic catchments : A prospective study on laboratory-heated soils from New Caledonia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13941, https://doi.org/10.5194/egusphere-egu23-13941, 2023.

EGU23-14211 | ECS | Posters on site | BG1.2

Impact of biomass burning on the chemical composition of Arctic aerosols using mass spectrometry 

Yvette Gramlich, Karolina Siegel, Sophie L. Haslett, Radovan Krejci, Paul Zieger, and Claudia Mohr

Biomass burning releases numerous aerosol particles into the air, influencing the radiative budget by scattering or absorbing solar radiation and by influencing cloud properties through acting as cloud condensation nuclei. These aerosol particles contain black and organic carbon and can be transported over large distances, reaching also pristine environments such as the Arctic. Due to the rising global temperature the fire activity has increased, and record-breaking black carbon concentrations have been observed in the Arctic (Stohl et al., 2007). Biomass burning events reaching the Arctic have been observed to increase the aerosol number concentration by about one to two orders of magnitude (Lathem et al., 2013). Although a lot of attention has been drawn to the physical characteristics of fire plumes, changes in chemical composition, specifically in the Arctic, are studied to a lesser extent. In this study we report molecular-level information on the chemical characteristics of biomass burning aerosol particles measured during different plumes reaching the island of Svalbard during 2020. These measurements were part of the year-long NASCENT (Ny-Ålesund aerosol cloud experiment; Pasquier et al., 2022) campaign, and were conducted using a filter inlet for gases and aerosols coupled to a high-resolution time-of-flight mass spectrometer (FIGAERO-CIMS) using iodide as reagent ion. We use the particle-phase levoglucosan, a well-known tracer for biomass burning released from cellulose combustion, obtained from the FIGAERO-CIMS to identify biomass burning events, and will discuss the chemical characteristics of the properties of the events compared to non-events and implications for aerosol radiative and hygroscopic properties. In addition to a better understanding of the chemical composition of aged fire plumes reaching the Arctic, our study will also give insights on the time scales on which the background Arctic air can be disturbed by fire activity. 

References:
Stohl et al., Atmospheric Chem. Phys., 7, 511–534, 2007
Lathem et al., Atmospheric Chem. Phys., 13, 2735–2756, 2013
Pasquier et al., Bull. Am. Meteorol. Soc., 103, E2533–E2558, 2022

How to cite: Gramlich, Y., Siegel, K., Haslett, S. L., Krejci, R., Zieger, P., and Mohr, C.: Impact of biomass burning on the chemical composition of Arctic aerosols using mass spectrometry, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14211, https://doi.org/10.5194/egusphere-egu23-14211, 2023.

EGU23-15549 | ECS | Posters on site | BG1.2

Regional precipitation variability modulates Holocene fire history of Iceland 

Nicolò Ardenghi, Gifford H Miller, Áslaug Geirsdóttir, David J Harning, Jonathan H Raberg, Thor Thordarson, and Julio Sepúlveda

We present the first continuous Holocene fire record of Iceland from a lacustrine archive in the northeast region. We use pyrogenic PAHs (polycyclic aromatic hydrocarbons) to trace shifts in fire regimes, paired to a continuous record of n-alkanes, faecal sterols, perylene, biogenic silica, and 13C, as proxies for soil erosion, lake productivity, and human presence.

Paleoclimate research across Iceland provides a template for changes in climate across the northern North Atlantic. The role of orbitally driven cooling, volcanism, and human impact as triggers of local environmental changes, such as fire and soil erosion, is debated. While there are indications that human impact could have reduced environmental resilience in a context of deteriorating climatic conditions, it is still difficult to resolve to what extent human and natural factors affected Iceland landscape instability, due also to a lack of data on natural fire regime prior and during human colonisation.

Pyrogenic PAHs can be formed during the incomplete combustion of biomass initiated by humans or natural wildfires. Factors such as fire temperature, biomass typology, and source distance can strongly affect pyrogenic PAH molecular weight and spatial distribution.
Faecal sterols/stanols and their ratios have been used in archaeological and paleoclimate studies to detect human and/or livestock/herbivore waste. The absence of large herbivorous mammals and humans in Iceland prior to settlement means that increases in the occurrence of faecal sterols and bile acids over natural background values should mark the arrival of humans and associated livestock in the catchment, which could be traced regionally.

Our results indicate that the Icelandic fire regime during the Holocene followed four main phases. Among these, a very long period centred around the Holocene climatic optimum (ca 9.5 – 4.5 ka BP) was characterised by a generally low frequency fire regime, both in the lake catchment as in the whole north-eastern Iceland. This same period was also marked by relatively low background levels of faecal sterols/stanols. At 4.5 ka BP a new phase started, with a general increase of all PAHs values. According to both our PAH and sterol data, there is no apparent human signal around the 9th century C.E., where an increase in man-made fires would likely be expected in connection to the historical data of Viking colonisation of Iceland (870s C.E.), suggesting that fire regimes have primarily been controlled by natural factors.
In addition, the pyrogenic PAHs record also differs from the trend of a general stepwise climatic “deterioration” previously highlighted by other lake proxies throughout Iceland, linked to decreasing summer insolation and related cooling, as highlighted also by our other proxies.

A comparison to recent palynological data from a nearby site and to δD data from the NW region suggest shifts in NAO regimes as the main forcing behind shifting fire regimes in Iceland. Changes in precipitation regimes would have determined shifts in the composition of the regional vegetational community, increasing fuel availability and flammability with decreasing precipitation, leading to widespread low temperature fires, easily trigged by frequent volcanic episodes.

How to cite: Ardenghi, N., Miller, G. H., Geirsdóttir, Á., Harning, D. J., Raberg, J. H., Thordarson, T., and Sepúlveda, J.: Regional precipitation variability modulates Holocene fire history of Iceland, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15549, https://doi.org/10.5194/egusphere-egu23-15549, 2023.

EGU23-15670 | ECS | Orals | BG1.2 | Highlight

Identifying tipping points and threshold values for ecosystem functioning in northern peatlands during the climate crisis (PEATFLAMES) 

Luke Andrews, Michał Słowiński, Harry Roberts, Katarzyna Marcisz, Piotr Kołaczek, Agnieszka Halaś, Dominika Łuców, and Mariusz Lamentowicz

Peatlands are globally important carbon sinks and stores. Climate change threatens to alter carbon cycling in some regions of the Northern Hemisphere, causing them to become net sources of atmospheric carbon, exerting a positive feedback upon global climate. Furthermore, enhanced drying, increased human activity and vegetation succession in response to a warming climate have increased the frequency of wildfires in some peat-bearing regions, including areas underlain by permafrost. Such events can cause thousands of years’ worth of formerly stable carbon to be rapidly released into the atmosphere, imparting further climate warming.

 

The future response of peatlands to climate warming and wildfire remains uncertain, and as a result peatlands are rarely included in Earth System Models, despite their importance in the global carbon system. Understanding how changes in climate and anthropogenic activity in the past affected peatland ecosystem functioning will improve our understanding of how these sensitive ecosystems may respond to future projected changes and thus reduce this uncertainty.

 

Our project aims to assess how warming, drought and wildfire have impacted the resilience of peatlands and permafrost in the Northern Hemisphere over the past c. 2000 years. Several peat cores spanning a latitudinal gradient covering several regions including Russia, Poland, the Baltic states and Scandinavia will be analysed using multiple palaeoecological proxies at high resolution to reconstruct past changes in wildfire frequency, hydrology and vegetation. This will allow us to define baselines and threshold values for ecosystem shifts relevant to future projected changes in climate.

 

How to cite: Andrews, L., Słowiński, M., Roberts, H., Marcisz, K., Kołaczek, P., Halaś, A., Łuców, D., and Lamentowicz, M.: Identifying tipping points and threshold values for ecosystem functioning in northern peatlands during the climate crisis (PEATFLAMES), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15670, https://doi.org/10.5194/egusphere-egu23-15670, 2023.

EGU23-16152 | Posters on site | BG1.2

Temporal analysis of wildfire emissions in the Northwest of Spain using ESA CCI data 

Patricia Oliva and César Quishpe

The Northwest of the Iberian Peninsula is one of the European regions with the highest frequency of forest fires. However, in the last decade fires in this region have burned larger areas and later in the fire season. Assessing the damage caused by fire and the pollutants released in the burning process is important to understand the effects on ecosystems and the carbon cycle, the recurrence of fires, and the effect on human health. In this work, we performed the estimation of emissions released in Galicia (Northwest Spain) in the last six years combining existing ESA CCI products. To quantify the area burned, we used the products from the Burned Area Algorithm developed within the Fire Climate Change Initiative (FireCCI) project. Then, the characterization and quantification of the total biomass were obtained from the Biomass CCI project at 100 m resolution by extracting the mean biomass by vegetation type from CORINE Land cover 2018. The burning efficiency factor was fitted using burn severity estimates from the dNBR calculation on the Sentinel-2 data. The emissions factors were selected from the literature. Our results show that during the last few years, there is a positive trend of annual emissions in Galicia. The sporadic maximums were registered in the years 2017 and 2022 when the climatic conditions aggravated the fire behaviour. In addition, Galicia is the region of Spain that registers the highest average estimates of emissions from fires since a high percentage of the affected area is occupied by pine and eucalyptus forests. These emissions contribute to a drastic decrease in air quality influencing the climate and affecting public health. Finally, we verified that adapting the burning efficiency factors to the specific conditions of the affected ecosystem generates more precise emission estimates.

How to cite: Oliva, P. and Quishpe, C.: Temporal analysis of wildfire emissions in the Northwest of Spain using ESA CCI data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16152, https://doi.org/10.5194/egusphere-egu23-16152, 2023.

EGU23-16241 | ECS | Posters virtual | BG1.2

Characterizing the fire regime evolution and land-use change in the Dry and Wet Chaco between 2001 and 2019 

Rodrigo San Martin, Catherine Ottle, and Anna Sörensson

Wildfires play an essential role in the biogeophysical cycles of different world ecosystems, from dry savannas to humid wetlands. During the last decades, fire regimes of several global regions began to present significant alterations due to climate change and human land-use pressure. The South American Gran Chaco ecoregion contains one of the most important reservoirs of native forests and biodiversity in the world, including the largest continuous dry tropical forest and some of the most extensive wetlands. The area presents a marked precipitation gradient from the East (wet) to the West (dry), which is manifested in vegetation (from wetlands to dry forests and shrublands). In this work, we mapped natural vegetation with the European Space Agency (ESA) Climate Change Initiative (CCI) medium-resolution land cover maps (MRLC v2.0.7; annual - 300m) and fires with the ESA CCI Fire product (FireCCI51; monthly - 250m) in the Gran Chaco between 2001 and 2019 to establish the past and current effects and dynamics of fires in the area (which are primarily human ignited). To assess the region’s climatology, we used the ERA5 bias-corrected reanalysis dataset (WFDE5; daily - 0.5º). Our results highlight the distinct dynamics of fires in the wet and dry areas of the Gran Chaco, showing two fire seasons - summer and winter - in the wet areas (where grasses predominate) and one fire season - winter - in the dry areas (where shrubs and trees are more abundant). Examining the correlations between annual rain anomalies and burnt area, we find that precipitation anomalies have different effects in dry and wet areas throughout the region’s precipitation gradient. Correlations change from positive in the drier areas to negative in the wetter areas. These results may reflect that summer and winter fires do not have the same drivers and the key role of the available biomass limiting the fire expansion. Since biomass is more dependent on precipitation in dry areas compared to wetter ones, the correlation of winter fires with precipitation is positive in the drier regions. The negative correlations obtained in the summer season could be explained by the fact that summer fires essentially occurred in the wetter part of the Chaco and are intended (through human ignition) to increase the grasslands’ productivity; this practice could be more frequent during negative precipitation anomalies compared to positive ones. Further analysis will try to confirm these findings with biomass satellite data.   

How to cite: San Martin, R., Ottle, C., and Sörensson, A.: Characterizing the fire regime evolution and land-use change in the Dry and Wet Chaco between 2001 and 2019, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16241, https://doi.org/10.5194/egusphere-egu23-16241, 2023.

EGU23-16504 | Posters on site | BG1.2

History of fire regime shifts during the last 1000 years in Northeastern Mongolia 

Michał Słowiński, Milena Obremska, Dashtseren Avirmed, Michał Woszczyk, Saruulzaya Adiya, Dominika Łuców, Agnieszka Mroczkowska, Agnieszka Halaś, Witold Szczuciński, Andrzej Kruk, Mariusz Lamentowicz, Joanna Stańczak, and Natalia Rudaya

Recent years have seen rapid climatic changes in Central Asia, particularly Mongolia. An increase in the thickness of the active layer above permafrost and considerable changes to the vegetation structure are likely outcomes of the long-term temperature rise and precipitation changes. The management of future habitats or the biodiversity of northern Mongolia faces significant difficulties from rising temperatures, prolonged and frequent droughts, and gradual permafrost degradation. Our knowledge of the historical processes involved in permafrost degradation and the ensuing ecological effects is still mostly incomplete. These connections may be used to explain changes in the fire regime, permafrost melting, and plant distribution in the Khentii mountains region. Therefore, based on a multiproxy study of peat archive data, we provide the first high-resolution fire history from northeastern Mongolia over the last 1000 years (micro- and macroscopic charcoals, charcoal size classes and morphotypes, peat geochemistry). We examined microscopic and macroscopic charcoal particles as a proxy for fire activity. We also tracked changes in regional and local plant composition using pollen data. To investigate how changes in fire regimes and the climate affect the functioning of the peatland ecosystem, we also conducted a geochemical analysis.

Additionally, to better comprehend the changes in earlier fire regimes and fire-vegetation connections, we employed the morphotypes of macrocharcoal to pinpoint vegetation burning. This study's primary objective is to evaluate the impact of human behavior, vegetation, and prolonged droughts on the incidence of fire regime transitions during the past 1000 years in Central Asia permafrost marginal zone (Mongolia). The findings showed that most of the fires in the area were probably started by natural causes, presumably connected to heatwaves that resulted in prolonged droughts. We have established a connection between increased fires and the local weather phenomena known as "dzud", a catastrophic confluence of winter snowfall and droughts that impacts fire intensity.

The study is the result of research project No. 2017/01/X/ST10/01216 and 2018/31/B/ST10/02498 funded by the Polish National Science Centre.

How to cite: Słowiński, M., Obremska, M., Avirmed, D., Woszczyk, M., Adiya, S., Łuców, D., Mroczkowska, A., Halaś, A., Szczuciński, W., Kruk, A., Lamentowicz, M., Stańczak, J., and Rudaya, N.: History of fire regime shifts during the last 1000 years in Northeastern Mongolia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16504, https://doi.org/10.5194/egusphere-egu23-16504, 2023.

EGU23-16912 | ECS | Posters on site | BG1.2

Fire, Work with Me: A PAH record from a Southwestern US speleothem 

Jonathan Smolen, Isabel Montañez, and Michael Hren

Polycyclic aromatic hydrocarbons (PAHs) are molecules produced during incomplete combustion of organic matter and have been increasingly utilized as paleo-proxies for wildfires. More recently, their incorporation from drip water into speleothems has been utilized in conjunction with the stable isotopic and trace elemental measurements of host carbonate and fluid inclusions in order to assess a coupled record of fire and hydroclimate. Numerous studies have focused on cave systems in the Southwestern U.S., which has experienced highly variable hydroclimate and massive wildfires with past climate changes. Here, we present a PAH record covering ~19-11.5 ka obtained from a precisely dated and well-studied ML-1 stalagmite obtained from McLean’s Cave in the central Sierran foothills, CA. Total concentrations of four-ring PAHs reach maximum values from ~16.8-15 ka, associated with the first stage (1a) of Heinrich Stadial 1 (HS1) interval – this is interpreted as increased levels of soil PAHs produced from regional wildfires. Covariance of isomeric diagnostic ratios with total concentration indicates a shift in the nature of the associated fires, separating effects of PAH mobility in altered soils as well as shifts in soil water transport, stalagmite growth rates, and precipitation amounts. Paired climate signals from independent regional proxies are discussed, as well as factors affecting the interpretation of PAH signals in speleothems. Considerations and methods using small (~1g) speleothem samples are presented, with a focus on simultaneous extraction of useful paleoenvironmental information from other molecular biomarkers entombed within speleothems.

How to cite: Smolen, J., Montañez, I., and Hren, M.: Fire, Work with Me: A PAH record from a Southwestern US speleothem, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16912, https://doi.org/10.5194/egusphere-egu23-16912, 2023.

EGU23-17450 | ECS | Orals | BG1.2 | Highlight

First results of a field campaign focused on overwintering zombie fires 

Thomas D. Hessilt, Sander Veraverbeke, Emily Ogden, Jason Paul, Merritt Turetsky, Max van Gerrevink, Raquel Alfaro-Sanchez, Oleg Melnik, Rebecca C. Scholten, and Jennifer Baltzer

Fire is a major disturbance in the boreal forests of the high northern latitude. Fire extent and severity have been increasing in recent decades, and the occurrence of overwintering ‘zombie’ fires has been linked to recent fire extremes. Overwintering fires are fires which were seemingly extinguished at the end of the boreal fire season yet smolder during winter to re-emerge as a flaming fire in the subsequent spring. So far, overwintering fires have only been investigated using satellite imagery. Here, for the first time, we show preliminary results from a field campaign that measured in situ impacts of fires that overwintered from 2014 to 2015 in the Canadian Northwest Territories. We measured among other the burn depth in organic soils, and characterized micro-topography. We also qualitatively assessed how fires may have overwintered. We compared nine overwintering fire sites, which burned during both 2014 and 2015, with six sites that only burned in 2014 and five nearby unburned sites. The average burn depth (±SD) of the overwintering fires was 6.8 ± 1.6 cm and significantly deeper compared to 6.1 ± 1.2 cm in the single fire sites (P < 0.01). Somewhat surprisingly, the majority of overwintering fires occurred in mesic sites with large productive trees. Only two overwintering sites were sampled in mesic-subhygric to subhygric sites dominated by black spruce (Picea mariana). The unburned control sites often featured a micro-topography of hummocks and hollows. This micro-topography was leveled in overwintering fires sites because of severe burning in organic soils. In overwintering sites, most of the organic layer was consumed. This may have led to prolonged smoldering in the root systems of trees. Our results are the first to quantify the burn depth of overwintering fires, and also show that overwintering does not only happen through deep smoldering in organic soils, yet can also occur from smoldering in tree boles and root systems of burned and fallen trees.

How to cite: Hessilt, T. D., Veraverbeke, S., Ogden, E., Paul, J., Turetsky, M., van Gerrevink, M., Alfaro-Sanchez, R., Melnik, O., Scholten, R. C., and Baltzer, J.: First results of a field campaign focused on overwintering zombie fires, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17450, https://doi.org/10.5194/egusphere-egu23-17450, 2023.

EGU23-1227 | Posters virtual | AS4 .8

Accumulation of atmospheric metal and nitrogen deposition in mosses 1990-2020, comparison with emission data and tree canopy drip effects 

Winfried Schröder, Stefan Nickel, Annekatrin Dreyer, and Barbara Völksen

Mosses are suitable for recording the bioaccumulation of atmospheric deposition over large areas at many sites. In Europe, such monitoring has been carried out every five years since 1990. Mosses have been collected and chemically analysed for metals (since 1990), nitrogen (since 2005), persistent organic pollutants (since 2010) and microplastics (2020). The aims of this study were: 1. To analyse the temporal trends of metal and nitrogen accumulation in mosses between 1990 or 2005, respectively, and 2020 in Germany; 2. To compare the accumulation trends with emission data; and 3. To determine the effect of tree canopy drip on metal and nitrogen accumulation in mosses. For the temporal trend analysis, the minimum sample number required for a reliable estimation of arithmetic mean values and statistical parameters based on it was calculated. It was only achieved for nitrogen, but not for metals. Therefore, the temporal trends of bioaccumulation of metals and nitrogen were calculated on the basis of median values. For the analyses of tree canopy effects on elements accumulation in mosses, 14 vegetation structure measures were used, which together with 80 other descriptors characterise each moss collection site and its environment. The comparison of the data obtained during the first monitoring campaign with those of the 2020 survey showed a significant decrease in metals bioaccumulation. However, in contrast to the emission data, an increase in accumulation of some metals was observed between 2000 and 2005 and of all metals from 2015 to 2020. Trends in Germany-wide nitrogen medians over the last three campaigns (2005, 2015, 2020) show that nitrogen medians decreased by -2% between 2005 and 2015 and increased by +8% between 2015 and 2020. These differences are not significant and do not match the emission trends. Inferential statistics confirmed significantly higher metal and nitrogen accumulation in mosses collected under tree canopies compared to adjacent open areas. Measured concentrations of metals and nitrogen were significantly higher under tree canopies than outside of them, by 18-150 %.

Keywords: Bioaccumulation; regression analysis; trend analysis

How to cite: Schröder, W., Nickel, S., Dreyer, A., and Völksen, B.: Accumulation of atmospheric metal and nitrogen deposition in mosses 1990-2020, comparison with emission data and tree canopy drip effects, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1227, https://doi.org/10.5194/egusphere-egu23-1227, 2023.

EGU23-2323 | Posters on site | AS4 .8

Using atmospheric models to simulate backward certain gases that are the result of illegal activities and locate the source 

Damianos Mantsis, Ilias Gialampoukidis, Stefanos Vrochidis, Theodora Tsikrika, and Ioannis Kompatsiaris

Illegal activities such as the manufacturing of home-made explosives may result in the dispersion of certain type of gases in the atmosphere or water pollutants. Our study addresses the methodology that can be used to track the source location of these gases after they have been detected. Traditionally, tracking the source location of a gas release requires the knowledge of the emission maps, however, given the nature of the task, this is unknown in our case. Our methodology, does not involve inverse modeling, and only requires the use of a network of instruments on the ground or mounted on aerial vehicles. The FLEXPART-WRF Lagrangian dispersion model is used to backward simulate the dispersion and transport of the gases at 0.5-1 Km horizontal resolution. The numerical experiments take place at two different geographical regions, i.e. one with strong topography and another over plain terrain with no topography, and over a wide range of meteorological conditions. Our results indicate that 5 to 10 ground measurements are enough to locate the source with an accuracy of a few kilometers. Identifying the time of the release, on the other hand, is more challenging especially if the initial release of the gas does not take place instantly and is gradual.

How to cite: Mantsis, D., Gialampoukidis, I., Vrochidis, S., Tsikrika, T., and Kompatsiaris, I.: Using atmospheric models to simulate backward certain gases that are the result of illegal activities and locate the source, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2323, https://doi.org/10.5194/egusphere-egu23-2323, 2023.

EGU23-2660 | Orals | AS4 .8

Microplastics and Persistent organic pollutants in moss samples from Germany 

Carmen Wolf, Mike Wenzel, Annekatrin Dreyer, Winfried Schroeder, Stefan Nickel, Barbara Voelksen, Christine Kube, and Jochen Tuerk

Introduction: Following their transport, atmospheric pollutants are deposited on the ground, on plants or on water. Depending on the substances involved, ecosystems can be adversely affected by the deposition of nutrients or pollutants. In order to be able to counteract the potential ecological risks through environmental policy measures, it is necessary to measure the atmospheric inputs of potentially harmful substances. For this reason, heavy metal concentrations in mosses used as accumulators of atmospherically deposited substances have been determined since 1990 for every five years at up to 7300 locations in up to 34 European countries. In 2005 nitrogen was added. Persistent organic compounds were determined for the first time in the European Moss Survey in 2010, in Germany firstly in the Moss Survey of 2015/2016. Microplastics were added to this group of substances for the 2020/2021 survey. Here, we are presenting results for microplastic and a variety of persistent organic pollutants (POP) from the 2020/2021 moss survey in Germany. Materials and Methods: Sampling was performed at 20 sites according to the recommendations of the Moss Survey Manual. Afterwards a sample preparation method was established for Thermo-Extraction-Desorption-GC-MS and RAMAN spectroscopy to analyze the microplastic concentration as well as number in the moss samples. Analyses for POPs were performed as described by Dreyer et al. 2018 with slight modifications. Overall, about 120 compounds (PAH, PCDD/F, PCB, PFAS, HBCD, PBB, PBDE, alternative halogenated flame retardants (HFR)) were analysed. Results: In all Moss samples microplastic were detected. The highest concentration in all samples was observed for polyethylene, followed by polyethylene terephthalate, polypropylene and styrene-butadiene and in one sample polystyrene. At the two sampling sites near the sea the highest microplastic concentrations were indicated, whereas no correlation with the other sampling location (urban, agriculture, forest) could be detected. PBB and indicator PCB were not observed above the LOQ in any sample. PFAS and dioxin-like PCBs were very rarely found above the LOQ. In contrast, certain PCDD/F, PAH, HBCD, PBDE and HFR were frequently observed. Current concentrations at sampling sites compared to those of sites that have also been investigated in 2015/2016 were in the same order of magnitude or declined. For HBCD, concentrations declined distinctly by a factor of up to 9. Conclusions: Microplastics and many POPs were observed in moss samples indicating their suitability to monitor atmospheric deposition of these substance groups by this bioindicator. Challenges exist for PBB, PCB or PFAS either because environmental concentrations are too low with respect to the LOQ or the pollutants’ environmental behavior limit accumulation in moss. Within the past five years, most POPs concentrations in moss samples from Germany stayed more or less the same or decreased.

Acknowledgements:

We are thankful to the German Environment Agency (Umweltbundesamt) for funding this study (FKZ 3720632010).

 References:

  • UNECE ICP VEGETATION (2020) Heavy metals, nitrogen and POP in European mosses: 2020 survey monitoring manual. https://icpvegetation.ceh.ac.uk/sites/default/files/ICP%20Vegetation%20moss% 20monitoring %20manual %202020.pdf
  • Dreyer A, Nickel S, Schröder W. et al. (2018). Environ. Sci. Eur. 30 (43): 1-14.

How to cite: Wolf, C., Wenzel, M., Dreyer, A., Schroeder, W., Nickel, S., Voelksen, B., Kube, C., and Tuerk, J.: Microplastics and Persistent organic pollutants in moss samples from Germany, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2660, https://doi.org/10.5194/egusphere-egu23-2660, 2023.

EGU23-3129 | Orals | AS4 .8

Rime – a non-negligible pathway of sulphur and nitrogen atmospheric deposition in middle-elevated Central European mountains   

Iva Hunova, Martin Novak, Pavel Kurfürst, Hana Skachova, Marketa Stepanova, Arnost Komarek, Jan Curik, Frantisek Veselovsky, Eva Prechova, and Leona Bohdalkova

Rime is an under-researched pathway of the atmospheric deposition of ecological and environmental relevance, in particular in mountain regions. Rime alongside with snow were sampled and assessed for S-SO42- and N-NO3- at ten border mountaintop sites across the Czech Republic (CR) in the three consecutive winters of 2009–2011. Our observations indicated significantly higher sulphur (S) and nitrogen (N) contents in rime as compared to snow at all sites.  Whereas the highest S contamination was found in the industrial North, the highest N contamination was found unexpectedly in the relatively unpolluted South. The measurements were put in context with data driven geo-spatial modeling results (Hůnová et al., 2016) of annual wet vertical (rain and snow) and horizontal (fog and rime) deposition. Despite relatively low hydrological input of rime, it contributed significantly to annual atmospheric deposition. At nine out of ten sites, the winter-time deposition of S via rime corresponded to 5–13% of annual wet-only S deposition, while it reached full 25% at the most S-polluted TET site in the Orlicke hory Mts., a region bordering Poland (Hůnová et al., 2022). Modelled results showed that mean winter rime deposition corresponded to about 6–25%, and mean winter snow deposition made up 25–72.5% of mean annual N-NO3- wet-only deposition (Hůnová et al., submitted). Model N-NO3-occult deposition estimated from throughfall and total (wet and dry) deposition is highly uncertain, however: N throughfall is not a relevant proxy for estimation of realistic total N deposition due to N exchange between the tree canopy and atmosphere.  Considering the fact that wet-only deposition is a year-long phenomenon, whereas rime forms under the climatological conditions of the Czech middle elevated mountains during only a few (2–3) months a year, we can conclude that the rime deposition pathway should not be neglected in quantifying the real atmospheric deposition flux in mountain regions as it might contribute to the real deposition flux substantially even in mountains of medium elevation, as was observed in the CR.

References:

Hůnová I., Kurfürst P., Vlček O., Stráník V., Stoklasová P., Schovánková J., Srbová D., 2016. Towards a Better Spatial Quantification of Nitrogen Deposition: A Case Study for Czech Forests. Environmental Pollution 213, 1028–1041. doi: 10.1016/j.envpol.2016.01.061.

Hůnová I., Novák M., Kurfürst P., et al., 2022. Contribution of rime to atmospheric sulphur deposition in Central Europe: A combined empirical and modelling approach. Atmospheric Environment 270, 118877. https://doi.org/10.1016/j.atmosenv.2021.118877.

Hůnová I., Novák M., Kurfürst P., et al., submitted. Comparison of vertical and horizontal atmospheric deposition of nitrate at Central European mountain-top sites during three consecutive winters.

How to cite: Hunova, I., Novak, M., Kurfürst, P., Skachova, H., Stepanova, M., Komarek, A., Curik, J., Veselovsky, F., Prechova, E., and Bohdalkova, L.: Rime – a non-negligible pathway of sulphur and nitrogen atmospheric deposition in middle-elevated Central European mountains  , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3129, https://doi.org/10.5194/egusphere-egu23-3129, 2023.

EGU23-3358 | ECS | Posters virtual | AS4 .8

Underestimation of potassium in forest dry deposition? – A simulation experiment in rural Germany 

Andreas Schmitz, Bernd Ahrends, Hartmut Herrmann, Alexander Moravek, Laurent Poulain, Tanja Sanders, Alfred Wiedensohler, and Andreas Bolte

Measurements of throughfall (TF) and wet deposition (WD) are a common method to assess nitrogen (N) and base cation (BC) deposition to forests. Using TF and WD, dry deposition (DD) is usually calculated with a canopy budget model (CBM) assuming similar BC to Na+ ratios in WD and DD. This assumption is especially uncertain for K+, since K+ is often bound to smaller particles compared to Na+. Here we asses this assumption by comparing the DD of K+ estimated with the CBM (DDKCBM) to the DD of K+ simulated with a process oriented DD model (“inferential model”, DDKINF). Simulation experiments were performed at two indicator forest stands (“virtual” broadleaved (BL) and coniferous (CF) forest) based on six years of daily PM2.5 and PM10 concentrations and weekly WD observations measured at the rural background research station Melpitz, Germany. On average, the K+:Na+ ratio in WD was 0.24 while the K+:Na+ ratio in DDINF was 0.43 (CF) and 0.40 (BL), respectively. Accordingly, DDKCBM would need to be multiplied by a correction factor of 1.77 (CF) and 1.66 (BL) to match DDKINF, with substantial variation between years (lowest correction factor: 0.98, highest correction factor: 3.89). However, applying the correction factors in CBM calculations at nearby ICP Forests monitoring sites had only little effect on total (WD+DD) deposition rates of N and BC. The results were robust against changes in the meteorological data used for the inferential model. Uncertainty arises from periods affected by presence of particles larger than 10 µm diameter, not covered by local measurements. A corresponding lower boundary estimate for the average underestimation of DDKCBM is a correction factor of 1.37 (CF) and 1.29 (BL). More work is required to assess to what extend the observed underestimation of DDKCBM is confirmed by other methods and at sites with different atmospheric conditions.

How to cite: Schmitz, A., Ahrends, B., Herrmann, H., Moravek, A., Poulain, L., Sanders, T., Wiedensohler, A., and Bolte, A.: Underestimation of potassium in forest dry deposition? – A simulation experiment in rural Germany, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3358, https://doi.org/10.5194/egusphere-egu23-3358, 2023.

EGU23-3607 | Orals | AS4 .8

Mediating Airborne Birch Modelling and Forecasting 

Willem W. Verstraeten, Nicolas Bruffaerts, Rostislav Kouznetsov, Mikhail Sofiev, and Andy Delcloo

Air pollution contributes to increased mortality and lower quality of life. It imposes additional distress on people suffering from respiratory diseases such as pollinosis. A quarter of the adult population and a third of all children in Europe are estimated to suffer from airborne allergenic pollen. In the future even more people might be subjected to pollen allergies since changes in climate and land-use tend to increase the amount of allergenic airborne pollen and prolong the pollen seasons. Good pollen mitigation measures may ease the symptoms but it requires proper knowledge on the modelling and forecasting of allergenic pollen in the air.

We start from the setup of the pollen transport model SILAM (System for Integrated modeLling of Atmospheric coMposition), driven by ECMWF ERA5 meteorology in a bottom-up emission approach for the period 1982-2019 for the Belgian territory. The dynamic vegetation component in the pollen transport model is determined by pollen emission source maps which have to be ingested in the model for every pollen season. The used maps are derived by merging multi-decadal datasets of spaceborne NDVI with forest inventory data in a Random Forest statistical framework.

Here we study the impact of spatially-varying pollen emission sources on the modelled airborne birch pollen levels compared with in-situ observations in a Monte-Carlo approach. Preliminary analysis indicates that by selecting the model scenario corresponding with median pollen levels, the correlation between the modelled and observed pollen levels increases with 16%. We show the importance of ingesting the appropriate pollen emission source map when the modelling and forecasting of airborne birch pollen levels is aimed for. Finally, we review methods to relate the pre-pollen season meteorology or vegetation state on the birch pollen loads of the up-coming season as tool for selecting the best emission source map in the forecasting framework.

How to cite: Verstraeten, W. W., Bruffaerts, N., Kouznetsov, R., Sofiev, M., and Delcloo, A.: Mediating Airborne Birch Modelling and Forecasting, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3607, https://doi.org/10.5194/egusphere-egu23-3607, 2023.

EGU23-4400 | Posters on site | AS4 .8

Total Reactive Nitrogen Flux Monitor Using CAPS NOx Detection 

Timothy B Onasch, J. Rob Roscioli, Matt Lund, Joanne Shorter, and Andrew Freedman

We are in the process of developing a comparatively inexpensive, robust, cavity attenuated phase shift (CAPS)‐based monitor to measure total reactive nitrogen (NR) emission and deposition rates. Total reactive nitrogen comprises both particle (ammonium and nitrate based) and gas phase species such as ammonia, nitrogen oxides, and various organo‐nitrogen compounds. The monitor will be capable of partitioning the emission/deposition rates between particle and gas allowing it to adapt sampling modes to optimize the operation of the monitor.

The monitor comprises a Total Reactive Atmospheric Nitrogen Converter (TRANC) (Marx et al. 2012), the output of which is coupled to a CAPS NOx monitor. The TRANC thermally decomposes and oxidizes both non‐refractory atmospheric particles into their gas phase constituents, and any volatile nitrogen-containing gases to NO + NO2. It does so by passing the sample through an oven operating at >900 ºC which has been shown to effectively operate at the residence times (i.e., flow rates) required for emission/deposition rate measurements such as eddy covariance (Ammann et al. 2012).

The output of the TRANC is sent to a CAPS NOx monitor which uses photolytically produced ozone to oxidize NO to NO2 with >98% efficiency without further oxidation to NO3. The resultant NO2 is measured using the Cavity Attenuated Phase Shift (CAPS) technique at 405 nm, a wavelength free from interference from the ozone in the flow (Kebabian, et al. 2007; Kebabian, et al., 2008; Roscioli, et al., 2022). The CAPS NOx monitor has been shown to have a sensitivity (2s, 1s) of less than 0.2 ppb and to be highly linear over a range of 0-1000 ppb. 

                Conversion efficiencies for gas phase ammonia and a range of nitrogen-containing particulate species are shown to be within 10% of unity. Aerosolized particles were size selected with an Aerodynamic Aerosol Classifier; equivalent gas phase concentrations were calculated by measuring particle concentrations with a condensation particle counter and assuming a per particle mass.  Within experimental error, gas phase ammonia and ammonium and nitrate containing particles were completely converted to gas phase NO + NO2. This holds true over a range of particle flow rates.

 

This work is supported by NASA, the U.S. Department of Energy and the U.S. Department of Agriculture, all under the Small Business Innovation Research program.

Kebabian, P.L., W.A. Robinson and A. Freedman (2007) Rev. Sci. Instrum., 78, 063102.

Kebabian, P.L., E.C. Wood, S.C. Herndon, and A. Freedman (2008) Environ. Sci. Technol., 42:6040-6045.

Ammann, C., Wolff, V., Marx, O., Brümmer, C., and Neftel, A. (2012). Biogeosciences 9 (11):4247–4261. doi:10.5194/bg-9-4247-2012.

Marx, O., Brümmer, C., Ammann, C., Wolff, V., and Freibauer, A. (2012). Atmospheric Meas. Tech. 5 (5):1045–1057. doi:10.5194/amt-5-1045-2012.

Roscioli, J., T.B. Onasch, and A. Freedman (2022) in preparation.

How to cite: Onasch, T. B., Roscioli, J. R., Lund, M., Shorter, J., and Freedman, A.: Total Reactive Nitrogen Flux Monitor Using CAPS NOx Detection, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4400, https://doi.org/10.5194/egusphere-egu23-4400, 2023.

EGU23-7040 | ECS | Posters on site | AS4 .8

Sulfur hexafluoride emissions – critical remarks on inversion techniques and inverse model results for the past two decades 

Martin Vojta, Andreas Plach, Rona Thompson, and Andreas Stohl

Inverse modeling provides a powerful tool to verify national greenhouse gas (GHG) emission inventories by using atmospheric observations. Often, inversions are based on Lagrangian Particle Dispersion Model simulations, where virtual particles are released from observation sites and traced backwards in time to establish a relationship between atmospheric concentrations and emission sources within the simulation period. The fact, that this simulation period is limited due to computational costs, raises two essential questions: (i) How to best define a baseline, that accounts for all emissions that occur prior to the simulation period? (ii) Which period length should be chosen for the backward-simulation?

We show that often used statistical baseline methods have large problems and present a superior global-distribution-based (GDB) approach, that is consistent with the backward-simulation period, accounts for meteorological variability, and leads to inversion results that agree well with known global emission estimates. Our results further show, that longer backward-simulation periods beyond the often used 5 to 10 days increase the correlation between modeled and observed concentrations, and lead to more robust inversion results. Furthermore, they can help to better constrain emissions in regions poorly covered by the observation network.

Based on these methodological results, we perform inversions for sulfur hexafluoride (SF6) - the most potent GHG regulated under the Kyoto Protocol with an estimated atmospheric lifetime of 3200 years. The inversions are based on 50-days backward-simulations, in-situ and flask measurements from various observation networks, and the GDB baseline method, to achieve globally and regionally consistent SF6 emissions from 2005 to present.

How to cite: Vojta, M., Plach, A., Thompson, R., and Stohl, A.: Sulfur hexafluoride emissions – critical remarks on inversion techniques and inverse model results for the past two decades, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7040, https://doi.org/10.5194/egusphere-egu23-7040, 2023.

EGU23-8887 | ECS | Posters on site | AS4 .8

Vegetation losses due to surface ozone concentrations from fires in Portugal mainland 

Catarina Alonso and Célia Gouveia

Tropospheric ozone (O3) is an important anthropogenic gas, and it is a secondary air pollutant. The combination of sunlight with non-methane hydrocarbons (NMHCs) and NOx (NO + NO2) from biomass burning results in significant photochemical production of O3. Since the fire season in Portugal occurs during the summer, these emitted O3 precursors lead to the production of O3. An excessive concentration of tropospheric O3 damage leaves, decreasing photosynthesis, plant growth and biomass accumulation and costing, therefore, billions of dollars annually in lost plant productivity.

The main objective of this work is to understand if there is a relationship between the loss in crop yields due to the concentration of O3 derived from fires, in Portugal mainland. Therefore, this work is divided into three phases: i) to evaluate the relationship between tropospheric O3 and extreme fires; ii) relate the contribution of O3 to vegetation productivity contraction; and iii) relate the fire-induced O3 increments to vegetation losses. To access to tropospheric O3 concentration data Atmospheric Infrared Sounder (AIRS) and Copernicus Atmosphere Monitoring Service (CAMS) products were used. The AIRS Version 7 Level 3 product are daily, gridded mean geophysical parameters on 1°x1° grid cells, with higher internal vertical resolution at 100 pressure levels (1000 hPa – 1 hPa). The CAMS reanalysis (CAMSRA) O3 data have a temporal resolution of 3 h and a spatial resolution of approximately 80 km (0.7°x0.7° grid cells) with 60 hybrid sigma–pressure (model) levels (13 levels, 400 - 100 hPa) in the vertical (top level at 0.1 hPa).  Vegetation productivity is assessed by means of Gross Primary Production (GPP) available from Moderate Resolution Imaging Spectroradiometer (MODIS) collections. It can be concluded that when fires occur in large areas, such as the fires of 2012 (Serra do Caldeirão) and 2018 (Monchique) the levels of surface O3 concentration have a high increase, which can lead to a decrease in vegetation and crop productivity.

Acknowledgements: This study is partially supported by the European Union’s Horizon 2020 research project FirEUrisk (Grant Agreement no. 101003890) and by the Portuguese Fundação para a Ciência e a Tecnologia (FCT) I.P./MCTES through national funds (PIDDAC) – UIDB/50019/2020- IDL,  DHEFEUS - 2022.09185.PTDC

How to cite: Alonso, C. and Gouveia, C.: Vegetation losses due to surface ozone concentrations from fires in Portugal mainland, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8887, https://doi.org/10.5194/egusphere-egu23-8887, 2023.

The bushfires in Australia during the 2019/2020 season were particularly severe, leading to the creation of a plume of smoke that rose into the Lower Stratosphere and resulted in record levels of smoke concentration.  In early January 2020, the plume disperses into independent transport paths in the stratosphere. Following a Lagrangian approach, we study the three dimensional atmospheric transport in the region at this time to better understand the cause of the splitting, the subsequent transport geometry, and the influence of the plume buoyancy on its movement. Aided by the Finite Time Lyapunov Exponent tool, we identify Lagrangian Coherent Structures (LCS) which simplify the three-dimensional transport description and make possible the characterization of the smoke plume evolution. 

Our numerical modeling results were able to replicate the observed behavior of the smoke plume during the bushfires in Australia, including the splitting of the plume into multiple pathways. In the model, we found parcels trajectories with the same behavior as the observed plume, highlighted the contribution of the passive advection of the plume by the wind versus the buoyancy effect of hot smoke, delineated the plume into regions destined to different fates, and showed that the division of the main path was affected by an eddy.

How to cite: Curbelo, J. and Rypina, I. I.: Lagrangian atmospheric transport of the smoke plume from the large Australian Wildfire Event of 2019/2020., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9344, https://doi.org/10.5194/egusphere-egu23-9344, 2023.

EGU23-10064 | ECS | Posters on site | AS4 .8

Changes in Organic Soil Mercury Concentrations Over 50 years at the Hubbard Brook Experimental Forest, New Hampshire, USA 

Connor Olson, Benjamin Geyman, Colin Thackray, Chris Johnson, Elsie Sunderland, and Charles Driscoll

Over the past half century, air quality management efforts have led to substantial decreases in mercury emission across North America and Europe. Subsequent declines of mercury concentrations in air and precipitation have been well documented, resulting in lower mercury fluxes in wet deposition. The responsiveness of ecosystems to these decreasing inputs is an on-going point of scientific inquiry and for some matrices, considerable uncertainty exists. Organic surface soils are one such example, with relatively little known about how and on what time scale soils react to changes in mercury deposition. Here, we present an analysis of total mercury in organic soils from the Hubbard Brook Experimental Forest (HBEF), New Hampshire USA, spanning over 50 years. Archived soil samples representing the Oie and Oa horizons in the reference watershed (WS6) were oven-dried, milled, and analyzed via direct mercury analyzer. Trends in total mercury concentration varied over time and among organic soil horizons, with overall mercury concentrations decreasing. Changes in Oie mercury concentration were more pronounced that the Oa horizon and matched modeled deposition for the experimental area (GEOS-Chem). Conversely, Oa mercury concentrations showed little agreement with deposition and are likely integrating atmospheric inputs over a much longer period. Overall, results suggest that organic soils at HBEF are dynamic and responsive to changes in atmospheric emissions.

How to cite: Olson, C., Geyman, B., Thackray, C., Johnson, C., Sunderland, E., and Driscoll, C.: Changes in Organic Soil Mercury Concentrations Over 50 years at the Hubbard Brook Experimental Forest, New Hampshire, USA, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10064, https://doi.org/10.5194/egusphere-egu23-10064, 2023.

An increasing body of evidence documents measurable levels of a broad range of PFAS compounds in precipitation - which translate into substantial deposition loads to terrestrial and aquatic resources. In many environments these atmospheric deposition fluxes can represent the dominant source of PFAS – however, very large gaps in our understanding of atmospheric sources and processing, and deposition fluxes of PFAS remain. 

To address these issues the University of Wisconsin-Madison Wisconsin State Laboratory of Hygiene (WSLH) and the WSLH managed National Atmospheric Deposition Program (NADP), initiated a program to evaluate the efficacy of the US NADP National Trends Network (NTN) for assessment of wet-deposition of PFAS and provide novel new data on levels of PFAS in precipitation across the US.  Dedicated experiments with a diverse suite of 34 PFAS compounds addressed system blanks and stability of the PFAS species in the NTN precipitation collectors. A robust standardized protocol was promulgated for PFAS wet-deposition measurements using the NADP-NTN infrastructure and analytical tools at the WSLH.

We have now applied this protocol in several studies, including in an intensive 5-month study in 2020 at NTN sites across Wisconsin, USA (Pfotenhauer et al., 2022), and in an on-going large-scale nationwide monitoring effort at 10 NTN sites initiated in 2020 and supported by the US Environmental Protection Agency-Office of Research & Development (EPA-ORD).  In the Wisconsin study, 91 precipitation samples, along with an array of QA/QC samples were collected from 8 NTN sites across Wisconsin, and analyzed for 34 PFAS compounds. Concentrations of individual PFAS compounds were generally less than 1 ng/L, however, summed PFAS concentrations ranged from 0.7 to 6.1 ng/L with a median of 1.5 ng/L. Perfluoro carboxylates (PFCAs) were detected most frequently and constituted an average of 83% of the total PFAS mass. Daily flux values ranged from 1.3 to 47.4 ng/m2/day with a median of 5.7 ng/m2/day. Differences in the PFAS fingerprints were observed among the 8 sampling sites, reflecting local sources.

How to cite: Shafer, M. and Gay, D.: Per- and Polyfluoroalkyl Substances (PFAS): Concentrations and Deposition in Precipitation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10074, https://doi.org/10.5194/egusphere-egu23-10074, 2023.

EGU23-11485 | ECS | Orals | AS4 .8

Evaluation of GEOS-Chem model performance for simulating transport and deposition of cosmogenic 10Be and 7Be using different production models 

Minjie Zheng, Hongyu Liu, Florian Adolphi, Raimund Muscheler, Zhengyao Lu, Mousong Wu, and Nønne Prisle

The cosmogenic radionuclides 7Be and 10Be are useful aerosol tracers for atmospheric transport studies. Combining 7Be and 10Be measurements with an atmospheric transport model, not only can improve our understanding of the radionuclide transport and deposition processes, but also can provide an evaluation of the transport process in the model. To simulate those aerosol tracers, it is critical to evaluate the influence of production uncertainties in simulations. Here we use the GEOS-Chem transport model to simulate 7Be and 10Be with different production scenarios: the default production scenario in GEOS-Chem based on an empirical approach, and two production scenarios from the CRAC: Be (Cosmic Ray Atmospheric Cascade: application to Beryllium) model. The model results are comprehensively evaluated with a large number of measurements including more than 490 sites for surface air concentrations and 300 sites for deposition flux. The model can reproduce the absolute values and temporal variability of 7Be and 10Be surface concentrations and deposition fluxes on annual and sub-annual scales. The simulations using the CRAC production scenarios yield a better agreement with the measured deposition flux (70% of data within a factor of 2) compared to the default production scenario in the GEOS-Chem model (59%).  This better agreement is also observed for the vertical profiles of air 7Be concentrations.  Independent of the production models, surface air concentrations and deposition fluxes from all simulations show similar seasonal variations, suggesting a dominant meteorological influence. Finally, we demonstrate the importance of including time-varying solar modulation in the production calculation, which can significantly improve the agreement between the model and measurements, especially from mid to high latitudes.

How to cite: Zheng, M., Liu, H., Adolphi, F., Muscheler, R., Lu, Z., Wu, M., and Prisle, N.: Evaluation of GEOS-Chem model performance for simulating transport and deposition of cosmogenic 10Be and 7Be using different production models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11485, https://doi.org/10.5194/egusphere-egu23-11485, 2023.

EGU23-13231 | ECS | Orals | AS4 .8

Gravitational settling of microplastic fibers: experimental results and implications for global transport 

Daria Tatsii, Gholamhossein Bagheri, Silvia Bucci, Lucie Bakels, and Andreas Stohl

Gravitational settling is a crucial parameter to study the transport and distribution of atmospheric concentrations, sources, and sinks of particles. Although the settling velocity is highly dependent on the particle shape, most atmospheric transport models assume particles to be spherical, ignoring other geometries. In this study, we focus on the gravitational settling of microplastics (MP) particles, which often deviate strongly from sphericity. For instance, MP fibers can be approximated more closely by cylinders rather than spheres. 

Here, we present the results of conducted experiments with extremely elongated MP particles to define their settling velocity. This was done with the settling column and 3D-printed MP particles of different shapes (straight cylinders, half-circled cylinders, and quarter-circled cylinders), lengths, and aspect ratios. The experimental data shows that the parameterization scheme for shape correction proposed by Bagheri and Bonadonna, 2016 is a reliable tool to predict the gravitational settling of fibers considering different types of particle orientation (random, horizontal, and average of both).

This scheme was implemented in the gravitational settling scheme of the Lagrangian transport model FLEXPART to eliminate uncertainties regarding the shape of a particle when simulating solid particle transport. As a study case, the mass concentration and deposition 3D fields of MP fibers were estimated according to the global population density to understand the contribution of the individual sites/regions to MP contamination of the atmosphere, land, and World Ocean.

How to cite: Tatsii, D., Bagheri, G., Bucci, S., Bakels, L., and Stohl, A.: Gravitational settling of microplastic fibers: experimental results and implications for global transport, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13231, https://doi.org/10.5194/egusphere-egu23-13231, 2023.

EGU23-13672 | ECS | Posters on site | AS4 .8

Elevated ammonia emission neutralized alleviation of nitrogen deposition to water pollution in China 

Sijie Feng, Wen Xu, Mengru Wang, Yuanhong Zhao, Maryna Strokal, Carolien Kroeze, Lin Ma, and Fusuo Zhang

Over the past few decades, human activities associated with energy and food production (e.g., industrial, traffic, agricultural, and waste disposal sources) have substantially increased emissions of reactive nitrogen (Nr) to the atmosphere which leads to excessive atmospheric nitrogen (N) deposition on land and rivers. Part of the deposited N on land is also transported to rivers (defined as indirect N deposition). China is a global hotspot of N deposition and has implemented strict atmospheric policies in the last decade. Yet, the responses of N deposition (including direct and indirect N deposition) to these policies and inputs into the river are not well known. We couple a global chemistry transport model with the native 0.5°×0.625° horizontal resolution with a water quality model to simulate direct and indirect N deposition from human activities on rivers in 33 Chinese sub-basins in 2011 and 2019. Compared with 2011, the fluxes of direct N deposition on both rivers and land changed from 10.9 to 10.8 Tg N yr-1 (including deposition of reduced nitrogen (NHx) changed 4.6 to 5.9 Tg N yr-1 and deposition of oxidized nitrogen (NOy) changed 6.3 to 4.9 Tg N yr-1) among the sub-basins in 2019. The results indicate that the strict air policies since 2013 released by the Chinese government significantly decreased NOy. However, the amounts of direct and indirect N deposition on water on average only declined by 2% across all sub-basins, mostly due to the increases in dry ammonia deposition. Agriculture was estimated as the largest source, contributing 30% and 37% to the total N deposition in 2011 and 2019. Thus, agricultural ammonia emission control is essential to reduce N deposition-induced water pollution. This integrated air-water model can assess the impacts of N deposition on water quality, providing insights to develop the pollution control policy for both air and water in sub-basins.

How to cite: Feng, S., Xu, W., Wang, M., Zhao, Y., Strokal, M., Kroeze, C., Ma, L., and Zhang, F.: Elevated ammonia emission neutralized alleviation of nitrogen deposition to water pollution in China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13672, https://doi.org/10.5194/egusphere-egu23-13672, 2023.

EGU23-15773 | ECS | Posters virtual | AS4 .8

Quantifying the Wet Deposition of Reactive Nitrogen over China: Synthesis of Observations and Models 

Jiani Tan, Hang Su, Syuichi Itahashi, Wei Tao, Siwen Wang, Rui Li, Hongbo Fu, Kan Huang, Joshua Fu, and Yafang Cheng

Accurate estimation on reaction nitrogen (Nr) deposition is highly demanded for assessing the impacts on the environment and human beings. This study investigated the wet deposition of inorganic nitrogen (IN) in mainland China by measurements from over 500 sites from five observational networks/databases and ensemble results of eleven chemical transport models (CTMs). Each data source has its focus and limitations and together formed a comprehensive view over China. But the inconsistency among different sources may hinder the appropriate usage of data. Model evaluation results demonstrated the models’ deficiency in simulating the wet NO3- deposition over Southeast China (40% underestimation) and showed an overall underestimation of wet NH4+ deposition over the hotspot regions (5-60% underestimation). A synthesis of this study and twelve reference studies was conducted to quantify the national amount of wet IN deposition. The estimations by CTMs ranged 2.4-3.9 Tg(N) yr-1 for wet NOy deposition and 4-6.7 Tg(N) yr-1 for wet NHx deposition, after adjusting the results with 10-19% underestimations in wet NOy deposition and 1-40% underestimations in wet NHx deposition. The estimations by ground observations ranged 7.1-9 Tg(N) yr-1 for wet NOy deposition and 8-13.1 Tg(N) yr-1 for wet NHx deposition, which were 20-275% higher than the estimation by CTMs, but the results were strongly influenced by the abundances and representative of measurements. Studies using statistical techniques to interpolate site observations predicted 3-5.5 Tg(N) yr-1 for wet NOy deposition and 3.9-7.2 Tg(N) yr-1 for wet NHx deposition. This approach benefited from high accuracy and good robustness of the statistical models, but the uncertainty in the interpolation methods could be a potential drawback.

How to cite: Tan, J., Su, H., Itahashi, S., Tao, W., Wang, S., Li, R., Fu, H., Huang, K., Fu, J., and Cheng, Y.: Quantifying the Wet Deposition of Reactive Nitrogen over China: Synthesis of Observations and Models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15773, https://doi.org/10.5194/egusphere-egu23-15773, 2023.

EGU23-15811 | Orals | AS4 .8

Origin of nitrogen deposition in Germany: Source allocation and influence of local emissions 

Richard Kranenburg, Martijn Schaap, Markus Geupel, Stefan Feigenspan, and Alexander Moravek

Eutrophication is one of the main reasons threatening biodiversity in Germany. To quantify the risk for biodiversity caused through nitrogen deposition, in Germany national data on the exceedance of critical loads for eutrophication are used as indicators for the National Strategy on Biodiversity and for the National Sustainability Development Strategy. In addition, to prevent ecosystems from unwanted further excessive nitrogen deposition, according to the German emission control and nature protection legislation, nitrogen deposition has to be assessed when new nitrogen emitting projects are submitted. To support the development of the national nitrogen strategy and devise regional emission targets an effort was made to provide insight into the geographic regions of origin of the nitrogen deposited within the federal states in Germany.

The atmospheric dispersion modelling was performed with chemistry transport model LOTOS-EUROS. Simulations over Germany were run with a resolution of 0.10° longitude by 0.05° latitude, nested in a European simulation. In addition to species concentrations and deposition fluxes, the contributions of predefined source categories were calculated and tracked using a labelling approach for the year 2019. The labels applied in this simulation encompass all emissions from the 16 individual German federal states, all 9 neighbouring countries of Germany and countries further away. Additionally, labels were attached to international shipping emissions, natural emissions, and boundary conditions to cover intercontinental transport. This result in a full source-receptor matrix with contributions to N-deposition in all federal states with contributions from all states and neighbouring countries. To assess contributions of local sources, an additional simulation was performed with emission reductions on three surface and two stack point sources.

Largest average depositions in Germany are found in Hamburg and Bremen followed by Niedersachsen, Nordrhein-Westfalen and Schleswig-Holstein. Hamburg and Bremen are small city states with relative high NOx emission densities. However, local emissions only contribute approximately 20%, main contributors are neighbouring areas Niedersachsen and Schleswig-Holstein due to their large agricultural sector with high ammonia emissions. A general trend can be spotted that states with dominant NHx emissions also have the highest local deposition. This holds for Baden-Württemberg, Bayern, Niedersachsen, Nordrhein-Westfalen and Schleswig-Holstein, where on average 40% of the nitrogen deposition originates from the sources within each state. For many states, there is also a considerable contribution of countries surrounding Germany. Emissions from the Netherlands contribute mainly in Bremen, Hamburg, Niedersachsen, Nordrhein-Westfalen and Schleswig-Holstein. The other main contributor is France, affecting mainly the states in southern Germany. The assessment of local contributions from the surface point sources shows that about 18-22 % of the emitted mass is deposited within a radius of 20 km from the source In contrast, for two the stack point sources, NHx deposition within 20 km of the source is only about 5% of the emission strength.

How to cite: Kranenburg, R., Schaap, M., Geupel, M., Feigenspan, S., and Moravek, A.: Origin of nitrogen deposition in Germany: Source allocation and influence of local emissions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15811, https://doi.org/10.5194/egusphere-egu23-15811, 2023.

Recent studies show that effective pollution control strategies have led to a significant reduction in air pollution in Cyprus. However, the same studies attributed a large number of pollution episodes to the long-range transport of pollutants from regional sources. Black carbon (BC) and carbon monoxide (CO), with a lifetime of several weeks to several months in the troposphere, are considered reliable aerosol and gaseous pollutants to quantify the contribution of regional sources. This study aims to investigate the contribution of anthropogenic sources to atmospheric pollutants over the Eastern Mediterranean. Using FLEXPART, a Lagrangian dispersion model, the origin and residence time of air masses over Cyprus from Europe and the MENA region have been simulated with a temporal resolution of 3 hours for each day of 2019. Then, by coupling FLEXPART simulations to global emission inventories, including MACCity and CAMS-GLOB, the contribution of sources to CO and BC simulations in Cyprus was determined separately for each sector and country in the study area. Results show that CO concentrations are mainly modulated by sources in Turkey. Secondary sources are found in MENA (Iran, Iraq, and Syria) in the cold period of the year and in Eastern (Ukraine and Russia) and Western Europe (Germany and Italy) in the warm seasons. While CAMS-GLOB simulations identify the main sources in agricultural (in the cold period) and residential (in the warm period) sectors, traffic sources have also been identified with the largest contributions in MACCity simulations. Regarding BC simulations, most sources are found in Turkey in the agricultural (in CAMS-GLOB simulations) and industrial (in MACCity simulations) sectors. Local sources were found influential only in the MACCity BC simulations. This can be attributed to uncertainties in the emission inventories and in the simulations of atmospheric residence times. Our results can inform policy- and decision-makers in implementing efficient abatement strategies, improving air quality, and reducing human exposure.

How to cite: nabavi, S. O. and Christoudias, T.: Long-range source apportionment of black carbon and carbon monoxide over Cyprus using FLEXPART and global emission inventories, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16207, https://doi.org/10.5194/egusphere-egu23-16207, 2023.

EGU23-17115 | ECS | Orals | AS4 .8

Modelling the atmospheric chlorine 36 dry deposition on grass using micrometeorology 

Deo-Gratias Sourabie, Didier Hebert, Lucilla Benedetti, Elsa Vitorge, Beatriz Lourino-Cabana, Valery Guillou, and Denis Maro

Chlorine 36 (36Cl, T1/2 = 301,000 years) is a radionuclide with natural and anthropogenic origin that can be rejected during decommissioning of nuclear power plants or chronically during recycling of used nuclear fuels. Once emitted into the atmosphere, chlorine 36 (gas and particles) can be transferred to the soil and vegetation cover by dry and wet deposition. However, quantitative constraints of these deposits are very scarce. Because of its relatively high mobility in the geosphere and its high bioavailability, chlorine 36 fate in the environment should be studied for environmental and human impact assessments.
The aim of this study is therefore to develop dry depositional models for the gaseous and particulate fractions of chlorine 36. The model used for the parameterization of gaseous chlorine 36 dry deposition on grass is the << Big-leaf >> model based on the electrical analogy (Seinfield 1985). It was adapted from the Bah (2020) model developed for iodine. For particulate chlorine 36, the Damay-Pellerin (2017) model was used. This model requiring the diameter of particulate chlorine 36 to be known, a sample of aerosol was taken in the chlorine 36 plume to determine on which particle size it is fixed. The sampling was performed on a low pressure impinger (LPI, DEKATI) of 13 levels for particles with diameters between 30nm and 10μm. In order to obtain model input data, meteorological and micrometeorological parameters were measured continuously at the IRSN La-Hague technical platform (PTILH, France). The PTILH is located 2 km north of Orano La-Hague plant which emits small quantities of chlorine 36. An ultrasonic anemometer (Young 81000V) installed at a height of 4,5 m from the ground measured the direction (°), the velocity u (m/s) and the air friction velocity u* (m/s), the sensible heat flux H, the Monin-Obukhov length (L) and the atmospheric stability (1/L). A weather station (Spectrum Watchdog, series 2000) measured temperature Ts (°C), relative humidity RH (%), dew point (°C), global radiation SR (Wat/m2) and photosynthetic active radiation PAR (μM/m2.s). Sampling campaigns of 2 weeks were also conducted at the PTILH site to determine experimental depositional rates of chlorine 36. Chlorine 36 measurements were carried out by acceleration mass spectrometry at CEREGE-LN2C (France).
The particle size distribution of the aerosol sample from chlorine 36 plume shows two peaks, a main one at 2μm and a second one at 10μm, typical distribution of marine aerosol. The models yield chlorine 36 depositional velocities between 6,7.10-3 and 10-2 m/s for the particulate fraction, and between 5.10-3 and 1,3.10-2 m/s for the gaseous one. The total dry depositional velocities (particles and gas) calculated from the model are less than one order of magnitude than the ones obtained experimentally.

How to cite: Sourabie, D.-G., Hebert, D., Benedetti, L., Vitorge, E., Lourino-Cabana, B., Guillou, V., and Maro, D.: Modelling the atmospheric chlorine 36 dry deposition on grass using micrometeorology, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17115, https://doi.org/10.5194/egusphere-egu23-17115, 2023.

EGU23-769 | ECS | PICO | AS4.9

A theoretical review of the air-ground coupling of 1D elastic media 

Zongbo Xu and Philippe Lognonné

The air-ground coupling is the conversion of the atmospheric pressure perturbation to the ground motion. This coupling includes the pressure static loading and the acoustic-to-seismic conversion. Studying this coupling can aid investigating the shallow subsurface using the pressure drops and monitoring explosive sources in the atmosphere (like meteorites). However, the theory link of the possible coupling scenarios is missing for 1D elastic media. We demonstrate that by utilizing the compliance, the ratio between the ground motion and the atmospheric pressure perturbation on the ground surface, we can analytically model the coupling scenarios: the static loading, the air-coupled Rayleigh wave, leaky mode, and the acoustic-to-body-wave conversion.

How to cite: Xu, Z. and Lognonné, P.: A theoretical review of the air-ground coupling of 1D elastic media, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-769, https://doi.org/10.5194/egusphere-egu23-769, 2023.

EGU23-2444 | PICO | AS4.9 | Highlight

Infrasonic observations of a rare earthgrazing fireball 

Elizabeth Silber, Miro Ronac Giannone, and Daniel Bowman

The Earth’s atmosphere is continuously bombarded by extraterrestrial objects (generally referred to as meteoroids) of various sizes and velocities (11.2–72.5 km/s). Such high kinetic energy interactions with exponentially increasing higher density atmosphere result in a visual phenomenon known as a meteor. Optically very bright events, or fireballs, are typically produced by objects larger than about 10 cm in diameter. A rare class of fireballs are earthgrazers which enter the atmosphere at an extremely shallow angle. Depending on their size and velocity, some earthgrazers return to space after a relatively short hypersonic flight through the upper regions of the atmosphere. Due to a variety of factors, including the lack of dedicated observational resources, there are only a handful of documented observations of earthgrazing fireballs in the last 50 years. Nevertheless, this category of extraterrestrial objects is of significant interest to the scientific community for a range of practical reasons, such as the analogous relationship with artificial platforms capable of reaching the boundary of the outer atmosphere. In general, typical fireballs are capable of generating shockwaves that can decay to very low frequency acoustic waves, also known as infrasound. Theoretically, the resulting shockwaves and subsequent infrasound from earthgrazers should have distinct signatures. In principle, fireballs can serve as natural laboratories for testing regional and global infrasound monitoring capabilities and provide an important leverage towards improving high-altitude source detection, characterization and geolocation efforts. Infrasound signatures from earthgrazers should further enhance our understanding of infrasonic signals generated in the upper atmopshere. We report infrasound detection of a rare earthgrazing fireball that was observed by casual witnesses and all-sky cameras across Europe on 22 September 2020. It entered at 03:53:40 UTC over northern Europe, and its luminous path extended from Germany to the UK. Despite the high-altitude trajectory (~100 km), the earthgrazer generated a pressure wave that reached the ground at low frequencies detectable by infrasonic instruments. Three infrasound stations of the Royal Netherlands Meteorological Institute (KNMI) network detected the signal. The airwave swept one of the arrays at a particularly high trace velocity (>1 km/s), indicative of a near-vertical arrival angle from a high-altitude cylindrical line source. 
SNL is managed and operated by NTESS under DOE NNSA contract DE-NA000352.

How to cite: Silber, E., Ronac Giannone, M., and Bowman, D.: Infrasonic observations of a rare earthgrazing fireball, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2444, https://doi.org/10.5194/egusphere-egu23-2444, 2023.

EGU23-3173 | PICO | AS4.9

3D Acoustic reconstruction of lightning by two dense acoustic networks 14 km apart 

Thomas Farges, Pierre Letournel, Alexis Le Pichon, and Constantino Listowski

Lightning emits electromagnetic (radio and optical) or acoustic waves, commonly called thunder. In recent years, studies have shown the contribution of acoustic measurements for the 3D reconstruction of cloud-to-ground or intracloud discharges. These acoustic reconstructions are in good agreement with LMA measurements and classical lightning location systems. Recent developments allow to infer the acoustic power of the source and its variability from one flash to another as well as within a flash.

In spring 2022, we set up a measurement campaign where four dense microphone arrays were deployed in the southeast of France. These arrays were composed of nine sensors distributed in a 3x3 matrix of a 20 meter square area. The signals were sampled at 100 Hz and time-stamped with the GPS reference. A thunderstorm occurred on April 23, 2022 and was observed by three of these four arrays. Comparisons with detections at a four array elements of comparable aperture highlights the contribution of denser networks in terms of detection and location capabilities. The storm of April 23 passed between two arrays 14 km apart. This campaign is a very good opportunity to demonstrate how lightning locations can be reconstructed by combining detection results at two acoustic arrays. We detail these new contributions in our presentation.

 

How to cite: Farges, T., Letournel, P., Le Pichon, A., and Listowski, C.: 3D Acoustic reconstruction of lightning by two dense acoustic networks 14 km apart, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3173, https://doi.org/10.5194/egusphere-egu23-3173, 2023.

EGU23-3534 | PICO | AS4.9

Evaluating long range middle atmospheric variability for global infrasound monitoring 

Alexis Le Pichon, Constantino Listowski, Patrick Hupe, and Lars Ceranna

Global scale infrasound observations confirm that the detection capability of the International Monitoring System (IMS) deployed to monitor compliance with the Comprehensive Nuclear-Test ban Treaty (CTBT) is highly variable in space and time. Previous studies estimated the radiated source energy from remote observations using empirical yield-scaling relations accounting for the along-path stratospheric winds. However, these relations simplified the complexities of infrasound propagation as the wind correction applied does not account for an accurate description of the middle atmosphere along the propagation path. In order to reduce the variance in the calculated transmission loss, massive frequency and range-dependent full-wave propagation simulations are carried out, exploring a wide range of realistic atmospheric scenarios. Model predictions are further enhanced by incorporating fine-scale atmospheric structures derived from a two-dimensional horizontal wave number spectrum model. A cost-effective approach is proposed to estimate the transmission losses at distances up to 4,000 km along with uncertainties derived from multiple gravity wave realizations. In the context of the future verification of the CTBT, this approach helps advance the development of network performance simulations in higher resolution and the evaluation of middle atmospheric models at a global scale with limited computational resources.

How to cite: Le Pichon, A., Listowski, C., Hupe, P., and Ceranna, L.: Evaluating long range middle atmospheric variability for global infrasound monitoring, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3534, https://doi.org/10.5194/egusphere-egu23-3534, 2023.

EGU23-3555 | PICO | AS4.9 | Highlight

Stratospheric gravity waves in high-resolution global models 

Claudia Stephan

As we enter the age of exascale computing, more and more global scale simulations with horizontal grid spacings in the range of 1-10 km become available. Yet, not the full spectrum of gravity waves (GWs) is resolved and new challenges emerge, some of which are directly linked to the representation of convection, which is only partially resolved, but the most important source of GWs in the tropics.

Unlike most climate models that use parameterizations for GWs, the DYAMOND simulations reproduce detailed, satellite-observed features of the global GW momentum flux (GWMF) distribution including the zonal mean. This can be attributed to realistic GWs from convection, orography and storm tracks. Yet, the GWMF magnitudes differ substantially among simulations. Differences in the strength of convection may help explain differences in the GWMF between simulations of the same model in the summer low latitudes where convection is the primary source. For ICON, simulations with explicit convection show 30-50% larger zonal-mean momentum fluxes in the summer hemisphere subtropics than simulations with parameterized convection. Explicit convection is associated with stronger updrafts and GW sources.

Since any kind of observations can only see a fraction of the GW spectrum, we also analyzed the spectra of the horizontal motions associated with inertia GWs and Rossby waves, respectively. A fundamental characteristic of the atmosphere is the distribution of wave energy across different horizontal scales. Observations and numerical modelling have supported the idea of a canonical energy spectrum. Horizontal kinetic energy scales with the horizontal wavenumber k as k**-3 at large scales with a transition towards k**-5/3 at mesoscales.

The simulations produce the expected canonical shape of the spectra, which is encouraging given that some models are stripped down to a minimum set of physical parameterizations. Yet, total energy levels, spectral slopes at sub-synoptic scales, and spectral crossing scales differ significantly. The contribution of inertia GWs to the total wave energy differs by factors of up to two between the simulations. The crossing scales between the inertia GW and Rossby wave spectra also differ by a factor of about two between the simulations and depend mostly on the ratio of integrated wave energies, rather than on spectral slope or details of the spectral shape. The spectra exhibit little variability in time and can serve as an almost instantaneous diagnostic.

How to cite: Stephan, C.: Stratospheric gravity waves in high-resolution global models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3555, https://doi.org/10.5194/egusphere-egu23-3555, 2023.

EGU23-3838 | PICO | AS4.9

Meteor infrasound recordings at a dense seismic broadband transect in Spain 

Daniel Stich, Josué Casado Rabasco, José María Madiedo, Juan Luis Guerrero Rascado, and Jose Morales

With the densification of seismic networks, recordings of atmospheric infrasound events through ground coupled signals are becoming more numerous. In particular, there’s an increasing probability of detecting direct arrivals at near distances from the source. Here, we analyze a meteor event with absolute magnitude m = −17 on December 11th 2016 that was recorded coincidentally along a dense seismic broadband transect near Granada, Spain. Using 44 near-field detections and the ERA5 atmospheric temperature and wind speed model, we can locate the acoustic source at 38 km height, consistent with the triangulation of the meteor terminal explosion from camera recordings.

The waveforms recorded along the seismic transect reveal important differences between nearby stations, emphasizing the importance of local conditions for acoustic wave propagation and acousto-seismic coupling. A common component of all waveforms are ~0.5 s long N-waves, inherited from the atmospheric shock wave, however waveform attributes such as peak velocity amplitudes and frequencies, signal duration and signal energy show variations of one order of magnitude. Also, the three-component signal polarization shows large variability among stations, suggesting that waveform complexity and the repetitions of N-waves reflects the interaction with local topography, in addition to multipathing through the small-scale structure of the atmosphere along the path. Our observations shed light on various causes of complexity in the conversion of the free-atmosphere acoustic wavefield to ground motion, and point to the difficulties involved in estimating the original pressure signal from acousto-seismic data.

How to cite: Stich, D., Casado Rabasco, J., Madiedo, J. M., Guerrero Rascado, J. L., and Morales, J.: Meteor infrasound recordings at a dense seismic broadband transect in Spain, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3838, https://doi.org/10.5194/egusphere-egu23-3838, 2023.

EGU23-5212 | PICO | AS4.9

Event clustering for infrasound monitoring system 

maurice charbit, alexis le pichon, benjamin poste, françois roueff, and julien vergoz
In the area of infrasonic monitoring system, an important task is to clustering the various cells containing a
signal of interest to a reduced event number. Indeed, to each time-frequency cell is attached a source direction of arrivals,
many of which arise from the same physical event spanning over a large time-frequency window. In PMCC (Progressive
Multi-Channel Cross-Correlation) the clustering is based on ad hoc rules and metrics provided by a large empirical expertise.

In this study we present a new approach based on a statistical model, associated to the multichannel maximum-
likelihood (MCML). More specifically, for each time-frequency cell, the MCML provides the estimations of the slowness
vector and of the signal-to-noise ratio (SNR), and the p-value computed from the generalized likelihood ratio (GLR).
These quantities are collected within a large window, typically 10 Hz by 1 hour. To reduce the computational time, only
the cells with p-values below a threshold are considered. The proposed mixture model (MM) is based on the following
4-dimensional vector: the time location, the log of the frequency location and the two components of the slowness vector.
 
Each cluster is modeled by a distribution, chosen in a flexible catalog that can still be improved. Today the catalog
consists of Gaussian distribution, uniform distribution and mixture of Gaussian and uniform. A few examples: short
time event is modeled by a 4D Gaussian, permanent event in a given frequency band, as microbarom or wind turbine, is modeled by
a 2D Gaussian for the DOA, a full time uniform distribution for the time location and a uniform distribution in the
known frequency band. For the DOA modeled by a Gaussian, the covariance is taken as the asymptotic covariance of
the MCML, using the estimated SNR in the corresponding cell. Moreover we introduce a specific cluster to trap falsely
detected signals, modeled by a full uniform distribution in the four dimensions.

The estimation of the parameters of the MM is performed by the so-called Expectation Maximization algorithm.
Then the maximum a posteriori provides the final clustering. We also present an estimation of the number of events
based on the Bayesian information criterion (BIC). Many real observations are considered to illustrate the method.

The main advantages of the proposed method are (i) taking into account the p-value for selecting the cells to cluster,
(ii) the flexibility of the model catalog, (iii) the statistical interpretation of the results.
 

How to cite: charbit, M., le pichon, A., poste, B., roueff, F., and vergoz, J.: Event clustering for infrasound monitoring system, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5212, https://doi.org/10.5194/egusphere-egu23-5212, 2023.

Simultaneous observations of infrasonic and seismic signals recorded with the Romanian seismo-acoustic arrays (BURAR, BURARI and IPLOR) are used to forensic tracking the repetitive explosion sources generated by the bombing and shelling taking place in Ukraine since 24 February 2022. Seismo-acoustic signature (signal shape and amplitude, frequency content, energy spectrum) analyzed are characterized by impulsive energetic signals. Events reported in the bulletins provided by IDC/CTBTO are used as reference for associating infrasound and seismic detections of the Romanian arrays. Infrasound signals observed with BURAR seismic array are added to better characterize the type of events in this region. Seismo-acoustic data are analyzed by using processing capabilities of the DTK-GPMCC and DTK-DIVA software embedded in NDC-in-a-Box package.
Infrasonic detections are strongly influenced both by seasonally dependent stratospheric winds and local turbulence-induced pressure fluctuations, i.e., level of wind-generated background noise increases with station altitude. Directions of IPLOR and BURARI infrasonic detections are estimated and the locations are obtained by cross-bearing the derived back azimuths. Deviating effects of zonal cross winds along the propagation path through the atmosphere affect the observed back azimuths: rays which arrive at BURARI are deflected towards the East with approx. 5o, whilst at IPLOR, the azimuthal deviation is negligible (below 1o).
The propagation path of infrasonic signals is analyzed by applying infraGA 2D ray tracer through NRL-G2S atmospheric model. Stratospheric and thermospheric infrasound phases are identified to be observed at BURARI and IPLOR stations.
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How to cite: Ghica, D. and Ionescu, C.: Analysis of infrasound and seismic signals recorded from repetitive explosion sources at near-regional distance, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5764, https://doi.org/10.5194/egusphere-egu23-5764, 2023.

EGU23-6609 | PICO | AS4.9

Swell and thunder : infrasound signatures of Mediterranean hurricanes 

Constantino Listowski, Edouard Forestier, Stavros Dafis, Thomas Farges, Marine De Carlo, Florian Grimaldi, Alexis Le Pichon, Julien Vergoz, Philippe Heinrich, and Chantal Claud

Infrasound detections of Mediterranean cyclones known as medicanes (for « Mediterranean hurricanes ») are demonstrated in low- and high- frequency ranges, respectively. We summarize the main findings of a recently published study [1]. We use data from the infrasound station IS48 of the International Monitoring System, in Tunisia, to investigate the infrasound signatures of these meso-cyclones, using a multi-channel correlation algorithm. We discuss cases of detections and non-detections, based on the state of the middle atmosphere and of the wind noise measured at the station. Detections and likely sources are discussed in light of other datasets, comprising satellite observations of deep convection [2] and cloud-to-ground lightning detections from a ground-based network. Detections of infrasound emitted by the cyclone-related swell are modelled using a microbarom source model [3] and are in agreement with observations, comforting the identification of the lower frequency sources. This multi-technology and modelling approach allows to discuss the various sources at plat that may contribute to the monitoring of such extreme meteorological events.

[1] Listowski, C.; Forestier, E.; Dafis, S.; Farges, T.; De Carlo, M.; Grimaldi, F.; Le Pichon, A.; Vergoz, J.; Heinrich, P.; Claud, C. Remote Monitoring of Mediterranean Hurricanes Using Infrasound. Remote Sens. 2022, 14, 6162. https://doi.org/10.3390/rs14236162

[2] Dafis, S.; Claud, C.; Kotroni, V.; Lagouvardos, K.; Rysman, J. Insights into the convective evolution of Mediterranean tropical-like cyclones. Q. J. R. Meteorol. Soc. 2020, 146, 4147–4169.

[3] De Carlo, M.; Accensi, M.; Ardhuin, F.; Le Pichon, A. ARROW (AtmospheRic InfRasound by Ocean Waves): A new real-time product for global ambient noise monitoring. In Proceedings of the EGU General Assembly 2022, Vienna, Austria, 23–27 May 2022

 

How to cite: Listowski, C., Forestier, E., Dafis, S., Farges, T., De Carlo, M., Grimaldi, F., Le Pichon, A., Vergoz, J., Heinrich, P., and Claud, C.: Swell and thunder : infrasound signatures of Mediterranean hurricanes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6609, https://doi.org/10.5194/egusphere-egu23-6609, 2023.

EGU23-6647 | ECS | PICO | AS4.9

The Multi-Channel Maximum-Likelihood (MCML) method: towards a multisource detection and wave parameter estimations using deep learning 

Benjamin Poste, Maurice Charbit, Alice Janela Cameijo, Alexis Le Pichon, Constantino Listowski, François Roueff, and Julien Vergoz

We present an improvement of the Multi-Channel Maximum-Likelihood (MCML) method [1]. This approach is based on the likelihood function derived from a multi-sensor stochastic model expressed in different frequency channels. Using the likelihood function, we determine, for the detection problem, the Generalized Likelihood Ratio (GLR) with a p-value threshold to discriminate signal of interest and noise. For the estimation of the slowness vector, we determine the Maximum Likelihood Estimation (MLE). Comparisons with synthetic and real datasets show that MCML, when implemented in the time-frequency domain, outperforms state-of-the-art detection algorithms in terms of detection probability and false alarm rate in poor signal-to-noise ratio scenarios. We evaluate the capability of MCML to detect overlapping coherent signals in the same time frequency domain, depending on various scenarios with varying signal-to-noise ratio (SNR), frequency bands and array geometry. We quantify the performance of deep learning method to discriminate between interfering coherent signals by predicting the number of sources in a given time-frequency cell using synthetics and real data recorded by stations part of the International Monitoring System (IMS).

 

[1] B Poste, M Charbit, A Le Pichon, C Listowski, F Roueff, J Vergoz (2022), The Multi-Channel Maximum-Likelihood (MCML) method: a new approach for infrasound detection and wave parameter estimation, Geophysical Journal International, https://doi.org/10.1093/gji/ggac377

How to cite: Poste, B., Charbit, M., Janela Cameijo, A., Le Pichon, A., Listowski, C., Roueff, F., and Vergoz, J.: The Multi-Channel Maximum-Likelihood (MCML) method: towards a multisource detection and wave parameter estimations using deep learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6647, https://doi.org/10.5194/egusphere-egu23-6647, 2023.

Sudden stratospheric warmings (SSWs) have significant impacts on the Arctic ozone. In this study, MERRA-2 provides the characteristics of the zonal-mean zonal wind and temperature influenced by the planetary waves during major SSWs. We present an analysis of ozone variations in the stratosphere over Ny-Ålesund, Svalbard (79°N, 12°E) based on the ground-based microwave radiometer GROMOS-C during the major SSW events that occurred from 2015 to 2022. The results are compared with Aura-MLS observations and MERRA-2 simulations. GROMOS-C captures the high variability of stratospheric ozone fluctuations during SSWs at polar latitudes very well. The stratospheric ozone dramatically increases after SSW onset day, which lasts up to two months. The polar vortex is disturbed or weakened by SSW resulting in the meridional transport of ozone from the mid-latitude into the polar regions. Therefore, this study assists in understanding the relationship between the interannual variability of stratospheric ozone and the occurrence of SSWs and has significant implications for stratospheric ozone trends in the northern polar regions.

How to cite: Shi, G. and Stober, G.: Analysing ozone variability at northern polar latitude during sudden stratospheric warming events using ground-based microwave radiometer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6931, https://doi.org/10.5194/egusphere-egu23-6931, 2023.

EGU23-6993 | ECS | PICO | AS4.9

Using infrasound from explosions for probing internal gravity waves in the middle atmosphere 

Ekaterina Vorobeva, Jelle Assink, Igor Chunchuzov, Toralf Renkwitz, Patrick Espy, and Sven Peter Näsholm

This study uses ground-based recordings of low-frequency, inaudible acoustic waves (infrasound) to probe the wind and temperature fluctuations associated with internal gravity waves breaking in the middle atmosphere. Building on the approach introduced by Chunchuzov et al., the recorded waveforms are used to retrieve the effective sound speed fluctuations in an inhomogeneous atmospheric layer of infrasound backscattering. The retrieval procedure was applied to infrasound from controlled blasts related to the disposal of military explosives in Hukkakero, Finland and recorded at the IS37 station in Norway over a four-year period from 2014 to 2017. Our findings indicate that infrasound scattering occurs in the lower mesosphere between 50 and 75 km in altitude in a region where gravity waves interact due to strong nonlinear effects and form thin layers with strong wind shears. The retrieved effective sound speed fluctuations were then analysed in terms of the vertical wave number spectra. The analysis revealed that the spectra follow a kz–3 power law that corresponds to the "universal" saturated spectrum of atmospheric gravity waves within kz ∈ [2.1·103; 2.7·102] cycles/m. Based on this wavenumber range, we estimate the outer and inner vertical scale of atmospheric inhomogeneities that infrasound is sensitive to as Linner= 33 – 37 m, Louter = 382 – 625 m.  

Furthermore, the spectra of the retrieved effective sound speed fluctuations were compared to theoretical linear and nonlinear gravity wave saturation theories as well as to independent wind measurements made by the Saura MF radar near the Andøya Space Center in Norway. The comparison showed a good agreement in terms of the amplitude and slopes of the vertical wavenumber spectra in both cases. The overall agreement allows us to suggest that the Saura radar and infrasound-based effective sound speed profiles represent the low- and high-wavenumber regimes of the same "universal" gravity wave spectrum. These results illustrate that the use of infrasound makes it possible to probe fine-scale motions that are not well captured by other techniques. The latter suggests that infrasound observations can be used as a complementary technique to probe internal gravity waves in the middle- and upper atmosphere. 

How to cite: Vorobeva, E., Assink, J., Chunchuzov, I., Renkwitz, T., Espy, P., and Näsholm, S. P.: Using infrasound from explosions for probing internal gravity waves in the middle atmosphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6993, https://doi.org/10.5194/egusphere-egu23-6993, 2023.

EGU23-7085 | ECS | PICO | AS4.9

Evaluating atmospheric models in the stratosphere using oceanic infrasound ambient noise. 

Pierre Letournel, Constantino Listowski, Marc Bocquet, Alexis Le Pichon, Alban Farchi, Julien Vergoz, and Marine De Carlo

Oceanic ambient noise (microbaroms) records are examined to retrieve information on the state of the middle atmosphere. We present an approach to compare ground-based infrasound observations with simulated infrasound detections obtained by combining a microbarom source model [1] with a semi-empirical attenuation law. Comparisons using this continuous and global infrasound source are presented for large time periods to assess performances on both seasonal and finer time scales. Infrasound detections obtained with a cross-correlation algorithm (PMCC) as well as with the new MCML (MultiChannel Maximum Likelihood) method [2] are considered. The sensitivity of simulated infrasound detections to the middle atmosphere model and to the propagation model (the transmission loss parametrisation) is evaluated. We discuss how this method may help to assess the performance of an atmospheric model in the middle atmosphere, as well as to select best members in an ensemble reanalysis.

 

[1] De Carlo, M., Accensi, M., Ardhuin, F., and Le Pichon, A.: ARROW (AtmospheRic InfRasound by Ocean Waves): a new real-time product for global ambient noise monitoring., EGU General Assembly 2022, Vienna, Austria, 23–27 May 2022, EGU22-7564, https://doi.org/10.5194/egusphere-egu22-7564, 2022.


[2] B Poste, M Charbit, A Le Pichon, C Listowski, F Roueff, J Vergoz, The multichannel maximum-likelihood (MCML) method: a new approach for infrasound detection and wave parameter estimation, Geophysical Journal International, Volume 232, Issue 2, February 2023, Pages 1099–1112, https://doi.org/10.1093/gji/ggac377

How to cite: Letournel, P., Listowski, C., Bocquet, M., Le Pichon, A., Farchi, A., Vergoz, J., and De Carlo, M.: Evaluating atmospheric models in the stratosphere using oceanic infrasound ambient noise., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7085, https://doi.org/10.5194/egusphere-egu23-7085, 2023.

EGU23-7121 | PICO | AS4.9 | Highlight

Summarizing the research of the MADEIRA project - Middle atmosphere dynamics: exploiting infrasound using a multidisciplinary approach at high latitudes 

Sven Peter Näsholm, Javier Amezcua, Jelle D. Assink, Evgenia Belova, Erik Mårten Blixt, Quentin Brissaud, Mari Dahl Eggen, Patrick J. Espy, Robert Hibbins, Johan Kero, Tormod Kvaerna, Alexis Le Pichon, Yvan J. Orsolini, Ismael Vera Rodriguez, Antoine Turquet, and Ekaterina Vorobeva

The MADEIRA project (Middle Atmosphere Dynamics: Exploiting Infrasound Using a Multidisciplinary Approach at High Latitudes) is a four-year basic research project finishing in the spring 2023, funded by the Research Council of Norway. 

Its primary objective has been in elucidating the 30-60 km altitude range over large spatial scales using wind and temperature constraints from infrasound data collected at Arctic stations. Wave propagation modelling and infrasound interpretation from well-characterized sources provide remote atmospheric sensing. These data are more continuous in space and time than from many other direct measurement techniques. An aim has been to constrain high-top atmospheric models and explore stratosphere-mesosphere coupling with meteor radar wind measurements sampling the 70-100 km altitude range in combination with the infrasonic data. Another ambition has been to develop real-time diagnostic tools for the stratospheric polar vortex circulation and extreme events like Sudden Stratospheric Warmings. 

Thanks to this project, the research teams have got the opportunity to explore several aspects and building blocks related to infrasound-based middle atmospheric probing and to work towards an assimilation of such datasets into atmospheric models. This paper reviews key research output from the project and highlights accomplishments in the domains of, e.g.: Tropospheric and stratospheric cross-wind estimation using infrasound from explosions; Assimilation of atmospheric infrasound data to constrain tropospheric and stratospheric winds; Atmospheric wind and temperature profile inversion in an ensemble model context; Microbarom radiation and propagation model benchmarking; Speeding up infrasound transmission loss estimation using deep learning; Probing internal middle atmospheric gravity waves; Using a machine learning and stochastics-founded model to provide near real-time stratospheric polar vortex diagnostics.

This project has included several high risk / high gain components and we highlight results that maybe could be labelled as unexpected successes, but we also discuss challenging research obstacles that occurred in our journey.

How to cite: Näsholm, S. P., Amezcua, J., Assink, J. D., Belova, E., Blixt, E. M., Brissaud, Q., Eggen, M. D., Espy, P. J., Hibbins, R., Kero, J., Kvaerna, T., Le Pichon, A., Orsolini, Y. J., Vera Rodriguez, I., Turquet, A., and Vorobeva, E.: Summarizing the research of the MADEIRA project - Middle atmosphere dynamics: exploiting infrasound using a multidisciplinary approach at high latitudes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7121, https://doi.org/10.5194/egusphere-egu23-7121, 2023.

EGU23-7641 | PICO | AS4.9 | Highlight

New observations showing temperature-wind interconnection during mesospheric inversion layer events 

Philippe Keckhut, Alexis Mariaccia, Alain Hauchecorne, Mathieu Ratynski, and Sergey Khaykin

It is known that propagation of atmospheric waves and their dissipation are responsible for the small and large disturbances governing the variability observed in the mesosphere (50-90 km). One of the main phenomena caused by these waves is the so-called mesospheric inversion layer (MIL) referring to a vertical layer of ~10 km where there is an enhanced temperature (15-50 K) lasting many days over thousands of kilometers in the mesosphere. Additionally, as perturbations in the mesosphere are crucial issues in aeronautics for the safe reentry of space shuttles or missiles, the study of MILs have aroused a large interest. However, the understanding of MIL’s formation mechanisms is still not fully complete as MILs’ impact on wind behavior has never been observed accurately in the middle atmosphere preventing to determine the shear profile or study how gravity waves propagate from the stratosphere to the thermosphere. Though numerous studies have suggested the important role of gravity waves in the MIL’s apparition. For instance, Hauchecorne and Maillard (1990) have simulated MIL’s formation by the breaking of gravity waves inside and above the MIL making decrease wind above the mesospheric jet, generating turbulence.

In this context, we report here, for the first time, an investigation of co-located temperature-wind observations in the altitude range 30-90 km during MIL events. According to these observations, the temperature inversion within the MIL is associated with a wind deceleration occurring in the same altitude range, confirming an inter-connection and arguing in favor of the role of gravity wave in the occurrence of MIL phenomenon.

How to cite: Keckhut, P., Mariaccia, A., Hauchecorne, A., Ratynski, M., and Khaykin, S.: New observations showing temperature-wind interconnection during mesospheric inversion layer events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7641, https://doi.org/10.5194/egusphere-egu23-7641, 2023.

EGU23-8117 | ECS | PICO | AS4.9

Limb temperature observations in the mesosphere with OMPS 

Pedro Da Costa, Philippe Keckhut, and Alain Hauchecorne

Global observations from space are not numerous and show some disagreements with ground-based NDACC lidars that are not fully explained or do not provide the required vertical resolution to reproduce large fluctuations (20-40 K) due to mesospheric inversions. Comparisons with ERA5 also confirm the lack of variability in the mesosphere. Temperature observations in the mesosphere are biased by migrating atmospheric solar tides with large amplitudes requiring more frequent measurements. Such observations can be easily handled by a constellation of cubesats.

Temperature profiles can be derived by existing satellite missions that were not initially designed for this purpose. This opportunity has been recently tested and processed using GOMOS/ENVISAT observations allowing to provide new and accurate temperature measurements in the mesosphere during 8 years of operation. OMPS/NPP is another limb sensor with a different technical implementation that can expend de 8 years duration of GOMOS to now providing more than 20 years of mesospheric temperature data.

How to cite: Da Costa, P., Keckhut, P., and Hauchecorne, A.: Limb temperature observations in the mesosphere with OMPS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8117, https://doi.org/10.5194/egusphere-egu23-8117, 2023.

EGU23-8239 | ECS | PICO | AS4.9

Correcting infrasound wave parameter estimations using in-situ calibration on defective wind-noise reduction systems 

Samuel Kristoffersen, Alexis Le Pichon, Paul Vincent, Michaela Schwardt, and Franck Larsonnier

Infrasound signals can be detected using a time-delay of arrival approach to derive the back azimuth and trace velocity of the coherent wave. For these calculations, it is necessary to have a calibrated measure of the pressure. Although the calibration of microbarometers can be performed in a laboratory setting with specific metrological means such as those developed by the CEA, it is much more difficult to determine the transfer function of the wind noise reduction systems (WNRS), designed to reduce the wind associated noise. In-situ calibration of these WNRS’s can be performed (as described by Gabrielson*) using a co-located reference sensor and comparing the response to that of the array sensor (considering only highly coherent signals) to determine the relative response of the WNRS. System defects, such as flooded pipes or blocked inlets, have significant impacts on the response, which in turn would influence the calculated infrasonic wave parameters. These defects can be characterized using in-situ calibration measurements. To demonstrate the importance of these measurements, experiments were undertaken at the infrasound station IS26, using a temporary detector whose defects on the WNRS can be produced. This will allow for the effects on real infrasound detections to be quantified and corrected using in-situ calibrations. Comparisons between models of these defects and experimental results allow for the characterization of their effects on infrasound parameter measurements and improvements of the models and WNRS designs.

* Thomas B. Gabrielson, “In situ calibration of atmospheric-infrasound sensors including the effects of wind-noise-reduction pipe systems”, The Journal of the Acoustical Society of America 130, 1154-1163 (2011) https://doi.org/10.1121/1.3613925

How to cite: Kristoffersen, S., Le Pichon, A., Vincent, P., Schwardt, M., and Larsonnier, F.: Correcting infrasound wave parameter estimations using in-situ calibration on defective wind-noise reduction systems, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8239, https://doi.org/10.5194/egusphere-egu23-8239, 2023.

EGU23-11344 | PICO | AS4.9

Sensitivity of the cancellation factor spectral variations for temperature investigation in the mesospheric nightglow layer 

Christophe Bellisario, Pierre Simoneau, Ewen Jaffré, Philippe Keckhut, and Alain Hauchecorne

The infrared emission lines observed between 80 and 100 km known as nightglow allow the investigation of dynamic phenomena such as gravity waves acting on local temperature and density. Swenson and Gardner (1998) introduced the cancellation factor as the link between the nightglow intensity observed and the local temperature. In a previous study, we investigated local changes in spectral intensity using the main source of the nightglow OH. The variations showed dependencies on vibrational levels due to the differences in their reaction coefficients. We now extend the sensitivity study by performing 3D spatial tests. We briefly describe the nightglow evolution model (NEMO), which is developed on a pressure level grid where the gravity wave perturbation is applied. Inherent parameters of the perturbation such as spatial wavelengths are confronted to their impacts on the nightglow layer. In addition, spectral integration over infrared InGaAs camera is applied to allow comparisons with measurement campaigns.

How to cite: Bellisario, C., Simoneau, P., Jaffré, E., Keckhut, P., and Hauchecorne, A.: Sensitivity of the cancellation factor spectral variations for temperature investigation in the mesospheric nightglow layer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11344, https://doi.org/10.5194/egusphere-egu23-11344, 2023.

EGU23-11941 | ECS | PICO | AS4.9

Temperature retrievals from a ground-based, fully polarymetric, 50 GHz radiometer 

Witali Krochin, Gunter Stober, Axel Murk, Roland Albers, and Tobias Plüss

Continuous temperature measurements in the stratosphere (12-50 km) and the mesosphere (50-80 km) are crucial for the deeper
understanding of the physical processes in the middle atmosphere and our understanding of the vertical coupling between the
different atmospheric layers. Several studies have shown the importance of atmospheric waves such as planetary waves, tides,
and gravity waves, their propagation and breaking at these altitudes, and its effect on the global circulation.


Investigating these effects requires long-term measurements with high temporal resolution and altitude coverage. Satellite data
covers the required altitude range but provides limited temporal resolution due to its fixed orbital geometry. Active measurement
techniques such as LIDAR are usually limited to nighttime and only a few instruments have daytime capability and therefore
are unsuitable for continuous observations. Ground-based microwave radiometry provides a robust observational method that
is independent of the daytime, almost independent of the weather conditions, and that permits to perform continuous soundings
from 20-60 km altitude.


TEMPERA (TEMPErature RAdiometer) is a ground-based radiometer developed at the University of Bern in 2013. It measures
microwave radiation spectra from atmospheric oxygen in a range between 52 GHz and 53 GHz. Atmospheric temperature profiles can be retrieved from these spectra. In the last 9 years, the accuracy and performance of this instrument were continuously
improved. The latest version of TEMPERA has a temporal resolution of one measurement per 30 min and temperature profiles
can be retrieved up to an altitude of about 50 km.


The reason for the altitude limitation is the Zeeman effect, which occurs due to the interaction of the atmospheric oxygen with
the Earths magnetic field. The polarisation of atmospheric radiation affected by the Zeeman effect depends on the orientation
of the propagation direction to the magnetic field. Therefore the altitude range for temperature retrievals could be further
improved by decomposing the measured radiation in its polarisation components. In addition, the inclusion of the Zeeman
effect in the retrieval algorithm provides the ability to retrieve the Earths magnetic field from measurements of atmospheric
microwave emissions.


The microwave group from the Institute of Applied Physics of the University of Bern, is currently developing a temperature
radiometer (TEMPERA-C), which is based on the former instrument (TEMPERA), but allows a fully polarymetric analysis of
the atmospheric emission spectra. In my talk I will present the technical details of TEMPERA-C as for example the challenges
in the calibration process. Furthermore I will present calibrated measurements of circular polarized atmospheric emission
spectra as well as temperature retrievals and discuss the effect of the Earth’s magnetic field on these measurements.

How to cite: Krochin, W., Stober, G., Murk, A., Albers, R., and Plüss, T.: Temperature retrievals from a ground-based, fully polarymetric, 50 GHz radiometer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11941, https://doi.org/10.5194/egusphere-egu23-11941, 2023.

EGU23-11977 | ECS | PICO | AS4.9 | Highlight

Using a machine learning and stochastics-founded model to provide near real-time stratospheric polar vortex diagnostics based on high-latitude infrasound data 

Mari Eggen, Alise Danielle Midtfjord, Ekaterina Vorobeva, Fred Espen Benth, Patrick Hupe, Quentin Brissaud, Yvan Orsolini, Alexis Le Pichon, Constantino Listowski, and Sven Peter Näsholm

Acoustic waves below the frequency limit of human hearing - infrasound - can travel for thousands of kilometres in the atmosphere. The global propagation signature of infrasound is highly sensitive to the wind structure of the stratosphere. 

This work exploits processed continuous data from three high-latitude infrasound stations to characterize an aspect of the stratospheric polar vortex. Concretely, a mapping is developed which takes the infrasound data from these three stations as input and outputs an estimate of the polar cap zonal mean wind averaged over 60-90 degrees in latitude at the 1 hPa pressure level. This stratospheric diagnostic information is relevant to, for example, sudden stratospheric warming assessment and sub-seasonal prediction.

The considered acoustic data is within a low-frequency regime globally dominated by so-called microbarom infrasound, which is continuously radiated into the atmosphere due to nonlinear interaction between counter-propagating ocean surface waves. 

We trained a stochastics-based machine learning model (delay-SDE-net) to map between a time series of five years (2014-2018) of processed infrasound data and the ERA5 (reanalysis-based) daily average polar cap wind at 1 hPa for the same period. The ERA5 data was hence treated as ground-truth. In the prediction, the delay-SDE-net utilizes time-lagged inputs and their dependencies, as well as the day of the year to account for seasonal differences. In the validation phase, the input was the 2019 and 2020 infrasound time series, and the model inference results in an estimate of the daily average polar cap wind time-series. This result was then compared to the ERA5 representation of the stratospheric diagnostic time-series for the same period. 

The applied machine learning model is based on stochastics and allows for an interpretable approach to estimate the aleatoric and epistemic prediction uncertainties. It is found that the mapping, which is only informed of the trained model, the day of year, and the infrasound data from three stations, generates a 1 hPa polar cap average wind estimate with a prediction error standard deviation of around 10 m/s compared to ERA5.

Focus should be put on the winter months because this is when the coupling between the stratosphere and the troposphere can mostly influence the surface conditions and provide additional prediction skill, in particular during strong and weak stratospheric polar vortex regimes. The infrasound data is available in real-time, and we discuss how the developed approach can be extended to provide near real-time stratospheric polar vortex diagnostics.

How to cite: Eggen, M., Midtfjord, A. D., Vorobeva, E., Benth, F. E., Hupe, P., Brissaud, Q., Orsolini, Y., Le Pichon, A., Listowski, C., and Näsholm, S. P.: Using a machine learning and stochastics-founded model to provide near real-time stratospheric polar vortex diagnostics based on high-latitude infrasound data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11977, https://doi.org/10.5194/egusphere-egu23-11977, 2023.

EGU23-12236 | ECS | PICO | AS4.9

Seismic and infrasound monitoring of military conflicts using machine learning 

Quentin Brissaud, Erik Myklebust, Ben Dando, Bettina Goertz-Allmann, Andreas Köhler, Johannes Schweitzer, and Tormod Kvaerna

The real-time seismo-acoustic monitoring of military conflicts can provide a unique alternative to conventional ground reports and sparse satellite coverage. The pressure waves generated by an explosion travel through the atmosphere and subsurface as sound and seismic waves, and their signature can be recorded by arrays of seismometers for ground motion or microbarometers for sound propagation. However, standard monitoring techniques can be both computationally expensive when localizing signals over large regions and/or prone to false detections when signals have low amplitudes. In this contribution we propose a Machine-Learning (ML) based solution to detect seismic and infrasound arrivals and locate sources close to real time. To validate our model we leverage the seismic data collected during the Russia-Ukraine conflict started in February 2022 using the Ukrainian primary station of the International Monitoring System (IMS), the Malin array (AKSAG). We test both the accuracy and computational efficiency of our approach against a threshold-based migration stacking model developed for near-real time monitoring in Ukraine. We hope that this first-ever ML detector of both seismic and acoustic phases could be employed for real-time monitoring of conflicts around the world across different network geometries and noise conditions.

How to cite: Brissaud, Q., Myklebust, E., Dando, B., Goertz-Allmann, B., Köhler, A., Schweitzer, J., and Kvaerna, T.: Seismic and infrasound monitoring of military conflicts using machine learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12236, https://doi.org/10.5194/egusphere-egu23-12236, 2023.

EGU23-13242 | PICO | AS4.9 | Highlight

25 years of infrasound monitoring: achievements and challenges 

Elisabeth Blanc, Alexis Le Pichon, Thomas Farges, Constantino Listowski, and Pierrick Mialle

The infrasound International Monitoring System (IMS, ) is a unique tool for atmospheric observations due to its high capacity for long-range detection and localisation. Its development, starting in the nineties, motivated technological innovations in sensors, array stations, network configuration and automatic detection algorithms. The rapidly increasing number of certified stations detected a large diversity of anthropic and natural infrasound events, well identified thanks to their accurate description. Numerical simulations, based on propagation laws and atmospheric models, determined the IMS specifications for infrasound monitoring. They were revisited at the end of the 2000s, integrating an improved representation of the variable atmospheric environment, showing the high performances of the network. Data analyses clearly demonstrated that most uncertainties originate from the middle atmosphere disturbances, which control the infrasound waveguides and are under-represented in models. Unexpectedly, relevant atmospheric parameters were identified in infrasound signals from well-known sources such as volcanoes, opening new infrasound remote sensing possibilities. The association of the infrasound IMS to complementary multi-instrument platforms provided new middle atmosphere data, needed for the determination of uncertainties in atmospheric models and infrasound simulations for more precise event analyses. New methods are developed for middle atmospheric remote sensing from IMS infrasound ocean swell noise observations. Such global observations could be relevant for future data assimilation systems used in numerical weather prediction models. A remote volcano information system is developed to provide in the future notification to civil aviation in case of large eruptions of non-instrumented volcanoes. Large-scale climatology systems, such as the inter-tropical convergence zone (ITCZ) of the winds and the semi-annual oscillation (SAO) of stratospheric winds were recently identified. They can provide relevant information about the evolution of climate related parameters. This shows the high IMS potential for weather, climate and civil safety applications.

How to cite: Blanc, E., Le Pichon, A., Farges, T., Listowski, C., and Mialle, P.: 25 years of infrasound monitoring: achievements and challenges, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13242, https://doi.org/10.5194/egusphere-egu23-13242, 2023.

EGU23-13253 | ECS | PICO | AS4.9

IMS infrasound data products for atmospheric studies and civilian applications – 2021 and 2022 updates 

Patrick Hupe, Lars Ceranna, Alexis Le Pichon, Robin S. Matoza, and Pierrick Mialle

We present recent and planned updates of the infrasound data products of all certified infrasound stations of the International Monitoring System, which was established in the late 1990s for verification of the Comprehensive Nuclear-Test-Ban Treaty (CTBT). The updates extend the four data products initially published for the 2003 to 2020 period (https://doi.org/10.5194/essd-14-4201-2022) by two years and thus complete a 20-year period.

Our intention for these data products is to facilitate using this unique global infrasound dataset for scientific applications. The products open up the IMS observations to user groups who do not have access to IMS data or are unfamiliar with data processing using the Progressive Multi-Channel Correlation (PMCC) method. We demonstrate the updated data products based on recent and global infrasound sources such as volcanic eruptions and ocean ambient noise and highlight the provided detection and quality parameters.

How to cite: Hupe, P., Ceranna, L., Le Pichon, A., Matoza, R. S., and Mialle, P.: IMS infrasound data products for atmospheric studies and civilian applications – 2021 and 2022 updates, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13253, https://doi.org/10.5194/egusphere-egu23-13253, 2023.

EGU23-14786 | PICO | AS4.9

Small aperture infrasound array in the Antarctic Peninsula region - the first observations experience 

Oleksandr Liashchuk, Yurii Andrushchenko, and Yurii Otruba

At the Ukrainian Antarctic Akademik Vernadsky station deployed a significant multidisciplinary complex of equipment, some of which has been providing data to the scientific community for more than half a century. In addition to existing measuring instruments, a small aperture infrasound array was installed at the Vernadsky Station in 2021. The distance between the Chaparral Physics Model 64Vx sensors is 100 meters. The shape of the array is in the form of a triangle with a central element. The signal from the sensor goes by wire to a four-channel 24-bit ADC and then to the SeisComP server, where the data archive is formed in the miniSEED format. Since 2022, data has been transmitted in real time via the SeedLink protocol via satellite internet to the National Data Center, where it is processed.

During the observation, a large number of interesting regional and global signals associated with the calving of icebergs, avalanches, tsunamis, and storm processes were recorded by the array. At the beginning of 2022, together with the global infrasound network, signals from the eruption of the Hunga volcano, Tonga, were also recorded at the infrasound array of the Vernadsky station.

During registration, some technical issues were discovered that need to be upgraded, in particular, to improve the noise reduction and power systems. It is also necessary to increase the aperture of the array.

In general, the infrasonic array showed good survivability and the ability to record a wide range of phenomena in the Antarctic Peninsula region. Processing of its data in combination with data from neighboring infrasound arrays of the International Monitoring System CTBTO in a number of cases makes it possible to locate and identify the source of the signal. In addition, the current observational experience can be used in the installation of the IMS infrasound station in the Antarctic Peninsula region, as previously planned.

How to cite: Liashchuk, O., Andrushchenko, Y., and Otruba, Y.: Small aperture infrasound array in the Antarctic Peninsula region - the first observations experience, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14786, https://doi.org/10.5194/egusphere-egu23-14786, 2023.

In order to reduce the observation of wind and turbulence on infrasound sensors, wind noise reduction filters are in place at most infrasound stations. The use of such filters is essential to obtain low background noise levels, which in turn facilitates detection of low signal-to-noise (SNR) infrasound signals. Most filters operate by spatially integrating the pressure field in the vicinity of an infrasound sensor. While the turbulent pressure (partially) de-correlates over the spatial length scale of the filter, the infrasound wave remains coherent. Infrasound arrays that are part of the International Monitoring System make use of advanced pipe array structures that have been designed for long-term deployments. The response is of these systems is stable and well understood. In contrast, many experimental infrasound arrays have relied on the use of porous hoses for wind noise reduction. Porous hoses appear to be efficient, yet cost-effective solutions for short term deployments. Over longer timescales, however, it is known that the response of the hoses can vary significantly and that the hoses can degrade over time.

 

In this work, we investigate the varying response of the porous hoses at the De Bilt Infrasound Array in the Netherlands, using a reference infrasound sensor without hoses. Since a weather station is co-located with the infrasound array, this allows us to study the relationship between the response of the hoses and various meteorological parameters. It is found that under dry conditions, the hoses act as a low-pass filter with a corner frequency around 1.8 Hz, which is consistent with earlier work. We shows that the higher frequency signals with sufficient SNR can be reasonably well reconstructed after a deconvolution step. Under wet conditions however, the hoses become highly absorptive. This can affect observations down to 0.1 Hz. The excess attenuation can be attributed to the presence of rain and/or dew. Although these effects appear to be reversible to some degree, this work shows that care must be taken in the interpretation of data from infrasound arrays that make use of porous hoses.

How to cite: Assink, J.: How does the weather affect the response of porous hose wind noise reduction systems?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15769, https://doi.org/10.5194/egusphere-egu23-15769, 2023.

EGU23-17492 | ECS | PICO | AS4.9

The use of infrasound monitoring in the 2022 São Jorge Island (Azores) seismovolcanic crisis 

Sandro Matos, Maria do Céu Jesus, and Nicolau Wallenstein and the CIVISA team²

Located in the middle of the North Atlantic Ocean, São Jorge is a volcanic island that belongs to the central group of the Azores Archipelago, Portugal. Very steep, with 54 km long and 7 km wide, São Jorge is different from all the other archipelago’s islands, being itself a WNW-ESE oriented fissure volcanic system composed of four volcanic units.

Since March 19, 2022, a seismovolcanic crisis has been ongoing beneath the active Manadas Volcanic Fissure System on the western half of the island, where historical eruptions occurred in 1580 and 1808. This unrest, characterized by the occurrence of several thousands of low magnitude earthquakes and some ground deformation, is being monitored by IVAR/CIVISA teams using several techniques (seismology, geodesy, infrasound, ground water geochemistry and CO2 and 222Rn emissions).

Infrasound detections were based on data from the IMS IS42 infrasound station located on the Graciosa Island (Azores) and a portable infrasound array (SJ1) that was deployed in the northwestern part of the island at ~7 km from the main epicentral area.

We describe the actual procedures to correlate seismic and infrasonic data, based on epicentral locations and infrasound back-azimuths and the main results obtained so far.

How to cite: Matos, S., do Céu Jesus, M., and Wallenstein, N. and the CIVISA team²: The use of infrasound monitoring in the 2022 São Jorge Island (Azores) seismovolcanic crisis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17492, https://doi.org/10.5194/egusphere-egu23-17492, 2023.

EGU23-185 | Orals | GI6.8

Space weather during extreme SEPs: new assessment of worst case scenario 

Alexander Mishev, Sanja Panovska, and Ilya Usoskin

An important topic in the field of space physics is the quantification of the cosmic-ray-induced effects in the atmosphere and the corresponding space weather effects. Space weather effects, specifically the exposure to radiation at aviation altitudes, represent an important threat. Here, we focus on a specific class of events due to solar energetic particles (SEPs), viz. events that can be registered at ground level: ground-level enhancements and more particularly extreme events with cosmogenic imprints,i.e. that have been registered by 14C records.

Naturally, for assessment of space weather effects during extreme SEP events, it is necessary to possess precise information on their spectra. Here we present results and application of an analysis of SEPs using neutron monitor (NM) records, that is derivation of their spectra, and application of numerical models. Using reconstructed spectra during the strongest directly recorded event, that is GLE # 5, occurred on 23 February 1956, and employing a convenient rescaling,  we assessed the space weather effect during the strongest indirectly reconstructed historical extreme SEP event, that is, 774 AD. Subseqeuntly, employing a state-of-the-art reconstruction of the magnetic field we study the worst-case scenario representing a combination of a geomagnetic excursion, that is the Laschamp excursion ca. 42 kyr ago and a 774 AD-like event. The possible implications are discussed.

How to cite: Mishev, A., Panovska, S., and Usoskin, I.: Space weather during extreme SEPs: new assessment of worst case scenario, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-185, https://doi.org/10.5194/egusphere-egu23-185, 2023.

EGU23-287 | ECS | Orals | GI6.8

A New Open-Source Geomagnetosphere Propagation Tool (OTSO) and its Applications 

Nicholas Larsen, Alexander Mishev, and Ilya Usoskin

We present a new open-source tool for magnetospheric computations, that is modelling of cosmic ray propagation in the geomagnetosphere, named "Oulu - Open-source geomagneToSphere prOpagation tool" (OTSO). A tool of this nature is required to interpret experiments and study phenomena within the cosmic ray research field.  Here, we demonstrate several applications of OTSO, namely the computation of asymptotic directions of selected cosmic ray stations, effective rigidity cut-off across the globe at various conditions within the design, and general properties, including the magnetospheric models employed. OTSO was applied to the investigation of several ground-level enhancement events after which comparison and validation of OTSO with older widely used tools such as MAGNETOCOSMICS was performed, and good agreement was achieved. The necessary background for the analysis of two notable ground-level enhancements was produced using OTSO and their spectral and angular characteristics show good agreement with prior studies and spacecraft data. This validation of OTSO's current abilities reveals its usefulness to the cosmic ray research field and its open-source nature further allows for the tool to be developed beyond its current capabilities by users to meet the needs of the research community.

How to cite: Larsen, N., Mishev, A., and Usoskin, I.: A New Open-Source Geomagnetosphere Propagation Tool (OTSO) and its Applications, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-287, https://doi.org/10.5194/egusphere-egu23-287, 2023.

EGU23-3095 | Posters on site | GI6.8

Effects of heterogeneous soil moisture distributions in cosmic-ray neutron sensing - the case of irrigation monitoring 

Heye Bogena, Cosimo Brogi, Markus Köhli, Harrie-Jan Hendricks Franssen, Olga Dombrowski, and Johan Alexander Huisman

Soil moisture (SM) sensors are widely used to monitor soil water dynamics and support irrigation management with the aim of achieving better yields while reducing water consumption. Unfortunately, due to the small measuring volume of point-scale sensors, their soil moisture readings are often not representative for heterogeneous agricultural fields. Therefore, in such cases, sensors with larger sensing volume are needed to address spatially variable SM. A suitable technique is the cosmic ray neutron sensor (CRNS) as it integrates SM over a large volume with a radius of ~130-210 m and a penetration depth of ~15-85 cm. The CRNS method is based on the inverse relationship between measured environmental neutron density and the presence of hydrogen pools (e.g., SM) in the instrument surroundings. However, the ability of CRNS to accurately monitor areas with complex SM heterogeneities (e.g., small irrigated fields) and the influence of detector design were not yet investigated. In this study, we used the neutron transport model URANOS to simulate the effect of SM variations on a CRNS placed in the centre of squared irrigated fields (0.5 to 8 ha dimensions). For this, SM in the irrigated field and in the surrounding was altered between 0.05 and 0.50 cm3 cm-3 (500 simulations in total). In addition, we investigated the effect of employing high-density polyethylene (HDPE) moderators with different thickness (5 to 35 mm) as well as a 25 mm HDPE moderator with an additional gadolinium oxide thermal shielding. Results showed that, in heterogeneous SM scenarios, the 2 e-folding lengths footprint (R86) can become smaller or larger than what previous studies showed in homogeneous SM distributions. In addition, a thin HDPE moderator will result in relatively smaller R86 whereas thicker moderators and the addition of a thermal shielding will result in relatively larger R86. However, we found that a relatively small footprint is not directly related to a better monitoring of SM nearby the instrument. In fact, in all the investigated field dimensions, the 25mm HDPE moderator with gadolinium shielding showed the largest values of R86 but also the largest variations of detected neutrons with changing SM. In addition, such moderator showed the highest chances of detecting irrigation events that increase SM by 0.05 or 0.10 cm3 cm-3 in the irrigated area. Generally, detection was uncertain only for SM variations of 0.05 cm3 cm-3 in fields of 0.5 ha when initial SM was 0.02 cm3 cm-3 or higher. Although the results of this study suggest the feasibility of monitoring and informing irrigation with CRNS, we found that SM variations outside the irrigated field have a considerable influence on CRNS measurements. Especially in fields of 0.5 and 1 ha dimension, it can be impossible to distinguish whether a relative change in detected neutrons is due to irrigation or to SM variations in the surroundings. These results are relevant for irrigation monitoring and the combination of neutron transport simulations and real-world installations has the potential to establish CRNS as a decision support system for irrigation management.

How to cite: Bogena, H., Brogi, C., Köhli, M., Hendricks Franssen, H.-J., Dombrowski, O., and Huisman, J. A.: Effects of heterogeneous soil moisture distributions in cosmic-ray neutron sensing - the case of irrigation monitoring, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3095, https://doi.org/10.5194/egusphere-egu23-3095, 2023.

EGU23-4506 | Orals | GI6.8

ORCA (Observatorio de Rayos Cósmicos Antártico), current status and future perspectives 

Juan José Blanco, Juan Ignacio García Tejedor, Sindulfo Ayuso de Gregorio, Óscar García Población, Alejandro López-Comazzi, Diego Sanz Martín, Ivan Vrublevskyy, Laura Gonzalvo Ballano, and Alberto Regadío

ORCA (2.37 GV) is a suit of two neutron monitors and a muon telescope. It was installed at Juan Carlos I Antarctic Base on January 2019 being in operation since. Because the low level of the solar activity, only a few of solar events have been detected. The GLE 73 and three Forbush decreases. A new ORCA like detector (ICaRO, 11.5 GV) is being installed at 2200 m a.s.l in Izaña Atmospheric Observatory (Tenerife Island, Spain). On the other hand, CaLMa neutron monitor (6.95 GV) will be updated with a muon telescope made by eight 1 m2 scintillators arranged in two layers of four scintillators at some point during the next two years. These three detector will measure muons and neutrons from cosmic ray interaction with atmosphere at three different locations allowing to study the solar activity from a new perspective

How to cite: Blanco, J. J., García Tejedor, J. I., Ayuso de Gregorio, S., García Población, Ó., López-Comazzi, A., Sanz Martín, D., Vrublevskyy, I., Gonzalvo Ballano, L., and Regadío, A.: ORCA (Observatorio de Rayos Cósmicos Antártico), current status and future perspectives, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4506, https://doi.org/10.5194/egusphere-egu23-4506, 2023.

EGU23-6045 | Posters on site | GI6.8

The concentration of cosmogenic radionuclide 7Be from the perspective of space weather and long-term trends in the stratospheric temperature and wind 

Kateřina Podolská, Michal Kozubek, Miroslav Hýža, and Tereza Šindelářová

Cosmogenic radionuclide Beryllium 7Be concentration is primarily determined by the solar activity level and space weather conditions. The 7Be is generated by cosmic ray reactions in the stratosphere and in the upper troposphere, binds to atmospheric aerosols and is transported horizontally and vertically by wind and gravity. The highest values of cosmic radiation are observed during the solar minima because, at that time the penetrability of the Earth’s and Sun magnetosphere is greatest.

The concentrations of the radionuclide 7Be are reliable indicators of various atmospheric processes. In our work, we try to contribute to better understanding of the dynamics of processes by associating them with long-term trends of stratospheric temperature dynamics. We investigate the coupling of concentrations of the cosmogenic radionuclide 7Be in the longitudinal view during the years 1986–2022 (time series of activity concentration of 7Be in aerosols evaluated by the corresponding activity in aerosols on a weekly basis at the National Radiation Protection Institute Monitoring Section in Prague) to space weather parameters (Kp planetary index, disturbance storm time Dst, proton density, proton flux), and stratospheric dynamics parameters (temperature, zonal component of wind, O3). On short timescales the intensity of cosmic radiation decreases by few percent in several days. On a longer timescale the intensity of galactic cosmic rays is strongly influenced by the degree of solar activity and by variations in the geomagnetic field. This corresponds with findings that the zonal wind climatology differences were largest in the decades of 2000–2010 than between others observed decades.

How to cite: Podolská, K., Kozubek, M., Hýža, M., and Šindelářová, T.: The concentration of cosmogenic radionuclide 7Be from the perspective of space weather and long-term trends in the stratospheric temperature and wind, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6045, https://doi.org/10.5194/egusphere-egu23-6045, 2023.

EGU23-6789 | Posters on site | GI6.8

Sensitivity of the Cosmic Ray Neutron Sensor (CRNS) to Seasonal Biomass Dynamics in Cherry and Olive Orchards 

Samir K. Al-Mashharawi, Marcel M. El Hajj, Kasper Johansen, Matthew F. McCabe, and Susan Steele-Dunne

Biomass estimation is important in many applications, such as carbon sequestration and precision agriculture. Developing a reliable method for biomass estimation from satellite, airborne and near-surface remote sensing sensors is an ongoing task due to the large uncertainty in current methods, which are often related to sensor limitations. Indeed, signals from optical sensors and synthetic aperture radar at high and medium frequencies suffer from saturation issues at high biomass levels. The Cosmic-Ray Neutron Sensor (CRNS) is a new non-invasive near-surface sensor used primarily to estimate soil water content (SWC), but it has also shown potential for retrieving other hydrological and environmental parameters such as biomass water equivalent and snow depth. The CRNS detects and counts the number of neutrons controlled by hydrogen atoms in the soil, air just above the ground, and vegetation. Biomass attenuates the intensity of cosmic ray neutrons, hence the ability to estimate biomass from a CRNS. Recent studies have used CRNS measurements to estimate biomass changes in crop areas and forest stands, while the use of CRNSs in orchards is limited. The objective of this study is to explore the potential of two CRNSs to estimate the biomass variation in irrigated cherry and olive tree orchards. The olive tree orchard is located in an arid region in northern Saudi Arabia (plantation density of 1667 trees/hectare) with an average tree height of 3 m and canopy diameter of 2 m. The cherry field is located in southern France (plantation density of 260 trees/hectare) with an average tree height of 3.5 m and canopy diameter of 5.5 m. Several soil moisture probes recording soil water content (SWC) at 15-min intervals at both sites were installed at different depths within the CRNS footprint. SWC measurements were used to assess the variations in the sensitivity of CRNS to soil moisture with increasing biomass. Tree parameters (height, canopy width, canopy length, leaf area index, and diameter at breast height) were measured in situ to estimate biomass using allometric equations. In addition, repetitive Light Detection and Ranging (LiDAR) scanning was performed over the cherry field to detect canopy volume changes over time. The results showed that the CRNS is sensitive to SWC variation, and this sensitivity is controlled by biomass evolution, indicating that CNRS measurements can also be used to estimate biomass. The sensitivity of CRNS neutron counts to SWC in the early season (before blooming) was twice as high as that during the mid- and late growing seasons (maximum leaf cover). The Cornish Pasdy model­, which models the measured neutron counts as a function of SWC and biomass contribution, was calibrated and then inverted to estimate the biomass in the cherry and olive tree orchards. 

How to cite: Al-Mashharawi, S. K., El Hajj, M. M., Johansen, K., McCabe, M. F., and Steele-Dunne, S.: Sensitivity of the Cosmic Ray Neutron Sensor (CRNS) to Seasonal Biomass Dynamics in Cherry and Olive Orchards, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6789, https://doi.org/10.5194/egusphere-egu23-6789, 2023.

EGU23-11071 | ECS | Posters on site | GI6.8

Updated heliospheric modulation potential of cosmic rays and station-specific scaling factors for 1964-2021 

Pauli Väisänen, Ilya Usoskin, Riikka Kähkönen, Sergey Koldobskiy, and Kalevi Mursula

Galactic cosmic rays (GCR) are energetic particles originating from galactic or extra-galactic sources. When they arrive inside our heliosphere, they are modulated by the magnetic irregularities in the solar wind flow from the Sun, deflecting and slowing down the GCR particles. The level of this modulation varies according to solar activity, especially the 11-year solar cycle. The heliospheric modulation potential, denoted by ϕ, describes the average energy loss of particle in MV and quantifies the level of modulation. It can be determined using ground-based neutron monitor (NM) measurements of GCRs by multiple stations. Here we use the most recent version of the NM yield function and a RMSE-minimization method to compute a new and more accurate version of the modulation potential ϕ and station-specific scaling factors κ, which can be used to scale the level of count rates to the theoretical NM count rate given by the model. The new version offers daily resolution of ϕ and can be conveniently updated with new measurements, stations, or updates to datasets whenever they might occur. The scaling factors and their variation can be used to scale the data for physical analyses or to identify outliers, errors or physical phenomena which do not match with the model.

How to cite: Väisänen, P., Usoskin, I., Kähkönen, R., Koldobskiy, S., and Mursula, K.: Updated heliospheric modulation potential of cosmic rays and station-specific scaling factors for 1964-2021, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11071, https://doi.org/10.5194/egusphere-egu23-11071, 2023.

EGU23-11326 | ECS | Posters on site | GI6.8

Monitoring soil moisture in the deeper vadose zone: A new approach using groundwater observation wells and cosmic ray neutrons 

Daniel Rasche, Jannis Weimar, Martin Schrön, Markus Köhli, Markus Morgner, Andreas Güntner, and Theresa Blume

Monitoring soil moisture at depths greater than one meter is generally challenging and often highly invasive as it requires opening large soil pits. As a result, this deeper vadose zone is often not monitored at all. On top of that, conventional soil moisture sensors usually have only a small measurement volume. On the other hand, soil moisture estimates derived from above-ground Cosmic-Ray Neutron Sensing (CRNS) are a representative average over an area of several hectares but only of the upper half meter of the soil. To this day, it is commonly believed that cosmic radiation cannot be used to monitor soil water content below this depth. As a consequence, large parts of the root-zone and deeper unsaturated zone have remained outside the observational window of the method. The estimation of soil moisture in greater depths typically requires additional invasive measurements, other active geophysical methods, or mathematical models which extrapolate surface soil moisture observations.

Against this background, we investigated the possibility of using passive detection of cosmogenic neutrons in existing monitoring infrastructure (e.g. groundwater wells). We hypothesized that this method provides a larger measurement volume than traditional techniques based on active neutron probes while requiring less safety restrictions.

Our neutron transport simulations demonstrated that this downhole-CRNS technique would be sensitive enough to detect changes of water content in depths down to 5 meters and above, depending on the temporal resolution of measurements. The simulations also revealed a large measurement radius of several tens of cm depending on the soil moisture content and soil bulk density.

From the theoretical results we derived a functional relationship between soil moisture and detectable neutrons and tested it in a groundwater observation well. Additional installations of supporting soil moisture sensors have been used to validate the model predictions as well as the neutron signals monitored by the CRNS detector. The study demonstrated the general applicability of downhole Cosmic-Ray Neutron Sensing for the estimation of soil moisture in greater depths and at temporal resolution of two days.

How to cite: Rasche, D., Weimar, J., Schrön, M., Köhli, M., Morgner, M., Güntner, A., and Blume, T.: Monitoring soil moisture in the deeper vadose zone: A new approach using groundwater observation wells and cosmic ray neutrons, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11326, https://doi.org/10.5194/egusphere-egu23-11326, 2023.

EGU23-11905 | Posters virtual | GI6.8

SEVAN European particle detector network for the atmospheric, solar and space weather studies 

Tigran Karapetyan, Ashot Chilingarian, and Balabek Sargsyan

Experiments during recent years with SEVAN detectors on mountain tops in Armenia, Slovakia, and Bulgaria reveal the broad potential of SEVAN detectors; The SEVAN detector on Lomnicky Stit (Slovakia) measured the largest thunderstorm ground enhancements (TGE), with particle fluxes exceeding the background 100-times. With muon and gamma ray fluxes, the maximum values of the potential difference in thunderclouds were measured, equal to 350 MV at Mt. Aragats, and 500 MV at the sharp peak of Lomnicky Stit. In Nov 2019, SEVAN detectors were installed at DESY (Hamburg and Zeuthen sites). Fluxes of electrons, photons, and muons and weather parameters are continuously monitored at all sites (at different latitudes, longitudes, and altitudes). To fully exploit the scientific potential of the SEVAN detectors, in 2023 is planned to install a new detector in the Umwelt-Forschungs-Station (UFS, Schneefernerhaus, 2650 m asl) near the top of the Zugspitze (2962 m), a site with a long history of atmospheric research. The new SEVAN module will be compact (SEVAN-light), and will enable the energy spectra measurements in the range from 0.3 to 50 MeV, allowing unambiguously separating Radon progeny gamma radiation from runaway electron-photon avalanches.

How to cite: Karapetyan, T., Chilingarian, A., and Sargsyan, B.: SEVAN European particle detector network for the atmospheric, solar and space weather studies, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11905, https://doi.org/10.5194/egusphere-egu23-11905, 2023.

Neutron monitor counting rates show, among others, a  $\sim$ 1.6--2.2-year period. This period has been associated with a solar origin affecting the cosmic ray propagation conditions through the heliosphere. The duration of this period varies from one Solar Cycle to another.
\cite{Comazzi_Blanco_2022} found the duration of the $\sim$ 1.6--2.2-year period ($\tau$) is linearly related to the averaged sunspot number ($SSN_a$) in each Solar Cycle.
In this piece of research, we have analyzed this relationship. This equation shows that shorter $\sim$1.6--2.2-year periods occur during stronger cycles when $SSN_a$ is higher. Drawing on this relationship given by $SSN_a = (-130 \pm 10) \: \tau + (330 \pm 30)$, we computed $\tau$ for the cycles previous to the existence of neutron monitors (Solar Cycles 7--19). 
By means of the Huancayo neutron monitor spectrum we checked the validity of this equation along the Solar Cycle 19. 
Once the previous relationship is checked, $\tau$ for the current Solar Cycle 25 is computed giving $\sim$ 2.22 years.

An internal mechanism of the solar dynamo called Rossby waves could produce these variations in the solar magnetic field  and, indirectly, in neutron monitor counting rates.
The harmonic of fast Rossby waves with $m=1$ and $n=8$ fit with the detected periodicity and the variation of the solar magnetic field strength from weaker to stronger Solar Cycles could explain the different periods detected in each cycle.
Finally, a solar magnetic field strength of $\sim$ 7--25 kG in the tachocline have been estimated based on the detected periodicities using the dispersion relation for fast Rossby waves. 

How to cite: López-Comazzi, A. and Blanco-Ávalos, J. J.: Study of the relationship between Sunspot number and the duration of the $\sim$1.6--2.2-year period in neutron monitor counting rates, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11981, https://doi.org/10.5194/egusphere-egu23-11981, 2023.

EGU23-12576 | ECS | Posters on site | GI6.8

Cosmic rays on snow: A combined analysis of fractional snow cover derived from Sentinel-2, MODIS and Cosmic Ray Neutron Sensors across Europe 

Nora Krebs, Paul Schattan, Sascha Oswald, Martin Schrön, Martin Rutzinger, and Johann Stötter

Epithermal neutrons from cosmic ray showers are slowed by hydrogen atoms in snow. The drop in the fast neutron abundance in the atmosphere can be measured with above-ground Cosmic Ray Neutron Sensing (CRNS), allowing for an estimation of the Snow Water Equivalent (SWE). SWE is an important variable that has a substantial role in hydrological modelling and forecasts. However, up to now, SWE is conventionally measured at point-scale, which holds only little information about the average SWE in areas of heterogeneous terrain and where snow drift is a predominant process. CRNS offers the prospect of closing this gap by sensing neutrons within a footprint of 10–20 hectares. Currently, further investigations are needed to reduce the uncertainties in the signal conversion from neutron counts to SWE. In this study, we compare the daily signals of 65 CRNS stations across Europe with the corresponding Fractional Snow Cover (FSC) products from Sentinel-2 and MODIS (Moderate-resolution Imaging Spectroradiometer) with a 20 m and 500 m spatial resolution, respectively. By analysing the FSC products, we were able to identify characteristic ranges of neutron counts at snow presence (winter signals) and absence (summer signals). Comparing these ranges and their overlap among stations, we were able to distinguish typical signal properties of lowland, pre-Alpine and Alpine sites. We found that altitude-related properties, such as soil and vegetation characteristics govern the general neutron level at the study sites. Snowfall typically leads to a major drop in the neutron count rate that is superimposed on the summer neutron count level. High-altitude stations are generally characterized by low ranges of count rates in summer and by high ranges in winter, while low-altitude stations show a reversed trend. Our results demonstrate that the suitability of a station for SWE measurements with CRNS depends highly on the site-specific hydrogen pool fluctuations that can be linked to altitude. Especially in heterogeneous mountain terrain with low soil formation, the advantages of CRNS come into play and can provide a spatial average of SWE with low uncertainties.

How to cite: Krebs, N., Schattan, P., Oswald, S., Schrön, M., Rutzinger, M., and Stötter, J.: Cosmic rays on snow: A combined analysis of fractional snow cover derived from Sentinel-2, MODIS and Cosmic Ray Neutron Sensors across Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12576, https://doi.org/10.5194/egusphere-egu23-12576, 2023.

EGU23-15343 | Posters on site | GI6.8

Measurements of cosmic rays by a mini neutron monitor aboard the German research vessel Polarstern 

Bernd Heber, Sönke Burmeister, Hanna Giese, Konstantin Herbst, Lisa Romaneehsen, Carolin Schwerdt, Du Toit Strauss, and Michael Walter

Neutron monitors are ground-based devices that measure the secondary particle population, i.e., neutrons produced by, e.g., galactic cosmic rays (GCRs). Due to their functionality, they are integral counters whose flux is proportional to the variation of the input spectrum. However, the measured flux also depends on the geomagnetic position and the static pressure at the monitor's location. To better understand the instrument response, the Christian-Albrechts-Universität zu Kiel, DESY Zeuthen, and the North-West University in Potchefstroom, South Africa, agreed on regular monitoring of the GCR intensity as a function of latitude, by installing a portable device aboard the German research vessel Polarstern in 2012. The vessel is ideally suited for this research campaign because it covers extensive geomagnetic latitudes (i.e., goes from the Arctic to the Antarctic) at least once per year. Since the installation aboard the vessel, 12 latitude scans were performed, allowing us to compute the so-called yield function by experimental means presented in this contribution.

The Kiel team received funding from the European Union's Horizon 2020 research and innovation program under grant agreement No 870405. The team would like to thank the crew of the Polarstern and the AWI for supporting our research campaign.

How to cite: Heber, B., Burmeister, S., Giese, H., Herbst, K., Romaneehsen, L., Schwerdt, C., Strauss, D. T., and Walter, M.: Measurements of cosmic rays by a mini neutron monitor aboard the German research vessel Polarstern, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15343, https://doi.org/10.5194/egusphere-egu23-15343, 2023.

EGU23-15523 | Posters on site | GI6.8

Buoy-based detection of low-energy cosmic-ray neutrons to monitor the influence of atmospheric effects 

Martin Schrön, Daniel Rasche, Jannis Weimar, Markus Köhli, Bertram Boehrer, Peter Dietrich, and Steffen Zacharias

Neutron monitors on the Earth’s surface are usually used to observe the dynamics of highly energetic cosmic-ray particles, assuming that local environmental conditions do not influence the measurement. In another young research field, low-energy cosmic-ray neutrons are used to monitor local dynamics of environmental water content. Water in soil, air, snow and vegetation determines the amount of ground albedo neutrons in the sensitive energy range from 1 eV to 100 keV. Plenty of small neutron detectors are operated on natural or agricultural sites all around the world. 

A major issue is the modulation of the neutron flux by the dynamics of incoming high-energy cosmogenic particles. Conventionally, independent data from neutron monitors are consulted to serve as a reference for the correction of the local detectors. However, the performance of this comparative correction approach is unreliable, because it does not account for geographical displacement, different energy windows of the detectors, or potential influence of atmospheric conditions on the referenced neutron monitor.

To test the traditional correction approaches for incoming cosmic radiation, air pressure, and air humidity, an experimental setup should avoid any influence of changes due to soil moisture. Therefore, a set of neutron detectors have been deployed in a buoy at the center of a lake for six months. The measurement period also included a Forbush Decrease in September, 2014. 

We found that the neutron signals correlated with air pressure, air humidity, and secondary cosmic radiation. The thermal neutron response to air humidity has been revealed to be different from the epithermal neutron response, while air pressure and incoming radiation similarly   influenced the thermal and epithermal signals. The results have been used to evaluate different existing strategies for air humidity correction of low-energy neutron data. Additionally, the potential effect of lake temperature on the thermal neutron count rate has been investigated. We have also analyzed the performance of the buoy  signal together with different neutron monitors in their capability to correct for the changes of incoming radiation and for the Forbush Decrease during the measurement period.

Overall, the study demonstrates how low-energy neutron detectors on a buoy  could be used to assess the influence of atmospheric and cosmogenic factors on the signal without the influence of soils. Despite the low count rate over water, the general principle could also serve as an alternative to remote neutron monitors as a more local reference signal at more comparable energies.

How to cite: Schrön, M., Rasche, D., Weimar, J., Köhli, M., Boehrer, B., Dietrich, P., and Zacharias, S.: Buoy-based detection of low-energy cosmic-ray neutrons to monitor the influence of atmospheric effects, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15523, https://doi.org/10.5194/egusphere-egu23-15523, 2023.

EGU23-15741 | ECS | Orals | GI6.8

Rigidity dependence of cosmic ray diurnal anisotropy using 22 years of GRAPES-3 muon telescope data 

Meeran Zuberi and the The GRAPES-3 Collaboration

The GRAPES-3 muon telescope (G3MT) has been recording high statistics of muons at a rate of ~50000 per second for the past two decades allowing us to probe the tiny variations in the muon flux caused by solar phenomena. The directional capabilities of G3MT enable us to look into 169 independent directions with a large median rigidity ranging from 64 to 141 GV. We have examined the 22 years (2000-2021) of G3MT data using the Fourier series technique to obtain the daily SDA amplitude and phase. The measured SDA amplitude and phase show a strong rigidity dependence. We found that the phase dominantly has the 22-year variation controlled by the drift effect due to solar polar magnetic field reversal, regardless of their rigidity. However, the higher rigidity bin phase variation shows an additional component of the 11 years controlled by the diffusion. The details of this work will be discussed during the talk.

How to cite: Zuberi, M. and the The GRAPES-3 Collaboration: Rigidity dependence of cosmic ray diurnal anisotropy using 22 years of GRAPES-3 muon telescope data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15741, https://doi.org/10.5194/egusphere-egu23-15741, 2023.

EGU23-15980 | ECS | Orals | GI6.8

Yield function of the DOSimetry TELescope (DOSTEL) count and dose rates aboard an aircraft 

Lisa Romaneehsen, Sönke Burmeister, Hanna Giese, Bernd Heber, and Konstantin Herbst

The Earth is continuously exposed to galactic cosmic rays. The magnetized solar wind in the heliosphere and the Earth's magnetic field alters the flux of these particles. If cosmic rays hit the atmosphere, they can form secondary particles. The total flux measured within the atmosphere depends on the atmospheric density above the observer. Therefore, the ability of a particle to approach an aircraft depends on its energy, the altitude, and the position of the plane. The cutoff rigidity describes the latter.
The radiation detector of the detector system NAVIDOS (NAVIgation DOSimetry) is the DOSimetry Telescope (DOSTEL), measuring the count and dose rates in two semiconductor detectors. From 2008 to 2011, two instruments were installed in two aircraft. First, we corrected the data for pressure variation by normalizing them to one flight level and determined their dependence on the cutoff rigidity by fitting a Dorman function to the observation. The latter was used to compute the yield function, which describes the ratio of incoming primary cosmic rays, approximated by a force field solution, to the measured count and dose rate for a particular instrument. As for neutron monitors, the sensitivity increases substantially above a rigidity of about 1 GV.
We received funding from the European Union's Horizon 2020 research and innovation program under grant agreement No 870405. 

How to cite: Romaneehsen, L., Burmeister, S., Giese, H., Heber, B., and Herbst, K.: Yield function of the DOSimetry TELescope (DOSTEL) count and dose rates aboard an aircraft, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15980, https://doi.org/10.5194/egusphere-egu23-15980, 2023.

EGU23-16004 | ECS | Posters on site | GI6.8

Impact and relevance of soil density changes on cosmic-ray neutron sensing for soil water estimation 

Katya Dimitrova Petrova, Lena Scheiffele, Lucile Verrot, Martin Schrön, and Josie Geris

Cosmic ray neutron sensor (CRNS) technology is becoming increasingly popular for monitoring volumetric soil water content (SWC) at the field (hectare) scale in a variety of environments. Applications include permanently installed (stationary) or the use of mobile (rover, trains, etc.) platforms. In agricultural settings, permanently installed CRNS have proven particularly useful for providing time series of footprint average SWC estimates. To derive the SWC product at a site, CRNS needs to be calibrated using gravimetric SWC, soil organic matter and bulk density (BD). Those variables may in the best case be derived from a large number of soil samples, collected ideally on multiple occasions and under a range of hydrometeorological conditions. Most CRNS applications use an average site-specific value of bulk density derived for a site from ≥1 field calibration and it is considered static over time.

However, while this is a safe assumption for many environments, in agricultural settings, management activities (e.g. tillage) may introduce substantial changes in BD over time. This may affect the accuracy of the CRNS SWC estimates, which in turn could affect management decisions (e.g. on irrigation) or modelling efforts, relying on these SWC inputs.

The importance of BD as a source of uncertainty in CRNS SWC estimation has been recognized with dedicated laboratory and neutron simulation experiments quantifying the effects. However, field-based studies are lacking. Therefore, the objective of this work is to quantify the impact and relevance of temporal variability in soil bulk density on the estimation of CRNS SWC in a variety of environments with different level of agricultural land use management. We used data from three sites (Scotland, Germany and China) with stationary CRNS, where BD was sampled on ≥3 or more occasions for sensor calibration. The sites display a varying intensity of land use management, cover different soil types and contrasting weather conditions. We quantify the differences in estimates of SWC by using the range of average BD values at a site and compare these differences to other sources of uncertainty (e.g. the integration time of neutron counts). We additionally consider existing theories on the interaction of neutrons and soil bulk density to evaluate the impact of BD changes. Finally, we make recommendations on when BD variability and thus its sampling over time may become important for the derivation of CRNS SWC outputs.

How to cite: Dimitrova Petrova, K., Scheiffele, L., Verrot, L., Schrön, M., and Geris, J.: Impact and relevance of soil density changes on cosmic-ray neutron sensing for soil water estimation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16004, https://doi.org/10.5194/egusphere-egu23-16004, 2023.

EGU23-17336 | ECS | Orals | GI6.8

Cosmic Ray Soil Moisture Sensors as an Asset to Space Weather Monitoring Activities 

Fraser Baird and Keith Ryden

Cosmic Ray Sensors (CRS) are used worldwide to measure soil moisture at intermediate scales, exploiting the neutrons produced in the air showers created by cosmic ray particles interacting with the atmosphere. Neutron Monitors also exploit these atmospheric neutrons, but they are shielded from local soil moisture variations so that information about the cosmic ray flux near Earth can be deduced from their observations. Neutron monitors remain the state of the art for observing variations in high-energy cosmic rays and are critically important to understanding ground-level enhancements of atmospheric radiation caused by high energy solar energetic particles.

This contribution explores how the UK CRS network (COSMOS-UK) can complement the neutron monitor network in monitoring these ground-level enhancements, as well as other space weather-driven variations in the ground-level neutron flux. Observations of such variations using COSMOS-UK are presented and discussed, and the sensitivity of COSMOS-UK to ground-level enhancements is also shown. Finally, the prospects and challenges of improving the space weather utility of CRS networks are discussed.

How to cite: Baird, F. and Ryden, K.: Cosmic Ray Soil Moisture Sensors as an Asset to Space Weather Monitoring Activities, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17336, https://doi.org/10.5194/egusphere-egu23-17336, 2023.

EGU23-17421 | Orals | GI6.8

Cosmic ray muons as a proxy for in-cruise galactic cosmic ray protons in 3He gas proportional counters 

Jack T. Wilson, Patrick N. Peplowski, Zachary W. Yokley, David J. Lawrence, and Richard C. Elphic

3He gas proportional counters have an extensive history in planetary neutron spectroscopy and several upcoming missions including Psyche, VIPER, MMX and Dragonfly will include this technology. In space, Galactic Cosmic Ray (GCR) protons deposit energy in the 3He gas in these detectors via ionization. This energy deposition constitutes a background on top of the neutron capture pulse-height spectrum that is particularly prominent at low energies. As planetary nuclear spectroscopy experiments are often count-rate limited using the full pulse height spectrum, including the proton and triton wall effect regions, has significant value. This will be particularly true for the upcoming VIPER mission that will explore the permanently shaded regions at the Moon’s south pole using the Neutron Spectrometer System (NSS).  The NSS does not include a neutron generator, so the count rates are low, and the rover will not spend long at any location.  However, using lower-energy parts of the spectrum requires understanding the GCR-originating background, which none of the previous missions were able to measure due to their low-energy cutoffs. GCR protons with mean energy around 400 MeV deposit similar amounts of energy to the 4 GeV mean-energy muons present at ground level as both represent minimum ionizing particles within the 3He sensors.  We therefore developed an experiment using a pair of plastic scintillators in coincidence with a 3He tube to measure energy deposition from muons while excluding room background gamma rays.  Here we will present results of this experiment to characterize the angular response to cosmic ray muons of a 3He flight spare detector from the VIPER NSS and explore the implications of these results for analysis of planetary neutron data sets.

How to cite: Wilson, J. T., Peplowski, P. N., Yokley, Z. W., Lawrence, D. J., and Elphic, R. C.: Cosmic ray muons as a proxy for in-cruise galactic cosmic ray protons in 3He gas proportional counters, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17421, https://doi.org/10.5194/egusphere-egu23-17421, 2023.

EGU23-17487 | ECS | Posters on site | GI6.8

Cosmic-ray neutron production and propagation inside snow packs characterized by multi-particle Monte Carlo simulations 

Jannis Weimar, Paul Schattan, Rebecca Gugerli, Benjamin Fersch, Darin Desilets, Martin Schrön, Markus Köhli, and Ulrich Schmidt

Cosmic-ray neutron sensors buried below a snow pack provide a passive and autonomous monitoring technique of snow water equivalent (SWE). The effective neutron flux is attenuated inside the snow volume resulting in an inverse relationship between neutron intensity and the water equivalent of the snow column above the sensor. Neutrons are moderated and absorbed within the snow. Simultaneously, highly energetic cosmic rays produce further neutrons via spallation and evaporation processes. A comprehensive assessment of the neutron flux therefore requires multi-particle simulations which involve all relevant incoming particle species and transient particles from cosmic-ray showers which play a crucial role in neutron production.

In our study, we used the Monte Carlo toolkit MCNP6 and validated its high-energy evaporation and spallation models against a measured data set of a neutron intensity profile in water. Based on that we fitted analytical functions to a large variety of simulation setups that describe the neutron intensity as a function of SWE and the moisture content of the soil below the sensor. Moreover, single-particle tracking revealed that the radial footprint of the method does not exceed few meters for detectors below thick snow layers. In the case of shallow snow, however, the diffusive long-range neutron flux in the atmosphere may penetrate through the snow pack to the buried sensor and thereby increases the influence of distant objects. Since the diffusive flux is further sensitive to the atmospheric water content, we developed an air humidity correction tailored to snow-buried neutron detectors.

In general, the study aims at a holistic understanding of neutron production and transport processes in snow and the adjacent soil and air volumes in order to improve SWE monitoring by buried cosmic-ray neutron sensors and compares the simulation results to field data.

How to cite: Weimar, J., Schattan, P., Gugerli, R., Fersch, B., Desilets, D., Schrön, M., Köhli, M., and Schmidt, U.: Cosmic-ray neutron production and propagation inside snow packs characterized by multi-particle Monte Carlo simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17487, https://doi.org/10.5194/egusphere-egu23-17487, 2023.

This study explores the potential of slow-varying components of the earth system to predict the monthly mean wind speeds over the seven homogenous climate zones of India at subseasonal to seasonal time-scales. The following set of predictors are selected for that purpose: sea-surface temperature, mean sea-level pressure, 10 m wind speed, wind speed at 850 hPa, and geopotential height at 850 hPa. With the exception of sea-surface temperature which is obtained from HadISST, the rest of the variables are obtained from the JRA55. Besides, the popular indices such as the Nino 3.4 index and the Dipole mode index are also used as predictors. The forecasts are made at 1, 2, 3, 4, and 5 months of leadtime for the monsoon months of June, July, August, and September when the wind speeds are the highest throughout the country. The regions of significant correlations of the predictor fields with the spatially-averaged wind speeds of each homogenous region are determined using the past 6 month lagged composites. Once identified, the variables over these regions are spatially averaged and are mapped to the 10 m wind speeds from JRA55, since it is the closest representation of observed wind speeds over India. This predictor-based forecasting is carried out using the following approaches: multi-linear regression, decision tree based regression, and K nearest neighbours regression. The models use data from 1958-2018 for training and 2019-2021 for testing. The deterministic predictions are evaluated using mean absolute error (MAE) and the skill compared to a climatological forecast is estimated using the root mean squared error skill score (RMSESS). Results show that different sets of predictor combinations are responsible for giving the best forecasts for individual months and leadtimes. These forecasts have MAE of  around 0.2 m/s and RMSESS values ranging from 0.5-0.7. Although we are looking at deterministic predictions here, a combination of multiple models and predictors used above can lead to the production of ensemble forecasts as well, which will be of further added value to the wind energy sector.

How to cite: Das, A. and Baidya Roy, S.: Exploiting the predictability of global teleconnections to forecast subseasonal to seasonal scale wind speeds over India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-507, https://doi.org/10.5194/egusphere-egu23-507, 2023.

EGU23-1119 * | Orals | ERE2.1 | Highlight

Meteorological challenges for renewable energy in the High Arctic 

Anna Sjöblom, Matthias Henkies, and Arthur Garreau

A transition to renewable energy is becoming increasingly more urgent in the High Arctic. In Svalbard (78°N), the previously coal based energy system is now, with a short transition period with diesel, moving to a completely renewable off-grid system. Both solar and wind energy are possible contributors to the energy mix. However, no renewable energy systems are specifically designed for the High Arctic and before implementing the systems they must be tested and adapted to Arctic conditions. Since 2020, the world’s northernmost higher education institution, The University Centre in Svalbard (UNIS), has developed a special focus on Arctic renewable energy meteorology, focussing especially on solar and wind energy. This is undertaken in close collaboration with local industry who are switching from coal mining to exporting renewable off-grid systems.

Many of the meteorological processes in the High Arctic are very different from further south with long periods of midnight sun, polar night, complex topography, low temperatures, stable stratification, snow and ice etc. What implications these processes will have on the solar and wind power are mostly unknown. To complicate matters further, numerical models are uncertain and unproved in these areas and there is a need for long-term measurements.

Long-term meteorological measurements to determine the energy potential as well as the impact of the Arctic climate have commenced around Longyearbyen, Svalbard, with a special focus on boundary layer processes. Initial results will be presented, including local wind processes important for wind energy and radiation properties for solar energy. The goal is to identify the most important meteorological processes and adapt the energy solutions accordingly.

How to cite: Sjöblom, A., Henkies, M., and Garreau, A.: Meteorological challenges for renewable energy in the High Arctic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1119, https://doi.org/10.5194/egusphere-egu23-1119, 2023.

Inclined and flat-plate photovoltaic (PV) solar panels have been widely used in many countries and regions for generating electric power. For exploiting the available solar energy in a region, prior knowledge of this potential is necessary. This work investigates the performance of solar panels in 82 locations in Saudi Arabia by calculating the annual energy received on inclined-plate with tilt angles from 15° – 55° inclined to south and flat-plate that continuously follow the daily motion of the sun.  Calculations are performed using a fixed surface albedo of 0.2 and with a near-real value. The analysis indicates that tilt angles of 20°, 25°, and 30° towards the south are the optimum ones depending on the site. These optimum tilt angles define three distinct solar energy zones in Saudi Arabia. The variation of the total energy in each energy zone on a monthly, seasonal, and annual basis is given. Regression analysis for the total energy as a function of time is derived for each zone. Moreover, the spatial distribution of the annual global inclined solar energy in Saudi Arabia is illustrated in a solar map where the total energy is found to vary from 1612 - 2977 kWhm−2year−1 for the southward-inclined plates and 2159 – 4078 kWhm−2year−1 for the flat-plates across Saudi Arabia. The correction factor, introduced in a recent publication, is used; it is found that the linear relationship between the correction factor and the ground-albedo ratio is general enough to be graphically representable as a nomogram.

How to cite: Farahat, A. and Kambezidis, H.: Solar Potential in Saudi Arabia: Spatio-temporal and Plates-inclination Effects on the Performance of Photovoltaic Solar Panels, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1790, https://doi.org/10.5194/egusphere-egu23-1790, 2023.

In 2021, Saudi Arabia, a leading global oil producer, announced its Middle East Green Initiative with many objectives including reducing carbon emissions by divagating the country away from an oil-based economy and towards renewable. Saudi Arabia has a high potential to become one of the global largest solar energy producers, as it is geographically located on a sunbelt. By 2030, the Saudi government targets building eight solar plants across the country which are expected to produce more than 3,600 MW, enough to power more than 500, 000 homes. However, the vast desert environment in Saudi Arabia increases the dust and aerosol loadings in the atmosphere, which affects the performance of the solar irradiance performance of photovoltaic panels due to the scattering of the solar radiation and the dust deposition on the solar panels. In this work, ground-based data from weather stations located in five Saudi cities: Dammam, Riyadh, Jeddah, Najran, and Arar along with data from the Moderate Resolution Imaging Spectroradiometer (MODIS) are used to estimate solar irradiance and its correlation with atmospheric and meteorological conditions like air temperature, wind, and aerosol physical parameters. We investigate the effect of three major dust storms that blew over different regions in Saudi Arabia on 20 March 2017, 23 April 2018, and 15 April 2021 on solar irradiance. It is found that there is a strong correlation between aerosol optical parameters like Aerosol Optical Depth (AOD), Ångström exponent, and solar irradiance. Maximum AOD (about 2) is recorded over Jeddah on 19 March 2017, (about 2.3) over Riyadh on 20 March 2017, (about 1.5) over Riyadh on 24 April 2018, and (about 0.9) over Najran on 15 April 2021. Large dust events are found to reduce air temperature by a few degrees in the regions affected by dust loadings. The study found large dust loading decreases the DNI, and GHI components on the solar irradiance, while increasing the DHI component over the cities of Jeddah, Riyadh, and Najran. This could be an indication that scattering from dust particles could play a significant role in the solar irradiance intensity. 

How to cite: Labban, A. and Farahat, A.: Effect of Major Dust Events on Atmospheric Temperature and Solar Irradiance Components over Saudi Arabia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1854, https://doi.org/10.5194/egusphere-egu23-1854, 2023.

EGU23-2107 | Posters on site | ERE2.1

Power generation forecast for a solar plant with a deep-learning method 

Yu-Ting Wu and Chang-Yu Lin

In this study, we perform power generation forecast of a solar farm using deep learning. A long short-term memory (LSTM) network is applied to forecast time series data of the overall power production from a solar farm. An LSTM network can be considered as a recurrent neural network (RNN) looping with input data (e.g., measured power data) over time steps to update the network information. The network information also has records over all previous time steps. One can use an LSTM network to predict subsequent values of a time series (denoted as open loop forecasting) or sequence using previous time steps as input (denoted as closed loop forecasting). Both forecasting methods are built in the LSTM network. Preliminary results show that closed loop forecasting can allow to have predictions of solar power in more time steps, but less accurate than the other method.  

How to cite: Wu, Y.-T. and Lin, C.-Y.: Power generation forecast for a solar plant with a deep-learning method, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2107, https://doi.org/10.5194/egusphere-egu23-2107, 2023.

Wind energy is essential in many decarbonization strategies and potentially vulnerable to climate change. While existing wind climate change assessments rely on regional or global climate models, a systematic investigation of the global-to-regional climate modeling chain is missing. In this presentation, I therefore address the differences in climate change impacts on winds according to  regional and global climate model ensembles under three different future scenarios.

 

I highlight two key limitations, namely (a) the differing representation of land-use change in global and regional climate models which compromises comparability, and (b) the consistency of large-scale features along the global-to-regional climate modeling chain. To this end, I analyze the large EURO-CORDEX ensemble (rcp85: N=49; rcp45: N=18; rcp26: N=22) along with the driving global models (rcp85: N=7; rcp45: N=5; rcp26: N=7), finding evidence that climate change reduces mean wind speeds by up to -0.8 m/s (offshore) and -0.3 m/s (onshore).

 

Moreover, I provide physical explanations for these changes by identifying two key drivers. First, onshore wind speeds drop in the driving global models in regions and scenarios with strong land use change but show no drop in EURO-CORDEX where land use is held constant. Second, offshore wind reductions follow decreases in the equator-to-pole temperature gradient remarkably well with correlations reaching around 0.9 in resource-rich European countries like Ireland, the United Kingdom and Norway, implying that arctic amplification is a severe risk for European offshore wind energy.

 

My results suggest that earlier conclusions of negligible climate change impacts on wind energy might be premature if either land use changes strongly or polar amplification is at or above the range sampled in global climate models. In conjunction with earlier work that demonstrated the relevance of multidecadal wind fluctuations caused by climate variability, these results call for a better inclusion of climate risk in wind energy planning.

 

Reference

 

Wohland, J. Process-based climate change assessment for European winds using EURO-CORDEX and global models. Environ. Res. Lett. (2022) doi:10.1088/1748-9326/aca77f.

How to cite: Wohland, J.: Climate change impacts on winds in Europe: do global and regional climate models tell the same story?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2317, https://doi.org/10.5194/egusphere-egu23-2317, 2023.

January 2007 was a bad storm month for much of central and northern Europe with a series of extratropical cyclones bringing high winds and precipitation to highly populated areas between Ireland and Russia.  Although Storm Kyrill on 18-19 January 2007 was the most serious for its infrastructure damage and insurance costs, Storm Franz from the preceding week on 11-12 January 2007 was actually more serious for its maritime impacts in western Europe. This contribution takes a closer look at Storm Franz, presenting an overview of its impact to energy infrastructure as well as transportation networks and societal infrastructure damage.  Maritime casualties are reviewed with respect to met-ocean conditions.  An analysis is carried out on water level recorders around the North Sea to assess the storm surge and short period oscillations that may reveal harbour seiches or meteotsunamis.  The results are compared with wave recorders, which had a fairly good coverage across the North Sea in 2007.  The issue of wave damage to offshore infrastructure was highlighted in events associated with Storm Britta on 31 October - 1 November, 2006.  Offshore wind energy in northwest Europe was in a growth phase during this time, and there were questions about the extreme met-ocean conditions that could be expected in the 20 year lifetime of an offshore wind turbine.

How to cite: Kettle, A.: Storm Franz: Societal and energy impacts in northwest Europe on 11-12 January 2007, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3218, https://doi.org/10.5194/egusphere-egu23-3218, 2023.

EGU23-3486 | ECS | Posters on site | ERE2.1 | Highlight

Solar energy potential assessment on urban rooftops using digital surface models 

Xinyuan Hou and Stelios Kazadzis

Rooftop solar photovoltaic (PV) systems have the advantage of producing electricity without air pollution and greenhouse gas emissions, at the same time reducing carbon footprint as well as urban heat island effect. This study aims to assess physical, geographical and economic levels of solar energy potentials in actual atmospheric conditions on urban rooftops, using two municipalities in Athens, Greece as an example. 

We utilize very high-resolution digital surface models for the computation of clear-sky solar irradiance considering surrounding shadows. For all-sky conditions, cloud and aerosol data from 2012 to 2021 are obtained from the Copernicus Atmosphere Monitoring Service radiation service and the ECMWF Atmospheric Composition Reanalysis 4 product, respectively. The goals are to quantify the effect of solar elevation, the shadowing effect from adjacent buildings and constructions, and the effects of clouds and aerosols on the solar radiation availability on the rooftops and to investigate their interconnections. The spatio-temporal resolution of the analyses ranges from individual rooftop to neighborhood scale (approximately 3000 buildings) and from hourly intervals to ten years periods.

The results of the solar potential assessment are made available as a web GIS map for potential public access, intended to aid urban planning and encourage widespread adoption of solar energy in the public and private sectors.

How to cite: Hou, X. and Kazadzis, S.: Solar energy potential assessment on urban rooftops using digital surface models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3486, https://doi.org/10.5194/egusphere-egu23-3486, 2023.

EGU23-4625 | Posters on site | ERE2.1

Medium and Long-term Forecast of Wind Power Trend Based on Regional Similarity 

Xianxun Wang, Yaru Liu, Defu Dong, and Suoping Wang

Accurate and efficient medium and long-term forecast of wind power can provide technical support for efficient development and utilization of wind resources. Taking into account the regional characteristics of wind resources, the regional similarity factor is introduced into the study of wind power forecasting, and the long-term dependence of wind power, the Long Short-Term Memory method is selected for medium and long-term forecasting of wind power trend, a case study is carried out in five provinces of Northwest China. The results show that the error is reduced by an average of 20.80% compared with the forecast of individual stations, which verifies the effectiveness of the proposed method. Different area division methods result in different effects on improving the prediction accuracy. This study provides a new method and reference for medium and long-term wind resource prediction.

How to cite: Wang, X., Liu, Y., Dong, D., and Wang, S.: Medium and Long-term Forecast of Wind Power Trend Based on Regional Similarity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4625, https://doi.org/10.5194/egusphere-egu23-4625, 2023.

EGU23-5382 | Posters on site | ERE2.1

The GASPOC project and the global offshore atlases of siting parameters 

Xiaoli Larsén, Marc Imberger, Neil Davis, Jacob Sørensen, Carsten Kofoed, Jim Nielsen, Bjarke Olsen, Jana Fischereit, and Jake Badger

The Global Atlas of Siting Parameters for Offshore and Coasts (GASPOC) project aims at shortening the project development period for offshore wind farms, with faster energy integration, lower capital expenditure and lower operating expense. This value is brought by the partners DHI, DTU Wind, Vento Maritime and DECK1 through automatic data driven downscaling techniques, that are applied to meteorological, ocean and wave modeling and analytics, including the application to real test scenarios. GASPOC provides metocean data, including siting parameters for offshore wind turbines such as extreme winds and turbulence intensity, as well as extreme waves and joint wind-wave statistics. An ensemble of reanalysis data together with the spectral correction method (Larsén et al. 2012) is used to obtain the effective 10-min extreme winds at 50 m, 100 m, 150 m and 200 m, while the calculation of the turbulence intensity at heights above the surface layer also takes the mesoscale turbulence into consideration. We show the data of the siting parameters from GASPOC which support seamless application to strategic planning of offshore wind energy development.

Reference

Larsén X., Ott S., Badger J., Hahmann A. N. and Mann J. 2012: Recipes for correcting the impact of effective mesoscale resolution on the estimation of extreme winds. Journal of applied meteorology and climatology, Doi:10.1175/JAMC-D-11.090, vol 51, No. 3, p521-533.

How to cite: Larsén, X., Imberger, M., Davis, N., Sørensen, J., Kofoed, C., Nielsen, J., Olsen, B., Fischereit, J., and Badger, J.: The GASPOC project and the global offshore atlases of siting parameters, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5382, https://doi.org/10.5194/egusphere-egu23-5382, 2023.

EGU23-5388 | ECS | Posters on site | ERE2.1

Spatial complementary of offshore wind farm Iberian Peninsula sites based on COSMO-REA6 high-resolution reanalysis. 

Noelia López-Franca, Miguel Ángel Gaertner, Enrique Sánchez, Clemente Gallardo, María Ofelia Molina, María Ortega, and Claudia Gutiérrez

The energy transition is a fundamental endeavour in the way towards a zero-carbon future that will allow us to mitigate anthropogenic climate change. There are plans at a European Union level and, also at Iberian Peninsula (IP) one, to strongly increase the installed wind power capacity by 2030, with the aim by 2050 of making Europe the first climate-neutral continent. Onshore wind and solar photovoltaic are currently by far the main renewable technologies installed on the IP, receiving other potential dispatchable energy resources such as offshore wind less attention. This resource should also be considered due to its high energy potential and the increasing difficulty of finding suitable land for new onshore wind farms. Although some areas, such as the western IP, show high potential, there are important spatial constraints for the deployment of floating offshore wind towers, related to wind infrastructure technologies and legislative limits. Together, wind power generation is, by nature, complex, irregular and hard to be forecasted. Thus, increasing interconnections between regions can dampen the impact of wind variability on local wind power generation. An analysis of the spatial complementarity of the top potential floating offshore wind farm sites across IP is then proposed in this work. For this purpose, hourly wind fields from COSMO-REA6 very high resolution reanalysis (0.055º) in the 1995-2018 period were used to compute the wind capacity. The wind speed was vertically interpolated to the hub height of 105 meters of a reference turbine at each grid point between the levels 36-39 (approximately 35 to 178 meters) of the reanalysis by a cubic polynomial function using the least squares fit. Then, a total of 55 potential locations of Iberian commercial floating wind farm projects were manually collected, mainly from publicly available information. Of these, ten potential sites were chosen by applying a methodology that finds the combination of sites that minimizes the coefficient of variation of the aggregate wind power. The first results indicate that, in the period considered, it is more advantageous for the Iberian electricity system to build wind farms farther apart, giving priority to wind farm projects located in the northeast and northwest coastal corners of IP. Thus, as more distant sites are added, the coefficient of variation decreases more than the capacity factor. This behaviour varies slightly by season, with the variation decreasing the most in winter and the capacity factor decreasing the most in summer.

How to cite: López-Franca, N., Gaertner, M. Á., Sánchez, E., Gallardo, C., Molina, M. O., Ortega, M., and Gutiérrez, C.: Spatial complementary of offshore wind farm Iberian Peninsula sites based on COSMO-REA6 high-resolution reanalysis., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5388, https://doi.org/10.5194/egusphere-egu23-5388, 2023.

EGU23-5763 | Posters on site | ERE2.1

Realistic Wake Simulation using the WRF-SADLES System 

Hai Bui and Mostafa Bakhoday-Paskyabi

Simulating wind turbine wakes with high accuracy is crucial for understanding their effects on nearby flow patterns and optimizing the design and operation of wind farms. However, current Large Eddy simulation (LES) models for this purpose often rely on highly idealized boundary layer conditions, which may not capture all relevant realistic processes. In this study, we present the development and application of a Simple Actuator Disc model for Large Eddy Simulation (SADLES) for simulating wakes in realistic conditions. SADLES was developed to utilize traditional thrust and power curves provided by turbine manufacturers, while also achieving an intermediate resolution of a few dozen meters to strike a balance between fidelity and computational cost. SADLES has been integrated into the Weather Research and Forecast (WRF) model, resulting in the WRF-SADLES system. Using this system, atmospheric conditions from ERA5 data were downscaled to a wake-enable scale of 40 m using a system of 5 nested domains. Selected transition events were simulated and the results were validated using real observations from the FINO1 meteorological mast and LiDAR data. Our WRF-SADLES approach represents a promising advancement in the simulation of wind turbine wakes and their impacts on surrounding flow fields.

How to cite: Bui, H. and Bakhoday-Paskyabi, M.: Realistic Wake Simulation using the WRF-SADLES System, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5763, https://doi.org/10.5194/egusphere-egu23-5763, 2023.

European countries are increasing their share of power production from wind and solar energy to mitigate climate change. Also the relative contributions from PV and wind power production in Europe change over time. At present, the installed capacity of photovoltaic (PV) power for all of Europe is smaller than that of wind power with a ratio of 3:4. Future scenarios for the installations of PV and wind power capacities for 2050 suggest that this ratio will substantially change. Namely, the PV power capacity might exceed the wind power capacity with a ratio of 3:2 to 2:1. We test the hypothesis that the weather dependency of anomalies in the PV plus wind power production will change in the future compared to today. Specifically, we examine which synoptic weather patterns are associated with anomalies in the PV plus wind power production for the present and future installed capacities in Europe. To that end, we developed a renewable energy model for the installed capacity of 2019 and 2050. This model allows us to simulate hourly PV and wind power production at 6 km horizontal resolution for all of Europe. We analyze the weather dependency of power-production anomalies by pairing our model output with results of the classification of weather patterns from the German Weather Service. Our results highlight similar weather patterns associated with positive anomalies in the hourly PV plus wind power production for the 2019 and 2050 installation, namely weather patterns with prevailing westerly winds. However, weather patterns associated with negative anomalies strongly change between the two installations. We also assess the dependency of the results on the duration of the production anomalies. Particularly for long production anomalies, the associated weather patterns are different for the 2019 and 2050 installation. One exception is the weather pattern Anticyclonic Southeasterly that is associated with the lowest 10-day power production in Europe for both 2019 and 2050. Regionally, weather patterns have different impacts on different regions in Europe, when comparing the associated patterns between the 2019 and 2050 installation. For instance, anomalously low power production differ for the Iberian peninsula and Southeastern Europe when the two installed capacities are compared. Taken together, our study gives a systematic overview on changes in the weather dependency of anomalies in the mix of PV and wind power between 2019 and 2050.

How to cite: Ho, L. and Fiedler, S.: Weather dependency of European wind and photovoltaic power production for present and future installations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5812, https://doi.org/10.5194/egusphere-egu23-5812, 2023.

EGU23-5918 | ECS | Posters on site | ERE2.1

AEOLIAN, the new Italian Wind Atlas for local energy planning support 

Martina Aiello, Davide Airoldi, and Alessandro Amaranto

The decarbonization objectives set by the EU Green Deal to increase the renewable generation heavily rely on the contribution of wind energy, both onshore, through the installation of new plants and repowering of existing plants, and offshore. The issuance of the new "Fit for 55" package of measures will result in an increase in the objectives already identified for 2030 for Italy, which in all probability will be set at over 21 GW of installed capacity for onshore wind (i.e., doubling the currently operating power) and at least 3 GW for offshore wind. An informed energy planning of the territory is therefore paramount to efficiently maximize renewable penetration. In these regards, the development of informatic tools aimed at disentangling both resource availability and generation potential can effectively play a key role in supporting optimal technology displacement through space. RSE has worked on these themes since the end of the 1990s, when the first version of the Italian Wind Atlas (ATLAEOLICO) WebGIS was released, providing a support tool for adequate energy planning of the territory. Throughout the years, the Wind Atlas has represented a reference for various stakeholders (wind plants developers, authorities responsible for spatial planning and companies involved in the electricity grid development) who recognized its great utility in quickly identifying the most suitable Italian areas for wind energy exploitation in terms of long-term annual average wind speed and full load hours.  With the purpose that this platform keeps providing tangible support for energy planning, we have worked on both renewing the anemological database and the WebGIS structure, which is the focus of this work.  The new Italian Wind Atlas AEOLIAN provides for a new anemological database consisting in 30 years (1990-2019) of hourly wind data at 1.4 km horizontal resolution (WGS84 UTM32) covering the whole Italian territory and marine areas. Wind trajectories are estimated through the Weather Research and Forecasting (WRF) meteorological model combined with a statistical post-processing based on Analog Ensemble (AnEn). The renewed AEOLIAN WebGIS, developed through the open access framework TerriaJS, integrates standard functions for visualizing and querying data, data download functions and advanced tools to support local energy planning. It shows the spatial distribution of onshore and offshore wind speed [m/s] and full load hours [MWh/MW]. Each variable is computed as the 30 years annual average at the heights of 50, 75, 100, 125 e 150 m. a.s.l. Within AEOLIAN, users can download both variable maps and historical series of wind speed for more accurate evaluations. Besides maps, AEOLIAN also includes a tool for the technical and economical evaluation of a hypothetical wind farm at a local scale. This tool allows assessing the energy performances in terms of the net annual energy production and the average cost of the energy produced, considering local distribution of the wind resource, energy performances of the wind farm and investments and management costs.  

How to cite: Aiello, M., Airoldi, D., and Amaranto, A.: AEOLIAN, the new Italian Wind Atlas for local energy planning support, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5918, https://doi.org/10.5194/egusphere-egu23-5918, 2023.

EGU23-5952 | ECS | Orals | ERE2.1

The Aspire campaign: Assessing the effects of aerosols on solar radiation and energy in SE Europe. 

Dimitra Kouklaki, Ioannis-Panagiotis Raptis, Stelios Kazadzis, Ilias Fountoulakis, Kyriakoula Papachristopoulou, and Kostas Eleftheratos

In recent years, solar power applications are growing rapidly worldwide, to meet the increasing power demand and the sustainable development planning. Estimation of solar radiation availability at surface level, its characteristics and various factors that affect it, play a key role in designing and achieving the optimal performance of systems employing solar energy. Various solar -PV related - applications are using radiative transfer modeling to characterize the radiation field, since accurate surface solar irradiance measurements are not always available, especially in remote regions. Understanding the effect of aerosols to the solar energy potential is highly important for the energy sector as well as for a variety of fields.    In areas and periods where cloudiness is limited and they are in the proximity of particle sources, the significance of aerosol effect is very high.

The objective of this study is to assess the impact of the variability of aerosols on the solar Direct Normal Irradiance (DNI), Global Horizontal Irradiance (GHI) and solar energy, using spectral solar measurements and aerosol optical properties retrievals, in the framework of the one-year experimental campaign (December 2020-December 2021) of the ASPIRE (Atmospheric parameters affecting SPectral solar IRradiance and solar Energy, https://aspire.geol.uoa.gr) project, which was held in Athens, Greece.

Main findings include an assessment of differences among different PV technology and their calculated outputs using actual and standard spectra, linking the differences with aerosol optical properties (optical depth, spectral dependence, absorption). Aerosol optical depth is the major factor of such differences for all PV technologies. Spectral aerosol characteristics affect differently PV technologies as a consequence of different spectral responsivities.

Finally, aerosol effect on solar nowcasting models have been investigated by comparing spectral solar measurements and aerosol properties with model inputs and outputs.

How to cite: Kouklaki, D., Raptis, I.-P., Kazadzis, S., Fountoulakis, I., Papachristopoulou, K., and Eleftheratos, K.: The Aspire campaign: Assessing the effects of aerosols on solar radiation and energy in SE Europe., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5952, https://doi.org/10.5194/egusphere-egu23-5952, 2023.

Probabilistic forecasts based on ensemble simulations of numerical weather prediction models have become a standard tool in weather forecasting and various application areas. However, ensemble forecasting systems tend to exhibit systematic errors such as biases, and fail to correctly quantify forecast uncertainty. Therefore, a variety of post-processing methods has been developed to correct these errors and improve predictions [1]. In particular, machine learning methods based on neural networks have been demonstrated to lead to substantial improvements compared to classical statistical techniques [2].
While post-processing can successfully correct the biases and dispersion errors in the weather variables, its effect but has not been evaluated thoroughly in the context of subsequent forecasts, such as wind and solar power generation forecasts and it is not obvious how to best propagate forecast uncertainty through to subsequent power forecasting models. Therefore, the work presented here will evaluate multiple strategies for applying ensemble post-processing to probabilistic wind and solar power forecasts. We use Ensemble Model Output Statistics (EMOS) as the post-processing method and evaluate four possible strategies: only using the raw ensembles without post-processing, a one-step strategy where only the weather ensembles are post-processed, a one-step strategy where we only post-process the power ensembles and a two-step strategy where we post-process both the weather and power ensembles. The presentation is based on recent work in Phipps et al. (2022) [3] and ongoing other work.

References

[1] Vannitsem, S., et al. (2021). Statistical Postprocessing for Weather Forecasts - Review, Challenges and Avenues in a Big Data World. Bulletin of the American Meteorological Society, 102, E681–E699.
[2] Rasp, S. and Lerch, S. (2018). Neural networks for post-processing ensemble weather forecasts. Monthly Weather Review, 146, 3885–3900.
[3] Phipps, K., Lerch, S., Andersson, M., Mikut, R., Hagenmeyer, V. and Ludwig, N. (2022). Evaluating ensemble post-processing for wind power forecasts. Wind Energy, 25, 1379-1405. 

How to cite: Lerch, S.: Evaluating ensemble post-processing for probabilistic energy prediction, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6644, https://doi.org/10.5194/egusphere-egu23-6644, 2023.

EGU23-6943 | Orals | ERE2.1 | Highlight

Impact assessment of future wind farm characteristics on cluster-scale wake losses in the North Sea 

Nicole van Lipzig and Ruben Borgers

Offshore wind zones are reaching sizes at which they start to affect each other and potentially also alter mesoscale weather systems, impacting the energy production. Here, we assess the impact of future wind farm characteristics, like turbine type and capacity density, on cluster-scale wake losses. For this we use the mesoscale model COSMO-CLM at the km-scale resolution, which skillfully models frequency distributions of wind speed and wind direction at turbine level compared to measurement masts, wind lidars and satellite data. It was found that inter-farm wakes can reduce the long-term capacity factor at the inflow edge of wind farms from 59% to between 55% and 40% depending on the degree of clustering and the size of the upwind farms, for a layout equipped with 5MW turbines at a capacity density of 8.1 MW / km². Moving to next-generation wind turbines (15MW) partly mitigates this degradation, as the total generation over all windfarms (TWh) is increased by 19% under the same wind farm capacity density. On the other hand, increases in the capacity density in this future layout lead to a less than proportional (0.8 to 1) increase in the basin-integrated, total generation as a consequence of more intense intra- and inter-farm wake effects. Generally, wind farm characteristics play an essential role in inter-farm wake losses, which should be included in future wind farm planning.

How to cite: van Lipzig, N. and Borgers, R.: Impact assessment of future wind farm characteristics on cluster-scale wake losses in the North Sea, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6943, https://doi.org/10.5194/egusphere-egu23-6943, 2023.

EGU23-8140 | ECS | Posters virtual | ERE2.1

From solar radiation estimation to solar energy potential in the High Arctic 

Arthur Garreau, Torodd Nord, Anna Sjöblom, and Aleksey Shestov

The High Arctic is a remote region with a harsh climate where communities mainly rely on fossil energy sources. In Longyearbyen, located in the archipelago of Svalbard at 78°N, solar energy is considered as one of the future energy sources. The available solar radiation must therefore be estimated to have solar energy as part of the energy mix. To achieve this goal, the University Centre in Svalbard has maintained a weather station that has recorded ten years of solar radiation data with a Kipp and Zonen CNR1 net radiometer. Additional pyranometers have been installed at other locations, at different altitudes, and with different configurations to establish a more complete atlas of the solar irradiance around Longyearbyen.

The solar irradiance in the High Arctic has different characteristics than that usually encountered at mid-latitudes. There are 24 hours of sunlight during summer and polar nights during winter. When the sun is present, its position and path in the sky differ from further south. In addition, the air mass, atmospheric aerosols, and albedo have an impact on radiation that is peculiar to the Arctic. All those specificities have yet to be completely understood for the Arctic, and hence some uncertainties remain about solar radiation.

A better understanding of the solar radiation received in Longyearbyen will help implement the future solar energy solution for the Arctic. The aim is to accurately estimate solar radiation at high latitudes, capture variability and predictability, and understand which solar cell configuration is optimal. In particular, differences between horizontal and plane-of-array irradiance have been investigated because of the very low elevation angle of the sun. The solar radiation distributions over different time scales have further been assessed using observations. Moreover, the impact of external factors on solar radiation, such as albedo, has been considered. In the future, the collected data will be used to assess Svalbard's solar PV potential.

How to cite: Garreau, A., Nord, T., Sjöblom, A., and Shestov, A.: From solar radiation estimation to solar energy potential in the High Arctic, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8140, https://doi.org/10.5194/egusphere-egu23-8140, 2023.

Near-surface wind fields are altered over mountainous topography, giving rise to complex wind flow patterns due to sheltering, acceleration, channelling, deflections, blocking or recirculation. However, the impact of the resulting spatio-temporal wind fields on wind energy potential remains largely unknown. While wind modelling approaches can describe highly resolved spatio-temporal wind fields in mountainous terrain rather well, wind fields cannot be generated in a reasonable amount of computational time. Models are therefore strongly limited in space and time for many applications. In mountainous regions, wind farm planning is thus much more challenging than in flat regions.

To investigate the variability of wind fields and its impact on wind energy production in mountainous terrain, we applied a computationally efficient statistical downscaling model approach to a small region in the Swiss Alps. This allowed us to analyze the impact of horizontal resolutions on spatial wind speeds and energy yield in a mountainous area. We applied the statistical approach of Helbig et al., 2017 to downscale coarse wind speed values to the fine scale based on local terrain parameters. This approach introduces two dominant local wind-topography interactions: sheltering and speed-up on coarse wind speed. Then, based on the resulting spatio-temporal near-surface wind fields and a common theoretical power curve, we calculated long-term wind energy yield. Through a sensitivity analysis, we assessed the impact of varying horizontal spatial resolutions in the mountainous environment on overall and local wind energy yield. Specifically, we addressed the impact when decreasing horizontal resolutions from grid cell sizes of 100 m down to 5 m. Resulting spatial variations will be discussed as functions of local terrain parameters, as well as wind speeds.

Helbig, N., Mott, R., van Herwijnen, A., Winstral, A. and Jonas, T. (2017): Parameterizing surface wind speed over complex topography. J. Geophys. Res., 122, 651–667.

How to cite: Helbig, N., Hammer, F., and Barber, S.: Characterizing the impact of spatial scales on near-surface wind speed and wind power generation in a mountainous environment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9025, https://doi.org/10.5194/egusphere-egu23-9025, 2023.

EGU23-9658 | Orals | ERE2.1

Renewable energy forecasting: results of the Smart4RES project and future research directions. 

Georges Kariniotakis and Simon Camal and the Smart4RES Team

The European Horizon 2020 project Smart4RES (http://www.smart4res.eu), which started in 2019 and runs until April 2023, aims at improving modelling and forecasting of weather variables necessary to optimize the integration of weather-dependent renewable energy (RES) production (i.e. wind, solar) into power systems and electricity markets. It gathers experts from several disciplines ranging from meteorology, data science, power systems a.o. It aims to contribute to the pathway towards energy systems with very high RES penetrations by 2030 and beyond.

This presentation has a double objective:

(1) To present a comprehensive overview in terms of KPI improvements of the final results obtained by the project. These results cover thematic objectives including:

  • Improvement of weather and RES forecasting;
  • Streamlined extraction of optimal value from the data through data sharing, data market places, and novel business models for the data;
  • New data-driven optimization and decision-aid tools for market and grid management applications;
  • Validation of new models in living labs and assessment of forecasting value vs costly remedies to hedge uncertainties (i.e. storage). 

The results obtained are numerous. Without being exhaustive, they include: improved forecasting of weather variables with focus on extreme situations and also through innovative measuring settings (i.e. a network of sky cameras); A seamless approach to couple outputs from different ensemble numerical weather prediction (NWP) models with different temporal resolutions; Advances from ultra-high resolution NWPs based on Large Eddy Simulation; Approaches for RES production forecasting aiming at efficiently combining highly dimensionally input (various types of satellite images, NWPs, spatially distributed measurements etc.); Seamless probabilistic RES forecasting covering multiple time frames and data inputs; Resilient energy forecasting. In the front of applications methods are proposed to optimally use forecasts for the management of storage systems coupled with renewables, for the optimal trading of renewables in multiple markets and for grid management optimization and dynamic security assessment. Prescriptive analytics and explainable AI methods are proposed to optimize decision making.  A cost benefit analysis is performed to assess the contribution of different types of data in forecasting problems.

(2) To present hierarchized proposals for future research directions. An international workshop is organized by the project (14/04/2023), where experts are invited to assess where RES predictability stands today and propose research directions for the future. In this presentation we will present the conclusions of this workshop. This will be a useful insight for academics, industrials as well as policy makers in the field.

How to cite: Kariniotakis, G. and Camal, S. and the Smart4RES Team: Renewable energy forecasting: results of the Smart4RES project and future research directions., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9658, https://doi.org/10.5194/egusphere-egu23-9658, 2023.

EGU23-10763 | Posters virtual | ERE2.1

Forecasting surface solar irradiance in Germany using Meteosat Rapid Scanning Service satellite images 

Mathieu Turpin, Sébastien Marchal, and Nicolas Schmutz

Photovoltaic (PV) production is strongly dependent on cloud cover behaviour. It can induce a very high variability of the production which is problematic for a safe and gainful injection into the power grid. Advanced forecasting solutions represent a major key to reliable PV systems. Satellite data are used to provide forecasts from 15 minutes until 6 hours ahead.

To achieve cloud cover forecast, the first step consists in converting two successive satellite images into a cloud index map. Then, the movement of the clouds between these two images is obtained by analysing the optical flow, transformed into a Cloud Motion Vector (CMV) which is then applied on the image taken at T0 to extrapolate it and forecast the various cloud index maps up to T0 + 6h. Finally, the cloud index is combined with a clear sky model in order to compute the effective Surface Solar Irradiance.

Over Europe, raw images are taken by EUMETSAT’s (European Organisation for the Exploitation of Meteorological Satellites) geostationary satellite. The satellite scans the Earth’s full disk in 15 minutes with the PRIME satellite positioned at 0°. However, the Rapid Scanning Service (RSS) scans the northern third of the Meteosat disk every five minutes, enabling more frequent data acquisition and lower delivery time. One satellite is dedicated to this operating mode and is positioned at 9.5°E.

TRUSTPV is a European Union’s Horizon 2020 Research project whose purpose is to investigate and demonstrate the development of O&M-friendly and grid-friendly solar solutions in large portfolios of distributed and utility scale photovoltaics. Within TRUSTPV, we demonstrate the performance improvement provided by using the geostationary meteorological satellite's RSS to obtain images more frequently and therefore improve intraday forecasts. In this work, we forecast cloud cover every 5 minutes with a 5-minute time step. Then, we simulate PRIME operation with forecasts generated every 15 minutes with a 15-minute time step by using the same optical flow and extrapolation algorithms. Moreover, we take into account the latency in the access to the data in real time. The model outputs are compared to 10-minute solar radiation measurements from Deutscher Wetterdienst (DWD) stations located in Germany over the period ranging from 2021-09-01 to 2022-08-31. We determine the quarterly performance in order to study the seasonal effects. The results are also expressed in terms of relative Root Mean Scare Error (RMSE), RMSE Skill Score, Mean Absolute Error (MAE), MAE Skill Score, and mean bias error.

Comparisons between forecasted surface solar irradiance at 30 minutes of time horizon and co-located pyranometric measurements show an improvement for all sites with a decrease of MAE around 4%. This gain brought by the RSS will improve the quality of power production forecasts of PV plants.

The research leading to these results has received funding from the Horizon 2020 Research and invention Programme, under Grant Agreement No 952957, Trust-PV project.

How to cite: Turpin, M., Marchal, S., and Schmutz, N.: Forecasting surface solar irradiance in Germany using Meteosat Rapid Scanning Service satellite images, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10763, https://doi.org/10.5194/egusphere-egu23-10763, 2023.

EGU23-11429 | ECS | Posters on site | ERE2.1

Improvements and validation of nextSENSE solar energy nowcasting and short-term forecasting system 

Kyriakoula Papachristopoulou, Ilias Fountoulakis, Alkiviadis F. Bais, Basil E. Psiloglou, Charalampos Kontoes, Maria Hatzaki, and Stelios Kazadzis

Solar energy is one of the main sources of renewable energy nowadays. Since there is a strong dependence of solar power generation on the presence of clouds and aerosols, operational nowcasting and short-term forecasting of solar resources are essential for its integration into the grid.

The aim of this study is the assessment of the downwelling surface solar irradiation (DSSI) estimates from the nextSENSE operational service. This service uses as input earth observational data for clouds (EUMETSAT), aerosols (Copernicus Atmosphere Monitoring Service - CAMS) and other important atmospheric parameters to the fast radiative transfer model (RTM) techniques (look-up table – LUT and multi-parametric equations) in order to derive DSSI in real time over Europe and North Africa in high spatial resolution (5 km at sub-satellite point), every 15 min. Recent modifications relative to the older versions are: (i) the use of multi-parametric equations to obtain the effect of clouds from cloud optical thickness (COT) instead of using Artificial Intelligence techniques, and (ii) the use of more detailed LUT. Forecasted DSSI values are also produced up to 3-hours ahead with a 15-min time step by applying a cloud motion vector (CMV) technique to the COT product based on Meteosat second generation (MSG) satellite data.

The new modeled (nowcasted and forecasted) DSSI values were validated against ground-based global horizontal irradiance measurements from pyranometers operating at the Baseline Surface Radiation Network (BSRN) stations and at two additional stations, these of Athens and Thessaloniki, Greece, for the year 2017. The nextSENSE forecasted DSSI values were also benchmarked against the smart-persistence forecast method. The performance of the modeled DSSI values were assessed for different cloud conditions in terms of real cloud modification factor (CMF) values derived by ground-based measurements in conjunction with a clear sky model. Additionally, the effects of aerosol related inputs for estimating DSSI were quantified by comparing the utilized CAMS aerosol optical depth (AOD) forecasts against surface retrievals of the AERONET network.

Acknowledgements

This study was funded by the European Commission project EuroGEO e-shape (grant agreement No 820852).

How to cite: Papachristopoulou, K., Fountoulakis, I., Bais, A. F., Psiloglou, B. E., Kontoes, C., Hatzaki, M., and Kazadzis, S.: Improvements and validation of nextSENSE solar energy nowcasting and short-term forecasting system, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11429, https://doi.org/10.5194/egusphere-egu23-11429, 2023.

EGU23-12367 | ECS | Posters on site | ERE2.1

Projected Changes in Türkiye's Wind Energy Potential Using Next-Generation Climate Models and Scenarios 

Zekican Demiralay, M. Tufan Turp, Nazan An, and M. Levent Kurnaz

Renewable energy is a cornerstone in reducing greenhouse gas emissions and, accordingly, mitigating changes in the global climate system. Wind energy is becoming more common among all renewable energy sources used for electricity generation in terms of generation capacity, rapid growth and technological maturity. The share of wind energy in Türkiye's total electricity production, whose installed capacity has been increasing in recent years, has nearly tripled in the last decade. However, given that wind energy potential varies with wind speed, even small changes in future wind patterns and characteristics can strongly affect future wind power generation dependent on projections. For this purpose, in this study, Türkiye's mid-future (2031-2060) wind energy potential is examined under optimistic (SSP2-4.5) and pessimistic (SSP3-7.0) scenarios. In the study, 0.25° x 0.25° spatial resolution CMIP6 models from the NASA Earth Exchange Global Daily Downscaled Projections (NEX-GDDP-CMIP6) dataset were used. The results point to regional differences in Turkey's mid-future (2031-2060) wind energy potential.

Acknowledgement: This research was supported by DaVinci Energy Investments and Consulting Industry and Trade Inc.

How to cite: Demiralay, Z., Turp, M. T., An, N., and Kurnaz, M. L.: Projected Changes in Türkiye's Wind Energy Potential Using Next-Generation Climate Models and Scenarios, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12367, https://doi.org/10.5194/egusphere-egu23-12367, 2023.

EGU23-12949 | Orals | ERE2.1

Post-processing and high-resolution downscaling of subseasonal ensemble forecasts with focus on renewables using statistics and machine learning 

Irene Schicker, Markus Dabernig, Petrina Papazek, Theresa Schellander-Gorgas, and Michael Tiefgraber

In the past decade, significant advances were made in improving the S2S and seasonal prediction using mainly numerical weather prediction models (NWP) and in some cases climate models for generating the predictions. Recently, the application of these models in real time forecasting through the S2S Real-Time Pilot Initiative (Robbins et al., 2020) was evaluated and is ongoing. There are, however, drawbacks. Computational costs for performing one forecast cycle are high (RAM, storage, ensemble for uncertainty) and limit the spatial, and to some extent temporal, resolution which are currently roughly 1.5° in spatial and at most 6-hourly in temporal resolution. Both resolutions are not sufficient for small scale renewable production sites.

 

In renewable energy applications, these time scales are getting more important as they can adapt their resource management strategies based on predictions of possible load/heating and cooling demand via anomalies to temperature, wind, precipitation amount, effects on the markets can be better estimated for trading, and scheduling of maintenance works. Thus, at least higher spatial resolutions could help improving the management and planning of these tasks.

 

Within the SSSEA project (SubSeasonal to Seasonal Ensemble prediction and Application), in project phase I, different methods for post-processing and downscaling the S2S challenge data to 1 km resolution and actual values instead of anomalies were implemented. The statistical methods EPISODES, GMOS, and SAMOS were adapted to be able to work with different time scales compared to their initial implementations (seasonal/hourly) and machine learning based methods were developed from scratch using a feed forward neural network, a Unet-based model, and a Random Forest. Temperature, precipitation, and in the currently ongoing project phase II, the wind components of the ECMWF S2S model were downscaled to daily analysis fields based on the INCA model.

 

For wind energy applications, specific indices were developed and applied to the downscaled results.  Verification and definition of suitable metrics is crucial to assess the skills of the different methodologies considered and a wide range of aspects and metrics were considered. Results on both grid and station verification for appx. 250 sites in Austria across nearly all altitude ranges show that all post-processing models are able to improve the ECMWF ensemble forecasts for the parameters considered, though, depending on lead time and season, differences in the models’ skill are visible. Furthermore, for most of the initial times and leadtimes in the forecast/testing period of 2020 we were able to outperform also the climatology. To assess the impact on renewable energy production, different indices were derived and evaluated with focus on wind energy and hydrology in project phases I and II. Results of SSSEA show clearly the added value of the post-processed and downscaled subseasonal predictions for both parameters and specified indices.

How to cite: Schicker, I., Dabernig, M., Papazek, P., Schellander-Gorgas, T., and Tiefgraber, M.: Post-processing and high-resolution downscaling of subseasonal ensemble forecasts with focus on renewables using statistics and machine learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12949, https://doi.org/10.5194/egusphere-egu23-12949, 2023.

EGU23-13992 | Orals | ERE2.1 | Highlight

Towards a paradigm of explainable AI applied in energy meteorology 

Konstantinos Parginos, George Kariniotakis, Ricardo Bessa, and Simon Camal

Standard practice of decision-making in energy systems relies largely on complex modeling chains to address technical constraints and integrate numerous sources of uncertainty. The increased penetration of Renewable Energy Sources (RES) such as solar and wind plants adds complexity due to the weather dependency of their electricity production. Artificial Intelligence (AI) based tools have proven their efficiency in different applications in the energy sector ranging from forecasting to optimization and decision making. They permit to simplify modeling chains and to improve performance due to higher learning capabilities compared to state-of-the-art methods. However, decision-makers of the energy sector need to understand how decision-aid tools construct their outputs from the data. AI-based tools are often seen as black-box models and this penalizes their acceptability by end-users (traders, power system operators a.o.). The lack of interpretability of AI tools is a major challenge for the wider adoption of AI in the energy sector and a fundamental requirement to better support humans in the decision-aid process. Agents of energy systems expect very high levels of reliability for the various services they provide. As energy systems are impacted by multiple uncertainty sources (e.g. available power of RES plants, weather and meteorological conditions, market conditions), developed AI tools should not only be performant on average situations but be able to guarantee robust solutions in the case of an extreme event. Therefore, our research focuses on understandable representations of data-driven decision-aid models for human operators in the energy sector. In order to enhance the interpretability of the AI models, a technique borrowed from the computer science domain is explored and further developed. Genetic programming and more precisely Symbolic Regression is used to derive a symbolic representation for the data-driven model that can take the form of a single equation. This equation results according to a specific reward function. The optimal solutions are selected naturally mimicking the biological theory of survival of the fittest. The main outcome is the production of symbolic representations of the AI models that require minimum changes when applied to different case studies. In this presentation a real-world use case is considered, to demonstrate the added value of the proposed tools for decision-making when trading the production of wind and solar power plants to the day-ahead market. An annual period of data is considered to train and test the proposed model. The typical modeling chain involves as many as 12 models for forecasting RES production, weather and meteorological conditions, together with stochastic optimization to derive trading decisions. A single AI-based model here replaces this complex chain. Such simplification is a significant enhancement to the modeling chain interpretability and facilitates trust to the human decision-maker. This work is carried out in part in the frame of the European project Smart4RES (Grant No  864337) supported by the H2020 Framework Program and in part in the frame the Marie-Curie COFUND project Ai4theSciences (Grant No  945304)

How to cite: Parginos, K., Kariniotakis, G., Bessa, R., and Camal, S.: Towards a paradigm of explainable AI applied in energy meteorology, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13992, https://doi.org/10.5194/egusphere-egu23-13992, 2023.

EGU23-14098 | ECS | Posters on site | ERE2.1

Offshore wind energy climate projections for the European region 

Stefano Susini and Melisa Menendez

The wind energy sector is experiencing a solid expansion towards the open sea, where higher-quality resources are available. This tendency is slowed down by the uncertainties in metocean characterization, with the wind playing a significant role as it represents both an action and a resource for the wind plant. The present study aims to investigate the climate change impact on the marine wind conditions, focusing on mean and extreme values.

Atmospheric circulation patterns over the European seas are classified based on combinations of the atmospheric sea level pressure and the directional wind speed data from the ERA5 reanalysis (1985-2015). These present climate patterns are then used to assess the performance of several General Circulation Model simulations from the sixth Climate Model Intercomparison Project (CMIP6) during the present climate. The best-performing models are then analyzed to provide projections of mean and extreme wind conditions in multiple shared socio-economic scenarios (SSP1-2.6, SSP2-4-5, and SSP5-8.5) and future horizons (2030-2060 and 2700-2100).

Results show a general decrease in the mean offshore wind speed over the European region, more intense in the Mediterranean Sea, while extreme wind speed will increase up to 3% along the Atlantic coast of Europe. The southeastern Atlantic coast appears to be favored in the analyzed climate change scenarios, as the extreme events are projected to reduce their intensity, while the wind resource is not expected to vary significantly.

How to cite: Susini, S. and Menendez, M.: Offshore wind energy climate projections for the European region, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14098, https://doi.org/10.5194/egusphere-egu23-14098, 2023.

EGU23-14422 | ECS | Posters virtual | ERE2.1

Use of Several Sources of Spatio-temporal Information to Improve Short-term Photovoltaic Power Forecasting. 

Kevin Bellinguer, Robin Girard, Guillaume Bontron, and Georges Kariniotakis

In recent years, the share of photovoltaic (PV) power in Europe has grown: the installed capacity increased from around 10 GW in 2008 to nearly 185 GW in 2021. Due to the intermittent nature of PV generation, new challenges arise regarding economic profitability and the safe operation of the power network. To overcome these issues, a special effort is made to develop efficient PV generation forecasting tools.

Several sources of information are currently investigated in the literature. Each one possesses different characteristics, which make them horizon-specific. For short-term forecasting (i.e. from a few minutes to 6-hour ahead), endogenous inputs, namely past PV production measurements, are typically the main drivers. With the development of PV plants, and the advances in smart monitoring and measurements, we observe a paradigm shift from temporal- to spatio-temporal (ST)-based forecasting models. This family of models considers features that exploit ST correlations in the data, such as observations from spatially distributed portfolios of PV plants. This new paradigm offers power producers the possibility to economically value information from geographically distributed plant networks in the form of forecast accuracy improvements, and prepares the ground for a data-sharing market.

Depending on its distribution or density, a PV network may partially account for the complex ST processes at stake (e.g. mainly sites located upwind or crosswind). To fill this gap, satellite-based observations are an appealing option. With recent developments, geostationary satellites can capture images of Earth at a temporal resolution of less than an hour, which enables operational uses. Contrary to the spatial inflexibility inherent to PV networks, satellite-based observations offer the possibility of covering the whole vicinity of the site location, and much more. In that context, relevant features selection tools need to be considered.

In this work, we propose the following contributions to the state of the art. Traditionally in the literature, observations from spatially distributed units and satellite-derived information are used separately. We propose an incremental approach to assess the impact of one or several sources of data on the forecasting performances of the considered regression model. This approach shows that the combination of various sources of ST information leads to higher accuracy than when inputs are considered individually. This is assumed to result from the difference in spatial resolutions of both features. In this specific case study, we highlight the limits of the PV plants portfolio through an analysis of the local topography and wind distribution at several altitudes Then, we consider cloud opacity maps obtained from infrared channels. Despite being under-represented in the literature (only two studies have been found), infrared channel-based data present the advantage of offering nighttime observations of cloud cover, which contributes to improving early morning forecasts.

The proposed approaches are evaluated using 9 PV plants in France and for a testing period of 12 months.

How to cite: Bellinguer, K., Girard, R., Bontron, G., and Kariniotakis, G.: Use of Several Sources of Spatio-temporal Information to Improve Short-term Photovoltaic Power Forecasting., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14422, https://doi.org/10.5194/egusphere-egu23-14422, 2023.

Solar energy from photovoltaics (PV) is a major contributor to the power production, e.g., in Germany, with a growing share. It is a major contributor to renewable power production but highly volatile as it is heavily influenced by atmospheric conditions. Especially shading by clouds can change within seconds to minutes and cause ramps in irradiance and solar power production. Accurate short-term predictions (nowcasts) of irradiance for the next minutes can help to alleviate the impact of this volatility and improve the integration of solar power into energy grids. One approach for nowcasting is the use of all-sky imagers (ASI), ground based fisheye cameras which capture the current cloud situation. Therefore, cloud information is extracted from current images, future cloud states are extrapolated and converted into an irradiance nowcast. Despite substantial progress in the quality of the applied methods, current ASI nowcasting models still exhibit significant nowcast errors and struggle to reliably outperform persistence nowcasts for all situations. Therefore, we assessed the implications for nowcast performance of two common fundamental simplifications of ASI nowcasting models. Firstly, cloud evolution is often modelled by advection, i.e. simple displacement over time. Growth, shrinking or reshaping of clouds is usually neglected in the models. Additionally, the ASI viewing geometry may introduce a misrepresentation of the depicted cloud scene, which is also commonly neglected. The ASI views surrounding clouds from a single ground position and under varying angles. For direct irradiance however, the horizontal distribution of clouds and their intersection in the direction of the sun is essential. While ASI images are usually reprojected to comply with the required horizontal representation, the original difference in actual and required viewing geometry cannot be fully compensated. E.g., breaks between distant clouds may not be clearly visible by the ASI although modulating the irradiance. Kurtz et al. (2017) demonstrated a major impact by this geometric limitation. We applied a nowcasting model to synthetic ASI images of a simulated cloud scene to extend this previous study and analyze the errors introduced by both of the two commonly used simplifications of ASI nowcasting models. A large fraction of the nowcasting error is attributable to the simplifications, which implies a systematic baseline error of common ASI nowcasting models. While the implementation of more evolved cloud evolution and a better representation of relevant cloud geometry are challenging, this work indicates, that efforts to implement these improvements in ASI nowcasting models are a chance for a leap in performance of future nowcasting models.

 

Kurtz, B., Mejia, F., and Kleissl, J.: A virtual sky imager testbed for solar energy forecasting, Solar Energy, 158, 753–759, https://doi.org/10.1016/j.solener.2017.10.036, 2017.

How to cite: Gregor, P., Zinner, T., and Mayer, B.: How good can we get? – An analysis of systematic errors in common models for all-sky imager based irradiance nowcasting for solar energy, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14645, https://doi.org/10.5194/egusphere-egu23-14645, 2023.

EGU23-14674 | Posters on site | ERE2.1

IEA Wind Task 51 Forecasting for the Weather Driven Energy System 

Gregor Giebel, Caroline Draxl, Helmut Frank, John Zack, Corinna Möhrlen, George Kariniotakis, Jethro Browell, Ricardo Bessa, and David Lenaghan
The energy system needs a range of forecast types for its operation in addition to the narrow wind power forecast. Therefore, the group behind the former IEA Wind Task 36 Forecasting for Wind Energy (running 6 years, from 2016-2021) has broadened its perspective on forecasting issues in part by reaching out to other IEA Technology Collaboration Programmes such as the ones for PV, hydropower, system integration, hydrogen etc. The three existing Work Packages (WPs) on NWP Improvements (WP1), Power and Uncertainty Forecasting (WP2) and optimal use of Forecasting Solutions (WP3), are complemented by thirteen work streams in a matrix structure.
 
The three work packages span three distinct areas of challenge in forecasting for the weather driven energy system. The first area is the continuing effort to improve the representation of physical processes in weather forecast models through both new high performance initializations and tailored parameterizations. The second area is the heterogeneity of the forecasters and end users, the full understanding of the uncertainties throughout the modelling chain and the incorporation of novel data into power forecasting algorithms. A third area is representation, communication, and use of these uncertainties to industry in forms that readily support decision-making in plant operations and electricity markets.
 
Task 51 will focus on facilitating communication and collaborations among international research groups engaged in the improvement of the accuracy and applicability of forecast models and their utility for the stakeholders in the wind industry, in the power sector and in the energy system.
 
The first two activities of Task 51 were (1) a workshop in Dublin on the State of the Art and Research Gaps for Forecasting. The results of the workshop will be compiled into a journal article, and (2) the publication of the IEA Recommended Practice for the Implementation of Renewable Energy Forecasting Solutions as an open access book by Elsevier. Other planned activities include further workshops on seasonal forecasting with emphasis on Dunkelflaute, storage and hydro in May 2023, a workshop on minute-scale forecasting (2024), and a workshop on extreme power system events (2025). The results of these interactive workshops will be compiled into a journal articles. Additionally, the Recommended Practice on Forecast Solution Selection will be updated to reflect the broader perspective.
 
Reference: Corinna Möhrlen, John Zack, Gregor Giebel (eds): IEA Wind Recommended Practice for the Implementation of Renewable Energy Forecasting Solutions. Elsevier, 348 pages, Nov. 2022. ISBN: 9780443186813. Download the individual chapters from https://www.sciencedirect.com/book/9780443186813/iea-wind-recommended-practice-for-the-implementation-of-renewable-energy-forecasting-solutions.

How to cite: Giebel, G., Draxl, C., Frank, H., Zack, J., Möhrlen, C., Kariniotakis, G., Browell, J., Bessa, R., and Lenaghan, D.: IEA Wind Task 51 Forecasting for the Weather Driven Energy System, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14674, https://doi.org/10.5194/egusphere-egu23-14674, 2023.

EGU23-14723 | Posters on site | ERE2.1

Analysis of Wind Energy production conditions in Catalonia (NE Spain) based on multiple data sources: station data, ERA-5 Reanalysis, WRF/CALMET, and EURO-CORDEX.  

Enric Aguilar, Oleg Skrynyk, Jon Xavier Olano Pozo, Anna Boqué Ciurana, and Antoni Domènech

Climate Change is largely affecting western societies and urgent decarbonization is a must to limit as much as possible global warming. Renewable energy is a critical component of this energy transition, as well as changes in human behavior. According to the Catalan Institute of Energy (ICAEN), Catalonia generated 2,706 GWh of wind energy in 2021, accounting for 6.4% of the total production.  

 

In this contribution, we explore the clear connection between wind energy capacity and weather and climate conditions. First, we use ERA-5 mean sea level pressure data (1959-2021) to identify the dominant circulation types and their evolution. Second, we combine these data with accurate local station data from the Catalan network of automatic weather stations (XEMA, from the acronym in Catalan) for the period 2009-2021 to identify the geographic patterns of wind energy production under the different circulation types. This analysis is refined using a coupled WRF/CALMET (on a 3km and 1km grid, respectively) hybrid dynamical/statistical downscaling of the GFS global data performed for the period 2016-2020. The investigation supports the assumption that, climatologically speaking, the southern areas in the mountains of Tarragona’s province and the northeastern area of Catalonia, bordering with France, are the most suitable for producing wind energy in most circumstances.  

 

Finally, using EURO-CORDEX climate model projections, we inspect future conditions.  

 

How to cite: Aguilar, E., Skrynyk, O., Olano Pozo, J. X., Boqué Ciurana, A., and Domènech, A.: Analysis of Wind Energy production conditions in Catalonia (NE Spain) based on multiple data sources: station data, ERA-5 Reanalysis, WRF/CALMET, and EURO-CORDEX. , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14723, https://doi.org/10.5194/egusphere-egu23-14723, 2023.

EGU23-14800 | Orals | ERE2.1

Integrated solar hydrogen production: Impact of the local climate 

Matthias M. May, Erica Schmitt, Johannes Grabenstein, Oliver Höhn, James Barry, Moritz Kölbach, and Kira Rehfeld

Hydrogen as a versatile, greenhouse gas-free energy carrier will play an important role in our future economy. Yet sustainable, competitive production and distribution of hydrogen remains a challenge. Highly integrated solar water splitting systems aim to combine solar energy harvesting and electrolysis in a single device, similar to a photovoltaic module.[1] Such a system can produce hydrogen locally without the requirement to be connected to the electricity grid. Unlike large electrolysis that draws power from the grid, the power density of such a device is reduced so far that it does not require active cooling, but its operating temperature will closely follow outdoor conditions.

Here, we present our work on high-efficiency integrated solar water splitting devices based on multi-junction solar absorbers. The light-absorbing component is sensitive to the shape of the solar spectrum and generally becomes more efficient at lower temperatures. Catalysis, on the other hand, benefits from higher temperatures. These conflicting trends wih respect to the temperature impact the design of the solar hydrogen production system. We analyse how the local climate affects production efficiency[2] and show in a lab study that adequate system design allows efficient operation at temperatures as low as -20°C.[3] These insights can help to design small-scale distributed solar hydrogen production for both temperate regions, but also more extreme climatic conditions.

[1] M.M. May et al., Nature Communications 6 (2015), 8286.
[2] M. Kölbach et al, Sustainable Energy & Fuels 6 (2022), 4062.
[3] M. Kölbach, K. Rehfeld, M.M. May, Energy & Environmental Sciences 14 (2021), 4410-4417.

How to cite: May, M. M., Schmitt, E., Grabenstein, J., Höhn, O., Barry, J., Kölbach, M., and Rehfeld, K.: Integrated solar hydrogen production: Impact of the local climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14800, https://doi.org/10.5194/egusphere-egu23-14800, 2023.

EGU23-14911 | ECS | Orals | ERE2.1

Wind farm wake recovery under different Planetary Boundary Layer schemes in WRF 

Oscar García-Santiago, Jake Badger, and Andrea N. Hahmann

Currently, to include the effects of wind farms in the Weather Research and Forecasting (WRF) model, a common choice is to use the Fitch wind farm parametrisation (WFP). This WFP has long been implemented into the WRF's standard repository and has been the subject of several wind resource assessment studies. However, one of the disadvantages of its current (WRF version 4.4) set-up is that it is constrained to one Planetary Boundary Layer (PBL) parametrisation. The Fitch scheme is coupled to the Mellor-Yamada Nakanishi Niino (MYNN) PBL parametrisation because it can inject Turbulent Kinetic Energy (TKE) from the turbines into the atmosphere. More importantly, it is the only PBL where the TKE advection can be activated. This feature is essential since it stores the TKE from one time step to the next and prevents the high TKE concentration at the turbine's location.

One way for the WFPs to become PBL-independent is to move away from focusing on the TKE source term and parametrise the turbulence in some other way. The Explicit Wake Parametrisation (EWP) is a WFP coupled to WRF that, as opposed to the Fitch scheme, does not include an explicit TKE source term and the turbulence is produced via enhanced vertical shear. The EWP is based on the assumption that the advection and diffusion terms in the RANS Navier-Stokes equations dominate the development of the wake. As a result, the drag equation is also related to the diffusion term from a 1.5 turbulence closure. The EWP then needs the turbine's information, wind speed and the turbulent diffusivity coefficient (Km) from the PBLs to calculate the wind deficit. Given the latter, the EWP can work if Km is present and comes from at least a 1.5-order turbulence closure PBL. However, studies have yet to attempt to prove this feature since it has only been used with the MYNN scheme.

In this study, we demonstrate the use of the EWP in WRF when other PBL schemes are used and the implications of this approach. We demonstrate this implementation under ideal neutral conditions with similar setups and forcings (surface roughness length, Coriolis parameter and hub-height wind speed) for two local (1.5-order closure) PBL schemes. Similarly, we test the possibility of coupling EWP into two non-local PBL schemes (first-order closure). The study focuses on the wake recovery behaviour, the drag strength and the power produced by an idealized wind farm under the four PBL schemes. Early results show faster wake recovery from non-local PBls than local ones, which could be related to the diffusivity coefficient values and the PBL's mixing rates.

How to cite: García-Santiago, O., Badger, J., and Hahmann, A. N.: Wind farm wake recovery under different Planetary Boundary Layer schemes in WRF, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14911, https://doi.org/10.5194/egusphere-egu23-14911, 2023.

EGU23-15319 | ECS | Posters on site | ERE2.1

A Temperature Profile Atlas based on Representative Profiles 

Sebastiaan Jamaer, Nicole van Lipzig, Dries Allaerts, and Johan Meyers

Vertical temperature profiles influence the wind power generation of large offshore wind farms through stability-dependent effects such as blockage and gravity waves. However, wind energy resource assessments often only consider idealized temperature profiles, which are not guaranteed to represent the atmospheric state and its variation. To assist the selection of atmospheric states, we created a temperature profile atlas and representative temperature profiles for Europe. To achieve this, we developed a new, generally applicable, analytical temperature model for the atmospheric boundary layer and lower troposphere with which the European temperature profiles over the period 2016-2020 are analyzed using a double clustering approach. This methodology results in eight representative profiles and spatial clusters with similarly behaving temperature profiles, which are quantified in cluster fingerprints. These representative profiles and cluster fingerprints can be used in the selection of background profiles for wind energy simulations such as LES models and can furthermore be used to make informed comparisons of results from different wind farm sites.

How to cite: Jamaer, S., van Lipzig, N., Allaerts, D., and Meyers, J.: A Temperature Profile Atlas based on Representative Profiles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15319, https://doi.org/10.5194/egusphere-egu23-15319, 2023.

East Asia is a highly industrialized region with elevated GHGs emissions from extensive fossil fuel use. To achieve the Paris Agreement’s primary goal, an increase in the production of renewable energy is required in this region. Renewable energy generation, such as photovoltaic or wind power, is directly affected by weather and climate. Therefore, a detailed investigation of present and future changes in future renewable energy production potential using high-resolution and reliable climate data should be conducted to develop renewable energy policies. This study investigated recent changes in Wind Energy Potential (Wpot) over East Asia and projected them for the future period using the CORDEX-East Asia phase Ⅱ high-resolution multiple regional climate models. The averaged Wpot over the past 40 years (1979-2018) was highest in western and eastern Inner Mongolia across all seasons, and the recent Wpot in East Asia generally increased in spring, autumn, and winter, and decreased in summer, but had large inter-regional variability. In particular, the recent increase in Korea and Inner Mongolia was the largest in spring. Moreover, in inner Mongolia, wind speeds from 12 m s-1 or higher to less than 25 m s-1, which are the highest efficiency sections, were the most frequent and had the highest rate of increase. In the case of the RCP2.6 scenario, Wpot will increase considerably in central and southern China in the near future from 2021 to 2050 and decrease in summer in Korea, and will increase throughout East Asia in the mid-future (2051-2080) than in the near future, and in the far future (2081-2099) is projected to decrease. In the RCP8.5 scenario, the difference between regions is larger than that of the RCP2.6 scenario, and the increase is projected to be larger in central and southern China.

 

Acknowledgments: This work was funded by the Korea Meteorological Administration Research and Development Program under Grant KMI(KMI2021-00913).

How to cite: Park, C., Shin, S.-W., and Cha, D.-H.: Future Projections of Wind Energy Potential in East Asia Using the CORDEX-East Asia High-Resolution Multiple Regional Climate Models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15469, https://doi.org/10.5194/egusphere-egu23-15469, 2023.

EGU23-15554 | ECS | Orals | ERE2.1

Surface solar radiation trends over Europe assessed from ground-based measurements and satellite imagery and their comparison with climate models 

Leandro Cristian Segado-Moreno, José Antonio Ruiz-Arias, and Juan Pedro Montávez

Downward surface solar radiation (SSR) is the main component in the surface energy balance and the climate system, as well as being the fundamental source of energy in various forms of solar and photovoltaic technologies. It is therefore of great importance to know in detail the spatio-temporal variation of SSR, as well as its long-term trends. Scientific evidence has shown that the amount of solar radiation incident on the Earth’s surface is not stable over the years, but undergoes significant variations every decade. Until recently, ground-based observations have been the most reliable data source for SSR monitoring. Nevertheless, satellite-derived SSR measurements have a better spatial and temporal coverage, though the scientific literature on the use of satellite imagery for the study of SSR is still limited.

This study covers several purposes. First, a direct comparison between ground-based observations and satellite-derived estimates has been carried out, to determine the capability of the latter to reproduce measurements from surface observations. Monthly averaged time series of 108 land stations from GEBA (Global Energy Balance Archive) dataset (ground observations) have been compared to those estimated from satellite imagery by the Solargis model over the same locations. Solargis is a company based in Bratislava, dedicated to the assessment of the solar resource worldwide, using GIS (Geographic Information Systems). SSR anomalies measured at the surface and estimated from satellite images have been compared over Europe for the period 1994-2019. Second, multiannual SSR trends have also been calculated in detail (station-averaged and station-separated) for both ground-based and satellite-derived datasets, in the period of study. Finally, SSR time series have been compared to several CMIP6 (Coupled Model Intercomparison Project Phase 6 ) climate models runs.

The results show that the method of estimating SSR from satellite images is able to reproduce around 94% of the variability of the SSR measured by ground-based methods in Europe. In addition, trend analysis shows a general increase of SSR over the continent in the period of this study, with an average trend of 3.5 Wm-2decade-1for the observational data and 1.7 Wm-2decade-1for the satellite estimations. This increase in SSR may be associated with changes in the transmission of the atmosphere due to variations in cloud properties and aerosols. Finally, CMIP6 time series average over all models for RCP8.5 scenario shows exactly the same trend as the satellite-derived dataset, which suggests there are still some variables not considered by satellite imagery methods and climate models.

How to cite: Segado-Moreno, L. C., Ruiz-Arias, J. A., and Montávez, J. P.: Surface solar radiation trends over Europe assessed from ground-based measurements and satellite imagery and their comparison with climate models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15554, https://doi.org/10.5194/egusphere-egu23-15554, 2023.

EGU23-15617 | ECS | Posters on site | ERE2.1

A Computational Fluid Dynamics based framework to assess the wind energy potential of an urban landscape: A case study in Brussels 

Sampath Kumar Raghunathan Srikumar, Gabriele Mosca, Ioannis Tsionas, Maider Llaguno-Munitxa, André Stephan, and Alessandro Gambale

Wind is a clean and renewable energy source that has the potential to significantly contribute to the electricity supply in urban areas. Electricity generation through Micro Wind Turbines (MWTs) in an urban setting is not often implemented given their expected low performance due to low wind speed. Wind speed is indeed generally lower in urban areas than in open, rural, and coastal areas: buildings and structures represent obstacles to the wind flow and reduce its velocity. But those same obstacles also locally accelerate the flow at some locations, so that accurate positioning of wind turbines can often result in a satisfactory performance. 

In the present work, a framework is detailed to assess the wind energy potential of an urban neighborhood using Computational Fluid Dynamics (CFD) and applied to the Northern District of Brussels, Belgium, a neighborhood that has the ambition to become a Positive Energy District. Assessing the wind energy potential of an urban area requires knowledge of local wind properties (speed, direction, turbulence) to a high spatial resolution, as conditions even on a single roof are not uniform. CFD is a powerful tool that can be used to discern wind patterns and aid in an accurate assessment of the wind energy potential. By using CFD, it is possible to accurately predict the wind speed, direction and turbulence within an urban landscape, taking into account the effects of buildings, terrain and other structures. 

Statistical wind data from the last 30 years collected by the nearest meteorological station is used to define the conditions for a large enough number (typically 5-10) of CFD simulations for each wind direction. Based on the obtained results, the potential energy output of a specific MWT can be predicted and sites with suitable conditions can be identified. Simulations are performed using the opensource finite-volume solver OpenFOAM v7. A modified RANS turbulence model (k-ω SST)  with the improved Atmospheric Boundary Layer (ABL) approach from Bellegoni et al  is used to solve the flow equations in order to improve the accuracy of results. 

The numerical analysis allowed to identify the most suitable locations for MWTs in Brussels Northern District, demonstrating how the described approach can be effectively used in assessing the wind energy potential in an urban environment. 

How to cite: Raghunathan Srikumar, S. K., Mosca, G., Tsionas, I., Llaguno-Munitxa, M., Stephan, A., and Gambale, A.: A Computational Fluid Dynamics based framework to assess the wind energy potential of an urban landscape: A case study in Brussels, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15617, https://doi.org/10.5194/egusphere-egu23-15617, 2023.

EGU23-17208 | ECS | Orals | ERE2.1

Statistical characterization of simulated wind ramps 

Harish Baki, Sukanta Basu, and George Lavidas

Wind ramps, or rapid changes in wind speed, are a crucial aspect of atmospheric dynamics and
have significant implications for various wind energy applications. For example, wind ramps tend
to increase uncertainty in power output predictions. Furthermore, they also induce fatigue damage
to wind turbines.


In a recent study, DeMarco and Basu (2018; Wind Energy) used long-term observational
data from four geographical locations to characterize the tails of the wind ramp probability
distribution functions (pdfs). They showed that the pdfs from these various sites (ranging from
offshore to complex terrain) portray quasi-universal behavior. The tails of the pdfs are much
heavier than the Gaussian pdf and decay faster with increasing time increments. The tail-index
statistics, computed via the so-called Hill plots, exhibited minimal height dependency up to
approximately one hundred meters above the land or sea surface level. However, wind ramp
statistics at higher altitudes at Cabauw (the Netherlands) were quite distinct.


In the present study, we investigate if state-of-the-art reanalysis datasets capture the
intrinsic traits of wind ramp pdfs. Specifically, we make use of the newly released Copernicus
European Regional ReAnalysis (CERRA) dataset in conjunction with the popular fifth-generation
ECMWF reanalysis (ERA5) dataset. These datasets allow us to describe the characteristics of wind
ramp pdfs at high altitudes (up to 500 m). Given the disparity of the spatial resolution of CERRA
(~5.5 km) and ERA5 (~32 km) datasets, we are also able to demonstrate the impact of spatial
resolution on simulated tail index characteristics. Lastly, the influence of natural climate patterns
such as El-Nino and La-Nina on wind ramp pdfs are examined.

How to cite: Baki, H., Basu, S., and Lavidas, G.: Statistical characterization of simulated wind ramps, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17208, https://doi.org/10.5194/egusphere-egu23-17208, 2023.

EGU23-17290 | Orals | ERE2.1 | Highlight

Improving the satellite retrieval of surface solar irradiance during an eclipse 

Arindam Roy, Annette Hammer, Marion Schroedter-Homscheidt, Jorge Lezaca, Faiza Azam, Ontje Lünsdorf, Detlev Heinemann, and Yves-Marie Saint-Drenan

Solar eclipse causes high magnitude fluctuations in the Surface Solar Irradiance (SSI) for a short duration and consequently reduces the output of solar PV systems. Grid operators try to estimate the impending loss in PV power generation prior to the occurrence of an eclipse in order to schedule conventional generators for compensating the loss. The worldwide installed capacity of grid connected solar PV systems is expected to steeply rise in the coming decade as a result of the various policy initiatives aimed to tackle the climate change. In future electric supply networks with a high penetration of solar PV systems, such large ramps in generation could impact the stability of the network. Although a solar eclipse is a purely deterministic phenomenon, it’s impact on the satellite retrieval of Surface Solar Irradiance (SSI) is complicated due to the possibility of cloud presence in the regions affected by the eclipse. The extraterrestrial solar irradiance is reduced by the moon during an eclipse. On the one hand this causes clouds to appear darker and they get assigned lower reflectance values than they should have in reality. This leads to predicting higher values for the solar irradiance under these clouds than expected. On the other hand, the eclipse also reduces the clear sky irradiance reaching the earth surface. We developed a method to make corrections for both of these effects on the High Resolution Visible (HRV) channel images from Meteosat-11 The results are validated against ground measurements of irradiance provided by BSRN, IEA-PVPS, DTN and the National Weather Services networks. The validation is performed for sites with locations across Europe and for the last two eclipses.  

How to cite: Roy, A., Hammer, A., Schroedter-Homscheidt, M., Lezaca, J., Azam, F., Lünsdorf, O., Heinemann, D., and Saint-Drenan, Y.-M.: Improving the satellite retrieval of surface solar irradiance during an eclipse, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17290, https://doi.org/10.5194/egusphere-egu23-17290, 2023.

EGU23-2364 | ECS | Orals | GMPV8.5

Measuring volcanic ash optical properties with high-spectral resolution infrared sounders: role of refractive indices 

Alexandre Deguine, Lieven Clarisse, Hervé Herbin, and Denis Petitprez

Hyperspectral infrared sounders like IASI are used to track and quantify volcanic ash in the atmosphere. The retrieval process of physical quantities like particle radius and mass depends critically on the assumed spectrally dependent complex refractive indices that are used. Traditionally, the Pollack et al. (1973) dataset were used almost exclusively. These indices are however based on measurements of rock slabs and in recent years two datasets have become available from laboratory measurements of ash in suspension, the Reed et al. (2018) and Deguine et al. (2020) dataset. In this work, we compare for the first time the three most important datasets of CRI with respect to the three most common ash types (basaltic, andesitic and rhyolitic). The results show significant influence of the dataset used on the retrieved physical quantities. When it comes to basaltic and andesitic ash, both the Deguine and Reed samples outperform Pollack in terms of able to reconstruct the satellite observed spectra. However, all datasets overestimate the extinction near 1250 cm−1, which could possibly be related to the lack of sensitivity of spectrometers (water vapour continuum) leading to a poor signal over noise ratio in this spectral region. While this is not a guarantee that the retrieved quantities are closer to the physical reality, being able to reconstruct the observed spectra is a prerequisite of constructing a consistent physical model. Finally, a case study on the 7 May 2010 plume of the Eyjafjallajokull eruption is presented. For this case study, the differences are found to be mostly related in retrieved altitudes. It is clear that while the availability of CRI based on ash suspended in air is an important milestone, a lot of further research is needed to strengthen the theoretical basis of infrared retrievals of volcanic ash. A comprehensive database of reliable in-situ measurements of volcanic clouds would in this perspective be most welcome.

A. Deguine, D. Petitprez, L. Clarisse, S. Gudmundsson, V. Outes, G. Villarosa, and H. Herbin, “Complex refractive index of volcanic ash aerosol in the infrared, visible, and ultraviolet,” Applied Optics, vol. 59, no. 4, p. 884, jan 2020.

J. B. Pollack, O. B. Toon, and B. N. Khare, “Optical properties of some terrestrial rocks and glasses,” Icarus, vol. 19, no. 3, pp. 372–389, jul 1973.

B. E. Reed, D. M. Peters, R. McPheat, and R. G. Grainger, “The complex refractive index of volcanic ash aerosol retrieved from spectral mass extinction,” Journal of Geophysical Research, vol. 123, no. 2, pp. 1339–1350, jan 2018.

How to cite: Deguine, A., Clarisse, L., Herbin, H., and Petitprez, D.: Measuring volcanic ash optical properties with high-spectral resolution infrared sounders: role of refractive indices, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2364, https://doi.org/10.5194/egusphere-egu23-2364, 2023.

Volcanic eruptions used to cause huge disasters which usually bring about many fatalities and property damages, especially a big city near the volcanoes. The Taipei metropolitan city is located at the foot of Tatun Volcano Group (TVO), which has been identified as an active volcano. Meanwhile, several volcanic islands are distributed in the offshore of northern Taiwan, which may be the active volcanoes. Thus, the past eruptive behaviors and mechanisms, characteristics of products, volcanic history and activity, etc.

Based on the field observations, geomorphologic analyses, characteristics of ejecta, as well as the cases of world volcanoes, the explosive craters distributed in both sides of Chihsingshan volcano were produced by the phreatic eruption. Generally, two models of phreatic eruption have been proposed. One is a deeper hydrothermal system fed by magmatic gases being sealed and produces overpressure sufficient to drive explosive eruptions, and the other where magmatic gases are supplied via open-vent degassing to a near-surface hydrothermal system, vaporizing liquid water which drives the phreatic eruptions. The mechanism of Chihsingshan phreatic eruption is similar to the type I, which has hydrothermal reservoir underneath the volcano. Comparing other types of phreatic eruption in the world, for example, Mt. Ontake (Japan)、Inyo Craters (USA) and Tarawera Rift (New Zealand), they have similar common characteristics, (i) occurred in rifting conditions, (ii) heat source from magma intruded along the faults, (iii) had water body, such as groundwater, lakes or hydrothermal fluids, etc. near the conduit of magma. The geology and mechanism of phreatic eruption in the Chihsingshan volcano is more or less similar to the 2014 phreatic eruption of Mt. Ontake, Japan.

How to cite: Song, S.-R.: Characteristics of Latest Eruption in the Tatun Volcano Group, North Taiwan, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3795, https://doi.org/10.5194/egusphere-egu23-3795, 2023.

EGU23-4626 | ECS | Orals | GMPV8.5

A millennial-scale tephra event-stratigraphic record of the South China Sea since the penultimate interglacial 

Deming Kong, Weijia Feng, jiawen Yang, Chuang Bao, and Min-Te Chen

Large volcanic eruptions have significant impacts on climate and environmental changes. The deposition of tephra in marine sediments may serve as an eruption recorder, but it has not been extensively studied in the western Pacific. This study explored a millennial-scale tephra event-stratigraphy with multiple indicators in a sediment core collected from the eastern South China Sea (SCS) basin. The magnetic susceptibility (MS), Fe and Mn concentration determined by X-ray fluorescence (XRF), and identification of individual ash particles were used to identify tephra layers and reconstruct the history of volcanic activity. Nine visible volcaniclastic units (VVU) and two cryptotephra layers have been identified based on their distinct features, as manifested by high MS, Fe, and Mn concentrations, and single-peak grain size distribution. The VVUs and cryptotephra layers reveal elevated volcanic activities. Using the radiocarbon age model and oxygen isotope stratigraphy, these episodes could roughly correspond to the following periods: 1-11 ka, 16-17 ka, 27-31 ka, 41-42 ka, 45-46 ka, 49-50 ka, 77-80 ka, 90-91 ka, 97-99 ka, 116-126 ka, and 132-140 ka. The alkenone-derived SST has significant glacial cycles and good synchronicity with other SCS SST records, which could partially help build the preliminary age model. Despite possible age errors larger than 1 kyr, the discovery and timing of tephra layers provide a preliminary framework to further investigate the impact of historical volcanic eruptions on climate changes.

How to cite: Kong, D., Feng, W., Yang, J., Bao, C., and Chen, M.-T.: A millennial-scale tephra event-stratigraphic record of the South China Sea since the penultimate interglacial, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4626, https://doi.org/10.5194/egusphere-egu23-4626, 2023.

Volcanic sulfur dioxide (SO2) is a gaseous precursor that is transformed into secondary sulfate aerosols (SO42-) by several intricate chemical and physical atmospheric processes. It is currently unclear how quickly sulfate aerosols are produced in volcanic plumes, particularly in tropospheric plumes. We jointly analyze Aura/OMI SO2 observations to constrain the sulfur-rich emissions and identify the volcanic plume dispersion pattern as well as multi-angle, multi-wavelength, and polarizing PARASOL/POLDER-3 observations that are particularly sensitive to fine mode particles to gain a better understanding of the lifecycle of volcanic sulfate aerosols. The GRASP/Component[1] (Generalized retrieval of Aerosol and Surface Properties) algorithm gives us details about the soluble and insoluble aerosol components in both fine and coarse modes based on their complex refractive indices in addition to standard optical characteristics. In order to provide insight into SO2 to particle conversion rate, we analyze the degassing of the Kilauea volcano (Hawaii, USA) between 2006 to 2012, which includes periods of passive and eruptive degassing.

We demonstrate that Kilauea SO2-rich pixels from OMI measurements are broadly collocated with poorly-absorbing fine aerosol-rich pixels from POLDER measurements (fine AOD (440nm) ranging from 0.1 to 0.4, SSA (440nm) ranging from 0.95 to 1.0). We show that these volcanic particles also differ from long-distance transported man-made and natural fine-absorbing particles seen across the Kilauea domain from the Asian region in terms of their absorption characteristics. We, therefore attribute these fine mode particles to sulfate aerosols that result from the conversion of Kilauea SO2 emissions.

In comparison to SO2-rich plumes, Kilauea aerosol-rich plumes have a significantly wider spread and are characterized by an excess anomaly in fine AOD and high SSA values. Irrespective of the degassing strength, a pattern consistent with the oxidation of SO2 to secondary sulfate aerosols is observed where the SO2 concentration gradually drops with plume dispersion while the fine AOD gradually increases, peaking at a distance of around 800–3000 km from the Kilauea source. Depending on the intensity of volcanic activity, the season, and enduring local meteorological conditions, different time scales for oxidation of SO2 and geographical dispersion of the Kilauea aerosol plumes are observed. We conducted additional analysis on the coarse AOD and coarse components to look for ash signals inside the plume. Furthermore, the complex refractive index of Kilauea particles, retrieved by the GRASP/Component algorithm, indicates an imaginary part (0.003-0.005) that is slightly higher than that of volcanic basaltic ash, as determined by laboratory experiments, while the real part (1.49-1.52) lies well in between pure sulfate (1.40-1.46) and basaltic ash (1.56-1.63). These refractive index values imply that Kilauea particles are not pure sulfate aerosols but instead contain some spectrally absorbing elements that may point to the existence of fine ash or sulfate-coated ash particles within the plume.

[1] Li, L., Dubovik, O., Derimian, Y., Schuster, G. L., Lapyonok, T., Litvinov, P., Ducos, F., Fuertes, D., Chen, C., Li, Z., Lopatin, A., Torres, B., and Che, H.: Retrieval of aerosol components directly from satellite and ground-based measurements, Atmos. Chem. Phys., 19, 13409–13443, https://doi.org/10.5194/acp-19- 13409-2019, 2019.

How to cite: Panda, S. R., Boichu, M., Derimian, Y., Dubovik, O., and Behera, A. K.: Insight into the conversion of SO2 to sulphate aerosols in volcanic plumes from the joint analysis of hyperspectral OMI and multi-angular polarimetric POLDER satellite observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5423, https://doi.org/10.5194/egusphere-egu23-5423, 2023.

EGU23-7027 | ECS | Posters on site | GMPV8.5

First archive of extensive N-fixation by volcanic lightning and implications for the prebiotic Earth 

Adeline Aroskay, Erwan Martin, Slimane Bekki, Joël Savarino, Jean-Luc Le Pennec, Abidin Temel, Nelida Manrique, Rigoberto Aguilar, Marco Rivera, and Sophie Szopa

On Earth, most of the nitrogen (N) accessible for life is trapped in dinitrogen (N2), which is the most stable atmospheric molecule. In order to be metabolised by living organisms, N2 has to be converted into assimilable forms, also called fixed N. Nowadays, nearly all the N-fixation is achieved through biological and anthropogenic processes. However, in early environments of the Earth, before the emergence of life, N-fixation must have occurred via natural abiotic processes. Electrical discharges, including from thunderstorms and also lightning associated with volcanic eruptions is one of the most invoked processes. The occurence of volcanic lightning during explosive eruptions is frequent, and convincing laboratory experimentations support the role of this phenomenon, however no evidence of substantial N-fixation has been found in volcanic records.
Here we report on the discovery of large amounts of nitrates in volcanic deposits from Neogene caldera-forming eruptions, which are well correlated with the concentrations of species directly emitted by volcanoes such as sulphur and chlorine. The multi-isotopic composition (δ18O, Δ17O) of the nitrates reveals that they originate from the atmospheric oxidation of nitrogen oxides formed by volcanic lightning that occur during the eruption. According to these volcanic nitrate records, our first estimates suggest that about 60 Tg of N can be fixed during a large explosive event. Our findings hint at a unique role potentially played by subaerial explosive eruptions in supplying essential ingredients for the emergence of life on Earth.

How to cite: Aroskay, A., Martin, E., Bekki, S., Savarino, J., Le Pennec, J.-L., Temel, A., Manrique, N., Aguilar, R., Rivera, M., and Szopa, S.: First archive of extensive N-fixation by volcanic lightning and implications for the prebiotic Earth, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7027, https://doi.org/10.5194/egusphere-egu23-7027, 2023.

EGU23-7268 | ECS | Orals | GMPV8.5

Dispersion modeling of the volcanic sulfur dioxide plumes from the simultaneous eruptive activity of Stromboli and Mt Etna on 28 August 2019 

Giuseppe Castorina, Agostino Semprebello, Alessandro Gattuso, Francesco Italiano, Giuseppe Salerno, Pasquale Sellitto, and Umberto Rizza

During the summer of 2019, both Mt. Etna and Stromboli volcanoes in Sicily were in the stage of no ordinary activity. Mt. Etna was featured by mild strombolian activity from the summit South East Crater producing a moderate SO2–ash rich plume 4 km above sea level (asl). Meanwhile, at 120 km far from Etna, on 3 July and 28August, the ordinary and typical mild explosive eruptive activity of Stromboli was interrupted by two paroxysms. Both events were characterized by pyroclastic flows and consistent emission of ash–SO2 rich plume, which spread up to height of 5–6 km asl.
In this work, we explored the spatial dispersion of the volcanic plumes released by both Mt. Etna and Stromboli on August 28 by employing the Weather Research and Forecasting Chemistry (WRF–Chem) model. The simulation was specifically configured and run by considering the time-variable Eruptive Source Parameters (ESPs) related to the SO2 flux data for Stromboli and Mount Etna observed from ground by the FLAME DOAS scanning spectrometers network.
In order to assess the predictive performance of the WRF–Chem model, the simulated SO2 dispersion maps were compared with data retrieved on 28 August from TROPOMI and OMI sensors onboard Sentinel–5p and Aura satellites. The results show a good agreement between WRF–Chem and satellite data. In fact, the simulated total mass of the emitted SO2 from the two volcanoes has the same order of magnitude as the satellite data. However, for the case of Stromboli, the total SO2 mass predicted by the WRF–Chem simulation is underestimated; this is likely due to inhibition of the real syn-eruptive SO2 detection by FLAME due to the extreme ash–rich volcanic plume released during the paroxysm.
In conclusion, the results of these two test–cases demonstrate the feasibility of WRF–Chem model with a time-variable ESPs in reproducing different levels of volcanic SO2 and their dispersion into the atmosphere. For these reasons, our approach could represent an effective support for the assessment of local–to-regional air quality and flight security and, in case of particularly intense events, also on a global scale.

How to cite: Castorina, G., Semprebello, A., Gattuso, A., Italiano, F., Salerno, G., Sellitto, P., and Rizza, U.: Dispersion modeling of the volcanic sulfur dioxide plumes from the simultaneous eruptive activity of Stromboli and Mt Etna on 28 August 2019, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7268, https://doi.org/10.5194/egusphere-egu23-7268, 2023.

EGU23-7369 | ECS | Orals | GMPV8.5 | Highlight

The evolution and dynamics of the sulfate aerosol plume in the stratosphere after the exceptional Tonga eruption of 15 January 2022 

Clair Duchamp, Bernard Legras, Pasquale Sellitto, Aurélien Podglajen, Elisa Carboni, Richard Siddans, Jens-Uwe Grooss, Felix Ploeger, and Sergey Khaykin

We use a combination of seven space-borne instruments to study the unprecedented stratospheric plume after the Tonga eruption of 15 January 2022.

The aerosol plume was initially formed of two clouds at 30 and 28 km mostly composed of submicron-sized sulfate particles, without ashes washed-out within the first day following the eruption. The large amount of injected water vapour led to a fast conversion of SO2 to sulfate aerosols and induced a descent of the plume to 24-26 km over the first 3 weeks by radiative cooling. Whereas SO2 has returned to background levels by the end of January, volcanic sulfates and water still persisted after 6 months, mainly confined between 35°S and 20°N until June due to the zonal symmetry of the summer stratospheric circulation at 22-26 km. Sulfate particles, undergoing hygroscopic growth and coagulation, sediment and gradually separate from the moisture anomaly entrained in the ascending branch Brewer-Dobson circulation. Sulfate aerosol optical depths derived from the IASI infrared sounder show that during the first two months the aerosol plume was not simply diluted and dispersed passively but rather organized in concentrated patches. Space-borne lidar winds suggest that those structures, generated by shear-induced instabilities, were associated with vorticity anomalies that may have enhanced the duration and impact of the plume.

Reference: ACP Highlight, DOI: 10.5194/acp-22-14957-2022

How to cite: Duchamp, C., Legras, B., Sellitto, P., Podglajen, A., Carboni, E., Siddans, R., Grooss, J.-U., Ploeger, F., and Khaykin, S.: The evolution and dynamics of the sulfate aerosol plume in the stratosphere after the exceptional Tonga eruption of 15 January 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7369, https://doi.org/10.5194/egusphere-egu23-7369, 2023.

EGU23-7516 | ECS | Posters on site | GMPV8.5

Rapid gas measurements in volcanic plumes with UAVs: online and offline measurements of various trace gases with light UAVs 

Niklas Karbach, Bastien Geil, Jonas Blumenroth, Heiko Bozem, Christian von Glahn, Peter Hoor, Nicole Bobrowski, and Thorsten Hoffmann

To protect people and infrastructures in the immediate vicinity of active volcanoes, monitoring the gas composition of the emitted plume is crucial. In order to react quickly to sudden changes in this composition, frequent measurements are key, as different ratios like the halogen/sulfur or the CO2/SO2 ratio can give hints on changing volcanic activity due to their different solubility in magma.   

However, monitoring the chemical composition of the volcanic plume is not an easy task, especially since stationary ground-based gas monitoring stations do not always measure the concentration in the plume, only under certain meteorological conditions, and remote sensing methods are not available for all gases of interest. In this case, human interaction is required to move the measurement equipment to the location of interest, which is close to the active vent. Not only does this pose a serious health risk, it is also burdensome, as the researcher must climb the volcano, take the measurements, climb back down, and analyze the results. This lengthy procedure can be sped up and facilitated by using lightweight drones to take the measurements. Sensors and various other instruments, such as miniaturized alkaline traps or impregnated syringe filters that employ an electrophilic addition to a double bond to selectively absorb halogen species in the oxidation states -1, ±0 and +1, can be mounted on the drone and controlled via a radio link to a ground station. The online results can then be used during the flight to locate the plume to ensure efficient sampling with the absorbers. The landing site of the drone is usually located far away from active vents, which significantly reduces health hazards and speeds up the process.

This poster presents such a drone with its advanced sensor system and absorbers for the determination and quantification of CO2, SO2, acidic gases and halogen species and its deployment during a measurement campaign on Etna in July 2022.

How to cite: Karbach, N., Geil, B., Blumenroth, J., Bozem, H., von Glahn, C., Hoor, P., Bobrowski, N., and Hoffmann, T.: Rapid gas measurements in volcanic plumes with UAVs: online and offline measurements of various trace gases with light UAVs, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7516, https://doi.org/10.5194/egusphere-egu23-7516, 2023.

EGU23-8281 | Posters on site | GMPV8.5

A case study of two simultaneous extreme aerosol events in the Mediterranean: The Mount Etna series of eruptions and major Saharan dust event in February 2021 

Pasquale Sellitto, Giuseppe Salerno, Stefano Corradini, Irène Xueref-Remy, Aurélie Riandet, Clémence Bellon, Sergey Khaykin, Gerard Ancellet, Simone Lilli, Ellsworth J. Welton, Antonella Boselli, Alessia Sannino, Juan Cuesta, Henda Guermazi, Maxim Eremenko, Luca Merucci, Dario Stelitano, Lorenzo Guerrieri, and Bernard Legras

During the extended activity of Mount Etna volcano in February-April 2021, three distinct paroxysmal events took place from 21 to 26 February, which were associated with a very uncommon transport of the injected upper-tropospheric plumes towards the north. A major Saharan dust outbreak to central Europe occurred in the same period. Using a synergy of observations and modelling, we characterise the three-dimensional dispersion of these volcanic plumes and we disentangle their optical and radiative signature from the simultaneous Saharan dust transport. In the region of interest for our study, the volcanic and the dust plumes remain completely vertically-separated, thus facilitating the detection and spatiotemporal characterisation of the dispersion, properties and radiative impacts of these two different aerosol plumes, using vertically-resolved observations. With a satellite-based source inversion, we estimate the emitted sulphur dioxide (SO2) mass at an integrated value of 55 kt and plumes injections at up to 12 km altitudes, which qualifies this series as an extreme event for Mount Etna activity spectrum. Then, we combine Lagrangian dispersion modelling, initialised with measured temporally-resolved SO2 emission fluxes and altitudes, with satellite observations to track the dispersion of the individual volcanic and dust plumes. The general transport towards the north allowed the height-resolved downwind monitoring of the volcanic and dust plumes at selected observatories in France, Italy and Israel, using LiDARs and photometric aerosol observations. A specific effort has been dedicated to the characterisation of the volcanic aerosol plumes. Volcanic-specific aerosol optical depths in the visible spectral range ranging from about 0.004 to 0.03 and local daily average shortwave radiative forcing ranging from about -0.2 to -1.2 W/m2 (at the top of atmosphere) and from about -0.2 to -3.0 W/m2 (at the surface) are found. The composition (possible presence of ash), aerosol optical depth and radiative forcing of the volcanic plumes has a large inter- and intra-plume variability and thus depend strongly on the position of the sampled section of the plumes. The dust optical depth and radiative impact largely outweigh volcanic aerosols when the two plumes are co-located, for this event. This case study points at the complexity of the Mediterranean aerosol environment and pave the way to future studies at longer timescales, exploiting the available observational and modelling capabilities and their synergies.

How to cite: Sellitto, P., Salerno, G., Corradini, S., Xueref-Remy, I., Riandet, A., Bellon, C., Khaykin, S., Ancellet, G., Lilli, S., Welton, E. J., Boselli, A., Sannino, A., Cuesta, J., Guermazi, H., Eremenko, M., Merucci, L., Stelitano, D., Guerrieri, L., and Legras, B.: A case study of two simultaneous extreme aerosol events in the Mediterranean: The Mount Etna series of eruptions and major Saharan dust event in February 2021, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8281, https://doi.org/10.5194/egusphere-egu23-8281, 2023.

EGU23-8559 | ECS | Orals | GMPV8.5

Laki 1783-84 AD tephra linked mercury enrichment in peat at Brackloon Wood, Mayo, Ireland. 

Lucy Blennerhassett and Dr. Emma Tomlinson

Mercury is a significant volcanic volatile species from effusive and explosive activity1. Understanding its emission to the atmosphere from volcanic activity, aids our understanding of the global mercury cycle and its environmental impacts. Sedimentary and ice core records can be archives of these mercury enrichments2,3.

The Laki 1783-84 AD fissure eruption in Iceland was significant due to its voluminous outpouring of basaltic lava, copious sulphur emissions and widespread environmental effects locally and across the Northern Hemisphere4,5. Extreme weather events were recorded in Europe and North America, owing to a veil of sulphur dioxide that remained at the tropopause for over a year5. Due to the phreatomagmatic and thus explosive nature of Laki, a significant eruption plume was produced4. As such, cryptotephra shards have been located at distal locations from Iceland including ice cores in Svalbard and Greenland6,7 and in an Irish woodland peat at Brackloon Wood, Co. Mayo8. There is evidence to suggest significant heavy metal emission to the atmosphere during the Laki eruption, however these records are currently restricted to Greenland ice cores9. Previous heavy metal findings linked to Laki do not include mercury, despite its significance as a volcanic volatile, and a potentially environmentally damaging heavy metal. Therefore, to expand our knowledge of the Laki 1783-84 AD eruption plume, its associated emissions, and environmental consequences we returned to the woodland peat site in Brackloon Wood, Co. Mayo, Ireland.

Analysis of a 50 cm peat core using an AMA 254 mercury analyser was combined with a novel technique to find tephra using BSE (back scattered electron) imaging and geochemical discrimination using SEM-EDX (scanning electron microscopy-energy dispersive x-ray). The Laki tephra is successfully located using this method and coincides with a visible enrichment in mercury relative to background concentrations and organic matter. An age-depth model developed using the tephra layer and two radiocarbon dates indicate a strong likelihood that such enrichments are a product of volcanic emission. Such a finding can expand our understanding of heavy metal deposition during Laki 1783-84 AD away from the poles and to our knowledge, demonstrates the first direct exploration of mercury enrichment in distal peat for this eruption. As a secondary test of volcanic volatile enrichment, trace element analysis of the same bulk peat will be conducted to explore enrichments in other volcanic volatiles such as sulphur, cadmium, lead, copper and zinc.

 

1. Pyle, D. M. & Mather, T. A. Atmos. Environ. 37, 5115–5124 (2003).

2. Schuster, P. F. et al.,. Environ. Sci. Technol. 36, 2303–2310 (2002).

3. Roos-Barraclough, F. et al.,. Earth Planet. Sci. Lett. 202, 435–451 (2002).

4. Thordarson, T. & Self, S. Bull. Volcanol. 55, 233–263 (1993).

5. Thordarson, T. & Self, S., J. Geophys. Res 108, 4011 (2003).

6. Kekonen, T. et al., Polar Res. 24, 33–40 (2005).

7. Wei, L. et al., Geophys. Res. Lett. 35, L16501 (2008).

8. Reilly, E. & Mitchell, F. J., Holocene 25, 241–252 (2015).

9. Hong, S. et al., Earth Planet. Sci. Lett. 144, 605–610 (1996).

 

How to cite: Blennerhassett, L. and Tomlinson, Dr. E.: Laki 1783-84 AD tephra linked mercury enrichment in peat at Brackloon Wood, Mayo, Ireland., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8559, https://doi.org/10.5194/egusphere-egu23-8559, 2023.

EGU23-9128 | Posters on site | GMPV8.5

Ground-based volcanic ash detection with low-cost sensors – a case study at the 2021 Cumbre Vieja eruption 

Jose Pacheco, Diogo Henriques, Sérgio Oliveira, Alexandra Moutinho, Fátima Viveiros, Diamantino Henriques, Pedro Hernández, and Nemesio Pèrez

The Tajogaite eruption of Cumbre Vieja volcano, in 2021, was a basaltic fissure eruption characterised by a variety of eruptive styles ranging from the predominantly strombolian activity, to lava fountaining, ash emission and effusive activity. The eruption lasted nearly 3 months, produced an extensive lava field and about 45.106 m3 of tephra. Although its intensity varied throughout the entire duration of the eruption, the eruptive plume had a typical height of about 3500 m asl and reached a maximum of 8500 m asl just hours before the end of the eruption, on the 13th of December. Ash is, therefore, a significant hazard to consider not only during the eruption, but also on the post-eruption phase.

To measure ash in the air around the volcano, during the last stage of the eruption and the following weeks, an experiment was devised based on a proximal network of several ground-based low-cost sensors, measuring suspended particulate matter (PM10, PM2.5) concentration, air temperature, and relative humidity.

The results showed that, during the documented period, the daily mass concentration of particulate matter in the air reproduced the peak on the eruptive column high at the end of the eruption. After the eruption several significant resuspension events were detected simultaneously in several stations; in addition, after the eruption, a major event of “calima” dust intrusion largely exceeded all recorded eruptive events. Overall, even after the eruption, the 24-hour average exposure to PM2.5 surpassed the guidelines of the World Health Organization.

 

 

This work was partially funded by FCT – Fundação para a Ciência e Tecnologia, under project SONDA - Synchronous Oceanic and Atmospheric Data Acquisition (PTDC/EME-SIS/1960/2020) and INTERREG MAC under the project VOLRISKMAC-II - Fortalecimiento de las capacidades de I+D+i para el desarrollo de la resiliencia frente a emergencias volcánicas en la Macaronesia.

How to cite: Pacheco, J., Henriques, D., Oliveira, S., Moutinho, A., Viveiros, F., Henriques, D., Hernández, P., and Pèrez, N.: Ground-based volcanic ash detection with low-cost sensors – a case study at the 2021 Cumbre Vieja eruption, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9128, https://doi.org/10.5194/egusphere-egu23-9128, 2023.

EGU23-9143 | Orals | GMPV8.5

Quantifying volcanic gas emission rates from infrasound and SO2 cameras: potentials, limitations, and volcanological implications. 

Dario Delle Donne, Giorgio Lacanna, Marcello Bitetto, Giacomo Ulivieri, Maurizio Ripepe, and Alessandro Aiuppa

Volcanic degassing, a persistent manifestation of active volcanoes, provides crucial information on the dynamics of the magmatic feeding systems, and allows identifying the phases of volcanic unrest in the runup to volcanic eruptions. While thus determining volcanic degassing rates is a central topic in modern Volcanology, direct volcanic gas flux observations by classic spectroscopic techniques are challenged by (i) the need of adequate illumination (by sunlight) and clear weather conditions (ii) difficulties in robustly estimating plume speed velocity and transport direction, and (iii) a variety of optical and radiative transfer issues. Because of these, volcanic gas flux records are often sparse and incomplete, and affected by intrinsic noise that may prevent from fully resolving the gas emission changes associated with changing volcanic activity. To overcome such limitations, measuring the infrasound produced by the expansion of over-pressurized volcanic gas in the atmosphere, using infrasonic arrays, offers as a promising alternative/complementary tool to quantify and locate degassing at active volcanoes. Here, we report on 2-year long (April 2017—March 2019) period of combined measurements of the SO2 flux and of volcano-acoustic emissions produced by regular mild persistent strombolian activity and passive degassing of Stromboli Volcano (Sicily, Italy). These were obtained by a permanent monitoring SO2 camera and a five-element short-aperture (~300 m) infrasonic array. Our results highlight substantial temporal changes in degassing activity, that reflect the recurrent episodes of activations/inactivation of multiple distinct degassing sources within the crater area, as coherently tracked by SO2 and infrasound together. A simple waveform modeling of the infrasonic record, assuming a monopole acoustical source, suggests that infrasonic degassing, comprising of explosive events and continuous puffing activity, dominates the total persistent degassing budget as tracked by the SO2 camera.

How to cite: Delle Donne, D., Lacanna, G., Bitetto, M., Ulivieri, G., Ripepe, M., and Aiuppa, A.: Quantifying volcanic gas emission rates from infrasound and SO2 cameras: potentials, limitations, and volcanological implications., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9143, https://doi.org/10.5194/egusphere-egu23-9143, 2023.

Sulfate aerosols are a primary driver of climate impacts during and following volcanic eruptions and form from erupted SO2 gas. However, the amount of SO2 that is delivered to the stratosphere is not clearly related to the amount dissolved in the magma (the ‘sulfur excess problem’). Therefore, magma properties and eruption magnitude are not necessarily predictive of climate impacts from eruptions, which is exacerbated by the as-yet unknown importance of the insulated, hot transport pathway. During a magnitude 6 explosive volcanic eruption there is up to 100 seconds of transport between the magma fragmentation depth – where volcanic ash is formed and the mixture accelerates – and the Earth’s surface. Here, we present a numerical implementation of a theoretical framework which predicts the rapid reactions between gases and volcanic ash in this transport interval, which include: (1) iron oxidation state changes; (2) SO2 uptake via calcium sulfate surface crystallization; (3) HCl uptake via NaCl surface crystallization; and (4) incipient nanolite crystallization that may be related to (1). In all cases, these processes are rate-limited by a suite of diffusive exchanges between the ash bulk and surface, for which our model solves. To demonstrate the upscaled importance of these processes, we couple our models to volcanic plume simulations (using a 1991 Pinatubo baseline simulation), and output the bulk SO2 that can be captured by ash. We find that depending on the source parameters of the eruption, anywhere between 30 and 100 wt.% of the total erupted SO2 can be removed from the plume gas and captured by ash. This effectively changes the sink of SO2 from the stratosphere to the hydrosphere, as CaSO4 crystals are soluble and ultimately wash into the environment following ash deposition. We propose that these hot sulfur scrubbing processes may be crucial in mediating SO2 delivery to the atmosphere, and therefore may explain much of the complexities associated with correlating eruption magnitude with climate impacts in the recent past or back into the Last Glacial period.

How to cite: Vasseur, J., Wadsworth, F., Paine, A., and Dingwell, D.: Hot volcanic ash filters eruptive SO2 during hot transport in conduits and the lower plume: A predictive model with implications for the climate impacts of volcanic eruptions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11407, https://doi.org/10.5194/egusphere-egu23-11407, 2023.

EGU23-11832 | Orals | GMPV8.5

Remote SO2 flux by UV and TIR ground based cameras at Sabancaya volcano (Peru), cross comparison and validation with satellite data 

Stefano Corradini, Giuseppe Salerno, Robin Campion, Lorenzo Guerrieri, Luca Merucci, and Dario Stelitano

During the 14th IAVCEI Field Workshop held in Peru from 6 to 14 November 2022, SO2 plume measurements were carried out remotely in the volcanic plume of Sabancaya volcano. Sabancaya is an active stratovolcano located in southern Peru (15.787°S, 71.857°W), Sabancaya’s first historical record of an eruption dates to 1750 and the most recent eruption began in November 2016. Volcanic activity consist of rhythm vulcanian explosions, which produce a gas-ash rich plumes which rose few km above the summit terrace. On 10 and 11 November 2022, side-by-side observation by UV and TIR ground-based cameras were remotely carried out with the object to observe the passive and active SO2 burden from the volcanic plume of Sambacaya. Two UV cameras systems were employed observing the volcanic plume at 2- and 5-seconds time steps and calibrating SO2 amounts by coupling SO2 DOAS inverted column densities ad and SO2-quartz cell amounts. The TIR camera (named VIRSO2) is a novel system developed for the detection of volcanic plumes, the estimation of the height and the determination of columnar content and the SO2 flux. It allows acquisition of high frequency data both during the day and at night. It is equipped with 3 cameras, two broadband TIR (7-14 micron) and a VIS, capable of acquiring data simultaneously. For the quantitative estimation of SO2, an 8.7 μm filter is installed in front of one of the TIR camera. Retrieved cameras products were cross-compared and validated in order to determinate limit an uncertainty of both methods and results were also compared with those obtained by S5p-TROPOMI instrument.

Preliminary results show a feasible strength between the three ground and space-based techniques. Within the uncertainties of each method, differences between inverted SO2 column densities and emission rates arise from field of view geometrical sampling set-up and radiative transfer. Results gathered in this study prove the promising application of ground-based TIR in volcanic plume SO2 observation.

How to cite: Corradini, S., Salerno, G., Campion, R., Guerrieri, L., Merucci, L., and Stelitano, D.: Remote SO2 flux by UV and TIR ground based cameras at Sabancaya volcano (Peru), cross comparison and validation with satellite data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11832, https://doi.org/10.5194/egusphere-egu23-11832, 2023.

EGU23-12069 | ECS | Orals | GMPV8.5

Explicit simulation of volcanic eruption plumes in atmospheric models: first results and implications 

Sascha Bierbauer, Gholam Ali Hoshyaripour, Julia Bruckert, Daniel Reinert, and Bernhard Vogel

Explosive volcanic eruptions emit large amounts of solid and gaseous materials into the atmosphere, thereby affect weather and climate and pose hazards to human health and aviation. To constrain those impacts it is important to understand dynamical, microphysical and chemical evolution of the eruption plumes. Especially the density of a plume and atmospheric conditions control the dynamical development of an eruption plume. To simulate those plumes correctly the flow field has to be described as a multi-constituent multiphase flow system. This is realized in eruption plume models but not in the conventional atmospheric models. The latter neglect the partial density of ash particles in relation to total air mass and cannot treat for the effect of ash particles on dynamics during simulations. To overcome this limitation, we use a modified version of ICOsahedral Nonhydrostatic model with Aerosols and Reactive Trace gases (ICON-ART) in which we extended the existing equation set. This version of ICON-ART can consider a source of total mass during the eruption as well as a mass sink due to sedimentation of ash and other constituents. The mass source is accounted by an additional source term for total density, and the mass sink is accounted by implementing the lower boundary condition of the vertical velocity at the surface. This leads to a conserved dry air mass and changing total air mass, which affects dynamics and is crucial for handling multiphase flows correctly. Additionally, a momentum forcing as well as a temperature forcing cause the strong updraft within the plume region.

We simulated the real case of the Raikoke eruption in 2019 in a LES-mode for more detailed investigations of the plume. In this experiment, in addition to ash, we also emit water vapor which might lead to an additional upward motion in the convective plume region due to latent heat release when clouds develop. The results show that the model is able to reproduce the observed plume geometry vertically and horizontally. Moreover, we simulated gravity waves that developed during the eruption around the volcano. In combination with microphysics and aerosol dynamics, the new implementations in ICON-ART enable detailed investigations of volcanic plume development across scales.

How to cite: Bierbauer, S., Hoshyaripour, G. A., Bruckert, J., Reinert, D., and Vogel, B.: Explicit simulation of volcanic eruption plumes in atmospheric models: first results and implications, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12069, https://doi.org/10.5194/egusphere-egu23-12069, 2023.

EGU23-13755 | ECS | Posters on site | GMPV8.5

Inversion techniques on volcanic emissions and the use for quantitative dispersion modeling: The case of Etna eruption on 12 March 2021 

Anna Kampouri, Vasilis Amiridis, Ondřej Tichý, Nikolaos Evangeliou, Stavros Solomos, Anna Gialitaki, Eleni Marinou, Antonis Gkikas, Emmanouil Proestakis, Simona Scollo, Luca Merucci, Lucia Mona, Nikolaos Papagiannopoulos, and Prodromos Zanis

Modeling the dispersion of volcanic particles released during explosive eruptions is crucially dependent on the knowledge of the source term of the eruption and the source strength as a function of altitude and time. Forecasting volcanic ash transport is vital for aviation but rather inaccurate for quantitative predictions of the fate of volcanic particle emissions. Here we demonstrate an inverse modeling framework that couples the output of a Lagrangian dispersion model with remote sensing observations to estimate the emission rates of volcanic particles released from the Etna eruption. We use an inversion algorithm (Tichy et al., 2020) where the distance between the model and observations is optimized under the assumption that the source term is either sparse or smooth. The Bayesian formalism allows the algorithm to estimate these characteristics together with the source term itself and thus normalize the inversion problem. This methodology uses source receptor relationships as an input from the FLEXPART (flexible particle dispersion) model constrained by ground-based Lidar measurements and satellite observations of SO2 and ash emissions. The case study analyzed here refers to the Etna eruption on 12 March 2021, with the volcanic plume being well captured by the lidar measurements of the PANGEA observatory located at Antikythera island in southwest Greece. A dense aerosol layer, suspending in the height range between 7.5 and 12.5 km (19:30 - 21:30 UTC), has been captured by the PollyXT lidar. For the inversion simulations, we also use data acquired by the Spin-stabilised Enhanced Visible and Infrared Imager (SEVIRI) instrument, mounted on the Meteosat Second Generation (MSG) geostationary satellite. The aforementioned observations serve as a priori source information to estimate the volcanic ash and SO2 source strength, depending on altitude and time, coupled with the output of the FLEXPART model. Our results are efficient for real-time application and could supply ash forecasting models with an accurate estimation of the mass rate of very fine ash during explosive eruptions. Improved forecasts of the dispersed volcanic plumes following the suggested inverse modeling framework would then allow for more effective emergency preparedness for aviation to ensure safety during volcanic eruptions.

 

This research was also supported by the following projects: ERC grant D-TECT (agreement no. 725698); EU H2020 E-shape project (Grant Agreement n. 820852); PANCEA project (MIS 502151) under the Action NSRF 2014-2020, co-financed by Greece and the European Union. The research was supported by data and services obtained from the PANhellenic Geophysical Observatory of Antikythera (PANGEA) of the National Observatory of Athens (NOA), Greece. O. Tichy was supported by the Czech Science Foundation, grant no. GA20-27939S.

 

Tichy, O.; Ulrych, L.; Smidl, V.; Evangeliou, N.; Stohl, A. On the tuning of atmospheric inverse methods: comparisons with the European Tracer Experiment (ETEX) and Chernobyl datasets using the atmospheric transport model FLEXPART, Geosci. Model Dev. (2020), 13, 5917-5934.

How to cite: Kampouri, A., Amiridis, V., Tichý, O., Evangeliou, N., Solomos, S., Gialitaki, A., Marinou, E., Gkikas, A., Proestakis, E., Scollo, S., Merucci, L., Mona, L., Papagiannopoulos, N., and Zanis, P.: Inversion techniques on volcanic emissions and the use for quantitative dispersion modeling: The case of Etna eruption on 12 March 2021, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13755, https://doi.org/10.5194/egusphere-egu23-13755, 2023.

EGU23-14820 | ECS | Posters on site | GMPV8.5

Pattern of volcanic degassing at open-vent volcanoes using TROPOMI SO2 time-series from COBRA retrievals 

Jordi Van Mieghem, Hugues Brenot, Benoît Smets, and Nicolas Theys

Sensitive and accurate detection of SO2 from remote sensing is essential to monitor volcanic degassing. The main objective of this study is to understand the dynamics of SO2 gas emissions at open-vent volcanoes between major eruptive events, using Sentinel-5P TROPOMI-based SO2 measurements.

Time-series of SO2 mass are analysed at 10 open-vent volcanoes (Ambrym, Erebus, Erta Ale, Kilauea, Masaya, Nyamuragira, Nyiragongo, Stromboli, Villarica, Yasur) using a newly developed TROPOMI SO2 product generated by the Covariance Based Retrieval Algorithm (COBRA; Theys et al., 2021). Compared to the current operational SO2 TROPOMI product (which uses the Differential Optical Absorption Spectroscopy technique), the COBRA dataset has improved performances and reduce both the noise and bias on the data, allowing a more refined study of degassing from open-vent volcanoes.

Time-series have been obtained for SO2 emissions over a period from 2018 to early 2023. For the 10 selected persistently active volcanoes, the SO2 behaviours are analysed and compared, showing cyclic and sporadic variations, as well as peaks of emission when a flank or major eruption occur. Patterns in SO2 time-series during and between major eruptive events are discussed to assess the potential use (and limitations) of these measurements as a tool for early warning and volcanic crisis management.

Reference:

Theys, N., Fioletov, V., Li, C., De Smedt, I., Lerot, C., McLinden, C., Krotkov, N., Griffin, D., Clarisse, L., Hedelt, P., Loyola, D., Wagner, T., Kumar, V., Innes, A., Ribas, R., Hendrick, F., Vlietinck, J., Brenot, H., Van Roozendael, M. (2021). A sulfur dioxide Covariance-Based Retrieval Algorithm (COBRA): application to TROPOMI reveals new emission sources. Atmospheric Chemistry and Physics, 21(22), 16727-16744.

How to cite: Van Mieghem, J., Brenot, H., Smets, B., and Theys, N.: Pattern of volcanic degassing at open-vent volcanoes using TROPOMI SO2 time-series from COBRA retrievals, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14820, https://doi.org/10.5194/egusphere-egu23-14820, 2023.

EGU23-15216 | ECS | Posters on site | GMPV8.5

Trace element transport processes in volcanic gases 

Celine Mandon and Andri Stefansson

Despite our perception of gold as a shiny precious metal, a small amount of gold is actually transported by magmatic gases and emitted in the atmosphere at most volcanoes on Earth. This gaseous transport is made possible by the very nature of volcanic gases: high-temperature non-ideal water vapor-dominated mixture of gases, also containing other major constituents such as sulfur, carbon dioxide and halogens. This combination allows for volatile transport of virtually all elements from the periodic table, through the formation of gaseous compounds between trace elements and major gas species. However, the complexity of volcanic gases also makes them difficult to apprehend; little is known on the solubility and behavior of trace elements. Moreover, the gas composition varies from one volcano to another, while changes in pressure and temperature occur between gas exsolution from the magma and emission at the surface. Interactions between the gas phase and surrounding rocks and fluids can furthermore affect volcanic gases on their way to the surface. In this work, we explore the transport processes controlling the abundance of trace elements in volcanic gases. We use major and trace element composition from fumarolic gases from Vulcano, Italy sampled over a 14-year period and during both background emissions and unrest. We also work with a compilation of high-temperature gas compositions, from fumaroles and volcanic plumes, from various tectonic settings. This data is then used for thermochemical calculations using the HSC Chemistry software. We will explore the factors that affect the trace element transport in volcanic gases, such as 1) cooling of the gas from the exsolution temperature to the emission temperature at the surface, 2) pressure decrease from the depth of exsolution to atmospheric pressure, 3) composition of the gas and therefore ligand availability, 4) transport rate and its effect on mineral deposition from the gas.

How to cite: Mandon, C. and Stefansson, A.: Trace element transport processes in volcanic gases, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15216, https://doi.org/10.5194/egusphere-egu23-15216, 2023.

EGU23-15716 | Posters on site | GMPV8.5

Tephrochronology and geochemical correlation of Middle Pleistocene distal tephra deposits in Armenia 

Edmond Grigoryan, Khachatur Meliksetian, Hripsime Gevorgyan, Ivan Savov, Gevorg Navasardyan, Marina Bangoyan, and Tatevik Boyakhchyan

Widespread volcanism played significant role in geological history of Anatolian-Armenian-Iranian orogenic plateau formed as a result of continental collision of Arabian and Eurasia. Among diverse chemical compositions and eruption styles, reported for volcanoes of Armenian highlands, noteworthy are distal tephra fallout deposits and voluminous ignimbrite shields resulted from violent explosive volcanic eruptions with VEI estimations ranging form 4 to 6. Obviously, such eruptions had significant impact on climate, human occupation and migrations in the entire region and provide insights to volcanic hazards in the region.  One difficulty in the identifying and studying explosive eruptions during Pleistocene, is that many tephra fallout deposits are not preserved in the geologic records, since unconsolidated deposits erode rapidly, particularly in mountain topography. In Armenia, there is a sparse geologic record of tephra fallouts, except where these deposits are preserved beneath pyroclastic flows, which presumably occurred very soon after tephra deposition. Such tephra deposits, are known in Armenia in underlying ignimbrite units related to activity of Aragats stratovolcano (Gevorgyan et al., 2018), beneath Ani ignimbrite in western part of Armenia and activity of Irind and Pemzashen volcanoes. Alternatively, tephra deposits can be preserved if layers are rapidly covered by loess deposits or colluvium deposits or landslides shortly after the eruption and tephra deposition occurs. Such conditions are known for distal tephra fall deposits from Ararat volcano in Ararat depression and in NE Armenia near Ijevan. A big number of finds of  Paleolithic stone tools, and resent achievements in studying Paleolithic archeology in south Caucasus region provide evidences of early human occupation in the territory of south Caucasus.  This contribution  aims to fill gaps in our knowledge of distal tephra layers identified in Armenia, namely in  north-east, south and central parts of Armenia.  New data based on detailed geochemical investigations and 40Ar/39Ar age determinations of distal tephra layers originated from violent explosive eruptions, reported in this study, can contribute to establish chronostratigraphic horizons as marker layers for paleoclimate and archaeological records during Middle-Upper Pleistocene in the entire region. Tephra layers preserved in Pleistocene sedimentary sequences in Armenia provide important information about these violent explosive eruptions that are significant for the geological evolution and the human geography of the entire region.

How to cite: Grigoryan, E., Meliksetian, K., Gevorgyan, H., Savov, I., Navasardyan, G., Bangoyan, M., and Boyakhchyan, T.: Tephrochronology and geochemical correlation of Middle Pleistocene distal tephra deposits in Armenia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15716, https://doi.org/10.5194/egusphere-egu23-15716, 2023.

EGU23-7 | ECS | Orals | ST1.10

Modeling the 2020 November 29 solar energetic particle event using EUHFORIA and iPATH models 

Zheyi Ding, Nicolas Wijsen, Gang Li, and Stefaan Poedts

We present the implementation of a coupling between EUropean Heliospheric FORcasting Information Asset (EUHFORIA) and improved Particle Acceleration and Transport in the Heliosphere (iPATH) models. In this work, we simulate the widespread solar energetic particle (SEP) event of 2020 November 29 and compare the simulated time-intensity profiles with measurements at Parker Solar Probe (PSP), the Solar Terrestrial Relations Observatory (STEREO)-A, SOlar and Heliospheric Observatory (SOHO), and Solar Orbiter (SolO). We examined the temporal evolution of shock parameters and particle fluxes during this event and we find that adopting a realistic solar wind background can significantly impact the expansion of the shock and, consequently, the shock parameters. Time-intensity profiles with an energetic storm particle event at PSP are well reproduced from the simulations. In addition, the simulated and observed time-intensity profiles of protons show a similar two-phase enhancement at STA. These results illustrate that modeling a shock using a realistic solar wind is crucial in determining the characteristics of SEP events. The decay phase of the modeled time-intensity profiles at Earth is in good agreement with the observations, indicating the importance of perpendicular diffusion in widespread SEP events. Taking into account the possible large curved magnetic field line connecting to SolO, the modeled time-intensity profiles show a good agreement with the observation. We suggest that the broadly distorted magnetic field lines, which are due to a stream interaction region, may be a key factor in understanding the observed SEPs at SolO.

How to cite: Ding, Z., Wijsen, N., Li, G., and Poedts, S.: Modeling the 2020 November 29 solar energetic particle event using EUHFORIA and iPATH models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7, https://doi.org/10.5194/egusphere-egu23-7, 2023.

EGU23-1741 | ECS | Posters virtual | ST1.10

Energy Spectrum of Solar Energetic Electron Events Over 25 Years 

Wen Wang, Linghua Wang, Zixuan Liu, Samuel Krucker, and Robert F. Wimmer-Schweingruber

Solar Energetic electron (SEE) events are the most common solar particle acceleration phenomenon detected in situ in the interplanetary medium and the energy spectrum of SEE events carries crucial information on the acceleration and/or transport processes of SEEs. In our research, we investigate the peak flux energy spectrum of 458 SEE events with a clear velocity dispersion detected at energies from ≤ 4.2 keV to ≥ 108 keV by Wind/3DP from 1994 December through 2019 December, utilizing a pan-spectrum fitting method. According to the fitted spectral parameters, these 458 events are self-consistently classified into five spectral shapes: 304 DDPL events, 32 UDPL events, 23 SPL events, 44 ER events and 55 LP events. The DDPL events can be further divided in to two types: 231 EB≥20 keV DDPL events and 73 EB<20 keV DDPL events, since the distribution of break energy EB exhibits a primary peak around 60 keV and a secondary peak around 7 keV, separated by a dip at ~20 keV. The EB≥20 keV (EB<20 keV) DDPL events exhibit a power-law spectral index of 2.0+0.2-0.2(2.1+0.3-0.3) (values shown in a form of A+B-C means the median value with the first and the third quartiles) at energies below EB=5.6+2.3-2.4 keV (60+23-12 keV) and index of 3.3+0.5-0.3 (3.9+0.6-0.7) at energies above.The UDPL events have a spectral index of 3.0+0.3-0.3 at energies below EB=5.1+4.2-1.8 keV and index of 2.2+0.2-0.3 at energies above. The SPL events shows a spectral index of 2.8+0.5-0.2. The ER events exhibit a spectral index 1.9+0.3-0.3 at energies below Ec=30+19-10 keV. The six spectrum types also behave differently in the relationship between spectral parameters and in solar cycle variations. Furthermore, propagation effects in the IPM from the Sun to 1 AU appear to have no obvious influence on the spectral shape of most SEE events. These results suggest that the formation of SEE events can involve complex processes/sources.

How to cite: Wang, W., Wang, L., Liu, Z., Krucker, S., and Wimmer-Schweingruber, R. F.: Energy Spectrum of Solar Energetic Electron Events Over 25 Years, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1741, https://doi.org/10.5194/egusphere-egu23-1741, 2023.

EGU23-2518 | ECS | Orals | ST1.10

Solar activity relations in energetic electron events measured by the MESSENGER mission 

Laura Rodríguez-García, Laura Balmaceda, Raúl Gómez-Herrero, Athanasios Kouloumvakos, Nina Dresing, David Lario, Yannis Zouganelis, Annamaria Fedeli, Francisco Espinosa Lara, Ignacio Cernuda, George Ho, Robert Wimmer-Schweingruber, and Javier Rodríguez-Pacheco

We perform a statistical study of the relations between the properties of solar energetic electron (SEE) events measured by the MESSENGER mission from 2010 to 2015 and the parameters of the respective parent solar activity phenomena to identify the potential correlations between them. During the time of analysis MESSENGER heliocentric distance varied between 0.31 and 0.47 au.

The main conclusion of the study is as follows. For this particular sample of events, with a majority of SEE events being widespread in heliolongitude and displaying relativistic electron intensity enhancements, a shock-related acceleration mechanism might be relevant in the acceleration of near-relativistic electrons. This conclusion is mainly based on three results. (1) The high and significant correlation found between the SEE peak intensities and the shock speed. (2) The ∼4 orders of magnitude in the SEE peak intensities for the same CME-driven shock speed that might be related to the presence of supra-thermal seed population that made local shock acceleration more efficient. (3) The asymmetry to the east of the range of connection angles (CAs) for which the SEE events present higher peak intensities and higher correlations with the solar activity, which might be related to the evolution of the magnetic field connection to the shock front. We note that the CA is defined as the angular distance between the footpoint of the magnetic field connecting to the spacecraft and the longitude of the source region.

How to cite: Rodríguez-García, L., Balmaceda, L., Gómez-Herrero, R., Kouloumvakos, A., Dresing, N., Lario, D., Zouganelis, Y., Fedeli, A., Espinosa Lara, F., Cernuda, I., Ho, G., Wimmer-Schweingruber, R., and Rodríguez-Pacheco, J.: Solar activity relations in energetic electron events measured by the MESSENGER mission, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2518, https://doi.org/10.5194/egusphere-egu23-2518, 2023.

EGU23-4398 | ECS | Posters on site | ST1.10

Analysis of the Energetic Storm Particle events of 6-7 September 2017 

Federica Chiappetta, Monica Laurenza, Fabio Lepreti, Simone Benella, and Giuseppe Consolini

Most of the energetic particles observed in the heliosphere are accelerated from a few keV up to MeV by shock fronts which are associated with the transit of coronal mass ejections (CMEs). The study of energetic storm particle events (ESP) can be very helpful for the investigation of the acceleration processes of particles at the shocks. We considered two ESP events occurring 6-7 September, 2017. The data used to study kinetic energy spectra are proton flux enhancements provided by WIND and ACE spacecraft that are both at the Lagrangian point L1, close to 1 AU along the Sun-Earth direction. The energy ranges are from 70 keV to 70 MeV and from 40 keV to 4.8 MeV, respectively. In order to broaden the range of the analyzed energies, we combine these data with the proton fluxes from SoHO spacecraft, also located at L1, which detects particles with energies from 1.3 MeV to 130 MeV. We used the Weibull functional form, the double power law and the Ellison-Ramaty form to fit the observed spectra. The implications of the obtained results for particle acceleration are discussed, taking also into account the properties of the shocks and of the magnetic turbulence in their surroundings.

This research has been carried out in the framework of the CAESAR project, supported by the Italian Space Agency and the National Institute of Astrophysics through the ASI-INAF n. 2020-35-HH.0 agreement for the development of the ASPIS prototype of scientific data centre for Space Weather.”

How to cite: Chiappetta, F., Laurenza, M., Lepreti, F., Benella, S., and Consolini, G.: Analysis of the Energetic Storm Particle events of 6-7 September 2017, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4398, https://doi.org/10.5194/egusphere-egu23-4398, 2023.

Radiation is one of the most important risks to deep space exploration programs such as manned missions to the Moon and Mars. In preparation for such programs, it requires a thorough understanding of interplanetary space weather conditions and a timely forecast of their potential effects as a baseline for the development of mitigation strategies. 

 

Radiation damage in space comes mainly from two sources, Galactic Cosmic Rays (GCRs) and Solar Energetic Particles (SEPs). In particular, intense SEP events could result in very high doses in a short time period that may exceed the threshold to induce deterministic radiation effects and to result in severe damages to humans and equipment leading to the failure of the entire mission. SEP events with radiation hazards, despite of being rather infrequent and sporadic, are however very difficult to forecast and remain as a major challenge for space weather studies in preparation for future deep space and Mars missions.

 

Specifically speaking, the SEP radiation reaching an astronaut on a Mars may be completely different from of that detected at (or predicted for) Earth’s vicinity, including the SEP onset time, spectra evolution, radiation intensity etc. This is due to (1) the different location of Mars and connectivity to the acceleration source which allow it to have difference access to the SEP population, and (2) the different planetary environment which modifies the energy and composition of the particles due to the interactions of primary particles with the atmosphere/regolith and the generation of secondaries. The synergistic analysis and modeling of these two processes are particularly important to understand and eventually forecast SEPs and their radiation effects on Mars in preparation for mitigating their potential hazardous effects.  We also emphasize the utmost importance of utilizing multi-spacecraft particle measurements at Mars and also other heliospheric locations to better understand such extreme events and their radiation effects for future deep space explorers.

How to cite: Guo, J.: The Impact of Solar Energetic Particles at Mars’ radiation environment: A synergistic approach combining measurements and Modeling efforts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5292, https://doi.org/10.5194/egusphere-egu23-5292, 2023.

EGU23-7171 | Posters on site | ST1.10

Modelling of atmospheric transport of SEP-induced cosmogenic 10Be  using CCM SOCOL-AER2-BE 

Kseniia Golubenko, Eugene Rozanov, Gennady Kovaltsov, Mélanie Baroni, and Ilya Usoskin

10Be is a cosmogenic isotope continuously produced in the Earth’s atmosphere by galactic cosmic rays (GCRs) and sporadically by solar energetic particles (SEPs). The long-living isotope, as measured in polar ice cores, typically with an annual resolution, serves as a proxy for long-term cosmic-ray variability, whose signal can, however, be distorted by atmospheric transport and deposition that need to be properly modelled. Atmospheric transport of 10Be depends on production, atmospheric circulation, and local orography. For an accurate physical description of the isotope's transport and deposition, we use the chemical climate model (CCM) SOCOL-AER2-BE. In combination with the production model CRAC, our model was verified using real measurements of beryllium in ice cores for Antarctic and Greenland locations. The model results agree with the measurements at the absolute level, implying that the production, decay, and lateral deposition are correctly reproduced. However, the exact time variability is not always well reproduced, particularly for the Greenland shore sites implying significant regional effects. Potentially, extreme SPEs that are orders of magnitude stronger than those observed during the recent decades can be recorded in cosmogenic isotope data, and a proper model is needed to study them. Here we present a model of the production and transport of 10Be for a major solar energetic particle event (GLE 69) and analyze the geographical pattern of the beryllium concentration.

How to cite: Golubenko, K., Rozanov, E., Kovaltsov, G., Baroni, M., and Usoskin, I.: Modelling of atmospheric transport of SEP-induced cosmogenic 10Be  using CCM SOCOL-AER2-BE, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7171, https://doi.org/10.5194/egusphere-egu23-7171, 2023.

EGU23-7905 | ECS | Orals | ST1.10 | Highlight

Development of an In-Progress Forecasting Model to Forecast Radiation Dose Rates Once a Ground-Level Enchancement has Begun 

Chris Davis, Charlotte Waterfall, Fan Lei, Silvia Dalla, Keith Ryden, Ben Clewer, and Clive Dyer

During major solar energetic particle events, radiation dose rates in Earth's atmosphere at aviation altitudes can increase by orders of magnitude relative to dose rates during quiet times in events known as Ground-Level Enhancements (GLEs). In the case of events of a scale such that they occur once every few decades, radiation dose rates could become high enough that they pose a threat to aircraft crew and electronics. It is not currently possible to predict when such an event will occur, and existing software systems are only capable of nowcasting the current atmospheric radiation dose rates using real-time data sources. However, while it is not possible to forecast when a major event will occur, it may be possible to generate forecasts for radiation dose rates once an event has been registered to have begun. The ability to provide forecasts for dose rates once a GLE has started would be vital for airlines and for pilots in any future where aircraft might be rerouted to avoid regions of high radiation, as pilots need to be able to know not just their current radiation dose rates but radiation dose rates at possible locations where their plane might be in say half an hour's time. We report on the development of a software system to do this. This 'in-progress' radiation dose rate forecasting system will be developed by integrating the FOrecasting Relativistic particles during GLE Events (FORGE) system being developed at the University of Central Lancashire with an anisotropic extension to the Models for Atmospheric Ionising Radiation Effects+ (MAIRE+) system being developed at the University of Surrey. We report on the development of both of these systems and their integration.

How to cite: Davis, C., Waterfall, C., Lei, F., Dalla, S., Ryden, K., Clewer, B., and Dyer, C.: Development of an In-Progress Forecasting Model to Forecast Radiation Dose Rates Once a Ground-Level Enchancement has Begun, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7905, https://doi.org/10.5194/egusphere-egu23-7905, 2023.

EGU23-8936 | ECS | Orals | ST1.10

Particle Energisation in a 3D Collapsing Magnetic Trap Model With a Braking Jet  

Kate Mowbray and Thomas Neukirch

Investigating the motion of charged particles in time- and space-dependent electromagnetic fields is central to many areas of space and astrophysical plasmas. Here we present results of studying the energy changes of particle orbits that are trapped in inhomogeneous and time-dependent magnetic fields with rapidly shortening field lines. These so-called collapsing magnetic trap (CMT) models can be useful to better understand the particle energisation processes occurring below the reconnection region in a solar flare. Braking jets may be associated with magnetic reconnection, for example when a sunward flow slows down as it approaches a stronger region of magnetic field. We generalise a 2D CMT model with braking jet (Borissov et al., 2016) to three dimensions and investigate the dynamics of particles in this 3D CMT model. The resulting particle orbits show a sensitive dependence of particle energies on the initial conditions of orbits, with initial pitch angles playing a particularly important role. This sensitive dependence relates to the time evolution of trapping regions that develop in the braking jet region of the CMT, ensuring that some orbits spend a significant time in the loop legs of field lines, whilst others escape these regions for the duration of the simulation. These loop leg trapped particle orbits see significantly lower energy gains than those orbits that repeatedly pass the loop top, with some of these particles even losing energy. This gives us greater insight into the importance of the curvature of collapsing loop tops for the Fermi acceleration mechanism acting on the particles. 

 

Borissov A. et al., Solar Physics 291, Issue 5, 1385 

How to cite: Mowbray, K. and Neukirch, T.: Particle Energisation in a 3D Collapsing Magnetic Trap Model With a Braking Jet , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8936, https://doi.org/10.5194/egusphere-egu23-8936, 2023.

A joint analysis approach is used to study flare signatures both in the low and higher corona. STIX, AIA and LOFAR data provide an extensive picture about different aspects of flare characteristics. Recent data by the STIX instrument complement the picture of accelerated electrons, which propagate along magnetic field lines towards the Sun. These observations are linked to the LOFAR data, which contain information about the elctrons propagating away from the Sun through the corona above the active region. Although, the active region and its thermal evolution (Differential Emission Measure (DEM) reconstruction of AIA data), flare accelerated electrons and their radio traces (LOFAR, STIX) are in principal all associated with the energy release during the flare process, they are often studied seperatly. Hence, the investigation of possible relations is part of this project. Solar magnetic fields as a binding element between low and high corona, accelerated electrons and heated flare loops are included in the analysis via a Potential Field Source Surface (PFSS) model.

How to cite: Bröse, M. and Vocks, C.: Flare-accelerated electrons and their traces in the solar corona observed by space- and ground-based instruments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9582, https://doi.org/10.5194/egusphere-egu23-9582, 2023.

EGU23-10509 | ECS | Posters on site | ST1.10

Radial Variation of Suprathermal Particles Associated with Corotating Interaction Regions 

Robert Allen, George Ho, Glenn Mason, Athanasios Kouloumvakos, Robert Wimmer-Schweingruber, and Javier Rodríguez-Pacheco

The first three years of Solar Orbiter operations have enabled robust sampling of the intensity and composition of suprathermal particles within the inner heliosphere. This includes a multitude of observations of suprathermal ions associated with Corotating Interaction Regions (CIRs), with corresponding observations at 1 au with measurements from the Ultra-Low-Energy Isotope Spectrometer (ULEIS) on the Advanced Composition Explorer (ACE) mission and the Suprathermal Ion Telescope (SIT) on the Solar-Terrestrial Relations Observatory-Ahead (STEREO-A) spacecraft. Comparing observations between these spacecraft allows for a statistical view of the radial variations of CIR-associated suprathermal particles by composition in the inner heliosphere, allowing for greater insight into energetic particle transport within the inner heliosphere. This study expands on early results from Solar Orbiter and ACE to now encompass the first three years of Solar Orbiter operations, as well as include STEREO-A measurements. Comparisons to historical studies of CIR-associated energetic protons are also expanded in the survey of CIR-associated suprathermal particles from Solar Orbiter, ACE, and STEREO-A.

How to cite: Allen, R., Ho, G., Mason, G., Kouloumvakos, A., Wimmer-Schweingruber, R., and Rodríguez-Pacheco, J.: Radial Variation of Suprathermal Particles Associated with Corotating Interaction Regions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10509, https://doi.org/10.5194/egusphere-egu23-10509, 2023.

EGU23-11362 | ECS | Posters virtual | ST1.10

Solar Energetic Electron Events with a Spectral Bump 

Wenyan Li, Linghua Wang, and Wen Wang

The energy spectrum of solar energetic electron (SEE) events carries crucial information on the origin/acceleration of energetic electrons at the Sun. Using  the Wind 3DP electron measurements at ~1 to 200 keV during 1995-2019, we select 11 good SEE events with a bump-like break in the peak flux vs. energy spectrum, different from the typical SEE events with a double-power-law spectrum. For the selected 11 events, the background-subtracted electron peak flux versus energy spectrum fits well to two functions: the sum of a single-power-law and a Gaussian function (spectral function #1) and the product of a single-power-law and the natural exponential form of a Gaussian function (spectral function #2). For the spectral function #1 (#2), on average, the fitted spectral index is 2.6±0.4 (2.7±0.6), significantly larger than the low-energy power-law index of typical SEE events, while the fitted center energy of spectral bump is 24±7 keV (75±38 keV) and the ratio of bump width and center is 2.0±0.7 (3.4±2.8). Among these 11 events, respectively, ~78%, ~89%, ~90%, 100% and ~55% are associated with GOES SXR flares, RHESSI HXR flares, west-limb CMEs, type III radio bursts and type II  radio bursts. Thus, these bump events have a stronger association with flares, coronal mass ejections (CMEs) and type II radio bursts, compared to the typical SEE events. In addition, we find a positive correlation between the center energy of bump and the CME speed. Therefore, we come up with an acceleration picture of these bump SEE events: the power-law portion is probably accelerated by flares with the acceleration efficiency larger at lower energies, while the bump portion is likely accelerated in CME-related processes with the acceleration efficiency increasing with the CME speed.

How to cite: Li, W., Wang, L., and Wang, W.: Solar Energetic Electron Events with a Spectral Bump, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11362, https://doi.org/10.5194/egusphere-egu23-11362, 2023.

EGU23-12330 | ECS | Orals | ST1.10 | Highlight

When are energetic electrons producing NO directly in the upper stratosphere? 

Josephine Salice, Hilde Nesse, Noora Partamies, Emilia Kilpua, Andrew Kavanagh, Eldho Babu, and Christine Smith-Johnsen

Compositional NOx changes caused by energetic electron precipitation (EEP) at a specific altitude are called the EEP direct effect. Changes co-dependent on vertical transport are referred to as the EEP indirect effect. The relative importance of EEP’s direct and indirect effect on NO and its subsequent impact on ozone and dynamic changes remain unresolved. The challenges are partly due to inadequate particle measurement and the relative scarcity of NO observations over the polar MLT region. Moreover, lower production rates in the mesosphere make it challenging to determine EEP’s direct impact on NO since small in-situ enhancements cannot be easily distinguished from the descending NO-rich air masses in the winter hemisphere. In this study, the uncertainty of the EEP observations is bypassed by exclusively identifying events applying NO-observations from the SOFIE instrument on board the AIM satellite. SOFIE daily averaged data from 2007 to 2014 is used to create a climatology based on the mean of the lower half of the data (lower 50 percentile mean). A direct EEP-produced NO-event at 90 km (“90km-event”) is identified when the NO density surpasses the climatology by 100%. If the NO density exceeds 25% above the climatology at 80, 70, 60, and 50 km, the event qualifies as a “50km-event”. By contrasting the 90km and 50km events, the characteristics of the solar wind and geomagnetic indices, as well as observed electron fluxes from POES, are studied. The goal is to unravel when EEP can produce NO directly in the upper stratosphere. The result will contribute to developing a parameterization of EEP from the radiation belt that includes both the direct and indirect impact of EEP to decipher the total EEP effect on the ozone and atmospheric dynamics.

How to cite: Salice, J., Nesse, H., Partamies, N., Kilpua, E., Kavanagh, A., Babu, E., and Smith-Johnsen, C.: When are energetic electrons producing NO directly in the upper stratosphere?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12330, https://doi.org/10.5194/egusphere-egu23-12330, 2023.

EGU23-13801 | ECS | Posters virtual | ST1.10

Witnessing a Forbush Decrease with a Microscintillator Ionisation Detector over the Atlantic Ocean 

Justin Tabbett, Karen Aplin, and Susana Barbosa

A novel ionisation detector, previously deployed on meteorological radiosonde flights, has demonstrated responsivity to X-rays and gamma radiation, and additionally, is thought to be sensitive to ionising radiation from cosmic rays. The PiN detector, composed of a 1x1x0.8 cm3 CsI(Tl) microscintillator coupled to a PiN photodiode, was deployed on the NRP Sagres sailing vessel on a cruise in the Atlantic between Portugal and the Azores in 2021. The instrument can determine both the count rate and energy of incoming ionising radiation particles.

The instrument was operational during the voyage in November 2021 when a coronal mass ejection event induced a sudden decrease in the observed cosmic ray intensity, known as a Forbush decrease. We present data recorded by the ionisation detector during this period, to characterise the instrument’s ability to detect cosmic ray events, and we compare the performance with neutron monitoring stations Oulu in Finland, and Dourbes in Belgium. As the PiN detector provides spectral and count rate data, it is possible to group events by their energy, and investigate the count rates of specific energy regimes. This approach is useful as many sources – including high and low energy ionising radiation from cosmic rays – contribute to the background energy spectrum. As a result, more meaningful comparisons and relationships can be established with the neutron monitoring stations.

How to cite: Tabbett, J., Aplin, K., and Barbosa, S.: Witnessing a Forbush Decrease with a Microscintillator Ionisation Detector over the Atlantic Ocean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13801, https://doi.org/10.5194/egusphere-egu23-13801, 2023.

EGU23-14711 | Orals | ST1.10

Monitoring of Solar Energetic Particles and Cosmic Rays with the RADEM instrument onboard the ESA JUICE mission 

Wojtek Hajdas, Patricia Goncalves, Marco Pinto, Andre Galli, and Olivier Witasse

The main goal of the radiation monitor RADEM flying onboard the ESA JUICE mission is to provide continuous information on particle fluxes and their energy spectra. The monitor measures electrons up to 40 MeV and protons up to 250 MeV. Such a range of energies detected by RADEM enables covering the most hazardous regimes in terms of radiation damage. Spectroscopic information on particle energies is provided using eight quasi-logarithmic energy bins. RADEM has also a dedicated heavy-ion detector designed to measure a variety of heavy ion species with their LET between 0.1 and 10 MeV/cm/mg-1. Moreover, the monitor contains an additional detector sensitive to the direction of incoming radiation. It expands the instrument's angular coverage up to 35% of the sky. Apart from its spectroscopic and angular distribution functions, RADEM will continuously provide values of the radiation dose deposited by each particle species. Its telemetry data will be stored in the data center for the JUICE mission operated by the European Space Astronomy Centre. After preprocessing the higher-level data will become available to the JUICE scientific team. RADEM will be switched on shortly after the JUICE launch planned for April 2023 and after a short commissioning phase will start its nominal operation. Apart from regular and short tuning and calibration periods, it will remain operating for the rest of the mission i.e. almost 10 years. While its primary purpose is to monitor the mission levels for safety concerns of the spacecraft and its scientific payload, its measurements open a unique opportunity for conducting real-time, continuous observations during its full cruise to Jupiter. RADEM will study all aspects of the radiation phenomena characteristic to the Earth and Solar System. Correlations with other instruments will allow for advanced observations of particle event propagation and a better understanding of processes related to the dynamics of particle environments including their links with solar activity and magnetic fields across the solar system. In particular, during its first two years of the cruise to Jupiter, RADEM will precisely map the radiation environment between Venus and Mars, providing uninterrupted time-resolved spectroscopy and dosimetry data from Solar Energetic Particles and Cosmic Rays.

How to cite: Hajdas, W., Goncalves, P., Pinto, M., Galli, A., and Witasse, O.: Monitoring of Solar Energetic Particles and Cosmic Rays with the RADEM instrument onboard the ESA JUICE mission, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14711, https://doi.org/10.5194/egusphere-egu23-14711, 2023.

EGU23-15517 | Posters on site | ST1.10

Proton energy spectra of energetic storm particle events and their relation with magnetic turbulence and intermittency nearby interplanetary shocks 

Fabio Lepreti, Federica Chiappetta, Monica Laurenza, Simone Benella, and Giuseppe Consolini

Shock waves propagating in the interplanetary space are efficient sources of energetic particles. In situ spacecraft observations, especially particle fluxes which can be used to obtain energy spectra, provide very useful data for the investigation of the acceleration mechanisms occurring at shocks. In this work we analyse the kinetic energy spectra of several proton flux enhancements associated with energetic storm particle (ESP) events observed by various spacecraft. ESP events occurring both in association with and in absence of Solar Energetic Particles (SEPs) are considered. Moreover, ESP events associated both with quasi-perpendicular and quasi parallel shocks are investigated.  Different functional forms (i.e. Weibull function, double power law, and Ellison-Ramaty) are used to fit the observed spectra and the obtained results are discussed in relation to the shock properties and to the magnetic turbulence and intermittency in the upstream and downstream regions. More specifically, the properties of magnetic turbulence and intermittency are analysed by calculating power spectral densities and structure functions of the fluctuations of the magnetic field components and the implications for particle acceleration are examined.

This research has been carried out in the framework of the CAESAR project, supported by the Italian Space Agency and the National Institute of Astrophysics through the ASI-INAF n. 2020-35-HH.0 agreement for the development of the ASPIS prototype of scientific data centre for Space Weather.

How to cite: Lepreti, F., Chiappetta, F., Laurenza, M., Benella, S., and Consolini, G.: Proton energy spectra of energetic storm particle events and their relation with magnetic turbulence and intermittency nearby interplanetary shocks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15517, https://doi.org/10.5194/egusphere-egu23-15517, 2023.

EGU23-15621 | ECS | Posters on site | ST1.10

The effect of magnetic reconnection on ICME-related GCR modulation 

Emma Davies, Camilla Scolini, Réka Winslow, and Andrew Jordan

The large-scale magnetic structure of interplanetary coronal mass ejections (ICMEs) has been shown to cause temporary decreases in the galactic cosmic ray (GCR) flux measured in situ by spacecraft, known as Forbush decreases (Fds). In some ICMEs, the magnetic ejecta exhibits a magnetic flux rope structure; the strong magnetic field strength and closed field line geometry of such ICME magnetic flux ropes has been proposed to act as a shield to GCR transport. However, as ICMEs propagate, they undergo many processes including interactions and magnetic reconnection with the interplanetary magnetic field (IMF) in large-scale solar wind structures and other solar transients. In this study, we investigate how ICME interaction and reconnection during propagation affects Fd size, shape, and duration. We hypothesize that the alteration of the ICME magnetic topology due to reconnection (specifically the opening of the closed magnetic field configuration in the ICME flux rope) will have a strong effect on the ICME’s ability to modulate GCRs. To test this hypothesis, we compare the Fds of ICMEs that likely underwent reconnection during propagation with ones that likely did not.

To this end, we identify ICMEs that exhibited open magnetic field line topologies (i.e., ones that likely underwent reconnection) and we compare their effects on GCRs with those of ICMEs that exhibited closed topologies (both ends connected to the Sun). We use magnetic field, solar wind plasma, and suprathermal electron pitch angle distribution data at ACE and Wind to select the ICMEs. Furthermore, we use data by the SOPO and McMurdo neutron monitors at Earth to investigate how the magnetic structure of the ICME ejecta modulates the GCRs by comparing the resulting Fds for the selected ICMEs. The results of our study yield new insights into how the modulation of GCRs is affected by ICME evolution and interaction during propagation and whether reconnection of the ICME flux rope weakens its modulation of GCRs.

How to cite: Davies, E., Scolini, C., Winslow, R., and Jordan, A.: The effect of magnetic reconnection on ICME-related GCR modulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15621, https://doi.org/10.5194/egusphere-egu23-15621, 2023.

EGU23-16136 | Posters on site | ST1.10

Energetic Electron Precipitation during Slot Region Filling Events 

Hilde Nesse, Eldho Midhun Babu, Josephine Salice, and Bernd Funke

The region separating the inner and outer radiation belt, typically devoid of energetic electrons, is termed the slot region. The outer edge of the slot region marks the equatorward edge of the energetic electron precipitation (EEP) originating from the outer radiation belt. Its varying location is strongly linked to the plasmasphere and geomagnetic activity. As such, geomagnetic indices are used to estimate the equatorward extent of the EEP region. There are, however, numerous reports where the energetic electrons cross these boundaries and fill the slot region, during which energetic electrons that can precipitate into the atmosphere long after the geomagnetic activity subsides. This is a missing source of energy input in current EEP estimates based on geomagnetic indices.

This study explores the occurrence rate, reformation, local time dependence, and energy deposition of slot region filling events. Medium energy electron measurements from the NOAA/POES over a full solar cycle from 2004 to 2014 are applied. We combine observations from the MEPED 0° and 90° detectors together with theory of pitch angle diffusion by wave-particle interaction to estimate the precipitating fluxes. To explore the energy dependent characteristics, each of the MEPED energy channels, > 43, >114, and >292 keV are evaluated independently. Finally, we investigate the potential EEP impact on the NO density utilizing seven years of Envisat MIPAS NO observations from 2005 to 2011.

How to cite: Nesse, H., Babu, E. M., Salice, J., and Funke, B.: Energetic Electron Precipitation during Slot Region Filling Events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16136, https://doi.org/10.5194/egusphere-egu23-16136, 2023.

EGU23-16177 | Orals | ST1.10 | Highlight

Risks of space radiation exposure to exploration astronauts: limitations in predictions based on the ground experiments and possible solutions 

Salman Khaksarighiri, Robert Wimmer-Schweingruber, Jingnan Guo, Cary Zeitlin, Thomas Berger, and Daniel Matthiä

Future expeditions into interplanetary space, and in particular to the Moon and Mars, will expose astronauts to very high levels of cosmic radiation, which are known due to years of research and instruments that have been sent to space. It is, however, a limitation in understanding the risks of this radiation for the human body due to difficulties in simulating the complex space environment on Earth or complex human phantom and the inability to extrapolate human clinical outcomes based on animal models or simulation results. 
As human spaceflight continues on its path to success, we need to develop appropriate and effective mitigation strategies for future missions to improve our understanding of the space radiation risk by identifying the constraints of radiation research on the Earth and finding possible solutions based on the existing technologies to be closer to the reality as much as possible and better understand human physiology in space.  
As part of this paper, we have identified several factors that hinder our understanding of radiation risks for human crews and have identified ways to cope with these restrictions for a better understanding and preparation for human spaceflights in the future.

How to cite: Khaksarighiri, S., Wimmer-Schweingruber, R., Guo, J., Zeitlin, C., Berger, T., and Matthiä, D.: Risks of space radiation exposure to exploration astronauts: limitations in predictions based on the ground experiments and possible solutions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16177, https://doi.org/10.5194/egusphere-egu23-16177, 2023.

AS5 – Methods and Techniques

Large-scale climate variability is analysed, modelled, and predicted mainly based on general circulation models and low-dimensional association analysis. The models’ equational basis makes it difficult to produce mathematical analysis results and clear interpretations, whereas the association analysis cannot establish causation sufficiently to make invariant predictions. However, the macroscale causal structures of the climate system may accomplish the tasks of analysis, modelling, and prediction according to the concepts of causal emergence and causal prediction’s invariance.

Under the assumptions of no unobserved confounders and linear Gaussian models, we examine whether the macroscale causal structures of the climate system can be inferred not only to model but also to predict the large-scale climate variability. Specifically, first, we obtain the causal structures of the macroscale air-sea interactions of El Niño–Southern Oscillation (ENSO), which are interpretable in terms of physics. The structural causal models constructed accordingly can model the ENSO diversity realistically and predict the ENSO variability. Second, this study identifies the joint effect of ENSO and three other winter climate phenomena on the interannual variability in the East Asian summer monsoon. Using regression, these causal precursors can predict the monsoon one season ahead, outperforming association-based empirical models and several climate models. Third, we introduce a framework that infers ENSO’s air-sea interactions from high-dimensional data sets. The framework is based on aggregating the causal discovery results of bootstrap samples to improve high-dimensional variable selection. It is also based on spatial-dimension reduction to allow of clear interpretations at the macroscale.

While further integration with nonlinear non-Gaussian models will be necessary to establish the full benefits of inferring causal structures as a standard practice in research and operational predictions, our study may offer a route to providing concise explanations of the climate system and reaching accurate invariant predictions.

How to cite: He, S., Yang, S., and Chen, D.: Inferring Causal Structures to Model and Predict ENSO and Its Effect on Asian Summer Monsoon, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-102, https://doi.org/10.5194/egusphere-egu23-102, 2023.

EGU23-239 | ECS | Orals | ITS1.14/CL5.8

Toward a hybrid tropical cyclone global model 

Roberto Ingrosso and Mathieu Boudreault

The future evolution of tropical cyclones (TCs) in a warming world is an important issue, considering their potential socio-economic impacts on the areas hit by these phenomena. Previous studies provide robust responses about the future increase in intensity and in the global proportion of major TCs (Category 4–5). On the other hand, high uncertainty is associated to a projected future decrease in global TCs frequency and to potential changes in TC tracks and translation speed.

Risk management and regulatory actions require more robust quantification in how the climate change affects TCs dynamics.  A probabilistic hybrid TC model based upon statistical and climate models, physically coherent with TCs dynamics, is being built to investigate the potential impacts of climate change. Here, we provide preliminary results, in terms of present climate reconstruction (1980-2021) and future projections (2022-2060) of cyclogenesis locations and TC tracks, based on different statistical models, such as logistic and multiple linear regressions and random forest.  Physical predictors associated with the TC formation and motion and produced by reanalysis (ERA5) and the Community Earth System Model (CESM) ensemble are considered in this study.

 

How to cite: Ingrosso, R. and Boudreault, M.: Toward a hybrid tropical cyclone global model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-239, https://doi.org/10.5194/egusphere-egu23-239, 2023.

EGU23-492 | ECS | Posters on site | ITS1.14/CL5.8

Separation of climate models and observations based on daily output using two machine learning classifiers 

Lukas Brunner, Sebastian Sippel, and Aiko Voigt

Climate models are primary tools to investigate processes in the climate system, to project future changes, and to inform decision makers. The latest generation of models provides increasingly complex and realistic representations of the real climate system while there is also growing awareness that not all models produce equally plausible or independent simulations. Therefore, many recent studies have investigated how models differ from observed climate and how model dependence affects model output similarity, typically drawing on climatological averages over several decades.

Here, we show that temperature maps from individual days from climate models from the CMIP6 archive can be robustly identified as “observation” or “model” even after removing the global mean. An important exception is a prototype high-resolution simulation from the ICON model family that can not be so  unambiguously classified into one category. These results highlight that persistent differences between observed and simulated climate emerge at very short time scales already, but very high resolution modelling efforts may be able to overcome some of these shortcomings.

We use two different machine learning classifiers: (1) logistic regression, which allows easy insights into the learned coefficients but has the limitation of being a linear method and (2) a convolutional neural network (CNN) which represents rather the other end of the complexity spectrum, allowing to learn nonlinear spatial relations between features but lacking the easy interpretability logistic regression allows. For CMIP6 both methods perform comparably, while the CNN is also able to recognize about 75% of samples from ICON as coming from a model, while linear regression does not have any skill for this case.

Overall, we demonstrate that the use of machine learning classifiers, once trained, can overcome the need for multiple decades of data to investigate a given model. This opens up novel avenues to test model performance on much shorter times scales.

How to cite: Brunner, L., Sippel, S., and Voigt, A.: Separation of climate models and observations based on daily output using two machine learning classifiers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-492, https://doi.org/10.5194/egusphere-egu23-492, 2023.

EGU23-753 | ECS | Orals | ITS1.14/CL5.8 | Highlight

Finding regions of similar sea level variability with the help of a Gaussian Mixture Model 

Lea Poropat, Céline Heuzé, and Heather Reese

In climate research we often want to focus on a specific region and the most prominent processes affecting it, but how exactly do we select the borders of that region? We also often need to use long-term in situ observations to represent a larger area, but which area exactly are they representative for? In ocean sciences we usually consider basins as separate regions or even simpler, just select a rectangle of the ocean, but that does not always correspond to the real, physically relevant borders. As alternative, we use an unsupervised classification model, Gaussian Mixture Model (GMM), to separate the northwestern European seas into regions based on the sea level variability observed by altimetry satellites.

After performing a principal component (PC) analysis on the 24 years of monthly sea level data, we use the stacked PC maps as input for the GMM. We used the Bayesian Information Criterion to determine into how many regions our area should be split because GMM requires the number of classes to be selected a priori. Depending on the number of PCs used, the optimal number of classes was between 12 and 18, more PCs typically allowing the separation into more regions. Due to the complexity of the data and the dependence of the results on the starting randomly chosen weights, the classification can differ to a degree with every new run of the model, even if we use the exact same data and parameters. To tackle that, instead of using one model, we use an ensemble of models and then determine which class does each grid point belong to by soft voting, i.e., each of the models provides a probability that the point belongs to a particular class and the class with the maximal sum of probabilities wins. As a result, we obtain both the classification and the likelihood of the model belonging to that class.

Despite not using the coordinates of the data points in the model at all, the obtained classes are clearly location dependent, with grid points belonging to the same class always being close to each other. While many classes are defined by bathymetry changes, e.g., the continental shelf break and slope, sometimes other factors come into play, such as for the split of the Norwegian coast into two classes or for the division in the Barents Sea, which is probably based on the circulation. The North Sea is also split into three distinct regions, possibly based on sea level changes caused by dominant wind patterns.

This method can be applied to almost any atmospheric or oceanic variable and used for larger or smaller areas. It is quick and practical, allowing us to delimit the area based on the information we cannot always clearly see from the data, which can facilitate better selection of the regions that need further research.

How to cite: Poropat, L., Heuzé, C., and Reese, H.: Finding regions of similar sea level variability with the help of a Gaussian Mixture Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-753, https://doi.org/10.5194/egusphere-egu23-753, 2023.

EGU23-849 | ECS | Orals | ITS1.14/CL5.8

Drivers of sea level variability using neural networks 

Linn Carlstedt, Lea Poropat, and Céline Heuzé

Understanding the forcing of regional sea level variability is crucial as many people all over the world live along the coasts and are endangered by the sea level rise. The adding of fresh water into the oceans due to melting of the Earth’s land ice together with thermosteric changes has led to a rise of the global mean sea level (GMSL) with an accelerating rate during the twentieth century, and has now reached a mean rate of 3.7 mm per year according to IPCCs latest report. However, this change varies spatially and the dynamics behind what forces sea level variability on a regional to local scale is still less known, thus making it hard for decision makers to mitigate and adapt with appropriate strategies.

Here we present a novel approach using machine learning (ML) to identify the dynamics and determine the most prominent drivers forcing coastal sea level variability. We use a recurrent neural network called Long Short-Term Memory (LSTM) with the advantage of learning data in sequences and thus capable of storing some memory from previous timesteps, which is beneficial when dealing with time series. To train the model we use hourly ERA5 10-m wind, mean sea level pressure (MSLP), sea surface temperature (SST), evaporation and  precipitation data between 2009-2017 in the North Sea region. To reduce the dimensionality of the data but still preserve maximal information we conduct principal component analysis (PCA) after removing the climatology which are calculated by hourly means over the years. Depending on the explained variance of the PCs for each driver, 2-4 PCs are chosen and cross-correlated to eliminate collinearity, which could affect the model results. Before being used in the ML model the final preprocessed data are normalized by min-max scaling to optimize the learning. The target data in the model are hourly in-situ sea level observations from West-Terschelling in the Netherlands. Using in-situ observations compared to altimeter data enhances the ability of making good predictions in coastal zones as altimeter data has a tendency to degrade along the coasts. The sea level time series is preprocessed by tidal removal and de-seasoned by subtracting the hourly means. To determine which drivers are most prominent for the sea surface variability in our location, we mute one driver at a time in the training of the network and evaluate the eventual improvement or deterioration of the predictions.

Our results show that the zonal wind is the most prominent forcing of sea level variability in our location, followed by meridional wind and MSLP. While the SST greatly affects the GMSL, SST seems to have little to no effect on local sea level variability compared to other drivers. This approach shows great potential and can easily be applied to any coastal zone and is thus very useful for a broad body of decision makers all over the world. Identifying the cause of local sea level variability will also enable the ability of producing better models for future predictions, which is of great importance and interest.

How to cite: Carlstedt, L., Poropat, L., and Heuzé, C.: Drivers of sea level variability using neural networks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-849, https://doi.org/10.5194/egusphere-egu23-849, 2023.

EGU23-984 | ECS | Orals | ITS1.14/CL5.8

Data-driven Attributing of Climate Events with Climate Index Collection based on Model Data (CICMoD) 

Marco Landt-Hayen, Willi Rath, Sebastian Wahl, Nils Niebaum, Martin Claus, and Peer Kröger

Machine learning (ML) and in particular artificial neural networks (ANNs) push state-of-the-art solutions for many hard problems e.g., image classification, speech recognition or time series forecasting. In the domain of climate science, ANNs have good prospects to identify causally linked modes of climate variability as key to understand the climate system and to improve the predictive skills of forecast systems. To attribute climate events in a data-driven way with ANNs, we need sufficient training data, which is often limited for real world measurements. The data science community provides standard data sets for many applications. As a new data set, we introduce a collection of climate indices typically used to describe Earth System dynamics. This collection is consistent and comprehensive as we use control simulations from Earth System Models (ESMs) over 1,000 years to derive climate indices. The data set is provided as an open-source framework that can be extended and customized to individual needs. It allows to develop new ML methodologies and to compare results to existing methods and models as benchmark. Exemplary, we use the data set to predict rainfall in the African Sahel region and El Niño Southern Oscillation with various ML models. We argue that this new data set allows to thoroughly explore techniques from the domain of explainable artificial intelligence to have trustworthy models, that are accepted by domain scientists. Our aim is to build a bridge between the data science community and researchers and practitioners from the domain of climate science to jointly improve our understanding of the climate system.

How to cite: Landt-Hayen, M., Rath, W., Wahl, S., Niebaum, N., Claus, M., and Kröger, P.: Data-driven Attributing of Climate Events with Climate Index Collection based on Model Data (CICMoD), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-984, https://doi.org/10.5194/egusphere-egu23-984, 2023.

EGU23-1135 | ECS | Posters on site | ITS1.14/CL5.8

Curation of High-level Molecular Atmospheric Data for Machine Learning Purposes 

Vitus Besel, Milica Todorović, Theo Kurtén, Patrick Rinke, and Hanna Vehkamäki

As cloud and aerosol interactions remain large uncertainties in current climate models (IPCC) they are of special interest for atmospheric science. It is estimated that more than 70% of all cloud condensation nuclei origin from so-called New Particle Formation, which is the process of gaseous precursors clustering together in the atmosphere and subsequent growth into particles and aerosols. After initial clustering this growth is driven strongly by condensation of low volatile organic compounds (LVOC), that is molecules with saturation vapor pressures (pSat) below 10-6 mbar [1]. These origin from organic molecules emitted by vegetation that are subsequently rapidly oxidized in the air, so-called Biogenic LVOC (BLVOC).

We have created a big data set of BLVOC using high-throughput computing and Density Functional Theory (DFT), and use it to train Machine Learning models to predict pSat of previously unseen BLVOC. Figure 1 illustrates some sample molecules form the data.

Figure 1: Sample molecules, for small, medium large sizes.     Figure 2: Histogram of the calculated saturation vapor pressures.

Initially the chemical mechanism GECKO-A provides possible BLVOC molecules in the form of SMILES strings. In a first step the COSMOconf program finds and optimizes structures of possible conformers and provides their energies for the liquid phase on a DFT level of theory. After an additional calculation of the gas phase energies with Turbomole, COSMOtherm calculates thermodynamical properties, such as the pSat, using the COSMO-RS [1] model. We compressed all these computations together in a highly parallelised high-throughput workflow to calculate 32k BLVOC, that include over 7 Mio. molecular conformers. See a histogram of the calculated pSat in Figure 2.

We use the calculated pSat to train a Gaussian Process Regression (GPR) machine learning model with the Topological Fingerprint as descriptor for molecular structures. The GPR incorporates noise and outputs uncertainties for predictions on the pSat. These uncertainties and data cluster techniques allow for the active choosing of molecules to include in the training data, so-called Active Learning. Further, we explore using SLISEMAP [2] explainable AI methods to correlate Machine Learning predictions, the high-dimensional descriptors and human-readable properties, such as functional groups.

[1] Metzger, A. et al. Evidence for the role of organics in aerosol particle formation under atmospheric conditions. Proc. Natl. Acad. Sci. 107, 6646–6651, 10.1073/pnas.0911330107 (2010)
[2] Klamt, A. & Schüürmann, G. Cosmo: a new approach to dielectric screening in solvents with explicit expressions for the
screening energy and its gradient. J. Chem. Soc., Perkin Trans. 2 799–805, 10.1039/P29930000799 (1993).
[3] Björklund, A., Mäkelä, J. & Puolamäki, K. SLISEMAP: supervised dimensionality reduction through local explanations. Mach Learn (2022). https://doi.org/10.1007/s10994-022-06261-1

How to cite: Besel, V., Todorović, M., Kurtén, T., Rinke, P., and Vehkamäki, H.: Curation of High-level Molecular Atmospheric Data for Machine Learning Purposes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1135, https://doi.org/10.5194/egusphere-egu23-1135, 2023.

EGU23-1244 | Posters on site | ITS1.14/CL5.8

Machine learning for non-orographic gravity waves in a climate model 

Steven Hardiman, Adam Scaife, Annelize van Niekerk, Rachel Prudden, Aled Owen, Samantha Adams, Tom Dunstan, Nick Dunstone, and Melissa Seabrook

There is growing use of machine learning algorithms to replicate sub-grid parametrisation schemes in global climate models.  Parametrisations rely on approximations, thus there is potential for machine learning to aid improvements.  In this study, a neural network is used to mimic the behaviour of the non-orographic gravity wave scheme used in the Met Office climate model, important for stratospheric climate and variability.  The neural network is found to require only two of the six inputs used by the parametrisation scheme, suggesting the potential for greater efficiency in this scheme.  Use of a one-dimensional mechanistic model is advocated, allowing neural network hyperparameters to be trained based on emergent features of the coupled system with minimal computational cost, and providing a test bed prior to coupling to a climate model.  A climate model simulation, using the neural network in place of the existing parametrisation scheme, is found to accurately generate a quasi-biennial oscillation of the tropical stratospheric winds, and correctly simulate the non-orographic gravity wave variability associated with the El Nino Southern Oscillation and stratospheric polar vortex variability.  These internal sources of variability are essential for providing seasonal forecast skill, and the gravity wave forcing associated with them is reproduced without explicit training for these patterns.

How to cite: Hardiman, S., Scaife, A., van Niekerk, A., Prudden, R., Owen, A., Adams, S., Dunstan, T., Dunstone, N., and Seabrook, M.: Machine learning for non-orographic gravity waves in a climate model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1244, https://doi.org/10.5194/egusphere-egu23-1244, 2023.

EGU23-1502 | ECS | Orals | ITS1.14/CL5.8

Adapting Transfer Learning for Multiple Channels in Satellite Data Applications 

Naomi Simumba and Michiaki Tatsubori

Transfer learning is a technique wherein information learned by previously trained models is applied to new learning tasks. Typically, weights learned by a network pretrained on other datasets are copied or transferred to new networks. These new networks, or downstream models, are then are then used for assorted tasks. Foundation models extend this concept by training models on large datasets. Such models gain a contextual understanding which can then be used to improve performance of downstream tasks in different domains. Common examples include GPT-3 in the field on natural language processing and ImageNet trained models in the field of computer vision.

Beyond its high rate of data collection, satellite data also has a wide range of meaningful applications including climate impact modelling and sustainable energy. This makes foundation models trained on satellite data very beneficial as they would reduce the time, data, and computational resources required to obtain useful downstream models for these applications.

However, satellite data models differ from typical computer vision models in a crucial way. Because several types of satellite data exist, each with its own benefits, a typical use case for satellite data involves combining multiple data inputs in configurations that are not readily apparent during pretraining of the foundation model. Essentially, this means that the downstream application may have a different number of input channels from the pretrained model, which raises the question of how to successfully transfer information learned by the pretrained model to the downstream application.

This research proposes and examines several architectures for the downstream model that allow for pretrained weights to be incorporated when a different number of input channels is required. For evaluation, models pretrained with self-supervised learning on precipitation data are applied to a downstream model which conducts temporal interpolation of precipitation data and requires two inputs. The effect of including perceptual loss to enhance model performance is also evaluated. These findings can be used to guide adaptation for applications ranging from flood modeling, land use detection, and more.

How to cite: Simumba, N. and Tatsubori, M.: Adapting Transfer Learning for Multiple Channels in Satellite Data Applications, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1502, https://doi.org/10.5194/egusphere-egu23-1502, 2023.

Unprecedented flash floods (FF) in urban regions are increasing due to heavy rainfall intensity and magnitude as a result of human-induced climate and land-use changes. The changes in weather patterns and various anthropogenic activities increase the complexity of modelling the FF at different spatiotemporal scales: which indicates the importance of multi-resolution forcing information. Towards this, developing new methods for processing coarser resolution spatio-temporal datasets are essential for the efficient modelling of FF. While a wide range of methods is available for spatial and temporal downscaling of the climate data, the multi-temporal downscaling strategy has not been investigated for ungauged stations of streamflow. The current study proposed a multi-temporal downscaling (MTD) methodology for gauged and ungauged stations using Adaptive Emulator Modelling concepts for daily to sub-daily streamflows. The proposed MTD framework for ungauged stations comprise a hybrid framework with conceptual and machine learning-based approaches to analyze the catchment behavior and downscale the model outputs from daily to sub-daily scales. The study area, Peachtree Creek watershed (USA), frequently experiences flash floods; hence, selected to validate the proposed framework. Further, the study addresses the critical issues of model development, seasonality, and diurnal variation of MTD data. The study obtained MTD data with minimal uncertainty on capturing the hydrological signatures and nearly 95% of accuracy in predicting the flow attributes over ungauged stations. The proposed framework can be highly useful for short- and long-range planning, management, and mitigation measurements, where the absence of fine resolution data prohibits flash flood modeling.

How to cite: Budamala, V., Wadhwa, A., and Bhowmik, R. D.: Multi-Temporal Downscaling of Streamflow for Ungauged Stations/ Sub-Basins from Daily to Sub-Daily Interval Using Hybrid Framework – A Case Study on Flash Flood Watershed, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1855, https://doi.org/10.5194/egusphere-egu23-1855, 2023.

EGU23-2289 | ECS | Posters on site | ITS1.14/CL5.8

Towards understanding the effect of parametric aerosol uncertainty on climate using a chemical transport model perturbed parameter ensemble. 

Meryem Bouchahmoud, Tommi Bergman, and Christina Williamson

Aerosols in the climate system have a direct link to the Earth’s energy balance. Aerosols interact directly with the solar radiation through scattering and absorption; and indirectly by changing cloud properties. The effect aerosols have on climate is one of the major causes of radiative forcing (RF) uncertainty in global climate model simulations. Thus, reducing aerosol RF uncertainty is key to improving climate prediction. The objective of this work is to understand the magnitude and causes of aerosol uncertainty in the chemical transport model TM5.

Perturbed Parameter Ensembles (PPEs) are a set of model runs created by perturbing an ensemble of parameters. Parameters are model inputs, for this study we focus on parameters describing aerosol emissions, properties and processes, such as dry deposition, aging rate, emissions to aerosols microphysics. PPEs vary theses parameters over their uncertainty range all at once to study their combine effect on TM5.

Varying these parameters along with others through their value range, will reflect on TM5 outputs. The TM5 outputs parameters we are using in our sensitivity study are the cloud droplet number concentration and the ambient aerosol absorption optical thickness at 550nm.

Here we discuss the design of the PPE, and one-at-a-time sensitivity studies used in this process. The PPE samples the parameter space to enable us to use emulation. Emulating is a machine learning technique that uses a statistical surrogate model to replace the chemical transport model. The aim is to provide output data with more dense sampling throughout the parameter space. We will be using a Gaussian process emulator, which has been shown to be an efficient technique for quantifying parameter sensitivity in complex global atmospheric models.

We also describe plans to extend this work to emulate an aerosol PPE for EC-Earth. The PPE for EC-Earth will also contain cloud parameters that will vary over their uncertainty range together with the aerosol parameters to examine the influence of aerosol parametric uncertainty on RF.

 

How to cite: Bouchahmoud, M., Bergman, T., and Williamson, C.: Towards understanding the effect of parametric aerosol uncertainty on climate using a chemical transport model perturbed parameter ensemble., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2289, https://doi.org/10.5194/egusphere-egu23-2289, 2023.

EGU23-2541 | ECS | Posters on site | ITS1.14/CL5.8

Machine learning based automated parameter tuning of ICON-A using satellite data 

Pauline Bonnet, Fernando Iglesias-Suarez, Pierre Gentine, Marco Giorgetta, and Veronika Eyring

Global climate models use parameterizations to represent the effect of subgrid scale processes on the resolved state. Parameterizations in the atmosphere component usually include radiation, convection, cloud microphysics, cloud cover, gravity wave drag, vertical turbulence in the boundary layer and other processes. Parameterizations are semi-empirical functions that include a number of tunable parameters. Because these parameters are loosely constraint with experimental data, a range of values are typically explored by evaluating model runs against observations and/or high resolution runs. Fine tuning a climate model is a complex inverse problem due to the number of tunable parameters and observed climate properties to fit. Moreover, parameterizations are sources of uncertainties for climate projections, thus fine tuning is a crucial step in model development.

Traditionally, tuning is a time-consuming task done manually, by iteratively updating the values of the parameters in order to investigate the parameter space with user-experience driven choices. To overcome such limitation and search efficiently through the parameter space one can implement automatic techniques. Typical steps in automatic tuning are: (i) constraining the scope of the study (model, simulation setup, parameters, metrics to fit and corresponding reference values); (ii) conducting a sensitivity analysis to reduce the parameter space and/or building an emulator for the climate model; and (iii) conducting a sophisticated grid search to define the optimum parameter set or its distribution (e.g., rejection sampling and history matching). The ICOsahedral Non-hydrostatic (ICON) model is a modelling framework for numerical weather prediction and climate projections. We implement a ML-based automatic tuning technic to tune a recent version of ICON-A with a spatial resolution typically used for climate projections. We evaluate the tuned ICON-A model against satellite observations using the Earth System Model Evaluation Tool (ESMValTool). Although automatic tuning technics allow to reach the optimum parameter values in less steps than with the manual tuning, they still require some experience-driven choices throughout the tuning process. Moreover, the performances of the tuned model is limited by the structural errors of the model, inherent to the mathematical description of the parameterizations included in the model.

How to cite: Bonnet, P., Iglesias-Suarez, F., Gentine, P., Giorgetta, M., and Eyring, V.: Machine learning based automated parameter tuning of ICON-A using satellite data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2541, https://doi.org/10.5194/egusphere-egu23-2541, 2023.

EGU23-3404 | ECS | Posters on site | ITS1.14/CL5.8 | Highlight

Deep learning-based generation of 3D cloud structures from geostationary satellite data 

Sarah Brüning, Stefan Niebler, and Holger Tost

Clouds and their interdependent feedback mechanisms remain a source of insecurity in climate science. This said, overcoming relating obstacles especially in the context of a changing climate emphasizes the need for a reliable database today more than ever. While passive remote sensing sensors provide continuous observations of the cloud top, they lack vital information on subjacent levels. Here, active instruments can deliver valuable insights to fill this gap in knowledge.

This study sets on to combine the benefits of both instrument types. It aims (1) to reconstruct the vertical distribution of volumetric radar data along the cloud column and (2) to interpolate the resultant 3D cloud structure to the satellite’s full disk by applying a contemporary Deep-Learning approach. Input data was derived by an automated spatio-temporally matching between high-resoluted satellite channels and the overflight of the radar. These samples display the physical predictors that were fed into the network to reconstruct the cloud vertical distribution on each of the radar’s height levels along the whole domain. Data from the entire year 2017 was used to integrate seasonal variations into the modeling routine.

The results demonstrate not only the network’s ability to reconstruct the cloud column along the radar track but also to interpolate coherent structures into a large-scale perspective. While the model performs equally well over land and water bodies, its applicable time frame is limited to daytime predictions only. Finally, the generated data can be leveraged to build a comprehensive database of 3D cloud structures that is to be exploited in proceeding applications.

How to cite: Brüning, S., Niebler, S., and Tost, H.: Deep learning-based generation of 3D cloud structures from geostationary satellite data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3404, https://doi.org/10.5194/egusphere-egu23-3404, 2023.

EGU23-3418 | ECS | Posters on site | ITS1.14/CL5.8

Building a physics-constrained, fast and stable machine learning-based radiation emulator 

Guillaume Bertoli, Sebastian Schemm, Firat Ozdemir, Fernando Perez Cruz, and Eniko Szekely

Modelling the transfer of radiation through the atmosphere is a key component of weather and climate models. The operational radiation scheme in the Icosahedral Nonhydrostatic Weather and Climate Model (ICON) is ecRad. The radiation scheme ecRad is accurate but computationally expensive. It is operationally run in ICON on a grid coarser than the dynamical grid and the time step interval between two calls is significantly larger. This is known to reduce the quality of the climate prediction. A possible approach to accelerate the computation of the radiation fluxes is to use machine learning methods. Machine learning methods can significantly speed up computation of radiation, but they may cause climate drifts if they do not respect essential physical laws. In this work, we study random forest and neural network emulations of ecRad. We study different strategies to compare the stability of the emulations. Concerning the neural network, we compare loss functions with an additional energy penalty term and we observe that modifying the loss function is essential to predict accurately the heating rates. The random forest emulator, which is significantly faster to train than the neural network is used as a reference model that the neural network must outperform. The random forest emulator can become extremely accurate but the memory requirement quickly become prohibitive. Various numerical experiments are performed to illustrate the properties of the machine learning emulators.

How to cite: Bertoli, G., Schemm, S., Ozdemir, F., Perez Cruz, F., and Szekely, E.: Building a physics-constrained, fast and stable machine learning-based radiation emulator, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3418, https://doi.org/10.5194/egusphere-egu23-3418, 2023.

EGU23-3457 | Orals | ITS1.14/CL5.8

Evaluating Vegetation Modelling in Earth System Models with Machine Learning Approaches 

Ranjini Swaminathan, Tristan Quaife, and Richard Allan

The presence and amount of vegetation in any given region controls Gross Primary Production (GPP) or  the flux of carbon into the land driven by the process of photosynthesis. Earth System Models (ESMs) give us the ability to simulate GPP through modelling the various interactions between the atmosphere and biosphere including under different climate change scenarios in the future. GPP is the largest flux of the global carbon cycle and plays an important role including in carbon budget calculations.  However, GPP estimates from ESMs not only vary widely but also have much uncertainty in the underpinning attributors for this variability.  

We use data from pre-industrial Control (pi-Control) simulations to avail of the longer time period to sample data from as well as to exclude the influence of anthropogenic forcing in GPP estimation thereby leaving GPP to be largely attributable to two factor - (a) input atmospheric forcings and (b) the processes using those input climate variables to diagnose GPP. 

We explore the processes determining GPP with a physically-guided Machine Learning framework applied to a set of Earth System Models (ESMs) from the Sixth Coupled Model Intercomparison Project (CMIP6). We use this framework to examine whether differences in GPP across models are caused by differences in atmospheric state or process representations. 

Results from our analysis show that models with similar regional atmospheric forcing do not always have similar GPP distributions. While there are regions where climate models largely agree on what atmospheric variables are most relevant for GPP, there are regions such as the tropics where there is more uncertainty.  Our analysis highlights the potential of ML to identify differences in atmospheric forcing and carbon cycle process modelling across current state-of-the-art ESMs. It also allows us to extend the analysis with observational estimates of forcings as well as GPP for model improvement. 

How to cite: Swaminathan, R., Quaife, T., and Allan, R.: Evaluating Vegetation Modelling in Earth System Models with Machine Learning Approaches, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3457, https://doi.org/10.5194/egusphere-egu23-3457, 2023.

EGU23-3619 | ECS | Posters on site | ITS1.14/CL5.8

TCDetect: A new method of Detecting the Presence of Tropical Cyclones using Deep Learning 

Daniel Galea, Julian Kunkel, and Bryan Lawrence

Tropical cyclones are high-impact weather events which have large human and economic effects, so it is important to be able to understand how their location, frequency and structure might change in a future climate.

Here, a lightweight deep learning model is presented which is intended for detecting the presence of tropical cyclones during the execution of numerical simulations for use in an online data reduction method. This will help to avoid saving vast amounts of data for analysis after the simulation is complete. With run-time detection, it might be possible to reduce the need for some of the high-frequency high-resolution output which would otherwise be required.

The model was trained on ERA-Interim reanalysis data from 1979 to 2017 and the training concentrated on delivering the highest possible recall rate (successful detection of cyclones) while rejecting enough data to make a difference in outputs.

When tested using data from the two subsequent years, the recall or probability of detection rate was 92%. The precision rate or success ratio obtained was that of 36%. For the desired data reduction application, if the desired target included all tropical cyclone events, even those which did not obtain hurricane-strength status, the effective precision was 85%.

The recall rate and the Area Under Curve for the Precision/Recall (AUC-PR) compare favourably with other methods of cyclone identification while using the smallest number of parameters for both training and inference. 

Work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. LLNL-ABS-843612

How to cite: Galea, D., Kunkel, J., and Lawrence, B.: TCDetect: A new method of Detecting the Presence of Tropical Cyclones using Deep Learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3619, https://doi.org/10.5194/egusphere-egu23-3619, 2023.

EGU23-3875 | ECS | Posters on site | ITS1.14/CL5.8

Explainable AI for oceanic carbon cycle analysis of CMIP6 

Paul Heubel, Lydia Keppler, and Tatiana Iliyna

The Southern Ocean acts as one of Earth's major carbon sinks, taking up anthropogenic carbon from the atmosphere. Earth System Models (ESMs) are used to project its future evolution. However, the ESMs in the Coupled Model Intercomparison Project version 6 (CMIP6) disagree on the biogeochemical representation of the Southern Ocean carbon cycle, both with respect to the phasing and the magnitude of the seasonal cycle of dissolved inorganic carbon (DIC), and they compare poorly with observations.

We develop a framework to investigate model biases in 10 CMIP6 ESMs historical runs incorporating explainable artificial intelligence (xAI) methodologies. Using both a linear Random Forest feature relevance approach to a nonlinear self organizing map - feed forward neural network (SOM-FFN) framework, we relate 5 drivers of the seasonal cycle of DIC in the Southern Ocean in the different CMIP6 models. We investigate temperature, salinity, silicate, nitrate and dissolved oxygen as potential drivers. This analysis allows us to determine dominant statistical drivers of the seasonal cycle of DIC in the different models, and how they compare to the observations. Our findings inform future model development to better constrain the seasonal cycle of DIC.

How to cite: Heubel, P., Keppler, L., and Iliyna, T.: Explainable AI for oceanic carbon cycle analysis of CMIP6, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3875, https://doi.org/10.5194/egusphere-egu23-3875, 2023.

EGU23-4044 | ECS | Orals | ITS1.14/CL5.8

DailyMelt: Diffusion-based Models for Spatiotemporal Downscaling of (Ant-)arctic Surface Meltwater Maps 

Björn Lütjens, Patrick Alexander, Raf Antwerpen, Guido Cervone, Matthew Kearney, Bingkun Luo, Dava Newman, and Marco Tedesco

Motivation. Ice melting in Greenland and Antarctica has increasingly contributed to rising sea levels. Yet, the exact speed of melting, existence of abrupt tipping points, and in-detail links to climate change remain uncertain. Ice shelves essentially prevent the ice sheet from slipping into the ocean and better prediction of collapses is needed. Meltwater at the surface of ice shelves indicates ice shelf collapse through destabilizing ice shelves via fracturing and flexural processes (Banwell et al., 2013) and is likely impacted by a warming climate ( Kingslake et al., 2017). Maps of meltwater have been created from in-situ and remote observations, but their low and irregular spatiotemporal resolution severely limits studies (Kingslake et al., 2019).

Research Gap. In particular, there does not exist daily high-resolution (< 500m) maps of surface meltwater. We propose the first daily high-resolution surface meltwater maps by developing a deep learning-based downscaling method, called DailyMelt, that fuses observations and simulations of varying spatiotemporal resolution, as illustrated in Fig.1. The created maps will improve understanding of the origin, transport, and controlling physical processes of surface meltwater. Moreover, they will act as unified source to improve sea level rise and meltwater predictions in climate models. 

Data. To synthesize surface meltwater maps, we leverage observations from satellites (MODIS, Sen-1 SAR) which are high-resolution (500m, 10m), but have substantial temporal gaps due to repeat time and cloud coverage. We fuse them with simulations (MAR) and passive microwave observations (MEaSURE) that are daily, but low-resolution (6km, 3.125km). In a significant remote sensing effort, we have downloaded, reprojected, and regridded all products into daily observations for our study area over Greenland’s Helheim glacier. 

Approach and expected results. Within deep generative vision models, diffusion-based models promise sharp and probabilistic predictions. We have implemented SRDiff (Li H. et al., 2022) and tested it on spatially downscaling external data. As a baseline model, we have implemented a statistical downscaling model that is a local hybrid physics-linear regression model (Noel et al., 2016). In our planned benchmark, we expect a baseline UNet architecture that minimizes RMSE to create blurry maps and a generative adversarial network that minimizes adversarial loss to create sharp but deterministic maps. We have started with spatial downscaling and will include temporal downscaling. 

In summary, we will create the first daily high-resolution (500m) surface meltwater maps, have introduced the first diffusion-based model for downscaling Earth sciences data, and have created the first benchmark dataset for downscaling surface meltwater maps.

 

References.

Banwell, A. F., et al. (2013), Breakup of the Larsen B Ice Shelf triggered by chain reaction drainage of supraglacial lakes, Geophys. Res. Lett., 40 

Kingslake J, et al. (2017), Widespread movement of meltwater onto and across Antarctic ice shelves, Nature, 544(7650)

Kingslake J., et al. (2019), Antarctic Surface Hydrology and Ice Shelf Stability Workshop report, US Antarctic Program Data Center

Li H., et al. (2022), SRDiff: Single image super-resolution with diffusion probabilistic models, Neurocomputing, 479

Noël, B., et al. (2016), A daily, 1 km resolution data set of downscaled Greenland ice sheet surface mass balance (1958–2015), The Cryosphere, 10

How to cite: Lütjens, B., Alexander, P., Antwerpen, R., Cervone, G., Kearney, M., Luo, B., Newman, D., and Tedesco, M.: DailyMelt: Diffusion-based Models for Spatiotemporal Downscaling of (Ant-)arctic Surface Meltwater Maps, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4044, https://doi.org/10.5194/egusphere-egu23-4044, 2023.

EGU23-4350 | ECS | Orals | ITS1.14/CL5.8

Physics-Constrained Deep Learning for Downscaling 

Paula Harder, Venkatesh Ramesh, Alex Hernandez-Garcia, Qidong Yang, Prasanna Sattigeri, Daniela Szwarcman, Campbell Watson, and David Rolnick

The availability of reliable, high-resolution climate and weather data is important to inform long-term decisions on climate adaptation and mitigation and to guide rapid responses to extreme events. Forecasting models are limited by computational costs and, therefore, often generate coarse-resolution predictions. Statistical downscaling can provide an efficient method of upsampling low-resolution data. In this field, deep learning has been applied successfully, often using image super-resolution methods from computer vision. However, despite achieving visually compelling results in some cases, such models frequently violate conservation laws when predicting physical variables. In order to conserve physical quantities, we develop methods that guarantee physical constraints are satisfied by a deep learning downscaling model while also improving their performance according to traditional metrics. We compare different constraining approaches and demonstrate their applicability across different neural architectures as well as a variety of climate and weather data sets, including ERA5 and WRF data sets.

How to cite: Harder, P., Ramesh, V., Hernandez-Garcia, A., Yang, Q., Sattigeri, P., Szwarcman, D., Watson, C., and Rolnick, D.: Physics-Constrained Deep Learning for Downscaling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4350, https://doi.org/10.5194/egusphere-egu23-4350, 2023.

EGU23-5431 | ECS | Orals | ITS1.14/CL5.8

Towards Robust Parameterizations in Ecosystem-level Photosynthesis Models 

Shanning Bao, Nuno Carvalhais, Lazaro Alonso, Siyuan Wang, Johannes Gensheimer, Ranit De, and Jiancheng Shi

Photosynthesis model parameters represent vegetation properties or sensitivities of photosynthesis processes. As one of the model uncertainty sources, parameters affect the accuracy and generalizability of the model. Ideally, parameters of ecosystem-level photosynthesis models, i.e., gross primary productivity (GPP) models, can be measured or inversed from observations at the local scale. To extrapolate parameters to a larger spatial scale, current photosynthesis models typically adopted fixed values or plant-functional-type(PFT)-specific values. However, the fixed and PFT-based parameterization approaches cannot capture sufficiently the spatial variability of parameters and lead to significant estimation errors. Here, we propose a Simultaneous Parameter Inversion and Extrapolation approach (SPIE) to overcome these issues. 

SPIE refers to predicting model parameters using an artificial neural network (NN) constrained by both model loss and ecosystem features including PFT, climate types, bioclimatic variables, vegetation features, atmospheric nitrogen and phosphorus deposition and soil properties. Taking a light use efficiency (LUE) model as an example, we evaluated SPIE at 196 FLUXNET eddy covariance flux sites. The LUE model accounts for the effects of air temperature, vapor pressure deficit, soil water availability (SW), light saturation, diffuse radiation fraction and CO2 on GPP using five independent sensitivity functions. The SW was represented using the water availability index and can be optimized based on evapotranspiration. Thus, we optimized the NN by minimizing the model loss which consists of GPP errors, evapotranspiration errors, and constraints on sensitivity functions. Furthermore, we compared SPIE with 11 typical parameter extrapolating approaches, including PFT- and climate-specific parameterizations, global and PFT-based parameter optimization, site-similarity, and regression methods using Nash-Sutcliffe model efficiency (NSE), determination coefficient (R2) and normalized root mean squared error (NRMSE).

The results in ten-fold cross-validation showed that SPIE had the best performance across various temporal and spatial scales and across assessing metrics. None of the parameter extrapolating approaches reached the same performance as the on-site calibrated parameters (NSE=0.95), but SPIE was the only approach showing positive NSE (=0.68) in cross-validation across sites. Moreover, the site-level NSE, R2, and NRMSE of SPIE all significantly outperformed per biome and per climate type. Ranges of parameters were more constrained by SPIE than site calibrations.

Overall, SPIE is a robust parameter extrapolation approach that overcomes strong limitations observed in many of the standard model parameterization approaches. Our approach suggests that model parameterizations can be determined from observations of vegetation, climate and soil properties, and expands from customary clustering methods (e.g., PFT-specific parameterization). We argue that expanding SPIE to other models overcomes current limits in parameterization and serves as an entry point to investigate the robustness and generalization of different models.

How to cite: Bao, S., Carvalhais, N., Alonso, L., Wang, S., Gensheimer, J., De, R., and Shi, J.: Towards Robust Parameterizations in Ecosystem-level Photosynthesis Models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5431, https://doi.org/10.5194/egusphere-egu23-5431, 2023.

EGU23-5487 * | ECS | Posters on site | ITS1.14/CL5.8 | Highlight

Harvesting historical spy imagery by evaluating deep learning models for state-wide mapping of land cover changes between 1965-1978 

Lucas Kugler, Christopher Marrs, Eric Kosczor, and Matthias Forkel

Remote sensing has played a fundamental role for land cover mapping and change detection at least since the launch of the Landsat satellite program in 1972. In 1995, the Central Intelligence Agency of the United States of America released previously classified spy imagery taken from 1960 onwards with near-global coverage from the Keyhole programme, which includes the CORONA satellite mission. CORONA imagery is a treasure because it contains information about land cover 10 years before the beginning of the civilian Earth observation and has a high spatial resolution < 2m. However, this imagery is only pan-chromatic and usually not georeferenced, which has so far prevented a large-scale application for land cover mapping or other geophysical and environmental applications.

Here, we aim to harvest the valuable information about past land cover from CORONA imagery for a state-wide mapping of past land cover changes between 1965 and 1978 by training, testing and validating various deep learning models.

To the best of our knowledge, this is the first work to analyse land cover from CORONA data on a large scale, dividing land cover into six classes based on the CORINE classification scheme. The particular focus of the work is to test the transferability of the deep learning approaches to unknown CORONA data.

To investigate the transferability, we selected 27 spatially and temporally distributed study areas (each 23 km²) in the Free State of Saxony (Germany) and created semantic masks to train and test 10 different U-shaped neuronal network architectures to extract land cover from CORONA data. As input, we use either the original panchromatic pixel values and different texture measures. From these input data, ten different training datasets and test datasets were derived for cross-validation.

The training results show that a semantic segmentation of land cover from CORONA data with the used architectures is possible. Strong differences in model performance (based on cross validation and the intersection over union metric, IOU) were detected among the classes. Classes with many sample data achieve significantly better IOU values than underrepresented classes. In general, a U-shaped architecture with a Transformer as Encoder (Transformer U-Net) achieved the best results. The best segmentation performance (IOU 83.29%), was obtained for forests, followed by agriculture (74.21%). For artificial surfaces, a mean IOU of 68.83% was achieved. Water surfaces achieved a mean IOU of 66.49%. For the shrub vegetation and open areas classes only IOU values mostly below 25% were achieved. The deep learning models were successfully transferable in space (between test areas) and time (between CORONA imagery from different years) especially for classes with many sample data. The transferability of deep learning models was difficult for the mapping of water bodies. Despite the general good model performance and successful transferability for most classes, the transferability was limited especially for imagery of very poor quality. Our approach enabled the state-wide mapping of land cover in Saxony between 1965 and 1978 with a spatial resolution of 2 m. We identify an increase in urban cover and a decrease in cropland cover

How to cite: Kugler, L., Marrs, C., Kosczor, E., and Forkel, M.: Harvesting historical spy imagery by evaluating deep learning models for state-wide mapping of land cover changes between 1965-1978, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5487, https://doi.org/10.5194/egusphere-egu23-5487, 2023.

EGU23-5583 | ECS | Posters on site | ITS1.14/CL5.8

Identifying and Locating Volcanic Eruptions using Convolutional Neural Networks and Interpretability Techniques 

Johannes Meuer, Claudia Timmreck, Shih-Wei Fang, and Christopher Kadow

Accurately interpreting past climate variability can be a challenging task, particularly when it comes to distinguishing between forced and unforced changes. In the  case of large volcanic eruptions, ice core records are a very valuable tool but still often not sufficient to link reconstructed anomaly patterns to a volcanic eruption at all or to its geographical location. In this study, we developed a convolutional neural network (CNN) that is able to classify whether a volcanic eruption occurred and its location (northern hemisphere extratropical, southern hemisphere extratropical, or tropics) with an accuracy of 92%.

To train the CNN, we used 100 member ensembles of the MPI-ESM-LR global climate model, generated using the easy volcanic aerosol (EVA) model, which provides the radiative forcing of idealized volcanic eruptions of different strengths and locations. The model considered global sea surface temperature and precipitation patterns 12 months after the eruption over a time period of 3 months.

In addition to demonstrating the high accuracy of the CNN, we also applied layer-wise relevance propagation (LRP) to the model to understand its decision-making process and identify the input data that influenced its predictions. Our study demonstrates the potential of using CNNs and interpretability techniques for identifying and locating past volcanic eruptions as well as improving the accuracy and understanding of volcanic climate signals.

How to cite: Meuer, J., Timmreck, C., Fang, S.-W., and Kadow, C.: Identifying and Locating Volcanic Eruptions using Convolutional Neural Networks and Interpretability Techniques, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5583, https://doi.org/10.5194/egusphere-egu23-5583, 2023.

EGU23-5967 | ECS | Posters on site | ITS1.14/CL5.8

Potentials and challenges of using Explainable AI for understanding atmospheric circulation 

Sebastian Scher, Andreas Trügler, and Jakob Abermann

Machine Learning (ML) and AI techniques, especially methods based on Deep Learning, have long been considered as black boxes that might be good at predicting, but not explaining predictions. This has changed recently, with more techniques becoming available that explain predictions by ML models – known as Explainable AI (XAI). These have seen adaptation also in climate science, because they could have the potential to help us in understanding the physics behind phenomena in geoscience. It is, however, unclear, how large that potential really is, and how these methods can be incorporated into the scientific process. In our study, we use the exemplary research question of which aspects of the large-scale atmospheric circulation affect specific local conditions. We compare the different answers to this question obtained with a range of different methods, from the traditional approach of targeted data analysis based on physical knowledge (such as using dimensionality reduction based on physical reasoning) to purely data-driven and physics-unaware methods using Deep Learning with XAI techniques. Based on these insights, we discuss the usefulness and potential pitfalls of XAI for understanding and explaining phenomena in geosciences. 

How to cite: Scher, S., Trügler, A., and Abermann, J.: Potentials and challenges of using Explainable AI for understanding atmospheric circulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5967, https://doi.org/10.5194/egusphere-egu23-5967, 2023.

EGU23-6061 | ECS | Orals | ITS1.14/CL5.8 | Highlight

Using reduced representations of atmospheric fields to quantify the causal drivers of air pollution 

Sebastian Hickman, Paul Griffiths, Peer Nowack, and Alex Archibald

Air pollution contributes to millions of deaths worldwide every year. The concentration of a particular air pollutant, such as ozone, is controlled by physical and chemical processes which act on varying temporal and spatial scales. Quantifying the strength of causal drivers (e.g. temperature) on air pollution from observational data, particularly at extrema, is challenging due to the difficulty of disentangling correlation and causation, as many drivers are correlated. Furthermore, because air pollution is controlled in part by large scale atmospheric phenomena, using local (e.g. individual grid cell level) covariates for analysis is insufficient to fully capture the effect of these phenomena on air pollution. 

 

Access to large spatiotemporal datasets of air pollutant concentrations and atmospheric variables, coupled with recent advances in self-supervised learning, allow us to learn reduced representations of spatiotemporal atmospheric fields, and therefore account for non-local and non-instantaneous processes in downstream tasks.

 

We show that these learned reduced representations can be useful for tasks such as air pollution forecasting, and crucially to quantify the causal effect of varying atmospheric fields on air pollution. We make use of recent advances in bounding causal effects in the presence of unobserved confounding to estimate, with uncertainty, the causal effect of changing atmospheric fields on air pollution. Finally, we compare our quantification of the causal drivers of air pollution to results from other approaches, and explore implications for our methods and for the wider goal of improving the process-level treatment of air pollutants in chemistry-climate models.

How to cite: Hickman, S., Griffiths, P., Nowack, P., and Archibald, A.: Using reduced representations of atmospheric fields to quantify the causal drivers of air pollution, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6061, https://doi.org/10.5194/egusphere-egu23-6061, 2023.

EGU23-6306 | ECS | Orals | ITS1.14/CL5.8 | Highlight

Data-Driven Cloud Cover Parameterizations 

Arthur Grundner, Tom Beucler, Pierre Gentine, Marco A. Giorgetta, Fernando Iglesias-Suarez, and Veronika Eyring

A promising approach to improve cloud parameterizations within climate models, and thus climate projections, is to train machine learning algorithms on storm-resolving model (SRM) output. The ICOsahedral Non-hydrostatic (ICON) modeling framework permits simulations ranging from numerical weather prediction to climate projections, making it an ideal target to develop data-driven parameterizations for sub-grid scale processes. Here, we systematically derive and evaluate the first data-driven cloud cover parameterizations with coarse-grained data based on ICON SRM simulations. These parameterizations range from simple analytic models and symbolic regression fits to neural networks (NNs), populating a performance x complexity plane. In most models, we enforce sparsity and discourage correlated features by sequentially selecting features based on the models' performance gains. Guided by a set of physical constraints, we use symbolic regression to find a novel equation to parameterize cloud cover. The equation represents a good compromise between performance and complexity, achieving the highest performance (R^2>0.9) for its complexity (13 trainable parameters). To model sub-grid scale cloud cover in its full complexity, we also develop three different types of NNs that differ in the degree of vertical locality they assume for diagnosing cloud cover from coarse-grained atmospheric state variables. Using the game-theory based interpretability library SHapley Additive exPlanations, we analyze our most non-local NN and identify an overemphasis on specific humidity and cloud ice as the reason why it cannot perfectly generalize from the global to the regional coarse-grained SRM data. The interpretability tool also helps visualize similarities and differences in feature importance between regionally and globally trained NNs, and reveals a local relationship between their cloud cover predictions and the thermodynamic environment. Our results show the potential of deep learning and symbolic regression to derive accurate yet interpretable cloud cover parameterizations from SRMs.

How to cite: Grundner, A., Beucler, T., Gentine, P., Giorgetta, M. A., Iglesias-Suarez, F., and Eyring, V.: Data-Driven Cloud Cover Parameterizations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6306, https://doi.org/10.5194/egusphere-egu23-6306, 2023.

EGU23-6450 | ECS | Orals | ITS1.14/CL5.8

The key role of causal discovery to improve data-driven parameterizations in climate models 

Fernando Iglesias-Suarez, Veronika Eyring, Pierre Gentine, Tom Beucler, Michael Pritchard, Jakob Runge, and Breixo Solino-Fernandez

Earth system models are fundamental to understanding and projecting climate change, although there are considerable biases and uncertainties in their projections. A large contribution to this uncertainty stems from differences in the representation of clouds and convection occurring at scales smaller than the resolved model grid. These long-standing deficiencies in cloud parameterizations have motivated developments of computationally costly global high-resolution cloud resolving models, that can explicitly resolve clouds and convection. Deep learning can learn such explicitly resolved processes from cloud resolving models. While unconstrained neural networks often learn non-physical relationships that can lead to instabilities in climate simulations, causally-informed deep learning can mitigate this problem by identifying direct physical drivers of subgrid-scale processes. Both unconstrained and causally-informed neural networks are developed using a superparameterized climate model in which deep convection is explicitly resolved, and are coupled to the climate model. Prognostic climate simulations with causally-informed neural network parameterization are stable, accurately represent mean climate and variability of the original climate model, and clearly outperform its non-causal counterpart. Combining causal discovery and deep learning is a promising approach to improve data-driven parameterizations (informed by causally-consistent physical fields) for both their design and trustworthiness.

How to cite: Iglesias-Suarez, F., Eyring, V., Gentine, P., Beucler, T., Pritchard, M., Runge, J., and Solino-Fernandez, B.: The key role of causal discovery to improve data-driven parameterizations in climate models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6450, https://doi.org/10.5194/egusphere-egu23-6450, 2023.

EGU23-7457 | ECS | Posters on site | ITS1.14/CL5.8

Towards the effective autoencoder architecture to detect weather anomalies 

Dusan Fister, Jorge Pérez-Aracil, César Peláez-Rodríguez, Marie Drouard, Pablo G. Zaninelli, David Barriopedro Cepero, Ricardo García-Herrera, and Sancho Salcedo-Sanz

To organise weather data as images, pixels represent coordinates and magnitude of pixels represents the state of the observed variable in a given time. Observed variables, such as air temperature, mean sea level pressure, wind components and others, may be collected into higher dimensional images or even into a motion structure. Codification of formers as a spatial and the latter as a spatio-temporal allows them to be processed using the deep learning methods, for instance autoencoders and autoencoder-like architectures. The objective of the original autoencoder is to reproduce the input image as much as possible, thus effectively equalising the input and output during the training. Then, an advantage of autoencoder can be utilised to calculate the deviations between (1) true states (effectively the inputs), which are derived by nature, and the (2) expected states, which are derived by means of statistical learning. Calculated deviations can then be interpreted to identify the extreme events, such as heatwaves, hot days or any other rare events (so-called anomalies). Additionally, by modelling deviations by statistical distributions, geographical areas with higher probabilities of anomalies can be deduced at the tails of the distribution. The capability of reproduction of the (original input) images is hence crucial in order to avoid addressing arbitrary noise as anomaly. We would like to run experiments to realise the effective architecture that give reasonable solutions, verify the benefits of implementing the variational autoencoder, realise the effect of selecting various statistical loss functions, and find out the effective architecture of the decoder part of the autoencoder.

How to cite: Fister, D., Pérez-Aracil, J., Peláez-Rodríguez, C., Drouard, M., G. Zaninelli, P., Barriopedro Cepero, D., García-Herrera, R., and Salcedo-Sanz, S.: Towards the effective autoencoder architecture to detect weather anomalies, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7457, https://doi.org/10.5194/egusphere-egu23-7457, 2023.

EGU23-7465 | ECS | Posters on site | ITS1.14/CL5.8

Invertible neural networks for satellite retrievals of aerosol optical depth 

Paolo Pelucchi, Jorge Vicent, J. Emmanuel Johnson, Philip Stier, and Gustau Camps-Valls

The retrieval of atmospheric aerosol properties from satellite remote sensing is a complex and under-determined inverse problem. Traditional retrieval algorithms, based on radiative transfer models, must make approximations and assumptions to reach a unique solution or repeatedly use the expensive forward models to be able to quantify uncertainty. The recently introduced Invertible Neural Networks (INNs), a machine learning method based on Normalizing Flows, appear particularly suited for tackling inverse problems. They simultaneously model both the forward and the inverse branches of the problem, and their generative aspect allows them to efficiently provide non-parametric posterior distributions for the retrieved parameters, which can be used to quantify the retrieval uncertainty. So far INNs have successfully been applied to low-dimensional idealised inverse problems and even to some simpler scientific retrieval problems. Still, satellite aerosol retrievals present particular challenges, such as the high variability of the surface reflectance signal and the often comparatively small aerosol signal in the top-of-the-atmosphere (TOA) measurements.

In this study, we investigate the use of INNs for retrieving aerosol optical depth (AOD) and its uncertainty estimates at the pixel level from MODIS TOA reflectance measurements. The models are trained with custom synthetic datasets of TOA reflectance-AOD pairs made by combining the MODIS Dark Target algorithm’s atmospheric look-up tables and a MODIS surface reflectance product. The INNs are found to perform emulation and inversion of the look-up tables successfully. We initially train models adapted to different surface types by focusing our application on limited regional and seasonal contexts. The models are applied to real measurements from the MODIS sensor, and the generated AOD retrievals and posterior distributions are compared to the corresponding Dark Target and AERONET retrievals for evaluation and discussion.

How to cite: Pelucchi, P., Vicent, J., Johnson, J. E., Stier, P., and Camps-Valls, G.: Invertible neural networks for satellite retrievals of aerosol optical depth, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7465, https://doi.org/10.5194/egusphere-egu23-7465, 2023.

The rapid development of deep learning approaches has conquered many fields, and precipitation prediction is one of them. Precipitation modeling remains a challenge for numerical weather prediction or climate models, and parameterization is required for low spatial resolution models, such as those used in climate change impact studies. Machine learning models have been shown to be capable of learning the relationships between other meteorological variables and precipitation. Such models are much less computationally intensive than explicit modeling of precipitation processes and are becoming more accurate than parametrization schemes.

Most existing applications focus either on precipitation extremes aggregated over a domain of interest or on average precipitation fields. Here, we are interested in spatial extremes and focus on the prediction of heavy precipitation events (>95th percentile) and extreme events (>99th percentile) over the European domain. Meteorological variables from ERA5 are used as input, and E-OBS data as target. Different architectures from the literature are compared in terms of predictive skill for average precipitation fields as well as for the occurrence of heavy or extreme precipitation events (threshold exceedance). U-Net architectures show higher skills than other variants of convolutional neural networks (CNN). We also show that a shallower U-Net architecture performs as well as the original network for this application, thus reducing the model complexity and, consequently, the computational resources. In addition, we analyze the number of inputs based on the importance of the predictors provided by a layer-wise relevance propagation procedure.

How to cite: Horton, P. and Otero, N.: Predicting spatial precipitation extremes with deep learning models. A comparison of existing model architectures., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7862, https://doi.org/10.5194/egusphere-egu23-7862, 2023.

EGU23-8085 | ECS | Posters on site | ITS1.14/CL5.8

Improving the spatial accuracy of extreme tropical cyclone rainfall in ERA5 using deep learning 

Guido Ascenso, Andrea Ficchì, Leone Cavicchia, Enrico Scoccimarro, Matteo Giuliani, and Andrea Castelletti

Tropical cyclones (TCs) are one of the costliest and deadliest natural disasters due to the combination of their strong winds and induced storm surges and heavy precipitation, which can cause devastating floods. Unfortunately, due to its high spatio-temporal variability, complex underlying physical process, and lack of high-quality observations, precipitation is still one of the most challenging aspects of a TC to model. However, as precipitation is a key forcing variable for hydrological processes acting across multiple space-time scales, accurate precipitation input is crucial for reliable hydrological simulations and forecasts.

A popular source of precipitation data is the ERA5 reanalysis dataset, frequently used as input to hydrological models when studying floods. However, ERA5 systematically underestimates TC-induced precipitation compared to MSWEP, a multi-source observational dataset fusing gauge, satellite, and reanalysis-based data, currently one of the most accurate precipitation datasets. Moreover, the spatial distribution of TC-rainfall in ERA5 has large room for improvement.

Here, we present a precipitation correction scheme based on U-Net, a popular deep-learning architecture. Rather than only adjusting the per-pixel precipitation values at each timestep of a given TC, we explicitly design our model to also adjust the spatial distribution of the precipitation; to the best of our knowledge, we are the first to do so. The key novelty of our model is a custom-made loss function, based on the combination of the fractions skill score (FSS) and mean absolute error (MAE) metrics. We train and validate the model on 100k time steps (with an 80:20 train:test split) from global TC precipitation events. We show how a U-Net trained with our loss function can reduce the per-pixel MAE of ERA5 precipitation by nearly as much as other state-of-the-art methods, while surpassing them significantly in terms of improved spatial patterns of precipitation. Finally, we discuss how the outputs of our model can be used for future research.

How to cite: Ascenso, G., Ficchì, A., Cavicchia, L., Scoccimarro, E., Giuliani, M., and Castelletti, A.: Improving the spatial accuracy of extreme tropical cyclone rainfall in ERA5 using deep learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8085, https://doi.org/10.5194/egusphere-egu23-8085, 2023.

EGU23-8496 | ECS | Posters on site | ITS1.14/CL5.8

Utilizing AI emulators to Model Stratospheric Aerosol Injections and their Effect on Climate 

Eshaan Agrawal and Christian Schroder de Witt

With no end to anthropogenic greenhouse gas emissions in sight, policymakers are increasingly debating artificial mechanisms to cool the earth's climate. One such solution is stratospheric atmospheric injections (SAI), a method of solar geoengineering where particles are injected into the stratosphere in order to reflect the sun’s rays and lower global temperatures. Past volcanic events suggest that SAI can lead to fast substantial surface temperature reductions, and it is projected to be economically feasible. Research in simulation, however, suggests that SAI can lead to catastrophic side effects. It is also controversial among politicians and environmentalists because of the numerous challenges it poses geopolitically, environmentally, and for human health. Nevertheless, SAI is increasingly receiving attention from policymakers. In this research project, we use deep reinforcement learning to study if, and by how much, carefully engineered temporally and spatially varying injection strategies can mitigate catastrophic side effects of SAI. To do this, we are using the HadCM3 global circulation model to collect climate system data in response to artificial longitudinal aerosol injections. We then train a neural network emulator on this data, and use it to learn optimal injection strategies under a variety of objectives by alternating model updates with reinforcement learning. We release our dataset and code as a benchmark dataset to improve emulator creation for solar aerosol engineering modeling. 

How to cite: Agrawal, E. and Schroder de Witt, C.: Utilizing AI emulators to Model Stratospheric Aerosol Injections and their Effect on Climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8496, https://doi.org/10.5194/egusphere-egu23-8496, 2023.

Multiple studies have now demonstrated that machine learning (ML) can give improved skill for simulating fairly typical weather events in climate simulations, for tasks such as downscaling to higher resolution and emulating and speeding up expensive model parameterisations. Many of these used ML methods with very high numbers of parameters, such as neural networks, which are the focus of the discussion here. Not much attention has been given to the performance of these methods for extreme event severities of relevance for many critical weather and climate prediction applications, with return periods of more than a few years. This leaves a lot of uncertainty about the usefulness of these methods, particularly for general purpose models that must perform reliably in extreme situations. ML models may be expected to struggle to predict extremes due to there usually being few samples of such events. 
 
This presentation will review the small number of studies that have examined the skill of machine learning methods in extreme weather situations. It will be shown using recent results that machine learning methods that perform reasonably for typical weather events can have very large errors in extreme situations, highlighting the necessity of testing the performance for these cases. Extrapolation to extremes is found to work well in some studies, however. 
 
It will be argued that more attention needs to be given to performance for extremes in work applying ML in climate science. Research gaps that seem particularly important are identified. These include investigating the behaviour of ML systems in events that are multiple standard deviations beyond observed records, which have occurred in the past, and evaluating performance of complex generative models in extreme events. Approaches to address these problems will be discussed.

How to cite: Watson, P.: Machine learning applications for weather and climate need greater focus on extremes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8615, https://doi.org/10.5194/egusphere-egu23-8615, 2023.

EGU23-8661 | Posters on site | ITS1.14/CL5.8

An urban climate neural network screening tool 

Robert von Tils and Sven Wiemers

Microscale RANS (Reynolds Averaged Navier Stokes) models are able to simulate the urban climate for entire large cities with a high spatial resolution of up to 5 m horizontally. They do this using data from geographic information systems (GIS) that must be specially processed to provide the models with information about the terrain, buildings, land use, and resolved vegetation. If high-performance computers, for example from research institutions, are not available for the simulations or are beyond the financial scope, the calculation on commercially available servers can take several weeks. The calculation of a reference initial state for a city is often followed by questions regarding adaptation measures due to climate change or the influence of smaller and larger future building developments on the urban climate. These changes lead locally to a change of the urban climate but are also influenced by the urban climate itself.

In order to save computational time and to comfortably give a quantitative fast initial assessment, we trained a neural network that predicts the simulation results of a RANS model (for example: air temperature at night and during the day, wind speed, cold air flow) and implemented this network in a GIS. The tool allows to calculate the impact of development projects on the urban climate in a fraction of the time required by a RANS simulation and comes close to the RANS model in terms of accuracy. It can also be used by people without in-depth knowledge of urban climate modeling and is therefore particularly suitable for use, for example, in specialized offices of administrative departments or by project developers.

How to cite: von Tils, R. and Wiemers, S.: An urban climate neural network screening tool, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8661, https://doi.org/10.5194/egusphere-egu23-8661, 2023.

EGU23-8666 | ECS | Posters on site | ITS1.14/CL5.8

Drivers of Natural Gas Use in United States Buildings 

Rohith Teja Mittakola, Philippe Ciais, Jochen Schubert, David Makowski, Chuanlong Zhou, Hassan Bazzi, Taochun Sun, Zhu Liu, and Steven Davis

Natural gas is the primary fuel used in U.S. residences, especially during winter, when cold temperatures drive the heating demand. In this study, we use daily county-level gas consumption data to assess the spatial patterns of the relationships and sensitivities of gas consumption by U.S. households considering outdoor temperatures. Linear-plus-plateau functions are found to be the best fit for gas consumption and are applied to derive two key coefficients for each county: the heating temperature threshold (Tcrit) below which residential heating starts and the rate of increase in gas consumption when the outdoor temperature drops by one degree (Slope). We then use interpretable machine learning models to evaluate the key building properties and socioeconomic factors related to the spatial patterns of Tcrit and Slope based on a large database of individual household properties and population census data. We find that building age, employment rates, and household size are the main predictors of Tcrit, whereas the share of gas as a heating fuel and household income are the main predictors of Slope. The latter result suggests inequalities across the U.S. with respect to gas consumption, with wealthy people living in well-insulated houses associated with low Tcrit and Slope values. Finally, we estimate potential reductions in gas use in U.S. residences due to improvements in household insulation or a hypothetical behavioral change toward reduced consumption by adopting a 1°C lower Tcrit than the current value and a reduced slope. These two scenarios would result in 25% lower gas consumption at the national scale, avoiding 1.24 million MtCO2 of emissions per year. Most of these reductions occur in the Midwest and East Coast regions. The results from this study provide new quantitative information for targeting efforts to reduce household gas use and related CO2 emissions in the U.S.

How to cite: Mittakola, R. T., Ciais, P., Schubert, J., Makowski, D., Zhou, C., Bazzi, H., Sun, T., Liu, Z., and Davis, S.: Drivers of Natural Gas Use in United States Buildings, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8666, https://doi.org/10.5194/egusphere-egu23-8666, 2023.

EGU23-8921 | ECS | Posters on site | ITS1.14/CL5.8

Identification of sensitive regions to climate change and anticipation of climate events in Brazil 

Angelica Caseri and Francisco A. Rodrigues

In Brazil, the water system is essential for the electrical system and agribusiness. Understanding climate changes and predicting long-term hydrometeorological phenomena is vital for developing and maintaining these sectors in the country. This work aims to use data from the SIN system (National Interconnected System) in Brazil, from the main hydrological basins, as well as historical rainfall data, in complex networks and deep learning algorithms, to identify possible climate changes in Brazil and predict future hydrometeorological phenomena. Through the methodology developed in this work, the predictions generated showed satisfactory results, which allows identifying regions more sensitive to climate change and anticipating climate events. This work is expected to help the energy generation system in Brazil and the agronomy sector, the main sectors that drive the country's economy.

How to cite: Caseri, A. and A. Rodrigues, F.: Identification of sensitive regions to climate change and anticipation of climate events in Brazil, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8921, https://doi.org/10.5194/egusphere-egu23-8921, 2023.

EGU23-9337 | ECS | Posters on site | ITS1.14/CL5.8

Modeling landscape-scale vegetation response to climate: Synthesis of the EarthNet challenge 

Vitus Benson, Christian Requena-Mesa, Claire Robin, Lazaro Alonso, Nuno Carvalhais, and Markus Reichstein

The biosphere displays high heterogeneity at landscape-scale. Vegetation modelers struggle to represent this variability in process-based models because global observations of micrometeorology and plant traits are not available at such fine granularity. However, remote sensing data is available: the Sentinel 2 satellites with a 10m resolution capture aspects of localized vegetation dynamics. The EarthNet challenge (EarthNet2021, [1]) aims at predicting satellite imagery conditioned on coarse-scale weather data. Multiple research groups approached this challenge with deep learning [2,3,4]. Here, we evaluate how well these satellite image models simulate the vegetation response to climate, where the vegetation status is approximated by the NDVI vegetation index.

Achieving the new vegetation-centric evaluation requires three steps. First, we update the original EarthNet2021 dataset to be suitable for vegetation modeling: EarthNet2021x includes improved georeferencing, a land cover map, and a more effective cloud mask. Second, we introduce the interpretable evaluation metric VegetationScore: the Nash Sutcliffe model efficiency (NSE) of NDVI predictions over clear-sky observations per vegetated pixel aggregated through normalization to dataset level. The ground truth NDVI time series achieves a VegetationScore of 1, the target period mean NDVI a VegetationScore of 0. Third, we assess the skill of two deep neural networks with the VegetationScore: ConvLSTM [2,3], which combines convolutions and recurrency, and EarthFormer [4], a Transformer adaptation for Earth science problems. 

Both models significantly outperform the persistence baseline. They do not display systematic biases and generally catch spatial patterns. Yet, both neural networks achieve a negative VegetationScore. Only in about 20% of vegetated pixels, the deep learning models do beat a hypothetical model predicting the true target period mean NDVI. This is partly because models largely underestimate the temporal variability. However, the target variability may partially be inflated by the noisy nature of the observed NDVI. Additionally, increasing uncertainty for longer lead times decreases scores: the mean RMSE in the first 25 days is 50% lower than between 75 and 100 days lead time. In general, consistent with the EarthNet2021 leaderboard, the EarthFormer outperforms the ConvLSTM. With EarthNet2021x, a more narrow perspective to the EarthNet challenge is introduced. Modeling localized vegetation response is a task that requires careful adjustments of off-the-shelf computer vision architectures for them to excel. The resulting specialized approaches can then be used to advance our understanding of the complex interactions between vegetation and climate.



 [1] Requena-Mesa, Benson, Reichstein, Runge and Denzler. EarthNet2021: A large-scale dataset and challenge for Earth surface forecasting as a guided video prediction task. CVPR Workshops, 2021.

 [2] Diaconu, Saha, Günnemann and Zhu. Understanding the Role of Weather Data for Earth Surface Forecasting Using a ConvLSTM-Based Model. CVPR Workshops, 2022.

 [3] Kladny, Milanta, Mraz, Hufkens and Stocker. Deep learning for satellite image forecasting of vegetation greenness. bioRxiv, 2022.

 [4] Gao, Shi, Wang, Zhu, Wang, Li and Yeung. Earthformer: Exploring Space-Time Transformers for Earth System Forecasting. NeurIPS, 2022.

How to cite: Benson, V., Requena-Mesa, C., Robin, C., Alonso, L., Carvalhais, N., and Reichstein, M.: Modeling landscape-scale vegetation response to climate: Synthesis of the EarthNet challenge, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9337, https://doi.org/10.5194/egusphere-egu23-9337, 2023.

EGU23-9434 | ECS | Posters on site | ITS1.14/CL5.8

Enhancing environmental sensor data quality control with graph neural networks 

Elżbieta Lasota, Julius Polz, Christian Chwala, Lennart Schmidt, Peter Lünenschloß, David Schäfer, and Jan Bumberger

The rapidly growing number of low-cost environmental sensors and data from opportunistic sensors constantly advances the quality as well as the spatial and temporal resolution of weather and climate models. However, it also leads to the need for effective tools to ensure the quality of collected data.

Time series quality control (QC) from multiple spatial, irregularly distributed sensors is a challenging task, as it requires the simultaneous integration and analysis of observations from sparse neighboring sensors and consecutive time steps. Manual QC is very often time- and labour- expensive and requires expert knowledge, which introduces subjectivity and limits reproducibility. Therefore, automatic, accurate, and robust QC solutions are in high demand, where among them one can distinguish machine learning techniques. 

In this study, we present a novel approach for the quality control of time series data from multiple spatial, irregularly distributed sensors using graph neural networks (GNNs). Although we applied our method to commercial microwave link attenuation data collected from a network in Germany between April and October 2021, our solution aims to be generic with respect to the number and type of sensors, The proposed approach involves the use of an autoencoder architecture, where the GNN is used to model the spatial relationships between the sensors, allowing for the incorporation of contextual information in the quality control process. 

While our model shows promising results in initial tests, further research is needed to fully evaluate its effectiveness and to demonstrate its potential in a wider range of environmental applications. Eventually, our solution will allow us to further foster the observational basis of our understanding of the natural environment.

How to cite: Lasota, E., Polz, J., Chwala, C., Schmidt, L., Lünenschloß, P., Schäfer, D., and Bumberger, J.: Enhancing environmental sensor data quality control with graph neural networks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9434, https://doi.org/10.5194/egusphere-egu23-9434, 2023.

EGU23-9810 | ECS | Orals | ITS1.14/CL5.8

Integration of a deep-learning-based fire model into a global land surface model 

Rackhun Son, Nuno Carvalhais, Lazaro Silva, Christian Requena-Mesa, Ulrich Weber, Veronika Gayler, Tobias Stacke, Reiner Schnur, Julia Nabel, Alexander Winkler, and Sönke Zaehle

Fire is an ubiquitous process within the Earth system that has significant impacts in terrestrial ecosystems. Process-based fire models quantify fire disturbance effects in stand-alone dynamic global vegetation models (DGVMs) and within coupled Earth system models (ESMs), and their advances have incorporated both descriptions of natural processes and anthropogenic drivers. However, we still observe a limited skill in modeling and predicting fire at global scale, mostly due to the stochastic nature of fire, but also due to the limits in empirical parameterizations in these process-based models. As an alternative, statistical approaches have shown the advantages of machine learning in providing robust diagnostics of fire damages, though with limited value for process-based modeling frameworks. Here, we develop a deep-learning-based fire model (DL-fire) to estimate gridded burned area fraction at global scale and couple it within JSBACH4, the land surface model used in the ICON ESM. We compare the resulting hybrid model integrating DL-fire into JSBACH4 (JDL-fire) against the standard fire model within JSBACH4 and the stand-alone DL-fire results. The stand-alone DL-fire model forced with observations shows high performance in simulating global burnt fraction, showing a monthly correlation (Rm) with the Global Fire Emissions Database (GFED4) of 0.78 and of 0.8 at global scale during the training (2004-10) and validation periods (2011-15), respectively. The performance remains nearly the same when evaluating the hybrid modeling approach JDL-fire (Rm=0.76 and 0.86 in training and evaluation periods, respectively). This outperforms the currently used standard fire model in JSBACH4 (Rm=-0.16 and 0.22 in training and evaluation periods, respectively) by far. We further evaluate the modeling results across specific fire regions and apply layer-wise relevance propagation (LRP) to quantify importance of each predictor. Overall, land properties, such as fuel amount and water contents in soil layers, stand out as the major factors determining burnt fraction in DL-fire, paralleled by meteorological conditions, over tropical and high latitude regions. Our study demonstrates the potential of hybrid modeling in advancing the predictability of Earth system processes by integrating statistical learning approaches in physics-based dynamical systems.

How to cite: Son, R., Carvalhais, N., Silva, L., Requena-Mesa, C., Weber, U., Gayler, V., Stacke, T., Schnur, R., Nabel, J., Winkler, A., and Zaehle, S.: Integration of a deep-learning-based fire model into a global land surface model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9810, https://doi.org/10.5194/egusphere-egu23-9810, 2023.

EGU23-10219 | ECS | Posters on site | ITS1.14/CL5.8

Identifying compound weather prototypes of forest mortality with β-VAE 

Mohit Anand, Friedrich Bohn, Lily-belle Sweet, Gustau Camps-Valls, and Jakob Zscheischler

Forest health is affected by many interacting and correlated weather variables over multiple temporal scales. Climate change affects weather conditions and their dependencies. To better understand future forest health and status, an improved scientific  understanding of the complex relationships between weather conditions and forest mortality is required. Explainable AI (XAI) methods are increasingly used to understand and simulate physical processes in complex environments given enough data. In this work, an hourly weather generator (AWE-GEN) is used  to simulate 200,000 years of daily weather conditions representative of central Germany. It is capable of simulating low and high-frequency characteristics of weather variables and also captures the inter-annual variability of precipitation. These data are then used to drive an individual-based forest model (FORMIND) to simulate the dynamics of a beech, pine, and spruce forest. A variational autoencoder β-VAE is used to learn representations of the generated weather conditions, which include radiation, precipitation and temperature. We learn shared and specific variable latent representations using a decoder network which remains the same for all the weather variables. The representation learning is completely unsupervised. Using the output of the forest model, we identify single and compounding weather prototypes that are associated with extreme forest mortality. We find that the prototypes associated with extreme mortality are similar for pine and spruce forests and slightly different for beech forests. Furthermore, although the compounding weather prototypes represent a larger sample size (2.4%-3.5%) than the single prototypes (1.7%-2.2%), they are associated with higher levels of mortality on average. Overall, our research illustrates how deep learning frameworks can be used to identify weather patterns that are associated with extreme impacts.

 

How to cite: Anand, M., Bohn, F., Sweet, L., Camps-Valls, G., and Zscheischler, J.: Identifying compound weather prototypes of forest mortality with β-VAE, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10219, https://doi.org/10.5194/egusphere-egu23-10219, 2023.

Hydrological models and machine learning models are widely used in streamflow simulation and data reconstruction. However, a global assessment of these models is still lacking and no synthesized catchment-scale streamflow product derived from multiple models is available over the globe. In this study, we comprehensively evaluated four conceptual hydrological models (GR2M, XAJ, SAC, Alpine) and four machine learning models (RF, GBDT, DNN, CNN) based on the selected 16,218 gauging stations worldwide, and then applied multi-model weighting ensemble (MWE) method to merge streamflow simulated from these models. Generally, the average performance of the machine learning model for all stations is better than that of the hydrological model, and with more stations having a quantified simulation accuracy (KGE>0.2); However, the hydrological model achieves a higher percentage of stations with a good simulation accuracy (KGE>0.6). Specifically, for the average accuracy during the validation period, there are 67% (27%) and 74% (21%) of stations showed a “quantified” (“good”) level for the hydrological models and machine learning models, respectively. The XAJ is the best-performing model of the four hydrological models, particularly in tropical and temperate zones. Among the machine learning models, the GBDT model shows better performance on the global scale. The MWE can effectively improve the simulation accuracy and perform much better than the traditional multi-model arithmetic ensemble (MAE), especially for the constrained least squares prediction combination method (CLS) with 82% (28%) of the stations having a “qualified” (“good”) accuracy. Furthermore, by exploring the influencing factors of the streamflow simulation, we found that both machine-learning models and hydrological models perform better in wetter areas.

How to cite: Zhang, J. and Liu, J.: Simulation and reconstruction of global monthly runoff based on hydrological models and machine learning models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10391, https://doi.org/10.5194/egusphere-egu23-10391, 2023.

Physical process-based numerical prediction models (NWPs) and radar-based probabilistic methods have been mainly used for short-term precipitation prediction. Recently, radar-based precipitation nowcasting models using advanced machine learning (ML) have been actively developed. Although the ML-based model shows outstanding performance in short-term rainfall prediction, it significantly decreases performance due to increased lead time. It has the limitation of being a black box model that does not consider the physical process of the atmosphere. To address these limitations, we aimed to develop a hybrid precipitation nowcasting model, which combines NWP and an advanced ML-based model via an ML-based ensemble method. The Weather Research and Forecasting (WRF) model was used as NWP to generate a physics-based rainfall forecast. In this study, we developed the ML-based precipitation nowcasting model with conditional Generative Adversarial Network (cGAN), which shows high performance in the image generation tasks. The radar reflectivity data, WRF hindcast meteorological outputs (e.g., temperature and wind speed), and static information of the target basin (e.g., DEM, Land cover) were used as input data of cGAN-based model to generate physics-informed rainfall prediction at the lead time up to 6 hours. The cGAN-based model was trained with the data for the summer season of 2014-2017. In addition, we proposed an ML-based blending method, i.e., XGBoost, that combines cGAN-based model results and WRF forecast results. To evaluate the hybrid model performance, we analyzed the performance of precipitation predictions on three heavy rain events in South Korea. The results confirmed that using the blending method to develop a hybrid model could provide an improved precipitation nowcasting approach.

 

Acknowledgements

 This work was supported by a grant from the National Research Foundation of Korea funded by the Ministry of Science, ICT & Future Planning (2020R1A2C2007670).

How to cite: Choi, S. and Kim, Y.: Developing hybrid precipitation nowcasting model with WRF and conditional GAN-based model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10431, https://doi.org/10.5194/egusphere-egu23-10431, 2023.

EGU23-10568 | ECS | Orals | ITS1.14/CL5.8

Extended-range predictability of stratospheric extreme events using explainable neural networks 

Zheng Wu, Tom Beucler, and Daniela Domeisen

Extreme stratospheric events such as extremely weak vortex events and strong vortex events can influence weather in the troposphere from weeks to months and thus are important sources of predictability of tropospheric weather on subseasonal to seasonal (S2S) timescales. However, the predictability of weak vortex events is limited to 1-2 weeks in state-of-the-art forecasting systems, while strong vortex events are more predictable than weak vortex events. Longer predictability timescales of the stratospheric extreme events would benefit long-range surface weather prediction. Recent studies showed promising results in the use of machine learning for improving weather prediction. The goal of this study is to explore the potential of a machine learning approach in extending the predictability of stratospheric extreme events in S2S timescales. We use neural networks (NNs) to predict the monthly stratospheric polar vortex strength with lead times up to five months using the first five principal components (PCs) of the sea surface temperature (SST), mean sea level pressure (MSLP), Barents–Kara sea-ice concentration (BK-SIC), poleward heat flux at 100 hPa, and zonal wind at 50, 30, and 2 hPa as precursors. These physical variables are chosen as they are indicated as potential precursors for the stratospheric extremes in previous studies. The results show that the accuracy and Brier Skill Score decrease with longer lead times and the performance is similar between weak and strong vortex events. We then employ two different NN attribution methods to uncover feature importance (heat map) in the inputs for the NNs, which indicates the relevance of each input for NNs to make the prediction. The heat maps suggest that precursors from the lower stratosphere are important for the prediction of the stratospheric polar vortex strength with a lead time of one month while the precursors at the surface and the upper stratosphere become more important with lead times longer than one month. This result is overall consistent with the previous studies that subseasonal precursors to the stratospheric extreme events may come from the lower troposphere. Our study sheds light on the potential of explainable NNs in searching for opportunities for skillful prediction of stratospheric extreme events and, by extension, surface weather on S2S timescales.

How to cite: Wu, Z., Beucler, T., and Domeisen, D.: Extended-range predictability of stratospheric extreme events using explainable neural networks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10568, https://doi.org/10.5194/egusphere-egu23-10568, 2023.

One of the main challenges for forecasting fire activity is the tradeoff between accuracy at finer spatial scales relevant to local decision making and predictability over seasonal (next 2-4 months) and subseasonal-to-seasonal (next 2 weeks to 2 months) timescales. To achieve predictability at long lead times and high spatial resolution, several analyses in the literature have constructed statistical models of fire activity using only antecedent climate predictors. However, in this talk, I will present preliminary seasonal forecasts of wildfire frequency and burned area for the western United States using SMLFire1.0, a stochastic machine learning (SML) fire model, that relies on both observed antecedent climate and vegetation predictors and seasonal forecasts of fire month climate. In particular, I will discuss results obtained by forcing the SMLFire1.0 model with seasonal forecasts from: a) downscaled and bias-corrected North American Multi-Model Ensemble (NMME) outputs, and b) skill-weighted climate analogs constructed using an autoregressive ML model. I will also comment upon the relative contribution of uncertainties, from climate forecasts and fire model simulations respectively, in projections of wildfire frequency and burned area across several spatial scales and lead times. 

How to cite: Buch, J., Williams, A. P., and Gentine, P.: Seasonal forecasts of wildfire frequency and burned area in the western United States using a stochastic machine learning fire model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11238, https://doi.org/10.5194/egusphere-egu23-11238, 2023.

EGU23-11355 | Posters on site | ITS1.14/CL5.8

Estimation of Fine Dust Concentration from BGR Images in Surveillance Cameras 

Hoyoung Cha, Jongyun Byun, Jongjin Baik, and Changhyun Jun

  This study proposes a novel approach on estimation of fine dust concentration from raw video data recorded by surveillance cameras. At first, several regions of interest are defined from specific images extracted from videos in surveillance cameras installed at Chung-Ang University. Among them, sky fields are mainly considered to figure out changes in characteristics of each color. After converting RGB images into BGR images, a number of discrete pixels with brightness intensities in a blue channel is mainly analyzed by investigating any relationships with fine dust concentration measured from automatic monitoring stations near the campus. Here, different values of thresholds from 125 to 200 are considered to find optimal conditions from changes in values of each pixel in the blue channel. This study uses the Pearson correlation coefficient to calculate the correlation between the number of pixels with values over the selected threshold and observed data for fine dust concentration. As an example on one specific date, the coefficients reflect their positive correlations with a range from 0.57 to 0.89 for each threshold. It should be noted that this study is a novel attempt to suggest a new, simple, and efficient method for estimating fine dust concentration from surveillance cameras common in many areas around the world.

 

Keywords: Fine Dust Concentration, BGR Image, Surveillance Camera, Threshold, Correlation Analysis

 

Acknowledgment

  This work was supported by the National Research Foundation of Korea(NRF) grant funded by the Korea government(MSIT) (No. NRF-2022R1A4A3032838) and this work was funded by the Korea Meteorological Administration Research and Development Program under Grant KMI2022-01910 and this work was supported by the National Research Foundation of Korea(NRF) grant funded by the Korea government(MSIT) (2020R1G1A1013624).

How to cite: Cha, H., Byun, J., Baik, J., and Jun, C.: Estimation of Fine Dust Concentration from BGR Images in Surveillance Cameras, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11355, https://doi.org/10.5194/egusphere-egu23-11355, 2023.

EGU23-12137 | ECS | Posters on site | ITS1.14/CL5.8

Identifying mechanisms of low-level jets near coast of Kurzeme using Principal Component Analysis 

Maksims Pogumirskis, Tija Sīle, and Uldis Bethers

Low-level jets are maximums in the vertical profile of the wind speed profile in the lowest levels of atmosphere. Low-level jets, when present, can make a significant impact on the wind energy. Wind conditions in low-level jets depart from traditional assumptions about wind profile and low-level jets can also influence the stability and turbulence that are important for wind energy applications.

In literature commonly an algorithm of identifying low-level jets is used to estimate frequency of low-level jets. The algorithm searches for maximum in the lowest levels of the atmosphere with a temperature inversion above the jet maximum. The algorithm is useful in identifying the presence of the low-level jets and estimating their frequency. However, low-level jets can be caused by a number of different mechanisms which leads to differences in low-level jet characteristics. Therefore, additional analysis is necessary to distinguish between different types of jets and characterize their properties. We aim to automate this process using Principal Component Analysis (PCA) to identify main patterns of wind speed and temperature. By analyzing diurnal and seasonal cycles of these patterns a better understanding about climatology of low-level jets in the region can be gained.

This study focuses on the central part of the Baltic Sea. Several recent studies have identified the presence of low-level jets near the coast of Kurzeme. Typically, maximums of low-level jets are located several hundred meters above the surface, while near the coast of Kurzeme maximums of low-level jets are usually within the lowest 100 meters of the atmosphere.

Data from UERRA reanalysis with 11 km horizontal resolution on 12 height levels in the lowest 500 meters of atmosphere was used. The algorithm that identifies low-level jets was applied to the data, to estimate frequency of low-level jets in each grid cell of the model. Jet events were grouped by the wind direction to identify main trajectories of low-level jets in the region. Several atmosphere cross-sections that low-level jets frequently flow through were chosen for further analysis.

Model data was interpolated to the chosen cross-sections and PCA was applied to the cross-section data of wind speed, geostrophic wind speed and temperature. Main patterns of these meteorological parameters, such as wind speed maximum, temperature inversion above the surface of the sea and temperature difference between sea and land were identified by the PCA. Differences of principal components between cross-sections and diurnal and seasonal patterns of principal components helped to gain better understanding of climatology, extent and mechanisms of low-level jets in the region.

How to cite: Pogumirskis, M., Sīle, T., and Bethers, U.: Identifying mechanisms of low-level jets near coast of Kurzeme using Principal Component Analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12137, https://doi.org/10.5194/egusphere-egu23-12137, 2023.

EGU23-12528 | ECS | Orals | ITS1.14/CL5.8

Evaluation of explainable AI solutions in climate science 

Philine Bommer, Marlene Kretschmer, Anna Hedstroem, Dilyara Bareeva, and Marina M.-C. Hoehne

Explainable artificial intelligence (XAI) methods serve as a support for researchers to shed light onto the reasons behind the predictions made by deep neural networks (DNNs). XAI methods have already been successfully applied to climate science, revealing underlying physical mechanisms inherent in the studied data. However, the evaluation and validation of XAI performance is challenging as explanation methods often lack ground truth. As the number of XAI methods is growing, a comprehensive evaluation is necessary to enable well-founded XAI application in climate science.

In this work we introduce explanation evaluation in the context of climate research. We apply XAI evaluation to compare multiple explanation methods for a multi-layer percepton (MLP) and a convolutional neural network (CNN). Both MLP and CNN assign temperature maps to classes based on their decade. We assess the respective explanation methods using evaluation metrics measuring robustness, faithfulness, randomization, complexity and localization. Based on the results of a random baseline test we establish an explanation evaluation guideline for the climate community. We use this guideline to rank the performance in each property of similar sets of explanation methods for the MLP and CNN. Independent of the network type, we find that Integrated Gradients, Layer-wise relevance propagation and InputGradients exhibit a higher robustness, faithfulness and complexity compared to purely Gradient-based methods, while sacrificing reactivity to network parameters, i.e. low randomisation scores. The contrary holds for Gradient, SmoothGrad, NoiseGrad and FusionGrad. Another key observation is that explanations using input perturbations, such as SmoothGrad and Integrated Gradients, do not improve robustness and faithfulness, in contrast to theoretical claims. Our experiments highlight that XAI evaluation can be applied to different network tasks and offers more detailed information about different properties of explanation method than previous research. We demonstrate that using XAI evaluation helps to tackle the challenge of choosing an explanation method.

How to cite: Bommer, P., Kretschmer, M., Hedstroem, A., Bareeva, D., and Hoehne, M. M.-C.: Evaluation of explainable AI solutions in climate science, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12528, https://doi.org/10.5194/egusphere-egu23-12528, 2023.

EGU23-12657 | Orals | ITS1.14/CL5.8 | Highlight

DeepExtremes: Explainable Earth Surface Forecasting Under Extreme Climate Conditions 

Karin Mora, Gunnar Brandt, Vitus Benson, Carsten Brockmann, Gustau Camps-Valls, Miguel-Ángel Fernández-Torres, Tonio Fincke, Norman Fomferra, Fabian Gans, Maria Gonzalez, Chaonan Ji, Guido Kraemer, Eva Sevillano Marco, David Montero, Markus Reichstein, Christian Requena-Mesa, Oscar José Pellicer Valero, Mélanie Weynants, Sebastian Wieneke, and Miguel D. Mahecha

Compound heat waves and drought events draw our particular attention as they become more frequent. Co-occurring extreme events often exacerbate impacts on ecosystems and can induce a cascade of detrimental consequences. However, the research to understand these events is still in its infancy. DeepExtremes is a project funded by the European Space Agency (https://rsc4earth.de/project/deepextremes/) aiming at using deep learning to gain insight into Earth surface under extreme climate conditions. Specifically, the goal is to forecast and explain extreme, multi-hazard, and compound events. To this end, the project leverages the existing Earth observation archive to help us better understand and represent different types of hazards and their effects on society and vegetation. The project implementation involves a multi-stage process consisting of 1) global event detection; 2) intelligent subsampling and creation of mini-data-cubes; 3) forecasting methods development, interpretation, and testing; and 4) cloud deployment and upscaling. The data products will be made available to the community following the reproducibility and FAIR data principles. By effectively combining Earth system science with explainable AI, the project contributes knowledge to advancing the sustainable management of consequences of extreme events. This presentation will show the progress made so far and specifically introduce how to participate in the challenges about spatio-temporal extreme event prediction in DeepExtremes.

How to cite: Mora, K., Brandt, G., Benson, V., Brockmann, C., Camps-Valls, G., Fernández-Torres, M.-Á., Fincke, T., Fomferra, N., Gans, F., Gonzalez, M., Ji, C., Kraemer, G., Marco, E. S., Montero, D., Reichstein, M., Requena-Mesa, C., Valero, O. J. P., Weynants, M., Wieneke, S., and Mahecha, M. D.: DeepExtremes: Explainable Earth Surface Forecasting Under Extreme Climate Conditions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12657, https://doi.org/10.5194/egusphere-egu23-12657, 2023.

EGU23-12889 | Orals | ITS1.14/CL5.8

New Berkeley Earth High Resolution Temperature Data Set 

Robert A. Rohde and Zeke Hausfather

Berkeley Earth is premiering a new high resolution analysis of historical instrumental temperatures.

This builds on our existing work on climate reconstruction by adding a simple machine learning layer to our analysis.  This new approach extracts weather patterns from model, satellite, and reanalysis data, and then layers these weather patterns on top of instrumental observations and our existing interpolation methods to produce new high resolution historical temperature fields.  This has quadrupled our output resolution from the previous 1° x 1° lat-long to a new global 0.25° x 0.25° lat-long resolution.  However, this is not simply a downscaling effort.  Firstly, the use of weather patterns derived from physical models and observations increases the spatial realism of the reconstructed fields.  Secondly, observations from regions with high density measurement networks have been directly incorporated into the high resolution field, allowing dense observations to be more fully utilized.  

This new data product uses significantly more observational weather station data and produces higher resolution historical temperature fields than any comparable product, allowing for unprecedented insights into historical local and regional climate change.  In particular, the effect of geographic features such as mountains, coastlines, and ecosystem variations are resolved with a level of detail that was not previously possible.  At the same time, previously established techniques for bias corrections, noise reduction, and error analysis continued to be utilized.  The resulting global field initially spans 1850 to present and will be updated on an ongoing basis.  This project does not significantly change the global understanding of climate change, but helps to provide local detail that was often unresolved previously.  The initial data product focuses on monthly temperatures, though a proposal exists to also create a high resolution daily temperature data set using similar methods.

This talk will describe the construction of the new data set and its characteristics.  The techniques used in this project are accessible enough that they are likely to be useful for other types of instrumental analyses wishing to improve resolution or leverage basic information about weather patterns derived from models or other sources.

How to cite: Rohde, R. A. and Hausfather, Z.: New Berkeley Earth High Resolution Temperature Data Set, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12889, https://doi.org/10.5194/egusphere-egu23-12889, 2023.

EGU23-12948 | ECS | Orals | ITS1.14/CL5.8

Identifying drivers of river floods using causal inference 

Peter Miersch, Shijie Jiang, Oldrich Rakovec, and Jakob Zscheischler

River floods are among the most devastating natural hazards, causing thousands of deaths and billions of euros in damages every year. Floods can result from a combination of compounding drivers such as heavy precipitation, snowmelt, and high antecedent soil moisture. These drivers and the processes they govern vary widely both between catchments and between flood events within a catchment, making a causal understanding of the underlying hydrological processes difficult.

Modern causal inference methods, such as the PCMCI framework, are able to identify drivers from complex time series through causal discovery and build causally aware statistical models. However, causal inference tailored to extreme events remains a challenge due to data length limitations. To overcome data limitations, here we bridge the gap between synthetic and real world data using 1,000 years of simulated weather to drive as state-of-the-art hydrological model (the mesoscale Hydrological Model, mHM) over a wide range of European catchments. From the simulated time series, we extract high runoff events, on which we evaluate the causal inference approach. We identify the minimum data necessary for obtaining robust causal models, evaluate metrics for model evaluation and comparison, and compare causal flood drivers across catchments. Ultimately, this work will help establish best practices in causal inference for flood research to identify meteorological and catchment specific flood drivers in a changing climate.

How to cite: Miersch, P., Jiang, S., Rakovec, O., and Zscheischler, J.: Identifying drivers of river floods using causal inference, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12948, https://doi.org/10.5194/egusphere-egu23-12948, 2023.

EGU23-13250 | ECS | Posters on site | ITS1.14/CL5.8

From MODIS cloud properties to cloud types using semi-supervised learning 

Julien Lenhardt, Johannes Quaas, and Dino Sejdinovic

Clouds are classified into types, classes, or regimes. The World Meteorological Organization distinguishes stratus and cumulus clouds and three altitude layers. Cloud types exhibit very different radiative properties and interact in numerous ways with aerosol particles in the atmosphere. However, it has proven difficult to define cloud regimes objectively and from remote sensing data, hindering the understanding we have of the processes and adjustments involved.

Building on the method we previously developed, we combine synoptic observations and passive satellite remote-sensing retrievals to constitute a database of cloud types and cloud properties to eventually train a cloud classification algorithm. The cloud type labels come from the global marine meteorological observations dataset (UK Met Office, 2006) which is comprised of near-global synoptic observations. This data record reports back information about cloud type and other meteorological quantities at the surface. The cloud classification model is built on different cloud-top and cloud optical properties (Level 2 products MOD06/MYD06 from the MODIS sensor) extracted temporally close to the observation time and on a 128km x 128km grid around the synoptic observation location. To make full use of the large quantity of remote sensing data available and to investigate the variety in cloud settings, a convolutional variational auto-encoder (VAE) is applied as a dimensionality reduction tool in a first step. Furthermore, such model architecture allows to account for spatial relationships while describing non-linear patterns in the input data. The cloud classification task is subsequently performed drawing on the constructed latent representation of the VAE. Associating information from underneath and above the cloud enables to build a robust model to classify cloud types. For the training we specify a study domain in the Atlantic ocean around the equator and evaluate the method globally. Further experiments and evaluation are done on simulation data produced by the ICON model.

How to cite: Lenhardt, J., Quaas, J., and Sejdinovic, D.: From MODIS cloud properties to cloud types using semi-supervised learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13250, https://doi.org/10.5194/egusphere-egu23-13250, 2023.

EGU23-13462 | ECS | Orals | ITS1.14/CL5.8

Double machine learning for geosciences 

Kai-Hendrik Cohrs, Gherardo Varando, Markus Reichstein, and Gustau Camps-Valls

Hybrid modeling describes the synergy between parametric models and machine learning [1]. Parts of a parametric equation are substituted by non-parametric machine learning models, which can then represent complex functions. These are inferred together with the parameters of the equation from the data. Hybrid modeling promises to describe complex relationships and to be scientifically interpretable. These promises, however, need to be taken with a grain of salt. With too flexible models, such as deep neural networks, the problem of equifinality arises: There is no identifiable optimal solution. Instead, many outcomes describe the data equally well, and we will obtain one of them by chance. Interpreting the result may lead to erroneous conclusions. Moreover, studies have shown that regularization techniques can introduce a bias on jointly estimated physical parameters [1].

We propose double machine learning (DML) to solve these problems [2]. DML is a theoretically well-founded technique for fitting semi-parametric models, i.e., models consisting of a parametric and a non-parametric component. DML is widely used for debiased treatment effect estimation in economics. We showcase its use for geosciences on two problems related to carbon dioxide fluxes: 

  • Flux partitioning, which aims at separating the net carbon flux (NEE) into its main contributing gross fluxes, namely, RECO and GPP.
  • Estimation of the temperature sensitivity parameter of ecosystem respiration Q10.

First, we show that in the case of synthetic data for Q10 estimation, we can consistently retrieve the true value of Q10 where the naive neural network approach fails. We further apply DML to the carbon flux partitioning problem and find that it is 1) able to retrieve the true fluxes of synthetic data, even in the presence of strong (and more realistic) heteroscedastic noise, 2) retrieves main gross carbon fluxes on real data consistent with established methods, and 3) allows us to causally interpret the retrieved GPP as the direct effect of the photosynthetically active radiation on NEE. This way, the DML approach can be seen as a causally interpretable, semi-parametric version of the established daytime methods. We also investigate the functional relationships inferred with DML and the drivers modulating the obtained light-use efficiency function. In conclusion, DML offers a solid framework to develop hybrid and semiparametric modeling and can be of widespread use in geosciences.

 

[1] Reichstein, Markus, et al. “Combining system modeling and machine learning into hybrid ecosystem modeling.” Knowledge-Guided Machine Learning (2022). https://doi.org/10.1201/9781003143376-14

[2] Chernozhukov, Victor, et al. “Double/debiased machine learning for treatment and structural parameters.” The Econometrics Journal, Volume 21, Issue 1, 1 (2018): C1–C68. https://doi.org/10.1111/ectj.12097

How to cite: Cohrs, K.-H., Varando, G., Reichstein, M., and Camps-Valls, G.: Double machine learning for geosciences, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13462, https://doi.org/10.5194/egusphere-egu23-13462, 2023.

EGU23-13622 | ECS | Posters on site | ITS1.14/CL5.8

Towards explainable marine heatwaves forecasts 

Ayush Prasad and Swarnalee Mazumder

In recent years, both the intensity and extent of marine heatwaves have increased across the world. Anomalies in sea surface temperature have an effect on the health of marine ecosystems, which are crucial to the Earth's climate system. Marine Heatwaves' devastating impacts on aquatic life have been increasing steadily in recent years, harming aquatic ecosystems and causing a tremendous loss of marine life. Early warning systems and operational forecasting that can foresee such events can aid in designing effective and better mitigation techniques. Recent studies have shown that machine learning and deep learning-based approaches can be used for forecasting the occurrence of marine heatwaves up to a year in advance. However, these models are black box in nature and do not provide an understanding of the factors influencing MHWs. In this study, we used machine learning methods to forecast marine heatwaves. The developed models were tested across four historical Marine Heatwave events around the world. Explainable AI methods were then used to understand and analyze the relationships between the drivers of these events.

How to cite: Prasad, A. and Mazumder, S.: Towards explainable marine heatwaves forecasts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13622, https://doi.org/10.5194/egusphere-egu23-13622, 2023.

EGU23-14493 | ECS | Orals | ITS1.14/CL5.8

Interpretable probabilistic forecast of extreme heat waves 

Alessandro Lovo, Corentin Herbert, and Freddy Bouchet
Understanding and predicting extreme events is one of the major challenges for the study of climate change impacts, risk assessment, adaptation, and the protection of living beings. Extreme heatwaves are, and likely will be in the future, among the deadliest weather events. They also increase strain on water resources, food security and energy supply. Developing the ability to forecast their probability of occurrence a few days, weeks, or even months in advance would have major consequences to reduce our vulnerability to these events. Beyond the practical benefits of forecasting heat waves, building statistical models for extreme events which are interpretable is also highly beneficial from a fundamental point of view. Indeed, they enable proper studies of the processes underlying extreme events such as heat waves, improve dataset or model validation, and contribute to attribution studies. Machine learning provides tools to reach both these goals.
We will first demonstrate that deep neural networks can predict the probability of occurrence of long-lasting 14-day heatwaves over France, up to 15 days ahead of time for fast dynamical drivers (500 hPa geopotential height field), and at much longer lead times for slow physical drivers (soil moisture). Those results are amazing in terms of forecasting skill. However, these machine learning models tend to be very complex and are often treated as black boxes. This limits our ability to use them for investigating the dynamics of extreme heat waves.
To gain physical understanding, we have then designed a network architecture which is intrinsically interpretable. The main idea of this architecture is that the network first computes an optimal index, which is an optimal projection of the physical fields in a low-dimensional space. In a second step, it uses a fully non-linear representation of the probability of occurrence of the event as a function of the optimal index. This optimal index can be visualized and compared with classical heuristic understanding of the physical process, for instance in terms of geopotential height and soil moisture. This fully interpretable network is slightly less efficient than the off-the-shelf deep neural network. We fully quantify the performance loss incurred when requiring interpretability and make the connection with the mathematical notion of committor functions.
This new machine learning tool opens the way for understanding optimal predictors of weather and climate extremes. This has potential for the study of slow drivers, and the effect of climate change on the drivers of extreme events.

How to cite: Lovo, A., Herbert, C., and Bouchet, F.: Interpretable probabilistic forecast of extreme heat waves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14493, https://doi.org/10.5194/egusphere-egu23-14493, 2023.

EGU23-14856 | ECS | Orals | ITS1.14/CL5.8

Classification of Indoor Air Pollution Using Low-cost Sensors by Machine Learning 

Andrii Antonenko, Viacheslav Boretskij, and Oleksandr Zagaria

Air pollution has become an integral part of modern life. The main source of air pollution can be considered combustion processes associated with energy-intensive corporate activities. Energy companies consume about one-third of the fuel produced and are a significant source of air pollution [1]. State and public air quality monitoring networks were created to monitor the situation. Public monitoring networks are cheaper and have more coverage than government ones. Although the state monitoring system shows more accurate data, an inexpensive network is sufficient to inform the public about the presence or absence of pollution (air quality). In order to inform the public, the idea arose to test the possibility of detecting types of pollution using data from cheap air quality monitoring sensors. In general, to use a cheap sensor for measurements, it must first be calibrated (corrected) by comparing its readings with a reference device. Various mathematical methods can be used for this. One of such method is neural network training, which has proven itself well for correcting PM particle readings due to relative humidity impact [2].

The idea of using a neural network to improve data quality is not new, but it is quite promising, as the authors showed in [3]. The main problem to implement this method is connected with a reliable dataset for training the network. For this, it is necessary to register sensor readings for relatively clean air and for artificially generated or known sources of pollution. Training the neural network on the basis of collected data can be used to determine (classify) types of air: with pollution (pollutant) or without. For this, an experiment was set up in the "ReLab" co-working space at the Taras Shevchenko National University of Kyiv. The sensors were placed in a closed box, in which airflow ventilation is provided. The ZPHS01B [4] sensor module was used for inbox measurements, as well as, calibrated sensors PMS7003 [5] and BME280 [6]. Additionally, IPS 7100 [7] and SPS30 [8] were added to enrich the database for ML training. A platform based on HiLink 7688 was used for data collecting, processing, and transmission.

Data was measured every two seconds, independently from each sensor. Before each experiment, the room was ventilated to avoid influence on the next series of experiments.

References

1. Zaporozhets A. Analysis of means for monitoring air pollution in the environment. Science-based technologies. 2017, Vol. 35, no3. 242-252. DOI: 10.18372/2310-5461.35.11844

2. Antonenko A, (2021) Correction of fine particle concentration readings depending on relative humidity, [Master's thesis, Taras Shevchenko National University of Kyiv], 35 pp.

3. Lee, J. Kang, S. Kim, Y. Im, S. Yoo , D. Lee, “Long-Term Evaluation and Calibration of Low-Cost Particulate Matter (PM) Sensor”, Sensors 2020, vol. 20, 3617, 24 pp., 2020.`

4. ZPHS01B Datasheet URL: https://pdf1.alldatasheet.com/datasheet-pdf/view/1303697/WINSEN/ZPHS01B.html

5. Plantower PMS7003 Datasheet URL: https://www.espruino.com/datasheets/PMS7003.pdf

6. Bosch 280 Datasheet URL: https://www.mouser.com/datasheet/2/783/BST-BME280-DS002-1509607.pdf

7. https://pierasystems.com/intelligent-particle-sensors/

8. https://sensirion.com/products/catalog/SPS30/

How to cite: Antonenko, A., Boretskij, V., and Zagaria, O.: Classification of Indoor Air Pollution Using Low-cost Sensors by Machine Learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14856, https://doi.org/10.5194/egusphere-egu23-14856, 2023.

EGU23-15000 | ECS | Orals | ITS1.14/CL5.8 | Highlight

Causal inference to study food insecurity in Africa 

Jordi Cerdà-Bautista, José María Tárraga, Gherardo Varando, Alberto Arribas, Ted Shepherd, and Gustau Camps-Valls

The current situation regarding food insecurity in the continent of Africa, and the Horn of Africa in particular, is at an unprecedented risk level triggered by continuous drought events, complicated interactions between food prices, crop yield, energy inflation and lack of humanitarian aid, along with disrupting conflicts and migration flows. The study of a food-secure environment is a complex, multivariate, multiscale, and non-linear problem difficult to understand with canonical data science methodologies. We propose an alternative approach to the food insecurity problem from a causal inference standpoint to discover the causal relations and evaluate the likelihood and potential consequences of specific interventions. In particular, we demonstrate the use of causal inference for understanding the impact of humanitarian interventions on food insecurity in Somalia. In the first stage of the problem, we apply different data transformations to the main drivers to achieve the highest degree of correlation with the interested variable. In the second stage, we infer causation from the main drivers and interested variables by applying different causal methods such as PCMCI or Granger causality. We analyze and harmonize different time series, per district of Somalia, of the global acute malnutrition (GAM) index, food market prices, crop production, conflict levels, drought and flood internal displacements, as well as climate indicators such as the NDVI index, precipitation or land surface temperature. Then, assuming a causal graph between the main drivers causing the food insecurity problem, we estimate the effect of increasing humanitarian interventions on the GAM index, considering the effects of a changing climate, migration flows, and conflict events. We show that causal estimation with modern methodologies allows us to quantify the impact of humanitarian aid on food insecurity.

 

References

 

[1] Runge, J., Bathiany, S., Bollt, E. et al. Inferring causation from time series in Earth system sciences. Nat Commun 10, 2553 (2019). https://doi.org/10.1038/s41467-019-10105-3

[2] Sazib Nazmus, Mladenova lliana E., Bolten John D., Assessing the Impact of ENSO on Agriculture Over Africa Using Earth Observation Data, Frontiers in Sustainable Food Systems, 2020, 10.3389/fsufs.2020.509914. https://www.frontiersin.org/article/10.3389/fsufs.2020.509914

[3] Checchi, F., Frison, S., Warsame, A. et al. Can we predict the burden of acute malnutrition in crisis-affected countries? Findings from Somalia and South Sudan. BMC Nutr 8, 92 (2022). https://doi.org/10.1186/s40795-022-00563-2

How to cite: Cerdà-Bautista, J., Tárraga, J. M., Varando, G., Arribas, A., Shepherd, T., and Camps-Valls, G.: Causal inference to study food insecurity in Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15000, https://doi.org/10.5194/egusphere-egu23-15000, 2023.

EGU23-15185 | ECS | Posters on site | ITS1.14/CL5.8

Deep learning to support ocean data quality control 

Mohamed Chouai, Felix Simon Reimers, and Sebastian Mieruch-Schnülle

In this study, which is part of the M-VRE [https://mosaic-vre.org/about] project, we aim to improve a quality control (QC) system on arctic ocean temperature profile data using deep learning. For the training, validation, and evaluation of our algorithms, we are using the UDASH dataset [https://essd.copernicus.org/articles/10/1119/2018/]. In the classical QC setting, the ocean expert or "operator", applies a series of thresholding (classical) algorithms to identify, i.e. flag, erroneous data. In the next step, the operator visually inspects every data profile, where suspicious samples have been identified. The goal of this time-consuming visual QC is to find "false positives", i.e. flagged data that is actually good, because every sample/profile has not only a scientific value but also a monetary one. Finally, the operator turns all "false positive" data back to good. The crucial point here is that although these samples/profiles are above certain thresholds they are considered good by the ocean expert. These human expert decisions are extremely difficult, if not impossible, to map by classical algorithms. However, deep-learning neural networks have the potential to learn complex human behavior. Therefore, we have trained a deep learning system to "learn" exactly the expert behavior of finding "false positives" (identified by the classic thresholds), which can be turned back to good accordingly. The first results are promising. In a fully automated setting, deep learning improves the results and fewer data are flagged. In a subsequent visual QC setting, deep learning relieves the expert with a distinct workload reduction and gives the option to clearly increase the quality of the data.
Our long-term goal is to develop an arctic quality control system as a series of web services and Jupyter notebooks to apply automated and visual QC online, efficient, consistent, reproducible, and interactively.

How to cite: Chouai, M., Simon Reimers, F., and Mieruch-Schnülle, S.: Deep learning to support ocean data quality control, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15185, https://doi.org/10.5194/egusphere-egu23-15185, 2023.

EGU23-15286 | ECS | Orals | ITS1.14/CL5.8

Spatio-temporal downscaling of precipitation data using a conditional generative adversarial network 

Luca Glawion, Julius Polz, Benjamin Fersch, Harald Kunstmann, and Christian Chwala

Natural disasters caused by cyclones, hail, landslides or floods are directly related to precipitation. Global climate models are an important tool to adapt to these hazards in a future climate. However, they operate on spatial and temporal discretizations that limit the ability to adequately reflect these fast evolving, highly localized phenomena which has led to the development of various downscaling approaches .

Conditional generative adversarial networks (cGAN) have recently been applied as a promising downscaling technique to improve the spatial resolution of climate data. The ability of GANs to generate ensembles of solutions from random perturbations can be used to account for the stochasticity of climate data and quantify uncertainties. 

We present a cGAN for not only downscaling the spatial, but simultaneously also the temporal dimension of precipitation data as a so-called video super resolution approach. 3D convolutional layers are exploited for extracting and generating temporally consistent  rain events with realistic fine-scale structure. We downscale coarsened gauge adjusted and climatology corrected precipitation data from Germany from a spatial resolution of 32 km to 2 km and a temporal resolution of 1 hr to 10 min, by applying a novel training routine using partly normalized and logarithmized data, allowing for improved extreme value statistics of the generated fields.

Exploiting the fully convolutional nature of our model we can generate downscaled maps for the whole of Germany in a single downscaling step at low latency. The evaluation of these maps using a spatial and temporal power spectrum analysis shows that the generated temporal and spatial structures are in high agreement with the reference. Visually, the generated temporally evolving and advecting rain events are hardly classifiable as artificial generated. The model also shows high skill regarding pixel-wise error and localization of high precipitation intensities, considering the FSS, CRPS, KS and RMSE. Due to the underdetermined downscaling problem a probabilistic cGAN approach yields additional information to deterministic models which we use for comparison. The method is also capable of preserving the climatology, e.g., expressed as the annual precipitation sum. Investigations of temporal aggregations of the downscaled fields revealed an interesting effect. We observe that structures generated in networks with convolutional layers are not placed completely at random, but can generate recurrent structures, which can also be discovered within other prominent DL downscaling models. Although they can be mitigated by adequate model selection, their occurrence remains an open research question.

We conclude that our proposed approach can extend the application of cGANs for downscaling to the time dimension and therefore is a promising candidate to supplement conventional downscaling methods due to the high performance and computational efficiency.

How to cite: Glawion, L., Polz, J., Fersch, B., Kunstmann, H., and Chwala, C.: Spatio-temporal downscaling of precipitation data using a conditional generative adversarial network, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15286, https://doi.org/10.5194/egusphere-egu23-15286, 2023.

EGU23-15540 | ECS | Posters on site | ITS1.14/CL5.8 | Highlight

USCC: A Benchmark Dataset for Crop Yield Prediction under Climate Extremes 

Adrian Höhl, Stella Ofori-Ampofo, Ivica Obadic, Miguel-Ángel Fernández-Torres, Ridvan Salih Kuzu, and Xiaoxiang Zhu

Climate variability and extremes are known to represent major causes for crop yield anomalies. They can lead to the reduction of crop productivity, which results in disruptions in food availability and nutritional quality, as well as in rising food prices. Extreme climates will become even more severe as global warming proceeds, challenging the achievement of food security. These extreme events, especially droughts and heat waves, are already evident in major food-production regions like the United States. Crops cultivated in this country such as corn and soybean are critical for both domestic use and international supply. Considering the sensitivity of crops to climate, here we present a dataset that couples remote sensing surface reflectances with climate variables (e.g. minimum and maximum temperature, precipitation, and vapor pressure) and extreme indicators. The dataset contains the crop yields of various commodities over the USA for nearly two decades. Given the advances and proven success of machine learning in numerous remote sensing tasks, our dataset constitutes a benchmark to advance the development of novel models for crop yield prediction, and to analyze the relationship between climate and crop yields for gaining scientific insights. Other potential use cases include extreme event detection and climate forecasting from satellite imagery. As a starting point, we evaluate the performance of several state-of-the-art machine and deep learning models to form a baseline for our benchmark dataset.

How to cite: Höhl, A., Ofori-Ampofo, S., Obadic, I., Fernández-Torres, M.-Á., Salih Kuzu, R., and Zhu, X.: USCC: A Benchmark Dataset for Crop Yield Prediction under Climate Extremes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15540, https://doi.org/10.5194/egusphere-egu23-15540, 2023.

EGU23-15817 | ECS | Posters on site | ITS1.14/CL5.8

Evaluating the generalization ability of a deep learning model trained to detect cloud-to-ground lightning on raw ERA5 data 

Gregor Ehrensperger, Tobias Hell, Georg Johann Mayr, and Thorsten Simon

Atmospheric conditions that are typical for lightning are commonly represented by proxies such as cloud top height, cloud ice flux, CAPE times precipitation, or the lightning potential index. While these proxies generally deliver reasonable results, they often need to be adapted for local conditions in order to perform well. This suggests that there is a need for more complex and holistic proxies. Recent research confirms that the use of machine learning (ML) approaches for describing lightning is promising.

In a previous study a deep learning model was trained on single spatiotemporal (30km x 30km x 1h) cells in the summer period of the years 2010--2018 and showed good results for the unseen test year 2019 within Austria. We now improve this model by using multiple neighboring vertical atmospheric columns to also address for horizontal moisture advection. Furthermore data of successive hours is used as input data to enable the model to capture the temporal development of atmospheric conditions such as the build-up and breakdown of convections.

In this work we focus on the summer months June to August and use data from parts of Central Europe. This spatial domain is thought to be representative for Continental Europe since it covers mountainous aswell as coastal regions. We take raw ERA5 parameters beyond the tropopause enriched with a small amount of meta data such as the day of the year and the hour of the day for training. The quality of the resulting paramaterized model is then evaluated on Continental Europe to examine the generalization ability.

Using parts of Central Europe to train the model, we evaluate its ability to generalize on unseen parts of Continental Europe using EUCLID data. Having a model that generalizes well is a building block for a retrospective analysis back into years where the structured recording of accurate lightning observations in a unified way was not established yet.

How to cite: Ehrensperger, G., Hell, T., Mayr, G. J., and Simon, T.: Evaluating the generalization ability of a deep learning model trained to detect cloud-to-ground lightning on raw ERA5 data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15817, https://doi.org/10.5194/egusphere-egu23-15817, 2023.

EGU23-16098 | Posters on site | ITS1.14/CL5.8

Identifying Lightning Processes in ERA5 Soundings with Deep Learning 

Tobias Hell, Gregor Ehrensperger, Georg J. Mayr, and Thorsten Simon

Atmospheric environments favorable for lightning and convection are commonly represented by proxies or parameterizations based on expert knowledge such as CAPE, wind shears, charge separation, or combinations thereof. Recent developments in the field of machine learning, high resolution reanalyses, and accurate lightning observations open possibilities for identifying tailored proxies without prior expert knowledge. To identify vertical profiles favorable for lightning, a deep neural network links ERA5 vertical profiles of cloud physics, mass field variables and wind to lightning location data from the Austrian Lightning Detection & Information System (ALDIS), which has been transformed to a binary target variable labelling the ERA5 cells as lightning and no lightning cells. The ERA5 parameters are taken on model levels beyond the tropopause forming an input layer of approx. 670 features. The data of 2010 - 2018 serve as training/validation. On independent test data, 2019, the deep network outperforms a reference with features based on meteorological expertise. Shapley values highlight the atmospheric processes learned by the network which identifies cloud ice and snow content in the upper and mid-troposphere as relevant features. As these patterns correspond to the separation of charge in thunderstorm cloud, the deep learning model can serve as physically meaningful description of lightning. 

How to cite: Hell, T., Ehrensperger, G., Mayr, G. J., and Simon, T.: Identifying Lightning Processes in ERA5 Soundings with Deep Learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16098, https://doi.org/10.5194/egusphere-egu23-16098, 2023.

EGU23-16163 | ECS | Posters on site | ITS1.14/CL5.8

A comparison of methods for determining the number of classes in unsupervised classification of climate models 

Emma Boland, Dani Jones, and Erin Atkinson

Unsupervised classification is becoming an increasingly common method to objectively identify coherent structures within both observed and modelled climate data. However, the user must choose the number of classes to fit in advance. Typically, a combination of statistical methods and expertise is used to choose the appropriate number of classes for a given study, however it may not be possible to identify a single ‘optimal’ number of classes. In this
work we present a heuristic method for determining the number of classes unambiguously for modelled data where more than one ensemble member is available. This method requires robustness in the class definition between simulated ensembles of the system of interest. For demonstration, we apply this to the clustering of Southern Ocean potential temperatures in a CMIP6 climate model, and compare with other common criteria such as Bayesian Information Criterion (BIC) and the Silhouette Score.

How to cite: Boland, E., Jones, D., and Atkinson, E.: A comparison of methods for determining the number of classes in unsupervised classification of climate models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16163, https://doi.org/10.5194/egusphere-egu23-16163, 2023.

EGU23-16186 | ECS | Posters on site | ITS1.14/CL5.8

A review of deep learning for weather prediction 

Jannik Thümmel, Martin Butz, and Bedartha Goswami

Recent years have seen substantial performance-improvements of deep-learning-based
weather prediction models (DLWPs). These models cover a large range of temporal and
spatial resolutions—from nowcasting to seasonal forecasting and on scales ranging from
single to hundreds of kilometers. DLWPs also exhibit a wide variety of neural architec-
tures and training schemes, with no clear consensus on best practices. Focusing on the
short-to-mid-term forecasting ranges, we review several recent, best-performing models
with respect to critical design choices. We emphasize the importance of self-organizing
latent representations and inductive biases in DLWPs: While NWPs are designed to sim-
ulate resolvable physical processes and integrate unresolvable subgrid-scale processes by
approximate parameterizations, DLWPs allow the latent representation of both kinds of
dynamics. The purpose of this review is to facilitate targeted research developments and
understanding of how design choices influence performance of DLWPs. While there is
no single best model, we highlight promising avenues towards accurate spatio-temporal
modeling, probabilistic forecasts and computationally efficient training and infer

How to cite: Thümmel, J., Butz, M., and Goswami, B.: A review of deep learning for weather prediction, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16186, https://doi.org/10.5194/egusphere-egu23-16186, 2023.

EGU23-16443 | ECS | Orals | ITS1.14/CL5.8

Hybrid machine learning model of coupled carbon and water cycles 

Zavud Baghirov, Basil Kraft, Martin Jung, Marco Körner, and Markus Reichstein

There is evidence for a strong coupling between the terrestrial carbon and water cycles and that these cycles should be studied as an interconnected system (Humphrey et al. 2018). One of the key methods to numerically represent the Earth system is process based modelling, which is, however, still subject to large uncertainties, e.g., due to wrong or incomplete process knowledge (Bonan and Doney 2018). Such models are often rigid and only marginally informed by Earth observations. This is where machine learning (ML) approaches can be advantageous, due to their ability to learn from data in a flexible way. These methods have their own shortcomings, such as their “black-box” nature and lack of physical consistency.

Recently, it has been suggested by Reichstein et al. (2019) to combine process knowledge with ML algorithms to model environmental processes. The so-called hybrid modelling approach has already been used to model different components of terrestrial water storage (TWS) in a global hydrological model (Kraft et al. 2022). This study follows-up on this work with the objective to improve the parameterization of some processes (e.g., soil moisture) and to couple the model with the carbon cycle. The coupling could potentially reduce model uncertainties and help to better understand water-carbon interactions.

The proposed hybrid model of the coupled water and carbon cycles is forced with reanalysis data from ERA-5, such as air temperature, net radiation, and CO2 concentration from CAMS. Water-carbon cycle processes are constrained using observational data products of water-carbon cycles. The hybrid model uses a long short-term memory (LSTM) model—a member of the recurrent neural networks family—at its core for processing the time-series Earth observation data. The LSTM simulates a number of coefficients which are used as parameters in the conceptual model of water and carbon cycles. Some of the key processes represented in the conceptual model are evapotranspiration, snow, soil moisture, runoff, groundwater, water use efficiency (WUE), ecosystem respiration, and net ecosystem exchange. The model partitions TWS into different components and it can be used to assess the impact of different TWS components on the CO2 growth rate. Moreover, we can assess the learned system behaviors of water and carbon cycle interactions for different ecosystems.

References:

Bonan, Gordon B, and Scott C Doney. 2018. “Climate, Ecosystems, and Planetary Futures: The Challenge to Predict Life in Earth System Models.” Science 359 (6375): eaam8328.

Humphrey, Vincent, Jakob Zscheischler, Philippe Ciais, Lukas Gudmundsson, Stephen Sitch, and Sonia I Seneviratne. 2018. “Sensitivity of Atmospheric CO2 Growth Rate to Observed Changes in Terrestrial Water Storage.” Nature 560 (7720): 628–31.

Kraft, Basil, Martin Jung, Marco Körner, Sujan Koirala, and Markus Reichstein. 2022. “Towards Hybrid Modeling of the Global Hydrological Cycle.” Hydrology and Earth System Sciences 26 (6): 1579–1614.

Reichstein, Markus, Gustau Camps-Valls, Bjorn Stevens, Martin Jung, Joachim Denzler, Nuno Carvalhais, et al. 2019. “Deep Learning and Process Understanding for Data-Driven Earth System Science.” Nature 566 (7743): 195–204.

How to cite: Baghirov, Z., Kraft, B., Jung, M., Körner, M., and Reichstein, M.: Hybrid machine learning model of coupled carbon and water cycles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16443, https://doi.org/10.5194/egusphere-egu23-16443, 2023.

EGU23-16449 | Orals | ITS1.14/CL5.8

Data-driven seasonal forecasts of European heat waves 

Stefano Materia, Martin Jung, Markus G. Donat, and Carlos Gomez-Gonzalez

Seasonal Forecasts are critical tools for early-warning decision support systems, that can help reduce the related risk associated with hot or cold weather and other events that can strongly affect a multitude of socio-economic sectors. Recent advances in both statistical approaches and numerical modeling have improved the skill of Seasonal Forecasts. However, especially in mid-latitudes, they are still affected by large uncertainties that can limit their usefulness.

The MSCA-H2020 project ARTIST aims at improving our knowledge of climate predictability at the seasonal time-scale, focusing on the role of unexplored drivers, to finally enhance the performance of current prediction systems. This effort is meant to reduce uncertainties and make forecasts efficiently usable by regional meteorological services and private bodies. This study focuses on seasonal prediction of heat extremes in Europe, and here we present a first attempt to predict heat wave accumulated activity across different target seasons. An empirical seasonal forecast is designed based on Machine Learning techniques. A feature selection approach is used to detect the best subset of predictors among a variety of candidates, and then an assessment of the relative importance of each predictor is done, in different European regions for the four main seasons.

Results show that many observed teleconnections are caught by the data-driven approach, while a few features that show to be linked to the heat wave propensity of a season deserve a deeper understanding of the underpinning physical process.

How to cite: Materia, S., Jung, M., Donat, M. G., and Gomez-Gonzalez, C.: Data-driven seasonal forecasts of European heat waves, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16449, https://doi.org/10.5194/egusphere-egu23-16449, 2023.

EGU23-16846 | ECS | Orals | ITS1.14/CL5.8

Learning causal drivers of PyroCb 

Emiliano Díaz, Gherardo Varando, Fernando Iglesias-Suarez, Gustau Camps-Valls, Kenza Tazi, Kara Lamb, and Duncan Watson-Parris

Discovering causal relationships from purely observational data is often not possible. In this case, combining observational and experimental data can allow for the identifiability of the underlying causal structure. In Earth Systems sciences, carrying out interventional experiments is often impossible for ethical and practical reasons. However, “natural interventions”, are often present in the data, and these represent regime changes caused by changes to exogenous drivers. In [3,4], the Invariant Causal Prediction (ICP) methodology was presented to identify the causes of a target variable of interest from a set of candidate causes. This methodology takes advantage of natural interventions, resulting in different cause variables distributions across different environments.  In [2] this methodology is implemented in a geoscience problem, namely identifying the causes of Pyrocumulunimbus (pyroCb), and storm clouds resulting from extreme wildfires. Although a set of plausible causes is produced, certain heuristic adaptations to the original ICP methodology were implemented to overcome some of the practical. limitations of ICP: a large number of hypothesis tests required and a failure to identify causes when these have a high degree of interdependence. In this work, we try to circumvent these difficulties by taking a different approach. We use a learning paradigm similar to that presented in [3] to learn causal representations invariant across different environments. Since we often don’t know exactly how to define the different environments best, we also propose to learn functions that describe their spatiotemporal extent. We apply the resulting algorithm to the pyroCb database in [1] and other Earth System sciences datasets to verify the plausibility of the causal representations found and the environments that describe the so-called natural interventions.. 

 

[1] Tazi et al. 2022. https://arxiv.org/abs/2211.13052

[2] Díaz et al. 2022 .https://arxiv.org/abs/2211.08883

[3] Arjovsky et al. 2019. https://arxiv.org/abs/1907.02893

[4] Peters et al.2016.  https://www.jstor.org/stable/4482904

[5] Heinze-Deml et al. 2018. https://doi.org/10.1515/jci-2017-0016

How to cite: Díaz, E., Varando, G., Iglesias-Suarez, F., Camps-Valls, G., Tazi, K., Lamb, K., and Watson-Parris, D.: Learning causal drivers of PyroCb, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16846, https://doi.org/10.5194/egusphere-egu23-16846, 2023.

EGU23-17082 | ECS | Posters on site | ITS1.14/CL5.8

A statistical approach on rapid estimations of climate change indices by monthly instead of daily data 

Kristofer Hasel, Marianne Bügelmayer-Blaschek, and Herbert Formayer

Climate change indices (CCI) defined by the expert team on climate change detection and indices (ETCCDI) profoundly contribute to understanding climate and its change. They are used to present climate change in an easy to understand and tangible way, thus facilitating climate communication. Many of the indices are peak over threshold indices needing daily and, if necessary, bias corrected data to be calculated from. We present a method to rapidly estimate specific CCI from monthly data instead of daily while also performing a simple bias correction as well as a localisation (downscaling). Therefore, we used the ERA5 Land data with a spatial resolution of 0.1° supplemented by a CMIP6 ssp5-8.5 climate projection to derive different regression functions which allow a rapid estimation by monthly data. Using a climate projection as a supplement in training the regression functions allows an application not only on historical periods but also on future periods such as those provided by climate projections. Nevertheless, the presented method can be adapted to any data set, allowing an even higher spatial resolution.

How to cite: Hasel, K., Bügelmayer-Blaschek, M., and Formayer, H.: A statistical approach on rapid estimations of climate change indices by monthly instead of daily data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17082, https://doi.org/10.5194/egusphere-egu23-17082, 2023.

EGU23-17197 | Posters on site | ITS1.14/CL5.8

Machine learning workflow for deriving regional geoclimatic clusters from high-dimensional data 

Sebastian Lehner, Katharina Enigl, and Matthias Schlögl

Geoclimatic regions represent climatic forcing zones, which constitute important spatial entities that serve as a basis for a broad range of analyses in earth system sciences. The plethora of geospatial variables that are relevant for obtaining consistent clusters represent a high-dimensionality, especially when working with high-resolution gridded data, which may render the derivation of such regions complex. This is worsened by typical characteristics of geoclimatic data like multicollinearity, nonlinear effects and potentially complex interactions between features. We therefore present a nonparametric machine learning workflow, consisting of dimensionality reduction and clustering for deriving geospatial clusters of similar geoclimatic characteristics. We demonstrate the applicability of the proposed procedure using a comprehensive dataset featuring climatological and geomorphometric data from Austria, aggregated to the recent climatological normal from 1992 to 2021.
 
The modelling workflow consists of three major sequential steps: (1) linear dimensionality reduction using Principal Component Analysis, yielding a reduced, orthogonal sub-space, (2) nonlinear dimensionality reduction applied to the reduced sub-space using Uniform Manifold Approximation and Projection, and (3) clustering the learned manifold projection via Hierarchical Density-Based Spatial Clustering of Applications with Noise. The contribution of the input features to the cluster result is then assessed by means of permutation feature importance of random forest models. These are trained by treating the clustering result as a supervised classification problem. Results show the flexibility of the defined workflow and exhibit good agreement with both quantitatively derived and synoptically informed characterizations of geoclimatic regions from other studies. However, this flexibility does entail certain challenges with respect to hyperparameter settings, which require careful exploration and tuning. The proposed workflow may serve as a blueprint for deriving consistent geospatial clusters exhibiting similar geoclimatic attributes.

How to cite: Lehner, S., Enigl, K., and Schlögl, M.: Machine learning workflow for deriving regional geoclimatic clusters from high-dimensional data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17197, https://doi.org/10.5194/egusphere-egu23-17197, 2023.

EGU23-17333 | ECS | Posters on site | ITS1.14/CL5.8

Emulating the regional temperature responses (RTPs) of short-lived climate forcers 

Maura Dewey, Hans Christen Hansson, and Annica M. L. Ekman

Here we develop a statistical model emulating the surface temperature response to changes in emissions of short-lived climate forcers as simulated by an Earth system model. Short-lived climate forcers (SLCFs) are chemical components in the atmosphere that interact with radiation and have both an immediate effect on local air quality, and regional and global effects on the climate in terms of changes in temperature and precipitation distributions. The short atmospheric residence times of SLCFs lead to high atmospheric concentrations in emission regions and a highly variable radiative forcing pattern. Regional Temperature Potentials (RTPs) are metrics which quantify the impact of emission changes in a given region on the temperature or forcing response of another, accounting for spatial inhomogeneities in both forcing and the temperature response, while being easy to compare across models and to use in integrated assessment studies or policy briefs. We have developed a Gaussian-process emulator using output from the Norwegian Earth System Model (NorESM) to predict the temperature responses to regional emission changes in SLCFs (specifically back carbon, organic carbon, sulfur dioxide, and methane) and use this model to calculate regional RTPs and study the sensitivity of surface temperature in a certain region, e.g. the Arctic, to anthropogenic emission changes in key policy regions. The main challenge in developing the emulator was creating the training data set such that we included maximal SLCF variability in a realistic and policy relevant range compared to future emission scenarios, while also getting a significant temperature response. We also had to account for the confounding influence of greenhouse gases (GHG), which may not follow the same future emission trajectories as SLCFs and can overwhelm the more subtle temperature response that comes from the direct and indirect effects of SLCF emissions. The emulator can potentially provide accurate and customizable predictions for policy makers to proposed emission changes with minimized climate impact.

How to cite: Dewey, M., Hansson, H. C., and Ekman, A. M. L.: Emulating the regional temperature responses (RTPs) of short-lived climate forcers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17333, https://doi.org/10.5194/egusphere-egu23-17333, 2023.

EGU23-582 | ECS | Posters on site | ITS1.13/AS5.2

Modeling the Variability of Terrestrial Carbon Fluxes using Transformers 

Swarnalee Mazumder and Ayush Prasad

The terrestrial carbon cycle is one of the largest sources of uncertainty in climate projections. The terrestrial carbon sink which removes a quarter of anthropogenic CO2 emissions; is highly variable in time and space depending on climate. Previous studies have found that data-driven models such as random forest, artificial neural networks and long short-term memory networks can be used to accurately model Net Ecosystem Exchange (NEE) and Gross Primary Productivity (GPP) accurately, which are two important metrics to quantify the direction and magnitude of CO2 transfer between the land surface and the atmosphere. Recently, a new class of machine learning models called transformers have gained widespread attention in natural language processing tasks due to their ability to learn from large volumes of sequential data. In this work, we use Transformers to model NEE and GPP from 1996-2022 at 39 Flux stations in the ICOS Europe network using ERA5 reanalysis data. We can compare our results with traditional machine learning approaches to evaluate the generalisability and predictive performance of transformers for carbon flux modelling.

How to cite: Mazumder, S. and Prasad, A.: Modeling the Variability of Terrestrial Carbon Fluxes using Transformers, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-582, https://doi.org/10.5194/egusphere-egu23-582, 2023.

EGU23-1825 | ECS | Orals | ITS1.13/AS5.2

Spatial representation learning for ensemble weather simulations using invariant variational autoencoders 

Jieyu Chen, Kevin Höhlein, and Sebastian Lerch

Weather forecasts today are typically issued in the form of ensemble simulations based on multiple runs of numerical weather prediction models with different perturbations in the initial states and the model physics. In light of the continuously increasing spatial resolutions of operational weather models, this results in large, high-dimensional datasets that nonetheless contain relevant spatial and temporal structure, as well as information about the predictive uncertainty. We propose invariant variational autoencoder (iVAE) models based on convolutional neural network architectures to learn low-dimensional representations of the spatial forecast fields. We specifically aim to account for the ensemble character of the input data and discuss methodological questions about the optimal design of suitable dimensionality reduction methods in this setting. Thereby, our iVAE models extend previous work where low-dimensional representations of single, deterministic forecast fields were learned and utilized for incorporating spatial information into localized ensemble post-processing methods based on neural networks [1], which were able to improve upon model utilizing location-specific inputs only [2]. By additionally incorporating the ensemble dimension and learning representation for probability distributions of spatial fields, we aim to enable a more flexible modeling of relevant predictive information contained in the full forecast ensemble. Additional potential applications include data compression and the generation of forecast ensembles of arbitrary size.

We illustrate our methodological developments based on a 10-year dataset of gridded ensemble forecasts from the European Centre for Medium-Range Weather Forecasts of several meteorological variables over Europe. Specifically, we investigate alternative model architectures and highlight the importance of tailoring the loss function to the specific problem at hand.

References:

[1] Lerch, S. & Polsterer, K.L. (2022). Convolutional autoencoders for spatially-informed ensemble post-processing. ICLR 2022 AI for Earth and Space Science Workshop, https://arxiv.org/abs/2204.05102.

[2] Rasp, S. & Lerch, S. (2018). Neural networks for post-processing ensemble weather forecasts. Monthly Weather Review, 146, 3885-3900.

How to cite: Chen, J., Höhlein, K., and Lerch, S.: Spatial representation learning for ensemble weather simulations using invariant variational autoencoders, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1825, https://doi.org/10.5194/egusphere-egu23-1825, 2023.

EGU23-3117 | Orals | ITS1.13/AS5.2

AtmoRep: Large Scale Representation Learning for Atmospheric Data 

Christian Lessig, Ilaria Luise, and Martin Schultz

The AtmoRep project asks if one can train one neural network that represents and describes all atmospheric dynamics. AtmoRep’s ambition is hence to demonstrate that the concept of large-scale representation learning, whose principle feasibility and potential was established by large language models such as GPT-3, is also applicable to scientific data and in particular to atmospheric dynamics. The project is enabled by the large amounts of atmospheric observations that have been made in the past as well as advances on neural network architectures and self-supervised learning that allow for effective training on petabytes of data. Eventually, we aim to train on all of the ERA5 reanalysis and, furthermore, fine tune on observational data such as satellite measurements to move beyond the limits of reanalyses.

We will present the theoretical formulation of AtmoRep as an approximate representation for the atmosphere as a stochastic dynamical system. We will also detail our transformer-based network architecture and the training protocol for self-supervised learning so that unlabelled data such as reanalyses, simulation outputs and observations can be employed for training and re-fining the network. Results will be presented for the performance of AtmoRep for downscaling, precipitation forecasting, the prediction of tropical convection initialization, and for model correction. Furthermore, we also demonstrate that AtmoRep has substantial zero-short skill, i.e., it is capable to perform well on tasks it was not trained for. Zero- and few-shot performance (or in context learning) is one of the hallmarks of large-scale representation learning and to our knowledge has never been demonstrated in the geosciences.

How to cite: Lessig, C., Luise, I., and Schultz, M.: AtmoRep: Large Scale Representation Learning for Atmospheric Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3117, https://doi.org/10.5194/egusphere-egu23-3117, 2023.

Numerical Earth system models (ESMs) are our primary tool for projecting future climate scenarios. Their simulation output is used by impact models that assess the effect of anthropogenic global warming, e.g., on flood events, vegetation changes or crop yields. Precipitation, an atmospheric variable with arguably one of the largest socio-economic impacts, involves various processes on a wide range of spatial-temporal scales. However, these cannot be completely resolved in ESMs due to the limited discretization of the numerical model. 
This can lead to biases in the ESM output that need to be corrected in a post-processing step prior to feeding ESM output into impact models, which are calibrated with observations [1]. While established post-processing methods successfully improve the modelled temporal statistics for each grid cell individually, unrealistic spatial features that require a larger spatial context are not addressed.
Here, we apply a cycle-consistent generative adversarial network (CycleGAN) [2] that is physically constrained to the precipitation output from Coupled Model Intercomparison Project phase 6 (CMIP6)  ESMs to correct both temporal distributions and spatial patterns. The CycleGAN can be naturally trained on daily ESM and reanalysis fields that are unpaired due to the deviating trajectories of the ESM and observation-based ground truth. 
We evaluate our method against a state-of-the-art bias adjustment framework (ISIMIP3BASD) [3] and find that it outperforms it in correcting spatial patterns and achieves comparable results on temporal distributions. We further discuss the representation of extreme events and suitable metrics for quantifying the realisticness of unpaired precipitation fields.

 [1] Cannon, A.J., et al. "Bias correction of GCM precipitation by quantile mapping: How well do methods preserve changes in quantiles and extremes?." Journal of Climate 28.17 (2015): 6938-6959.

[2] Zhu, J.-Y., et al. "Unpaired image-to-image translation using cycle-consistent adversarial networks." Proceedings of the IEEE international conference on computer vision. 2017.

[3] Lange, S. "Trend-preserving bias adjustment and statistical downscaling with ISIMIP3BASD (v1.0)." Geoscientific Model Development 12.7 (2019): 3055-3070.

How to cite: Hess, P., Lange, S., and Boers, N.: Improving global CMIP6 Earth system model precipitation output with generative adversarial networks for unpaired image-to-image translation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3128, https://doi.org/10.5194/egusphere-egu23-3128, 2023.

EGU23-3256 | Orals | ITS1.13/AS5.2

Emulating radiative transfer in a numerical weather prediction model 

Matthew Chantry, Peter Ukkonen, Robin Hogan, and Peter Dueben

Machine learning, and particularly neural networks, have been touted as a valuable accelerator for physical processes. By training on data generated from an existing algorithm a network may theoretically learn a more efficient representation and accelerate the computations via emulation. For many parameterized physical processes in weather and climate models this being actively pursued. Here, we examine the value of this approach for radiative transfer within the IFS, an operational numerical weather prediction model where both accuracy and speed are vital. By designing custom, physics-informed, neural networks we achieve outstanding offline accuracy for both longwave and shortwave processes. In coupled testing we find minimal changes to forecast scores at near operational resolutions. We carry out coupled inference on GPUs to maximise the speed benefits from the emulator approach.

How to cite: Chantry, M., Ukkonen, P., Hogan, R., and Dueben, P.: Emulating radiative transfer in a numerical weather prediction model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3256, https://doi.org/10.5194/egusphere-egu23-3256, 2023.

EGU23-3321 | ECS | Orals | ITS1.13/AS5.2

Using machine learning to improve dynamical predictions in a coupled model 

Zikang He, Julien Brajard, Yiguo Wang, Xidong Wang, and Zheqi Shen

Dynamical models used in climate prediction often have systematic errors that can bias the predictions. In this study, we utilized machine learning to address this issue. Machine learning was applied to learn the error corrected by data assimilation and thus build a data-driven model to emulate the dynamical model error. A hybrid model was constructed by combining the dynamical and data-driven models. We tested the hybrid model using synthetic observations generated by a simplified high-resolution coupled ocean-atmosphere model (MAOOAM, De Cruz et al., 2016) and compared its performance to that of a low-resolution version of the same model used as a standalone dynamical model.

To evaluate the forecast skill of the hybrid model, we produced ensemble predictions based on initial conditions determined through data assimilation. The results show that the hybrid model significantly improves the forecast skill for both atmospheric and oceanic variables compared to the dynamical model alone. To explore what affects short-term forecast skills and long-term forecast skills, we built two other hybrid models by correcting errors either only atmospheric or only oceanic variables. For short-term atmospheric forecasts, the results show that correcting only oceanic errors has no effect on atmosphere variables forecasts but correcting only atmospheric variables shows similar forecast skill to correcting both atmospheric and oceanic errors. For the long-term forecast of oceanic variables, correcting the oceanic error can improve the forecast skill, but correcting both atmospheric and oceanic errors can obtain the best forecast skill. The results indicate that for the long-term forecast of oceanic variables, bias correction of both oceanic and atmospheric components can have a significant effect.

How to cite: He, Z., Brajard, J., Wang, Y., Wang, X., and Shen, Z.: Using machine learning to improve dynamical predictions in a coupled model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3321, https://doi.org/10.5194/egusphere-egu23-3321, 2023.

EGU23-3340 | ECS | Orals | ITS1.13/AS5.2

An iterative data-driven emulator of an ocean general circulation model 

Rachel Furner, Peter Haynes, Dan(i) Jones, Dave Munday, Brooks Paige, and Emily Shuckburgh

Data-driven models are becoming increasingly competent at tasks fundamental to weather and climate prediction. Relative to machine learning (ML) based atmospheric models, which have shown promise in short-term forecasting, ML-based ocean forecasting remains somewhat unexplored. In this work, we present a data-driven emulator of an ocean GCM and show that performance over a single predictive step is skilful across all variables under consideration. Iterating such data-driven models poses additional challenges, with many models suffering from over-smoothing of fields or instabilities in the predictions. We compare a variety of methods for iterating our data-driven emulator and assess them by looking at how well they agree with the underlying GCM in the very short term and how realistic the fields remain for longer-term forecasts. Due to the chaotic nature of the system being forecast, we would not expect any model to agree with the GCM accurately over long time periods, but instead we expect fields to continue to exhibit physically realistic behaviour at ever increasing lead times. Specifically, we expect well-represented fields to remain stable whilst also maintaining the presence and sharpness of features seen in both reality and in GCM predictions, with reduced emphasis on accurately representing the location and timing of these features. This nuanced and temporally changing definition of what constitutes a ‘good’ forecast at increasing lead times generates questions over both (1) how one defines suitable metrics for assessing data-driven models, and perhaps more importantly, (2) identifying the most promising loss functions to use to optimise these models.

How to cite: Furner, R., Haynes, P., Jones, D., Munday, D., Paige, B., and Shuckburgh, E.: An iterative data-driven emulator of an ocean general circulation model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3340, https://doi.org/10.5194/egusphere-egu23-3340, 2023.

EGU23-4337 | Orals | ITS1.13/AS5.2 | Highlight

Towards a new surrogate model for predicting short-term NOx-O3 effects from aviation using Gaussian processes 

Pratik Rao, Richard Dwight, Deepali Singh, Jin Maruhashi, Irene Dedoussi, Volker Grewe, and Christine Frömming

While efforts have been made to curb CO2 emissions from aviation, the more uncertain non-CO2 effects that contribute about two-thirds to the warming in terms of radiative forcing (RF), still require attention. The most important non-CO2 effects include persistent line-shaped contrails, contrail-induced cirrus clouds and nitrogen oxide (NOx) emissions that alter the ozone (O3) and methane (CH4) concentrations, both of which are greenhouse gases, and the emission of water vapour (H2O). The climate impact of these non-CO2 effects depends on emission location and prevailing weather situation; thus, it can potentially be reduced by advantageous re-routing of flights using Climate Change Functions (CCFs), which are a measure for the climate effect of a locally confined aviation emission. CCFs are calculated using a modelling chain starting from the instantaneous RF (iRF) measured at the tropopause that results from aviation emissions. However, the iRF is a product of computationally intensive chemistry-climate model (EMAC) simulations and is currently restricted to a limited number of days and only to the North Atlantic Flight Corridor. This makes it impossible to run EMAC on an operational basis for global flight planning. A step in this direction lead to a surrogate model called algorithmic Climate Change Functions (aCCFs), derived by regressing CCFs (training data) against 2 or 3 local atmospheric variables at the time of emission (features) with simple regression techniques and are applicable only in parts of the Northern hemisphere. It was found that in the specific case of O3 aCCFs, which provide a reasonable first estimate for the short-term impact of aviation NOx on O3 warming using temperature and geopotential as features, can be vastly improved [1]. There is aleatoric uncertainty in the full-order model (EMAC), stemming from unknown sources (missing features) and randomness in the known features, which can introduce heteroscedasticity in the data. Deterministic surrogates (e.g. aCCFs) only predict point estimates of the conditional average, thereby providing an incomplete picture of the stochastic response. Thus, the goal of this research is to build a new surrogate model for iRF, which is achieved by :

1. Expanding the geographical coverage of iRF (training data) by running EMAC simulations in more regions (North & South America, Eurasia, Africa and Australasia) at multiple cruise flight altitudes,

2. Following an objective approach to selecting atmospheric variables (feature selection) and considering the importance of local as well as non-local effects,

3. Regressing the iRF against selected atmospheric variables using supervised machine learning techniques such as homoscedastic and heteroscedastic Gaussian process regression.

We present a new surrogate model that predicts iRF of aviation NOx-O3 effects on a regular basis with confidence levels, which not only improves our scientific understanding of NOx-O3 effects, but also increases the potential of global climate-optimised flight planning.

References

[1] Rao, P.; et al. Case Study for Testing the Validity of NOx-Ozone Algorithmic Climate Change Functions for Optimising Flight Trajectories. Aerospace 20229, 231. https://doi.org/10.3390/aerospace9050231

How to cite: Rao, P., Dwight, R., Singh, D., Maruhashi, J., Dedoussi, I., Grewe, V., and Frömming, C.: Towards a new surrogate model for predicting short-term NOx-O3 effects from aviation using Gaussian processes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4337, https://doi.org/10.5194/egusphere-egu23-4337, 2023.

Time transfer functions describe the change of state variables over time in geoscientific numerical simulation models. The identification of these functions is an essential but challenging step in model building. While traditional methods rely on qualitative understanding or first order principles, the availability of large spatio-temporal data sets from direct measurements or extremely detailed physical-based system modelling has enabled the use of machine learning methods to discover the time transfer function directly from data. In this study we explore the feasibility of this data driven approach for numerical simulation of the co-evolution of soil, hydrology, vegetation, and grazing on landscape scale, at geological timescales. From empirical observation and hyper resolution (1 m, 1 week) modelling (Karssenberg et al, 2017) it has been shown that a hillslope system shows complex behaviour with two stable states, respectively high biomass on deep soils (healthy state) and low biomass on thin soils (degraded or desertic state). A catastrophic shift from healthy to degraded state occurs under changes of external forcing (climate, grazing pressure), with a transient between states that is rapid or slow depending on system characteristics. To identify and use the time transfer functions of this system at hillslope scale we follow four procedural steps. First, an extremely large data set of hillslope average soil and vegetation state is generated by a mechanistic hyper resolution (1 m, 1 week) system model, forcing it with different variations in grazing pressure over time. Secondly, a machine learning model predicting the rate of change in soil and vegetation as function of soil, vegetation, and grazing pressure, is trained on this data set. In the third step, we explore the ability of this trained machine learning model to predict the rate of system change (soil and vegetation) on untrained data. Finally, in the fourth step, we use the trained machine learning model as time transfer function in a forward numerical simulation of a hillslope to determine whether it is capable of representing the known complex behaviour of the system. Our findings are that the approach is in principle feasible. We compared the use of a deep neural network and a random forest. Both can achieve great fitting precision, although the latter performs much faster and requires less training data. Even though the machine learning based time transfer function shows differences in the rates of change in system state from those calculated using expert knowledge in Karssenberg et al. (2017), forward simulation appeared to be possible with system behaviour generally in line with that observed in the data from the hyper resolution model. Our findings indicate that discovery of time transfer functions from data is possible. Next steps need to involve the use observational data (e.g., from remote sensing) to test the approach using data from real-world systems.

 

Karssenberg, D., Bierkens, M.F.P., Rietkerk, M., Catastrophic Shifts in Semiarid Vegetation-Soil Systems May Unfold Rapidly or Slowly. The American Naturalist 2017. Vol. 190, pp. E145–E155.

How to cite: Pomarol Moya, O. and Karssenberg, D.: Machine learning for data driven discovery of time transfer functions in numerical modelling: simulating catastrophic shifts in vegetation-soil systems, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4454, https://doi.org/10.5194/egusphere-egu23-4454, 2023.

EGU23-4695 | Posters on site | ITS1.13/AS5.2

Development of PBL Parameterization Emulator using Neural Networks 

Jiyeon Jang, Tae-Jin Oh, Sojung An, Wooyeon Park, Inchae Na, and Junghan Kim

Physical parameterization is one of the major components of Numerical Weather Prediction system. In Korean Integrated Model (KIM), physical parameterizations account for about 30 % of the total computation time. There are many studies of developing neural network based emulators to replace and accelerate physics based parameterization. In this study, we develop a planetary boundary layer(PBL) emulator which is based on Shin-Hong (Hong et al., 2006, 2010; Shin and Hong, 2013, 2015) scheme that computes the parameterized effects of vertical turbulent eddy diffusion of momentum, water vapor, and sensible heat fluxes. We compare the emulator performance with Multi-Layer Perceptron (MLP) based architectures: simple MLP, MLP application version, and MLP-mixer(Tolstikhin et al., 2021). MLP application version divides data into several vertical groups for better approximation of each vertical group layers. MLP-mixer is MLP based architecture that performs well in computer vision without using convolution and self-attention. We evaluate the resulting MLP based emulator performance. MLP application version and MLP-mixer showed significant performance improvement over simple MLP.

How to cite: Jang, J., Oh, T.-J., An, S., Park, W., Na, I., and Kim, J.: Development of PBL Parameterization Emulator using Neural Networks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4695, https://doi.org/10.5194/egusphere-egu23-4695, 2023.

EGU23-4817 | ECS | Posters on site | ITS1.13/AS5.2

Algorithmic optimisation of key parameters of OpenIFS 

Lauri Tuppi, Madeleine Ekblom, Pirkka Ollinaho, and Heikki Järvinen

Numerical weather prediction models contain parameters that are inherently uncertain and cannot be determined exactly. Traditionally, the parameter tuning has been done manually, which can be an extremely labourious task. Tuning the entire model usually requires adjusting a relatively large amount of parameters. In case of manual tuning, the need to balance a number of requirements at the same time can lead the tuning process being a maze of subjective choices. It is, therefore, desirable to have reliable objective approaches for estimation of optimal values and uncertainties of these parameters. In this presentation we present how to optimise 20 key physical parameters having a strong impact on forecast quality. These parameters belong to the Stochastically Perturbed Parameters Scheme in the atmospheric model Open Integrated Forecasting System.

The results show that simultaneous optimisation of O(20) parameters is possible with O(100) algorithm steps using an ensemble of O(20) members, and that the optimised parameters lead to substantial enhancement of predictive skill. The enhanced predictive skill can be attributed to reduced biases in low-level winds and upper-tropospheric humidity in the optimised model. We find that the optimisation process is dependent on the starting values of the parameters that are optimised (starting from better suited values results in a better model). The results also show that the applicability of the tuned parameter values across different model resolutions is somewhat questionable since the model biases seem to be resolution-specific. Moreover, our optimisation algorithm tends to treat the parameter covariances poorly limiting its ability to converge to the global optimum.

How to cite: Tuppi, L., Ekblom, M., Ollinaho, P., and Järvinen, H.: Algorithmic optimisation of key parameters of OpenIFS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4817, https://doi.org/10.5194/egusphere-egu23-4817, 2023.

EGU23-5003 | ECS | Posters on site | ITS1.13/AS5.2

Towards machine-learning calibration of cloud parameters in the kilometre-resolution ICON atmosphere model 

Hannah Marie Eichholz, Jan Kretzschmar, Duncan Watson-Parris, Josefine Umlauft, and Johannes Quaas

In the preparation of the global kilometre-resolution coupled ICON climate model, it is necessary to calibrate cloud microphysical parameters. Here we explore the avenue towards optimally calibrating such parameters using machine learning. The emulator developed by Watson-Parris et al. (2021) is employed in combination with a perturbed-parameter ensemble of limited-area atmosphere-only ICON simulations for the North Atlantic ocean. In a first step, the autoconversion scaling parameter is calibrated, using satellite-retrieved top-of-atmosphere and bottom-of-atmosphere radiation fluxes. For this purpose, limited area simulations of the north atlantic are performed with ICON. In which different cloud microphysical parameters are changed, in order to evaluate possible influences on the output of radiation fluxes.

How to cite: Eichholz, H. M., Kretzschmar, J., Watson-Parris, D., Umlauft, J., and Quaas, J.: Towards machine-learning calibration of cloud parameters in the kilometre-resolution ICON atmosphere model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5003, https://doi.org/10.5194/egusphere-egu23-5003, 2023.

EGU23-5149 | ECS | Posters on site | ITS1.13/AS5.2

Machine Learning Parameterization for Super-droplet Cloud Microphysics Scheme 

Shivani Sharma and David Greenberg

Machine learning approaches have been widely used for improving the representation of subgrid scale parameterizations in Earth System Models. In our study we target the Cloud Microphysics parameterization, in particular the two-moment bulk scheme of the ICON (Icosahedral Non-hydrostatic) Model. 

 

Cloud microphysics parameterization schemes suffer from an accuracy/speed tradeoff. The simplest schemes, often heavy with assumptions (such as the bulk moment schemes) are most common in operational weather prediction models. Conversely, the more complex schemes with fewer assumptions –e.g. Lagrangian schemes such as the super-droplet method (SDM)– are computationally expensive and used only within research and development. SDM allows easy representation of complex scenarios with multiple hydrometeors and can also be used for simulating cloud-aerosol interactions. To bridge this gap and to make the use of more complex microphysical schemes feasible within operational models, we use a data-driven approach. 

 

Here we train a neural network to mimic the behavior of SDM simulations in a warm-rain scenario in a dimensionless control volume. The network behaves like a dynamical system that converts cloud droplets to rain droplets–represented as bulk moments–with only the current system state as the input. We use a multi-step training loss to stabilize the network over long integration periods, especially in cases with extremely low cloud water to start with. We find that the network is stable across various initial conditions and in many cases, emulates the SDM simulations better than the traditional bulk moment schemes. Our network also performs better than any previous ML-based attempts to learn from SDM. This opens the possibility of using the trained network as a proxy for imitating the computationally expensive SDM within operational weather prediction models with minimum computational overhead. 

How to cite: Sharma, S. and Greenberg, D.: Machine Learning Parameterization for Super-droplet Cloud Microphysics Scheme, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5149, https://doi.org/10.5194/egusphere-egu23-5149, 2023.

EGU23-5523 | ECS | Orals | ITS1.13/AS5.2

Using weak constrained neural networks to improve simulations in the gray zone 

Yvonne Ruckstuhl, Raphael Kriegmair, Stephan Rasp, and George Craig

Machine learning represents a potential method to cope with the gray zone problem of representing motions in dynamical systems on scales comparable to the model resolution. Here we explore the possibility of using a neural network to directly learn the error caused by unresolved scales. We use a modified shallow water model which includes highly nonlinear processes mimicking atmospheric convection. To create the training dataset, we run the model in a high- and a low-resolution setup and compare the difference after one low-resolution time step, starting from the same initial conditions, thereby obtaining an exact target. The neural network is able to learn a large portion of the difference when evaluated on single time step predictions on a validation dataset. When coupled to the low-resolution model, we find large forecast improvements up to 1 d on average. After this, the accumulated error due to the mass conservation violation of the neural network starts to dominate and deteriorates the forecast. This deterioration can effectively be delayed by adding a penalty term to the loss function used to train the ANN to conserve mass in a weak sense. This study reinforces the need to include physical constraints in neural network parameterizations.

How to cite: Ruckstuhl, Y., Kriegmair, R., Rasp, S., and Craig, G.: Using weak constrained neural networks to improve simulations in the gray zone, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5523, https://doi.org/10.5194/egusphere-egu23-5523, 2023.

EGU23-5766 | ECS | Orals | ITS1.13/AS5.2

Best Practices for Fortran-Python Bridges to Integrate Neural Networks in Earth System Models 

Caroline Arnold, Shivani Sharma, Tobias Weigel, and David Greenberg

In recent years, machine learning (ML) based parameterizations have become increasingly common in Earth System Models (ESM). Sub-grid scale physical processes that would be computationally too expensive, e.g., atmospheric chemistry and cloud microphysics, can be emulated by ML algorithms such as neural networks.

Neural networks are trained first on simulations of the sub-grid scale process that is to be emulated. They are then used in so-called inference mode to make predictions during the ESM run, replacing the original parameterization. Training usually requires GPUs, while inference may be done on CPU architectures.

At first, neural networks are evaluated offline, i.e., independently of the ESM on appropriate datasets. However, their performance can ultimately only be evaluated in an online setting, where the ML algorithm is coupled to the ESM, including nonlinear interactions.

We want to shorten the time spent in neural network development and offline testing and move quickly to online evaluation of ML components in our ESM of choice, ICON (Icosahedral Nonhydrostatic Weather and Climate Model). Since ICON is written in Fortran, and modern ML algorithms are developed in the Python ecosystem, this requires efficient bridges between the two programming languages. The Fortran-Python bridge must be flexible to allow for iterative development of the neural network. Changes to the ESM codebase should be as few as possible, and the runtime overhead should not limit development.

In our contribution we explore three strategies to call the neural network inference from within Fortran using (i) embedded Python code compiled in a dynamic library, (ii) pipes, and (iii) MPI using the ICON coupler YAC. We provide quantitative benchmarks for the proposed Fortran-Python bridges and assess their overall suitability in a qualitative way to derive best practices. The Fortran-Python bridge enables scientists and developers to evaluate ML components in an online setting, and can be extended to other parameterizations and ESMs.

How to cite: Arnold, C., Sharma, S., Weigel, T., and Greenberg, D.: Best Practices for Fortran-Python Bridges to Integrate Neural Networks in Earth System Models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5766, https://doi.org/10.5194/egusphere-egu23-5766, 2023.

EGU23-6287 | Orals | ITS1.13/AS5.2

Approximation and Optimization of Atmospheric Simulations in High Spatio-Temporal Resolution with Neural Networks 

Elnaz Azmi, Jörg Meyer, Marcus Strobl, Michael Weimer, and Achim Streit

Accurate forecasts of the atmosphere demand large-scale simulations with high spatio-temporal resolution. Atmospheric chemistry modeling, for example, usually requires solving a system of hundreds of coupled ordinary partial differential equations. Due to the computational complexity, large high performance computing resources are required, which is a challenge as the spatio-temporal resolution increases. Machine learning methods and specially deep learning can offer an approximation of the simulations with some factor of speed-up while using less compute resources. The goal of this study is to investigate the feasibility, opportunities but also challenges and pitfalls of replacing the compute-intensive chemistry of a state-of-the-art atmospheric chemistry model with a trained neural network model to forecast the concentration of trace gases at each grid cell and to reduce the computational complexity of the simulation. In this work, we introduce a neural network model (ICONET) to forecast trace gas concentrations without executing the traditional compute-intensive atmospheric simulations. ICONET is equipped with a multifeature Long Short Term Memory (LSTM) model to forecast atmospheric chemicals iteratively in time. We generated the training and test dataset, our ground truth for ICONET, by execution of an atmospheric chemistry simulation in ICON-ART. Applying the ICONET trained model to forecast a test dataset results in a good fit of the forecast values compared to our ground truth dataset. We discuss appropriate metrics to evaluate the quality of models and present the quality of the ICONET forecasts with RMSE and KGE metrics. The variety in the nature of trace gases limits the model's learning and forecast skills according to the variable. In addition to the quality of the ICONET forecasts, we described the computational efficiency of ICONET as its run time speed-up in comparison to the run time of the ICON-ART simulation. The ICONET forecast showed a speed-up factor of 3.1 over the run time of the atmospheric chemistry simulation of ICON-ART, which is a significant achievement, especially when considering the importance of ensemble simulations.

How to cite: Azmi, E., Meyer, J., Strobl, M., Weimer, M., and Streit, A.: Approximation and Optimization of Atmospheric Simulations in High Spatio-Temporal Resolution with Neural Networks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6287, https://doi.org/10.5194/egusphere-egu23-6287, 2023.

EGU23-6836 | ECS | Posters on site | ITS1.13/AS5.2

Parameterising melt at the base of Antarctic ice shelves with a feedforward neural network 

Clara Burgard, Nicolas C. Jourdain, Pierre Mathiot, and Robin Smith

One of the largest sources of uncertainty when projecting the Antarctic contribution to sea-level rise is the ocean-induced melt at the base of Antarctic ice shelves. This is because resolving the ocean circulation and the ice-ocean interactions occurring in the cavity below the ice shelves is computationally expensive.

Instead, for large ensembles and long-term projections of the ice-sheet evolution, ice-sheet models currently rely on parameterisations to link the ocean temperature and salinity in front of ice shelves to the melt at their base. However, current physics-based parameterisations struggle to accurately simulate basal melt patterns.

As an alternative approach, we explore the potential use of a deep feedforward neural network as a basal melt parameterisation. To do so, we train a neural network to emulate basal melt rates simulated by highly-resolved circum-Antarctic ocean simulations. We explore the influence of different input variables and show that the neural network struggles to generalise to ice-shelf geometries unseen during training, while it generalises better on timesteps unseen during training. We also test the parameterisation on separate coupled ocean-ice simulations to assess the neural network’s performance on independent data.  

How to cite: Burgard, C., Jourdain, N. C., Mathiot, P., and Smith, R.: Parameterising melt at the base of Antarctic ice shelves with a feedforward neural network, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6836, https://doi.org/10.5194/egusphere-egu23-6836, 2023.

EGU23-7281 | ECS | Posters on site | ITS1.13/AS5.2

Neural network surrogate models for multiple scattering: Application to OMPS LP simulations 

Michael Himes, Natalya Kramarova, Tong Zhu, Jungbin Mok, Matthew Bandel, Zachary Fasnacht, and Robert Loughman

Retrieving ozone from limb measurements necessitates the modeling of scattered light through the atmosphere.  However, accurately modeling multiple scattering (MS) during retrieval requires excessive computational resources; consequently, operational retrieval models employ approximations in lieu of the full MS calculation.  Here we consider an alternative MS approximation method, where we use radiative transfer (RT) simulations to train neural network models to predict the MS radiances.  We present our findings regarding the best-performing network hyperparameters, normalization schemes, and input/output data structures.  Using RT calculations based on measurements by the Ozone Mapping and Profiling Suite's Limb Profiler (OMPS/LP), we compare the accuracy of these neural-network models with both the full MS calculation as well as the current MS approximation methods utilized during OMPS/LP retrievals.

How to cite: Himes, M., Kramarova, N., Zhu, T., Mok, J., Bandel, M., Fasnacht, Z., and Loughman, R.: Neural network surrogate models for multiple scattering: Application to OMPS LP simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7281, https://doi.org/10.5194/egusphere-egu23-7281, 2023.

EGU23-7368 | ECS | Posters on site | ITS1.13/AS5.2

Comparison of Methods for Learning Differential Equations from Data 

Christof Schötz

Some results from the DEEB (Differential Equation Estimation Benchmark) are presented. In DEEB, we compare different machine learning approaches and statistical methods for estimating nonlinear dynamics from data. Such methods constitute an important building block for purely data-driven earth system models as well as hybrid models which combine physical knowledge with past observations.

Specifically, we examine approaches for solving the following problem: Given time-state-observations of a deterministic ordinary differential equation (ODE) with measurement noise in the state, predict the future evolution of the system. Of particular interest are systems with chaotic behavior - like Lorenz 63 - and nonparametric settings, in which the functional form of the ODE is completely unknown (in particular, not restricted to a polynomial of low order). To create a fair comparison of methods, a benchmark database was created which includes datasets of simulated observations from different dynamical systems with different complexity and varying noise levels. The list of methods we compare includes: echo state networks, Gaussian processes, Neural ODEs, SINDy, thin plate splines, and more.

Although some methods consistently perform better than others throughout different datasets, there seems to be no silver bullet.

How to cite: Schötz, C.: Comparison of Methods for Learning Differential Equations from Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7368, https://doi.org/10.5194/egusphere-egu23-7368, 2023.

EGU23-7391 | ECS | Posters on site | ITS1.13/AS5.2

Learning fluid dynamical statistics using stochastic neural networks 

Martin Brolly
Many practical problems in fluid dynamics demand an empirical approach, where statistics estimated from data inform understanding and modelling. In this context data-driven probabilistic modelling offers an elegant alternative to ad hoc estimation procedures. Probabilistic models are useful as emulators, but also offer an attractive means of estimating particular statistics of interest. In this paradigm one can rely on proper scoring rules for model comparison and validation, and invoke Bayesian statistics to obtain rigorous uncertainty quantification. Stochastic neural networks provide a particularly rich class of probabilistic models, which, when paired with modern optimisation algorithms and GPUs, can be remarkably efficient. We demonstrate this approach by learning the single particle transition density of ocean surface drifters from decades of Global Drifter Program observations using a Bayesian mixture density network. From this we derive maps of various displacement statistics and corresponding uncertainty maps. Our model also offers a means of simulating drifter trajectories as a discrete-time Markov process, which could be used to study the transport of plankton or plastic in the upper ocean.

How to cite: Brolly, M.: Learning fluid dynamical statistics using stochastic neural networks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7391, https://doi.org/10.5194/egusphere-egu23-7391, 2023.

EGU23-7492 | Posters on site | ITS1.13/AS5.2

Machine Learning and Microseism as a Tool for Sea Wave Monitoring 

Flavio Cannavo', Vittorio Minio, Susanna Saitta, Salvatore Alparone, Alfio Marco Borzì, Andrea Cannata, Giuseppe Ciraolo, Danilo Contrafatto, Sebastiano D’Amico, Giuseppe Di Grazia, and Graziano Larocca

Monitoring the state of the sea is a fundamental task for economic activities in the coastal zone, such as transport, tourism and infrastructure design. In recent years, regular wave height monitoring for marine risk assessment and mitigation has become unavoidable as global warming impacts in more intense and frequent swells.
In particular, the Mediterranean Sea has been considered as one of the most responsive regions to global warming, which may promote the intensification of hazardous natural phenomena as strong winds, heavy precipitation and high sea waves. Because of the high density population along the Mediterranean coastlines, heavy swells could have major socio-economic consequences. To reduce the impacts of such scenarios, the development of more advanced monitoring systems of the sea state becomes necessary.
In the last decade, it has been demonstrated how seismometers can be used to measure sea conditions by exploiting the characteristics of a part of the seismic signal called microseism. Microseism is the continuous seismic signal recorded in the frequency band of 0.05 and 0.4 Hz that is likely generated by interactions of sea waves together and with seafloor or shorelines.
In this work, in the framework of i-WaveNET INTERREG project, we performed a regression analysis to develop a model capable of predicting the sea state in the Sicily Channel (Italy) using microseism, acquired by onshore instruments installed in Sicily and Malta. Considering the complexity of the relationship between spatial sea wave height data and seismic data measured at individual stations, we used supervised machine learning (ML) techniques to develop the prediction model. As input data we used the hourly Root Mean Squared (RMS) amplitude of the seismic signal recorded by 14 broadband stations, along the three components, and in different frequency bands, during 2018 - 2021. These stations, belonging to the permanent seismic networks managed by the National Institute of Geophysics and Volcanology INGV and the Department of Geosciences of the University of Malta, consist of three-component broadband seismometers that record at a sampling frequency of 100 Hz.
As for the target, the significant sea wave height data from Copernicus Marine Environment Monitoring Service (CMEMS) for the same period were used. Such data is the hindcast product of the Mediterranean Sea Waves forecasting system, with hourly temporal resolution and 1/24° spatial resolution. After a feature selection step, we compared three different kinds of ML algorithms for regression: K-Nearest-Neighbors (KNN), Random Forest (RF) and Light Gradient Boosting (LGB). The hyperparameters were tuned by using a grid-search algorithm, and the best models were selected by cross-validation.  Different metrics, such as MAE, R2 and RMSE, were considered to evaluate the generalization capabilities of the models and special attention was paid to evaluate the predictive ability of the models for extreme wave height values.
Results show model predictive capabilities good enough to develop a sea monitoring system to complement the systems currently in use.

How to cite: Cannavo', F., Minio, V., Saitta, S., Alparone, S., Borzì, A. M., Cannata, A., Ciraolo, G., Contrafatto, D., D’Amico, S., Di Grazia, G., and Larocca, G.: Machine Learning and Microseism as a Tool for Sea Wave Monitoring, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7492, https://doi.org/10.5194/egusphere-egu23-7492, 2023.

EGU23-7561 | ECS | Posters on site | ITS1.13/AS5.2

Deep Learning guided statistical downscaling of climate projections for use in hydrological impact modeling in Danish peatlands 

Thea Quistgaard, Peter L. Langen, Tanja Denager, Raphael Schneider, and Simon Stisen

A course of action to combat the emission of greenhouse gasses (GHG) in a Danish context is to re-wet previously drained peatlands and thereby return them to their natural hydrological state acting as GHG sinks. GHG emissions from peatlands are known to be closely coupled to the hydrological dynamics through the groundwater table depth (WTD). To understand the effect of a changing and variable climate on the spatio-temporal dynamics of hydrological processes and the associated uncertainties, we aim to produce a high-resolution local-scale climate projection ensemble from the global-scale CMIP6 projections.

With focus on hydrological impacts, uncertainties and possible extreme endmembers, this study aims to span the full ensemble of local-scale climate projections in the Danish geographical area corresponding to the CMIP6-ensemble of Global Climate Models (GCMs). Deep learning founded statistical downscaling methods are applied bridge the gap from GCMs to local-scale climate change and variability, which in turn will be used in field-scale hydrological modeling. The approach is developed to specifically accommodate the resolutions, event types and conditions relevant for assessing the impacts on peatland GHG emissions through their relationship with WTD dynamics by applying stacked conditional generative adversarial networks (CGANs) to best downscale precipitation, temperature, and evaporation. In the future, the approach is anticipated to be extended to directly assess the impacts of climate change and ensemble uncertainty on peatland hydrology variability and extremes.

How to cite: Quistgaard, T., Langen, P. L., Denager, T., Schneider, R., and Stisen, S.: Deep Learning guided statistical downscaling of climate projections for use in hydrological impact modeling in Danish peatlands, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7561, https://doi.org/10.5194/egusphere-egu23-7561, 2023.

EGU23-8288 | Orals | ITS1.13/AS5.2

Learning operational altimetry mapping from ocean models 

Quentin Febvre, Ronan Fablet, Julien Le Sommer, Clément Ubelmann, and Simon Benaïchouche

In oceanography, altimetry products are used to measure the height of the ocean surface, and ocean modeling is used to understand and predict the behavior of the ocean. There are two main types of gridded altimetry products: operational sea level products, such as DUACS, which are used for forecasting and reconstruction, and ocean model reanalyses, such as Glorys 12, which are used to forecast seasonal trends and assess physical characteristics. However, advances in ocean modeling do not always directly benefit operational forecast or reconstruction products.

In this study, we investigate the potential for deep learning methods, which have been successfully applied in simulated setups, to leverage ocean modeling efforts for improving operational altimetry products. Specifically, we ask under what conditions the knowledge learned from ocean simulations can be applied to real-world operational altimetry mapping. We consider the impact of simulation grid resolution, observation data reanalysis, and physical processes modeled on the performance of a deep learning model.

Our results show that the deep learning model outperforms current operational methods on a regional domain around the Gulfstream, with a 50km improvement in resolved scale. This improvement has the potential to enhance the accuracy of operational altimetry products, which are used for a range of important applications, such as climate monitoring and understanding mesoscale ocean dynamics.

How to cite: Febvre, Q., Fablet, R., Le Sommer, J., Ubelmann, C., and Benaïchouche, S.: Learning operational altimetry mapping from ocean models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8288, https://doi.org/10.5194/egusphere-egu23-8288, 2023.

EGU23-9285 | ECS | Orals | ITS1.13/AS5.2

Stabilized Neural Differential Equations for Hybrid Modeling with Conservation Laws 

Alistair White and Niklas Boers

Neural Differential Equations (NDEs) provide a powerful framework for hybrid modeling. Unfortunately, the flexibility of the neural network component of the model comes at the expense of potentially violating known physical invariants, such as conservation laws, during inference. This shortcoming is especially critical for applications requiring long simulations, such as climate modeling, where significant deviations from the physical invariants can develop over time. It is hoped that enforcing physical invariants will help address two of the main barriers to adoption for hybrid models in climate modeling: (1) long-term numerical stability, and (2) generalization to out-of-sample conditions unseen during training, such as climate change scenarios. We introduce Stabilized Neural Differential Equations, which augment an NDE model with compensating terms that ensure physical invariants remain approximately satisfied during numerical simulations. We apply Stabilized NDEs to the double pendulum and Hénon–Heiles systems, both of which are conservative, chaotic dynamical systems possessing a time-independent Hamiltonian. We evaluate Stabilized NDEs using both short-term and long-term prediction tasks, analogous to weather and climate prediction, respectively. Stabilized NDEs perform at least as well as unstabilized models at the “weather prediction” task, that is, predicting the exact near-term state of the system given initial conditions. On the other hand, Stabilized NDEs significantly outperform unstabilized models at the “climate prediction” task, that is, predicting long-term statistical properties of the system. In particular, Stabilized NDEs conserve energy during long simulations and consequently reproduce the long-term dynamics of the target system with far higher accuracy than non-energy conserving models. Stabilized NDEs also remain numerically stable for significantly longer than unstabilized models. As well as providing a new and lightweight method for combining physical invariants with NDEs, our results highlight the relevance of enforcing conservation laws for the long-term numerical stability and physical accuracy of hybrid models.

How to cite: White, A. and Boers, N.: Stabilized Neural Differential Equations for Hybrid Modeling with Conservation Laws, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9285, https://doi.org/10.5194/egusphere-egu23-9285, 2023.

EGU23-10135 | ECS | Orals | ITS1.13/AS5.2

Exploring physics-informed machine learning for accelerated simulation of permafrost processes 

Brian Groenke, Moritz Langer, Guillermo Gallego, and Julia Boike

Permafrost, i.e. ground material that remains perennially frozen, plays a key role in Arctic ecosystems. Monitoring the response of permafrost to rapid climate change remains difficult due to the sparse availability of long-term, high quality measurements of the subsurface. Numerical models are therefore an indispensable tool for understanding the evolution of Arctic permafrost. However, large scale simulation of the hydrothermal processes affecting permafrost is challenging due to the highly nonlinear effects of phase change in porous media. The resulting computational cost of such simulations is especially prohibitive for sensitivity analysis and parameter estimation tasks where a large number of simulations may be necessary for robust inference of quantities such as temperature, water fluxes, and soil properties. In this work, we explore the applicability of recently developed physics-informed machine learning (PIML) methods for accelerating numerical models of permafrost hydrothermal dynamics. We present a preliminary assessment of two possible applications of PIML in this context: (1) linearization of the nonlinear PDE system according to Koopman operator theory in order to reduce the computational burden of large scale simulations, and (2) efficient parameterization of the surface energy balance and snow dynamics on the subsurface hydrothermal regime. By combining the predictive power of machine learning with the underlying conservation laws, PIML can potentially enable researchers and practitioners interested in permafrost to explore complex process interactions at larger spatiotemporal scales.

How to cite: Groenke, B., Langer, M., Gallego, G., and Boike, J.: Exploring physics-informed machine learning for accelerated simulation of permafrost processes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10135, https://doi.org/10.5194/egusphere-egu23-10135, 2023.

EGU23-10256 | ECS | Posters on site | ITS1.13/AS5.2

Foehn Wind Analysis using Unsupervised Deep Anomaly Detection 

Tobias Milz, Marte Hofsteenge, Marwan Katurji, and Varvara Vetrova

Foehn winds are accelerated, warm and dry winds that can have significant environmental impacts as they descend into the lee of a mountain range. For example, in the McMurdo Dry Valleys in Antarctica, foehn events can cause ice and glacial melt and destabilise ice shelves, which if lost, resulting in a rise in sea level. Consequently, there is a strong interest in a deeper understanding of foehn winds and their meteorological signatures. Most current automatic detection methods rely on rule-based methodologies that require static thresholds of meteorological parameters. However, the patterns of foehn winds are hard to define and differ between alpine valleys around the world. Consequently, data-driven solutions might help create more accurate detection and prediction methodologies. 

State-of-the-art machine learning approaches to this problem have shown promising results but follow a supervised learning paradigm. As such, these approaches require accurate labels, which for the most part, are being created by imprecise static rule-based algorithms. Consequently, the resulting machine-learning models are trained to recognise the same static definitions of the foehn wind signatures. 

In this paper, we introduce and compare the first unsupervised machine-learning approaches for detecting foehn wind events. We focus on data from the Mc Murdo Dry Valleys as an example, however, due to the unsupervised nature of these approaches, our solutions can recognise a more dynamic definition of foehn wind events and are therefore, independent of the location. The first approach is based on multivariate time-series clustering, while the second utilises a deep autoencoder-based anomaly detection method to identify foehn wind events. Our best model achieves an f1-score of 88%, matching or surpassing previous machine-learning methods while providing a more flexible and inclusive definition of foehn events. 

How to cite: Milz, T., Hofsteenge, M., Katurji, M., and Vetrova, V.: Foehn Wind Analysis using Unsupervised Deep Anomaly Detection, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10256, https://doi.org/10.5194/egusphere-egu23-10256, 2023.

EGU23-10351 | ECS | Orals | ITS1.13/AS5.2

Deep learning of systematic sea ice model errors from data assimilation increments 

William Gregory, Mitchell Bushuk, Alistair Adcroft, and Yongfei Zhang

Data assimilation is often viewed as a framework for correcting short-term error growth in dynamical climate model forecasts. When viewed on the time scales of climate however, these short-term corrections, or analysis increments, closely mirror the systematic bias patterns of the dynamical model. In this work, we show that Convolutional Neural Networks (CNNs) can be used to learn a mapping from model state variables to analysis increments, thus promoting the feasibility of a data-driven model parameterization which predicts state-dependent model errors. We showcase this problem using an ice-ocean data assimilation system within the fully coupled Seamless system for Prediction and EArth system Research (SPEAR) model at the Geophysical Fluid Dynamics Laboratory (GFDL), which assimilates satellite observations of sea ice concentration. The CNN then takes inputs of data assimilation forecast states and tendencies, and makes predictions of the corresponding sea ice concentration increments. Specifically, the inputs are sea ice concentration, sea-surface temperature, ice velocities, ice thickness, net shortwave radiation, ice-surface skin temperature, and sea-surface salinity. We show that the CNN is able to make skilful predictions of the increments, particularly between December and February in both the Arctic and Antarctic, with average daily spatial pattern correlations of 0.72 and 0.79, respectively. Initial investigation of implementation of the CNN into the fully coupled SPEAR model shows that the CNN can reduce biases in retrospective seasonal sea ice forecasts by emulating a data assimilation system, further suggesting that systematic sea ice biases could be reduced in a free-running climate simulation.

How to cite: Gregory, W., Bushuk, M., Adcroft, A., and Zhang, Y.: Deep learning of systematic sea ice model errors from data assimilation increments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10351, https://doi.org/10.5194/egusphere-egu23-10351, 2023.

Current numerical weather prediction models contain significant systematic errors, due in part to indeterminate ground forcing (GF). This study considers an optimal virtual GF (GFo) derived by training observed and simulated datasets of 10-m wind speeds (WS10) for summer and winter. The GFo is added to an offline surface multilayer model (SMM) to revise predictions of WS10 in China by the Weather Research and Forecasting model (WRF). This revision is a data-based optimization under physical constraints. It reduces WS10 errors and offers wide applicability. The resulting model outperforms two purely physical forecasts (the original WRF forecast and the SMM with physical GF parameterized using urban, vegetation, and subgrid topography) and two purely data-based revisions (i.e., multilinear regression and multilayer perceptron). Compared with original WRF forecasting, using the GFo scheme reduces the Root Mean Square Error (RMSE) in WS10 across China by 25% in summer and 32% in winter. The frontal area index of GFo indicates that it includes both the effects of indeterminate GF and other possible complex physical processes associated with WS10.

How to cite: Feng, J.: Mitigate forecast error in surface wind speed using an offline single-column model with optimal ground forcing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10394, https://doi.org/10.5194/egusphere-egu23-10394, 2023.

EGU23-10726 | Posters virtual | ITS1.13/AS5.2

A hybrid VMD-WT-InceptionTime model for multi-horizon short-term air temperature forecasting in Alaska 

Jaakko Putkonen, M. Aymane Ahajjam, Timothy Pasch, and Robert Chance

The lack of ground level observation stations outside of settlements makes monitoring and forecasting local weather and permafrost challenging in the Arctic. Such predictive pieces of information are essential to help prepare for potentially hazardous weather conditions, especially during winter. In this study, we aim at enhancing predictive analytics in Alaska of permafrost and temperature by using a hybrid forecasting technique. In particular, we propose VMD-WT-InceptionTime model for short-term air temperature forecasting.

This proposed technique incorporates data preprocessing techniques and deep learning to enhance the accuracy of the next seven days air temperature forecasts. Initially, the Spearman correlation coefficient is utilized to examine the relationship between different inputs and the forecast target temperature. Following this, Variational Mode Decomposition (VMD) is used to decompose the most output-correlated input variables (i.e., temperature and relative humidity) to extract intrinsic and non-stationary time-frequency features from the original sequences. The Wavelet Transform (WT) is then employed to further extract intrinsic multi-resolution patterns from these decomposed input variables. Finally, a deep InceptionTime model is used for multi-step air temperature forecasting using these processed sequences. This forecasting technique was developed using an open dataset holding 20+ years of data from three locations in Alaska: North Slope, Alaska, Arctic National Wildlife Refuge, Alaska, and Diomede Island region, Bering Strait. Model performance has been rigorously evaluated of metrics including RMSE, MAPE and error.

Results highlight the effectiveness of the proposed hybrid model in providing more accurate short-term forecasts than several baselines (GBDT, SVR, ExtraTrees, RF, ARIMA, LSTM, GRU, and Transformer). More specifically, this technique reported RMSE and MAPE average increase rates amounting to 11.21% and 16.13% in North Slope, 30.01% and 34.97% in Arctic National Wildlife Refuge, and 16.39%, 23.46% in Diomede Island region. In addition, the proposed technique produces forecasts over all seven horizons with a maximum error of <1.5K, a minimum error of >-1.2K, and an average error lower than 0.18K for North Slope. For Arctic National Wildlife Refuge, a maximum error of <1K, a minimum error of >-0.9K, and an average of < 0.1K. While a maximum error of <0.9K, a minimum error of >-0.8K, and an average of <0.13K, for Diomede Island region. However, the worst performances achieved were errors of around 6K in the third horizon (i.e., 3rd day) for North Slope and the Arctic National Wildlife Refuge and the last horizon (i.e., 7th day) for the Diomede Islands region. Most of the worst performances of the proposed technique in all three locations can be attributed to having to produce forecasts of higher variations and wider temperature ranges than their averages.

Overall, this research highlights the potential of the decomposition techniques and deep learning to: 1) reveal and effectively learn the underlying cyclicity of air temperatures at varying resolutions that allows for accurate predictions without any knowledge of the governing physics, 2) produce accurate multi-step temperature forecasts in Arctic climates.

How to cite: Putkonen, J., Ahajjam, M. A., Pasch, T., and Chance, R.: A hybrid VMD-WT-InceptionTime model for multi-horizon short-term air temperature forecasting in Alaska, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10726, https://doi.org/10.5194/egusphere-egu23-10726, 2023.

EGU23-10810 | ECS | Orals | ITS1.13/AS5.2

Oceanfourcast: Emulating Ocean Models with Transformers for Adjoint-based Data Assimilation 

Suyash Bire, Björn Lütjens, Dava Newman, and Chris Hill

Adjoints have become a staple of the oceanic and atmospheric numerical modeling community over the past couple of decades as they are useful for tuning of dynamical models, sensitivity analyses, and data assimilation. One such application is generation of reanalysis datasets, which provide an optimal record of our past weather, climate, and ocean. For example, the state-of-the-art ocean-ice renanalysis dataset, ECCO, is created by optimally combining a numerical ocean model with heterogeneous observations through a technique called data assimilation. Data assimilation in ECCO minimizes the distance between model and observations by calculating adjoints, i.e., gradients of the loss w.r.t. simulation forcing fields (wind and surface heat fluxes). The forcing fields are iteratively updated and the model is rerun until the loss is minimized to ensure that the numerical model does not drastically deviate from the observations. Calculating adjoints, however, either requires  disproportionately high computational resources  or rewriting the dynamical model code to be autodifferentiable. 

Therefore, we ask if deep learning-based emulators can provide fast and accurate adjoints. Ocean data is smooth, high-dimensional, and has complex spatiotemporal correlations. Therefore, as an initial foray into ocean emulators, we leverage a combination of neural operators and transformers. Specifically, we have adapted the FourCastNet architecture, which has successfully emulated ERA5 weather data in seconds rather than hours, to emulate an idealized ocean simulation.

We generated a ground-truth dataset by simulating a double-gyre, an idealized representation of the North Atlantic Ocean, using MITgcm, a state-of-the-art dynamical model. The model was forced by zonal wind at the surface and relaxation to a meridional profile of temperature — warm/cold temperatures at low/high latitudes. This simulation produced turbulent western boundary currents embedded in the large-scale gyre circulation. We performed 4 additional simulations by modifying the magnitude of SST relaxation and wind forcing to introduce diversity in the dataset. From these simulations, we used 4 state variables (meridional and zonal surface velocities, pressure, and temperature) as well as the forcing fields (zonal wind velocity and relaxation SST profile) sampled in 10-day steps. The dataset was split into training, validation, and test datasets such that validation and test datasets were unseen during training. These datasets provide an ideal testbed for evaluating and comparing the performance of data-driven ocean emulators.

We used this data to train and evaluate Oceanfourcast. Our initial results in the following figure show that our model, Oceanfourcast, can successfully predict the streamfunction and pressure for a lead time of 1 month. 

We are currently working on generating adjoints from Oceanfourcast.  We expect the adjoint calculation to require significantly less compute time than that from a full-scale dynamical model like MITgcm.  Our work shows a promising path towards deep-learning augmented data assimilation and uncertainty quantification.

How to cite: Bire, S., Lütjens, B., Newman, D., and Hill, C.: Oceanfourcast: Emulating Ocean Models with Transformers for Adjoint-based Data Assimilation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10810, https://doi.org/10.5194/egusphere-egu23-10810, 2023.

EGU23-10904 | ECS | Posters on site | ITS1.13/AS5.2

On the choice of turbulence eddy fluxes to learn from in data-driven methods 

Feier Yan, Julian Mak, and Yan Wang

Recent works have demonstrated the viability of employing data-driven / machine learning 
methods for the purposes of learning more about ocean turbulence, with applications to turbulence parameterisations in ocean general circulation models. Focusing on mesoscale geostrophic turbulence in the ocean context, works thus far have mostly focused on the choice of algorithms and testing of trained up models. Here we focus instead on the choice of eddy flux data to learn from. We argue that, for mesoscale geostrophic turbulence, it might be beneficial from a theoretical as well as practical point of view to learn from eddy fluxes with dynamically inert rotational fluxes removed (ideally in a gauge invariant fashion), instead of the divergence of the eddy fluxes as has been considered thus far. Outlooks for physically constrained and interpretable machine learning will be given in light of the results. 

How to cite: Yan, F., Mak, J., and Wang, Y.: On the choice of turbulence eddy fluxes to learn from in data-driven methods, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10904, https://doi.org/10.5194/egusphere-egu23-10904, 2023.

EGU23-10959 | Orals | ITS1.13/AS5.2

Deep learning parameterization of small-scale vertical velocity variability for atmospheric models 

Donifan Barahona, Katherine Breen, and Heike Kalesse-Los

Small-scale fluctuations in vertical wind velocity, unresolved by climate and weather forecast models play a particularly important role in determining vapor and tracer fluxes, turbulence and cloud formation. Fluctuations in vertical wind velocity are challenging to represent since they depend on orography, large scale circulation features, convection and wind shear. Parameterizations developed using data retrieved at specific locations typically lack generalization and may introduce error when applied on a wide range of different conditions. Retrievals of vertical wind velocity are also difficult and subject to large uncertainty. This work develops a new data-driven, neural network representation of subgrid scale variability in vertical wind velocity. Using a novel deep learning technique, the new parameterization merges data from high-resolution global cloud resolving model simulations with high frequency Radar and Lidar retrievals.  Our method aims to reproduce observed statistics rather than fitting individual measurements. Hence it is resilient to experimental uncertainty and robust to generalization. The neural network parameterization can be driven by weather forecast and reanalysis products to make real time estimations. It is shown that the new parameterization generalizes well outside of the training data and reproduces much better the statistics of vertical wind velocity than purely data-driven models.

How to cite: Barahona, D., Breen, K., and Kalesse-Los, H.: Deep learning parameterization of small-scale vertical velocity variability for atmospheric models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10959, https://doi.org/10.5194/egusphere-egu23-10959, 2023.

EGU23-11293 | ECS | Posters on site | ITS1.13/AS5.2

National scale agricultural development dynamics under socio-political drivers in Saudi Arabia since 1990 

Ting Li, Oliver López Valencia, Kasper Johansen, and Matthew McCabe

Driven in large part by policy initiatives designed to increase food security and realized via the construction of thousands of center-pivot irrigation fields since the 1970s, agriculture development in Saudi Arabia has undergone tremendous changes. However, little is known about the accurate number, acreage, and the changing dynamics of the fields. To bridge the knowledge gap between the political drivers and in-field response, we leveraged a hybrid machine learning framework by implementing Density-Based Spatial Clustering of Applications with Noise, Convolutional Neural Networks, and Spectral Clustering in a stepwise manner to delineate the center-pivot fields on a national scale in Saudi Arabia using historical Landsat imagery since 1990. The framework achieved producer's and user's accuracies larger than  83.7% and 90.2%, respectively, when assessed against 28,000 manually delineated fields collected from different regions and periods. We explored multi-decadal dynamics of the agricultural development in Saudi Arabia by quantifying the number, acreage, and size distribution of center-pivot fields, along with the first and last detection year of the fields since 1990. The agricultural development in Saudi Arabia experienced four stages, including an initialization stage before 1990, a contraction stage from 1990 to 2010, an expansion stage from 2010 to 2016, and an ongoing contraction stage since 2016. Most of the fields predated 1990, representing over 8,800 km2 in that year, as a result of the policy initiatives to stimulate wheat production, promoting Saudi Arabia as the sixth largest exporter of wheat in the 1980s. A decreasing trend was observed from 1990 to 2010, with an average of 8,011 km2 of fields detected during those two decades, which was a response to the policy initiative implemented to phase-out wheat after 1990. As a consequence of planting fodder crops to promote the dairy industry, the number and extent of fields increased rapidly from 2010 to 2015 and reached its peak in 2016, with 33,961 fields representing 9,400 km2. Agricultural extent has seen a continuous decline since 2016 to a level lower than 1990 values in 2020. This decline has been related to sustainable policy initiatives implemented for the Saudi Vision 2030. There is some evidence of an uptick in 2021 — also observed in an ongoing analysis for 2022 — which might be in response to global influences, such as the COVID-19 pandemic and the more recent conflict in the Ukraine, which has disrupted the international supply of agricultural products. The results provide a historical account of agricultural activity throughout the Kingdom and provide a basis for informed decision-making on sustainable irrigation and agricultural practices, helping to better protect and manage the nation's threatened groundwater resources, and providing insights into the resilience and elasticity of the Saudi Arabian food system to global perturbations.

How to cite: Li, T., López Valencia, O., Johansen, K., and McCabe, M.: National scale agricultural development dynamics under socio-political drivers in Saudi Arabia since 1990, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11293, https://doi.org/10.5194/egusphere-egu23-11293, 2023.

EGU23-11687 | ECS | Orals | ITS1.13/AS5.2

Objectively Determining the Number of Similar Hydrographic Clusters with Unsupervised Machine Learning 

Carola Trahms, Yannick Wölker, and Arne Biastoch

Determining the number of existing water masses and defining their boundaries is subject to ongoing discussion in physical oceanography. Traditionally, water masses are defined manually by experts setting constraints based on experience and previous knowledge about the hydrographic properties describing them. In recent years, clustering, an unsupervised machine learning approach, has been introduced as a tool to determine clusters, i.e., volumes, with similar hydrographic properties without explicitly defining their hydrographic constraints. However, the exact number of clusters to be looked for is set manually by an expert up until now. 

We propose a method that determines a fitting number of clusters for hydrographic clusters in a data driven way. In a first step, the method averages the data in different-sized slices along the time or depth axis as the structure of the hydrographic space changes strongly either in time or depth. Then the method applies clustering algorithms on the averaged data and calculates off-the-shelf evaluation scores (Davies-Bouldin, Calinski-Harabasz, Silhouette Coefficient) for several predefined numbers of clusters. In the last step, the optimal number of clusters is determined by analyzing the cluster evaluation scores across different numbers of clusters for optima or relevant changes in trend. 

For validation we applied this method to the output for the subpolar North Atlantic between 1993 and 1997 of the high-resolution Atlantic Ocean model VIKING20X, in direct exchange with domain experts to discuss the resulting clusters. Due to the change from strong to weak deep convection in these years, the hydrographic properties vary strongly in the time and depth dimension, providing a specific challenge to our methodology. 

Our findings suggest that it is possible to identify an optimal number of clusters using the off-the-shelf cluster evaluation scores that catch the underlying structure of the hydrographic space. The optimal number of clusters identified by our data-driven method agrees with the optimal number of clusters found by expert interviews. These findings contribute to aiding and objectifying water mass definitions across multiple expert decisions, and demonstrate the benefit of introducing data science methods to analyses in physical oceanography.

How to cite: Trahms, C., Wölker, Y., and Biastoch, A.: Objectively Determining the Number of Similar Hydrographic Clusters with Unsupervised Machine Learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11687, https://doi.org/10.5194/egusphere-egu23-11687, 2023.

EGU23-11906 | ECS | Orals | ITS1.13/AS5.2

Untapping the potential of geostationary EO data to understand drought impacts with XAI 

Basil Kraft, Gregory Duveiller, Markus Reichstein, and Martin Jung

Ecosystems are affected by extreme climate conditions such as droughts worldwide but we still lack understanding of the involved dynamics. Which factors render an ecosystem more resilient, and on which temporal scales do weather patterns affect vegetation state and physiology? Traditional approaches to tackle such questions involve assumption-based land surface modeling or inversions. Machine learning (ML) methods can provide a complementary perspective on how ecosystems respond to climate in a more data-driven and assumption-free manner. However, ML depends heavily on data, and commonly used observations of vegetation at best contain one observation per day, but most products are provided at 16-daily to monthly temporal resolution. This masks important processes at sub-monthly time scales. In addition, ML models are inherently difficult to interpret, which still limits their applicability for process understanding.

In the present study, we combine modern deep learning models in the time domain with observations from the geostationary Meteosat Second Generation (MSG) satellite, centered over Africa. We model fractional vegetation cover (representing vegetation state) and land surface temperature (as a proxy for water stress) from MSG as a function of meteorology and static geofactors. MSG collects observations at sub-daily frequency, rendering it into an excellent tool to study short- to mid-term land surface processes. Furthermore, we use methods from explainable ML for post-hoc model interpretation to identify meteorological drivers of vegetation dynamics and their interaction with key geofactors.

From the analysis, we expect to gather novel insights into ecosystem response to droughts with high temporal fidelity. Drought response of vegetation can be highly diverse and complex especially in arid to semi-arid regions prevalent in Africa. Also, we assess the potential of explainable machine learning to discover new linkages and knowledge and discuss potential pitfalls of the approach. Explainable machine learning, combined with potent deep learning approaches and modern Earth observation products offers the opportunity to complement assumption-based modeling to predict and understand ecosystem response to extreme climate.

How to cite: Kraft, B., Duveiller, G., Reichstein, M., and Jung, M.: Untapping the potential of geostationary EO data to understand drought impacts with XAI, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11906, https://doi.org/10.5194/egusphere-egu23-11906, 2023.

EGU23-11958 | ECS | Posters on site | ITS1.13/AS5.2

Modelling Soil Temperature and Soil Moisture in Space, Depth, and Time with Machine Learning Techniques 

Maiken Baumberger, Linda Adorf, Bettina Haas, Nele Meyer, and Hanna Meyer

Soil temperature and soil moisture variations have large effects on ecological processes in the soil. To investigate and understand these processes, high-resolution data of soil temperature and soil moisture are required. Here, we present an approach to generate data of soil temperature and soil moisture continuously in space, depth, and time for a 400 km² study area in the Fichtel Mountains (Germany). As reference data, measurements with 1 m long soil probes were taken. To cover many different locations, the available 15 soil probes were shifted regularly in the course of one year. With this approach, around 250 different locations in forest sites, on meadows and on agricultural fields were captured under a variety of meteorological conditions. These measurements are combined with readily available meteorological data, satellite data and soil maps in a machine learning approach to learn the complex relations between these variables. We aim for a model which can predict the soil temperature and soil moisture continuously for our study area in the Fichtel Mountains, with a spatial resolution of 10 m x 10 m, down to 1 m depth with segments of 10 cm each and in an hourly resolution in time. Here, we present the results of our pilot study where we focus on the temperature and moisture change within the depth down to 1 m at one single location. To take temporal lags into account, we construct a Long Short-Term Memory network based on meteorological data as predictors to make temperature and moisture predictions in time and depth. The results indicate a high ability of the model to reproduce the time series of the single location and highlight the potential of the approach for the space-time-depth mapping of soil temperature and soil moisture.

How to cite: Baumberger, M., Adorf, L., Haas, B., Meyer, N., and Meyer, H.: Modelling Soil Temperature and Soil Moisture in Space, Depth, and Time with Machine Learning Techniques, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11958, https://doi.org/10.5194/egusphere-egu23-11958, 2023.

EGU23-12218 | Posters on site | ITS1.13/AS5.2

Bias correction of aircraft temperature observations in the Korean Integrated Model based on a deep learning approach 

Hui-nae Kwon, Hyeon-ju Jeon, Jeon-ho Kang, In-hyuk Kwon, and Seon Ki Park

The aircraft-based observation is one of the important anchor data used in the numerical weather prediction (NWP) models. Nevertheless, the bias has been noted in the temperature observation through several previous studies. As the performance on the hybrid four-dimensional ensemble variational (hybrid-4DEnVar) data assimilation (DA) system of the Korean Integrated Model (KIM) ⸺ the operational model in the Korea Meteorological Administration (KMA) ⸺ has been advanced, the need for the aircraft temperature bias correction (BC) has been confirmed. Accordingly, as a preliminary study on the BC, the static BC method based on the linear regression was applied to the KIM Package for Observation Processing (KPOP) system. However, the results showed there were limitations of a spatial discontinuity and a dependency on the calculation period of BC coefficients.

In this study, we tried to develop the machine learning-based bias estimation model to overcome these limitations. The MultiLayer Perceptron (MLP) based learning was performed to consider the vertical, spatial and temporal characteristics of each observation by flight IDs and phases, and at the same time to consider the correlation among observation variables. As a result of removing the predicted bias from the bias estimation model, the mean of the background innovation (O-B) decreases from 0.2217 K to 0.0136 K in a given test period. Afterwards, in order to verify the analysis field impact for BC, the bias estimation model will be grafted onto the KPOP system and then several DA cycle experiments will be conducted in the KIM.

How to cite: Kwon, H., Jeon, H., Kang, J., Kwon, I., and Park, S. K.: Bias correction of aircraft temperature observations in the Korean Integrated Model based on a deep learning approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12218, https://doi.org/10.5194/egusphere-egu23-12218, 2023.

EGU23-12355 | ECS | Orals | ITS1.13/AS5.2

Comparison of NWP Models Used in Training Surrogate Wave Models 

Ajit Pillai, Ian Ashton, Jiaxin Chen, and Edward Steele

Machine learning is increasingly being applied to ocean wave modelling. Surrogate modelling has the potential to reduce or bypass the large computational requirements, creating a low computational-cost model that offers a high level of accuracy. One approach integrates in-situ measurements and historical model runs to achieve the spatial coverage of the model and the accuracy of the in-situ measurements. Once operational, such a system requires very little computational power, meaning that it could be deployed to a mobile phone, operational vessel, or autonomous vessel to give continuous data. As such, it makes a significant change to the availability of met-ocean data with potential to revolutionise data provision and use in marine and coastal settings.

This presentation explores the impact that an underlying physics-based model can have in such a machine learning driven framework; comparing training the system on a bespoke regional SWAN wave model developed for wave energy developments in the South West of the UK against training using the larger North-West European Shelf long term hindcast wave model run by the UK Met Office. The presentation discusses the differences in the underlying NWP models, and the impacts that these have on the surrogate wave models’ accuracy in both nowcasting and forecasting wave conditions at areas of interest for renewable energy developments. The results identify the importance in having a high quality, validated, NWP model for training such a system and the way in which the machine learning methods can propagate and exaggerate the underlying model uncertainties.

How to cite: Pillai, A., Ashton, I., Chen, J., and Steele, E.: Comparison of NWP Models Used in Training Surrogate Wave Models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12355, https://doi.org/10.5194/egusphere-egu23-12355, 2023.

EGU23-12403 | ECS | Orals | ITS1.13/AS5.2

PseudoSpectralNet: A hybrid neural differential equation for atmosphere models 

Maximilian Gelbrecht and Niklas Boers

When predicting complex systems such as parts of the Earth system, one typically relies on differential equations which often can be incomplete, missing unknown influences or include errors through their discretization. To remedy those effects, we present PseudoSpectralNet (PSN): a hybrid model that incorporates both a knowledge-based part of an atmosphere model and a data-driven part, an artificial neural network (ANN). PSN is a neural differential equation (NDE): it defines the right-hand side of a differential equation, combining a physical model with ANNs and is able to train its parameters inside this NDE. Similar to the approach of many atmosphere models, part of the model is computed in the spherical harmonics domain, and other parts in the grid domain. The model consists of ANN layers in each domain, information about derivatives, and parameters such as the orography. We demonstrate the capabilities of PSN on the well-studied Marshall Molteni Quasigeostrophic Model.

How to cite: Gelbrecht, M. and Boers, N.: PseudoSpectralNet: A hybrid neural differential equation for atmosphere models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12403, https://doi.org/10.5194/egusphere-egu23-12403, 2023.

EGU23-12458 | ECS | Posters on site | ITS1.13/AS5.2

Training Deep Data Assimilation Networks on Sparse and Noisy Observations 

Vadim Zinchenko and David Greenberg

Data Assimilation (DA) is a challenging and expensive computational problem targetting hidden variables in high-dimensional spaces. 4DVar methods are widely used in weather forecasting to fit simulations to sparse observations by optimization over numerical model input. The complexity of this inverse problem and the sequential nature of common 4DVar approaches lead to long computation times with limited opportunity for parallelization. Here we propose using machine learning (ML) algorithms to replace the entire 4DVar optimization problem with a single forward pass through a neural network that maps from noisy and incomplete observations at multiple time points to a complete system state estimate at a single time point. We train the neural network using a loss function derived from the weak-constraint 4DVar objective, including terms incorporating errors in both model and data. In contrast to standard 4DVar approaches, our method amortizes the computational investment of training to avoid solving optimization problems for each assimilation window, and its non-sequential nature allows for easy parallelization along the time axis for both training and inference. In contrast to most previous ML-based data assimilation methods, our approach does not require access to complete, noise-free simulations for supervised learning or gradient-free approximations such as Ensemble Kalman filtering. To demonstrate the potential of our approach, we show a proof-of-concept on the chaotic Lorenz'96 system, using a novel "1.5D Unet" architecture combining 1D and 2D convolutions.

How to cite: Zinchenko, V. and Greenberg, D.: Training Deep Data Assimilation Networks on Sparse and Noisy Observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12458, https://doi.org/10.5194/egusphere-egu23-12458, 2023.

EGU23-12566 | Posters on site | ITS1.13/AS5.2

Comparison of PM2.5 concentrations prediction model performance using Artificial Intelligence 

Kyung-Hui Wang, Chae-Yeon Lee, Ju-Yong Lee, Min-Woo Jung, Dong-Geon Kim, Seung-Hee Han, Dae-Ryun Choi, and Hui-young Yun

Since PM2.5 (particulate matter with an aerodynamic diameter of less than 2.5 µm) directly threatens public health, in order to take appropriate measures(prevention) in advance, the Korea Ministry of Environment(MOE) has been implementing PM10 forecast nationwide since February 2014. PM2.5 forecasts have been implemented nationwide since January 2015. The currently implemented PM forecast by the MOE subdivides the country into 19 regions, and forecasts the level of PM in 4 stages of “Good”, “Moderate”, “Unhealthy”, and “Very unhealthy”.

Currently PM air quality forecasting system operated by the MOE is based on a numerical forecast model along with a weather and emission model. Numerical forecasting model has fundamental limitations such as the uncertainty of input data such as emissions and meteorological data, and the numerical model itself. Recently, many studies on predicting PM using artificial intelligence such as DNN, RNN, LSTM, and CNN have been conducted to overcome the limitations of numerical models.

In this study, in order to improve the prediction performance of the numerical model, past observational data (air quality and meteorological data) and numerical forecasting model data (chemical transport model) are used as input data. The machine learning model consists of DNN and Seq2Seq, and predicts 3 days (D+0, D+1, D+2) using 6-hour and 1-hour average input data, respectively. The PM2.5 concentrations predicted by the machine learning model and the numerical model were compared with the PM2.5 measurements.

The machine learning models were trained for input data from 2015 to 2020, and their PM forecasting performance was tested for 2021. Compared to the numerical model, the machine learning model tended to increase ACC and be similar or lower to FAR and POD.

Time series trend was showed machine learning PM forecasting trend is more similar to PM measurements compared with numerical model. Especially, machine learning forecasting model can appropriately predict PM low and high concentrations that numerical model is used to overestimate.

Machine learning forecasting model with DNN and Seq2Seq can found improvement of PM forecasting performance compared with numerical forecasting model. However, the machine learning model has limitations that the model can not consider external inflow effects.

In order to overcome the drawback, the models should be updated and added some other machine learning module such as CNN with spatial features of PM concentrations.

 

Acknowledgements

This study was supported in part by the ‘Experts Training Graduate Program for Particulate Matter Management’ from the Ministry of Environment, Korea and by a grant from the National Institute of Environmental Research (NIER), funded by the Ministry of Environment (ME) of the Republic of Korea (NIER-2022-04-02-068).

 

How to cite: Wang, K.-H., Lee, C.-Y., Lee, J.-Y., Jung, M.-W., Kim, D.-G., Han, S.-H., Choi, D.-R., and Yun, H.: Comparison of PM2.5 concentrations prediction model performance using Artificial Intelligence, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12566, https://doi.org/10.5194/egusphere-egu23-12566, 2023.

EGU23-13013 | ECS | Posters on site | ITS1.13/AS5.2

Using cGAN for cloud classification from RGB pictures 

Markus Rosenberger, Manfred Dorninger, and Martin Weißmann

Clouds of all kinds play a large role in many atmospheric processes including, e.g. radiation and moisture transport, and their type allows an insight into the dynamics going on in the atmosphere. Hence, the observation of clouds from Earth's surface has always been important to analyse the current weather and its evolution during the day. However, cloud observations by human observers are labour-intensive and hence also costy. In addition to this, cloud classifications done by human observers are always subjective to some extent. Finding an efficient method for automated observations would solve both problems. Although clouds have already been operationally observed using satellites for decades, observations from the surface shed a light on a different set of characteristics. Moreover, the WMO also defined their cloud classification standards according to visual cloud properties when observations are done at the Earth’s surface. Thus, in this work a utilization of machine learning methods to classify clouds from RGB pictures taken at the surface is proposed. Explicitly, a conditional Generative Adversarial Network (cGAN) is trained to discriminate between 30 different categories, 10 for each cloud level - low, medium and high; Besides showing robust results in different image classification problems, an additional advantage of using a GAN instead of a classical convolutional neural network is that its output can also artificially enhance the size of the training data set. This is especially useful if the number of available pictures is unevenly distributed among the different classes. Additional background observations like cloud cover and cloud base height can also be used to further improve the performance of the cGAN. Together with a cloud camera, a properly trained cGAN can observe and classify clouds with a high temporal resolution of the order of seconds, which can be used, e.g. for model verification or to efficiently monitor the current status of the weather as well as its short-time evolution. First results will also be presented.

How to cite: Rosenberger, M., Dorninger, M., and Weißmann, M.: Using cGAN for cloud classification from RGB pictures, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13013, https://doi.org/10.5194/egusphere-egu23-13013, 2023.

EGU23-13143 | ECS | Posters on site | ITS1.13/AS5.2

Comparison of LSTM, GraphNN, and IrradPhyDNet based Approaches for High-resolution Solar Irradiance Nowcasting 

Petrina Papazek, Irene Schicker, and Pascal Gfähler

With fast parallel computing hardware, particularly GPUs, becoming more accessible in the geosciences the now efficiently running deep learning techniques are ready to handle larger amounts of recorded observation and satellite derived data and are able to learn complex structures across time-series. Thus, a suitable deep learning setup is able to generate highly-resolved weather forecasts in real-time and on demand. Forecasts of irradiance and radiation can be challenging in machine learning as they embrace a high degree of diurnal and seasonal variation.

Continuously extended PV/solar power production grows into one of our most important fossil-fuel free energy sources. Unlike the just recently emerging PV power observations, solar irradiance offers long time-series from automized weather station networks. Being directly linked to PV outputs, forecasting highly resolved solar irradiance from nowcasting to short-range plays a crucial role in decision support and managing PV.

In this study, we investigate the suitability of several deep learning techniques adopted and developed to a set of heterogeneous data sources on selected locations. We compare the forecast results to traditional – however computationally expensive - numerical weather prediction models (NWP) and rapid update cycle models. Relevant input features include 3D-fields from NWP models (e.g.: AROME), satellite data and products (e.g.: CAMS), radiation time series from remote sensing, and observation time time-series (site observations and close sites). The amount of time-series data can be extended by a synthetic data generator, a part of our deep learning framework. Our main models investigated includes a sequence-to-sequence LSTM (long-short-term-memory) model using a climatological background model or NWP for post-processing, a Graph NN model, and an analogs based deep learning method. Furthermore, a novel neural network model based on two other ideas, the IrradianceNet and the PhyDNet, was developed. IrradPhyDNet combines the skills of IrradianceNet and PhyDNet and showed improved performance in comparison to the original models.

Results obtained by the developed methods yield, in general, high forecast-skills. For selected case studies of extreme events (e.g. Saharan dust) all novel methods could outperform the traditional methods.  Different combinations of inputs and processing-steps are part of the analysis.

How to cite: Papazek, P., Schicker, I., and Gfähler, P.: Comparison of LSTM, GraphNN, and IrradPhyDNet based Approaches for High-resolution Solar Irradiance Nowcasting, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13143, https://doi.org/10.5194/egusphere-egu23-13143, 2023.

EGU23-13322 | ECS | Posters on site | ITS1.13/AS5.2

Nodal Ambient Noise Tomography and automatic picking of dispersion curves with convolutional neural network: case study at Vulcano-Lipari, Italy 

Douglas Stumpp, Elliot Amir Jiwani-Brown, Célia Barat, Matteo Lupi, Francisco Muñoz, Thomas Planes, and Geneviève Savard

The ambient noise tomography (ANT) method is widely adopted to reconstruct shear-wave velocity anomalies and to generate high-resolution images of the crust and upper-mantle. A critical step in this process is the extraction of surface-wave dispersion curves from cross-correlation functions of continuous ambient noise recordings, which is traditionally performed manually on the dispersion spectrograms through human-machine interfaces. Picking of dispersion curves is sometimes prone to bias due to human interpretation. Furthermore, it is a laborious and time-consuming task that needs to be resolved in an automatized manner, especially when dealing with dense seismic network of nodal geophones where the large amount of generated data severely hinders manual picking approaches. In the last decade, several studies successfully employed machine learning methods in Earth Sciences and across many seismological applications. Early studies have shown versatile and reliable solutions by treating dispersion curve extraction as a visual recognition problem. 

We review and adapt a specific machine learning approach, deep convolutional neural networks, for use on dispersion spectrograms generated with the usual frequency-time analysis (FTAN) processing on ambient noise cross-correlations. To train and calibrate the algorithm we use several available datasets acquired from previous experiments across different geological settings. The main dataset consists of records acquired with a dense local geophone network (150 short period stations sampling at 250 Hz) deployed for one month in October 2021. The dataset has been acquired during the volcanic unrest of the Vulcano-Lipari complex, Italy. The network also accounts for additional 17 permanent broadband stations (sampling at 100 Hz) maintained by the National Institute of Geophysics and Volcanology (INGV) in Italy. We evaluate the performance of the dispersion curves extraction algorithm. The automatically-picked dispersion curves will be used to construct a shear-wave velocity model of the Vulcano-Lipari magmatic plumbing system and the surrounding area of the Aeolian archipelago.

 

How to cite: Stumpp, D., Amir Jiwani-Brown, E., Barat, C., Lupi, M., Muñoz, F., Planes, T., and Savard, G.: Nodal Ambient Noise Tomography and automatic picking of dispersion curves with convolutional neural network: case study at Vulcano-Lipari, Italy, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13322, https://doi.org/10.5194/egusphere-egu23-13322, 2023.

EGU23-13367 | ECS | Posters on site | ITS1.13/AS5.2

Framework for creating daily semantic segmentation maps of classified eddies using SLA along-track altimetry data 

Eike Bolmer, Adili Abulaitijiang, Luciana Fenoglio-Marc, Jürgen Kusche, and Ribana Roscher

Mesoscale eddies are gyrating currents in the ocean and have horizontal scales from 10 km up to 100 km and above. They transport water mass, heat, and nutrients and therefore are of interest among others to marine biologists, oceanographers, and geodesists. Usually, gridded sea level anomaly maps, processed from several radar altimetry missions, are used to detect eddies. However, operational processors create multi-mission (processing level 4) SLA grid maps with an effective spatiotemporal resolution far lower than their grid spacing and temporal resolution. 

This drawback leads to erroneous eddy detection. We, therefore, investigate if the higher-resolution along-track data could be used instead to solve the problem of classifying the SLA observations into cyclonic, anticyclonic, or no eddies in a more accurate way than using processed SLA grid map products. With our framework, we aim to infer a daily two-dimensional segmentation map of classified eddies. Due to repeat cycles between 10 and 35 days and cross-track spacing of a few 10 km to a few 100 km, ocean eddies are clearly visible in altimeter observations but are typically covered only by a few ground tracks where the spatiotemporal context within the input data is highly variable each day. However conventional convolutional neural networks (CNNs) rely on data without varying gaps or jumps in time and space in order to use the intrinsic spatial or temporal context of the observations. Therefore, this is a challenge that needs to be addressed with a deep neural network that on the one hand utilizes the spatiotemporal context information within the modality of along-track data and on the other hand is able to output a two-dimensional segmentation map from data of varying sparsity. Our approach with our architecture Teddy is to use a transformer module to encode and process the spatiotemporal information along with the ground track's sea level anomaly data that produces a sparse feature map. This will then be fed into a sparsity invariant convolutional neural network in order to infer a two-dimensional segmentation map of classified eddies. Reference data that is used to train Teddy is produced by an open-source geometry-based approach (py-eddy-tracker [1]). 

The focus of this presentation is on how we implemented this approach in order to derive two-dimensional segmentation maps of classified eddies with our deep neural network architecture Teddy from along-track altimetry. We show results and limitations for the classification of eddies using only along-track SLA data from the multi-mission level 3 product of the Copernicus Marine Environment Monitoring Service (CMEMS) within the 2017 - 2019 period for the Gulf Stream region. We find that using our methodology, we can create two-dimensional maps of classified eddies from along-track data without using preprocessed SLA grid maps.

[1] Evan Mason, Ananda Pascual, and James C. McWilliams, “A new sea surface height–based code for oceanic mesoscale eddy tracking,” Journal of Atmospheric and Oceanic Technology, vol. 31, no. 5, pp. 1181–1188, 2014.

How to cite: Bolmer, E., Abulaitijiang, A., Fenoglio-Marc, L., Kusche, J., and Roscher, R.: Framework for creating daily semantic segmentation maps of classified eddies using SLA along-track altimetry data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13367, https://doi.org/10.5194/egusphere-egu23-13367, 2023.

EGU23-13771 | Orals | ITS1.13/AS5.2

Machine Learning Emulation of 3D Shortwave Radiative Transfer for Shallow Cumulus Cloud Fields 

Jui-Yuan Christine Chiu, Chen-Kuang Kevin Yang, Jake J. Gristey, Graham Feingold, and William I. Gustafson

Clouds play an important role in determining the Earth’s radiation budget. Despite their complex and three-dimensional (3D) structures, their interactions with radiation in models are often simplified to one-dimensional (1D), considering the time required to compute radiative transfer. Such a simplification ignores cloud Inhomogeneity and horizontal photon transport in radiative processes, which may be an acceptable approximation for low-resolution models, but can lead to significant errors and impact cloud evolution predictions in high-resolution simulations. Since model developments and operations are heading toward a higher resolution that is more susceptible to radiation errors, a fast and accurate 3D radiative transfer scheme becomes important and necessary. To address the need, we develop a machine-learning-based 3D radiative transfer emulator to provide surface radiation, shortwave fluxes at all layers, and heating rate profiles. The emulators are trained for highly heterogeneous shallow cumulus under different solar positions. We will discuss the performance of the emulators in accuracy and efficiency and discuss their potential applications.

How to cite: Chiu, J.-Y. C., Yang, C.-K. K., Gristey, J. J., Feingold, G., and Gustafson, W. I.: Machine Learning Emulation of 3D Shortwave Radiative Transfer for Shallow Cumulus Cloud Fields, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13771, https://doi.org/10.5194/egusphere-egu23-13771, 2023.

EGU23-14051 | ECS | Posters on site | ITS1.13/AS5.2

Multi-modal data assimilation of sea surface currents from AIS data streams and satellite altimetry using 4DVARNet 

Simon Benaïchouche, Clément Le Goff, Brahim Boussidi, François Rousseau, and Ronan Fablet

Over the last decades, space oceanography missions, particularly altimeter missions, have greatly advanced our ability to observe sea surface dynamics. However, they still struggle to resolve spatial scales below ~ 100 km. On a global scale, sea surface current are derived from sea surface height by a geostrophical assumption. While future altimeter missions should improve the observation of sea surface height, the observation of sea surface current using altimetry techniques would remains indirect. In the other hands, recent works have considered the use of AIS (automated identification system) as a new mean to reconstruct sea surface current : AIS data streams provide an indirect observational models of total currents including ageostrophic phenomenas. In this work we consider the use of the supervised learning framework 4DVARNet, a supervised data driven approach that allow us to perform multi-modal experiments : We focus on an Observing System Simulation Experiment (OSSE) in a region of the Gulf-Stream and we show that the joint use of AIS and sea surface height (SSH) measurement could improve the reconstruction of sea surface current with respect to product derived solely from AIS or SSH observations in terms of physical and time scale resolved. 

How to cite: Benaïchouche, S., Le Goff, C., Boussidi, B., Rousseau, F., and Fablet, R.: Multi-modal data assimilation of sea surface currents from AIS data streams and satellite altimetry using 4DVARNet, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14051, https://doi.org/10.5194/egusphere-egu23-14051, 2023.

EGU23-15183 | ECS | Orals | ITS1.13/AS5.2

Deep learning approximations of a CFD model for operational wind and turbulence forecasting 

Margrethe Kvale Loe and John Bjørnar Bremnes

The Norwegian Meteorological Institute has for many years applied a CFD model to downscale operational NWP forecasts to 100-200m spatial resolution for wind and turbulence forecasting for about 20 Norwegian airports. Due to high computational costs, however, the CFD model can only be run twice per day, each time producing a 12-hour forecast. An approximate approach requiring far less compute resources using deep learning has therefore been developed. In this, the relation between relevant NWP forecast variables at grids of 2.5 km spatial resolution and wind and turbulence from the CFD model has been approximated using neural networks with basic convolutional and dense layers. The deep learning models have been trained on approximately two year of the data separately for each airport. The results show that the models are to a large extent able to capture the characteristics of their corresponding CDF simulations, and the method is in due time intended to fully replace the current operational solution. 

How to cite: Loe, M. K. and Bremnes, J. B.: Deep learning approximations of a CFD model for operational wind and turbulence forecasting, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15183, https://doi.org/10.5194/egusphere-egu23-15183, 2023.

EGU23-15684 | ECS | Posters on site | ITS1.13/AS5.2

Semi-supervised feature-based learning for prediction of Mass Accumulation Rate of sediments 

Naveenkumar Parameswaran, Everardo Gonzalez, Ewa Bur­wicz-Ga­ler­ne, David Greenberg, Klaus Wallmann, and Malte Braack

Mass accumulation rates of sediments[g/cm2/yr] or sedimentation rates[cm/yr] on the seafloor are important to understand various benthic properties, like the rate of carbon sequestration in the seafloor and seafloor geomechanical stability. Several machine learning models, such as random forests, and k-Nearest Neighbours have been proposed for the prediction of geospatial data in marine geosciences, but face significant challenges such as the limited amount of labels for training purposes, skewed data distribution, a large number of features etc. Previous model predictions show deviation in the global sediment budget, a parameter used to determine a model's predicitve validity, revealing the lack of accurate representation of sedimentation rate by the state of the art models. 

Here we present a semi-supervised deep learning methodology to improve the prediction of sedimentation rates, making use of around 9x106  unlabelled data points. The semi-supervised neural network implementation has two parts: an unsupervised pretraining using an encoder-decoder network. The encoder with the optimized weights from the unsupervised training is then taken out and fitted with layers that lead to the target dimension. This network is then fine-tuned with 2782 labelled data points, which are observed sedimentation rates from peer-reviewed sources. The fine-tuned model then predicts the rate and quantity of sediment accumulating on the ocean floor, globally.

The developed semi-supervised neural network provide better predictions than supervised models trained only on labelled data. The predictions from the semi-supervised neural network are compared with that of the supervised neural network with and without dimensionality reduction(using Principle Component Analysis).

How to cite: Parameswaran, N., Gonzalez, E., Bur­wicz-Ga­ler­ne, E., Greenberg, D., Wallmann, K., and Braack, M.: Semi-supervised feature-based learning for prediction of Mass Accumulation Rate of sediments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15684, https://doi.org/10.5194/egusphere-egu23-15684, 2023.

EGU23-15756 | ECS | Posters on site | ITS1.13/AS5.2

Physiography improvements in numerical weather prediction digital twin engines 

Thomas Rieutord, Geoffrey Bessardon, and Emily Gleeson

The next generation of numerical weather prediction model (so-called digital twin engines) will reach hectometric scale, for which the existing physiography databases are insufficient. Our work leverages machine learning and open-access data to produce a more accurate and higher resolution physiography database. One component to improve is the land cover map. The reference data gathers multiple high-resolution thematic maps thanks to an agreement-based decision tree. The input data are taken from the Sentinel-2 satellite. Then, the land cover map generation is made with image segmentation. This work implements and compares several algorithms of different families to study their suitability to the land cover classification problem. The sensitivity to the data quality will also be studied. Compared to existing work, this work is innovative in the reference map construction (both leveraging existing maps and fit for end-user purpose) and the diversity of algorithms to produce our land cover map comparison.

How to cite: Rieutord, T., Bessardon, G., and Gleeson, E.: Physiography improvements in numerical weather prediction digital twin engines, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15756, https://doi.org/10.5194/egusphere-egu23-15756, 2023.

EGU23-15892 | ECS | Posters on site | ITS1.13/AS5.2

Towards emulated Lagrangian particle dispersion model footprints for satellite observations 

Elena Fillola, Raul Santos-Rodriguez, and Matt Rigby

Lagrangian particle dispersion models (LPDMs) have been used extensively to calculate source-receptor relationships (“footprints”) for use in greenhouse gas (GHG) flux inversions. However, because a backward-running model simulation is required for each data point, LPDMs do not scale well to very large datasets, which makes them unsuitable for use in GHG inversions using high-resolution satellite instruments such as TROPOMI. In this work, we demonstrate how Machine Learning (ML) can be used to accelerate footprint production, by first presenting a proof-of-concept emulator for ground-based site observations, and then discussing work in progress to create an emulator suitable to satellite observations. In Fillola et al (2023), we presented a ML emulator for NAME, the Met Office’s LPDM, which outputs footprints for a small region around an observation point using purely meteorological variables as inputs. The footprint magnitude at each grid cell in the domain is modelled independently using gradient-boosted regression trees. The model is evaluated for seven sites, producing a footprint in 10ms, compared to around 10 minutes for the 3D simulator, and achieving R2 values between 0.6 and 0.8 for CH4 concentrations simulated at the sites when compared to the timeseries generated by NAME. Following on from this work, we demonstrate how this same emulator can be applied to satellite data to reproduce footprints immediately around any measurement point in the domain, evaluating this application with data for Brazil and North Africa and obtaining R2 values of around 0.5 for simulated CH4 concentrations. Furthermore, we propose new emulator architectures for LPDMs applied to satellite observations. These new architectures should tackle some of the weaknesses in the existing approach, for example, by propagating information more flexibly in space and time, potentially improving accuracy of the derived footprints and extending the prediction capabilities to bigger domains.

How to cite: Fillola, E., Santos-Rodriguez, R., and Rigby, M.: Towards emulated Lagrangian particle dispersion model footprints for satellite observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15892, https://doi.org/10.5194/egusphere-egu23-15892, 2023.

EGU23-15994 | ECS | Posters on site | ITS1.13/AS5.2

Uncertainty quantification in variational data assimilation with deep learning 

Nicolas Lafon, Philippe Naveau, and Ronan Fablet

The spatio-temporal reconstruction of a dynamical process from some observationaldata is at the core of a wide range of applications in geosciences. This is particularly true for weather forecasting, operational oceanography and climate studies. However, the re35 construction of a given dynamic and the prediction of future states must take into ac36 count the uncertainties that affect the system. Thus, the available observational measurements are only provided with a limited accuracy. Besides, the encoded physical equa38 tions that model the evolution of the system do not capture the full complexity of the real system. Finally, the numerical approximation generates a non-negligible error. For these reasons, it seems relevant to calculate a probability distribution of the state system rather than the most probable state. Using recent advances in machine learning techniques for inverse problems, we propose an algorithm that jointly learns a parametric distribution of the state, the dynamics governing the evolution of the parameters, and a solver. Experiments conducted on synthetic reference datasets, as well as on datasets describing environmental systems, validate our approach.

How to cite: Lafon, N., Naveau, P., and Fablet, R.: Uncertainty quantification in variational data assimilation with deep learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15994, https://doi.org/10.5194/egusphere-egu23-15994, 2023.

EGU23-16287 | ECS | Posters on site | ITS1.13/AS5.2

A machine learning emulator for forest carbon stocks and fluxes 

Carolina Natel de Moura, David Martin Belda, Peter Antoni, and Almut Arneth

Forests are a significant carbon sink of the total carbon dioxide (CO2) emitted by humans. Climate change is expected to impact forest systems, and their role in the terrestrial carbon cycle in several ways – for example, the fertilization effect of increased atmospheric CO2, and the lengthening of the growing season in northern temperate and boreal areas may increase forest productivity, while more frequent extreme climate events such as storms and windthrows or drought spells, as well as wildfires might reduce disturbances return period, hence increasing forest land loss and reduction of the carbon stored in the vegetation and soils. In addition, forest management in response to an increased demand for wood products and fuel can affect the carbon storage in ecosystems and wood products. State-of-the-art Dynamic Global Vegetation Models (DGVMs) simulate the forest responses to environmental and human processes, however running these models globally for many climate and management scenarios becomes challenging due to computational restraints. Integration of process-based models and machine learning methods through emulation allows us to speed up computationally expensive simulations. In this work, we explore the use of machine learning to surrogate the LPJ-GUESS DGVM. This emulator is spatially-aware to represent forests across the globe in a flexible spatial resolution, and consider past climate and forest management practices to account for legacy effects. The training data for the emulator is derived from dedicated runs of the DGVM sampled across four dimensions relevant to forest carbon and yield: atmospheric CO2 concentration, air Temperature, Precipitation, and forest Management (CTPM). The emulator can capture relevant forest responses to climate and management in a lightweight form, and will support the development of the coupled socio-economic/ecologic model of the land system, namely LandSyMM (landsymm.earth). Other relevant scientific applications include the analysis of optimal forestry protocols under climate change, and the forest potential in climate change mitigation.

 

How to cite: Natel de Moura, C., Belda, D. M., Antoni, P., and Arneth, A.: A machine learning emulator for forest carbon stocks and fluxes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16287, https://doi.org/10.5194/egusphere-egu23-16287, 2023.

EGU23-16597 | Posters on site | ITS1.13/AS5.2 | Highlight

Global Decadal Sea Surface Height Forecast with Conformal Prediction 

Nils Lehmann, Jonathan Bamber, and Xiaoxiang Zhu

One of the many ways in which anthropogenic climate change impacts our planet is
rising sea levels. The rate of sea level rise (SLR) across the oceans is,
however, not uniform in space or time and is influenced by a complex interplay
of ocean dynamics, heat uptake, and surface forcing. As a consequence,
short-term (years to a decade) regional SLR patterns are difficult to model
using conventional deterministic approaches. For example, the latest climate
model projections (called CMIP6) show some agreement in the globally integrated
rate of SLR but poor agreement when it comes to spatially-resolved
patterns. However, such forecasts are valuable for adaptation planning in
coastal areas and for protecting low lying assets.
Rather than a deterministic modeling approach, here we explore the possibility
of exploiting the high quality satellite altimeter derived record of sea surface
height variations, which cover the global oceans outside of ice-infested waters
over a period of 30 years. Alongside this rich and unique satellite record,
several data-driven models have shown tremendous potential for various
applications in Earth System science. We explore several data-driven deep
learning approaches for sea surface height forecasts over multi-annual to
decadal time frames. A limitation of some machine learning approaches is the
lack of any kind of uncertainty quantification, which is problematic for
applications where actionable evidence is sought. As a consequence, we equip
our models with a rigorous measure of uncertainty, namely conformal prediction which
is a model and dataset agnostic method that provides calibrated predictive
uncertainty with proven coverage guarantees. Based on a 30-year satellite
altimetry record and auxiliary climate forcing data from reanalysis such as
ERA5, we demonstrate that our methodology is a viable and attractive alternative
for decadal sea surface height forecasts.

How to cite: Lehmann, N., Bamber, J., and Zhu, X.: Global Decadal Sea Surface Height Forecast with Conformal Prediction, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16597, https://doi.org/10.5194/egusphere-egu23-16597, 2023.

EGU23-16936 | ECS | Orals | ITS1.13/AS5.2

Analysis of marine heat waves using machine learning 

Said Ouala, Bertrand Chapron, Fabrice Collard, Lucile Gaultier, and Ronan Fablet

Sea surface temperature (SST) is a critical parameter in the global climate system and plays a vital role in many marine processes, including ocean circulation, evaporation, and the exchange of heat and moisture between the ocean and atmosphere. As such, understanding the variability of SST is important for a range of applications, including weather and climate prediction, ocean circulation modeling, and marine resource management.

The dynamics of SST is the compound of multiple degrees of freedom that interact across a continuum of Spatio-temporal scales. A first-order approximation of such a system was initially introduced by Hasselmann. In his pioneering work, Hasselmann (1976) discussed the interest in using a two-scale stochastic model to represent the interactions between slow and fast variables of the global ocean, climate, and atmosphere system. In this paper, we examine the potential of machine learning techniques to derive relevant dynamical models of Sea Surface Temperature Anomaly (SSTA) data in the Mediterranean Sea. We focus on the seasonal modulation of the SSTA and aim to understand the factors that influence the temporal variability of SSTA extremes. Our analysis shows that the variability of the SSTA can indeed well be decomposed into slow and fast components. The dynamics of the slow variables are associated with the seasonal cycle, while the dynamics of the fast variables are linked to the SSTA response to rapid underlying processes such as the local wind variability. Based on these observations, we approximate the probability density function of the SSTA data using a stochastic differential equation parameterized by a neural network. In this model, the drift function represents the seasonal cycle and the diffusion function represents the envelope of the fast SSTA response.

 

How to cite: Ouala, S., Chapron, B., Collard, F., Gaultier, L., and Fablet, R.: Analysis of marine heat waves using machine learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16936, https://doi.org/10.5194/egusphere-egu23-16936, 2023.

EGU23-1254 | ECS | Orals | AS5.3

Balanced data assimilation with a blended numerical model 

Ray Chew, Tommaso Benacchio, Gottfried Hastermann, and Rupert Klein

Physical imbalances introduced by local sequential Bayesian data assimilation pose a problem for numerical weather prediction. For example, fast-mode acoustic imbalances of the order of the relevant slower dynamics destroy solution quality. We introduce a novel dynamics-driven method that suppresses imbalances arising from data assimilation. Specifically, we employ a blended numerical model with seamless access to compressible, soundproof, and hydrostatic dynamics. After careful numerical and asymptotic analysis, we introduce a one-step blending strategy to switch between model regimes within a simulation run. Upon assimilation of data, the model configuration is switched for one timestep to the limit soundproof pseudo-incompressible or hydrostatic regime. After that, the model configuration is switched back to the compressible regime for the duration of the assimilation window. The switching between model regimes is repeated for each subsequent assimilation window. Idealised experiments involving the travelling vortex, buoyancy-driven rising thermals, and internal gravity wave pulses demonstrate that our method successfully eliminates imbalances from data assimilation, yielding up to two orders-of-magnitude improvements in the analysis fields. While our studies involved eliminating acoustic and hydrostatic imbalances, this novel dynamics-driven method of achieving balanced data assimilation can be extended to eliminate other undesired imbalances, with significant prospective applications in real-world weather prediction.

How to cite: Chew, R., Benacchio, T., Hastermann, G., and Klein, R.: Balanced data assimilation with a blended numerical model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1254, https://doi.org/10.5194/egusphere-egu23-1254, 2023.

EGU23-1688 | Orals | AS5.3

Implementation Of The Novel Duo-Grid Within The GFDL FV3 Dynamical Core 

Joseph Mouallem and Lucas Harris

The current edge handling of the cubed sphere grid introduces numerical errors in simulations and creates grid imprinting due to the discontinuity of the great­-circle grid lines between two adjacent tiles. In this work, we implement a new edge/corner handling method to greatly reduce the grid imprinting in GFDL's dynamical core FV3. First, we extend on the duo-grid method (Chen 2021) to support halo updates of staggered variables. Second, we implement a corner handling algorithm to fill the corner regions using a lagrangian polynomial interpolation. Results of idealized shallow water test cases show that the new halo update methods are able to reduce the numerical noise at the edges/corners and thus reduce the grid imprinting in the numerical solution. This improvement is especially useful for coarse-grid models such as climate models in which the cube edges are most noticeable.

How to cite: Mouallem, J. and Harris, L.: Implementation Of The Novel Duo-Grid Within The GFDL FV3 Dynamical Core, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1688, https://doi.org/10.5194/egusphere-egu23-1688, 2023.

EGU23-1841 | ECS | Posters on site | AS5.3

AtmoFlow: Thermo-electrohydrodynamic convection in the thermally driven spherical shell with differential rotation 

Yann Gaillard, Peter Szabo, and Christoph Egbers

In a geophysical point of view, large scale prediction of atmospheric flows become more and more important to forecast e.g. extreme weather conditions that are observed in recent days more frequent and may relate to the overall climate change.  The AtmoFlow experiment is a small scaled laboratory spherical shell to investigate such atmospheric flow fields in a miniaturized model of a planet. Besides this physical experiment, numerical simulations are performed to analyze the resulting convective patterns in more detail. The experiment is composed of two spherical shells, which can rotate independently. The temperature on the shell's surface can be defined as a heated equator and a cooled pole. To model the terrestrial gravitation, an electric potential is applied on a dielectric fluid confined between the shells. This so called dielectrophoretic force triggers the formation of buoyant patterns, and is in fact the artificial equivalent of terrestrial gravitation. 


The simulations are processed with a custom programmed solver in the OpenFOAM ecosystem. It covers all predefined rotation combinations starting with no rotation, solid body rotation and differential rotation. The latter are the latest results of the computational simulation campaign and used to investigate the influence of the artificial central force field to differential rotation. While differential rotation can cause the well known Taylor vortices, it has to be noted that the cell formation induced by the central dielectrophoretic force field maybe significantly extubated and thus new convection patterns may arise.  This in fact is the overall focus of this study to understand the underlying physical process of such pattern formations. The analyses focus first on the amount of convective heat that these patterns are able to transport, and second to quantify their shape and intensity via a spatial Fast Fourier Transformation to identify the most dominant structures. Finally, statistical moments will provide an estimation about the shape and location of vacillating patterns.

How to cite: Gaillard, Y., Szabo, P., and Egbers, C.: AtmoFlow: Thermo-electrohydrodynamic convection in the thermally driven spherical shell with differential rotation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1841, https://doi.org/10.5194/egusphere-egu23-1841, 2023.

EGU23-2394 | Orals | AS5.3

Coupling simple dry physics to a dynamically adaptive global atmosphere model 

Nicholas Kevlahan, Gabrielle Ching-Johnson, and Thomas Dubos

Adaptive global circulation models (GCMs) have the potential to significantly improve the computational efficiency and accuracy of climate simulations by dynamically adjusting the local grid resolution to ensure a specified numerical tolerance or to track features of interest.  We have developed the global dynamical cores WAVETRISK-ATMOSPHERE and WAVETRISK-OCEAN to explore the strengths and weaknesses of dynamical GCMs. 

The main open challenge of adaptive climate modelling is how to appropriately couple the dynamical core to the physics. The physics should ideally be “scale-aware”: adjusting the parameterization as necessary based on the current local resolution (or disabling it entirely if the physical phenomenon becomes fully resolved).  A related question is whether the grid adaptation criteria should be based on the physics as well as the dynamics. Such scale-aware physics parameterizations remain poorly understood.  In this talk we report on initial progress in coupling WAVETRISK-ATMOSPHERE to Hourdin’s (1992) “simple dry physics”.

A better understanding of scale-aware physics will also improve non-adaptive climate modelling, since such models currently require extensive tuning each time the resolution is increased. An additional goal of this project is to develop a set of test cases for the simple physics that could be used to compare dynamical cores using a well-understood and standardized physics package.

This is joint work with Gabrielle Ching-Johnson (MSc student, McMaster University, Canada) and Thomas Dubos (LMD, École Polytechnique, France)

How to cite: Kevlahan, N., Ching-Johnson, G., and Dubos, T.: Coupling simple dry physics to a dynamically adaptive global atmosphere model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2394, https://doi.org/10.5194/egusphere-egu23-2394, 2023.

EGU23-3029 | Posters on site | AS5.3

Apply a positivity-preserving limiter of spectral element method to KIM 

Hyun Nam and Suk-Jin Choi

 As for a tracer transport scheme, the spectral element method (SEM) has a good accuracy in the  L2-norm error analysis since it uses relatively high-order continuous polynomials. However, the fact  that the basis functions for SEM are globally continuous makes it difficult to preserve important property such as positivity of tracer advection, which results in oscillations in numerical solutions. Moreover, this may cause difficulties in maintaining conservation of mass in long-term integration. Therefore, in many studies, many efforts have been made to reduce or eliminate these oscillations. Among them, this study attempts to apply a positivity-preserving limiter used in finite volume and discontinuous finite element method to SEM. It was proposed by Zhang and Shu (2010) in the highorder positivity-preserving discontinuous Galerkin schemes without losing local conservation or high-order accuracy. 

 The Korean Integrated Model (KIM) is employing SEM for a tracer transport scheme and has a kind of sign-preserving limiter to reduce oscillations currently (Guba et al.). The limiter prevents all undershoots up to machine precision in a highly deformational advection test case. As a primary result, this study aims to analyze the numerical results in terms of accuracy, mass conservation, oscillation magnitude, comparing to two types of limiters (positivity-preserving limiter & sign-preserving limiter) with original one of KIM. 

How to cite: Nam, H. and Choi, S.-J.: Apply a positivity-preserving limiter of spectral element method to KIM, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3029, https://doi.org/10.5194/egusphere-egu23-3029, 2023.

EGU23-3660 | ECS | Posters on site | AS5.3

Moisture with Gusto: towards moist shallow water test cases using the Gusto dynamical core toolkit 

Nell Hartney, Jemma Shipton, and Thomas Bendall

The shallow water equations are widely used in the development of weather and climate models, being computationally cheap while still retaining many pertinent features of atmospheric dynamics. The usual shallow water equations, however, model a ‘dry’ atmosphere and so neglect moist processes and moisture effects. Including moisture in the shallow water system offers a framework in which to develop more challenging test cases for parallel time-stepping schemes, arising through numerical complexities that moisture introduces and relevant because of changing trends in supercomputer architectures necessitating interest in parallel-in-time. This talk will discuss the implementation of moist shallow water models in the dynamical core toolkit Gusto, which mirrors the compatible finite element approach being taken in the next-generation UK Met Office model. We will highlight the advantages Gusto offers for rapid prototyping and flexible implementation of different moist shallow water models and describe progress towards running moist shallow water tests cases (both from the literature and newly-devised for this purpose) in Gusto.

How to cite: Hartney, N., Shipton, J., and Bendall, T.: Moisture with Gusto: towards moist shallow water test cases using the Gusto dynamical core toolkit, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3660, https://doi.org/10.5194/egusphere-egu23-3660, 2023.

We introduce a stochastic representation of the rotating shallow water equations and a corresponding structure preserving finite element discretization in Firedrake. The stochastic flow model follows from using a stochastic transport principle and a decomposition of the fluid flow into a large-scale component and a noise term that models the unresolved flow components. Similarly to the deterministic case, this stochastic model (denoted as modeling under location uncertainty (LU)) conserves the global energy of any realization. Consequently, it permits us to generate an ensemble of physically relevant random simulations with a good trade-off between the representation of the model error and the ensemble's spread. Applying a compatible finite element discretisation of the deterministic part of the equations combined with a standard weak finite element discretization of the stochastic terms, the resulting stochastic scheme preserves (spatially) the total energy. To address the enstrophy accumulation at the grid scale, we applied an anticipated potential vorticity method (APVM) to stabilize the stochastic scheme. Using this setup, we compare different realizations of noise parametrizations in the context of geophysical flow phenomena and study potential pathways to fully energy preserving stochastic discretizations.

How to cite: Bauer, W. and Li, L.: Towards compatible finite element discretizations of stochastic rotating shallow water equations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4133, https://doi.org/10.5194/egusphere-egu23-4133, 2023.

EGU23-4139 | Posters on site | AS5.3

The double-ITCZ problem in CMIP6 and the influences of deep convection and model resolution 

Shuyun Zhao, Xinyu Ma, Hua Zhang, and Wuke Wang

The double Intertropical Convergence Zone (ITCZ) bias is an outstanding bias in many climate models. This work assesses the annual-mean double-ITCZ problem in the models participating in the Coupled Model Intercomparison Project Phase 6 (CMIP6) based on several quantitative indices. Within the forty-six CMIP6 models, nine models from mainland China are evaluated as a group to verify the effort of model development from one perspective. The double-ITCZ bias and its large inter-model spread still exist in CMIP6 models. The overall performance of the models from Chinese mainland is similar with all CMIP6 models. It is found that the top-five models with relatively low double-ITCZ biases can effectively restrain the frequency of deep convection and related sea surface temperature (SST) bias in the southeastern Pacific dry subsidence region, which highlights the necessity of improving convective physics in climate models. Impacts of model resolution on the double-ITCZ problem are examined by comparing the high- and low-resolution groups in CMIP6 and High Resolution Model Intercomparison Project (HighResMIP) historical experiments, respectively. Increased resolution in atmospheric models is found to be able to reduce the positive precipitation bias over the tropical southern Atlantic, and improve the simulation of deep convection frequency and convective precipitation ratio there. However, the double-ITCZ bias over the Pacific is not improved significantly by increased resolution.

How to cite: Zhao, S., Ma, X., Zhang, H., and Wang, W.: The double-ITCZ problem in CMIP6 and the influences of deep convection and model resolution, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4139, https://doi.org/10.5194/egusphere-egu23-4139, 2023.

EGU23-7333 | Orals | AS5.3

Acceleration of the non-hydrostatic dynamical core of RegCM using GPUs 

Alessio Sclocco, Gijs van den Oord, Graziano Giuliani, Ivan Girotto, Erwan Raffin, and Ben van Werkhoven

Within the ESiWACE-2 project, a work package was dedicated toward providing services to the European earth system modeling community; the primary aspect of these services was the advancement of weather and climate model components towards exascale hardware architectures. As the bulk of this software is MPI-parallelized Fortran code, significant leaps have to be made in design and engineering to utilize the potential of e.g. GPU-equipped supercomputers that constitute the majority of (pre-)exascale systems that will emerge in the near future in Europe. The service was organized in the form of a call for projects, where awarded modeling groups would benefit from a 6 person-month collaboration with HPC experts within the ESiWACE consortium.

One such project has been the regional climate model RegCM, a state of the art limited area model, developed by the Earth System Physics section of the Abdus Salam International Centre for Theoretical Physics (ICTP) for long-term regional climate simulation. RegCM has participated in numerous intercomparison projects and is designed to be a public, open source, user-friendly and portable code that can be applied to any region of the world. The RegCM userbase extends beyond Europe, both toward industrialized countries (e.g. the US) as well as developing nations. Its development iteration has seen the addition of a non-hydrostatic dynamical core which, coupled with model 1D packages solving the sub-grid scale physics of convection, water phase change, boundary layer, short and long wave solar and long wave earth radiation interaction, permit the model a time integration to produce a climate scenario simulation. The model has an internal coupling with a surface community land model for atmosphere surface interaction description (CLM4.5).

Within the ESiWACE-2 service project, we have accelerated this dynamical core to GPUs using the OpenACC programming model. Within the limited timeframe we have adopted three main optimizations: (i) the restructuring of zonal and meridional advection loops to expose full three-dimensional parallelism, (ii) the use of direct GPU-to-GPU communication through device-aware MPI calls, and (iii) the minimization of GPU-CPU exchanges by excluding any data transfers back to the host, except for I/O and physics parameterizations.

Using these programming techniques, we were able to construct a dynamical core for RegCM that runs exclusively on the GPU. For benchmarking, we use the ‘Alps’ test case, a 3km-resolution mesh with ~14M grid columns over the Alpine region, representative of the future convection permitting model configurations. Benchmarks on the JUWELS-Booster supercomputer show an acceleration by more than a factor of two at low node counts (1-3) which diminishes when higher node allocations are used; at 8 nodes, both CPU- and GPU-versions have comparable speed. For the previous-generation system Marconi-100, the accelerated version is observed to be consistently faster by a factor ~2.7.

Looking forward, performance profiles indicate that the GPU-resident code is mostly bound by MPI-communication latency within the advection substepping. Techniques to mitigate these penalties are currently being investigated. Moreover, more fine-grained parallelisation of complex loops, such as tuned tiling instructions, can further improve the performance of the nonhydrostatic dynamical core of RegCM.

How to cite: Sclocco, A., van den Oord, G., Giuliani, G., Girotto, I., Raffin, E., and van Werkhoven, B.: Acceleration of the non-hydrostatic dynamical core of RegCM using GPUs, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7333, https://doi.org/10.5194/egusphere-egu23-7333, 2023.

EGU23-9496 | Posters on site | AS5.3

Towards parallel-in-time algorithms for numerical weather prediction 

Jemma Shipton, Colin Cotter, and Beth Wingate

Parallel-in-time algorithms provide a route to increased parallelism for weather and climate models, addressing the issue of how to make efficient use of future supercomputers. In this talk I will present an overview of the approaches implemented in Gusto, the compatible finite element dynamical core toolkit build on top of the Firedrake finite element library. Compatible finite element methods are of interest for weather and climate modelling due to their conservation and wave propagation properties on non-orthogonal meshes such as the cubed-sphere. These non-orthogonal meshes allow for better scaling from spatial domain decomposition than meshes based on the latitude-longitude grid which have grid points clustered at the poles. However, the sequential nature of classical timestepping algorithms is a bottleneck to increased parallelisation. Numerical weather prediction is a challenging application for time-parallel schemes due to the hyperbolic nature of the partial differential equations that make up the dynamical core. Several different time-parallel schemes are under investigation in Gusto: parallel exponential integrators using a rational approximation (REXI); asymptotic parareal, which uses averaged equations to construct the coarse approximation; and schemes based on deferred correction. I will give an overview of these methods and present the latest results and challenges.

How to cite: Shipton, J., Cotter, C., and Wingate, B.: Towards parallel-in-time algorithms for numerical weather prediction, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9496, https://doi.org/10.5194/egusphere-egu23-9496, 2023.

EGU23-9551 | ECS | Posters on site | AS5.3

z-coordinates with surface layer insertion/removal  for accurate representation of free-surface flows in ocean models 

Luca Arpaia, Christian Ferrarin, Marco Bajo, and Georg Umgiesser

Ocean model performances are highly related to the vertical coordinate system implemented. We study geo-potential (or z-) coordinates and we focus on the numerical treatment of the moving free surface. Typically z-coordinate models are coded with a surface layer with varying but not-vanishing thickness, which limits the vertical resolution in areas with high tidal range. We propose a z-coordinate algorithm that, thanks to the insertion and removal of surface layers, can deal with an arbitrary large tidal oscillation independently of the vertical resolution. The algorithm is based on a classical two steps procedure used in numerical simulations with moving boundaries (grid movement followed by a grid topology change) which leads to a stable and accurate numerical discretization. With ad-hoc treatment of advection terms at non-conformal edges that may appear due to insertion/removal operations, mass conservation and tracer constancy are preserved. This algorithm can be reverted, in the particular case when all layers are moving, to other surface-following z-coordinates, such as z-star. With a simple truncation error analysis and realistic numerical experiments, we show the performances of z-coordinates with surface layer insertion/removal in coastal environments.

How to cite: Arpaia, L., Ferrarin, C., Bajo, M., and Umgiesser, G.: z-coordinates with surface layer insertion/removal  for accurate representation of free-surface flows in ocean models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9551, https://doi.org/10.5194/egusphere-egu23-9551, 2023.

EGU23-10012 | Orals | AS5.3

The Unified Forecast System: linking operational and research environmental modeling through an open source community approach 

Hendrik Tolman, Neil Jacobs, Louisa Nanace, and Henrique Alves

In the last few years, operational modeling of the environment at the National Oceanic and Atmospheric Administration  (NOAA) in the USA has been moving towards a Unified Forecast System (UFS) approach based on open source community models and tools. For NOAA, the main benefits of this approach are to more rapidly transition innovations into operations, and simplifying NOAA’s production suite of models around selected UFS applications. For the broader community, this approach makes operational models easily available for a broad range of research, as well as for testing new ideas in a vetted, near-operational environment. The collaboration and cooperation of the UFS community are powered by the Earth Prediction Innovation Center (EPIC). EPIC is a virtual center managed by the Weather Program Office at NOAA’s Oceanic and Atmospheric Research and designed to ensure that the UFS is an efficient, effective, and user-friendly community modeling system. Additionally, EPIC ensures that NOAA’s operational needs and the Research and Development community are supported with effective Research to Operations and Operations to Research processes. NOAA furthermore drives the development of the UFS by a focus of internal NOAA resources on UFS applications. And by generally requiring applicants to NOAA Funding Opportunities to perform their research and development with UFS tools and approaches.  The presentation will outline the basic principles of the UFS, as well as progress made so far. The latter will highlight code releases and operational implementations, UFS governance, and progress with pre-operational prototype coupled models. 

How to cite: Tolman, H., Jacobs, N., Nanace, L., and Alves, H.: The Unified Forecast System: linking operational and research environmental modeling through an open source community approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10012, https://doi.org/10.5194/egusphere-egu23-10012, 2023.

EGU23-11818 | ECS | Posters on site | AS5.3

A set of deterministic and stochastic model improvements for the AWI-CM3 climate model 

Jan Streffing, Tido Semmler, Dmitry Sidorenko, Felix Pithan, and Stephan Juricke

We present intermediate results as well as ongoing work on improving the post-CMIP6 climate model of the Alfred Wegener Institute, AWI-CM3. A baseline version of the model was completed in 2021 with an above average performance when compared to other CMIP6 models. Close investigation of surfaces fluxes revealed that v3.0 can be further improved in a number of ways which will also benefit other climate models.

As a first step we reevaluated old coupling simplifications and assumptions made years ago. At the air-sea ice interface we corrected the gradient of surface sensible heat flux / wind speed vs. (2m air temp - sea ice surf temp), by using a nudged version of AWI-CM3 and evaluating against in situ data from the MOSAiC-Expedition. We added the coupling of ocean current feedback, as well as new latent and sensible heat fluxes resulting from precipitation entering the ocean with a different temperature and state than the ocean surface. As a precursor to subsequent Earth System Model (ESM) development we included the coupling of mass and heat fluxes of snow falling on ice-sheets. The resulting AWI-CM3 v3.1 shows increased ability to represent the current climate and historic climate change.

Furthermore we present ongoing work towards AWI-CM3 v3.2, where among other improvements we will include the coupling of sub atmospheric gridscale information from the higher resolution ocean grid, via a stochastic method. Finally we give a brief outlook on our efforts to link up with the EC-Earth climate and earth system model community for common cryosphere, vegetation and isotope developments towards two comprehensive ESMs.

How to cite: Streffing, J., Semmler, T., Sidorenko, D., Pithan, F., and Juricke, S.: A set of deterministic and stochastic model improvements for the AWI-CM3 climate model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11818, https://doi.org/10.5194/egusphere-egu23-11818, 2023.

EGU23-12375 | ECS | Orals | AS5.3

Parallel-in-time solution of finite element atmospheric models using ParaDiag 

Josh Hope-Collins and Colin Cotter

Modern numerical weather prediction requires vast amounts of computing power, so highly scalable algorithms are essential on massively parallel modern hardware. However, once the strong scaling limit is reached for spatial parallelism, the wallclock time increases with the number of timesteps. This limits the ability to provide higher resolution forecasts on an operational schedule. Parallel-in-time methods overcome this limit by exposing time parallelism, in addition to the spatial parallelism exposed by traditional domain decomposition.

ParaDiag is one such method, which reduces the coupled system for multiple time-steps into a block-diagonal matrix that can be solved in parallel. We will present recent progress on the application of ParaDiag to compatible finite element discretisations of PDEs for atmospheric flow, which are particularly challenging for time-parallel methods due to their highly oscillatory nature. These solvers are implemented as an open source general library using Firedrake, an automated code generation framework for the solution of finite element methods.

Various ParaDiag formulations are explored for linear and non-linear models, and their parallel scaling is compared. Their performance is compared against time serial methods to find the parameter ranges where the greatest speedups are achieved. We identify the main difficulties faced by ParaDiag and describe our approaches to overcoming these, including solution strategies for the block systems within the ParaDiag matrix, and improving the convergence of nonlinear models.

How to cite: Hope-Collins, J. and Cotter, C.: Parallel-in-time solution of finite element atmospheric models using ParaDiag, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12375, https://doi.org/10.5194/egusphere-egu23-12375, 2023.

EGU23-13070 | ECS | Orals | AS5.3

Higher-Efficiency Inverse Atmospheric Modelling by Virtue of a Global Hexagonal Mesh 

Sakina Takache, Frederic Chevallier, Zoé Lloret, and Anne Cozic

Emission sources and sinks of long-lived greenhouse gases (GHGs), such as CO2 and N2O, can be localized and scaled by inversely modelling existing distributions of these tracers in the atmosphere. This is particularly useful for monitoring GHG emissions at a global level, for comparison, for instance, with the national inventory reports of the United Nations Framework Convention on Climate Change (UNFCCC).

To achieve inverse transport numerically, multiple approaches can be taken, notably variational data assimilation. This involves the optimization of the Bayesian cost function accounting for prior state errors and observation errors. Variational data assimilation can be implemented by adjoint modelling. This method is based on the modification of the tracer transport equations of general circulation models (GCMs). The transpose of the tangent-linear operator, called the “adjoint”, is applied to find the initial sources and sinks. Eulerian backtracking, also called “retro-transport”, is a simplified approach to adjoint modelling, where the roles of updraughts and entrainment are switched with downdraughts and detrainment, respectively, and vice versa (Hourdin et al., 2005a).

In our presented work, we implement both the adjoint method for inverse modelling (Lions, 1971; Marchuk, 1974, 1982) and the retro-transport method put forth by Hourdin et al. (2005a). Our newfound approach consists of adapting these methods to a hexagonal mesh. For this, we use the DYNAMICO dynamical core of the the Laboratoire de Météorologie Dynamique-Zoom (LMDZ) GCM, which computes forward-in-time transport equations on a hexagonal mesh (Dubos et al., 2015). We add routines to DYNAMICO’s source code for the adjoint method, and alter the direction of fluxes to implement Eulerian backtracking.

The hexagonal mesh permits to reduce the computational cost traditionally attributed to inverse atmospheric modelling. Without the decreasing cell size as we approach the poles in a regular lon-lat grid, a hexagonal mesh covers the globe with a smaller number of nearly fixed-size cells. This directly reduces the size of input data and the number of operations. Further, the hexagonal mesh allows modellers to bypass the need for nonlinear cell-treatment at the poles of a regular lon-lat grid, increasing the accuracy of the retro-transport approximation. The increased computational efficiency of the hexagonal mesh paves the way for higher horizontal resolutions for global atmospheric inversion.

How to cite: Takache, S., Chevallier, F., Lloret, Z., and Cozic, A.: Higher-Efficiency Inverse Atmospheric Modelling by Virtue of a Global Hexagonal Mesh, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13070, https://doi.org/10.5194/egusphere-egu23-13070, 2023.

EGU23-14086 | ECS | Posters on site | AS5.3

Quantifying the accuracy of large time-steps in highly oscillatory systems 

Timothy Andrews, Beth Wingate, and Jemma Shipton

There is an ever-increasing demand for longer and higher resolution numerical simulations of the weather and climate. To achieve this with reasonable wall-clock times, it is desirable to use as large a time-step as possible, whilst retaining a stable and accurate solution. However, this is very challenging in the presence of highly oscillatory linear waves; there are explicit time-step limits and losses in accuracy with implicit methods. This talk will highlight where non-linear errors can result from large time-steps and provide metrics for quantifying this. We begin by re-casting the non-linearity as a product of linear waves. In the Rotating Shallow Water Equations (RSWEs), this allows for key dynamics to be expressed as three-wave ‘triad’ interactions. A non-linear ‘triadic’ time-stepping error is computed using linear stability polynomials. A number of explicit and implicit time-stepping methods (such as RK4, TR-BDF2, ETD-RK2) will be compared analytically in the RSWEs. Next, two new test problems enable analyses of large time-step simulations. The first is of a Gaussian perturbation to a RSWE height field. A proposed metric, relating to the kinetic energy distribution over temporal frequency, quantifies phase errors in the height reformation. The second test case initialises linear waves which, via direct- and near- resonant triad interactions, will construct non-linear dynamics. Phase errors with large time-steps can be identified in the corresponding height fields. A first variant of this case will initialise only two waves; this will primarily instigate an energy exchange within a dominant triad. A second version, containing more slow modes, enables a re-distribution of fast mode energy into rings in wavenumber space.

How to cite: Andrews, T., Wingate, B., and Shipton, J.: Quantifying the accuracy of large time-steps in highly oscillatory systems, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14086, https://doi.org/10.5194/egusphere-egu23-14086, 2023.

EGU23-15904 | ECS | Orals | AS5.3

Towards a Performance-Portable Finite-Volume Dynamical Core for Numerical Weather Prediction 

Stefano Ubbiali, Till Ehrengruber, Nicolai Krieger, Christian Kühnlein, Lukas Papritz, and Heini Wernli

We present the ongoing development of a Python implementation of a finite-volume non-hydrostatic dynamical core at ECMWF and its member state partners. The main drivers behind the model formulation are suitability for convective-scale resolutions and increasing multi-level parallelism. Sustainable software design with respect to emerging and future heterogeneous computing platforms is addressed by leveraging the GT4Py domain-specific framework. We further address aspects of implementing and coupling selected ECMWF model physical parametrizations using GT4Py. 

How to cite: Ubbiali, S., Ehrengruber, T., Krieger, N., Kühnlein, C., Papritz, L., and Wernli, H.: Towards a Performance-Portable Finite-Volume Dynamical Core for Numerical Weather Prediction, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15904, https://doi.org/10.5194/egusphere-egu23-15904, 2023.

EGU23-16453 | ECS | Orals | AS5.3 | Highlight

Storm- and eddy-resolving simulations with IFS-FESOM/NEMO at the kilometre scale 

Thomas Rackow, Xabier Pedruzo Bagazgoitia, Tobias Becker, Sebastian Milinski, Irina Sandu, Michail Diamantakis, Helge F. Goessling, Ioan Hadade, Jan Hegewald, Nikolay Koldunov, Alexei Koldunov, Tobias Kölling, Kristian Mogensen, Dmitry Sidorenko, Jan Streffing, Nils Wedi, Lorenzo Zampieri, and Florian Ziemen

Global coupled simulations that can resolve atmospheric storms and mesoscale oceanic features at the kilometre-scale have recently become possible to run over short time slices, for example on a seasonal timescale. Here we give an overview of the first multi-year simulations performed with ECMWF’s Integrated Forecasting System (IFS), coupled to both the NEMO and FESOM2 ocean-sea ice models, for the H2020 Next Generation Earth Modelling Systems (nextGEMS) project. The project aims to build a new generation of eddy- and storm-resolving global coupled Earth System Models. Along with ICON, the other model participating in nextGEMS, the IFS-based models form the basis also for Digital Climate Twins of Earth as envisioned in the European Union’s ambitious Destination Earth project. nextGEMS relies on several model development cycles, in which the models are run and improved based on community feedback. In an initial set of storm-resolving coupled simulations (Cycle 1), the IFS was integrated for 75 days. For Cycle 2, IFS has been run at the operational 9 km resolution as a baseline, and at 4.4 km and 2.8 km global spatial resolution for up to 1 year of simulation (4.4 km). To our knowledge, the 8-months long 2.8 km simulation in Cycle 2 represents the first fully coupled simulation ever of this duration at this high level of spatial detail and is made available to the public. The runs at 9 km were performed with the parameterization for deep convection active as in the operational system, while at 4.4 km and 2.8 km, separate experiments with IFS were run both with and without the deep convection parameterization.

We document the model improvements made to IFS-FESOM/NEMO based on the lessons learned from the first Cycle 1 runs, which were included for the second round of Cycle 2 simulations; these mainly consist in vastly improved conservation properties of the coupled model systems in terms of water and energy balance, which are crucial for longer climate integrations, and in a more realistic representation of the snow and surface drag. Cycle 2 also targeted eddy-resolving resolution in large parts of the mid- and high-latitude ocean (better than 5km) to resolve mesoscale eddies and linear kinematic features (i.e. leads or cracks) in sea ice. For IFS-FESOM, this is made possible thanks to a recently refactored ocean model code that can be linked as an external library and that allows for efficient coupled simulations in the single-executable context with IFS, via hybrid parallelization with MPI and OpenMP.

How to cite: Rackow, T., Pedruzo Bagazgoitia, X., Becker, T., Milinski, S., Sandu, I., Diamantakis, M., Goessling, H. F., Hadade, I., Hegewald, J., Koldunov, N., Koldunov, A., Kölling, T., Mogensen, K., Sidorenko, D., Streffing, J., Wedi, N., Zampieri, L., and Ziemen, F.: Storm- and eddy-resolving simulations with IFS-FESOM/NEMO at the kilometre scale, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16453, https://doi.org/10.5194/egusphere-egu23-16453, 2023.

EGU23-16797 | Orals | AS5.3 | Highlight

EarthWorks 

David Randall, James Hurrell, Andrew Gettelman, William Skamarock, Donald Dazlich, Thomas Hauser, Sheri Mickelson, Brian Medeiros, and Lantao Sun

EarthWorks is a high-resolution, coupled, global storm-resolving Earth System Model which is aimed at both weather and climate applications. All components share the same geodesic grid. The target grid spacing is 3.75 km for all components, and the target performance is one simulated year per wall clock day by 2025. 

While EarthWorks uses the CESM framework, its atmosphere, ocean and sea ice components are based on the MPAS (“Model for Prediction Across Scales”) dynamical cores. These components are coupled using the CMEPS (Community Mediator for Earth Prediction Systems) developed for CESM. 

Our presentation will focus on the results of both fully coupled and AMIP simulations with various horizontal grid spacings. We will also mention various problems encountered and overcome along the way.

How to cite: Randall, D., Hurrell, J., Gettelman, A., Skamarock, W., Dazlich, D., Hauser, T., Mickelson, S., Medeiros, B., and Sun, L.: EarthWorks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16797, https://doi.org/10.5194/egusphere-egu23-16797, 2023.

EGU23-1095 | Orals | NP5.2

Recent offline land data assimilation results and future steps towards coupled DA at Meteo-France 

Jean-Christophe Calvet, Bertrand Bonan, and Yiwen Xu

Land data assimilation aims to monitor the evolution of soil and vegetation variables. These variables are driven by climatic conditions and by anthropogenic factors such as agricultural practices. Monitoring terrestrial surfaces involves a number of variables of the soil-plant system such as land cover, snow, surface albedo, soil water content and leaf area index. These variables can be monitored by integrating satellite observations into models. This process is called data assimilation. Integrating observations into land surface models is particularly important in changing climate conditions because environmental conditions and trends never experienced before are emerging. Because data assimilation is able to weight the information coming from contrasting sources of information and to account for uncertainties, it can produce an analysis of terrestrial variables that is the best possible estimation. In this work, data assimilation is implemented at a global scale by regularly updating the model state variables of the ISBA land surface model within the SURFEX modelling platform: the LDAS-Monde sequential assimilation approach. Model-state variable analysis is done for initializing weather forecast atmospheric models. Weather forecast relies on observations to a large extent because of the chaotic nature of the atmosphere. Land variables are not chaotic per se but rapid and complex processes impacting the land carbon budget such as forest management (thinning, deforestation, ...), forest fires and agricultural practices are not easily predictable with a good temporal precision. They cannot be monitored without integrating observations as soon as they are available. We focus on the assimilation of leaf area index (LAI), using land surface temperature (LST) for verification. We show that (1) analyzing LAI together with root-zone soil moisture is needed to monitor the impact of irrigation and heat waves on the vegetation, (2) LAI can be forecasted after properly initializing ISBA. This paves the way to more interactive assimilation of land variables into numerical weather forecast and seasonal forecast models, as well as in atmospheric chemistry models.

 

How to cite: Calvet, J.-C., Bonan, B., and Xu, Y.: Recent offline land data assimilation results and future steps towards coupled DA at Meteo-France, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1095, https://doi.org/10.5194/egusphere-egu23-1095, 2023.

EGU23-1846 | Posters on site | NP5.2 | Highlight

Hybrid covariance super-resolution data assimilation 

Sébastien Barthélémy, Julien Brajard, Laurent Bertino, and François Counillon

This work extends the concept of "Super-resolution data assimilation" (SRDA, Barthélémy et al. 2022)) to the case of mixed-resolution ensembles pursuing two goals: (1) emulate the Ensemble Kalman Filter while (2) benefit from high-resolution observations. The forecast step is performed by two ensembles at two different resolutions, high and low-resolution. Before the assimilation step the low-resolution ensemble is downscaled to the high-resolution space, then both ensembles are updated with high-resolution observations. After the assimilation step, the low-resolution ensemble is upscaled back to its low-resolution grid for the next forecast. The downscaling step before the data assimilation step is performed either with a neural network, or with a simple cubic spline interpolation operator. The background error covariance matrix used for the update of both ensembles is a hybrid matrix between the high and low resolution background error covariance matrices. This flavor of the SRDA is called "Hybrid covariance super-resolution data assimilation" (Hybrid SRDA). We test the method with a quasi-geostrophic model in the context of twin-experiments with the low-resolution model being twice and four times coarser than the high-resolution one. The Hybrid SRDA with neural network performs equally or better than its counterpart with cubic spline interpolation, and drastically reduces the errors of the low-resolution ensemble. At equivalent computational cost, the Hybrid SRDA outperforms both the SRDA (8.4%) and the standard EnKF (14%). Conversely, for a given value of the error, the Hybrid SRDA requires as little as  50% of the computational resources of  the EnKF. Finally, the Hybrid SRDA can be formulated as a low-resolution scheme, in the sense that the assimilation is performed in the low-resolution space, encouraging the application of the scheme with realistic ocean models.

How to cite: Barthélémy, S., Brajard, J., Bertino, L., and Counillon, F.: Hybrid covariance super-resolution data assimilation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1846, https://doi.org/10.5194/egusphere-egu23-1846, 2023.

All-sky radiance assimilation often has non-Gaussian observation error distributions, which can be exacerbated by high model spatial resolutions due to better resolved nonlinear physical processes. For ensemble Kalman filters, observation ensemble perturbations can be approximated by linearized observation operator (LinHx) that uses the observation operator Jacobian of ensemble mean rather than full observation operator (FullHx). The impact of observation operator on infrared radiance data assimilation is examined here by assimilating synthetic radiance observations from channel 1025 of GIIRS with increased model spatial resolutions from 7.5 km to 300 m. A tropical cyclone is used, while the findings are expected to be generally applied. Compared to FullHx, LinHx provides larger magnitudes of correlations and stronger corrections around observation locations, especially when all-sky radiances are assimilated at fine model resolutions. For assimilating clear-sky radiances with increasing model resolutions, LinHx has smaller errors and improved vortex intensity and structure than FullHx. But when all-sky radiances are assimilated, FullHx has advantages over LinHx. Thus for regimes with more linearity, LinHx provides stronger correlations and imposes more corrections than FullHx; but for regimes with more nonlinearity, LinHx provides detrimental non-Gaussian prior error distributions in observation space, unrealistic correlations and overestimated corrections, compared to FullHx.

How to cite: Lei, L.: Impacts of Observation Forward Operator on Infrared Radiance Data Assimilation with Fine Model Resolutions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3011, https://doi.org/10.5194/egusphere-egu23-3011, 2023.

EGU23-3086 | Posters on site | NP5.2

Comparison of optimization methods for the maximum likelihood ensemble filter 

Takeshi Enomoto and Saori Nakashita

The Newton method, which requires the Hessian matrix, is prohibitively expensive in adjoint-based variational data assimilation (VAR). It may be rather attractive for ensemble-based VAR because the ensemble size is usually several orders of magnitude smaller than that of the state size. In the present paper the Newton method is compared against the conjugate-gradient (CG) method, which is one of the most popular choices in adjoint-based VAR. To make comparisons, the maximum likelihood ensemble filter (MLEF) is used as a framework for data assimilation experiments. The Hessian preconditioning is used with CG as formulated in the original MLEF. Alternatively we propose to use the Hessian in the Newton method. In the exact Newton (EN) method, the Newton equation is solved exactly, i.e. the step size is fixed to unity avoiding a line search. In the 1000-member wind-speed assimilation test, CG is stagnated early in iteration and terminated due to a line search error while EN converges quadratically. This behaviour is consistent with the workings of the EN and CG in the minimization of the Rosenbrock function. In the repetitive cycled experiments using the Korteweg-de Vries-Burgers (KdVB) model with a quadratic observation operator, EN performs competitively in accuracy to CG with significantly enhanced stability. These idealized experiments indicate the benefit of adopting EN for the optimization in MLEF.

How to cite: Enomoto, T. and Nakashita, S.: Comparison of optimization methods for the maximum likelihood ensemble filter, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3086, https://doi.org/10.5194/egusphere-egu23-3086, 2023.

EGU23-3761 | ECS | Posters on site | NP5.2

Observation space localizations for the maximum likelihood ensemble filter 

Saori Nakashita and Takeshi Enomoto

The maximum likelihood ensemble filter (MLEF) can handle nonlinearity of observation operators more appropriately than conventional ensemble Kalman filters. Here we consider the observation space localization method for MLEF to enable application to large-scale problems in the atmosphere. Optimization of the cost function in MLEF, however, impedes local analysis, suitable for massive parallel computers, in the same manner as the local ensemble transform Kalman filter (LETKF). In this study two approaches to observation space localization for MLEF (LMLEF) are compared. The first method introduces local gradients to minimize the global cost function (Yokota et al. 2016). An alternative approach, proposed here, defines a local cost function for each grid assuming a constant ensemble weight in the local domain to enable embarrassingly parallel analysis. The two approaches are compared to LETKF in cycled data assimilation experiments using the Lorenz-96 and the SPEEDY models. LMLEFs are found to be more accurate and stable than LETKF when nonlinear observations are assimilated into each model. Our proposed method is comparable to Yokota's global optimization method when dense observations are assimilated into the Lorenz-96 model. This result is consistent with the fact that ensemble weights have high spatial correlations with those at neighboring grids. Although our method also yields similar analysis in the SPEEDY experiments with a more realistic observation network, Yokota’s global optimization method shows faster error convergence in the earlier cycles. The error convergence rate seems to be related to the difference between global and local optimization and the validity of the assumption of constant weights, which depends strongly on the observation density.

How to cite: Nakashita, S. and Enomoto, T.: Observation space localizations for the maximum likelihood ensemble filter, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3761, https://doi.org/10.5194/egusphere-egu23-3761, 2023.

EGU23-4668 | ECS | Posters virtual | NP5.2 | Highlight

A particle filter based target observation method and its application to two types of El Niño events 

Meiyi Hou and Youmin Tang

The optimal observational array for improving the El Niño-Southern Oscillation (ENSO) prediction is investigated by exploring sensitive areas for target observations of two types of El Niño events in the Pacific. A target observation method based on the particle filter and pre-industrial control runs from six coupled model outputs in Coupled Model Intercomparison Project Phase 5 (CMIP5) experiments are used to quantify the relative importance of the initial accuracy of sea surface temperature (SST) in different Pacific areas. The initial accuracy of the tropical Pacific, subtropical Pacific, and extratropical Pacific can influence both types of El Niño predictions. The relative importance of different areas changes along with different lead times of predictions. Tropical Pacific observations are crucial for decreasing the root mean square error of predictions of all lead times. Subtropical and extratropical observations play an important role in reducing the prediction uncertainty, especially when the prediction is made before and throughout the boreal spring. To consider different El Niño types and different start months for predictions, a quantitative frequency method based on frequency distribution is applied to determine the optimal observations of ENSO predictions. The final optimal observational array contains 31 grid points, including 21 grid points in the equatorial Pacific and 10 grid points in the North Pacific, suggesting the importance of the initial SST conditions for ENSO predictions in the tropical Pacific and also in the area outside the tropics. Furthermore, the predictions made by assimilating SST in sensitive areas have better prediction skills in the verification experiment, which can indicate the validity of the optimal observational array designed in this study. This result provided guidance on how to initialize models in predictions of El Niño types. 

How to cite: Hou, M. and Tang, Y.: A particle filter based target observation method and its application to two types of El Niño events, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4668, https://doi.org/10.5194/egusphere-egu23-4668, 2023.

EGU23-5421 | ECS | Posters on site | NP5.2

Estimation of Spatially and Temporally Varying Biogeochemical Parameters in a Global Ocean Model 

Nabir Mamnun, Christoph Völker, Mihalis Vrekoussis, and Lars Nerger

Ocean biogeochemical (BGC) models are, in addition to measurements, the primary tools for investigating ocean biogeochemistry, marine ecosystem functioning, and the global carbon cycle. These models contain a large number of not precisely known parameters and are highly uncertain regarding those parametrizations.  The values of these parameters depend on the physical and biogeochemical context, but in practice values derived from limited field measurements or laboratory experiments are used in the model keeping them constant in space and time. This study aims to estimate spatially and temporally varying parameters in a global ocean BGC model and to assess the effect of those estimated parameters on model fields and dynamics. Utilizing the BGC model Regulated Ecosystem Model 2 (REcoM2), we estimate ten selected BGC parameters with heterogeneity in parameter values both across space and over time using an ensemble data assimilation technique. We assimilate satellite ocean color and BGC-ARGO data using an ensemble Kalman filter provided by the Parallel Data Assimilation Framework (PDAF) to simultaneously estimate the BGC model states and parameters. We assess the improvement in the model predictions with space and time-dependent parameters in reference to the simulation with globally constant parameters against both assimilative and independent data. We quantify the spatiotemporal uncertainties regarding the parameter estimation and the prediction uncertainties induced by those parameters. We study the effect of estimated parameters on the biogeochemical fields and dynamics to get deeper insights into modeling processes and discuss insights from spatially and temporally varying parameters beyond parameter values.

How to cite: Mamnun, N., Völker, C., Vrekoussis, M., and Nerger, L.: Estimation of Spatially and Temporally Varying Biogeochemical Parameters in a Global Ocean Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5421, https://doi.org/10.5194/egusphere-egu23-5421, 2023.

EGU23-5506 | ECS | Posters on site | NP5.2

Empirical optimal vertical localization derived from large ensembles 

Tobias Necker, Philipp Griewank, Takemasa Miyoshi, and Martin Weissmann

Ensemble-based estimates of error covariances suffer from limited ensemble size due to computational restrictions in data assimilation systems for numerical weather prediction. Localization of error covariances can mitigate sampling errors and is crucial for ensemble-based data assimilation. However, finding optimal localization methods, functions, or scales is challenging. We present a new approach to derive an empirical optimal localization (EOL) from a large ensemble dataset. The EOL allows for a better understanding of localization requirements and can guide toward improved localization.

Our study presents EOL estimates using 40-member subsamples assuming a 1000-member ensemble covariance as truth. The EOL is derived from a 5-day training period. In the presentation, we cover both model and observation space vertical localization and discuss:

  • vertical error correlations and EOL estimates for different variables and settings;

  • the effect of the EOL compared to common localization approaches, such as distance-dependent localization with a Gaspari-Cohn function;

  • and vertical localization of infrared and visible satellite observations in the context of observation space localization.

Proper observation space localization of error covariances between non-local satellite observations and state space is non-trivial and still an open research question. First, we evaluate requirements for optimal localization for different variables and spectral channels. And secondly, we investigate the situation dependence of vertical localization in convection-permitting NWP simulations, which suggests an advantage of using adaptive situation-dependent localization approaches.

How to cite: Necker, T., Griewank, P., Miyoshi, T., and Weissmann, M.: Empirical optimal vertical localization derived from large ensembles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5506, https://doi.org/10.5194/egusphere-egu23-5506, 2023.

EGU23-6050 | ECS | Posters on site | NP5.2 | Highlight

Unbalanced emission reductions of different species and sectors in China during COVID-19 lockdown derived by multi-species surface observation assimilation 

Lei Kong, Xiao Tang, Jiang Zhu, Zifa Wang, Yele Sun, Pingqing Fu, Meng Gao, Huangjian Wu, Jie Li, Xiaole Pan, Lin Wu, Hajime Akimoto, and Gregory R. Carmichael

The unprecedented lockdown of human activities during the COVID-19 pandemic have significantly influenced the social life in China. However, understanding of the impact of this unique event on the emissions of different species is still insufficient, prohibiting the proper assessment of the environmental impacts of COVID-19 restrictions. Here we developed a multi-air pollutant inversion system to simultaneously estimate the emissions of NOx, SO2, CO, PM2.5 and PM10 in China during COVID-19 restrictions with high temporal (daily) and horizontal (15km) resolutions. Subsequently, contributions of emission changes versus meteorology variations during COVID-19 lockdown were separated and quantified. The results demonstrated that the inversion system effectively reproduced the actual emission variations of multi-air pollutants in China during different periods of COVID-19 lockdown, which indicate that the lockdown is largely a nationwide road traffic control measurement with NOx emissions decreased substantially by ~40%. However, emissions of other air pollutants were found only decreased by ~10%, both because power generation and heavy industrial processes were not halted during lockdown, and residential activities may actually have increased due to the stay-at-home orders. Consequently, although obvious reductions of PM2.5 concentrations occurred over North China Plain (NCP) during lockdown period, the emission change only accounted for 8.6% of PM2.5 reductions, and even led to substantial increases of O3. The meteorological variation instead dominated the changes in PM2.5 concentrations over NCP, which contributed 90% of the PM2.5 reductions over most parts of NCP region. Meanwhile, our results also suggest that the local stagnant meteorological conditions together with inefficient reductions in PM2.5 emissions were the main drivers of the unexpected COVID-19 haze in Beijing. These results highlighted that traffic control as a separate pollution control measure has limited effects on the coordinated control of O3 and PM2.5 concentrations under current complex air pollution conditions in China. More comprehensive and balanced regulations for multiple precursors from different sectors are required to address O3 and PM2.5 pollution in China.

How to cite: Kong, L., Tang, X., Zhu, J., Wang, Z., Sun, Y., Fu, P., Gao, M., Wu, H., Li, J., Pan, X., Wu, L., Akimoto, H., and Carmichael, G. R.: Unbalanced emission reductions of different species and sectors in China during COVID-19 lockdown derived by multi-species surface observation assimilation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6050, https://doi.org/10.5194/egusphere-egu23-6050, 2023.

EGU23-7480 | ECS | Orals | NP5.2 | Highlight

Supermodelling: synchronising models to further improve predictions 

Francine Schevenhoven, Mao-Lin Shen, Noel Keenlyside, Jeffrey B. Weiss, and Gregory S. Duane

Instead of combining data from an ensemble of different models after the simulations are already performed, as in a standard multi-model ensemble, we let the models interact with each other during their simulation. This ensemble of interacting models is called a supermodel. By exchanging information, models can compensate for each other's errors before the errors grow and spread to other regions or variables. Effectively, we create a new dynamical system. The exchange between the models is frequent enough such that the models synchronize, in order to prevent loss of variance when the models are combined. In previous work, we experimented successfully with combining atmospheric models of intermediate complexity in the context of parametric error. Here we will show results of combining two different AGCMs, NorESM1-ATM and CESM1-ATM. The models have different horizontal and vertical resolutions. To combine states from the different grids, we convert the individual model states to a ‘common state space’ with interpolation techniques. The weighted superposition of different model states is called a ‘pseudo-observation’. The pseudo-observations are assimilated back into the individual models, after which the models continue their run. We apply recently developed methods to train the weights determining the superposition of the model states, in order to obtain a supermodel that will outperform the individual models and any weighted average of their outputs.

How to cite: Schevenhoven, F., Shen, M.-L., Keenlyside, N., Weiss, J. B., and Duane, G. S.: Supermodelling: synchronising models to further improve predictions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7480, https://doi.org/10.5194/egusphere-egu23-7480, 2023.

EGU23-7719 | ECS | Orals | NP5.2

The role of anchor observations in disentangling observation and model bias corrections in 4DVar 

Devon Francis, Alison Fowler, Amos Lawless, Stefano Migliorini, and John Eyre

Data assimilation theory relies on the assumption that the background, model, and observations are unbiased. However, this is often not the case and, if biases are left uncorrected, this can cause significant systematic errors in the analysis. When bias is only present in the observations, Variational Bias Correction (VarBC) can correct for observation bias, and when bias is only present in the model, Weak-Constraint 4D Variational Assimilation (WC4DVar) can correct for model bias. However, when both observation and model biases are present, it can be very difficult to understand how the different bias correction methods interact, and the role of anchor (unbiased) observations becomes crucial for providing a frame of reference from which the biases may be estimated. This work presents a systematic study of the properties of the network of anchor observations needed to disentangle between model and observation biases when correcting for one or both types of bias in 4DVar.

We extend the theory of VarBC and WC4DVar to include both biased and anchor observations, to find that the precision and timing of the anchor observations are important in reducing the contamination of model/observation bias in the correction of observation/model bias. We show that anchor observations have the biggest impact in reducing the contamination of bias when they are later in the assimilation window than the biased observations, as such, operational systems that rely on anchor observations that are earlier in the window will be more susceptible to the contamination of model and/or observation biases. We also compare the role of anchor observations when VarBC/WC4DVar/both are used in the presence of both observation and model biases. We find that the ability of VarBC to effectively correct for observation bias when model bias is present, is very dependent on precise anchor observations, whereas correcting model bias with WC4DVar or correcting for both biases performs reasonably well regardless of the precision of anchor observations (although more precise anchor observations reduces the bias in the state analysis compared with less precise anchor observations for all three cases). This demonstrates that, when it is not possible to use anchor observations, it may be better to correct for both observation and model biases, rather than relying on only one bias correction technique.

We demonstrate these results in a series of idealised numerical experiments that use the Lorenz 96 model as a simplified model of the atmosphere.

How to cite: Francis, D., Fowler, A., Lawless, A., Migliorini, S., and Eyre, J.: The role of anchor observations in disentangling observation and model bias corrections in 4DVar, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7719, https://doi.org/10.5194/egusphere-egu23-7719, 2023.

EGU23-8030 | Posters on site | NP5.2

Assessment of short-range forecast atmosphere-ocean cross-covariances from the Met Office coupled NWP system 

Amos Lawless, Maria Valdivieso, Nancy Nichols, Daniel Lea, and Matthew Martin

As part of the design of future coupled forecasting systems, operational centres such as the Met Office are starting to include interactions between the atmosphere and the ocean within the data assimilation system. This requires an improved understanding and representation of the correlations between short-range forecast errors in different variables. To understand the potential benefit of further coupling in the data assimilation scheme it is important to understand the significance of any cross-correlations between atmosphere and ocean short-range forecast errors as well as their temporal and spatial variability. In this work we examine atmosphere-ocean cross-covariances from an ensemble of the Met Office coupled NWP system for December 2019, with particular focus on short-range forecast errors that evolve at lead times up to 6 hours.

We find that significant correlations exist between atmosphere and ocean forecast errors on these timescales, and that these vary diurnally, from day to day, spatially and synoptically. Negative correlations between errors in sea-surface temperature (SST) and 10m wind correlations strengthen as the solar radiation varies from zero at night (local time) to a maximum insolation around midday (local time). In addition, there are significant variations in correlation intensities and structures in response to synoptic-timescale forcing. Significant positive correlations between SST and 10m wind errors appear in the western North Atlantic in early December and are associated with variations in low surface pressures and their associated high wind speeds, that advect cold, dry continental air eastward over the warmer Atlantic ocean. Negative correlations across the Indo-Pacific Warm Pool are instead associated with light wind conditions on these short timescales.

When we consider the spatial extent of cross-correlations, we find that in the Gulf Stream region positive correlations between wind speed and sub-surface ocean temperatures are generally vertically coherent down to a depth of about 100m, consistent with the mixing depth; however, in the tropical Indian and West Pacific oceans, negative correlations break down just below the surface layer. This is likely due to the presence of surface freshwater layers that form from heavy precipitation on the tropical oceans, manifested by the presence of salinity-stratified barrier layers within deeper isothermal layers that can effectively limit turbulent mixing of heat between the ocean surface and the deeper thermocline.

How to cite: Lawless, A., Valdivieso, M., Nichols, N., Lea, D., and Martin, M.: Assessment of short-range forecast atmosphere-ocean cross-covariances from the Met Office coupled NWP system, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8030, https://doi.org/10.5194/egusphere-egu23-8030, 2023.

EGU23-8640 | Orals | NP5.2

Forecast error growth: A stochastic differential equation model 

Michael Ghil, Eviatar Bach, and Dan Crisan

There is a history of simple error growth models designed to capture the key properties of error growth in operational numerical weather prediction models. We propose here such a scalar model that relies on the previous ones, but captures the effect of small scales on the error growth via additive noise in a nonlinear stochastic differential equation (SDE). We nondimensionalize the equation and study its behavior with respect to the error saturation value, the growth rate of small errors, and the magnitude of noise. We show that the addition of noise can change the curvature of the error growth curve. The SDE model seems to improve substantially the fit to operational error growth curves, compared to the deterministic counterparts.

How to cite: Ghil, M., Bach, E., and Crisan, D.: Forecast error growth: A stochastic differential equation model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8640, https://doi.org/10.5194/egusphere-egu23-8640, 2023.

EGU23-9529 | Orals | NP5.2

Nonlinear Data Assimilation for State and Parameter Estimation in Earthquake Simulation 

Femke Vossepoel, Arundhuti Banerjee, Hamed Diab Montero, Meng Li, Celine Marsman, Rob Govers, and Ylona van Dinther

The highly nonlinear dynamics of earthquake sequences and the limited availability of stress observations near subsurface faults make it very difficult, if not impossible, to forecast earthquakes. Ensemble data-assimilation methods provide a means to estimate state variables and parameters of earthquake sequences that may lead to a better understanding of the associated fault-slip process and contribute to the forecastability of earthquakes. We illustrate the challenges of data assimilation in earthquake simulation with an overview of three studies, each with different objectives and experiments.

In the first study, by reconstructing a laboratory experiment with an advanced numerical simulator we perform synthetic twin experiments to test the performance of an ensemble Kalman Filter (EnKF) and its ability to reconstruct fault slip behaviour in 1D and 3D simulations. The data assimilation estimates and forecasts earthquakes, even when having highly uncertain observations of the stress field. In these experiments, we assume the friction parameters to be perfectly known, which is typically not the case in reality.

A bias in a friction parameter can cause a significant change in earthquake dynamics, which will complicate the application of data assimilation in realistic cases. The second study addresses how well state estimation and state-parameter estimation can account for friction-parameter bias. For this, we use a 0D model for earthquake recurrence with a particle filter with sequential importance resampling. This shows that in case of intermediate to large uncertainty in friction parameters, combined state-and-parameter estimation is critical to correctly estimate earthquake sequences. The study also highlights the advantage of a particle filter over an EnKF for this nonlinear system.

The post- and inter-seismic deformations following an earthquake are rather gradual and do not pose the same challenges for data assimilation as the deformation during an earthquake event. To estimate the model parameters of surface displacements during these phases, a third study illustrates the application of the Ensemble Smoother-Multiple Data Assimilation and the particle filter with actual GPS data of the Tohoku 2011 earthquake.

Based on the comparison of the various experiments, we discuss the choice of data-assimilation method and -approach in earthquake simulation and suggest directions for future research.

How to cite: Vossepoel, F., Banerjee, A., Diab Montero, H., Li, M., Marsman, C., Govers, R., and van Dinther, Y.: Nonlinear Data Assimilation for State and Parameter Estimation in Earthquake Simulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9529, https://doi.org/10.5194/egusphere-egu23-9529, 2023.

EGU23-11889 | ECS | Posters on site | NP5.2

Data Assimilation and Subsurface Flow Modeling: Interactions between Groundwater and the Vadose Zone 

Bastian Waldowski, Insa Neuweiler, and Natascha Brandhorst

Reliable estimates of soil water content and groundwater levels are essential in evaluating water availability for plants and as drinking water and thus both subsurface components (vadose zone and groundwater) are commonly monitored. Such measurements can be used for data assimilation in order to improve predictions of numerical subsurface flow models. Within this work, we investigate to what extent measurements from one subsurface component are able to improve predictions in the other one.
For this purpose, we utilize idealized test cases at a subcatchment scale using a Localized Ensemble Kalman Filter to update the water table height and soil moisture at certain depths with measurements taken from a numerical reference model. We do joint, as well as single component updates. We test strongly coupled data assimilation, which implies utilizing correlations between the subsurface components for updating the ensemble and compare it to weakly coupled data assimilation. We also update soil hydraulic parameters and examine the role of their heterogeneity with respect to data assimilation. We run simulations with both a complex 3D model (using TSMP-PDAF) as well as a more simplified and computationally efficient 2.5D model, which consists of multiple 1D vadose-zone columns coupled iteratively with a 2D groundwater-flow model. In idealized settings, such as homogeneous subsurface structures, we find that predictions in one component consistently benefit from updating the other component.

How to cite: Waldowski, B., Neuweiler, I., and Brandhorst, N.: Data Assimilation and Subsurface Flow Modeling: Interactions between Groundwater and the Vadose Zone, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11889, https://doi.org/10.5194/egusphere-egu23-11889, 2023.

EGU23-12304 | ECS | Posters on site | NP5.2

Analysis of airborne-derived sea ice emissivities up to 340 GHz in preparation for future satellite missions 

Nils Risse, Mario Mech, Catherine Prigent, Gunnar Spreen, and Susanne Crewell

Passive microwave radiometers onboard polar-orbiting satellites provide global information on the atmospheric state. The underlying retrievals require accurate knowledge of the surface radiative properties to distinguish atmospheric from surface contributions to the measured radiance. Polar surfaces such as sea ice contribute up to 400 GHz to the measured radiance due to the high atmospheric transmissivity under cold and dry conditions. Currently, we lack an understanding of sea ice parameters driving the variability in its radiative properties, i.e., its emissivity, at frequencies above 200 GHz due to limited field data and the heterogeneous sea ice structure. This will limit the use of future satellite missions such as the Ice Cloud Imager (ICI) onboard Metop-SG and the Arctic Weather Satellite (AWS) in polar regions.

To better understand sea ice emission, we analyze unique airborne measurements from 89 to 340 GHz obtained during the ACLOUD (summer 2017) and AFLUX (spring 2019) airborne campaigns and co-located satellite observations in the Fram Strait. The Polar 5 aircraft carried the Microwave Radar/radiometer for Arctic Clouds (MiRAC) cloud radar MiRAC-A with an 89 GHz passive channel and MiRAC-P with six double-sideband channels at 183.31 GHz and two window channels at 243 and 340 GHz. We calculate the emissivity with the non-scattering radiative transfer equation from observed upwelling radiation at 25° (MiRAC-A) and 0° (MiRAC-P) and Passive and Active Microwave radiative TRAnsfer (PAMTRA) simulations. The PAMTRA simulations are based on atmospheric profiles from dropsondes and surface temperatures from an infrared radiometer.

The airborne-derived sea ice emissivity (O(0.1km)) varies on small spatial scales (O(1km)), which align with sea ice properties identified by visual imagery. High-resolution airborne-derived emissivities vary more than emissivities from co-located overflights of the GPM constellation due to the smaller footprint size, which resolve sea ice variations. The emissivity of frozen and snow-free leads separates clearly from more compact and snow-covered ice flows at all frequencies. The comparison of summer and spring emissivities reveals an emissivity reduction due to melting. We will also conduct evaluations of emissivity parameterizations (e.g. TELSEM²) and provide insights into observations at ICI and AWS frequencies over Arctic sea ice. Findings based on the field data may be useful for the assimilation of radiances from existing and future microwave radiometers into weather prediction models in polar regions.

How to cite: Risse, N., Mech, M., Prigent, C., Spreen, G., and Crewell, S.: Analysis of airborne-derived sea ice emissivities up to 340 GHz in preparation for future satellite missions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12304, https://doi.org/10.5194/egusphere-egu23-12304, 2023.

EGU23-14227 | Orals | NP5.2

Combining sea-ice and ocean data assimilation with nudging atmospheric circulation in the AWI Coupled Prediction System 

Svetlana N. Losa, Longjiang Mu, Marylou Athanase, Jan Streffing, Miguel Andrés-Martínez, Lars Nerger, Tido Semmler, Dmitry Sidorenko, and Helge F. Goessling

Assimilation of sea ice and ocean observational data into coupled sea-ice, ocean and atmosphere models is known as an efficient approach for providing a reliable sea-ice prediction (Mu et al. 2022). However, implementations of the data assimilation in the coupled systems still remain a challenge. This challenge is partly originated from the chaoticity possessed in the atmospheric module, which leads to biases and, therefore, to divergence of predictive characteristics. An additional constrain of the atmosphere is proposed as a tool to tackle the aforementioned problem. To test this approach, we use the recently developed AWI Coupled Prediction System (AWI-CPS). The system is built upon the AWI climate model AWI-CM-3 (Streffing et al. 2022) that includes FESOM2.0 as a sea-ice ocean component and the Integrated Forecasting System (OpenIFS) as an atmospheric component. An Ensemble-type Kalman filter within the Parallel Data Assimilation Framework (PDAF; Nerger and Hiller, 2013) is used to assimilate sea ice concentration, sea ice thickness, sea ice drift, sea surface height, sea surface temperature and salinity, as well as temperature and salinity vertical profiles. The additional constrain of the atmosphere is introduced by relaxing, or “nudging”, the AWI-CPS large-scale atmospheric dynamics to the ERA5 reanalysis data. This nudging of the large scale atmospheric circulation towards reanalysis has allowed to reduce biases in the atmospheric state, and, therefore, to reduce the analysis increments. The most prominent improvement has been achieved for the predicted sea ice drift. Comprehensive analyses will be presented based upon the new system’s performance over the time period 2003 – 2022.

Mu, L., Nerger, L., Streffing, J., Tang, Q., Niraula, B., Zampieri, L., Loza, S. N. and H. F. Goessling, Sea-ice forecasts with an upgraded AWI Coupled Prediction System (Journal of Advances in Modeling Earth Systems, 14, e2022MS003176. doi: 10.1029/2022MS003176.

Nerger, L. and Hiller, W., 2013. Software for ensemble-based data assimilation systems—Implementation strategies and scalability. Computers & Geosciences, 55, pp.110-118.

Streffing, J., Sidorenko, D., Semmler, T., Zampieri, L., Scholz, P., Andrés-Martínez, M., Koldunov, N., Rackow, T., Kjellsson, J., Goessling, H., Athanase, M., Wang, Q., Sein, D., Mu, L., Fladrich, U., Barbi, D., Gierz, P., Danilov, S.,  Juricke, S., Lohmann, G. and Jung, T. (2022) AWI-CM3 coupled climate model: Description and evaluation experiments for a prototype post-CMIP6 model, EGUsphere, 2022, 1—37, doi: 10.5194/egusphere-2022-32

How to cite: Losa, S. N., Mu, L., Athanase, M., Streffing, J., Andrés-Martínez, M., Nerger, L., Semmler, T., Sidorenko, D., and Goessling, H. F.: Combining sea-ice and ocean data assimilation with nudging atmospheric circulation in the AWI Coupled Prediction System, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14227, https://doi.org/10.5194/egusphere-egu23-14227, 2023.

EGU23-14826 | Posters virtual | NP5.2 | Highlight

Inverse modelling for trace gas surface flux estimation, impact of a non-diagonal B-matrix 

Ross Bannister
One of the most appealing uses of data assimilation is to infer useful information about a dynamical system that is not observed directly. This is the case for the estimation of surface fluxes of trace gases (like methane). Such fluxes are not easy to measure directly on a global scale, but it is possible to measure the trace gas itself as it is transported around the globe. This is the purpose of INVICAT (the inverse modelling system of the chemical transport model TOMCAT), which has been developed here. INVICAT interprets observations of (e.g.) methane over a time window to estimate the initial conditions (ICs) and surface fluxes (SFs) of the TOMCAT model.
This talk will show how INVICAT has been expanded from a diagonal background error covariance matrix (B-matrix, DB) to allow an efficient representation of a non-diagonal B-matrix (NDB). The results of this process are mixed. A NDB-matrix for the SF field improves the analysis against independent data, but a NDB-matrix for the IC field appears to degrade the analysis. This paper presents these results and suggests that a possible reason for the degraded analyses is the presence of a possible bias in the system.

How to cite: Bannister, R.: Inverse modelling for trace gas surface flux estimation, impact of a non-diagonal B-matrix, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14826, https://doi.org/10.5194/egusphere-egu23-14826, 2023.

EGU23-14985 | ECS | Orals | NP5.2

Reconstructing North Atlantic Ocean Heat Content Using Convolutional Neural Networks 

Simon Lentz, Dr. Sebastian Brune, Dr. Christopher Kadow, and Prof. Dr. Johanna Baehr

Slowly varying ocean heat content is one of the most important variables when describing cli-
mate variability on interannual to decadal time scales. Since observation-based estimates of
ocean heat content require extensive observational coverage, incomplete observations are often
combined with numerical models via data assimilation to simulate the evolution of oceanic heat.
However, incomplete observations, particularly in the subsurface ocean, lead to large uncertain-
ties in the resulting model-based estimate. As an alternative approach, Kadow et al (2020) have
proven that artificial intelligence can successfully be utilized to reconstruct missing climate in-
formation for surface temperatures. In the following, we investigate the possibility to train their
three-dimensional convolutional neural network to reconstruct missing subsurface temperatures
to obtain ocean heat content estimates with a focus on the North Atlantic ocean.
The network is trained and tested to reconstruct a 16 member Ensemble Kalman Filter assimi-
lation ensemble constructed with the Max-Planck Institute Earth System Model for the period
from 1958 to 2020. Specifically, we examine whether the partial convolutional U-net represents
a valid alternative to the Ensemble Kalman Filter assimilation to estimate North Atlantic sub-
polar gyre ocean heat content.
The neural network is capable of reproducing the assimilation reduced to datapoints with ob-
servational coverages within its ensemble spread with a correlation coefficient of 0.93 over the
entire time period and of 0.99 over 2004 – 2020 (the Argo-Era). Additionally, the network is
able to reconstruct the observed ocean heat content directly from observations for 12 additional
months with a correlation of 0.97, essentially replacing the assimilation experiment by an extrap-
olation. When reconstructing the pre-Argo-Era, the network is only trained with assimilations
from the Argo-Era. The lower correlation in the resulting reconstruction indicates higher un-
certainties in the assimilation outside of its ensemble spread at times with low observational
density. These uncertainties are highlighted by inconsistencies in the assimilation’s represen-
tations of the North Atlantic Current at times and grid points without observations detected
by the neural network. Our results demonstrate that a neural network is not only capable of
reproducing the observed ocean heat content over the training period, but also before and after
making the neural network a suitable candidate to step-wise extend or replace data assimilation.

How to cite: Lentz, S., Brune, Dr. S., Kadow, Dr. C., and Baehr, P. Dr. J.: Reconstructing North Atlantic Ocean Heat Content Using Convolutional Neural Networks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14985, https://doi.org/10.5194/egusphere-egu23-14985, 2023.

EGU23-15189 | ECS | Orals | NP5.2

A coupled data assimilation framework with an integrated surface and subsurface hydrological model 

Qi Tang, Hugo Delottier, Oliver S. Schilling, Wolfgang Kurtz, and Philip Brunner

We developed an ensemble based data assimilation (DA) system for an integrated hydrological model to facilitate real-time operational simulations of water quantity and quality. The integrated surface and subsurface hydrologic model HydroGeoSphere (HGS) (Brunner & Simmons, 2012) which simulates surface water and variably saturated groundwater flow as well as solute transport, was coupled with the Parallel Data Assimilation Framework (PDAF) (Nerger et al., 2005). The developed DA system allows joint assimilation of multiple types of observations such as piezometric heads, streamflow, and tracer concentrations. By explicitly considering tracer and streamflow data we substantially expand the hydrologic information which can be used to constrain the simulations.    Both the model states and the parameters can be separately or jointly updated by the assimilation algorithm.  

A synthetic alluvial plain model set up by Delottier et al., (2022) was used as an example to test the performance of our DA system.  For flow simulations, piezometric head observations were assimilated, while for transport simulations, noble gas concentrations (222Rn, 37Ar, and 4He) were assimilated. Both model states (e.g., hydraulic head or noble gas concentrations) and parameters (e.g. hydraulic conductivities and porosity) are jointly updated by the DA. Results were evaluated by comparing the estimated model variables with independent observation data between the assimilation runs and the free run where no data assimilation was conducted. In a further evaluation step, a real-world, field scale model featuring realistic forcing functions and material properties was set up for a site in Switzerland and carried out for numerical simulations with the developed DA system. The synthetic and real-world examples demonstrate the significant potential in combing state of the art numerical models, data assimilation and novel tracer observations such as noble gases or Radon.

How to cite: Tang, Q., Delottier, H., Schilling, O. S., Kurtz, W., and Brunner, P.: A coupled data assimilation framework with an integrated surface and subsurface hydrological model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15189, https://doi.org/10.5194/egusphere-egu23-15189, 2023.

EGU23-16806 | Orals | NP5.2

Coupled data assimilation for numerical weather prediction at ECMWF 

Patricia de Rosnay, Phil browne, Eric de Boisséson, David Fairbairn, Sébastien Garrigues, Christoph Herbert, Kenta Ochi, Dinand Schepers, Pete Weston, and Hao Zuo

In this presentation we introduce coupled assimilation activities conducted in support of seamless Earth system approach developments for Numerical Weather Prediction and climate reanalysis at the European Centre for Medium-Range Weather Forecasts (ECMWF). For operational applications coupled assimilation requires to have reliable and timely access to observations in all the Earth system components and it relies on consistent acquisition and monitoring approaches across the components. We show recent and future infrastructure developments and implementations to support consistent observations acquisition and monitoring for land and ocean at ECMWF. We discuss challenges of surface sensitive observations assimilation and we show ongoing forward operator and coupling developments to enhance the exploitation of interface observations over land and ocean surfaces. We present plans to use new and future observation types from future observing systems such as the Copernicus Expansion missions.

How to cite: de Rosnay, P., browne, P., de Boisséson, E., Fairbairn, D., Garrigues, S., Herbert, C., Ochi, K., Schepers, D., Weston, P., and Zuo, H.: Coupled data assimilation for numerical weather prediction at ECMWF, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16806, https://doi.org/10.5194/egusphere-egu23-16806, 2023.

EGU23-164 | ECS | Orals | ITS1.8/AS5.5 | Highlight

Improvement and verification of urban extreme temperature predictions with satellite and ground observations in Austria (VERITAS-AT) 

Sandro Oswald, Stefan Schneider, Maja Zuvela-Aloise, Claudia Hahn, and Clemens Wastl

Extreme temperatures, especially long-lasting heat and cold waves in urban areas, lead to thermal stress of the population and increase the number of weather-related health risks and deaths. The observed climate trend and the associated increase of extreme weather events are expected to continue in the future. Thus, the evaluation of urban thermal stress and the associated health effects becomes an important issue for urban planning and risk management. For Austrian cities, an information system for temperature warnings already exists (Weather warnings, ZAMG), which is based on the information of regional weather forecast models. However, this information does not have the required spatial resolution needed to resolve urban structure and thus to account for the urban heat island effect or cold stress situations in winter.

The aim of this project is to provide the basis for the improvement of extreme weather/thermal (dis)comfort warning systems in Austrian major cities by using high-resolution weather predictions (100 m). Therefore, the soil model SURFEX (developed by Météo France) coupled with the AROME numerical weather forecast model is applied to selected cities in Austria and used to determine the best model configuration to compute short-term forecasts (+60 hours). This method provides not a full dynamical model, but a way of pyhsical downscaling with height corrections and a high-resolution surface model.

In this project, land use parameterization will be updated and improved based on Pan-European High Resolution Layers (e.g. Urban Atlas) of the Copernicus Land Monitoring service in ECOCLIMAP (predefined land use classes for SURFEX). The model output will be verified with in-situ operational and crowd-sourced observations. Furthermore, the results will be compared to the micro-scale urban climate model MUKLIMO_3 from the German Weather Service (100 m) and various thermal infrared (TIR with 150 to 250 m) datasets. The novel modeling approach for simulating thermal stress in urban areas serves as the basis for improving the operational prediction system of extreme temperatures, for optimizing the future extreme weather warning system at the ZAMG, and for decision-making for the involved cities and their stakeholders.

How to cite: Oswald, S., Schneider, S., Zuvela-Aloise, M., Hahn, C., and Wastl, C.: Improvement and verification of urban extreme temperature predictions with satellite and ground observations in Austria (VERITAS-AT), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-164, https://doi.org/10.5194/egusphere-egu23-164, 2023.

EGU23-353 | ECS | Posters on site | ITS1.8/AS5.5

The added value of regional climate simulations at kilometre-scale resolution to describe daily wind speed: the CORDEX FPS-Convection multi-model ensemble runs over the Alps 

María Ofelia Molina, Joao Careto, Claudia Gutiérrez, Enrique Sánchez, and Pedro Soares

In the recent past, the increase in computational resources allowed researchers to run simulations at increasingly horizontal and time resolutions. One such project is the World Climate Research Program’s Coordinated Regional Downscaling Experiments Flagship Pilot Studies (FPS) on convective phenomena. This FPS encompasses a set of simulations driven by the ERA-Interim reanalysis for the period from 2000-2009 (hindcast) and by the Coupled Model Intercomparison Project Phase 5 Global models for the 1996-2005 period (historical). Most models feature a horizontal resolution of 2.2 to 3 km, nested in an intermediate resolution of 12-25 km. An extended Alpine domain is considered for the simulations, due to the complexity of the mountain system together with heavy precipitation events, a large observational network and the high population density of the area. This initiative aims to build first-of-its-kind ensemble climate experiments of convective-permitting models to investigate convective processes over Europe and the Mediterranean.

 

In this study, the Distribution Added Value metric is used to determine the improvement of the representation of all available FPS hindcast and historical simulations for the daily mean wind speed. The analysis is performed on normalized empirical probability distributions and considers station observation data as a reference. The use of a normalized metric allows for spatial comparison among the different altitudes and seasons. This approach permits a direct assessment of the added value between the higher resolution convection-permitting regional climate model simulations against their global driving simulations and respective coarser resolution Regional Model counterparts. Although the complexity of such simulations, those not always reveal an added value. In general, results show that models add value to their reanalysis or forcing global model, but the nature and magnitude of the improvement on the representation of wind speed vary depending on the model, the spatial distribution and the season.

 

How to cite: Molina, M. O., Careto, J., Gutiérrez, C., Sánchez, E., and Soares, P.: The added value of regional climate simulations at kilometre-scale resolution to describe daily wind speed: the CORDEX FPS-Convection multi-model ensemble runs over the Alps, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-353, https://doi.org/10.5194/egusphere-egu23-353, 2023.

EGU23-617 | ECS | Posters on site | ITS1.8/AS5.5

Applying statistical downscaling to CMIP6 projections of precipitation for South America: Analysis of pre and post-processed simulations 

Glauber Willian de Souza Ferreira, Michelle Simões Reboita, and João Gabriel Martins Ribeiro

Global Climate Models (GCMs) are fundamental for simulating future climate conditions. However, such tools have limitations like their coarse resolution, systematic biases, and considerable uncertainties and spread among the projections generated by different models. Thus, raw outputs from GCMs are insufficient for regional-scale studies, which can be solved using downscaling techniques. These methods are particularly relevant for South America (SA), given the continent's climate regimes and topographic complexity. Moreover, critical socio-economic activities developed in SA, such as rainfed agriculture and hydroelectric power generation, are highly dependent on climate conditions and susceptible to extreme events, which can lead to intense droughts or floods depending on the region. Given the background, this study aims to analyze the performance of the statistical downscaling technique Quantile Delta Mapping (QDM) applied to precipitation projections simulated by an ensemble composed of eight GCMs from the Coupled Model Intercomparison Project Phase 6 (CMIP6) for SA. In this manner, we evaluate both the original precipitation projections from the GCMs, and after applying the QDM statistical downscaling technique. Daily precipitation data from the Climate Prediction Center (CPC), with a horizontal resolution of 0.5°, and from the Multi-Source Weighted-Ensemble Precipitation version 2 (MSWEPV2), with a horizontal resolution of 0.1°, are used as a reference, so the final resolution of the GCMs (and the ensemble) projections after the QDM technique application is the same from the different validation databases. Preliminary results with CPC indicate a satisfactory performance of the technique on precipitation simulations over SA.

 

The authors thank the CAPES, the R&D Program regulated by ANEEL, and the companies Engie Brasil Energia and Energética Estreito for their financial support.

How to cite: de Souza Ferreira, G. W., Simões Reboita, M., and Martins Ribeiro, J. G.: Applying statistical downscaling to CMIP6 projections of precipitation for South America: Analysis of pre and post-processed simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-617, https://doi.org/10.5194/egusphere-egu23-617, 2023.

Two main approaches to downscale global climate projections are possible: dynamical and statistical downscaling. Both families have been widely evaluated, but intercomparison studies between the two families are scarce, and usually limited to temperature and precipitation. In this work, we present a comparison between a Statistical Downscaling Model (SDM) based on Machine Learning and six Regional Climate Models (RCMs) from EURO-CORDEX, for five variables of interest: temperature, precipitation, wind, humidity and solar radiation. The study expands at a continental scale over Europe, with a spatial resolution of 0.11o and daily data. Both the SDM and the RCMs are driven by the ERA-Interim reanalysis, and observations are taken from the gridded dataset E-OBS. Several aspects have been evaluated: daily series, mean values and extremes, spatial patterns and also temporal aspects. Additionally, in order to analyze the intervariable consistency, a multivariable index (Fire Weather Index) derived from the fundamental variables has been included. The SDM has reached better scores than the RCMs for all the evaluated aspects with only a few exceptions, mainly related to an underestimation of the variance. After bias correction, both the SDM and the six RCMs present similar results, with no significant differences among them. Results presented here, combined with the low computational expense of SDMs and the limited availability of RCMs over some CORDEX domains, should motivate the consideration of statistical downscaling at the same level as RCMs by official providers of regional information, and its inclusion in reference sites. Nonetheless, further analysis on crucial aspects such as the impact on long-term trends or the sensitivity of different methods to being driven by Global Climate Models instead of by a reanalysis, is needed.

How to cite: Hernanz, A., Correa, C., Domínguez, M., Rodríguez-Guisado, E., and Rodríguez-Camino, E.: Can Statistical Downscaling based on Machine Learning compete with Regional Climate Models? A comparison for temperature, precipitation, wind, humidity and radiation over Europe under present conditions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1296, https://doi.org/10.5194/egusphere-egu23-1296, 2023.

The reliable prediction of flash flood relevant heavy precipitation events under climate change conditions remains a challenging task for the downscaling community. Therefore, a huge variety of downscaling approaches have been proposed and successfully applied, however, there is still potential for improvements. The conducted study aims to investigate potential improvements by circulation pattern (CP) trends conservation and their utilization for CP conditional statistical downscaling of daily summer precipitation in the (pre-)alpine region of Bavaria. The CPs have been created taking only atmospheric variables into consideration and the link to precipitation is established via CP conditional cumulative distribution functions (CDF) of the observed precipitation at selected measurement sites across the region. The derived CDFs allow for the sampling of CP conditional precipitation values at the station scale which are subsequently bias corrected by quantile mapping (QM) and parametric transfer functions (PTFs) as tested methods. The predicted precipitation values have been evaluated against obervations using different performance measures such as Kling-Gupta Efficiency (KGE), Root Mean Squared Error (RMSE) and Mean Absolute Error (MAE). In order to properly account for extreme events the evaluation has been conducted for the complete precipitation distribution and for the distribution above the 95th percentile seperately. The results show that the described CP conditional downscaling approach is capable of yielding more accurate daily precipitation values especially in the extremes compartment in which an average gain in prediction skill of + 0.24 and a maximum gain of + 0.6 in terms of KGE has been observed. This shows that the conservation of trends and atmospheric information through CPs and their utilization for downscaling can lead to improved precipitation downscaling results.

How to cite: Böker, B., Laux, P., Olschewski, P., and Kunstmann, H.: Accurate heavy precipitation prediction in an (pre-)alpine area: The benefit of trend conservation in circulation pattern conditional statistical downscaling., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2260, https://doi.org/10.5194/egusphere-egu23-2260, 2023.

While much effort has been devoted to analyzing long-term changes of temperature and precipitation in mean values and extremes, studies on changes in variability have been rather scarce. Trends in variability are, however, important, among others because their interaction with trends in mean values determines the degree with which extremes would change. The knowledge of long-term changes in temporal variability is essential for assessments of climate change impacts on various sectors, including hydrology (floods and droughts), agriculture, health, and energy demand and production.

SPAGETTA is a stochastic spatial daily weather generator (WG), which uses first-order multivariate (dimension = number of variables X number of gridpoints) autoregressive model to represent the spatial and temporal variability of surface weather variables (including precipitation and temperature). We consider the generator to be a suitable tool for assessing changes in the spatial and temporal variability of the weather series because of following reasons: (A) The inter-gridpoint lag-0 and lag-1(day) correlations included in a set of WG parameters may serve as representatives for spatial and temporal variability of input weather variables. (B) Statistical significance of changes in the lag-0 and lag-1 correlations derived from the input series may be easily assessed by comparing the changes with a variability of the lag-0 and lag-1 correlations related to the stochasticity in input weather series (the variability is assessed across a set of multiple realisations of the synthetic series). (C) Separate effects of changes in various statistical characteristics on any climatic characteristic may be easily assessed. Specifically, having analysed changes in the means, variability and inter-gridpoint correlations (e.g. based on RCM simulations of the future climate), we may modify only a selected (possibly only a single one) WG parameter(s) before producing the synthetic series and analysing effect of climate change on the climatic characteristics.

In the first part of the contribution, we employ SPAGETTA generator to analyse changes in interdiurnal variability of precipitation and temperature in 8 European regions (defined in Dubrovsky et al 2020, Theor Appl Climatol) using (a) gridded observational (last N years vs. first N years in available E-OBS times series) and (b) RCM-simulated surface weather series (2070-2099 vs 1971-2000; outputs from 19 RCMs available from the CORDEX database are analysed). In doing this, we assess the statistical significance of the detected changes. In the second part, we assess separate effects of changes in the means, variability and lag-0 & lag-1 correlations of temperature and precipitation (the changes based on a set of 19 RCM simulations are used to modify the corresponding WG parameters) on a set of climatic indices - including a set of compound precipitation-temperature characteristics representing spells of days with spatially significant extent of significantly non-normal weather (e.g. hot-dry spells).

How to cite: Dubrovský, M., Huth, R., Stepanek, P., Lhotka, O., Miksovsky, J., and Meitner, J.: Spatial and Temporal Variability of Precipitation and Temperature: Analysis of Recent Changes and Future Development with Use of the Weather Generator and RCM-Based Climate Change Scenarios, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2735, https://doi.org/10.5194/egusphere-egu23-2735, 2023.

EGU23-3343 | Orals | ITS1.8/AS5.5 | Highlight

Conceptual development and use of downscaled climate model information 

Robert Wilby and Christian Dawson

Statistical and dynamical downscaling techniques are widely applied in the development of local climate change scenarios. This talk traces the conceptual development of downscaling as a decision-support tool for climate risk assessment, resilience and adaptation planning. Four epochs are identified: (1) early exploration of local changes in key climate variables, such as temperature and precipitation extremes; (2) application of downscaled scenarios to climate impacts modelling (such as for agriculture yield or water resource assessments); (3) advent of ensemble-based methods and more sophisticated handling of uncertainty in the downscaling-impacts workflow; and (4) use of downscaled scenarios to stress-test adaptation options under plausible ranges of climate and non-climatic conditions. Each phase is illustrated by and reflected in the development of the Statistical DownScaling Model – Decision Centric (SDSM-DC) over more than two decades. Questions around fitness for purpose and appropriate uses of the tool are explored. The talk concludes by considering: where next for downscaling?

How to cite: Wilby, R. and Dawson, C.: Conceptual development and use of downscaled climate model information, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3343, https://doi.org/10.5194/egusphere-egu23-3343, 2023.

An atmospheric single-column model (SCM) developed in the framework of the Canadian Regional Climate Model, CRCM, driven by NCEP-NCAR reanalyses is applied to study the non-linear interactions between the surface and the planetary boundary layer (Goyette et al., 2020). The approach to solve the model equations and the technique described may be implemented in any RCM system environment as a model option. The working hypothesis underlying this SCM formulation is that a substantial portion of the variability simulated in the column can be reproduced by processes operating in the vertical dimension and a lesser portion comes from processes operating in the horizontal dimension. This SCM offers interesting prospects as the horizontal and vertical resolution of the RCM is ever increasing. Due to its low computational cost, multiple simulations may be carried out in a short period of time. In this paper, a range of possible results obtained by changing the lower boundary from open water surface to land, and by varying model parameters are mainly shown for central Mediterranean but also for other applications. Results show that the model responded in a highly nonlinear but coherent manner in the lowest levels with changes in air temperature, moisture and windspeed profiles. The latter are consistent with those of the surface vertical sensible, latent heat and momentum fluxes. For example in the central Mediterranean, during a simulated year, air temperature is increased during all the seasons. Specific humidity is increased during the autumn and winter seasons but decreased by during the spring and summer seasons thus showing the contrasting influence of the land surface. The potential for further developments, as well as some guidance as to how to handle mixed land/open water coupling in RCMs, is also provided.

GOYETTE, Stéphane, FONSECA, Cédric, TRUSCELLO, Léonard. Assessment of nonlinear effects of a deep subgrid lake with an atmospheric single‐column model. In: International Journal of Climatology, 2020. doi: 10.1002/joc.6890

How to cite: Goyette, S. and Kasparian, J.: Numerical investigation with a coupled single-column surface-atmosphere model and an application to central Mediterranean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3479, https://doi.org/10.5194/egusphere-egu23-3479, 2023.

EGU23-3741 | ECS | Orals | ITS1.8/AS5.5

Validation of MVT bias correction in dynamical downscaling simulations for climate extreme 

Meng-Zhuo Zhang, Ying Han, Zhongfeng Xu, and Weidong Guo

Dynamical downscaling is a widely-used approach to generate regional projections of future climate extremes at a finer scale. Previous studies indicated that the global climate model (GCM) bias correction method prior to dynamical downscaling can improve the simulation of the climate extreme to a certain extent. Recently, a new bias correction method termed MVT was developed. Note that this method did not correct the GCM biases of the climate extreme event explicitly. In this study, we evaluate the MVT method in terms of various climate extreme events through three dynamical downscaling simulations over Asia-western North Pacific with 25 km grid spacing throughout 1980–2014, and further investigate to what extent and how this bias correction method can improve the simulation of downscaled climate extreme events. The dynamical downscaling simulations driven by the original GCM dataset derived from the MPI-ESM1-2-HR (hereafter WRF_GCM), the bias-corrected GCM (hereafter WRF_GCMbc) are validated against that driven by the European Centre for Medium-Range Weather Forecasts Reanalysis 5 dataset, respectively. The results suggest that compared with the WRF_GCM, the WRF_GCMbc shows more than 26% decrease in root mean square errors of the precipitation and temperature extreme indices, and even 61% out of seasonal extreme indices show more than 50% reduction. Such improvements in the WRF_GCMbc are primarily caused by the correct simulation of the large-scale circulation due to the GCM bias correction. The large-scale circulation in turn improves the simulation of the precipitation and cloud by the water vapor transport and further improves the simulation of the 2m temperature by the radiation process and the surface energy balance, which contribute to the better simulation of the precipitation and temperature extreme indices.

How to cite: Zhang, M.-Z., Han, Y., Xu, Z., and Guo, W.: Validation of MVT bias correction in dynamical downscaling simulations for climate extreme, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3741, https://doi.org/10.5194/egusphere-egu23-3741, 2023.

EGU23-3922 | ECS | Posters on site | ITS1.8/AS5.5

Scale Heterogeneity Avoided Dasymetric Mapping for the Gridded Population 

Weipeng Lu and Qihao Weng

The gridded population, crucial for resource allocation and emergency support, is mainly downscaled from the census data with administrative divisions. A common dasymetric mapping approach is building a regression model between aggregated geospatial properties and population potential at the administrative level and then applying this model directly to the grid level. The aggregation of geospatial properties often relies on statistical methods like averaging. However, the difference in scale between the two levels can lead to the heterogeneity of geospatial properties, which causes a gap between the training domain and the target domain and makes these methods fail to preserve the physical meaning of geographic properties. To address this issue, we propose a deep learning-based approach, in which a sophisticated loss function involving tripartite elements, gridded geospatial properties, gridded population potential, and administrative population potential, is designed. In this way, scale heterogeneity both in aggregation and domains can be avoided. In this study, a 30-meter resolution population density map of Hong Kong is produced through the proposed approach. The validation result shows that compared with both the machine learning-based or the artificial neural network-based one, the proposed approach gets a lower RMSE and potentially provides a more accurate reference for detailed urban management.

How to cite: Lu, W. and Weng, Q.: Scale Heterogeneity Avoided Dasymetric Mapping for the Gridded Population, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3922, https://doi.org/10.5194/egusphere-egu23-3922, 2023.

EGU23-4495 | Orals | ITS1.8/AS5.5

Implications of statistical bias adjustment for uncertainties in regional model projections 

Muralidhar Adakudlu, Elena Xoplaki, and Niklas Luther

Regional climate models, due to their systematic biases, are not usable for impact assessment and policy-relevant applications. It is common to post-process the regional model outputs with appropriate bias correction methodologies to provide reliable climate change information. We apply a distribution-based, trend-preserving quantile mapping procedure to bias correct the projections of daily precipitation and temperature from an ensemble of 5 RCMs driven by 5 GCMs, each at a resolution of 0.11°, chosen from the EURO-CORDEX initiative. The gridded observations from the German Weather Service, DWD-HYRAS, has been used as a reference for the bias correction. The impact of the bias correction is found to be more pronounced on precipitation than on temperature, as the precipitation biases are larger. The models are wetter and underestimate (overestimate) the daily maximum (minimum) temperature. The correction method eliminates large parts of these biases and maps the distributions of both the variables well with that of observations. The bias adjustment also leads to the narrowing down of the uncertainties in the projected changes of both the variables. The decomposition of total variance into model uncertainty and internal variability suggests that the bias correction acts mostly on the former component. The internal variability component does not seem, however, to undergo considerable changes following the bias correction. Due to the reduction of the uncertainty, we find a slight improvement in the signal-to-noise ratio in the projections. 

How to cite: Adakudlu, M., Xoplaki, E., and Luther, N.: Implications of statistical bias adjustment for uncertainties in regional model projections, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4495, https://doi.org/10.5194/egusphere-egu23-4495, 2023.

In this study, a multi-model ensemble of regional climate and air quality coupling model system was established to evaluate current climate and air pollution in China during 2010-2014. Meteorological initial and boundary conditions were obtained from the multi earth system models used in the Coupled Model Intercomparison Project Phase 6 (CMIP6) with a dynamical downscaling method and the National Centers for Environmental Prediction Final Analysis (NCEP-FNL) reanalysis data. These downscaling data under the historical scenario and FNL data were applied to driven the Weather Research and Forecasting model coupled to Chemistry (WRF-Chem) to simulate current climate and air quality. A comprehensive evaluation of the current five years was conducted against the ground-level meteorological and chemical observations. The performances for the 2 m temperature were very well and consistently overestimated the wind speed at 10 m by 0.8~1.2 m/s. PM2.5 and ozone concentrations were underestimated by the downscaling data driven simulations compared with the FNL data. The model performance was relatively well and can be used to study the impacts of climate change on China's future air quality and pollution events in the context of carbon neutrality and clean air, which may shed light on policy formulation for medium and long-term air quality management and climate change alleviation.

How to cite: Cui, M.: Multi-model downscaling simulations of regional climate and air quality in China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5321, https://doi.org/10.5194/egusphere-egu23-5321, 2023.

Floods are highly destructive natural hazards causing widespread impacts on socio-ecosystems. This hazard could be further amplified with the ongoing climate change, which will likely alter magnitude and frequency of floods. Estimating how flood-rich periods could change in the future is however challenging. The classical approach is to estimate future changes in floods from hydrological simulations forced by time series scenarios of weather variables for different future climate scenarios. The development of relevant weather scenarios for this is often critical. To be adapted to the critical space and time scales of the considered basins, weather scenarios are thus typically produced from climate models with downscaling models, either dynamical or statistical.

In this study, we assessed the ability of two typical simulations chains to reproduce over the last century (1902-2009) and from large-scale atmospheric information only observed temporal variations of river discharges and flood events of the Upper Rhône River (10,900 km²). The modeling chains are made up of (i) the atmospheric reanalysis ERA-20C, (ii) either the statistical downscaling model SCAMP (Raynaud et al., 2020) or the dynamical downscaling model MAR (Gallée and Schayes, 1994), and (iii) the glacio-hydrological model GSM-SOCONT (Schaefli et al., 2005).

The daily Mean Areal Temperature (MAT) and Precipitation (MAP) time series were compared to the observed ones over the period 1961-2009. The meteorological results highlight the need for a bias-correction for both downscaling models. To avoid irrelevant simulations of the snowpack dynamics, especially for high elevations, the bias-correction was needed not only for the precipitation and temperature scenarios but also for the lapse scenarios of the dynamical downscaling chain. Simulated discharges are globally in very good agreement with the reference ones in the bias-corrected simulations. Whatever the river basin considered, the multi-scale observed variations of discharges are well reproduced (daily, seasonal and interannual). The reconstruction power of the chains is lower for low frequency hydrological situations, namely low flow sequences and annual discharge maxima. Flood events tend to be underestimated by each simulation chain.

Flood activity was also estimated from the discharge time series using the Peak Over Threshold (POT) method. The results over the last century are very promising, and encourage us to continue towards simulations over the last millennium. Outputs from the PMIP4 experiments (CESM1 Last Millennium Ensemble) will be statistically downscaled with the SCAMP model (for reasons of computation costs) and used as forcings in the GSM-SOCONT model.

References: 
- Raynaud et al. (2020) HESS doi.org/10.5194/hess-24-4339-2020 
- Gallée and Schayes, 1994 MWR doi:10.1175/1520-0493(1994)122<0671:DOATDM>2.0.CO;2
- Schaefli et al. (2005) HESS doi.org/10.5194/hess-9-95-2005

How to cite: Legrand, C., Wilhelm, B., and Hingray, B.: Simulating river discharges variations and flood events from large-scale atmospheric information with statistical and dynamical downscaling models: Example of the Upper Rhône River, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6168, https://doi.org/10.5194/egusphere-egu23-6168, 2023.

Climate simulations often need to be adjusted before carrying out climate impact studies at regional scale in order to reduce the biases often present in climate models. To do that, bias adjustment methods are usually applied to climate output simulations and are calibrated over a reference period. This period ideally includes good observational coverage and is often defined as the 2 or 3 more recent decades. However, on these timescales, the climate state may be influenced by the low-frequency internal climate variability. There is therefore a risk of introducing a bias to the climate projections by bias-adjusting simulations with low-frequency variability in a different phase to that of the observations. We proposed here a new pseudo-reality framework using an ensemble of simulations performed with the IPSL-CM6A-LR climate model in order to assess the impact of the low-frequency internal climate variability of the North Atlantic sea surface temperatures on bias-adjusted projections of mean and extreme surface temperature over Europe. We show that adjusting a simulation in a similar phase of the Atlantic Multidecadal Variability to that of the pseudo-observations reduces the pseudo-biases in temperature projections. Therefore, for models and regions where low frequency internal variability matters, it is recommended to sample relevant climate simulations to be bias adjusted in a model ensemble or alternatively to use a very long reference period when possible.

How to cite: Bonnet, R., Vrac, M., Boucher, O., and Jin, X.: Sensitivity of bias adjustment methods to low-frequency internal climate variability over the reference period: an ideal model study, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6529, https://doi.org/10.5194/egusphere-egu23-6529, 2023.

The nature and severity of climate change impacts varies significantly from region to region. Consequently, high-resolution climate information is needed for meaningful impact assessments and the design of mitigation strategies. This demand has lead to an increase in the coupling of Empirical Statistical Downscaling (ESD) models to General Circulation Model (GCM) simulations of future climate. Here, we present a new open-source Python package (pyESD; github.com/Dan-Boat/PyESD) that implements several Perfect Prognosis ESD (PP-ESD) methods and the whole downscaling cycle. The latter includes routines for data preparation, predictor selection and construction, model selection and training, evaluation, utility tools for relevant statistical tests, visualisation, and more. The package includes a collection of well-established Machine Learning algorithms and allows the user to choose a variety of estimators, cross-validation schemes, objective function measures, hyperparameter optimization, etc., in relatively few lines of codes. The package is highly modular and flexible, and allows quick and reproducible downscaling of any climate information, such as precipitation, temperature, wind speed or even glacial retreat. We demonstrate the effectiveness of the new PP-ESD framework by generating station-based downscaling products of precipitation and temperature for complex mountainous terrain in Southwest Germany.

How to cite: Mutz, S. G. and Boateng, D.: pyESD: An open-source Python framework for empirical-statistical downscaling of climate information, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7470, https://doi.org/10.5194/egusphere-egu23-7470, 2023.

EGU23-8234 | ECS | Posters on site | ITS1.8/AS5.5 | Highlight

Weather reconstruction and application for Switzerland: Long-term changes of spring weather impacts since 1763 

Imfeld Noemi and Brönnimann Stefan

Numerous historical sources report on hazardous past climate and weather events that had considerable impacts on society. Studying changes in their occurrence or mechanisms behind such events is however hampered by a lack of spatial weather information. For Switzerland, we created a daily high-resolution (1x1 km2) reconstruction of temperature and precipitation fields for the years 1763 to 1960 using an analog resampling method based on observational data. The resampled fields are further post-processed by assimilating temperature observations and quantile mapping the precipitation fields. Together with the present-day meteorological fields, this forms a more than 250-year long gridded data set.

We use this data set to evaluate changes in spring weather impacts over the last 250 years. The spring season receives fewer attention since it has no extreme events in absolute terms. However, it is relevant since weather conditions in spring can delay vegetation onset and growth, and can create substantial vegetation damages due to for example late frost and snow events. We evaluate therefore the long-term changes of spring fresh snow days, late frost days, frost days, and warm days, and compare it to changes of spring onset and reconstructed phenological stages.

How to cite: Noemi, I. and Stefan, B.: Weather reconstruction and application for Switzerland: Long-term changes of spring weather impacts since 1763, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8234, https://doi.org/10.5194/egusphere-egu23-8234, 2023.

EGU23-8829 | ECS | Posters on site | ITS1.8/AS5.5

A soil moisture downscaling playground of multiple resolution physics-based simulations 

Elena Leonarduzzi and Reed M Maxwell

Knowing soil moisture conditions accurately is extremely important for natural hazards prediction, agriculture, and other water resources management practices. Remote sensing products have been used more and more in these contexts. Their main advantage is the spatial coverage, which allows one to obtain continental or even global products. Nevertheless, there are limitations associated with them, such as reduced penetrating depth, impact of cloudiness and snow/ice, and low spatial and temporal resolutions. To compensate for the low spatial resolution, downscaling techniques have been developed that combine different remote sensing products and/or other data considered to affect soil moisture redistribution. The main limitation in their development, is the lack of data to validate the techniques and the final product. Oftentimes in situ measurements are used for the calibration/training and for the testing/verification. These are very sparse, i.e., only available at few locations, and hard to compare directly, as both the satellite products and the downscaled estimates are volumetric and not point estimates.

Here, we create a soil moisture downscaling playground by generating soil moisture estimates with a physics-based hydrological model (ParFlow-CLM) at different resolutions, from a few kilometers to 100 meters. Having continuous gridded estimates of high- and low- resolution soil moisture with a reliable physics-based model, allows us to test and compare different downscaling techniques as well as the impact on the scaling of individual inputs/parameters. As an initial experiment, we model the East Taylor catchment (Colorado, USA) at 100m and 1000m resolution, by only changing the topography (i.e., all other inputs are resolved at 1000m), which is not only the best-known input even at high resolutions, but also the most impactful in soil moisture redistribution. The best performing downscaling technique will allow us, in an operational setup, to run the physics-based model at a coarser resolution but still have a high-resolution product in a computationally inexpensive manner. Beyond our application, the high- and low- resolution simulations generated in this work can be used for the validation of any downscaling technique also applicable with remote sensing products.

How to cite: Leonarduzzi, E. and Maxwell, R. M.: A soil moisture downscaling playground of multiple resolution physics-based simulations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8829, https://doi.org/10.5194/egusphere-egu23-8829, 2023.

EGU23-9644 | ECS | Orals | ITS1.8/AS5.5

Analysis of Ensemble Uncertainty Transfer in AI-Based Downscaling of C3S Seasonal Forecast 

Qing Lin, Fatemeh Heidari, Edgar Fabián Espitia Sarmiento, Muralidhar Adakudlu, Andrea Toreti, and Elena Xoplaki

Copernicus Climate Change Service (C3S) integrates multiple seasonal forecast models of climate variables with multiple ensemble realizations. Assessing the risks of natural hazards with high impacts on human and natural systems and providing actionable services at the local scale require high-resolution predictions. We implement the AI-based approach proposed by Heidari et al. (2023) to address such needs and reach a kilometer scale. While downscaling seasonal forecasts, it is crucial to transfer the full range of the uncertainties given by the ensembles.

This study assesses how uncertainty is transferred by an AI-based downscaling approach. Quantile-based metrics are here used to measure the ensemble variability between seasonal forecasts and their downscaled products. On the other side, quantile-based metrics can also give an alternative description of the ensemble variabilities, which could replace the raw ensemble members in the downscaling process. In this study, the AI-downscaling system is tested by inputting (a) raw ensemble members and (b) quantile-based metrics. Transferred uncertainty and downscaling accuracy are then evaluated to develop and implement an optimal downscaling approach with hazard-dependent inputs being selected at  regional and local scales.

 

Heidari F., Lin Q., Espitia Sarmiento E.F., Toreti A., and Xoplaki E. (2023): A deep learning technique to realistically bias correct and downscale seasonal forecast ensembles of climate variables towards the development of an AI-based early warning system, EGU 2023 abstract

How to cite: Lin, Q., Heidari, F., Espitia Sarmiento, E. F., Adakudlu, M., Toreti, A., and Xoplaki, E.: Analysis of Ensemble Uncertainty Transfer in AI-Based Downscaling of C3S Seasonal Forecast, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9644, https://doi.org/10.5194/egusphere-egu23-9644, 2023.

The lack of long-term and consistent meteorological observations limits the application of land-surface simulators (e.g., of phenomena in hydrology, the cryosphere, ecology) at remote locations. For example, most permafrost areas are remote and lacking consistent meteorological time series, models that describe permafrost change over time cannot be driven for comparison with observations or for impact studies. Reanalysis-derived time series are valuable because they are available with global coverage, for a long time period, and for a broad set of physically consistent variables. Multiple reanalyses can be used to provide estimates of uncertainty. Practically, however, this data is difficult to use for several reasons: grid-scale reanalyses must be downscaled and interpolated horizontally (and vertically within the atmospheric column for mountains regions) to the site‑scale, differences in variables, units, and delivery between reanalyses must be reconciled, and large volumes of data need to be handled. Globsim is an open-source python library (available via GitHub) that was developed to handle these challenges and to facilitate a simulation workflow that takes advantage of the multiple reanalysis products available today. It outputs sub-daily meteorological time series that resemble meteorological stations for any location on the planet. Since the release of the first version of Globsim, we have improved usability, refactored code for maintainability and speed, and fixed a number of bugs. We also added support for ERA5 ensemble data, and added more sophisticated heuristic downscaling algorithms, including TOPOscale for elevation-adjusted radiative fluxes. We use Globsim as a core tool in a multi-model permafrost simulation workflow and, as a future step, we intend to use it as part of a debiasing routine to make predictions of permafrost using climate scenarios. We expect this tool to be broadly applicable to climate change impact modelers and other scientists using climate driven simulations working in (remote) locations that lack meteorological data of sufficient quality and duration for their application.

How to cite: Brown, N., Gruber, S., and Cao, B.: Globsim v.3 – Improvements to an open-source software library for utilizing atmospheric reanalyses in point-scale land surface simulation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10595, https://doi.org/10.5194/egusphere-egu23-10595, 2023.

EGU23-11124 | Orals | ITS1.8/AS5.5

Reducing negative impacts of bias adjustment on the distribution tail and extreme climate indicators in MIdAS 

Peter Berg, Thomas Bosshard, Lars Bärring, Johan Södling, Renate Wilcke, Wei Yang, and Klaus Zimmermann

Bias adjustment of climate models is today normally performed with quantile mapping methods that account for the whole distribution of the parameter. The bulk of the distribution is well described as long as sufficient data records are used (Berg et al., 2012), however, the extreme tails will always suffer from large uncertainties. These uncertainties stem from both the climate model and the reference data set, which prevents a robust and detailed identification of bias in the extreme tail. Empirical quantile mapping methods are therefore prone to overfitting, and may introduce substantial bias when applied outside the calibration period. Commonly, a constant adjustment is applied for values outside the range of the calibration period, but there is room for improvements of the extrapolation method.

While working with a climate service for Sweden, a clear offset was identified between data adjusted within and outside the calibration period for an extreme indicator of daily maximum precipitation. This study explores different extrapolation methods for the extreme tail of the distribution in the spline-based empirical quantile mapping method of the MIdAS bias adjustment method (Berg et al., 2022). By limiting the bias adjustment to the first 95% of the distribution, and thereafter applying a constant or a linear fit to the remaining 5% of data in the tail, the offset is strongly reduced and the adjusted extremes become more robust and plausible.

Berg, P., Feldmann, H., & Panitz, H. J. (2012). Bias correction of high resolution regional climate model data. Journal of Hydrology448, 80-92.

Berg, P., Bosshard, T., Yang, W., & Zimmermann, K. (2022). MIdASv0. 2.1–MultI-scale bias AdjuStment. Geoscientific Model Development15(15), 6165-6180.

How to cite: Berg, P., Bosshard, T., Bärring, L., Södling, J., Wilcke, R., Yang, W., and Zimmermann, K.: Reducing negative impacts of bias adjustment on the distribution tail and extreme climate indicators in MIdAS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11124, https://doi.org/10.5194/egusphere-egu23-11124, 2023.

EGU23-11595 | ECS | Orals | ITS1.8/AS5.5

Understanding the double-ITCZ problem over the Atlantic with bias-corrected downscaling 

Shuchang Liu, Christian Zeman, and Christoph Schär

The long-existing double-ITCZ problem in GCMs affects not only the models' ability in simulating the current climate, but also implies limitations regarding the assessment of climate sensitivity and global climate change. Using a regional climate model (RCM) with explicit convection at a horizontal grid spacing of 12 km in a large computational domain covering the tropical and sub-tropical Atlantic, we develop a bias-correction downscaling methodology to remove the biases of a driving GCM. The methodology is related to the pseudo-global warming (PGW) approach. Normally this method is used to impress the climate-change signal to a reanalysis-driven RCM simulation, but it can also be used to modulate the lateral-boundary conditions of a GCM, such as to remove the large-scale biases. We show that the double ITCZ problem persists with classical dynamical downscaling (i.e. when driving the RCM directly by the GCM output), but with our bias-corrected downscaling the double ITCZ problem can be removed. Detailed analysis reveals that the main cause of the double ITCZ problem can be attributed to the GCMs' SST bias. Compared to the GCMs' AMIP simulations, RCMs with higher resolution allow explicit deep convection and enable a better simulation of tropical convection and clouds. By improving the corresponding radiative forcing, vertical motion is better simulated. Subsidence stronger to the south of the ITCZ pushes the ITCZ more north in the boreal spring, which is consistent with the observation of the ITCZ. The developed methodology provides an opportunity for better constraining climate sensitivity by removing double-ITCZ biases.

How to cite: Liu, S., Zeman, C., and Schär, C.: Understanding the double-ITCZ problem over the Atlantic with bias-corrected downscaling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11595, https://doi.org/10.5194/egusphere-egu23-11595, 2023.

Enel, as most of the Energy Players, has an important exposure on weather risk due to the indirect effect of the power demand and to the direct effects on renewable production. A large component of such risk comes from the hydroelectric production, this is especially true in Southern America where, in some countries, it can represent up to 70% of the total production. We present a practical development of an operational chain to extract information from the seasonal forecasts produced by SEAS5. It works on some catchments in Colombia and Peru with the aim to provide an ensemble forecast of monthly precipitations at a high resolution from the fields at low resolution provided by Copernicus. To produce the high-resolution fields of precipitations we developed a procedure based on Lorenz et al. (2021); for our scope, the biases of the SEAS5 forecasts are corrected following a reference climatology obtained from the SEAS5 hindcasts that is calibrated over the cumulative distribution function calculated be mean of historical measurements of the IDEAM weather stations. The method and preliminary results as well as the validation will be shown in this work.

How to cite: Rea, G., Galuzzo, D., and Formenton, M.: Development of an operational seasonal forecast in Colombia and Peru by mean of statistical downscaling of the SEAS5-Copernicus data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12395, https://doi.org/10.5194/egusphere-egu23-12395, 2023.

EGU23-12899 | ECS | Orals | ITS1.8/AS5.5

A downscaling exercise for the Adriatic Sea in a perfect model approach 

Renata Tatsch Eidt, Giorgia Verri, Vladimir Santos da Costa, Murat Gunduz, and Antonio Navarra

In this study, the predictability of the coastal ocean is assessed in a downscaling exercise for the Adriatic Sea using NEMO 3.6 over a 19 years’ time window (2001-2019). Inspired by the perfect model approach (Denis et al. 2002, De Elia et al. 2002) using a dynamical downscaling setup, a high resolution (2 km) experiment (Big Brother – BB) for the entire Adriatic Sea is used as the “true” reference for a smaller domain, downscaling experiment (Little Brother – LB) in the Northern Adriatic subbasin. The LB experiment has the same horizontal resolution as the BB (2 km) and is downscaled from a low resolution parent model (6 km), in a ratio of 1/3 resolution jump. The 2 km horizontal resolution fits the purpose of reaching an eddy-permitting grid spacing in the Adriatic basin (Masina and Pinardi, 1994; Cushman-Roisin et al. 2002).

Power spectral density analysis is used to evaluate the kinetic energy variance on the frequency domain among the experiments and compare them with the BB experiment. Overall, the LB is more energetic than the parent model, and the timing of the peaks of energy coincides with the ones of the BB. The energy on the 1 year signal is higher in the LB than the BB. The LB can recover a significant amount of energy for all peaks, with special attention to the 6 months period, which is poorly captured by the parent model. The 4 months signal is equally represented in BB and LB, while there is an underestimation of the 6 months signal of LB with respect to BB. Energy in the LB does not deviate from BB more than ~20% in the low frequencies and ~10% in the high frequencies, while the parent model presents in a whole lower energy than the BB, with higher differences on the low frequencies.

The Northern Adriatic circulation is largely influenced by the surface buoyancy flux and the wind forcing (Cessi et al., 2014), which play a significant role in the energy budget and the anti-estuarine overturning circulation of the Adriatic basin. Differences between LB and parent model results may be associated with the energy cascade due to interactions of internal dynamic processes which are differently represented at different resolutions. Differences between LB and BB results are the effect of the downscaling method and the horizontal resolution ratio between the parent model and the nested LB.

Moreover, the analysis of the wavenumber spectra allows a clear overview of the energy distribution in the space domain among the experiments and the representation of small-scale features in the LB. Small scale features less than twice the grid spacing (~12 km) are absent in the low-resolution parent model outputs. Therefore, the comparison with the true reference, BB, reveals the energy spectrum of the parent model solves only the larger scales, while the downscaling LB can recover the smaller scales absent in the initial and lateral boundary conditions.

How to cite: Tatsch Eidt, R., Verri, G., Santos da Costa, V., Gunduz, M., and Navarra, A.: A downscaling exercise for the Adriatic Sea in a perfect model approach, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12899, https://doi.org/10.5194/egusphere-egu23-12899, 2023.

EGU23-13876 | ECS | Posters on site | ITS1.8/AS5.5

Evaluating state-of-art statistical downscaling and analogs approaches on historical climate statistics over European regions 

Daniele Peano, Lorenzo Sangelantoni, and Carmen Alvarez-Castro

Climate change impacts assessment crucially relies on climate information at high temporal and spatial resolutions, not available from global climate models (GCMs) involved in the coupled model intercomparison project (CMIP). At the same time, dynamically downscaled regional climate model simulations do not provide global-scale coverage and in several cases are computationally too expensive.

For this reason, downscaling techniques are commonly applied to bridge the resolution gap between GCM simulations and impact studies. The most common methodology is the statistical downscaling approach. However, statistical downscaling fast computation comes at a price, it does not account for physical and dynamic processes potentially inflates temporal variability of the original simulations’ resolution. Given this limitation, the analogs technique may represent a valuable alternative since it considers both large and local scales dynamics balanced by a reasonable increase in computational costs.

The present study explores differences, added value, and limitations characterizing state-of-the-art bias adjustment/statistical downscaling based on a stochastic quantile mapping approach and the analogs technique. In particular, the comparison applies to the data computed in the inter-sectoral impact model intercomparison project (ISIMIP) and data obtained by applying the analogs method based on the same ISIMIP reference dataset. The two approaches are compared and evaluated in terms of the historical period observed statistics reproduction for a few climate variables over European regions.

This study is performed in the framework of GoNEXUS and NEXOGENESIS European projects.

How to cite: Peano, D., Sangelantoni, L., and Alvarez-Castro, C.: Evaluating state-of-art statistical downscaling and analogs approaches on historical climate statistics over European regions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13876, https://doi.org/10.5194/egusphere-egu23-13876, 2023.

EGU23-14253 | ECS | Orals | ITS1.8/AS5.5 | Highlight

Downscaling with a machine learning-based emulator of a local-scale UK climate model 

Henry Addison, Elizabeth Kendon, Suman Ravuri, Laurence Aitchison, and Peter Watson

High resolution rainfall projections are useful for planning for climate change [1] but are expensive to produce using physical simulations. We make novel use of a state-of-the-art generative machine learning (ML) method, diffusion models [2], to more cheaply generate high resolution (8.8km) daily mean rainfall samples over England and Wales conditioned on low resolution (60km) climate model variables. The downscaling model is trained on output from the Met Office UK convection-permitting model (CPM) [3]. We then apply it to predict high-resolution rainfall based on either coarsened CPM output or output from the Met Office HadGEM3 general circulation model (GCM). The downscaling model is stochastic and able to produce samples of high-resolution rainfall that have realistic spatial structure, which previous methods struggle to achieve. It is also easy to train and should better estimate the probability of extreme events compared to previous generative ML approaches.

The downscaling model samples match well the rainfall distribution of CPM simulation output. We use as our conditioning variables We obtained further improvements by also including high-resolution, location-specific parameters that are learnt during the ML training phase. We will discuss the challenges of applying the model trained on coarsened CPM variables to GCM variables and present results about the method’s ability to reproduce the spatial and temporal behaviour of rainfall and extreme events that are better represented in the CPM than the GCM due to the CPM’s ability to model atmospheric convection.

References

[1] Kendon, E. J. et al. (2021). Update to the UKCP Local (2.2km) projections. Science report, Met Office Hadley Centre, Exeter, UK. [Online]. Available: https://www.metoffice.gov.uk/pub/data/weather/uk/ukcp18/science-reports/ukcp18_local_update_report_2021.pdf

[2] Song, Y. et al. (2021). Score-Based Generative Modeling through Stochastic Differential Equations. ICLR.

[3] Met Office Hadley Centre. (2019). UKCP18 Local Projections at 2.2km Resolution for 1980-2080, Centre for Environmental Data Analysis. [Online]. Available: https://catalogue.ceda.ac.uk/uuid/d5822183143c4011a2bb304ee7c0baf7

How to cite: Addison, H., Kendon, E., Ravuri, S., Aitchison, L., and Watson, P.: Downscaling with a machine learning-based emulator of a local-scale UK climate model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14253, https://doi.org/10.5194/egusphere-egu23-14253, 2023.

Statistical bias adjustment is now common practice when using climate models for impact studies, prior to or in conjunction with downscaling methods. Examples of widely used methodologies include CDFt (Vrac et al. 2016), ISIMIP3BASD (Lange 2019) or equidistant CDF matching (Li et al. 2010). Though common practice, recent papers (Maraun et al. 2017) have found fundamental issues with statistical bias adjustment. When multivariate aspects are not evaluated, improper use of bias adjustment is not detected. Fundamental misspecifications of the climate model, such as the displacement of large-scale circulation, cannot be corrected. Furthermore, results are sensitive to internal climate variability over the reference period (Bonnet et al 2022). If applied, bias adjustment methods should therefore be evaluated carefully in multivariate aspects and targeted to the use-case at hand.

However, good practice in the evaluation and application of bias adjustment methods is inhibited by what we frame as practical issues. If at all, published bias adjustment methods are often published as individual software packages across different programming languages (mostly R and Python) that do not allow users to adapt aspects of the method, such as the fit distribution, to their use-case. Existing open-source software packages, such as ISIMIP3BASD or CDFt, often do not offer an evaluation framework that covers multivariate (spatial, temporal, multi-variable) aspects necessary to detect misuse of methods, or user-specific impact metrics. Several of these issues apply to downscaling similarly.

To address some of these practical issues, we developed the open-source software package ibicus in collaboration with ECWMF (available on PyPi, extensive documentation https://ibicus.readthedocs.io/en/latest/index.html, published under Apache 2.0 licence). The package implements eight peer-reviewed bias adjustment methods in a common framework. It also includes an extensive evaluation framework covering multivariate aspects as well as the ETCCDI climate indices. The package thereby contributes to enhanced flexibility and ease-of-use of better evaluation practises in bias adjustment.

Our contribution presents three case studies using ibicus, highlighting a number of pitfalls in the usage of bias adjustment for climate impact modelling, and shows possible ways to address these issues. We investigate extreme indices of precipitation and compound extreme temperature-precipitation indices, modification of the climate change trend, and dry spell length as an example of a temporal index, over northern Spain and Turkey.

We evaluate how bias adjustment adds to the ‘cascade of uncertainty’ and how this can be made transparent in the different use-cases. We also demonstrate how some of the fundamental issues that can arise when applying bias adjustment can be detected and how evaluation of spatial and temporal aspects such as dry spell length can be made specific to the use-case at hand to detect improper use of bias adjustment. Lastly, we demonstrate how the ‘best’ bias adjustment method may depend on the metric of interest, and therefore a user-centric design of comparison and evaluation methods is necessary.

How to cite: Spuler, F., Wessel, J., Cagnazzo, C., and Comyn-Platt, E.: Case studies in bias adjustment: addressing potential pitfalls through model comparison and evaluation using a new open-source python package, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14254, https://doi.org/10.5194/egusphere-egu23-14254, 2023.

EGU23-15537 | ECS | Posters virtual | ITS1.8/AS5.5

Analysis of the statistical bias correction of ERA5-Land on different time aggregations in Trentino-Alto Adige 

Andrea Menapace, Pranav Dhawan, Daniele Dalla Torre, Michele Larcher, and Maurizio Righetti

Global and regional climate models are constantly improving the quality of their outputs with increasingly fine spatial and temporal resolutions. These products, which comprise, for instance, reanalysis, reforecast and forecast, can be used for several applications, such as boundary conditions for climate simulations, initial conditions for local weather forecasting, and reference datasets for environmental and energy uses. Nevertheless, many authors have pointed out that such climate models are not suitable for direct use in local applications due to the presence of biases between the model results and the metered data. At this aim, several statistical methodologies have been proposed to correct and downscale the climate models outputs and make it available also for local purposes. Therefore, the purpose of this contribution is to analyse the current state-of-the-art statistical bias correction methods on different time aggregation to assess the capabilities of these methods from monthly to hourly temporal scale.

This study is carried out on the Trentino- Alto Adige, which is an alpine region in north Italy equipped with several measuring weather stations, around 300. The temperature and precipitation observations have been then used to produce a reference dataset through the geostatistical interpolation method called kriging. Instead, ERA5-Land, the reanalysis of ECMWF, has been adopted for the bias correction analysis. Several methods have been tested comprising of univariate and multivariate method including: linear scaling, variance scaling, local intensity scaling, local power transformation, quantile mapping, quantile delta mapping, and multivariate bias correction methods such as MBCn, MBCp, and MBCr. The time scale investigated are monthly, daily and hourly aggregations.

The results show a general decreasing of the performance of all the bias correction methods with the increase in the time-frequency of the weather variables. In particular, the mean absolute error of the corrected daily temperature is 50% larger than the monthly one, and the same 50% increase in error is found between daily and hourly corrected data. The increase in error with decreasing temporal resolution is even more pronounced for the precipitation variable, which is known to be discontinuous with respect to temperature. Multivariate bias correction methods seem to have difficulty maintaining dependencies between variables in the case of high-frequency data.

Although the results on the hourly data are not so scarce, it is evident that more depth analysis of temporal high-resolution climate data is needed, including sub-hourly data in the future, and therefore become crucial to develop new methodologies capable of correcting sub-daily bias. In conclusion, with this work, the authors seek to support research in the direction of providing high-frequency weather data for local applications, which are crucial, for example, in hydrological simulations for the assessment of hydrogeological risks and the management of renewable energy in the electricity market.

How to cite: Menapace, A., Dhawan, P., Dalla Torre, D., Larcher, M., and Righetti, M.: Analysis of the statistical bias correction of ERA5-Land on different time aggregations in Trentino-Alto Adige, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15537, https://doi.org/10.5194/egusphere-egu23-15537, 2023.

EGU23-17077 | ECS | Orals | ITS1.8/AS5.5

Extending A Posteriori Random Forests for Multivariate Statistical Downscaling of Climate Change Projections 

Mikel N. Legasa, Soulivanh Thao, Mathieu Vrac, Ana Casanueva, and Rodrigo Manzanas
Under the perfect prognosis approach, statistical downscaling (SD, Gutiérrez et al., 2019) methods aim to learn the relationships between large-scale variables from reanalysis and local observational records. Typically, these statistical relationships, which can be learnt employing many different statistical and machine learning models, are subsequently applied to downscale future global climate model (GCM) simulations, obtaining local projections for the region and variables of interest. 
A posteriori random forests (APRFs) were introduced in a recent paper (Legasa et al., 2021) for precipitation downscaling, but can be potentially used to estimate any probabilitydistribution. While performing similarly to other state-of-the-art machine learning methodologies like convolutional neural networks in terms of predictive performance (as measured in terms of correlation of the downscaled series with the observed series), APRFs produce less biased simulations, as measured by several distributional indicators.Furthermore, climate change signals projected by APRFs are consistent with those given by the raw GCM outputs, thus proving suitable for downscaling local climate change scenarios (Legasa et al. 2023, in review). Moreover, they also automatically select the most adequate large-scale variables and geographical domain of interest, a time-consuming task and potential source of uncertainty (Manzanas et al. 2020) when downscaling climate change projections.
In this work we show how the APRF methodology can be easily extended to more complex and multivariate distributions. One of the proposed extensions is temporal APRFs, which explicitly model the transition in time for a variable and location of interest (e.g. the rainfall probability conditioned to the dry/wet state of the previous day), thus improving the temporal consistency of the downscaled series in terms of several temporal (e.g. spells) indicators. Other possible extensions within the APRF framework include predicting the joint probability distribution of several geographical locations, thus improving the spatial consistency of the downscaled series; and modeling the multivariate joint distribution of different meteorological variables (e.g. precipitation, humidity and temperature).
 
References
Gutiérrez, J.M., Maraun, D., Widmann, M. et al. An intercomparison of a large ensemble of statistical downscaling methods over Europe: Results from the VALUE perfect predictor cross-validation experiment. Int. J. Climatol. 2019; 39: 3750– 3785. doi: https://doi.org/10.1002/joc.5462
Legasa, M. N., Manzanas, R., Calviño, A., & Gutiérrez, J. M. (2022). A posteriori random forests for stochastic downscaling of precipitation by predicting probability distributions. Water Resources Research, 58 (4), e2021WR030272. doi: https://doi.org/10.1029/2021WR030272
Legasa, M. N., Thao, S., Vrac, M., & Manzanas, R. (2023). Assessing Three Perfect Prognosis Methods for Statistical Downscaling of Climate Change Precipitation Scenarios. Submitted to Geophysical Research Letters.
Manzanas, R., Fiwa, L., Vanya, C. et al. Statistical downscaling or bias adjustment? A case study involving implausible climate change projections of precipitation in Malawi. Climatic Change 162, 1437-1453 (2020). doi: https://doi.org/10.1007/s10584-020-02867-3

How to cite: Legasa, M. N., Thao, S., Vrac, M., Casanueva, A., and Manzanas, R.: Extending A Posteriori Random Forests for Multivariate Statistical Downscaling of Climate Change Projections, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17077, https://doi.org/10.5194/egusphere-egu23-17077, 2023.

EGU23-135 | ECS | Orals | GI4.2

Deep-Pathfinder: A machine learning algorithm for mixing layer height detection based on lidar remote sensing data 

Jasper Wijnands, Arnoud Apituley, Diego Alves Gouveia, and Jan Willem Noteboom

The mixing layer height (MLH) indicates the change between vertical mixing of air near the surface and less turbulent air above. MLH is important for the dispersion of air pollutants and greenhouse gases, and assessing the performance of numerical weather prediction systems. Existing lidar-based MLH detection algorithms typically do not use the full resolution of the ceilometer, require manual feature engineering, and often do not enforce temporal consistency of the MLH profile. Given the large-scale availability of lidar remote sensing data and the high temporal and spatial resolution at which it is recorded, this domain is very suitable for machine learning approaches such as deep learning. This presentation introduces a completely new approach to estimate MLH: the Deep-Pathfinder algorithm, based on deep learning techniques for image segmentation.

The concept of Deep-Pathfinder is to represent the 24-hour MLH profile as a mask (i.e., black indicating the mixing layer, white indicating the non-turbulent atmosphere above) and directly predict the mask from an image with lidar observations. Range-corrected signal (RCS) data at 12-second temporal and 10-meter vertical resolution was obtained from Lufft CHM 15k ceilometers at five locations in the Netherlands (2020–2022). High-resolution annotations were created for 50 days, informed by a visual inspection of the RCS image, the manufacturer's layer detection algorithm, gradient fields, thermodynamic MLH estimates, and humidity profiles of the 213-meter mast at Cabauw.

Our model is based on a customised U-Net architecture with MobileNetV2 encoder to ensure fast inference times. A nighttime variable indicated whether the sample occurred between sunset and sunrise and hence, whether an estimate of the stable or convective boundary layer was required. Model calibration was performed on the Dutch National Supercomputer Snellius. First, input samples were randomly cropped to 224x224 pixels, covering a 45-minute period and maximum altitude of 2240 meters. Then, the model was pre-trained on 19.4 million samples of unlabelled data. Finally, the labelled data was used to fine-tune the model for the task of mask prediction. Performance on a test set was compared to MLH estimates from ceilometer manufacturer Lufft and the STRATfinder algorithm.

Results showed that days with a clear convective boundary layer were captured well by all three methods, with minimal differences between them. The Lufft wavelet covariance transform algorithm contained a slight temporal shift in MLH estimates. Further, it had more missing data in complex atmospheric conditions. STRATfinder estimates for the nocturnal boundary layer were consistently low due to guiding restrictions in the algorithm. In contrast, Deep-Pathfinder followed short-term fluctuations in MLH more closely due to the use of high-resolution input data. Path optimisation algorithms like STRATfinder have good temporal consistency but can only be evaluated after a full day of ceilometer data has been recorded. Deep-Pathfinder retains the advantages of temporal consistency by assessing MLH evolution in 45-minute samples, however, it can also provide real-time estimates. This makes a deep learning approach as presented here valuable for operational use, as real-time MLH detection better meets the requirements of users in aviation, weather forecasting and air quality monitoring.

How to cite: Wijnands, J., Apituley, A., Alves Gouveia, D., and Noteboom, J. W.: Deep-Pathfinder: A machine learning algorithm for mixing layer height detection based on lidar remote sensing data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-135, https://doi.org/10.5194/egusphere-egu23-135, 2023.

EGU23-1387 | ECS | Posters on site | GI4.2

Optical properties of birch pollen using a synergy of three lidar instruments 

Maria Filioglou, Ari Leskinen, Ville Vakkari, Minttu Tuononen, Xiaoxia Shang, and Mika Komppula

Pollen has important implications for health, but also for the climate as it can act as cloud condensation nuclei or ice nuclei in cloud processing. Active remote sensing instruments equipped with polarization capability can extend the detection of pollen from the surface up to several kilometres in the atmosphere maintaining continuous and high time resolution operation. In this study, we use a synergy of three lidars, namely, a multi-wavelength PollyXT lidar, a Vaisala CL61 ceilometer and a Halo Photonics StreamLine Doppler lidar, to investigate the optical properties of birch pollen particles. All three lidars are equipped with polarization channels enabling the investigation of the wavelength dependence at 355, 532, 910 and 1565 nm. Together with pollen observations from a Hirst-type spore sampler and aerosol in situ observations, we were able to characterize the linear particle depolarization ratio (PDR) and backscatter-related Angstrom exponents of the pollen particles. Both optical properties have been extensively used in aerosol classification algorithms and they are therefore highly desired in the lidar community. We found that birch pollen exhibits a spectral dependence in the PDR, and its classification is feasible when, preferably, two or more polarization wavelengths are available.

How to cite: Filioglou, M., Leskinen, A., Vakkari, V., Tuononen, M., Shang, X., and Komppula, M.: Optical properties of birch pollen using a synergy of three lidar instruments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1387, https://doi.org/10.5194/egusphere-egu23-1387, 2023.

Ice clouds in the Arctic are expected to have different radiative properties compared to mid latitude cirrus, because of the different humidity and temperature profile and also the prevalent aerosol loading in northern latitudes which govern their formation. During the late winter and early spring 2022 the HALO-(AC)3 campaign was conducted out of Kiruna (Sweden) to probe artic clouds with an airborne remote sensing payload. For this purpose, the German research aircraft HALO was equipped with a water vapor Differential Absorption Lidar (DIAL), a cloud radar, micro-wave radiometers, radiation measurements in the visible, near infrared and thermal region and a drop-sonde dispenser. A total of 25 flights where performed mainly over the sea between Svalbard and Greenland and up to nearly 90°N.

The primary observable to study ice cloud formation is the relative humidity, which is not directly measurable by lidar, but can only be computed with the aid of additional temperature information. By comparison with a large number of dropsondes launched during flight, we will show that the temperature field from ECMWF IFS analyses and short-term forecasts provides sufficient accuracy to retrieve the relative humidity for ice cloud studies. Using this method we will analyse different scenarios of arctic cirrus formation: under stable artic conditions, during a warm air intrusion and while a cold air outbreak. An interesting special case is the modification of cirrus properties by the presence of an aerosol layer which is most probably composed of long range transported Sharan dust. 

How to cite: Wirth, M. and Groß, S.: Characterisation of Arctic Cirrus by Airborne Water Vapor and High Spectral Resolution Lidar, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2024, https://doi.org/10.5194/egusphere-egu23-2024, 2023.

The atmospheric boundary layer is a layer that directly responds to energy emitted or absorbed from the ground into the atmosphere, and is greatly affected by various meteorological factors, which change the concentration of air pollutants. There is generally an inversion layer above the atmospheric boundary layer, so most of the air pollutants emitted by humans cannot escape to the outside of the atmospheric boundary layer and remain there. Ulsan Metropolitan City in Korea is known as the largest industrial city in Korea. These industrial cities generally emit more air pollutants than other cities. Since these air pollutants are greatly affected by the boundary layer, it is important to accurately calculate the height of the boundary layer. In this study, we compare the height of the atmospheric boundary layer based on LiDAR and the height of the atmospheric boundary layer in the Weather Research and Forecasting numerical model, and examine how the height of the atmospheric boundary layer affects the change in the concentration of air pollutants.

How to cite: Choi, K. and Song, C.: Effect of air pollutant concentration according to the height of the Planetary boundary layer in Ulsan, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3042, https://doi.org/10.5194/egusphere-egu23-3042, 2023.

EGU23-3068 | ECS | Posters on site | GI4.2

Improvement of wind vector retrieval method for increasing data acquisition rate of the wind profiler and the wind lidar 

Yujin Kim, Byung Hyuk Kwon, Jiwoo Seo, Geon Myeong Lee, and KyungHun Lee

Representative meteorological instruments that utilize the Doppler effect include Doppler radar, wind profiler, and wind lidar. The latter two instruments produce a vertical profile of winds in high spatio-temporal resolution, in the atmospheric boundary layer. Wind lidar observes with a vertical resolution of 50 m or less and a temporal resolution in minutes, so it fills the observation gap in the lower layer where the wind profiler misses meteorological data. The wind lidar makes the wind vector using DBS (Doppler Beam Swinging) and VAD (Velocity Azimuth Display) methods. It is known that the wind by the VAD method is more accurate than the wind by the DBS method. The DBS method has the advantage of obtaining a wind profile with a fast scan time. On the other hand, there is a restriction that requires at least two beams including vertical beams (one of the east and west beams, and one of the south and north beams), which causes a decrease in the data acquisition rate. The VAD method was improved to produce more wind vector of the wind profiler as well as the wind lidar, which generally uses 5 beams. First, the Fourier series was estimated with the radial velocity by the DBS method. Next, the wind vector was determined by setting the azimuth interval and applying the radial velocity by the Fourier series to the VAD method. The wind vectors were retrieved at the altitude where the wind was not calculated by the DBS method, and the results of the two methods were consistent at the altitude where the wind was calculated by the DBS and the improved VAD method. In this study, we propose a method to increase the data acquisition rate even if the vertical beam or one of the inclined beams is insufficient.

How to cite: Kim, Y., Kwon, B. H., Seo, J., Lee, G. M., and Lee, K.: Improvement of wind vector retrieval method for increasing data acquisition rate of the wind profiler and the wind lidar, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3068, https://doi.org/10.5194/egusphere-egu23-3068, 2023.

EGU23-4339 | Orals | GI4.2

Climatological assessment of the vertically resolved optical aerosol properties by lidar measurements and their influence on radiative budget over the last two decades at UPC Barcelona 

Simone Lolli, Adolfo Comeron, Cristina Gíl-Diaz, Tony Landi, Constantin Munoz-Porcar, Daniel Oliveira, Alejandro Rodriguez-Gomez, Michael Sïcard, Andrés Alastuey, Xavier Querol, and Cristina Reche

In the last two decades, several scientific studies have highlighted the adverse effects, primarily on population health, transportation, and climate, of urban atmospheric particulate due to anthropogenic emissions. For these reasons, aerosols have been monitored through both, remote sensing and in-situ observation platforms, also to establish if the reduction emission policies implemented at the government level have had positive outcomes. In this study, for the first time, we assess how the vertically resolved properties of the atmospheric particulate have changed and consequently their radiative effect during the last twenty years in Barcelona, Spain, one of the largest metropolitan areas of the Mediterranean basin. This study is carried out in the frame of the ACTRIS project through synergy between lidar measurements and the meteorological variables, e.g. wind, temperature, and humidity at the surface. This research, thanks to twenty-year measurements, can shed some light on the meteorological processes and conditions that can lead to haze formation and can help decision-makers to adopt mitigation strategies to preserve large marine Mediterranean metropolitan regions.

How to cite: Lolli, S., Comeron, A., Gíl-Diaz, C., Landi, T., Munoz-Porcar, C., Oliveira, D., Rodriguez-Gomez, A., Sïcard, M., Alastuey, A., Querol, X., and Reche, C.: Climatological assessment of the vertically resolved optical aerosol properties by lidar measurements and their influence on radiative budget over the last two decades at UPC Barcelona, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4339, https://doi.org/10.5194/egusphere-egu23-4339, 2023.

EGU23-5753 | Posters on site | GI4.2

Latent flow measurement by Wind Lidar and Raman Lidar during WaLiNeas campaign 

Donato Summa, Paolo Di Girolamo, Noemi Franco, Ilaria Gandolfi, Marco Di Paolantonio, Marco Rosoldi, Fabio Madonna, Aldo Giunta, and Davide Dionisi

A network of water vapor Raman lidars  WaLiNeas (Lidar Network Assimilation) for improving heavy precipitation forecasting in the Mediterranean Sea has been designed among with the aim of providing water vapor measurements with high spatial-temporal resolution and accuracy, in order to be assimilated into AROME mesoscale models using a four-dimensional ensemble-variational approach with 15-min updates. The CONCERNIG Lidar from University of Basilicata and a Wind Lidar form CNR–IMAA are co-located in the University of Toulone between October 2022 and January 2023 in order to reach the campaign objective. For this scope a of vertical profiles of latent heat flux were obtained  as a  Covariance matrices from vertical wind component (w') and mixing ratio (q') are estimated as a retrieval of a Wind Lidar and Raman Lidar UV respectively.

In this way, a time series of vertical wind profiles from the selected case (31 Oct to 03 Nov) are computed. with temporal resolution Δt = 15 min and vertical resolution Δz = 90 m.  The specific humidity flux < w’ · q’>  [g/kg · m/s] is converted into the flux of latent heat (W/m2) by multiplication with the air density ρ obtained from the radiosonde and the latent heat of vaporization of water Lv. A flux comparison with ground-based water vapour Raman and wind lidar shows agreement within the instruments and the results will be presented during the conference

How to cite: Summa, D., Di Girolamo, P., Franco, N., Gandolfi, I., Di Paolantonio, M., Rosoldi, M., Madonna, F., Giunta, A., and Dionisi, D.: Latent flow measurement by Wind Lidar and Raman Lidar during WaLiNeas campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5753, https://doi.org/10.5194/egusphere-egu23-5753, 2023.

EGU23-7065 | Orals | GI4.2

Nitrous Oxide, N2O: Spectroscopic Investigations for Future Lidar Applications 

Christoph Kiemle, Christian Fruck, and Andreas Fix

Nitrous Oxide, N2O, is the third most important GHG contributing to human-induced global warming, after carbon dioxide and methane. Its growth rate is constantly increasing and its global warming potential is estimated to be 273 times higher than that of CO2 over 100 years. The major anthropogenic source is nitrogen fertilization in croplands. Soil N2O emissions are increasing due to interactions between nitrogen inputs and global warming, constituting an emerging positive N2O-climate feedback. The recent increase in global N2O emissions exceeds even the most pessimistic emission trend scenarios developed by the IPCC, underscoring the urgency of mitigating N2O emissions (Global Carbon Project, 2020). Estimating N2O emissions from agriculture is inherently complex and comes with a high degree of uncertainty, due to variability in weather and soil characteristics, in agricultural management options and in the interaction of field management with environmental variables. Further sources of N2O are processes in the chemical industry and combustion processes. The sink of N2O in the stratosphere increases the NOx concentration which catalytically depletes ozone. Better N2O measurements thus are urgently needed, particularly by means of remote sensing.

Airborne or satellite based N2O lidar remote sensing combines the advantages of high measurement accuracy, large-area coverage and nighttime measurement capability. Past initial feasibility studies revealed that Integrated-Path Differential-Absorption (IPDA) lidar providing vertical column concentrations of N2O would be the method of choice. In this current study we use the latest HITRAN spectroscopic data in order to identify appropriate N2O absorption lines in the wavelength region between 2.9 and 4.6 µm. The infrared spectral region challenges both lidar transmission and detection options. On the transmitter side, the use of optical parametric conversion schemes looks promising, while HgCdTe avalanche photodiode (APD), superconducting nanowire single-photon (SNSPD) or upconversion detectors (UCD) could offer high-efficiency low-noise signal detection. These options are implemented into a lidar simulation model in order to identify the optimal lidar system configuration for measuring N2O from aircraft or satellite using state-of-the-art technology.

How to cite: Kiemle, C., Fruck, C., and Fix, A.: Nitrous Oxide, N2O: Spectroscopic Investigations for Future Lidar Applications, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7065, https://doi.org/10.5194/egusphere-egu23-7065, 2023.

EGU23-7093 | ECS | Orals | GI4.2

Ceilometer aerosol retrieval and comparison with in-situ tower-measurements 

Marcus Müller, Ulrich Löhnert, and Birger Bohn

In recent years there is a growing interest in real-time aerosol profiling and in this context, the use of automated lidars and ceilometers (ALC) for aerosol remote sensing increased. Ceilometers were originally developed to measure cloud-base height automatically. Apart from this, they also provide vertically resolved backscatter information. Several algorithms have been developed to calibrate this signal and to derive aerosol concentration from it, bringing up new opportunities in air quality monitoring and boundary layer research.

The quality of ALCs is often evaluated by comparing the attenuated backscatter to measurements from high-power lidars. This approach is suitable to validate the backscatter signal. However, for the validation of the aerosol concentration, a direct comparison with an in-situ, optical aerosol measurement is more significant.

In this work, a comparison study was performed using the Jülich Observatory for Cloud Evolution. Data were processed and calibrated with algorithms by E-Profile (https://www.eumetnet.eu/activities/observations-programme/current-activities/e-profile/alc-network/). The aerosol retrieval was performed using a Klett inversion algorithm. Close to the JOYCE site a 120 m meteorological tower is located. This tower was used as a platform for the in-situ aerosol measurement, where an optical particle sizer was mounted 100 m above the ceilometer position.

We will show the setup and data processing of the in-situ measurements as well as an approach how ceilometer raw data can be processed, calibrated and used to retrieve aerosol concentration. First results of the comparison will be presented to evaluate the quality of ALC aerosol-measurement.

How to cite: Müller, M., Löhnert, U., and Bohn, B.: Ceilometer aerosol retrieval and comparison with in-situ tower-measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7093, https://doi.org/10.5194/egusphere-egu23-7093, 2023.

EGU23-7775 | Posters on site | GI4.2

Several months of continuous operation of two thermodynamic Raman lidars in the frame of WaLiNeAs 

Paolo Di Girolamo, Noemi Franco, Marco Di Paolantonio, Donato Summa, Davide Dionisi, Annalisa Di Bernardino, Anna Maria Iannarelli, and Tatiana Di Iorio

The University of Basilicata, in cooperation with ISMAR-CNR, deployed two compact Raman lidars, namely the system CONCERNING and the system MARCO, in Southern France in the frame of the “Water Vapor Lidar Network Assimilation (WaLiNeAs)” experiment. WaLiNeAs, primarily funded by the “French National Research Agency” (ANR), is an international field experiment aimed at studying extreme precipitation events and improving their predictability through the assimilation of water vapour profile measurements from a network of Raman lidar systems into mesoscale numerical models. The experiment has a specific geographical focus on Southern France. The measurement strategy implies the exploitation of seven Raman lidars along the Mediterranean coasts of Spain and France, capable to provide real-time measurements of water vapour mixing ratio profiles over a three-month period starting on October 1st, 2022.

CONCERNING (COmpact RamaN lidar for Atmospheric CO2 and ThERmodyNamic ProfilING), developed in the frame of a cooperation between University of Basilicata, ISMAR-CNR and University of Rome, is a compact and transportable Raman lidar system designed for long-term all-weather continuous operation, capable to perform high-resolution and accurate carbon dioxide and water vapour mixing ratio profile measurements, together with temperature and multi-wavelength (355, 532 and 1064 nm) particle backscattering/extinction/depolarization profile measurements. The system relies on a 45-cm diameter Newtonian telescope and on a diode-pumped Nd:Yag laser source, capable of emitting pulses at the three traditional wavelengths of this laser source(355, 532 and 1064 nm), with a single pulse energy at 355 nm of 110 mJ and an average emitted power of 11 watts, based on a pulse repetition frequency of 100 Hz.

MARCO (Micropulse Atmospheric Optical Radar for Climate Observations) is also a compact and easily transportable Raman lidar system, developed around a high- frequency laser source (20 kHz), capable to perform 24/7 high-resolution and accurate CO2 and water vapour mixing ratio profile measurements, together with temperature and single-wavelength (355 nm) particle backscattering/extinction/depolarization measurements. In the frame of WaLiNeAs, as a result of the restrictions imposed by air traffic authority in the use of the visible and infrared laser radiation, only the 355 wavelength was exploited in CONCERNING, the temperature channel was not available in MARCO, while the CO2 channels, not needed for the purposes of WaLiNeAs, were temporarily deactivated in both systems.

Both systems have been recently designed and developed and WaLiNeAs represents the first international field deployment for both. CONCERNING was deployed at the University of Toulon in La Garde (Lat.: 43.136040 N, Long.: 6.011650 E, Elev.: 65 m, with continuous measurements since 29 September 2022, i.e. over more than 100 days up to now), while MARCO, was deployed at the Direction de Services Techniques in Port-Saint-Louis-du-Rhône, Camargue (Lat.: 43.392570 N, Long.: 4.813480 E, Elev.: 5 m, with continuous measurements since 19 October 2022, i.e. over more than 80 days up to now). At the time of the submission of this abstract, both system are still operational with a tbc date for the stop of the operation of 31 January 2023. Preliminary results from these two systems will be illustrated and discussed during the Conference.

How to cite: Di Girolamo, P., Franco, N., Di Paolantonio, M., Summa, D., Dionisi, D., Di Bernardino, A., Iannarelli, A. M., and Di Iorio, T.: Several months of continuous operation of two thermodynamic Raman lidars in the frame of WaLiNeAs, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7775, https://doi.org/10.5194/egusphere-egu23-7775, 2023.

EGU23-8014 | ECS | Posters on site | GI4.2

A compact general-purpose Doppler Lidar for lidar networks 

Jan Froh, Josef Höffner, Alsu Mauer, Thorben Mense, Ronald Eixmann, Gerd Baumgarten, Franz-Josef Lübken, Alexander Munk, Sarah Scheuer, Michael Strotkamp, and Bernd Jungbluth

We present the state of the VAHCOLI (Vertical and Horizontal COverage by Lidar) project for investigating small- to large-scale processes in the atmosphere. In the future, an array of compact lidars with multiple fields of view will allow for measurements of temperatures, winds and aerosols with high temporal and vertical resolution.

Doppler lidars, in particular resonance Doppler lidars, with daylight capability are challenging systems because of the small field of view, spectral filtering and other additional subsystems required compared to observations at night. We developed a universal Doppler lidar platform (~1m3, ~500kg) with all required technologies for automatic operation. The system is capable of studying Mie scattering (aerosols), Rayleigh scattering (air molecules), and resonance fluorescence on free potassium atoms in the middle atmosphere from 5 km to 100 km. Unique spectral methods and narrowband optical components allow precise wind, temperature, and aerosol measurements by studying the Doppler shift and broadening of the scattered signals. The combination of cost-efficient design and fast assembling of such a system allows the construction of a Doppler lidar network with identical units

We will show the latest results and discuss the next scientific and technical steps for network operation and transferring the technology into industry.

How to cite: Froh, J., Höffner, J., Mauer, A., Mense, T., Eixmann, R., Baumgarten, G., Lübken, F.-J., Munk, A., Scheuer, S., Strotkamp, M., and Jungbluth, B.: A compact general-purpose Doppler Lidar for lidar networks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8014, https://doi.org/10.5194/egusphere-egu23-8014, 2023.

EGU23-8149 | ECS | Orals | GI4.2

Water vapor retrieval from mini Raman lidar HORUS in the framework of the WaLiNeAs campaign 

Frédéric Laly, Patrick Chazette, Julien Totems, and Jérémy Lagarrigue

The Mediterranean Rim, and more particularly the western Mediterranean area, is one of the most sensitive regions to climate change. The associated environmental changes are already evident through periods of drought and intense rainfall. The predictions of these phenomena are a major societal issue, which led us to use lidar systems to constrain regional modelling. The Raman lidars HORUS-1 and -2 are each composed of two telescopes of 15 cm diameter.  For each telescope N2 and H2O channels are associated. Lidars components have been specifically defined for this task and put into operation during the international Water vapor Lidar Network Assimilation (WaLiNeAs) campaign led by French research teams. Among the three stations managed by the LSCE team, two of them were equipped with HORUS lidar systems at the Port Camargue (43.52 N 4.13 E) and Coursan (43.23 N 3.06 E) sites. The main difference between the two HORUS lidars is the laser used. For HORUS-1 we used an ULTRA laser (optimally pumped by a flash lamp at 30 mJ/20Hz) which showed a good reliability since the beginning of the lidar installation. However, the MERION-C laser (optimally pumped by diodes at 30 mJ/100 Hz) installed in HORUS-2 did not live up to our expectations with several failures, to the point of stopping the measurements in Coursan. We will nevertheless discuss the relative interest of these two lasers in projection of future Raman lidar networks. Observations available from these two lidar systems will be presented and discussed with respect to the meteorological processes encountered during their operating periods.

We give a special acknowledgment to the ANR grant #ANR-20-CE04-0001 for the contribution to the WaLiNeAs program and a special acknowledgment to Meteo France and to the CNRS INSU national LEFE program for their financial contribution for this project. The CEA is acknowledged for the provision of its staff and facilities.

How to cite: Laly, F., Chazette, P., Totems, J., and Lagarrigue, J.: Water vapor retrieval from mini Raman lidar HORUS in the framework of the WaLiNeAs campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8149, https://doi.org/10.5194/egusphere-egu23-8149, 2023.

Since there are only a very few suitable remote sensing measurements, the thermodynamic field of the atmospheric boundary layer and lower free troposphere is largely still Terra Incognita. To close this gap, we developed an automated thermodynamic profiler based on the Raman lidar technique, the Atmospheric Raman Temperature and Humidity Sounder (ARTHUS) (Lange et al. 2019).

It uses only the ice-safe 355-nm radiation of an injection-seeded Nd:YAG laser as transmitter. The laser power is about 20 W at 200 Hz. The diameter of the receiving telescope is 40 cm. Four receiving channels (elastic, water vapor, two rotational Raman signals) allow for four independently measured parameters: temperature (T), water vapor mixing ratio (WVMR), particle extinction coefficient, and particle backscatter coefficient.

With these data, ARTHUS resolves, e.g., the strength of the inversion layer at the atmospheric boundary layer (ABL) top, elevated lids in the free troposphere, and turbulent fluctuations. Furthermore, in combination with Doppler lidars, sensible and latent heat flux profiles in the convective ABL and thus flux-gradient relationships can be studied (Behrendt et al. 2020). Consequently, ARTHUS can be applied for process studies of land-atmosphere feedback, weather and climate monitoring, model verification, and data assimilation.

Resolutions of the measurements are a few seconds and meters in the lower troposphere. With the data, also the statistical uncertainties of the measured parameters are derived. Continuous operations over long periods were achieved not only at the Land Atmosphere Feedback Observatory (LAFO) at University of Hohenheim but also during several field campaigns elsewhere covering a large variety of atmospheric conditions.

During the EUREC4A field campaign (Stevens et al, 2020), ARTHUS was deployed onboard the research vessel Maria S Merian between 18 January and 18 February 2020 to study ocean-atmosphere interaction. Here, ARTHUS was collocated with two Doppler lidars: one in vertically pointing mode and one in a 6-beam scanning mode.

Between 15 July and 20 September 2021, ARTHUS was deployed at the Lindenberg Observatory of the German Weather Service (DWD). The objective of the campaign was to investigate the long-term stability of ARTHUS by comparisons with four local radiosondes. Indeed, the very high accuracy during day and night were verified.

ARTHUS participated in WaLiNeAs (Water Vapor Lidar Network Assimilation) between 15 September and 10 December 2022. For this campaign, ARTHUS was deployed at the west coast of Corsica. The objective was to implement an integrated prediction tool to enhance the forecast of heavy precipitation events in southern France, primarily demonstrating the benefit of assimilating vertically resolved WVMR lidar data in the new version of the French operational AROME numerical weather prediction system.

At the conference, highlights of ARTHUS’ measurements during WaLiNeAs will be shown.

References:

Behrendt et al. 2020, https://doi.org/10.5194/amt-13-3221-2020

Lange et al. 2019, https://doi.org/10.1029/2019GL085774

Stevens et. al. 2021, https://doi.org/10.5194/essd-2021-18

How to cite: Lange, D., Behrendt, A., and Wulfmeyer, V.: The Atmospheric Raman Temperature and Humidity Sounder: Highlights of Four Years of Automated Measurements of the Atmospheric Boundary Layer and Free Troposphere, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10606, https://doi.org/10.5194/egusphere-egu23-10606, 2023.

The increasing atmospheric carbon dioxide (CO2) is the most important factor forcing climate change. However, due to lack of observation data about large-scale range-resolved CO2, there remains substantial uncertainty in current global atmospheric CO2 budget, which hinders giving insight into CO2 cycle and modeling its forcing to climate change. Space-based range-resolved differential absorption lidar (range-resolved DIAL), is a promising and powerful means for obtaining large-scale range-resolved CO2 data, but has been rarely studied. Prior to developing spaceborne range-resolved DIAL, a preliminary study on optimization of on/off-line wavelengths must be performed to ensure high signal-to-noise (SNR), high sensitivity to near surface region and minimize the interference of atmospheric factors. This study aims to find the optimum wavelength scenarios in terms of random errors determined by SNR, weighting functions used to assess sensitivity to near-surface region, and systematic errors affected by atmospheric factors. Firstly, we find the optimal on/off-line wavelengths at 1.57μm and 2.05μm, which are widely used and show good results for measuring CO2 concentration, after estimating on-line and off-line wavenumbers separately using evaluation indexes called  and . Furthermore, we get the optimum wavelength scenarios of spaceborne range-resolved DIAL by comparing the random, systematic errors and weighting functions of optimal on-line and off-line wavelengths at 1.57μm and 2.05μm. Results show that the wavelength scenario at 2.05μm is the optimal for spaceborne range-resolved CO2 detection. To satisfy the requirement that the relative random errors are smaller than 0.01 (<1%), systems at 2.05μm wavelength scenario with vertical resolution of 0.5 km, 0.7 km, 0.8 km, 0.9 km separately require that SNR values of on-line wavelength at 0 km height are larger than 10, 9, 8, 7.

How to cite: Hu, L., Yu, Z., Huang, Y., and Ma, R.: Performance Simulation of Spaceborne Range-resolved Differential Absorption Lidar System For CO2 Profile Detection At 1.57μm and 2.05μm Wavelength Scenarios, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11104, https://doi.org/10.5194/egusphere-egu23-11104, 2023.

Cirrus clouds, forming in the cold upper troposphere, are composed of ice crystals with various sizes and nonspherical shapes. They are observed at all latitudes covering over 30% of the Earth’s surface. Studies reveal that they have a significant impact on the radiation balance of our planet and, consequently, on the climate evolution. The radiative effect of cirrus clouds is strongly determined by the cloud microphysical, thermal, and optical properties. Furthermore, global aviation affects the Earth’s radiation balance by inducing contrails and exerting an indirect effect on the microphysical properties of naturally-formed cirrus clouds. In the last decades, the Arctic surface has been warming faster than other regions of the globe, which is known as Arctic Amplification. The thin and small-coverage cirrus clouds over the Arctic are presumed to largely contribute to it. Unfortunately, however, the optical and microphysical properties of cirrus clouds over the Arctic and the exact role they play in the elevated warming of the Arctic are far from understanding. Compared with the intensive studies of cirrus clouds in the tropics and midlatitude regions, cirrus cloud measurements and model studies at high latitudes are sparse. In this study, we present the comparisons of the particle linear depolarization ratio (PLDR) and occurrence rates of cirrus clouds at midlatitudes (35–60 oN; 30 oW–30 oE) and high latitudes (60–80 oN; 30 oW–30 oE) based on the analysis of lidar measurements of CALIPSO in the years 2018–2021. The results show that cirrus clouds at high latitudes appear at lower altitudes than the midlatitude cirrus clouds. The PLDR and occurrence rates of cirrus clouds at high latitudes are smaller than the midlatitude cirrus clouds. Furthermore, air traffic over Europe was significantly reduced in 2020 (starting from March) and only moderately reduced in 2021 due to the COVID-19 pandemic. Under this condition we are able to study the difference in the aviation impacts on the cirrus cloud properties at high latitudes and midlatitudes.

How to cite: Li, Q. and Groß, S.: CALIPSO observations of cirrus cloud properties: investigation of latitude differences and possible aviation impacts, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11893, https://doi.org/10.5194/egusphere-egu23-11893, 2023.

EGU23-12585 | Posters on site | GI4.2

Investigation of 2021 summer wildfires in the Eastern Mediterranean: The ERATOSTHENES Centre of Excellence capabilities for atmospheric studies 

Rodanthi-Elisavet Mamouri, Dragos Ene, Holger Baars, Ronny Engelmann, Argyro Nisantzi, Maria Prodromou, Diofantos Hadjimitsis, and Albert Ansmann

In the summer of 2021, several wildfires were reported in the south of Turkey, fires that are considered one of the worst in the history of Turkey. Due to atmospheric conditions, the smoke plume travelled south between 27 July to 5 August 2021, and smoke layers arrived above Cyprus. 

In this work, the capabilities of the newly established ERATOSTHENES Centre of Excellence (CoE), to study large-scale atmospheric events is presented. The study is based on the synergistic use of different datasets of remote sensing techniques both from ground and space. The EARLINET multiwavelength-Raman-polarization lidar PollyXT-CYP hosted by the ERATOSTHENES CoE is continuously running since October 2020 in Limassol, and during summer 2021, the lidar observed smoke plumes from these extreme wildfires on the south coast of Turkey.  

The PollyXT-CYP is a key research infrastructure of the Cyprus Atmospheric Remote Sensing Observatory (CARO) of the ERATOSTHENES CoE established through the EXCELSIOR H2020 EU Teaming project coordinated by the Cyprus University of Technology. CARO will consist of two high-tech containers housing the PollyXT-CYP lidar and state-of-the art doppler lidar, cloud radar and radiometric equipment which will be used to measure the air quality, the dust transport, and the cloud properties over Cyprus. The CARO is a planning National Facility of the Republic of Cyprus for Aerosol and Cloud Remote Sensing Observations.

Land cover information which shows the type of burned vegetation is used together with satellite products to capture additionally the burned area and to investigate the carbon monoxide of the smoke plume. The study is focusing on the optical characteristics of the plume, as it was detected by the PollyXT-CYP lidar at Limassol. An intense fresh smoke layer was detected on 28-29 July 2021, at an altitude between 2.5 to 4.0 km, having a volume depolarization ratio of ~15% at 355n and ~20% at 532nm, and lidar ratio of 75-80sr at 355nm and 65-70sr at 532nm.

 

Acknowledgements

The authors acknowledge the ‘EXCELSIOR’: ERATOSTHENES: EΧcellence Research Centre for Earth Surveillance and Space-Based Monitoring of the Environment H2020 Widespread Teaming project (www.excelsior2020.eu). The ‘EXCELSIOR’ project has received funding from the European Union’s Horizon 2020 research and innovation programme under Grant Agreement No 857510, from the Government of the Republic of Cyprus through the Directorate General for the European Programmes, Coordination and Development and the Cyprus University of Technology. The PollyXT-CYP was funded by the German Federal Ministry of Education and Research (BMBF) via the PoLiCyTa project (grant no. 01LK1603A). The study is supported by “ACCEPT” project (Prot. No: LOCALDEV-0008) co-financed by the Financial Mechanism of Norway (85%) and the Republic of Cyprus (15%) in the framework of the programming period 2014 - 2021.

How to cite: Mamouri, R.-E., Ene, D., Baars, H., Engelmann, R., Nisantzi, A., Prodromou, M., Hadjimitsis, D., and Ansmann, A.: Investigation of 2021 summer wildfires in the Eastern Mediterranean: The ERATOSTHENES Centre of Excellence capabilities for atmospheric studies, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12585, https://doi.org/10.5194/egusphere-egu23-12585, 2023.

A newly available Raman lidar (Purple Pulse Lidar Systems) for vertical profiling of atmospheric water vapor, temperature and aerosols was evaluated during the TEAMx pre-campaign (TEAMx-PC22) in summer 2022 in the Inn Valley (Austria). TEAMx (Multi-scale transport and exchange processes in the atmosphere over mountains – programme and experiment) is an international research program addressing exchange processes in the atmosphere over mountains and their parametrization in numerical weather models and climate models. Prior to the multi disciplinary measurement campaign, planned in 2024/2025, the pre-campaign 2022 was rather performed for testing (new) instruments and measurement sites and finding synergies between certain devices.

The Raman lidar system is capable of profiling water vapor and temperature throughout the entire planetary boundary layer (typically 3 km to 4 km agl. on summer days) continuously with a basic temporal resolution of 10 s and a reasonable vertical resolution of 30 m to 100 m. Depending on conditions and temporal averaging, water vapor profiles could even be obtained up to ~7.5 km agl. during nighttime. The lidar system was located at the University of Innsbruck (downtown). It was operated side by side with a vertically staring Doppler wind lidar and a nearby (50 m) scanning Doppler wind lidar on the rooftop of the university building, which provide vertical profiles of the vertical wind component at a 1-s interval and vertical profiles of the three-dimensional wind vector at a 10-min interval, respectively. During the measurement period (Aug 2022 to Sep 2022), operational radiosondes were launched in close proximity, at Innsbruck Airport, roughly 3 km to the west of the lidar site. In addition to the daily ascent at 2 UTC, radiosondes were launched at about 8, 14 and 20 UTC on selected days with potentially complex meteorological conditions. We present a first assessment of the Raman lidar measurements through comparisons with the radiosonde data. Together with data from the wind lidars, we also present an interpretation for significant meteorological situations and events, such as foehn, a passing front, a thunderstorm and the formation of a convective boundary layer during a warm period.

How to cite: Vogelmann, H., Federer, M., Speidel, J., and Gohm, A.: Assessing the performance of a Combined Water Vapor / Temperature / Aerosol Raman Lidar within the TEAMx pre-campaign in the Inn Valley (Innsbruck, Austria) during Summer 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13101, https://doi.org/10.5194/egusphere-egu23-13101, 2023.

EGU23-13218 | ECS | Orals | GI4.2

ARC and ATLAS: CARS software tools for the data analysis and quality assurance of lidar measurements performed within ACTRIS 

Nikolaos Siomos, Ioannis Binietoglou, Peristera Paschou, Mariana Adam, Giuseppe D'Amico, Benedikt Gast, Moritz Haarig, and Volker Freudenthaler

We present newly developed software for the data analysis and quality assurance of lidar systems operated in the ACTRIS (Aerosol Clouds and Trace Gases Research Infrastructure) research infrastructure. The software development is coordinated by the Meteorological Institute of Munich (MIM), which operates as one of the central facilities of the Center of Aerosol Remote Sensing (CARS) of ACTRIS. In the frame of ACTRIS, a large number of national facilities (NF) are operating lidar systems for aerosol remote sensing. In order to ensure homogeneously high data quality, CARS is developing appropriate common software tools to assist data processing, system intercomparison, and routine quality assurance of lidar data. Here, we present two such software tools, developed and tested using the long experience of the EARLINET (European Aerosol Research Lidar Network) community.

The ARC (Algorithm for Rayleigh Calculations) has been designed to calculate the cross-section and depolarization ratio of molecular back-scattering. The effect of Rotational Raman (RR) scattering is included line-by-line in ARC considering especially the partial blocking of the RR spectrum due to transmission through narrow-band interference filters. The algorithm supports calculation in variable meteorological conditions for an atmosphere that consists of up to five major gas components (N2, O2, CO2, Ar, H2O). Such a tool is needed in order to properly take into account the effect of air temperature in the molecular depolarization ratio measured by the NF lidar systems. It is also crucial for designing lidars that rely on RR scattering such as temperature and RR aerosol lidars and can even be applied for the algorithmic correction of unwanted effects introduced by the interference filter in such systems.

The second software package developed by CARS-MIM is ATLAS (AuTomated Lidar Analysis Software). It has been designed for the operational analysis of the quality assurance tests that should be regularly performed and submitted to CARS by the NF for the ACTRIS labeling process. ATLAS currently supports the analysis of all main CARS test procedures, that is, the Rayleigh fit, the Telecover, and the Polarization Calibration. It can also be used to directly compare signals from two lidar systems; It has already been applied in the first intercomparison campaign of CARS reference systems, organized in September 2022 in Magurele, Romania. The software takes raw lidar data as input so the user can detect otherwise-hidden issues in the preprocessing steps. At the time of writing, ATLAS is compatible with all ACTRIS lidar systems. Future updates will include automated syncing of the system metadata from the handbook of instruments of the network, currently hosted by the Single Calculus Chain (SCC), and a graphical user interface that will facilitate its adoption by the NF users. Both software packages are written in python and are open-source projects.

How to cite: Siomos, N., Binietoglou, I., Paschou, P., Adam, M., D'Amico, G., Gast, B., Haarig, M., and Freudenthaler, V.: ARC and ATLAS: CARS software tools for the data analysis and quality assurance of lidar measurements performed within ACTRIS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13218, https://doi.org/10.5194/egusphere-egu23-13218, 2023.

EGU23-13416 | Orals | GI4.2

Merging clouds retrieved from ALADIN/Aeolus and CALIOP/CALIPSO spaceborne lidars 

Artem Feofilov, Hélène Chepfer, and Vincent Noël

Clouds play an important role for the energy budget of Earth. But, when it comes to predicting the climate's future, their behavior in response to climate change is a major source of uncertainty. To understand and accurately predict the Earth's energy budget and climate, it is necessary to have a thorough understanding of the cloud variability, including their vertical distribution and optical properties.

Satellite observations have been able to provide ongoing monitoring of clouds all around the globe. Among them, active sounders hold a special place thanks to their capability of measuring the vertical position of the cloud with an accuracy of about 100 meters and with a typical horizontal sampling on the order of hundreds of meters. However, clouds retrieved from two spaceborne lidars are different, because the instruments use different wavelengths, pulse energies, pulse repetition frequencies, telescopes, and detectors. In addition, they do not overpass the atmosphere at the same local time.

In this work, we discuss the approach to merging the clouds retrieved from the space-borne lidar ALADIN/Aeolus, which has been orbiting the Earth since August 2018 and operating at 355nm wavelength with the clouds measured since 2006 by CALIPSO lidar, which operates at 532nm.

We demonstrate how to compensate for the existing instrumental differences to get an almost comparable cloud dataset and we discuss the importance of the aforementioned differences between the instruments. The method developed in this study sets the path for adding future lidars (e.g. ATLID/EarthCare) to the global climate lidar cloud record.

How to cite: Feofilov, A., Chepfer, H., and Noël, V.: Merging clouds retrieved from ALADIN/Aeolus and CALIOP/CALIPSO spaceborne lidars, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13416, https://doi.org/10.5194/egusphere-egu23-13416, 2023.

EGU23-13419 | ECS | Orals | GI4.2

Columnar heating rate and  radiative effects of dust aerosols using 20 years of lidar observations. 

Benedetto De Rosa, Lucia Mona, Simone Lolli, Aldo Amodeo, and Michalis Mytilinaios

The uncertainties of the Earth-atmosphere energy budget are associated with a poor understanding of direct and indirect aerosol effects. Dust is a mixture of different minerals, and its chemical and microphysical properties change during transport. Therefore, the influence of dust aerosols on radiative effects is characterized by great uncertainty. Due to meteorological atmospheric patterns, aerosol intrusions are very frequent in the Mediterranean, which is a climatic hot spot and where climate change is much stronger than in other parts of the world. In this study, we analyzed and assessed long-term trends of the surface and columnar heating rate and the radiative effects of dust aerosols using lidar observations. These measurements were taken in the framework of the European Aerosol Research Lidar Network (EARLINET) at Istituto di Metodologie per l'Analisi Ambientale (IMAA) with the Raman/elastic lidar MUSA (40°36′N, 15°44′E). The radiative transfer model Fu–Liou–Gu (FLG) was used to solve aerosol (no clouds) radiative fluxes, with aerosol extinction coefficient profiles from lidar observations as input data. All the cases of dust intrusion that occurred in the last twenty years were selected to understand how they affected the Earth-atmosphere radiative budget, both at the surface and at the top-of-the-atmosphere. In the future, these studies will be important for improving the accuracy of climate predictions.

How to cite: De Rosa, B., Mona, L., Lolli, S., Amodeo, A., and Mytilinaios, M.: Columnar heating rate and  radiative effects of dust aerosols using 20 years of lidar observations., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13419, https://doi.org/10.5194/egusphere-egu23-13419, 2023.

EGU23-13643 | ECS | Orals | GI4.2

Is your aerosol backscatter retrieval afflicted by a sign error? 

Johannes Speidel and Hannes Vogelmann

Precise knowledge about the prevailing aerosol content in the atmosphere is very important for several reasons, as aerosols are involved in multiple important processes that not only have a direct impact on air quality, but also influence cloud formation and the earth's radiation budget. Besides that, continuous aerosol observations provide valuable information on atmospheric transport dynamics.
Aerosol backscatter coefficient measurements with elastic backscatter lidars are conducted since multiple decades [1], while the implemented retrieval algorithms predominantly refer to the seminal publications by Klett 1985, Fernald 1984 and Sasano 1985 [2,3,4]. The respective inversion algorithm is often simply called the 'Klett inversion', being a main reason why this algorithm is most often adapted. While more sophisticated aerosol lidars (e.g. Raman lidars, HSRL, ...) have been developed since, simple elastic backscatter lidar measurements are still very frequently conducted as they are technically easy to implement, often as a byproduct. In most cases, the corresponding retrieval algorithms still refer to the 'Klett inversion'.
Unfortunately, the inversion algorithm by Klett 1985 is afflicted by a sign error. In his publication, the sign error is hidden within a substitute, making it very hard to be recognized, representing a major pitfall. A comprehensive literature review revealed, that large parts of the aerosol lidar community are aware of this problem and have tacitly corrected it or, to a much smaller amount, even referred to an erratum which was published by Kaestner in 1986 [5].
However, at the same time and up to this date, a considerable error propagation can be found in literature as well, using and referring to the incorrect algorithm with the sign error included.
Therefore, we want to renew the awareness towards this sign error and show a corrected and slightly improved Klett inversion algorithm. In addition, we present the overall implication resulting from the uncorrected inversion algorithm by using exemplary case studies. Depending on the lidar location and prevailing atmospheric conditions, potential errors reach from marginal to major, often preventing error detection solely based on the magnitude of the calculated results. Simple a posteriori corrections are not possible, as the error magnitude depends on multiple factors.

[1] T. Trickl, H. Giehl, H. Jäger, and H. Vogelmann. 35 yr of stratospheric aerosol measurements at Garmisch-Partenkirchen: From Fuego to Eyjafjalla-   jökull, and beyond. Atmospheric Chemistry and Physics, 13(10):5205–5225, 2013.
[2] James D. Klett. Lidar inversion with variable backscatter/extinction ratios. Appl. Opt., 24(11):1638–1643, June 1985.
[3] Frederick G. Fernald. Analysis of atmospheric lidar observations: Some comments. Appl. Opt., 1984.
[4] Yasuhiro Sasano, Edward V. Browell, and Syed Ismail. Error caused by using a constant extinction/backscattering ratio in the lidar solution. Appl. Opt., 24(22):3929–3932, November 1985.
[5] Martina Kaestner. Lidar inversion with variable backscatter/extinction ratios: Comment. Applied Optics, 25(6):833–835, March 1986.

How to cite: Speidel, J. and Vogelmann, H.: Is your aerosol backscatter retrieval afflicted by a sign error?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13643, https://doi.org/10.5194/egusphere-egu23-13643, 2023.

EGU23-13823 | ECS | Posters on site | GI4.2

Development of a Carbon Dioxide Raman Lidar 

Moritz Schumacher, Andreas Behrendt, Diego Lange, and Volker Wulfmeyer

Carbon dioxide (CO2) is one of the most important greenhouse gases and therefore its detailed measurement is of high interest. As the concentration varies significantly with altitude and time, it is desirable to be able to measure vertical CO2 profiles with high temporal resolution. Profiles of high resolution will improve our understanding of atmospheric systems and the impact of the local environment, e.g., due to natural and anthropogenic sources and sinks. The use of these data in data assimilation provides the potential of improving climate models.

For water vapor and temperature the Atmospheric Raman Temperature and Humidity Sounder (ARTHUS) system has proven to be able to provide profiles with high resolution (10-60 s in time and 7.5-100 m vertically) and accuracy in the lower troposphere. Now this successful system will be expanded with a CO2 Raman channel, which is currently in development. After successful integration it will be possible to simultaneously measure CO2, water vapor and temperature profiles. Challenges are the weak signal of the backscattered light due to the low concentration and the small Raman backscatter cross section of CO2.

Further information on the CO2 Raman lidar will be given at the conference.

How to cite: Schumacher, M., Behrendt, A., Lange, D., and Wulfmeyer, V.: Development of a Carbon Dioxide Raman Lidar, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13823, https://doi.org/10.5194/egusphere-egu23-13823, 2023.

Extreme heavy precipitation events (HPEs) pose a threat to human life but, despite regular improvement, remain difficult to predict because of the lack of adequate high frequency and high-resolution water vapor (WV) observations in the low troposphere (below 3 km). To fill this observational gap, The Water vapor Lidar Network Assimilation (WaLiNeAs) initiative aims at implementing an integrated prediction tool (IPT), coupling network measurements of WV profiles, and a numerical weather prediction system to try to improve the  forecasts of  the amount, timing, and location of rainfall associated with HPEs in southern France (struck by ~ 7 HPEs per year on average during the fall).

In the fall/winter of 2022-2023, a network of 6 mobile Raman WV lidars was specifically implemented in Southern France (Aude, Gard, Var and Bouche du Rhone) and in Corsica. The network was complemented by 2 fixed Raman WV lidars in Barcelona and Valencia with the aim to provide measurements with high vertical resolution and accuracy to be assimilated in the French Application of Research to Operations at Mesoscale (AROME-France) model, using a four-dimensional ensemble-variational approach with 15-min updates in addition to the observations operationally assimilated (radar, satellites, …). This innovative IPT is expected to enhance the model capability for kilometer-scale prediction of HPEs over southern France up to 48 h in advance.

The field campaign was conducted from October of 2022 to January 2023, to cover the period most propitious to heavy precipitation events in southern France. A consortium of French, German, Italian, and Spanish research groups operated the Raman WV lidar network

In this presentation, we will provide an overview of the precipitation events in southern France during the WaLiNeAs campaign, as well as an outline of the operations period of the different Raman WV lidars and the lidar data monitoring procedure implemented during the experiment. We will highlight the cases of interest and provide an outlook at next steps towards lidar data assimilation in AROME.

How to cite: Flamant, C. and the WaLiNeAs Team: A network of water vapor Raman lidars for improving heavy precipitation forecasting in southern France: introducing the WaLiNeAs initiative and first highlights from the 2022 field campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14747, https://doi.org/10.5194/egusphere-egu23-14747, 2023.

Each year, during both boreal winter and summer, large amounts of Saharan mineral dust particles get carried westwards over the Atlantic Ocean towards the Caribbean. During their transport, Saharan dust particles can affect the Earth’s radiation budget in different ways. They can either directly scatter, absorb and emit radiation or have an indirect effect by modifying cloud properties through their interactions as cloud condensation nuclei or ice nucleating particles. While during the summer months – the peak season of transatlantic mineral dust transport – the particles are mostly advected in elevated Saharan Air Layers at altitudes of up to 6 km and at latitudes around 15°N, wintertime transport takes place at lower atmospheric levels (<3 km altitude) and lower latitudes. Our recent studies have shown that, during both boreal winter and summer, transported Saharan dust layers are characterized by enhanced concentrations of water vapor compared to the surrounding atmosphere. In this way the dust layers have to potential to modify the radiation budget not only through particle-radiation-interactions, but also through the absorption and emission of radiation by water vapor. This in turn may affect the atmospheric stability and stratification in and around the aerosol layers.

In this study, the turbulent structure as well as the atmospheric stability in and around transported Saharan mineral dust is analyzed and possible differences between summer and wintertime are investigated. Therefore, measurements by both the water vapor and aerosol lidar WALES as well as by dropsondes are studied. They were collected upstream the Caribbean island of Barbados aboard the German research aircraft HALO (High Altitude and Long Range). To identify possible seasonal differences, not only data collected in boreal summer in the framework of the NARVAL-II campaign (August 2016), but also data collected in winter during the EUREC4A research campaign (January & February 2020) are analyzed. During both campaigns several research flights were designed to lead over long-range-transported Saharan mineral dust, thus allowing and in-depth investigation of their properties. The analysis shows that dust layers are highly turbulent and therefore help dust particles to stay airborne for a longer time. Additionally, the dust layers modify the atmospheric stability in a way that the evolution of marine clouds can be affected.

In our presentation, we will give an overview of the performed measurements over long-range-transported Saharan dust layers and present the conducted analyses on atmospheric stability and turbulence from dropsonde measurements and calculated power spectra from lidar data.

How to cite: Gutleben, M. and Groß, S.: Atmospheric turbulence and stability in and around long-range-transported Saharan dust layers as observed by airborne lidar and dropsondes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15538, https://doi.org/10.5194/egusphere-egu23-15538, 2023.

EGU23-15605 | Posters on site | GI4.2

How good are temperature and humidity measurements with lidar? 

Andreas Behrendt, Diego Lange, and Volker Wulfmeyer

In this contribution, we will discuss the performance of state-of-the-art automatic temperature and humidity lidar (e.g., Wulfmeyer and Behrendt 2022). As example, we will investigate ARTHUS (Lange et al., 2019), a lidar system developed at University of Hohenheim. This automatic mobile instrument participated in recent years in a number of field campaigns.

ARTHUS technical configuration is the following: A strong diode-pumped Nd:YAG laser is used as transmitter. It produces 200 Hz laser pulses with up to 20 W average power at 355 nm. Only this UV light is sent after beam expansion into the atmosphere so that the system remains eye safe. The atmospheric backscatter signals are collected with a 40 cm telescope. A polychromator extracts the elastic backscatter signal and three inelastic signals, namely the vibrational Raman signal of water vapor, and two pure rotational Raman signals. The detection resolution of these backscatter signals are 1 to 10 s and 3.75 to 7.5 m. All four signals are simultaneously analyzed and stored in both photon-counting (PC) mode and voltage (so-called “analog” mode) in order to make optimum use of the large intensity range of the backscatter signals covering several orders of magnitude.

From these eight primary signals measured by ARTHUS, four independent atmospheric parameters are calculated merging the PC and analog signals: temperature, water vapor mixing ratio, particle backscatter coefficient, and particle extinction coefficient. The temporal resolution of these data is also 1 to 10 s, allowing studies of boundary layer turbulence (Behrendt et al, 2015) and - in combination with a vertical pointing Doppler lidar - sensible and latent heat fluxes (Behrendt et al, 2020).

From the measured number of photon counts in each range bin, the statistical uncertainty of the measured data due to so-called shot-noise can directly be calculated. This value, however, while determining the major part of the uncertainty, does not cover the total uncertainty because additional noise of the analog signals is not included. So the shot-noise uncertainty alone underestimates the uncertainties in the near range where the analog data is used. To solve with this problem, higher-order analyses of the turbulent fluctuations can be performed which allow to determine the total statistical uncertainty of the measurements (Behrendt et al, 2020).

Finally, to investigate the stability of the calibration and thus the accuracy of the measured data, we decided to compare averaged ARTHUS data with local radiosondes. In order to cope with the unavoidable sampling of different air masses between these different instruments, we are investigating the average of a larger number of profiles.  We found that the performance of the measured data of ARTHUS reaches even the stringent requirements of WMO.

The results will be presented at the conference.

 

References:

Behrendt et al. 2015, https://doi.org/10.5194/acp-15-5485-2015

Behrendt et al. 2020, https://doi.org/10.5194/amt-13-3221-2020

Lange et al. 2019, https://doi.org/10.1029/2019GL085774

Wulfmeyer and Behrendt 2022, https://doi.org/10.1007/978-3-030-52171-4_25

How to cite: Behrendt, A., Lange, D., and Wulfmeyer, V.: How good are temperature and humidity measurements with lidar?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15605, https://doi.org/10.5194/egusphere-egu23-15605, 2023.

EGU23-15696 | Posters on site | GI4.2

A new filtering approach for multiple Doppler Lidar setups 

Kevin Wolz, Christopher Holst, Frank Beyrich, and Matthias Mauder

We compare the wind measurements of a virtual tower triple Doppler Lidar setup to those of a sonic anemometer located at a height of 90 m above ground on an instrumented tower and with those of a single Doppler Lidar. The instruments were set up at the boundary-layer field site of the German Meteorological Service (DWD) in July and August of 2020 during the FESST@MOL (Field Experiment on sub-mesoscale spatio-temporal variability at the Meteorological Observatory Lindenberg) 2020 campaign.  The triple Lidar setup was operated in a stare and in a step/stare mode at six heights between 90 and 500 m above ground, while the single Lidar was operated in a continuous scan Velocity-Azimuth-Display (VAD) mode with an azimuthal resolution of around 1.5 ° and a zenith angle of 55.5 °. Overall, both Lidar methods showed a good agreement for the whole study period for different averaging times and scan modes compared to the sonic anemometer. Additionally, we developed and show a new filtering approach based on a Median Absolute Deviation (MAD) filter for the virtual tower setup and compare it to a filtering approach based on a signal-to-noise ratio SNR threshold. The advantage of the MAD filter is that it is not based on a strict threshold but on the MAD of each 30-second period and can, therefore, better adapt to changing atmospheric conditions. In the comparison the MAD filter leads to a greater data availability while upholding similar comparability and bias values between the triple Lidar and sonic anemometer setups. Our results also show that a single Doppler Lidar is a viable method for measuring wind speed and direction with only small disadvantages, at least for measurement heights similar to our investigation and for comparable heterogeneous but flat landscapes.

How to cite: Wolz, K., Holst, C., Beyrich, F., and Mauder, M.: A new filtering approach for multiple Doppler Lidar setups, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15696, https://doi.org/10.5194/egusphere-egu23-15696, 2023.

EGU23-15942 | ECS | Posters on site | GI4.2

Study of the Atmospheric Boundary Layer and Land-Atmosphere Interaction with Lidars 

Syed Abbas, Andreas Behrendt, Florian Späth, Diego Lange, Osama Alnayef, and Volker Wulfmeyer

Investigating the dynamics of the atmospheric boundary layer (ABL) is essential for studies of air quality, the energy and water cycles and for the improvement of weather and climate models. During daytime in convective conditions, the convective boundary layer (CBL) is formed. Here, we present our approach of how to continuously study CBL characteristics with an improved algorithm including fuzzy logic. The Land-Atmosphere Feedback Observatory (LAFO) of University of Hohenheim consists of two Doppler lidars, a Doppler Cloud Radar, the Atmospheric Raman Temperature and Humidity Sounder (ARTHUS), and Eddy covariance stations. These are excellent tools for observing high resolution atmospheric wind profiles, clouds and precipitation events, as well as thermodynamic profiles and surface fluxes. The data are collected at LAFO by operating continuously two Doppler lidars, one in vertical and one in six-beam scanning mode, to obtain vertical and horizontal wind profiles. Both Doppler lidars are operated with resolutions of 1 s and 30 m. The six-beam staring Doppler lidar is used for obtaining time series of turbulent kinetic energy (TKE), momentum flux, TKE dissipation rate and horizontal wind profiles statistics. The vertically staring Doppler lidar is used to compute statistics of higher-order moments of vertical wind fluctuations, the CBL height, and cloud base height. With these data, the land-atmosphere coupling processes and the associated nonlinear feedbacks are investigated as well as their impact on the turbulent structure of the CBL.

We will present analyses of two three-month periods covering different weather conditions: 1 May to 31 July 2021 and 2022.

How to cite: Abbas, S., Behrendt, A., Späth, F., Lange, D., Alnayef, O., and Wulfmeyer, V.: Study of the Atmospheric Boundary Layer and Land-Atmosphere Interaction with Lidars, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15942, https://doi.org/10.5194/egusphere-egu23-15942, 2023.

EGU23-16149 | ECS | Orals | GI4.2

Performance Simulation and Preliminary Measurements of a Raman Lidar for the Retrieval of CO2 Atmospheric Profiles 

Marco Di Paolantonio, Paolo Di Girolamo, Davide Dionisi, Annalisa Di Bernardino, Tatiana Di Iorio, Noemi Franco, Giovanni Giuliano, Anna Maria Iannarelli, Gian Luigi Liberti, and Donato Summa

Within the frame of the project CONCERNING (COmpact RamaN lidar for Atmospheric CO2 and ThERmodyNamic ProfilING), we investigated the feasibility and the limits of a ground-based Raman lidar system dedicated to the measurement of CO2 profiles. The performance of the lidar system was evaluated through a set of numerical simulations. The possibility of exploiting both CO2 Raman lines of the ν1:2ν2 resonance was explored. An accurate quantification of the contribution of the Raman O2 lines on the signal and other (e.g., aerosol, absorbing gases) disturbance sources was carried out. The signal integration over the vertical and over time required to reach a useful signal to noise ratio both in day-time and night-time needed for a quantitative analysis of carbon dioxide sources and sinks was evaluated. The above objectives were obtained developing an instrument simulator software consisting of a radiative transfer model able to simulate, in a spectrally resolved manner, all laser light interaction mechanisms with atmospheric constituents, a consistent background signal, and all the devices present in the considered Raman lidar experimental setup. The results indicate that the simulated lidar system, provided to have a low overlap height, could perform measurements on the low troposphere (<1 km) gradients (1-5 ppm) with sufficient precision both in day-time and night-time with an integration time of 1-3 h and a vertical resolution of 75 m. The selected Raman lidar setup is currently being tested and we aim to present preliminary results during the conference.

How to cite: Di Paolantonio, M., Di Girolamo, P., Dionisi, D., Di Bernardino, A., Di Iorio, T., Franco, N., Giuliano, G., Iannarelli, A. M., Liberti, G. L., and Summa, D.: Performance Simulation and Preliminary Measurements of a Raman Lidar for the Retrieval of CO2 Atmospheric Profiles, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16149, https://doi.org/10.5194/egusphere-egu23-16149, 2023.

EGU23-16192 | ECS | Posters on site | GI4.2

Investigation of Boundary Layer Aerosol Processes with Turbulence-Resolving Lidar 

Osama Alnayef, Andreas Behrendt, Diego Lange, Florian Späth, Volker Wulfmeyer, and Syed Abbas

Our research focuses on the vertical transport of aerosol particles, and the properties of these aerosol particles in dependence on relative humidity. For this, we use the synergy of Raman and Doppler lidar systems operated during the Land-Atmosphere Feedback Experiment (LAFE) (see https://www.arm.gov/research/campaigns/sgp2017lafe).

We will present our first results of investigating the aerosol flux. For this, we use the aerosols backscatter coefficient and vertical wind velocity collected with Raman lidar and Doppler lidar.

The LAFE project was executed at the Southern Great Plains (SGP) site of the Atmospheric Radiation Measurement (ARM) program in August 2017 in the USA.  In addition, data collected at the Land-Atmosphere Feedback Observatory (LAFO) at the University of Hohenheim, Germany is used. Results of the combined aerosol backscatter measurements with water-vapor and temperature lidar measurements to detail insights into the relative humidity dependencies on the growth of aerosols.

How to cite: Alnayef, O., Behrendt, A., Lange, D., Späth, F., Wulfmeyer, V., and Abbas, S.: Investigation of Boundary Layer Aerosol Processes with Turbulence-Resolving Lidar, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16192, https://doi.org/10.5194/egusphere-egu23-16192, 2023.

EGU23-16695 | ECS | Orals | GI4.2

Preliminary Studies and Performance Simulations in support of the mission “CALIGOLA” 

Noemi Franco, Paolo Di Girolamo, Donato Summa, Marco Di Paolantonio, and Davide Dionisi

CALIGOLA (Cloud Aerosol Lidar for Global Scale Observations of the Ocean-Land-Atmosphere System) is a mission funded by the Italian Space Agency (ASI), aimed at the development of a space-borne Raman Lidar. A Phase A study to assess the technological feasibility of the laser source and receiver system is currently underway at the Leonardo S.p.A., while scientific studies in support of the mission are conducted by the University of Basilicata. Scientific and technical studies are furthermore supported by other Italian institutions (CNR-ISMAR, CNR-IMAA), with NASA also having expressed an interest in contributing to the mission .

Mission objectives include the observation of the Earth atmosphere, surface (ocean and land). Among the atmospheric objectives, the characterization of the global scale distribution of natural and anthropogenic aerosols, their radiative properties and interactions with clouds, and the measurements of ocean color, suspended particulate matter and marine chlorophyll.

The expected performance of CALIGOLA has been assessed based on the application of an end-to-end lidar simulator. Specifically, sensitivity studies have been carried out to define the technical specifications for the laser source, the telescope, the optics of transceiver, the detectors and the acquisition system. Simulations reveal that the system can measure Rotational Raman echoes from nitrogen and oxygen molecules stimulated at the three lengths wavelength of 355, 532 and 1064 nm. Simulations also reveal that elastic signals are strong enough to meet the requirements under different environmental conditions. As reference signal, several options have been considered. Among others, a temperature-insensitive rotational Raman signal including rotational lines from nitrogen and oxygen molecules.

A careful analysis of different potential orbits is ongoing, with the goal to identify solutions which maximize performance and scientific impact of both atmospheric and oceanic measurements. Near noon-midnight equatorial crossing times are preferable on the ocean side for diel vertical migration and phytoplankton observations, but degrade significantly the performances of atmospheric measurements due to the high solar background. For this reason is essential to find an orbit in which the solar contribution is low enough to obtain acceptable atmospheric results and at the same time the oceanic measurements are far enough from the night-day transitions for as many days a year as possible to assure correct interpretation of phytoplankton physiology. To counterbalance the degraded signal performances also lower obit height are considered, as well as the use of polarized filters to reduce the amount of solar radiation. The estimated performances under different conditions and considering different orbits will be showed during the presentation.

How to cite: Franco, N., Di Girolamo, P., Summa, D., Di Paolantonio, M., and Dionisi, D.: Preliminary Studies and Performance Simulations in support of the mission “CALIGOLA”, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16695, https://doi.org/10.5194/egusphere-egu23-16695, 2023.

EGU23-808 | ECS | PICO | AS5.7

Comparison of mineral dust scattering properties simulated by the spheroid and irregular-hexahedral models 

Yuyang Chang, Qiaoyun Hu, and Philippe Goloub

Monitoring of the vertical structure of airborne mineral dust, the most abundant aerosol species in the atmosphere, is a significant task for lidar measurements. However, due to the complex morphology and large range of particle size, precise modeling of scattering properties of dust aerosol, particularly for the backward direction, is needed to link lidar measurements to particle microphysical properties. In this study, we investigate two scattering models for non-spherical dust aerosol simulation: the Spheroid model (Dubovik et al., 2006) and the Irregular-Hexahedral model (Saito et al., 2021). The Spheroid model characterizes non-spherical particles as a mixture of spheroids, while the latter utilizes an ensemble of 20 irregular hexahedral particles. Previous studies have proved their feasibilities of simulating the scattering properties of coarse non-spherical particles. Nevertheless, there is a lack of direct comparison between the two models, especially the capability of simulating backward lidar measurements.

In this regard, firstly, a comprehensive sensitivity study was conducted to compare the sensitivities of particle scattering properties produced respectively by the two models to the change of particle microphysical properties. The particle microphysical properties are characterized by bimodal lognormal size distributions and wavelength independent refractive index (RI) to mimic mineral dust aerosols. Preliminary results show the two models produce same variation tendencies of scattering properties as RI and the fine-mode volume fraction (FVF) change. However, discrepancy between the two models increases with the increase of FVF. Particularly, the spectral depolarization ratio produced by the Irregular-Hexahedral model is evidently larger than that by the Spheroid model. Furthermore, backscattering properties produced by the Irregular-Hexahedral model show larger sensitivity to particle imaginary part of the RI. In the second step, we are going to investigate how these differences influence the retrieval of dust aerosol microphysical properties from the measurements of multi-wavelength Mie-Raman-polarization lidars by incorporating the models into BOREAL (Basic algOrithm for REtrieval of Aerosol with Lidar) (Chang et al., 2022). Scenarios of different types of dust aerosols (pure, polluted, fresh, transported, etc.) will be identified and used for the retrieval and a better understanding of the retrieval differences will be gained based on both specific case studies and statistical analysis.

How to cite: Chang, Y., Hu, Q., and Goloub, P.: Comparison of mineral dust scattering properties simulated by the spheroid and irregular-hexahedral models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-808, https://doi.org/10.5194/egusphere-egu23-808, 2023.

Absorbing aerosols from dust, industrial emissions and biomass combustion have a strong impact on solar radiation in the atmosphere, and they are considered to be an important source of regional air pollution[1], especially in East Asia, where the degree of variation of absorbable aerosols is very large, so it will have a significant impact on regional climate change. Aerosol single scattering albedo (SSA) is a key variable of aerosol absorption and a key metric of climate impact. Accurate estimation of SSA is crucial to reduce uncertainties in the study of atmospheric pollution and climate effects.

The aerosol model of the current aerosol inversion algorithm is several typical regional aerosol candidate models obtained by cluster analysis of selected ground observation data[2]. These independent candidates' aerosol models result in the estimation of SSA being just a few simple constants, leading to a large bias in the results of SSA.

In the current study, an atmospheric radiative transfer model parameterized by a two-stream approximation is used to construct a genetic algorithm for application to geostationary satellite Himawari-8 / AHI data to retrieve the aerosol SSA. The inversion process is constrained by AOD and the surface bidirectional reflectance distribution function (BRDF). Using this algorithm, hourly SSA data were retrieved was retrieved during day time.

The algorithm was tested using the hourly L1 grid data of AHI from 00:00 to 07:00(UTC) from January to March 2020. Examples of the 10km satellite-retrieved SSA on March 15, 2020, are shown in Fig. 1. It can be seen that the SSA value in East China is significantly lower than in other regions. This may be due to the developed industries in southern cities that emit a large number of black carbon aerosols, while the temperature in winter is low, and the aerosol particles are not easily diffused, resulting in the SSA value of some areas maintaining a stable low value.

To evaluate the retrieval SSA results, AERONET V3 datasets were used for validation. The AERONET datasets were selected in East Asia. Fig. 2 shows the scatter plots of AHI SSA retrievals versus AERONET at 470nm, (a) all AOD, and (b) only high aerosol loading (AOD>0.4 at 470nm), respectively. This indicates that the algorithm has great advantages for SSA inversion of heavy pollution conditions.

The retrieval results from three months of AHI data were evaluated against the ground-based AERONET measurements. The AHI SSA shows good agreement with AERONET measurements, especially in heavy pollution conditions. This algorithm has been proven to be to characterize the temporal and spatial distribution of aerosol SSA.

How to cite: Xue, Y. and Jiang, X.: Retrieval of aerosol single scattering albedo over land using geostationary satellite data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2610, https://doi.org/10.5194/egusphere-egu23-2610, 2023.

Spaceborne Doppler profiling radars (SDPR) are among the leading instruments considered by space agencies to study atmospheric dynamics. For instance, the European and Japan space agencies are developing the Earth Cloud Aerosol Radiation Explorer (EarthCARE) mission, which will carry the first spaceborne Doppler profiling radar [1,2], while NASA is currently developing the Atmosphere Observing System mission, with a constellation of Doppler radars [3]. 

However, operating an SDPR from low-Earth Orbit (LEO) is challenging due to the large instantaneous speed of the spacecraft (VSAT ~7200 m/s), which affects velocity measurements by broadening the Doppler spectrum that is being measured. Three major error sources that are caused by this spectral broadening are 1) Non-Uniform BeamFilling (NUBF) biases, 2) prohibitive broadening of the measured spectral widths, and 3) a noisiness of the velocity and width measurements [4,5].

In this presentation we will discuss a novel method that we have developed to overcome NUBF and spectral broadening errors that affect SDPR measurements. This method, coined the ExpliSyT approach, is based on the explicit hierarchical representation of the various Doppler moments. For instance, it allows to correct for the broadening of the measured spectral width (second-order Doppler moment), using the measured mean velocity (first-order Doppler moment) and reflectivity factor (zeroth-order Doppler moment). The resulting corrections enable accuracte retrievals of the full spectrum, which in turns enables a higher-order Doppler characterization of atmospheric dynamics. 

The method will be illustrated with simulations of EarthCARE’s radar, and of a notional Displaced Phase Center Antenna (DPCA) configuration developed at JPL [6]. The DPCA configuration uses a pair of collimated antennas to reduce the severity of the spacecraft-induced fading. 

REFERENCES:
[1] A.J. Illingworth et al., “The EarthCARE satellite: The next step forward in global measurements of clouds, aerosols, precipitation, and radiation,” Bull. Amer. Meteorol. Soc., vol. 96, no. 8, pp. 1311–1332, 2015.
[2] H. Kumagai, H. Kuroiwa, S. Kobayashi, and T. Orikasa, “Cloud profiling radar for EarthCARE mission,” Proc. SPIE, vol. 4894, pp. 118–125, Apr. 2003.
[3] https://aos.gsfc.nasa.gov/
[4] R. Meneghini and T. Kozu, Spaceborne Weather Radar. Boston, MA, USA: Artech House, 1990.
[5] P. Kollias, S. Tanelli, A. Battaglia, and A. Tatarevic, “Evaluation of EarthCARE cloud profiling radar Doppler velocity measurements in particle sedimentation regimes,” J. Atmos. Ocean. Technol., vol. 31, no. 2, pp. 366–386, Feb. 2014.
[6] S. L. Durden, P. R. Siqueira, and S. Tanelli, “On the use of multi-antenna radars for spaceborne Doppler precipitation measurements,” IEEE Geoscience and Remote Sensing Letters, vol. 4, no. 1, pp. 181–183, 2007.

How to cite: Sy, O. O. and Tanelli, S.: Novel ExpliSyT method to Correct Dynamic Measurements from Spaceborne Doppler Cloud Profiling Radars, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2975, https://doi.org/10.5194/egusphere-egu23-2975, 2023.

Dust storms often occur in the spring season and influence large areas of Korean peninsula. During a dust storm event, the concentration of dust particles in the atmosphere increases significantly. Satellite monitoring is a powerful tool for studying the properties of large-scale dust storms. however, amidst all uncertainties associated with aerosol properties, the inadequate information about the chemical composition of the dust also greatly affects the radiation field at the top of atmosphere (TOA). GEO-KOMPSAT-2A is a South Korean geostationary meteorological satellite for the meteorological mission and the space weather monitoring mission. It has been equipped with AMI (Advanced Meteorological Imager) and KSEM (Korean Space Environment Monitor) payloads. In this study, an algorithm will be investigated that uses four infrared channels: 8.6 μm, 10.4 μm, 11.2 μm and 12.4 μm, on the AMI. updating Asian dust components according to 25 samples collected during 14 Asian dust events occurring between 2005 and 2018 on the Korean Peninsula and compared them to 34 soil samples (<20 µm) obtained from the Mongolian Gobi Desert, which is a major source of Asian dust will be presented. We used the libRadtran radiative transfer model for simulation of the atmospheric condition, presence of the aerosols and radiance reaching TOA. according to the refractive index and size distribution dataset of new components and strong dependency of TIR wavelength bands to the optical properties of the dust we expect this method will increase the accuracy of the algorithm.

How to cite: Parsa Javid, E. and Park, S. S.: Improvement of the dust retrieval algorithm using GK-2A Geostationary satellite by updating Asian dust chemical composition, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4725, https://doi.org/10.5194/egusphere-egu23-4725, 2023.

Over the past decades there has been both rapid economic growth and increase in energy use in Asia. This has led to a rapid change in the emissions of aerosols and trace gases associated with climate and air pollution, having dramatic effects on the atmosphere. Aerosol absorption optical depth (AAOD) is a measure of the optical-physical-chemical information of particles which absorb visible and UV radation, including: black carbon (BC), dust, and brown carbon (BrC). This subset of total aerosols has a significant and unique effect on air pollution and climate change, including altering the radiative balance and impacting the hydrological cycle. Different unbiased models and methods based on non-aerosol measurments are used to disaggregate urban and industrial areas from suburban and rural areas. These regions are then sampled as constrained in space and time by MISR to elucidate and quantify information about the absorbing particle size distribution, ageing, and emissions in these rapidly changing and/or heavily polluted areas.

To better understand AAOD and its impact on the atmosphere, this work uses both empirical orthogonal decomposition (EOF) and a MIE model based on a core/shell assumption, combining information from from both MISR AAOD and OMI NO2, to determine information about the geospatial and temporal distribution of absorbing aerosols, the size of these particles, regional differences, and physical and chemical properties. The AAOD is constrained by inverted NO2 emissions profiles to find the regional distribution of particulate matter. The differences in the observed values of SSA and AAOD over the four different visible bands are then used to drive the MIE model, which in turn is used to produce a probability distribution of the core size, shell size, and arosol mixing state. The inverse performance of the particle size distributions and mixing state are observed to be dramatically different over urban, industrial, and suburban areas, in specific during the times as constrained by OMI. The impacts of these changes to the atmospheric and radiative profiles over both the source regions are analyzed and used to further evaluate the atmospheric loading, transport, aging, and emissions of abosbing aerosols, with the goal of developing and quantifying the impacts on these regions undergoing the largest amount of change in the region.

How to cite: Liu, Z. and Cohen, J. B.: Characterizing Emissions from Energy Sources Using Aerosol Properties Over Multiple-Wavelengths, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4996, https://doi.org/10.5194/egusphere-egu23-4996, 2023.

NASA’s future Earth System Observatory (ESO) will provide key information related to understanding climate change processes, mitigating natural hazards, fighting forest fires, and improving real-time agricultural processes. The Atmosphere Observing System (AOS) constellation is a key component of the ESO, providing the atmospheric part of the ESO and focusing on two of the five designated observables from the 2017 NASA Earth Science Decadal Survey: aerosols and clouds, convection, and precipitation (CCP). AOS is made up of two projects, one in an inclined orbit (referred to as AOS-I) and the other in a polar, sun synchronous orbit (AOS-P), with both projects addressing synergistic aerosol and CCP science. The constellation is expected to deliver a comprehensive suite of observations to address coupled aerosol-cloud-precipitation interactions, with science objectives focused on low and high cloud feedbacks; the dynamics and structure of convective systems and properties of the aerosol environment; phase partitioning and precipitation formation in frozen and mixed-phase clouds; aerosol microphysical and optical properties, aerosol sources, and relationships to air quality; aerosol vertical redistribution and processing by clouds and precipitation; and aerosol direct and indirect effects. AOS-I and AOS-P are expected to launch no earlier than July 2028 and December 2030, respectively. This talk will describe the science objectives of AOS and the mission architecture and measurement capabilities.

How to cite: Braun, S., Yorks, J., Thorsen, T., and Cecil, D.: The NASA Atmosphere Observing System (AOS): Future Space-Based and Suborbital Observations for the Study of Coupled Aerosol-Cloud-Precipitation Interactions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5092, https://doi.org/10.5194/egusphere-egu23-5092, 2023.

EGU23-5222 | ECS | PICO | AS5.7

Aerosol optical depth validation and aerosol identification using satellite and ground-based data over the high-mountain protected area of Sierra Nevada (Spain) 

Ana del Águila, Domingo Alcaraz-Segura, Javier Martínez-López, and Francisco Navas-Guzmán

High-mountain protected areas are of great interest from the ecological perspective and have a strong impact on the socioeconomic system. However, protected areas such as National Parks, are scarcely investigated from the climatological point of view. Furthermore, the aerosol loading at high elevation locations is not fully characterized. Thus, the analysis of the aerosol optical depth (AOD) in these areas is crucial to assess the role of aerosols in regional climate change and in several ecosystem processes.

We have analyzed the long-term AOD ground-based and satellite remote sensing data in order to provide an accurate picture of the aerosol loading from local to regional scale, respectively. In addition, reanalysis data has been used to provide information of the aerosol typing at larger scale. The Moderate Resolution Imaging Spectroradiometer (MODIS) Version 6 global Multi-Angle Implementation of Atmospheric Correction (MAIAC) (hereafter MODIS+MAIAC) provides daily AOD data at 1 km spatial resolution. The ground-based AOD dataset is obtained from the Aerosol Robotic Network (AERONET) over Granada (South-Eastern Iberian Peninsula) and the high-mountain protected area of Sierra Nevada. Specifically, there are three AERONET stations in the region of interest: Granada at 680 m above sea level (a.s.l), Cerro Poyos at 1809 m a.s.l. and Albergue UGR at 2500 m a.s.l., which have been used for validation. Additionally, the latest reanalysis data from MERRA-2 has been employed for aerosol typing at regional scale, with a spatial resolution of 55 km x 69 km, covering the city of Granada and Sierra Nevada high-mountain protected area.

In this study, we will present the validation results of AODs from MODIS+MAIAC and MERRA-2 against AERONET stations at different altitudes. Moreover, a trend analysis of the AOD for the long-term database at the different seasons is investigated. Finally, the classification of the major aerosol types at regional scale has been performed, indicating the dominant aerosol types and the increase of Saharan dust events in the recent years over the high-mountain protected area of Sierra Nevada.

How to cite: del Águila, A., Alcaraz-Segura, D., Martínez-López, J., and Navas-Guzmán, F.: Aerosol optical depth validation and aerosol identification using satellite and ground-based data over the high-mountain protected area of Sierra Nevada (Spain), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5222, https://doi.org/10.5194/egusphere-egu23-5222, 2023.

EGU23-5819 | PICO | AS5.7

Research infrastructure for the observation of clouds and aerosol in Cyprus 

Dragoș Ene, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Silas Michaelides, Diofantos Hadjimitsis, Albert Ansmann, Johannes Bühl, and Patric Seifert

The presence of aerosol and clouds constitutes one of the highest uncertainties regarding the energy budget of the Earth. Therefore, their continuous observation can help reduce these uncertainties, by providing more information about aerosol-cloud interactions and how these atmospheric components contribute to climate change.

To study the properties of aerosols and clouds, new infrastructure will soon be set up in Cyprus by the Eratosthenes Centre of Excellence, which was recently established through the ‘EXCELSIOR’ H2020 Widespread Teaming Project. Eratosthenes Centre of Excellence is a digital innovation hub for Earth Observation, Space Technology and Geospatial Information, aiming to become the reference centre in the East Mediterranean, north Africa and the Middle East (EMMENA region). The infrastructure will be installed in Limassol, on the south coast of the island. Apart from the fact that the site is less than 2 km from the island’s coastline, this location is extremely important in terms of the regional atmospheric composition, as the air masses affecting the site originate from the surrounding areas of EMMENA, as well as from south-eastern Europe.

Infrastructure to sample aerosol is already represented by a state-of-the-art PollyXT lidar, with measurements being registered continuously since October 2020. By the end of 2023, a similar LACROS multi-instrument platform will be available for the continuous monitoring of clouds and aerosols. This new ground-based remote sensing platform consists of a 35GHz cloud radar, a ceilometer, a microwave radiometer, a Doppler lidar, and a disdrometer. The infrastructure will be integrated into the Cyprus Atmospheric Remote Sensing Observatory (CARO).

An example of the value of the observations about cloud formation and the role of aerosol in the process of cloud formation that will be provided from the site in Limassol, can be reflected in the data collected during the CyCARE campaign, executed between October 2016 and March 2018, during which similar ground-based infrastructure was deployed.  

The authors acknowledge the ‘EXCELSIOR’: ERATOSTHENES: EΧcellence Research Centre for Earth Surveillance and Space-Based Monitoring of the Environment H2020 Widespread Teaming project (www.excelsior2020.eu). The ‘EXCELSIOR’ project has received funding from the European Union’s Horizon 2020 research and innovation programme under Grant Agreement No 857510, from the Government of the Republic of Cyprus through the Directorate General for the European Programmes, Coordination and Development and the Cyprus University of Technology.

How to cite: Ene, D., Mamouri, R.-E., Nisantzi, A., Michaelides, S., Hadjimitsis, D., Ansmann, A., Bühl, J., and Seifert, P.: Research infrastructure for the observation of clouds and aerosol in Cyprus, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5819, https://doi.org/10.5194/egusphere-egu23-5819, 2023.

EGU23-7292 | PICO | AS5.7

Open Source Application of Fusing Aerosol Products from GEO and LEO Satellites 

Jennifer Wei, Sally Zhao, Neil Gutkin, Xiaohua Pan, Pawan Gupta, and Robert Levy

Retrieving aerosol optical depths (AODs) from sun-synchronous polar orbiting (aka low earth orbit, LEO) satellites, such as MODISs, and VIIRSs, OMI, TROPOMI, etc,  has become well-established as a tool for extracting information on particulate matter (PM) and related processes in the atmosphere. However, with recently launched geostationary satellites (GEO), such as GOES-16/17/18,  and Himawari-8/9, and Meteosat Third Generation (MTG)   they provide a much higher temporal resolution (order of 10 minutes), typically an image once or more per hour during daylight compared to LEO once per day.  By combining these observations, we may be able to characterize the diurnal cycle of global AOD at the local, regional and global scale.  

While the science community is still exploring the new data from GEO observations, we have been thinking about how to properly combine/merge/fuse those data considering differences in their spatial and temporal resolutions.  However, this poses a “Big Data” challenge. The big data challenge is not just about data storage,  but also about data discoverability,  and accessibility, and even more, about data migration/mirroring in the cloud-computing environment.   This paper is merely showing some of the efforts and approaches we have attempted in fusing six satellites’ Level 2 aerosol data (three are from GEO (GOES-16/17 and Himawari-8), and the other three are from LEO (TERRA/MODIS, AQUA/MODIS, SNPP-VIIRS) from Dark Target (DT) aAerosol rRetrieval aAlgorithm. Having the on-demand capability of fusing remote sensing products onto the desired temporal and spatial domain enables researchers and application practitioners to better manipulate and work with satellite and sensor data. It is our hopeWe hope that by making such an open-source package, and the accompanying functionality, the scientific community will be granted easier access to aerosol data processing resources.

How to cite: Wei, J., Zhao, S., Gutkin, N., Pan, X., Gupta, P., and Levy, R.: Open Source Application of Fusing Aerosol Products from GEO and LEO Satellites, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7292, https://doi.org/10.5194/egusphere-egu23-7292, 2023.

EGU23-7341 | ECS | PICO | AS5.7

Sensing of rainy clouds using an IR lidar 

Bhavani Kumar Yellapragada

LIDAR is an optical profiler that generally works during clear sky periods.  Lidars operation during disturbed weather conditions is rare [1]. An Infrared lidar sensor was developed indigenously at NARL site to profile clouds and rain during thunderstorm periods. The lidar operates in slant mode through a window and make measurements continuously during cloudburst periods. The developed lidar employs a Nd:YAG laser that operates at its fundamental spectrum in the Infrared band and works in pulsed mode. A spare optical tube assembly (OTA) is employed in the experimental work for collecting the backscattered infrared photons. A high degree of alignment made between laser and OTA units to collect light photons from far ranges. An adjustable conical pin-hole system is employed in the present work, which permitted lidar to function in daylight period. A silicon avalanche photodiode (APD) is used in the demonstration work for optical sensing and signal conditioning. Thin-film interference (IF) filter doublet and a peltier cooled APD supported the lidar measurements at room temperature conditions. An Ethernet interfaced single channel transient recorder unit employed in the receiver measurements, which digitizes signal at 40 MHz rate. The experimental data were recorded at one-second sampling with 7.5 m range resolution. The pump laser uses an in-line optical attenuator that switches at 20 pulses per second. The laser radar probes the atmosphere at a slant angle through a window of the lidar room. The lidar first measurement during thunder clouds and rain is shown in Figure 1. Figure 1 contains two panels. The first panel illustrates the range time intensity map generated using the lidar data that collected between 1200 and 1300 Hrs LT on November 2018 at NARL site. The data plotted in Figure 1 correspond to 7.5 m range resolution at one second time sampling. The other panel of Figure 1 indicates the height profile of lidar range corrected signal (RCS) that obtained at 1203 Hrs LT, which has been shown indicate the lidar signal strength during cloud conditions.  One can notice from Figure 1 the downward movement of thunderstorm cloud deck with time, which further leads fall of rain over land.  One can see rainfall as varying streaks of intensity with range. Different color bands shown in Figure 1 indicate the variations in the intensity of lidar RCS. The red color band indicates the peak value that represents the thunderstorm cloud base. The yellow-orange represents heavy rain events, whereas the shades of green and blue color indicate light rain. The lidar signal overlap occurs at a range of around 100 m, which is 50 m above ground level.

Figure 1. Infrared lidar measurements of cloud and rain during thunderstorm period over NARL site through a window.

 

References

 

[1]. R. Vishnu, Y. Bhavani Kumar, T. Narayana Rao, Anish Kumar M. Nair, A. Jayaraman , “Development of lidar sensor for cloud-based measurements during convective conditions,”, Proc. SPIE. 9876, Remote Sensing of the Atmosphere, Clouds, and Precipitation VI

 

How to cite: Yellapragada, B. K.: Sensing of rainy clouds using an IR lidar, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7341, https://doi.org/10.5194/egusphere-egu23-7341, 2023.

EGU23-8642 | ECS | PICO | AS5.7

NO2 absorption correction for enhanced AOD retrieval 

Ioannis Panagiotis Raptis, Theano Drosoglou, Massimo Valeri, Stefano Casadio, Francesca Barnaba, Gabriele Brizzi, Fabrizio Niro, Monica Campanelli, and Stelios Kazadzs

Aerosol Optical Depth (AOD) retrieval from sunphotometric measurements is sensitive to the concentration of atmospheric gases (e.g. NO2), particularly in UV and lower visible spectral range. Current algorithms used in aerosol networks  either use  climatological NO2 to estimate the corresponding absorption or it is totally ignored . NO2 in the atmosphere is characterized by high spatial and temporal variations, especially in urban areas. Thus, climatological values are rarely representative of the actual NO2 concentration, introducing non-negligible errors in AOD retrievals at specific spectral regions.

We propose a correction approach, using synchronous data from different networks/instruments. AOD is retrieved by sunphotometers (CIMEL and PREDE-POM) in AERONET and SKYNET networks. NO2 total column is calculated by direct sun measurements of PANDORA spectroradiometers, part of PANDONIA network. Data from three stations, with colocation of these instruments are used in presented study to apply the correction and evaluate the new datasets. Two stations in Rome, Italy (Sapienza University at City Center and CNR-ISAC at Tor Vergata in suburban area) and one in Athens, Greece (National Observatory of Athens at city center). More specifically the NO2 correction is applied on AOD at four bandwidths (340, 380, 400 and 440 nm). Propagation of the correction to the calculated Ångström Exponent is also estimated.

Highest mean relative differences are found at 440nm which are up to 1.7% for AERONET data and 5.3% at 400 nm for SKYNET (which’s algorithm does not consider NO2). Highest absolute AOD difference found was 0.037 at 440nm. For Ångström Exponent 440-870 absolute maximum difference found was 0.31.Finally, cases of days with high NO2 variability and the corresponding effect on AOD calculations will be presented.

How to cite: Raptis, I. P., Drosoglou, T., Valeri, M., Casadio, S., Barnaba, F., Brizzi, G., Niro, F., Campanelli, M., and Kazadzs, S.: NO2 absorption correction for enhanced AOD retrieval, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8642, https://doi.org/10.5194/egusphere-egu23-8642, 2023.

EGU23-10050 | ECS | PICO | AS5.7

Cloud Identification and Classification from Ground Based and Satellite Sensors on the Antarctic Plateau 

Michele Martinazzo, Viviana Volonnino, Tiziano Maestri, Fabrizio Masin, Gianluca Di Natale, Giovanni Bianchini, Massimo Del Guasta, and Luca Palchetti

Cloud identification from satellites is considerably challenging in polar environments due to the similar radiative properties of surface and ice clouds, making it difficult to detect and distinguish cloud features. CIC (Cloud Identification and Classification) is a machine learning algorithm adopted as the official software in the ESA Far-infrared Outgoing Radiation Understanding and Monitoring (FORUM) (Palchetti et al., 2020) End2End simulator (FE2ES). CIC is based on Principal Component Analysis and performs cloud detection and multi-scene classification. It is adaptable to every type of sensor and is particularly suitable when a small number of elements are available for the Training Set. Assessment studies have already been conducted to evaluate the performances of the algorithm in multiple conditions. In Maestri et al. (2019), CIC was applied to simulated radiance all over the globe, while Magurno et al. (2020) used the algorithm to analyze airborne interferometric spectra. Finally, in Cossich et al. (2021) the algorithm was tested on downwelling radiances collected at Dome-C in Antarctica. In this work, CIC is applied to high spectrally resolved data taken from ground and, for the first time, from satellites. Ground-based data are collected by the REFIR-PAD sensor (Di Natale et al., 2020), covering the far and mid-infrared part of the spectrum. Collocated satellite data are measured by IASI (Infrared Atmospheric Sounding Interferometer) which collects upwelling radiance between 3.4 and 15.5 μm. The period under study spans from 2012 to 2022. CIC results applied to ground-measured spectra are compared to IASI’s L2 classification products. Large discrepancies between the two classifications are observed, indicating an overestimation of the cloud occurrence in case of IASI. A verification is obtained using collocated ground-based LIDAR measurements, which are available for subsets of the collocated radiances. Finally, the CIC algorithm is trained with a subset of IASI data collocated with REFIR-PAD and LIDAR measurements. The training set is defined also with the help of the Advanced Very High Resolution Radiometer (AVHRR) on board of MetOp satellites. The AVHRR has 1 km resolution (at the nadir) and its collocated measurements are used to evaluate the scene homogeneity in the satellite field of view. Statistical analyses are then performed on IASI spectra using the CIC classification. Results indicate a much better agreement with ground-based data, improving the cloud occurrence provided in IASI L2 products.

How to cite: Martinazzo, M., Volonnino, V., Maestri, T., Masin, F., Di Natale, G., Bianchini, G., Del Guasta, M., and Palchetti, L.: Cloud Identification and Classification from Ground Based and Satellite Sensors on the Antarctic Plateau, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10050, https://doi.org/10.5194/egusphere-egu23-10050, 2023.

Aerosol lidar is widely used in the planetary boundary layer (PBL) height calculation due to its high spatiotemporal resolution. Most of the PBL height (PBLH) algorithms for aerosol lidar are valid for single aerosol layer structure, but overestimate the PBLH under multilayer aerosol/cloud structures. To fill the gap, a new algorithm of PBLH calculation based on multilayer recognition and idealized-profile (MR-IP) is developed. In this algorithm, residual layer and/or suspended aerosol/cloud layer are first recognized based on the signal to noise ratio (SNR) of lidar, the range squared correction signal (RCS) and its gradient (∇RCS). In residual and/or suspended aerosol/cloud layer, positive and negative ∇RCS exist simultaneously, while inside the PBL only a single negative ∇RCS exists. These characteristics are used to discern residual layer and/or suspended aerosol/cloud layers. Aerosol and cloud layers are further distinguished by the ratio of RCS in the objective layer (RCS(rs)) to the mean RCS in the background layer. After multilayer recognition, the PBLH is calculated based on idealized-profile (IP) method. A yearlong (642 samples) comparison of the PBLH calculated by lidar and radiosonde verified the new algorithm in PBLH calculation under complicated structures (R=0.81). The mean PBLH calculated by the MR-IP method is 635.4 m, consistent with the PBLH defined by radiosonde (665.3 m). Furthermore, the residual layer, suspended aerosol layer and cloud layer can also be discerned by the new algorithm.

How to cite: Pan, Y. and Wang, Y.: A new algorithm for planetary boundary layer height calculation based on multilayer recognition, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10843, https://doi.org/10.5194/egusphere-egu23-10843, 2023.

EGU23-11608 | ECS | PICO | AS5.7

Depicting the regime of different aerosol types in NAMEE (North Africa - Middle East - Europe) based on CALIOP-CALIPSO retrievals 

Anna Moustaka, Emmanouil Proestakis, Vassilis Amiridis, Stelios Kazadzis, Kleareti Tourpali, and Antonis Gkikas

The aerosol-induced perturbations of the Earth-Atmosphere system radiation budget are determined by the load and the nature of the suspended particles. Therefore, it is crucial to identify accurately various aerosol types characterized by different optical properties, which regulate aerosol-radiation interactions. The discrimination among aerosol species can be sufficiently achieved from ground-based observations in contrast to those derived by satellite sensors subjected to several limitations. In the case of CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) and the CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) aerosol product, such deficiencies are attributed either to the erroneous classification of the detected aerosol layers or to the incorrect modelling of aerosol microphysics for particular aerosol subtypes.

In the present study, we are developing and demonstrating a simplified aerosol classification scheme capable of identifying dust, marine, clean continental, smoke and urban/smoke particles. For its development, we are relying on quality-assured CALIOP-CALIPSO vertically resolved retrievals (Level 2, Version 4.20) of the backscatter coefficient and the linear particle depolarization extracted from the LIVAS (LIdar climatology of Vertical Aerosol Structure for space-based lidar simulation studies) database. In addition, simulated relative humidity (RH) profiles from MERRA-2 (Modern-Era Retrospective analysis for Research and Applications version 2) as well as the land cover type from the IGBP (International Geosphere–Biosphere Programme) dataset are jointly processed. Moreover, we are applying a discrimination technique suitable for decoupling the individual components of dust-marine and dust-smoke-urban categories, assuming external aerosol mixtures. Finally, for each defined aerosol type we are setting a representative lidar ratio (LR), derived via an extensive literature review of studies utilizing ground-based measurements, required for the derivation of the extinction coefficient at 532nm. Our algorithm is implemented within the NAMEE (North Africa – Middle East – Europe) domain, hosting a variety of aerosol species of natural and anthropogenic origin, and it is applied over a 14-year period (2007-2020).

At the first step of the analysis we are evaluating the columnar aerosol optical depth (AOD), derived from our new classification algorithm, against the corresponding measurements from the ground-based AERONET stations situated within NAMEE as well as versus quality-assured spaceborne (MODIS-Aqua) retrievals. In order to justify the added-value of our approach, we are comparing the assessment results against those obtained from the corresponding evaluation of the raw CALIOP-CALIPSO retrievals using the default and upgraded LRs. After final adjustments in our classification scheme, the aerosol type dependent backscatter and extinction coefficient profiles are gridded at 1° x 1° spatial resolution and on a monthly basis for presenting a 4D climatology within the NAMEE domain. Finally, for each aerosol category we are defining the optical properties required as inputs in a radiative transfer model for estimating the aerosol-induced direct radiative effects within the Earth-Atmosphere system.           

Acknowledgements: Authors acknowledge support by the Hellenic Foundation for Research and Innovation (H.F.R.I.) under the “2nd Call for H.F.R.I. Research Projects to support Post-Doctoral Researchers” (Project Acronym:  ATLANTAS, Project number:  544).

How to cite: Moustaka, A., Proestakis, E., Amiridis, V., Kazadzis, S., Tourpali, K., and Gkikas, A.: Depicting the regime of different aerosol types in NAMEE (North Africa - Middle East - Europe) based on CALIOP-CALIPSO retrievals, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11608, https://doi.org/10.5194/egusphere-egu23-11608, 2023.

EGU23-12228 | ECS | PICO | AS5.7

Impact of parallax correction on Deep Convection Clouds detection frequency. 

Zuzanna Babicka, Andrzej Z. Kotarba, and Izabela Wojciechowska

Satellite data is becoming a progressively accurate source of weather information. An increasing resolution and the number of spectral channels allows to determine the location and recognition of clouds due to their optical and thermal properties.

Predicting the movement of correctly defined deep convection clouds (DCC) is of great importance in forecasting the course of dangerous phenomena for households as well as human health and life. The analysis of trends and occurrence of DCC will make it possible to verify the current climate models, which estimate that the aforementioned phenomena will intensify in the future.

The most common method of detecting DCC is based on the cloud tops temperature. The lower the temperature, the higher and more extensive the cloud is.

The aim of the study is to determine the influence of parallax shift on the frequency of deep convection clouds (DCC).

A geostationary satellite is located at a fixed point in the orbit, which means that the angle of view at higher latitudes is smaller. The higher the object, the greater the parallax shift of the object in relation to its true location. In order to verify the shift and its significance in the analysis of the trend of DCC occurrence, it is necessary to check what values the shift takes and whether it causes significant losses in the number of detected DCC.

The data used for the analysis come from the geostationary satellite Meteosat Second Generation 1 (MSG1) - Meteosat-8, whose sub-satellite point has coordinates: 0oN and 3.4° W. And from the circumpolar satellite Moderate Resolution Imaging Spectroradiometer (MODIS), which it flies at an altitude of 705 km and its cycle lasts 16 days. The cloud tops temperature was obtained from both satellites and used to estimate the cloud tops height.

The analyzes were carried out for the case study of July 4, 2005.

To perform the parallax correction of the geostationary satellite, the existing parallax correction methods were used. For the first time, an attempt was also made to perform parallax correction for a circumpolar satellite.

This research was funded by the National Science Institute of Poland. Grand no. UMO-2020/39/B/ST10/00850.

How to cite: Babicka, Z., Kotarba, A. Z., and Wojciechowska, I.: Impact of parallax correction on Deep Convection Clouds detection frequency., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12228, https://doi.org/10.5194/egusphere-egu23-12228, 2023.

Atmospheric aerosols not only scatter or absorb solar radiation and affect the Earth’s radiation balance, which plays an important role in climate change, but also react with air pollutants and affect public health. In East Asia, due to naturally occurring Asian dust and anthropogenic air pollution resulting from urbanization and industrialization, continuous aerosol monitoring is crucial. Atmospheric aerosols are quantified by satellite- or model-derived Aerosol Optical Depth (AOD), which is defined as the extinction of solar radiation due to aerosols integrated over the atmospheric columns. In this study, machine learning-based models were developed to estimate daytime and nighttime AODs in East Asia using a geostationary satellite Geo-KOMPSAT-2A (GK-2A). Two machine learning approaches, random forest (RF) and light gradient boosting machine (LightGBM), were used in this study. Top-of-atmosphere (TOA) reflectance and brightness temperature (BT) from visible and infrared channels of GK-2A, meteorological data, geographical information, and auxiliary variables were used as input features to the machine learning models. The estimated AOD by the model was evaluated with ground-based AOD data from Aerosol Robotic Network (AERONET) by 10-fold cross-validation methods. To consider the model continuity of day and night and the model performance, two schemes using different combinations of input variables from GK-2A were examined: scheme 1 uses the same composition of input variables of BT for both daytime and nighttime for day-and-night continuity, and scheme 2 additionally uses TOA reflectance only during the daytime based on scheme 1 for high model performance. The LightGBM model (R2 = 0.78, RMSE = 0.1099 for scheme 1, R2 = 0.82, RMSE = 0.0993 for scheme 2) showed higher performance than RF model (R2 = 0.76, RMSE = 0.1213 for scheme 1, R2 = 0.76, RMSE = 0.1214 for scheme 2). Especially in LightGBM model, scheme 2 showed higher performance than scheme 1, and it is supported by the SHapley Additive exPlanations (SHAP) feature importance showing that TOA reflectance of visible and NIR channels of daytime of scheme 2 played an important influence on the model result. The estimated AOD from machine learning-based models were compared with GK-2A level 2 AOD and Copernicus Atmosphere Monitoring Service (CAMS) AOD forecast products. The spatiotemporal distribution in East Asia and time series trend at ground-based stations of estimated AOD show similar patterns to CAMS AOD forecast product, and generally agreed well with AERONET AOD. In conclusion, using the machine learning-based models proposed in this study, it is expected to contribute to continuous satellite-based aerosol and air quality monitoring over a specific region including nighttime, when geostationary satellite-based AOD retrieval is not available. 

How to cite: Song, S., Kang, Y., and Im, J.: Estimation of geostationary satellite-based hourly daytime and nighttime AOD using machine learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12334, https://doi.org/10.5194/egusphere-egu23-12334, 2023.

As a result of progressive global warming, in some regions the frequency of Deep Convective Clouds (DCCs) is expected to increase. However, reliable information about DCCs presence still remains one of the greatest challenges in modern atmospheric sciences, so the misconclusions about existing trends can be avoid. The most accurate data seems to be radar and lidar profiles; unfortunately, the limited spatial resolution of those data, as well as the few years’ time of the operation of radar&lidar missions, makes them not sufficient in terms of providing long-term climatological research. On the other hand, traditional ground-based synoptic observations are mostly limited to land surfaces and are becoming to be provided increasingly rarely. The most promising datasets for present and future DCCs climatologies are those retrieved from geostationary satellite imagers, among which are the METEOSAT First (MFG) and Second Generation (MSG) instruments.

The most commonly used methods for detecting DCCs from satellites are the ones based on brightness temperature (BT), where the specified threshold indicate the presence of convective clouds on satellite images. The simplest of BT-based methods uses the radiances from only one spectral channel: 11 µm (BT11 method). More advances approaches additionally need radiances at 6 µm water vapor absorption channel (BT6-BT11 method) and 9.7 µm oxygen absorption channel (BT11-BT6-BT9.7 method). An utterly different method is to analyze cloud properties, such as cloud top pressure (CTP) and cloud optical thickness (COT), and to determine DCCs presence due to International Satellite Cloud Climatology Project (ISCCP) classification (COT-CTP method). Convective clouds detection can be also supported by meteorological reanalyses.

METEOSAT instruments operates since early 1980s. However, the first generation of METEOSAT imagers were retrieving radiances at only three spectral channels and thus MFG datasets would allow to use only two of the above-mentioned methods: BT11 and BT6-BT11. The rest of approaches could be applied only for MSG datasets (2000s+ time period). This study aims to investigate how many information about DCCs presence are being missed while using only the BT11 or BT6-BT11 methods (which are possible to employ for METEOSAT both First and Second Generation Imagers data) in comparison to the other methods (available for MSG, but not for MFG instruments).

We use data High Rate SEVIRI Level 1.5 Image Data - MSG - 0 degree data, as well as the CLAAS-2.1 (MSG, 0 degree) data containing cloud properties such as CTP and COT for summer season of 2005 (full disk). We compare the frequencies of DCCs determined in accordance to the following methods: BT11 (with ranging brightness temperature thresholds), BT11-BT6, BT11-BT6-BT9.7, COT-CTP, BT11+meteorological reanalyses. The study answers the question how the climatological statistics of DCCs vary depending on the method adopted for detecting these clouds.

This research was funded by the National Science Centre of Poland. Grant no. UMO-2020/39/B/ST10/00850.

How to cite: Wojciechowska, I. and Kotarba, A.: Methods for detecting Deep Convective Clouds (DCCs) from METEOSAT Second Generation Imagers: A case study for 2005 summer season, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12608, https://doi.org/10.5194/egusphere-egu23-12608, 2023.

EGU23-13246 | ECS | PICO | AS5.7

Investigation of Saharan dust plumes in Western Europe by remote sensing, in situ measurements, and transport modelling 

Hengheng Zhang, Frank Wagner, Gholam Ali Hoshyaripour, Heike Vogel, and Harald Saathoff

Atmospheric dust has significant impact on the Earth’s climate system but different aspects of the impact remain highly uncertain. These uncertainties can be attributed to the larger spatial-temporal variability of aerosol dust and its complex interaction with other atmospheric constituents, radiation, and clouds.  To investigate Saharan dust plumes in Western Europe, we collected a comprehensive set of observational data and compared it with global transport model simulations to achieve a better understanding of the distribution, evolution, and potential impact of dust plumes in southwest Germany for four characteristic cases during April 2018, February 2021, June 2021, and March 2022. Remote sensing methods including lidars and sunphotometers were used to study the dust events employing different retrieval methods and comparing these retrievals with ICON-ART simulations. In situ measurements (e.g. Optical Particle Counters (OPC), Aerodynamic Particle Sizer (APS), and Scanning Mobility Particle Sizer (SMPS)) were used to determine e.g. size distributions and particle number concentrations of dust particles, which were compared for suitable cases with remote sensing measurements and ICON-ART simulations. One major objective was to quantify the uncertainties of the different measurements and retrieval methods including a demonstration how useful scanning lidar measurements can be in addition to vertical lidar and sun photometer data and what kind of understanding of the aerosol properties can be achieved by combining the different measurement techniques. Furthermore, we compared these observational data with predictions by the state-of-the-art transport model, ICON-ART, to evaluate the quality of its predictions for different meteorological conditions. In this contribution, we will discuss the systematic comparison between observational data and ICON-ART model results.

How to cite: Zhang, H., Wagner, F., Hoshyaripour, G. A., Vogel, H., and Saathoff, H.: Investigation of Saharan dust plumes in Western Europe by remote sensing, in situ measurements, and transport modelling, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13246, https://doi.org/10.5194/egusphere-egu23-13246, 2023.

EGU23-13515 | ECS | PICO | AS5.7

Machine-learning algorithm for 24h Detection of Fog and Low Stratus over Europe based on MSG-SEVIRI infrared bands 

Babak Jahani, Steffen Karalus, Tobias Zech, Julia Fuchs, Jan Cermak, and Marina Zara

In this communication we present a pixel-based algorithm for detection of fog and low stratus (FLS) during the 24H day cycle over land and across Europe, based on geostationary satellite observations.

Fog and low Stratus are both a persistent aggregation of water particles in liquid and/or solid phases (cloud) close to the Earth surface. As the cloud-base-altitude is the only real difference between the two (fog: touching the ground; low stratus: above ground), they are frequently treated together as a single category from satellite perspective (FLS). This study presents a pixel-based method for detection of FLS over land across Europe based on Meteosat-11 SEVIRI (Spinning Enhanced Visible and InfraRed Imager) infrared observations. The method is based on a gradient boosting machine learning model that is trained with the observations from Meteorological Aviation Routine Weather Reports (METAR) and German Weather Service (DWD) stations. An intensive validation of the product over 356 METAR stations across Europe over five years of daytime winter data revealed that the method proposed is well capable of detecting FLS over land.  Specifically, the algorithm is found to detect FLS with probabilities of detection (POD) ranging from 0.83 to 0.88 (for different inter-comparison approaches), and false alarm ratios (FAR) between 0.34 and 0.36. As the algorithm operates based on the SEVIRI infrared observations only, it can be applied over day and night, making it feasible to continuously monitor the FLS status over large areas over the 24H day cycle.

How to cite: Jahani, B., Karalus, S., Zech, T., Fuchs, J., Cermak, J., and Zara, M.: Machine-learning algorithm for 24h Detection of Fog and Low Stratus over Europe based on MSG-SEVIRI infrared bands, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13515, https://doi.org/10.5194/egusphere-egu23-13515, 2023.

EGU23-13975 | ECS | PICO | AS5.7

High-resolution AOD retrievals using MODIS data and machine learning over East Asia 

Eunjin Kang, Seonyoung Park, Miae Kim, Cheolhee Yoo, and Jungho Im

Atmospheric aerosols are closely related to climate phenomena such as Earth’s energy budget and the formation of clouds. Anthropogenic aerosols have rapidly increased since the industrial revolution, which is damaging to human health, leading to cardiovascular, respiratory, and allergic diseases. Consequently, comprehensive knowledge of aerosol distribution is critical, particularly at detailed spatial scales. AOD measures the vertically integrated extinction of solar radiation by atmospheric aerosol particles. Ground-based sun photometers and satellite remote sensing are mainly used to retrieve AOD as a trade-off relationship. Ground-based measurements have been considered ground truth data, and satellite remote sensing has been used to derive the spatial variability of AOD over vast areas in near real-time. The Moderate Resolution Imaging Spectroradiometer (MODIS) sensor onboard the Terra and Aqua satellite is one of the main operation instruments to retrieve AOD, which has conducted atmospheric observations for almost two decades. MODIS has two well-known aerosol retrieval algorithms, Dark Target (DT) and Deep Blue (DB). Recently, the Multi-Angle Implementation of Atmospheric Correction (MAIAC) algorithm was developed to retrieve high-resolution AOD at a 1 km scale with better performance than DT and DB products. However, DT, DB, and MAIAC algorithms used radiative transfer models (RTM) and lookup tables (LUTs). LUTs was precalculated for a specific aerosol model using meteorological data, atmospheric gases, and constant geometry viewings, which required a high computation. The current LUT-based AOD model has reported uncertainties by aerosol model assumptions. Thus, there is room for complementing the existing AOD retrieval. Recently, machine learning (ML) has been applied with great performance for AOD retrieval. The ML-based AOD retrievals can be processed much faster and simpler without sensitive assumptions of the existing MODIS AOD algorithms. This study developed ML-based AOD retrievals that produce different resolutions of AODs (250m, 500m, and 1km) using MODIS data. The developed AODs at 250m, 500 m, and 1 km showed comparable performance, and 250 m AOD especially caught the spatial dynamics over urban areas well. When compared to MAIAC, 77.8 % of the 250 m AOD values are within the MODIS expected error (EE) envelope of ± (0.05 + 15%), followed by 500 km (76.5 % within EE), 1 km (76.3 % within EE), and MAIAC (70.08% within EE). Even ML-based AOD showed similar performance to MAIAC with three times more samples in the region where MAIAC AOD was unavailable. Our findings suggest the feasibility of ML-based estimation of high-resolution AOD using only satellite data.

How to cite: Kang, E., Park, S., Kim, M., Yoo, C., and Im, J.: High-resolution AOD retrievals using MODIS data and machine learning over East Asia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13975, https://doi.org/10.5194/egusphere-egu23-13975, 2023.

EGU23-14536 | ECS | PICO | AS5.7

Infrared Radiation Effects of Aerosols in the Atmospheric Window during Wet Growth Process 

Denghui Ji, Mathias Palm, and Justus Notholt

Aerosols increase the down-welling infrared (IR) radiation flux in the Arctic. The activation of aerosols increases the down-welling IR flux further, depending on the type of the aerosol. A new instrument, NYAEM-FTS has been installed in Ny-Alesund, Spitsbergen to measure the down-welling IR flux. Ny-Alesund is located on the archipelago of Spitsbergen in the most Northern part of the Atlantic Ocean. It is affected by influx of air from Europe and Asia which leads to import of Aerosols from the polluted areas of Europe and Asia.

We use the measurements of NYAEM -FTS for observing (non-activated) aerosols in cloud-free conditions. We improved this algorithm that it can be used for determining the type of activated aerosol as well.

We present first analysis of the IR measurements to show the dependence of the down-welling infrared radiation on the humidity in the aerosol layer and the chemical composition of the aerosols. This helps to close the gap between the warming effect on the Arctic climate of aerosols on one hand and the warming effect of clouds on the other hand.

 

 

How to cite: Ji, D., Palm, M., and Notholt, J.: Infrared Radiation Effects of Aerosols in the Atmospheric Window during Wet Growth Process, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14536, https://doi.org/10.5194/egusphere-egu23-14536, 2023.

EGU23-14913 | ECS | PICO | AS5.7

Consistency of Aerosol Optical Depth from different Aerosol retrieval algorithms and instruments 

Ulrike Stöffelmair and Thomas Popp

Aerosols affect climate in several ways. Aerosols together with clouds contribute the largest uncertainties to the Earth’s radiative forcing estimates, according to IPCC. Consequently, accurate retrieval of the Aerosol Optical Depth (AOD) from satellite measurements is important to improve the knowledge about aerosols in the global atmosphere and the associated influence of natural and anthropogenic events on the amount of aerosols. Since the retrieval of AOD is typically under-determined it needs assumptions concerning aerosol properties and the surface of the Earth – consequently, there are several different algorithms. We analyse data from the Copernicus Climate Change Service of retrieved AOD with Dual-View Instruments (Along Track Scanning Radiometer 2 (ATSR2), Advanced Along Track Scanning Radiometer (AATSR), Sea and Land Surface Temperature Radiometer (SLSTR)) and the Infrared Atmospheric Sounding Interferometer (IASI) for the retrieval of Dust AOD.

For reliable conclusions the results of these algorithms and of different instruments should be consistent. When looking at different regions we observe, that the consistency between different algorithms differs depending on the type of surface or the geographical location. Looking at fractions of AOD measured by different instruments, we find inconsistencies over deserts and part of the oceans with much sea salt AOD. Apart from that, the results are consistent.

Based on these results, we plan to develop a new retrieval ​​combining the different instruments in order to use their respective advantages and to reduce the errors. In a first step data from SLSTR, IASI and additionally GOME-2 will be combined.

How to cite: Stöffelmair, U. and Popp, T.: Consistency of Aerosol Optical Depth from different Aerosol retrieval algorithms and instruments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14913, https://doi.org/10.5194/egusphere-egu23-14913, 2023.

EGU23-16043 | ECS | PICO | AS5.7

Evaluating and improving the retrieval of cloud droplet number: case studies in an urban region and orographic environments in the E. Mediterranean 

Romanos Foskinis, Alexandros Papayannis, Athanasios Nenes, Konstantinos Eleftheriadis, Stergios Vratolis, Prodromos Fetfatzis, Maria Gini, Evagelia Diapouli, Olga Zografou, Konstantinos Granakis, Alexis Berne, Anne-Claire Marie Billault-Roux, Mika Komppula, and Ville Vakkari

It is well established that the Aerosol-Cloud Interaction (ACI) processes play a key-role in global precipitation and are a strong modulator of cloud radiative forcing and climate, and yet remain poorly understood despite decades of research. Aerosol-cloud interactions are one of the most uncertain aspects of anthropogenic climate change (Seinfeld et al., 2016a; IPCC, 2021).

Global datasets on cloud microphysical state – especially droplet number concentration and size distribution – provide important constraints that are required for reducing the ACI uncertainty. Recently, Quaas et al. (2020) showed that satellite remote sensing is the only approach that offers the potential of obtaining global datasets with frequent coverage; current retrieval algorithms, however, carry many uncertainties and require constraints that can only be addressed with in situ and/or ground-based remote sensing observations.

Our study aims to evaluate retrievals of cloud droplet number (Nd), effective radius (reff) and optical thickness provided by the CLoud property dAtAset using SEVIRI - Edition 3 (CLAAS-3) cloud products of Satellite Application Facility on Climate Monitoring (CM SAF).  For this reason, we used co-located in-situ measurements of aerosols and cloud dynamical properties in conjunction with remote sensing observations at the high-altitude regional background station Hellenic Atmospheric Aerosol and Climate Change (HAC2) during the Cloud-AerosoL InteractionS in the Helmos background TropOsphere (CALISHTO) campaign, which took place from Fall 2021 to Spring 2022 at Mount Helmos in Peloponnese, Greece (https://calishto.panacea-ri.gr/).

In this study, we adopt an approach first applied to droplet retrievals in an urban environment (Foskinis et al. 2022). Ground-based remote sensing instrumentation involved includes a Doppler depolarization lidar (HALO) at 1550 nm to provide the vertical velocity (w) of the air masses, a Doppler cloud radar at 94 GHz (RPG) to provide the equivalent reflectivity factor (Z), and the mean Doppler velocity (VD), and a radiometer at 89 GHz provides the liquid water path (LWP). Furthermore, the in-situ instrumentations employed a co-located scanning Mobility Particle Size (SMPS) measuring the size distribution of submicron aerosol, and a Time-of-Flight Aerosol Chemical Speciation Monitor (ToF-ACSM) to provide the aerosol chemical composition of the aerosols. The in-situ dataset together with the airmass vertical velocity distributions are used as input to a state-of-the art parameterization to predict the droplet number (Nd) in clouds formed in the vicinity of the HAC2 station. Retrievals with the the CLAAS-3 cloud properties product from CMSAF are then evaluated with in-situ observations carried out with a cloud probe instrument (PVM-100) and the droplet number calculations.

Compared to our previous study (Foskinis et al. 2022), this study is implemented in a different physical system, where we examined again the dependence of the Spectral Dispersion of Droplets (SDD) on Nd and we found a new optimized expression between SDD-Nd which can be used on the established droplet number retrieval algorithm (Bennartz et al., 2007) for non-precipitating planetary boundary layer clouds in order to mitigate the bias.

How to cite: Foskinis, R., Papayannis, A., Nenes, A., Eleftheriadis, K., Vratolis, S., Fetfatzis, P., Gini, M., Diapouli, E., Zografou, O., Granakis, K., Berne, A., Billault-Roux, A.-C. M., Komppula, M., and Vakkari, V.: Evaluating and improving the retrieval of cloud droplet number: case studies in an urban region and orographic environments in the E. Mediterranean, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16043, https://doi.org/10.5194/egusphere-egu23-16043, 2023.

EGU23-17366 | ECS | PICO | AS5.7

Retrieving cloud properties based on MTG/IRS (Meteosat Third Generation/InfraRed Sounder) 

Xuemei Chen, Gaëlle Kerdraon, Sonia Péré, Jérôme Vidot, and Emmanuel Fontaine

The next generation Meteosat Third Generation sounding satellite (MTG-S) is expected to be launched at the end of 2024. MTG-S will carry a hyperspectral interferometer, namely InfraRed Sounder (IRS), to provide a four-dimensional look at the atmosphere from a geostationary orbit. IRS will measure the radiance emission from the earth at 1960 infrared spectral channels at two bands (2250 ~ 1600 cm-1 and 1210 ~ 680 cm-1), with a spectral resolution of around 0.60 cm-1.

Satellite-based cloud information is essential for the subsequent retrievals of atmospheric and surface products or for data assimilation in numerical weather prediction (NWP) models. Our project aims at studying the feasibility of retrieving cloud properties from MTG/IRS simulated data, notably cloud mask, cloud classification, and cloud top pressure/temperature/height following NWC SAF threshold methodologies. In this poster, the radiative transfer modelling by RTTOV is carried out at various atmospheric and cloud conditions to study the IRS spectral behaviours, especially at window channels. We will also discuss our preliminary retrieval of a cloud mask by brightness temperature thresholds using the selected IRS channels.

How to cite: Chen, X., Kerdraon, G., Péré, S., Vidot, J., and Fontaine, E.: Retrieving cloud properties based on MTG/IRS (Meteosat Third Generation/InfraRed Sounder), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17366, https://doi.org/10.5194/egusphere-egu23-17366, 2023.

EGU23-309 | ECS | Orals | AS5.9

Measurement of Highly Oxygenated Organic Compounds at the Rambouillet forest during the ACROSS Campaign 

Estephanie Alhajj Moussa, Vincent Michoud, Paola Formenti, Manuela Cirtog, Bénédicte Picquet-Varrault, Sergio Harb, Mathieu Cazaunau, Aline Gratien, Claudia Di Biagio, Emmanuel Tison, Joel F. de Brito, Sebastien Dusanter, Veronique Riffault, Nadine Locoge, Ahmad Lahib, Alexandre Tomas, Marina Jamar, Pablo Espina-Martin, and Christopher Cantrell

Global population increase has placed pressure on available resources and has resulted in the emission of a variety of trace gases into the troposphere that includes volatile organic compounds (VOCs). This class of molecules plays major roles in the formation of secondary products such as secondary organic aerosol (SOA) and tropospheric ozone, which adversely affect Earth’s climate and human health. Research has continued to reveal more details of complex atmospheric degradation processes involving VOCs of both anthropogenic and biogenic origins, but relatively few have been directly studied including the possible impacts of mixing of air masses of anthropogenic and biogenic origins. The ACROSS (Atmospheric ChemistRy Of the Suburban foreSt) project aims to improve our knowledge of atmospheric chemical processes that occur in such mixed air masses and their impact on air quality. The experimental strategy of ACROSS is based on ground-based and airborne observations during an international, large-scale, comprehensive, multi-platform, multi-site field campaign that took place in the summer of 2022 in the greater Paris and suburban forested areas.

As VOCs are processed in the atmosphere, secondary compounds are produced including highly oxygenated organic molecules (HOMs) that are a subset of low volatility organic compounds characterized by their contribution to formation and ageing of SOA. Nitrate ion chemical ionization (CI), coupled with an Atmospheric Pressure Interface−Time-Of-Flight Mass Spectrometer (API-TOF-MS) is an online analytical technique that detects and quantifies gas-phase HOMs (and other compounds) with high sensitivity and mass resolution in the atmosphere or laboratory systems. This instrument provides measurements that help to fill the observational gap between the aerosol and gas phases.

The instrument was deployed at the top of a 40 m tower (above the canopy) in the Rambouillet forest site during the ACROSS field campaign to measure and identify HOMs formed mainly under two different composition regimes: biogenic emissions only, and biogenic air/urban air mixtures. The data collected by the instrument will be presented and used to enhance understanding of the chemical formation pathways of HOMs and their contribution to the composition of aerosols.

How to cite: Alhajj Moussa, E., Michoud, V., Formenti, P., Cirtog, M., Picquet-Varrault, B., Harb, S., Cazaunau, M., Gratien, A., Di Biagio, C., Tison, E., F. de Brito, J., Dusanter, S., Riffault, V., Locoge, N., Lahib, A., Tomas, A., Jamar, M., Espina-Martin, P., and Cantrell, C.: Measurement of Highly Oxygenated Organic Compounds at the Rambouillet forest during the ACROSS Campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-309, https://doi.org/10.5194/egusphere-egu23-309, 2023.

EGU23-420 | ECS | Orals | AS5.9

Aerosol complex refractive index retrieval in the Paris urban area and its forested surroundings during the ACROSS field campaign: variability and constraint for direct radiative effect estimation in regional models 

Ludovico Di Antonio, Claudia Di Biagio, Matthias Beekmann, Aline Gratien, Paola Formenti, Astrid Bauville, Antonin Bérge, Joel Ferreira de Brito, Mathieu Cazaunau, Servanne Chevaillier, Barbara D’Anna, David Owen De Haan, Olivier Favez, Cecile Gaimoz, Olivier Garret, Leila N. Hawkins, Julien Kammer, Brigitte Language, Franck Maisonneuve, Griša Močnik, Anne Monod, Gael Noyalet, Diana Pereira, Sebastien Perrier, Jean-Eudes Petit, Drew Pronovost, Véronique Riffault, Sydney Riley, Matthieu Riva, Marwa Shahin, Guillaume Siour, Brice Temime-Roussel, Chenjie Yu, Pascal Zapf, Gilles Foret, Jean-François Doussin, Christopher Cantrell, and Vincent Michoud

The complex refractive index (CRI) is one of the key parameter driving aerosol spectral optical properties and direct radiative effects (DRE). Its value and spectral variation under different conditions, such as anthropogenic− and biogenic−dominated environments and anthropogenic−biogenic mixing situations, remains not fully understood. As a consequence, oversimplified representations of aerosol optical properties are generally used in climate models. Therefore, measurements of aerosol CRI in different environments and their inclusion in models are needed. The field observations from the ACROSS campaign, performed in June-July 2022 in the Ile de France region, are used in this study to deepen the knowledge of aerosol optical properties, aiming to improve the aerosol representation in the CHIMERE model and provide the best constraint for DRE simulations. Measurements obtained both at the Paris city center and the Rambouilllet rural forest sites during ACROSS are considered, in order to explore the CRI variability from anthropogenic−dominated to biogenic−dominated environments, including anthropogenic−biogenic mixing situations. The CRI retrievals at seven different wavelengths, performed by combining the Mie theory with optical and size distribution measurements, are representative of different atmospheric conditions, aerosol loadings as well as type and chemical compositions. In fact, the June-July 2022 period was characterized by highly diversified weather conditions: 1) two strong heatwaves, promoting SOA build-up and favoring the export of the Paris pollution plume towards the forest site; 2) Saharan dust events transported from the upper atmosphere to the ground; 3) biomass burning episode; 4) periods with reduced anthropogenic influence. The CRI retrievals under these different conditions and their link to particulate chemical composition is investigated. Hence, the CRI dataset presented here constitutes a unique dataset from which models can benefit to validate and constrain simulations and DRE estimations, under both urban and biogenic emissions influence. These data, in conjunction with those from the aircraft observations during ACROSS, are used to initialize and perform sensitivity studies on the aerosol DRE, using the CHIMERE−WRF coupled model, the OPTSIM model for the aerosol optical properties and the Rapid Radiative Transfer Model for GCMs (RRTMG).

Keywords: Complex refractive index, direct radiative effect, aerosol mixing, urban, forest

How to cite: Di Antonio, L., Di Biagio, C., Beekmann, M., Gratien, A., Formenti, P., Bauville, A., Bérge, A., de Brito, J. F., Cazaunau, M., Chevaillier, S., D’Anna, B., De Haan, D. O., Favez, O., Gaimoz, C., Garret, O., Hawkins, L. N., Kammer, J., Language, B., Maisonneuve, F., Močnik, G., Monod, A., Noyalet, G., Pereira, D., Perrier, S., Petit, J.-E., Pronovost, D., Riffault, V., Riley, S., Riva, M., Shahin, M., Siour, G., Temime-Roussel, B., Yu, C., Zapf, P., Foret, G., Doussin, J.-F., Cantrell, C., and Michoud, V.: Aerosol complex refractive index retrieval in the Paris urban area and its forested surroundings during the ACROSS field campaign: variability and constraint for direct radiative effect estimation in regional models, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-420, https://doi.org/10.5194/egusphere-egu23-420, 2023.

EGU23-437 | ECS | Orals | AS5.9 | Highlight

Nighttime concentrations of NO3 and N2O5 in mixed anthropogenic/biogenic air masses during the ACROSS campaign 

Sergio Harb, Manuela Cirtog, Mathieu Cazaunau, Maxime Feingesicht, Vincent Michoud, Xavier Landsheere, Edouard Pangui, Estephanie Alhajj Moussa, Antonin Berge, Christopher Cantrell, and Benedicte Picquet-Varrault

The nitrate radical (NO3) is mainly formed in the atmosphere through the reaction of nitrogen dioxide (NO2) with ozone (O3). It accumulates at night because during the day its photolysis in sunlight and its rapid reaction with nitric oxide (NO) can rapidly consume it. NO3 radical is a major nighttime atmospheric oxidant of biogenic volatile organic compounds (BVOCs), which represent alone 75 to 90% of global non-methane VOC emissions.

Nighttime chemistry between NO3 and BVOCs has received increased attention in the recent literature due to its potential influences on climate, air quality, health and visibility through the formation of many gaseous and particulate secondary pollutants such as organic nitrates, secondary organic aerosol (SOA), ozone and other functionalized products. In several studies conducted in clean forested environments,  NO3 concentrations were found to be very low, mostly below the detection limits (2-6pptv), which can be explained by the low concentrations of precursors (NO2 and O3) and the high reactivity of NO3 with unsaturated BVOCs. However, significant contribution of NO3-BVOC reactions to the secondary pollutants formation in these clean areas have been found.

Since NO3 radicals are formed more rapidly in polluted air masses, it is expected that reactions with BVOCs are even more important in mixed atmospheres, i.e. influenced by both biogenic and anthropogenic sources and characterized by relatively high concentrations of both VOCs and NO2. The ACROSS (Atmospheric ChemistRy Of the Suburban foreSt) field campaign was carried out in June and July 2022 in Ile-de-France region and aims, among other objectives, to assess the potential impact of NO3-BVOC nocturnal processes on SOA formation. For this purpose, a newly developed field instrument, called "NOyBox", was deployed on top of a 40-meter tower, which is above the canopy, located at the Rambouillet Forest supersite southwest of Paris. The instrument allows the measurement of NO3 radicals, N2O5 and HONO (IBB-CEAS, Incoherent Broad Band Cavity Enhanced Absorption Spectroscopy), NO2 (CAPS, Cavity Attenuated Phase Shift) and NOy (gold heated converter coupled with a NO chemiluminescence analyzer). Significant concentrations of NO3 and N2O5 were detected on several nights with situations characterized by air masses coming from the direction of Paris, high concentrations of ozone and NO2, and moderate relative humidity levels. Concentrations of these species as well as concentrations of species of interest for NO3 chemistry are presented and the resulting implications on nighttime chemistry are discussed.

How to cite: Harb, S., Cirtog, M., Cazaunau, M., Feingesicht, M., Michoud, V., Landsheere, X., Pangui, E., Alhajj Moussa, E., Berge, A., Cantrell, C., and Picquet-Varrault, B.: Nighttime concentrations of NO3 and N2O5 in mixed anthropogenic/biogenic air masses during the ACROSS campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-437, https://doi.org/10.5194/egusphere-egu23-437, 2023.

EGU23-493 | ECS | Posters on site | AS5.9

Addressing the chemical composition of secondary organic aerosol in the rural/ urban Paris area 

Diana L Pereira, Aline Gratien, Chiara Giorio, Gael Noyalet, Servanne Chevaillier, Thomas Bertin, Emmanuelle Mebold, Christopher Cantrell, Vincent Michoud, Claudia Di Biagio, Bénédicte Picquet-Varrault, Lelia Hawkins, Olivier Favez, Olivier Garret, Drew Pronovost, Ludovico Di Antonio, Joel F. de Brito, Véronique Riffault, Chenjie Yu, and Paola Formenti

Organic aerosol (OA) from natural or anthropogenic origin can be directly emitted into the atmosphere (primary organic aerosols, POA) or formed by secondary processes via the oxidation of volatile organic compounds (VOC). However, the formation pathways and their chemical composition of these secondary organic aerosols (SOA), which may contribute up to 90% of the OA mass, are not well understood to date, which is problematic due to the relevance of SOA on climate. To address this issue, this study uses a tracer-based approach to identify and quantify the contribution of different anthropogenic/biogenic VOCs precursors to the SOA formation. To do so, we combine experiments in a large scale atmospheric simulations chamber, CESAM (which means Multiphase Atmospheric Experimental Simulation Chamber), and field measurements during the ACROSS (Atmospheric ChemistRy Of the Suburban foreSt) campaign conducted in the Paris area in summer 2022. This approach provides both a mechanistic study of the oxidation of targeted VOCs in simulated and controlled rural/urban atmospheres and the identification of targeted tracers in the real atmosphere, to quantify their concentrations in ambient air.

The ACROSS dataset consists in atmospheric samples of submicron aerosols collected twice a day (day and night) in the urban area of Paris and the Rambouillet forest on the south-west of Paris, as well as samples collected onboard the Safire ATR-42 research aircraft on low-level flights targeting the  evolution and dilution of the Paris urban plume. The CESAM chamber dataset consists in samples of SOA generated by the OH oxidation of toluene/ m-xylene in various conditions.

Filters are analyzed to provide with the chemical composition at the molecular scale by SFE-GC-MS (Supercritical Fluid Extraction Gas Chromatography- Mass Spectrometry) and UPLC-QTOF-MS (Ultra Performance Liquid Chromatography Time of Flight Mass Spectrometry). The organic mass and chemical speciation are obtained by aerosol mass spectrometry and the organic carbon (OC) concentrations by thermal-optical analysis.

The first results of the ambient samples of Paris revealed that the OC concentration varied between 0.69 ± 0.07 and 9.48 ± 0.51 µgC/m3, which correspond to the 28% and 53% of the total mass of the submicron aerosols, for background and polluted (fire) conditions, respectively. These diverse conditions are favorable to trace the compounds identified during the simulation chamber experiments, such as benzoic acid, succinic acid, and 2-methyl-4-nitrophenol. These attempts will be presented and discussed in order to determine the contribution of specific precursors to SOA formation.

How to cite: Pereira, D. L., Gratien, A., Giorio, C., Noyalet, G., Chevaillier, S., Bertin, T., Mebold, E., Cantrell, C., Michoud, V., Di Biagio, C., Picquet-Varrault, B., Hawkins, L., Favez, O., Garret, O., Pronovost, D., Di Antonio, L., F. de Brito, J., Riffault, V., Yu, C., and Formenti, P.: Addressing the chemical composition of secondary organic aerosol in the rural/ urban Paris area, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-493, https://doi.org/10.5194/egusphere-egu23-493, 2023.

EGU23-763 | ECS | Posters on site | AS5.9 | Highlight

Airborne measurement of aerosol physicochemical properties along the Paris urban plume 

Chenjie Yu, Paola Formenti, Peter DeCarlo, Eleonora Aruffo, Piero Di Carlo, Edouard Pangui, Mathieu Cazaunau, Diana L. Pereira, Kevin Tu, Astrid Bauville, Grégoire Cayez, Noel Grand, Pascal Zapf, Vincent Michoud, and Christopher Cantrell

Atmospheric aerosols make significant contributions to several atmospheric chemical and physical processes. Aerosols from anthropogenic emissions have negative impact on air quality and human health. In recent years, significant progress has been made in understanding the anthropogenic pollutants. However, it is still not clear how mixtures of anthropogenic and biogenic emissions impact the regional climate and human health. To better understand aerosol physicochemical properties within the Paris urban plume when mixed with biogenic emissions, a comprehensive airborne measurement platform was deployed in the Île-de-France region in summer 2022 as part of the ACROSS (Atmospheric ChemistRy Of the Suburban foreSt) campaign. In this study, the vertical and spatial distributions of aerosol chemical composition, size distributions, and optical properties during urban plume aging are characterized based on couples of in-situ measurement techniques like aerosol mass spectrometer (c-ToF-AMS), Ultra-High Sensitivity Aerosol Spectrometer (UHSAS) and AVIRAD staged onboard the Safire ATR 42 research aircraft. Gas phase components are also detailed characterized by Proton-transfer-reaction mass spectrometry (PTR-ToF-MS) to act as tracers of anthropogenic and biogenic emissions. Based on gas and particulate phase organic information provided by laser-induced fluorescence technique (TDLIF), the production rate of particulate organic nitrate (pON) can also be estimated. These detailed airborne measurements of aerosol properties provide data that can contribute to modelling studies of aerosol characteristics.

How to cite: Yu, C., Formenti, P., DeCarlo, P., Aruffo, E., Di Carlo, P., Pangui, E., Cazaunau, M., L. Pereira, D., Tu, K., Bauville, A., Cayez, G., Grand, N., Zapf, P., Michoud, V., and Cantrell, C.: Airborne measurement of aerosol physicochemical properties along the Paris urban plume, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-763, https://doi.org/10.5194/egusphere-egu23-763, 2023.

EGU23-3467 | Posters on site | AS5.9 | Highlight

Report on selected measurements in the canopy of a Rambouillet forest site during the ACROSS field campaign 

Alexandre Kukui, Chaoyang Xue, Jérôme Houny, Max Mcgillen, Fanny Bachelier, Benoit Grosselin, Véronique Daële, and Wahid Mellouki

In this contribution we report on a subset of ground-based measurements performed by LPC2E and ICARE at a forest site of Rambouillet during June-July of 2022 in the frame of the project ACROSS (Atmospheric ChemistRy Of the Suburban foreSt). In particular, we present the following time-concentration profiles:

-    OH and sum of peroxy radicals (CIMS , LPC2E);
-    gaseous H2SO4 (CIMS, LPC2E);
-    large number of volatile organic compounds (VOCs) and their oxidation products, including  N-containing oxygenated organic molecules (OOMs) (Orbitrap High Resolution CIMS, LPC2E);
-    directly emitted VOCs and their oxidation products measured by GC-MS/FID (ICARE)
-    HONO (LOPAP, ICARE)
-    NO and NO2 (ICARE)

Based on a first analysis of this reduced data-set some preliminary conclusions are made about an influence of VOCs emissions and NOx variability on the composition of OOMs oxidation products, HONO formation and oxidation capacity in the forest canopy.

How to cite: Kukui, A., Xue, C., Houny, J., Mcgillen, M., Bachelier, F., Grosselin, B., Daële, V., and Mellouki, W.: Report on selected measurements in the canopy of a Rambouillet forest site during the ACROSS field campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3467, https://doi.org/10.5194/egusphere-egu23-3467, 2023.

EGU23-3503 | ECS | Posters on site | AS5.9

Field measurements of organic and inorganic composition in the Rambouillet Forest during ACROSS campaign 

Fanny Bachelier, Chaoyang Xue, Jérôme Houny, Max McGillen, Alexandre Kukui, Benoit Grosselin, Abdelwahid Mellouki, and Véronique Daële

Rambouillet Forest is a large forested location, situated about 50km from central Paris. It covers some 200km² and contains mainly a mix of oak and pine trees. Its size and proximity towards Paris makes it an interesting site to study the interaction between polluted air masses and biogenic emissions and the impact on air quality in areas surrounding polluted cities. The ACROSS (Atmospheric ChemistRy Of the Suburban forest) campaign represents a large international collaboration between various French, European and American institutes, which aims to further characterize these interactions. For our contribution, different instruments from ICARE and LPC2E CNRS Orléans performed in-situ measurements in this forest during June and July of 2022, including: VOCs/ BVOCs (GC-MS/FID); oxidants (OH radicals, CIMS); oxidant precursors (NOx, NOy, Ecophysics, CAPS, LOPAP); and highly oxidized products (orbitrap). In general, data coverage for all instrumentation was high throughout the campaign, furthermore this instrumentation was calibrated and characterized under field condition where possible. These observations represent a broad look at the composition of the forested environment, and contain information on organic emissions, their oxidized products, oxidants and oxidant precursors. We therefore anticipate that these measurements will contribute significantly to the understanding of the atmospheric chemistry operating during the ACROSS campaign.

How to cite: Bachelier, F., Xue, C., Houny, J., McGillen, M., Kukui, A., Grosselin, B., Mellouki, A., and Daële, V.: Field measurements of organic and inorganic composition in the Rambouillet Forest during ACROSS campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3503, https://doi.org/10.5194/egusphere-egu23-3503, 2023.

EGU23-4813 | ECS | Posters on site | AS5.9

Air pollution in rural India: Analysis of satellite NO2 measurements 

Mansi Pathak and Jayanarayanan Kuttippurath

India is a country having more than 67% of its population (947 million) residing in rural areas as of 2020. Therefore, health of the people in rural India becomes important for development plans, economy and growth of the nation. As the sources of NO2 are closely linked to the industrial and economic development of a country, we use satellite measurements of NO2 in rural and urban areas of India to analyse the air quality in these areas. Our findings for rural areas show strong seasonal variations, with winter having the highest NO2 (2.0×1015molec./cm2) whereas monsoon having the lowest (1.5×1015molec./cm2) levels. Around 40% of the total NOpollution comes from rural sources with 45% of it attributed to road transport, however urban areas with more than 90% of their NO2 from power sector were focused in the past studies. Our assessment shows that the NO2 exposure in rural regions is as severe as in urban areas; indicating the need for more effective reduction measures of population exposure and protection of public health. Henceforth, this study reveals that rural India is gradually getting polluted from its nearby regions as well as from the new sources within, which is a big concern for the health of the large rural population of India.

 

How to cite: Pathak, M. and Kuttippurath, J.: Air pollution in rural India: Analysis of satellite NO2 measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4813, https://doi.org/10.5194/egusphere-egu23-4813, 2023.

EGU23-5061 | ECS | Posters on site | AS5.9

NO3 reactivity in a temperate forest impacted by anthropogenic and biogenic emissions during the ACROSS campaign 

Patrick Dewald, Simone T. Andersen, Gunther N.T.E. Tuerk, Jan Schuladen, Tobias Seubert, and John N. Crowley

Terpenoids are readily released into the environment via biogenic emissions. One of their major nighttime oxidizing agent is the nitrate radical (NO3), which is formed from the reaction between ozone (O3) and nitrogen dioxide (NO2). The NO3-initiated oxidation of such biogenic volatile organic compounds (BVOCs) leads to the formation of organic nitrates that can deposit on particles to form secondary organic aerosols. This reaction path thus can lead to irreversible removal of NO2, usually of anthropogenic origin, from the gas phase. Alternatively, NO3 rapidly reacts with nitric oxide (NO) with reformation of NO2. Assigning the contribution of BVOCs and NO to the NO3 reactivity therefore provides insight into the fate of NOx (= NO + NO2).

We used a flow-tube coupled to a cavity-ring-down spectrometer (FT-CRDS) to make direct measurements of the NO3 reactivity in air (at a height of ~ 6 m above ground level) during the ACROSS field campaign in the forest of Rambouillet in the vicinity of Paris, France. Measured reactivities ranged from < 0.006 s-1 to 2.3 s-1, with high average daytime and nighttime reactivities of 0.13 s-1 and 0.25 s-1, respectively. In addition, vertical profiles of NO3 reactivity (up to 40 m) were made and are compared to data previously observed in a boreal forest. Reactivities in Rambouillet forest were highest close the ground (0.36 s-1 at 0 m) and drastically decreased with height (0.08 s-1 at 24 m).

By comparing direct NO3 reactivity measurements with those calculated from trace gas mixing ratios and their corresponding rate coefficients, we identify the contributions of BVOCs and NO to NO3 losses.

How to cite: Dewald, P., Andersen, S. T., Tuerk, G. N. T. E., Schuladen, J., Seubert, T., and Crowley, J. N.: NO3 reactivity in a temperate forest impacted by anthropogenic and biogenic emissions during the ACROSS campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5061, https://doi.org/10.5194/egusphere-egu23-5061, 2023.

EGU23-5065 | ECS | Posters on site | AS5.9

IAQMS-street v2.0: a two-way coupled regional-urban–street-network model system for Beijing, China 

Tao Wang, Jie Li, Youngseob Kim, and Zifa Wang

Owing to the substantial traffic emissions in urban areas, especially near road areas, the concentrations of pollutants, such as ozone (O3) and its precursors, have a large gap with the regional averages and their distributions cannot be captured accurately by traditional single-scale air-quality models. In this study, a new version of a regional-urban-street-network model (IAQMS-street v2.0) is presented. An upscaling module is implemented in IAQMS-street v2.0 to calculate the impact of mass transfer to regional scale from street network. The influence of pollutants in street network is considered in the concentration calculation on regional scale, which is not considered in a previous version (IAQMS-street v1.0). In this study, the simulated results in Beijing during August 2021 by using IAQMS-street v2.0, IAQMS-street v1.0, and the regional model (NAQPMS) are compared. On-road traffic emissions in Beijing, as the key model-input data, were established using intelligent image-recognition technology and real-time traffic big data from navigation applications. The simulated results showed that the O3 and nitrogen oxides (NOx) concentrations in Beijing were reproduced by using IAQMS-street v2.0 both on regional scale and street scale. The prediction fractions within a factor of two (FAC2s) between simulations and observations of NO and NO2 increased from 0.11 and 0.34 in NAQPMS to 0.78 and 1.00 in IAQMS-street v2.0, respectively. The normalized mean biases (NMBs) of NO and NO2 decreased from 2.67 and 1.33 to -0.25 and 0.08. the concentration of NOx at street scale is higher than that at the regional scale, and the simulated distribution of pollutants on regional scale was improved in IAQMS-street v2.0 compared with that in IAQMS-street v1.0.  We further used the IAQMS-street v2.0 to quantify the contribution of local on-road traffic emissions to the O3 and NOx emissions and analyze the effect of traffic-regulation policies in Beijing. Results showed that heavy-duty trucks are the major source of on-road traffic emissions of NOx. The relative contributions of local traffic emissions to NO2, NO, and O3 emissions were 53.41, 57.45, and 8.49%, respectively. We found that traffic-regulation policies in Beijing largely decreased the concentrations of NOx and hydrocarbons (HC); however, the O3 concentration near the road increased due to the decrease consumption of O3 by NO. To decrease the O3 concentration in urban areas, controlling the local emissions of HC and NOx from other sources requires consideration.

How to cite: Wang, T., Li, J., Kim, Y., and Wang, Z.: IAQMS-street v2.0: a two-way coupled regional-urban–street-network model system for Beijing, China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5065, https://doi.org/10.5194/egusphere-egu23-5065, 2023.

EGU23-5240 | ECS | Posters on site | AS5.9

First ground-deployment of a new small-footprintcavity-ring-down spectrometer for NO3 and N2O5 in a temperate forest during the ACROSS campaign 

Gunther N. T. E. Türk, Simone T. Andersen, Patrick Dewald, Jan Schuladen, Tobias Seubert, and John N. Crowley

At nighttime, when concentrations of the OH-radical are low, the nitrate radical, NO3, over takes the role of major initiator of the oxidation of many organic trace gases, especially those containing one or more double bonds. In contrast to daytime, where the lifetime of NO3 is very short due to its photolysis and reaction with NO, NO3 can reach mixing ratios of several tens of ppt at night. NO3 can also react with NO2 to form N2O5. As N2O5 is thermally stable, the three trace-gases usually exist in equilibrium:

NO3 + NO2 + M                ⇌ N2O5 + M

Measurements of NO3 and N2O5 are central to our understanding of the fate of NOx at night. Loss of NO3 to gas-phase reactions (forming e.g. organic nitrates) has a different impact on NOx than formation of N2O5 which may hydrolyse on aerosol to form particulate nitrate.

During the ACROSS campaign in Rambouillet Forest (France), a recently built two-channel cavity-ring-down spectrometer was deployed for the first time to record mixing ratios of NO3 and N2O5 at night over a period of several weeks. NO3 was detected directly at 662nm in one channel while N2O5 was first converted to NO3 in a thermal dissociation inlet before being detected in the same way.

In this work, we describe the new instrument in detail and compare obtained data with those measured by an established cavity-ring-down instrument. We show that, at a sampling height of about 6m, NO3 and N2O5 mixing ratios were low and frequently below the detection limit of both instruments; the likely reasons for this are discussed.

How to cite: Türk, G. N. T. E., Andersen, S. T., Dewald, P., Schuladen, J., Seubert, T., and Crowley, J. N.: First ground-deployment of a new small-footprintcavity-ring-down spectrometer for NO3 and N2O5 in a temperate forest during the ACROSS campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5240, https://doi.org/10.5194/egusphere-egu23-5240, 2023.

EGU23-7568 | Orals | AS5.9 | Highlight

French ACROSS 2022 campaign – First results from CO2/H2O, energy and VOC fluxes measurements at the Rambouillet tower supersite 

Pauline Buysse, Benjamin Loubet, Florence Lafouge, Alain Fortineau, Jeremie Depuydt, Raluca Ciuraru, Baptiste Esnault, Celine Decuq, Pedro-Henrique Herig-Coimbra, Mathis Lozano, Vincent Michoud, and Christopher Cantrell

Volatile organic compounds (VOC) contribute to the production of pollutants harmful to human health and the environment. Most VOC (90 %) are biogenic. At the European scale, forests account for 55 % of the total VOC emissions, crops 27 %, and grasslands, wetlands and shrubs 18 % (Karl, 2009). These estimates are hampered by lack of data acquired at the ecosystem scale. In this work we measured VOC fluxes above the mixed (oaks and pines) forest of Rambouillet (about 60 km south west of Paris) during the ACROSS 2022 summer campaign. The objectives were (1) to quantify emission and deposition of constitutive VOC, and those occurring in response to heat and drought stresses, and (2) to study VOC formation in the canopy.

VOC fluxes were measured at the top of a 40 m-tall tower located at the Rambouillet ACROSS super site. A PTR-Qi-TOF-MS was installed in a shelter at the foot of the tower, and the air sucked through a 50 m heated line by a high-volume pump to ensure short residence time. The PTR-MS was synchronised at 10 Hz with an ultrasonic anemometer to compute fluxes by eddy covariance. Additionally, VOC concentrations were measured along a 5-level profile between 2m and 40m. Preliminary results show emission and deposition of more than 80 VOC compounds. The forest at this location was a strong emitter of monoterpenes, but also of isoprene and sesquiterpenes. A heatwave event has led to a clear decrease in photosynthesis and transpiration during week 28. This period also corresponded to the highest emissions observed during the whole campaign. Deposition of heavy VOC compounds (m/z  > 220) was also observed, possibly corresponding to nitrogen or sulphur containing compounds.

How to cite: Buysse, P., Loubet, B., Lafouge, F., Fortineau, A., Depuydt, J., Ciuraru, R., Esnault, B., Decuq, C., Herig-Coimbra, P.-H., Lozano, M., Michoud, V., and Cantrell, C.: French ACROSS 2022 campaign – First results from CO2/H2O, energy and VOC fluxes measurements at the Rambouillet tower supersite, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7568, https://doi.org/10.5194/egusphere-egu23-7568, 2023.

EGU23-7865 | Posters on site | AS5.9 | Highlight

Hygroscopic and optical properties of complex aerosol mixtures at the Rambouillet forest super-site of the ACROSS project 

Paola Formenti and the ACROSS/Rambouillet aerosol team

The ACROSS (Atmospheric ChemistRy Of the Suburban foreSt) project is an integrative and innovative large-scale initiative that seeks to definitively improve the understanding of the impacts of mixing urban and biogenic air masses in the largest Paris area (the Île-de-France region), where the Paris anthropogenic emissions and the biogenic emissions from the forested surroundings  give rise to the coexistence of several particulate and gaseous species. This scheme promotes the formation of complex mixtures and also influences the physico-chemical aging of aerosol plumes, with consequences on the optical and hygroscopic properties of aerosols, and ultimately on their impacts. Representing the physico-chemical properties, distribution and radiative effect of aerosols at the regional scale of Ile de France is a challenge, limiting our ability to provide reliable climate projections.

ACROSS is based on a multiple platform intensive measurement campaign which was held in June-July 2022. In this paper, we present the first results of the ground-based observations of the aerosol hygroscopic and optical properties at the ACROSS supersite within the downwind Rambouillet forest, located on the south-west of Paris. Here, the PEGASUS (PortablE Gaz and Aerosol Sampling UnitS) mobile facility was operated to deploy an HTDMA (humidified tandem differential mobility analyser) to measure the size-resolved aerosol hygroscopic properties, and a suite of optical analysers including a spectral aethalometer (Magee sci model AE33), a spectral nephelometer (TSI Inc model 3596), and three CAPS-type instruments (Aerodyne Inc, models PMEx and SSA) to measure the particle absorption, scattering and extinction coefficients at wavelengths ranging between 370 and 950 nm. The HDTMA was set to operate primarily at 85% relative humidity. . The observational period was characterised by variable conditions ranging from clean to very polluted depending on the weather.  The surface mass concentrations of submicron particles varied between 2 and 15 µg m-3 through the experimental campaign. The aerosol single scattering albedo at 450 nm varied between 0.88 and 1 during the campaign, the lowest values being observed during the heatwave period between 15 and 22 June when the aerosol optical depth reached 0.5 at 440 nm. The size growth factor (GF) for particles of 200 nm varied between 1 and 2 depending on air mass type and time of the day. The observations will be linked to the aerosol chemical composition and aerosol mixing state also observed during the campaign.

How to cite: Formenti, P. and the ACROSS/Rambouillet aerosol team: Hygroscopic and optical properties of complex aerosol mixtures at the Rambouillet forest super-site of the ACROSS project, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7865, https://doi.org/10.5194/egusphere-egu23-7865, 2023.

EGU23-8093 | ECS | Orals | AS5.9

Investigation of Organic Nitrates in a European Temperate Forest 

Simone Andersen, Patrick Dewald, Laura Wüst, Tobias Seubert, Jan Schuladen, Gunther N. T. E. Türk, Lucy J. Carpenter, and John N. Crowley

Biogenic volatile organic compounds (BVOCs) are to a great extent oxidized by NO3 radicals at night leading to the formation of organic nitrates and secondary organic aerosols (SOA), which have an impact on human health and air quality. One of the focus points of the ACROSS (Atmospheric ChemistRy Of the Suburban forest) campaign, which took place in a temperate forest influenced by emissions from Paris over a period of 6 weeks during the Summer of 2022, was nighttime chemistry between NO3 radicals and BVOCs and its relative importance to daytime chemistry for organic nitrate formation.

Measurements of total alkyl and peroxy nitrates and NO2 mixing ratios were performed using multi-channel cavity-ring-down spectroscopy (CRDS) with thermal dissociation inlets operated at different temperatures to distinguish between alkyl nitrates and peroxy-nitrates.

NO2 were on average 1500 pptv across the entire campaign with an average diel maximum of 2200 pptv at nighttime and minimum of 800 pptv in the afternoon. Both total alkyl and peroxy nitrates showed a diel profile with average daytime maxima of 250 and 450 pptv, respectively, and average nighttime minima of 150 and 250 pptv, respectively.

The relative contributions of day- and nighttime chemistry for generation of ANs will be assessed as will the lifetime of ANs in this environment and the efficiency of NOx conversion into organic nitrates.

How to cite: Andersen, S., Dewald, P., Wüst, L., Seubert, T., Schuladen, J., Türk, G. N. T. E., Carpenter, L. J., and Crowley, J. N.: Investigation of Organic Nitrates in a European Temperate Forest, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8093, https://doi.org/10.5194/egusphere-egu23-8093, 2023.

EGU23-8457 | ECS | Posters on site | AS5.9

Three-dimensional distribution of anthropogenic and natural aerosols over France measured using TROPOMI satellite observations during the ACROSS campaign 

Prem Maheshwarkar, Juan Cuesta, Paola Formenti, Chenjie Yu, Farouk Lemmouchi, and Christopher Cantrell

ACROSS is an extensive field campaign that was conducted over the greater Paris region in summer 2022 to study the interaction between the urban pollution plume and biogenic volatile organic compounds emitted from the surrounding forests. This is mainly done by synergism of in-situ ground-based and airborne observations of the composition of the atmosphere (Cantrell and Michoud, 2022). Satellite observations are complementary to these measurements, providing a regional and continental framework of the atmospheric composition.

In this study, we present new satellite observations of the 3D distribution of anthropogenic and natural atmospheric aerosols over France during the ACROSS campaign. For this, we use a so-called AEROS5P approach which derives vertical profiles of aerosol extinction for each cloud free TROPOspheric Monitoring Instrument (TROPOMI) pixel using hyperspectral top of atmosphere (TOA) reflectance measurements in the visible and near infrared. This method uses a priori knowledge on particle properties, such as their size and refractive index, along with meteorological parameters from meteorological analyses (ECMWF), surface albedo properties, and a unique a priori aerosol vertical profile. The initial version of AEROS5P was able to monitor the 3D distribution of biomass burning aerosols over Australia, which is a single aerosol type (Lemmouchi et al., 2022).

In this study, we present a new version of AEROS5P for deriving the 3D distribution of several aerosol types present in the same atmospheric scene, from both anthropogenic and natural origins. This is done by taking for each TROPOMI pixel the co-localised aerosol type from the VIIRS aerosol product and then processing it with an associated aerosol model of microphysical and optical properties. These aerosol properties are taken from an AERONET sun photometer inversion climatology (Dubovik et al., 2002). This new multi aerosol type AEROS5P method is used for studying dust transport from North Africa, urban pollution from the Paris region, and smoke aerosol transport from South France during the ACROSS campaign. These results are compared against total aerosol extinction from MODIS, vertical aerosol backscatter from CALIOP, airborne and ground-based measurements of aerosol composition, optical and microphysical properties performed in the framework of ACROSS.

References

Cantrell, Christopher, and Vincent Michoud. "An Experiment to Study Atmospheric Oxidation Chemistry and Physics of Mixed Anthropogenic–Biogenic Air Masses in the Greater Paris Area." Bulletin of the American Meteorological Society 103.8 (2022): 599-603.

Dubovik, Oleg, et al. "Variability of absorption and optical properties of key aerosol types observed in worldwide locations." Journal of the atmospheric sciences 59.3 (2002): 590-608

Lemmouchi, Farouk, et al. "Three-Dimensional Distribution of Biomass Burning Aerosols from Australian Wildfires Observed by TROPOMI Satellite Observations." Remote Sensing 14.11 (2022): 2582.

 

How to cite: Maheshwarkar, P., Cuesta, J., Formenti, P., Yu, C., Lemmouchi, F., and Cantrell, C.: Three-dimensional distribution of anthropogenic and natural aerosols over France measured using TROPOMI satellite observations during the ACROSS campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8457, https://doi.org/10.5194/egusphere-egu23-8457, 2023.

EGU23-8905 | ECS | Orals | AS5.9

Particle hygroscopicity in an urban background environment during the ACROSS campaign 

Shravan Deshmukh, Laurent Poulain, Birgit Wehner, Jean-Eudes Petit, Pauline Fombelle, Oliver Favez, Hartmut Herrmann, and Mira Pöhlker

Hygroscopicity strongly influences aerosol particle properties and multiphase chemistry, which also plays an essential role in several atmospheric processes. Although CCN (cloud condensation nuclei) properties are commonly measured, sub-saturation hygroscopicity measurements remain rare. Within the ACROSS campaign, which took place in the Paris region, France, during the summer of 2022, the particle’s hygroscopic growth at 90 % relative humidity (RH) and chemical composition were concurrently measured using a Hygroscopicity Tandem Differential Mobility Analyser (HTDMA, scanning at 100, 150, 200, and 250 nm) and Aerodyne High-Resolution Time-of-Flight Aerosol Mass Spectrometer (HR-ToF-AMS) respectively, at the ACTRIS (the European Aerosol, Clouds and Trace gases Research Infrastructure) SIRTA near facility, a peri-urban site representative of the Greater Paris background conditions. Growth factor probability density distributions (GF-PDF) show two distinct modes: hydrophobic and hygroscopic, indicating that the particles are internally and externally mixed. The hygroscopic mode is always more prominent in the GF-PDF, indicating a change in the particles' mixing state. The dominance of the hygroscopic mode becomes more pronounced with increasing particle size. The mean hygroscopicity parameter values, κ of 100, 150, 200, and 250 nm particles derived from hygroscopicity measurements are respectively 0.23, 0.29, 0.36, and 0.38 during the sampling period. The size dependence is reflected in the averaged values of κ and the GF distributions. A diurnal pattern was observed with an average daytime κ higher than during night-time, which could be linked to aging processes and secondary aerosol formation during the day. The Zdanovskii-Stokes-Robinson (ZSR) mixing rule was applied on the particle chemical to make accurate quantitative predictions of the mean GF of mixed atmospheric aerosol particles.

Keywords: Hygroscopicity, Growth factor, hygroscopicity parameter κ.

How to cite: Deshmukh, S., Poulain, L., Wehner, B., Petit, J.-E., Fombelle, P., Favez, O., Herrmann, H., and Pöhlker, M.: Particle hygroscopicity in an urban background environment during the ACROSS campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8905, https://doi.org/10.5194/egusphere-egu23-8905, 2023.

EGU23-11676 | ECS | Posters on site | AS5.9

In situ VOC measurements in the center of Paris under local biogenic influence ( Spring- Summer 2022) 

Carmen Kalalian, Valérie Gros, Leïla Simon, Vincent Douet, Aurélien Faucheux, Christophe Boitel, Nathalie Bocquet, Julien Kammer, Barbara D'anna, Jean-Eudes Petit, Olivier Favez, Juliette Leymarie, and Christophe Boissard

It is generally acknowledged that urban vegetation improves the environmental quality of cities around the world as they can provide ecosystem services like mitigation of urban heat island effect, and capture of atmospheric pollutants by the leaf surfaces. However, vegetation is also a source of Biogenic Volatile Organic Compounds (BVOC), that can be targets of oxidants produced from chemical interactions with anthropogenic atmospheric pollutants. Such oxidation phenomena trigger the formation of secondary pollutants like ozone (O3) and secondary organic aerosols (SOA). As part of the sTREEt (Impact of sTress on uRban trEEs and on city air quality) project, the present work aims to (i) characterize the ambient gaseous composition in the center of Paris (Town Hall) impacted by a local biogenic source (an urban garden and street trees) and subjected to significant anthropogenic contributions (mainly traffic), and (ii) estimate the contribution of BVOC (vs Anthropogenic VOC) and ultimately their impact on the ambient air quality (O3, SOA). A field campaign took place in Paris city center, from June 8th to July 6th, 2022, notably including a heat wave period on June 17th and 18th (with temperature up to 37°C). The experimental set-up comprised continuous measurements of VOC (using PTR-ToF-MS), NOx (as traffic tracer), aerosol chemical composition (using ACSM) and meteorological parameters (i.e., temperature, wind, light irradiation). VOCs speciation (including terpenes) was also performed off-line based on cartridges analyses for selected days. Results are presented and compared here with measurements at a suburban site at the SIRTA-ACTRIS facility (20 km SW of Paris).

The overall VOC concentrations at the town hall site were higher than at the SIRTA site. Furthermore, isoprene and monoterpenes were mainly of anthropogenic origin, with a diurnal variability and a strong correlation with traffic markers (NOx and aromatic VOC). However, during the heat wave, the concentrations of isoprene and monoterpenes increased and showed a different variability than that of the traffic markers. The concentration of isoprene became very significant with levels around 6 ppb (comparable to the SIRTA site), due to the increase in the biotic component, which may promote the formation of ozone. On the other hand, the moderate increase in monoterpene concentrations (0.1 to 0.7 ppb), due as well to the increase in the biotic component, could contribute significantly to the SOA formation. Thus, assuming a near future increase in the frequency and intensity of heat waves, the contribution of the biogenic source to the ambient air quality may be even more important in urban areas with strong anthropogenic contributions.

How to cite: Kalalian, C., Gros, V., Simon, L., Douet, V., Faucheux, A., Boitel, C., Bocquet, N., Kammer, J., D'anna, B., Petit, J.-E., Favez, O., Leymarie, J., and Boissard, C.: In situ VOC measurements in the center of Paris under local biogenic influence ( Spring- Summer 2022), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11676, https://doi.org/10.5194/egusphere-egu23-11676, 2023.

EGU23-11896 | ECS | Orals | AS5.9

Atmospheric Chemistry linked to HOx radicals of a Suburban Forest during the ACROSS summer Field Campaign 

Nesrine Shamas, Sebastien Batut, Amaury Lahccen, Vincent Michoud, Christopher Cantrell, Sébastien Dusanter, Joel Brito, Alexandre Tomas, Ahmad Lahib, Marina Jamar, Christa Fittschen, and Coralie Schoemaecker

Atmospheric Chemistry linked to HOx radicals of a Suburban Forest during the ACROSS summer Field Campaign

Nesrine. Shamas1, Sebastien. Batut1, Amaury. Lahccen1, Vincent Michoud2, Christopher Cantrell3, Sébastien Dusanter4, Joel Brito4, Alexandre Tomas4, Ahmad Lahib4, Marina Jamar4, Christa. Fittschen1, Coralie. Schoemaecker1

1 PC2A, CNRS – University Lille, Bât. C11, Cité Scientifique, Villeneuve d’Ascq, France

2 LISA, CNRS – Université Paris Cité and Université Paris-Est Créteil, F-94010 Créteil, France

3 LISA, CNRS – Université Paris-Est Créteil and Université Paris Cité, F-94010 Créteil, France

41IMT Nord Europe, Institut Mines-Télécom, Univ. Lille, Center for Energy and Environment, F-59000 Lille, France

Paris, one of the largest European megacities, transports pollution to different surrounding areas depending on the variation of the wind direction associated with specific meteorological conditions. The relatively unique situation of this isolated megacity from other urban areas make it a suitable location to study the impact of urban emissions on the chemistry of close biogenic environments such as forests and vice versa. In order to investigate this influence, the ACROSS (Atmospheric ChemistRy Of the Suburban foreSt) field campaign was performed during summer 2022, with a measurement site located in the Rambouillet forest. The combination of the data provided during this field campaign from different research groups (such as measurements of VOCs, inorganic species, particle concentration and composition, …) will allow a better understanding of the influence of mixing anthropogenic urban or oceanic air masses, leading to different NO concentrations, with biogenic forestry emissions on the oxidation of tropospheric VOCs. This will ultimately help improving this chemistry within atmospheric models. The UL-FAGE instrument was deployed during the ACROSS campaign, where different types of measurements were performed: OH, HO2, ROx radical quantification at the ground level and OH reactivity. The OH reactivity was alternatively measured at two different levels: below (ground level) and above the forest canopy (top of a 40 m tower). Clear stratification was observed during the night with a higher OH reactivity at the ground level than above the canopy. Comparison between the measured and the calculated OH reactivity allows to identify the diurnal missing reactivity at both levels. Preliminary results of the OH reactivity and the radical quantification will be presented.

References

[1] Baklanov et al., Advances in Science and Research, 4, 115–120, 2010

[2] MEGAPOLI campaign 2009-2010 special issue, https://acp.copernicus.org/articles/special_issue248.html page, accessed 24 May 2019

How to cite: Shamas, N., Batut, S., Lahccen, A., Michoud, V., Cantrell, C., Dusanter, S., Brito, J., Tomas, A., Lahib, A., Jamar, M., Fittschen, C., and Schoemaecker, C.: Atmospheric Chemistry linked to HOx radicals of a Suburban Forest during the ACROSS summer Field Campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11896, https://doi.org/10.5194/egusphere-egu23-11896, 2023.

EGU23-12435 | Posters on site | AS5.9

Overview of the ACROSS Campaign near Paris in Summer 2022 

Christopher Cantrell, Vincent Michoud, Jean-Francois Doussin, Paola Formenti, Manuela Cirtog, Patrice Coll, Ludovico Di Antonio, Claudia Di Biagio, Aline Gratien, Benedicte Picquet-Varrault, and Guillaume Siour and the ACROSS Measurement and Modeling Team

ACROSS (Atmospheric ChemistRy Of the Suburban foreSt) is an integrative, innovative, multi-scale project within the “Make Our Planet Great Again” (MOPGA) initiative designed to advance understanding of the fate of the photochemical processing of urban and biogenic air mass mixtures in the Paris region. An ACROSS hypothesis is that the anthropogenic-biogenic air mass mixing leads to changes in the production of oxygenated volatile organic compounds (VOCs) whose properties alter their importance in incorporation into secondary organic aerosols (SOA) and their roles in production of ozone and other relevant secondary species. A likely important factor is NOx transport to suburban biogenic environments and the resulting modification of key chemical processes.

The key highlight of ACROSS was an intensive, multi-platform measurement campaign that took place in the summer of 2022. The campaign included measurements from multi-instrumented ground sites located in the urban, rural, and semi-rural Paris region including a 40-meter tower and from the ground in the Rambouillet suburban forest southwest of Paris, and airborne regional observations following the urban plume downwind of Paris and areas within 150 km (coordinated with other projects in the framework of the PANAME initiative). As the analysis proceeds, the data collected from this campaign will provide a unique snapshot of the properties that are characteristic of combinations of urban and biogenic air masses around one of the largest European megacities. This new knowledge will contribute to advancement of our understanding at the process level and will lead to the ability to better represent such complex systems in numerical models, ultimately resulting in improved capability to predict the impacts on air quality, regional climate, and global climate change.

This presentation consists of a summary of the campaign organization and measurements. Some preliminary findings from the analysis of the observations in the early stages are shown as a complement to other, more focused evaluations that are given at this meeting.

How to cite: Cantrell, C., Michoud, V., Doussin, J.-F., Formenti, P., Cirtog, M., Coll, P., Di Antonio, L., Di Biagio, C., Gratien, A., Picquet-Varrault, B., and Siour, G. and the ACROSS Measurement and Modeling Team: Overview of the ACROSS Campaign near Paris in Summer 2022, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12435, https://doi.org/10.5194/egusphere-egu23-12435, 2023.

EGU23-15788 | Posters on site | AS5.9

Forest fire plumes in the Paris region (France) during summer 2022, the spoor of a schorching summer 

Jean-Eudes Petit, Valérie Gros, Olivier Favez, Leila Simon, Carmen Kalalian, Etienne Brugère, Agnès Borbon, Jean-Charles Dupont, Grégory Abbou, Véronique Ghersi, Vincent Michoud, Claudia Di Biagio, Paola Formenti, Christopher Cantrell, Aline Gration, Joêl Brito, Sebastien Dusanter, Marina Jamar, and Martial Haeffelin

In the context of climate change with increasingly pronounced impacts, year 2022 in France has been the warmest year ever observed. It has been the case more specifically during July, when a severe heatwave occurred across North-Western Europe. Sea-level temperature anomalies jumped over +12°C, especially in the Western half of France, pushing back all-time records. Associated to extreme temperature occurred a severe drought, with long-lasting precipitation deficit throughout the year, which was amplified during July. With around 80% deficit, July 2022 in France has also been the driest ever recorded. These singular meteorological conditions were therefore a fertile ground for forest fires. Around 70 000 ha of forest have burned in France during 2022. The South-West region has been particularly impacted during July 2022, as well as other areas which are not usually subject to this kind of events (Brittany, Center, Paris region).

During July 2022 occurred the ACROSS field campaign within the Paris region, where several sites following a South-West to North-East transect provided comprehensive characterization of atmospheric composition. Namely Rambouillet station (forest, SW of Paris), SIRTA (peri-urban, SW of Paris), PRG (urban, Paris center) and Chatelet Les Halles (urban, Paris center). These sites were equiped with state-of-the-art instrumentations to characterize aerosols and reactive gases. On July 19th, an intense biomass burning plume went through the Paris region, with PM10 concentrations reaching more than 150µg/m3. The experimental effort during that period is therefore a unique asset in order to characterize the composition of this episode.

Most of the sites, during that episode, record high concentrations of carbonaceous aerosols (organic matter and black carbon) and Volatile Organic Compounds tracers of biomass burning (eg acetonitrile, benzene, toluene). Temporality of the episode, atmospheric dynamics and air mass pathways, suggest the transport of a biomass burning plume from South-Western France, more than 600km away from Paris. However, aerosol size distribution surpringly reveals the influence of local fires occuring near some of the sites, at almost the same time. This work is therefore focusing on the different properties of different plumes mixing at the same time over a densely urbanized region. These differences can be highlighted by source apportionment, combined with size distribution, as well as oxydation state of organic aerosols.

How to cite: Petit, J.-E., Gros, V., Favez, O., Simon, L., Kalalian, C., Brugère, E., Borbon, A., Dupont, J.-C., Abbou, G., Ghersi, V., Michoud, V., Di Biagio, C., Formenti, P., Cantrell, C., Gration, A., Brito, J., Dusanter, S., Jamar, M., and Haeffelin, M.: Forest fire plumes in the Paris region (France) during summer 2022, the spoor of a schorching summer, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15788, https://doi.org/10.5194/egusphere-egu23-15788, 2023.

EGU23-17265 | Orals | AS5.9 | Highlight

Observations of trace gases above & below a forest canopy during ACROSS 

Sébastien Dusanter, Joel de Brito, Ahmad Lahib, Alexandre Tomas, Marina Jamar, Estephanie Alhajj Moussa, Astrid Bauville, Christopher Cantrell, Vincent Michoud, Mathieu Cazaunau, Paola Formenti, Fanny Bachelier, Benoit Grosselin, Max McGillen, Veronique Daele, Wahid Mellouki, Chaoyang Xue, Jérôme Houny, and Alexandre Kukui

The ACROSS campaign (Atmospheric chemistry of the suburban forest) is a collaborative effort to better understand how the mixing between urban and biogenic air masses impacts atmospheric composition and reactivity. A main objective is to provide a detailed description of physico-chemical processes involved in atmospheric transformations of biogenic Volatile Organic Compounds (VOCs), and the myriad of intermediate species formed as a consequence, which have yet to be characterized. This multi-platform campaign took place during summer 2022 for a duration of 6 weeks and included a supersite in the Rambouillet forest located on the path of pollution plumes from Paris. An unprecedented suite of analytical instruments was deployed at this site to probe air masses at the ground level and above the forest canopy using a 40-m tower.
This presentation will focus on trace gas observations, including VOCs, ROx (OH+HO2+RO2) and selected inorganic species (O3, NOx – NO+NO2), both above and below the forest canopy. A descriptive analysis will be presented to highlight biogenic VOC oxidation regimes taking place under unpolluted (oceanic air masses) and polluted (Paris plumes) conditions, with a focus on primary/secondary species. Chemical compositions observed above and below-canopy will also be contrasted. On the basis of these observations, this presentation will highlight scientific questions related to ROx, VOC and NOx budgets that will be further investigated to fill important gaps in our understanding of biogenic VOC transformations and secondary organic aerosol formation.


Acknowledgments. This work is supported by the French national research agency (ANR-20-CE01-0010) & LABEX-CaPPA (ANR-11-LABX-005-01) and the French national program LEFE/CHAT INSU.

How to cite: Dusanter, S., de Brito, J., Lahib, A., Tomas, A., Jamar, M., Alhajj Moussa, E., Bauville, A., Cantrell, C., Michoud, V., Cazaunau, M., Formenti, P., Bachelier, F., Grosselin, B., McGillen, M., Daele, V., Mellouki, W., Xue, C., Houny, J., and Kukui, A.: Observations of trace gases above & below a forest canopy during ACROSS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17265, https://doi.org/10.5194/egusphere-egu23-17265, 2023.

EGU23-17306 | Orals | AS5.9

Contrasting aerosol composition in and out of Paris plume during the ACROSS campaign at the Rambouillet supersite 

Joel Ferreira de Brito, Paola Formenti, Sebastien Dusanter, Marina Jamar, Alexandre Tomas, Laurent Alleman, Esperanza Perdrix, Pablo Espina, Veronique Riffault, Chenjie Yu, Claudia Di Biagio, Aline Gratien, Ludovico Di Antonio, Lelia Hawkins, Barbara D'Anna, Julien Kammer, Anne Monod, Jean-Eudes Petit, Shravan Deshmukh, and Laurent Poulain and the ACROSS Leadership

Based on a combination of ground-sites and aircraft observations, the ACROSS (Atmospheric ChemistRy Of the Suburban foreSt) project seeks to better understand how the pollution from Paris affects air quality over large regional scales, particularly through interaction with biogenic species. A field campaign took place in June-July 2022 at three sites: a forested remote site (Rambouillet, 50 km southwest from downtown Paris) a peri-urban (SIRTA) and an urban ones (PRG). The extensive instrumentation deployed at those sites allows to gain insights into the transformation of gaseous and particulate species from local to regional scales. Besides, the Rambouillet site has not only served as a receptor site from Paris plume but also led to detailed observations of freshly emitted biogenic compounds and their role in local chemistry, reactivity, and aerosol properties.

This work focuses on the real-time aerosol composition at the Rambouillet site. High resolution time-of-flight aerosol mass spectrometry sampled air from below (3 m above ground level) and above the canopy (40 m), and has been complemented by a suite of aerosol instruments including PTRMS-CHARON (targeting semi-volatile species above the canopy), and the PEGASUS mobile facility sampling below the canopy. Furthermore, data will be combined with SIRTA and PRG observations for case studies where Paris plume was transported into the supersite, or conversely, clean air masses were first observed at the remote site, and then advected towards the urban area. During the six-week observation period, the average PM1 (non-refractory PM1 + equivalent BC) was 8.4 µg m-3, with significant variability (10th-90th percentiles of 2.3 and 17.9 µg m-3). The dominant component was organics with an average contribution to PM1 of 62%, and peak contribution during periods of warm temperature of up to 90%. The organic aerosol was fairly oxidized at the site (average O:C ratio of 0.6), as expected for such an environment, with a negative trend of oxidation with organic aerosol loading, indicating primary or relatively fresh particles contributing the most to polluted episodes. Secondary inorganic aerosols (sulfate, nitrate, and ammonium) represented about 34% of PM1, with the highest contribution during cold, rainy periods, and equivalent BC only had a minor contribution of about 4%. This presentation aims at providing a large picture of aerosol composition in the Ile-de-France region during the ACROSS experiment.

Acknowledgments. This work is supported by the French national research agency (ANR-20-CE01-0010), the Labex CaPPA (ANR-11-LABX-005-01) and the French national program LEFE/CHAT INSU.

How to cite: Ferreira de Brito, J., Formenti, P., Dusanter, S., Jamar, M., Tomas, A., Alleman, L., Perdrix, E., Espina, P., Riffault, V., Yu, C., Di Biagio, C., Gratien, A., Di Antonio, L., Hawkins, L., D'Anna, B., Kammer, J., Monod, A., Petit, J.-E., Deshmukh, S., and Poulain, L. and the ACROSS Leadership: Contrasting aerosol composition in and out of Paris plume during the ACROSS campaign at the Rambouillet supersite, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17306, https://doi.org/10.5194/egusphere-egu23-17306, 2023.

EGU23-17469 | ECS | Posters on site | AS5.9

Presence of siloxanes in the ambient air of urban Paris during the ACROSS field campaign 

Rulan Verma, Sebastien Perrier, Vincent Michoud, Claudia Di Biagio, Aline Gratien, Lelia Hawkins, Barbara D'Anna, Julien Kammer, Anne Monod, Christopher Cantrell, Christian George, and Matthieu Riva

Cyclic volatile methyl Siloxanes (cVMS) are a group of silicon-based organic compounds of anthropogenic origin that are found ubiquitously in the ambient air. They find wide application in many industrial, automotive products, consumer, and personal care products such as paints, solvents, adhesives, cosmetics, polymers, etc. About 90% of the environmentally released cyclic siloxanes diffuse directly into the atmosphere. They are high–production volume chemicals with some having an annual production rate of 45 to 227 thousand tons worldwide. Siloxanes have been observed in both urban and rural areas. Among the different siloxanes emitted into the atmosphere hexamethylcyclotrisiloxane (D3), octamethylcyclotetrasiloxane (D4), and decamethylcyclopentasiloxane (D5) are of great importance due to their subsequent concentrations. It should be mentioned that siloxanes are not readily biodegradable which means they can persist in the environment for a long duration. The D4 species has already been identified as a potential persistent organic pollutant (PoPs). D4 and D5 are very persistent and bioaccumulative and have evinced or potential hazards to both humans and the environment.

Taking advantage of the Vocus proton-transfer-reaction time-of-flight mass spectrometer (VOCUS PTR–TOF–MS) the D3, D4, and D5 species were measured in real-time downtown Paris in the June–July 2022 period. The measurements were performed during the ACROSS (Atmospheric ChemistRy Of the Suburban foreSt) field campaign at the urban site located at Université Paris Cité (48.83°N, 2.38°E) sampling at about 25 m above the ground level. The data collected during the summer 2022 showed that the mean concentrations were 0.099±0.009, 0.045±0.009, and 0.131±0.089 ppb for D3, D4, and D5, respectively. A strong diurnal cycle was observed for the different siloxanes. Concentrations for the D5 siloxane peaked in the morning with an averaged maximum of 0.298± 0.119 ppb while the 25th and the 75th quantile are 0.221 and 0.377 ppb, respectively. In the afternoon concentrations show a minimum value, followed by a slight increase during the night. The D5 is the most abundant siloxane species and shows the strongest diurnal cycle compared to the other two identified siloxanes. Observations during the campaign and the potential reaction products and sources of siloxanes will be discussed in this work.

KEYWORDS: Siloxanes; Cyclic Siloxanes; D3,D4 and D5; Ambient Air; PoPs; ACROSS; HR- Mass Spectrometry; VOCUS PTR-Tof

How to cite: Verma, R., Perrier, S., Michoud, V., Di Biagio, C., Gratien, A., Hawkins, L., D'Anna, B., Kammer, J., Monod, A., Cantrell, C., George, C., and Riva, M.: Presence of siloxanes in the ambient air of urban Paris during the ACROSS field campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17469, https://doi.org/10.5194/egusphere-egu23-17469, 2023.

EGU23-17485 | Orals | AS5.9 | Highlight

Meteorological variability and regional pollutant distributions during the summer 2022 ACROSS/PANAME campaign 

Matthias Beekmann, Guillaume Siour, Ludovico Di Antonio, Gilles Foret, Frederic Meleux, Augustin Colette, Amandine Rosso, Claudia Di Biagio, Juan Cuesta, Paola Formenti, Aline Gratien, Martial Haeffelin, Simone Kotthaus, Valery Masson, Vincent Michoud, and Christopher Cantrell

The international ACROSS (Atmospheric ChemistRy Of the Suburban forest) intensive field measurement campaign (supported by the Make Our Planet Great Again initiative) took place from June 13 to July 25 2022 in and around the Ile-de-France during an exceptional hot (more than 3°C above the climatological mean for France) and dry summer season. This work will provide a broad classification of weather conditions that occurred during the campaign, useful for further analysis of observations and simulations. Weather scenarios will be analysed in terms of synoptic weather situations, relating transport patterns (regional advection to the Ile-de-France region, plumes from Paris agglomeration), temperature and relative humidity evolution. During the June-July 2022 period, several distinct weather and pollution patterns occurred, among which: (1) two strong heatwaves, with large photochemical activity promoting secondary pollutants build-up (O3, SOA), (2) advection of relatively clean oceanic air masses, and (3) Saharan dust and intense forest fire events with dust and fire aerosol advection to the Ile-de-France region. The analysis is based on meteorological data from several models (GFS, WRF, ARPEGE, AROME) and observations, pollution forecasts from the French Prev’Air system (http://www2.prevair.org/), and from the AirParif Esmeralda platform (http://www.esmeralda-web.fr/accueil/)  that have been used for the airborne campaign support. In addition, dedicated simulations with the CHIMERE model (see companion abstract by Di Antonio et al. for this session), and major pollutant observations by air quality networks, from satellites, or performed within ACROSS will be used to analyse how meteorological conditions and weather patterns impacted the spatial distributions of major primary and secondary chemical species. Especially tracers of anthropogenic and biogenic emissions and photochemical activity (O3, PM2.5, OA, BC, NOx, BVOC) will be analysed. 

 

Keywords: Meteorology, pollutant distributions, transport patterns, ACROSS, MOPGA  

How to cite: Beekmann, M., Siour, G., Di Antonio, L., Foret, G., Meleux, F., Colette, A., Rosso, A., Di Biagio, C., Cuesta, J., Formenti, P., Gratien, A., Haeffelin, M., Kotthaus, S., Masson, V., Michoud, V., and Cantrell, C.: Meteorological variability and regional pollutant distributions during the summer 2022 ACROSS/PANAME campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17485, https://doi.org/10.5194/egusphere-egu23-17485, 2023.

EGU23-17525 | ECS | Posters on site | AS5.9

Organic particles and gaseous precursors in suburban Paris during the ACROSS campaign in summer 2022: first deployment of a PTR-ToF-MS coupled with CHARON at the SIRTA observatory 

Etienne Brugère, Shravan Deshmukh, Aurélie Lambreschi, Leïla Simon, Carmen Kalalian, Nicolas Bonnaire, Aurélie Colomb, Evelyn Freney, Valérie Gros, Jean-Eudes Petit, Laurent Poulain, Mickaël Ribeiro, Junteng Wu, and Agnès Borbon

Atmospheric organic aerosols (OA) are important because of their ubiquity and significance. They are the key drivers of air quality and climate change. While the secondary fraction of OA, namely SOA, is dominant in mass (between 50 to 85%), our capability to predict SOA is still uncertain because of the influence of multiple parameters (ie. humidity, temperature, NOx, nature and vapor pressure of organic gaseous precursors). Quantifying the partitioning between the gas and particle phases of semi-volatile organic compounds (SVOCs) in real conditions is one relevant approach to better constraint the budget of SOA and to develop accurate parametrization for organic aerosol formation in climate models.

During the summer of 2022, the ACROSS field campaign (Atmospheric ChemistRy Of the Suburban foreSt) took place in the Paris region at several sites located along a southwest to northeast transect for a comprehensive characterization of the gaseous and particulate atmospheric composition. For the first time, a PTR-ToF-MS (Proton Transfer Reaction-Time of Flight Mass Spectrometry) coupled with a CHARON (Chemical Analysis of aeRosol ON-line) inlet as part of the MOCCA set-up (Mass spectrOmetry for the multiphasic Composition of the Cloudy Atmosphere) was deployed at the SIRTA observatory. SIRTA is a suburban site being part of the Aerosols, Cloud, and Trace gases Research InfraStructure (ACTRIS), where long-term monitoring of in-situ reactive gases and particles has been performed for more than a decade [Simon et al. 2022]. Such deployment is a unique opportunity to qualify and intercompare the technical performances of the CHARON-PTR-ToF-MS system with other state of the art instrumentation at the site [Petit et al. 2015/Zhang et al., 2019] (PTR-Q-MS, quadrupole Aerosol Chemical Speciation Monitor (Q-ACSM), Scanning Mobility Particle Sizer (SMPS), Condensation Particle Counter (CPC)), or aerosol size spectrometer for PM-10 and PM-2.5 and also a High-Resolution Time-of-Flight Aerosol Mass Spectrometer (HR-ToF-AMS) by TROPOS institute.

In this work, I will present the technical evaluation of the CHARON-PTR-ToF-MS system with respects to other conventional mass spectrometry methods such as the ACSM, under both controlled laboratory conditions and ambient conditions. Using the unique features of the CHARON-PTR-ToF-MS system, it will consider the analysis of the temporal variability of trace gases and aerosol observations, meteorology and air mass trajectories, relevant and contrasting periods, thus, the partitioning between the particle phase and the gaseous phase could be estimated. These observations will be compared to collocated measurements of trace gases and aerosols and will be used to evaluate model predictions using equilibrium partitioning theory.

 

References :

Petit, J.-E., et al..: Two years of near real-time chemical composition of submicron aerosols in the region of Paris using an Aerosol Chemical Speciation Monitor (ACSM) and a multi-wavelength Aethalometer, Atmos. Chem. Phys., 15, 2985–3005, https://doi.org/10.5194/acp-15-2985-2015, 2015.

Simon, L., et al.: Two years of Volatile Organic Compounds online in-situ measurements at SIRTA (Paris region, France) using Proton-Transfer-Reaction Mass Spectrometry, Earth Syst. Sci. Data Discuss. [preprint], https://doi.org/10.5194/essd-2022-406, in review, 2022.

Zhang, Y., et al., A.: Six-year source apportionment of submicron organic aerosols from near-continuous highly time-resolved measurements at SIRTA (Paris area, France), Atmos. Chem. Phys., 19, 14755–14776, https://doi.org/10.5194/acp-19-14755-2019, 2019.

How to cite: Brugère, E., Deshmukh, S., Lambreschi, A., Simon, L., Kalalian, C., Bonnaire, N., Colomb, A., Freney, E., Gros, V., Petit, J.-E., Poulain, L., Ribeiro, M., Wu, J., and Borbon, A.: Organic particles and gaseous precursors in suburban Paris during the ACROSS campaign in summer 2022: first deployment of a PTR-ToF-MS coupled with CHARON at the SIRTA observatory, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17525, https://doi.org/10.5194/egusphere-egu23-17525, 2023.

The so-called sea spray effect is known to considerably influence the stable isotope fingerprint of coastal samples (plants, soil, bones, teeth). However, the impact of sea spray on radiocarbon analyses in environmental samples from coastal sites has not been investigated, yet. Sea spray aerosols, containing, e.g., HCO3- or CO32- of marine origin, enter the terrestrial environment, shifting stable isotope values of terrestrial samples towards a seemingly marine isotope signature. Moreover, the sea spray is always accompanied by physiological effects in the sprayed plants, e.g., due to the salinity of the incorporated water, also visible in, e.g., stable carbon isotope data. A terrestrial herbivore, never consuming any marine food, can show a marine isotope signal due to the sea spray effect. While the marine reservoir effect, resulting from the consumption of marine food sources, can be investigated by calculating isotopic mixing models based on the δ13Ccollagen and δ15Ncollagen values of archaeological animal and human bones, the sea spray effect remains undetected in the δ13Ccollagen and δ15Ncollagen values of individuals consuming terrestrial protein (i.e., plant sources) influenced by marine aerosols. Therefore, it is important to investigate the influence of the sea spray on the radiocarbon signature.

The impact of either the direct or the accompanied, indirect sea spray effect can be visualized by an artificial sea spray experiment which was performed in a greenhouse. European beach grass (Ammophila arenaria, L.) was sprayed with mineral salt solution of different ion concentration but only traces of NaCl, with salty water from the Schlei inlet, collected next to the archaeological site of Haithabu (Germany), and with seawater from the Baltic Sea, collected at the western coast of Fehmarn island (Germany), respectively. Plants of all treatment groups were irrigated with Munich tap water (mainly originating from Mangfall valley). Radiocarbon analyses (F14C), stable as well as radiogenic isotope analyses (δ13CDIC, δ13Cbulk, δ13Ccellulose, δ18Ocellulose, δ18Osulfate, δ34Ssulfate, δ34Stotal S, 87Sr/86Sr), and (trace) elemental analyses were conducted on the plant, soil, and water samples (spray water, irrigation water) using mass spectrometry (AMS, IRMS, TIMS, ICP-MS, IC).

Radiocarbon analyses of the plants showed an impact due to the artificial sea spray. The indirect sea spray effect, resulting from either salinity (NaCl) or HCO3- stress, has an impact on plants’ F14C. The study demonstrates that a substantial proportion of 14C, which is taken up by the sprayed plants, originates from either irrigation or spray water. Stomatal conductance is markedly reduced due to both salinity and bicarbonate stress. Accordingly, less atmospheric 14CO2 can enter the plants via their stomata, while H14CO3-/14CO32-/14CO2 (aq.) can still be incorporated via the roots.

A multi-dimensional approach with a combined analysis of stable (δ13C, δ18O, δ34S), radiogenic (87Sr/86Sr), and radiocarbon isotopes in environmental samples allows to depict a detailed image of biochemical and physiological processes associated with the sea spray effect and will help to reveal new insights into the sea spray impact on the isotopic fingerprint of plants, animals, and humans, including potential caveats for radiocarbon analyses in coastal regions.

How to cite: Göhring, A., Hüls, C. M., Hölzl, S., Mayr, C., and Strauss, H.: Indirect sea spray effects on radiocarbon data of coastal plants – how physiological reactions in plants can be visualized by a combined investigation of stable, radiogenic, and radiocarbon isotopes in a greenhouse experiment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-128, https://doi.org/10.5194/egusphere-egu23-128, 2023.

Last glacial loess in Poland was deposited under periglacial conditions nearby to the regional maximum advance of the Scandinavian Ice Sheet during the Weichselian glaciation. Its glacier advance and retreat stages are expected to be mirrored in Loess-Paleosol Sequences (LPS) calling for reliable and exact dating. In the Bayreuth luminescence laboratory (BT) established modern SAR protocols of optical dating (OSL, pIRSL) were applied to the 4-11µm fine grain fraction of 38 loess samples from four LPS, distributed from Silesia to the Volhynian upland. Results were compared to published results from the Gliwice luminescence laboratory. Pleasing basic agreement even for surprising results is overshadowed however by somewhat differing apparent ages complicating a sound palaeoclimatic interpretation. A comparison of OSL and pIRIR ages obtained in BT poses a similar problem. OSL ages from quartz are prone to dose-dependent age underestimates but the critical absorbed dose may be grainsize-dependent. Experiences in BT resulted in favoring the fine grains from quartz, allowing for higher credible ages. Nevertheless, our quartz ages > ca. 50 ka are possibly but not necessarily underestimated, obviously dependent on the site and the providence of the quartz grains. In contrast, pIRIR ages turn out to be prone to overestimates due to incomplete bleaching leaving an unknown residual dose at deposition, a serious problem for beds with strong periglacial reworking.

Loess stratigraphy in Poland is well-based mainly on lithostratigraphy, palaeopedology, and periglacial geomorphology. Apart from – often problematic – radiocarbon dating and contradictory previous TL and OSL ages there is a lack however of independent physical dating methods and also of tephrostratigraphic markers. But at least the age of a prominent interstadial soil (or soil complex) now labelled L1SS1 at the end of the Middle Pleniglacial can now be fixed between ca. 30 and ca. 40 ka. Interpretation of dating results from samples older than L1SS1 is challenging. The observed diverging ages (OSL, pIRIR) are critical for the accurate time bracketing of geomorphologic and pedostratigraphic features such as ice wedging, thermokarst erosion events and interstadial soil formations and for their attribution to marine isotope stages. Alternative interpretations are discussed including possible periglacial mirroring of pre-LGM regional ice advances (Ristinge and Klintholm advances) in the southwestern Baltic Sea area.

I suggest that the strange behavior of quartz ages from different grain sizes is caused by various sources (ranging from Paleozoic crystalline rocks to Quaternary glacial drift) with very different geological and thermal histories, stored due to the very high resistance of quartz against weathering. Local and remote sources contribute to individual sedimentary beds of LPSs to varying extents. Thus, fine grains and coarser grains from an individual sample may be derived from diverse sources. In spite of the addressed uncertainties, for honesty reasons it is so far recommended aiming at age bracketing as narrowly as possible, simultaneously using OSL from different quartz fractions and pIRIR from fine polymineral grains. A refinement of this approach remains challenging as far as the sole reliable dating protocol is not ensured.

How to cite: Zoeller, L.: Ambiguity of luminescence ages from periglacial loess in Poland – “As you like it” or honesty with users?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1003, https://doi.org/10.5194/egusphere-egu23-1003, 2023.

EGU23-1396 | ECS | Posters on site | CL5.2

Tephra compositional data: are we doing it right? 

Simon Larsson and Matthew Bolton

Tephrochronology is often used for dating of natural archives and for correlation between study sites. Volcanic ashes (tephra) extracted from cores used for climate reconstructions function as common time-marker horizons and become anchor points in comparisons of age models from different studies. Given these uses, tephrochronology is well placed to help overcome the chronological challenges that hinder sufficiently precise dating of palaeoclimate records.

Tephras are identified based on their geographic and stratigraphic contexts, glass shard morphology, and geochemical composition. The geochemistry is most commonly analysed by electron probe microanalyser and presented as weight percentages of oxides of the nine or ten most abundant elements, often normalised to a 100 % total for ease of comparison. A simple exploration of such results and comparison to published data of previous tephra findings is usually enough for confident identification. However, compositional data of tephra findings from new studies continuously add to the complexity of tephrochronological investigations by increasing the amount of data available for comparison, including the addition of new potential candidates for identification. The increased likelihood of multiple candidates—sometimes with overlapping geochemistries—means that statistical data analyses are increasingly necessary.

Tephrochronologists have used principal component analysis and discriminant function analysis in situations needing statistical approaches, but these methods’ validity often requires certain assumptions not to be violated. A rarely considered example of such an issue is that compositional data suffers from the constant-sum constraint and must be converted by log-ratio transformations for some statistical analyses to function properly. As there is presently no consensus on a tephra compositional data curation procedure including log-ratio transformations, we have explored several variations and compared the results to see if a formal recommendation for such a procedure is relevant for the tephra community.

How to cite: Larsson, S. and Bolton, M.: Tephra compositional data: are we doing it right?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1396, https://doi.org/10.5194/egusphere-egu23-1396, 2023.

EGU23-1481 | Orals | CL5.2

How accurate are marine Δ14CDIC modelling approaches? 

Martin Butzin, Peter Köhler, Christoph Völker, Ying Ye, and Gerrit Lohmann

It has been estimated that Δ14C values of marine dissolved inorganic radiocarbon (Δ14CDIC) are primarily governed by transport and radioactive decay. This implies that Δ14CDIC can be considered as a radioconservative tracer which can be implemented into Earth system models without a full marine carbon cycle model. Here we evaluate the accuracies of the radioconservative modelling approach and of a further modelling approach which considers a different simplified representation of the marine radiocarbon cycle, presenting simulation results obtained with the ocean general circulation model FESOM and the marine biogeochemistry model REcoM. The relative uncertainties between the two simplified and the comprehensive treatments of the marine radiocarbon cycle are less than 5%. Therefore, the simplified Δ14CDIC modelling approaches should be sufficiently accurate for many marine radiocarbon studies. 

How to cite: Butzin, M., Köhler, P., Völker, C., Ye, Y., and Lohmann, G.: How accurate are marine Δ14CDIC modelling approaches?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1481, https://doi.org/10.5194/egusphere-egu23-1481, 2023.

EGU23-1551 | ECS | Posters on site | CL5.2

Continuous Radiocarbon Records by Laser Ablation – Status Report 

Melina Wertnik, Lukas Wacker, Nicolas Brehm, and Caroline Welte

The unique laser ablation (LA) setup at ETH Zurich (Switzerland), coupled to a MICADAS accelerator mass spectrometer (AMS), enables rapid 14C analyses and has been successfully employed for a broad range of carbonate archives such as stalagmites (Welte et al., 2021), otoliths (Andrews et al., 2019), and shells of Arctica islandica. An 193 nm ArF excimer laser is used to liberate CO and CO2 from the sample surface by ablation. The gas is then flushed with helium into the gas ion source of the AMS for online measurement.

Advantages of the novel techniques are a significant reduction in labour-intensive sample preparation and the speed of measurement, which minimises the expensive beam-time of the AMS. However, as a transient signal is measured where each sampling location is only measured for a short duration, uncertainties associated with LA-AMS are significantly higher than for conventional measurement techniques. Still, it is possible to locate strong signals such as a growth stop or the bomb spike very rapidly and precisely using only two scans of the sample. Here we present the status of the setup and progress on data reduction aimed at reducing the larger uncertainties. Preliminary results from comparisons of parallel tracks on a stalagmite allow testing the data reduction strategy and will be shown.

Andrews, A. et al. (2019), Marine and Freshwater Research, https://doi.org/10.1071/mf18265

Welte, C. et al. (2021), Climate of the Past, 17(5), 2165–2177, https://doi.org/10.5194/cp-17-2165-2021

How to cite: Wertnik, M., Wacker, L., Brehm, N., and Welte, C.: Continuous Radiocarbon Records by Laser Ablation – Status Report, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1551, https://doi.org/10.5194/egusphere-egu23-1551, 2023.

EGU23-2836 | ECS | Orals | CL5.2

The Role of Aged Organic Carbon in North Atlantic Fjord Sediments 

Craig Smeaton, Negar Haghipour, William Austin, and Timothy Eglington

Fjords are recognised as important hotspots for the burial and storage of organic carbon (OC) within their sediment, which potentially provides a long-term climate regulation service. Annually, it is estimated that 18 Mt of OC is buried within fjord sediments with between 55 – 62% of the OC originating from the terrestrial environment. The transfer of OC from the terrestrial environment to the fjord sediments is likely a significant pathway for aged OC to reach the coastal ocean. By estimating the quantity and mapping the spatial distribution of aged OC within the fjord sediments, we can develop a better understanding of the processes that govern the transfer of terrestrial OC from the catchment to the sediment of fjords, further constraining their role in long-term climate regulation.

Here we bring together radiocarbon analysis with isotopic and biomarker measurements to investigate the age of the surficial sediments within 46 fjords across the North Atlantic. The fjords in this study range from Scottish systems with catchments dominant with OC rich peat to the glaciated systems of Svalbard and Greenland.  The results from this analysis highlight that a multiple natural and anthropogenic processes govern the quantity and distribution of aged OC across North Atlantic fjords ranging between glacial input of fossil OC to the erosion of aged terrestrial material facilitated by deforestation.  This study highlights the fundamental need to understand the processes that govern the transfer of OC across the land-ocean interface to allow the role these marine sedimentary systems play in long-term climate regulation to be constrained.    

How to cite: Smeaton, C., Haghipour, N., Austin, W., and Eglington, T.: The Role of Aged Organic Carbon in North Atlantic Fjord Sediments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2836, https://doi.org/10.5194/egusphere-egu23-2836, 2023.

EGU23-2934 | ECS | Posters on site | CL5.2

Novel methods for determining the 14C age of microbially assimilated soil carbon 

Kari Finstad, Erin Nuccio, Katherine Grant, Jennifer Pett-Ridge, and Karis McFarlane

Soils are a significant component of the Earth’s carbon (C) cycle, yet a mechanistic understanding of what controls the turnover of this large C pool remains elusive. Microbial respiration of organic C accounts for roughly half of the total CO2 production from soils, though limited options exist for accurately identifying the source of C assimilated by microbial communities. Currently, radiocarbon (14C) analysis of evolved CO2 from soil incubations is the most common laboratory method for this, however they can introduce artifacts due to sample disruption and processing and can take months to produce sufficient CO2 for analysis. We present novel extraction methods which allow for the direct 14C analysis of microbial biomolecules and compare the results to laboratory incubations. Preliminary results suggest that in the upper 50 cm soil depths, the Δ14C from incubations is indistinguishable from that of extracted microbial biomass. Below 50 cm, the Δ14C of the microbial biomass is more depleted than that of the incubations, either due to the stimulation of labile C decomposition in the incubations, or the inclusion of biomolecules from non-living cells in the biomass extractions. Work is ongoing to identify the source of the extracted biomass pool and additional methods for isolating specific, short-lived biomolecules such as RNA, are underway to unambiguously determine the Δ14C of organic molecules being assimilated by active microbial communities.

How to cite: Finstad, K., Nuccio, E., Grant, K., Pett-Ridge, J., and McFarlane, K.: Novel methods for determining the 14C age of microbially assimilated soil carbon, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2934, https://doi.org/10.5194/egusphere-egu23-2934, 2023.

EGU23-4545 | Orals | CL5.2

Evaluating the accuracy of the Greenland Ice-Core Chronology (GICC) 

Sune Olander Rasmussen, Giulia Sinnl, Anders Svensson, and Bo Møllesøe Vinther

The full potential of palaeoclimate data relies on reliable time scales, i.e., a relation tying the physical dimension of the palaeoclimate archive with age. For many records, including ice cores, identification and counting of annual layers is the most direct and accurate way to obtain a time scale provided that high-resolution measurements of parameters showing annual variability are available. Annual-layer counting can provide very precise estimates of event durations and rates of change, but as errors accumulate with age, the accuracy decreases with depth/time. In contrast, radiometric methods often have good accuracy, and in principle, the two approaches can be combined to form highly accurate and precise time scales provided that the archives and their time scales can be robustly aligned. This can be done based on e.g. volcanic markers, common and correlatable features in cosmogenic isotope records, or on climatic wriggle-matching when the possible leads and lags between records is considered.

The Central Greenland ice cores are drilled in the interior areas of the ice sheet where precipitation rates are appropriate for the formation and preservation of annual layers, thereby allowing annual layers to be identified in the Holocene period and well into the last glacial period. The Greenland Ice-Core Chronology (GICC) is an attempt to derive a consistent, common time scale for the Greenland ice cores by combining data from multiple cores, using for each time period all available annually resolved data and then applying the time scale to the other cores by means of matching patterns of volcanic eruptions and other reference horizons. In this way, data from all the ice cores can be interpreted together on a common time scale (i.e., with very small relative dating uncertainty), greatly reducing the risk of artificial offsets due to misinterpretation of individual records. The first version of GICC, named GICC05, was published in 2006 and 2008, where the dating covered the time period back to 60 ka b2k, at which point the layers had thinned too much to continue with continuous annual layer counting.

Since then, high-resolution data from the newer Greenland ice cores NEEM and EGRIP have appeared, and comparisons to other palaeoclimate records on radiometric time scales have shown that in some sections, GICC05 was not as accurate as initially estimated, motivating a revision on the time scale. The top 3.8 ka of the time scale was recently revised, leading to changes in age of 10-15 years for the section older than 2500 years (see presentation by Giulia Sinnl). Here, we review the older sections of GICC05 in the context of other well-dated palaeoclimate archives and cosmogenic isotope records, as well as model-based estimates of climate leads and lags relevant when aligning climate records, and outline a plan for how to continue the revision of GICC05.

How to cite: Rasmussen, S. O., Sinnl, G., Svensson, A., and Vinther, B. M.: Evaluating the accuracy of the Greenland Ice-Core Chronology (GICC), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4545, https://doi.org/10.5194/egusphere-egu23-4545, 2023.

EGU23-6028 | Posters on site | CL5.2

Radiocarbon signatures of carbon phases exported by swiss rivers in the Anthropocene 

Timo Rhyner, Lisa Bröder, Margot White, Benedict Mittelbach, Florian Storck, Lucas Passera, Negar Haghipour, and Timothy Eglinton

Lateral carbon mobilization processes are particularly prone to anthropogenic perturbations due to human intervention of the land surface as well as aquatic corridors yet remain poorly constrained despite their importance as a key component of the C-cycle. A major source of this uncertainty involves processes modulating the sources and fate of carbon along the freshwater aquatic continuum. This study examines the radiocarbon (14C) signatures of particulate and dissolved organic carbon (POC, DOC, respectively) and dissolved inorganic carbon (DIC) transported by Swiss rivers with a view to assessing controls on the origin and cycling of carbon within corresponding watersheds. Twenty-one rivers were selected that span a range of watershed properties and are monitored by the National Long-Term Surveillance of Swiss Rivers (NADUF) program, enabling radiocarbon data to be interpreted within a broader hydrological and geochemical context.  Samples were collected during high-flow conditions in summer 2021, a year of extreme rain events. Average discharge of our sample set (n=21) was 299.76 +/- 513.87 m3/s, while the annual average discharge of all stations was 184.90 ± 264.92 m3/s. The range of D14C values of POC was -158‰ to - 446‰ (n = 21), while corresponding ranges of  D14C values for DOC and DIC were - 43‰ to - 377‰ and - 40‰ to - 301‰, respectively, indicating the presence of pre-aged carbon in all three pools. Hydrological properties such as discharge, runoff and precipitation did not appear as major significant controlling factors. Except for DI14C where annual average runoff of the past decade showed a significant negative correlation. Instead, based on Multivariate Regression Analysis, “alpine” variables such as mean basin elevation, slope, and barren areas were negatively correlated with D14C values of all three D14C-phases, while rivers draining lower elevation terrain, where agricultural land-use is more extensive were associated with higher D14C values in -the organic carbon pools (POC, DOC). Repeated sampling under different hydrological conditions and associated 14C (and 13C) measurements are being used to provide additional insights into the controls on the amount and nature of carbon exported by Swiss rivers, the interconnectivity between different carbon pools within the corresponding drainage basins and ecoregions, as well as to predict long-term trends in the context of changing climate and anthropogenic forcing.

How to cite: Rhyner, T., Bröder, L., White, M., Mittelbach, B., Storck, F., Passera, L., Haghipour, N., and Eglinton, T.: Radiocarbon signatures of carbon phases exported by swiss rivers in the Anthropocene, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6028, https://doi.org/10.5194/egusphere-egu23-6028, 2023.

EGU23-6579 | Posters on site | CL5.2

An empirical study on the variability of luminescence ages for coeval loess samples 

Daniela Constantin, Robert Begy, Dimitri Vandenberghe, Daniel Veres, and Alida Timar-Gabor

An increasing number of studies exploit the advantages of a single-aliquot regenerative-dose protocol (SAR) for equivalent dose determination with sampling at relatively closely-spaced vertical intervals (of the order of 10-30 cm). The resulting ages are, at least in principal, ideally suited for age-depth modelling. The modelling, however, is made difficult owing to the variety and complex combination of uncertainties associated with luminescence dating. Moreover, we previously reported on a variability in age results for coeval loess samples that is significantly larger than expected and remains to be understood.

In this study, we examine this problem explicitly by observing the degree of precision and accuracy that can be achieved by luminescence dating of multiple coeval loess samples of known age. The main goal is to improve our understanding of how luminescence ages are to be incorporated into age-depth models, thus increasing their robustness and accuracy.

Fourteen samples were taken at closely-spaced horizontal intervals from loess deposits immediately over- and underlying the Campanian Ignimbrite/Y5 tephra layer (40Ar/39Ar dated to 39.2±0.1 ka), as exposed at a section in the Lower Danube Basin in southeastern Europe. Luminescence analyses were carried out using the single-aliquot regenerative-dose (SAR) protocol and OSL signals from 63-90 µm quartz fraction. We report an average age of 46 ka for the samples collected below the tephra layer and 40 ka for the samples collected above it. The individual random and systematic uncertainties contributing to the individual ages vary from 1.9 % to 5.4 % and from 6.0 % to 6.1 %, respectively. We obtain an improved overall precision on the age of the sedimentary context by calculating the weighted average age and combining the individual random and systematic uncertainties following Aitken (1985, Appendix B). Thus we report weighted average ages of 46 ka and 40 ka for the horizontally sampled sediment layers intercalating the ash layer and associated overall random uncertainties of 1.3 % and 1.1 %. The overall systematic uncertainties are 6.1 % and 6.0 %. The insights gained from this are discussed in relation to age-modelling studies of luminescence-dated paleoclimate archives, and loess deposits in particular.

Keywords: luminescence dating; precision; random uncertainty; quartz

How to cite: Constantin, D., Begy, R., Vandenberghe, D., Veres, D., and Timar-Gabor, A.: An empirical study on the variability of luminescence ages for coeval loess samples, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6579, https://doi.org/10.5194/egusphere-egu23-6579, 2023.

EGU23-7006 | ECS | Posters on site | CL5.2

A global synthesis of speleothem radiocarbon data – is it a sensitive proxy for past ecosystem processes? 

Franziska A. Lechleitner, Christopher Day, Jens Fohlmeister, Sophie Warken, Norbert Frank, Heather Stoll, and Caroline Welte

Speleothems, secondary cave carbonate precipitates, can serve as tools to reconstruct past terrestrial ecosystem processes, particularly related to soil and vegetation. Radiocarbon, often in conjunction with other geochemical proxies, has been increasingly used for this purpose, as the speleothem reservoir effect retains useful information on local ecosystem conditions. On the other hand, speleothems are also of interest to the radiocarbon community as they can be dated very precisely with the U-Th method, which may allow the reconstruction of atmospheric radiocarbon levels in time if the reservoir effect remained constant.

Over the past decades, a growing number of speleothem radiocarbon records have been generated from vastly different climate zones and ecosystem types. While much progress has been made in the interpretation of these records, a unified and global view of the factors driving variability in speleothem radiocarbon is still lacking. We compiled a global dataset of averaged speleothem radiocarbon measurements, and provide a critical evaluation of the applicability of the radiocarbon reservoir effect as a proxy for past ecosystem conditions. We compare our dataset to geographic (latitude, elevation), climatic (temperature and precipitation), and ecosystem and geological parameters (soil and bedrock thickness, soil age, vegetation type, and land cover). Our preliminary results show that it is difficult to extract a strong globally relevant driving factor for the mean absolute value in the reservoir effect at the investigated cave sites, and highlights the importance of detailed reporting of local conditions.

To provide insight into the amplitude range of processes affecting published speleothem radiocarbon records we perform a series of numerical forward modeling experiments. We test how the effects of changing soil age, soil pCO2, carbonate dissolution regime, and pyrite oxidation affect carbon isotopes in stalagmites.

Together, the global synthesis and modeling experiments provide us with the first global overview of how cave site parameters and climate and ecosystem processes affect speleothem radiocarbon records, and allow us to assess the sensitivity of this proxy as a tool for past ecosystem conditions.

How to cite: Lechleitner, F. A., Day, C., Fohlmeister, J., Warken, S., Frank, N., Stoll, H., and Welte, C.: A global synthesis of speleothem radiocarbon data – is it a sensitive proxy for past ecosystem processes?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7006, https://doi.org/10.5194/egusphere-egu23-7006, 2023.

EGU23-7936 | ECS | Posters on site | CL5.2

Sources of cave CO2 at Milandre cave, Switzerland constrained through multipool analysis of 14C and δ13C. 

Sarah Rowan, Marc Luetscher, Sönke Szidat, Thomas Laemmel, Oliver Kost, and Franziska Lechleitner

The cycling of subsurface karst CO2 is not well constrained in terms of its source and transportation pathway. The classical model suggests that cave CO2 is produced by the respiration of soils and vegetation in the catchment. In contrast, several new studies have proposed that the dominant source of CO2 is from the respiration of older organic matter situated deeper within the karst, or from the degassing of supersaturated drip water.

We present over a year of monitoring data from Milandre cave, northern Switzerland, whereby we evaluated the 14CO2 and δ13CO2 composition of the atmosphere in the cave catchment, catchment soil gas, well gas, and cave air. Drip waters located throughout the cave also underwent various analysis. The cave 14CO2 is more depleted compared to the soil and gas samples. The Keeling plot intercept of atmospheric and cave δ13CO2 is ~-26‰, indicating a dominant contribution from biological respiration. The dissolved inorganic carbon from various cave drips have an F14C from ~ 0.84 to 0.96 and δ13C from ~ -16‰ to -11‰. F14C and δ13C are inversely correlated.  Considering both the 14C and δ 13C results, this suggests either a source of CO2 from an aged reservoir of respiring organic matter contributing to the cave gas or substantial influence from degassing of 14C fossil carbonate CO2 from drip water. These results have implications for the understanding of the subterranean carbon cycle and the interpretation of speleothem carbon isotope records for paleoclimate studies.

How to cite: Rowan, S., Luetscher, M., Szidat, S., Laemmel, T., Kost, O., and Lechleitner, F.: Sources of cave CO2 at Milandre cave, Switzerland constrained through multipool analysis of 14C and δ13C., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7936, https://doi.org/10.5194/egusphere-egu23-7936, 2023.

The surficial 10 cm of Scotland’s saltmarshes are estimated to store 1.35 ± 0.33 Mt CO2 equivalent, approximately 3.37% of Scotland’s national greenhouse gas emissions in 20201,2. This is largely achieved through effective preservation of organic matter (OM) in low oxygen, sulphidic soils1. Saltmarshes gain organic carbon (OC) through in-situ (autochthonous) production by vegetation and benthic microalgae, and the accumulation of marine and terrestrial material during tidal inundation (allochthonous)3.

A key blue carbon challenge is to empirically understand, under current and predicted warmer conditions, the sources of OC accreted into and respired from saltmarshes. This can determine the proportion of the total OC pool which is additional through in-situ sequestration or from increased preservation of allochthonous OM3. Alongside 13C and 15N isotopes, radiocarbon (14C) analysis/dating can be used to determine the sources of saltmarsh surficial soil OC4.

We hypothesise that at ambient temperatures the younger and more labile, and predominantly autochthonous OM, will be preferentially decomposed.  But at elevated temperatures the aged, and predominantly allochthonous, OM pool will increasingly contribute to the respired greenhouse gases.

To test this hypothesis, we collected soil cores and surficial sediment samples from three contrasting Scottish saltmarshes. We analysed them for 14C to gain an understanding of the age and sources of the autochthonous and allochthonous OM accumulating. We also aerobically incubated sub-samples of the soil in temperature-controlled experiments at 11.1 ± 1°C (ambient) and 20 ± 1°C (elevated). The evolved CO2 was collected on molecular sieve traps and analysed for 14C content/age.

Our results will facilitate comparison of the age of the bulk OM and the respired CO2 to the thermogravimetrically measured reactivity of the OM determined using the recently developed Carbon Reactivity Index5. We will present our findings and introduce our ongoing work on anaerobic incubations of the same soils, which includes the novel measurement of the evolved 14CH4.

Our research contributes to a growing evidence base for emissions from saltmarshes, and the sources of OC accreting in their soils, which is vital for understanding how they cycle carbon and their ability to mitigate climate change. It will contribute to the creation of saltmarsh carbon cycle models and inform work to include saltmarshes in the UK’s Nationally Determined Contributions.

References

  • Smeaton C, Burden A, Ruranska P, et al. Using citizen science to estimate surficial soil Blue Carbon stocks in Great British saltmarshes. Front Mar Sci. 2022;9. Accessed November 28, 2022. https://www.frontiersin.org/articles/10.3389/fmars.2022.959459
  • Scottish Goverment. Scottish Greenhouse Gas Statistics 2020.; 2022. https://www.gov.scot/publications/scottish-greenhouse-gas-statistics-2020/
  • McTigue ND, Walker QA, Currin CA. Refining Estimates of Greenhouse Gas Emissions From Salt Marsh “Blue Carbon” Erosion and Decomposition. Front Mar Sci. 2021;8. Accessed January 26, 2022. https://www.frontiersin.org/article/10.3389/fmars.2021.661442
  • Hajdas I, Ascough P, Garnett MH, et al. Radiocarbon dating. Nat Rev Methods Primer. 2021;1(1):1-26. doi:10.1038/s43586-021-00058-7
  • Smeaton C, Austin WEN. Quality Not Quantity: Prioritizing the Management of Sedimentary Organic Matter Across Continental Shelf Seas. Geophys Res Lett. 2022;49(5):e2021GL097481. doi:10.1029/2021GL097481

How to cite: Houston, A., Austin, W., and Garnett, M.: A Novel Method for Radiocarbon Dating Greenhouse Gas Emissions from Saltmarsh Soils to Address Key Blue Carbon Challenges, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8033, https://doi.org/10.5194/egusphere-egu23-8033, 2023.

EGU23-8148 | ECS | Posters on site | CL5.2

Using the radiocarbon bomb spike to constrain the age of soil organic carbon delivered to Lake Constance sediments. 

Benedict V.A. Mittelbach, Margot E. White, Timo Rhyner, Stephan Wartenweiler, Negar Haghipour, Martin Wessels, Thomas M. Blattmann, Nathalie Dubois, and Timothy I. Eglinton

The residence time of carbon in terrestrial ecosystems, such as soils and freshwater, sets the pace of the terrestrial carbon cycle. Understanding export pathways and turnover times of soil organic carbon (OCSoil) is crucial to assess responses to climate and land use changes. Our study aims to quantify the average turnover time of OCSoil in the catchment of perialpine Lake Constance. Lake sedimentary sequences integrate organic carbon from their catchment and aquatic primary productivity. They act as both burial sites of organic carbon (OC) and time series archives of catchment processes. Thus, they can bridge the gap between plot scale observations, e.g., on soil carbon turnover, and observations made at the outlet of major river systems.

Sedimentary organic carbon sources include aquatic primary productivity, OCSoil, and rock-derived (petrogenic) OC. Stable carbon isotopes (δ13C) can be used to identify the relative contribution of these pools. The 5700-year half-life of radiocarbon (14C) coupled with the atmospheric nuclear bomb spike in the early 1960s can be used to infer the age and turnover rate of the OC pools on millennial to annual timescales. Bulk OC isotope analysis of a varved sediment core spanning the past ca. 110 years at quasi-annual resolution was used to constrain the age of soil carbon delivered to Lake Constance. We combined the geochemical data with a Markov-Chain-Monte-Carlo-based approach to identify the most probable age structure of aquatic and soil-derived OC components and to quantify their respective contributions in addition to petrogenic OC.

Radiocarbon analysis of sedimentary bulk OC reveals a well-defined but muted bomb spike in the early 1960s. However, bulk Δ14COC values remain below 0‰, implying a predominance of aged OC. Based on the δ13C-based three-component linear mixing model, we found these values to be the result of an OC mixture containing approx. 40% pre-aged soil carbon and up to 20% fossil petrogenic carbon.  Accounting for these inputs, we estimated that soil-derived OC delivered to Lake Constance is centennial in age, implying interim storage prior or subsequent to erosion from the landscape.

How to cite: Mittelbach, B. V. A., White, M. E., Rhyner, T., Wartenweiler, S., Haghipour, N., Wessels, M., Blattmann, T. M., Dubois, N., and Eglinton, T. I.: Using the radiocarbon bomb spike to constrain the age of soil organic carbon delivered to Lake Constance sediments., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8148, https://doi.org/10.5194/egusphere-egu23-8148, 2023.

EGU23-8195 | Orals | CL5.2

Lateglacial to interglacial sediment infills in Alpine valleys: timing, sediment provenance and paleo-environmental conditions 

Pierre Valla, Yann Rolland, Romain Delunel, Julien Carcaillet, and Christian Crouzet

Glacial/interglacial transitions in mountainous areas are marked by significant glacier retreat from forelands to inner massifs, resulting in large-scale and ephemeral lake formation that are subsequently filled (or not) by sediment transfer during lateglacial to postglacial times. When valley paleo-infills are preserved, they form precious archives to investigate (1) Alpine erosion dynamics and paleo-environmental conditions during key transition periods from full glacial stages to interglacials, and (2) glacial erosion patterns during susbequent glaciation.

In this contribution, we investigate such sedimentary deposits (locally called as "banquettes") in the French western Alps, and more precisely along the Isère valley and Val du Bourget. Previous research have attributed these deposits to the Riss – Würm transition due to their position under a basal compact till and to the MIS 6/5 transition up to early MIS 4 from palynological constraints, although no absolute ages has been available so far. Based on existing mapping of their spatial distribution and stratigraphic reconstructions, we sampled coarse-sand and sandy-gravel layers within these deposits for constraining both sediment deposition time (OSL dating) and provenance (glacial/postglacial origin, using terrestrial cosmogenic nuclide TCN 10Be in quartz). In addition, their spatial distribution provides estimates of maximum glacial erosion during the last glacial cycle, which can be subsequently used as spatial constraints for ice model predictions.

Our results confirm deposition times of these sedimentary units at the MIS 6/5 transition, with dating constraints from the late MIS 6 (ca. 145 ka) to the early MIS 5 (Eemien, 115-130 ka) for sandy layers. Upper sandy-gravel layers have younger deposition ages of ca. 80 ka, illustrating sediment fluxes at the transition from late MIS 5 to early MIS 4. We compare this temporal sequence to more recent sediment infills of the Isère valley (14C and OSL dating) during the Lateglacial to Holocene (MIS 2/1) transition. TCN data from sand samples also illustrate the sharp transition from full glacial to interglacial conditions, with a significant increase in 10Be concentrations from Lateglacial to post-glacial sediments. We propose that the observed signal can reflect changes in erosion rates, but also in glacier expansion or in paleo-environmental conditions, with export of stored subglacial sediments as well as the re-establishment of sediment/soil production and transfer along the catchment routing system following glacier retreat.

How to cite: Valla, P., Rolland, Y., Delunel, R., Carcaillet, J., and Crouzet, C.: Lateglacial to interglacial sediment infills in Alpine valleys: timing, sediment provenance and paleo-environmental conditions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8195, https://doi.org/10.5194/egusphere-egu23-8195, 2023.

EGU23-8323 | ECS | Orals | CL5.2

Using radiocarbon to identify the impact of climate and mineralogy on soil organic matter turnover 

Margaux Moreno Duborgel, Luisa Isabell Minich, Negar Haghipour, Beatriz González-Domíngez, Timothy Eglinton, and Frank Hagedorn

Soils are the largest carbon (C) reservoir in terrestrial ecosystems. There are still numerous uncertainties concerning the fate of soil organic carbon and its feedback on climate change. Radiocarbon is a useful approach to better understanding the carbon cycle. The nuclear weapon testing in the 1960s induced a peak in 14C atmospheric concentration – a signal that can be used to trace the incorporation and turnover of C in soil. By separating the soil in different fractions and measuring the 14C in them, we can quantify how much C and for how long is stored in soils, and where soil organic carbon is stabilised.

Our study aimed at identifying the impact of climate and mineralogy on soil organic matter turnover on a regional scale. We analysed C pools and 14C contents in the organic layer, mineral soil (0-20cm) and its fractions from 54 sites across Switzerland. These 54 sites are systematically spread across natural climatic and geological gradients and were repeatedly sampled in the 1990s and 2014. The mineral soil was incubated for 181 days and 14C was measured in the respired CO2. The mineral soil was fractionated according to density into particulate organic matter (POM) and mineral-associated organic matter (MAOM). We then oxidised the mineral-associated organic matter with hydrogen peroxide to remove its labile fraction of carbon. Our 14C dataset was analysed together with ancillary data comprising soil properties and climatic variables from the studied sites.

Our radiocarbon dataset showed that the carbon that was respired from the mineral soil originated predominantly from particulate organic matter. The bomb spike signal was incorporated in the organic layer and in the particulate organic matter, while the mineral-associated organic matter had turnover times on centennial to millennial time scales (from 94 to 3060 years). Further chemical oxidation of MAOM using hydrogen peroxide revealed a stronger depletion in radiocarbon of the residual fraction with Δ14C values ranging between -173 ‰ and -47 ‰. This indicates that the MAOM is a mixture of 14C-enriched organic matter and very old material.

With respect to the controlling factors of soil organic matter turnover time, the radiocarbon signature of the POM is most strongly affected by climatic variables such as mean annual temperatures. In contrast to POM, the mineral-associated organic matter, comprising the greatest pool of soil organic carbon is driven by chemical soil properties. For instance, older 14C ages are found in acidic soils with low pH values ranging between 3 and 4. In these soils, Al and Fe oxides concentrations are high. We showed that the concentrations of pedogenic oxides in the soil correlate with soil organic carbon concentrations in the mineral-associated organic matter. In soils with higher pH (>7), we can also find old 14C ages. In these soils, C is stabilised by interactions with calcium ions and carbonates.

Overall, our regional scale dataset shows that the net accumulation of labile soil organic matter seems to be climate sensitive, while mineralogy and weathering contribute most significantly to the stabilisation of organic carbon in the soil.

 

 

How to cite: Moreno Duborgel, M., Minich, L. I., Haghipour, N., González-Domíngez, B., Eglinton, T., and Hagedorn, F.: Using radiocarbon to identify the impact of climate and mineralogy on soil organic matter turnover, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8323, https://doi.org/10.5194/egusphere-egu23-8323, 2023.

EGU23-8974 | Posters on site | CL5.2

New developments in techniques for the sampling and analysis of atmospheric 14CO2 and 14CH4 at ETHZ and UNIBE, Switzerland 

Soenke Szidat, Thomas Laemmel, Dylan Geissbühler, Sarah Rowan, Philip Gautschi, Franziska Lechleitner, and Lukas Wacker

Radiocarbon (14C) measurements of atmospheric greenhouse gases such as carbon dioxide (CO2) and methane (CH4) are central in our capability to identify their provenance. The 14C content of these gases provides more insight into the age of their sources and mainly allows the distinction between fossil and modern ones. 14CO2 measurements can be used to analyze the nature of anthropogenic emissions (mostly fossil), or to discern on what organic matter pool respiration is taking place in a given environment. 14CH4 can also be used to detect anthropogenic emissions (from leaks of natural gas, for example) as well as natural emissions produced by methanogenesis, for example from ruminants or in wetlands.

The 14C analysis of atmospheric gases is made challenging due to their usual low concentration. Thus making the use of appropriate sampling methods, preconcentration and extraction techniques necessary to reach a sufficient amount of carbon for Accelerator Mass Spectrometry (AMS) analysis. We propose here a general view of the techniques that were developed at the Laboratory for Ion Beam Physics (ETHZ, Zurich), and at the Laboratory for the Analysis of Radiocarbon with AMS (UNIBE, Bern) for the purpose of analyzing CO2 and CH4 in atmospheric samples. We then discuss the practicability and the potential bias introduction of each of them.

The techniques are as follows :

  • Automated Graphitization Equipment with Automated Loading Facility (AGE-ALF)
  • Automated Graphitization Equipment with Cryogenic Trap (AGE-CT)
  • Methane Preconcentration and Purification System (MPPS)

Generally, samples were collected in sampling bags, either in 5-15L capacity for CO2 or larger than 60L for CH4. Types of samples that are considered are atmospheric CO2 and CH4 samples, CO2 from soil respiration, and CO2 from cave air. The different techniques are presented, and 14C results from standard gases are compared between the extraction lines and two MICADAS AMS systems at ETHZ and UNIBE.

How to cite: Szidat, S., Laemmel, T., Geissbühler, D., Rowan, S., Gautschi, P., Lechleitner, F., and Wacker, L.: New developments in techniques for the sampling and analysis of atmospheric 14CO2 and 14CH4 at ETHZ and UNIBE, Switzerland, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8974, https://doi.org/10.5194/egusphere-egu23-8974, 2023.

EGU23-9064 | ECS | Orals | CL5.2

Paleoclimate and weathering on volcanic islands: insights from well-dated paleosols spanning the last Myr in the Central Azores 

Francisco Hevia-Cruz, Anthony Hildenbrand, Nathan D. Sheldon, François Chabaux, Fernando O. Marques, Julie Carlut, and Vittorio Zanon

Paleosols (PSs) contain valuable information about the climatic conditions under which they formed and constitute an outstanding archive of past weathering processes. Nevertheless, paleosol dating over most of the Quaternary remains challenging. Volcanic environments are unique sites for such purposes, as precise radiometric age determination can be achieved on volcanic units ‘bracketing’ PSs. Here, we present a combined geochemical and geochronological study of PSs spanning the last Myr in the Central Azores archipelago (Pico, Faial and São Jorge Islands; central North Atlantic). Precise K-Ar dating of lava flows on groundmass separates (unspiked Cassignol-Gillot technique) yield ages with a typical uncertainty of a few kyr, allowing us to tightly constrain PS ages and weathering rates near key paleoclimatic transitions. PS geochemistry further allowed us to reconstruct weathering conditions and estimate Mean Annual Precipitation and Temperature (MAP & MAT) by two proxies previously validated for other volcanic terranes (CIA-K and Clayeyness).

Four periods of PSs formation are constrained at 870-845 ka, ~725 ka, 320-280 ka and 130-45 ka. Most PSs formed just after interglacial peaks, with a few exceptions. Our MAP reconstructions are variable (600-1,500 mm/yr), but generally lower than current annual precipitations (~1,000 mm/yr). MAT estimates (14-28°C) are higher than present-day annual temperatures (~17.5°C). MAP & MAT variations are in general agreement with global climatic curves; the highest values (28°C, 1,500 mm/yr) are reached at ~855 ka, coinciding with an interglacial peak. The younger PSs (130-45 ka) indicate more stable MAP & MAT in the ranges 650-1,000 mm/yr and 15-20°C, respectively and seem to show a temperature decrease after the MIS5e interglacial stage.

Most paleosols were formed in a few kyr under high MAT (>17°C) and moderate to high MAP (>700 mm/yr), supporting a major influence of temperature on weathering kinetics. Parental material texture also had an important role, as several PSs formed upon pyroclastic deposits over most of their depth, whereas those developed on lava flows were generally restricted to the highly fragmented upper brecciated parts. Minimum vertical soil formation rates are in the range of ~0.3-4.5 cm/kyr, with a mean of ~1.7 cm/kyr and an outlier around ~10 cm/kyr. Those generally high values can be explained by the highly vesicular parental material, and by an exceptionally feldspar-rich (easily weathered) parental rock for the outlier.

As current precipitation and temperatures are higher than the threshold values of ~700 mm/yr and ~17°C under which most PSs formed, enhanced soil formation is expected for the near future, especially in the context of global warming and particularly in volcanic contexts. This may have important and fast impacts on local human activities, but also regarding CO2 consumption by rock weathering and geological hazards.

How to cite: Hevia-Cruz, F., Hildenbrand, A., Sheldon, N. D., Chabaux, F., Marques, F. O., Carlut, J., and Zanon, V.: Paleoclimate and weathering on volcanic islands: insights from well-dated paleosols spanning the last Myr in the Central Azores, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9064, https://doi.org/10.5194/egusphere-egu23-9064, 2023.

EGU23-10967 | ECS | Posters on site | CL5.2

Initial radiocarbon (14C) results of compound class persistence across a climate gradient in California grassland soils 

Katherine Grant, Marisa Repasch, Kari Finstad, Taylor Broek, Jennifer Pett-Ridge, and Karis McFarlane

Soils mediate the rapid cycling of carbon through the critical zone. Soil organic carbon (SOC) is composed of a complex mixture of plant and microbial derived organic compounds with distinct cycling timescales. The residence time of individual SOC components depends on a combination of factors, including compound reactivity, mineral association, and climate conditions, making it difficult to accurately quantify. However, radiocarbon analysis of specific compound classes can disentangle the mixture of SOC ages within a single sample. We modified methods to measure the Δ14C of distinct compound classes (lipids, amino acids, and carbohydrates) from bulk and physically fractionated grassland soils. Additionally, we measured the Δ14C of the water-extractable fraction (WEOC) and the residual acid-insoluble fraction. Samples were collected from a series of grassland meadows across California ranging in climatic conditions including temperature and precipitation. Sites include grassland meadows in Angelo Coast Range Reserve, Hopland Extension Reserve and Sedgwick reserve, and which receives 2160, 940, and 380 mm yr-1 of rainfall and is dominated by Avena spp. We sampled 1m soil pits by ~10cm intervals to study changes in SOC persistence with depth. We used solid state 13C-NMR to measure the relative abundance of the target compound classes in soil. The Δ14C of bulk soil decreased from about +50‰ to about +10‰ in the O-horizons to a range of about -150‰ to about -650‰ in the deepest horizons. At the Hopland site, the clay fraction (<63μm) had higher Δ14C values than both the bulk (<2mm) and sand (<2mm to >63μm) fractions. WEOC Δ14C values ranged from modern to about -45.6‰. Δ14C values of total extracted lipids ranged from 36±4‰ at the surface to -215±3‰ at depth. Quantifying the age distribution of distinct compound classes gives a direct measurement of the persistence between these phases.

How to cite: Grant, K., Repasch, M., Finstad, K., Broek, T., Pett-Ridge, J., and McFarlane, K.: Initial radiocarbon (14C) results of compound class persistence across a climate gradient in California grassland soils, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10967, https://doi.org/10.5194/egusphere-egu23-10967, 2023.

EGU23-11287 | ECS | Orals | CL5.2

14C-based deconvolution of relationships between carbon pools in Icelandic rivers and streams 

Nora Gallarotti, Lisa Bröder, Julie Lattaud, Negar Haghipour, and Timothy Eglinton

Rivers are important agents in the lateral transfer of carbon from terrestrial to the marine realm, thus forming a key component of the global carbon cycle. Carbon sources and transformations along the land-ocean aquatic continuum are dynamic with a complex interplay between dissolved and particulate, and inorganic and organic carbon pools. Elucidating interrelationships between these pools is hindered by multiple sources and processes that influence the carbon signatures of these pools in a dissimilar fashion. Icelandic streams and rivers offer an opportunity to directly assess the fluvial carbon pool dynamics due to the virtual absence of sedimentary rocks (e.g., shales, carbonates with a radiocarbon dead signature) that otherwise “muddy the waters” with respect to apparent sources and turnover times.

In order to characterize carbon transport patterns of Icelandic rivers and streams, we collected water samples from 43 river systems with watersheds that cover a wide range of catchment properties such as size, water discharge, climate as well as landcover. Here we assess the concentrations as well as the isotopic composition (13C, 14C) of particulate and dissolved organic carbon (POC; DOC, respectively) as well as dissolved inorganic carbon (DIC) alongside stable water isotopes (δ2H, δ18O) and major ion geochemistry.
Radiocarbon content (reported as fraction modern; F14C) of POC, DOC and DIC show similar patterns: lower F14C values (i.e., highest radiocarbon ages) are mostly associated with glacial runoff while higher F14C values (younger carbon) correspond to higher soil organic carbon content within the respective catchment. This dataset is but a first glimpse at carbon transport patterns in Icelandic rivers. Biomarker concentrations and isotopic compositions such as leaf waxes (n-alkanes, n-alkanoic acids) and soil derived lipids (branched glycerol dialkyl glycerol tetraether) will be used to further investigate provenance, transport and storage mechanisms in the diverse suite of Icelandic catchments.

How to cite: Gallarotti, N., Bröder, L., Lattaud, J., Haghipour, N., and Eglinton, T.: 14C-based deconvolution of relationships between carbon pools in Icelandic rivers and streams, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11287, https://doi.org/10.5194/egusphere-egu23-11287, 2023.

EGU23-11860 | Posters on site | CL5.2

A new UV-Oxidation set up for AMS radiocarbon analysis for small dissolved organic carbon in marine and fresh water samples 

Negar Haghipour, Maarten Lupker, Lukas Wacker, Margot White, Lisa Bröder, and Timothy I. Eglinton

Radiocarbon measurements of dissolved organic carbon (DOC) can give us valuable information about origin and age of DOC, a major, yet little understood component in the global carbon cycle. One way to measure DOC in water is to remove dissolved inorganic carbon first, oxidize organic carbon with UV irradiation and ultimately analyses the formed inorganic CO2 for 14C. The main challenge of UV-Oxidation (UVox) methods is to extract the typically low concentrations of DOC with low blanks required for relatively high precision 14C measurements. A disadvantage of currently used UVox methods is that only one sample can be oxidized in a laborious process at the same time in large volume. Here we present a UV-Oxidation system where up to 12 water samples can be oxidized simultaneously in 12 separate quartz reactors arranged around a single UV lamp in a compact setup. The simple setup further uses helium instead of vacuum typically used by conventional extraction lines to speed up the extraction of the formed CO2 after oxidation. The key improvements of the new UVox setup are: 1) Reduced amount of water needed (30- 60 ml) as samples are measured for 14C with the Micadas gas ion source., 2) UV oxidation efficiency for standards is high (96%), 3) No KI trap is needed, 4) Required time for sample preparation of up to 12 samples is 4-6 h, 5) combined the CO2 from different reactors to one trap.  We obtained 2.6 ± 0.6 µgC with F14C= 0.27±0.05 for processing blank.  We will present the first measurments of DOC samples from Swiss lakes, Canadian Beaufort Sea and the reproducibility of the line.

How to cite: Haghipour, N., Lupker, M., Wacker, L., White, M., Bröder, L., and Eglinton, T. I.: A new UV-Oxidation set up for AMS radiocarbon analysis for small dissolved organic carbon in marine and fresh water samples, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11860, https://doi.org/10.5194/egusphere-egu23-11860, 2023.

EGU23-12735 | Orals | CL5.2

14C analysis of atmospheric methane: development of a portable sampling system 

Giulia Zazzeri, Lukas Wacker, Negar Haghipour, Philip Gautschi, and Heather Graven

Measurements of radiocarbon (14C) in atmospheric methane (CH4) provide a powerful tool to distinguish fossil from biogenic methane emissions, because fossil methane is completely devoid of 14C. However, these measurements are particularly challenging as CH4 is at low concentration in the atmosphere and large volumes of air must be sampled.

At the Laboratory of Ion Beam Physics (LIP), ETH, we developed a portable sampler based on the laboratory prototype in Zazzeri et al. 2021 [1]. The new system enables extraction of carbon from CH4 while sampling in the field, reducing the sample processing in the laboratory and allowing collection of a hundred liters of air onto a 0.5 g zeolite trap.

Here we present an overview of the sampling system and the technical developments that have been implemented at LIP. The relatively small size of the sampler and its interface with the gas ion source of the AMS system make 14CH4 measurements much easier to perform. Its portability will enable collection of CH4 samples in any environment, with the potential of assessing the radiocarbon signature of methane emissions that have not been yet characterized.

[1] Zazzeri, G., Xu, X., & Graven, H. (2021). Environmental Science & Technology, 55(13), 8535-8541.

How to cite: Zazzeri, G., Wacker, L., Haghipour, N., Gautschi, P., and Graven, H.: 14C analysis of atmospheric methane: development of a portable sampling system, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12735, https://doi.org/10.5194/egusphere-egu23-12735, 2023.

EGU23-14183 | ECS | Posters on site | CL5.2

Radiocarbon constraints on lateral export of soil organic carbon in rivers of Switzerland 

Alexander Brunmayr, Heather Graven, Timo Rhyner, Margaux Moreno Duborgel, and Negar Haghipour

Lateral carbon transport through inland waters plays a critical yet often overlooked role in the delicate balance of carbon exchanges controlling the net uptake and storage of anthropogenic carbon in terrestrial ecosystems. Though new terrestrial carbon cycle models are increasingly making an effort to explicitly represent these traditionally neglected lateral fluxes, the parameters governing lateral carbon transport, particularly the composition and ages of exported soil carbon, remain ill-constrained. In this study, we explore the power of combined river and soil 14C datasets as a parameter constraint when calibrating a novel carbon cycle model connecting the terrestrial and riverine systems in catchments of Switzerland. For the riverine data, we use 14C measurements of particulate organic carbon (POC), dissolved organic carbon (DOC) and dissolved inorganic carbon (DIC) for water samples collected during high-discharge events in 2021 across Switzerland. Within those river catchments, we have forest soil 14C data at various depths down to 60cm for up to three samples in time (mid 1990s, 2014, and 2022). The soil samples were split into the following representative fractions: soil dissolved organic carbon (soil-DOC), particulate organic carbon (soil-POC), and mineral-associated organic carbon (soil-MOC), which represents the older and more recalcitrant component of soil carbon. This study investigates to what extent using these fraction-specific 14C measurements together with 13C and nitrogen data for both rivers and soils allows us to not only distinguish the different sources of riverine carbon but further analyze the composition and age of the soil organic carbon ending up in Swiss rivers.

How to cite: Brunmayr, A., Graven, H., Rhyner, T., Moreno Duborgel, M., and Haghipour, N.: Radiocarbon constraints on lateral export of soil organic carbon in rivers of Switzerland, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14183, https://doi.org/10.5194/egusphere-egu23-14183, 2023.

EGU23-1405 | Posters on site | G5.2

Variability of GNSS PWV in global tropics over different time scales 

Zofia Bałdysz, Grzegorz Nykiel, Dariusz B. Baranowski, and Beata Latos

The variability of water vapour in the global tropics has impacts on global circulation patterns through atmospheric teleconnections. Various timescales of its fluctuations strongly affect weather, including interannual to daily changes. Although traditional techniques of water vapour measurements have always been vital in understanding complex thermodynamic processes, they still face some limitations related to e.g. temporal sampling, non-automatic data collection, or cost efficiency. In light of this, global navigation satellite systems (GNSS) can state for a valuable source of precipitable water vapour (PWV) data. Taking advantage of a long time series of collected by International GNSS Service (IGS) observations, we performed an analysis of the variability of 18-year GNSS PWV over the tropics, from interannual to daily time scales. Results have proved, that the GNSS technique is capable of capturing long-term changes in PWV resulting from climate modes, such as El Nino Southern Oscillations or Indian Ocean Dipole. Additionally, analysis of diurnal GNSS variability, together with satellite-based precipitation and cloudiness data, taken from the Tropical Rainfall Measurement Mission gridded dataset (TRMM 3B42 v7) and the global, merged infrared (IR) dataset, have enabled reliable estimation of changes that are in line with various regimes of tropical deep convection.  In particular, our results show that the diurnal cycle of PWV and TB were almost entirely dominated by mono-modal distributions. The diurnal cycle of precipitation onshore (continental areas or big islands; continental regime) had a single late afternoon peak, and that offshore (small islands; oceanic regime) had both a midday and a nocturnal peak. The daily amplitude phase shift of PWV and precipitation at onshore stations with a continental regime consistently occurred at the same time, while TB maximum peaked about five hours later. Furthermore, results show that the daily mean and the amplitude of the diurnal cycle of PWV, precipitation, and TB appeared smaller on offshore stations, exhibited to an oceanic regime, than on onshore, continental stations.

How to cite: Bałdysz, Z., Nykiel, G., Baranowski, D. B., and Latos, B.: Variability of GNSS PWV in global tropics over different time scales, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1405, https://doi.org/10.5194/egusphere-egu23-1405, 2023.

Global long-term stable wind fields are valuable information for climate analyses of atmospheric dynamics. Given shortcomings of available observations their monitoring remains a challenging task. One promising option for progress are radio occultation (RO) satellite data, where the winds are estimated using the geostrophic approximation. Hence, in this study we focus on two goals, explored through European Re-Analysis ERA5 and RO datasets, using monthly-mean January and July data over 2007-2020 with 2.5° × 2.5° resolution. First, we compare actual and geostrophic ERA5 wind speeds to evaluate the validity of the geostrophic approximation. Second, we test how well ERA5 and RO geostrophic winds agree. We find the geostrophic approximation to work well within 2 m/s accuracy almost globally (5°-85° latitude), especially over the summer hemisphere; larger differences (up to about 5 m/s) may occur in the winter stratosphere. We noticed the effect of large mountain ranges on the wind flow as a wave-like pattern, also in the difference between RO and ERA5 geostrophic winds, pointing to effects of different geopotential height estimations. Generally, RO and ERA5 geostrophic winds showed very good agreement. In the long-term, systematic differences in decadal trends of higher than 0.5 m/s per decade were found at subtropical latitudes, mainly related to observing system changes in the year 2016 that influenced ERA5. Together with the validity of the geostrophic approximation, this indicates that the long-term stability of RO-derived wind field monitoring can provide added value to reanalysis winds, for the benefit of climate monitoring and analyses.

How to cite: Danzer, J., Nimac, I., and Kirchengast, G.: Validation of the geostrophic approximation and the potential of long-term radio occultation data for wind field monitoring, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1442, https://doi.org/10.5194/egusphere-egu23-1442, 2023.

EGU23-2615 | Orals | G5.2

Fast observation operator for GNSS tropospheric gradients 

Florian Zus, Rohith Thundathil, Galina Dick, and Jens Wickert

Raw data collected at a single Global Navigation Satellite System (GNSS) station allow the estimation of the Zenith Total Delay (ZTD) and the tropospheric gradient. In order to make use of such data in Numerical Weather Prediction (NWP) the observation operators must be developed. Our current observation operator for tropospheric gradients is based on a linear combination of ray-traced tropospheric delays (Zus et al., 2022). Although this observation operator is tuned for high speed and precision it remains difficult to be implemented into NWP Data Assimilation (DA) systems. In this contribution we introduce a simple and fast observation operator which is based on the closed-form expression depending on the north–south and east–west horizontal gradients of radio refractivity (Davis et al., 1993). We run the Weather Research and Forecasting (WRF) model (horizontal resolution of 10km) and find that for the considered geographical region (central Europe) and time period (summer season) the root-mean-square deviation between the tropospheric gradients calculated by the fast and original approach is about 0.15 mm. In essence, the observation operator error is non negligible but acceptable for assimilation. In a first step we implemented the developed operator in our experimental DA system (Zus et al., 2019) and run a series of experiments to check the usefulness of the new approach. We present results from this assimilation experiments where we utilize both simulated and real observations. In the next step we will implement the fast observation operator in the WRF DA system in support of the research project EGMAP (Exploitation of GNSS tropospheric gradients for severe weather Monitoring And Prediction).

Davis, J., Elgered, G., Niell, A., and Kuehn, K.: Ground-based measurement of gradients in the “wet” radio refractivity of air, Radio Sci., 28, 1003–1018, 1993. 

Zus, F.; Douša, J.; Kačmařík, M.; Václavovic, P.; Dick, G.; Wickert, J. Estimating the Impact of Global Navigation Satellite System Horizontal Delay Gradients in Variational Data Assimilation. Remote Sens. 2019, 11, 41.

Zus, F., Galina, D., and Wickert, J.: Development of a cost efficient observation operator for GNSS tropospheric gradients, EGU General Assembly 2022, Vienna, Austria, 23–27 May 2022, EGU22-1079

How to cite: Zus, F., Thundathil, R., Dick, G., and Wickert, J.: Fast observation operator for GNSS tropospheric gradients, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2615, https://doi.org/10.5194/egusphere-egu23-2615, 2023.

EGU23-2992 | Posters virtual | G5.2

Multi-source water vapor tomography based on ray-tracing technique 

Ming Shangguan, Meng Dang, and Xu Cheng

GNSS water vapor tomography has proven to be a near-real-time cost-effective method to obtain the three-dimensional distribution of atmospheric water vapor. Many previous studies have used various methods to derive the GNSS water vapor tomography. However, the number and distribution of GNSS signals limit the accuracy and spatial resolution of GNSS water vapor tomography, which could cause an ill-posed inverse problem. This study tries to use multi-source observations (GNSS, MODIS and ERA5) in Hongkong with the help of the ray-tracing technique to increase the number of signals and voxels crossed by rays for the water vapor reconstruction. Water vapor tomography are derived based on multi-source data and validated with the radiosonde data. Experimental results demonstrate that the proposed method is helpful to improve the quality of water vapor tomography.

How to cite: Shangguan, M., Dang, M., and Cheng, X.: Multi-source water vapor tomography based on ray-tracing technique, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2992, https://doi.org/10.5194/egusphere-egu23-2992, 2023.

Continuously operating reference stations (CORS) are widely used to provide near realtime estimates of zenith tropospheric delays and tropospheric gradients to be assimilated in numerical weather models. Due to the latest evolution of global satellite navigation systems and ground based augmentation services, it became feasible to estimate the 3D distribution of wet refractivities in near realtime.

This paper presents a near realtime tomographic reconstuction algorithm utilizing the zenith tropospheric delays and tropospheric gradients obtained from the processing of several GNSS networks in Hungary (HU), Slovakia (SK), Romania (RO) and Ukraine (UK). The estimated zenith tropospheric delays (ZTDs) and tropospheric gradients are used to restore the slant wet delays (SWD) affecting the observed satellite-receiver range. The SWDs are used as input for a tomographic reconstruction algorithm based on the multiplicative algebraic reconstruction technique. The developed software tool includes a stepwise outlier detection module to select the most reliable slant wet delays for the tomographic reconstruction. It provides the wet refractivities in a pre-defined voxel model on an hourly basis over the HU-SK-RO-UA cross-border region.

The derived refractivity profiles have been validated with radiosonde observations. The results show that our GNSS tomography approach could reconstruct the refractivities with the standard deviation of 5 ppm below 3 km of altitude, while the standard deviation decreased to the level of 0.3 ppm at the altitude of 10 km.

The estimated tropospheric delays as well as the refractivity profiles are made available online to the meteorologists community in Little-R format and can be directly assimilated in the Weather Research & Forecast numerical model.

 

How to cite: Rozsa, S., Turak, B., and Khaldi, A.: Near realtime tomographic reconstruction of atmospheric water vapour using multi-GNSS observations in Central Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4465, https://doi.org/10.5194/egusphere-egu23-4465, 2023.

EGU23-5596 | ECS | Posters on site | G5.2

Troposphere Monitoring Based on Crowdsourced Smartphone GNSS Data 

Yuanxin Pan, Grzegorz Kłopotek, Markus Rothacher, Linda See, Rudi Weinacker, Tobias Sturn, Ian McCallum, Vicente Navarro, and Benedikt Soja

Global Navigation Satellite System (GNSS) is an essential tool for troposphere monitoring. Currently, GNSS meteorology depends mainly on the data from geodetic receivers of global or regional networks. However, these geodetic-grade GNSS stations are costly, and thus cannot be densely deployed, especially in less developed regions. Since the release of the Android 7 operating system in 2016, Android smartphones can be used to collect raw GNSS data. Considering that nowadays there are about 3 billion Android smartphones worldwide, a smartphone GNSS data crowdsourcing campaign was launched on March 17th 2022 as a part of the CAMALIOT project. About 5 TB of raw GNSS observations were collected around the world by more than 12 thousand users of the CAMALIOT Android application. In this contribution, we highlight the results related to the dedicated pipeline developed to process the crowdsourced smartphone GNSS data. Firstly, all the collected data were classified by a machine learning-based model to disregard observations of low quality. It was found that only about 2% of the collected data could potentially be used for troposphere delay estimation. The high-quality observations were then processed in the relative-positioning mode by forming baselines with the nearby geodetic stations. Several crowdsourced data sets were used to demonstrate that the zenith wet delays (ZWD) derived from smartphone data could achieve an accuracy of better than 10 mm. However, uncalibrated phase center variations of the smartphone antennas and multipath errors are still the main limitations to further improve the ZWD estimation. Overall, our study indicates that crowdsourced smartphone GNSS data is promising to densify the existing GNSS networks in terms of troposphere monitoring.

How to cite: Pan, Y., Kłopotek, G., Rothacher, M., See, L., Weinacker, R., Sturn, T., McCallum, I., Navarro, V., and Soja, B.: Troposphere Monitoring Based on Crowdsourced Smartphone GNSS Data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5596, https://doi.org/10.5194/egusphere-egu23-5596, 2023.

Precipitable water vapor PWV is one of the major greenhouse gases. Monitoring Long-term variations in water vapor concentrations, which have a direct effect as a greenhouse gas and involve amplifying other feedbacks such as albedo and clouds. Monitoring of Precipitable water vapor on a continuous and steady basis has become possible over the recent decades due to the increased ground-based GPS receivers at global scale. However, the High Atlas Mountains remained a data-void zone until recently, when some ground-based GPS receiving stations were deployed to monitor geodynamic movements in the High Atlas belt. This paper investigates seasonal changes in precipitable water vapor, moisture transport, and precipitation over the central High Atlas using data from three ground-based GPS (FSSM, OUCA, and TIOU), Aeronet (AErosol RObotic NETwork) (Saada), GPCP, and NCEP reanalysis II over seven years (2016 to 2022). The ZTD (Zenith Tropospheric Delay) and the PWV results using the GipsyX/RTGx software show significantly better results than the Aeronet PWV measurements based on the acquired data. The reanalysis and observations are in good correlation regarding moisture transport and precipitation. Precipitable water increases in late summer, but precipitation peaks in winter and spring over the central high atlas.

Keywords: Precipitable water vapor, GPS, Zenith total delay, Aeronet, NCEP.

How to cite: Lakhouidsi, K. and Fadil, A.: Seasonal-scale atmospheric water cycle study using ground-based GPS receivers, Aeronet, and NWP models over the central High Atlas Mountains (Morocco), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6426, https://doi.org/10.5194/egusphere-egu23-6426, 2023.

GNSS interferometric reflectometry is a well-established technique in Ocean Remote Sensing that can be used for the retrieval of sea surface characteristics. In particular, the evaluation of interference patterns in GNSS signal-to-noise ratio (SNR) observations allows for an estimation of the Significant Wave Height (SWH), e.g. by relating the SWH to the attenuation that is typically present in the oscillating interference pattern for increasing elevation angle of the signal-emitting GNSS satellite.

Recently, we developed new machine learning methods for the analysis of GNSS SNR observation data obtained from the research platform FINO 2 in the Baltic Sea. The core element thereof is the extraction of various engineered features from SNR interference patterns  by means of kernel regression and clustering techniques. The various engineered features were used as input for the prediction of the SWH with supervised machine learning models (artificial neural networks, bagged regression trees, linear models). In a case study, these predictions provided a remarkable improvement in accuracy compared to predictions which solely use a common feature stemming from the aforementioned attenuation in the SNR interference pattern.  

However, an optimized extraction of information from the various and partially redundant engineered features for the prediction task is desirable, aiming at the reduction of model complexity without reducing predictive performance. This goal is successfully addressed in the present work by applying a forward selection scheme and a principal component analysis for the set of available  engineered features. The usage of the engineered features can also be optimized by tuning the hyperparameters of complex supervised machine learning models used for the SWH prediction. Such a tuning is performd by means of a grid search for a random forest model applied to the engineered features. This optimization represents an advancement of the application of the bagged regression trees with an improvement in accuracy of the respective SWH predictions.

The improved methods for SWH prediction at FINO2 are outlined and the impact of the involved optimizations concerning the use of the engineered features is evaluated and discussed in detail in a case study.

How to cite: Becker, J. and Roggenbuck, O.: Optimized Use of Engineered Features from GNSS Reflectometry for Prediction of Significant Wave Heights , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8052, https://doi.org/10.5194/egusphere-egu23-8052, 2023.

EGU23-8800 | ECS | Orals | G5.2

Sensing the tropospheric water vapor from grazing-angle Spaceborne GNSS-R 

Yang Wang and Jade Morton

In this work, we investigate a novel method to estimate the tropospheric wet delay, and further the vertically integrated water vapor (VIWV) and its horizontal gradients, using the coherent-reflection GNSS signals received by a CubeSat in the low-Earth orbit (LEO).  It can complement existing observation approaches over some polar and ocean regions where GNSS signals can be coherently reflected.

The precise altimetry using coherent-reflection GNSS signal carrier phase measurements has gained popularity over the past couple of decades for the observation of ocean, sea ice, lake, and river surfaces.  The troposphere delay error is found to be a major error source for GNSS-R phase altimetry, especially at a low elevation angle.  However, if we can model the reflection surface elevation relatively well, then the estimated residual phase from GNSS-R signal can be dominantly contributed by the mis-modeled tropospheric wet delay, and GNSS-R signal can become a new data source for tropospheric water vapor sensing.  The GNSS-R approach can observe the horizontal gradients of VIWV along the specular point (SP) track, as the SP moves at high speeds of ~5 km/s, and the spatial resolution is 10s of km by ~1 km.

In the presentation, we will provide examples using Spire Global’s grazing-angle GNSS-R data and comparisons with the ECMWF reanalysis VIWV data.  We will also discuss the applicable regions, performance, and error mitigations of the proposed method in estimating tropospheric wet delay and issues to be addressed in the further retrieval of VIWV.

How to cite: Wang, Y. and Morton, J.: Sensing the tropospheric water vapor from grazing-angle Spaceborne GNSS-R, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8800, https://doi.org/10.5194/egusphere-egu23-8800, 2023.

EGU23-9059 | Posters virtual | G5.2

Water vapour monitoring over France using the low-cost GNSS collaborative network Centipede 

Pierre Bosser, Julien Ancelin, Marianne Métois, Lucie Rolland, and Maurin Vidal

In recent years, the significant growth of positioning applications has come with the development of low-cost dual frequency Global Navigation Satellite Systems (GNSS) receivers. Such receivers allow high precision positioning to be achieved. They are becoming increasingly popular for geosciences as they allow for large numbers of equipment at affordable prices. 

Founded in 2019, the Centipede network is a collaborative permanent GNSS network that aims to offer free real-time centimetric positioning to any user. The network is currently made up of more than 330 low-cost reference stations located mainly in France and has nearly 500 regular users. Since July 2022, the GNSS raw data acquired by the stations forming this network have been archived by the Réseau National GNSS (RENAG) scientific network data centre in order to evaluate their suitability for geosciences applications such as tectonic, sea-level monitoring, troposphere and ionosphere studies. 

In this study, we present a first evaluation of the use of this dataset for the retrieval of integrated water vapour content (IWV) over five months in 2022. Troposphere delays are estimated from a PPP analysis and are converted to IWV using a standard procedure. Then, the IWV are compared with those retrieved for GNSS stations from the “conventional” French permanent GNSS networks, the Réseau GNSS Permanent (RGP) and RENAG. The results of these comparisons are conclusive, with root mean square differences in the range of 0.5-2 kg/m2 and high correlations of the time series registered by nearby low-cost and geodetic-class receivers. 

These results confirm the high potential of low-cost GNSS networks. The development of such network is a real opportunity for geoscience applications, particularly in poorly instrumented areas.  In such areas, their contribution could be especially significant for meteorological or climatological applications for which the monitoring of water vapour by GNSS is widely used. 

How to cite: Bosser, P., Ancelin, J., Métois, M., Rolland, L., and Vidal, M.: Water vapour monitoring over France using the low-cost GNSS collaborative network Centipede, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9059, https://doi.org/10.5194/egusphere-egu23-9059, 2023.

EGU23-9910 | ECS | Posters on site | G5.2

Tropospheric tomography – integration of ground- and space-based GNSS observations 

Natalia Hanna and Robert Weber

On the way transmitter-receiver, the Global Navigation Satellite Systems (GNSS) signal is attenuated and delayed by the presence of water vapor. This information serves as the input to the GNSS tomography - a robust technique in water vapor estimation concerning its amount and distribution in the troposphere.

GNSS rays pass through the tomographic grid built over a dense network of ground-based GNSS stations. Due to the constant movement of the GNSS satellites influencing their elevation angle and visibility, the measurement geometry varies in time. The model elements are either over or under-determined during the chosen time span within the area of interest; hence, the system of observation equations is mixed-determined.

However, to enhance the tomographic solution, the model can be supplied with additional data, e.g., from the radio occultation (RO). The RO technique provides the space-based signal delay between the low Earth orbit (LEO) and GNSS satellites. Products obtained from the RO measurements consist of bending angles and vertical dry- and wet-atmosphere data.

In this study, we analyze the COSMIC-1 radio occultation events in the tomographic domain located in the Netherlands in February 2018. The observation system in the ATom GNSS software was extended with the space-based wet refractivity profiles (level 2 data). We compare the obtained 3D wet refractivity field to the GNSS ground-based-only tomographic solution and the radiosonde measurements. The drawbacks and potential development of the applied solution are also discussed.

How to cite: Hanna, N. and Weber, R.: Tropospheric tomography – integration of ground- and space-based GNSS observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9910, https://doi.org/10.5194/egusphere-egu23-9910, 2023.

The Global Navigation Satellite System (GNSS) is an all-weather, high-precision space geodetic technique that can solve positioning results while providing high-precision tropospheric products. Abundant studies have demonstrated the positive impact of traditional ground-based GNSS on numerical weather prediction using data assimilation tools. As tropospheric profile information is promisingly to satisfy the increasing data demand for improving short-range forecast accuracy, it is very important to obtain and assimilate high accuracy, high spatial and temporal resolution, and three-dimensional GNSS tropospheric products. Fortunately, the aerial vehicle market is booming and represented by unmanned aerial vehicle, providing convenient platforms for obtaining richer GNSS tropospheric products at different position and heights. However, there are still some key challenges in processing and assimilating GNSS tropospheric products from such highly dynamic platforms. In our study, we firstly improve the accuracy of aerial-based GNSS tropospheric products up to millimeter level by applying a new data processing method which optimizes the stochastic constraint for GNSS zenith wet delay. Thereafter, we evaluate the impact of those high spatial and temporal tropospheric products on meteorological application by assimilating them into numerical weather models. Experiments are conducted to prove the feasibility of aerial-based GNSS meteorology and point out some topics for further investigation.

How to cite: Zhang, Z., Zhang, W., and Lou, Y.: High-precision tropospheric product processing and meteorological application based on GNSS observations from aerial-based highly dynamic platforms, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10506, https://doi.org/10.5194/egusphere-egu23-10506, 2023.

This study examined the impact of the vertical shapes of water vapour on GNSS atmospheric observations. The standard model used in GNSS measurements to represent the vertical distribution of water vapour is a natural logarithm function based on the water vapour scale height. This model is effective in describing the variation of vertical structure of water vapour below the water vapour scale height (similar to the atmospheric boundary layer). However, in very humid conditions, it is important to measure water vapour above the water vapour scale height to predict whether a heavy rain system will persist. The presentation will discuss the characteristics of the vertical structure and an improved model for these structures.

How to cite: Fujita, M.: Sensitivity of water vapor vertical shape in GNSS atmospheric observation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10661, https://doi.org/10.5194/egusphere-egu23-10661, 2023.

EGU23-10991 | Posters virtual | G5.2

Enabling subfield scale soil moisture mapping in near real-time by recycling L-band GNSS signals from drones 

Mehmet Kurum, Mehedi Farhad, Volkan Senyurek, and Ali Gurbuz

Accurate measurement of soil moisture (SM) at high spatiotemporal resolutions is one of the critical challenges of site-specific precision agriculture. Traditionally SM is measured manually or using in-situ SM probes scattered in the field. Although these observations are generally accurate and reliable up to the sensitivity level of the SM probe, it is very time-consuming, costly, and inefficient for large heterogeneous fields to acquire high-resolution SM measurements. Over the last several decades, microwave remote sensing approaches have become popular for measuring spatially distributed SM. Several space-borne missions, such as SMAP and SMOS, have been launched to provide surface SM measurements globally. Although all current satellite missions and their SM products are critical for many large-scale research and studies, their coarse spatial resolution (about 40km) makes it impractical for precision agriculture applications.

 

To enable subfield scale soil moisture mapping in near real-time, our team has recently developed an unmanned aircraft systems ( UAS) -based multi-sensory system with Global Navigation Satellite System (GNSS) reflectometry (GNSS-R), a multispectral camera, and a LIDAR. A down-facing GNSS antenna with a ground plane blocks the direct GNSS signals, and it collects reflected carrier-to-noise density ratio (C/N0) measurements from multiple specular points on the ground for each visible GNSS satellite. The multispectral camera provides spectral images in blue, green, red, red edge, and near-infrared (NIR) bands. The LIDAR offers a 3D representation of the surface and vegetation. Such a comprehensive dataset has been collected in a field under different management practices for the last three years. The study field was organized with a split-plot arrangement and was planted with corn and cotton as the main crops. We have performed 581 flights over the study field and collected more than 4 TB of data, including visual and multispectral images and LIDAR point clouds. More than 2.5 million L-band reflection samples have been collected over the field. In addition, in-situ SM and intense manual SM observations over the field have been collected as ground truth information.

 

Observed GNSS-R data is dependent not only on the SM but also on the vegetation, surface roughness, topography, soil texture, GNSS satellites' positions, transmitter characteristics, receiver orientation, and flight parameters through a combination of linear and nonlinear relations. To learn such a relationship, we developed a machine learning (ML) model using multiple sensory input features for high-resolution, low-cost, and easily accessible SM mapping for precision agriculture. In this study, we will present the multi-year field campaigns and the development of the ML framework with convolutional and fully connected neural network layers for SM mapping that can utilize multiple imageries jointly with other physical and microwave data and calculate features relevant to SM. During the model development, site and time-independent cross-validation methods are used for better model generalization and performance evaluation.

How to cite: Kurum, M., Farhad, M., Senyurek, V., and Gurbuz, A.: Enabling subfield scale soil moisture mapping in near real-time by recycling L-band GNSS signals from drones, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10991, https://doi.org/10.5194/egusphere-egu23-10991, 2023.

EGU23-13749 | ECS | Posters on site | G5.2

3D ground and space-based ray tracing tomography model – methodology and implementation 

Adam Cegla, Witold Rohm, Paweł Hordyniec, Gregor Moeller, Estera Trzcina, and Natalia Hanna

One of the indispensable elements of high-resolution weather forecast systems is the provision of reliable initial conditions using observations. Among the methods for collecting meteorological data, besides the quality of measurements, their time and space variability play a crucial role. Hence, GNSS observations stand out as stable, bias-free alternatives for weather stations, radiosondes, or microwave satellites.

Current studies of GNSS observations in weather forecasting give promising results. However, the observations themselves are subject to errors due to their geometry, mainly caused by insufficient vertical and horizontal resolution. Therefore, applying them in an operational forecasting model is challenging. A possible way to solve this is to integrate space and ground-based observations into one tomography model.

The solution should be able to detect local, extreme weather phenomena with repeatable uncertainty and high numerical stability. Hence, we propose a precise 3D ray tracing solution for effective simulations of the ray path between the GNSS satellite and the GNSS receiver (Low Earth Orbiting LEO satellite), along with the ground receiver. Although, the combination of these results in one computationally efficient and stable model is a complex task.

The following step is the 3D ray tracing simulation integration into a modified TOMO2 operator dedicated to the tomography of 3D wet refractivity fields. The ray tracing module collects information on ray points’ refractivity and distance traversed in models’ voxels along the ray path. Then delivers it to mutual observational matrices for ground- and space-based simulations. 

This study focuses on the methodology of integrated tomography modeling.  Results are compared to the ground-based only GNSS tomography solution and validated with radiosondes profiles. The case studies are based on severe weather events in Poland with RO data delivered by SPIRE company and GNSS ground-based observations produced by UPWr. Numerical Weather Model input comes from European Centre for Medium-Range Weather Forecasts (ECMWF) ERA5.

How to cite: Cegla, A., Rohm, W., Hordyniec, P., Moeller, G., Trzcina, E., and Hanna, N.: 3D ground and space-based ray tracing tomography model – methodology and implementation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13749, https://doi.org/10.5194/egusphere-egu23-13749, 2023.

EGU23-14626 | ECS | Orals | G5.2

A generic approach to parameterize the scaling properties of atmospheric delays in InSAR time-series 

Gert Mulder, Freek van Leijen, and Ramon Hanssen

The observed phase in time-series of Interferometric Synthetic Aperture Radar (InSAR) products is a combination of primarily differential topography, line-of-sight displacement and atmospheric delay contributions. These components need to be disentangled to derive accurate atmospherical products from InSAR. However, isolating the atmospheric component from InSAR has been proven difficult as it is spatiotemporally highly dynamic and a superposition of two atmospheric states.

Here we propose an approach to parameterize the stochastic properties of the single-epoch atmospheric delay field as a way to represent the atmospheric signal in InSAR.

We found that the atmospheric signal of a time-series of interferograms can be characterized by structure functions, which can be used to isolate the single-epoch structure functions. Using two isotropic and three anisotropic scaling parameters it is then possible to construct a structure function characterizing the atmospheric signal per SAR acquisition. Especially, the isotropic parameters for the small scale and large scale atmospheric delay variations, can be used to characterize the atmospheric signal. For a test set of 150 Sentinel-1 acquisitions, this results in a difference in signal strength of the InSAR atmospheric signal with a factor of about 10 for small scale and 50 for large scale variations.

Our parametrization demonstrates that the scaling properties of the InSAR atmospheric signal for different SAR acquisitions are very similar and can be described using only five parameters. After parameter estimation we can then provide time-series of the expected atmospheric signal using distance and direction only for any combination of points within the InSAR image.

 

How to cite: Mulder, G., van Leijen, F., and Hanssen, R.: A generic approach to parameterize the scaling properties of atmospheric delays in InSAR time-series, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14626, https://doi.org/10.5194/egusphere-egu23-14626, 2023.

EGU23-14654 | ECS | Posters on site | G5.2

Ionospheric Impact on GNSS Reflectometry in the Tropical Region: A Simulation Study with NEDM model 

Mario Moreno, Maximilian Semmling, Mainul Hoque, and Jens Wickert

The ionosphere is a layer of Earth's upper atmosphere that is ionized by solar radiation. It plays a crucial role in the propagation of Global Navigation Satellite System (GNSS) signals, as these signals pass through the ionosphere on their way from the GNSS satellite to the receiver. The irregularities in the ionospheric electron density may have a significant impact on the GNSS signals, causing delays and phase and amplitude scintillations.

GNSS reflectometry (GNSS-R) is a promising technique for atmospheric sounding. Multiple studies have been successfully conducted in the recent decade by using GNSS-R ground-based, airborne and spaceborne data e.g., to estimate ionospheric disturbances from the reflected signals. However, further investigations are needed to precisely characterize ionospheric effects for GNSS-R altimetric applications.

This study presents simulation results of ionospheric delay for reflection events in tropical regions. The first-order ionospheric effects are estimated along the ray paths by deriving the slant total electron content from the Neustrelitz Electron Density Model (NEDM). The geometry of the simulated events refers to reflectometry records of the SPIRE satellite constellation and the satellite navigation system GPS on 2021/03/01.

Initial analysis has shown promising results. As solar activity increases (indicated by solar radio flux F10.7 index), an increase in the total ionospheric phase delay is evident.  Between 0h and 8h local time, there is a delay of 2 to 10 meters. For the time interval from 8h to 16h, the delay is from 14 up to 22 meters, with the maximum at noon. In the sunset period from 16h to 24h, the ionospheric delay reduces from 9 to 3 meters, respectively. The height above the Earth’s surface at which the highest amount of electron content is found along the ray path is ~290 km. This altitude corresponds to the F-region which has the highest concentration of free electrons. The analyzed events correspond to elevation angles from 5 to 30 degrees. The highest ionospheric delay is found at elevation angles between 10 and 20 degrees also depending on the local time.

How to cite: Moreno, M., Semmling, M., Hoque, M., and Wickert, J.: Ionospheric Impact on GNSS Reflectometry in the Tropical Region: A Simulation Study with NEDM model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14654, https://doi.org/10.5194/egusphere-egu23-14654, 2023.

EGU23-16054 | Orals | G5.2

Assessment of parameters describing the signal delay in the neutral atmosphere derived from VGOS sessions 

Rüdiger Haas, Periklis-Konstantinos Diamantidis, Gunnar Elgered, Jan Johansson, Tobias Nilsson, and Tong Ning

The VLBI Global Observing System (VGOS) is the next generation VLBI system for geodetic and astrometric VLBI. It has been designed by the International VLBI Service for Geodesy and Astrometry (IVS) to improve the accuracy and precision of the estimated geodetic parameters by one order of magnitude compared to the so-called legacy S/X VLBI system. During the VGOS design phase, small-scale and rapid variations in the signal propagation delay caused by the neutral atmosphere were identified as one of the major limiting error sources in terms of accuracy of geodetic VLBI. Performing as many observations as possible per time unit to cover the local sky at the stations as uniformly as possible, has been developed as a strategy to address this topic. The VGOS idea is to achieve this goal by employing fast-slewing radio telescopes ,of typically 12–13 m diameter, that are equipped with broad-band receiving devices of reasonably high sensitivity and digital backends with high sampling capability. Compared to standard S/X legacy VLBI sessions, at least a factor of two in the number of observations per station is currently achieved within operational VGOS sessions (VO). Dedicated VGOS Research and Development (R&D) sessions (VR) achieve an even larger number of observations through minimizing the scan lengths.

VGOS is still in its build-up phase and by 2022 the VGOS operational network has reached 10 internationally distributed stations. Among those is the Onsala Space Observatory which is operationally active with its VGOS twin telescopes since 2019. We analyse VGOS sessions of both VO- and VR-series and assess the current ability of VGOS to sense small-scale, rapid variations in the signal propagation delay caused by the neutral atmosphere. We compare the VGOS-derived results to corresponding results from simultaneous observation with co-located instrumentation at VGOS sites, i.e. receiving equipment for Global Navigation Satellite System (GNSS) observations. For the Onsala station we compare also to the results derived from the ground-based microwave radiometer.

How to cite: Haas, R., Diamantidis, P.-K., Elgered, G., Johansson, J., Nilsson, T., and Ning, T.: Assessment of parameters describing the signal delay in the neutral atmosphere derived from VGOS sessions, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16054, https://doi.org/10.5194/egusphere-egu23-16054, 2023.

EGU23-17311 | Orals | G5.2

Assessing long-term ZTD trends for climate 

Marcelo C. Santos, Jordan Rees, Kyriakos Balidakis,, Anna Klos, and Rosa Pacione

In this presentation we showcase results of an ongoing effort to assess long-term ZTD trends for eventual use in climate models, either for assimilation or validation. We have been analyzing the ZTD time series estimated from six REPRO3 IGS Analysis Centers (ACs), namely, COD, ESA, GFZ, GRG, JPL, TUG, to compare their long-term trends. Long-term here means 20 years or longer. About thirty stations have been selected globally for this purpose. The estimated ZTD time series have gone through a process of homogenization using ERA-5 derived ZTDs as reference. The homogenized data is then averaged to daily values to minimize potential influences coming from different estimation strategies used by individual ACs. As mentioned, our interest is with the long-term signal. Similar averaging is applied to the ERA-5 ZTDs. Two combinations, using weighted mean and (a robust) least median of squares, are being generated from the six homogenized ACs. The combinations serve as quality control to each ACs. Analysis of the trends generated from each one of the seven ZTD times series is performed looking at their similarities in both time and frequency domains. Results obviously vary depending on the geographical location. For example, for station ALBH, in Canada, inter-AC scatter is 0.47 mm/decade for the trends, 0.11 mm for the annual amplitudes, and 0.29 degrees for the annual phase. 

How to cite: C. Santos, M., Rees, J., Balidakis,, K., Klos, A., and Pacione, R.: Assessing long-term ZTD trends for climate, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17311, https://doi.org/10.5194/egusphere-egu23-17311, 2023.

EGU23-638 | ECS | Posters on site | AS5.13

Assessing the variability in emissions from crop residue burning in north India using remote sensing data 

Apoorva Yadav, Santosh Kumar Sasanapuri, Hitesh Upreti, and Sailesh N. Behera

Open biomass burning is the major cause for air pollution in north India, particularly in the months around the harvest of the major crops viz. rice and wheat. Crop residue burning, in the two agricultural powerhouse states of Punjab and Haryana, is major contributor for emissions from open biomass burning in the region. A district-wise emission inventory is needed to quantify the variations of crop residue burning emissions within various districts of Punjab and Haryana. In this study, bottom-up approach is used to determine the spatial variation of these emissions. In this approach, burned area is detected by using two MODIS satellite data products i.e., MODIS burned area product (MCD64A1) having resolution of 500m and MODIS active fire product (MOD14A1) having spatial resolution of 1km which can detect fires up to 1/20 of a pixel. Combining these two products the small fires data can also be detected and the accuracy in detection of burned area is improved. After detecting the burned area, the emissions of major pollutants were estimated in grids of (3×3) km2 during 2008-2017 in order to analyze their spatial and temporal variability. Also, the emissions for the study region are estimated using top-down approach where the crop residue burned is determined using IPCC guidelines and the comparison is done using both the approaches.

In Punjab, the average emissions of PM2.5, PM10, CO2 & CO are 153.3 Gg, 173.6 Gg, 21185.7 Gg, 1791.6 Gg, respectively during 2008-17 using top-down approach. During 2008-2017, the average emissions of PM2.5, PM10, CO2 & CO are 117.2 Gg, 120.7 Gg, 18859.9 Gg, 1133.7 Gg, respectively using bottom-up approach. The major contribution of emissions in Punjab is from Sangrur district followed by Patiala and Ludhiana district.  In Haryana, the average emissions of PM2.5, PM10, CO2 & CO are 68.9 Gg, 78.0 Gg, 9518.4 Gg, 804.9 Gg, respectively during 2008-17 using top-down approach. During 2008-2017, the average emissions of PM2.5, PM10, CO2 & CO are 28.2 Gg, 26.4 Gg, 5214.0 Gg, 214.0 Gg, respectively using bottom-up approach. The major contribution of emissions in Haryana is from Fatehabad district followed by Karnal and Kaithal district. For Haryana, the peak emissions during 2008-17 are in the month of May and November and for Punjab the peak emissions are in the month of October and November. From the results, it is observed that the top-down approach overestimates the emissions when compared to the bottom-up approach. For example, the CO2 emissions calculated using top-down approach is 1.1 and 1.8 times higher than the bottom-up approach for Punjab and Haryana, respectively. This is because a fixed value of fraction of biomass burnt is taken to estimate the amount of crop residue burned from the crop production values instead of accounting for area which are actually burned.

The development of the longer term emission inventory from crop residue burning may provide useful information for policy making on air pollution control in the region.

How to cite: Yadav, A., Sasanapuri, S. K., Upreti, H., and Behera, S. N.: Assessing the variability in emissions from crop residue burning in north India using remote sensing data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-638, https://doi.org/10.5194/egusphere-egu23-638, 2023.

EGU23-1096 | ECS | Posters on site | AS5.13

Assessment of aerosols over five cities of Angola based on MERRA-2 reanalysis data 

Pascoal Campos, José Pires, and Anabela Leitão

The use of Aerosol Optical Depth (AOD) has been proven as an alternative to the traditional ground-level monitoring of air quality in many countries across the world. Therefore, this study based on MERRA-2 data aims: (i) to characterize the spatiotemporal and component variations of aerosols in the atmosphere over the capital cities (Luanda, Sumbe, Benguela, Huambo and Lubango) of the five most densely populated provinces of Angola from 2010 to 2020; (ii) to analyze the relationship between the monthly mean variation of the total AOD and the meteorological parameters (precipitation, temperature, wind speed, and relative humidity) in those five cities; and (iii) to assess the influence of emissions from the Nyamuragira volcano, located in the Democratic Republic of Congo, on the air quality at the five cities. The most significant contribution to the total AOD was derived from organic carbon, in all the cities, whereby the highest values (0.19 - 0.23) were in Luanda. Ranges of sulphates across the coastal cities were higher when compared to the interior cities caused by the emissions inventory data. The value of AOD in all the cities increased and reached the peak during the dry season. The HYSPLIT model showed that air masses from Nyamuragira at various heights in November 2011 reached Luanda and Sumbe, and CALIPSO could confirm the existence of volcanic aerosols in this same period. This study allowed to conclude that the variability of AOD loading depends on seasons and regions, thus providing a little more information about the matter.

How to cite: Campos, P., Pires, J., and Leitão, A.: Assessment of aerosols over five cities of Angola based on MERRA-2 reanalysis data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1096, https://doi.org/10.5194/egusphere-egu23-1096, 2023.

EGU23-1112 | ECS | Posters on site | AS5.13

COVID-19 Pandemic Hopeful Prospect: Air Quality Improvements over Indo-Gigantic Plain 

Saadia Hina, Farhan Saleem, and Muhammad Ibrahim

The COVID-19 pandemic has received enormous attention worldwide due to its environmental, and societal impacts. The present study highlights the spatio-temporal variations in air quality parameters (AOD, SO2, NO2, and O3) due to lockdown over the IGP, one of the world's most populated regions. The satellite retrievals of aerosol optical depth (AOD), sulfur dioxide (SO2), nitrogen dioxide (NO2), and Ozone (O3) were used to estimate the spatial-temporal extent of major air pollutants in the region during lock down period (March-May, 2020) in comparison to the pre-lockdown period (March-May 2015-2019) and post-lockdown (March-May, 2021) across the IGP. To provide more insight into the changes in air pollutants status, country and city scale percentage increase/decrease have also been calculated. Following strict lockdown implementation, reduction in anthropogenic activities led to a significant decline in AOD, SO2 and NO2, whereas a considerable increase in tropospheric O3 concentration has been noticed that in turns significantly improved the regional air quality. But these trends reversed as soon as the lockdown was relieved and human activities normalized.  Moreover, the comparative analysis among meteorological parameters and ambient air pollutants presented that meteorological factors were not the main reason for the dramatic reductions of pollutants in the atmosphere. The outcome of this study can be a reference to introduce new public policies for promoting adaptive socio-ecological models to understand the synergies and trade-offs between the reduced human interventions and the environmental health of cities systematically.

How to cite: Hina, S., Saleem, F., and Ibrahim, M.: COVID-19 Pandemic Hopeful Prospect: Air Quality Improvements over Indo-Gigantic Plain, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1112, https://doi.org/10.5194/egusphere-egu23-1112, 2023.

EGU23-1617 | ECS | Orals | AS5.13

Near road urban air pollution due to vehicular traffic: Effect of real-world driving conditions and vehicle composition 

Sohana Debbarma, Bajrang Lal, and Harish C. Phuleria

Rapid economic growth with ongoing urbanization trends has led to exponential growth in global transport demand, especially in Asia. The growing vehicle population in India is one of the major contributors to congestion and air pollution causing related health and climate risks in urban areas. In this study, we assessed the impact of motor vehicles on near-road air pollution using roadway tunnel and roadside measurements under real-world traffic conditions based on speed, type of roads, vehicle types (LDV: light duty vehicles, HDDV: heavy-duty diesel vehicles), and fuel composition (gasoline and diesel vehicles). Portable real-time and gravimetric instruments were used to measure emissions from high-speed urban traffic (at Freeway tunnel: all LDV fleet), low-speed creeping traffic (at LBS road: 5% HDDVs and rest LDV fleet), and idling traffic (at Mulund toll plaza: 8% HDDVs and rest LDV fleet) in Mumbai city, and high-speed inter-city traffic (at Kamshet-I tunnel on Mumbai-Pune expressway: 20% HDDV and 80% LDV), covering both peak and off-peak traffic hours. A very small fraction of electric vehicles was also observed in the fleet at LBS road and Toll plaza. Simultaneous measurements were also carried out at an urban background location in Powai, Mumbai. All measured gaseous (CO2, CO, NO2, and VOCs) and particulate (PM2.5 and BC) pollutants at the roadsides and the tunnels were 1.2 to 3.8 times higher than in the background. Total fine carbonaceous species, comprising of elemental carbon (EC) and organic carbon (OC) accounted for up to 47%(±5%) of total PM2.5, highest in the inter-city traffic which could be attributed to its high HDDV and super-emitter fraction followed by the urban idling traffic which had significant HDDV fraction. The OC/EC ratio was 1.8 (± 0.3), highest in the high-speed urban traffic with all light-duty vehicles (LDV) fleet, and the higher HDDV fraction in the inter-city traffic attributed to the low OC/EC ratio of 0.7 (±0.4).  The water-soluble organic carbon (WSOC) fraction that affects aerosol hygroscopicity accounted for up to 70% of the total OC. WSOC was found highest during the afternoon period at the roadsides as well as the background site indicating the contribution of other sources, including photochemical processes. Our study finds that while the near-road emission levels are inevitably higher due to the significant contribution from on-road vehicles, the emission profiles vary significantly depending on the vehicle and fuel composition. Higher HDDV fraction and super-emitters in the fleet contributed to 2.8 folds of higher EC concentrations.  These findings can help in making informed policy decisions towards urban vehicle emission control and monitoring by focusing on targeted vehicles that are polluting disproportionately more than the rest of the vehicles.

How to cite: Debbarma, S., Lal, B., and Phuleria, H. C.: Near road urban air pollution due to vehicular traffic: Effect of real-world driving conditions and vehicle composition, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1617, https://doi.org/10.5194/egusphere-egu23-1617, 2023.

In urban set-ups, the use of charcoal as a source of energy is predominant among the urban poor (low-income earners). In the urban informal settlements such as the Korogocho slums in Nairobi, households rely on kerosene and charcoal for cooking. In some cases, it has been reported that some poorest households in these informal settlements use plastic waste, cloth rags, and other unconventional fuels due to unaffordability to access conventional sources of energy. As a result, the fuels generate high levels of harmful indoor air pollutants. This study was part of the wider project in which we assessed exposure to in-kitchen particulate matter (PM2.5 and PM10) in 60 low-income homes across 12 cities, including Nairobi (Kenya). We aim to ensure cleaner air in homes and promote the development of equitable, inclusive, social, and environmental benefits in one of Nairobi’s informal settlements as indoor environments have become more important during the Covid-19 pandemic thereby necessitating the need to ensure less exposure of households to harmful pollutants. We assess indoor air pollution exposure by monitoring aerosol and carbon dioxide data in five different households in the informal settlement of Korogocho in Nairobi. We engaged stakeholders through co-designed webinars, outreach, and capacity-building activities. The study aimed at developing exposure strategies and assessing the feasibility of similar studies in other parts of the country. The results showed that fuel, kitchen volume, cooking type, and ventilation were the most prominent factors affecting in-kitchen exposure. There is an urgent need for increased awareness of improved cooking practices and minimizing passive occupancy in kitchens to mitigate harmful cooking emissions.

 

How to cite: Sitati, C.: In-kitchen aerosol exposure in Korogocho informal settlement in Nairobi, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2211, https://doi.org/10.5194/egusphere-egu23-2211, 2023.

EGU23-2495 | Orals | AS5.13 | Highlight

Application of satellite data in air quality management: Lessons learned in India 

Sagnik Dey, Alok Kumar, Varun Katoch, Fahad Imam, Debajit Sarkar, and Kirtika Sharma

Exposure to ambient PM2.5 is the leading environmental health risk in India. An efficient air quality management plan requires a consistent and long-term database at high spatial and temporal scale. We have developed a satellite-based PM2.5 data for India by filling the gaps in satellite AOD to complement the paucity in ground monitoring. The average population-weighted exposure during 2017-2021 was estimated as 52.5 μg/m3, 18.1% lower than the estimates without adjusting for the sampling gaps. The annually averaged mortality burden attributable to ambient PM2.5 exposure during this period was estimated to be 0.45 million (95% UI: 0.36-0.55), 0.27 million (95% UI: 0.22-0.33) and 0.24 million (95% UI: 0.19-0.28) for low, medium and high sociodemographic index states, respectively. If the sampling gaps in satellite AOD is not filled, the health burden in India would be overestimated by 0.1 million (95% UI: 0.07-0.13).  We demonstrated  use of this satellite data in various air quality management practices. We have delineated 9 to 11 major seasonal air sheds in India using k-means clustering. We have found that the number of days daily PM2.5 exceeding the national standard have decreased during 2017 to 2021 in all air sheds. We have identified the potential sites for future expansion of the ground network under the National Clean Air Program. We examined the representativeness of the existing ground monitors in the non-attainment cities. These lessons learned in India could be valuable for other developing countries with limited or no ground monitoring.   

How to cite: Dey, S., Kumar, A., Katoch, V., Imam, F., Sarkar, D., and Sharma, K.: Application of satellite data in air quality management: Lessons learned in India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2495, https://doi.org/10.5194/egusphere-egu23-2495, 2023.

EGU23-3027 | ECS | Posters virtual | AS5.13

An emission model to predict hourly street level traffic emission for air quality management in megacity Delhi 

Akash Biswal, Vikas Singh, Leeza Malik, Geetam Tiwari, Khaiwal Ravindra, and Suman Mor

Road traffic emission is considered to be the major source of pollution exposure in megacities around the globe. Traffic emission makes urban air pollution to be highly spatially heterogeneous with sharp concentration gradients that can vary substantially within a few meters near the road. The spatially heterogeneous and temporally varying emissions are required to account for  concentration gradients that have a direct impact on the population exposure to outdoor air pollution. However, estimating such a detailed emission is very complex as it requires multi-category emission factors and a huge amount of georeferenced detailed traffic activity data such as traffic volume and speed, distance traveled, vehicle category share, fuel share, engine share, technology share etc. In the absence of detailed data, emission estimations have been limited to coarser resolution which may not be suitable for high resolution air quality modeling, exposure assessment and management..

Here we present an emission model to estimate multi-pollutant hourly gridded on-road traffic emission over Delhi. The model uses the globally adopted COPERT (Computer Programme to Calculate Emissions from Road Transport) emission functions to calculate the emission as a function of speed for 127 vehicle categories. For traffic activity, the emission model uses advanced traffic volume and speed data for Delhi obtained from TRIPP (Transportation Research and Injury Prevention Programme, IIT Delhi). Further the model considers the congestion (travel time delay based on TOMTOM) and speed-volume relation for different road categories to estimate hourly traffic volume and speed for each road link in Delhi that is used to calculate the hourly emissions using the COPERT emission functions Further, the emissions are gridded at 100 m × 100 m resolution to generate high-resolution spatio-temporal emission maps for Delhi and shown in Fig. 1 for four different hours of the day.

We analyzed the modeled emissions to identify peak emission hours, pollution hotspots and most polluting vehicles. The hourly variation of emissions show distinct bimodal distribution with morning and dominant evening peaks for almost all pollutants linked with congestion and peak traffic.

Figure 1. Estimated gridded NOx emission at 100m × 100m spatial resolution at different time of the day; the time is displayed in the upper-right corner of each subplot.

The emissions are high near the busy roads and traffic junctions. The emission flux in the central areas of Delhi (Fig. 1) is 40-50% higher than mean emission flux due to the higher road and traffic density and lower average speed. Diesel vehicles have been found to be the dominant contributor to PM, BC and NOx emission. Our results suggest that the top 5 polluting vehicle categories account for more than half (55% - 91%) of the emissions. This study provides very detailed spatio-temporal emission maps for megacity Delhi, which can be used in air quality models for developing suitable strategies to reduce the traffic related pollution. The developed model can be applied for developing emission inventory and real-time emission with the growing availability of real-time traffic data.

How to cite: Biswal, A., Singh, V., Malik, L., Tiwari, G., Ravindra, K., and Mor, S.: An emission model to predict hourly street level traffic emission for air quality management in megacity Delhi, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3027, https://doi.org/10.5194/egusphere-egu23-3027, 2023.

EGU23-3110 | ECS | Posters on site | AS5.13

Correcting PM2.5 data from low-cost sensors using machine learning techniques 

Pratyush Agrawal, Srishti Srishti, Padmavati Kulkarni, Hrishikesh Gautam, Meenakshi Kushwaha, Sreekanth Vakacherla, and Pratima Singh

Low-cost sensors (LCSs) used for measuring air quality have become popular because of their portability, affordability, and ease of operation. However, LCS data often have accuracy and bias issues that need to be addressed before using them for research. LCSs are, therefore, collocated with reference-grade instruments, and various statistical and machine learning (ML) approaches are used to correct the observed bias in data. In this study, collocation experiments were conducted in Bengaluru, India, for about nine months (December 2021 to August 2022). We used nine PM2.5 LCSs that were collocated with a beta attenuation monitor (BAM), which is certified by the United States Environmental Protection Agency (USEPA). Hourly averaged data from LCSs and BAM were used to train various ML correction models. The LCSs included in the study—Airveda, Atmos, Prana Air, BlueSky, Aurassure, Aerogram, PurpleAir, and Prkruti—are widely available in the Indian market. The ML models include support vector regression (SVR), decision tree (DT), random forest (RF), and eXtreme gradient boosting (XGBoost). For the LCSs used in the study, a total of 170 ML models were built to identify the best-performing correction model for each sensor. Model performances were evaluated based on the following metrics: mean absolute error (MAE), root mean square error (RMSE), and normalised RMSE (NRMSE). During the study period, the average hourly BAM concentration was ~32 µg/m3. Hourly averaged PM2.5 from LCSs and BAM exhibited a linear relationship. The NRMSE values of the raw (uncorrected) LCSs PM2.5 with respect to BAM PM2.5 varied between 0.26 and 0.89 across various sensors. The Plantower-based LCSs (Atmos I, PurpleAir, and Aerogram) performed better, characterised by the lowest RMSE/NRMSE values. SVR was found to be the best-performing model for most of the sensors in correcting raw LCSs PM2.5 data. The NRMSE of the ML models’ corrected LCSs PM2.5 was reduced by 46% to 74% across various sensors compared to the uncorrected LCSs PM2.5. As a case study, we also added black carbon (BC) data to our ML models, but no significant change (improvement by 6% RMSE) in performance was observed.

How to cite: Agrawal, P., Srishti, S., Kulkarni, P., Gautam, H., Kushwaha, M., Vakacherla, S., and Singh, P.: Correcting PM2.5 data from low-cost sensors using machine learning techniques, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3110, https://doi.org/10.5194/egusphere-egu23-3110, 2023.

EGU23-3307 | Posters on site | AS5.13

Sharing Air Quality Monitoring Activities at a University in Nigeria 

Rabia Salihu Sa'id, Najib Yusuf Galadanci, Murtala Muhammad Badamasi, A. Babatunde Rabiu, and Gregory S. Jenkins

Breathing is life and the quality of air we breathe is important for good quality of living. At the Bayero University in Kano, Nigeria, the Space Weather and Atmospheric Physics Laboratory has collaborated with the Center for Atmospheric Research to establish a network of air quality monitoring and data gathering techniques through setthing up monitoring stations and recently collaborating with the Alliance for education, Science, Engineering and Design in Africa (AESEDA), using low cost air quality monitoring devices and combining the ground-based data with sattelite data to give meaningful and useful data for safety. Data of air pollutants measured and how they correlate with increasein respiratory tract infections during the pandemic were studied. We present the activities of air quality monitoring during the period of 2020; the hieght of the pandemic and the period thereafter. Findings show that there is a need to be concerned as readings of impact of air pollutants are high and most times hiher than the minimum EPA standards.

How to cite: Sa'id, R. S., Galadanci, N. Y., Badamasi, M. M., Rabiu, A. B., and Jenkins, G. S.: Sharing Air Quality Monitoring Activities at a University in Nigeria, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3307, https://doi.org/10.5194/egusphere-egu23-3307, 2023.

EGU23-3805 | ECS | Orals | AS5.13

Monitoring the Diurnal and Seasonal Variation of Ambient of Ambient Particulate Matter (PM2.5) using Low-Cost Sensors in Juja, Kenya 

Josephine Kanyeria Ndiang'ui, Paul Njogu, and Daniel Westervelt

Air pollution is a major environmental concern that affects human health worldwide. Despite recent studies indicating ambient air pollution is a growing global concern strongly linked to rapid global urbanization, little has been done to monitor the air quality levels in Africa. Traditionally, air quality monitoring has relied on environmental monitoring stations, that are expensive to build and maintain. In Kenya, for example there is no publicly available national air quality monitoring data. Thus, low-cost sensors offer a practical and cost-effective means of monitoring air quality. We carried out a study in Juja town, located in central Kenya within the outskirts of Nairobi. Juja is one of the largest growing towns and is located along the busy Thika Superhighway. The purpose of this study was to assess the diurnal and seasonal variations of Ambient Particulate Matter (PM2.5) in Juja, Kenya. The data was collected as from November 2019 to April 2021 at JKUAT Institute of Energy and Environmental Technology (IEET) department, a residential area within Toll and Kibariti and an additional site along the busy Thika Superhighway. The PM level was measured using the Purple Air Monitoring Sensor – PA-II-SD in μg/m3 on a 24hour cycle. The PM2.5 level from the low-cost Purple Air Sensors were later calibrated against a reference BAM-1022 to yield corrected PM values. The results revealed that the overall PM2.5 concentration was higher during the dry season (June - August 2020) compared to March - May 2020 (wet season) where it dropped by 5-10μg/m3 on average. The average daily PM2.5 levels were recorded at 44μg/m3 (Pine Breeze), 20μg/m3 (Toll) and 16μg/m3 (Kibariti) all exceeding the WHO guideline of 15μg/m3. JKUAT had an annual mean concentration of 15μg/m3, also exceeding the WHO guidelines of 5μg/m3. The study also found that PM2.5 levels were highly correlated with vehicle emissions, as the site closest to the highway had the highest PM2.5 levels. The levels also peaked twice a day at 5am and 5pm, possibly due to morning and evening traffic. It is thus evident that traffic related emissions are a great concern within the town and effective mitigation measures are needed to protect the residents. In addition, comparing the month of April 2021 to the previous year, the daily mean dropped by 5-10μg/m3 – the period of the new Covid -19 lockdown. These results can then be used to model and predict urban air quality within the town. Overall, low-cost sensors have provided an increased availability of data that can be used to identify patterns and trends in air quality over time. Their use can also facilitate greater community engagement, as individuals and organizations can participate in data collection, monitoring and analysis. To conclude, this research provides an important tool for informing urban planning and environmental policies. By understanding the sources, patterns and impacts of air pollution, decision makers can develop strategies to address these issues and improve the health and well-being of urban residents.

How to cite: Kanyeria Ndiang'ui, J., Njogu, P., and Westervelt, D.: Monitoring the Diurnal and Seasonal Variation of Ambient of Ambient Particulate Matter (PM2.5) using Low-Cost Sensors in Juja, Kenya, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3805, https://doi.org/10.5194/egusphere-egu23-3805, 2023.

EGU23-3903 | ECS | Orals | AS5.13 | Highlight

Enhancing the spatial and temporal resolution of air quality monitoring in low – and middle-income countries using low-cost sensors 

Collins Gameli Hodoli, Anthony Amoah, Dominic Buer Boyetey, Iq Mead, Frederic Coulon, Pallavi Pant, Cesunica E. Ivey, Victoria Owusu Tawiah, James Nimoo, John-Terry Morladza, Garima Raheja, Mawuli Amedofu, Felix Allison Hughes, Nelson Kowu, Emmanuel Appoh, Benjamin Essien, Carl Malings, and Daniel M. Westervelt

Air pollution is one of the leading risk factors for poor health in Africa, resulting in millions of premature deaths and economic losses. Of particular interest is exposure to fine particulate matter (PM2.5) which is the driver for a majority of deaths across the continent. However, PM monitoring, and by extension, ground-level data on PM2.5 is very limited; this limits our understanding of the widespread societal and health impacts linked to PM pollution. The robustness of low-cost PM sensors and their ability to report in situ data in tropical environments via internet-based platforms as well as relative affordability has created the opportunity to employ low-cost sensors (LCS) for air quality monitoring but calibration methodologies and the usefulness of the high-temporal resolution data for source identification remain a challenge. Increasingly, local governments in African countries are also turning to low-cost sensors to monitor air quality. In this study, two Airnote PM monitors were colocated with reference-grade Teledyne PM mass monitor T640 for ~4 weeks at the University of Ghana, Accra to establish their performance using a simplified data correction methodology - multiple linear regression (MLR) model. A split ratio of 80% and 20% was used to train and test the populated Airnote PM2.5 data respectively based on measurements from Teledyne T640 with temperature and relative humidity values from the Airnote monitor. Sectoral and calendar analysis with wind component data were used to triangulate the sources of PM2.5. We observed a high consistency between the two Airnote monitors. Hourly and 24-hour average PM2.5 values ranged from 25 to 95 μg/m3, and 29 to 54 μg/m3 respectively, and in most cases, were significantly higher than the WHO Air Quality Guideline. MLR using Pearson’s correlation analysis improved the out-of-the-box quality of low-cost Airnote PM2.5 data; the R2 improved from 0.69 to 0.84 and the mean absolute error from 11.75 to 4.20 μg/m3 respectively. Also, the MLR correction model was found to improve the Airnote PM2.5 data quality for higher relative humidity (between 50 and 90%) but not lower. PM2.5 pollution was local and from N, NE and SW winds for the raw, corrected and Teledyne PM mass monitor T640 measurements. Together, these results indicate that with appropriate corrections, low-cost PM sensors can generate the much needed data for air pollution research and mitigation in areas with limited air quality monitoring and data.

How to cite: Hodoli, C. G., Amoah, A., Buer Boyetey, D., Mead, I., Coulon, F., Pant, P., Ivey, C. E., Owusu Tawiah, V., Nimoo, J., Morladza, J.-T., Raheja, G., Amedofu, M., Allison Hughes, F., Kowu, N., Appoh, E., Essien, B., Malings, C., and Westervelt, D. M.: Enhancing the spatial and temporal resolution of air quality monitoring in low – and middle-income countries using low-cost sensors, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3903, https://doi.org/10.5194/egusphere-egu23-3903, 2023.

EGU23-4018 | ECS | Posters virtual | AS5.13

Investigation of Endocrine disruptor - PAEs and Carcinogenic - PAHs bound to ambient fine particulate matter over Northwest Indo-Gangetic Plain 

Durga Prasad Patnana, Boggarapu Praphulla Chandra, Pooja Chaudhary, Baerbel Sinha, and Vinayak Sinha

 

Phthalic acid esters (PAEs) and polycyclic aromatic hydrocarbons (PAHs) are classified as priority pollutants by United States Environment Protection Agency (USEPA). Some of the PAEs and PAHs are considered as human carcinogens by International Agency for Research on Cancer (IARC). In the present study, an ultra-high performance liquid chromatography coupled to triple quadruple mass spectrometry (LC-MS QQQ) method was developed and validated for the simultaneous determination of PAEs and PAHs bound to ambient particulate matter. After the method validation, it was deployed for the quantification of PAEs and PAHs bound to PM2.5 collected at a sub urban site in the Northwest Indo-Gangetic Plain. The targeted PAEs in this study are dimethyl phthalate (DMP), diethyl phthalate (DEP), benzyl butyl phthalate (BBP), di butyl phthalate (DBP), bis (2-ethyl hexyl) phthalate (DEHP), bis (2-ethylhexyl) adipate (DEHA), di-n-octyl phthalate (DNOP) and PAHs are benzo[a]anthracene (B[a]A), benzo[b]fluorenthene (B[b]F), benzo[k]fluorenthene (B[k]F), benzo[a]pyrene (B[a]P), dibenzo[ah]anthracene (D[ah]A), benzo[ghi]perylene (B[ghi]P), and indeno[1,2,3-cd]pyrene (IND). The measured concentrations of PAEs and PAHs are seasonally varied and the higher concentrations of PAEs were observed in summer and PAHs in winter. DEHP (17.94 ng m-3) and B[b]F (36.13 ng m-3) are the most abundant PAE and PAH measured at the sampling site. The concentrations of B[a]P (4.66 ng m-3; Group 1 carcinogen) exceeded the threshold limits (1 ng m-3) set by the National Ambient Air Quality Standards of India (NAAQS). Further, the incremental lifetime cancer risk due to inhalation exposure to DEHP and B[a]P were estimated for adults (0.3678 × 10-6 and 1.40 × 10-5 respectively) and children (0.8792 × 10-6 and 3.272 × 10-5 respectively). Also, the cancer risk associated with the inhalation exposure to B[a]P has exceeded the limits (1 ×10-3) set by USEPA at the measurement site.

How to cite: Patnana, D. P., Praphulla Chandra, B., Chaudhary, P., Sinha, B., and Sinha, V.: Investigation of Endocrine disruptor - PAEs and Carcinogenic - PAHs bound to ambient fine particulate matter over Northwest Indo-Gangetic Plain, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4018, https://doi.org/10.5194/egusphere-egu23-4018, 2023.

EGU23-4512 | Orals | AS5.13

Visibility as a proxy for air quality in Nigeria from 1950 to 2020 

Francis Pope and Vitalis Nwokorie

Nigeria is the largest country in Africa by population. Currently, the population is estimated to be 219 million making it the 7th largest country worldwide. Demographic trends suggest that rapid population growth will lead to a population of approximately 400 million by 2050, which would make it the 3rd largest country worldwide. 

Air quality in Nigeria is routinely reported to be poor due to both natural and anthropogenic sources of air pollution.  There are a limited number of air monitoring stations within Nigeria, and a corresponding lack of long-term air quality data, with which to assess its long-term trends. With the advent of low-cost monitoring, there has been a recent upsurge in measurements in Nigeria, but these measurement campaigns tend to short term and difficult to discern long term trends from. Nonetheless, these measurements show clearly that particulate matter (PM) air pollution regularly exceeds the WHO guidelines for both PM10 and PM2.5 size fractions, and hence PM places a high health burden upon the population.

This study uses visibility readings in Nigeria, measured since the 1950s, to study and understand historical and contemporary levels of air pollution. Visibility is related to the atmospheric extinction coefficient that is largely determined by the amount of PM in the atmosphere. New machine learning calibration techniques allow for PM2.5 mass concentrations to be estimated directed from visibility and other meteorological measurements.  This presentation will discuss the visibility derived PM findings for the different regions of Nigeria. It will highlight trends in both regional scale and more localized sources of PM.  The implications of population growth and other socio-economic factors upon potential air quality scenarios for Nigeria will also be discussed.

How to cite: Pope, F. and Nwokorie, V.: Visibility as a proxy for air quality in Nigeria from 1950 to 2020, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4512, https://doi.org/10.5194/egusphere-egu23-4512, 2023.

EGU23-4750 | ECS | Posters virtual | AS5.13

Performance of Low-Cost Sensors in Measuring Particulate Matter Concentrations in Indoor and Outdoor Environments 

Rubal Rubal, Anirudha Ambekar, and Thaseem Thajudeen

Air pollution is one of the major causes of early death worldwide and is especially widespread in many low-and middle-income nations (LMICs). Preliminary monitoring networks, satellite retrievals of air-quality-relevant species, and air quality models show that in Asian countries, ambient fine particulate matter (PM) concentrations exceed World Health Organization guidelines, despite the fact that many areas generally remain unmonitored and understudied. The size of PM in the air and the ratio of fine to coarse PM determine the ability to affect the environment and health. Although better monitoring of the air quality levels is of prime importance, the costs involved in setting up monitoring stations are often a big hurdle. This study investigates the distribution and proportion of PM1, PM2.5, and PM10 at multiple locations in an educational institute in Goa. In addition to continuous monitoring using low-cost sensors (LCS), including PMS5003, PMS A003, PMS 7003, Winsen ZH 06, SPS 30, Novafitness SDS 011, and Honeywell HPMA, we have also attempted to compare the performance of these sensors with Alphasense OPC N3 at Indian Institute of Technology Goa. The performance of LCS was examined in a variety of environmental settings throughout the research period. The factors such as reference bias, temporal drift, particle composition effect, Pearson correlation, sensor repeatability, and climatic influence on sensor data have been analyzed to assess their significance in the analytical results. Pearson correlations (r = 0.64 - 0.83) between the investigated devices demonstrated the efficacy of low-cost Plantower PM sensors in monitoring PM10 and PM 2.5 in the field. The correlation between the low-cost sensor and OPC was lower in sites with a more significant concentration of coarse particles. As expected, the measurements are also influenced by atmospheric conditions, particularly temperature and relative humidity. The time-series results also clearly show the increased concentration levels during the winter (greater than the national standards) but less in summer and winter. This study also attempts to analyze the air quality at different locations in Goa with LCS, and the PM concentration is compared with gravimetric samplers at those locations.

How to cite: Rubal, R., Ambekar, A., and Thajudeen, T.: Performance of Low-Cost Sensors in Measuring Particulate Matter Concentrations in Indoor and Outdoor Environments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4750, https://doi.org/10.5194/egusphere-egu23-4750, 2023.

Phthalate esters (PEs) are a group of synthetic organic compounds that are frequently employed as plasticizers, additives in the production of plastic products, as well as in cosmetics, personal care items, medical products, and insecticides. Since PEs are not chemically linked to polymers, they can easily be released into the environment both during production and use, as well as following the disposal of plastic items. These compounds  also belong to the class of endocrine disrupting species and have gained research attention due to their widespread environmental occurrence and associations with respiratory system diseases, and higher incidence of allergies. However, very little is known regarding the inhalation exposure to endocrine disrupting PEs. In this study an analytical approach- thermal desorption gas chromatography coupled with mass spectrometry (TD-GC/MS) was optimized for the measurement of particle-bound PEs. We report monthly (Jan, Feb, Mar, and Apr, 2019) concentrations of 6 PEs, viz., Dimethyl Phthalate (DMP), Diethyl Phthalate (DEP), Di-N-Butyl Phthalate (DnBP), Butyl Benzyl Phthalate (BBZP), Bis(2-Ethylhexyl) Phthalate (DEHP), Di-N-Octyl Phthalate (DNOP) measured every other day in ambient PM2.5 over Bhopal – one of the regionally representative sites of the COALESCE network (Lekinwala et al., 2020).

Two endocrine disrupting compounds – DEHP and DBP exhibited high concentrations during  the months of Jan (23.6 ± 7.1 ng m-3 and 12.3 ± 4.2 ng m-3) and Feb (21.3 ± 10 ng m-3 and 11.0 ± 3.5 ng m-3). The average daily intake of Σ6 PEs and DEHP via inhalation were 0.11-0.21 μg/Kg day and 0.01-0.1 μg/Kg day, respectively, for adults in Bhopal. The inhalation cancer risk metric revealed that the estimated exposure to DEHP (3.9 × 10-5) exceeded the acceptable risk threshold. These results provide critical information that suggests that PEs from ambient and indoor sources should be considered when exploring the inhalation health risks to PM exposure.

How to cite: Yadav, K. and Sunder Raman, R.: Phthalate esters in atmospheric PM2.5 in Bhopal, central India: Identification, Concentrations, and Health Risk Assessment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4958, https://doi.org/10.5194/egusphere-egu23-4958, 2023.

EGU23-5586 | ECS | Orals | AS5.13

Development of land use regression (LUR) models for criteria air pollutants in Delhi: Use of regulatory monitoring data 

Adithi Upadhya, Padmavati Kulkarni, Mahesh Kalshetty, Srishti Srishti, Meenakshi Kushwaha, Pratyush Agrawal, and Sreekanth Vakacherla

High-resolution spatial maps of air pollution can be useful for air quality management. In low- and middle-income countries, regulatory measurements of criteria pollutants are typically insufficient to generate spatial maps, due to the sparsely located monitoring stations. Alternatively, high-resolution spatial maps of air pollution can be achieved by dispersion (physics-based) and statistical regression (training-based) modelling. Resolutions of up to ~25 meters can be achieved by Land Use Regression (LUR) modelling based spatial predictions. In this study, we leveraged the high density of regulatory monitors located in New Delhi, India, and developed LUR models for all the major criteria pollutants (PM10, PM2.5, SO2, NO2, and Ozone). New Delhi is one of the most heavily polluted cities in the world. We used data from 40 continuous ambient air quality monitoring stations’ (CAAQMS) for the year 2019 to develop seasonal and annual LUR models, following the ESCAPE (European Study of Cohorts for Air Pollution Effects) stepwise supervised regression method. Model predictors included land use parameters, road lengths, rail track lengths, population, satellite pollution, and NDVI data, along with air pollution point source location data and reanalysis meteorology. The models were validated using leave one station out (LOSO) and 10-fold cross validations (CV). The model adjusted R2 values varied between 0.08 and 0.64. Particle pollutant models (PM2.5 and PM10) performed better than those of gaseous pollutants. Further, ozone models performed the least. Across seasons, summer models performed the best (least) for PM (gaseous pollutants). Models with adjusted R2 were used for spatial predictions at 50-m resolution for the Delhi National Capital Territory region. Spatio-seasonal characteristics of air pollution were studied using the generated high-resolution maps.

How to cite: Upadhya, A., Kulkarni, P., Kalshetty, M., Srishti, S., Kushwaha, M., Agrawal, P., and Vakacherla, S.: Development of land use regression (LUR) models for criteria air pollutants in Delhi: Use of regulatory monitoring data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5586, https://doi.org/10.5194/egusphere-egu23-5586, 2023.

EGU23-5925 | ECS | Orals | AS5.13 | Highlight

Impact of low clouds and boundary layer height on regional air quality over Delhi-NCR 

Jaswant Rathore and Dilip Ganguly

In this study, Ceilometer measurements of attenuated backscatter coefficient over Delhi-NCR during monsoon (June-September) and post-monsoon (October-November) of 2022 are analyzed to determine cloud base height (CBH) and atmospheric boundary layer (ABL) height. The derived CBH and ABL height are used to assess the impact of low clouds (CBH < 2km) and ABL height on regional air quality. The Ceilometer measurements are augmented by ERA5 reanalysis dataset of hourly averaged CBH and ABL height and radiosonde measurements. The aerosol loading over Delhi-NCR is derived using Moderate Resolution Imaging Spectroradiometer (MODIS) Terra aerosol optical depth (AOD) measurements and Dusttrack retrieved particulate matter with aerodynamic diameter ≤ 10 µm (PM10) concentrations. We also used Ceilometer measurements for non-cloudy days to interpolate missing PM10 values during the study period. To evaluate the dilution and diffusion of pollutants, we calculated ventilation coefficient from ABL height and wind speed data.

The results reveal that out of the total measurements during monsoon season, 41% cloud occurrence was observed, out of which 24% of clouds were low-level clouds. In post-monsoon season, cloud occurrence was low (nearly 12%), out of which 40% of clouds were low-level clouds. The ABL results show that during monsoon season, average ABL height was 0.85±0.6 km and during post-monsoon, it was 0.53±0.45 km. The seasonal difference is not only noted in the average values but also in the growth of ABL with full growth of ABL happening 2 hours later in post-monsoon season than monsoon season. The MODIS derived AOD results show average AOD values of 0.72±0.29 and 0.97±0.54 in monsoon and post-monsoon season respectively.

The comparison of PM10 & AOD values indicate that during the cloudy days, both PM10 values and AOD values were higher suggesting the abundance of cloud nuclei which could facilitate low cloud formation. For cloudy days, the correlation of observed CBH of low clouds with PM10 and AOD shows a strong negative correlation (-0.78 and -0.83 respectively) suggesting that under same atmospheric thermodynamic conditions, CBH lowers under polluted conditions. The seasonal characteristics show that this tendency is predominant in post-monsoon than monsoon which might require further investigation. We observed strong negative correlation of ABL height with PM10 and AOD (-0.84 and -0.89 respectively) during the study period. The derived ventilation coefficient shows a strong negative correlation with PM10 and AOD values (-0.67 and -0.69 respectively). Both seasons showed similar characteristics indicating that the dissipation of pollutants depends more on ABL during both the seasons. However, substantiation of the diffusion and dilution processes over Delhi-NCR may require further investigation with different meteorological conditions. This will be added to this study along with the impact of clouds and ABL on different size distributions of aerosols. In conclusion, we used advanced instrumentation to study the interlinkages of atmospheric vertical structure with air quality. Our findings are relevant for the Indo Gangetic Plain (IGP) having population more than 400 million and can be applied to other places in the global south experiencing high pollution episodes often linked to unfavourable meteorology.

How to cite: Rathore, J. and Ganguly, D.: Impact of low clouds and boundary layer height on regional air quality over Delhi-NCR, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5925, https://doi.org/10.5194/egusphere-egu23-5925, 2023.

EGU23-6046 | ECS | Posters on site | AS5.13

Fireworks: A Major source of elemental aerosols during Diwali in Delhi-NCR 

Mohd Faisal, Umar Ali, Vikram Singh, and Mayank Kumar

Fireworks activities worldwide seem to play a significant role in air quality degradation, especially during different events that lead to worsening air quality in the form of ambient particulate matter (PM) pollution. The fireworks activity in Delhi is one of the primary cause for the considerable increase in the particulate concentration during Diwali in Delhi. The substantial increase due to extensive firework activity results in enhanced metal concentration in the atmosphere. Therefore a comprehensive understanding of fireworks induced into the atmosphere is crucial to develop an enhanced mitigation strategy. Thus this study focuses on the comparative analysis of fireworks used in Diwali for the years 2019, 2020 and 2021. The current analysis studies the impact of Diwali for three consecutive years on the concentration, composition, and sources of ambient PM2.5. The measurement of elements in PM2.5 was performed with half-hourly time resolution using the Xact 625 Ambient Metals Monitor. The 12-hour average concentration of metals during Diwali night for 2019, 2020 and 2021 are 181 ug/m3, 117 ug/m3, and 151 ug/m3, respectively. Concentration levels of species like K, Al, Sr, Ba, and S displayed distinct peaks during the firework event and were identified as tracers for the same. We conducted source apportionment by positive matrix factorization (PMF) of the elemental mass measurable by the Xact. The source apportionment study indicated that more than 85% of elemental mass had been apportioned to firecrackers during Diwali. The reported enhancement in the mass concentration of elemental metals like Al, Ba, Cl, Pb, and Mn poses a severe threat to the health of the exposed population as the average mass concentration of these species exceeded the standard EPA risk-based levels by orders of magnitude during the Diwali phase. Moreover, possible carcinogens like As also exceeded the risk-based concentration significantly.

How to cite: Faisal, M., Ali, U., Singh, V., and Kumar, M.: Fireworks: A Major source of elemental aerosols during Diwali in Delhi-NCR, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6046, https://doi.org/10.5194/egusphere-egu23-6046, 2023.

EGU23-6113 | ECS | Orals | AS5.13

Study of aerosol trace elements over three COALESCE network locations in India: Spatio-temporal variability, dry deposition and health risks 

Diksha Haswani, Ramya Sunder Raman, Kajal Yadav, Abisheg Dhandapani, Iqbal Jawed, R Naresh Kumar, Laxmi Prasad Sanyasihally Vasanth Kumar, Adi Yogesh, Sadashiva Murthy, and Kaggere Shivananjaiah Lokesh

A small fraction (5-10 %) of PM2.5 (fine particulate matter, with aerodynamic diameter ≤ 2.5 µm) mass constitutes trace elements (TEs) and plays an important role in controlling human health, ecological systems and air quality. TE/groups of TE are used as tracers to identify specific PM sources, predominantly due to their persistence and stability in the atmosphere. As a part of the COALESCE network ambient aerosol measurement campaign, 24-h integrated collocated PM2.5 filter sampling was carried out for 2019 in all the three distinctly different geographical locations in India, viz., Bhopal, Mesra and Mysuru, and 15 TE concentrations were analyzed using Energy Dispersive X-Ray Fluorescence. For all sites, annual mean sulfur contributed highest (~7 %) to PM2.5 mass among all analyzed elements followed by silicon (~3 %). Elements from multiple sources exhibited differentiable seasonal variations like crustal origin elements peaked during the pre-monsoon season, while other anthropogenic activities driven elements increased during the winter and post- monsoon seasons. Spatial heterogeneity of elements between the sites was examined using statistical tools like coefficient of divergence and spearman correlation coefficient (SCC), and revealed that they had different sources/source regions or were processed differently in the atmosphere. Further, SCC coupled with hierarchical clustering analysis categorized the data set into three common groups to yield likely sources of TEs that included crustal and mineral dust; biomass burning; non-exhaust traffic emissions and industrial sources, for all three locations. The computed dry deposition flux of both crustal (3377.41 ± 3224.65 µg m-2 d-1 to 27.83 ± 21.91 µg m-2 d-1) and non-crustal elements (53.47 ± 78.57 µg m-2 d-1 to 0.72 ± 0.59 µg m-2 d-1) was in compliance with modeled deposition flux for the entire Northern Indian Ocean and were similar to the fluxes over different regions across the globe. The United States Environment Protection Agency health risk assessment method in all sites revealed that the route of exposure of metals was highest via inhalation pathway for both adults and children, followed by dermal contact and ingestion. Total potential non-carcinogenic health risk for all pathways were below safe level (Hazard Quotient < 1) for Bhopal and Mysuru, and above safe level (Hazard Quotient > 1) for Mesra. These findings suggest that the non-carcinogenic adverse effects from multi-elemental exposure to PM2.5 was greater in Mesra, than other two sites and might be due to influence of elemental pollutants from more dominant sources of agricultural burning and industrial activities in this region (1). On the other hand, the carcinogenic risk of all metal exposure was within acceptable limits (1×10-6 – 1×10-4), through all three pathways in all the sites. Overall, the multiple site analysis presented in this study provides information on spatiotemporal patterns, dry deposition fluxes of elements in ambient PM, in addition to potential human health risks upon exposure to these species.

 

1.Maheshwarkar, Prem, et al. "Understanding the influence of meteorology and emission sources on PM2. 5 mass concentrations across India: first results from the COALESCE network." Journal of Geophysical Research: Atmospheres 127.4 (2022): e2021JD035663.

How to cite: Haswani, D., Raman, R. S., Yadav, K., Dhandapani, A., Jawed, I., Kumar, R. N., Sanyasihally Vasanth Kumar, L. P., Yogesh, A., Murthy, S., and Lokesh, K. S.: Study of aerosol trace elements over three COALESCE network locations in India: Spatio-temporal variability, dry deposition and health risks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6113, https://doi.org/10.5194/egusphere-egu23-6113, 2023.

EGU23-6516 | Posters on site | AS5.13

Health Risk Assessment and Source Apportionment of Elemental Particulate Contents from a South Asian Future Megacity 

Muhammad Ibrahim, Afifa Aslam, Abid Mahmood, Muhammad Alvi, Fariha Jabeen, and Umara Tabassum

Many factors cause air pollution in Pakistan, which poses a significant threat to human health. Diesel fuel and gasoline motor vehicles, as well as industrial companies, pollute the air in Pakistan's cities. The study's goal is to determine the level of air pollution in a Pakistani industrial city and to establish risk levels for the health of the population. We measured the intensity of air pollution by chemical characterization and examination of air samples collected at stationary remark sites. The PM10 levels observed at all sampling sites including residential, commercial, high traffic and industrial areas were well above the limits imposed by Pakistan EPA, United States EPA, and WHO. We assessed the health risk via chemical factors using methodology approved for risk assessment. All Igeo index values greater than one were considered moderately contaminated or moderately to severely contaminated. Heavy metals have a substantial risk of acute adverse effects. In Faisalabad, Pakistan, there was an enormously high risk of chronic effects producing of heavy metal acquaintance. Concerning specified toxic metals, intolerable levels of carcinogenic risks have been determined for the entire population. As a result, in most of the investigated areas of Faisalabad, the indices and hazard quotients for chronic and acute exposure exceeded the permissible level of 1.0. In the current study, re-suspended roadside mineral dust, anthropogenic exhaust emissions from traffic and industry and industrial dust were identified as major emission sources of elemental particulate contents. Because of the unacceptable levels of risk in the research area, it is strongly suggested that a comprehensive study of the population's health status as a result of air pollution should be conducted for policies to be developed against these risks.

How to cite: Ibrahim, M., Aslam, A., Mahmood, A., Alvi, M., Jabeen, F., and Tabassum, U.: Health Risk Assessment and Source Apportionment of Elemental Particulate Contents from a South Asian Future Megacity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6516, https://doi.org/10.5194/egusphere-egu23-6516, 2023.

EGU23-6686 | Orals | AS5.13 | Highlight

Emissions Inventory of Air Pollutants from Anthropogenic Sources in Jakarta 

Puji Lestari, Maulana Khafid Arrohman, Seny Damayanti, and Zbigniew Klimont

Emission inventory is an important tool for air quality management. Jakarta as a capital city of Indonesia has a very high air pollution as a result of urban activities from various anthropogenic sources. This study aims to conduct emission inventory and emission spatial distribution of NOX, CO, PM2.5, PM10, NMVOC, BC, and SO2 from anthropogenic sources in Jakarta from 2015 to 2030, using 2015 as a baseline year. The results from this study can be very important to improve the emission data for Jakarta and contribute to the global emission model. This result can also be used for air quality management and lesson learnt cases for other regions in South East Asian countries.   Emissions of these pollutants were calculated using GAINS (Greenhouse gas Air pollution INteractions and Synergies) model, considering implementation of emission standards for transport and stationary combustion sources as well as policies stimulating accelerated electrification of vehicle fleets and vehicle scrapping programs. The impact of current policies to emission reduction was also evaluated in this study. The total 2015 emissions of NOX, CO, PM2.5, PM10, NMVOC, BC and SO2 were estimated at around 53 kt, 144 kt, 4.6 kt, 6 kt, 48.6 kt, 1.2 kt, and 20 kt, respectively. The biggest contribution for NOx, CO, BC and NMVOC emissions originated from road transportation sector which contributed about 57%, 93% and 75%, 96% respectively, while for SO2, industrial combustion contributed about 67%. Heavy duty vehicles contribute the most NOx and BC emissions in the transport sector, while motorcycles emit the most CO. Meanwhile PM2.5 and PM10 in Jakarta are mostly emitted from road transportation and industrial combustion sectors, which contributed around 43%-46% for each sector. Heavy duty vehicles were still the highest contributor of PM2.5 emission in the transport sector. In addition to air pollutants, GHG (CO2 eq) emission was also calculated in this study and the results indicating that the main contributor in 2015 were road transport  and power & heating plant which contributed 34% and 32 % respectively.  Based on emission spatial distribution, the highest concentration of all pollutants was found in the central of Jakarta, where traffic activities are very busy. Policy implementation could effectively reduce pollution levels in Jakarta. The accelerated implementation of electric vehicles, stringent emission standards, and transport management measures like electronic road pricing could significantly contribute to the reduction of PM2.5, PM10 as well as BC.

Keywords: Emission inventory, pollutants, power plant, industry, residential and commercial, PM2.5, NOx, SO2, NMVOC, GAINS.

 

How to cite: Lestari, P., Arrohman, M. K., Damayanti, S., and Klimont, Z.: Emissions Inventory of Air Pollutants from Anthropogenic Sources in Jakarta, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6686, https://doi.org/10.5194/egusphere-egu23-6686, 2023.

EGU23-6701 | ECS | Orals | AS5.13

Emission Inventories for 76 Cities In India for Clean Air Strategies 

Pratima Singh, Anirban Banerjee, Udhaya Kumar, Amishi Tiwari, Hrishikesh Gautam, and Sameer Mishra

Understanding polluting sources, for improving Air Quality (AQ) levels at the city/airshed level is required to solve the air pollution challenge. Scientific evidence like Emission Inventory (EI); identification of efficient technologies; implementation roadmap; and cost and resources required, are needed to develop clean air strategies.

This study considered 76 Non-Attainment (NA) cities in India, for developing EI at an airshed level. Various polluting sectors and activities were identified. Data from various sources and ground surveys were used to generate evidence. The EI was developed for the base year 2019 for 4 pollutants– Particulate Matter (PM10 and PM2.5), Sulphur dioxide (SO2), and oxides of Nitrogen (NOX). Based on the city EI, sector-specific technologies and control measures were identified and prioritized using Techno-Economic Assessment (TEA) and the emission reduction potential. Gap Analysis was conducted to identify sectoral targets for reducing emissions.

The Emission load varied for types of cities (tier I, II, or III) based on landscape, and anthropogenic activities. It was observed that city-level PM2.5 emissions from three sectors - transportation (tailpipe: 30%-50%; road dust: 8%-17%); domestic (14%-30%); and Industries (6%-29%) were high for all the cities. In a few cities, heavy industries within the city boundary dominated the industrial share in the city’s total PM2.5 emission load (34%-88%). Hence, heavy industries were excluded from the analysis to better understand the city's emission level. The study helped to understand the city vs airshed emission load. In 46% of the cities, it was found that the airshed emission load (excluding city emission) was high due to the presence of heavy industries.

Using TEA, the study estimated the associated cost of the identified control measures feasible for implementation at the city level. The required cost was based on the existing gaps in the current infrastructure needs of the city. In tier 2 cities, the transportation sector required heavy infrastructure. Capital investment, for transportation, was estimated between INR 300 – 800 Cr on measures such as a) improving public transportation, b) LNG for freight transport, and c) replacing older vehicles. However, in tier 3 cities increasing LPG connections and strategies to reduce solid fuel usage (advanced chullah’s) were found to be critical interventions, which required investment of less than 50cr. The study also carried out emission reduction scenarios till 2030. In comparison to the business-as-usual scenario, under a high emission reduction scenario, PM2.5 emission reduction for tier 2 cities were up to 45%, and for tier 3 cities up to 54%. The study found that developing clean air strategies need to adopt an airshed approach.

How to cite: Singh, P., Banerjee, A., Kumar, U., Tiwari, A., Gautam, H., and Mishra, S.: Emission Inventories for 76 Cities In India for Clean Air Strategies, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6701, https://doi.org/10.5194/egusphere-egu23-6701, 2023.

EGU23-8038 | ECS | Orals | AS5.13 | Highlight

Stabilized Criegee Intermediates are important nocturnal oxidants in the summertime air of the Indo-Gangetic Plain. 

Muhammed Shabin, Ashish Kumar, Haseeb Hakkim, Yinon Rudich, and Vinayak Sinha

Night-time oxidation significantly affects concentrations of both primary and secondary air pollutants but is poorly constrained over South Asia. Here, we investigate the chemistry, formation and abundance of Stabilized Criegee Intermediates (SCI) in the summertime air of the Indo-Gangetic Plain using measurements of its precursors and sinks. This includes ethene, propene, 1-butene, cis-2-butene, trans-2-butene, 1-pentene, cis-2-pentene, trans-2-pentene, and 1-hexene for which this work also reports the first summertime dataset from the IGP. Ethene, propene, and 1-butene were the highest ambient alkenes in both summer and winter. Morning and noon-time concentrations in summer were ~5.6 and ~3.3 times higher relative to winter, suggesting stronger alkene emission sources in summer. Applying chemical steady-state to the measured precursors, the average calculated SCI concentrations were 4.5 (± 3.8) × 103 molecules cm-3, with Z-CH3CHOO (55 %) as the major SCI. SCI production rates drove ambient SCI with Z-RCHOO (35 %) and α-pinene derived PINOO (34 %) as the largest contributors to the SCI production rate of 7.8 × 105 molecules cm-3 s-1. Peak SCI occurred during evenings. All SCI loss was dominated (>70 %) by unimolecular decomposition or reactions with water vapour. Pollution events influenced by crop biomass fires resulted in significantly elevated SCI production (2.1 times higher relative to non-polluted periods) reaching as high as (7.4 ± 2.5) × 105 molecules cm-3 s-1. Among individual SCI species, Z-CH3CHOO was highest in all the plume events with a contribution of at least ~41 % and among alkenes, trans-2-butene was the highest contributor to P(SCI) in plume events with values ranging from 22-32 %. SCIs dominated the night-time oxidation of sulphur dioxide with rates as high as 1.5 (± 1.3) × 104 molecules cm-3 s-1at midnight, suggesting this pathway could be a significant source of fine mode sulphate aerosols over the Indo-Gangetic Plain, especially during summertime pollution episodes.

How to cite: Shabin, M., Kumar, A., Hakkim, H., Rudich, Y., and Sinha, V.: Stabilized Criegee Intermediates are important nocturnal oxidants in the summertime air of the Indo-Gangetic Plain., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8038, https://doi.org/10.5194/egusphere-egu23-8038, 2023.

Over the past decade the air pollution problem in the bowl-shaped Kathmandu Valley in Nepal – South Asia’s Mini-Mexico City – has become one of the most studied in the region.  Several international field campaigns resulted  50+ journal papers, while three separate networks now provide live air quality data to policymakers and the public.  They valley’s air pollution meteorology, emissions, ozone chemistry, aerosol chemical composition, health impacts, and the role of pollution transport have all been studied in detail.  At the same time, interdisciplinary task forces have laid out clear regulatory priorities and action plans for the Kathmandu Valley. 

Yet except for a decline in coarse dust (due to more roads getting paved), air quality has not improved in the Kathmandu Valley. Regulatory interventions have mostly been spontaneous, devoid of expert inputs, and short-lived.  There exists today sufficient scientific understanding to design a sophisticated regulatory framework that would respond to changing situations in real time to maintain the valley’s air quality.  But today that is just a dream.  

As a front-row participant in the design of the field campaigns in the Kathmandu Valley, in policy making, and most recently in alternative politics, the author has unique insights into challenges that need to be overcome for there to be serious government action to clean up the Kathmandu Valley’s air.  At EGU he will share his insights into which scientific results did or did not end up being useful in shaping the public policy narrative, and why.  He will conclude his presentation by taking the lessons from the Kathmandu Valley from the past decade to provide general principals for other cities with air pollution problems but little data.

How to cite: Panday, A.: The Kathmandu Valley as a science-policy laboratory: When science is insufficient to achieve clean air, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8285, https://doi.org/10.5194/egusphere-egu23-8285, 2023.

EGU23-8342 | Orals | AS5.13 | Highlight

Can India leapfrog into a clean air future – perspectives from measurements, source-receptor modelling and emission inventories 

Baerbel Sinha, Haseeb Hakkim, Gaurav Sharma, Pooja Chaudhary, Ashish Kumar, Harshita Pawar, Praphulla B. Chandra, and Vinayak Sinha

India struggles with frequent exceedances of the ambient air quality standard for particulate matter, ozone and benzene. The situation in the Indo-Gangetic plain (IGP) is particularly severe during post monsoon and winter season.

We show that despite strong governmental efforts to make clean energy accessible and affordable, residential solid fuel usage is still the largest source of particulate matter pollution and carcinogenic benzene in India. Particularly cow dung as a cooking and heating fuel contributes disproportionally to the residential sector emissions and India’s air quality challenge. In addition, crop residue burning, open burning of waste, solid fuel usage in industrial boilers, and power generation units also contribute significantly to the particulate matter and benzene emissions over the region. In urban agglomerations, transport sector emissions aggravate the already poor air quality further.

In this talk we present several recently updated gridded emission inventories with detailed VOC speciation for these air pollution sources. We also look at future projection under different Shared Socioeconomic Pathways (SSPs) for several sources.

We focus on the most polluted part of the year, namely post-monsoon and winter season, to evaluate and compare these updated emission inventories against other available emission inventories and measurements studies. We find that that existing inventories tend to underestimate the magnitude of residential sector emissions and their strong seasonality. The use of solid fuels for heating purposes results in a strong temperature induced emission feedback that can aggravate the wintertime fog. Existing inventories also underestimate the magnitude of crop residue burning emissions and lack open waste burning as a source.

A combination of measurement-based assessments and emission inventories for different air quality intervention strategies are used to evaluate a number of possible air quality interventions for their potential impact. We specifically look at the sectoral coupling between the residential sector, waste management, crop residue management, and the transport sector to propose interventions that maximize air quality gains.

How to cite: Sinha, B., Hakkim, H., Sharma, G., Chaudhary, P., Kumar, A., Pawar, H., Chandra, P. B., and Sinha, V.: Can India leapfrog into a clean air future – perspectives from measurements, source-receptor modelling and emission inventories, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8342, https://doi.org/10.5194/egusphere-egu23-8342, 2023.

EGU23-8701 | ECS | Posters virtual | AS5.13

Carbonaceous Aerosol Characterization and their Association with Meteorological Parameters at an Industrial Region in Delhi, India 

Saurabh Sonwani, Pallavi Saxena, and Anuradha Shukla

The present study has been carried out focusing on the characterization of carbonaceous aerosol near an industrial region in New Delhi, India. It also determines the variation of carbonaceous species during the summer monsoon (SM) and winter monsoon (WM), interprets the morphological description of aerosol particles, identifies the major sources of carbonaceous aerosol, and recognizes the role of meteorological parameters in terms of OC-EC variability. PM10 samples were collected and atmospheric organic carbon (OC) and elemental carbon (EC) were determined during SM and WM seasons in 2016–2017. Owing to high combustion and emission activities in the industrial area, the OC concentration was 70.3±53.7 and 94.3 ± 40.3 μgC/m3 during the SM and WM, respectively, with an overall average of 79.9±44.9 μgC/m3, and the EC concentration was 50.8 ± 53 and 62.6±49.8 μgC/m3, respectively, with an overall average of 58.3±46.7 μgC/m3. The morphological observations of collected particles were studied and the char/soot particles, iron-rich particles, and aggregates of calcium sulfate particles were observed during both seasons. The OC/EC ratio suggested the presence of mixed sources at the industrial location, predominated by industry and motor vehicle emissions. The relationship of carbonaceous aerosol with meteorological variables was also studied, and it was found that temperature, atmospheric stability, wind direction, and rain intensity significantly affect the levels of OC as compared to that of EC during both seasons. Furthermore, it was also noticed that high-intensity rain decreases the carbonaceous aerosol significantly and vice versa.

How to cite: Sonwani, S., Saxena, P., and Shukla, A.: Carbonaceous Aerosol Characterization and their Association with Meteorological Parameters at an Industrial Region in Delhi, India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8701, https://doi.org/10.5194/egusphere-egu23-8701, 2023.

EGU23-8742 | Orals | AS5.13

Air quality studies using long-term observations at Welgegund, South Africa 

Ville Vakkari, Kerneels Jaars, Miroslav Josipovic, Markku Kulmala, Lauri Laakso, Tuukka Petäjä, and Pieter G. van Zyl

Quality-controlled long-term measurements of atmospheric composition are central in identifying the sources and processes that are most important for air quality in a particular environment. In South Africa, continuous measurements of various atmospheric constituents have been carried out at the Welgegund measurement station since May 2010 in close collaboration between North-West University, Finnish Meteorological Institute and University of Helsinki. Welgegund is a regionally representative continental site approx. 100 km west of Johannesburg with no local sources. Before Welgegund, measurements were operated at Marikana village, which is an urban location with large industrial point sources in the vicinity. At both sites measurements included particulate matter smaller than 10 µm in diameter (PM10), black carbon (BC) and trace gases (SO2, NO, NOx, O3, CO) among others.

Numerous industrial point sources surrounding Johannesburg result in elevated NOx and SO2 levels in the region, but these concentrations remain below air quality standards. On the other hand, PM10 does exceed 50 µg m3 rather frequently and more often at Marikana than at Welgegund. However, strong correlation with CO suggests that the periods of elevated PM10 are related to incomplete combustion rather than the industrial emissions at both locations. At Marikana the major source appears to be domestic heating during winter time, while at Welgegund landscape fires seem more important. Also, O3 exceeds air quality standards frequently at both sites and the highest O3 cases appear to be linked with landscape fires. Furthermore, our observations suggest that O3 formation is not NOx-limited but rather VOC-limited.

How to cite: Vakkari, V., Jaars, K., Josipovic, M., Kulmala, M., Laakso, L., Petäjä, T., and van Zyl, P. G.: Air quality studies using long-term observations at Welgegund, South Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8742, https://doi.org/10.5194/egusphere-egu23-8742, 2023.

EGU23-9708 | ECS | Posters on site | AS5.13 | Highlight

Development of a low-cost black carbon sensor for air quality monitoring in Ghana               

Nyasha Milanzi, Stewart Isaacs, and Heather Beem

The International Energy Agency estimates that 970 million Africans use biomass for cooking [1], emissions from which expose them to pollutants like particulate matter (PM) and black carbon (BC). Due to its small size (range: 135 - 145 nm) [2], BC is easily inhalable and presents worse health impacts than many other PM species [3]. A considerable challenge is accessing affordable standard BC sensors; most cost US$3,000 to US$20,000 and are thus too expensive to deploy in large numbers [3] to provide high spatial resolution. Therefore, in recent low-cost air pollution sensor networks, there has been a noticeable gap in the absence of a BC emissions inventory [3]. In this research, we have designed a BC sensor that costs less than US$200 and incorporates a rechargeable battery & LoRa communication to enable long-term, remote operation. Leveraging Pugh Charts, we chose materials and components available in Ghana. Drawing from recent studies in developing low-cost BC sensors, the sensor uses an optical measurement technique to measure the absorption coefficient from the degree of weakened light intensity of 880 nm wavelength to invert the BC aerosol concentration. We chose absorption measurement at 880 nm to define BC concentration because, at this wavelength, BC is the predominant PM species to absorb light [3]. We developed a low-fidelity prototype using a flame sensor to test the optical measurement concept. The flame sensor detected light wavelengths between 760 nm – 1100 nm with high sensitivity and a resolution of 0.98 mV using a 12-bit analog-to-digital converter (ADC). In the next prototype stage, we aim to achieve a resolution of less than 0.1 mV leveraging a 16-bit ADC. Additionally, components will be integrated to enable the measurement of carbon monoxide (CO) and nitrogen dioxide (NO2) concentrations as well, leveraging the MiCS-4514 sensor module. Simultaneous detection of high BC & CO and BC & NO2 concentrations can aid in indicating nearby biomass combustion and diesel engine emissions, respectively [4], thus painting a complete picture of major BC pollution drivers. These emissions data will aid policymakers to devise data-driven solutions to BC-associated human health impacts.

References 

[1] IEA (2022), Africa Energy Outlook 2022, IEA, Paris https://www.iea.org/reports/africa-energy-outlook-2022, License: CC BY 4.

[2] Y. Cheng, S.-M. Li, M. Gordon, and P. Liu, "Size distribution and coating thickness of black carbon from the Canadian oil sands operations," Atmospheric Chem. Phys., vol. 18, no. 4, pp. 2653–2667, Feb. 2018, doi: 10.5194/acp-18-2653-2018.

[3] J. J. Caubel, T. E. Cados, and T. W. Kirchstetter, “A New Black Carbon Sensor for Dense Air Quality Monitoring Networks,” Sensors, vol. 18, no. 3, Art. no. 3, Mar. 2018, doi: 10.3390/s18030738.

[4] B. Alfoldy, A. Gregorič, M. Ivančič, I. Ježek, and M. Rigler, "Source apportionment of black carbon and combustion-related CO2 for the determination of source-specific emission factors," Aerosols/In Situ Measurement/Instruments and Platforms, preprint, Apr. 2022. doi: 10.5194/amt-2022-53.



 

How to cite: Milanzi, N., Isaacs, S., and Beem, H.: Development of a low-cost black carbon sensor for air quality monitoring in Ghana              , EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9708, https://doi.org/10.5194/egusphere-egu23-9708, 2023.

EGU23-9753 | Orals | AS5.13

Internet of Things Lab for Air Quality Monitoring 

Bertrand Tchanche and Ibrahima Fall

Anthropogenic activities emit particulate matter (PM) and gaseous substances that are harmful. PM has adverse effects on different parts of the body. Atmospheric pollution is a global threat with an increasing social and economic costs. Poor air quality is a concern in African cities, but governments have been too slow to react, one of the reasons being the scarcity of data on different air pollutants. Instruments based on low-cost sensors and Internet of Things are being considered as solution to evaluate the concentration of different pollutants. Increasing number of manufacturers are proposing sensing devices with good accuracy. Low-cost sensors are an alternative to expensive high graded equipment. They are cheap and can be easily deployed. Here we present the IoT4AQ project. It is funded by the International Astronomical Union (IAU). The main objective is to organize training sessions for researchers and students on the design and implementation of low-cost sensors for air quality monitoring. The project will use astronomy instrumentation knowledge and skills. Participants will be trained in IoT techniques showing how to build low-cost sensors-based instruments and deploy them. The project starts on February 2023, will last for two years and trainers will be invited on various aspects of the trainings. Two hands-on trainings and two online seminars will be organized each year. The project will be implemented in Senegal and the first year will see the participation of local trainees and in the second phase it will open to participants from other African countries. Specific objectives are: (1) organize hands-on trainings and online seminars on IoT and air quality monitoring, (2) train researchers, teachers, and students on various aspects of air quality monitoring and (3) improve Physics education in Africa through low-cost sensors and IoT. Expected outcome are as follows: (1) train a minimum of 100 participants on IoT and air quality monitoring; (2) improve the experimental skills of participants; and (3) increase awareness of the threat that represents atmospheric pollution.

How to cite: Tchanche, B. and Fall, I.: Internet of Things Lab for Air Quality Monitoring, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9753, https://doi.org/10.5194/egusphere-egu23-9753, 2023.

EGU23-9929 | Orals | AS5.13 | Highlight

Enhanced Quantification and Source Apportionment Capabilities of a New Higher-Resolution Aerosol Chemical Speciation Monitor for Long-Term Measurements of Non-Refractory Aerosol 

Philip Croteau, Benjamin Nault, Manjula Canagaratna, Edward Fortner, Andrew Lambe, Harald Stark, Donna Sueper, Benjamin Werden, Anandi Williams, Leah Williams, Douglas Worsnop, and John Jayne

Long-term measurements of the composition and mass concentration of particulate matter (PM) are essential for source apportionment, epidemiological studies, and air quality trends. Over the past ten years, the Aerosol Chemical Speciation Monitor (ACSM) has been widely used for long-term, in situ, high time resolution measurements. However, to date there are limited measurements with these instruments in Africa and South/Southeast Asia. The measurements that have been made in these regions suggest the presence of varied and complex sources. Current ACSMs have unit mass resolution (UMR), which impacts detection limits and separation and identification of ions, limiting source apportionment. Here, we present a new instrument, the Time-of-Flight ACSM with eXtended resolution (TOF-ACSM-X) with updated analysis software (Tofware) to allow for high-resolution peak fitting. The TOF-ACSM-X has a mass resolution of ~2000 m/Δm, which is approximately an order of magnitude higher than the other versions of the ACSM. This enhanced resolution improves ammonium detection limits by approximately 2-orders of magnitude, from ~0.200 μg m-3 to ~0.008 μg m-3 (TOF-ACSM versus TOF-ACSM-X, respectively), for 15-minute integration times. Intercomparisons of the TOF-ACSM-X with other measurements show improved performance in source apportionment and elemental analysis.

How to cite: Croteau, P., Nault, B., Canagaratna, M., Fortner, E., Lambe, A., Stark, H., Sueper, D., Werden, B., Williams, A., Williams, L., Worsnop, D., and Jayne, J.: Enhanced Quantification and Source Apportionment Capabilities of a New Higher-Resolution Aerosol Chemical Speciation Monitor for Long-Term Measurements of Non-Refractory Aerosol, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9929, https://doi.org/10.5194/egusphere-egu23-9929, 2023.

EGU23-10315 | ECS | Posters virtual | AS5.13 | Highlight

Air Quality Study to Analyze PM2.5 Sources and their Possible Mitigation pathways in Nairobi 

Ezekiel Waiguru Nyaga, Matthias Beekmann, Subramanian R., Mike R. Giordano, Savannah Ward, Daniel Westervelt, Michael Gatari, Moses Njeru, John Mungai, Godwin Opinde, Tedy Mwendwa, Albert Presto, Emilia Tjernstrom, and Faye v. McNeill

Anthropogenic activities in cities can be major sources of fine particulate matter which contribute significantly to increased mortality and disease. In rapidly developing cities of eastern Africa, lack of routine air pollution measurements have hampered formulation of actionable air quality policies. This study integrates ground-based observations of low-cost sensors (LCS) and regional chemical transport modelling (CHIMERE, https://www.lmd.polytechnique.fr/chimere/) to quantify spatial-temporal variability of PM2.5 and NO2 concentrations, primary/secondary aerosol loading, local versus regional pollution share, and  contribution of key economic sectors. Prior to deployment, LCS PM2.5 mass concentrations were calibrated with a reference instrument (BAM-1020), while LCS NO2 measurements could only be normalized internally. Between June-December 2021 period, sensors were deployed at urban background site (IPA, and UoN), urban traffic sites (KUCC, BuruBuru, and Marurui), and a peri-urban site (Ngong). BuruBuru and Marurui are in addition exposed to nearby residential emissions. Daily average PM2.5 varied from 26.3 to 27.6 µg/𝑚3 at traffic sites, 17.8 to 21.7 µg/𝑚3 at urban background sites,  while it was 20.3 µg/𝑚3 at peri-urban site. PM2.5 and NO2 diurnal patterns mimicked daily traffic cycle with constantly higher evening peaks compared to morning peaks indicating residential emissions. A link of  “large pollution” events with PM2.5 concentrations above 50 µg/m3 and low wind speeds (<4 m/s) was made evident and points to local sources. Preliminary modelling results of a nested CHIMERE run over Eastern Africa down to 2 km horizontal resolution show satisfying results when compared to measurements. They point to a strong urban source of fine particle pollution, with the strongest mass contribution of primary organic aerosol. Analysis of final model output will help to better understand air quality dynamics in Nairobi and ultimately help evaluation of possible future emission mitigation scenarios.

How to cite: Nyaga, E. W., Beekmann, M., R., S., Giordano, M. R., Ward, S., Westervelt, D., Gatari, M., Njeru, M., Mungai, J., Opinde, G., Mwendwa, T., Presto, A., Tjernstrom, E., and v. McNeill, F.: Air Quality Study to Analyze PM2.5 Sources and their Possible Mitigation pathways in Nairobi, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10315, https://doi.org/10.5194/egusphere-egu23-10315, 2023.

EGU23-10366 | ECS | Orals | AS5.13 | Highlight

Air Quality Monitoring & Data Sharing in Africa and South/Southeast Asia: A Scoping Review 

Colleen Marciel Rosales, Viraj Sawant, Margaret Isied, Russ Biggs, and Chris Hagerbaumer

Reliable data on air pollution are fundamental to understanding and taking corrective action to improve air quality. In addition, where data are shared with the public, everyone across private, public and civil society can innovate, collaborate, and apply effective solutions towards clean air. However, air quality (AQ) monitoring, as well as AQ data sharing, are both limited in many low- and middle-income countries. While a few reviews of air quality in Africa and South/Southeast Asia exist, a review focused on monitoring capabilities and data sharing is necessary, especially with growth in non-traditional, non-reference monitoring technologies. We conducted a scoping review based on the Arksey and O’Malley methodological framework along with updates proposed in literature consistent with the PRISMA-ScR (Scoping Review Extension). We implemented a search strategy that was iteratively refined to review diverse sources including scientific and gray literature, air quality data aggregators, and publicly internet-available documents of national governments. We complemented our findings by consulting with experts. We found that AQ monitoring in Africa and South/Southeast Asia is lacking, with very few countries having reference-grade monitoring programs and few sharing the data they collect publicly. We recommend leveraging emerging lower-cost alternatives along with traditional (“reference”) technologies. This is supported by our review of emerging approaches and highlighted case studies of countries like Uganda and Cambodia that have adopted such approaches. 

How to cite: Rosales, C. M., Sawant, V., Isied, M., Biggs, R., and Hagerbaumer, C.: Air Quality Monitoring & Data Sharing in Africa and South/Southeast Asia: A Scoping Review, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10366, https://doi.org/10.5194/egusphere-egu23-10366, 2023.

EGU23-10385 | Orals | AS5.13 | Highlight

Investigating expanding air pollution and climate change on the African continent using TROPOMI data 

Pieternel Levelt, Deborah Stein, Sara-Eva Martinez, Wenfu Tang, Helen Worden, Louisa Emmons, Benjamin Gaubert, Henk Eskes, Ronald van der A, and Pepijn Veefkind

In the coming decades, a large increase in population is expected to occur on the African continent, leading to a doubling of the current population, which will reach 2.5 billion by 2050. At the same time, the African continent is experiencing substantial economic growth. As a result, air pollution and greenhouse gas emissions will increase considerably with expected health impacts on the African population. The impact of wildfires also needs to be carefully assessed. Will the frequency of fire episodes increase? And how will this perturbation compare with anthropogenic emissions in urban areas? In the decades ahead, Africa’s contribution to climate change and air pollution will become increasingly important.  

Time has come to address the changing role of Africa in understanding and quantifying global environmental change.  What can we learn from the new TROPOMI satellite data for Africa, in combination with emerging modelling efforts including the MUSICA development at NCAR and the development of inverse modelling techniques? How can we deal with the lack of surface observations in many areas of Africa?

We will show several recent achievements related to Africa, using space observations and modeling approaches as a contribution towards the development of an integrated community effort to better characterize air quality and climate-related processes in this continent.  This presentation will mainly focus on the potential of the use of TROPOMI data for Africa Research.

How to cite: Levelt, P., Stein, D., Martinez, S.-E., Tang, W., Worden, H., Emmons, L., Gaubert, B., Eskes, H., van der A, R., and Veefkind, P.: Investigating expanding air pollution and climate change on the African continent using TROPOMI data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10385, https://doi.org/10.5194/egusphere-egu23-10385, 2023.

EGU23-10764 | ECS | Posters on site | AS5.13

PM2.5 Reconstruction using MERRA-2 using Ensemble Machine Learning Approach and Long-term Analysis for India (1980-2021) 

Vikas Kumar, Vasudev Malyan, and Manoranjan Sahu

Particle exposure affects more humans globally than any other air pollutant. However, due to expensive instruments and infrastructural deficiency, a high spatiotemporal network of monitoring stations is not possible, leading to data-scarce regions. Satellite and reanalysis datasets can be implemented to estimate particulate matter, but they do not provide surface concentration and needs to be reconstructed from the components. In this study, a machine learning (ML) framework is implemented to reconstruct PM2.5 from MERRA-2 data components, namely black carbon (BC), organic carbon (OC), dust (DUST), sea salt (SS), and sulfate (SO4). The ground level and respective MERRA-2 data were collected from India's 335 continuous ambient air quality monitoring stations (CAAQMS) for 2017-2021 at hourly resolution. Random forest (RF) performs better with train and test scores (R2) of 0.86 and 0.74, respectively, while the empirical equation provides an R2 of only 0.27 on test data. The estimated PM2.5 for Indian states from 1980-2021 indicates a significant increase in most cases. However, states in the Indo-Gangetic plain such as Delhi, Punjab, Haryana, and Uttar Pradesh are the most polluted regions of India. The major shift in concentration is from 2000 onwards, which can be seen as a direct result of the economic liberalization policies implemented in 1991. The results provide evidence for the limitations of the broad application of the empirical equation and the feasibility of ML algorithms as a potential reconstruction technique for developing robust and accurate region-specific models from MERRA-2 data.

How to cite: Kumar, V., Malyan, V., and Sahu, M.: PM2.5 Reconstruction using MERRA-2 using Ensemble Machine Learning Approach and Long-term Analysis for India (1980-2021), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10764, https://doi.org/10.5194/egusphere-egu23-10764, 2023.

EGU23-11184 | ECS | Orals | AS5.13 | Highlight

Has the redressal mechanism for air pollution-related cases in India evolved since the inception of the National Green Tribunal? 

Abinaya Sekar, Muhammed Siddik Abdul Samad, and George K Varghese

The National Green Tribunal (NGT) was established in accordance with the National Green Tribunal Act, 2010. NGT is the specialized judicial body, consisting of technical members and judicial members, constituted for adjudicating environmental cases and reducing the burden of litigation in other courts in the country. In matters involving air pollution, anyone seeking relief or compensation for environmental damage concerning issues included in the Air (Prevention and Control of Pollution) Act of 1981 may approach the tribunal. Before the establishment of the NGT, the country’s apex court played a vital role in delivering land-mark decisions concerning air pollution. The objective of the current study is to assess if the involvement of technical experts in the tribunal has improved the redressal mechanism. The judgments were reviewed in SCC online’s case finder and NGT official portal. The methodology involved analyzing cases decided by the NGT for five indicators that signal the use of technical expertise in decision-making. These indicators are (i) scientific/ technical content of the ratio decidendi, (ii) technical investigation of the case directly by NGT, including site visits by its technical experts, (iii) Assessment of technical reports directly by NGT, without the help of external experts (iv) insistence by NGT on studies using latest techniques as part of the investigation (v) Evaluating reversal of NGT verdict following the Supreme Court appeal on technical grounds. In general, this study assesses the role of the scientific experts as decision-makers in the environmental redress process. Reported cases, supported by existing literature show that scientific experts had a significant policy impact, which is crucial in air quality management. A guideline document, similar to the Environmental crime investigation manual of INTERPOL can improve the situation further by helping the investigator choose the suitable approach for a given scenario. 

 

How to cite: Sekar, A., Samad, M. S. A., and Varghese, G. K.: Has the redressal mechanism for air pollution-related cases in India evolved since the inception of the National Green Tribunal?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11184, https://doi.org/10.5194/egusphere-egu23-11184, 2023.

EGU23-11237 | ECS | Posters virtual | AS5.13

Statistical Trends and Characterization of Atmospheric Pollutants Levels Using Low-Cost and Satellite Total Column Data in the Greater Accra Metropolitan Assembly (GAMA), Ghana 

James Nimo, Azoda Koffi, Alabi Omowumi, Benjamin Essien, Emmanuel K.-E Appoh, Ramachandran Subramanian, Nana Ama Browne Klutse, and Allison Felix Hughes

High concentration of pollutants is known to have adverse implication on climate and public health. Every year, poor air quality is responsible for about 7 million deaths globally as it is estimated by the WHO. In sub- Saharan Africa with increasing population growth and urban emissions, the situation is no different since poor air quality is increasing at an alarming rate. Therefore, regular monitoring is required to assess the levels of pollutant in both local and regional scale. However, this is scarce in sub-Saharan Africa as it is expensive to acquire, install and maintain large number of high-grade air quality monitoring sensors. And thus, has limited studies to investigate associations between particulates with aerodynamic diameter less than 2.5 microns (PM2.5) and gas pollutants like nitrogen dioxide (NO2) and ozone (O3) for a long time in sub-Saharan African cities. Hence, this study sort to bridge this gap by utilizing 5 Clarity Node-S sensors PM2.5 data, total column particulates or Aerosol Optical Depth (AOD), NO2 and O3 data from satellites over 5 different Ghana Environmental Protection Agency (GEPA) air quality  traffic stations in the Greater Accra Metropolitan Assembly (GAMA). AOD, NO2 and O3 were retrieved from NASA Moderate Resolution Imaging Spectro-Radiometer (MODIS) Terra and Ozone Monitoring Instrument (OMI). Long-term trends over the 5 stations on (25 x 25) km resolution for OMI and (50 x 50) km resolution for MODIS Terra AOD from 2012 to 2021 were assessed using Mann-Kendall test to ascertain the impact of population growth coupled with increasing traffic, biomass burning and climate change on air quality for the past decade in the GAMA. Further, characterization of PM2.5, AOD, NO2, and O3 levels in the GAMA was also assessed while the Pearson correlation coefficient was used to find correlations between the pollutants. Overall, there was an increasing trend in NO2 (p < 0.05), no trend in O3 (p > 0.05) and a decreasing trend in AOD (p < 0.01). Pearson correlation coefficients between PM2.5 data and MODIS Terra AOD on (50 x 50) km resolution across the stations were (R2 = 0.72, 0.72, 0.67, 0.58 and 0.57) respectively. Correlation coefficient between column NO2 and O3 was (R2 = -0.83 ± 0.030, p < 0.01), AODand O3 (R2 = -0.43 ± 0.003, p < 0.01) and NO2 and AOD(R2 = 0.21 ± 0.010, p > 0.01). PM2.5, AOD and NO2 levels were generally high during the dry season while high concentrations of O3 were observed in the wet season across the stations. Also, PM2.5 daily mean level of 32.8 μgm-3 for 25 months between 2018 and 2021 was more than twice WHO recommended daily mean level of 15 μgm-3. Again, an increasing and decreasing trends in NO2 and AOD levels shows that sources of poor air quality may be shifting from the usual biomass burning to traffic emissions. High population growth with increasing traffic and climate change in growing sub-Saharan African cities requires urgent policy measures and regulations as ground air quality monitoring sensors are limited.

How to cite: Nimo, J., Koffi, A., Omowumi, A., Essien, B., K.-E Appoh, E., Subramanian, R., Klutse, N. A. B., and Hughes, A. F.: Statistical Trends and Characterization of Atmospheric Pollutants Levels Using Low-Cost and Satellite Total Column Data in the Greater Accra Metropolitan Assembly (GAMA), Ghana, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11237, https://doi.org/10.5194/egusphere-egu23-11237, 2023.

EGU23-11384 | ECS | Orals | AS5.13 | Highlight

Impact of planetary boundary layer in dense haze /smog event over South Asian Mega City; Lahore Pakistan 

Imran Shahid and Muhammad Imran Shahzad

Air quality over North Eastern region of Pakistan is rapidly worsening over the years, especially over Lahore and adjacent areas reporting world record levels of pollutant concentrations including highest particulate matter (PM) levels during the autumn and winter seasons. Meteorological parameter plays an important role in extreme pollution episodes. In order to study the impact of meteorological condition such as planetary boundary layer (PBL) an intensive PBL measurements were conducted over Lahore from October 2019 to March 2021 using LUFT CHM15K Ceilometer LIDAR. The impacts of PBL structure on heavy haze pollution and the relationship with PM2.5 concentrations were studied. The boundary layer height drops clearly during winter period (December 2019 and 2020, usually lower than 500m. The PM2.5 concentrations increases when the PBL drops and vice versa. Key finding in this study is that the dynamics of the Planetary Boundary Layer (PBL) change significantly during heavily polluted days during intense autumn / winter smog periods, which indicates the role of aerosols in influencing meteorological conditions, besides having other impacts in the region of study.   

How to cite: Shahid, I. and Shahzad, M. I.: Impact of planetary boundary layer in dense haze /smog event over South Asian Mega City; Lahore Pakistan, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11384, https://doi.org/10.5194/egusphere-egu23-11384, 2023.

EGU23-11895 | ECS | Orals | AS5.13 | Highlight

Densification of air quality monitoring in Nigeria: Progress and challenges 

Samuel Ogunjo, Babatunde Rabiu, Ibiyinka Fuwape, Gregory Jenkins, and Aderonke Obafaye

Pollution is a major problem in developing countries.  There has been much studies on water pollution and its relation to communicable diseases with little attention to air pollution.  Air quality problem in sub-Saharan Africa is pervasive due to lack of awareness and paucity of reliable data.  The lack of reliable data has limited our underestanding and quantification of its impact on the population.  To address this problem, the the Centre for Atmospheric Research, Nigeria, and the Alliance for Education, Science, Engineering and Design in Africa of the Penn State University collaborated to densify air quality monitoring networks in Nigeria.  The programme has succeeded in deploying over 70 monitoring networks across the country within the last two years. Using data from the network, the impact of air quality especially in relation to diseases have been assessed within Nigeria.   This approach has revealed significant association between air quality and COVID-19 infections.  Furthermore, the available data has helped in understanding the sources of air pollution in different regions of the country.  This is helping in formulating environmental policy, planning, and monitoring for reduction of air pollution.  In this presentation, the progress and challenges in the densification of air quality monitoring stations across the country will be presented.

How to cite: Ogunjo, S., Rabiu, B., Fuwape, I., Jenkins, G., and Obafaye, A.: Densification of air quality monitoring in Nigeria: Progress and challenges, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11895, https://doi.org/10.5194/egusphere-egu23-11895, 2023.

EGU23-12426 | Orals | AS5.13 | Highlight

Predicting PM2.5 based on micro-satellite imagery and low-cost sensor network using CNN-RT-RF Joint Model 

Sachchida Tripathi, Vaishali Jain, Avideep Mukherjee, Soumya Banerjee, Piyush Rai, and Sandeep Madhwal

Presently, 17 out of 30 Indian cities are ranked worst in air quality around the globe due to high emissions of fine particulate matter, PM2.5 (particles less than 2.5 µm diameter). These particles can reach deeper into the lungs and cause serious health problems, including cardiovascular obstructive pulmonary disease, lung cancer, stroke, and asthma. To take prompt actions towards mitigating and controlling the adverse effects of air pollution, it is important to monitor the ambient air quality regularly and at the neighbourhood level. However, the distribution of the regulatory central ambient air quality monitoring stations (CAAQMS) in India is sparse, and many states and cities lack any regulatory stationary monitors (RSMs). Conventional air quality monitoring techniques are inefficient and incapable of mapping PM2.5 at a sub-Km level. The heterogeneity of PM2.5 concentrations at large-scale and high spatial resolution has numerous applications in epidemiological studies, detecting hotspots within neighbourhoods and implementing policy interventions at local, regional and city levels. Therefore, an integrated monitoring framework is needed to fill gaps in the existing air quality measurements. This study proposes a tribrid approach of using the low-cost sensor (LCS) network to supplement the RSMs in generating more ground-truth PM2.5 concentrations along with high-resolution micro-satellite imageries (PlanetScope, ~3m/pixel) to estimate and generate the PM2.5 concentration maps at the sub-Km level (~500m by 500m). In the present study, an extensive LCS network of 70 nodes deployed at optimally selected locations within and around the boundaries of Lucknow city, Uttar Pradesh, India, along with six existing RSMs for one year (December 2021 onwards). It has increased monitoring ten folds at a moderate cost, covering remote urban and rural areas. The locations of these LCS and RSMs (76 nodes) have been used to precisely extract the daily (every day Dec 2021-2022) high-resolution satellite imageries by forming the area of interest (AOI) of size 224 by 224-pixel around the node while keeping the node in the middle of AOI. These imageries have been labelled with the ground truth PM2.5  values from the nodes with geographical location and meteorological parameters such as relative humidity, atmospheric temperature, and barometric pressure. These labelled data are then fed into a deep learning CNN-RT-RF (Convolutional neural network- random trees-random forest) joint model to predict PM2.5 at sub-Km level, which provides RMSE~ 2.74 and 7.50 for training and test data, respectively. The study further compares model performance with existing datasets of Delhi and Beijing. The results show that the predicted PM2.5 using satellite imagery shows a strong co-relation with LCS and RSMs network and thus can be used as a soft sensor for large-scale monitoring. This study is the first study to integrate LCS sensor data with microsatellite imagery, leveraging over costly, conventional methods using machine learning approaches.

 

How to cite: Tripathi, S., Jain, V., Mukherjee, A., Banerjee, S., Rai, P., and Madhwal, S.: Predicting PM2.5 based on micro-satellite imagery and low-cost sensor network using CNN-RT-RF Joint Model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12426, https://doi.org/10.5194/egusphere-egu23-12426, 2023.

EGU23-12530 | ECS | Posters on site | AS5.13

Current gaps in air quality management over India: A study on stakeholder consultation 

Arindam Roy, Athanasios Nenes, and Satoshi Takahama

As a part of the National Clean Air Program (NCAP) in India, non-attainment cities have begun implementing city-wide action plans for air quality monitoring and management. Air quality action plan implementation is supported by a collaboration of academic institutions, non-governmental organizations, and governmental bodies,  but each of these stakeholder groups perceives different challenges in this effort. Here, we report on the results of a stakeholder consultation study conducted through semi-structured anonymous interviews to identify varying perspectives on the key challenges. Three types of stakeholders were selected for the interview; a) academic researchers (10 participants); b) experts from non-governmental agencies (10 participants), and, c) group leads from government implementation bodies (8 participants). The governmental stakeholders are from state agencies and municipalities that are actually responsible for the ground implementation of air quality control. The questionnaire was broadly divided into three categories; a) the role and sufficiency of current air quality monitoring operations and NCAP; b) how information is shared or used by different agencies, and, c) how the research data is being used in implementation (“data to action”).

 

The majority of stakeholders (~95%) identify NCAP and its resource support as the driving force for the recent implementation on air quality. They also raise concerns regarding the post-funding sustainability of implementation strategies beyond the five-year lifetime of NCAP. According to implementation agency leads, there are three types of data required for action: 1) the proportion of transported and local pollutants; 2) what implementation will improve the air quality at the neighborhood scale for a particular city; and 3) how to evaluate the effectiveness of an ongoing implementation project. Receptor modeling studies currently conducted to identify major source classes in the study area often do not answer these questions; most participants (irrespective of stakeholder types) state that receptor modeling is costly and often unaffordable. We found that only a fraction of non-attainment cities is interested to use allocated funds for air quality management toward receptor modeling. Instead, building emission inventories followed by numerical modeling are perceived to be a good starting point for actionable information such as identifying prioritized sectors for air pollution management, particularly for Indian cities that lack resources. Regarding monitoring and evaluation strategies, academics and governmental implementation agencies raise concerns about the deployment of low cost sensors (LCS) and satellite data for regulatory purposes, while NGOs are advocating for mainstreaming the LCS measurement. Governmental implementation agencies are neutral about the number of stations or methods of monitoring as they believe measurement is not directly helping in implementation and evaluation.

 

Our study suggests that there is a gap between knowledge generated by academic air pollution research and knowledge required for decision-making by implementation agencies in Indian municipalities. Therefore, we identify a necessity for establishing a fourth type of entity, independent of the three preexisting ones, that transfers actionable information from research institutes to governmental agencies and devise locale-specific strategies for air pollution management. Cooperating among government departments, such entities can further provide unified action plans on air quality, climate change adaptation, and development.

How to cite: Roy, A., Nenes, A., and Takahama, S.: Current gaps in air quality management over India: A study on stakeholder consultation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12530, https://doi.org/10.5194/egusphere-egu23-12530, 2023.

According to WHO, air pollution is associated with 7 million premature deaths annually. Lack of air pollution monitoring systems is one of the major challenges in developing regulations and policies for air pollution control as well as health risk assessments in majority of the developing nations. Ground based monitoring stations are sparsely distributed in major cities only. The major reason for lack of monitoring stations is the heavy cost associated with their establishment and operations, whereas low-cost sensors come with different variety of challenges related to the calibration, accuracy and reliability. This problem could be solved by combining remote sensing data with machine learning to estimate particulate matter concentrations. Modern satellite sensors hold the potential to provide high-quality aerosol optical depth (AOD) data at a resolution of 10m × 10m. Current approaches for estimating particle (PM2.5) concentrations rely on AOD with meteorological data such as relative humidity, ambient temperature, wind speed, etc. However, the prediction accuracy decreases dramatically if these results are extrapolated over a wider timeline and a broader region. This is owing to the fact that traditional methods take many assumptions based on the training data set. We implemented and validated the conventional method of predicting particle concentration to evaluate prediction accuracy using five distinct machine learning models. The light gradient boosting regression model generated the highest prediction accuracy, i.e., 92.46% for a training data set of one year (January 2019 – December 2019) for the city of Mumbai, with a resolution of 0.5° × 0.625° (latitude × longitude). This work presents a hybrid approach combining the physics-based relations and statistical methods, to predict surface level concentration. It uses the vertical distribution of aerosols along with the optical properties like single scattering albedo and angstrom exponent for determining particle characteristics and meteorological parameters for a greater prediction accuracy over a wider timeline and a broader region. Since AOD provides a measure of total particles above a location, we employed data from multi-angular satellite sensor (CALIOPS) to generate vertical distribution profiles and ultimately surface-level concentration. Also, the physics based empirical relations are considered while determining the input parameters for model training, which significantly increases the prediction accuracy of model. When the particle size distribution curve was combined with the surface level concentration from vertical distribution profile, a more accurate surface level PM2.5 concentration was obtained. Unlike previous approaches that make several assumptions based on the location of training data, this method, by removing those assumptions, is valid over a broader area and a wider timescale.

 

How to cite: Moni, M. and Sahu, M.: Development of high-resolution particle concentration prediction model - an application of remote sensing and machine learning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12994, https://doi.org/10.5194/egusphere-egu23-12994, 2023.

EGU23-13204 | ECS | Posters on site | AS5.13

Significance of sources and size distribution on calibration of low-cost particle sensors: Evidence from a field sampling campaign 

Vasudev Malyan, Vikas Kumar, and Manoranjan Sahu

Low-cost sensors (LCS) are gathering the interest of researchers and monitoring agencies worldwide due to their compact size and economic feasibility. However, the data recorded by LCS is often of low quality owing to its calibration dependencies and biases. An intensive field sampling campaign was conducted at five sites inside the IIT Bombay campus to understand the fundamental issues associated with LCS. PA-II and OPC-N2 LCS were collocated with BAM-1020 and OPS- 3330 at the sampling locations for inter-comparison. LCS shows a good correlation with BAM-1020 at sites where the contributing sources produce more particles in the 1–2.5 μm size range than particles in below 1 μm (PM1) and 2.5–10 μm size range. The performance decreased with an increase in mass fractions of PM1 and PM10. The overall performance of both PA-II (R2 = 0.72) and OPC-N2 (R2 = 0.73) are comparable. Both PA-II and OPC-N2 have substandard performance with R2 in the range of 0.30–0.39 and 0.42–0.53 at the construction and main gate site respectively. Comparing the two calibration approaches used in this study indicates the importance of including size distribution parameters in the calibration of LCS. The calibration models were developed for each site and were compared with the general model developed for PA-II and OPC-N2. Results indicate that the site-specific models are in better agreement with the reference instrument than the general calibration model. The number concentration recorded by PA-II was poorly correlated with OPS-3330, especially for particles >1 μm and vice versa for OPC-N2. The particle count for PM > 2.5 μm recorded by PA-II is predominantly zero, which is inconsistent with the mass concentration data recorded by the sensor. The size distribution results indicate that LCS assumes a universal monotonically decreasing function of number concentration with respect to the particle diameter. It is one of the critical problems with LCS measurements as any error in the number measurement is increased 3-fold in the mass conversion. This study shows the need for site-specific robust calibration of LCS based on the particle size distribution and provides a direction in their development.

How to cite: Malyan, V., Kumar, V., and Sahu, M.: Significance of sources and size distribution on calibration of low-cost particle sensors: Evidence from a field sampling campaign, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13204, https://doi.org/10.5194/egusphere-egu23-13204, 2023.

EGU23-13453 | ECS | Posters on site | AS5.13

Characterizing aerosol emissions from traditional clay fired clamp kilns in South Asia 

Anurag Kumar Gupta, Taveen Singh Kapoor, Navinya Chimurkar, Chandra Venkatraman, and Harish C. Phuleria

Fired clay brick kiln (FCBK) industry is one of the unorganized and often overlooked sectors in terms of its regional air quality and health impacts. Approximately 87% of the 1.5 trillion clay bricks produced worldwide annually are made in Asia. These bricks are typically fired in small-scale traditional kilns that burn coal or biomass without air pollution controls. Clamp kiln is the most traditional technology of brick manufacturing. It is a batch-style kiln that produces 10,000-200,000 bricks per batch in a time period of two to four weeks. It uses coal as primary and firewood and rice husk as supplementary fuel. There is no chimney, and hence the smoke escapes from the cracks at the top and from the sides of the kiln. Very little information is available on aerosols emitted from these kilns. Therefore, it’s important to accurately estimate aerosol emissions and their chemical properties from FCBK to understand their impact on regional air quality and climate. This study examines the chemical and optical properties of emitted aerosols during different stages of combustion in clamp kilns. The National Carbonaceous aerosol programme- Carbonaceous aerosol emissions, source apportionment and climate impacts (NCAP-COALESCE) network source emission measurement system was used to measure absorption and scattering properties using the Aethalometer and Integrating Nephelometer, respectively. Measurements were done for clamp kilns of different firing stages, namely ignition, propagation, and end. The combustion efficiency was >97% during the end, propagation and ignition stages. The average BC (SO2) concentration measured during the ignition, propagation and end stage was 12.5 (10) 18.5 (9), and 13.3 μg-m-3(19 ppm), respectively against background of 2 μg-m-3 (0 ppm) . The corresponding values of average AAE370/660 (AAE660/880) during the three combustion phases were 3.6 (1.3), 2.6 (1.1) and 1.8 (1.2), respectively. The relatively high AAEs indicate a strong contribution by brown carbon aerosol, likely emitted from fuelwood and rice husk combustion during the ignition and propagation stages, respectively. This study would help characterise the combustion stage specific emissions. Further analysis is ongoing to understand the potential impacts on regional air quality and climate. 

Figure 1: Emission measurement setup and different position of the multi-arm during measurement based on incoming plume

How to cite: Gupta, A. K., Kapoor, T. S., Chimurkar, N., Venkatraman, C., and Phuleria, H. C.: Characterizing aerosol emissions from traditional clay fired clamp kilns in South Asia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13453, https://doi.org/10.5194/egusphere-egu23-13453, 2023.

Design, development and application of a particulate matter control technology with special consideration for indoor air quality management

Aiswarya Kumar1, Manoranjan Sahu1*

1Environmental science and engineering, Indian Institute of Technology Bombay (IITB), India

*Corresponding email: mrsahu@iitb.ac.in

ABSTRACT

Indoor air quality is a major concern in the modern environment since people especially those in urban areas spend 80-90% of their time in living, workspaces as well as in different means of transportation and also due to construction of tightly sealed buildings because of space constraints in developing and populated countries like Indian subcontinent. Among different indoor pollutants, particles are major concern for health due to their smaller size and easy attachment to different species. Particle exposure indoors depends on the characteristics of indoor sources, activities causing resuspension of particles and infiltration from an outdoor polluted environment. Conventional particle cleaning technologies such as filtration and ionisers have lot of draw backs such as high energy consumption, maintenance difficulties and reduced efficiency with time. Electrostatic precipitation (ESP) is a promising emerging technology in indoor environments due to benefits like high efficiency removal, minimal pressure drop, flexibility of keeping as standalone/induct, lesser energy consumption and low maintenance requirements. Therefore current study designed and developed a miniature wire-plate ESP for capture of indoor particles. Designed ESP was operated at a voltage of 6 kV considering voltage-current characteristics, different empirical formulas, visualization of corona and based on number of ions generated. Flow rate was kept at 8 LPM considering migration-residence times as well as uniform velocity distribution obtained from computational fluid dynamics (CFD) modelling. Characteristics of discharge wire were selected such as keeping by-product emission and power consumption minimal which are required optimal conditions for an indoor application. Designed ESP provided high capture efficiency for standard laboratory aerosols such as sodium chloride, ammonium chloride and magnesium chloride achieving promising results with a total removal efficiency of 95-99% for wide particles sizes from 10 nm to 10 µm as measured by sophisticated instruments like scanning mobility particle sizer (SMPS) and optical particle sizer (OPS). To simulate performance in a real scenario experiments were also carried out with major indoor particle sources like incense sticks, burning candles, mosquito coils and bio-aerosols such as Mycobacterium smegmatis as well as  Escherichia coli having varied particle number distributions and obtained total particle capture efficiency 99.99, 99.97, 99.98 and 95% respectively. Designed ESP also removed particles from ambient as well as infiltrated particles at a total capture efficiency of 99.8%. Nonthermal plasma (NTP) ionisation process happening inside the ESP has provided bioaerosol deactivation efficiency and volatile organic compound (VOC) degradation efficiency of 70 and 85% respectively. Additionally, this multipollutant removal technology  has an  lower energy consumption/Clean air delivery rate (CADR) (0.32 W/m³/hr) and emission of by-products like ozone and ultrafine particles compared to best commercial purifiers thereby suggesting its possible applicability as a product for air quality management

How to cite: Kumar, A. and Sahu, M.: Design, development and application of a particulate matter control technology with special consideration for indoor air quality management, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13497, https://doi.org/10.5194/egusphere-egu23-13497, 2023.

EGU23-15034 | Orals | AS5.13

Light-NMHCs in the Central Himalayas and associated IGP Region: Role in Ozone and Secondary Organic Aerosols-Formation 

Mahendar Rajwar, Manish Naja, Shyam Lal, Sethuraman Venkataramani, Prajjwal Rawat, and Rakesh K. Tiwari

Non-methane hydrocarbons (NMHCs) are important precursors of tropospheric ozone and secondary organic aerosols (SOAs). The air quality in South Asia is rapidly deteriorating due to increasing pollution levels, and transporting these pollutants to pristine regions in the Himalayas also exacerbates the problem. Despite this, air quality studies are very limited in South Asia, particularly in remote Himalayan regions. This study presents first time, a comprehensive analysis of light NMHCs (C2-C5) at the central Himalayas mountain site (Nainital; 29.37°N, 79.45°E, 1958 m a.m.s.l.) and an Indo Gangetic Plain (IGP) site (Haldwani; 29.22°N 79.51°E, 554 m a.m.s.l.). Observations were made from January 2017 to December 2020 using a Thermal Desorption Gas Chromatograph equipped with Flame Ionization Detectors (TD-GC-FID). The continuous online observations showed diurnal variation in light-NMHCs with higher values in the daytime throughout the year except for the summer/monsoon months. The mixing levels of alkanes, alkenes and alkynes vary from the lowest level of 1.96±0.77 ppbv, 0.29±0.06 ppbv, and 0.22±0.20ppbv respectively, to the highest levels of 4.43±0.84 ppbv, 1.03±0.39 ppbv, and 0.75±0.40ppbv in November, respectively. However, an IGP site showed much higher levels at nighttime than in the daytime, where alkanes, alkenes and alkyne showed 19.24±0.24 ppbv, 2.88±1.76 ppbv, 1.41±1.21 ppbv levels during winter and 13.41±9.33 ppbv,1.88±1.65 ppbv, 0.67±0.59 ppbv. Among eight light-NMHCs, the observed levels of ethane, ethylene, propane, n-butane and acetylene were highest during winter and spring and minimum in summer/monsoon at both sites. Ethane is most dominant at the Himalayan site, while propane is at the IGP site. The investigation of the natural logarithmic ratio between two different pairs (ln([n-butane]/[ethane]) to ln([i-butane]/[ethane]) and ln([Propane]/[ethane]) to ln([n-butane]/[ethane]) suggested the role of oxidation of OH mechanism for light-NMHCs removal in the atmosphere at both the sites and globally compared results showed a heterogeneous nature of these light NMHCs in the atmosphere. There is a strong inter-correlation among ethane, i-butane, propane, and n-butane acetylene, which supports the influence of natural gas, LPG leakage and biomass burning. Additionally, a good correlation of combustion tracer carbon monoxide (CO) with ethane, propane, and acetylene reconfirmed that biomass burning is the source of these light-NMHCs at the central Himalayas site, especially during spring. The OH reactivity, ozone formation potential (OFP) and secondary organic aerosol potential (SOAP) is also studied. The OH-reactivity is minimal at a mountain site compared to an IGP site. Propylene (25%-30) and ethylene (10-25%) strongly contributed to OH-reactivity. Both sites have maximum OFP during the winter and a minimum. The OFP during the summer/monsoon for all the seasons. Propylene (23%-35%) and ethylene (18- 22%) are species dominated by OFP throughout the year at both sites. SOAP showed wintertime maxima and springtime minima with the dominance of propylene (35%-45%) and i-butane (15%-38%) at the Himalayan site, whereas propylene (%) and n-butane (%) dominance at the IGP site. Further, these datasets can be used to develop emission inventories and validate various chemical transport models. The results from these studies are also useful for policymakers in formulating and implementing effective emission reduction strategies. 

How to cite: Rajwar, M., Naja, M., Lal, S., Venkataramani, S., Rawat, P., and Tiwari, R. K.: Light-NMHCs in the Central Himalayas and associated IGP Region: Role in Ozone and Secondary Organic Aerosols-Formation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15034, https://doi.org/10.5194/egusphere-egu23-15034, 2023.

EGU23-16203 | Posters virtual | AS5.13

Seasonal variation and source apportionment of Oxygenated (OPAHs) and Nitrated (NPAHs) Polycyclic Aromatic Hydrocarbons in PM2.5 in Ulaanbaatar, Mongolia 

Soyol-Erdene Tseren-Ochir, Iderkhangai Erdenebat, Urangoo Tumurbat, Ji Yi Lee, Amgalan Natsagdorj, and Youngpyu Kim

Nitrogen and oxygen containing polycyclic aromatic hydrocarbons (NPAHs and OPAHs) are the most dangerous substances for public health and are of increasing interest due to their high toxicity and oxidative properties. Ulaanbaatar, the capital city of Mongolia, has occasionally been considered the most polluted city in the world. The high emissions from various anthropogenic sources of pollutants coupled with unique weather and geographical conditions lead to the formation of haze over the city in winter. The main purpose of this study is to determine the concentration, main sources and seasonal changes of nitrogen and oxygen containing polycyclic aromatic compounds (Oxygenated PAHs and Nitro-PAHs) in atmospheric fine inhalable particulate matter (PM2.5) in Ulaanbaatar city and to compare it with other big cities in East Asia in order to define their risk to human health. Samples were taken in winter (December 2020 and January 2021) and summer (June 2021) and the concentration of 12 types of OPAHs and 8 types of NPAHs were analyzed by Gas Chromatography/Mass Spectrometry (GC/MS).  As a result, the mean concentration of OPAHs in atmospheric PM2.5 particles in Ulaanbaatar is 21.5 and 35.3 times higher than that in Seoul, Korea in winter and summer, respectively. While the concentration of NPAHs was 5.1 times higher in winter and 11.2 times higher in summer than that in Seoul. Major sources and their contributions of NPAHs and OPAHs in atmospheric PM2.5 in Ulaanbaatar were identified based on correlation analysis and Positive Matrix Factorization (PMF) modeling.

How to cite: Tseren-Ochir, S.-E., Erdenebat, I., Tumurbat, U., Lee, J. Y., Natsagdorj, A., and Kim, Y.: Seasonal variation and source apportionment of Oxygenated (OPAHs) and Nitrated (NPAHs) Polycyclic Aromatic Hydrocarbons in PM2.5 in Ulaanbaatar, Mongolia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16203, https://doi.org/10.5194/egusphere-egu23-16203, 2023.

EGU23-16373 | Orals | AS5.13

An Integrated approach of dispersed source mapping and hyperlocal monitoring for air quality management: A case study of hotspots in Delhi 

Adeel Khan, Sairam Dhandapan, Saurabh Mendiratta, Mohammad Rafiuddin, Priyanka Singh, Nimisha Biswas, Shreya Chadha, Tanushree Ganguly, and Karthik Ganeshan

Limited actionable data is one of the main constraints for urban local bodies and regulatory agencies to improve air quality. Emission inventories and source apportionment are important components of air quality management. However, they provide limited information about the location of pollution sources and how the sources are changing dynamically. To overcome these limitations, a field reconnaissance survey and hyperlocal monitoring through low-cost sensors were conducted for one of the hotspots in Delhi. Field reconnaissance survey helps identify and geolocate dispersed pollution sources (unpaved roads, road dust, biomass and waste burning, construction activities, etc.). The operation of the survey includes route planning, training of field surveyors, field survey, data quality control and analysis. Through the survey, 786 dispersed sources of 14 distinct types were identified. Construction and Demolition waste, potholes, road dust and garbage dumps constitute 40 % of the sources. The concerned agencies and sub-departments were mapped through consultation with stakeholders, and sources were prioritised based on factors like population density, predominant wind direction, etc. A network of low-cost sensors is also being deployed, taking the different land use categories within the hotspot into consideration to study the impact of tackling these dispersed sources. The present approach was found to be both cost as well time effective and has the potential to scale and can be used for other scientific applications like spatial bias correction in air quality models. The approach can also be used to develop targeted strategies for improving air quality and mitigating the negative impacts of air pollution on human health and the environment.

How to cite: Khan, A., Dhandapan, S., Mendiratta, S., Rafiuddin, M., Singh, P., Biswas, N., Chadha, S., Ganguly, T., and Ganeshan, K.: An Integrated approach of dispersed source mapping and hyperlocal monitoring for air quality management: A case study of hotspots in Delhi, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16373, https://doi.org/10.5194/egusphere-egu23-16373, 2023.

EGU23-16697 | ECS | Orals | AS5.13 | Highlight

Data management in resource-limited settings: Unpacking the role of robust digital solutions for air quality data management in African cities. 

Deo Okure, Daniel Ogenrwot, Noah Nsimbe, Lillian Muyama, Priscilla Adong, Richard Sserunjogi, Martin Bbaale, and Engineer Bainomugisha

Increasing awareness of air pollution requires access to timely and reliable air quality data and information, and yet many African cities lack effective air quality monitoring infrastructure, largely because of the resource constraints of establishing and managing a continuous monitoring network. Low-cost sensor platforms have the potential to close the air quality data gaps in resource-strained settings such as Africa, but the continued lack of accessible and reliable infrastructure for data management is a major hindrance to effective air quality management.

Moreso, managing a large Internet of Things (IoT)-based sensor network can be complex, and the demand for a case-specific and highly customizable platform, coupled with its conceptualization & implementation complexities, renders most existing IoT platforms ineffective. There is a need for a platform infrastructure for continuous support and management of air quality data with a high spatial and temporal resolution to facilitate sophisticated analysis; while taking care of the associated structural challenges of low-cost sensors.  The AirQo platform, a robust could-native software is a novel communityaware digital platform for managing large-scale air quality networks, applicable in resource-strained environments. This customisable and scalable platform attempts to address the data access challenges, with capabilities to become a ‘one-stop centre’ for management of other third party IoT sensor networks. Different interfaces through mobile application, web-based dashbord and platform cater for diverse data needs. The robust approach enables decision makers and other stakeholder communities have access to timely and quality assured air quality data. Using a set of metrics, user-experiece can be computed and compared with existing IoT management platforms. Software design considerations including (1) Multi-tenancy, (2) Data pipeline, (2) Sharded Database Cluster, (3) Microservices architecture, (4) Containerized deployment, and (5) Interoperability are recommended to support replication in other use-cases.

 

 

How to cite: Okure, D., Ogenrwot, D., Nsimbe, N., Muyama, L., Adong, P., Sserunjogi, R., Bbaale, M., and Bainomugisha, E.: Data management in resource-limited settings: Unpacking the role of robust digital solutions for air quality data management in African cities., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16697, https://doi.org/10.5194/egusphere-egu23-16697, 2023.

EGU23-17038 | ECS | Orals | AS5.13

Traffic-related Air Pollution (TRAP) and Its Exposure to Cardiorespiratory Outcomes to Active Commuters in a University Outdoor Environment 

Eliani Ezani, Nur Izah Ab Razak, Josfirin Uding Rangga, Hasni Idayu Saidi, and Sairam Dhandaphani

Air pollutants are a major by-product of urbanisation and motorisation of society. In lower and upper middle-income Asian countries, in cities with rapid population growth such as Malaysia, traffic emissions are responsible for almost 90% of urban air pollution, so cycling or walking outdoor can be a major route of exposure for active commuters. Our study aims to examine the association between traffic-related air pollution and cardiorespiratory health symptoms among pedestrian and cyclists in a university campus located in Selangor, Malaysia.  PM2.5 concentrations were monitored using SidePak Personal Aerosol Monitor AM510 on weekday morning cycling and walking commutes into designated high and low-traffic areas nearby campus roadsides. Volunteers cycled (n=21) and walked (n=30) for about 60-minutes in high and low-traffic cycling and walking routes respectively. The cardiorespiratory health status of blood pressure and lung function were measured before, immediately after, after 15 minutes and after 1 hour of volunteers’ commutes. The average commute exposure to PM2.5 was determined, and the inhaled dosage was estimated. Results showed that pedestrian are exposed to higher PM2.5 levels than cyclists traveling in the same high-traffic areas. However, the inhalation dose per kilometre travelled, DL (µg/km) for cyclist was observed higher compared to the pedestrian due to the ventilation rate of physical activity. We also observed that there were increase in the systolic blood pressure and lung function (force-vital capacity-FVC) of pedestrians after the exposure to high PM2.5 concentrations at high traffic walking routes (61.6 ± 14.6 µg/m³). PM2.5 concentrations while walking in the university campus were approximately three times higher compared to cities in Europe (26 μg m−3). Our observation techniques can be applied in resource-constrained countries with heavy traffic emissions that may have an impact on the health of active commuters. To characterise the exposure patterns of other traffic-related air pollutant surrogates (such as soot/black carbon and nitrogen dioxide) and their influence on acute and chronic health outcomes in different Asian traffic microenvironments, further research based on the results of our study is needed.

How to cite: Ezani, E., Ab Razak, N. I., Uding Rangga, J., Saidi, H. I., and Dhandaphani, S.: Traffic-related Air Pollution (TRAP) and Its Exposure to Cardiorespiratory Outcomes to Active Commuters in a University Outdoor Environment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17038, https://doi.org/10.5194/egusphere-egu23-17038, 2023.

EGU23-17264 | ECS | Orals | AS5.13

Climate modelling and futures scenarios: Civil society perceptions of and proposed solutions for air pollution’s effects on health and wellbeing in two Thai cities 

Kelly Perry, Weenarin Lulitanonda, Tharinya Supasa, Siripha Junlakarn, and Bhushan Tuladhar

In Thailand—the fourth most polluted nation in Southeast Asia—air pollution is estimated to take an average three years off people’s lives. While all of Thailand’s 68 million people live in areas that exceed the World Health Organization’s (WHO) guidelines for airborne fine particulate matter less than 2.5 microns (PM2.5), Bangkok and Chiang Mai in particular (the focus of this study) are among the provinces carrying the highest health burden.

Currently, while the science behind air pollution is unequivocal, its public representation is, with official accounts perpetuating existing inequities by narrowly determining how crises are defined and selectively narrating who is impacted by them—pushing civil society voices to the fringes of public conversations on air pollution. To decenter this inequity, this study uses innovative participatory futures methods to gather civil society perspectives on the plausible, possible, and probable future solutions to air pollution and its impact on people’s health as well as social and economic implications on wellbeing. This is to ensure that civil society perspectives on solutions inform future advocacy, policy, and programmatic recommendations for addressing air pollution.

This research proposes to use modelling and air quality forecasting (the Stockholm Environment Institute’s Low Emissions Analysis Platform, Integrated Benefits Calculator) to create four sets of projections for air pollution 30 years from now (in 2053) that will then form the basis for four futures scenarios to be presented to civil society study participants as a direct form of citizen engagement.

Based on modelling results, scientists, subject matter experts, and civil society stakeholders will be engaged in online scenario-building workshops to create four futures scenarios. For instance, health, economic, political, and social implications will be generated from workshop dialogue, informed by model projections, and used to construct imaginary narratives within each of the four futures scenarios (that will then serve as the basis for the futures visioning interviews with civil society participants). Final scenarios will include depictions of social, economic, and health standards for Thai people in 2053. Once the four scenarios have been developed and stress tested, online individual participatory futures interviews will be conducted with civil society participants based in Bangkok and Chiang Mai (n=20 per city to reach an inductive thematic saturation point for primary data collection), using a blend of purposive (selective) sampling and snowball sampling methods. The University of Hawaii’s Manoa Futures Visioning Process and Krishnan’s decolonial futures/foresight framework will be employed to ensure an equitable and participant-centered approach.

Data collection and analysis will be completed by the start of the EGU General Assembly in April 2023; the AS5.13 session will be used to share experiences and lessons learned through integrating climate modelling with citizen science within this study to inform potential regional futures work within South and Southeast Asia (and beyond). Results from the study will inform the work that the Thailand Clean Air Network is doing regarding air quality policy advocacy in Thailand, among other avenues.

How to cite: Perry, K., Lulitanonda, W., Supasa, T., Junlakarn, S., and Tuladhar, B.: Climate modelling and futures scenarios: Civil society perceptions of and proposed solutions for air pollution’s effects on health and wellbeing in two Thai cities, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17264, https://doi.org/10.5194/egusphere-egu23-17264, 2023.

EGU23-1224 | ECS | Posters on site | ITS1.2/AS5.14

Implications for engineering design of shorter more extreme rainfalls and increased flood variability 

Conrad Wasko, Michelle Ho, Rory Nathan, Ashish Sharma, Caleb Dykman, and Elisabeth Vogel

Increases in extreme rainfall intensities as a result of climate change pose a great risk due to the possible increases in pluvial flooding. But evidence is emerging that the observed increases in extreme rainfall are not resulting in universal increases in flooding. Here, we begin by presenting historical evidence for changes in extreme rainfalls and floods discussing the underlying mechanisms for the changes, before examining the implications of climate change projections on engineering design.

Extreme rainfall is intensifying universally across the globe with more extreme events experiencing larger degrees of intensification. Simultaneously, and somewhat paradoxically, the magnitude of frequent floods (those expected to occur on average once per year) are in general decreasing, particularly in the tropical and arid regions of the world. We suggest this is likely due to the dominance of drying antecedent soil moisture conditions and shorter storm durations at higher temperatures offsetting any increases in rainfall intensity. However, for rare magnitude floods (those expected, on average, to occur less than once every twenty years) the increase in rainfall appears to outweigh any decrease in soil moisture or change in the temporal pattern of the storm.

Climate model projections, downscaled through a continental scale water balance model and locally calibrated rainfall-runoff models, show that future projections of flood responses follow historical trends – with the rarer the flood, the more likely it is to be increasing. To deepen our understanding, we focus our analysis on event runoff coefficients as an indicator of future runoff changes. Across Australia we find runoff coefficients are projected to decrease, that is, reduced runoff resulting from the same amount of rainfall. These results indicate drier conditions and a compounding of the reduced average rainfall and drier conditions already being experiences in many arid parts of the world.

With these historical changes and projections in mind we conclude with some insights and implications on how best to incorporate the additional uncertainty due to climate change when estimating floods for planning and design purposes. As floods constitute a large portion of the inflows into reservoirs, we suggest that future water resources planning will need to account for reduced runoff yields. To assess the potential impacts of future climate change for planning and design purposes we need to consider how changes to rainfall intensity vary with both storm duration and storm rarity, as well as how antecedent conditions influence the proportion of rainfall that appears as runoff. There remains significant work in adapting our current flood guidance to reflect these historical and projected changes.

How to cite: Wasko, C., Ho, M., Nathan, R., Sharma, A., Dykman, C., and Vogel, E.: Implications for engineering design of shorter more extreme rainfalls and increased flood variability, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1224, https://doi.org/10.5194/egusphere-egu23-1224, 2023.

EGU23-5418 | ECS | Posters virtual | ITS1.2/AS5.14

High resolution exposure model for a flood displacement risk assessment 

Daria Ottonelli, Sylvain Ponserre, Lauro Rossi, Roberto Rudari, and Eva Trasforini

Disaster risk determines the potential loss of life, injury, or destroyed or damaged assets which could occur to a system, society or a community in a specific period of time, determined probabilistically as a function of hazard, exposure, vulnerability and capacity. This paper focuses on the exposure elements, that expresses people, infrastructure, housing, production capacities and other tangible human assets located in hazard-prone areas (UNDRR, 2017).  In performing risk analyses, an accurate exposure model should be constructed and specified according to the purpose and spatial scale of the assessment.

The scope of the present work is the flood displacement risk assessment for two small island developing states in the Pacific Ocean, Fiji and Vanuatu, where a new methodology is proposed, that considers different but intrinsically linked components in assessing the contribution of disasters to displacement. In this assessment, three main elements are supposed to trigger (or at least contribute to cause) flood displacements: the loss of housing, the loss of livelihoods or the loss of access to basic services. This implies that, besides the classical vulnerability characterization of a asset based on occupancy (residential, commercial, industrial, etc.) and structural elements (number of stories, basement, etc.), the exposure model must also consider a spatial representation of the population relying on the specific function of that asset: residential population in case of residential building; population working in that building in case of commercial, industrial, or service buildings; population working in crop or grazing areas in case of agricultural field; number of students in case of school.

In this context, a procedure for avoiding potential double counting was also implemented. It means that, to evaluate the ratio of population that could suffer impacts due to floods on both livelihoods and housing, each worker must be associated to his/her home with his/her workplace.

Regarding the spatial scale, the small size of the countries allows for the definition of a high-resolution exposure model, that entails a characterization at building Level.

The construction of the exposure model is articulated in three main steps: 1) analysis and integration of different sources of employment and residential data (from global to local information); 2) physical characterization of assets at building scale, using building footprints from the Open Street Map layer and attributes from existing exposure models, such as Pacific Catastrophe Risk Assessment and Financing Initiative (PCRAFI) project that lasted from 2012 to 2017 and Global Earthquake Model (GEM) within the project Global Exposure Map (v2018.1); 3) the procedure to avoid double counting, which associates each worker to his/her home with his/her workplace, following the criterion of minimum geometric distance between workplace and residence.

The exposure model is then used in a probabilistic risk assessment, where different flood scenarios and related damage scenarios are computed at building scale. Physical damage above a certain threshold is considered to cause the unavailability of asset function (residence, workplace), thus triggering the displacement of people relying on that function.

How to cite: Ottonelli, D., Ponserre, S., Rossi, L., Rudari, R., and Trasforini, E.: High resolution exposure model for a flood displacement risk assessment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5418, https://doi.org/10.5194/egusphere-egu23-5418, 2023.

EGU23-5563 | Posters virtual | ITS1.2/AS5.14

From vulnerability to vulnerabilities for a probabilistic flood displacement risk model: the case study of Fiji and Vanuatu. 

Eva Trasforini, Lauro Rossi, Sylvain Ponserre, Lorenzo Campo, Andrea Libertino, Daria Ottonelli, and Roberto Rudari

Floods have triggered about 166 million displacements globally since 2008, according to the Internal Displacement Monitoring Center (IDMC). Since 2008, most of the displacements triggered by floods have been localized in Asia and the Pacific and with an overall estimate of 129 million displacements. Small Island Developing States (SIDS) states bear the greatest displacement risk relative to their population size. Climate change combined with vulnerability of exposed infrastructure, and housing poses an existential threat for some Pacific islands that could see their populations move not only internally but also across borders. These magnitudes of forced movement highlight the importance of the phenomenon. In this context, we present a first attempt to estimate present and future riverine flood displacement risk at the national and sub-national level for two countries in the Pacific Ocean: Fiji and Vanuatu.

This work proposes a new methodology that provides a more comprehensive assessment of vulnerability in the context of disaster displacement risk and recognizes that people’s vulnerability depends on several physical and social factors. Such elements, however, are not yet included in standard risk models because difficultly quantifiable. While quantitative approaches to disaster displacement risk assessment generally consider the likelihood of housing rendered unhabitable as a proxy for displacement, this new methodology expands this concept by taking into account different elements that may trigger displacements or may increase the susceptibility to forced movement: 1) impact on houses; 2) impact on livelihoods; 3) impact on critical facilities and services.

A probabilistic risk assessment was performed at building scale in present and future climate conditions: under current climate conditions (1979-2016); under medium-term projected climate conditions (2016 - 2060); under long-term projected climate conditions (2061 – 2100). As results, displacement risk information - expressed in annual average displacement (AAD) and probable maximum displacement (PMD) - were calculated at national and subnational (NUTS2) scales, allowing for a geographic and quantitative comparison both within and between countries. The computation performed at building scale also allowed for result aggregation by sectors.

The outputs of the probabilistic model  show an important role of climate change in determining future likelihood to displacement due to riverine floods in the area. Flood displacement risk is likely to double by 2060 in both countries, and under the pessimistic long-term scenarios AAD is expected to triple in Fiji and quadruple in Vanuatu. These analyses are an important step in risk awareness processes and key to pushing for risk reduction, adaptation, and management mechanisms to be put in place.

 

 

How to cite: Trasforini, E., Rossi, L., Ponserre, S., Campo, L., Libertino, A., Ottonelli, D., and Rudari, R.: From vulnerability to vulnerabilities for a probabilistic flood displacement risk model: the case study of Fiji and Vanuatu., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5563, https://doi.org/10.5194/egusphere-egu23-5563, 2023.

EGU23-5564 | ECS | Posters virtual | ITS1.2/AS5.14

Flood Modelling and Simulation using HEC-RAS 

Mohd. Usman Saeed Khan, Maaz Abdullah, and Arisha Aslam Khan

Natural disasters are one of the main causes of worry for the majority of nations because they severely harm the global economy. One of the natural disasters that occur on a global scale that seriously damages infrastructure and claims thousands of lives is flooding. Due to its geographical location, India is one of the high-risk nations that is negatively impacted by floods every year. It ranks in the top 20% of countries worldwide for the number of flood-related fatalities. A natural tragedy cannot be prevented. However, if some preventative actions were taken in advance, a sizable portion of the potential damage may be prevented. Professionals and authorities need accurate figures regarding flood depth, amount of flow, scale, and distinct datasets in order to reduce and manage the effects of such catastrophes. The management of flood risk is heavily dependent on flood modelling. One of the many software tools that assists in computing the discharge, depth, magnitude, and statistics of rivers located in high-risk flood zones is HEC-RAS (Hydrologic Engineering Centre-River Analysis System).This study employed the Purna River's 1D hydrodynamic floods modelling (50 and 100 years out) on HEC-RAS and it has been found that the great portion of populated area will be affected in future. The goal of this study is to assess the prediction power and carry out a sensitivity analysis to identify the sensitive zones. This research project would enable different flood modelling and risk zone delineation for diverse flood-affected areas in India and around the world. In places affected by flooding, these technologies can also be used to create emergency response protocols.

How to cite: Khan, M. U. S., Abdullah, M., and Khan, A. A.: Flood Modelling and Simulation using HEC-RAS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5564, https://doi.org/10.5194/egusphere-egu23-5564, 2023.

EGU23-7110 | ECS | Orals | ITS1.2/AS5.14

Combining future projections of land-use and climate change to assess their impact on biodiversity 

Chantal Hari, Inne Vanderkelen, Markus Fischer, and Édouard Davin

Biodiversity loss, land degradation, and climate change are acknowledged environmental challenges faced by humanity. Human activities including land-use changes are key stressors for biodiversity, thus, future projections of biodiversity impacts need to include both climate change and land-use change. While a lot of studies focused on mapping and projecting the vulnerability of multiple species based on different climate mitigation scenarios or warming levels, land-use trajectories are often not included in these projections. Recent work made first steps to address these deficiencies. For example, Hof et al. (2018) evaluated potential future impacts of climate and land-use changes on global species richness of terrestrial vertebrates under a low and high emission scenario. However, they used the same land-use change assumptions for both emission scenarios. In this study, we aim to fill the described research gap by combining future climate scenarios and a matrix of land-use projections derived from integrated assessment modeling (IAM) to estimate the fractional land-use patterns, underlying land-use transitions, and key agricultural management information, to assess the impact of climate change on biodiversity and quantify the additional impact of land-use change.

 

To this end, we use the global simulations with a species distribution model from the Hof et al. (2018) study forced by four GCMs and both RCP2.6 and RCP6.0 climate scenarios following the ISIMIP2b simulation protocol and apply a land-use filter on the species occurrence probabilities to determine the implications for the world’s amphibians, mammals and reptiles at a 0.5° resolution. The land use data used to include future projections of land-use change is the Land Use Harmonization dataset v2 (LUH2). LUH2 reconstructs and projects changes in land use among 12 categories. To match the species’ habitat preferences, data from IUCN Habitat and Classification Scheme for each species is mapped onto the 12 land-use types represented in the LUH2 dataset according to the conversion table from Carlson et al. (2022). The land-use data is then used to refine the climatic envelope and filter out regions where species cannot persist.

 

This approach allows to quantify the change of the proportion of affected species distributions between different climate and land-use scenarios and combinations of both. In addition, it provides quantitative information on the impact of future climate change on biodiversity accounting for the combination of land-use change projections and climate-driven species distribution models.

 

Key Reference:

Hof, C., Voskamp, A., Biber, M. F., Böhning-Gaese, K., Engelhardt, E. K., Niamir, A., Willis, S. G., & Hickler, T. 2018: Bioenergy cropland expansion may offset positive effects of climate change mitigation for global vertebrate diversity. Proceedings of the National Academy of Sciences of the United States of America, 115(52), 13294–13299.

How to cite: Hari, C., Vanderkelen, I., Fischer, M., and Davin, É.: Combining future projections of land-use and climate change to assess their impact on biodiversity, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7110, https://doi.org/10.5194/egusphere-egu23-7110, 2023.

EGU23-7346 | Orals | ITS1.2/AS5.14 | Highlight

End-to-end modelling of flood risk and impact for climate change resilience 

Anne Jones, Andrew Taylor, Junaid Butt, Blair Edwards, Jorge Luis Guevara Diaz, and Priscilla Barreria Avegliano

Climate change is driving increased urgency for better quantification of climate hazards and their impacts for stakeholders across multiple economic sectors. Flooding has been highlighted as one of the most significant climates risk to UK economic infrastructure, with costs expected to increase with climate-driven changes to rainfall, such as increased intensity of summer storms. To accelerate climate change adaptation and enable economic resilience to climate change impacts, close collaboration is needed between climate scientists, impact modellers, and stakeholders, and technology advances can support this by enabling and streamlining the process of developing and deploying climate impact modelling workflows to translate complex datasets and scientific models into actionable information.

In this presentation, we describe the application of such a technology for the case of pluvial flooding, undertaken as part of the IBM Research and Science and Technology Facilities Research Council partnership, the Hartree National Centre for Digital Innovation (HNCDI), a 5-year programme established to develop and apply new technology to key economic challenges in the UK. Here, we model pluvial flood hazard for a case study region in northeastern England, using a 2-d physical simulation model of flood inundation, driven by open-access geospatial and climate datasets. Flood hazard maps are translated to impact using open asset location data and damage functions.

We consider the sensitivity and scalability (in terms of computational cost) of the hazard and impact predictions to multiple factors, including (1) DEM/DSM representation of land surface (2) soil and land use parameterisation, and (3) model spatial resolution. We also contrast the use of drivers in the form of extreme rainfall scenarios created using a traditional design storm approach, and ensembles of synthetic storms from a stochastic weather generator, both derived from hourly 1km gridded rainfall observations. Finally, we reflect on key gaps to be addressed in the models, data and technology to meaningfully inform climate adaptation across industry sectors.

How to cite: Jones, A., Taylor, A., Butt, J., Edwards, B., Diaz, J. L. G., and Avegliano, P. B.: End-to-end modelling of flood risk and impact for climate change resilience, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7346, https://doi.org/10.5194/egusphere-egu23-7346, 2023.

EGU23-7522 | ECS | Orals | ITS1.2/AS5.14

A transdisciplinary chain to assess the risk of direct and indirect impacts linked to extreme climate events from regional to local scale 

Marcello Arosio, Alessandro Caiani, Giorgia Fosser, and Jlenia Di Noia

Climate change is causing increased risks linked to extreme weather events. In order to develop effective adaptation strategies and policies, there is an urgent need for methodologies able to assess how the socio-economic risks associated with extreme climate-related events will change in the coming decades especially at local scale. The development of these methodologies require the expertise from many different scientific disciplines, including: modelling of global and local climatic phenomena, assessment of the intensity and probability of extreme events, representation of their impacts on the society and quantification of the associated risk.

In this work we propose a methodological chain linking the risk of extreme events in a changing climate with both direct and indirect impacts on the socio-economic sector from regional to local scale. The proposed chain integrates the knowledge of three scientific fields: climatologists, engineers and macro-economist. Here, we present agreements and differences between communities (e.g., aim, terminology, methodology, etc.), and evaluate advantages and constrains of the combined used of high-resolution regional climate models, engineering risk assessment models and economic input-output models compared to the state of the art in this field.

To illustrate the advantages of the proposed methodology and its practical feasibility, we present preliminary results from an applied pilot study in the Italian context.

How to cite: Arosio, M., Caiani, A., Fosser, G., and Di Noia, J.: A transdisciplinary chain to assess the risk of direct and indirect impacts linked to extreme climate events from regional to local scale, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7522, https://doi.org/10.5194/egusphere-egu23-7522, 2023.

EGU23-9246 | ECS | Posters on site | ITS1.2/AS5.14

Assessing the appropriateness of different climate modelling approaches for the estimation of aviation NOx climate effects 

Jin Maruhashi, Mariano Mertens, Volker Grewe, and Irene Dedoussi

Aviation’s contribution to anthropogenic global warming is estimated to be between 3 – 5% [1]. This assessment comprises two contributions: the well understood atmospheric impact of carbon dioxide (CO2) and the more uncertain non-CO2 effects. The latter pertain to persistent contrails and pollutants like nitrogen oxides (NOx), water vapor (H2O), sulfur oxides (SOx) and soot particles. NOx emissions are involved in non-linear processes that result in the short-term production of ozone (O3) and longer-term destruction of methane (CH4), stratospheric water vapor (SWV), and primary mode ozone (PMO). The aviation-attributable impacts arising from this short-term increase in O3 can vary by more than a factor of 1.5 depending on the selected modelling approach. This O3 increase is associated with the second largest warming effect across aviation’s main climate forcers [1]. We therefore quantify this figure using three modelling approaches (an Eulerian and a Lagrangian tagging scheme as well as a perturbation approach) at three potential aircraft cruise altitudes (200, 250 and 300 hPa) at which NOx pulse emissions are introduced in the Americas, Africa, Eurasia and Australasia. In general, the tagging method computes the contribution by an emission source to the concentration of a chemical species while a perturbation approach consists in calculating the total impact of an emission to the concentration of a species by means of subtracting two simulations: one with all emissions and a second without the specific source’s emissions. We compare results from Eulerian and Lagrangian simulations using the same climate-chemistry code: the ECHAM5/MESSy Atmospheric Chemistry (EMAC) model. With the Eulerian setup, we are able to capture non-linear processes and feedback effects, but not track the transport of emitted species in detail. The Lagrangian setup [2], on the other hand, allows for the accompaniment of thousands of air parcel trajectories, but at the cost of assuming a simplified linear chemistry mechanism. We find that the Lagrangian tagging approach provides the largest estimates for O3 production and radiative forcing (RF), followed by the Eulerian tagging scheme and lastly by the perturbation method. We therefore investigate the appropriateness of each of these in quantifying aviation’s total and marginal climate effects by addressing the following research questions: 1) By how much are the estimates for the short-term NOx-induced O3 perturbation and consequent RF varying across the three modelling approaches and why? 2) How does this RF vary with emission altitude within the upper Troposphere/lower Stratosphere (UTLS)?

[1] Lee, D.S., Fahey, D.W., Skowron, A., Allen, M.R., Burkhardt, U., Chen, Q., Doherty, S.J., Freeman, S., Forster, P.M., Fuglestvedt, J., Gettelman, A., De León, R.R., Lim, L.L., Lund, M.T., Millar, R.J., Owen, B., Penner, J.E., Pitari, G., Prather, M.J., Sausen, R., and Wilcox, L.J.: The contribution of global aviation to anthropogenic climate forcing for 2000 to 2018, Atmos. Environ., 244, 117834, https://doi.org/10.1016/j.atmosenv.2020.117834, 2021.

[2] Maruhashi, J., Grewe, V., Frömming, C., Jöckel, P., and Dedoussi, I. C.: Transport patterns of global aviation NOx and their short-term O3 radiative forcing – a machine learning approach, Atmos. Chem. Phys., 22, 14253–14282, https://doi.org/10.5194/acp-22-14253-2022, 2022.

How to cite: Maruhashi, J., Mertens, M., Grewe, V., and Dedoussi, I.: Assessing the appropriateness of different climate modelling approaches for the estimation of aviation NOx climate effects, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9246, https://doi.org/10.5194/egusphere-egu23-9246, 2023.

EGU23-9338 | ECS | Orals | ITS1.2/AS5.14

Future changes in sub-daily extreme precipitation over a complex-orography area from a convection-permitting climate model 

Eleonora Dallan, Giorgia Fosser, Christoph Schaer, Bardia Roghani, Antonio Canale, Marco Marani, Marco Borga, and Francesco Marra

Sub-daily extreme precipitation can generate fast hydro-geomorphic hazards such as flash floods and debris flows, which cause fatalities and damages especially in mountainous regions. Reliable projections of extreme future precipitation is fundamental for risk management and adaptation strategies. Convection-permitting climate models (CPMs) esplicitely resolve large convective systems and represent local processes, especially sub-daily extreme precipitation, more realistically than coarser resolution models, thus leading to higher confidence in their projections. Given their high computation cost, however, the available CPM simulations cover relatively short time periods (10–20 years), too short for deriving precipitation frequency analyses with conventional extreme value methods based on annual maxima or threshold exceedances.

In this work, we evaluate the potential of a non-asymptotic approach based on “ordinary” events, the so-called Simplified Metastatistical Extreme Value (SMEV), to provide information on the future change of short-duration precipitation extremes. We focus on a complex-orography region in the Eastern Italian Alps, where significant changes in sub-daily annual maxima have been already observed. The study is based on COSMO-crCLIM model simulations at 2.2 km resolution under the RCP8.5 scenario and uses three 10-year time periods: historical 1996-2005 (the control period), near-future 2041-2050 and far future 2090-2099. We estimate extreme precipitation for durations ranging from 1 h to 24 h and assess the projected changes with respect to the control period. Specifically, we analyze annual maxima, return levels up to 50 years, and the parameters of the statistical model. A bootstrap procedure is used to evaluate the uncertainty of the estimates, and a permutation test is applied to assess the statistical significance of the projected changes. We compare our results with a modified Generalized Extreme Value (GEV) approach, recently applied for the study of extremes in CPM future time periods.

We found that annual maxima and higher return levels exhibit a general increase in the future especially for the far future and the shorter event durations. On average, the magnitude of the far future change decreases with the precipitation temporal scale. The changes show an interesting spatial organization that can be associated with the orography of the region: significant future increases are mostly located at high elevations, while lowlands and coastal zones show no clear pattern.

This work shows that SMEV reduces the uncertainty in the estimates of higher return levels compared to GEV and can thus provide improved estimates of their future changes from short CPM runs. These findings advance our knowledge about the projected changes in extreme precipitation and their spatial distribution at the different time scales. They can thus help improving risk management and adaptation strategies.

How to cite: Dallan, E., Fosser, G., Schaer, C., Roghani, B., Canale, A., Marani, M., Borga, M., and Marra, F.: Future changes in sub-daily extreme precipitation over a complex-orography area from a convection-permitting climate model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9338, https://doi.org/10.5194/egusphere-egu23-9338, 2023.

EGU23-9379 | Posters on site | ITS1.2/AS5.14

Three Hundred and Fifty Views on what the Natural Hazard Community should do to Support the Implementation of the SDGs 

Bruce D. Malamud, Robert Šakić Trogrlić, and Amy Donovan

We present the results of an NHESS (Natural Hazards and Earth System Sciences) 20th anniversary survey, in which 350 natural hazard community members responded to two questions: (Q1) “what are the top three scientific challenges you believe are currently facing our understanding of natural hazards” and (Q2) “what three broad step changes should or could be done by the natural hazard community to address natural hazards in achieving the Sustainable Development Goals”? We have analysed the data quantitatively and qualitatively. According to the 350 respondents, the most significant challenges (Q1) are the following (within brackets % of 350 respondents who identified a given theme): (i) shortcomings in the knowledge of risk and risk components (64 %), (ii) deficiencies of hazard and risk reduction approaches (37 %), (iii) influence of global change, especially climate change (35 %), (iv) integration of social factors (18%), (v) inadequate translation of science to policy and practice (17 %), and (vi) lack of interdisciplinary approaches (6 %). In order for the natural hazard community to support the implementation of the Sustainable Development Goals (Q2), respondents called for (i) enhanced stakeholder engagement, communication and knowledge transfer (39 %), (ii) increased management and reduction of disaster risks (34 %), (iii) enhanced interdisciplinary research and its translation to policy and practice (29 %), (iv) a better understanding of natural hazards (23 %), (v) better data, enhanced access to data and data sharing (9 %), and (vi) increased attention to developing countries (6 %). We note that while the most common knowledge gaps are felt to be around components of knowledge about risk drivers, the step changes that the community felt were necessary related more to issues of wider stakeholder engagement, increased risk management and interdisciplinary working.

How to cite: Malamud, B. D., Šakić Trogrlić, R., and Donovan, A.: Three Hundred and Fifty Views on what the Natural Hazard Community should do to Support the Implementation of the SDGs, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9379, https://doi.org/10.5194/egusphere-egu23-9379, 2023.

EGU23-10210 | ECS | Orals | ITS1.2/AS5.14

Can annual streamflow volumes be characterised by flood events alone? 

Caleb Dykman, Ashish Sharma, Conrad Wasko, and Rory Nathan

Can total annual streamflow in any given year be largely characterised by a relatively small number of high flow events? A comprehensive assessment of this is of high value as there is evidence to suggest that as flood events increase in rarity a more consistent response between streamflow extremes and temperature increases can be established — providing greater reliability in projections of rare events. We propose here a novel methodology to characterise streamflow regimes in the context of total annual streamflow for water supply. Using the Australian Bureau of Meteorology’s Hydrologic Reference Station database, we developed annual event flow distributions that standardise the relationship between total annual streamflow and event flows. It was found that the annual event flow distributions are primarily a function of local climate and catchment size and were largely insensitive to interannual variability represented by the El Nino Southern Oscillation Index, mean annual temperature, or total annual rainfall volume. Statistically significant trends were found in the timeseries of annual event flow distribution values, signalling a move to a less even distribution in the southern latitudes and a more even distribution in the northern latitudes. Our results show that total annual streamflows can be characterised by a small number of high flow events. This suggests that for Australia’s most critical surface drinking water supply catchments the streamflow yields can be represented by changes in a few, high flow events, independent of interannual variability. As these relationships are non-stationary, they may provide a basis for understanding changes in water supply into the future.

How to cite: Dykman, C., Sharma, A., Wasko, C., and Nathan, R.: Can annual streamflow volumes be characterised by flood events alone?, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10210, https://doi.org/10.5194/egusphere-egu23-10210, 2023.

EGU23-10715 | Posters on site | ITS1.2/AS5.14

Towards global km-scale greenhouse warming simulations with the AWI-CM3 

Sun-Seon Lee, Axel Timmermann, Thomas Jung, Tido Semmler, Jung-Eun Chu, Jan Streffing, and Pavan Harika Raavi

In the past 5 years large efforts have been made to improve our understanding of scale-interactions in the Earth system, and to better resolve atmospheric and oceanic meso-scale processes and their response to greenhouse warming. Here, we provide an overview of the technical and scientific achievements of a new collaboration between the IBS Center for Climate Physics (South Korea) and the Alfred Wegener Institute for Polar and Marine Research (Germany) to simulate the climate system at km-scale resolution using the AWI Climate Model, version 3 (AWI-CM3). AWI-CM3 is based on the OpenIFS-FESOM2 coupled model and we conducted several control simulations and transient greenhouse warming runs in a medium-resolution (MR) configuration (31 km in the OpenIFS and 5~27 km in the FESOM2, ‘Tco319-DART’). These simulations will be used in future as initial conditions for shorter coupled storm-resolving (SR) simulations with target resolutions of 9 km and 4 km (Tco1279 and Tco2559). Our presentation focuses on the performance of the MR configuration (with a throughput of about 7 simulation years per day on 350 nodes) and its representation of the mean climate, climate variability such as the El Niño-Southern Oscillation, tropical cyclone statistics. We will also present preliminary estimates of the expected scaling behavior of the AWI-CM3 SR configuration on different multi-Petaflop supercomputing systems.

How to cite: Lee, S.-S., Timmermann, A., Jung, T., Semmler, T., Chu, J.-E., Streffing, J., and Raavi, P. H.: Towards global km-scale greenhouse warming simulations with the AWI-CM3, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10715, https://doi.org/10.5194/egusphere-egu23-10715, 2023.

EGU23-11320 | Posters on site | ITS1.2/AS5.14

Econometric modelling for the  estimation of direct flood damage to enterprises: a local-scale approach from post-event records in Italy 

Marta Ballocci, Daniela Molinari, Francesco Ballio, and Giovanni Marin

Flood-related damage has increased dramatically in recent decades with direct and indirect economic impacts accounting for a large share of gross national products. Therefore, there is an urgent need to acquire more quantitative knowledge about flood damage to mitigate economic losses and reduce exposure to flood risk.

Firms are especially affected in case of flood. Still, flood damage assessment to businesses is hindered by the paucity of available data to characterize the enterprises, the lack of high-quality damage data to derive new models or validate existing ones, and the high variability of activity types which hampers generalization. This study contributes at improving knowledge about types and extent of damage of flood events on economic activities through the analysis of empirical data, focusing on direct damage and with specific reference to the Italian context.

In detail, the investigated dataset is composed by around a thousand of observed damage records collected after four flood events in Italy, along with additional information on the dimension (i.e., surface and number of employees) and the typology of the affected firms (i.e., NACE category) as well as on local water depth levels. Damage data are further classified in damage to the building structure, the stock, and the equipment.

Several econometric models have been implemented to better understand the links among the damage, the characteristics of the economic activities and the water depth. Since the heterogeneity of the affected firms is very high, in terms of surface, water depth levels, and number of employees and this might have had influence on the firm’s damage reporting, data has been analyzed with Heckman's selection bias model.

Obtained results show the absence of a constant return scale relationship, therefore, the total damage increases less than proportionally to the firm’s surface; the water depth plays an important role to explain the damage to the stock that results the more vulnerable asset.  Information on the NACE category made it possible to quantify the differences in damage by economic sector. The results reveal as the most vulnerable sectors for building structure, stock and equipment, respectively, human health, commercial, and manufacture. The accuracy of the prediction models represented by adjusted R2 varies between 0.25, 0.36 depending on the damage component.

Despite characterized by significant uncertainty, obtained results supply a first model for the prediction of flood damage to firms for the Italian context, in the support of more effective risk mitigation actions. In fact, the model identifies the more vulnerable elements within the business sectors orienting modelers and decision-makers choices.

Acknowledgements:

Authors acknowledge with gratitude: Francesca Carisi, Alessio Domeneghetti and Armando Brath (from University of Bologna), Giovanni Menduni, Giulia Pesaro and Guido Minucci (from Politecnico di Milano), Simone Sterlacchini and Marco Zazzeri (from the Italian National Research Council) for their collaboration in collecting the observed damage records analysed in the research. A special thanks to Marta Galliani (from Politecnico di Milano) for providing the refined dataset used in this study.

How to cite: Ballocci, M., Molinari, D., Ballio, F., and Marin, G.: Econometric modelling for the  estimation of direct flood damage to enterprises: a local-scale approach from post-event records in Italy, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11320, https://doi.org/10.5194/egusphere-egu23-11320, 2023.

EGU23-11432 | ECS | Orals | ITS1.2/AS5.14

Using domestic weather disturbances and price transmission for maize price predictions in Southern Africa 

Patrese Anderson, Frank Davenport, Kathy Baylis, and Shraddhanand Shukla

In this paper we combine traditional econometric time series techniques and machine learning algorithms to construct skillful monthly maize price prediction models for four southern African countries – namely, Malawi, Mozambique, Zambia, and Zimbabwe. Theoretical models of price transmission commonly assume that shocks are transmitted from an external market (typically modeled as the world market) to the largest domestic city or port within a country and then, depending on the degree of market integration within the country, these shocks are transmitted to local markets. However recent evidence suggests that internal shocks have a larger impact on prices than external shocks. In an analysis of 554 local commodity markets across 51 countries during the period between 2008-2012, Brown and Kshirsagar (2015) find that 20% of local market prices were affected by domestic weather disturbances in the short-run in comparison to 9% by international price changes. This finding has prompted more recent literature to relax assumptions about international price transmission to investigate how shocks are transmitted through local and regional markets. 

Here we investigate the effects of domestic weather disturbances on regional maize price transmission. We then use these results of to build skillful price prediction models that use limited price data, weather disturbances, and other readily accessible free secondary data to predict monthly grain prices three, six, and nine months ahead in four Southern African countries. The collection of subnational price data in developing countries is costly and often difficult to obtain. We limit the amount of price data used by first determining if monthly price series in each country co-move and how these co-movements are influenced by domestic climate disturbances. We then use bivariate error correction models to both assess whether price movements in each country follow well-defined paths and identify influencing and influenced markets.

From this analysis we classify markets that act as price anchors in each country. Because local climate conditions have been found to affect and accurately predict agricultural prices, price dispersion, and yields in developing countries we use climate conditions at both the market location and anchor market locations as predictors. We show that during periods classified by drought, price prediction models using anchor market prices and high-resolution climate data have high degrees of predictive accuracy. We hope the results presented in this paper will assist policymakers, government stakeholders, and researchers in systematically constructing subnational price forecasts with minimal price data to be used in early warning and food security monitoring models.

 

How to cite: Anderson, P., Davenport, F., Baylis, K., and Shukla, S.: Using domestic weather disturbances and price transmission for maize price predictions in Southern Africa, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11432, https://doi.org/10.5194/egusphere-egu23-11432, 2023.

EGU23-13826 | ECS | Posters on site | ITS1.2/AS5.14

Change in the Tropical Storms activity in the future over the Ganges basin 

Haider Ali, Hayley Fowler, Malcolm Roberts, and Benoit Vanniere

The understanding of climate change impacts on tropical storms (TS) activity is crucial for better planning and risk assessment. Despite the theory and modeling suggest an increase in the TS activity with warming, the change in TS characteristics remain uncertain due to the limitations in the global climate models and tracking algorithms (tracker). Here, we performed tracker-inter-comparison and model-evaluation to find out the reliability of trackers and models at simulating the TS characteristics. We found that both trackers produce qualitatively similar results but quantitative different results due to different specifications of the algorithms and model bias. Our results show a decline in the frequency but rise in the strength of TS in the future for the Ganges and the Mekong basin.

How to cite: Ali, H., Fowler, H., Roberts, M., and Vanniere, B.: Change in the Tropical Storms activity in the future over the Ganges basin, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13826, https://doi.org/10.5194/egusphere-egu23-13826, 2023.

EGU23-15643 | ECS | Posters on site | ITS1.2/AS5.14

Measuring Carbon: A Tool for Analysing Gridded, Continuous, Carbon Measurements at High Temporal and Spatial Resolution 

Mitchell Odhiambo, Raunaq Jain, Yash Gorana, Nikita Kaushal, and Abhilash Mishra

Measuring carbon emissions at high temporal and spatial resolution covering all parts of the globe is key to understanding the sources and sinks of carbon. These measurements are critical for informing both climate modeling and policy decisions to mitigate climate change. Fragmented data sources and the requirement of significant programming knowledge to retrieve, clean, and analyze data from existing data sources pose a significant barrier for climate researchers. As understanding of climate science becomes crucial for fields beyond geophysical sciences, it is especially urgent to build tools that can enable researchers from diverse academic backgrounds to analyze carbon emission data from satellites. 

In this presentation, we will present a novel, user-friendly platform which has pre-built functions and analysis pipelines allowing scientists to perform common data analysis tasks without the need to write code. The underlying data lake combines NASA’s Orbiting Carbon Observatory (OCO-2 and OCO-3) data with other data sources (e.g. MODIS-based fire data) that facilitate a more accurate and complete understanding of the dynamics of the carbon cycle and the factors that influence it. 

We highlight how our approach integrating data discovery, access, and analysis of climate data can help democratize climate research and inform policymaking.

Potential research questions that can be addressed using this approach include: 

(i) studying the impacts of fires on the global carbon cycle with MODIS fire products providing information on the location, intensity, and types of fires, 

(ii) studying the photosynthetic activity of plants and the carbon cycle assimilating OCO-2 SIF data. OCO2-SIF data measures the fluorescence emitted by plants as a result of photosynthesis, which can be used as an indicator of plant health and productivity and 

(iii) AI-assisted audit of industrial emissions incorporating publicly available data on critical CO2 emitting sectors e.g. power plants, steel mills, cement plants, atmospheric “spillover” from agricultural and forest fires, traffic emissions, demographic and economic variables, etc

How to cite: Odhiambo, M., Jain, R., Gorana, Y., Kaushal, N., and Mishra, A.: Measuring Carbon: A Tool for Analysing Gridded, Continuous, Carbon Measurements at High Temporal and Spatial Resolution, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15643, https://doi.org/10.5194/egusphere-egu23-15643, 2023.

EGU23-17497 | Posters on site | ITS1.2/AS5.14

Bridging the Gap: Cervest's Climate Intelligence Approach for Effective Adaptation Strategies 

Edward Peter Morris Boyne, Chloé Prodhomme, Adam Jay Pain, and Benjamin Laken

Cervest, a climate intelligence startup, addresses the need for effective adaptation strategies by bridging the gap between disciplines. We use cutting-edge science techniques such as high-resolution convection-permitting models, remote sensing, hydrology, bayesian statistical modeling, machine learning, and data science to provide accurate, localized physical risk assessments for assets. Our climate intelligence product also accounts for assets vulnerability and multi-hazard, multi-risks. It can be used to assess not only the direct impacts of extreme events but also their indirect effects on supply chains and economic production networks. In this session, we will present our vision for the future of climate intelligence and share our novel probabilistic approach to assessing the impacts of climate change.

How to cite: Morris Boyne, E. P., Prodhomme, C., Pain, A. J., and Laken, B.: Bridging the Gap: Cervest's Climate Intelligence Approach for Effective Adaptation Strategies, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17497, https://doi.org/10.5194/egusphere-egu23-17497, 2023.

EGU23-17504 | Posters on site | ITS1.2/AS5.14

Cost-Effective Climate-Friendly Aircraft Flight Planning 

Abolfazl Simorgh and Manuel Soler

The aviation-induced non-CO2 climate effects, being responsible for two-thirds of aviation radiative forcing [1], have a direct dependency on atmospheric location and time of emissions. This implies that their associated impacts can be mitigated by planning climate-aware trajectories to avoid areas of airspace with large climate effects [2]. However, for the efficiency of such a mitigation strategy, one needs to consider various sources of uncertainty. In fact, if not accounted for within flight planning a priori, the rather immature scientific understanding of aviation-induced climate effects and uncertainty associated with emissions calculation and meteorological conditions can lead to inefficient aircraft trajectories. In addition, the mitigation potential achieved by the climate-optimal routing option increases the operating costs as the aircraft flies longer by re-routing climate-sensitive areas. In this respect, there is a need to plan robust climate-optimal aircraft trajectories having a minimum cost increase compared to the Business-as-usual (BAU) scenario.

In the current study, we present robust climate optimal aircraft trajectory planning, considering meteorological uncertainties. The airspace is assumed to be fully free routing. The information on the spatio-temporal dependency of aviation-induced climate effects is based on the latest version of the prototype algorithmic climate change functions (aCCF V1.1) [3]. An ensemble prediction weather forecast is used to characterize meteorological uncertainty. The flight planning objective is to find an efficient balance between the increased operating costs and the mitigated climate effects with acceptable ranges of uncertainty. The general approach for decision-making between conflicting objectives relies on building a Pareto-frontier by running the optimization many times, each corresponding to a weighting parameter in the objective function (see e.g., [4]). In this study, by proposing a more efficient modeling scheme in the definition of the aircraft trajectory optimization within the context of optimal control theory, we provide an ability to determine the highest possible mitigation potential with a user-specified limit on the increased operating cost and vice versa only in two iterations. In this approach, we define the “Lagrangian” term of the performance index (used to represents climate effects in the objective function) as an additional state variable, enabling to impose path and boundary constraints on the climate effect and its dispersion.

The effectiveness of the proposed approach is illustrated by considering the optimization of 10 flights on June 13, 2018, 0000UTC. Due to the strong variability among different members of relative humidity within the EPS weather forecast, the climate impact of contrails is highly uncertain. This in turn leads to high uncertainty in quantifying the net climate effects due to the dominant impact of contrails compared to the remaining species. For the considered case studies, it is shown that by employing the proposed trajectory optimizer, it is possible to minimize the climate effects while respecting the specified available extra operating cost in US dollars. In addition, the uncertainty on the quantified climate effects lies within the user-defined range, implying that the sensitivity of climate impact to the uncertainty in the forecasted weather conditions can be controlled.

How to cite: Simorgh, A. and Soler, M.: Cost-Effective Climate-Friendly Aircraft Flight Planning, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17504, https://doi.org/10.5194/egusphere-egu23-17504, 2023.

The aviation industry contributes to global warming by releasing CO2 and non-CO2 species into the atmosphere. The climate impacts of non-CO2 emissions have been claimed to be two times higher than the effects of CO2 alone [1]. Unlike CO2 emission, the climate impacts of non-CO2 species highly depend on geographical location, altitude, and time of the emissions. Thus, performing more efficient maneuvers to avoid climate hotspots can potentially mitigate their associated climate effects. So far, several studies have been conducted on micro-scale climate optimal aircraft trajectory planning (i.e., trajectory level) [2]. However, generating a climatically optimal flight plan for each aircraft is not the ultimate solution to this problem when it comes to global traffic scenarios.  
 
  Besides increasing the operating costs as the aircraft fly longer routes ( mainly due to the tendency to avoid climate-sensitive regions), the climate-optimal trajectories also alter the traffic pattern by increasing the congestion around climate hotspots, which may have negative implications, including, but not limited to, high traffic density, increased workload, complexity, and conflicts. Therefore, the evolution toward an environmentally friendly trajectory planning framework required a holistic perspective on the consequences of adopting climate-optimal routes at network scale. Nonetheless, in the literature, the problem of aircraft trajectory planning for the benefits of climate at a network scale is explored only in a free-routing airspace, considering a regional scenario (i.e., only Spain airspace), and constant altitude for trajectory optimization [3].
 
 
  In this study, we aim to explore this problem considering a real large-scale scenario including ≈ 6000 flights on December 20th, 2018, from 12:00 to 16:00 over European airspace. The flight information, including the time and altitude of the first crossed waypoint within the considered time interval, has been extracted from the DDR2 dataset. For flights that start or land outside ECAC airports, we model only the segment of the flight that takes place within ECAC airspace. The algorithmic climate change functions proposed by [4] are employed to quantify the climate impact of each species, including contrails, and emissions of nitrogen oxides, CO2, and water vapor, in terms of average temperature response over the next 20 years. Our recently developed tool for climate-optimal aircraft trajectory planning, ROOST, is then used to optimize each trajectory 1 within the current structured airspace [5]. The effects of adopting climate optimized trajectories are assessed in terms of complexity, demand, and the number of conflicts. A performance map associated with each indicator is generated to spatially analyze the overall behavior of optimized trajectories and detect congested areas.  
  
  For the considered scenario, the results indicate that by adopting trajectories with less climate impact, the complexity, demand, and conflicts are increased around climate hotspots. This trend is mainly due to the tendency to avoid climate-sensitive regions. In order to mitigate such changes in traffic patterns, an efficient resolution strategy is needed to find the optimal mechanisms to manage the ATM system from a climatic perspective.  

How to cite: Baneshi, F. and Soler, M.: Network Assessment of the Aviation Climate Impact Considering the European Structured Airspace, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17517, https://doi.org/10.5194/egusphere-egu23-17517, 2023.

The deposition of heavy metals on water bodies and soil has adverse consequences on
human health. The elevated Coal-based energy production and increased industrial emissions
have also prompted us to study about heavy metals reactive nitrogen species in the
atmosphere. In the present work, the samples of rain water were collected from a residential
site in south-west Delhi. The samples were analyzed for selected heavy metals by using ICP-
OES. The heavy metals analysis involved voltammetry method using 797 VA Computrace
(Metrohm, Switzerland) instrument. The analysis of Total Nitrogen (TN) and dissolved
organic carbon (DOC) was carried out by using chemiluminescence based TN/TOC analyzer
(Shimadzu model TOC-LCPH E200 ROHS). The mean values of Cu, Mn, Zn, Al, As and Hg
were calculated as 34.5 mg/l, 19.5 mg/l, 52.7 mg/l, 392.3 mg/l, 9.8 mg/l and 1.6 mg/l
respectively. The mean values for TN and DOC were 12.7mg/l and 2.8 mg/l respectively. The
detailed results will be discussed in the EGU General Assembly Meeting.

Keywords: Total Nitrogen, wet deposition, ICP-OES, voltammetry, agricultural area.

How to cite: sunaina, S.: Wet deposition of heavy metals, reactive nitrogen species and dissolved organic carbonat a residential site in Delhi region, India, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-345, https://doi.org/10.5194/egusphere-egu23-345, 2023.

EGU23-1075 | ECS | Posters on site | GI1.3

What can we learn from nested IoT low-cost sensor networks for air quality?  A case study of PM2.5 in Birmingham UK. 

Nicole Cowell, Clarissa Baldo, William Bloss, and Lee Chapman

Birmingham is a city within the West Midlands region of the United Kingdom. In June 2021, coinciding with the introduction of the Clean Air Zone by Birmingham City Council (BCC), multiple low-cost IoT sensor networks for air pollution were deployed across the city by both the University of Birmingham and BCC. Low-cost sensor networks are growing in popularity due to their lower costs compared to regulatory instruments (£10’s-£1000’s per unit compared to £10,000+ per unit) and the reduced need for specialised staff allow for deployments at greater spatial scales (1-3).  Although such low-cost sensing is often associated with uncertainty, the measurement of PM2.5 optical particle counters have been generally shown to perform well, giving indicative insight into concentrations following calibrations and corrections for external influence such as humidity (4-7). 

One common problem with sensor networks is they tend to be isolated and unopen deployments, deployed and maintained by an interested party with the focus of their own monitoring goal. To tackle this, Birmingham Urban Observatory was an online platform created and used by researchers at the University of Birmingham to host and share open access meteorological and air pollution data from low-cost sensor deployments. Whilst hosting and displaying data from two of their own deployments of air quality sensors (Zephyrs by Earthsense and AltasensePM: an in-house designed PM sensor), the platform also pulled data from the DEFRA AURN sites and collaborated with local government to pull data from their own low-cost sensor network. The result was a real-time view of environmental data produced from a series of nested arrays of sensors.

This poster presents findings from this combined low-cost network, considering the successes and pitfalls of the low-cost monitoring network alongside insight into regional and local PM2.5 concentrations. Colocations against reference instruments within the network demonstrate good performance of the low-cost sensors after calibration and data validation but the project experienced challenges in deploying the network and sensor reliability. Low-cost sensor data generally gives novel insight into spatial analysis of PM2.5 across the city and this is presented alongside other experiences of deploying and using sensor networks for air quality.

1 Lewis et al., (2016) https://doi.org/10.1039/C5FD00201J

2 Chong and Kumar. (2003) doi: 10.1109/JPROC.2003.814918

3 Snyder et al., (2013) https://doi.org/10.1021/es4022602

4 Magi et al., (2020) https://doi.org/10.1080/02786826.2019.1619915

5 Crilley et al., (2018) https://doi.org/10.5194/amt-11-709-2018

6 Cowell et al., (2022) https://doi.org/10.3389/fenvs.2021.798485

7 Cowell et al., (2022) https://doi.org/10.1039/D2EA00124A

How to cite: Cowell, N., Baldo, C., Bloss, W., and Chapman, L.: What can we learn from nested IoT low-cost sensor networks for air quality?  A case study of PM2.5 in Birmingham UK., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1075, https://doi.org/10.5194/egusphere-egu23-1075, 2023.

EGU23-2847 | Posters on site | GI1.3

Atmospheric ammonia in-situ long-term monitoring: review worldwide strategies and recommendations for implementation 

Aude Bourin, Pablo Espina-Martin, Anna Font, Sabine Crunaire, and Stéphane Sauvage

Ammonia (NH3) is the major alkaline gas in the atmosphere and the third most abundant N-containing species, after N2 and N2O. It plays an important role in N deposition processes, responsible of several damages on ecosystems, and it is also a precursor of fine particulate matter, known to cause numerous impacts on human health. Despite this, not many countries have implemented long-term monitoring of NH3 in their air quality programs due to the lack of consensus on limit values for ambient levels and a reference method of measuring this gas. In the climate change context, governments and health organizations are increasingly concerned about NH3 and its effects. As a proof, the revision of the EU air quality directives proposes the inclusion of NH3 as a mandatory pollutant for several urban and rural supersites for all member states.

Currently, there are only 12 long term programs worldwide dedicated specifically to measure NH3 or including gas-phase measurements of NH3. The longest NH3 time series come from UK and Africa, where measurements start in mid-1990. The rest of locations have started after 2000 and they have lower temporal coverage, between 5 and 22 years. The objectives pursued by these networks are to follow long term spatio-temporal trends, assess the N deposition on sensitive ecosystems, validate emission and/or chemistry transport models and help to understand the effectiveness of air pollution control and mitigation policies. Most of these networks operate using a combination of low-cost samplers with a high spatial density with few collocated sites with high time resolution instrumentation to help calibrate passive samplers and to better monitor the fine temporal variability of NH3. This combined approach has proven to be successful for most of the proposed objectives.

However, there are several differences that may difficult harmonizing the information at both the technical and scientific level. At the technical level these include type and number of passive samplers per site, calibration protocol, data control and quality analysis, exposure duration and type of high time resolution sampling method. On the scientific level, increased difficulty understanding the operative parameters and scientific results may come from language barriers (non-English reports), availability of the data (whether it is public or not), and gaps on the knowledge of NH3 levels on a spatial scale due to differences in the implementation of monitoring strategies within the same country.

This work aims to review synthetically the world current long-term NH3 networks and provide some insight and recommendations for other countries and supranational programs aiming to establish long term monitoring networks of NH3, based on cost-effective, technical, and operational criteria.

How to cite: Bourin, A., Espina-Martin, P., Font, A., Crunaire, S., and Sauvage, S.: Atmospheric ammonia in-situ long-term monitoring: review worldwide strategies and recommendations for implementation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2847, https://doi.org/10.5194/egusphere-egu23-2847, 2023.

EGU23-2984 | ECS | Posters virtual | GI1.3

The COllaborative Carbon Column Observing Network COCCON: Showcasing GHG observations at the COCCON Tsukuba site 

Matthias Max Frey, Isamu Morino, Hirofumi Ohyama, Akihiro Hori, Darko Dubravica, and Frank Hase

Greenhouse gases (GHGs) play a crucial role regarding global warming. Therefore, precise and accurate observations of anthropogenic GHGs, especially carbon dioxide and methane, are of utmost importance for the estimation of their emission strengths, flux changes and long-term monitoring. Satellite observations are well suited for this task as they provide global coverage. However, like all measurements these need to be validated.

The COllaborative Carbon Column Observing Network (COCCON) performs ground-based observations to retrieve column-averaged dry air mole fractions of GHGs (XGAS) with reference precision. The instrument used by the network is the EM27/SUN, a solar-viewing Fourier Transform infrared (FTIR) spectrometer. COCCON data are of high accuracy as COCCON uses species dependent airmass-independent and airmass-dependent adjustments for tying the XGAS products to TCCCON (Total Carbon Column Observing Network) and thereby to the World Meteorological Organization (WMO) reference scale. Moreover, instrument specific characteristics are measured for each COCCON spectrometer, and taken into account in the data analysis.

Here we first introduce the COCCON network in general and summarize its capabilities for various challenges including satellite and model validation, long-term observation of GHGs, and local and regional GHG source emission strength estimations. By example of the COCCON Tsukuba station we highlight in detail its usefulness for the above-mentioned applications.

How to cite: Frey, M. M., Morino, I., Ohyama, H., Hori, A., Dubravica, D., and Hase, F.: The COllaborative Carbon Column Observing Network COCCON: Showcasing GHG observations at the COCCON Tsukuba site, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2984, https://doi.org/10.5194/egusphere-egu23-2984, 2023.

EGU23-7462 | ECS | Orals | GI1.3

Data infrastructure for nitrogen compound emissions monitoring 

Daniel Bertocci, Burcu Celikkol, Shaojie Zhuang, and Jasper Fabius

Emissions of nitrogen compounds, including nitrogen dioxide (NO2) and ammonia (NH3), have significant impacts on air quality and the environment. To effectively monitor the spatial and temporal variability of these emissions and the efficacy of emission mitigation measures, OnePlanet Research Center is developing a low-cost sensor system to monitor outdoor NO2 and NH3concentrations. This sensor system is designed to be deployable in fine-grained networks to accurately capture the dispersion from an emitting source. The deployment of multitudes of such sensor systems will result in large volumes of data. For this purpose, we developed a data infrastructure using the OGC SensorThings API and TimescaleDB, a time-series database extending PostgreSQL. This infrastructure allows for the efficient storage, management, and analysis of large volumes of spatiotemporal data from various sources, such as air quality monitoring networks, meteorological data, and agricultural practices. We demonstrate the potential of this infrastructure by using it in citizen science project COMPAIR, combining data from various sensors to gain insights on the air quality impact of urban circulation policies. The resulting data platform will facilitate the development of decision support tools and the implementation of targeted emission reduction strategies.

How to cite: Bertocci, D., Celikkol, B., Zhuang, S., and Fabius, J.: Data infrastructure for nitrogen compound emissions monitoring, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7462, https://doi.org/10.5194/egusphere-egu23-7462, 2023.

Even in the presence of more reliable air quality tools, low-cost sensors have the benefit of recording data on highly localized spatial and temporal scales, allowing for multiple measurements within a single satellite pixel and on pixel boundaries. However, they are less accurate than their regulatory-grade counterparts, requiring regular co-locations with accepted instruments to ensure their validity. Thus, the addition of low-cost sensors to a field campaign – where reference-grade air quality instruments are abundant – not only provides ample opportunities for low-cost sensor co-location and calibration, but also allows the low-cost instruments to be used for sub-pixel validation, covering more surface area than the regulatory instruments alone with a network of sensors. During the summer of 2014, our low-cost sensor network was deployed during the Front Range Air Pollution and Photochemistry Éxperiment (FRAPPÉ) campaign conducted to sample the composition of air at and above ground level in northeastern Colorado, USA. The low-cost sensor platform included a suite of gas-phase sensors, notably NO2 and two generalized volatile organic compound (VOC) sensors, which were leveraged together to quantify speciated hydrocarbons such as formaldehyde. These key pollutants were chosen for their impacts on human health and climate change, as well as their inclusion on the TEMPO satellite launching this year. Airborne campaign measurements included slant column optical observations of formaldehyde (HCHO), nitrogen dioxide (NO2), and ozone (O3). Myriad additional in-situ instruments described chemical composition up to approximately 5 km above surface level. Ground-based instrumentation included both stationary and mobile regulatory-grade instruments, which were used for sensor calibration. Machine learning techniques such as artificial neural networks (ANNs) were used to match the low-cost signals to that of the reference-grade instruments. Here, we compare calibrated low-cost sensor data collected at ground level in a variety of locations along Colorado’s Front Range to various data sources from the FRAPPÉ campaign to better understand how well airborne and regulatory ground-based measurements can be extrapolated to other locations. Further, as the slant column measurements act as satellite simulators, we explore how low-cost instruments can be used for satellite validation purposes. Comparisons among these different data types also have important implications in data fusion.

How to cite: Okorn, K., Iraci, L., and Hannigan, M.: Comparing Low-Cost Sensors with Ground-Based and Airborne In-Situ and Column Observations of NO2 and HCHO during the FRAPPE Field Campaign in Colorado, USA, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7839, https://doi.org/10.5194/egusphere-egu23-7839, 2023.

EGU23-8631 | Posters on site | GI1.3 | Highlight

Ambient conditions and infrared sky brightness in the Chilean Atacama Desert 

Wolfgang Kausch, Stefan Kimeswenger, Stefan Noll, and Roland Holzlöhner

The Atacama Desert in the Chilean Andes region is one of the dryest areas in the world. Due to its unique location with stable subtropical meteorological conditions and high mountains, it is an ideal site for the astronomical telescope facilities of the European Southern Observatory (ESO). The special meteorological conditions are continuously monitored at Cerro Paranal (the location of the Very Large Telescope) by measuring various parameters like temperature, pressure, humidity, precipitable water vapour (PWV), wind speed and direction, and sky radiance and bolometric sky temperature, respectively, the latter being crucial for astronomical observations in the thermal infrared regime. ESO operates several site monitoring systems for that purpose, e.g. the ESO MeteoMonitor, the Differential Image Motion Monitor (DIMM) and a Low Humidity And Temperature PROfiler (L-HATPRO) microwave radiometer providing detailed water vapour and temperate profiles up to a height of 12km in various directions. 


We have assembled all available data for a period of 4.5 years (2015-07-01 through 2019-12-31) and created a unique data set from it. This period also covers the strong El Niño event at the end of 2015. In this poster we present statistical results on the overall conditions and trends, and compare our measurements of the nocturnal sky brightness with an empirical model as function of the ambient temperature, PWV and zenith distance.

How to cite: Kausch, W., Kimeswenger, S., Noll, S., and Holzlöhner, R.: Ambient conditions and infrared sky brightness in the Chilean Atacama Desert, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8631, https://doi.org/10.5194/egusphere-egu23-8631, 2023.

Air quality monitoring networks provide invaluable data for studying human health, environmental impacts, and the effects of policy changes,  but obtaining high quality data can be costly, with each site in a monitoring network requiring instrumentation and skilled operator time. It is therefore important to ensure that each monitor in the network is providing unique data to maximize the value of the entire network.  Differences in measurement approaches for the same chemical between monitoring stations may also result in discontinuities in the network data.  Both of these factors suggest the need for objective, machine-learning methodologies for monitoring network data analysis.   

Air quality models are another valuable tool to augment monitoring networks.  The models simulate air quality over a large region where monitoring may be sparse. The gridded output from air-quality models thus contain inherent information on the similarity of sources, chemical oxidation pathways and removal processes for chemicals of interest, provided appropriate tools are available to identify these similarities on a gridded basis.  The output from these models can be immense, again requiring the use of special, highly optimized tools for post-processing analysis.

Spatiotemporal clustering is a family of techniques that have seen widespread use in air quality, whereby time-series taken at different locations are grouped based on the level of similarity between time-series data within the dataset.   Hierarchical clustering is one such algorithm, which has the advantage of not requiring an a priori assumption about how many clusters there might be (unlike K-means).  However, traditional approaches for hierarchical clustering become computationally expensive as the number of time-series increases in size, resulting in prohibitive computational costs  when the total number of time-series to be compared rises above 30,000, even on a supercomputer.  Similarly, the comparison and clustering of large numbers of discrete data (such as multiple mass spectrometer data sampled at high time resolution from a moving laboratory platform) becomes computationally prohibitive using conventional methods. 

In this study we present a high-performance hierarchical clustering algorithm which is able to run in parallel over many nodes on massively parallel computer systems, thus allowing for efficient clustering for very large monitoring network and model output datasets.   The new high-performance program is able to cluster 290,000 annual time series (from either monitoring network data or gridded model output) in 13 hours on 800 nodes. We present here some example results showing how the algorithm can be used to analyse very large datasets, providing new insights into “airsheds” depicting regions of similar chemical origin and history, different spatial regimes for nitrogen, sulphur, and base cation deposition, .  These analyses show how different processes control each species at different potential monitoring site locations, via cluster-generated airshed maps for each species. The efficiency and flexibility of the algorithm allows for extremely large datasets to be analysed in hours of wall-clock time instead of weeks or months. The new algorithm is being used as the numerical engine for a new tool for the analysis of EU monitoring network data. 

How to cite: Lee, C., Makar, P., and Soares, J.: Spatio-temporal clustering on a high-performance computing platform for high-resolution monitoring network analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8841, https://doi.org/10.5194/egusphere-egu23-8841, 2023.

22 cost-efficient (aka ‘low-cost’) commercially available particulate matter (PM) measurement devices were installed in a diverse urban area in Leipzig, Germany. The instruments measure mostly PM2.5, some additionally PM10, and are equipped with methods for quality assurance such as conditioning to a defined temperature and regular internal calibration. In order to investigate the spread between the instruments and to enable a pre-campaign calibration, all instruments were setup in the laboratory and the outside air and compared against the same reference measurements.

Since July 2022, the measurement network was installed. It covers roughly 2x2 km2 and holds different urban features like residential and commercial buildings, important main roads, city parks, and small open building gaps. Within the network there is an official air quality monitoring station located directly at a main road. In addition, at two further official monitoring stations as well as at observation stations of the Leibniz Institute for Tropospheric Research instruments were installed to study the long-term performance, dependence on meteorological conditions and comparison to reference measurements. The measurements will take place until end of 2023.

The cost-efficient instruments perform generally quite well after the calibration. In particularly for higher PM loads > 10 µg m-3 the agreement against references is mostly satisfying. However, under very high relative humidity and cold temperatures, some instruments lacked to condition the air sufficiently. Despite these difficulties, the chosen instruments have the potential for application in monitoring of air quality limit values, i.e. the answer the question how often are certain limits exceeded.

Furthermore, differences between different local features in the observation area could be observed in e.g., the diurnal cycle but also peak and mean concentrations.

This work is co-financed with tax funds on the basis of the budget passed by the Saxon State Parliament (funding number 100582357).

How to cite: Schrödner, R., Alas, H., and Voigtländer, J.: Application of cost-efficient particulate matter measurement devices in an urban network and comparison to state-of-the-art air quality monitoring, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9356, https://doi.org/10.5194/egusphere-egu23-9356, 2023.

EGU23-9537 | Posters on site | GI1.3

The Global Environmental Measurement and Monitoring Initiative – An International Network for Local Impact 

Daniel Klingenberg, D. Michelle Bailey, David Lang, and Mark Shimamoto

The Global Environmental Measurement and Monitoring (GEMM) Initiative is an international project of Optica and the American Geophysical Union seeking to provide precise and usable environmental data for local impact. The Initiative brings together science, technology, and policy stakeholders to address critical environmental challenges and provide solutions to inform policy decisions on greenhouse gases (GHGs) and air and water quality. GEMM Centers are currently established in Scotland, Canada, New Zealand, and the United States. These Centers represent partnerships with leading institutions that are actively working toward developing or deploying new measurement technology and improved climate models. Additional Centers are under development in India and Australia with plans to expand to Asia and Africa.

In addition to establishing monitoring centers worldwide, GEMM actively engages with other sectors (including industry, standards organizations, and regional or national governments) to support the incorporation or adoption of these evidence-based approaches into decision making processes. For example, Glasgow, Scotland is piloting the GEMM Urban Air Project, deploying a low-cost, real-time, ground-based network of devices that continuously monitors GHGs and air pollutants at a neighborhood scale. The sensor network in Glasgow is increasing the precision of local models that can provide the city with information to assess current policies and support future action. Here we will share the progress and outputs of the GEMM Initiative to date and highlight paths forward to grow the network.

How to cite: Klingenberg, D., Bailey, D. M., Lang, D., and Shimamoto, M.: The Global Environmental Measurement and Monitoring Initiative – An International Network for Local Impact, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9537, https://doi.org/10.5194/egusphere-egu23-9537, 2023.

Since the discovery of the chlorofluorocarbons (CFCs) implication in stratospheric ozone destruction, the Montreal Protocol (1987) has aimed at controlling the production of CFCs and other ozone depleting substances (ODS) in order to protect and then recover the ozone layer. Consequently, temporary substitutes for CFCs have been developed and produced by the industry. First substitute molecules were hydrochlorofluorocarbons (HCFCs), which have smaller ozone depletion potentials (ODP) than CFCs since their atmospheric lifetimes are shorter. Nevertheless, HCFCs still contain chlorine atoms and hence, also deplete the stratospheric ozone, requiring them to be banned in turn. Thus, chlorine-free molecules, i.e. hydrofluorocarbons (HFCs) such as CH2FCF3 (HFC-134a) were introduced to replace both CFCs and HCFCs. Even if HFCs do not contribute to ozone depletion, they are very powerful greenhouse gases since they have great global warming potentials (GWPs). Consequently, the Kigali amendment (2016) to the Montreal Protocol aimed for their phase-out.

The atmospheric concentrations of CFCs have decreased in response to the phase-out and ban of their production by the Montreal Protocol and its subsequent amendments, while the HCFCs burden is now leveling off. In contrast, the atmospheric concentrations of HFCs have increased notably in the last two decades.

We present the first retrievals of HFC-134a from Fourier Transform Infra-Red (FTIR) solar spectra obtained from a remote site of the Network for the Detection of Atmospheric Composition Change (NDACC.org): the Jungfraujoch station (Swiss Alps). We discuss of the applicability of our retrieval strategy to other NDACC sites, for future quasi global monitoring from ground-based observations. We further perform first comparisons with other datasets as ACE-FTS satellite observations.

 

How to cite: Pardo Cantos, I. and Mahieu, E.: First HFC-134a retrievals and analysis of long-term trends from FTIR solar spectra above NDACC network stations: the Jungfraujoch case, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11033, https://doi.org/10.5194/egusphere-egu23-11033, 2023.

Monitoring networks, able to effectively provide high-frequency geochemical data for characterizing the geochemical behavior of the main greenhouse gases (i.e., CO2 and CH4) and pollutants (e.g., heavy metals) are crucial tools for the assessment of air quality and its role in climate changes. However, the provision of measurement stations dedicated to monitor gas species and particulate in polluted areas is complicated by the high cost of their set-up and maintenance. In the last decade, traditional instruments have tentatively been coupled with low-cost sensors for improving spatial coverage and temporal resolution of air quality surveys. The main concerns of this new approach regard the in-field accuracy of the low-cost sensors, being significantly dependent on: (i) cross-sensitivities to other atmospheric pollutants, (ii) environmental parameters (e.g., relative humidity and temperature), and (iii) detector signal degradation over time.

This study presents the results of a geochemical survey carried out in the Greve River Basin (Chianti territory, Central Italy) from May to September 2022 by adopting two measuring strategies: (i) deployment of a mobile station, along predefined transepts within the Greve valley, equipped with a Picarro G2201-i analyzer to measure CO2 and CH4 concentrations and δ13C-CO2 and δ13C-CH4 values (‰ vs. V-PDB) by Wavelength-Scanned Cavity Ring-Down Spectroscopy (WS-CRDS); (ii) continuous monitoring, at five fixed sites positioned at different altitudes, of CO2 and CH4 concentrations through prototyped low-cost stations, coupled with atmospheric deposition and rain samplers to collect particulate samples for chemical lab analysis. The low-cost monitoring stations housed (i) a non-dispersive infrared (NDIR) sensor for CO2 concentrations, (ii) a solid-state metal oxide sensor (MOS) for CH4 concentrations, (iii) a laser light scattering sensor (LSPs) for PM2.5 and PM10 concentrations, and (iv) a sensor for temperature and relative humidity in the air. The CO2 and CH4 sensors have been calibrated in-field based on parallel measurements with the Picarro G2201-i and elaborating the calibration data with the Random Forest machine learning-based algorithm.

The measurements carried out along the transepts showed that the downstream areas next to the metropolitan city of Florence were affected by the highest concentrations of CO2 and CH4, marked by isotopic signatures revealing a clear anthropogenic origin, mainly ascribed to vehicular traffic. The distribution of these carbon species reflected the evolution of the atmospheric boundary layer, displaying higher concentrations during the early morning, when gas accumulation occurred due to stable atmospheric conditions, and lower concentrations during daytime when the heating of the surface favored the dilution of air pollutants due to the establishment of convective turbulence. These observations were confirmed by the network of low-cost stations, which allowed to simultaneously monitor the distribution of the atmospheric pollutants at different altitudes in the valley. The distribution of particulate was consistent with that of the gaseous species, and the main sources were clearly distinguished based on the chemical composition of the atmospheric deposition in the collection sites. The promising results from the present study could result in an affordable approach to effectively improve air quality monitoring strategies and support data-driven policy actions to reduce carbon emissions.

How to cite: Biagi, R., Ferrari, M., Tassi, F., and Venturi, S.: Multi-instrumental approach for air quality monitoring: characterization and distribution of greenhouse gases and atmospheric metal deposition in the Greve River Basin (Chianti territory, Central Italy)., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11385, https://doi.org/10.5194/egusphere-egu23-11385, 2023.

EGU23-13997 | ECS | Posters on site | GI1.3

Correction, gap filling and homogenization on daily level of the historical DMI station network temperature data 

Dina Rapp, Bo Møllesøe Vinther, Jacob L. Høyer, and Eigil Kaas

As climate change is amplified in the Arctic, it is crucial to have temperature records of high temporal resolution and quality in this area. This will help improve understanding of the involved physical mechanisms, assessment of the past changes and improve predictions for the future temperature development in the Arctic. In this study temperature measurements from the DMI Greenland station network spanning 1784-present day are corrected, gap-filled and homogenized on a daily level. Currently homogenized data is only available on a monthly level, and the more recent data has not been homogenized. The data is currently used for purposes like assessment and predictions of the surface mass balance of the Greenland Ice Sheet, temperature/climate reanalyses, validation of proxy data, etc.  

This study presents a method for improving the calculation of daily average temperatures, from the current practice of averaging the available measurements without considering what time of day they are from and how the measurements are distributed. The method is based on a moving average taking into consideration time of day, time of year and latitude/longitude of the station in question. An estimate of the related uncertainty is also calculated. Following the generation of daily average temperatures, different gap filling methods are tested. The different algorithms tested and compared are: simple gap filling by linear interpolation with other stations, single station temporal linear interpolation and MEM (Maximum Entropy Method). Finally, homogenization on daily level is performed. These steps will in turn also improve the monthly and annual average temperatures for the DMI Greenland station network. 

How to cite: Rapp, D., Møllesøe Vinther, B., L. Høyer, J., and Kaas, E.: Correction, gap filling and homogenization on daily level of the historical DMI station network temperature data, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13997, https://doi.org/10.5194/egusphere-egu23-13997, 2023.

The Global Atmosphere Watch (GAW) Programme was established in 1989 in recognition of the need for improved scientific understanding of the increasing influence of human activities on atmospheric composition and subsequent societal impacts. It is implemented as an activity of the World Meteorological Organization, a specialized agency of the United Nations system, and is funded by the organization member countries.

As an international programme, GAW supports a broad spectrum of applications from atmospheric composition-related services to contribution to environmental policy. The examples of the later include provision of a comprehensive set of high quality and long-term globally harmonized observations and analysis of atmospheric composition for the United Nations Framework Convention on Climate Change (UNFCCC), the Montreal Protocol on Substances that Deplete the Ozone Layer and follow-up amendments, and the Convention on Long-Range Transboundary Air Pollution (CLRTAP).

The programme includes six focal areas: Greenhouse Gases, Ozone, Aerosols, Reactive Gases, Total Atmospheric Deposition and SolarUltraviolet Radiation.

The surface-based observational network of the programme includes Global (31 stations) and Regional (about 400 stations) stations where observations of various GAW parameters occur. These stations are complemented by regular ship cruises and various contributing networks. All observations are linked to common reference standards and the observational data are made available at seven designated World Data Centres (WDC).

Surface-based observations are complemented by airborne and space-based observations that help to characterize the upper troposphere and lower stratosphere, with regards to ozone, solar radiation, aerosols, and certain trace gases.

Requirements to become a GAW station are detailed in the GAW Implementation Plan 2016-2023 (WMO, 2017). A new IP is in preparation, the four strategic objectives will be presented.

  • The GAW Quality Management comprises: Data Quality Objectives, Measurement Guidelines, Standard Operating Procedures and Data Quality Indicators. Throughout the programme the common quality assurance principles apply, that include requirements for the long-term sustainability of the observations, use of one network standard for each variable and implementation of the measurement practices that satisfy the set data quality objectives. GAW implements open data policy and requires observational data be made available in the dedicated data centers operated by WMO Member countries.

The programme relies on different types of central facilities: Central Calibration Laboratories, Quality Assurance/Science Activity Centres, World and Regional Calibration Centres, which are also directly supported and implemented by the individual Member countries for the global services.

Majority of the recommendations regarding measurement and quality assurance procedures are developed by the expert and advisory groups within the programme, often those rely on the expertise withing the contributing networks and collaborating organizations, like the Aerosol, Clouds and Trace Gases Research Infrastructure (ACTRIS) or the Integrated Carbon Observation System (ICOS).

One of the GAW priorities is to expand and strengthen partnerships with contributing networks, through development of statements and strategies to articulate the mutual benefits for the collaborations and stream-line processes of data reporting and exchange of QA standards and metadata. This involves collaboration with national and regional environmental protection agencies and the development of harmonized metadata and data exchange and quality information.

How to cite: Moreno, S.: The WMO Global Atmosphere Watch Programme new implementation plan and strategic objectives, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14442, https://doi.org/10.5194/egusphere-egu23-14442, 2023.

EGU23-14459 | ECS | Orals | GI1.3

Developing and testing a validation procedure to successfully use on-the-move sensors in urban environments 

Francesco Barbano, Erika Brattich, Carlo Cintolesi, Juri Iurato, Vincenzo Mazzarella, Massimo Milelli, Abdul Ghafoor Nizamani, Maryam Sarfraz, Antonio Parodi, and Silvana Di Sabatino

With the increasing attempt to empower citizens and civil society in promoting virtuous behaviours and relevant climate actions, novel user-friendly and low-cost tools and sensors are nowadays being developed and distributed on the market. Most of these sensors are typically easy to install with a ready-to-use system, while measured data are automatically uploaded on a mobile application or a web dashboard which also guarantees secure and open access to measurements gathered by other users. However, the quality of the datum and the calibration of these sensors are often ensured against research-grade instrumentations only in the laboratory and rarely in real-world measurement. The discrepancies arising between these low-cost sensors and research-grade instrumentations are such that the first might be impossible to use if a validation (and re-calibration if needed) under environmental conditions is not performed. Here we propose a validation procedure applied to the MeteoTracker, a recently developed portable sensor to monitor atmospheric quantities on the move. The ultimate scope is to develop and implement a general procedure to test and validate the quality of the MeteoTracker data to compile user guidelines tailored for on-the-move sensors. The result will evaluate the feasibility of MeteoTracker (and potentially other on-the-move sensors) to integrate the existing monitoring networks on the territory, improve the atmospheric data local coverage and support the informed decision by the authorities. The procedure will include multi-sensor testing of all the sensor functionalities, validation of all data simultaneously acquired by several sensors under similar conditions, methods and applications of comparisons with research-grade instruments. The first usage of the MeteoTracker will be also presented for different geographical contexts where the sensors will be used for citizen science activities and develop a monitoring network of selected Essential Variables within the HORIZON-EU project I-CHANGE (Individual Change of HAbits Needed for Green European transition).

How to cite: Barbano, F., Brattich, E., Cintolesi, C., Iurato, J., Mazzarella, V., Milelli, M., Nizamani, A. G., Sarfraz, M., Parodi, A., and Di Sabatino, S.: Developing and testing a validation procedure to successfully use on-the-move sensors in urban environments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14459, https://doi.org/10.5194/egusphere-egu23-14459, 2023.

EGU23-15087 | Posters on site | GI1.3

Applications of an advanced clustering tool for EU AQ monitoring network data analysis 

Joana Soares, Christoffer Stoll, Islen Vallejo, Colin Lee, Paul Makar, and Leonor Tarrasón

Air quality monitoring networks provide invaluable data for studying human health, environmental impacts, and the effects of policy changes. In a European legislative context, the data collected constitutes the basis for reporting air quality status and exceedances under the Ambient Air Quality Directives (AAQD) following specific requirements. Consequently, the network's representativity and ability to accurately assess the air pollution situation in European countries become a key issue. The combined use of models and measurements is currently understood as the most robust way to map the status of air pollution in an area, allowing it to quantify both the spatial and temporal distribution of pollution. This spatial-temporal information can be used to evaluate the representativeness of the monitoring network and support air quality monitoring design using hierarchical clustering techniques.

The hierarchical clustering methodology applied in this context can be used as a screening tool to analyse the level of similarity or dissimilarity of the air concentration data (time-series) within a monitoring network. Hierarchical clustering assumes that the data contains a level of (dis)similarity and groups the station records based on the characteristics of the actual data. The advantage of this type of clustering is that it does not require an a priori assumption about how many clusters there might be, but it can become computationally expensive as the number of time-series increases in size. Three dissimilarity metrics are used to establish the level of similarity (or dissimilarity) of the different air quality measurements across the monitoring network: (1) 1-R, where R is the Pearson linear correlation coefficient, (2) the Euclidean distance (EuD), and (3) multiplication of metric (1) and (2). The metric based on correlation assesses dissimilarities associated with the changes in the temporal variations in concentration. The metric based on the EuD assesses dissimilarities based on the magnitude of the concentration over the period analysed. The multiplication of these two metrics (1-R) x EuD assesses time variation and pollution levels correlations, and it has been demonstrated to be the most useful metric for monitoring network optimization.

This study presents the MoNET webtool developed based on the hierarchical clustering methodology. This webtool aims to provide an easy solution for member states to quality control the data reported as a tier-2 level check and evaluate the representativeness of the air quality network reporting under the AAQD. Some examples from the ongoing evaluation of the monitoring site classification carried out as a joint exercise under the Forum for Air Quality Modeling (FAIRMODE) and the National Air Quality Reference Laboratories Network (AQUILA) are available to show the usability of the tool. MoNet should be able to identify outliers, i.e., issues with the data or data series with very specific temporal-magnitude profiles, and to distinguish, e.g., pollution regimes within a country and if it resembles the air quality zones required by the AAQD and set by the member states; stations monitoring high-emitting sources; background regimes vs. a local source driving pollution regime in cities.

How to cite: Soares, J., Stoll, C., Vallejo, I., Lee, C., Makar, P., and Tarrasón, L.: Applications of an advanced clustering tool for EU AQ monitoring network data analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15087, https://doi.org/10.5194/egusphere-egu23-15087, 2023.

EGU23-15609 | ECS | Posters on site | GI1.3

A compact and customisable street-level sensor system for real-time weather monitoring and outreach in Freiburg, Germany 

Gregor Feigel, Marvin Plein, Matthias Zeeman, Ferdinand Briegel, and Andreas Christen

Climate adaptation and emergency management are major challenges in cities, that benefit from the incorporation of real-time weather, air quality, differential exposure and vulnerability data. We therefore need systems that allow us to map, for example, localised thermal heat stress, heavy precipitation events or air quality spatially resolved across cities at high temporal resolution. Key to the assessment of average conditions and weather extremes in cities are systems that are capable of resolving intra-urban variabilities and microclimates at the level of people, hence in the urban canopy layer at street-level. Placing sensors at street-level, however, is challenging: Sensors need to be small, rugged, safe, and they must measure a number of quantities within limited space. Such systems may ideally require little or no external power, provide remote accessibility, sensor interoperability and real-time data transfer and must be cost-effective for mass deployment. However, these characteristics as well as a wide spectrum of observed variables are not available in current commercial sensor network solutions, hence we designed and implemented a custom partly in-house developed two-tiered sensor system for mounting and installation at 3 m height on city-owned street lights in Freiburg, Germany.

Our partly in-house developed two-tiered sensor network, consisting of fifteen fully self-developed, cost-effective “Tier-I stations” and 35 commercial “Tier-II stations” (LoRAIN, Pessl Instruments GmbH), aims to fill these gaps and to provide a modular, user-friendly WSN with a high spatial density and temporal resolution for research, practical applications and the general public. The Tier-I stations were designed and optimised from the ground up, including the printed circuit board (PCB), for temporally high-resolution WSNs that support wide ranges of sensors and that is expandable. The core of the system is a low-power embedded computer (Raspberry Pi Zero) running a custom multithreaded generic logging and remote control software that locally stores the data and transmits it to a custom vapor-based TCP server via GSM. The software also features system monitoring and error detection functions, as well as remote logging. The setup can easily be expanded on the fly by adding predefined sensors to a configuration file. For better modularity, each station registers itself on the server and will be automatically integrated in all further processes and vice versa. Custom frontends as well as bidirectional communication and task distribution protocols enable remote access and across node interaction, resulting in a more easy-to-maintain system. 

In addition to air temperature, humidity and precipitation measured by the Tier II stations, the Tier-I station feature a ClimaVUE 50 all-in-one weather sensor and a BlackGlobe (Campbell Scientific, Inc.) that provides data on wind, radiation, pressure, lightning, solar radiation and black globe temperatures. That allows for calculation of thermal comfort indices in real-time. A webpage and the self-developed “uniWeather” (iOS-App, API) offers near-realtime data access and data interpretation for stakeholders and public outreach.

How to cite: Feigel, G., Plein, M., Zeeman, M., Briegel, F., and Christen, A.: A compact and customisable street-level sensor system for real-time weather monitoring and outreach in Freiburg, Germany, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15609, https://doi.org/10.5194/egusphere-egu23-15609, 2023.

EGU23-16779 | Orals | GI1.3 | Highlight

An integrated meteorological forecasting system for emergency response 

Alexander Haefele, Maxime Hervo, Philipp Bättig, Daniel Leuenberger, Claire Merker, Daniel Regenass, Pirmin Kaufmann, and Marco Arpagaus

EMER-Met is the new meteorological forecasting system for the protection of the population in Switzerland. It provides the meteorological basis for coping with all types of emergencies, especially in case of nuclear and chemical accidents. EMER-Met consists of a dedicated upper air measurement network and a high-resolution numerical weather prediction model. The measurement network is composed of state-of-the-art remote sensing instruments to measure accurate wind and temperature profiles in the boundary layer. At three sites, a radar wind profiler PCL1300, a Doppler lidar Windcube-200s and a microwave radiometer Hatpro-G5 are installed. The data from the measurement network are assimilated into the operational 1-km ensemble numerical weather prediction (NWP) system. In the case of the microwave radiometers, we assimilate the brightness temperatures using an adapted version of the RTTOV observation operator. To ensure best impact on the NWP results, the data quality of the measurements is of high importance and is monitored closely on a daily and monthly basis against radiosondes and the NWP model itself. EMER-Met is operational since 2022 and to our best knowledge, it is the first time that the brightness temperatures measured by surface-based microwave radiometers are assimilated operationally. This presentation will focus on the upper air network performance and its impact on NWP. 

How to cite: Haefele, A., Hervo, M., Bättig, P., Leuenberger, D., Merker, C., Regenass, D., Kaufmann, P., and Arpagaus, M.: An integrated meteorological forecasting system for emergency response, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16779, https://doi.org/10.5194/egusphere-egu23-16779, 2023.

EGU23-17535 | ECS | Orals | GI1.3

ACTRIS - CiGas side-by-side interlaboratory comparison of new and classical techniques for formaldehyde measurement in the nmol/mol range 

Therese Salameh, Emmanuel Tison, Evdokia Stratigou, Sébastien Dusanter, Vincent Gaudion, Marina Jamar, Ralf Tillmann, Franz Rohrer, Benjamin Winter, Teresa Verea, Amalia Muñoz, Fanny Bachelier, Véronique Daele, and Audrey Grandjean

Formaldehyde is an important hazardous air pollutant, classified as carcinogenic to humans by the International Agency for Research on Cancer (IARC). It is emitted directly by many anthropogenic and natural sources, and formed as a secondary product from volatile organic compounds (VOCs) photo-oxidation. Formaldehyde is, as well, a significant source of radicals in the atmosphere resulting in ozone and secondary organic aerosols formation. Routine measurements of formaldehyde in regulatory networks within Europe (EMEP) and USA (EPA Compendium Method TO 11A) rely on sampling with DNPH (2,4-Dinitrophenylhydrazine)- impregnated silica cartridges, followed by analysis with HPLC (High-performance liquid chromatography).

In the framework of the EURAMET-EMPIR project « MetClimVOC » (Metrology for climate relevant volatile organic compounds: http://www.metclimvoc.eu/), the European ACTRIS (Aerosol, Cloud and Trace Gases Research InfraStructure: https://www.actris.eu/) Topical Centre for Reactive Trace Gases in-situ Measurements (CiGas), IMT Nord Europe unit – France, organized a side-by-side intercomparison campaign in Douai-France, dedicated to formaldehyde measurement in a low amount fraction range of 2 - 20 nmol/mol, from 30 May to 8 June 2022. The objectives of the intercomparison are to evaluate the instruments metrological performance under the same challenging conditions, and to build best practices and instrumental knowledge.

Here, we present the results from the intercomparison, where ten instruments belonging to seven different techniques were challenged with the same formaldehyde gas mixture generated either from a cylinder or from a permeation system, in different conditions (amount fractions, relative humidity, interference, blanks, etc.), flowing through a high-flow (up to 50 L/min) Silcosteel-coated manifold. The advantages/drawbacks of the techniques will be discussed.

How to cite: Salameh, T., Tison, E., Stratigou, E., Dusanter, S., Gaudion, V., Jamar, M., Tillmann, R., Rohrer, F., Winter, B., Verea, T., Muñoz, A., Bachelier, F., Daele, V., and Grandjean, A.: ACTRIS - CiGas side-by-side interlaboratory comparison of new and classical techniques for formaldehyde measurement in the nmol/mol range, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17535, https://doi.org/10.5194/egusphere-egu23-17535, 2023.

EGU23-943 | Orals | AS5.17

Five-year PM Chemical Composition and Organic Aerosol (OA) Sources in a European Megacity, London 

Gang Chen, Max Priestman, Anna Font, Anja Tremper, and David Green

Improving air quality in urban areas is essential since 97% of European cities exceed the annual PM2.5 value of the WHO guidelines (10 μg/m3). Therefore, in order to mitigate adverse health outcomes of air pollutants, it is extremely important to understand the long-term chemical compositions and organic aerosol (OA) sources in the largest European city, London. North Kensington (50.52° N, 0.21° W) is an urban background monitoring station located in a residential area of west London. A Quadrupole Aerosol Chemical Speciation Monitors, Q-ACSM (Aerodyne Research Inc., MA, USA), was deployed to continuously monitor submicron non-refractory particulate matter (NR-PM1) from March 2013 until May 2018. The knowledge of OA sources is crucial not only because OA is the main constituent of particulate matter (PM), but also because different sources of OA are known to have different toxicities. Positive matrix factorization (PMF) on the OA matrix of ACSM data remains the most common technique to conduct source apportionment (SA) analyses. By following the standardized protocol developed by Chen et al. (2022), we have retrieved high-quality SA results in these 5 years using the most advanced SA techniques (i.e., rolling PMF (Parworth et al., 2015), the ME-2 solver (Paatero, 1999), and bootstrap resampling (Erfon, 1979)). Additionally, back trajectory analysis has helped identify the geographical origin of OA sources. A variety of auxiliary measurements have been conducted on the same site, which has been used to validate our SA results. Overall, this study provided a rare opportunity to investigate the long-term trends of PM composition and OA sources in a European megacity and provided valuable information for policymakers to understand the effects of mitigation strategies and design more efficient policies.

How to cite: Chen, G., Priestman, M., Font, A., Tremper, A., and Green, D.: Five-year PM Chemical Composition and Organic Aerosol (OA) Sources in a European Megacity, London, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-943, https://doi.org/10.5194/egusphere-egu23-943, 2023.

EGU23-944 | Orals | AS5.17

Source apportionment analysis at an urban background site, a roadside site, and the resulting roadside increment in London, UK 

Anja H. Tremper, William A. Hicks, Max Priestman, Gang Chen, Manousos-Ioannis Manousakas, Andre S. H. Prevot, and David Green

Traffic remains a key source of PM2.5 and PM10 in urban environments and contributes to PM in the form of exhaust related particles and non-exhaust related particles (Grigoratos and Martini, 2014). It is expected that due to traffic fleet changes and stricter exhaust emissions controls the relative contribution of non-exhaust traffic related particles, such as brake and tyre wear, but also of other urban sources, such as wood smoke and cooking aerosols, will become more significant. To understand these changes in relative contribution, sources need to be identified and quantified in different urban environments. High time resolution measurements of PM composition, such as those from the Xact instrument allow for a more accurate identification and quantification of sources as the high time resolution reflects short term changes due to emission and atmospheric processing. Here we present a comparison of positive matrix factorisation (PMF) analysis at an urban background site, a roadside site, and of the resulting roadside increment. This work aims to improve the identification of non-exhaust traffic emissions.

Hourly PM10 measurements of a range of elements were made with the Xact at an urban background and a roadside location in London between Aug. 2019 and Aug. 2020. Source contributions were determined with PMF using the Source Finder software (SoFi) (Canonaco et al., 2013). PMF is carried out in steps: i) initial factor profiles are established for the roadside and background location; ii) factor profiles of the roadside increment are established; iii) the roadside increment profiles are used to improve the factor identification at the roadside and background and results evaluated in comparison with the initial profiles. Black carbon, PM10, PM2.5 mass concentrations and NOx were used to verify PMF results.

PMF analysis was initially performed on roadside increment data. The profiles identified were then used to improve the combined PMF for both sites. In this novel approach, the advantages of utilizing the roadside increment are explored to investigate the identification of factors which can be used to quantify traffic impact more accurately at roadside and background locations.

This work was supported by the Natural Environment Research Council (NERC) under grant NE/T001909/2.

References

Canonaco et al, (2013). AMT 6, 3649-2013

  • Grigoratos and G. Martini, 2014; Non-exhaust traffic-related emissions - Brake and tyre wear PM. Report no. Report EUR 26648 EN

How to cite: Tremper, A. H., Hicks, W. A., Priestman, M., Chen, G., Manousakas, M.-I., Prevot, A. S. H., and Green, D.: Source apportionment analysis at an urban background site, a roadside site, and the resulting roadside increment in London, UK, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-944, https://doi.org/10.5194/egusphere-egu23-944, 2023.

EGU23-1011 | ECS | Orals | AS5.17

Monitoring and apportioning sources of outdoor and indoor air quality using low-cost particulate matter sensors. 

Dimitrios Bousiotis, Leah-Nani Alconcel, Roy M. Harrison, Davis C. S. Beddows, and Francis Pope

Air quality is the leading environmental factor for public health globally. Source apportionment of air pollution is a key aspect of understand and ameliorating air quality problems. However, its use has been rather limited primarily due to the high cost that comes with instrument deployment. The emergence of low-cost sensors provides a new tool for assessing air quality and assigning sources within outdoor and indoor environments.

We have developed low-cost source apportionment techniques that can be used with single and multiple point measurements in outdoor environments. We have demonstrated its applicability for understanding sources at urban background sites, as well as assessing the pollution footprint of several industrial activities. The application of our methodology greatly improved our understanding of major pollution sources, by pinpointing and quantifying their effect in the surrounding area, at only a fraction of the cost of regulatory approaches. The information of the effect of any polluting activity, as well as the conditions that enhance or reduce it, is crucial information for the remediation of air quality problems.

Continuing our successful work on apportioning pollution in outdoor environments, we now focus on the indoor environment. Indoor environments can be particularly important because of the duration of time spent within them, and hence the potential for high exposure. These environments can be highly heterogenous, with different sources and concentrations varying from room to room.  In our latest study, four low-cost sensors were deployed both inside and outside a typical family house close to Birmingham, UK. While the average PM concentrations in all rooms were within the latest World Health Organisation (WHO) guidelines, great variation was found on the PM concentrations among the rooms. Using the source apportionment methods the effect of the indoor and outdoor sources of particles was quantified. Up to 95% of the PM1 was found to be from outdoor sources in all the rooms. This effect was reduced as particle size increased, though the outdoor sources were still contributing more than 65% of the PM2.5 and up to 50% of the PM10, depending on the room studied. These measurements allowed for the estimation of the average exposure of a work-at-home day. The implications on increased working from home will be discussed with respect to total exposure.

 

This study reveals new insights into the how different indoor and outdoor sources combine within households to contribute to total air pollution exposures.  It highlights that total exposure is a function of the geographic situation of the household, the physical infrastructure of the household including filtration and appliances. This methodology will also be tested and used within the RI-URBANS pilot project to assess the air quality of the area surrounding the University of Birmingham. The presentation will finish with a roadmap on how low cost source apportionment can help to improve indoor and outdoor air quality.

How to cite: Bousiotis, D., Alconcel, L.-N., Harrison, R. M., Beddows, D. C. S., and Pope, F.: Monitoring and apportioning sources of outdoor and indoor air quality using low-cost particulate matter sensors., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1011, https://doi.org/10.5194/egusphere-egu23-1011, 2023.

EGU23-3202 | ECS | Orals | AS5.17

Modelling the dispersion of particle number concentrations in the West Midlands, UK 

Jian Zhong and Roy Harrison

Ultrafine particles (UFPs with a diameter less than 100 nm) are tiny and respirable particles. Because of their small sizes, UFPs can penetrate cells and tissue, accumulate in lungs, and cause health effects. Although UFPs are currently not regulated in the same way as mass concentrations for large particles such as PM2.5 and PM10, the 2021 WHO global air quality guidelines have highlighted the pressing issue of UFPs with a good practice statement. Particle number concentrations (PNC) are the most common measure for UFPs with tiny mass. UFPs often dominate the total ambient PNC in urban environments. There is a strong need to quantify the PNC in the ambient air through measurements and modelling. This study simulates the dispersion of particle number concentrations in the West Midlands (WM), UK using the local scale ADMS-Urban model, which is an advanced quasi-Gaussian plume dispersion modelling system. ADMS-Urban implements a physics-based approach to represent the characteristics of the atmospheric boundary layer. It can represent a variety of source types (such as road and grid emissions) occurring in urban environments and requires a range of input data. Grid sources of PNC for SNAP (Selected Nomenclature for Air Pollution) sectors across the WM were obtained from TNO. Road sources were derived based on the local traffic activity maps (from Transport for West Midlands and Birmingham City Council) and PNC emission factors available in the literature. Meteorological data for Birmingham Airport was used to drive the dispersion. Particle number was used as a passive scalar, with no inclusion of aerosol microphysics. Background data from the rural Chilbolton air quality site was downloaded from Defra UK-Air website. Advanced canyon and urban canopy parameters were derived based on the building data and road network shapefiles using ArcGIS tools. The model was run on the University of Birmingham’s BlueBEAR HPC. Model evaluation was conducted by comparing the modelled (from a receptor run) and measured data at the Birmingham Air Quality Supersite. Overall, the model performed well. Based on the modelling output from a contour run, street scale resolution maps for annual PNC were generated, which could be linked to local population and health data for potential epidemiological studies.        

How to cite: Zhong, J. and Harrison, R.: Modelling the dispersion of particle number concentrations in the West Midlands, UK, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3202, https://doi.org/10.5194/egusphere-egu23-3202, 2023.

EGU23-3833 | Posters virtual | AS5.17

High time resolution PM 10 chemical composition of urban city influenced by industry and North-African dust outbreaks in SW Europe 

Jesus de la Rosa, Ana M Sánchez de la Campa, and Daniel A Sánchez-Rodas

In this work, we present the results of high time resolution PM10 chemical composition using online XRF spectrometer (Xact 625i) in the city of Huelva (SW of Spain) in September 2021-september 2022. The sampling was performed at the Campus monitoring station, which is belonging to Air Quality Network of the junta de Andalucía in the western part of the city of Huelva. Since 1970, Population is submitted to the hourly impact of industrial plumes related to Cu-metallurgy, phosphate production and petrochemical complex.

A total of 30 elements were analyzed in an hourly resolution. Moreover, other on-line pollutants were analyzed (N, BC, SO2, NO2, O3 and PM10). To compare the results obtained by Xact 625i to conventional chemical procedures using ICP-MS, ICPOES, IC and TOT, daily chemical composition of PM10 was characterized every 4 days during one year of sampling.

The results have shown how the impact of the industry occurs in the city of Huelva around 20% of the days every year. Days with poor air quality are influenced by the simultaneous impact of industry and North African air masses.

Nucleation of PM is synchronous with elements related to industrial activity (SO2, As, Cu, Bi, Se, Pb, Ni, Zn and P). Another source of nucleation is traffic (BC, NO2, Sn and Sb ). The highest concentrations of mineral dust are related to north African outbreak air masses Two elements (Si +Al) may contribute more than the daily limit value for this pollutant (50 µg m-3).

How to cite: de la Rosa, J., Sánchez de la Campa, A. M., and Sánchez-Rodas, D. A.: High time resolution PM 10 chemical composition of urban city influenced by industry and North-African dust outbreaks in SW Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-3833, https://doi.org/10.5194/egusphere-egu23-3833, 2023.

EGU23-5280 | ECS | Posters on site | AS5.17

Variability and vertical structure of gaseous air quality indicators above urban areas: IAGOS in-situ profiling of nitrogen oxides, ozone, and carbon monoxide 

Christoph Mahnke, Ulrich Bundke, Norbert Houben, Torben Blomel, Philippe Nédélec, Valérie Thouret, Hannah Clark, and Andreas Petzold

Nitrogen oxides (NOX), ozone (O3), and carbon monoxide (CO) are important air quality indicators which have anthropogenic and natural sources at ground (e.g.: transport emissions, industry, agriculture, biomass burning) and within the troposphere (e.g.: lighting, aircraft emissions). Furthermore, their concentrations in the atmosphere are strongly affected by photochemistry. The European Research Infrastructure IAGOS (www.iagos.org) is using in-service passenger aircraft as observation platforms, equipped with instrumentation for measuring gaseous species, aerosols, and cloud particles. IAGOS monitors the vertical profiles of climate and air quality relevant trace gases like CO, O3, NO, NO2 and NOX near airports of highly populated urban areas (e.g.: Frankfurt (Main) and Paris) during take-off and landing. These profiles provide essential information about the chemical composition of the lower troposphere, which is not available from surface-based stations or remote sensing instrumentation.

Here, we characterize the variability and the vertical structure of these trace gases in the background atmosphere in the lower free troposphere that interacts with the urban boundary layer. In addition, layers of enhanced pollution level can be detected that were advected from distant source regions and have the potential to affect the urban air quality at the receptor site due to downmixing. This data provides valuable information that is complementary to the surface-based air quality network stations, facilitating the link to high-resolution models and satellite observations, where IAGOS can provide information about e.g., the vertical profile of the NO to NO2 ratio. The latter being difficult to retrieve from remote sensing measurements.

Acknowledgments: This work is part of the RI-URBANS project and has received funding from the European Union’s Horizon 2020 research and innovation program under grant agreement No 101036245. We thank all airlines contributing to IAGOS, in particular Deutsche Lufthansa and Lufthansa Technik for enabling the observations. The German Federal Ministry of Education and Research (BMBF) is acknowledged for financing the instruments operation and data analysis as part of the joint project IAGOS-D under grant 01LK1301A.

How to cite: Mahnke, C., Bundke, U., Houben, N., Blomel, T., Nédélec, P., Thouret, V., Clark, H., and Petzold, A.: Variability and vertical structure of gaseous air quality indicators above urban areas: IAGOS in-situ profiling of nitrogen oxides, ozone, and carbon monoxide, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5280, https://doi.org/10.5194/egusphere-egu23-5280, 2023.

EGU23-5896 | ECS | Orals | AS5.17

Oxidative potential modelling of PM10 : an indicator of aerosol health risk studied in France with the CHIMERE model 

Matthieu Vida, Gilles Foret, Guillaume Siour, Samuel Weber, Olivier Favez, Jean-Luc Jaffrezo, Gaelle Uzu, and Matthias Beekmann

Air pollution remains an outstanding issue due to its hazardous health and environmental impacts. For France, the number of premature deaths is estimated around 40,000 people per year mostly due to particulate matter (PM), while associated economical coast is estimated at 100 billion euros per year. In this context, action plans are implemented in order to reduce the PM mass concentrations in ambient air. However, considering mass concentration only can lead to an obvious bias: for instance, at equal mass concentrations, the exposure to fresh sea salts is assumed to have the same toxicity as soot particles containing toxic compounds. Therefore, accurate abatment measures need thorough knowledge on the PM chemical composition, which can then be used within receptor and/or chemical transport models to apportion their emission sources and secondary formation processes. The PM chemistry is also relevant in terms of adverse health effects. Based on the PM chemical species ability to generate oxidative stress through reactive oxygen species, the oxidative potential (OP) indicates the consumption of antioxidant per particles mass. This proxy estimates the imbalance between oxidants and antioxidants, responsible for inflammatory processes and chronic diseases. As a result, the aerosol’s oxidative potential has emerged as a promising indicator of PM adverse health impacts.

To better evaluate PM health effects, we set-up a strategy to implement OP in the state-of-art air quality model CHIMERE and to simulate particles OP over the whole French territory for the year 2013 and 2014. To do so, a measurement derived and source specific OP determined by Positive Matrix Factorization (PMF) receptor modelling approach is combined with particle sources apportionment in CHIMERE using a tagging method called Particulate Source Apportionment Technology (PSAT). Alternatively, a source specific OP is obtained by linear regression of observed OP and simulated sources. Both methods are used to simulate OP over France for the years 2013 and 2014, and to determine the most affected areas and responsible sources.

How to cite: Vida, M., Foret, G., Siour, G., Weber, S., Favez, O., Jaffrezo, J.-L., Uzu, G., and Beekmann, M.: Oxidative potential modelling of PM10 : an indicator of aerosol health risk studied in France with the CHIMERE model, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5896, https://doi.org/10.5194/egusphere-egu23-5896, 2023.

EGU23-5899 | ECS | Orals | AS5.17

Personal exposure to UFP from bicycling measurements in Birmingham, UK 

Seny Damayanti, Roy M. Harrison, and Francis Pope

Cycling activity has benefits for both health and the environment. However, there are also health risks for cyclists due to their direct exposure to air pollutants from on-road vehicle emissions. Higher breathing rates and the proximity to the emission sources while cycling could also increase the health risk for the cyclist. Airborne particle exposure, particularly ultrafine particles (UFP, Dp smaller than 100nm) has been considered to have a detrimental effect on human health. The assessment of exposure to UFP is essential for UFP management, which is also included in a Good Practice Statement by WHO.

In this study, we estimated the personal exposure to UFP using mobile measurements (bicycling) between 17 October and 18 November 2022, in Birmingham, UK. The measurements were conducted at three (3) different times (morning, afternoon, and evening) on weekdays and weekends. A miniature particle counter (DiscMini) that measures particle number concentration (PNC), and average diameter with 1s resolution was used. Besides, a similar instrument was also deployed at an urban background site which was passed during the bicycling measurements.

A total of 34 trips (~1.5 hours, and ~12km per trip) were completed. Overall, the result revealed that the exposure to PNC varied substantially both spatially and temporally. Relatively higher PNC exposure was found during the morning (MWD) and evening (EWD) trips on weekdays, while the lowest was during morning weekend (MWE) trips. The mean concentration of MWD, EWD, and MWE was 16664#/cm3, 15255 #/cm3, and 4004#/cm3, respectively. A moderate level was observed during the afternoon on weekdays and weekend (AWD, AWE), and evening weekend (EWE) ranging from 8321-9676 #/cm3.

During weekend trips, the average geometric mean diameter was observed to be larger (43-52.3 nm), suggesting a greater relative background contribution during the weekend, especially in the morning. All the average PNC from bicycling measurements were 2.3-2.6x higher than that measured at the background site due to more emission sources being present along the route. However, PNC and average diameter measured at the background site revealed similar behaviour to the mobile measurement with high concentrations during morning and evening on  weekdays.

Spatial analysis indicated some hotspots that were at intersections and traffic lights. A construction area and shopping park area also exhibited high concentrations, especially during afternoon and evening weekend trips. These results may be of value in support of strategies to mitigate UFP personal exposure, particularly for cyclists who commute daily in this area and on similar routes elsewhere.

How to cite: Damayanti, S., Harrison, R. M., and Pope, F.: Personal exposure to UFP from bicycling measurements in Birmingham, UK, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5899, https://doi.org/10.5194/egusphere-egu23-5899, 2023.

EGU23-5970 | Orals | AS5.17 | Highlight

Ultrafine Particles and Black Carbon in Two Roadside Sites in Europe: Long-term Data Analysis 

Roy M. Harrison, Seny Damayanti, Francis Pope, and Jarkko V. Niemi

Road vehicles are typically the main source of ultrafine particles (UFP, Dp <100nm) in urban areas. A high spatio-temporal variation of UFP is found even in similar types of sites e.g roadside. We analyzed long-term particle datasets (number count or PNC, and number size distribution or NSD), and Black Carbon (BC) from two roadside sites in Europe, London Marylebone Road (LMR) in the UK, and Mäkelänkatu Street in Finland (Mäk). We evaluated 11 years (2010-2021) and 5 years (2015-2020) of particle data derived from SMPS (16.55-604.3nm) and DMPS (6-798.42nm) for LMR and Mäk, respectively.

The initial analysis shows that at LMR, PNC reduced by 64% over 2010-2021 (~20000#/cm3 to less than 10000#/cm3), while the BC declined by 86% (~9 µg/m3 to 1.2 µg/m3). Meanwhile, PNC at Mäk remained constant at ~15000#/cm3 during 2015-2018, then decreased to ~10000#/cm3 in 2020. BC decreased by 58% (1.3 to 0.6 µg/m3) during 2015-2020.

Using the same size range (16.5–604nm) from both sites during 2015-2019, the TNC at LMR were 1.4-1.6 times higher than that at Mäk, and 2.4-3.9 higher for BC. Particles less than 16.39 nm at Mäk account for approximately 50% of TNC over the full measured size range. When particles are classified into nucleation, Aitken and accumulation ranges, the nucleation mode contributes most at Mäk (68% of the full size range), while the Aitken mode is dominant at LMR (51%).

A downward trend was observed during 2015-2019 at both sites. However, the pollutant concentration reduced faster at LMR, apart from the Nucleation mode which slightly increased. BC showed the fastest decline (9.6%/yr and 14.2%/yr in Mäk and LMR, respectively). Further investigation using wind direction data shows that in LMR, the most significant reduction of pollutants mainly occurred from the southerly wind sector, which is associated with the emissions from road vehicles on the adjacent road, suggesting that interventions applied to the road vehicle fleet have effectively decreased pollutants concentration. In Mäk, pollutant concentrations decreased much faster on winds from the NW and SE sectors, corresponding to the alignment of the road. The Nucleation mode proportion has increased since 2014 from the southern and westerly sectors at LMR, and NW and west at the Mäk due to the rapid reduction of the Aitken or Accumulation mode, rather than an increase of Nucleation mode concentration, which has changed little.

The annual mean PNSD shows a bimodal pattern at both sites. A change was observed from a minor peak at ~60-70nm that gradually disappeared over the period seen more clearly at LMR.

We interpret the rapid reduction in BC and PNC as being largely attributable to the progressive uptake of diesel particle filters as Euro 5 and 6 standard vehicles have entered the fleet since 2011.  However, the greatest impact has been upon the BC and Aitken and Accumulation mode particles, with little change seen in the Nucleation mode particles, which are comprised largely of condensed lubricating oil, and form in the cooling exhaust after passage through the particle filter (Harrison et al., 2015).

How to cite: Harrison, R. M., Damayanti, S., Pope, F., and Niemi, J. V.: Ultrafine Particles and Black Carbon in Two Roadside Sites in Europe: Long-term Data Analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5970, https://doi.org/10.5194/egusphere-egu23-5970, 2023.

EGU23-6361 | Orals | AS5.17

Near real-time source apportionment of carbonaceous aerosols in 13 sites across Europe 

Hilkka Timonen and Jean-Eudes Petit and the RI-URBAN NRT-SA pilot sites

Source apportionment by receptor modeling is used to determine the contributions of different emission sources to ambient levels of bulk Particulate Matter (PM), Black Carbon (BC), the Oxidative Potential (OP), among others. Source apportionment can be based e.g. on statistical approaches such as PMF (Positive Matrix Factorization), CMB (Chemical Mass Balance) or different properties such as absorption of particles originating from different sources (Aethalometer model). Often source apportionment analysis is time consuming and based on subjective decisions of an experienced user. 

As a part of RI-URBANs project an automated Near real-time source apportionment (NRT-SA) of carbonaceous aerosols is piloted on 13 sites across Europe during 2023. In all cities real-time measurements of aerosol chemical composition are conducted with the Aerosol Chemical Speciation monitor (ACSM: organics, sulphate, ammonium, nitrate and chloride) and Aethalometer (AE33: Black carbon (BC) and Brown carbon (BrC)). The measurement sites include two traffic, nine urban, one regional and one background site. NRT-SA based on PMF (Gang et al., 2022) will be used to separate the different primary (e.g. traffic, cooking, biomass combustion, coffee roastery, coal combustion) and secondary sources of organics from the ACSM data and aethalometer model (Sandradewi et al., 2008) to separate the BClf (from liquid fuel combustion) and BrCwb (from solid fuel combustion).  Prior information about the sources of organics like number of factors and reference mass spectra of primary sources from previously conducted source apportionment studies (Chen et al., 2022) in pilot cities have been utilized. The results of the NRT-SA have been validated by comparison to the offline calculated source apportionment results. Based on these extensive measurements, the chemical composition and origins of the fine aerosol fraction will further be discussed regarding the different environments of the investigated pilot sites throughout the European continent.

The measurements and NRT-SA are conducted as a part of RI-URBANS’ project (Grant #101036245) , that aims to demonstrate how service tools from atmospheric research infrastructures can be adapted and enhanced in air quality monitoring networks in an interoperable and sustainable way.

 

Chen, G., Canonaco, F., Slowik, J. G., Daellenbach, K. R., Tobler, A., Petit, J.-E., Favez, O., Stavroulas, I., Mihalopoulos, N., Gerasopoulos, E., El Haddad, I., Baltensperger, U., and Prévôt, A. S. H.: Real-Time Source Apportionment of Organic Aerosols in Three European Cities, Environ. Sci. Technol., https://doi.org/10.1021/acs.est.2c02509, 2022.

Sandradewi, J., Prévôt, A. S. H., Szidat, S., Perron, N., Alfarra, M. R., Lanz, V. A., Weingartner, E., and Baltensperger, U.: Using Aerosol Light Absorption Measurements for the Quantitative Determination of Wood Burning and Traffic Emission Contributions to Particulate Matter, Environ. Sci. Technol., 42, 3316–3323, https://doi.org/10.1021/es702253m, 2008.

How to cite: Timonen, H. and Petit, J.-E. and the RI-URBAN NRT-SA pilot sites: Near real-time source apportionment of carbonaceous aerosols in 13 sites across Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6361, https://doi.org/10.5194/egusphere-egu23-6361, 2023.

EGU23-6503 | Posters on site | AS5.17

Modeling terrestrial water balance using regionalization of hydrological model parameters at Kalli watershed, Estonia. 

Steffen M. Noe and Emílio Graciliano Ferreira Mercuri

Terrestrial water storage and evapotranspiration (ET) have strong dependence on vegetation type at the catchment scale, and they also play an important role in the forest management and carbon exchange. Regionalization methods dependent on rainfall-runoff models comprise techniques for transferring calibrated parameters in instrumented basins (donor basins) to non-instrumented basins (target basins). In this study, regionalization was used to transfer of parameters from the GR4J-Cemaneige model calibrated in Reola hydrographic basin to predict daily flows in Kalli basin, both watersheds located in the south-east of Estonia. The basins are covered with hemi-boreal forests and we used the hypothesis that both basins have physiographic and climate similarity, besides being close to each other. ET historical data was collected from the Station for Measuring Ecosystem-Atmosphere Relations (SMEAR Estonia), located in Järvselja forest in Kalli basin. Precipitation data was collected from Tartu-Tõravere and SMEAR stations, and the river flow from Reola hydrometric station. The time series period adopted for model calibration was 2015-2018 and the 2019 year was used for validation. Point precipitation measurements are generally used to calculate average precipitations at the watershed scale. However, several studies point out that the use of rain gauges can generate errors in undermeasurement of precipitation, both for snow (solid precipitation) and rain (liquid precipitation), mainly due to the effect of wind. Water Balance Method (WBM) was used to correct the precipitation from Reola Watershead and then GR4J-Cemaneige model was calibrated at Reola Basin, with Nash-Sutcliffe Efficiency index of 0.77. The precipitation series from SMEAR at Kalli watershed was corrected to consider the solid precipitation, using data from Tartu-Tõravere station. For modeling the Kalli watershed streamflow an iterative process was created and it consists of: i) run the hydrological model and obtain the streamflow, ii) apply the WBM correction on the precipitation data, iii) repeat step (i) until the correction factor stabilizes to a fixed value. This methodology allowed to obtain the terrestrial water storage daily variation from the beginning of 2015 to the end of 2019 with high reliability, since the watershed is treated as a system. The results indicate that the terrestrial water storage is positive in winter and negative in the summer period, reaching absolute maximum values of 200 mm.  This research allows a better understanding of the Järvselja hemi-boreal forest water dynamics and its variation through the seasons, especially in the context of climate change. Next steps are to analyze the relations between carbon, energy and water balance at stand and catchment scales.

How to cite: Noe, S. M. and Ferreira Mercuri, E. G.: Modeling terrestrial water balance using regionalization of hydrological model parameters at Kalli watershed, Estonia., EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6503, https://doi.org/10.5194/egusphere-egu23-6503, 2023.

EGU23-7178 | Posters on site | AS5.17

Trends of atmospheric composition over Eurasia and their response on global climate changes 

Vadim Rakitin, Andrey Skorokhod, Yury Shtabkin, Natalia Kirillova, and Eugenia Fedorova

Based on the analysis of orbital measurements, as well as GEOS-Chem model calculations, a study of trends in the total content of CO, CH4 and NO2 in different periods and seasons of 2003-2022 was made for the Eurasia domain, -20°E - 180°E, 0°N - 80°N. Data from the AIRS and OMI instruments were used as orbital information.

Before calculating the trend distributions, we compared the trend estimates obtained from orbital and ground-based measurements using only synchronous observations, i.e., days when the measurements were carried out by both orbital (AIRS, OMI) and ground-based (IAP RAS and NDACC stations) instruments.

A good agreement has been established between trend distributions obtained from the orbital data and the same distributions obtained from the GEOS-Chem model calculations.

In general, according to average annual estimates, trends over most of Eurasia regions in the period 2003-2022 was negative; however, after 2008 the downward trend slowed down, and in some areas the CO content began to rise.

Thus, a positive trend (change) in CO TC trends after about 2008 was established. In the entire domain under study, this change was about 2–2.5%/year. In the autumn months of 2008-2022 (including November) increase in CO TC was established over almost the entire Eurasia, including Arctic regions and Europe. This growth (at least in Europe) cannot be explained by either anthropogenic emissions or releases from fires. A possible reason for this rising may be the formation of additional CO from methane, the increase in concentrations of which began around the same time (after 2007), and change in the source/sink ratio for CO.

Based on GEOS-Chem calculations with different scenarios for specifying anthropogenic emissions and emissions from fires, the response of CO trends to climate change was calculated. The study was supported by Russian Science Foundation under grant №21-17-00210.

How to cite: Rakitin, V., Skorokhod, A., Shtabkin, Y., Kirillova, N., and Fedorova, E.: Trends of atmospheric composition over Eurasia and their response on global climate changes, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7178, https://doi.org/10.5194/egusphere-egu23-7178, 2023.

EGU23-7266 | Posters on site | AS5.17

Air-water gas transfer coefficient for shallow water 

Irina Repina

Fluxes of GH gases across the water surface constitute an important part of the global climate. Because of the combination of small concentrations and  small fluxes, the determination of air–water gas fluxes presents unusual measurement difficulties. Direct measurements (i.e., eddy correlation) of the fluxes are rarely attempted.  Used in gas transport parameterization models were mainly developed for the open ocean. The differences, especially those between shallow sheltered systems and the open waters best fit by some published relationships, are ecologically important and do not appear yet to be measurable by other methods.

The report discusses the determination of the transfer coefficient from direct measurements of methane and carbon dioxide fluxes in the case of shallow water bodies. Coastal zones, an estuary, a small lake and a river of differing bathymetry and local terrain are considered. The influence of footprint, surface condition, and atmospheric stability is investigated. In the case of a river, the current may also have an influence. It is shown that the inhomogeneous relief significantly affects the results of the convergence of measurements and model calculations. Determined that the model overestimates the fluxes in low winds. For CH₄, most of the transport appears to be by ebullition rather than diffusion and model would have underestimated the exchange by two orders of magnitude. New dependencies are proposed for determining the gas transfer coefficient for methane and carbon dioxide under conditions of shallow water and inhomogeneous relief. The work was supported by the Russian Science Foundation grant 22-47-04408.

How to cite: Repina, I.: Air-water gas transfer coefficient for shallow water, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7266, https://doi.org/10.5194/egusphere-egu23-7266, 2023.

EGU23-7684 | Orals | AS5.17

Mobile Air Quality monitoring with daily commuters in Rotterdam 

Martine Van Poppel, Jelle Hofman, Jan Peters, Gerard Hoek, Jules Kerckhoffs, Saskia Willers, and Emre Özdemir

Air pollution is the fourth cause of premature mortality (HEI, 2020) and in Europe, more than 0.3 million premature deaths are due to air pollution (EEA, 2021). In urban environments, people are exposed to a complex mixture of air pollutants with a large spatial variability. However, highly spatially resolved measurement data on air pollutants is lacking. These fine-grained data is needed to correctly assess personal exposure to air pollution for epidemiolocal studies and to support air quality management scenarios.

Within RI-URBANS different innovative approaches to get insights into novel air quality parameters, source contributions, exposure to air pollution and associated health effects will be developed and tested. One of the approaches relies on mobile measurements with citizens to derive spatial air pollution maps. Mobile measurements can contribute to understand spatial variability of short-living constituents of air pollution from a diversity of pollution sources.

The monitoring campaign is performed with volunteers, who are all employees of DCMR or the city of Rotterdam. They are asked to measure during their daily bicycle commutes. Before the measurement campaign, a training session was organized for the volunteers. Measurements were performed in winter (November 2022 – February 2023) and will be repeated in spring 2023.

Measurements are based on the airQmap approach; more information on the approach and previous studies can be found on https://www.airQmap.com. Measurements of Black Carbon (BC) are performed using a microaethalometer (microAeth®, AE51, AethLabs) and a GPS.  BC is measured at 1s temporal resolution and a flow rate of 150 mL min-1. To reduce the noise in BC measurements, the ONA (Optimized Noise-reduction Averaging, Hagler et al., 2011) algorithm was used with an attenuation threshold of 0.05. The geo-tagged measurements were aggregated (trimmed mean) and attributed to fixed points 20 m apart from each other along the cycling route.

The dataset will be used to test different data processing techniques (a.o. temporal aggregation, background correction approaches) to construct representative BC maps.  The collected spatiotemporal BC measurements will be analysed to identify main sources of BC in the area. The pilot study will result in guidance on best practices for mobile air quality monitoring involving citizens.

This paper will present the results of the winter campaign.

____________________

EEA, 2021. HI of Air Pollution in EU

Hagler, G.S., Yelverton, T.L., Vedantham, R., Hansen, A.D., Turner, J.R., 2011. Postprocessing method to reduce noise while preserving high time resolution in Aethalometer real-time black carbon data. Aerosol Air Qual. Res. 11, 539-546.

HEI, 2020. State of Global Air

How to cite: Van Poppel, M., Hofman, J., Peters, J., Hoek, G., Kerckhoffs, J., Willers, S., and Özdemir, E.: Mobile Air Quality monitoring with daily commuters in Rotterdam, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7684, https://doi.org/10.5194/egusphere-egu23-7684, 2023.

EGU23-8931 | ECS | Posters virtual | AS5.17

The Italian Automated Lidar Ceilometer Network ALICENET: retrievals and applications in support to  urban air quality monitoring 

Annachiara Bellini, Henri Diémoz, Luca Di Liberto, Gian Paolo Gobbi, and Francesca Barnaba

ALICENET is the Italian network of Automated Lidar-Ceilometers (ALCs) coordinated by CNR-ISAC, operationally running (24/7) several systems across the country, including main urban areas. Particulate matter and atmospheric dynamics monitoring through profiling remote sensing techniques is explored within the H2020 RI-URBANS project (WP1) and, in this framework, ALC-based products will be made available to the scientific and stakeholder communities. These include, among others, aerosol extinction and mass concentration profiles, directly usable by the research community as well as by environmental, meteorological, health and aviation safety agencies.

In this work, the ALICENET data processing is applied and showcased for three RI-URBANS pilot sites: Milan, Rome (Italy) and Paris (France). These are characterized by different aerosol and atmospheric conditions: Milan is strongly influenced by high anthropic emissions and transport dynamics within the Po Basin, Rome is an example of urban conditions in the Mediterranean area, and Paris is representative of aerosol conditions affected by both local and continental sources. The ALC-retrieved aerosol quantities are compared with both advanced in-situ/remote sensing observations and modeled fields  to identify potential upscaling issues of the data inversion procedure.

The work will focus  on the added value of the aerosol profile products for air quality monitoring in urban sites.

How to cite: Bellini, A., Diémoz, H., Di Liberto, L., Gobbi, G. P., and Barnaba, F.: The Italian Automated Lidar Ceilometer Network ALICENET: retrievals and applications in support to  urban air quality monitoring, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8931, https://doi.org/10.5194/egusphere-egu23-8931, 2023.

EGU23-9843 | Orals | AS5.17

Toward Climate Smart and Sustainable cities: Integrated Urban System Methodology and Key Performance Indicators 

Alexander Baklanov and the WMO IUS and U4SSC Expert Teams

Accelerating growth of urban populations has become a driving force of human development, especially in developing countries. Crowded cities are centres of creativity and economic progress; however, extreme weather conditions, flooding, water quality, air pollution and other hazards create substantial vulnerability and challenges in the urban environment.

The third United Nations Conference on Housing and Sustainable Urban Development (HABITAT III) in October 2016 adopted the New Urban Agenda (United Nations, 2017), which brings into focus urban resilience, climate and environment sustainability, and disaster risk management. Following the event at the United Nations Economic and Social Council, efforts are required from WMO to consolidate its input to the revision of the New Urban Agenda (NUA) and support urban related activities in a comprehensive manner. Urban development is now a cornerstone of the United Nations 2030 Sustainable Development Goals. It has its own sustainable development goal (SDG 11): Make cities inclusive, safe, resilient and sustainable.

To support implementation of urban activities the WMO inter-programme Urban Expert Team under the Commission for Atmospheric Sciences and Commission for Basic Systems (2018) supported by a dedicated team of urban focal points in the Secretariat developed the Guidance on Integrated Urban Hydro-Meteorological, Climate and Environmental Services (IUS). The needs for integrated urban services (IUS) include information for short-term preparedness (e.g. hazard response and early warning systems), longer-term planning (e.g. adaptation and mitigation to climate change) and support for day-to-day operations (e.g. water resources). The aim is to build urban systems and services that meet the special needs of cities through a combination of dense observation networks, high-resolution forecasts, multi-hazard early warning systems, disaster management plans and climate services. This approach gives cities the tools they need to reduce emissions, build thriving and resilient communities and implement the UN Sustainable Development Goals.

WMO with its urban cross-cutting approach is involved in joint UN urban activities for development of and implementation of NUA and SDG 11 with a number of external partners, e.g. UN-Habitat, WHO, ITU, GEO, International Association for Urban Climate (IAUC), etc. The IUS methodology is integrated into more broad Multi-Agency UN system U4SSC: United for Smart Sustainable Cities and its key performance indicators (KPIs) for smart sustainable cities.

This presentation provides an overview of the current efforts towards future IUSs on urbanization under climate change undertaken by the WMO and UN international initiatives for building climate smart, sustainable and resilient cities.

How to cite: Baklanov, A. and the WMO IUS and U4SSC Expert Teams: Toward Climate Smart and Sustainable cities: Integrated Urban System Methodology and Key Performance Indicators, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9843, https://doi.org/10.5194/egusphere-egu23-9843, 2023.

The meteorological observation data of the early period (1840-1950) in China were  manually corrected the input and clerical errors, and then according to the length or coverage of time, the main series was determined. The observation time system of unknown sites is determined by the difference method introduced. After these operations, the data of all sites are unified into the same format. Then, through the ridge regressions established by data from modern reference stations, the missing maximum temperature (T-max) and minimum temperature (T-min) are interpolated, and then combined with modern data to form the heterogeneous extreme temperature data set of 1840-2020 in China. RHtest software was used to adjust the homogenate problem in  data set. Finally, the century-long homogenized daily temperature data set including 45 key city stations in China was obtained. There are 20 stations with observation record more than one hundred year. The length of temperature observation series of 17 stations is between 80 and 100 years. The series length of the remaining 7 sites is between 68 and 80 years. The data integrity of 5 stations is 50 - 60%, 9 stations is 60 - 70%, 8 stations is 70 - 75%, 5 stations is 75 - 80% and 18 stations is 85 - 100%. Finally, the angular distance weighting (ADW) method is used to interpolate the dataset into grid products, and the grid accuracy is 2.5 ° * 2.5 °. Climatic research unit dataset (CRU data set) was compared to verify the new dataset. The correlation between the four longest sequences in the newly developed data set  and the corresponding sites in the CRU data set is very good, and the correlation coefficient is very high, and the correlation between the remaining sites of the two data sets is also very good so the quality of CUG dataset is still trustworthy.

How to cite: zheng, X.: Development of the century-long homogenized daily temperature data set in China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-10313, https://doi.org/10.5194/egusphere-egu23-10313, 2023.

EGU23-11497 | Posters virtual | AS5.17

Methane Emission from lakes on continuous and isolate permafrost in Russia 

Irina Fedorova, Anna Shornikova, Ekaterina Chulkova, and Irina Arestova

Greenhouse gases emission from lakes is quite significant environment question in the cryosphere. Up to know the volume of storage and reason that influence on it are underestimated. If GHG emission for the Arctic landscapes and boreal wetlands are measuring on seldom stations, data from permafrost border is insufficient.

There are continuous and isolated permafrost with many lakes in Russia. Emission from the surface of thermokarst and periglacial lakes were measured in Yamal peninsula and Tunkinskaya valley (the Russian Arctic and Baikal region) in summer 2022. Both regions have natural and anthropogenic changed aquatic ecosystems. Several geochemical, ecological and hydrodynamical features of lakes were consider as well.

CH4 emission from thermokarst lake near Salekhard city was 237 mgCH4·m-2·day-1 in site of volume for thermokarst lake Shorshonka in Tunkinskaya valley was more than 2000 mgCH4·m-2·day-1 (the air temperature was equal). Eutrophic lake near Tunkinskiye Goltsy Mountain Ridge gave 1020 mgCH4·m-2·day-1 in summer period. Methane concentration in lake sediments was 2.1-8.3 µg/l for lakes in southern Yamal and reached 13.6 µg/l in Baikal region. Biogenic elements concentration in all lakes as usual was in the limit. Isotope content was also a little bit strange for Shorshonka lake (4.67 δ18O, ‰). Other lakes near Salekhard city and Baikal lake had amplitude 11-16 δ18O, ‰.   

Therefor we can tell about strong differences for methane emission from thermokarst lakes in continuous and isolated permafrost that flux should be studied more detail.   

How to cite: Fedorova, I., Shornikova, A., Chulkova, E., and Arestova, I.: Methane Emission from lakes on continuous and isolate permafrost in Russia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11497, https://doi.org/10.5194/egusphere-egu23-11497, 2023.

EGU23-12039 | Posters virtual | AS5.17

An analysis of daily ice coverage changes for the Yenisei River from 2002 to 2021 

Yubao Qiu, Yixiao Zhang, Yang Li, Matti Leppäranta, Wenshan Liang, Zhengxin Jiang, and Bin Cheng

Since the beginning of the 20th century, the surface air temperature in the Arctic has increased more than three times faster than the global average. River ice is an important component of the terrestrial cryosphere, which is very sensitive to air temperature. The Yenisei River originates from the Sayan Mountains in Mongolia and is the largest watersheds drained by Arctic Ocean, which covers latitudes from 46°N to 73°N. The changes of river ice for Yenisei River provides reflect the response of great rivers in the high latitudes of the Northern Hemisphere to climate change. In this study, the daily river ice coverage in the Yenisei River was firstly estimated with a grid of resolution at , derived from the Moderated Resolution Imaging Spectroradiometer (MODIS) daily observations for the period 2002-2021. The classical Normalized-Difference Snow Index (NDSI) algorithm was employed to extract the ice cover; a cloud removal and filtering method were used to reduce errors caused by cloud contamination and the polar night influence. The validation with dependence to the Landsat data showed that an overall accuracy was achieved by 86%. By applying the Theil–Sen nonparametric statistical slope method and the Mann–Kendall test to the results, it was found that the river ice coverage shows a decreasing trend. Over the past 20-year period, 82.8% of the Yenisei River Basin experienced a decreasing ice coverage, of which 21.9% is significant at the 0.05 level of significance. A correlation analysis indicated that the winter river ice coverage is driven by the mean winter air temperature () and that the ice coverage shows a strong latitude dependence (). River ice coverage is highly sensitive to the air temperature in the south part of the Yenisei basin, where the latitudes are low and the altitudes are high. It was also found that, during the winter, the accumulated negative temperature correlates with river ice coverage similarly with the average temperature (). In Lake Baikal, the largest freshwater lake in the Yenisei basin, apart from air temperature the distribution characteristics of ice coverage was most probably affected by heat inflows from streams, dynamics and water depth.

How to cite: Qiu, Y., Zhang, Y., Li, Y., Leppäranta, M., Liang, W., Jiang, Z., and Cheng, B.: An analysis of daily ice coverage changes for the Yenisei River from 2002 to 2021, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-12039, https://doi.org/10.5194/egusphere-egu23-12039, 2023.

EGU23-13154 | Orals | AS5.17

Urban atmosphere dynamics for air quality applications: Atmospheric boundary layer height and wind profiles from ground-based remote sensing networks 

Simone Kotthaus, Martial Haeffelin, Jonnathan Céspedes, Melania Van Hove, Marc-Antoine Drouin, Jean-Charles Dupont, and Gilles Foret

Atmospheric boundary layer (ABL) dynamics severely impact the horizontal transport of pollutants as well as their vertical dilution. Despite this, observations of vertical wind profiles and the ABL height are still rare, particularly in cities. Thanks to recent technological advances compact ground-based remote sensing instruments are now available to monitor the heterogeneous urban atmosphere across dense sensor networks. In urban settings, Doppler wind lidars (DWL) and automatic lidars and ceilometers (ALC) are particularly useful as they operate continuously and automatically with very low maintenance under all weather conditions. Thanks to those novel profiling instruments, high-resolution (time and vertical) wind information as well as aerosol backscatter profiles can be recorded.

Based on the RI-URBANS (and ICOS-cities) pilot city of Paris, France, we demonstrate what advanced products can be derived using different detailed algorithms, including vertical profiles of horizontal wind and turbulence, boundary layer heights based on aerosol or turbulence indicators, as well as low-level jet characteristics. In Paris, RI-URBANS is embedded in the PANAME initiative that coordinates the synergy between numerous projects that are investigating the urban atmosphere. Clear measurement standards, careful quality control and advanced processing algorithms are required to ensure harmonised products are obtained from the diverse sensor networks that involve instruments of different models from various manufacturers with respective capabilities and limitations.

Using the synergy of the different ABL products obtained in the Paris region, it is investigated how the urban boundary layer interacts with the synoptic scale flow, the underlying topography and the urban surface. A combination of wind direction, atmospheric stability and terrain clearly affect shallow boundary layer heights and the low-level jet characteristics. But also spatial variations across the region are registered during deep convective boundary layer development.

How to cite: Kotthaus, S., Haeffelin, M., Céspedes, J., Van Hove, M., Drouin, M.-A., Dupont, J.-C., and Foret, G.: Urban atmosphere dynamics for air quality applications: Atmospheric boundary layer height and wind profiles from ground-based remote sensing networks, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13154, https://doi.org/10.5194/egusphere-egu23-13154, 2023.

EGU23-13319 | ECS | Orals | AS5.17

Towards a better understanding of fine PM sources: online and offline datasets combination in a single PMF 

Marta Via, Jesús Yus-Díez, Francesco Canonaco, Jean-Eudes Petit, Philip Hopke, Cristina Reche, Marco Pandolfi, Matic Ivančič, Martin Rigler, Xavier Querol, Andrés Alastuey, and María Cruz Minguillón

Source apportionment (SA) techniques allow matching the measured ambient pollutants with their potential source origin. Hence, they are a powerful tool for assessing air pollution mitigation strategies. The Positive Matrix factorization (PMF) model is one of the most widely used SA approaches, and its multi-time resolution add-on (MTR-PMF), which enables mixing different instrument data in their original time resolution, is the focus of this study.

Co-located one-year measurements of non-refractory submicronic particulate matter (NR-PM1), black carbon (BC) and metals, obtained respectively, by a Q-ACSM (Aerodyne Research Inc.), an Aethalometer (Aerosol d.o.o.) and offline fine PM samples collected on quartz-fibre filters, were combined in a single PMF in two different resolutions (30 minutes for the NR-PM1 and BC, and 24h every 4 days for the offline samples). The multi-time resolution PMF (MTR-PMF) was run varying both the time resolution (averaging the dataset) and the uncertainty weightings of both datasets in order to assess the impact of these variations on the model output. The resolution assessment revealed that averaging the high-resolution data was disadvantageous in terms of model residuals and environmental feasibility. Regarding uncertainty weightings, overweighting the uncertainties of the 24-h dataset dividing them by two provided the most optimal scaled residuals adjustment.

The MTR-PMF was run with the optimised time resolution and uncertainty weightings retrieving eight PM1 sources: ammonium sulphate (AS) + heavy oil combustion (24%), ammonium nitrate (AN) and ammonium chloride (15%), fresh SOA (15%), traffic (14%), biomass burning (11%), aged SOA + mineral dust (8%), urban mix (7%) and cooking-like organic aerosol + industry (6%). The MTR-PMF technique allowed the identification of two more sources respect a dataset containing the same species at a 24h time resolution (base case) and four more respect to the conventional offline and PMF, proving that the combination of both high and low time resolution data through MTR-PMF is significantly beneficial for SA. This is especially true for those sources which have been disentangled with respect to the conventional and base case PMFs.

 

How to cite: Via, M., Yus-Díez, J., Canonaco, F., Petit, J.-E., Hopke, P., Reche, C., Pandolfi, M., Ivančič, M., Rigler, M., Querol, X., Alastuey, A., and Minguillón, M. C.: Towards a better understanding of fine PM sources: online and offline datasets combination in a single PMF, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13319, https://doi.org/10.5194/egusphere-egu23-13319, 2023.

EGU23-15235 | ECS | Orals | AS5.17

Source apportionment of ultrafine particle size distributions in urban Europe 

Meritxell Garcia Marlès, Andrés Alastuey, Xavier Querol, and Philip K. Hopke

Ultrafine particles (UFP, particles sized <100 nm)  significantly impact health and the environment. However, their study is still a challenge, and a specific regulation is required. The measurement of UFP-PSD (Ultrafine Particles – Particle Size Distribution) and its application in air quality assessment is a significant goal of RI-URBANS. 2017-2019 hourly UFP-PSD data from 26 sites in urban Europe and one site in the US have been compiled and evaluated according to the instrumental and methodological approaches implemented; the comparison of urban concentrations across Europe; the identification of similarities and major differences; and the evaluation of relationships with other pollutants, such as BC, PMx and gaseous pollutants (SO2, NOx, O3, CO), and with meteorological parameters. The results of this study have recently been published by Trechera et al. (2023).

To continue the study by Trechera et al. (2023) in UFP, source apportionment for the previous 27 urban sites is being analyzed with an extended period from 2009 to 2019. This study aims to identify and quantify sources contributing to UFP-PSD using Positive Matrix Factorization (PMF), comparing the differences between the sites. PMF is a widely used multivariate factor analysis tool to identify the source types that may be contributing to the sample using measured source profile information. According to a recent review on UFP source apportionment based on UFP-PSD measurements by Hopke et al. (2022), the typically reported sources of UFP include nucleation, several traffic sources (fresh to aged), domestic and residential heating, regional secondary inorganic aerosols (i.e., regional nitrate and sulfate), particles associated with oxidants as represented by O3 (i.e., regional secondary organic and inorganic aerosols) and other sources (such as biomass burning, urban background sources, industrial emissions, diverse sources, dust and unknown sources). In the near future we expect to publish the results of source apportionment for the datasets mentioned above.

 

 

 

 

 

 

Cassee F., Morawska L., Peters A. (Eds)., 2019. The White Paper on Ambient Ultrafine Particles: evidence for policy makers. ‘Thinking outside the box’ Team, October 2019, 23 pp, https://efca.net/files/WHITE%20PAPER-UFP%20evidence%20for%20policy%20makers%20(25%20OCT).pdf

Hopke, P.K., Feng, Y., Dai, Q., 2022. Source apportionment of particle number concentrations: A global review. Sci. Total Environ. 819, 153104. https://doi.org/10.1016/j.scitotenv.2022.153104

Paatero, P., and U. Tapper, 1994. Positive matrix factorization: A non-negative factor model with optimal utilization of error estimates of data values., Environmetrics, 5, 111–126, doi:10.1002/env.3170050203

Rivas, I., Vicens, L., Basagaña, X., Tobías, A., Katsouyanni, K., Walton, H., Hüglin, C., Alastuey, A., Kulmala, M., Harrison, R.M., Pekkanen, J., Querol, X., Sunyer, J., Kelly, F.J., 2021. Associations between sources of particle number and mortality in four European cities. Environ. Int. 155. https://doi.org/10.1016/j.envint.2021.106662

Trechera, P., Garcia-Marlès, M., Liu, X., et al., 2023. Phenomenology of ultrafine particle concentrations and size distribution across urban Europe. Environ. Int. Accepted (Publication in progress).

How to cite: Garcia Marlès, M., Alastuey, A., Querol, X., and Hopke, P. K.: Source apportionment of ultrafine particle size distributions in urban Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15235, https://doi.org/10.5194/egusphere-egu23-15235, 2023.

EGU23-15713 | Posters on site | AS5.17

Quantification of Secondary Sulfate emissions in Europe and Central Asia 

Stergios Vratolis and Konstantinos Eleftheriadis

The scope of this work is to quantify the emission rate of Secondary Sulfate across a wide region in the Northern hemisphere, mainly in Europe and Western Asia. The data employed are deducted by Positive Matrix Factorization (PMF) on a PM2.5 chemical composition dataset from 16 European and Asian cities for the period 2014 to 2016. The spatial resolution of the method corresponds to the geographic grid cell size of the Lagrangian particle dispersion model (FLEXPART) which was utilized for the air mass backward simulations. The area covered is also related to the location of the 16 cities under study.

Species with an aerodynamic geometric mean diameter of 400 nm and geometric standard deviation of 1.6 were used to model the Secondary Sulfate aerosol transport. Generalized Tikhonov regularization was applied so as to acquire potential source areas and quantify their emission rate. The results acquired by this process indicate a significant source area for Secondary Sulfate on the East of the Caspian Sea. The maximum emission rate in that area is as high as 10 g m-2 s-1. Significant source areas also include South Poland and the Balkans. The results display many similarities to the SO2 emission map provided by ECLIPSE database.

 

Acknowledgements

This research has been funded by the program “RER/1/015 - Apportioning air pollution sources on a regional scale”, 2016 - 2017.

 

References

Vratolis, S., Diapouli, E., Manousakas, M. I., Almeida, S. M., Beslic, I., Kertesz, Z., Samek, L., and Eleftheriadis, K.: A new method for the quantification of ambient particulate matter emissions, Atmos. Chem. Phys. Discuss. [preprint], https://doi.org/10.5194/acp-2022-843, in review, 2023.

How to cite: Vratolis, S. and Eleftheriadis, K.: Quantification of Secondary Sulfate emissions in Europe and Central Asia, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15713, https://doi.org/10.5194/egusphere-egu23-15713, 2023.

EGU23-16079 | ECS | Orals | AS5.17

Phenomenology of ultrafine particle concentrations and size distribution across urban Europe 

Pedro Trechera, Meritxell Garcia-Marlès, Andrés Alaustey, and Xavier Querol and the RI-URBANS collaborators

In spite of the important advances in the science of aerosols and air quality, important scientific and environmental challenges remain unsolved, especially those related to source apportionment of the specific components of atmospheric particulate matter (PM), atmospheric processes influencing aerosols, and the associated climate and health impacts. Moreover, ultrafine particle (UFP) studies are growing, they are still insufficient and much needed. Furthermore, there is a clear lack of information and guidance on UFP measurement, especially in smaller ranges. In addition, it is widely recognised that exposure to PM negatively impacts human health (WHO, 2021). In 2016, ambient air pollution accounted for almost seven million premature deaths per year (WHO, 2016), as derived from the aggravation of cardiovascular and respiratory diseases and cancers. Several studies have also shown that UFP can deeply penetrate the respiratory system, thus causing respiratory and cardiovascular diseases in humans (Cassee et al., 2019).

The 2017-2019 hourly particle number size distributions (PNSD) from 26 sites in Europe and 1 in the US were evaluated focusing on 16 urban background (UB) and 6 traffic (TR) sites in the framework of RI-URBANS project. The main objective was to describe the phenomenology of urban ultrafine particles in Europe with a significant air quality focus. The varying lower size detection limits made it difficult to compare PN concentrations (PNC), particularly PN10-25, from different cities. PNCs follow a TR>UB>Suburban (SUB) order. PNC and Black Carbon (BC) progressively increase from Northern Europe to Southern Europe and from Western to Eastern Europe. At the UB sites, typical traffic rush hour PNC peaks are evident, many also showing midday-morning PNC peaks anti-correlated with BC. These peaks result from increased PN10-25, suggesting significant PNC contributions from nucleation, fumigation and shipping.

Site types to be identified by daily and seasonal PNC and BC patterns are: (i) PNC mainly driven by traffic emissions, with marked correlations with BC on different time scales; (ii) marked midday/morning PNC peaks and a seasonal anti-correlation with PNC/BC; (iii) both traffic peaks and midday peaks without marked seasonal patterns. Groups (ii) and (iii) included cities with high insolation. PNC, especially PN25-800, was positively correlated with BC, NO2, CO and PM for several sites. The variable correlation of PNSD with different urban pollutants demonstrates that these do not reflect the variability of UFP in urban environments. Specific monitoring of PNSD is needed if nanoparticles and their associated health impacts are to be assessed. Implementation of the CEN-ACTRIS recommendations for PNSD measurements would provide comparable measurements, and measurements of <10 nm PNC are needed for full evaluation of the health effects of this size fraction.

WHO, 2021. Ambient (outdoor) air pollution. 22 September 2021, https://www.who.int/news-room/fact-sheets/detail/ambient-(outdoor)-air-quality-and-health

WHO, 2016. Ambient air pollution: a global assessment of exposure and burden of disease. World Health Organization., 121 pp, https://apps.who.int/iris/handle/10665/250141

Cassee F., Morawska L., Peters A. (Eds)., 2019. The White Paper on Ambient Ultrafine Particles: evidence for policy makers. ‘Thinking outside the box’ Team, October 2019, 23 pp, https://efca.net/files/WHITE%20PAPER-UFP%20evidence%20for%20policy%20makers%20(25%20OCT).pdf

How to cite: Trechera, P., Garcia-Marlès, M., Alaustey, A., and Querol, X. and the RI-URBANS collaborators: Phenomenology of ultrafine particle concentrations and size distribution across urban Europe, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16079, https://doi.org/10.5194/egusphere-egu23-16079, 2023.

EGU23-16601 | Posters virtual | AS5.17

Sensors, Mobile Monitoring & Citizen Involvement: Complementary Tools for More Accurate Air Quality Exposure Assessments 

Jelle Hofman, Martine Van Poppel, Gerard Hoek, Mar Viana, Jan Theunis, Jan Peters, Jules Kerckhoffs, Teresa Moreno, Ioar Rivas, Xavier Basagaña, Vanessa Nogueira dos Santos, Roy Harrison, Dimitrios Bousiotis, David Green, Tuukka Petäja, Martha Zaidan, Naser Hossein Motlagh, and Aikaterini Bougiatioti

Traditional fixed air quality monitoring networks fulfill requirements as set in the European Air Quality Directive (2008/50/EC) and provide valuable information on ambient concentrations and temporal trends of air quality at the international, national, regional and urban level. Some short-lived pollutants or constituents, like ultrafine particle (UFPs), black carbon (BC) and nitrogen oxides (NOx), exhibit a high spatial (street-level) variability, requiring a higher monitoring resolution for more accurate exposure assessments in health or epidemiological studies. Advances in sensing and Internet of Things (IoT) technologies have resulted in smaller and more affordable stationary and mobile monitoring solutions, enabling data collection at unprecedented  scales. Moreover, citizens can contribute in data collection resulting in more wide-scale data collection, dissemination and resulting impact. The collected data, however, needs adequate processing and validation in order to obtain representative exposure maps (i.e., long-term averaged concentration maps) for epidemiological studies and policy assessment.

RI-URBANS aims to develop and test innovative and complementary air quality monitoring approaches in different European pilot cities. This methodological work focusses on the potential of mobile and stationary sensor applications as complementary tools for traditional (low-density) monitoring networks (Figure 1). Complementary measurements can contribute to understand spatial variability of short-lived constituents of air pollution from a diversity of pollution sources.

Figure 1: Mobile and fixed sensor applications, resulting data resolution and associated requirements in terms of device (devices) and monitoring strategy (setup).

We identify different data users and use cases for mobile, stationary (or combined) sensor applications and their resulting implications regarding device specifications, monitoring strategy and data processing needs. By reflecting on past studies and projects, we summarize common methodological approaches and best practices to increase the spatial resolution of air quality data. Moreover, the role of citizen engagement is evaluated, both in generating more data and air quality impact (awareness raising).

This work serves as methodological input for the RI-URBANS service tools that will be tested in the pilot cities and is openly available at https://riurbans.eu/wp-content/uploads/2022/10/RI-URBANS_D13_D2.5.pdf 

How to cite: Hofman, J., Van Poppel, M., Hoek, G., Viana, M., Theunis, J., Peters, J., Kerckhoffs, J., Moreno, T., Rivas, I., Basagaña, X., Nogueira dos Santos, V., Harrison, R., Bousiotis, D., Green, D., Petäja, T., Zaidan, M., Hossein Motlagh, N., and Bougiatioti, A.: Sensors, Mobile Monitoring & Citizen Involvement: Complementary Tools for More Accurate Air Quality Exposure Assessments, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16601, https://doi.org/10.5194/egusphere-egu23-16601, 2023.

EGU23-16835 | Posters virtual | AS5.17

Overview of RI-URBANS project - an update 

Tuukka Petäjä, Xavier Querol, Paolo Laj, and Eija Juurola and the RI-URBANS team

In the urban areas, regional and local air quality monitoring networks (AQMN) provide the concentrations of regulated air quality parameters. However, there is a rising concern of aerosol particle number concentrations, lung deposited surface area and black carbon (BC) as novel health indicators that connect closely to the well-being of the citizens. The capacities of the AQMNs need to be improved to be able to respond to the need of novel air quality data.

Aerosols, Clouds and TRace gases Research InfraStructure (ACTRIS) provides harmonized high-quality data on the variability of aerosols, aerosol precursors and their complex interactions through remote-sensing and in-situ measurement techniques. More specifically, ACTRIS has observations on surface aerosol levels, including nanoparticle-size distribution, PM size distributions, nanoparticles, online (aerosol mass spectrometers, MS and aerosol chemical speciation monitors ACSM) and offline (filter-based chemistry) chemical composition, BC, Volatile Organic Compounds as precursors of PM, nanoparticles and O3, radiative properties of aerosols, and 4D (3- dimensions and online in time) atmospheric measurements. 

There is a need to connect the ACTRIS expertise and that of the air quality monitoring networks. This provides the starting point of Research Infrastructures Services Reinforcing Air Quality Monitoring Capacities in European Urban & Industrial AreaS (RI-URBANS), a European Commission funded project in the Horizon 2020 Call H2020-LC-GD-2020 (Building a low-carbon, climate resilient future: Research and innovation in support of the European Green Deal).

The challenge of RI-URBANS is therefore to develop innovative urban AQ service tools, in clear complementarity with the AQMNs, and provide innovative tools to better quantify the impact of atmospheric species most deleterious to human health. Under the complex and changing AQ situation of urban pollution as described above, obtaining monitoring data on PM composition, source contributions to PM, nanoparticles, and gaseous precursors, as well as spatially resolved exposure maps of urban pollutants, will contribute to enhanced AQ policy assessment and evaluation of health effects in Europe. For such assessment both urban scale modelling (for nanoparticles, and other pollutants such as exhaust and non-exhaust vehicles PM emissions, and BC) and regional ones (for SOA and Secondary Inorganic Aerosols (SIA) and for the background levels of all the other pollutants) are also needed. RI-URBANS is based on the premise that advanced monitoring and modelling tools developed by RIs and science teams can be used to supplement current AQMNs of regulated pollutants.

On one hand, the overarching objective of RI-URBANS is to demonstrate how Service Tools (STs from atmospheric Research Infrastructures (RIs) can be adapted and enhanced in a RIs-AQ Monitoring Networks (AQMNs) interoperable and sustainable way to better address the challenges and societal needs related to AQ in European cities (and industrial, harbour, airport and traffic hotspots) as areas with especially significant levels of air pollution and associated health effects. On the other hand, ACTRIS has then the opportunity provide harmonized pan-European observation capacity of urban air quality and therefore to contribute to the well-being of the population.

In this work we will summarize the key developments of the RI-URBANS project acquired during the first year of the project.

How to cite: Petäjä, T., Querol, X., Laj, P., and Juurola, E. and the RI-URBANS team: Overview of RI-URBANS project - an update, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-16835, https://doi.org/10.5194/egusphere-egu23-16835, 2023.

EGU23-17305 | Posters virtual | AS5.17

Enviro-HIRLAM Seamless Modelling: Research, Development, Application 

Alexander Mahura, Roman Nuterman, Alexander Baklanov, Mykhailo Savenets, Larysa Pysarenko, Svitlana Krakowska, Igor Ezau, Behzad Heibati, Benjamin Foreback, Michael Boy, Risto Makkonen, Hanna K. Lappalainen, Tuukka Petäjä, and Markku Kulmala

The Enviro-HIRLAM (Environment - HIgh Resolution Limited Area Model) is seamless/ online integrated numerical weather prediction and atmospheric chemical transport modelling system. It is capable of simultaneous simulation of meteorology – atmospheric composition and downscaling/nesting for regional–subregional–urban scales. The research and development are focused on: multi-scale modelling up to fine resolution; improving parameterizations describing urban processes, boundary/surface layer structures; implementation of emissions, aerosol/chemistry mechanisms, aerosol feedback and interactions. The Enviro-components includes: gas-phase chemistry; aerosol microphysics and deposition processes; urban sublayer physics parameterisations; direct/indirect/combined aerosol feedbacks due to radiation; locally  mass-conserving  semi-Lagrangian  numerical  advection  scheme; natural and anthropogenic emission inventories. The model has modules for pre-processing of the ECMWF’s initial/ boundary conditions for meteorology-chemistry-aerosols, observations for data assimilation, and selected emission inventories. The model has been developed through HPC projects such as Enviro-HIRLAM at CSC and Enviro-PEEX(Plus) at ECMWF, as well as other research projects.

The research and development of Enviro-HILRAM and its application will be demonstrated on examples, where this model is used as a research tool  for studies in domain of the Pan-Eurasian Experiment (PEEX; https://www.atm.helsinki.fi/peex) programme. The examples include: Integrated modelling for assessment of potential pollution regional atmospheric transport as result of accidental wildfires; Integrated modelling and analysis of influence of land cover changes on regional weather conditions/ patterns; High-resolution integrated urban environmental modelling with integration of the urban large-eddy simulation (PALM model) and meteorological simulations into a seamless modelling chain; Effects of spring air pollution and weather on Covid-19 infection/situation in Finland; Meteorology integration between seamless and trajectory (FLEXPART model) models; and others. The Enviro-HIRLAM model generated output provides valuable input (3D meteorology and atmospheric composition) to assessment studies, and it as can be integrated into GIS environment for further risk/ vulnerability/ consequences/ etc. estimation, and other studies.

How to cite: Mahura, A., Nuterman, R., Baklanov, A., Savenets, M., Pysarenko, L., Krakowska, S., Ezau, I., Heibati, B., Foreback, B., Boy, M., Makkonen, R., Lappalainen, H. K., Petäjä, T., and Kulmala, M.: Enviro-HIRLAM Seamless Modelling: Research, Development, Application, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17305, https://doi.org/10.5194/egusphere-egu23-17305, 2023.

EGU23-17327 | Posters virtual | AS5.17

Prospects for development of a climate service system in Ukraine 

Sergiy Stepanenko, Oleh Shablii, and Inna Khomenko

Adaptation to climate change and mitigation of its consequences is one of the goals of sustainable development. Therefore, one of the main priorities of national hydrometeorological services is elaboration of climate service systems at the national level. The global framework for climate services established in 2009 provided a powerful impulse for development of such services in many countries including Ukraine.

It is for establishment of the national climate services in Ukraine that the Erasmus+ ClimEd (Multilevel Local, Nation- and Regionwide Education and Training in Climate Services, Climate Change Adaptation and Mitigation; http://climed.network) project was initiated and supported by the European Union. One of the ClimEd main objectives is to determine a competence base for development of climate educational courses on climate with the content that meets the expectations and requirements of both the national and international legislation and the needs of climate-dependent sectors of Ukrainian economy.

To determine the requirements of various sectors of the economy for climate information as well as to comprehend the nature and extent of its use in their daily and planned activities, 297 respondents were interviewed. The surveys covered 7 sectors of the economy such as healthcare, urban management, water management, energy, agriculture, civil engineering and architecture, nature conservation. Several international transdisciplinary discussion panels, the international scientific and practical conference “Climate Services: Science and Education” and the 2nd All-Ukrainian Hydrometeorological Congress were held. These allowed to adapt the surveys’ results to national and international standards in the field of the climate education. To learn and follow the best European Universities educational practices, three trainings were held (see details at http://climed.network/events/climed-trainings). Moreover, 48 representatives of the Hydrometeorological Service of Ukraine were also interviewed as well as meetings with discussions were held with the heads of Ukrainian regional hydrometeorological centers. This allowed to assess the needs for modernisation the Ukrainian National Meteorological Service. In principle, all these obtained results can be updated annually and used for future continuous modernisation of the climate related educational system and for its effective response to demands of the modern labour market.

Although the ClimEd project has been temporarily suspended (Feb 2022 - Aug 2023), development of educational and teaching materials will be resumed starting autumn 2023. Such materials are crucially important for: continual and comprehensive professional training of specialists in the field of climate services, inter- and transdisciplinary training of specialists in climate-dependent sectors of the economy, and decision-makers in the field of climate change and climate adaptation.

How to cite: Stepanenko, S., Shablii, O., and Khomenko, I.: Prospects for development of a climate service system in Ukraine, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17327, https://doi.org/10.5194/egusphere-egu23-17327, 2023.

EGU23-17331 | Posters virtual | AS5.17

Climate-related education for the healthcare industry in Ukraine 

Tetiana Shablii, Sergiy Stepanenko, Oleh Shablii, and Inna Khomenko

In the frameworks of the European educational project Erasmus+ ClimEd (Multilevel Local, Nation- and Regionwide Education and Training in Climate Services, Climate Change Adaptation and Mitigation), further climate-related education is provided for professionals in the healthcare industry, as one of the climate-associated industries in Ukraine.

A trans-disciplinary approach in developing distance and blended advanced training courses for medical doctors constitutes knowledge transfer in basics of Climatology and Economics of Climate Change at the pre-course and post-course stages. The main course includes modules on climate-associated pathology in Pulmonology, Cardiology, Neurology, Infectious Diseases and Epidemiology, Obstetrics and Gynecology, and Psychiatry. In view of the climate change an increase in occurrence of floods, wildfires, droughts and other natural disasters alongside extreme weather events is observed thus crucially setting down a requirement for development of a module on emergency primary healthcare.

All the modules are to be developed and taught by high-level professionals, who hold at least a PhD degree. It is under the ClimEd project that blended courses on climate change and climate adaptation are to be designed and delivered for the target audiences of decision-makers in the healthcare industry and the wider public. This will bring in stabilization to the industry-specific aspects of nationwide economy through introduction of the aggregate of all settings, the online, onsite, and hybrid, to be applied in the educational process to ensure maximum efficiency in accordance with the stakeholders’ needs.

How to cite: Shablii, T., Stepanenko, S., Shablii, O., and Khomenko, I.: Climate-related education for the healthcare industry in Ukraine, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17331, https://doi.org/10.5194/egusphere-egu23-17331, 2023.

An improved understanding of the land - atmosphere - ocean feedbacks and interactions is needed for the future strategies for sustainable development of the Arctic region. An understading of the Arctic climate system and  the implementation of the related processes in climate models are required to provide advice for policy actions.  In this presenation, we highlight key areas for Arctic research from the atmospheric, oceanic, cryospheric, and social perspectives, and summarize recent developments in a holistic understanding of the Arctic climate system carried out in in a frame of AASCO Arctic Science Collaboration project in 2020-2022. We also provide an outlook of the links between research and its societal impacts.

How to cite: Lappalainen, H., Petäjä, T., and Baklanov, A.: “ARCTIC SCIENCE COLLABORATIONS” -  A HOLISTIC SYSTEM UNDERSTANDING OF THE ARCTIC ENVIRONMENTAL SYSTEM FOR WELL-TARGETED POLICY ACTIONS- Future perspectives, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-17357, https://doi.org/10.5194/egusphere-egu23-17357, 2023.

EGU23-1619 | ECS | Posters virtual | AS5.18

Evaluation and measurement of tropospheric glyoxal retrieved from MAX-DOAS in Shenzhen, China 

Hairong Zhang, Ang Li, and Zhaokun Hu

We investigated the spatio-temporal variation characteristics of glyoxal through observations over a 23-day period. Sensitivity analysis of simulated and actual observed spectra revealed that the accuracy of glyoxal fitting is primarily controlled by the wavelength range selected. Within the range of 420–459 nm, the value calculated using the simulated spectra was 12.3×1014 molecules/cm2 lower than the actual value, and the results obtained using the actual spectra included a large number of negative values. Overall, the wavelength range has a far stronger influence than other parameters. The wavelength range of 420–459 nm (excluding 442–450 nm) is the most suitable because it ensures minimal influence from interference components in the same wavelength. Within this range, the calculated value of the simulated spectra is the closest to the actual value, with a deviation of only 0.89×1014 molecules/cm2. Therefore, the 420–459 nm range (excluding 442–450 nm) was selected for further observation experiments. The fourth polynomial order was used in DOAS fitting, and constant terms were used to correct the actual spectral offset. In the experiments, the glyoxal slant column density primarily ranged from -4×1015 molecules/cm2 to 8×1015 molecules/cm2, and the near-ground glyoxal concentration ranged from 0.02 to 0.71 ppb. Glyoxal was concentrated below 500 m and the pollution height began to rise around 09:00 and reached the maximum value around 12:00, after which they declined. 

How to cite: Zhang, H., Li, A., and Hu, Z.: Evaluation and measurement of tropospheric glyoxal retrieved from MAX-DOAS in Shenzhen, China, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-1619, https://doi.org/10.5194/egusphere-egu23-1619, 2023.

EGU23-2046 | ECS | Posters on site | AS5.18

DOAS applied to shipping emission monitoring: compliance assessment and comparison to satellite measurements 

Maxime Prignon, Vladimir Conde, Smyth Timothy J., Sundström Anu-Maija, van Vliet Jasper, and Mellqvist Johan

While shipping is generally the most energy-efficient freight transportation mode (in terms of gCO2 t-1 km-1), its intensive use (80 % to 90 % of global merchandise trade volume), coupled with high pollutant emission factors, leads to serious impact on the environment and the human health. The primary pollutants emitted by ships, nitrogen oxides (NOx = NO2 + NO), sulphur oxides (SOx, mainly SO2) and particulate matter (PM), degrade the air quality and are involved in the formation of secondary pollutants as tropospheric ozone (O3). As 70 % of ship emissions occur within 400 km of coastlines, ship emissions have strong impact in harbour cities and coastal areas situated along high traffic shipping lanes.

Compliance monitoring for fuel sulphur content (FSC) is usually done by the collection and the analysis of fuel samples by competent authorities from ships at berth. The complexity of the method results in very few ships being formally controlled. In consequence, various remote compliance monitoring techniques of FSC have been developed in the last years, mainly involving sniffer techniques (extractive methods coupled with analyser instruments) performed from fixed or moving (e.g., manned and unmanned aircrafts, ships) platforms. Optical remote sensing techniques such as differential optical absorption spectroscopy (DOAS) have also been applied to shipping emission monitoring in the past years.

Here we present results of several ship-based campaigns conducted in the last years (in the Mediterranean Sea in 2019 and 2021, and in the English Channel in May 2022), with a focus on the DOAS technique. While the performed DOAS zenith measurements are not fully suitable to conduct a quantitative monitoring of the ship compliance to the FSC regulations, we propose a method to qualitatively identify potential non-compliant ships. Comparisons are made with state-of-the-art sniffer measurements. Despite the larger uncertainty yielded by this technique in comparison to sniffer systems, it may be applied for the guidance of formal controls (e. g., authorities at port).

During the English Channel campaign in May 2022, we modified our DOAS setup in order to sequentially scan various elevation angles from the horizon to the zenith (i.e., multi axis DOAS, MAX-DOAS) and, thus, to retrieve vertical tropospheric columns of NO2. Here we compare our shipborne MAX-DOAS NO2 columns to the ones retrieved from TROPOMI (TROPOspheric Monitoring Instrument). TROPOMI could be further involved in the monitoring of shipping emissions as it has been recently used to identify the emission plumes of single (or group of) ships. Therefore, its validation with independent datasets at sea is needed to strengthen the monitoring of shipping emissions.

How to cite: Prignon, M., Conde, V., Timothy J., S., Anu-Maija, S., Jasper, V. V., and Johan, M.: DOAS applied to shipping emission monitoring: compliance assessment and comparison to satellite measurements, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2046, https://doi.org/10.5194/egusphere-egu23-2046, 2023.

EGU23-2310 | Posters on site | AS5.18

First MAX- DOAS results of the SO292-2 cruise across the Pacific in June/July 2022: Nouméa (New-Caledonia) to Dutch Harbor (Alaska, USA) 

Steffen Ziegler, Bianca Lauster, Steffen Beirle, Sebastian Donner, and Thomas Wagner

Transit cruises of German research vessels across oceans provide a unique platform for MAX-DOAS measurements of atmospheric trace gases such as nitrogen dioxide (NO2), formaldehyde (HCHO) and sulphur dioxide (SO2). The Deep Blue/PORD campaign took place from 24 June to 21 July 2022. During that period the research vessel SONNE was crossing the Pacific in meridional direction from 22° S to 54° N in an area that is typically used as reference for satellite data due to its large distance from anthropogenic emission sources.

In this study we focus on three trace gases: NO2 columns provide information on the meridional distribution of stratospheric NO2 as well as the distribution of tropospheric background NO2 above the marine boundary layer. For the analysis, high signal “peaks” that only last a short time are filtered as they most likely originate from the ship exhaust. First results show a minimum of total NO2 columns between the equator and about 15° N. HCHO and SO2 mainly appear as plumes from nearby islands and/or volcanoes in the Solomon Sea, where biogenic and volcanic activities are naturally high. In combination with the onboard instrumentation (Ceilometer, Pyranometer and a cloud camera) this data set provides a detailed description of the atmosphere along the cruise track.

How to cite: Ziegler, S., Lauster, B., Beirle, S., Donner, S., and Wagner, T.: First MAX- DOAS results of the SO292-2 cruise across the Pacific in June/July 2022: Nouméa (New-Caledonia) to Dutch Harbor (Alaska, USA), EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-2310, https://doi.org/10.5194/egusphere-egu23-2310, 2023.

EGU23-4611 | ECS | Posters on site | AS5.18

A novel hyperspectral remote sensing technique for horizontal distribution of atmospheric gaseous pollutant: to fill the spatio-temporal resolution limitations of satellite and in-situ observations 

Qihua Li, Chuan Lu, Chengzhi Xing, Qihou Hu, Wei Tan, Hua Li, Jinan Li, Zhiguo Zhang, Bowen Chang, and Cheng Liu

High spatial-temporal resolution distribution of atmospheric gaseous pollutant is an important basis for tracing its emission, transport and transformation. At present, methods commonly used to obtain the regional horizontal distribution of trace gas are based on satellite remote sensing or numerous in-situ observation. However, typical trace gas monitoring satellites only have a few fixed overpassing times with a spatial resolution limited to several kilometers, which make it hard to locate minor emission sources. Limited in-situ observations have limited coverage, and can only obtain trace gas concentration information near the observation point. In this study, we propose a method for the long-term detection of the horizontal distribution of trace gas. The spatial resolution in the direction of rotation was up to 0.1°, and the spatial resolution in the optical path direction, reached the kilometer level. Meanwhile, the temporal resolution of the results reached the hourly level during the daytime. The obtained trace gas horizontal distribution was consistent with the in-situ and mobile measurements. Compared with satellite remote sensing, this method achieved horizontal distribution results with higher spatial and temporal resolutions, and located several small high-value areas in Hefei, China. The satellite NO2 vertical column density (VCD) distribution results were evaluated via the NO2 horizontal distribution obtained from the hyperspectral NO2 horizontal distribution at 13:30 (local time) (UTC+8:00) on April 2, 2022. The Tropospheric NO2 VCD results of the satellite at transit time (13:30) were consistent with the hyperspectral NO2 horizontal distribution results at 13:00–14:00 on the same day but were not consistent with the daily average NO2 results. The hourly NO2 concentration in each area was 10–40% lower than the daytime average obtained by the hyperspectral remote sensing result. Based on these results, we approximated the errors associated with the calculation of NO2 emissions based on the satellite results, with a maximum bias of approximately 69.45–83.34%.

How to cite: Li, Q., Lu, C., Xing, C., Hu, Q., Tan, W., Li, H., Li, J., Zhang, Z., Chang, B., and Liu, C.: A novel hyperspectral remote sensing technique for horizontal distribution of atmospheric gaseous pollutant: to fill the spatio-temporal resolution limitations of satellite and in-situ observations, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4611, https://doi.org/10.5194/egusphere-egu23-4611, 2023.

EGU23-4636 | ECS | Posters on site | AS5.18

Preliminary Results of the GMAP/SIJAQ Campaign: Remote Sensing Measurements of Air Pollution over Korea 

Kangho Bae, Chang-Keun Song, Andreas Richter, Thomas Wagner, Michel van Roozendael, Kezia Lange, Tim Boesch, Steffen Ziegler, Alexis Merlaud, Sang Seo Park, Jong-Uk Park, and Hyunkee Hong

GEMS (Geostationary Environmental Monitoring Spectrometer), the world’s first geostationary environmental satellite was successfully launched in February 2020 and keeps monitoring the trace gases around East Asia. For improving the GEMS retrieval algorithms and validation of the products, NIER (National Institute of Environmental Research) organized two international field campaigns in Korea: GMAP2021 (GEMS MAP of Air Pollution) and SIJAQ2022 (Satellite Integrated Joint monitoring of Air Quality), respectively in winter and summer season. In the framework of these campaigns, to fill the gap of the reference ground remote sensing observation network, additional Pandora and MAX-DOAS instruments were installed in SMA (Seoul Metropolitan Area), Ulsan, and Busan. In addition, we operated Car-DOAS and GCAS (GeoCAPE Airborne Simulator) flight measurements around the SMA and the Southeastern region to catch the detailed distribution of emission sources. Preliminary results indicate different diurnal variation patterns of NO2 columns in SMA and the Southeastern region, visible both in ground-based and GEMS data. Car-DOAS measurements show a detailed distribution of trace gases at city level and for a few days during the summer season (SIJAQ2022), Car-DOAS even caught some well-synchronized high SO2 and HCHO signals with NO2, which can be related to anthropogenic emissions around the industrial area and in the case of the SMA emission estimation measurement, nice plumes were observed along the wind direction on good meteorological condition days.

How to cite: Bae, K., Song, C.-K., Richter, A., Wagner, T., Roozendael, M. V., Lange, K., Boesch, T., Ziegler, S., Merlaud, A., Park, S. S., Park, J.-U., and Hong, H.: Preliminary Results of the GMAP/SIJAQ Campaign: Remote Sensing Measurements of Air Pollution over Korea, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4636, https://doi.org/10.5194/egusphere-egu23-4636, 2023.

The Tibetan Plateau (TP) plays a key role in regional environment and global climate change, however, the lack of vertical observation hinders a deeper understanding of the atmospheric chemistry and atmospheric oxidation capacity (AOC) on the TP. In this study, we conducted MAX-DOAS measurements at Nam Co, central TP, to observe the vertical profiles of aerosol, water vapor, NO2, HONO and O3 from May to July 2019. In addition to NO2 mainly exhibiting a Gaussian shape with the maximum value appearing at 300-400 m, other four species all showed an exponential shape and decreased with the increase of height. The maximum values of monthly averaged aerosol (0.17 km-1) and O3 (66.71 ppb) occurred on May, water vapor (3.68×1017 molec cm-3) and HONO (0.13 ppb) appeared on July, while NO2 (0.39 ppb) occurred on June at 200-400 m layer. Water vapor, HONO and O3 all exhibited a multi-peak pattern, and aerosol appeared a bi-peak pattern for their averaged diurnal variation. Moreover, we found O3 and HONO were the main contributors to OH on the TP. The averaged vertical profiles of OH production rates from O3 and HONO all exhibited an exponential shape, and decreased with the increase of height with the maximum values of 2.61 ppb/h and 0.49 ppb/h at the bottom layer, respectively. In addition, source analysis for HONO and O3 were conducted based on vertical observations. The heterogeneous reaction of NO2 on wet surfaces was a significant source of HONO, which obviously associated with water vapor concentration and aerosol extinction. The maximum values of HONO/NO2 appeared around water vapor being 1.0×1017 molec cm-3 and aerosol being lager 0.15 km-1 under 1.0 km, and the maximum values usually accompanied with water vapor being 1.0-2.0×1017 molec cm-3 and aerosol being lager 0.02 km-1 at 1.0-2.0 km. O3 was potentially sourced from south Asian subcontinent and Himalayas through long-range transport. Our results enrich the new understanding of vertical distribution of atmospheric components and explained the strong AOC on the TP.

How to cite: Xing, C., Liu, C., and Hu, Q.: Observations of the vertical distributions of summertime atmospheric pollutants in Nam Co: OH production and source analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4660, https://doi.org/10.5194/egusphere-egu23-4660, 2023.

EGU23-4852 | Orals | AS5.18

Ozone profiles without blind area retrieved from MAX-DOAS observations: methodology, validations and applications 

Xiangguang Ji, Cheng Liu, Yang Wang, Qihou Hu, and Thomas Wagner

    Tropospheric ozone (O3) profiles, especially within the boundary layer, are essential for studying the vertical, temporal, spatial variations, as well as the formation sensitivity and regional transport of O3. However, it is rare to find continuous tropospheric O3 profiles with high temporal and spatial resolutions without blind areas using current remote sensing technologies, with issues such as low near-surface sensitivity or systematic blind areas from satellite and LiDAR observations, respectively, being encountered. Here, multi-source data including stratospheric O3 profiles from external datasets and local monthly dependent a priori profiles were fused in the retrieval algorithm, then vertical O3 profiles from the near-surface to the free troposphere were retrieved from multi-axis differential optical absorption spectroscopy (MAX-DOAS) measurements. This study mainly includes the following three points: First, with the aim of deriving a set of best practice recommendations for applying a profile inversion algorithm to long-term observations, we comprehensively investigated the influence of various settings on profile retrieval, with emphasis on the selection of a Fraunhofer reference spectrum and appropriate a priori profiles in the upper troposphere. Secondly, tropospheric O3 profiles were retrieved for operational MAX-DOAS observations in Beijing, and the results, especially for the boundary layer, were evaluated in detail with respect to well-established independent O3 datasets, including one-year ozonesonde profiles and tower-based in-situ measurements at different altitudes. A good level of agreement was found for both near-surface and elevated-altitude results, and the MAX-DOAS O3 profiles were able to reproduce the vertical distributions measured by ozonesonde. Then, the characteristics of ozone vertical temporal variations during the pollution episode were concluded. At the meanwhile, vertical ozone formation sensitivities across the Chinese metropolis, such as Beijing, Guangzhou, etc., were studied basing on the retrieval of O3, HCHO and NO2 from MAX-DOAS observations.

How to cite: Ji, X., Liu, C., Wang, Y., Hu, Q., and Wagner, T.: Ozone profiles without blind area retrieved from MAX-DOAS observations: methodology, validations and applications, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-4852, https://doi.org/10.5194/egusphere-egu23-4852, 2023.

EGU23-5253 | ECS | Orals | AS5.18

Ground-based imaging of NO2 emission plumes from Bełchatów Power Station using a hyperspectral camera 

Felix Külheim, Marvin Knapp, Leon Scheidweiler, Ralph Kleinschek, Paweł Jagoda, Jarosław Nęcki, and André Butz

Nitrogen oxides (NOx  = NO + NO2) are atmospheric pollutants that are detrimental to air quality and human health and play a major role in tropospheric ozone chemistry. Combustion processes produce NOx; thus, coal-fired power plants contribute significantly to the emission total (EEA 2017). Imaging atmospheric NOxcolumns with the Differential Optical Absorption Spectroscopy (DOAS) method is a well-established tool for NOx  emission monitoring (e.g. Lohberger 2004; Manago 2018).

During field measurements in June 2022, we deployed a ground-based hyperspectral camera (HySpex) for the visible to near-infrared (VNIR) spectral range at a distance of 6 km from the largest coal-fired power plant in Europe, the Bełchatów Power Station in Poland. We present preliminary results of NOemission plume images using sky-scattered sunlight as the light source. Our HySpex VNIR-1800 hyperspectral camera records spatially highly resolved images with 2400 pixels horizontally and 1800 pixels vertically covering a 22°x16.5° field of view at a temporal resolution of 1 minute. The camera covers the spectral range between 400 nm and 1000 nm with a spectral resolution of 5 nm and sampling intervals of 3.2 nm. We retrieve pixel-wise differential slant column densities of NO2  using DOAS in the 420 - 550 nm spectral interval. Despite the low spectral resolution, NO2  absorption structures can be identified and fitted, as we demonstrate by lab measurements with pre-calibrated NO2  cells.

We examine the performance of the NO2  camera and the potential for combining it with a co-deployed carbon dioxide (CO2) HySpex camera that operates in the shortwave-infrared spectral range. Simultaneous observations of NO2  and CO2  might enable insights into plume dynamics, photochemical processing in the plume and the emission ratio of the two species.

 

References:

European Environment Agency, 2017. Releases of pollutants to the environment from Europe’s industrial sector – 2015. url: https://www.eea.europa.eu /publications/releases-of-pollutants-to-the/releases-of-pollutants-from-industrial-sector (visited on 01/04/2023).

Lohberger, Falko et al.,  Aug. 2004. “Ground-based imaging differential optical absorption spectroscopy of atmospheric gases”. In: Applied Optics 43.24, p.4711. doi: 10.1364/ao.43.004711. url: https://doi.org/10.1364/ao.43.004711.

Manago, Naohiro et al.,  July 2018. “Visualizing spatial distribution of atmospheric nitrogen dioxide by means of hyperspectral imaging”. In: Applied Optics 57.21, p. 5970. doi: 10.1364/ao.57.005970. url: https://doi.org/10.1364/ao.57.005970.

How to cite: Külheim, F., Knapp, M., Scheidweiler, L., Kleinschek, R., Jagoda, P., Nęcki, J., and Butz, A.: Ground-based imaging of NO2 emission plumes from Bełchatów Power Station using a hyperspectral camera, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5253, https://doi.org/10.5194/egusphere-egu23-5253, 2023.

EGU23-5483 | Posters on site | AS5.18

Regional transport of air pollutants from stereoscopic remote sensing observation 

Qihou Hu, Yizhi Zhu, Chengxin Zhang, Wenjing Su, Xiangguang Ji, Chengzhi Xing, Haoran Liu, Wei Tan, Qihua Li, and Cheng Liu

  In addition to local emissions and atmospheric chemical reactions, regional transport is also an important source of atmospheric pollutants. Satellite-based remote sensing can obtain the spatial distribution of air pollutants in a large range. However, due to the influence of cloud coverage, there is the problem of data missing, which make it difficult to directly use satellite data for quantitative assessment of regional transport. In this study, we used satellite remote sensing from TROPOMI to update the emissions of WRF-Chem modeling. Then, the spatial distribution of regional transport fluxes was obtained through the updated modeling, and the output areas of air pollutants were identified in a large range of regional pollution events. We find that with the overall improvement of air quality in the Beijing-Tianjin-Hebei region, the contribution of external input to air pollution in Beijing from surrounding cities shows a downward trend, while the impact of local emissions become more prominent. Besides, the transports through elevated altitude were investigated through ground-based remote sensing. We found that the transport heights and source regions for different pollutants are quite different. Aerosols and sulfur dioxide (SO2) are significantly affected by the long-distance transport across the upper boundary layer; nitrogen dioxide (NO2) is mainly from local emissions and transport from surrounding area across the lower boundary layer; while the regional transport of formaldehyde (HCHO) is not obvious. Moreover, regional transport through elevated altitudes not only directly brings air pollutants, but also can cause the inversion of the vertical structure of aerosols. The inverse structure of aerosols can further induce adverse meteorological conditions through the interaction between pollution and meteorology, and then aggravate air pollution.

How to cite: Hu, Q., Zhu, Y., Zhang, C., Su, W., Ji, X., Xing, C., Liu, H., Tan, W., Li, Q., and Liu, C.: Regional transport of air pollutants from stereoscopic remote sensing observation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-5483, https://doi.org/10.5194/egusphere-egu23-5483, 2023.

EGU23-6091 | Orals | AS5.18

A CNN - SVR model for NO2 profile Prediction based on MAX-DOAS observation 

Xin Tian, Yifeng Pan, Pinhua Xie, Jin Xu, Ang Li, Zijie Wang, Zhaokun Hu, and Jiangyi Zheng

In the Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) trace gases profile retrieval, it needs to obtain the vertical profile of aerosols as the a priori, and depends on the atmospheric radiative transfer model (RTM). Therefore, a data mining method named CNN-SVR was adopted to achieve the prediction of NO2 profile, which combines the advantages of convolutional neural network (CNN), support vector regression (SVR) and MAX-DOAS. The optimization core of the hybrid model is embodied in three aspects. (1) CNN extracting the effective features of MAX-DOAS spectral data. The input data are MAX-DOAS spectrum, wind direction, wind speed, season, temperature, relative humidity, aerosol optical depth (AOD), cloud cover. Feature variables of MAX-DOAS spectra were extracted by CNN. The output data set is the NO2 profile retrieved by MAX-DOAS profile inversion algorithm PriAM. The data set is processed by normalization to unify the dimensions to ensure the accelerated convergence of the program. (2) The mean impact value (MIV) method selecting the input variables sensitive to NO2 profile forecasting. The MAX-DOAS spectral data, temperature, AOD and low cloud cover are finally determined as the best input parameters of the prediction model. (3) The hybrid forecasting method. Combined with the advantages that CNN can reduce the amount of data processing and retain useful information, and SVR does not depend on the dimension of input space, a CNN-SVR hybrid prediction model is proposed. The average percentage error (MAPE) of the CNN-SVR model is 9.14%. Compared with the separately constructed CNN, SVR and backpropagation models, the MAPE of CNN-SVR is reduced by 8.22%, 6.00% and 32.28% respectively. Therefore, CNN-SVR can effectively predict tropospheric NO2 profiles by using MAX-DOAS observation.

How to cite: Tian, X., Pan, Y., Xie, P., Xu, J., Li, A., Wang, Z., Hu, Z., and Zheng, J.: A CNN - SVR model for NO2 profile Prediction based on MAX-DOAS observation, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-6091, https://doi.org/10.5194/egusphere-egu23-6091, 2023.

EGU23-7316 | ECS | Orals | AS5.18 | Highlight

MAX-DOAS Network in China and Its Applications 

Haoran Liu, Cheng Liu, Chengzhi Xing, Qihou Hu, Wei Tan, and Xiangguang Ji

Entering the “14th Five-Year Plan”, the coordinated control of PM2.5 and O3 has become a major issue of air pollution prevention and control in China. In order to achieve this goal, the stereoscopic monitoring of regional PM2.5 and O3 and their precursors (NO2, HCHO etc.) is extremely necessary. Yet, current monitoring networks are inadequate to monitor the vertical profiles of all above atmospheric compositions simultaneously, and to support air quality control. We have established a nationwide ground-based hyperspectral stereoscopic remote sensing network based on MAX-DOAS since 2015. This monitoring network provides a significant opportunity for the regional coordinated control of PM2.5 and O3 in China. One-year vertical profiles of aerosol, NO2, HCHO and O3 monitored from four MAX-DOAS stations (CAMS, SH_XH, SUST and CQ) installed in four megacities (Beijing, Shanghai, Shenzhen and Chongqing) are used to characterize their vertical distribution differences in four key regions of Jing-Jin-Ji (JJJ), Yangtze River Delta (YRD), Pearl River Delta (PRD) and Sichuan Basin (SB), respectively. The normalized and yearly averaged aerosol vertical profiles in JJJ and PRD exhibit a box shape under 400 m and a Gaussian shape, respectively, and they all show exponential shapes in YRD and SB. The NO2 vertical profiles in four regions all exhibit exponential shapes due to the obvious vehicle emissions. The shape of HCHO vertical profile in JJJ and PRD shows Gaussian, and it exhibits exponential shape in YRD and SB. The averaged O3 vertical profiles in four regions all exhibit box shape and linear shape in pollution and non-pollution periods, respectively. Moreover, a regional transport event occurred at an altitude of 600-1000 m was monitored in the southwest-northeast pathway of North China Plain (NCP) by five MAX-DOAS stations (SJZ, WD, NC, CAMS and UCAS) belonging to above network. The aerosol optical depths (AOD) in these five stations varied in the order of SJZ > WD > NC > CAMS > UCAS. The short-distance regional transport of NO2 in 800 m layer was monitored between WD and NC. As an important precursor of secondary aerosol, NO2 air mass in WD and NC all occurred 1 hr earlier than aerosol. Similarly, the short-distance regional transport of HCHO in 800 m layer between NC and CAMS, and it potentially affected the O3 concentration in Beijing. Finally, CAMS was selected as a typical site to learn O3-NOx-VOCs sensitivities in vertical space. We found the production of O3 changed from predominantly VOC-limited condition to mainly mixed VOC-NOx-limited condition from 0-100 m layer to 200-300 m layer. In addition, the downward transport of O3 could make a contribute to the increase of ground surface O3 concentration. ground-based hyperspectral stereoscopic remote sensing network provide a promising strategy to support PM2.5 and O3 and their precursors management and attribution of sources.

How to cite: Liu, H., Liu, C., Xing, C., Hu, Q., Tan, W., and Ji, X.: MAX-DOAS Network in China and Its Applications, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7316, https://doi.org/10.5194/egusphere-egu23-7316, 2023.

EGU23-7447 | ECS | Posters on site | AS5.18

Estimating Nitrogen Oxides emissions from inland waterway vessels using MAX-DOAS measurements – Results of pioneering measurements and plans to advance the method 

Simona Ripperger-Lukosiunaite, Steffen Ziegler, Sebastian Donner, Leon Kuhn, Thorsten Hoffmann, Peter Hoor, and Thomas Wagner

Nitrogen oxides (NOx, i.e. NO and NO2) are a major contributor to urban air pollution and have negative impacts on human health, relating to respiratory and cardiovascular problems. NO2 is also a precursor of secondary particulate matter and tropospheric ozone, which are also associated with adverse effects on human health. Inland waterway vessels are a significant source of NOx emissions due to their diesel engines operating at high temperatures. Emissions from inland ships are concentrated in the vicinity of waterways, and could be a significant local air pollution source, particularly in residential areas located along intensively used waterways, narrow and steep river valleys, and small villages without heavy road traffic or nearby power plants. Hence, quantifying the influence of inland ship emissions on air quality and humans is important.

We demonstrate the use of ground-based MAX-DOAS (Multi AXis-Differential Optical Absorption Spectroscopy) measurements to estimate NOx emissions from inland ships on the Rhine River in western Germany. We show that this method can be used to derive ship emissions of NOx for individual plumes and as an average over several plumes. However, we also identify several challenges with this approach and propose ways to improve it.

The combination of MAX-DOAS and in situ measurements, particularly knowledge of the NO/NO2 ratio could lead to more accurate estimates of ship emissions. In addition, we introduce planned systematic measurements at selected locations, such as narrow parts of the Rhine and Moselle valleys, where ship emissions may be a major pollution source. We plan to apply regional models to estimate the effect of the updated ship emissions on local NOx concentrations.

How to cite: Ripperger-Lukosiunaite, S., Ziegler, S., Donner, S., Kuhn, L., Hoffmann, T., Hoor, P., and Wagner, T.: Estimating Nitrogen Oxides emissions from inland waterway vessels using MAX-DOAS measurements – Results of pioneering measurements and plans to advance the method, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-7447, https://doi.org/10.5194/egusphere-egu23-7447, 2023.

EGU23-8101 | ECS | Posters on site | AS5.18

Validation of a MAX-DOAS instrument-based cloud classification algorithm 

Lucas Reischmann, Steffen Ziegler, Steffen Beirle, Vinod Kumar, Sebastian Donner, and Thomas Wagner

A major challenge in Differential Optical Absorption Spectroscopy (DOAS) is the characterization of the light path. For the determination of the light path length, cloud conditions are essential. While instruments like a LIDAR/ceilometer provide information on cloud base height in zenith direction, it is often quite challenging to obtain information on cloud coverage in the line of sight of a Multi-Axes-DOAS (MAX-DOAS) instrument.

In this study, we apply an existing cloud classification algorithm using combined information from the colour index and the O4 slant column density (Wagner et al., 2013) on spectra recorded by a MAX-DOAS instrument. In order to validate the algorithm, a MAX-DOAS with camera measurements of the sky conditions carried out at the Max Planck Institute for Chemistry in Mainz for several months. The results of the cloud classification algorithm are compared to the recordings of the cameras in order to analyse the performance of the algorithm.

How to cite: Reischmann, L., Ziegler, S., Beirle, S., Kumar, V., Donner, S., and Wagner, T.: Validation of a MAX-DOAS instrument-based cloud classification algorithm, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-8101, https://doi.org/10.5194/egusphere-egu23-8101, 2023.

EGU23-9561 | Orals | AS5.18

CHAPS: A New, Compact Hyperspectral Imager for Air Pollution Remote Sensing 

William Swartz, Nickolay Krotkov, Lok Lamsal, Frank Morgan, Benjamin Stewart, Walter Zimbeck, Gerard Otter, Floris van Kempen, Pieternel Levelt, and Pepijn Veefkind

Current and planned low Earth orbit and geostationary satellite instruments have long provided global surveys, revealing air pollution characteristics and trends. Targeted pollution observations with even finer spatial and temporal resolution would better characterize, quantify, and monitor emissions from urban areas, power plants, and other anthropogenic activities, with both scientific and societal benefits. The Compact Hyperspectral Air Pollution Sensor (CHAPS) is an imaging spectrometer in a CubeSat form factor, made possible by the use of freeform optics and additive manufacturing. CHAPS has the potential to complement global surveyors and provide targeted observations valuable for understanding air quality at urban scales. The instrument is designed to make measurements of atmospheric composition at 300–500 nm (@ 0.6-nm spectral resolution) at unprecedented spatial resolution from low Earth orbit (1 x 1 km2). The NASA Earth Science Technology Office has funded the development of a CHAPS–Demonstrator (CHAPS-D), which will result in an airborne demonstration of a CHAPS prototype instrument. The CHAPS-D project is a joint collaboration of JHU/APL (USA) and TNO (The Netherlands). CHAPS-D freeform optics derive heritage from the Sentinel-5 Precursor (TROPOMI) mission. Freeform optics has potentially huge advantages over traditional optical designs, including fewer optical surfaces and lower mass and volume, while maintaining optical performance, and CHAPS-D will fit within the design constraints of a 6U CubeSat. The CHAPS-D mechanical structure and some optical elements will be fabricated using additive manufacturing, using a next-generation aluminum alloy. This approach simplifies the construction of the instrument and allows for integral stray light baffling features not possible using traditional fabrication approaches. The compact size and relatively lower cost of CHAPS makes a constellation feasible for the first time, with unprecedented spatiotemporal sampling of global point pollution sources. The project will culminate in an airborne demonstration of CHAPS-D, with 30-m spatial resolution. We will retrieve NO2, SO2, HCHO, ozone, and other trace species relevant to air quality from solar backscatter measurements. We present the science context, measurement requirements, and preliminary design of CHAPS-D, as well as results from breadboard testing.

How to cite: Swartz, W., Krotkov, N., Lamsal, L., Morgan, F., Stewart, B., Zimbeck, W., Otter, G., Kempen, F. V., Levelt, P., and Veefkind, P.: CHAPS: A New, Compact Hyperspectral Imager for Air Pollution Remote Sensing, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9561, https://doi.org/10.5194/egusphere-egu23-9561, 2023.

EGU23-9615 | ECS | Orals | AS5.18 | Highlight

First measurements of spatial NO2 variability in Bremen with a newly developed tram DOAS instrument 

Kezia Lange, Andreas Richter, Lisa K. Behrens, and John P. Burrows

Mobile DOAS measurements are a good option to determine the spatial distribution of NO2 or other trace gases such as HCHO and SO2 within a city. In previous works, such measurements have been performed using cars and have provided interesting insights into spatial inhomogeneities of the NO2 distribution and valuable contributions to satellite validation. A disadvantage of car DOAS measurements is the time required for driving the car.

Therefore, a new DOAS instrument was developed and installed on a tram in Bremen in November 2021. The instrument is mostly operating in zenith-sky mode, but also takes measurements at 20° elevation every 7 minutes. The advantage of the tram DOAS instrument is that it performs measurements during the normal operation of the tram. As a result, regular measurements along the route network can be carried out without additional time spent driving.

Up to now, the instrument has gathered one year of data all over the Bremen tram network. It can be clearly seen that the areas of increased tropospheric NO2 VCDs change throughout the day, but certain areas show reproducibly higher NO2 pollution. We found elevated NO2 levels in the industrially dominated northwest and lower levels in the more rural northeast of Bremen. This is confirmation for a very similar distribution visible in the TROPOMI tropospheric NO2 VCDs data. In addition, the tram DOAS measurements are compared to the measurements from a stationary MAX-DOAS instrument installed close to one of the tram lines.   

How to cite: Lange, K., Richter, A., Behrens, L. K., and Burrows, J. P.: First measurements of spatial NO2 variability in Bremen with a newly developed tram DOAS instrument, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-9615, https://doi.org/10.5194/egusphere-egu23-9615, 2023.

EGU23-11128 | ECS | Posters on site | AS5.18

McPrA - a new trace gas profile retrieval algorithm for MAX-DOAS 

Jiangyi Zheng, Pinhua Xie, Xin Tian, Jin Xu, Ang Li, Bo Ren, Feng Hu, Zhaokun Hu, Yinsheng Lv, and Zhidong Zhang

Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) has been widely used in the three-dimensional monitoring of air pollutants. It is of great significance for MAX-DOAS to reconstruct the state of air pollutants by establishing an accurate vertical profile retrieval algorithm. At present, the profile retrieval algorithm of MAX-DOAS mainly adopts the iterative method based on a priori profile, which leads to strong dependence on priori profiles. We try to reduce the dependence on priori profiles by first calculating the vertical column density and then calculating the vertical distribution from observation. Therefore, we propose a new MAX-DOAS trace gas profile inversion algorithm - McPrA (Monte Carlo profile inversion algorithm by Anhui Institute of Optics and Fine Mechanics (AIOFM)). The algorithm uses Monte Carlo method to solve the optimal estimation problem of the gas profile. Firstly, the gas vertical column density is obtained through the air mass factor calculated by the radiative transfer model SCIATRAN. Secondly, the vertical distribution of trace gas is retrieved by combining the weight function with the a priori profile. Besides, we introduce the normalization process in the vertical distribution solution to make the prior profile better match the weight function. McPrA can set the vertical resolution of profile by modifying the grid, and we increase the vertical resolution of gas profile to 50m. By conducting sensitivity experiments on parameters such as Monte Carlo sampling, covariance matrix and the priori profiles, the optimal configuration of retrieval parameter is obtained. At the same time, the degree of freedom is more than 3.0. Finally, comparative verification experiments were carried out to compare with in situ data from LP-DOAS and National Air Quality Monitoring Station. The correlation coefficient for NO2 VMR at the first layer retrieved by McPrA in 50 m grid reached above 0.89. The comparison of NO2 profiles retrieval by McPrA with that from WRF-Chem and simulation of synthetic data also shows that McPrA algorithm can retrieve trace gas profiles accurately.

How to cite: Zheng, J., Xie, P., Tian, X., Xu, J., Li, A., Ren, B., Hu, F., Hu, Z., Lv, Y., and Zhang, Z.: McPrA - a new trace gas profile retrieval algorithm for MAX-DOAS, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11128, https://doi.org/10.5194/egusphere-egu23-11128, 2023.

EGU23-11189 | Orals | AS5.18

Towards tomographical MAX DOAS profile retrieval:  sensitivity studies 

Janis Pukite, Steffen Beirle, Sebastian Donner, Bianca Lauster, Simona Ripperger-Lukosiunaite, Steffen Ziegler, and Thomas Wagner

The ground-based Multiple Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) measurement technique is of high interest to measure local scale pollution events like trace gas plumes above cities or power plants. Besides vertical column densities and especially for the comparison with in-situ measurements and model simulations, vertical profiles of aerosol extinction and trace gas concentrations are retrieved. In this the horizontal extent of the plume is usually neglected in the forward modelling (i.e. horizontally homogeneous distribution is assumed).

Here we investigate by sensitivity studies on simulated measurements 1) the systematic errors induced when in fact a horizontally limited plume is measured while neglecting the limited horizontal  plume extent in the retrieval, 2) the capabilities to correct for these errors by a tomographic measurement scheme scanning the same air masses by two instruments, and 3) we provide an outlook to the practical applicability of such a measurement concept.

 

How to cite: Pukite, J., Beirle, S., Donner, S., Lauster, B., Ripperger-Lukosiunaite, S., Ziegler, S., and Wagner, T.: Towards tomographical MAX DOAS profile retrieval:  sensitivity studies, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11189, https://doi.org/10.5194/egusphere-egu23-11189, 2023.

EGU23-11376 | Posters on site | AS5.18

Measurements of trace gases with a MAX-DOAS system during a ship cruise from the Canaries to Ecuador (SO287) on board of RV Sonne 

Tim Bösch, Miriam Latsch, Andreas Richter, Folkard Wittrock, and John P. Burrows

Ship-based trace gas measurements are of particular interest to the scientific community as they fill a gap in knowledge of trace gas concentrations in the marine boundary layer (MBL) on the open ocean. Remote sensing techniques, such as Multi AXis Differential Optical Absorption Spectroscopy (MAX-DOAS), offer the capability of probing air masses located further away from the ship, compared to in situ instruments. In this way, MAX-DOAS measurements taken during ship cruises can be used to examine larger volumes of air in the MBL where routinely measured data is sparse.

We present measurements of a MAX-DOAS system installed on the research vessel Sonne during the cruise SO287 from Las Palmas (Gran Canaria, Spain) to Guayaquil (Ecuador) from the 11th of December 2021 until the 11th of January 2022.    
Ship-based anthropogenic emissions have been identified as higher slant column densities (SCD) of nitrogen dioxide (NO2) and sulphur dioxide (SO2) while biogenic emissions are mainly found close to land, as indicated by higher SCDs of formaldehyde (HCHO). On the open ocean, the frequently detected abundance of iodine monoxide (IO) emphasizes that the MBL is mainly dominated by emissions from the ocean (algae) in the absence of anthropogenic emissions.               
In a second step, these SCD results have been analysed with the profiling algorithm BOREAS to further assess the vertical extent of trace gases in the MBL. Since trace gas concentrations are highest in the lowest kilometre, emission sources close to the shipping route and the ocean surface dominate the measurements taken during cruise SO287.

How to cite: Bösch, T., Latsch, M., Richter, A., Wittrock, F., and Burrows, J. P.: Measurements of trace gases with a MAX-DOAS system during a ship cruise from the Canaries to Ecuador (SO287) on board of RV Sonne, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11376, https://doi.org/10.5194/egusphere-egu23-11376, 2023.

EGU23-11861 | ECS | Posters on site | AS5.18

The TROPOMI Ozone Profile retrieval algorithm and its use for stratospheric and tropospheric atmospheric research 

Serena Di Pede, Pepijn Veefkind, Maarten Sneep, Mark ter Linden, and Arno Keppens

The status and the most recent developments of the algorithm of the operational TROPOMI (Tropospheric Monitoring Instrument) Ozone Profile product will be presented in this contribution. TROPOMI is the payload onboard of the single-satellite Sentinel-5 Precursor (S5P), an atmospheric composition mission that is part of the EU Copernicus program. The aim of the TROPOMI ozone profile product is to continue the record of the stratospheric ozone, monitor changes, improve the accuracy of the retrieved stratospheric profiles and focus on the tropospheric ozone, which is also important for climate studies. The monitoring of the evolution of stratospheric and tropospheric ozone is important as the ozone plays an important role in atmospheric chemistry and radiative balance throughout the atmosphere. The stratospheric ozone layer from 15 to 50 km absorbs the harmful UV radiation, protecting life at the surface. Tropospheric ozone is a greenhouse gas affecting the climate. In addition, ozone in the lower troposphere is a toxic component of air pollution with significant public health and agricultural impacts.

The operational ozone profile product of TROPOMI provides the ozone profile at 33 pressure levels in the atmosphere and as 6 sub-columns with a vertical sampling depending on the altitude. The ozone profile is derived from the UV spectral range (270-330 nm), with an horizontal spatial resolution of approximately 28x28 km2. The derived ozone profile contains 6-7 independent pieces of information, providing a vertical resolution in the range 7 – 15 km. The retrieval is based on the Optimal Estimation method, which combines the information from the measured spectra with the a-priori information. In addition to the a-priori profile, the retrieved profiles and their errors, the algorithm also provides diagnostic information, such as the averaging kernel matrix of the ozone profile elements, an essential parameter also for the product validation operated by the ESA/Copernicus Atmospheric Mission Performance Cluster/Validation Data Analysis Facility (ATM-MPC/VDAF).

The algorithm also relies on accurate Level 1B radiometric calibration of both radiance and irradiance data, which addresses in particular the spectral region below 310 nm. From comparison to other satellites sensors as well as to forward models, it is known that the TROPOMI UV spectral bands show systematic radiometric deviations. To address this issue, a radiometric correction based on a comparison with forward models has been developed. The derived correction parameters are updated regularly in the operational product in order to follow the changes of the instrument over time due to its optical degradation.

The improvements in the operational algorithm, regarding the radiometric calibration and the choice of a new climatology for the ozone profile a-priori information and its uncertainty, are crucial aspects for the ozone retrieval and they will be shown during this talk.

Finally, with the availability of the reprocessed ozone profile data from the beginning of the mission, this contribution will also show the results of the algorithm performances throughout the TROPOMI mission, in ozone hole conditions and for tropospheric enhancements.

How to cite: Di Pede, S., Veefkind, P., Sneep, M., ter Linden, M., and Keppens, A.: The TROPOMI Ozone Profile retrieval algorithm and its use for stratospheric and tropospheric atmospheric research, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-11861, https://doi.org/10.5194/egusphere-egu23-11861, 2023.

EGU23-13464 | Posters on site | AS5.18

Enhancing the AOTF-based NO2 camera with light polarization sensitivity for aerosol retrievals 

Emmanuel Dekemper and Jurgen Vanhamel

The AOTF-based NO2 camera is a remote sensing instrument primarily aimed at imaging and quantifying the NO2 field above cities or in industrial plumes. The measurement principle consists in acquiring a number of spectral images of the scene at selected wavelengths. Each pixel is therefore recording a discrete spectrum of the radiance collected in its acceptance cone, enabling the retrieval of the NO2 column density in its optical path by application of the DOAS method on the measured spectrum.

The core element of the instrument principle is the acousto-optical tunable filter (AOTF). This device works under the principle of the acousto-optical interaction, the coupling of the light electric field with the modulation of the crystal lattice by a shear acoustic wave created by a transducer. The coupling takes place at a single wavelength, and diffracts that part of the spectrum into another direction. By blocking the undiffracted light beam, and imaging the diffracted order, one can capture a monochromatic image of the scene.

We propose to expand the capabilities of the NO2 camera by exploiting another aspect of the acousto-optic interaction. The coupling between light and sound actually takes place in a birefringent crystal (TeO2), and one usually works with a single linear polarization of the incoming light (e-light, or o-light). The two polarization components are diffracted in different directions. If the current design is modified such that the two components can be imaged, then an information on the degree of linear polarization of the light can be obtained.

In the atmosphere, the scattering of light by air (Rayleigh), and particles (Mie) is controlling the state of polarization of the scattered solar light. Hence, aerosols not only introduce a smooth spectral signatures, but also a change of the state of polarization. The proposed modification of the NO2 camera design can provide some sensitivity on this, potentially enhancing the scientific return of the instrument with aerosol retrievals capabilities. The new instrumental design will be presented, and vector radiative transfer simulations will be produced to estimate the benefit of this change.

How to cite: Dekemper, E. and Vanhamel, J.: Enhancing the AOTF-based NO2 camera with light polarization sensitivity for aerosol retrievals, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13464, https://doi.org/10.5194/egusphere-egu23-13464, 2023.

EGU23-13645 | Posters on site | AS5.18

MAX-DOAS measurements of AOT, NO2 and HCHO in Kinshasa (DR Congo): comparisons with TROPOMI and GEOS-CHEM 

Alexis Merlaud, Rodriguez Yombo Phaka, Gaia Pinardi, Jean-Pierre Mbungu Tsumbu, Richard Bopili Mbotia Lepiba, Bunenimio Lomami Djibi, Martina Friedrich, Isabelle De Smedt, Jenny Stavrakou, Jean-François Muller, François Hendrick, Emmanuel Mahieu, and Michel Van Roozendael

African megacities suffer from air pollution and the problem is expected to worsen in the near-future, with the ongoing explosive demographic growth in these areas. The sources of pollutants in Africa are different from those found in Europe. Agricultural burnings and charcoal-based cooking largely contribute to the NO2 and HCHO burdens. However, many large African cities, such as the City of Kinshasa, capital of the Democratic Republic of Congo, do not have local pollution monitoring capabilities. In these polluted places, space-based measurements are often the only source of data available regarding air quality. Together with the validation of TROPOMI in a poorly sampled area, this context motivated ground-based DOAS observations in Kinshasa since 2017. We first operated a single-axis instrument, which we upgraded as a MAX-DOAS instrument in December 2019.  

We describe the observation site in Kinshasa, the MAX-DOAS instrument, and the retrievals which use the algorithmic tools developed within the FRM4DOAS project. We compare the MAX-DOAS database (2019-2023) of ground-based observations of aerosol optical thickness (AOT), NO2 and HCHO with MODIS and TROPOMI, and with simulations using the GEOS-CHEM Chemistry and Transport Model. Such comparisons enable to assess the quality of the satellite products and model performances around Kinshasa. The ground and satellite-based observations have different sensitivities to the trace gas profiles. Combining the observations and model datasets sheds light on the true atmospheric state above Kinshasa. Another objective of this work is to constrain emission inventories in central Africa. 

How to cite: Merlaud, A., Yombo Phaka, R., Pinardi, G., Mbungu Tsumbu, J.-P., Bopili Mbotia Lepiba, R., Lomami Djibi, B., Friedrich, M., De Smedt, I., Stavrakou, J., Muller, J.-F., Hendrick, F., Mahieu, E., and Van Roozendael, M.: MAX-DOAS measurements of AOT, NO2 and HCHO in Kinshasa (DR Congo): comparisons with TROPOMI and GEOS-CHEM, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13645, https://doi.org/10.5194/egusphere-egu23-13645, 2023.

EGU23-13808 | Orals | AS5.18

Nitrosat, a Satellite Mission Concept for Mapping Reactive Nitrogen at the Landscape Scale 

Lieven Clarisse and the Nitrosat team

Two key forms of reactive nitrogen (Nr) in the atmosphere are nitrogen oxides (NO+NO2) and ammonia (NH3). Both species are abundantly emitted from anthropogenic sources (fossil fuel combustion, agriculture) with devastating consequences on the environment, human health and climate. Complementing sparse ground-based measurements, current satellite sounders provide daily coverage of their global distribution. However, the spatial resolution of these instruments (>20 km² for NO2 and >100km² for NH3) is orders of magnitudes greater than the typical size of the main Nr sources (industries, farms, roads), which makes identification of the emitters, and corresponding quantification of their emission strengths particularly challenging.

To understand and address the impacts of a perturbed nitrogen cycle, and in response to the current observational gap, a dedicated satellite for the monitoring of NO2 and NH3 at high spatial resolution has been conceptualised. Nitrosat, as it is being called, is currently in Phase 0 of ESA’s Earth Explorer 11 call. Its main objective is to quantify simultaneously the emission sources of NH3 and NOx at the landscape scale (<0.25 km²) and to characterize seasonal patterns (<1 month) in their emissions. The two imaging spectrometers onboard Nitrosat will operate respectively in the infrared for NH3 and the visible for NO2, offering gapless coverage in a single swath.

Starting from representative examples of measurement techniques that are presently used to derive emission fluxes from NH3 and NO2 satellite observations, we discuss the limitations of current sounders. We introduce the Nitrosat measurement concept and, exploiting both model simulations and aircraft campaign data, provide examples from the Phase 0 studies of how Nitrosat will enable retrieval of emission fluxes from local and diffuse sources in a way that will not be possible with other current or planned missions.

How to cite: Clarisse, L. and the Nitrosat team: Nitrosat, a Satellite Mission Concept for Mapping Reactive Nitrogen at the Landscape Scale, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-13808, https://doi.org/10.5194/egusphere-egu23-13808, 2023.

EGU23-14162 | Orals | AS5.18

Methodological improvements and processing software of SO2 fluxes from UV cameras 

Hugues Brenot, Martina Friedrich, Nicolas Theys, Alexis Merlaud, Christian Hermans, Caroline Fayt, and Michel Van Roozendael

With its high temporal and spatial resolution, SO2 UV cameras are very attractive tools for monitoring emission and estimating fluxes (volcanic or anthropogenic sources). Their measurements can also contribute to warning systems (e.g., in the mitigation of volcanic crisis and its impact on aviation).

The first part of this contribution will briefly review the methodology with the pros and cons of this technique. In the calibration process (to obtain SO2 amounts by using a collocated spectrometer as a part of our EnviCam3 SO2 UV camera), we show means to mitigate some of the effect on UV light propagation (i.e., dilution and saturation) by using a multi-window DOAS analysis approach. We will show some tests of the saturation effect for sets of SO2 concentrations (from 10 to 10000 ppm.m) obtained in our laboratory (device with a vacuum pump).

 In the second part, we will present a new GUI Python software developed at BIRA, for both fast analysis during field campaigns and more detailed post-processing analysis of SO2 fluxes. The functionalities of this software consist of: 1) automatic or manual correction of X/Y shifts between the images from the two cameras; 2) correction of the vignetting effect in each image; 3) automatic detection of spectrometer field of view by correlation with time series of QDOAS retrieved SO2 slant columns for calculating the conversion factor to SO2 concentrations  4) estimation of the plume speed using optical flow computing; 5) retrievals of SO2 fluxes (box, traverse or delta-M methods).

Data measured in the harbour of Antwerp (in 2022 and 2023), at Etna (in 2022) and Nyiragongo (in 2017) volcanoes will be shown.

How to cite: Brenot, H., Friedrich, M., Theys, N., Merlaud, A., Hermans, C., Fayt, C., and Van Roozendael, M.: Methodological improvements and processing software of SO2 fluxes from UV cameras, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14162, https://doi.org/10.5194/egusphere-egu23-14162, 2023.

EGU23-14246 | Posters on site | AS5.18

The ALTIUS mission: status and performance 

Antonin Berthelot, Noel Baker, Philippe Demoulin, Quentin Errera, Ghislain Franssens, Didier Fussen, Nina Mateshvili, Didier Pieroux, Sotiris Sotiriadis, and Emmanuel Dekemper

ALTIUS (Atmospheric Limb Tracker for the Investigation of the Upcoming Stratosphere) is an atmospheric limb mission being implemented in ESA's Earth Watch programme and planned for launch in early 2026. The primary objective of the mission is to measure high-resolution stratospheric ozone concentration profiles. Secondary objectives are the retrievals of stratospheric aerosols particle density, NO2, water vapor and other minor species concentrations.

This innovative instrument consists of three spectral high-resolution imagers: UV (250-355 nm), VIS (440-675 nm) and NIR (600-1040 nm) channels. The UV channel uses a stack of four Fabry-Pérot interferometers, while the VIS and NIR channels each rely on an AOTF (Acousto-Optical Tunable Filter). Each channel can image scenes independently of the others at given wavelengths and with a moderate spectral resolution, and high spatial sampling. The agility of ALTIUS allows for series of observations at desired wavelengths carefully chosen to retrieve the vertical profiles of species of interest.

The instrument will perform measurements in different geometries to maximize global coverage: observing limb-scattered solar light in the dayside, solar occultations at the terminator, and stellar, lunar, and planetary occultations in the nightside.

The status of the ALTIUS mission will be presented as well as the foreseen quality of the Level-1 observations.  The quality of the retrieved profile densities will be discussed with a particular focus on the high vertical resolution that can be achieved using this instrument. The added-value of the native imaging capabilities of ALTIUS in terms of observations, and in-flight calibrations, will be highlighted.

How to cite: Berthelot, A., Baker, N., Demoulin, P., Errera, Q., Franssens, G., Fussen, D., Mateshvili, N., Pieroux, D., Sotiriadis, S., and Dekemper, E.: The ALTIUS mission: status and performance, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-14246, https://doi.org/10.5194/egusphere-egu23-14246, 2023.

EGU23-15430 | ECS | Posters on site | AS5.18

The airborne greenhouse gas observation systems MAMAP2D-Light and MAMAP2D – Characterization and performance assessment 

Jakob Borchardt, Konstantin Gerilowski, Oke Huhs, Sven Krautwurst, Heinrich Bovensmann, Hartmut Bösch, and John P. Burrows

Remote sensing measurements of greenhouse gases from aircraft to detect and quantify greenhouse gas emissions began about 15 years ago. These measurements have been exploited to detect and quantify predominantly anthropogenic emissions. However, with new satellite systems targeting especially methane (CH4) emissions on different scales, high-precision airborne measurements are needed to validate these satellite systems and detect and quantify emissions too small to be detected from space-based sensors.

For this, the MAMAP2D family of airborne passive imaging remote sensing instruments has been and is being built at the Institute of Environmental Physics of the University of Bremen. MAMAP2D-Light, the first of this family, is a lightweight, compact spectrometer measuring carbon dioxide (CO2) and CH4 enhancements in a short-wave infrared band around 1.6 µm with a spectral resolution of ~1.1 nm. It was flown successfully on a Diamond HK36 TTC-ECO motor glider aircraft of the Jade University of Applied Sciences in Wilhelmshaven and the High Altitude Long Range operations (HALO) aircraft of DLR during the COMET 2.0 Arctic campaign in Canada. The MAMAP2D instrument, the next biggest in the MAMAP2D family, covers the SWIR band with a higher spectral resolution and additionally contains a near-infrared channel covering O2 absorption around 760 µm for path-length correction and is currently assembled in the laboratory.

In this poster, we will present the spectral characterization of the MAMAP2D-Light instrument as flown during the COMET 2.0 Arctic campaign and assess its performance for detecting local CH4 and CO2 gradients. Additionally, initial laboratory characterizations of the MAMAP2D breadboarding activity will be presented.

How to cite: Borchardt, J., Gerilowski, K., Huhs, O., Krautwurst, S., Bovensmann, H., Bösch, H., and Burrows, J. P.: The airborne greenhouse gas observation systems MAMAP2D-Light and MAMAP2D – Characterization and performance assessment, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15430, https://doi.org/10.5194/egusphere-egu23-15430, 2023.

EGU23-15635 | ECS | Posters on site | AS5.18

CO2Image retrieval studies and performance analysis 

Philipp Hochstaffl, Andreas Baumgartner, Sander Slijkhuis, Guenter Lichtenberg, Claas H. Koehler, Franz Schreier, Anke Roiger, Dietrich G. Feist, Julia Marshall, André Butz, and Thomas Trautmann

Current and planned satellite missions such as the Japanese GOSAT (Greenhouse Gases Observing Satellite) and NASA’s OCO (Orbiting Carbon Observatory) series and the upcoming Copernicus Carbon Dioxide Monitoring (CO2M) mission aim to constrain national and regional-scale emissions down to scales of urban agglomerations and large point sources. The CO2Image demonstrator mission of the German Aerospace Center (DLR) is specifically designed to detect and quantify carbon dioxide (CO2) and methane (CH4) emissions from medium-size point sources. To this end its COSIS (Carbon dioxide Sensing Imaging Spectrometer) push-broom grating spectrometer measures reflected solar radiation with a high spatial resolution of 50x50 m2, covering tiles of ~50x50 km2 extent. The instrument has a moderate spectral resolution of approximately ~1 nm and observes in a single spectral window in the 2 µm region.

Here we present and discuss the impact of the expected COSIS performance on the retrieved level-2 data. The level-1 data (spectra) are generated using the Py4CAtS (Python for Computational ATmospheric Spectroscopy) line-by-line radiative transfer model and the COSIS SIMulator (COSIS-SIM). Based on the COSIS instrument parameters the analysis examines the retrieval errors related to noise which allows to estimate the detection and quantification limit of CO2 and CH4 emission rates at the instrument’s spatial and spectral resolution. We further discuss the effect of heterogeneous scenes, i.e. high contrast surfaces that cause an effective distortion of the spectral response function by non-uniform illumination of the entrance slit. Finally, we assess the influence of initial guess values for the plume's vertical extent and shape on the retrieval.

How to cite: Hochstaffl, P., Baumgartner, A., Slijkhuis, S., Lichtenberg, G., Koehler, C. H., Schreier, F., Roiger, A., Feist, D. G., Marshall, J., Butz, A., and Trautmann, T.: CO2Image retrieval studies and performance analysis, EGU General Assembly 2023, Vienna, Austria, 23–28 Apr 2023, EGU23-15635, https://doi.org/10.5194/egusphere-egu23-15635, 2023.

AS6 – Short Courses

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